Presentation type:
AS – Atmospheric Sciences

The process of new particle formation from gas-phase precursors holds significant importance in Earth's atmosphere and introduces a notable source of uncertainty in climate change predictions. Typical conditions for new particle formation are moderate temperatures, clear sky and low background aerosol contamination. This general paradigm was challenged by the puzzling observation of frequent new particle formation in megacities. The pre-existing aerosol loadings in such environments seemed to be too high to allow clusters of being formed and grow fast enough before they encounter a collision with a background particle and get lost from the number budget.

Here, we show how nanoparticle growth in urban atmospheres is facilitated enabling efficient survival of nanoclusters providing an explanation for the occurrence of NPF in heavily polluted environments. We outline the tool set, which we have developed over the recent years to address this puzzle. Significant uncertainty in the particle number size distribution measurements and growth rate estimates were addressed through new instrumentation and analysis approaches. At the same time, we refined growth models to account for the challenges of a wide variety of potentially condensable vapors and updated our understanding of particle survival in the atmosphere.

We could demonstrate that new particle formation takes a decisive role in air quality issues in megacities, especially as nanoparticles seem to grow at surprisingly constant rates even when no new particle formation is observed. The “unique atmospheric experiment” of the Covid-19 lockdowns finally provided the chance to estimate how sensitive the urban environment is to changes in the atmospheric chemistry, especially with respect to new particle formation. While we speculated that other condensable vapors than previously thought could be part of the puzzle, we can finally show that also the population dynamics are crucial for more efficient nanoparticle survival than previously thought. However, severe challenges remain, as the outlined methodological improvements also revealed that sometimes the little ones even grow slower than expected.

How to cite: Stolzenburg, D.: How do the little ones grow? Solving the puzzling occurrence of new particle formation in megacities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2853, https://doi.org/10.5194/egusphere-egu25-2853, 2025.

Clouds are fascinating objects because of their myriad shapes and the optical phenomena that they cause. They are also scientifically challenging to understand because their formation and dissipation require knowledge about both the large-scale meteorological environment as well as about the details of cloud droplet and ice crystal formation on the microscale. While we have reduced the uncertainty in the radiative forcing of aerosol-cloud interactions over the last decades, the effect of climate change on clouds, precipitation forecasts and cloud dynamics still pose lots of open questions.

With the advancement of better in-situ and remote sensing instruments, unprecedented observations of clouds are now possible. Simultaneously, the increasing amount of computing power enables us to simulate clouds at increasingly finer scales over larger domains, making convection parameterizations obsolete and allowing us to resolve larger eddies. Cloud research is also being revolutionized by machine learning. We have used machine learning in combination with satellite data to disentangle the response of stratocumulus clouds to aerosol perturbations, for understanding how cirrus clouds respond to the presence of mineral dust as well as for classifying ice crystals down to aggregated monomer scale in in-situ measurements.

We have exploited these advancements in our CLOUDLAB project, where we employed cloud seeding technology to better our understanding of mixed-phase cloud processes: by releasing silver iodide-containing particles from uncrewed aerial vehicles in supercooled low stratus clouds over the Swiss plateau, we were able to observe and measure downstream ice crystals in a controlled way. From these measurements, we quantifed their diffusional growth rates, aggregation rates and riming rates. Additional high-resolution modeling supported the experiments and provided insights for weather forecasts and climate projections. The CLOUDLAB results can also be translated to the potential climate mitigation idea of thinning mixed-phase clouds.

I have great hope that the open questions in cloud research will be tackled by a combination of advanced measurement devices, AI-driven methods, and further advances in computing power enabling high-resolution modeling.

How to cite: Lohmann, U.: From the microscale to climate: combining observations, laboratory data, and numerical simulations for aerosol-cloud interactions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5678, https://doi.org/10.5194/egusphere-egu25-5678, 2025.

EGU25-56 | Posters virtual | VPS2

Links between the Indian Ocean Dipole and Persistent Dry Spells in the Eastern Mediterranean Winter 

Sigalit Berkovic and Assaf Hochman

Persistent Dry Spells (PDS) during winter in the eastern Mediterranean are crucial to understanding the regional challenges of water resources and mitigating agricultural and economic impacts. Winter dry spells significantly affect ecosystem stability, public health, and socioeconomic conditions in a region susceptible to climate variability. Therefore, extending the forecast horizon of these extreme weather events to subseasonal time scales is a key challenge. With this aim, we examine the covariability of the sea surface temperature of the Indian Ocean and Persistent Dry Spells during winter over the eastern Mediterranean. The positive Indian Ocean Dipole (IOD) phase alters global circulation patterns, notably increasing the geopotential height at 500 hPa and the sea-level pressure over western Russia, eastern Europe, and the eastern Mediterranean during PDS events. Concurrently, the positive IOD phase enhances moisture fluxes and decreases sea level pressure and geopotential height at 500 hPa in the Western Mediterranean, suggesting increased cyclonic activity in that region. This type of activity probably influences the formation of PDS in the eastern Mediterranean through latent heating and the formation of ridges downstream of the cyclones. The baroclinic, subtropical, and polar regimes are large-scale synoptic regimes alternately prevailing during PDS events. Changes due to the DMI phase are not identical under these regimes and sometimes have opposite trends. The baroclinic regime is the most frequent regime during PDS events. Consequently, the average changes in pressure intensity during PDS events strongly resemble those during baroclinic days. Positive DMI case studies exemplify the effect of these large-scale regimes. We provide evidence for a link between the positive phase of IOD in December and the frequency of longer (> 15 days) PDS events. The normalized frequencies of persistent 15-20-day events under the positive dipole mode index (DMI) are ~ 2% higher than the frequency of negative DMI. The frequencies of 6-7 day events are ~20% lower. Finally, we emphasize the sensitivity of persistent dry spells during winter to event definition, the chosen precipitation data source, and threshold definitions for climate indices. These considerations are essential for improving the accuracy of regional weather and climate predictions, further enhancing our understanding of the climatic impacts of IOD and other teleconnection patterns in the eastern Mediterranean and worldwide.

How to cite: Berkovic, S. and Hochman, A.: Links between the Indian Ocean Dipole and Persistent Dry Spells in the Eastern Mediterranean Winter, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-56, https://doi.org/10.5194/egusphere-egu25-56, 2025.

Quantifying uncertainties is a key aspect of data assimilation systems since it has a large impact on the quality of the forecasts and analyses. Sequential data assimilation algorithms, such as the Ensemble Kalman Filter (EnKF), describe the model and observation errors as additive Gaussian noises and use both inflation and localization to avoid filter degeneracy and compensate for misspecifications. This introduces different stochastic parameters which need to be carefully estimated in order to get a reliable estimate of the latent state of the system. A classical approach to estimate unknown parameters in data assimilation consists in using state-augmentation, where the unknown parameters are included in the latent space and are updated at each iteration of the EnKF. However, it is well-known that this approach is not efficient to estimate stochastic parameters because of the complex (non-Gaussian and non-linear) relationship between the observations and the stochastic parameters which can not be handled by the EnKF. A natural alternative for non-Gaussian and non-linear state-space models is to use a particle filter (PF), but this algorithm fails to estimate high-dimensional systems due to the curse of dimensionality. The strengths of these two methods are gathered in the proposed algorithm, where the PF first generates the particles that estimate the stochastic parameters, then using the mean particle the EnKF generates the members that estimate the geophysical variables. This generic method is first detailed for the estimation of parameters related to the model or observation error and then for the joint estimation of inflation and localization parameters. Numerical experiments are performed using the Lorenz-96 model to compare our approach with state-of-the-art methods. The results show the ability of the new method to retrieve the geophysical state and to estimate online time-dependent stochastic parameters. The algorithm can be easily built from an existing EnKF with low additional cost and without further running the dynamical model. 

How to cite: Guillot, J.: State and Stochastic Parameters Estimation with Combined Ensemble Kalman and Particle Filters, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-125, https://doi.org/10.5194/egusphere-egu25-125, 2025.

EGU25-243 | ECS | Posters virtual | VPS2

Envisioning the Role of Physics-Informed Neural Networks in Atmospheric Science: Advancements, Challenges, and Future Prospects 

Johanne Ayeley Ekue, Desmond Hammond, and Ebenezer Agyei-Yeboah

Since the inception of physics-informed neural networks (PINNs) by Raissi et al. in 2019, it has been seen as a promising approach to outperform conventional algorithms in terms of computational efficiency, reduced costs, and improved prediction accuracy, especially in small data regimes.PINNs incorporate known physical governing equations in the form of partial differential equations (PDEs) or ordinary differential equations (ODEs) into neural networks, and occasionally the governing equations are derived from observational or simulated data, allowing PINNs to address specific atmospheric systems.Moreover, depending on the problem being solved, most work adds the physical constraints directly into the loss or cost function, while others enhance performance using modified architectures or preprocessing techniques.In the realm of atmospheric sciences, challenges remain, including a heavy reliance on simulated data and limited use of observational datasets, which does not show the real-world applicability of PINNs. A detailed review of available results shows critical gaps in scalability, hybrid data integration, and standardization in atmospheric science.We identified a hybrid methodology by combining simulated and observational data, which includes optimizing hybrid loss functions to balance physics-based and observational accuracy, applying adaptive training techniques, and standardizing preprocessing schemes to handle multi-scale atmospheric phenomena.Results demonstrate the ability of PINNs to deliver faster computation, enhanced prediction accuracy, and robustness in sparse data environments. This highlights the transformative advantages of PINNs over traditional methods and suggests future directions for leveraging their capabilities in atmospheric science applications.

How to cite: Ekue, J. A., Hammond, D., and Agyei-Yeboah, E.: Envisioning the Role of Physics-Informed Neural Networks in Atmospheric Science: Advancements, Challenges, and Future Prospects, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-243, https://doi.org/10.5194/egusphere-egu25-243, 2025.

EGU25-888 | ECS | Posters virtual | VPS2

Evaluation of Vertically Integrated Liquid Water Content in Indian Summer Monsoon Clouds Using Dual-Polarimetric Doppler Weather Radar 

Albin Sabu, Hamid Ali Syed, Someshwar Das, Subrat Kumar Panda, Devesh Sharma, and Jayanti Pal

Accurate evaluation of cloud microphysical variables is essential for improving cloud parameterization and weather forecasting. However, obtaining high-resolution, spatially and temporally extensive observation dataset remains a challenge due to the limitations of in situ measurements. Therefore, this study addresses this gap by assessing existing equations for estimating vertically integrated liquid water content (VIL, kg/m²) from liquid water content (LWC, g/m3) using C-band dual-polarised doppler weather radar (DWR) data from IMD Jaipur station over 78 deep convective summer monsoon days in the years 2020-2022. A long-term climatological study (2003-2023) of total column cloud liquid water (TCCLW, kg/m2) from ERA5, liquid water cloud water content (LWCP, kg/m2) from MODIS and rainfall data from IMD, IMERG, and GPCP datasets is also performed. VIL is computed as the vertical integral of LWC across atmospheric layers using four reflectivity-LWC (Z-LWC) relationships and one reflectivity-differential reflectivity (Z, ZDR-LWC) relationship from existing literature. The performance of each equation is evaluated by comparing radar-derived VIL with satellite-derived parameters like MODIS cloud liquid water path (LWP, kg/m2) and TCCLW. The results show that VIL values increase with rainfall intensity and cloud vertical height, leading to higher estimation errors. Among the equations tested, the hybrid ZDR-based equation consistently demonstrated superior performance, particularly during high-intensity rainfall events, with lower root mean square error (RMSE) and mean absolute error (MAE) values which also captured more detailed spatial patterns of liquid water distribution and reduced bias, making it the most reliable estimator. Despite some limitations, such as beam blockage and slight spatial shifts due to interpolation, the study highlights the advantages of incorporating polarimetric radar products for VIL estimation. These findings provide a foundation for improving real-time precipitation forecasts and understanding cloud microphysics, with future work aimed at refining the methodology by addressing data gaps and enhancing cloud-type-specific estimators.

How to cite: Sabu, A., Syed, H. A., Das, S., Panda, S. K., Sharma, D., and Pal, J.: Evaluation of Vertically Integrated Liquid Water Content in Indian Summer Monsoon Clouds Using Dual-Polarimetric Doppler Weather Radar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-888, https://doi.org/10.5194/egusphere-egu25-888, 2025.

EGU25-1073 | ECS | Posters virtual | VPS2

Building Equitable Air Quality Networks: Low-Cost Sensors and Community-Led Monitoring in Dublin 

Harish Daruari, Saul Crowley, Chiara Cocco, and José P. Gómez Barrón

Air quality monitoring remains a significant challenge in urban areas, particularly where high-cost infrastructure is unavailable or difficult to maintain. Traditional monitoring systems are often limited in scope due to expense and logistical constraints, leading to data gaps, especially in resource-constrained environments. Low-cost air quality sensors have the potential to transform environmental monitoring by providing accessible, affordable tools for collecting air quality data, especially in urban settings. As part of the SCORE project, a low-cost sensor system was developed to support real-time air quality monitoring across European cities. These sensors provide a more granular understanding of air pollution trends, making air quality data collection both scalable and accessible to a wider range of stakeholders, including local communities. This presentation will highlight the deployment of these sensors in Dublin, Ireland, where they have been successfully integrated into citizen science initiatives, enabling communities to actively participate in environmental data collection and contribute to air quality management.

Ensuring data accuracy and reliability is a key challenge in the use of low-cost sensors. We will examine the technical challenges of deploying low-cost sensors, such as calibration, accuracy, and long-term reliability in small-scale urban environments. The presentation will also discuss strategies for integrating sensor data into authoritative air quality monitoring networks to enhance overall data quality and spatial coverage.

In Dublin, the citizen science air quality initiative has built strong connections between local communities, researchers and policymakers. This collaboration exemplifies how co-created initiatives, backed by accessible technology, can empower citizens and bridge the gap between public engagement and formal policy processes. The outcomes of the Dublin case study suggest broader applicability for the SCORE model in other cities facing similar air quality challenges. By offering a replicable and scalable solution, low-cost sensors provide an affordable alternative to high-end monitoring stations, enabling resource-limited municipalities to expand their air quality infrastructure. The project demonstrates how engaging local communities in the data collection process can foster long-term, sustainable environmental stewardship. These insights underscore the importance of equitable partnerships between citizens, researchers, and governments in tackling air pollution, particularly in cities where financial or technical constraints have traditionally limited comprehensive air quality monitoring.

How to cite: Daruari, H., Crowley, S., Cocco, C., and Barrón, J. P. G.: Building Equitable Air Quality Networks: Low-Cost Sensors and Community-Led Monitoring in Dublin, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1073, https://doi.org/10.5194/egusphere-egu25-1073, 2025.

EGU25-1542 | ECS | Posters virtual | VPS2

Rainfall Prediction using Hybrid CNN-LSTM approach: A case study in the Boudh district, Odisha, India 

Sandeep Samantaray, Abinash Sahoo, and Deba P Satapathy

The forecast of monthly rainfall is a significant topic for water resource management and hydrological disaster prevention. A critical need for precise hydrological forecasts in water resource management is addressed in this study by analyzing machine learning (ML) models for precipitation forecasting in the Boudh district of Odisha, India. Although machine learning (ML) models have demonstrated significant promise in rainfall forecasting due to their high performance, often surpassing that of certain physical models, the intricate physical processes involved in rainfall creation mean that a single ML model is typically insufficient to provide reliable rainfall projections. A thorough set of meteorological parameters, including precipitation wind speed, temperature, and humidity, are utilized to create four distinct models: Support Vector Regression (SVR), long and short memory neural networks (LSTM), Bi-LSTM and Convolutional neural network with LSTM (CNN-LSTM). The performance of these models is thoroughly assessed utilizing a range of evaluation metrics. In this work, the correlations between precipitation and climate factors are assessed using the cross-correlation function (XCF). With maxima consistently reported during months across all four sites, the XCF analysis shows a number of significant trends, including a strong correlation amid precipitation and maximum temperature. Moreover, precipitation is significantly correlated with wind speed and relative humidity. The results demonstrate the effectiveness of hybridized ML techniques in raising the precision of precipitation forecasts. The CNN-LSTM models, which have R2 values between 0.93 and 0.97, generally perform better. Their remarkable accuracy highlights their efficacy in precipitation forecasting, outperforming rival models during both training and testing. These findings have important ramifications for hydrological processes, particularly in Odisha's Boudh region, where sustainable water resources management depends on precise precipitation forecasting.

How to cite: Samantaray, S., Sahoo, A., and Satapathy, D. P.: Rainfall Prediction using Hybrid CNN-LSTM approach: A case study in the Boudh district, Odisha, India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1542, https://doi.org/10.5194/egusphere-egu25-1542, 2025.

EGU25-2672 | ECS | Posters on site | AS1.23

Genesis, structure and propagation of synoptic systems over the Indian Ocean during the Northeast Monsoon  

Shrutee Jalan, Jai Sukhatme, and Ashwin Seshadri

The Northeast Monsoon (NEM) in South Asia, occurring from October to January, plays a pivotal role in precipitation, often giving rise to extreme weather events. This study aims to elucidate the diverse synoptic systems responsible for rainfall during the NEM and track their origins. Specifically, using a synoptic system tracking algorithm, we identify and characterise the genesis locations, propagation, and structures of these synoptic systems.  

Our findings reveal a seasonally evolving latitude dependence in genesis locations, with a bimodal distribution that shifts southwards and becomes more meridionally confined as the season progresses. These genesis locations coincide with regions of high relative vorticity and column-integrated Moist Static Energy (MSE).  Based on the pressure level at which maximum vorticity is observed at genesis, we classify these systems into three categories: Lower Tropospheric Cyclones (LTCs), Mid-Tropospheric Cyclones (MTCs), and Upper Tropospheric Cyclones (UTCs).  Each category exhibits an evolving preference for genesis location, generally evolving southwards and eastwards, as the season advances. The UTCs are further categorised into two subtypes: one forming near the equator (up to 15°N/S) and another of subtropical origin (poleward of 15°N/S). Composites of near-equatorial UTCs display westward tilt with height, warm temperature anomalies at upper levels, and cold anomaly below, with vorticity maximum near 400 mb. This structure resembles that of MTCs, which exhibit a similar westward tilt and warm-over-cold core structure, but with maximum vorticity near 600 mb. In contrast, LTCs exhibit an upright structure with a warm core aloft and vorticity maximum centred around 800 mb. The joint distribution of MSE and relative vorticity at genesis indicates that LTCs are typically associated with stronger values of both variables, whereas UTCs and MTCs each appear in two distinct regimes: one with higher values of MSE and vorticity and another with lower values of these variables.  

UTCs account for 14% of all systems, MTCs 44%, and LTCs 42%. Despite being fewer, on average a UTC produces rainfall of comparable magnitude to an MTC. UTCs predominantly generate precipitation over the Bay of Bengal shifting to the southwest Indian Ocean in January. MTCs generate significant rainfall over the Arabian Sea, Bay of Bengal, and South China Sea until December, and over Indo-Pacific region and the tropical South Indian Ocean in January. LTCs produce the largest rainfall, mainly over the Bay of Bengal and South China Sea, throughout the season and over the tropical South Indian Ocean as the season progresses. Lastly, while cyclonic propagation trajectories show overall westward movement for all categories, there are important differences: LTCs tend to have a more meridional motion towards northwest, while MTCs and UTCs exhibit a comparatively more zonally directed motion. Given the structural differences between systems, especially MTCs and LTCs, and their potential to morphologically evolve (e.g., MTC transitioning to LTC and vice versa), our study focussing on the genesis of these systems offer valuable insight into their formation mechanism. 

How to cite: Jalan, S., Sukhatme, J., and Seshadri, A.: Genesis, structure and propagation of synoptic systems over the Indian Ocean during the Northeast Monsoon , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2672, https://doi.org/10.5194/egusphere-egu25-2672, 2025.

EGU25-3008 | Posters virtual | VPS2

Aerosol-Radiation Interaction During Dense Fog in the Indo-Gangetic Plains Region  

Shweta Bhati, Theethai Jacob Anurose, Aravindakshan Jayakumar, Saji Mohandas, and Vijapurapu Srinivasa Prasad

The Indo-Gangetic plains (IGP) in India are frequently affected by fog during the winter months of December, January, and February, which manifests in severe consequences for air and road traffic, thereby leading to health as well as economic losses. This region, which includes highly populated cities like the National Capital Territory of Delhi, also experiences a high concentration of aerosols during this period. While studies have indicated the importance of the role of aerosols in fog processes in the region, the role of different aspects of aerosol-radiation interaction (ARI) has not been studied in detail for the formation of fog in the region. Current numerical weather prediction models (NWP) still struggle to predict fog accurately because of the uncertainties in the representation of processes leading to fog formation, sustenance, and dissipation. The present study aims to understand the influence of aerosols and ARI on the fog over IGP with a focus on dense fog conditions using the Delhi Model with Chemistry and aerosol framework (DM-Chem1.0), which is a high-resolution (330 m) model used for operational forecasting of wintertime visibility and air quality at the National Centre for Medium-Range Weather Forecasting (NCMRWF), India. Four experiments (along with a Control experiment) were designed to analyze how both the scattering and absorbing nature of ARI influence the evolution of dense fog from temporal and spatial perspectives. Two experiments isolated the absorbing and scattering effect of aerosols, while the third excluded both these effects. The fourth experiment analyzed pristine conditions with minimal aerosol presence. The study indicated that turning off absorption had the greatest impact, significantly increasing dense fog-impacted areas and fog-associated parameters like cloud liquid water mixing ratio and cloud droplet number concentration (CDNC). Satellite data for the absorbing aerosol index also corroborated the greater contribution of absorbing aerosols in the model domain. Further, the study also indicates the importance of a realistic representation of aerosol for better model performance during daytime. The study highlights the importance of correctly representing radiative interactions in the numerical models for fog prediction. The policy measures need to focus on regulating high aerosol concentrations over IGP to mitigate the adverse effects of fog.

How to cite: Bhati, S., Anurose, T. J., Jayakumar, A., Mohandas, S., and Prasad, V. S.: Aerosol-Radiation Interaction During Dense Fog in the Indo-Gangetic Plains Region , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3008, https://doi.org/10.5194/egusphere-egu25-3008, 2025.

EGU25-3431 | ECS | Posters virtual | VPS2

Exploring the spatiotemporal variations and key environmental conditions of convective initiations in the Western Jiangnan Region of China 

Zhenzhen Wu, Yu Han, Nan Song, Chengzhi Ye, and Gang Xiang

This study investigated convective initiations (CIs) in the western Jiangnan region of China using radar data spanning April to September from 2018 to 2021. An integrated approach combining objective identification and subjective validation was applied to identify, track and validate CIs, resulting in a more accurate CIs dataset. Based on this dataset, this study delved into the spatiotemporal variations and key environmental conditions associated with CIs. The results indicated distinct seasonal and diurnal patterns in CIs events. Seasonally, the spatial variations of CIs were demarcated by the Nanling Mountains, exhibiting higher frequency to the south and lower to the north. Generally, the seasonal distribution of CIs followed a unimodal pattern, peaking during June to August and reaching minima in April and September. Notably, CIs exhibited a pronounced convection feature in the afternoon, particularly during June to August, when the majority of CIs occurred between 11:00 and 19:00. Furthermore, the spatial variations influenced by terrain were prominent. With the Nanling Mountains as the dividing line, CIs in the northern region were located near relatively higher mountains, while in the southern region, they were concentrated in smaller mountains and coastal areas. Utilizing the K-means clustering method, CIs that could develop into Mesoscale Convective Systems are classified into four circulation types: the Western Pacific Subtropical High (WPSH) Control type (Type I), the WPSH Edge type (Type II), the Southwest Airflow type (Type III), and the Low Trough Shear type (Type IV). CIs under Type I and II were primarily attributed to afternoon thermal convection occurring under conditions of strong moisture and thermal instability. The distribution of CIs triggers for these types tended to cluster in the vicinity of high-elevation terrain. In contrast, CIs belonging to Type III and IV were primarily driven by the synergy of abundant moisture conditions and systematic dynamic factors such as low-level jets, upper-level troughs, and shear lines. These exhibited a north-low and south-high frequency distribution, with high-frequency CIs trigger zones observed particularly in regions of strong moisture flux convergence and near complex terrain.

How to cite: Wu, Z., Han, Y., Song, N., Ye, C., and Xiang, G.: Exploring the spatiotemporal variations and key environmental conditions of convective initiations in the Western Jiangnan Region of China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3431, https://doi.org/10.5194/egusphere-egu25-3431, 2025.

EGU25-3896 | Posters virtual | VPS2

Dynamics and Characteristics of Climatic Extremes over East Asia Monsoon region 

Kyung-Ja Ha, Ji-Hye Yeo, and Ye-Won Seo

In this talk, I will highlight our recent advances and findings in changes in climatic extremes over east Asia monsoon region. I will focus specifically on monsoon duration, intensity, rainfall extremes changes, and mechanism, with dynamic and thermodynamic factors controlling rainfall extremes over East Asia in late summer. Moreover, I will present our latest research on climatic extremes such as heatwaves based on dry conditions and stationary waves. Despite increasing future rainfall, rainfall extremes and rainfall variability in many areas, our recent studies suggest also an increase in drought risk over eastern Asia as a result of changes in evapotranspiration. However, the underlying mechanisms of heat waves and potential atmospheric and land feedbacks are still not fully understood. Through feedback attribution analysis, we found that there are dry and hot heat waves with very different underlying physical processes and feedbacks. The increasing global warming is expected to exacerbate atmospheric water demand, worsening future conditions of extreme droughts and heatwaves. Compound drought and heatwaves (DHW) events have much attention due to their notable impacts on socio-ecological systems. However, studies on the mechanisms of DHW related to land-atmosphere interaction are not still fully understood in regional aspects. Here, we investigate drastic increases in DHW from 1980 to 2019 over northern East Asia, one of the strong land-atmosphere interaction regions. Heatwaves occurring in severely dry conditions have increased after the late 1990s, suggesting that the heatwaves in northern East Asia are highly likely to be compound heatwaves closely related to drought. Moreover, the soil moisture–temperature coupling strength increased in regions with strong increases in DHW through phase transitions of both temperature and heat anomalies that determine the coupling strength. As the soil moisture decreases, the probability density of low evapotranspiration increases through evaporative heat absorption. This leads to increase evaporative stress and eventually amplify DHW since the late 1990s. Focusing on changes in stomatal conductance due to CO2 changes, our research results reveal an increase in surface resistance with CO2 elevation. Particularly under drought conditions, potential evapotranspiration tends to overestimate drought severity in the East Asian region by approximately 17% when scenarios considering vegetation are not taken into account. Additionally, intensified land-atmosphere interactions due to soil moisture deficiency lead to more frequent and amplified occurrences of compound heatwaves and droughts over northern East Asia. Understanding the relationship between soil moisture and vegetation can contribute to comprehending future severe droughts and heatwaves under diverse surface conditions with warming and moistening.

How to cite: Ha, K.-J., Yeo, J.-H., and Seo, Y.-W.: Dynamics and Characteristics of Climatic Extremes over East Asia Monsoon region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3896, https://doi.org/10.5194/egusphere-egu25-3896, 2025.

Based on the minute by minute precipitation observation data from 46 national weather stations in the Yangtze River Delta region of China and hourly ERA5 reanalysis data from June to August 2018 to 2021, the temporal and spatial characteristics and environmental parameters of short-term heavy precipitation were analyzed. The short-term heavy rainfall was classified and compared according to the 19 environmental parameters representing water vapor, dynamic and thermal conditions. The results showed that:(1) There were more short-term heavy rainfall in the Yangtze River Delta in summer, and 58.7% of the weather stations appeared more than 5 times a year on average; most of short-term heavy rainfall appeared in August, accounting for 40.7%; From 14:00 PM to 17:00 PM was the high incidence period of short-term heavy rainfall; The duration of short-term heavy rainfall was mostly within 60 minutes, accounting for 85.9%, and the longest process lasted 282 minutes.(2) At the beginning of short-term heavy rainfall, water vapor was sufficient, PWAT generally exceeded 63mm, and the relative humidity at 850 hPa and 700 hPa exceeded 80%; The energy condition was good, and the average value of cape was 1516.9 J/kg; The vertical wind shear of 0-6 km was mainly distributed in the range of 8.1~16.7 m/s, belonging to medium weak or weak intensity; The thickness of warm clouds was large, most of which were more than 4395.2 m, which was conducive to higher precipitation efficiency.(3) The environmental parameters of the three types of short-term heavy rainfall were quite different. The water vapor of the first type was mainly concentrated in the lower layer, with high cloud base height and large Cape value, 75% of which was more than 1700 J/kg. The thermal conditions were prominent, and the dynamic effect was weak. The water vapor of the whole layer of the second type was sufficient, and the Cape value was high, with an average value of 1401.1 J/kg, the uplift condition of the middle and low layers was the best of the three types. The water vapor, thermal and dynamic effects were relatively balanced; The third type was rich in water vapor, with prominent water vapor conditions, large vertical wind shear in the lower layer and weak thermal effect. 

How to cite: Zhang, C. and Peng, L.: Characteristics of environmental parameters of short-term heavy rainfall in the Yangtze River Delta region in summer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3935, https://doi.org/10.5194/egusphere-egu25-3935, 2025.

EGU25-4905 | ECS | Posters virtual | VPS2

Deep learning-based ENSO modeling and its prediction and predictability study 

Lu Zhou and Rong-hua Zhang

A novel deep learning (DL) transformer model, named the 3D-Geoformer, has been developed for ENSO-related modeling studies in the tropical Pacific. Multivariate input predictors and output predictands are selected to adequately represent ocean-atmosphere interactions; so, this purely data-driven model is configured in such a way that key fields for the coupled ocean-atmosphere system are collectively and simultaneously utilized, including three-dimensional (3D) upper-ocean temperature and surface wind stress fields, which represents the coupled ocean-atmosphere interactions known as the Bjerknes feedback in the region. The 3D-Geoformer achieves high correlation skills for ENSO prediction at lead times of up to one and a half years. The reasons for the successful prediction with interpretability are explored comprehensively by performing perturbation experiments to predictors and quantifying input‐output relationships in predictions using the 3D-Geoformer. This is achieved by investigating how the thermal precursors contribute to ENSO prediction skills, with the dependence of the precursor representations on preconditioning multi-month input predictors elucidated. Results reveal the existence of ENSO‐related upper‐ocean temperature anomaly pathways and consistent phase propagations of thermal precursors around the tropical Pacific in the DL framework. The research demonstrates that 3D thermal fields and their basinwide evolution during multi-month time intervals act to enhance long‐lead prediction skills of ENSO. It is demonstrated that the 3D-Geoformer can not only have its ability to effectively improve prediction skills of sea surface temperature variability in the eastern equatorial Pacific, but also explain how and why it is so, thus enhancing model explainability.

How to cite: Zhou, L. and Zhang, R.: Deep learning-based ENSO modeling and its prediction and predictability study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4905, https://doi.org/10.5194/egusphere-egu25-4905, 2025.

EGU25-5045 | Posters on site | AS1.31

Ozone anomalies over Eastern and Western Hemisphere Antarctic stations during sudden stratospheric warming life cycle 

Gennadi Milinevsky, Ruixian Yu, Asen Grytsai, Oleksandr Evtushevsky, Andrew Klekociuk, and Oksana Ivaniha

Sudden stratospheric warming (SSW), a well-known phenomenon in the polar atmosphere, changes the distribution of various atmospheric parameters due to the enhanced activity of planetary waves. These processes produce zonal asymmetry in total ozone content (TOC) with a wave-1 pattern. However, regional characteristic properties of the Antarctic TOC anomalies that occur during the SSW life cycle have not been studied in detail. We aim to analyze the connection of zonally asymmetric variations of TOC with SSW events. The analysis is based on a time series of ten research stations in the Antarctic region and gridded fields from MSR-2 TOC data. Here, we compare the evolution of TOC and wave amplitudes in three Southern Hemisphere SSW events. The TOC time series over ten stations in the Antarctic region and superposed epoch analysis for ±60-day time lags relative to the SSW central date were used. A regional division according to the geographic location of the stations and TOC climatology was introduced. According to the TOC asymmetry pattern, a division between Eastern and Western Hemisphere stations is used. We observe zonally asymmetric ozone responses in the two hemispheres during the SSW life cycle, including distinct precursor properties before the SSW onset. This research clarifies the different SSW properties in local ozone observations under the zonally asymmetric TOC field. The previously unknown regional manifestations of Antarctic TOC anomalies in the early stage of the SSW are discussed. The role of wave-1 and the zonally asymmetric Brewer-Dobson circulation in the Eastern–Western Hemisphere difference in the Antarctic TOC variability is also discussed. We also characterize total ozone levels in the years immediately preceding and following the three most significant SSW events. We examine the influence of planetary wave activity and large-scale climate modes on the level of interannual ozone variability and its regional patterns. There is evidence that Antarctic total ozone in the years adjacent to these SSW events is reduced, which may serve as a precursor signal of these events and an indicator of their longer-lasting influence. We discuss the implications and importance of these ozone perturbations for the regional Antarctic climate.

How to cite: Milinevsky, G., Yu, R., Grytsai, A., Evtushevsky, O., Klekociuk, A., and Ivaniha, O.: Ozone anomalies over Eastern and Western Hemisphere Antarctic stations during sudden stratospheric warming life cycle, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5045, https://doi.org/10.5194/egusphere-egu25-5045, 2025.

EGU25-5789 | Posters virtual | VPS2

Lessons learned from a UAS survey of methane emissions from multiple biogas plants in France 

Jean-Louis Bonne, Nicolas Dumelie, Thomas Lauvaux, Charbel Abdallah, Jérémie Burgalat, Grégory Albora, Julien Vincent, Julien Cousin, Florian Parent, Vincent Moncourtois, and Lilian Joly

An on-going campaign monitors the greenhouse gases emissions of biogas plants in the Grand Est region, in France, using airborne in situ CO2 and CH4 concentrations and wind measurements from Uncrewed Aerial System, associated with a mass balance method. During 16 days in 2024, we quantified the instantaneous emissions of 19 agricultural biogas plants, with installed methane productions ranging from 128 to 312 Nm3.h-1,producing biogas injected into the network mainly from manure, energy crops and agricultural wastes.

Observations obtained to date were used to quantify emissions either representative of the globality of a biogas plant or of specific targeted sources inside a site (inputs, effluents, digesters or biogas purification). Global plant methane emissions among all sites range from 1.5 to 26 kg.h-1, with average emissions of 10 kg.h-1. Repeated measurements of emissions on the same site at different dates depict a significant temporal variability, however overwhelmed by the variability of emissions among all sites. We estimated instantaneous methane losses ranging from 1.7 to 10 %, comparing monitored emissions with the installed productions. Emissions of targeted sources among sites suggest that inputs and effluents might be the predominant methane sources on the sites, while biogenic CO2 emissions might be mostly attributed to the biogas purification process.

This campaign highlighted several limits intrinsically linked with the mass balance method. One of them is the sensitivity to contamination by parasite sources, which has to be anticipated during the field campaign preparation. Another difficulty is the risk of measuring truncated plumes, as the mass balance method requires the monitoring of an entire plume cross-section to provide quantifications representative of the complete source emissions. These limitations could be overturned in the future by alternative quantification methods, such as inversion methods based on Large Eddy Simulation of the atmospheric transport, considering the highly variable nature of the turbulent plume. These new developments, associated with evolutions of the monitoring protocol, may improve the reliability and precision of the results.

How to cite: Bonne, J.-L., Dumelie, N., Lauvaux, T., Abdallah, C., Burgalat, J., Albora, G., Vincent, J., Cousin, J., Parent, F., Moncourtois, V., and Joly, L.: Lessons learned from a UAS survey of methane emissions from multiple biogas plants in France, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5789, https://doi.org/10.5194/egusphere-egu25-5789, 2025.

Based on the traditional satellite-based convective initiation (CI) detection method, an improved algorithm for the identification and tracking of CIs using satellite data has been proposed. This algorithm then undergoes spatio-temporal matching with ground-based observation data such as radar and precipitation data. Incorporating experts domain knowledge, the algorithm utilizes a subjective-objective interactive approach to complete the verification and calibration of the satellite-drived CI identification results. This process results in a high-resolution annotation dataset of convective initiation that can be used for detection and forecasting of CI and artificial intelligence models.

Firstly, within a spatial-temporal window of 30 minutes before and after the satellite CIs trigger time and a radius of 20km, the satellite-derived CIs are matched with radar-identified CIs. Additionally, within a spatial-temporal window of 60 minutes after the satellite CI trigger and extending 2km outside the CI cloud clusters movement zone, the satellite-derived CIs are also matched with precipitation data. The two matching results are combined to form a comprehensive identification of CIs. Furthermore, using a calibration system and a back-to-back verification method by forecasters, the CI annotation results are revised, resulting in a high-resolution and reliable CI annotation dataset.

Using this methodology, a high spatio-temporal resolution CI dataset was established for the years 2018-2023, which allowed for the statistical analysis of CI distributions across different precipitation levels in each month. The highest proportion of CI events occurred in August, followed by July. Among these, CI events with moderate precipitation accounted for 46.2%, weak precipitation accounted for 34.4%, and strong precipitation accounted for 19.3%.

It can be seen that there is a noticeable northward shift in the occurrence of CI events, especially those associated with heavy precipitation, from April to August. In April, these events are mainly concentrated in a few provinces in the central and southern parts of the country. Subsequently, they gradually expand from south to north, covering the entire central and eastern research area by August. In September, they retreat back to the central and southern regions. This spatial evolution pattern of CI events once again verifies that the occurrence of severe convection events is closely related to the position changes of the Intertropical Convergence Zone (ITCZ) and the monsoon.The frequency of CI occurrences has also been proven to peak between 11 a.m. and 3 p.m., regardless of precipitation intensity.

How to cite: Peng, L., Ye, C., and Ou, X.: Convection Initiation Identification and The Construction of A High-value Dataset Using the Fengyun-4A Satellite, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6767, https://doi.org/10.5194/egusphere-egu25-6767, 2025.

EGU25-7147 | ECS | Posters virtual | VPS2

An Enigmatic Variability in the Tropical Middle Atmosphere 

Neelakantan Koushik and Karanam Kishore Kumar

The tropical middle atmosphere is characterized by long-period oscillations such as the Quasi Biennial Oscillation and the Semiannual Oscillation which are primarily driven by the interaction of a broad spectrum of atmospheric waves with the background flow. Using reanalysis datasets and independent rocket soundings from a low latitude location, we identified a hitherto unreported variability in the tropical middle atmosphere that appears at a variable interval of 2-5 years in the late 20th century and 7-9 years in the early 21st century. The newly identified variability, Quasi-Periodic Easterly Bursts (QPEBs) as we call them, manifests as enhanced easterlies during the easterly phase of the Stratopause Semiannual Oscillation around May-July. QPEBs are found to have remote influences on the Southern Hemispheric polar vortex as well as residual circulation in the lower mesosphere. A momentum budget analysis reveals that QPEBs are found to be primarily caused by enhanced cross-equatorial advection as well as gravity wave drag. Even though a close association with the Quasi Biennial Oscillation winds is observed, the cause of the observed periodicity remains elusive.

How to cite: Koushik, N. and Kumar, K. K.: An Enigmatic Variability in the Tropical Middle Atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7147, https://doi.org/10.5194/egusphere-egu25-7147, 2025.

In past few decades there has been a noticeable increase in the frequency and intensity of extreme rainfall events (EREs) globally, including India. The Clausius-Clapeyron relationship explains how the warmer air can significantly hold more moisture. Hence, in present climate change scenario increasing temperature along with other factors can lead to further increase in EREs. Effective management strategeis in various sectors like disaster preparedness, smart-city planning, water quality, public health, agriculture planning, etc. can get improved, through proper understanding on the distribution and frequency of EREs. Keeping in mind the socio-economic impacts of EREs; this study aimed to identify the hotspot regions for EREs in India.

India is a country with vast spatio-temporal variability in rainfall pattern. Hence, this study implemented objective criteria to identify the spatio-temporal rainfall variability of EREs over four rainfall homogeneous regions for pre-monsoon, monsoon and post-monsoon seasons. Based on frequency distribution of daily accumulated rainfall, suitable rainfall threshold values for defining EREs are identified for each homogeneous region and each season. These threshold values vary region-wise as well as season-wise. Distribution of EREs show interannual as well as seasonal variability.

Clustering algorithms, popular unsupervised Machine Learning (ML) techniques, are handy tools to identify hotspots of extreme rainfall regions with similar spatial variability. To understand the ERE distribution and to identify rainfall hotspots based on long term daily gridded rainfall data, this study implemented K-means clustering and DBSCAN (Density-Based Spatial Clustering of Applications with Noise) clustering algorithms. Comparative area distribution study between K-means and DBSCAN clustering help to identify the EREs hotspots in India. Overall, the K-means method shows more scattered hotspots compared to DBSCAN method, which are further validated using Davies-Boulding Index (DBI), Silhouette score, Calinski-Harabasz (CH) score and Dunn's Index. These score analysis methods serve as potential tools to support the clustering validation method. In addition to the area distribution, this study has addressed the temporal variability of the EREs hotspots. ST-OPTICS ( Spatio-Temporal Ordering Points to Identify the Clustering Structure) algorithm results clustering of hotspots based on their spatial and temporal similarity. This study shows that ML algorithms prove to be promising techniques for detecting and analyzing spatial as well as temporal variability of EREs hotspots which is effective for future management practice in various sectors.

Keywords: Extreme Rainfall Events; DBSCAN Clustering; K-Means Clustering; ST-OPTICS.

How to cite: Putatunda, I. and Vasudevan, R.: Extreme rainfall hotspots in India based on spatio-temporal variability of rainfall using unsupervised clustering techniques, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7852, https://doi.org/10.5194/egusphere-egu25-7852, 2025.

EGU25-7965 | Posters virtual | VPS2

An Explainable AI-Driven Feature Reduction Framework for Enhanced Agricultural Yield Prediction 

Anamika Dey, Arkadipta Saha, Somrita Sarkar, Arijit Mondal, and Pabitra Mitra

Agricultural yield prediction plays a crucial role in food security and economic planning, yet existing models often struggle with the complexity and high dimensionality of agricultural data. This study presents a framework that combines explainable artificial intelligence (XAI) with feature reduction methodology to enhance the accuracy and efficiency of rice yield prediction. Our approach addresses the dual challenges of model interpretability and computational efficiency while maintaining high prediction accuracy.

The framework begins with a systematic development of prediction models utilizing advanced machine learning (ML) and deep learning (DL) techniques. We implemented comprehensive pre-processing steps, including data normalization, feature engineering, and missing value handling, to ensure data quality. Our evaluation encompassed various models, including Random Forest, Gradient Boosting Machines, Convolutional Neural Networks (CNNs), and Long Short-Term Memory (LSTM) networks with attention mechanisms. To optimize model performance, we employed hyperparameter tuning through grid search, effectively mitigating issues of overfitting and underfitting.

A notable innovation of our framework is the incorporation of SHapley Additive exPlanations (SHAP), enabling transparent insights into the model's decision-making process. Leveraging this XAI approach, we introduced a novel feature reduction methodology that systematically identifies and removes negatively contributing features while maintaining model accuracy. Our analysis of a multivariate dataset which is a public dataset from rice fields in the an Giang province of the Mekong Delta, Vietnam, required the integration of diverse satellite datasets, including optical data from Landsat and radar data from Sentinel-1. This revealed distinct patterns of feature influence on yield prediction, facilitating the optimization of the feature set for maximum effectiveness. Key radar polarization bands, VV (Vertical-Vertical) and VH (Vertical-Horizontal), provided crucial surface backscatter data, capturing information on crop structure, growth stages, and post-harvest soil conditions. Notably, the feature min_vh consistently emerged as the most significant predictor.

The implementation of our feature reduction strategy resulted in significant improvements in both model performance and computational efficiency. By removing 15-20 number of identified negatively contributing features, we achieved approximately 3-5% improvement in prediction accuracy while substantially reducing the computational overhead and model training time. This enhancement in efficiency did not compromise the model's interpretability, demonstrating the robust nature of our framework.

Our methodology represents a significant advancement in agricultural modeling by successfully addressing the challenges of high-dimensional data while maintaining model interpretability. The framework's ability to identify and eliminate non-contributing features while improving prediction accuracy demonstrates its potential for wide-scale application in agricultural yield prediction. Furthermore, the reduced computational requirements make it a practical solution for real-world applications where computational resources may be limited.

These results validate the effectiveness of our integrated approach in handling complex agricultural data while providing actionable insights for yield prediction. The framework offers a scalable, interpretable, and computationally efficient solution that can be adapted for various agricultural prediction tasks, potentially transforming how we approach agricultural yield forecasting.

How to cite: Dey, A., Saha, A., Sarkar, S., Mondal, A., and Mitra, P.: An Explainable AI-Driven Feature Reduction Framework for Enhanced Agricultural Yield Prediction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7965, https://doi.org/10.5194/egusphere-egu25-7965, 2025.

EGU25-9946 | ECS | Posters virtual | VPS2

 Long-term changes in black carbon aerosols and their health effects in rural India during the past two decades (2000–2019) 

Mansi Pathak, Jayanarayanan Kuttippurath, and Rahul Kumar

Black carbon (BC) is a short-lived atmospheric aerosol having light absorbing properties with climate-changing potential. In addition, BC aerosols are also responsible for several adverse health effects including cardiovascular and respiratory problems. Here, we examine the long-term changes in BC, using MERRA-2 (Modern-Era Retro spective analysis for Research and Applications) and Emissions Database for Global Atmospheric Research (EDGAR) data for the period 2000–2019, and the associated health burden in rural India. This study finds a decreasing trend in BC in the rural IGP (Indo-Gangetic Plain) and NWI (North West India) during 2007–2019, at about -0.004 and –0.005 μg/m3/yr, respectively. A significant reduction in BC (from 0.03 to 0.01 μg/m3/yr after 2006) is observed in the rural Peninsular India (PI), where the reduced wind speed limits the transport of BC aerosols from other regions and thus, limits the BC concentration there. Our assessment finds that government policies such as BS (Bharat Stage) emission norms, electrification of rail routes, use of electric and compressed natural gas-based vehicles, the transformation of brick kilns to zig-zag technology, mechanised farming for on- site handling of crop residues and recent changes in atmospheric drivers (e.g. winds in IGP) contributed to this reduction in BC. However, the health burden associated with BC causes the highest all-cause mortality to be around 5,17,651 and 34,082 inhabitants in winter (December-February) and post-monsoon (October-November) seasons, respectively, in the rural IGP in the latest year 2019. In brief, the reduction of BC in rural India indicates that it complements the government policies. However, an improvement in the policy implementation might prove to be conducive to reduce the BC-driven mortality and regional climate warming.

How to cite: Pathak, M., Kuttippurath, J., and Kumar, R.:  Long-term changes in black carbon aerosols and their health effects in rural India during the past two decades (2000–2019), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9946, https://doi.org/10.5194/egusphere-egu25-9946, 2025.

EGU25-10268 | Posters virtual | VPS2

Bridging the Gap: Smart Benches for Accessible Urban Air Quality Monitoring and Public Engagement in the Region of Attica 

Vasiliki Assimakopoulos, Kyriaki - Maria Fameli, Angelos Kladakis, Chrysanthi Efthymiou, Chrysa Charalampidou, Maria Sotiropoulou, Iro – Maria Antoniou, Aikaterini Kytrilaki, Alex Massas, and Margarita-Niki Assimakopoulos

The rapid urbanization of modern cities presents significant challenges, with air pollution emerging as a critical concern for public health and environmental sustainability. In Greece, while the government collects extensive air quality data as mandated by the EU Directive 2881/2024 (recast of 2008/50, 2004/107), limited efforts are made to communicate this data to the public. The existing network of large monitoring stations is often inaccessible to the pubic and primarily serving scientists and policymakers.

Addressing this gap, the FAIRCITY (ATTP4-0360457) project—a collaboration between the National Observatory of Athens, the National and Kapodistrian University of Athens and the Greek Innovation Company Energy4Smart—introduces the “Smart Stations” an innovative solution incorporating public benches powered by photovoltaics, equipped with free charging sockets for people with electrical wheelchairs as well as other smart city sevices, with embedded low cost air quality sensors, designed to make air quality data accessible, timely, and engaging. This initiative not only aligns with global sustainability goals but also serves as a model for other cities seeking to improve urban liveability. The low-cost sensors embedded within the bench at a height of approximately 3 meteres above ground, were selected based on size, technology and price criteria to continuously monitor eight key pollutants: three fractions of Particulate Matters (PM1, PM2.5, PM10), carbon monoxide (CO), carbon dioxide (CO2), nitrogen dioxide (NO2), ozone (O3) and sulfur dioxide (SO2).

The Smart Stations are deployed in open, public spaces (e.g., commercial areas, residential zones, parks), at a distance from major pollutant sources and in collaboration with interested municipalities of the Attica Region. Their aim is to record the local air quality and pollutant diurnal variations in order to highlight the sources responsible (i.e., Korydallos high NO2, NO, PM concentrations from traffic) and estimate the population exposure. Citizens can walk up to these stations, sit down and instantly access critical information about their local air quality from digital displays that provide in near real-time the simplified Air Quality Index (AQI) along with health protection and other environmental infomation.

Preliminary results indicate that the diurnal variations of the monitored pollutants follow closely the local anthropogenic activities (traffic by passing the area, central heating, cooking). The pollutant levels are similar across the different municipalities, presenting peaks at different times depending on the type of area. The hourly AQI is mainly affected by larger scale events such as an extensive air pollution episode or dust intrusion event.  

How to cite: Assimakopoulos, V., Fameli, K.-M., Kladakis, A., Efthymiou, C., Charalampidou, C., Sotiropoulou, M., Antoniou, I. –. M., Kytrilaki, A., Massas, A., and Assimakopoulos, M.-N.: Bridging the Gap: Smart Benches for Accessible Urban Air Quality Monitoring and Public Engagement in the Region of Attica, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10268, https://doi.org/10.5194/egusphere-egu25-10268, 2025.

EGU25-10631 | ECS | Posters virtual | VPS2

Harmonizing Low-Cost Air Quality Sensors for a Hybrid Monitoring Network 

Alexandru Luchiian

Air quality monitoring is crucial for assessing environmental health and supporting mitigation strategies. This research focuses on the co-location of various low-cost particulate matter (PM) sensors—uRADMonitor, AirGradient, PurpleAir, Clarity, and sensors from community initiatives—alongside a mobile laboratory equipped with a reference-grade GRIM EDM 180 analyzer. The primary goal is to identify and quantify bias among these low-cost sensors for PM2.5 and PM10 measurements at the same location.

By systematically analyzing the measurement discrepancies, a generalized correction formula is derived, enabling the harmonization of readings across different sensor types. The corrected data will form the basis of a hybrid air quality monitoring network, which standardizes PM2.5 and PM10 concentrations regardless of the sensor manufacturer. This approach leverages the affordability and scalability of low-cost sensors while ensuring data quality comparable to reference instruments.

The results aim to address limitations in the current low-cost sensor ecosystem, enhance interoperability, and provide communities and policymakers with reliable, high-resolution air quality data. Ultimately, this study supports the development of inclusive and sustainable monitoring frameworks that empower both urban and rural regions with actionable environmental insights, using all kinds of sensors.

How to cite: Luchiian, A.: Harmonizing Low-Cost Air Quality Sensors for a Hybrid Monitoring Network, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10631, https://doi.org/10.5194/egusphere-egu25-10631, 2025.

EGU25-11635 | ECS | Posters virtual | VPS2

Spatio-Temporal Distribution of PM 2.5 and its Association with Agricultural Fires in Northern Argentina. 

Rodrigo G. Gibilisco, Mariela Aguilera Sammaritano, Facundo Reynoso Posse, Kathrin Huber, Jazmín Elizondo, Sofía Torkar, María Marta Saez, Ariel Scaglioti, Florencia Tames, Enrique Puliafito, María José Castellano, Mariana Diaz, Nicolás Parellada, Gustavo Ciancaglini, Bettina Schillman, Ralf Kurtenbach, Peter Wiesen, Antonio Caggiano, Aída Ben Altabef, and Mariano Teruel

Agricultural burning in Tucumán, Argentina, has been a major contributor to air pollution, particularly during the dry season (April to September). This environmental issue is mainly due to the limited availability of modern machinery for sustainable harvesting, leading to heavy reliance on traditional biomass burning for crop residue management. The combustion process generates large amounts of fine particulate matter (PM2.5), which severely affects air quality and public health. To address this challenge, an inter-institutional collaboration under the Networking Initiative Breathe2Change.org, supported by the Alexander von Humboldt Foundation, facilitated the creation of the first air quality monitoring network in Tucumán. This initiative aimed to raise awareness and provide actionable data to local communities and scientists.

A custom sensor module was designed, integrating an OPC Plantower PMS5003 sensor for real-time PM2.5 detection, CO2 sensors using NDIR technology, as well as humidity and temperature sensors. A forced ventilation system was also incorporated to ensure representative air circulation inside the module without affecting airflow into the OPC sensor. The network, consisting of 25 sensor modules deployed throughout the 22,500 square kilometers of Tucumán, provided continuous data collection for 12 months in 2023. The data were shared on a publicly accessible data platform, developed as part of the Breathe2Change Initiative, which facilitated both citizen consultation and analysis by the scientists involved in the project.

During an initial 3-week intercomparison phase, 10 sensor modules were assessed for consistency, yielding a high correlation (R² > 0.9), confirming the reliability of the modules. Afterward, 23 of the 25 sensors were deployed across urban, suburban, and rural areas, including regions directly affected by agricultural fires. High- and low-flow reference samplers were used to collect daily PM2.5 concentrations from August to December, coinciding with the peak biomass burning period. During this period, two of the sensor modules were co-located with the reference samplers to allow for direct comparison. This phase was essential for deriving a local correction factor for the sensors.

Results showed considerably high PM2.5 concentrations, with monthly averages exceeding 60 µg/m³ in fire-impacted areas, well above the daily limits set by the World Health Organization (WHO). Even urban areas recorded average levels of 30 µg/m³, surpassing WHO guidelines. The region’s mountainous terrain and climate further exacerbated the pollution, triggering thermal inversion phenomena that trapped pollutants near ground level. Using the corrected sensor network, spatial distribution maps of PM2.5 were generated through Kriging interpolation, revealing a strong correlation between elevated pollutant levels and fire activity. Higher PM2.5 concentrations were observed in the central-eastern part of the province, likely linked to sugarcane production areas, and possibly influenced by rural traffic and biomass burning. Kriging analysis confirmed this spatial trend, with a marked reduction in localized concentrations after September, likely due to rainfall events.

This study underscores the degradation of air quality during biomass burning events and the need for regulatory measures and sustainable agricultural practices to mitigate environmental and health impacts. It also highlights the potential of low-cost sensors as effective tools for monitoring air pollution in resource-limited regions.

How to cite: Gibilisco, R. G., Aguilera Sammaritano, M., Reynoso Posse, F., Huber, K., Elizondo, J., Torkar, S., Saez, M. M., Scaglioti, A., Tames, F., Puliafito, E., Castellano, M. J., Diaz, M., Parellada, N., Ciancaglini, G., Schillman, B., Kurtenbach, R., Wiesen, P., Caggiano, A., Ben Altabef, A., and Teruel, M.: Spatio-Temporal Distribution of PM 2.5 and its Association with Agricultural Fires in Northern Argentina., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11635, https://doi.org/10.5194/egusphere-egu25-11635, 2025.

EGU25-13882 | ECS | Posters virtual | VPS2

Leveraging Large Language Models for Enhancing and Reasoning Adverse Weather Hazard Classification 

Adarsha Neupane, Nima Zafarmomen, and Vidya Samadi

Severe weather events often develop rapidly and cause extensive damage, resulting in billions of dollars in losses annually. This paper explores Large Language Models (LLMs) to effectively reason about the adversity of weather hazards. To tackle this issue, we gathered National Weather Service (NWS) flood reports covering the period from June 2005 to September 2024. Two pre-trained LLMs including Bidirectional and Auto-Regressive Transformer (BART) models (large) and Bidirectional Encoder Representations from Transformers (BERT) were employed to classify flood reports according to predefined labels. These models encompass a range of sizes with parameter counts of 406 million, and 110 million parameters, respectively. We employed the Low-Rank Adaptation (LoRA) fine-tuning technique to enhance performance and memory efficiency. The fine-tuning and few-shot learning capabilities of these models were evaluated to adapt pre-trained language models for specific tasks or domains. The methodology was applied in Charleston County, South Carolina, USA— a vulnerable region to compound flooding. Extreme events reported during the training periods were unevenly distributed across training period, resulting in imbalanced datasets. The “Cyclonic” category represents significantly fewer instances in the report text data, while the “Flood” and “Thunderstorm” categories appeared more frequent.  The findings revealed that while few-shot learning significantly reduced computational costs, fine-tuned models resulted in more stable and reliable performance. Among multiple LLMs applied in this research, the BART model achieved higher F1 scores in the “Flood,” “Thunderstorm,” and “Cyclonic” categories—requiring fewer training epochs to reach optimized performance levels. Furthermore, the BERT model demonstrated a shorter overall training time (12 hours 17 minutes) compared to other LLMs, demonstrating efficient cost of computing. This comprehensive evaluation of LLMs across diverse NWS flood reports enhanced our understanding of their capabilities in text classification and offered valuable insights into leveraging these advanced techniques for weather disaster assessment.

How to cite: Neupane, A., Zafarmomen, N., and Samadi, V.: Leveraging Large Language Models for Enhancing and Reasoning Adverse Weather Hazard Classification, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13882, https://doi.org/10.5194/egusphere-egu25-13882, 2025.

EGU25-14960 | Posters virtual | VPS2

Air Quality Assessment In The University Of The Philippines Diliman Campus Through The Integration Of Small Sensors, Satellite Data, And Kriging Interpolation Techniques 

John Richard Hizon, Rodyvito Angelo Torres, Adrian Cahlil Eiz Togonon, Bernadette Anne Recto, Frauline Anne Apostol, Percival Magpantay, John Jairus Eslit, Jomari Ganhinhin, Marc Rosales, Isabel Austria, Jaybie de Guzman, Maria Theresa de Leon, Rhandley Cajote, Paul Jason Co, and Roseanne Ramos

Air quality monitoring is an essential procedure to ensure that pollutant levels remain within safe limits and do not pose a threat to public health, particularly for vulnerable populations. The deployment and maintenance of stationary air quality monitoring stations can be expensive, especially when a large number is required to create a comprehensive network. As a result, there has been growing interest in utilizing small, low-cost sensors that are easier to deploy and provide a more flexible and cost-effective alternative. In addition to these sensors, satellite systems have become valuable tools for air quality monitoring, offering high temporal resolution data that facilitates the assessment of air pollution over larger areas. This study looks into data fusion techniques to combine data from both stationary and mobile low-cost sensors with satellite data to analyze the air quality at the University of the Philippines, Diliman campus. Seven small sensors were deployed across the university, a mixed-use area with both vegetation and buildings, to measure pollutant concentrations, such as particulate matter. Satellite data from MODIS, Sentinel-5P, and ERA5 reanalysis were used to monitor aerosol optical depth (AOD), sulfur dioxide (SO2), nitrogen dioxide (NO2), and meteorological conditions. The time-series analysis focused on a three-day period during which mobile air quality data from an e-trike were collected around the university. The data from these mobile sensors, along with the stationary sensor measurements, were used to estimate PM2.5 concentrations across the campus. Kriging interpolation, a geostatistical method that estimates unknown values based on the spatial correlation of known data points, was employed to generate smooth surfaces of PM2.5 concentration across the university.  Kriging interpolation was used on the stationary sensor dataset to predict the PM2.5 levels at the location of the mobile sensors at a given timeframe. Moreover, cokriging was also applied by incorporating multiple correlated variables, improving predictions by utilizing relationships between the primary variable (PM2.5) and secondary variables, such as aerosol optical depth or SO2 and NO2 concentrations. The results obtained from both Kriging and Cokriging methods were compared with data collected from mobile sensors to assess the air quality at the University of the Philippines, Diliman. The interpolated PM2.5 values were compared with the data from the mobile sensors (SEN55 and PMS7003) as ground truth, and a mean absolute percentage error (MAPE) of 43.00% to 57.23% was obtained. Initial results of cokriging with NO2 showed MAPE of 36.67% to 52.55%. Further work is expanding the dataset and refining the interpolation models to enhance the accuracy and reliability of air quality assessments across the university. By integrating more data and conducting additional tests, this approach can provide more comprehensive air quality monitoring at reduced costs and address data gaps.

How to cite: Hizon, J. R., Torres, R. A., Togonon, A. C. E., Recto, B. A., Apostol, F. A., Magpantay, P., Eslit, J. J., Ganhinhin, J., Rosales, M., Austria, I., de Guzman, J., de Leon, M. T., Cajote, R., Co, P. J., and Ramos, R.: Air Quality Assessment In The University Of The Philippines Diliman Campus Through The Integration Of Small Sensors, Satellite Data, And Kriging Interpolation Techniques, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14960, https://doi.org/10.5194/egusphere-egu25-14960, 2025.

EGU25-14973 | Posters virtual | VPS2

Automated Nighttime Fog Detection and Masking Using Machine Learning from Near Real-Time Satellite Observations 

Narendra Reddy Nelli, Diana Francis, Cherfeddine Cherif, Ricardo Fonseca, and Hosni Ghedira

Fog significantly reduces visibility, impacting transportation and safety, particularly in regions like the United Arab Emirates (UAE) where it is a regular
occurrence, in particular in the winter months. This study develops a machine learning-based approach for automated fog detection and masking from near real-time observations from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) instrument onboard the Meteosat Second Generation spacecraft to enhance fog detection and forecast. We evaluated six basic machine learning (ML) models trained with four different methods: (1) supervised training using SEVIRI pixel data and fog observations over airport stations; (2) as approach (1) but incorporating infrared channel data; (3) training with labeled fog and no-fog regions identified in SEVIRI night microphysics Red-Green-Blue (RGB) images through k-means clustering; and, (4) a fusion approach combining station-labeled data (approach 1) and k-means clustered-labeled data (approach 3). Among the models, the eXtreme Gradient Boosting (XGBoost) demonstrated slightly higher performance. Models trained on station data (approach 1) achieved a Probability of Detection (POD) of 0.73 and a False Alarm Ratio (FAR) of 0.11. For spatial fog masking, models trained on a combination of station-labeled and k-means cluster-labeled data (approach 4) performed best. Overall, the XGBoost method and the fusion approach (4) are recommended for fog detection and masking in the hyper-arid UAE. These findings demonstrate the potential for trained ML models to deliver accurate, near real-time fog detection and masking, enhancing monitoring over broad areas.

How to cite: Nelli, N. R., Francis, D., Cherif, C., Fonseca, R., and Ghedira, H.: Automated Nighttime Fog Detection and Masking Using Machine Learning from Near Real-Time Satellite Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14973, https://doi.org/10.5194/egusphere-egu25-14973, 2025.

EGU25-15784 | ECS | Posters on site | AS1.24

Changes in MJO Propagation Characteristics and Regional Variations under a Changing Climate 

Hye-Ryeom Kim and Kyung-Ja Ha

The Madden-Julian Oscillation (MJO) is a crucial atmospheric phenomenon characterized by large-scale, eastward-propagating disturbances in the tropical atmosphere. It profoundly influences global climate and weather patterns and serves as a key source of predictability for subseasonal forecasts. In particular, the propagation characteristics of the MJO are critical parameters that impacts the timing and intensity of its effects. Variability in these characteristics can alter the MJO’s interaction with other climate components, thereby affecting weather patterns. Therefore, it is essential to investigate the variability of MJO propagation characteristics.

In this study, we aim to examine the changes in propagation characteristics of the MJO, such as propagation speed, across three primary regions: Indian Ocean, Maritime Continent, western Pacific. These changes will be compared between two distinct period (P1: 1979-1998, P2: 2003-2022). Furthermore, we will investigate the mechanisms driving variations in MJO propagation speed within each tropical region and assess potential future changes using reanalysis data and model outputs. By addressing these questions, this study can contribute to improve the predictability and accuracy of climate models in representing the MJO.

How to cite: Kim, H.-R. and Ha, K.-J.: Changes in MJO Propagation Characteristics and Regional Variations under a Changing Climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15784, https://doi.org/10.5194/egusphere-egu25-15784, 2025.

 In order to solve the problem of quantity traceability of precipitation phenomenon instrument, a precipitation phenomenon checking device was developed. By simulating the precipitation particles of 4.3 mm and 9.5 mm, corresponding to the velocities of 2m/s, 7M/s and 12M/s respectively, the on-site verification of the precipitation phenomenometer and the test program of the upper computer software are carried out, the relevant particle channels are recorded and displayed in the map, and the performance of the precipitation phenomenometer is judged automatically. It has many advantages, such as complete function, reasonable design, easy to carry, friendly software interface, one-button detection, automatically judge whether the equipment is qualified, and according to the template to generate a verification report. The practical application proves that the device provides a strong support for the meteorological department's equipment support personnel to carry out the verification work of the precipitation phenomenometer, improves the working efficiency, and plays a role in supervising and inspecting the quality of the precipitation phenomenometer's equipment, it has a good application prospect in the field verification of precipitation phenomenometer.

How to cite: Han, Y.: Development and application of the calibration device of precipitation phenomenometer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17395, https://doi.org/10.5194/egusphere-egu25-17395, 2025.

EGU25-17568 | ECS | Posters virtual | VPS2

Improving forecasts of extreme precipitation with MAD-WRF mesoscale model 

Anton Gelman, Efrat Morin, Pedro Jiménez, Rong-Shyang Sheu, and Dorita Rostkier-Edelstein

The Multi-sensor Advection Diffusion Weather Research and Forecast (MAD-WRF) model is a state-of-the-art addition to the WRF model that includes a fast cloud-initialization procedure, making it more suitable for hydrometeors analysis and clouds forecasts. The MAD-WRF cloud initialization combines a cloud parameterization that infers the presence of clouds based on relative humidity with observations of the cloud mask and cloud top/base height to provide a three-dimensional cloud analysis. During the forecasts, the hydrometeors can be advected and diffused with no microphysics, in what we refer to as the MAD-WRF passive mode. Alternatively, these passive hydrometeors can be integrated into the explicitly resolved hydrometeors during a nudging phase, designated the MAD-WRF active mode (Jiménez et al., 10.1016/j.solener.2022.04.055). As such, MAD-WRF has been extensively used for solar energy predictions.

Here we have investigated the feasibility of using MAD-WRF to improve the accuracy of intense precipitation forecasts. An extreme precipitation event over Israel that led to urban floods and two casualties in Tel-Aviv during January 4th, 2020, has been chosen as a case study. The extreme accumulated precipitation responsible for noon and early afternoon floods was triggered by a persistent cloud train that developed over the area several hours before. MAD-WRF model has been configured with 3-nested domains with 9, 3 and 1 km grid-sizes. We have run MAD-WRF in active mode incorporating satellite-retrieved cloud-top heights provided by the European Space Agency EUMETSAT in all three domains. EUMETSAT data are available in near real-time making it suitable for operational forecasts.

Independent precipitation data measured by the Israel Meteorological Service radar at Bet-Dagan (about 10 km south-east of Tel-Aviv) has been used for forecasts verification. Comparison between radar data and MAD-WRF forecasts with and without incorporation of EUMETSAT cloud-tops retrievals reveal the advantage MAD-WRF cloud initialization. The significant improvement in the forecast of the location and rate of the precipitation is observed up to 12 hours ahead in time.

On-going work focuses on the evaluation of the precipitation distributions and improvement of the forecast of dry areas.

How to cite: Gelman, A., Morin, E., Jiménez, P., Sheu, R.-S., and Rostkier-Edelstein, D.: Improving forecasts of extreme precipitation with MAD-WRF mesoscale model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17568, https://doi.org/10.5194/egusphere-egu25-17568, 2025.

EGU25-19687 | ECS | Posters virtual | VPS2

Verification of weather variables linked to Dengue incidence inthe sub‐seasonal scale in Vietnam 

Iago Perez, Sarah Sparrow, Antje Weisheimer, Matthew Wright, and Lucy Main

Dengue fever outbreaks impose a severe healthcare burden in Vietnam, therefore the development of an early Dengue warning system is key to improve public health planning and mitigate the future burden produced by this disease. This study assessed the ECMWF ensemble re-forecast skill for relative humidity, temperature and precipitation, which are key factors for vector-borne disease transmission in Vietnam between 1-4 weeks in advance. We focused the analysis on the rainy season (May-October) using ERA5 reanalysis as a reference dataset. Re-forecast data was pre-processed using a quantile mapping technique to reduce the bias between re-forecast and observations. Results showed that corrected re-forecasts of weekly mean temperature, relative humidity and accumulated precipitation are skilful up to 2-3 weeks in advance and rank histograms verified the forecast reliability. Nonetheless the model is less skillful for the region of South Vietnam and seems to struggle at predicting extremely high/low values of temperature, relative humidity and precipitation. Results from this study demonstrate that ECMWF ensemble forecasts are suitable to use as inputs for a dengue early warning system up to 14-21 days in advance

How to cite: Perez, I., Sparrow, S., Weisheimer, A., Wright, M., and Main, L.: Verification of weather variables linked to Dengue incidence inthe sub‐seasonal scale in Vietnam, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19687, https://doi.org/10.5194/egusphere-egu25-19687, 2025.

EGU25-20267 | ECS | Posters virtual | VPS2

Air Quality Monitoring in Nairobi City, Kenya: Role of Collocation in Low Cost Sensor Deployment  

Joshua Nyamondo, Nicholas Oguge, Stephen Anyango, Augustine Afulloh, Noah Adera, and Beldine Okoth

Background: The increasing availability and usage of low-cost air quality sensors (LCS) presents both opportunities and challenges in terms of data accuracy, reliability, precision and interpretation. Various low cost sensors types differ in the degree of accuracy reliability and precision They can also be influenced by environmental conditions like temperatures and humidity. This study assesses three LCS, E-Samplers, ModulairTM and AirQO, deployed alongside a reference-grade Beta Attenuation Monitor (BAM-1022) in Nairobi, Kenya, to upraise their performance under varying conditions and explore the strategies for calibration and integration into the monitoring networks.

Methods: The study used BAM-1022 data to validate and calibrate the LCS installed at the University of Nairobi’s Parklands Campus (27 February 2024 to 26 December 2024).  We analyzed sensor accuracy, precision and response to pollution across wet and dry seasons and varying temperature and humidity levels. We aligned the LCS data with BAM-1022 measurements using tailored correction factors and multiple linear regression (MLR) models. We used the coefficient of determination, represented by R-squared (R2), a statistical measure of how close the data from the LCS are from the data from the BAM and the Pearson correlation, r to show the strength of the linear relationship between the sensor measurements and reference measurements. Additionally, we conducted paired t-tests to determine whether statistically significant differences existed between the BAM-1022 and each LCS, and one-sample t-tests to find out if there was a statistically significant difference in the values recorded by low-cost sensors themselves. The study also explored the potential of LCS to improve spatial coverage and resolution while addressing challenges like sensor drift and environmental interference.

Results: The ModulairTM sensor showed closer measurements in reference to BAM-1022 measurements (R2= 0.82, r =0.9458) followed by AirQO (R2=0.54, r =0.8933) and E-Sampler (R2=0.36, r =0.7166). During wet season, ModulairTM maintained the closer measurements (R2=0.73, r =0.9123) with AirQO (R2=0.36, r =0.7219) and E-Sampler (R2=0.21, r =0.7812) showing lower alignment. Similar trend was observed in dry season with ModulairTM (R2=0.8, r=0.8124) followed by AirQO (R2=0.51, r=0.7001) and E-Sampler (R2=0.28, r=0.6996). During high PM2.5 concentration periods (July to December), ModulairTM reported higher values than the BAM on certain days. AirQO generally recorded lower values except during these high concentration periods while the E-Samplers fluctuated between higher or lower values across the collocation period. Consequently, correction factors of -12.5, 31.55 and 29.65 were derived for ModulairTM,AirQO and E-Samplers respectively. Statistical analysis revealed a significant difference between the BAM measurements and LCS (p-value < 0.001). However, no significant differences were observed between the measurements of each of the low-cost sensors.

Conclusion: The LCS can enhance air quality monitoring networks when collocated appropriately and, consistently and carefully calibrated. The readings should be corrected against reference sensor for accurate and reliable data.  Collocation with reference monitors or among the LCS units for regions with limited access to high-end monitoring infrastructure such as Nairobi is key before deployment. Air quality modeling can create a comprehensive monitoring networks hence improved spatial resolution and public health insights. 

How to cite: Nyamondo, J., Oguge, N., Anyango, S., Afulloh, A., Adera, N., and Okoth, B.: Air Quality Monitoring in Nairobi City, Kenya: Role of Collocation in Low Cost Sensor Deployment , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20267, https://doi.org/10.5194/egusphere-egu25-20267, 2025.

Tropical deep convective clouds (DCCs) play a pivotal role in Earth's hydrological cycle, with their dynamics strongly influenced by aerosols. Depending on their properties, aerosols can either invigorate or suppress cloud formation and development. Previous observational studies and cloud-resolving model simulations have shown that aerosols such as black carbon (BC) and sulfates modify cloud microphysics, affecting droplet size distribution, latent heat release, and precipitation patterns. However, the use of global climate models (GCMs) to study these aerosol-cloud interactions remain limited, despite their ability to capture large-scale circulation patterns and associated non-linear feedback. This study investigates the sensitivity of aerosol-induced cloud invigoration and suppression (AIVe) to major aerosol species during the Indian summer monsoon (ISM) season using the Community Earth System Model, specifically its atmospheric component, the Community Atmosphere Model version 5 (CESM-CAM5). The analysis focuses on DCCs over central India during the monsoon months of June–September (JJAS) for the period 2005–2008. Aerosol and cloud parameters from CESM-CAM5 simulations, conducted at 0.5-degree horizontal resolution, are compared with satellite observations. Five Atmospheric Model Intercomparison Project (AMIP)-style simulations were performed: one with aerosols at pre-industrial level (PI) levels, another at present-day (PD) levels, and three additional simulations perturbing specific aerosol species (dust, BC, and sulfate) under PD conditions to isolate their individual effects on AIVe. The findings highlight that aerosol physico-chemical properties critically influence DCC behavior. Black carbon near the boundary layer increases cloud condensation nuclei (CCN) concentrations, delaying precipitation, enhancing warm-phase invigoration, and strengthening updrafts. In the upper troposphere, BC absorbs solar radiation, causing atmospheric warming that promotes cloud deepening and cold-phase processes. Additionally, BC intensifies both shortwave and longwave heating, prolonging cloud lifetimes and supporting deeper convection. Sulfate aerosols primarily enhance warm-phase invigoration through increased CCN concentrations at lower altitudes. However, their weaker vertical transport limits their impact on cold phase processes and deep convection compared to BC and dust. Dust aerosols with high concentrations in the mid-troposphere, act as efficient ice-nucleating particles (INPs), enhancing cold phase invigoration. However, suppressed updrafts in the upper troposphere reduce their overall effect on deep convective systems, emphasizing the importance of aerosol size, number concentration, and properties in shaping AIVe. This study underscores the complex interplay between aerosol characteristics and their vertical distribution in influencing cloud dynamics during the ISM. Detailed results and further implications will be presented.

How to cite: Sharma, P., Ganguly, D., and Kant, S.: Sensitivity of Cloud Invigoration and Suppression Effects to Major Aerosol species During the Indian Summer Monsoon in a Global Climate Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-886, https://doi.org/10.5194/egusphere-egu25-886, 2025.

EGU25-1100 | ECS | Posters on site | AS3.22

Modulation of temporal evolution of black carbon aerosols at a rural location in the Western Ghats by meteorology and boundary layer dynamics 

Devika Sunil S, Anand Narayana Sarma, Sunilkumar Kudilil, Satheesh Sreedharan Krishnakumari, and Krishnamoorthy Krishnaswamy

Black carbon (BC) aerosols have been reported to influence the precipitation patterns over South-East Asia. In this study, we present surface measurements of BC carried out from a rural location in the Western Ghats and covering all the seasons. Despite being a remote location with negligible anthropogenic emissions, the total BC concentration is strongly modulated by particles originating from fossil fuel burning (~75%). Contrary to the prominent role played by boundary layer dynamics in the diurnal variations of BC in the tropics, our measurements reveal a disconnection between boundary layer dynamics and BC concentration mostly due to the advection from a distant urban location being the dominant source of BC. However, this influence is conspicuous on the concentration of particles originating from biomass burning. Seasonal variations in the wind fields, surface temperature, and rainfall are observed to influence the BC concentration, thereby leading to distinct diurnal variations seldom reported elsewhere. Reanalysis data sets fail to capture these changing patterns in BC, with daily mean concentrations exhibiting large differences with our observations (particularly in winter months) and diurnal patterns being different throughout the season. Under this backdrop, incorporation of these measurements could possibly improve the monsoon forecast in global climate models and provide deeper insights on the role of meteorology and boundary layer dynamics on aerosol fields in complex environments.

How to cite: Sunil S, D., Narayana Sarma, A., Kudilil, S., Sreedharan Krishnakumari, S., and Krishnaswamy, K.: Modulation of temporal evolution of black carbon aerosols at a rural location in the Western Ghats by meteorology and boundary layer dynamics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1100, https://doi.org/10.5194/egusphere-egu25-1100, 2025.

EGU25-1370 | ECS | Posters virtual | VPS3

Evaluating WRF-Chem for simulating fog episodes: A Case Study from The National Capital Region Delhi, India 

Anie K Lal, Ravi Kumar Kunchala, and Manju Mohan

During winter, dense fog occurrences in the Indo-Gangetic Plain pose severe risks to visibility, air quality, and public health, emphasizing the need for improved fog forecasting in India. This study employs a high-resolution WRF-Chem model (2 km × 2 km) to identify optimal configurations for simulating fog in the region and investigate the impact of urbanization-induced UHI/UDI (Urban Heat Island/Urban Dry Island) and elevated emissions on the fog life cycle in and around the megacity of Delhi.

A comprehensive sensitivity analysis explores model configurations across microphysics, planetary boundary layer (PBL), land surface models (LSM), radiation schemes, chemistry, and emission inputs. Simulations of surface and vertical meteorology are evaluated against data from weather stations and radiosonde profiles, while modeled chemistry is compared with ground-based measurements. Results demonstrate that specific combinations of microphysics, PBL, and LSM schemes coupled with chemistry effectively simulate Liquid Water Content (LWC), a critical fog proxy. Modeled relative humidity, particulate matter concentrations, and fog life cycles show strong agreement with observations. We then utilize this optimized model configuration to quantitatively analyze individual and combined effects of urbanization and aerosols on fog formation.

How to cite: K Lal, A., Kunchala, R. K., and Mohan, M.: Evaluating WRF-Chem for simulating fog episodes: A Case Study from The National Capital Region Delhi, India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1370, https://doi.org/10.5194/egusphere-egu25-1370, 2025.

Satellite remote sensing has the advantage of wide spatial coverage and high data consistency, which is an important technology for global atmospheric environment monitoring. However, due to the influence of cloud cover, satellite remote sensing faces the problem of data missing; moreover, the direct object of hyperspectral satellite remote sensing is the total amount of pollution gases in the atmosphere, which is different from the near-ground concentration that directly affects human health. To solve these problems, this research developed a remote sensing technology combining satellite spectral analysis and artificial intelligence. We use artificial intelligence to increase the spatial coverage of satellite and ground-based remote sensing, and make future short term predictions and their applications. Preliminary results show that the reconstruction of satellite remote sensing data supported by artificial intelligence is of great significance for environmental pollution monitoring and control.

How to cite: Liu, C., Hu, Q., Li, Q., and Zhang, C.: Spatiotemporal reconstruction of gas pollutants with high resolution and coverage using hyperspectral remote sensing and artificial intelligence, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1923, https://doi.org/10.5194/egusphere-egu25-1923, 2025.

EGU25-2082 | ECS | Posters virtual | VPS3

Exploring the Nexus of Two-Wheeler Gaseous Contributions and Driver Exposure in a Million-Plus Population City 

Saket Ranjan, Sudheer K. Kuppili, and Shiva Nagendra SM

In Indian metropolitan cities, two-wheelers (2W) constitute 60–70% of traffic, making their emissions a significant contributor to urban air pollution. This study measured 2W exhaust emissions and driver exposure under real-world traffic conditions in the Chennai metropolitan area. Emission factors for CO, HC, and NO were 1.1, 0.02, and 0.03 g/km, respectively. However, limited studies on 2W are available due to the complexity of real-world measurements in Indian traffic conditions. The gaseous emissions from the measured vehicles are lower than their respective Bharat Stage (BS) standards except for CO. Personal exposure levels for PM10, PM2.5, and PM1 were 212.5, 78.1, and 58.9 µg/m³, with the highest exposures occurring during idling and driving behind heavy-duty vehicles. The Multiple Particle Path Dosimetry (MPPD) model was used to estimate the deposition fractions in the human respiratory tract (HRT). Results indicated that PM2.5 and PM1 deposition fractions are higher in the pulmonary region, whereas PM10 deposition is higher in the head region. 2W drivers are exposed to higher concentrations than any other motor vehicle driver. Since there is no substantiation of a tolerable limit of PM1 exposure or a threshold beyond which no detrimental health implications occur, cautious planning is needed when developing the roads.

How to cite: Ranjan, S., K. Kuppili, S., and Nagendra SM, S.: Exploring the Nexus of Two-Wheeler Gaseous Contributions and Driver Exposure in a Million-Plus Population City, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2082, https://doi.org/10.5194/egusphere-egu25-2082, 2025.

EGU25-2443 | Posters virtual | VPS3

Two Typical Case Studies of Volcanic Eruption Trace Gases Based on EMI Observations 

Yuhan Luo, Qidi Li, Kaili Wu, Yuanyuan Qian, Haijin Zhou, and Fuqi Si

Volcano eruption is one of the most destructive natural disasters, and its direct release of toxic gases and volcanic ash can lead to atmospheric pollution, posing significant threats to human health and ecological balance. To investigate the environmental impact of volcanic emissions, we retrieved the vertical column densities (VCDs) of sulfur dioxide (SO2) and bromine monoxide (BrO) using the Chinese highest-resolution atmospheric trace gas remote sensing satellite payloads: the Environmental Trace Gas Monitoring Instrument (EMI) series on-board the GaoFen (GF5-02) and DaQi (DQ-1) satellites.

Here, we present our study on two significant volcanic emission events. On January 15, 2022, a violent eruption occurred near the South Pacific Island nation of Tonga, which is a typical submarine volcano. During this eruption, the volcanic plume ascended directly into the stratosphere (above 20 km), releasing a substantial amount of SO2 and spreading rapidly westward (~30 m/s). In contrast, the majority of the BrO dispersed southeastward slowly (~10 m/s) within the altitude range of 8–15 km on January 16. The differences in eruption height and timing resulted in the transport of SO2 and BrO in distinct directions in the Southern Hemisphere.

Another case is the Sundhnukagigar volcano on Iceland's Reykjanes Peninsula, which is a typical fissure volcano. A significant eruption began at 21:00 on August 22nd, following an earthquake swarm; this was the largest eruption in the region since December 2023. Satellite data indicated that the volcanic eruption released high concentrations of SO2, with the maximum SO2 VCD exceeding 15 Dobson Units (DU). By the morning of the 26th, part of the air mass had been transported northward to the Arctic Svalbard region. Simultaneously, ground observations from Ny-Ålesund revealed that an unprecedented Arctic haze event occurred, with the SO2 VCD reaching approximately 40 times the usual level. It is also important to note that, in the context of global warming, the ongoing activity of Iceland's volcanoes will further exacerbate the melting of local glaciers and permafrost. This, in turn, disrupts the gravitational balance of the overlying crust, leading to an intensification of volcanic activity. Therefore, it is essential to employ multi-instrument, multi-scale, and high-resolution observations to monitor volcanic activity and assess its impact on both regional and global climate and the environment.

How to cite: Luo, Y., Li, Q., Wu, K., Qian, Y., Zhou, H., and Si, F.: Two Typical Case Studies of Volcanic Eruption Trace Gases Based on EMI Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2443, https://doi.org/10.5194/egusphere-egu25-2443, 2025.

EGU25-3222 | ECS | Posters virtual | VPS3

City-level Disparities in NOX Emission Trends and Their Inhibitory Effects on O3 Mitigation in China 

Hao Kong, Jintai Lin, Lulu Chen, Yuhang Zhang, and Sijie Wang

As a major air pollutant and precursor of ozone (O3), anthropogenic nitrogen oxides (NOX = NO + NO2) have been effectively controlled in China since peaking around 2012. However, the evolving contrast of emissions across cities and its impacts on secondary pollutants such as O3 remain poorly understood, primarily due to the limitations of existing emission inventories. Here we track the historical high-resolution (5 km) NOX emissions based on POMINO-OMI and POMINO-TROPOMI NO2 VCDs, adopting our previously developed inversion, PHLET. The results demonstrate significantly weaker NOX emission declines in economically small cities where environmental pollution received much less attentions, leading to a shift of emission burdens toward western and non-capital cities. Moreover, simulations based on GEOS-Chem indicate that such disparities in NOX emission trends have inhibited the mitigation of O3 mainly in the western China, and even added up to the O3 increase in some areas of the North China Plain. Our study points to the value of satellite-based inversion to access historical environmental regulations, and emphasizes the importance of collaborative pollution control across regions for comprehensive pollution control in China and other Global South countries undergoing rapid emission changes.

How to cite: Kong, H., Lin, J., Chen, L., Zhang, Y., and Wang, S.: City-level Disparities in NOX Emission Trends and Their Inhibitory Effects on O3 Mitigation in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3222, https://doi.org/10.5194/egusphere-egu25-3222, 2025.

EGU25-3841 | ECS | Posters virtual | VPS3

SeParation of Ice Nuclei via Density Layers (SPINDL): A new method for characterizing ice nuclei using density gradient centrifugation 

Gurcharan K. Uppal, Soleil E. Worthy, Lanxiadi Chen, Cally Yeung, Olenna McConville, and Allan K. Bertram

Atmospheric ice nucleating substances (INSs) play a crucial role in ice cloud formation above -35°C, impacting cloud radiative properties, cloud lifetime, and the hydrological cycle. Characterizing inorganic (e.g., mineral dusts, volcanic ash, metals) and organic (e.g., bacterial cells, fungal spores, pollen, and various biomacromolecules) INSs has typically involved: 1) single-particle analyses, which offer high resolution but require specialized equipment, and 2) bulk sample treatment (e.g., heat, H2O2, (NH₄)₂SO₄) analyses, which are more accessible but may overestimate or underestimate INS concentrations due to non-target effects. There is a need for additional methods to quantify inorganic and organic INSs concentrations in the atmosphere to test and improve climate models.

Here we show a new density gradient centrifugation method to differentiate and quantify inorganic (densities ≥ 2.1 g cm-3) and organic INSs (densities ≤ 1.6 g cm-3). Density gradient centrifugation was used to separate the INSs suspension into their respective density isolate. This was followed by a wash procedure consisting of sequential differential centrifugation and ultrafiltration. Lastly, the INSs were quantified using a droplet freezing assay.

Our method successfully recovered organic water-soluble INSs (lignin, birch pollen washing water and filtered Fusarium acuminatum) and organic water-insoluble INSs (Snomax and Pseudomonas syringae) in the low-density isolate. We recovered inorganic water-insoluble INSs (K-feldspar) in the high-density isolate. In an INS mixed suspension, we recovered K-feldspar in the high-density isolate and lignin in the low-density isolate both at concentrations similar to the isolated K-feldspar or lignin tests. 

This work demonstrates the broad applicability of density gradient centrifugation for characterizing a wide range of inorganic and organic atmospheric INSs.

 

How to cite: Uppal, G. K., Worthy, S. E., Chen, L., Yeung, C., McConville, O., and Bertram, A. K.: SeParation of Ice Nuclei via Density Layers (SPINDL): A new method for characterizing ice nuclei using density gradient centrifugation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3841, https://doi.org/10.5194/egusphere-egu25-3841, 2025.

EGU25-4493 | Posters virtual | VPS3

Comparison of nitrogen dioxide tropospheric columns retrieved by TEMPO and Pandora 

Alexander Radkevich, Hazem Mahmoud, and Daniel Kaufman

Monitoring emissions of nitrogen dioxide is crucial for understanding the atmospheric composition and its impacts on air quality and climate. This study aims to evaluate the accuracy of retrievals of nitrogen dioxide tropospheric column by the Tropospheric Emissions: Monitoring of Pollution (TEMPO) by comparing them against retrievals of the ground-based Pandora instruments.

The TEMPO is a visible and ultraviolet spectrometer flying aboard of a commercial telecommunications satellite, Intelsat 40e, in geostationary orbit over 91˚ W longitude, thus maintaining a continuous view of North America. High resolution measurements of radiance reflected by the Earth's back to the instrument's detectors enable retrievals of columns of nitrogen dioxide involved in the chemical dynamics of Earth’s atmosphere. TEMPO V03 Level 1, 2, and 3 data were recently made available from the Atmospheric Science Data Center (ASDC) via NASA EarthData Search.

Direct-Sun Pandora spectrometer is used to retrieve columnar amounts of trace gases in the atmosphere by the means of differential optical absorption spectroscopy at numerous locations around the globe.

ASDC has developed a set of Jupyter notebooks dedicated to TEMPO vs. Pandora comparisons of the columns of individual trace gases including one dealing with NO2 tropospheric column. The notebooks allow a user to select a specific Pandora station and a timeframe of interest. The code downloads all relevant TEMPO L2 granules as well as the Pandora dataset. The latter is sub-set to the selected timeframe. Time series of the gas column retrievals along with their uncertainties are then derived with accounting for the quality flags from both datasets. Since Pandora measurements are significantly more frequent, a procedure computing weighted averages of them at the times of TEMPO retrievals was incorporated to the notebooks allowing direct comparison of gaseous columns from two sensors against each other.

The results derived by the ASDC tool show only qualitative agreement between the TEMPO and Pandora retrievals of nitrogen dioxide tropospheric column. it was also found that the discrepancies between the two are site dependent which may point to a potential problem with Pandora quality flags. Two attempts were made to improve comparison. Since TEMPO algorithm allows for negative NO2 tropospheric columns, such retrievals were removed from consideration. There are also multiple TEMPO retrievals accompanied by uncertainty greater that the retrieved column. Removal of such retrievals constitutes another approach to improve comparison.

The findings of this study will contribute to the understanding of the reliability and applicability of space-based trace gases monitoring for air quality applications. The results will enhance our understanding of atmospheric processes related to tropospheric NO2.

How to cite: Radkevich, A., Mahmoud, H., and Kaufman, D.: Comparison of nitrogen dioxide tropospheric columns retrieved by TEMPO and Pandora, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4493, https://doi.org/10.5194/egusphere-egu25-4493, 2025.

EGU25-4697 | ECS | Posters virtual | VPS3

Direct and indirect effects of biomass burning and dust aerosols under various synoptic processes during the April 2020 pollution case in Ukraine 

Mykhailo Savenets, Alexander Mahura, Roman Nuterman, and Tuukka Petäjä

Wildfires and dust storms significantly contribute to air pollution, causing adverse health impacts and intensifying various aerosol-meteorology feedbacks in the atmosphere through direct and indirect aerosol effects. These effects, however, are highly variable and depend on prevailing synoptic conditions. In April 2020, Ukraine experienced one of its most severe air pollution episodes, which had a profoundly negative impact on the Kyiv metropolitan area. This event was triggered by wildfires in the abandoned exclusion zone around the Chornobyl Nuclear Power Plant (northern Ukraine) and a dust storm that swept across the entire territory of Ukraine from the west to the east. Despite similar aerosol emissions – characterized by elevated levels of dust, organic carbon (OC), and black carbon (BC) – the atmospheric effects varied significantly under different synoptic processes during April 2020. This study presents seamless modeling results that analyze the meteorological response to direct (DAE) and indirect aerosol effects (IDAE) under varying synoptic conditions during this pollution episode in Ukraine.

Using the Environment – HIgh-Resolution Limited Area Model (Enviro-HIRLAM) at a 1.5 km horizontal resolution, four simulations/runs were conducted to investigate the role of aerosols: DAE run, IDAE run, combined aerosol effects (COMB run), and a reference (REF run) representing a standard Numerical Weather Prediction configuration without aerosol effects. The uniform and continuous effects of biomass burning and dust aerosols were primarily observed in radiation parameters, leading to a reduction in downwelling global and net short-wave radiation by 25-40 W/m². A clear correspondence between aerosol distribution and changes in the spatial patterns of other meteorological parameters was evident during the atmospheric fronts and the dust storm episode. Notably, the movement of a warm front caused near-surface air temperature to decrease and specific humidity to increase ahead of the front, with the opposite effects observed behind it. Compared to the REF run, these parameters exhibited local variations ranging from -2.6°C to +1.0°C for air temperature and from -1.5 g/kg to +1.0 g/kg for specific humidity. Aerosol effects during the stationary cold front led to an increase in air temperature and cloud liquid water content. However, transported sulfur aerosols significantly influenced these effects against the background of OC and BC emissions. In contrast, the subsequent dust storm and cold front had the opposite effect on air temperature, also impacting changes in turbulent kinetic energy. Most of these effects were associated with areas in model domain affected by elevated concentrations of dust, BC, and OC in their coarse and accumulation modes.

We acknowledge support through the grant HPC-Europa3 Transnational Access Programme for projects “Integrated modelling for assessment of potential pollution regional atmospheric transport as result of accidental wildfires”; projects Horizon Europe programme under Grant Agreement No 101137680 CERTAINTY (Cloud-aERosol inTeractions & their impActs IN The earth sYstem); project No 101036245 RI-URBANS (Research Infrastructures Services Reinforcing Air Quality Monitoring Capacities in European Urban & Industrial AreaS) and No 101056783 European Union via FOCI-project (Non-CO2 Forcers And Their Climate, Weather, Air Quality And Health Impacts).

How to cite: Savenets, M., Mahura, A., Nuterman, R., and Petäjä, T.: Direct and indirect effects of biomass burning and dust aerosols under various synoptic processes during the April 2020 pollution case in Ukraine, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4697, https://doi.org/10.5194/egusphere-egu25-4697, 2025.

EGU25-5297 | Posters virtual | VPS3

Sulfur dioxide trends in Iranian urban areas: assessing the impact of mitigation policies

Robabeh Yousefi, Fang Wang, Amaneh Kaveh-Firouz, Abdallah Shaheen, and Quansheng Ge

EGU25-5323 | ECS | Posters virtual | VPS3

Assessing black carbon dynamics in Iran: the role of urban growth and land use changes in long-term trends (1980–2023) 

Abdallah Shaheen, Robabeh Yousefi, Fang Wang, Amaneh Kaveh-Firouz, and Quansheng Ge

Black carbon (BC), the primary light-absorbing aerosol, has significant implications for atmospheric heating and climate change, with far-reaching effects on regional air quality and public health. In Iran, BC concentrations, primarily resulting from combustion processes such as industrial emissions, vehicular exhaust, and biomass burning, constitute a significant air quality challenge, particularly in urban regions with high levels of anthropogenic activity. However, there is a lack of studies on the long-term trends of BC in Iran, particularly regarding the effects of urban growth and land use changes on air quality and human health. This study systematically analyzes trends in BC concentrations from 1980 to 2023, both on a national and regional scales, using high-resolution data from the Modern-Era Retrospective Analysis for Research and Applications version 2 (MERRA-2).  The analysis includes temporal and spatial variations to evaluate the impact of anthropogenic and natural factors on BC levels over this period. A substantial increase in BC concentrations was observed from 1980 to 2023, followed by a decline after 2010. Regional analysis revealed higher BC levels in western Iran, driven by concentrated anthropogenic and industrial activities, compared to the sparsely populated, desert-dominated eastern regions, characterized by arid landscapes. Seasonal variations in BC concentrations were observed nationwide, with peak levels occurring in Tehran and Ahvaz during the winter. Trend analysis across various land use and land cover (LULC) types indicated that urban and agricultural expansion were the primarily drivers of increasing BC concentrations. Positive correlations were observed between the aforementioned factors and aerosol emissions, while water and grassland coverage were associated with reduced emissions in most regions. These findings underscore the necessity of expanding natural land use, such as forest coverage, and promoting sustainable urbanization as strategies to mitigate BC emissions.

How to cite: Shaheen, A., Yousefi, R., Wang, F., Kaveh-Firouz, A., and Ge, Q.: Assessing black carbon dynamics in Iran: the role of urban growth and land use changes in long-term trends (1980–2023), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5323, https://doi.org/10.5194/egusphere-egu25-5323, 2025.

EGU25-5362 | ECS | Posters virtual | VPS3

Turbulence-induced Non-Monotonic Influence of Aerosols on Cloud Droplet Size Distribution 

Yiqi Chen, Jingyi Chen, and Chunsong Lu

Cloud droplet size distribution is essential for quantifying the role of clouds in earth system, including cloud albedo, precipitation formation, and cloud lifetime. The response of cloud droplet spectral relative dispersion (ε) to aerosol number concentration (Na) is highly uncertain, and the role of turbulence in εNa relationships is yet puzzling. This study uses large eddy simulation to examine the εNa relationship and derives an expression for ε from a minimal model to elucidate this relationship. Our findings indicate that as Na increases, ε initially decreases due to the aerosol’s effect on weakening the intensity of turbulence-induced broadening greater than its effect on weakening the intensity of condensational narrowing. However, as Na continues to increase, ε increases due to the aerosol’s effect on weakening the intensity of condensational narrowing more significant than its effect on weakening the intensity of turbulence-induced broadening. These findings improve the understanding of the aerosol effects on cloud droplet size distribution and address the challenge of quantifying aerosol indirect effects considering turbulence, potentially leading to new cloud microphysics parameterizations.

How to cite: Chen, Y., Chen, J., and Lu, C.: Turbulence-induced Non-Monotonic Influence of Aerosols on Cloud Droplet Size Distribution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5362, https://doi.org/10.5194/egusphere-egu25-5362, 2025.

EGU25-5764 | ECS | Posters virtual | VPS3

Volatile organic compounds in ambient air of Delhi 

Richa Sharma

Delhi is one of the most polluted cities in the world with a rapidly growing population. Huge amount of VOCs is released into the atmosphere from both anthropogenic and biogenic emissions. Various types of VOCs are released from anthropogenic sources such as disinfectants and cleansers, paints and varnishes, wood preservatives, aerosol sprays, room fresheners, dry cleaners and organic solvents. Another important anthropogenic source is burning of fossil fuels in motor vehicles, which also releases VOCs. Various plants species also release VOCs like isoprene (biogenic VOCs) which upon oxidation with atmospheric oxidants like ozone (O3), nitrate (NO3) and hydroxyl radicals (OH) forms less volatile products which on further reaction forms secondary organic aerosols (SOA). VOCs are also responsible for formation of tropospheric ozone which is one of the major criterion air pollutants and causes various health issues.

Around 32 samples of VOCs have been collected in the NCT of Delhi using charcoal tubes from the selected sites, VIZ., Okhla Phase 2 (OKHL, Industrial site), Sri Aurobindo Marg (SAM, traffic intervention site), Income tax office (ITO, traffic intervention site), Jawaharlal Nehru University (JNU, Institutional site). Sample preparation has been done following the protocol given by NIOSH 1501 method for xylene analysis, which is widely accepted as a “golden standard” for Industrial Hygiene sampling. Collected samples were run on GC-FID and concentration of VOCs is determined. The average concentration of Total VOCs at SAM is found to be 382.07µg/m3 while it is 200.14, 242.63 and 452.62 µg/m3 at JNU, OKHL and ITO, respectively. Out of all the VOCS, benzene and toluene represents the highest percentage with benzene representing a percentage of 17%  and 18% at SAM, JNU, Okhla and ITO, respectively and Toluene  contributing to a percentage concentration of 15% , 13%, 16% and 15% respectively at SAM , JNU, Okhla and  ITO thus owing to high vehicular emissions in Delhi. Individual average concentration at evening is higher than individual average concentration at morning at all chosen sites.  Also individual concentration of benzene and toluene is higher than other VOCs being 64.14 µg/m3 and 59.13 µg/m3 respectively at SAM, 35.64 µg/m3 and 25.83 µg/m3 at JNU, 79.6 µg/m3 and 69.9 µg/m3 at ITO and 41.92 µg/m3 and 37.80 µg/m3 at Okhla. It has planned to evaluate both the carcinogenic and non-carcinogenic risk associated with the chosen VOCs. This research will help us to get knowledge of sources of emission of VOCs. Further we will get a knowledge of the carcinogenic and non-carcinogenic impacts of VOCs and the percentage of population in Delhi which is getting directly or indirectly exposed to the carcinogenic VOCs. Hence it would help us in determining the health risk associated with VOC emission which would help in formulating effective strategies for controlling VOC emission. This would further aid us in reducing tropospheric ozone which is also a pollutant of concern. This study can also be used further in understanding atmospheric chemical reactions, photochemical smog pollution, assessment and forecast of possible change in atmospheric environment on the regional/global scale.

 

How to cite: Sharma, R.: Volatile organic compounds in ambient air of Delhi, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5764, https://doi.org/10.5194/egusphere-egu25-5764, 2025.

NASA’s Atmospheric Science Data Center (ASDC) at Langley Research Center will present an overview of the Tropospheric Emissions: Monitoring of Pollution (TEMPO) mission, focusing on the cutting-edge tools and services available to users for air quality research and environmental monitoring. TEMPO is a pioneering geostationary satellite that provides day light hourly observations of pollutants over North America, including measurements of ozone, nitrogen dioxide, and other critical pollutants.This presentation will highlight the ASDC’s role in archiving, distributing, and providing user support for TEMPO data. Attendees will be introduced to data access tools, visualization platforms, and analysis services designed to facilitate the use of TEMPO observations for scientific research and decision-making. Key resources, such as NASA Earthdata Search, Earth GIS, OPeNDAP, Worldview, Github Tutorials and Harmony services on the cloud, will be showcased, demonstrating how researchers can efficiently explore and download high-resolution data products.Additionally, the presentation will cover the application of TEMPO data in studying air quality trends, emission sources, and the impacts of pollution on public health and climate. Attendees will also gain insights into ASDC's open science initiatives, which encourage collaboration and data sharing to enhance the impact of TEMPO and NASA’s broader Earth science mission.Through this presentation, the ASDC aims to empower the scientific community with the tools and knowledge needed to harness the full potential of TEMPO data in addressing pressing environmental challenges.

How to cite: Mahmoud, H. and Radkevich, A.: Leveraging TEMPO Data: Tools and Services for Air Quality Monitoring and Research from the Atmospheric Science Data Center, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7314, https://doi.org/10.5194/egusphere-egu25-7314, 2025.

EGU25-7978 | ECS | Posters virtual | VPS3

Atmospheric deposition of anthropogenic microfibers in different indoor environments of Chennai, India  

Angel Jessieleena, Iniyan Kambapalli Ezhilan, Amit Singh Chandel, Sancia Verus D'sa, Nilofer Mohamed, and Indumathi Nambi

Microplastics, particularly microplastic fibers, are an emerging pollutant of growing concern, frequently detected in the atmosphere. However, recent studies emphasized the predominance of artificial and natural microfibers over microplastic fibers. Despite this, research focusing on all types of microfibers, commonly grouped as anthropogenic microfibers (MFs) remains limited, especially in residential indoor environments. Therefore, this study explored the indoor atmospheric deposition of microfibers, in the residential homes of Chennai, India, marking the first such study in the country. Additionally, workplaces, including offices, laboratories, and hostel rooms, were examined. Bedrooms (16,736±7,263 MFs/m²/day) and student hostels (5,572±2,898 MFs/m²/day) recorded the highest contamination in respective categories, and this could be attributed to the abundance of textile products, such as bedsheets, carpets, quilts, towels, and curtains in the indoors of both the rooms. MFs shorter than 500 µm dominated the samples, comprising 78.8 and 65.9 % of total MFs in residential and workplace categories, respectively. The diameter of MFs ranged from 2.02–23 µm in residential spaces and 2.04–36.4 µm in workplaces, indicating their potential to penetrate human lungs. µ-FTIR analysis revealed the predominance of semi-synthetic MFs (48.2 %), followed by natural (29.3%) and synthetic (22.5 %) MFs, underscoring the need to consider all categories of MFs. Further classification revealed rayon (94.5±6.40 %), cotton (68.1±6.12 %), and polyethylene terephthalate (PET) (48.1±11.5 %) as major MFs, indicating textiles as a significant contamination source. The detection of black rubber/latex MFs indicates additional contributions from road dust. Surface morphological analysis, correlations with environmental and meteorological factors, and backward trajectory analysis further highlighted the primary role of indoor/local sources in MFs contamination. Overall, the study emphasizes the need to monitor all categories of MFs and calls for comprehensive investigations into the impact of indoor textile products and road dust on indoor atmospheric contamination in future research.

How to cite: Jessieleena, A., Kambapalli Ezhilan, I., Chandel, A. S., D'sa, S. V., Mohamed, N., and Nambi, I.: Atmospheric deposition of anthropogenic microfibers in different indoor environments of Chennai, India , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7978, https://doi.org/10.5194/egusphere-egu25-7978, 2025.

Nitrogen dioxide (NO2), an atmospheric pollutant produced by fossil fuel combustion in vehicles and industrial processes, is harmful to human health, worsening respiratory and cardiovascular diseases. The main effects of NO2 pollution on human health are respiratory infections, airway inflammation, asthma, and low birth weight, among others. Vehicle traffic in cities is one of the main sources of NO2, affecting the health of the population living near highways. The highest NO2 concentration occurs at distances between 200 and 500 meters from high-traffic highways. The study area, the metropolitan region of Campinas (MRC), Brazil, is a technological, industrial and economic hub with 3.3 million inhabitants and busy transport corridors that connect the southeast and central-west regions of the country. It is composed of 20 municipalities and is located in São Paulo state, the most developed and populated Brazilian state. The aims of this work are to map atmospheric NO2 pollution and estimate NO2 concentrations near the highways in the MRC using average daily vehicle flow (DVF) and NO2 concentrations estimated from satellite images. Data on the tropospheric vertical column of nitrogen dioxide (in mol/cm2) values from 32 daily images from the Sentinel 5P satellite TROPOMI spectrometer that were collected from April 15 to May 20, 2024, were used. During that period, there was no rain, and the sky remained clear and cloudless. The images were processed to produce NO2 median images during the study period. The NO2 pollution map was produced by the spline interpolation algorithm method. To estimate the concentration of NO2 near the MRC highways, a road map was used, and a 500 m buffer was drawn around the highways. The NO2 pollution map was combined with the buffer map, and the median NO2 concentration within the 500 m buffer around the highways was estimated. Pearson regression analysis was performed between the average DVF and the NO2 concentration. The results revealed a positive and significant correlation (r=0.692; p= 0.004) between the DVF and NO2 concentration near the highways estimated from satellite data. The highest NO2 concentrations were observed near highways SP-083 (1.5591 mol/cm2; 45,000 vehicles/day), SP-330 (1.521 mol/cm2; 38,815 vehicles/day), and SP-075 (1.485 mol/cm2; 37,813 vehicles/day). The results of this study can be used in epidemiological research to identify neighborhoods and populations that live near high NO2 concentration highways and are exposed to respiratory and cardiovascular disease risks. In the next step of this research, the NO2 concentration values ​​estimated from Sentinel 5P images in mol/cm2 units will be converted to µg/m3 units using data from ground-based measurement stations located in the MRC. In the future, this methodology can be used to produce highway NO2 pollution maps for areas in which ground measurement station data are unavailable.

How to cite: Ferreira, M.: Using Sentinel 5P satellite and vehicle flow data to map NO2 air pollution near highways in the Metropolitan Region of Campinas, Brazil, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9328, https://doi.org/10.5194/egusphere-egu25-9328, 2025.

Extreme weather events, such as extreme temperatures, water vapor transport, and the resulting extreme precipitation, have been occurring with increasing frequency and are projected to intensify further in a warming climate. Understanding how these events respond to climate change is critically important. Numerical models serve as essential tools for uncovering the mechanisms behind these phenomena, with spatial resolution being one of the key challenges. Leveraging advanced supercomputing resources, we have recently made significant advancements in developing high-resolution Earth system models based on the Community Earth System Model (CESM), featuring a 25 km atmospheric resolution and a 10 km oceanic resolution. Compared to the commonly used CMIP5 and CMIP6 models, the high-resolution Earth system model demonstrates substantial improvements in reproducing extreme weather events, thereby greatly enhancing the confidence in future projections.

How to cite: Gao, Y.: Enhancing the Simulation and Prediction of Extreme Temperature and Water Vapor in a Warming Climate Using a High-Resolution Earth System Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11612, https://doi.org/10.5194/egusphere-egu25-11612, 2025.

The Indo-Gangetic Plain (IGP) is a globally recognized hotspot for high aerosol loading, necessitating precise modelling to understand its spatial and temporal dynamics. This study evaluates the performance of differently parameterized Seasonal Autoregressive Integrated Moving Average (SARIMA) models in forecasting the Aerosol Optical Depth (AOD) at 550 nm retrieved from the CERES (Clouds and the Earth's Radiant Energy System) satellite platform across eight  locations: Delhi, Dhaka, Jaipur, Kanpur, Karachi, Kolkata, Lahore, and Varanasi in the IGP. Using long-term AOD datasets from CERES during the period of 2005 to 2020, we tested various SARIMA configurations to capture seasonal trends and irregular variations specific to urban environments. The SARIMA configurations tested include configure_1: (1,0,1)(1,0,1)₁₂, configure_2: (1,1,1)(1,1,1)₁₂, configure_3: (2,0,1)(2,0,1)₁₂, and configure_4: (2,1,1)(2,1,1)₁₂ These configure models were compared with CERES-derived observations for AOD at the study sites for the next two years, that is, Jan, 2021 to Dec, 2022. Each configuration was assessed for data stationarity using the Augmented Dickey-Fuller (ADF) test and if not follows, then the differentiation method has been used to stationaries the series. The Model performance was evaluated using multiple statistical metrics, including normalized Akaike Information Criterion (AIC), Bayesian Information Criterion (BIC), Root Mean Squared Error (RMSE), Mean Bias Error (MBE), and Mean Absolute Percentage Error (MAPE) for every configuration showed the low metric values. The result indicates high correlation coefficients, ranging from 0.54 to 0.91, and R-squared values, varying between 0.31 and 0.81 for all configurations that significantly determined the best-suited models for each location. Every modelled configuration has been checked with 95% and 99% confidence interval (with alpha=0.05 and 0.01, respectively) showing the p-value <0.001. These results emphasize the models' ability to replicate observed AOD patterns effectively. It reveal that parameter sensitivity plays a critical role in predictive accuracy, with optimal configurations varying across locations due to heterogeneity in aerosol sources and meteorological conditions. The present study underlines the importance of site-specific model tuning for reliable aerosol forecasting in densely populated and pollution-prone regions. These insights provide a foundation to enhance air quality prediction studies and address health, and climate impacts associated with aerosols in the IGP.

How to cite: Mall, A. and Singh, S.: Comparison of Differently Parameterized SARIMA Models using CERES-Derived Aerosol Optical Depth over Indo-Gangetic Plain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12277, https://doi.org/10.5194/egusphere-egu25-12277, 2025.

EGU25-13295 | Posters virtual | VPS3

Multiple lines of evidence help identify the sources and formation mechanisms of Nitrogen and Carbon in Particulate Matter sampled in the historical center of Naples (Italy) 

Mauro Rubino, Carmina Sirignano, Elena Chianese, Miguel Ángel Hernández-Ceballos, Anikó Angyal, Fabio Marzaioli, Davide Di Rosa, Giuseppe Caso, and Angelo Riccio

The aim of this study is to investigate Particulate Matter (PM) sources and mechanisms of formations over the city of Naples (Italy) and their seasonal and day-to-day variations.

We have sampled fine particles with diameter < 2.5 μm (PM2.5) and < 10 μm (PM10) daily on pre-cleaned (700 °C for 2 h) quartz filters, during the months of May and November 2016-January 2017, on top of the historical building complex in Largo San Marcellino, Naples. We have measured the concentrations of total N/C together with their isotopic composition (δ15N and δ13C). We have also measured the concentration of major ions and interpreted the results with data of gaseous compounds, as well as consideration of the meteorology, using data and state of the art models of atmospheric circulation (Hysplit). Our point was to show that the uncertainty associated with quantification of sources contribution with an apportionment model decreases when the model is constrained with information derived from different methods.

Seasonal differences: the results show that the concentrations of total PM10/PM2.5, N/C measured in autumn are more variable than those measured in spring. This is related to a different wind regime, whereby in spring air masses mostly originated from West and South (the “clean” Mediterranean sea), whereas in autumn the wind blew air from North (over the highly urbanized and “dirty” European continent). This interpretation is supported by the concentration of major ions showing more scattered values in autumn for species typically originating from land (K+, NH4+, NO3-), with high values on the 9th and the 26-27th of December and the 2nd of January 2017. However, neither the monthly mean δ15N and δ13C, nor the daily values corresponding to the spikes show significant changes, suggesting that the isotopic composition of total N/C has limited power in identifying changes of mean monthly sources or for the spikes. 

Day-to-day variations: a significant change of the main species measured is found around the middle of May. This event is associated with a change in weather pattern going from a typical land-sea breeze wind regime (typically causing poor air circulation and stagnation of air masses) to an intense synoptic with winds originating mostly from South/South-West (the sea). Correspondingly, there is a peak in the concentration of major ions originating mostly from land (NO3-, SO42-, Ca2+, C2O42-, K+) towards the end of the land-sea breeze regime (9-11th May), followed (10-15th May) by an increase of the concentration of major ions originating mostly from the sea (Na+, Mg2+, Cl-). The entire period (9-14th) is characterized by a concurrent variation of total N, C, δ15N and δ13C. While the changes of δ15N are caused mainly by isotope fractionations, associated with the dissociation of NH4Cl producing NH3 and HCl, the changes of δ13C are caused mostly by a change of the source of total C, associated with carbonate (CO32-) apportion.

We conclude that the concentrations and isotopic compositions of N/C in PM are useful tools only when coupled with other tools like the analysis of the meteorology and the concentration of major ions.

How to cite: Rubino, M., Sirignano, C., Chianese, E., Hernández-Ceballos, M. Á., Angyal, A., Marzaioli, F., Di Rosa, D., Caso, G., and Riccio, A.: Multiple lines of evidence help identify the sources and formation mechanisms of Nitrogen and Carbon in Particulate Matter sampled in the historical center of Naples (Italy), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13295, https://doi.org/10.5194/egusphere-egu25-13295, 2025.

Active and passive sensors onboard satellites and suborbital measurements have shown frequent aerosol-cloud overlapping situations over several regions worldwide on a monthly to seasonal scale. However, retrieving the optical properties of aerosols lofted over clouds poses challenges. Primarily, the assumption of aerosol single-scattering albedo (SSA) in the satellite-based algorithms is known to be one of the largest sources of uncertainty in quantifying the above-cloud aerosol optical depth (ACAOD). On the radiative forcing aspect, the sign and magnitude of the aerosol radiative forcing over clouds are determined mainly by the aerosol loading, the absorption capacity of aerosols (SSA), and the brightness of the underlying cloud cover.

 

We contribute to addressing the uncertainties surrounding the absorbing aerosols-cloud radiative interactions by offering a novel, NASA’s A-train-centric, one-and-half decade long (2006-2022) global retrieval product of aerosols above cloud that delivers 1) spectral ACAOD, 2) spectral SSA of light-absorbing aerosols lofted over the clouds, and 3) aerosol-corrected cloud optical depth (COD). The synergy algorithm combines lidar retrievals of ACAOD derived from the ‘De-polarization Ratio’ method applied to CALIOP and the top-of-atmosphere (TOA) spectral reflectance from OMI (354-388 nm) and MODIS (470-860 nm) sensors to deduce the joint aerosol-cloud product. The availability of accurate ACAOD accompanied by a marked sensitivity of the TOA measurements to ACAOD, SSA, and COD allow retrieval of SSA for above-cloud aerosols scenes using the ‘color ratio’ algorithm applied to UV and VIS sensors.

 

We will present multiyear (2006-2022), regional retrievals of UV-VIS spectral aerosol SSA above clouds, and it’s a comparison against ORACLES airborne in situ and remote sensing measurements and ground-based AERONET inversions. A preliminary uncertainty analysis suggests that an uncertainty of 20% in ACAOD can result in an error of ~0.02 at 388 nm and ~0.01 at 470 nm in the retrieved SSA from OMI and MODIS, respectively. Furthermore, the presented aerosol-cloud remote sensing algorithm assumes implications for the recently launched EarthCARE and PACE missions with potential synergy of ATLID lidar and OCI imager. The availability of the global aerosol-cloud joint product will reenergize the community by offering 1) an improved representation of aerosol extinction and absorption properties over clouds and 2) much-needed observational estimates of the radiative effects of aerosols in cloudy regions for constraining the climate models.

How to cite: Jethva, H., Torres, O., Kayetha, V., and Hu, Y.: One-and-half Decade Long Global Retrieval Dataset of UV-VIS Spectral Optical Depth and Single-scattering Albedo of Absorbing Aerosols above Clouds from A-train Active-Passive Synergy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14363, https://doi.org/10.5194/egusphere-egu25-14363, 2025.

EGU25-14596 | Posters virtual | VPS3

The Tropospheric Emissions: Monitoring of Pollution (TEMPO) Level 0-1 Processor – Radiometric calibration and intercomparison 

Heesung Chong, Xiong Liu, John Houck, David E. Flittner, James Carr, and Weizhen Hou and the TEMPO instrument calibration team

We present the status of the Level 0-1 processor for the Tropospheric Emissions: Monitoring of Pollution (TEMPO), with a primary focus on radiometric calibration. Multiple version updates have significantly improved the TEMPO Level 1 products, enhancing the quality of Level 2 products and enabling the detection of city lights, nightglow, and aurora signals during twilight hours. However, assessments of TEMPO Level 1 data (versions 1 to 3) indicated overestimations of Sun-normalized radiances when compared to radiative transfer calculations. To investigate these biases, we compared TEMPO solar irradiance measurements to those from multiple independent instruments and a high-resolution reference solar spectrum. For Earth radiance assessments, we conducted intercomparisons with spaceborne measurements from the Advanced Baseline Imager (ABI) instruments onboard the Geostationary Operational Environmental Satellite (GOES)-16 and -19. Located at the checkout position of 89.5°W for post-launch testing, GOES-19 ABI has provided comparable viewing geometries with TEMPO (at 91.0°W) over North America. On the other hand, comparisons with GOES-16 ABI (located at 75.2°W) may require corrections for viewing angles and bidirectional reflectance distribution function (BRDF) effects due to larger differences in geometries. Additionally, we compared TEMPO Sun-normalized radiances with radiative transfer simulations over Railroad Valley, which use ground-based surface reflectance measurements as input. In this work, we present the intercomparison results and propose potential approaches to mitigate the radiometric biases.

How to cite: Chong, H., Liu, X., Houck, J., Flittner, D. E., Carr, J., and Hou, W. and the TEMPO instrument calibration team: The Tropospheric Emissions: Monitoring of Pollution (TEMPO) Level 0-1 Processor – Radiometric calibration and intercomparison, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14596, https://doi.org/10.5194/egusphere-egu25-14596, 2025.

EGU25-14804 | ECS | Posters virtual | VPS3

Investigation of the Cyclohexene Oxidation Mechanism Through the Direct Measurement of Organic Peroxy Radical 

Yang Li, Xuefei Ma, Keding Lu, and Yuanhang Zhang

Monoterpenes, the second most abundant biogenic volatile organic compounds globally, are crucial in forming secondary organic aerosols, making their oxidation mechanisms vital for addressing climate change and air pollution. This study utilized cyclohexene as a surrogate to explore first-generation products from its ozonolysis through laboratory experiments and mechanistic modeling. We employed proton transfer reaction mass spectrometry with NH4+ ion sources (NH4+-CIMS) and a custom-built OH calibration source to quantify organic peroxy radicals (RO2) and closed-shell species. Under near-real atmospheric conditions in a Potential Aerosol Mass-Oxidation Flow Reactor, we identified 30 ozonolysis products, expanding previous data sets of low-oxygen compounds. Combined with simulations based on the Generator for Explicit Chemistry and Kinetics of Organics in the Atmosphere and relevant literature, our results revealed that OH dominates over ozone in cyclohexene oxidation at typical atmospheric oxidant levels with H-abstraction contributing 30% of initial RO2 radicals. Highly oxidized molecules primarily arise from RO2 autoxidation initiated by ozone, and at least 15% of ozone oxidation products follow the overlooked nonvinyl hydroperoxides pathway. Gaps remain especially in understanding RO2 cross-reactions, and the structural complexity of monoterpenes further complicates research. As emissions decrease and afforestation increases, understanding these mechanisms becomes increasingly critical.

How to cite: Li, Y., Ma, X., Lu, K., and Zhang, Y.: Investigation of the Cyclohexene Oxidation Mechanism Through the Direct Measurement of Organic Peroxy Radical, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14804, https://doi.org/10.5194/egusphere-egu25-14804, 2025.

EGU25-14890 | ECS | Posters virtual | VPS3

Quantifying the sources of anthropogenic aerosols over western India 

Shashank Shekhar, Shubham Dhaka, Aditya Vaishya, Narendra Ojha, Andrea Pozzer, and Amit Sharma

Anthropogenic aerosols significantly deteriorate the urban air quality and climate of the western Indian region, nevertheless, the contributions from different sources (power, residential, transport and industries) to ambient particulate pollution has been uncertain. In this regard, high-resolution simulations have been conducted employing the WRF-Chem (v3.9.1) model to comprehensively assess contribution from major anthropogenic sources in post-monsoon (November 2019), when air quality is typically poor in the region. Model evaluation is conducted by comparing simulated near-surface aerosol concentrations (PM2.5 and PM10) and aerosol optical depth (AOD) against ground-based measurements (CPCB), satellite data (MODIS), and the reanalysis dataset (MERRA-2). The results show that the model captures the spatial distribution of AOD satisfactorily, with WRF-Chem simulated AOD (0.38 ± 0.10) aligning well with MERRA-2 AOD (0.54 ± 0.10) and MODIS AOD (0.50 ± 0.20). Surface PM2.5 and PM10 concentrations also meet performance metrics of Fractional Bias ≤ 60% and Fractional Error ≤ 75%, with FAC2 values of 0.9 and 0.7, respectively. Sensitivity analysis reveals spatial heterogeneity in dominant sector that contributes to PM2.5 concentration over western India. The power sector dominates in most areas with an average contribution of ~14% from regional power sources, followed by regional industries (~12%), regional residential emissions (~9%), and regional transport (~5%). In the trans-regional emissions from the Indo-Gangetic Plain (IGP) and central India also, the power sector remains the largest contributor (~15%), followed by industry (10.5%). Our findings underscore the need for targeted emission reductions in high-impact sectors to improve air quality over western India.

How to cite: Shekhar, S., Dhaka, S., Vaishya, A., Ojha, N., Pozzer, A., and Sharma, A.: Quantifying the sources of anthropogenic aerosols over western India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14890, https://doi.org/10.5194/egusphere-egu25-14890, 2025.

EGU25-14891 | ECS | Posters virtual | VPS3

Impacts of anthropogenic emissions on monsoon precipitation over western India: Insights from high-resolution regional modeling 

Shubham Dhaka, Shipra Lakshmi, Aditya Vaishya, Narendra Ojha, Andrea Pozzer, Tabish Ansari, and Amit Sharma

Air quality and climate over the western Indian region have been shown to be strongly influenced by trans-regional anthropogenic emissions originated from the Indo-Gangetic Plain (IGP) and central India, besides the local and regional processes. Nevertheless, the relative roles of local versus remote anthropogenic processes in changing precipitation over western India have remained unclear. In this regard, numerical simulations have been conducted using the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) to quantify regional versus trans-regional anthropogenic effects on cloud droplet number concentration (CDNC) and precipitation during monsoon (August 2019). WRF-Chem simulations show a good agreement with the ERA5 reanalysis for cloud fraction (CF) (r = 0.88, MB = 0.08 mm/day) and accumulated monthly precipitation (AMP) (r = 0.84, MB = -0.14 mm/day). Sensitivity simulations reveal that regional plus trans-regional anthropogenic emissions enhance CDNC by up to 5.1×106 number/cm2 (~121% of the average CDNC over WI) but significantly reduce the precipitation by up to 45 mm (~15% of the average precipitation). The findings also revealed that the impact of trans-regional emissions in perturbing CDNC and precipitation is higher than that of regional emissions. Our results suggest that anthropogenic emissions can substantially lower water resources in this already stressed arid region in India. The study also highlights that policies need to aim emission reductions ubiquitously and not only over western India for mitigating pollution impacts on regional precipitation.

How to cite: Dhaka, S., Lakshmi, S., Vaishya, A., Ojha, N., Pozzer, A., Ansari, T., and Sharma, A.: Impacts of anthropogenic emissions on monsoon precipitation over western India: Insights from high-resolution regional modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14891, https://doi.org/10.5194/egusphere-egu25-14891, 2025.

Dhaka, the capital of Bangladesh, is currently experiencing critically alarming levels of air pollution, with its Air Quality Index (AQI) exceeding 200, indicating hazardous conditions. This study investigates the factors contributing to Dhaka's deteriorating air quality over the past two decades by integrating AQI data with Land Use and Land Cover (LULC) analyses. Particular attention is given to the impacts of major development projects, including the Metro Rail, Elevated Expressway, and International Airport Terminal 3, on the city’s air quality. Comparative assessments of AQI before and after the completion of these projects reveal a significant worsening of air quality, attributed to increased construction activity and subsequent urbanization. The rapid expansion of impervious surfaces is identified as another critical factor exacerbating the AQI. The findings emphasize the urgent need for sustainable urban planning and air quality management strategies to mitigate the adverse effects of development on public health and the environment in Dhaka.

How to cite: Akhter, J. and Rayhan, M.: Assessing the Impact of Urban Development and Land Use Changes on Dhaka's Hazardous Air Quality, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14892, https://doi.org/10.5194/egusphere-egu25-14892, 2025.

EGU25-14903 | Posters virtual | VPS3

Advancing Greenhouse Gas Mapping with JPL Imaging Spectrometers: AVIRIS, EMIT, and Carbon-I 

Andrew Thorpe, Robert Green, Christian Frankenberg, Anna Michalak, David Thompson, Philip Brodrick, Dana Chadwick, Michael Eastwood, Valerie Scott, William Frazier, Jay Fahlen, Red Willow Coleman, Chuchu Xiang, Daniel Jensen, Claire Villanueva-Weeks, Amanda Lopez, Quentin Vinckier, Holly Bender, Adam Chlus, and John Chapman

Over the past 15 years, imaging spectrometers developed at the NASA Jet Propulsion Laboratory have significantly advanced the field of remote sensing of methane (CH4) and carbon dioxide (CO2) point source emissions. This began in 2008 with airborne observations from the Airborne Visible/Infrared Imaging Spectrometer (AVIRIS), 2013 with the next generation AVIRIS-NG instrument, and has culminated with the launch of NASA’s Earth Surface Mineral Dust Source Investigation (EMIT) in 2022.

These instruments have identified thousands of CH4 and CO2 point source emissions across the oil and gas, waste, and energy sectors, contributing in some cases to emission mitigation efforts. As part of an extended mission, EMIT coverage will expand beyond the arid regions of Earth to cover terrestrial surfaces between +51.6° and −51.6° latitude, enabling direct attribution of anthropogenic emissions on a global scale. EMIT's measurements and greenhouse gas data products are accessible through NASA’s Land Processing DAAC and the U.S. GHG Center, with all associated code available as open source. These data are already being utilized by public, private, and non-profit organizations, including UNEP IMEO and the Carbon Mapper Coalition. Additionally, new airborne instruments, such as AVIRIS-3 (2023) and the planned AVIRIS-5, promise enhanced sensitivity to CH4 and CO2 point sources, offering the potential for direct comparisons with satellite-based EMIT observations.

The Carbon Investigation (Carbon-I), a proposed mission for the NASA Earth System Explorer Program, reflects a dramatic advancement in greenhouse gas mapping capability. It provides a unique combination of coverage, high spatial sampling, and very high sensitivity, to permit quantification of emissions that cannot be observed with current technology. With contiguous global observations of CH4, CO2, and CO at 300 m sampling every 28 days with targeted observations at 30 m sampling, Carbon-I will permit emission quantification at the global to regional scales as well as for localized point sources. Consistent with NASA’s Open Source Science Initiative, all Carbon-I data and code will be publicly accessible, empowering Earth Action initiatives worldwide.

How to cite: Thorpe, A., Green, R., Frankenberg, C., Michalak, A., Thompson, D., Brodrick, P., Chadwick, D., Eastwood, M., Scott, V., Frazier, W., Fahlen, J., Coleman, R. W., Xiang, C., Jensen, D., Villanueva-Weeks, C., Lopez, A., Vinckier, Q., Bender, H., Chlus, A., and Chapman, J.: Advancing Greenhouse Gas Mapping with JPL Imaging Spectrometers: AVIRIS, EMIT, and Carbon-I, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14903, https://doi.org/10.5194/egusphere-egu25-14903, 2025.

EGU25-15068 | ECS | Posters virtual | VPS3

Stratospheric Circulation in the Southern Hemisphere: links to tropical winds, ozone and Hunga Eruption 

Xinyue Wang, Wandi Yu, William Randel, and Rolando Garcia

The Southern Hemisphere (SH) stratosphere circulation can be organized around the development of the low-latitude jet (LLJ) in the upper stratosphere during winter months. The LLJ is associated with weak planetary wave activity, reduced residual circulation, and connections to westerly anomalies of the middle and upper stratosphere during early and mid-winter. The 2022 Hunga eruption coinciding with an anomalously strong LLJ year. Additionally, the LLJ is linked to a persistent, strong polar vortex in the lower stratosphere during October–December. This strong vortex, primarily driven by dynamical processes in winter, is further associated with enhanced ozone losses in spring, with ozone feedback reinforcing the vortex as sunlight returns in October.

How to cite: Wang, X., Yu, W., Randel, W., and Garcia, R.: Stratospheric Circulation in the Southern Hemisphere: links to tropical winds, ozone and Hunga Eruption, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15068, https://doi.org/10.5194/egusphere-egu25-15068, 2025.

EGU25-15097 | ECS | Posters virtual | VPS3

Advancing load-dependent emission factors for ships: Integrating alternative fuels, biofuels, and control technologies 

Achilleas Grigoriadis, Theofanis Chountalas, Evangelia Fragkou, Dimitrios Chountalas, and Leonidas Ntziachristos

Shipping is a high-energy-consuming sector and a significant source of climate-related and harmful pollutant emissions. In response to growing environmental concerns, the maritime sector has been subject to stringent regulations aimed at reducing emissions, achieved through the adoption of alternative fuels and emission control technologies. Accurate and diverse emission factors (EFs) are critical for quantifying shipping’s contribution to current emission inventories and projecting future trends under various policy scenarios. This study presents advancements in the development of emission factors for ships, incorporating alternative fuels, biofuels and emission control technologies. The methodology integrates statistical analysis of emission data from an extensive literature review with newly acquired on-board emission measurements. To ensure high resolution and applicability across diverse operational conditions, the emission factors are formulated as functions of engine load and categorized by engine type and fuel used. The results provide insights into the emission performance of ships and intend to support the development of robust, up-to-date emission models and inventories, contributing to the broader goal of sustainable maritime transport.

How to cite: Grigoriadis, A., Chountalas, T., Fragkou, E., Chountalas, D., and Ntziachristos, L.: Advancing load-dependent emission factors for ships: Integrating alternative fuels, biofuels, and control technologies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15097, https://doi.org/10.5194/egusphere-egu25-15097, 2025.

EGU25-15191 | Posters virtual | VPS3

Nitrous Acid (HONO) Retrievals from wildfire events by using Geostationary Environment Monitoring Spectrometer (GEMS) ultraviolet spectra 

Hyeji Cha, Jhoon Kim, Heesung Chong, Gonzalo González Abad, Sang Seo Park, and Won-jin Lee

Nitrous acid (HONO) is known to be the significant source of hydroxyl radicals (OH), impacting air quality and climate as a major oxidant in the atmosphere. Many studies have highlighted that the photolysis of HONO can produce substantial amounts of OH throughout the day. Despite the crucial role of HONO in tropospheric chemistry, more research is needed to improve understanding of global HONO budgets. To address this, we developed a prototype HONO retrieval algorithm from the Geostationary Environment Monitoring Spectrometer (GEMS). The retrieval algorithm comprises two major processes, commencing with the spectral fitting of UV spectral range (343-371 nm) using the direct fitting method to obtain the slant columns. Subsequently, the conversion of slant columns into vertical columns is achieved by applying the air mass factor. The last step involves background correction, wherein the slant column amounts of HONO included in the radiance reference spectrum are added to the differential slant columns. Enhancements of HONO resulting from wildfire events in Asia were detected using GEMS. Refining the GEMS HONO retrieval algorithm is expected to enhance our understanding of the diurnal cycle of HONO, along with tropospheric chemistry in Asia.

How to cite: Cha, H., Kim, J., Chong, H., González Abad, G., Park, S. S., and Lee, W.: Nitrous Acid (HONO) Retrievals from wildfire events by using Geostationary Environment Monitoring Spectrometer (GEMS) ultraviolet spectra, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15191, https://doi.org/10.5194/egusphere-egu25-15191, 2025.

EGU25-15708 | Posters virtual | VPS3

"Investigating Regional and Long-Range Transport Contributions to GHG Concentrations of a Mid-Latitude Urban Site"  

Thomas Panou, Marios Mermigkas, Chrysanthi Topaloglou, Dimitrios Balis, Darko Dubravica, and Frank Hase

Increasing concentrations of greenhouse gases (GHGs) in the atmosphere are the primary driver of the observed rise in global surface temperatures, meanwhile exceeding 1°C above pre-industrial levels. Addressing this challenge requires linking GHG concentrations to specific anthropogenic and natural sources as part of the global carbon budget. This study investigates the relationship between GHG concentrations measured in Thessaloniki, Greece, and potential long-range transport sources using a clustering approach.

The GHG data were obtained from the EM27/SUN Fourier Transform Infrared (FTIR) spectrometer, a ground-based low-resolution infrared spectrometer operated in the framework of the Collaborative Carbon Column Observing Network (COCCON) at a mid-latitude urban site. The instrument provides column-averaged dry air molar fractions of CH₄, CO₂, CO, and H₂O. Meteorological data for trajectory simulations were derived from the Global Data Assimilation System (GDAS) with a spatial resolution of 1° × 1°.

Clustering analysis was performed using the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model. Seven-day kinematic back trajectories were calculated for the period 2019–2024 at two arrival heights, 1500 m and 3000 m above mean sea level. The findings aim to specify the influence of long-range transport on GHG concentrations over Thessaloniki, contributing to a more complete understanding of regional GHG source-receptor relationships and transport patterns.

How to cite: Panou, T., Mermigkas, M., Topaloglou, C., Balis, D., Dubravica, D., and Hase, F.: "Investigating Regional and Long-Range Transport Contributions to GHG Concentrations of a Mid-Latitude Urban Site" , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15708, https://doi.org/10.5194/egusphere-egu25-15708, 2025.

EGU25-15895 | Posters virtual | VPS3

Tracing Black Carbon's Historical Impact on Regional Precipitation 

Camilla Weum Stjern, Bjørn H. Samset, Kari Alterskjaer, and Ane Nordlie Johansen

Black carbon (BC) aerosols, strong absorbers of solar radiation, induce atmospheric heating, altering vertical profiles of temperature, water vapor, and clouds. These impacts can lead to localized precipitation changes, and may also initiate changes to atmospheric circulation, with potentially far-reaching impacts on precipitation patterns.

While prior studies suggest BC's significant influence on precipitation, its role in both local and remote precipitation change remains insufficiently quantified. To address this gap, we explore the extent to which historical BC emissions have shaped regional precipitation. Specifically, we ask: how much could future BC changes influence regional precipitation, based on insights from the historical period?

Using the Community Earth System Model version 2 (CESM2), we have generated a 20-member ensemble of simulations of 1950–2014 with anthropogenic BC emissions fixed at 1950 levels. By comparing these to standard historical simulations with evolving emissions, we isolate the impacts of BC emission trends from 1950 to 2014 on global and regional climates.

Our results reveal that BC emissions have caused localized drying in regions of high emissions, notably over Europe during the 1980s–1990s and Eastern China in the early 21st century. Furthermore, we find indications that BC exerts a dampening effect on the most extreme precipitation events, highlighting its historical role in modulating climate extremes.

How to cite: Stjern, C. W., Samset, B. H., Alterskjaer, K., and Johansen, A. N.: Tracing Black Carbon's Historical Impact on Regional Precipitation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15895, https://doi.org/10.5194/egusphere-egu25-15895, 2025.

EGU25-16374 | ECS | Posters virtual | VPS3

Voyage Optimization with the VISIR-2 Model on the Shanghai–Los Angeles Green Corridor of shipping 

Mario Leonardo Salinas and Gianandrea Mannarini

In 2018, international shipping accounted for significant anthropogenic greenhouse gas emissions, contributing approximately 740 million tons of CO₂ according to the voyage-based method of the Fourth International Maritime Organization (IMO) Greenhouse Gases Study [1] and 880 million tons based on the CEDS and EDGAR inventories [2]. Recognizing this impact, the IMO adopted a long-term strategy in 2023 to achieve decarbonisation of global shipping by mid-century. However, concrete measures remain under development. A recent assessment of the 2018–2022 period suggests emissions are once again approaching 2008 levels, attributed to stagnation in improving energy efficiency [3]. This highlights the urgency of evaluating the potential of operational measures to mitigate emissions.

Voyage optimization, or ship weather routing, is an operational strategy leveraging meteo-oceanographic data to minimize energy consumption. This reduction can be achieved through spatial diversions, speed variations, or a combination of both. VISIR-2 [4], an open-source Python-based model, computes least-CO₂ routes by optimizing spatial diversions. Using a validated graph-search algorithm, the model integrates ocean currents and avoids adverse sea conditions [5].

In this study, we apply VISIR-2 to an ocean-going vessel operating on the Shanghai–Los Angeles/Long Beach route, identified as one of the first green corridors of shipping [6]. Simulations are conducted for both eastbound and westbound voyages over an entire calendar year, with and without the influence of ocean currents. We evaluate the resulting CO₂ savings, analysing their dependence on engine load and environmental conditions.

These results demonstrate the potential of operational measures like voyage optimization to contribute to shipping decarbonisation. The VISIR-2 model is currently employed within the EDITO-Model Lab project [7], contributing to developing a digital twin of the ocean. This work underscores the importance of open-source tools in fostering sustainable maritime practices and achieving the IMO's decarbonisation goals.

 

References
[1] https://www.imo.org/en/ourwork/Environment/Pages/Fourth-IMO-Greenhouse-Gas-Study-2020.aspx
[2] Deng, S., Mi, Z. A review on carbon emissions of global shipping. Mar Dev 1, 4 (2023). https://doi.org/10.1007/s44312-023-00001-2
[3] https://www.shippingandoceans.com/post/international-shipping-emissions-return-to-peak-2008-levels-due-to-insufficient-energy-efficiency-im
[4] https://doi.org/10.5281/zenodo.8305526
[5] Mannarini, G., Salinas, M. L., Carelli, L., Petacco, N., and Orović, J.: VISIR-2: ship weather routing in Python, Geosci. Model Dev., 17, 4355–4382, https://doi.org/10.5194/gmd-17-4355-2024, 2024
[6] https://www.c40.org/news/la-shanghai-implementation-plan-outline-green-shipping-corridor/
[7] https://www.edito-modellab.eu/

How to cite: Salinas, M. L. and Mannarini, G.: Voyage Optimization with the VISIR-2 Model on the Shanghai–Los Angeles Green Corridor of shipping, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16374, https://doi.org/10.5194/egusphere-egu25-16374, 2025.

EGU25-16376 | ECS | Posters virtual | VPS3

Regional and climatic variations in atmospheric microplastic deposition 

Sajjad Abbasi, Reda Dzingelevičienė, and Andrew Turner

The atmosphere is a critical reservoir for and transporter of microplastics (MPs) but little is known about the nature and drivers of their regional and climatic variability. In this study, dry deposition of MPs is quantified simultaneously over a seven-day period in nine Iranian cities encompassing different populations and climates and relationships with meteorological conditions and gaseous and particulate air quality parameters investigated. Overall, deposition ranged from < 5 to > 100 MP m-2 h-1 and was dominated by fibres of various sizes and constructed of different polymers (mainly polyethylene, polyethylene terephthalate, polypropylene, polystyrene and nylon), and there were clear and significant differences in mean values between the different cities that were not a simple function of climate or population. On a local scale, both positive and negative relationships between MP deposition and various meteorological and air quality parameters were observed among the cities. However, the pooled depositional data for MPs and various shapes and sizes thereof exhibited significant inverse relationships with wind speed and specific measures of airborne particulate matter (e.g., dust, PM-2.5, PM-10). The results suggest that there is a broadly consistent, fibre-dominated regional population of MPs whose deposition (and presumably resuspension) is influenced by variations in wind speed, but additional location-specific factors and sources contribute to temporal variations within the different cities. Despite the relationships between deposition and some gaseous and particulate air quality parameters identified at specific locations, it may be difficult to introduce a sharp parameter that can be used as a regional proxy for MP deposition.

 

Acknowledgements

We thank Shiraz University and Klaipeda University for technical support. This project has received funding from the Research Council of Lithuania (LMTLT), agreement No. S-PD-24-51.

How to cite: Abbasi, S., Dzingelevičienė, R., and Turner, A.: Regional and climatic variations in atmospheric microplastic deposition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16376, https://doi.org/10.5194/egusphere-egu25-16376, 2025.

Aerosol-cloud interactions contribute to 75–80% of the total radiative effect of aerosols and remain a major source of uncertainty in predicting future climate. Aerosols significantly influence the warm cloud properties by serving as cloud condensation nuclei (CCN). An increase in CCN leads to the formation of more numerous and smaller cloud droplets, suppresses warm rain by reducing the efficiency of collision and coalescence processes, and extends the cloud lifetime, and liquid water path (LWP) and/or cloud fraction (CF). The activation of a CCN into a cloud droplet is strongly influenced by its size and chemical composition, which subsequently affects the size distribution of cloud droplets and other cloud properties. Although the physical processes of nucleation are well documented for individual particles, the impact of aerosol size on cloud properties is often underestimated because both fine and coarse aerosols co-exist together. To bridge this gap, this study aims to address the impact of size-differentiated aerosols on warm cloud properties over the Northern Indian Ocean (NIO) by utilizing ~20 years of multi-satellite observation data.

The Arabian Sea (AS) and the Bay of Bengal (BoB) in the NIO were chosen in this study as these regions experience a continuous load of aerosols from natural and anthropogenic sources with high seasonal variations. Comparative analysis of size-segregated aerosol optical depth (AOD) revealed the dominance of coarse mode particles (c-AOD) over AS, and fine mode (f-AOD) over BoB. However, a significant increasing trend in the mean f-AOD, particularly during the post-monsoon (ON) and winter (DJF) seasons, is observed over both the AS (0.05/decade) and BoB (0.045/decade) from 2000 to 2021, primarily driven by rising anthropogenic emissions. Further, a climatological analysis of warm cloud CF during these seasons reveals a corresponding increasing trend over the AS (0.07/decade) and BoB (0.05/decade). A correlation analysis of c-AOD and f-AOD with warm CF was conducted, which revealed a stronger annual positive correlation of warm CF with c-AOD (AS: r = 0.56, BOB: r = 0.41) compared to f-AOD (AS: r = 0.37, BOB: r = 0.27). To further investigate the impact of f-AOD and c-AOD on cloud effective radius (CER) for a fixed LWP, an additional correlation analysis was performed. For low LWP (up to 70 gm-2), an increase in CER was observed with both c-AOD and f-AOD, with a more pronounced increase in CER associated with c-AOD over both the AS and BoB regions. However, as LWP increased, f-AOD exhibited a faster decrease in CER over the BoB compared to the AS. In contrast, c-AOD consistently showed an increasing CER with rising LWP, indicating a contrasting effect relative to f-AOD. These results indicate the dominant radiative effect of fine mode aerosols on cloud formation against the classical microphysical effect of coarse mode aerosols.  Further analysis, incorporating meteorological parameters such as relative humidity and atmospheric stability, is essential to better understand these relationships and enhance the robustness of this study.

How to cite: Bangar, V. and Mishra, A. K.: Satellite-Based Analysis of Size-Segregated Aerosols and Their Effects on Warm Cloud Properties over the Northern Indian Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16951, https://doi.org/10.5194/egusphere-egu25-16951, 2025.

EGU25-18095 | ECS | Posters virtual | VPS3

New Particle Formation and Condensable Vapours in an Arctic Site: Ny-Ålesund 

Aarni Vaittinen, Nina Sarnela, Mikko Sipilä, Zoé Brasseur, Matthew Boyer, Cecilia Righi, Roseline Thakur, Mauro Mazzola, and Lauriane Quéléver

INTRODUCTION 

New particle formation (NPF) is an important source of aerosol particles in the Arctic, the dynamics and drivers of which are still not fully understood. The concentrations of precursor gases, such as sulfuric acid (SA), methane sulfonic acid (MSA), iodic acid (IA), and highly oxygenated organic molecules (HOMs), are strongly linked with the occurrence and strength of NPF. Currently, though, measurement data of NPF, as well as precursor gases, in the Arctic remains extremely limited.

Here we present some preliminary results of our in-situ measurements deployed to study NPF in the Svalbard archipelago. The region is mapped by snow-, ice-, and permafrost-covered land, limited vegetation, and a strong marine influence of the sea ice. SA, MSA, and IA concentrations at the site are interlinked with the behaviour of ocean and sea ice. The terrestrial vegetation emits volatile organic compounds (VOC), which in the atmosphere convert to HOMs. As the Arctic is rapidly transforming due to climate change, all these ecosystems are being altered, which also affects the dynamics of NPF.

METHODS

The measurements considered in this work have been conducted at the Ny-Ålesund Research Station (Svalbard) and, originally started in 2017, represent the longest time series of aerosol data measured with mass spectrometry in the Arctic. In this work, the Arctic summer of 2024 is studied. 

A nitrate-based chemical ionisation atmospheric pressure interface time-of-flight mass spectrometer (CI-APi-TOF, Tofwerk AG.) is used to measure precursor vapour concentrations and identify ion clusters in the ambient air. A neutral cluster and air ion spectrometer (NAIS, Airel Ltd) and a cluster ion counter (CIC, Airel Ltd) are used to monitor neutral particle (2-42nm) and ion cluster (0.8-42nm) size distribution. The measurements are paired with solar radiation data gathered at the Climate Change Tower by CNR (Mazzola et al., Rend. Fis. Acc. Lincei 27, 2016).

RESULTS AND DISCUSSION

A SA/MSA ratio larger than 1 was observed almost throughout the measurement period (Figure 1). This is contrary to previous results from the site by Beck et al. (Geophysical Research Letters 48, 2021). The difference could be due to yearly variation in the oceanic phytoplankton spring bloom, which affects atmospheric MSA concentrations Arctic.

From the preliminary analysis for one week, a diurnal cycle for SA and MSA was observed (Figure 2). NPF occurrence appeared to correlate with radiation intensity, as well as SA and MSA concentrations.

CONCLUSIONS 

These preliminary results highlight the importance of long-term data sets in monitoring Arctic NPF, as they imply strong inter-annual variation in precursor gas concentrations, which may initiate NPF and growth of particles at the study site.

 

Figure 1. Daily mean values for precursor gas concentrations measured with CI-APi-TOF (May-August 2024).  

 

Figure 2. Upper panel: 1.5-hour average values of net short-wave radiation and precursor gas concentrations from a seven-day period with NPF. Lower panel: particle size distribution measured with NAIS, from the same period.

How to cite: Vaittinen, A., Sarnela, N., Sipilä, M., Brasseur, Z., Boyer, M., Righi, C., Thakur, R., Mazzola, M., and Quéléver, L.: New Particle Formation and Condensable Vapours in an Arctic Site: Ny-Ålesund, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18095, https://doi.org/10.5194/egusphere-egu25-18095, 2025.

EGU25-18600 | Posters virtual | VPS3

A tropical EM27/SUN network for satellite validation and long term observations 

Morgan Lopez, Maixent Cassagne, Hippolyte Leuridan, Laura Ticona, Benoit Burban, Wahid Mellouki, Lynn Hazan, and Michel Ramonet

The EM27/SUN instrument is a FTIR spectrometer allowing to retrieve total atmospheric column abundance of CO2, CH4, CO and H2O. LSCE is currently developing a tropical network in the framework of the OBS4CLIM French project.

OBS4CLIM aims at deploying five EM27 at observatories located in tropical (Bolivia, French Guiana, Morocco, Ivory Coast) and background regions (Amsterdam Island, Indian Ocean) for long-term observations and satellite validation purposes (TROPOMI, OCO-2/3, GOSAT, MicroCarb). The chosen stations are also part of French National Observation Service and benefit from in situ greenhouse gas measurements.

The rapid growth of this EM27/SUN network requires developing tools to ensure data quality and availability. Therefore, LSCE has developed:

- An automatic data treatment chain based on PROFFAST (developed and maintained at KIT). Two models are used as a priori profiles (GGG2020, and CAMS) allowing to retrieve daily data in near real-time (NUBICOS project).

- Automatic enclosure systems to protect the instrument from a rough environment. This system allows increasing drastically the daily observations and data availability.

Four of the five stations are fully operational. We will present in details the network construction and the first measurement results.

How to cite: Lopez, M., Cassagne, M., Leuridan, H., Ticona, L., Burban, B., Mellouki, W., Hazan, L., and Ramonet, M.: A tropical EM27/SUN network for satellite validation and long term observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18600, https://doi.org/10.5194/egusphere-egu25-18600, 2025.

EGU25-19010 | Posters virtual | VPS3

Pre-normative research on hydrogen release assessment 

Andy Connor, Alessandro Guzzini, Jadwiga Holewa-Rataj, Paolo Piras, Julie Claveul, Matteo Robino, and Alexandra Kostereva

Hydrogen could play a crucial role in achieving climate neutrality by serving as an energy carrier for renewable sources, offering an alternative to traditional fossil fuels. However, researchers are investigating the impact of hydrogen emissions, as its leakage into the atmosphere poses a concern due to its potential to indirectly influence methane’s atmospheric lifetime and thereby extending its greenhouse effect. Therefore, minimising hydrogen emissions would reduce any potential environmental impact while enhancing safety and efficiency throughout the hydrogen value chain. Thus far, the literature lacks a verified data inventory on the amount of hydrogen emitted from the value chain. Little to no standardized data are present for many elements of the value chain. Otherwise, when present, efforts are still needed for their collection and validation in a unique inventory. The research community needs to address this by improving the capability to quantify small and large emissions and delivering validated methodologies and techniques for measuring or calculating them. An open-access and comprehensible user-friendly tool is urgently needed to better quantify the emissions from the whole hydrogen value chain. The pre-normative research on hydrogen release assessment (NHyRA) project is specifically designed to address these urgent needs. As a first step in this process, the project defined the hydrogen value chain, identifying its main components’ typical operative conditions and recognizing the potential sources of hydrogen emissions.  The next step, the project is working to update an open-access first version of the hydrogen emissions inventory to serve as a reference for the scientific and industrial community. Therefore, by welcoming and validating any contribution of new data, including from outside the NHyRA Consortium, subsequent versions of the inventory will include a more significant amount of data for some of the archetypes (i.e. processes or equipment) in the hydrogen value chain section, to ensure consistent scenario analysis and provide mitigation action recommendations. Furthermore, the NHyRA Consortium experts have identified hydrogen detection and quantification techniques and instruments, covering those which are commercially available and emerging. In this regard, partners of the Consortium have identified three monitoring categories: Detection of emissions at the component level, Detection and quantification of emissions at the component level, and detection and quantification of emissions at the area/site level. Additionally, new or adequately adapted experimental, theoretical, and simulation methodologies will be validated to perform laboratory or in-field measurements to achieve the ambitious goal. Experimental tests will also be performed on the most critical elements of the hydrogen value chains by the partners of the Consortium. A complete picture of the hydrogen emission scenarios, applied on the middle (2030) and long (2050) term European hydrogen economy, will be developed to enable decision-makers to quantify the impact of hydrogen emissions in the energy system transition, identifying  and prioritizing effective risk mitigation actions. Finally, the project will formulate recommendations for Standards and Technical Specifications.

 

How to cite: Connor, A., Guzzini, A., Holewa-Rataj, J., Piras, P., Claveul, J., Robino, M., and Kostereva, A.: Pre-normative research on hydrogen release assessment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19010, https://doi.org/10.5194/egusphere-egu25-19010, 2025.

EGU25-19307 | ECS | Posters virtual | VPS3

Evaluation of Chamber-based soil greenhouse gas emissions in contrasted land use of the Sudanian savanna 

Francis E. Oussou, Souleymane Sy, Jan Bliefernicht, Ines Spangenberg, Samuel S. Guug, Rainer Steinbrecher, Anja Schäffler-Schmidt, Ralf Kiese, Michael Ayamba, Nicaise Yalo, Ayodele Y. Asiwaju-Bello, Windmanagda Sawadogo, Christiana F. Olusegun, Leonard K Amekudzi, and Harald Kunstmann

The effects of major greenhouse gas (GHG) emissions in West Africa remain insufficiently documented. Over two consecutive years, we monitored soil GHG emissions using a chamber-based experimental setup across four contrasting land management conditions in the Sudanian savanna. The environmental drivers of the emissions were assessed through stepwise linear regression and ANOVA statistical tests. Our results show that, regardless of land management conditions, N2O release occurs at the highest rate in rice fields (4.29±2.9 µg N m-2 h-1). The soil acts as a sink for CH4 in the forest reserve (-1.09±7.67 µg C m-2 h-1), whereas degraded lands, such as cropland and rainfed rice farms, exhibit CH4 release at rates of 1.03±13.1 µg C m-2 h-1 and 5.93±12.28 µg C m-2 h-1, respectively. Livestock breeding contributes significantly to CH4 emissions in grasslands, where the annual mean CH4 flux is the highest (16.79±6.69 µg C m-2 h-1). The statistical analysis indicates that 53.8% and 50.2% variability in the CH4 flux is explained by soil moisture and soil temperature respectively in the grassland and rice field. Soil moisture is negatively correlated with N2O release, while the relationship with CH4 is positive in grassland and rice fields, where higher CH4 emissions are observed. N2O flux shows a positive correlation with soil temperature. These findings suggest that land degradation exacerbates CH4 emissions, and the effect of fertilizer use on biomass during the growing season increases CH4 release in rice fields by approximately threefold. At the peak of the raining season, the forest CH4 sink reaches the highest -6.08±14.7 µg C m-2 h-1 while the rainfed rice field releases 9.14±29.57 µg C m-2 h-1. Overall, there is intra annual variability of GHG fluxes with dry and wet years showing different magnitude of N2O and CH4 emissions. The patterns of GHG flux dynamics in this data-scarce region is better clarified through our investigation. We conclude that GHG emissions in response to land cover degradation and agricultural practices, such as fertilizer use, are significant in the Sudanian savanna and urgent decisions are needed to mitigate these effects.

How to cite: Oussou, F. E., Sy, S., Bliefernicht, J., Spangenberg, I., Guug, S. S., Steinbrecher, R., Schäffler-Schmidt, A., Kiese, R., Ayamba, M., Yalo, N., Asiwaju-Bello, A. Y., Sawadogo, W., Olusegun, C. F., Amekudzi, L. K., and Kunstmann, H.: Evaluation of Chamber-based soil greenhouse gas emissions in contrasted land use of the Sudanian savanna, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19307, https://doi.org/10.5194/egusphere-egu25-19307, 2025.

EGU25-19539 | ECS | Posters virtual | VPS3

Quantifying regional and temporal heterogeneity in greenhouse gas emissions from Indian diets 

Saumya Yadav and Srinidhi Balasubramanian

 Providing sufficient and nutritious food while reducing climate emissions footprints from food systems is a Grand Engineering Challenge for India. The increasing dietary emissions pose a serious threat to achieving the national net-zero goal by 2070, yet such emissions are not yet accounted for in India’s Climate Action Plans. Since the 1990s, India’s dietary transitions have been largely propelled by economic development and intensive urbanization, yet such transitions have occurred unequally between urban and rural regions across India.

The regional and temporal heterogeneity in dietary consumption patterns across different populations and the corresponding GHG emissions is not well known. Here, we apply a life-cycle approach to quantify the regional, demographical, and food commodity-specific GHG emissions (CO2, N2O, and CH4) based on detailed household-expenditure data across three national-scale censuses (1999, 2011, 2022). We differentiate such emissions across twelve major food groups that are typically consumed in 88 distinct NSSO regions with demographics (rural and urban) differentiated by income. Our findings suggest that between 1999-2022, the per capita consumption of animal-based products has increased by ~20% respectively, and a ~15% decrease in wholegrain intake. Emissions from dairy (34%), wholegrain (31%), and meat (18%) food groups contributed more than 80% of total dietary emissions for 2011.

The demographical analysis suggested that household expenditure directly influences GHG emissions. For example, the highest expenditure decile of the population was 2.2 kgCO2eq cap-1 day-1  with 0.7 kgCO2eq cap-1 day-1  for the lowest decile in 2011Both rural and urban regions have per capita GHG emissions similarly, but the total emissions and share of food groups varied extremely with the household expenditure. The disparities in total emissions remain as high as 65% among poor and rich households, with poor houses having wholegrain-dominated emissions and rich households having dairy-dominated emissions. The spatial examination further showed the high heterogeneity in emissions among and within Indian states. Our findings highlight the opportunities and challenges in using food consumption as a lever for climate change while also reducing food inequality by shifting to healthier diets. Such findings can help strengthen State Climate Action Plans to help towards green agriculture and sustainable consumption.

How to cite: Yadav, S. and Balasubramanian, S.: Quantifying regional and temporal heterogeneity in greenhouse gas emissions from Indian diets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19539, https://doi.org/10.5194/egusphere-egu25-19539, 2025.

EGU25-19628 | Posters virtual | VPS3

Estimation and validation of direct aerosol radiative forcing in the Korean peninsula using the GEMS dataset 

Ja-Ho Koo, Juhee Lee, and Jeong-Ah Yoo

In this study, we conducted the estimation of shortwave aerosol radiative forcing using the aerosol optical depth (AOD) and supplementary information from the Geostationary Environment Monitoring Spectrometer (GEMS) dataset. We used the libRadtran package for the radiative transfer modeling (RTM), and used the radiative forcing values provided from the Aerosol Robotic Network (AERONET) system for the input value of RTM and the validation task. Total 6 sites in the Korean peninsula are target regions, such as Seoul (Yonsei University and Seoul National university), Anmyeon, Gwangju, Gangneung, and Ulsan. In detail, we used the climatological mean of surface albedo and asymmetry parameter at 4 shortwave channels (440, 675, 870, and 1020 nm), and used daily representative single scattering albedo provided from the GEMS dataset in order to consider the different aerosol type (dust, non-absorbing, and black carbon types). These set-up conditions were finally decided after a number of sensitivity tests. As a result, our estimation of direct aerosol radiative forcing (DARF) at the surface and top of the atmosphere (TOA) shows high correlations with the DARF from the AERONET (correlation coefficient is 0.65 to 0.85 in all 6 sites). Our estimated DARF is a little underestimated compared to the DARF of AERONET, and it seems natural due to the spatial resolution difference. With this high performance, we can provide the daytime hourly variation of DARF over the whole Korean peninsula, which can be useful information to a number of application in the future.

How to cite: Koo, J.-H., Lee, J., and Yoo, J.-A.: Estimation and validation of direct aerosol radiative forcing in the Korean peninsula using the GEMS dataset, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19628, https://doi.org/10.5194/egusphere-egu25-19628, 2025.

EGU25-20229 | ECS | Posters virtual | VPS3

Life cycle assessment of milk production: integrating changes in soil carbon stock with eddy covariance and DNDC modeling 

Yajie Gao, Teng Hu, Marja Roitto, Tapani Jokiniemi, Mari Sandell, Mari Pihlatie, and Hanna Tuomisto

Background aims: Life cycle assessment (LCA) is widely used to evaluate the carbon footprint (CF) of milk production. Changes in soil organic carbon (SOC) stock play a vital role in agricultural greenhouse gas emissions. However, no consensus has been reached to incorporate SOC changes into agricultural LCA. This study aims to evaluate the CF of milk production using LCA methodology with integrating  SOC balance based on data from Viikki Research Farm at Helsinki. Methods: The CF of milk production was analyzed for 2022 and 2023 using the Solagro Carbon Calculator. Furthermore, the study explored the soil carbon and nitrogen balances using the DNDC model, for a comparison with IPCC Tier 1 & Tier 2 methods and the real measurements. Results and conclusions: Real measurements demonstrated substantial SOC loss from grassland and subsequent annual cropland, which was 607 and 3939 kg C ha-1 in 2022 and 2023, respectively. Incorporation of those results increased the CF of milk production. Estimated based on DNDC modeling, the SOC loss exceeded the measured results in 2022 and was underestimated in 2023, while the IPCC method showed SOC sequestration in 2022. The observed emissions fluctuation between the two years was related to the rotation between perennial grass and annual crop, and harsh wintertime conditions affecting crop growth. This study underscores the importance of SOC change in agricultural LCAs. While direct measurements may have limitations, a more profound understanding of SOC dynamics and better calculation is crucial to minimize bias in CF estimations.

How to cite: Gao, Y., Hu, T., Roitto, M., Jokiniemi, T., Sandell, M., Pihlatie, M., and Tuomisto, H.: Life cycle assessment of milk production: integrating changes in soil carbon stock with eddy covariance and DNDC modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20229, https://doi.org/10.5194/egusphere-egu25-20229, 2025.

EGU25-20571 | ECS | Posters virtual | VPS3

Characterization and machine learning prediction of atmospheric pollutants in an urban region of the Cerrado biome 

Marco Aurélio Franco and Márcio Teixeira

The Cerrado biome, a globally significant biodiversity hotspot, is undergoing rapid degradation primarily due to anthropogenic activities. Large-scale conversion of native vegetation for agriculture, particularly soybean and cattle ranching, and strong urbanization rates are the main drivers of the biome losses. Additionally, unsustainable water use, infrastructure development, and recurrent fires exacerbate ecosystem degradation, leading to significant biodiversity decline and ecosystem service impairment. A direct consequence of this change in land use is the generation of substantial quantities of air pollutants, mainly particulate matter of 2.5 and 10 𝜇m (PM2.5 and PM10, respectively). These particles, emitted from biomass burning, soil erosion, and dust storms, can penetrate the respiratory tract, leading to various health issues, including respiratory infections, cardiovascular disease, and increased mortality rates. Using measurements of meteorological variables and air pollutants from CETESB (Environmental Company of the State of São Paulo) from 2017 to 2023 in an important urbanized region of the Brazilian Cerrado, we characterized the seasonal distribution of PM2.5 and PM10, together with other pollutants, such as nitrogen oxides (NOx), carbon monoxide (CO) and ozone (O3). In addition, using different combinations of meteorological and air pollution variables, we trained machine learning models to predict the concentration of PM2.5 and PM10. We list Random Forest, XGBoost, and Artificial Neural Networks (ANN) among these models. Our results show that a lower concentration of air pollutants (PM10, PM2.5, CO, and NOx) is observed during summer, while, in contrast, the peak occurs during winter. This is directly related to the seasons with higher and lower precipitation rates. Curiously, O3 peaks in spring and is minimal in autumn, likely related to cloud occurrence. During the whole analyzed period, NOx, PM10, and PM2.5 exceeded the daily average limits of the World Health Organization by about 15, 22 and 35%, respectively. Regarding the predictive models, the random forest better predicted PM10 and PM2.5 concentrations. For PM10, the statistical results for the train (80% of the data)/test (20% of the data) set were R² = 0.79/ 0.92 (p-value < 0.05), with RMSE of 10.7 and 6.5 𝜇g m-3. For PM2.5, the model returned R² = 0.74/0.91, with RMSE of 4.3 and 2.6 𝜇g m-3 for the train/test set, respectively. Although not the best, the ANN also worked relatively well after proper tuning. Future investigations will extend and validate the predictions obtained in this study to other stations in the Cerrado biome with multiple models to spatialize the PM prediction and obtain the regions in which the most air pollutants are emitted. 

How to cite: Franco, M. A. and Teixeira, M.: Characterization and machine learning prediction of atmospheric pollutants in an urban region of the Cerrado biome, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20571, https://doi.org/10.5194/egusphere-egu25-20571, 2025.

Oxygenated volatile organic compounds (OVOCs) significantly contribute to the radical formation in the troposphere, enhancing atmospheric oxidation capacity and driving secondary pollutant production. However, uncertainties in OVOC emissions hinder accurate assessments of their regional impacts. This study updates OVOC emission profiles for the Yangtze River Delta (YRD) region and integrates them into the Community Multiscale Air Quality (CMAQ) model to refine OVOC estimations. The updated model effectively captures the diurnal variations of most OVOCs, significantly reducing biases compared to simulations based on previous inventories. OVOCs, particularly formaldehyde (HCHO), are key precursors of hydroperoxyl radicals (HO2), which play a dominant role in ozone production across the YRD. Anthropogenic emissions, primarily from industrial activities and vehicular sources, account for 40−60% of total OVOCs. Sensitivity simulations reveal that reducing emissions of reactive OVOCs, such as HCHO and glyoxal, effectively lowers regional ozone levels. These findings underscore the pivotal role of OVOCs in radical chemistry and ozone formation, providing insights for mitigating ozone pollution in rapidly urbanizing regions like the YRD.

How to cite: Li, J.: Photooxidation of Oxygenated Volatile Organic Compounds as a Major Source of Hydroperoxyl Radicals Driving Ozone Formation in the Yangtze River Delta Region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21194, https://doi.org/10.5194/egusphere-egu25-21194, 2025.

AS1 – Meteorology

EGU25-1679 | ECS | Orals | AS1.1

Effect of boundary layer low-level jet on fog fast spatial propagation 

Shuqi Yan, Hongbin Wang, Xiaohui Liu, Fan Zu, and Duanyang Liu

The spatiotemporal variation of fog reflects the complex interactions among fog, boundary layer thermodynamics and synoptic systems. Previous studies revealed that fog can present fast spatial propagation feature and attribute it to boundary layer low-level jet (BLLJ), but the effect of BLLJ on fog propagation is not quantitatively understood. Here we analyze a large-scale fog event in Jiangsu, China from 20 to 21 January 2020. Satellite retrievals show that fog propagates from southeast coastal area to northwest inland with the speed of 9.6 m/s, which is three times larger than the ground wind speeds. The ground meteorologies are insufficient to explain the fog fast propagation, which is further investigated by WRF simulations. The fog fast propagation could be attributed to the BLLJ occurring between 50 and 500 m, because the wind speeds (10 m/s) and directions (southeast) of BLLJ core are consistent with fog propagation. Through sensitive experiments and process analysis, three possible mechanisms of BLLJ are revealed: 1) The abundant oceanic moisture is transported inland, increasing the humidity of boundary layer and promoting condensation; 2) The oceanic warm air is transported inland, enhancing the inversion layer and favouring moisture accumulation; 3) The moisture advection probably promotes low stratus formation, and later it subsides to be ground fog by turbulent mixing of fog droplets. The fog propagation speed would decrease notably by 6.4m/s (66%) in the model if the BLLJ-related moisture and warm advections are turned off.

How to cite: Yan, S., Wang, H., Liu, X., Zu, F., and Liu, D.: Effect of boundary layer low-level jet on fog fast spatial propagation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1679, https://doi.org/10.5194/egusphere-egu25-1679, 2025.

During 29th July to 1st August in 2023, a persistent heavy rainfall event (“23·7” event) hit North China causing severe floods, enormous infrastructure damage and large economy loss. Observational analysis shows that the extremely large accumulation of precipitation and long duration of this event are closely related to a slowly moving landfall typhoon “Dusuari” over North China due to the blocking effect of an anomalous high over the mid- and high-latitude Asia. The anomalous southeasterly flow induced by the typhoon “Dusuari” and another typhoon “Kanu” over the East China Sea jointly built a highly efficient channel of water vapor supplying from southern oceans towards North China. A water vapor budget analysis indicates that precipitation of this event is mainly caused by dynamic process involving strong ascending motion. Accompanying strong water vapor transportation and convergence over North China, large amount of latent heat is released in the middle and lower troposphere. The physical mechanisms of heavy rainfall-induced diabatic heating in maintaining the precipitation over North China is further investigated using statistics analysis and numerical experiments. On one hand, the latent heating released by heavy rainfall induces significant uplifting flows which causes more precipitation. On the other hand, the heavy rainfall-induced diabatic heating contributes to enhancement of the westward extension of high-pressure dam around the Mongolian Plateau through a regional meridional circulation. This strengthened high pressure dam sustained the cyclonic circulation of “Dusuari” over North China, leading to continuous heavy rainfall there.

How to cite: Zhao, W.: Mechanisms of persistent extreme rainfall event in North China, July 2023: Role of atmospheric diabatic heating, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1762, https://doi.org/10.5194/egusphere-egu25-1762, 2025.

EGU25-1763 | ECS | Orals | AS1.1

Wind profile warning characteristics of short-term heavy rain during the Meiyu season 

Jingyu Wang, Chunguang Cui, Xiaokang Wang, and Xiaofang Wang

This study examines the spatial and temporal distributions of short-term heavy rain (SHR) in the middle Yangtze River basin (MYRB) in the summers of the past decade. SHR events are most frequent during the annual Meiyu periods, significantly contributing to total precipitation. Additionally, these events generally last longer and tend to peak at night. The occurrence of SHR events decrease from southeast to northwest, influenced by the monsoonal flow and the small-scale terrain. Moisture convergence prior to Meiyu SHR events is predominantly influenced by both southerly and easterly winds below 700 hPa. Frequent low-level jets and quasi-steady cyclonic circulation lead to strong southerly winds prevailing over the eastern MYRB, while weaker easterly winds dominate in the west. Wind profiles derived from wind profile radar products illustrate the preceding changes in wind speed, wind directions, and vertical wind shear below 4 km above ground level (AGL), as well as the timing of these changes. In the plain area of southeastern MYRB, accelerated southwesterlies are observed 3 to 4 hours before SHR events, accompanied by an intensification of southerly winds near the boundary layer top 2 hours prior. Within the hour leading up to the SHR events, wind speeds sharply rise to their peak. In front of the mountains in west MYRB, southwesterlies strengthen 5 hours in advance but then weaken as they shift to northerlies. Just before the SHR events, however, reinforced northerlies occur near the surface. In the mountainous region of western MYRB, while changes in wind speed are minimal due to topographic blocking, the frequency of southeasterly components below 2 km AGL significantly increases 4 hours before SHR events. The preceding timing of significant vertical wind shear coincides with the increase in wind speed and the change in wind direction. Understanding the detailed characteristics of wind profiles preceding the SHR events during the Meiyu seasons can provide valuable insights for localized severe weather early warning systems. 

How to cite: Wang, J., Cui, C., Wang, X., and Wang, X.: Wind profile warning characteristics of short-term heavy rain during the Meiyu season, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1763, https://doi.org/10.5194/egusphere-egu25-1763, 2025.

Convective clouds during the Mei-yu season contribute significantly to the total rainfall and related disasters over the middle and lower reaches of the Yangtze River in China. Studying the effects of aerosols on convective clouds is of great importance to weather and climate research. However, there are still many open questions to address. This study investigated the effects of aerosol on convections with different cloud geometrical thickness (CGT) bins during the 2018 Mei-yu season, which lasted for 17 days from 18 June to 5 July. Contrasting aerosol effects on shallow and deep convective clouds were revealed by means of anthropogenic aerosol experiments in the Weather Research and Forecasting model with Chemistry (WRF-Chem). Specifically, increased anthropogenic aerosols lead to a 9% reduction in total rainfall and a 7.17% decrease in convection occurrences during the Mei-yu season. After adopting a methodology that stratifies the convective clouds by fixing the CGT, we found that increasing aerosols suppress shallow convections with CGT less than 4 km and invigorate deep convections with CGT greater than 4 km. Increased aerosols enhance the scattering of shortwave radiation, resulting in cooling of the surface air and increasing the stability of the regional lower atmosphere, potentially suppressing shallow convection. Meanwhile, in deep convection, with its stronger updraft and more latent heat, convective invigoration occurs under polluted conditions due to the aerosol-related microphysical and dynamical responses. Considering the high-humidity environment during the Mei-yu season, additional relative humidity tests show that the competing aerosol effects come from convective core invigoration and convective periphery processes which enhance evaporation and dissipation, demonstrating relative humidity is a critical factor in maintaining the net aerosol effects on convections. These results contribute to a better understanding of the effects of anthropogenic aerosols on convections during the Mei-yu season and the competing effects of aerosols depending on the ambient environmental conditions.

How to cite: liu, L.: Contrasting aerosol effects on shallow and deep convections during the Mei-yu season in China , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1775, https://doi.org/10.5194/egusphere-egu25-1775, 2025.

The present study assesses the simulated precipitation and cloud properties using three microphysics schemes (Morrison, Thompson, and MY) implemented in the Weather Research and Forecasting model. The precipitation, differential reflectivity (ZDR), specific differential phase (KDP) and mass-weighted mean diameter of raindrops (Dm) are compared with measurements from a heavy rainfall event that occurred on 27 June 2020 during the Integrative Monsoon Frontal Rainfall Experiment (IMFRE). The results indicate that all three microphysics schemes generally capture the characteristics of rainfall, ZDR, KDP, and Dm, but tend to overestimate their intensity. To enhance the model performance, adjustments are made based on the MY scheme, which exhibited the best performance. Specifically, the overall coalescence and collision parameter (Ec) are reduced, which effectively decreases Dm and makes it more consistent with observations. Generally, reducing Ec leads to an increase in the simulated content (Qr) and number concentration (Nr) of raindrops across most time steps and altitudes. With a smaller Ec, the impact of microphysical processes on Nr and Qr varies with time and altitude. Generally, the autoconversion of droplets to raindrops primarily contributes to Nr, while the accretion of cloud droplets by raindrops plays a more significant role in increasing Qr. In this study, it is emphasized that even the precipitation characteristics could be adequately reproduced, accurately simulating microphysical characteristics remains challenging and it still needs adjustments in the most physically based parameterizations to achieve more accurate simulation.

How to cite: Zhou, Z.: An evaluation and improvement of microphysical parameterization for a heavy rainfall process in Meiyu season, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1816, https://doi.org/10.5194/egusphere-egu25-1816, 2025.

EGU25-1939 | Orals | AS1.1

Stochastic Galerkin method for cloud simulation 

Alina Chertock

In this talk, we consider a mathematical model of cloud physics that consists of the Navier-Stokes equations coupled with the cloud evolution equations for water vapor, cloud water, and rain. In this model, the Navier-Stokes equations describe weakly compressible flows with viscous and heat conductivity effects, while microscale cloud physics is modeled by the system of advection-diffusion-reaction equations. We aim to explicitly describe the evolution of uncertainties arising from unknown input data, such as model parameters and initial or boundary conditions. The developed stochastic Galerkin method combines the space-time approximation obtained by a suitable finite volume method with a spectral-type approximation based on the generalized polynomial chaos expansion in the stochastic space. The resulting numerical scheme yields a second-order accurate approximation in both space and time and exponential convergence in the stochastic space. Our numerical results demonstrate the reliability and robustness of the stochastic Galerkin method. We also use the proposed method to study the behavior of clouds in certain perturbed scenarios, for example, the ones leading to changes in macroscopic cloud patterns as a shift from hexagonal to rectangular structures.

How to cite: Chertock, A.: Stochastic Galerkin method for cloud simulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1939, https://doi.org/10.5194/egusphere-egu25-1939, 2025.

EGU25-2024 | Posters on site | AS1.1

Analysis and research on the impact of terrain on the "23.7" extremely heavy rainstorm 

xiaoyu huang, zhenzhen wu, feng xue, and chenghao fu

From 08:00 on July 29 to 08:00 on August 2, 2023, under the influence of typhoon "Dussuri", an extremely heavy rainstorm process occurs in Hebei and Beijing. The precipitation in some areas of the windward slope of Taihang Mountains exceeds 250mm, and in some areas it exceeds 500mm. The distribution of heavy precipitation is basically consistent with the terrain of the windward slope. Using the 6-minute radar retrieved wind field network data developed by the CMA (China meteorological administration) Meteorological Observation Center for analysis, it is found that from 13:00 on July 29th to 20:00 on August 1st, a southeast-oriented ultra-low-level jet greater than 12 m/s was maintained in the 925-hPa field over Hebei and Beijing. The angle between the jet and the Taihang Mountains is almost 90°, and at the same time, a 850-hPa typhoon trough stays on the windward slope for a long time, resulting in stable and less movement of heavy precipitation echoes. This series of factors together led to the occurrence of the extremely heavy rainstorm process. Using the ERA5 hourly reanalysis data as the initial field and based on the WRF4.5 model, a sensitivity test is conducted on this process using three-layer bidirectional nesting (grid spacing of 9km, 3km, and 1km, respectively). The experiment reduces the Yanshan and Taihang Mountains to half of their original heights and 50 meters, respectively (equivalent to the altitude of Beijing). The experimental results indicate that: (1) Precipitation impact: Due to the easterly winds brought by typhoons, the eastern side of Taihang Mountains is on the windward slope, which has a significant impact on precipitation. When the height of Taihang Mountains decreases, the precipitation intensity significantly weakens; When the terrain height drops to 50m, the precipitation location is biased to the west compared to the actual situation. (2) The experiment showed that the blocking effect of Taihang Mountains formed mesoscale low vortex and convergence line on the windward slope. When the height of Taihang Mountains drops to half of its original height or only 50 meters, the mesoscale low vortex and convergence line move westward to Shaanxi Province. (3) The vertical profile analysis along the east-west direction of Taihang Mountains shows strong upward movement in the windward slope area, with positive vorticity in the lower level and negative vorticity in the upper level. When the height of Taihang Mountains decreases, the upward movement significantly weakens, and the positive and negative vorticity weakens until it disappears, indicating that the dynamic effect of terrain has a significant impact on precipitation processes. (4) The Yanshan Mountains are oriented east-west, and parallel to the environmental winds. Therefore, when its height decreases, its impact on physical quantities such as precipitation, wind field, vertical velocity, and vorticity is relatively small.

Key words: terrain, "23.7" extremely heavy rainstorm, analysis

How to cite: huang, X., wu, Z., xue, F., and fu, C.: Analysis and research on the impact of terrain on the "23.7" extremely heavy rainstorm, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2024, https://doi.org/10.5194/egusphere-egu25-2024, 2025.

EGU25-2044 | Orals | AS1.1

A New Method for Calculating Highway Blocking due to High Impact Weather Conditions 

Duanyang Liu, Tian Jing, Mingyue Yan, and Ismail Gultepe

 Fog, rain, snow, and icing are the high-impact weather events often lead to the highway blockings, which in turn causes serious economic and human losses. At present, there is no clear calculation method for the severity of highway blocking which is related to highway load degree and economic losses. Therefore, there is an urgent need to propose a method for assessing the economic losses caused by high-impact weather events that lead to highway blockages, in order to facilitate the management and control of highways and the evaluation of economic losses. The goal of this work is to develop a method to be used to assess the high impact weather (HIW) effects on the highway blocking. Based on the K-means cluster analysis and the CRITIC (Criteria Importance through Intercriteria Correlation) weight assignment method, we analysed the highway blocking events occurred in Chinese provinces in 2020. Through cluster analysis, a new method of severity levels of highway blocking is developed to distinguish the severity into five levels. The severity levels of highway blocking due to high-impact weather are evaluated for all weather types. As a part of calculating the degree of highway blocking, the highway load in each province is evaluated. The economic losses caused by dense fog are specifically assessed for the entire country.

How to cite: Liu, D., Jing, T., Yan, M., and Gultepe, I.: A New Method for Calculating Highway Blocking due to High Impact Weather Conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2044, https://doi.org/10.5194/egusphere-egu25-2044, 2025.

I will introduce a flux globalization-based well-balanced path-conservative central-upwind scheme on Cartesian meshes for the two-dimensional (2-D) two-layer thermal rotating shallow water equations. The scheme is well-balanced in the sense that it can exactly preserve a variety of physically relevant steady states. In the 2-D case, preserving general "moving-water" steady states is difficult, and to the best of our knowledge, none of existing schemes can achieve this ultimate goal. The proposed scheme can exactly preserve the 𝑥- and 𝑦-directional jets in the rotational frame as well as certain genuinely 2-D equilibria. Numerical experiments demonstrate the performance of the proposed scheme in computationally non-trivial situations: in the presence of shocks, dry areas, non-trivial topographies, including discontinuous ones, and in the case of hyperbolicity loss. The scheme works equally well in both the 𝑓-plane and beta-plane frameworks.

How to cite: Kurganov, A., Cao, Y., Liu, Y., and Zeitlin, V.: Flux Globalization-Based Well-Balanced Path-Conservative Central-Upwind Scheme for Two-Dimensional Two-Layer Thermal Rotating Shallow Water Equations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2053, https://doi.org/10.5194/egusphere-egu25-2053, 2025.

EGU25-2224 | ECS | Posters on site | AS1.1

Interpretable ultivariate scoring rules based on aggregation and transformation 

Romain Pic, Clément Dombry, Philippe Naveau, and Maxime Taillardat

Proper scoring rules are an essential tool to assess the predictive performance of probabilistic forecasts. However, propriety alone does not ensure an informative characterization of predictive performance and it is recommended to compare forecasts using multiple scoring rules. With that in mind, interpretable scoring rules providing complementary information are necessary. We formalize a framework based on aggregation and transformation to build interpretable multivariate proper scoring rules. Aggregation-and-transformation-based scoring rules can target application-specific features of probabilistic forecasts, which improves the characterization of the predictive performance. This framework is illustrated through examples taken from the weather forecasting literature and numerical experiments are used to showcase its benefits in a controlled setting. Additionally, the framework is tested on real-world data of postprocessed wind speed forecasts over central Europe. In particular, we show that it can help bridge the gap between proper scoring rules and spatial verification tools.

How to cite: Pic, R., Dombry, C., Naveau, P., and Taillardat, M.: Interpretable ultivariate scoring rules based on aggregation and transformation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2224, https://doi.org/10.5194/egusphere-egu25-2224, 2025.

EGU25-2650 | ECS | Orals | AS1.1

Constraining Future Changes in Extreme Precipitation Using Typical Synoptic Patterns 

Yang Hu, Yanluan Lin, Jiawei Bao, and Yi Deng

The middle and lower reaches of the Yangtze River (MLYR) suffers from extreme precipitation (EP) during summer, which has a huge impact on human society and ecosystem. However, the large spreads among climate models hinder their application in future risk assessment. In this work, four typical synoptic patterns (SPs) triggering EP over MLYR are identified based on the clustering algorithm. And we found a significant linear correlation between the CMIP6 (sixth phase of Coupled Model Intercomparison Project) models’ ability to reproduce the observed typical SPs in present-day climate and the projected future changes of EP over MLYR. Then we proposed an emergent constraint method for EP projections based on this linear correlation and the observed SPs. Using this method, the model spread is evidently narrowed, which increases the credibility of projected future EP changes.

How to cite: Hu, Y., Lin, Y., Bao, J., and Deng, Y.: Constraining Future Changes in Extreme Precipitation Using Typical Synoptic Patterns, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2650, https://doi.org/10.5194/egusphere-egu25-2650, 2025.

From July 29 to August 1, 2023, extreme heavy rainfall occurred in the Chinese HUABEI region. Heavy rainstorm occurred in the most areas of Beijing, Tianjin and Hebei province. The daily precipitation of 14 national meteorological observatories  exceeded the historical extreme value. The process intensity exceeded the three extreme rainstorm processes in the history of HUABEI region. Studying the causes of extreme heavy precipitation in HUABEI and evaluating the predictive performance of the model for extreme heavy precipitation is beneficial for improving the application and forecasting ability of the model. This article analyzes the weather scale characteristics and anomalies of this precipitation process from factors such as height field, wind field, divergence field, vorticity field, and water vapor. The dynamic and thermal structure of the vortex and the cause of the upper level continental high  are analyzed using the method of cyclone phase space map and full type vorticity equation. Finally, the predictive ability of the model for extreme precipitation is tested. The following main conclusions have been drawn:(1) The precipitation process is divided into two stages. Before the 31st, it was caused by the residual vortex circulation of the "Dussuri", with strong precipitation intensity and range. After the 31st, it was formed by the convergence of the easterly jet on the west side of the subtropical high pressure and its interaction with the terrain. Precipitation was mainly concentrated in the northern part of China, with weaker rainfall intensity compared to the previous period.(2) The key impact systems of this process are the 200hPa high trough and continental high pressure, the 500hPa blocking high pressure, and the residual circulation of the low-level "Dussuri". The divergence in front of the 200hPa high altitude trough is beneficial for maintaining upward movement in the North China region; At 500hPa, there is a blocking high pressure in the northern and eastern parts of North China, which is conducive to the maintenance of low-level vortex systems. The "Dussuri" convergence circulation is the triggering system of the process.(3) The water vapor conditions during this process were exceptionally good, mainly consisting of three water vapor transport paths: the southerly water vapor transport of the South China Sea monsoon, the eastward water vapor transport of the residual circulation of "Dussuri", and the southeast water vapor transport path of typhoon "Kanu".(4) During the northward movement, the residual vortex of the Dussuri maintains a quasi symmetric and warm center structure, with weak cold advection in the upper level of the vortex on the 30th.(5) The uneven vertical distribution of condensation latent heat heating generates negative vorticity in the upper troposphere, ensuring the stable maintenance of continental high pressure.(6) In global model forecasting, the CMA model cannot report a blocking high pressure above 96 hours of time. The EC deterministic model can predict heavy precipitation processes within a 120 hour time frame, and the ensemble forecast can have a predictable time frame of up to 7 days.

How to cite: guan, Y.: Analysis and Model Verification of Extreme rainfall Processes in Huabei of China in 2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2697, https://doi.org/10.5194/egusphere-egu25-2697, 2025.

This article introduces the five-year research plan of the project and the preliminary progress made over the past two years: 1. Implemented tracking observation experiments on the Mei-Yu frontal extreme precipitation associated in the middle and lower reaches of the Yangtze River for the years 2023 and 2024; 2. Investigated the triggering and maintenance mechanisms of extreme precipitation related to multi-scale interactions and associated thermodynamic conditions; 3. Conducted studies on the microphysical structure and evolution simulation of extreme precipitation. To be specific, the mechanism of low-level jet formation is analyzed during the rainy season in the Yangtze River Basin in 2024.

How to cite: Cui, C. and Wang, B.: Preliminary results on the Mei-Yu Frontal Heavy Rainfall Tracking Observation Experiment and Related Studies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3219, https://doi.org/10.5194/egusphere-egu25-3219, 2025.

In this study, the microphysical characteristics of summer and winter liquid rainfall are analyzed by 4 Parsivel sites in Hubei Province in the middle reaches of the Yangtze River during 2015-2018. The possible reasons for summer and winter DSD differences are also discussed. The main conclusions are summarized as follows:

(1) Hubei Province is dominated by stratified rainfall in winter, while summer includes convective, stratified, and mixed rainfall. Compared with winter, the average rain rate and Dm in summer are larger, the number concentration Nw is relatively smaller, while difference between δM is very small. The PDF distribution of Dm peak value are about 1.0 mm both in summer and winter, and the Dm data is skewed to the right while the Nw show the opposite.

(2) With increasing rain rate, the Dm increases in both summer and winter. For rain rate R < 2 mm h-1, there are larger Dm and smaller Nw in summer than that in winter, while for the rain rete R > 2 mm h-1 shows the opposite.

(3) There are differences in the μ-λ and Z-R relationships between summer and winter in the middle reaches of the Yangtze River. The relationships also different from those in the lower reaches of the Yangtze River.

(4) The middle reaches of the Yangtze River are mainly influenced by the warm and humid air transport originates in the subtropical South Indian Ocean. In summer, the convective rainfall raindrops grow by collision–coalescence mechanism, and the break-up mechanism also plays an important role which makes smaller diameter. The ice particles could grow sufficiently and fall to the ground with enough time by the accretion mechanism in winter.

In summary, this study gives an insight into the seasonal characteristics of rainfall microphysics in summer and winter, which are very useful for radar QPE and numerical forecasting models modify in the middle reaches of the Yangtze River. However, due to the limitation of observation data, more types of observation data and numerical models simulation should be included to understand the mechanism of the microphysical processes for future reach.

How to cite: Wang, B. and Fu, Z.: The seasonal characteristics of summer and winter raindrops size distribution in Central China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3232, https://doi.org/10.5194/egusphere-egu25-3232, 2025.

EGU25-3272 | Orals | AS1.1

Climate change will increase aircraft take-off distances and reduce payloads, but by how much? 

Jonny Williams, Paul Williams, Federica Guerrini, and Marco Venturini

Climate model output at 30 European airports (including 25 of the busiest) is used to investigate summer take-off distance required – TODR – and maximum take-off mass – MTOM – and how they may change in the future. We compare data from 2035–2064 to a historical baseline of 1985–2014 using three future forcing scenarios which represent low (SSP1-2.7), medium (SSP3-7.0), and high (SSP5-8.5) future emissions trajectories defined by the widely used Shared Socioeconomic Pathways, SSPs.

This work presents data for the A320 aircraft manufactured by Airbus but the calculation framework is widely applicable to any similar fixed-wing aircraft and uses entirely open-access input data.

We use 10 models from the 6th Coupled Model Intercomparison Project (CMIP6) which have a range of equilibrium climate sensitivity values; a measure of the amount of global warming they give for a doubling of carbon dioxide concentrations.

We use a numerical scheme which considers the resultant forces on an aircraft in the runway acceleration phase of its take-off and show that 30-year average values of TODR could increase by up to 100 m by mid-century. There is, however, significant variability since daily data is used throughout.

We quantify the changing probability distribution of TODR using kernel density estimation and illustrate this using an example showing how increases in extreme daily maximum temperature could alter distributions of TODR.

Additionally, we project that the 99th percentile (a one in a hundred day event) of the TODR from 1985-2014 may by exceeded on as many as half the summer days for some sites in the future.

Four of the airports studied (Chios, Pantelleria, San Sebastian and Rome Ciampino) have runway lengths which are shorter than the TODR when the aircraft is carrying its maximum payload. This means that the weight they carry must be reduced to fulfil safety constraints, which will only become more stringent as temperatures increase further. Relative to the mean weight-restriction amount for the historical period, we find that the number of passengers may have to be reduced by up to 10-12 passengers per flight, again accompanied by a significantly increased chance of exceeding extreme historical values.

How to cite: Williams, J., Williams, P., Guerrini, F., and Venturini, M.: Climate change will increase aircraft take-off distances and reduce payloads, but by how much?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3272, https://doi.org/10.5194/egusphere-egu25-3272, 2025.

EGU25-3417 | Posters on site | AS1.1

Evolution and Cause Analysis of a Heavy Precipitation Process of Meiyu Along Yangtze River 

Houfu Zhou, Nan Ge, and Wen Qi

Based on the observational and forecast datasets from precipitation merging product, radiosonde, Doppler radar, wind profiler radar and ECMWF product, the evolution and causes of the heavy precipitation process of Meiyu in the middle and lower reaches of the Yangtze River in China from June 21 to 22, 2024 were analyzed. The results show as the followings. (1) The heavy precipitation was mainly distributed in the northern part of Hunan Province, the southeastern part of Hubei Province and the western part of Anhui Province, with the main period from 15:00 on June 21 to 15:00 on June 22, especially in the early morning of June 22. The rain belt was located to the north of the subtropical high, in the north of the low-level jet, and at the front side of the moving trough line. (2) The K index exceeded 38℃ in all areas, and the CAPE before and after this heavy precipitation process was over 800 J/kg and less than 100 J/kg, respectively, indicating the evolution characteristics of unstable atmospheric stratification as well as the energy accumulation and release. (3) In the early stage of this process, the surface high temperature was distributed to the south of Wuhan, and the near-surface convergence line extended from the eastern part of Henan Province to the central part of Hubei Province. In the middle stage of this process, the convergence line moved eastward. In the later stage of this process, there was a significant cold pool over the land surface along the Yangtze River. The near-surface high temperature and convergence line were the triggering mechanisms of the heavy precipitation, while the cold pool led to the gradual weakening of the precipitation. (4) The water vapor flux was mainly located in the northern part of Hunan Province, the eastern part of Hubei Province as well as the southern part of Anhui Province, and gradually moved eastward. The flux values in the middle and lower layers were relatively high in the early morning of June 22. There were two water vapor transport belts in the lower layer, corresponding to different heavy precipitation centers. (5) The approximately east-west oriented echo band moved from west to east through the forms of merging, strengthening and dissipating. The south side of the echo band was the mesoscale linear or hook-shaped strong echo accompanied by high echo top and strong VIL. The meso-β scale convective system was composed of several meso-γ scale convective cells, and the meso-γ scale convective cells caused strong cumulative precipitation through the ‘train effect’.

How to cite: Zhou, H., Ge, N., and Qi, W.: Evolution and Cause Analysis of a Heavy Precipitation Process of Meiyu Along Yangtze River, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3417, https://doi.org/10.5194/egusphere-egu25-3417, 2025.

EGU25-3842 | Posters on site | AS1.1

 IAGOS estimates of climate-process costs for trans-Atlantic flights 

Corwin Wright

IAGOS, or the In-service Aircraft for a Global Observing System project, is a European Infrastructure project consisting of scientific measurement packages attached to commercial aircraft. Operating since 1994, this programme provides a unique long-timeseries dataset of flight data across the globe, with thousands of flights per year providing a strong base for statistical studies.

Here, we use flight times derived from IAGOS metadata to quantify the role of the El Nino - Southern Oscillation (ENSO), the Quasi-Biennial Oscillation, the solar cycle and the North Atlantic Oscillation (NAO) on trans-Atlantic flight times. We do this both by subsetting the data in various ways and via regression methods. This allows us to statistically assess the effects of these large-scale atmospheric-dynamical processes on trans-Atlantic flight times. We also calculate the additional costs associated with these effects in terms of both carbon dioxide emissions and fuel costs, allowing us to understand how climate processes drive them.

Depending on season and direction of flights, we show that these four climate indices can explain as much as 1/3 of the total variance in trans-Atlantic flight times. At a flight-time level and particularly in winter, the NAO dominates flight times and is the most important factor in one-way fuel costs: flights at peak NAO+ can be as much as 83 minutes longer than the equivalent flight at peak NAO- when crossing the Atlantic. However, at a whole-dataset level, ENSO is shown to be much more important in driving net round-trip costs. We further estimate that the monthly cost of these four climate indices can be as high as 100 kT of additional CO2 or USD 20 million at 2023 flight volumes and fuel prices.

How to cite: Wright, C.:  IAGOS estimates of climate-process costs for trans-Atlantic flights, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3842, https://doi.org/10.5194/egusphere-egu25-3842, 2025.

The MicroWave Humidity Sounder II (MWHS II) is a cross-track microwave sounder flying on FengYun (FY)-3C satellite. It has 15 channels ranging from 89.0 to 191.0 GHz, eight (channels 2-9) of which are located near 118.75 GHz along an oxygen absorption line, five (channels 11-15) of which are located near 183.31 GHz water vapor absorption line and the remaining two channels 1 and 10 are two window channels centered at 89.0 and 150.0 GHz. A new precipitation detection algorithm for 118GHz channels was developed based on the radiation characters of the double O2 absorption bands (118 and 50-60 GHz). Since both of the 118 GHz and 50-60 GHz oxygen absorption bands are sensitive to atmospheric temperature, the radiation observed in the two bands has a specific inherent constraint relationship under the clear-sky conditions. However, the frequencies of 118 GHz channels are approximately twice that of the 50-60 GHz channels, and the two bands have different absorption and scattering characteristics for atmospheric hydrometeors. The radiance transfer mode VDISORT was used to simulate the sensitivity of the 118 GHz and 50-60 GHz channels to five kinds of hydrometeors (cloud water, rainwater, ice, snow, and graupel) in the cloud atmosphere. The results show that the 50-60 GHz channels are more sensitive to rainwater, and the 118 GHz channels are more sensitive to the other four types of hydrometeors. Therefore, the inherent constraint of the observational radiance between 118 GHz and 50-60 GHz channels under clear-sky condition is no longer valid for a cloudy scenario. In this paper, the machine learning system TensorFlow was used to construct a model for predicting the brightness of 118 GHz channels using 50-60 GHz observations under clear-sky conditions, and the accuracy of the prediction model was validated using independent samples. Then this neural network-based predictive model was used for 118 GHz channel precipitation detection. When the difference between actual observed and predicted bright temperature for 118 GHz channel is more massive than three times of the standard deviation of the prediction model, it is thought that the MWHS II observation is contaminated by precipitation or cloud. At last, this new precipitation detection algorithm for 118 GHz was validated by simulated measurements. The results show that both the precipitation detection POD (test probability) and PC (correct rate) for 118 GHz channels are above 90%.

How to cite: Guo, Y.: A precipitation detection algorithm for 118GHz channels based on FY-3C MWHS II and FY-3C MWTS II, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3880, https://doi.org/10.5194/egusphere-egu25-3880, 2025.

EGU25-4138 | ECS | Orals | AS1.1

Methodological Focus on Hyperparameters for Different Rain Nowcasting Models 

Baptiste Guigal, Aymeric Chazottes, Laurent Barthès, Nicolas Viltard, Erwan Le Bouar, Emmanuel Moreau, and Cécile Mallet

Precipitation nowcasting plays an essential role in operational weather forecasting services. Sudden precipitation events have significant socio-economic impacts, including natural disasters like flash floods. This challenge is becoming increasingly critical as climate change alters weather patterns and the frequency of extreme weather events continues to increase.

Over the last decade, radar observations, offering high temporal and spatial resolution, have facilitated the development of machine learning methods for precipitation nowcasting. Once trained, these methods are well suited to processing large datasets with low latency, especially in a real-time context. Recent advances in the field of nowcasting have focused on optimizing model architectures, improving loss functions for imbalanced data, and integrating multivariate inputs, including radar and satellite observations.

This study explores some critical hyperparameters, such as temporal context length, edge effect during training, influence of the output horizons prediction, and convolution kernel size. To do this, we investigate the performance of several models, including both machine learning approaches from different families, in particular SmaAt-Unet, ConvLSTM , and DGMR (trained on UK rains) , as well as non-machine learning methods such as  STEPS. An eleven years consistent radar precipitation dataset covering the Paris region was set up from Météo-France mosaic. Nine years were used for training machine learning models, and two years were reserved to evaluate the models’ performances. To assess the model in different weather conditions, the data set is divided into four groups with distinct characteristics corresponding to various meteorological phenomena. To ensure consistent evaluation, we evaluated the models on the same two-year test dataset, focusing on three criteria, namely: spatial consistency (Pearson correlation coefficient), location accuracy (CSI), and precipitation intensity (MSE).

Our analysis reveals that machine learning models consistently outperform traditional optical flow methods, with notable variations in performance across timescales and rainfall intensities. We also highlight that performance is nearly identical for all models in the presence of stratiform rain, while there are substantial differences in the convective rain group. Additionally, we show that for deep learning models, considering edge effects during training prevents the propagation of inevitable errors and helps avoid the appearance of ghost rain cells at the edges of the map. Furthermore, we show that the size of the kernels of the first layers plays an important role and must be large enough to allow correlation between distant pixels.

Finally, our study provides guidelines for the development of precipitation nowcasting models.

How to cite: Guigal, B., Chazottes, A., Barthès, L., Viltard, N., Le Bouar, E., Moreau, E., and Mallet, C.: Methodological Focus on Hyperparameters for Different Rain Nowcasting Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4138, https://doi.org/10.5194/egusphere-egu25-4138, 2025.

EGU25-5038 | Posters on site | AS1.1

On the Dynamical Core of Aeolus 2.0: An Atmospheric Model Using a Moist-Convective Thermal Rotating Shallow Water Framework 

Masoud Rostami, Stefan Petri, Bijan Fallah, and Farahnaz Fazel-Rastgar

This study introduces Aeolus 2.0[1, 2], a novel multilayer moist-convective Thermal Rotating Shallow Water (mcTRSW) model designed to simulate atmospheric dynamics under various forcings, such as increased radiative or thermal forcing, as well as the effects of latent heat release and radiative transfer on meso- and large-scale dynamics. The model incorporates a novel moist-convective scheme that respects conservation laws, a new bulk aerodynamic scheme for sea surface evaporation and sensible heat flux, and provides a computationally efficient yet physically robust framework, bridging the gap between idealized models and complex general circulation models. Aeolus 2.0 integrates barotropic and baroclinic processes, enabling detailed investigations of phenomena such as zonal wind variability, heatwaves, and seasonal energy fluxes.

The model has already been applied to various atmospheric phenomena, such as simulating the Madden-Julian Oscillation (MJO)[3], large-scale localized extreme heatwaves[4], and atmospheric responses to increased radiative forcing during solstices and equinoxes[1]. In this presentation, we showcase the results of the latter. The findings highlight significant changes in zonal wind velocity and meridional temperature gradients, with notable hemispheric asymmetry. Specifically, increased radiative forcing enhances subtropical westerly jet velocities and mid-latitude temperatures during the solstices, while reducing polar cyclone zonal wind velocities in the affected hemisphere. Poleward eddy heat fluxes were consistently observed across hemispheres, and heatwave intensity and duration were amplified over both land and ocean regions.

References:

[1] Rostami, M., Petri, S., Fallah, B., Fazel-Rastgar, F. (2025). Aeolus 2.0's thermal rotating shallow water model: A new paradigm for simulating extreme heatwaves, westerly jet intensification, and more. Physics of Fluids, 37 (1), 016604. https://doi.org/10.1063/5.0244908.

[2] Rostami, M., Petri, S., Guimaräes, S.O., Fallah, B. (2024). Open-source stand-alone version of atmosphere model Aeolus 2.0 Software. Geoscience Data Journal, 11, 1086–1093. https://doi.org/10.1002/gdj3.249. (Link to Zenodo: https://doi.org/10.5281/zenodo.10054154)

[3] Rostami, M., Zhao, B. & Petri, S. (2022). On the genesis and dynamics of madden–Julian oscillation-like structure formed by equatorial adjustment of localized heating. Quarterly Journal of the Royal Meteorological Society, 148, 3788–3813.  https://doi.org/10.1002/qj.4388.

[4] Rostami, M., Severino, L., Petri, S., & Hariri, S. (2023). Dynamics of localized extreme heatwaves in the mid-latitude atmosphere: A conceptual examination. Atmospheric Science Letters, e1188. https://doi.org/10.1002/asl.1188 .

 

How to cite: Rostami, M., Petri, S., Fallah, B., and Fazel-Rastgar, F.: On the Dynamical Core of Aeolus 2.0: An Atmospheric Model Using a Moist-Convective Thermal Rotating Shallow Water Framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5038, https://doi.org/10.5194/egusphere-egu25-5038, 2025.

Based on the brightness temperature observed by the Fengyun-4A satellite, eight hundred mesoscale convective systems (MCSs) are identified in the middle reaches of the Yangtze River Basin during the warm seasons of 2018–2021, and these MCSs are categorized into the quasistationary (QS) type and the outward-moving (OM) type. Afterward, the initiations of the MCSs are backward tracked using a hybrid method of areal overlapping and optical flow. Then, the intensity, evolution and distribution of cloud-to-ground (CG) lightning and radar composite reflectivity (CR) associated with MCSs are explored.

The QS-MCSs primarily occur in July and August and are mainly initiated in the afternoon. The OM-MCSs mostly occur in June and July with two initiation peaks at noon and late night, respectively. The QS-MCSs are mainly initiated in mountainous areas. In contrast, the OM-MCSs are mainly initiated in plain areas. Compared to the OM-MCSs, the QS-MCSs show notable diurnal variation in intensity and develop more rapidly. The geographical distribution of CG lightning associated with MCSs shows that the highest occurrence tends to appear over the transition zone of the Poyang Lake Plain and the surrounding mountains. The CG lightning associated with MCSs features a relative lower proportion of negative CG lightning occurrences. An overall negative correlation between brightness temperature and the peak current of CG lightning is documented with seasonal variations. The advection of ice particles associated from convective cores into nearby stratiform regions caused by relatively stronger mid-to-upper-level winds, may explain the positive correlations in May and September. A time lag of 0–2 h between the CG lightning occurrence peak and the MCS extent maximum is found. As the MCS develops, the proportion of convective clouds decreases, the proportion of nonprecipitating anvil increases, and the proportion of stratiform consistently maintains 50%–60% of the MCS extent, dominating throughout its life span. The main region for stratiform is primarily in the southern part of the MCS, while convective clouds are mainly in the northern part, possibly due to the influence of the Meiyu front.

 

How to cite: Sun, J. and Fu, Y.: The Intensity, Evolution, and Distribution of Cloud-to-Ground Lightning and Radar Reflectivity throughout the Life Cycle of Mesoscale Convective Systems over Southern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5335, https://doi.org/10.5194/egusphere-egu25-5335, 2025.

EGU25-5755 | ECS | Orals | AS1.1

Informing the Unification of a Single Cloud Fraction Scheme in the Met Office’s Unified Model   

Francesca Cottrell, Paul Barrett, Steven Abel, Michael Whitall, Keith Williams, and Paul Field

The choice of cloud fraction parametrization scheme in weather and climate models significantly influences model performance. Currently in the Met Office’s Unified Model (UM), two different approaches are used to represent sub-grid clouds: a prognostic scheme in the global atmosphere and land (GAL) configuration, and a diagnostic scheme in the regional atmosphere and land (RAL) configuration.  Historically, prognostic schemes have performed better at climate resolutions where memory is important, whilst diagnostic schemes have been sufficient for higher resolution numerical weather prediction (NWP). Due to recent increases in computational power, both climate simulations and NWP are being run at higher resolutions. This blurs the boundary between the two configurations, and it would therefore be beneficial to unify a single large-scale cloud fraction scheme which works seamlessly across all resolutions. 

A framework for testing candidate cloud fraction schemes has been developed, using high resolution (300m grid spacing) simulations. This grid spacing was chosen as previous comparisons of the UM with observational data show a cloud fraction scheme is required, however most deep convection will be resolved at this resolution and so there is no need for a convection scheme.  

We investigate four different cloud fraction schemes: Smith (diagnostic), Bi-Modal (diagnostic), PC2 (prognostic), and a new hybrid cloud scheme combining PC2 for ice and Bi-Modal for liquid. We also look at two cloud microphysics schemes: Wilson & Ballard (single moment), and Cloud AeroSol Interacting Microphysics (CASIM; double moment).  

Simulations of shallow cumulus and stratocumulus cloud regimes have been performed over a south UK domain for several case study dates. Through comparisons of rainfall rates and storm cell sizes against 1 km radar observations, it’s been demonstrated that all model configurations overpredict the number of small cells even at this high resolution, particularly GAL9 which also hugely overpredicts rainfall rates. Further comparisons against 3D radar composites provide information on timing and morphology errors. In addition, comparisons against the observations from the Wessex UK Summertime Convection Experiment (WesCon) provide further constraints for single-site model output for parameters including liquid water path and cloud-base height. Together, these comparisons will help to identify the configuration that best represents observed cloud at high resolutions, thereby informing the development of a unified physics configuration.   

How to cite: Cottrell, F., Barrett, P., Abel, S., Whitall, M., Williams, K., and Field, P.: Informing the Unification of a Single Cloud Fraction Scheme in the Met Office’s Unified Model  , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5755, https://doi.org/10.5194/egusphere-egu25-5755, 2025.

Cloudburst is a new post-processing system at the Met Office, leveraging Amazon Web Services (AWS) to provide a route for easy deployment of post processing pipelines allowing for the generation of replacement data as legacy sources are retired. The focus is primarily on generating diagnostics where consistency across multiple variables is required to provide a coherent weather narrative. Thus far all provided parameters have utilised the Met Office’s global and UK deterministic models but the system is made to be versatile so ensemble forecasts could be used in future.

The diagnostics generated in Cloudburst use code from the open-source IMPROVER (Integrated Model post-PROcessing and VERification) repository, which offers a versatile toolbox of post-processing plugins. By enhancing this toolbox with new plugins and functionalities, we promote the reusability of post-processing components, fostering collaboration between the Blended Probabilistic Forecast team and the Cloudburst team. Any code added to the IMPROVER repository by Cloudburst is made as adaptable as possible so that it could be applied to deterministic forecasts or ensemble members.

In this presentation we will describe the first diagnostic generated within Cloudburst: precipitation type. This diagnostic was required to be consistent with the rain and snow rate so these were also rederived from the precipitation rate. Precipitation type, along with rain and snow rates, have now been operationalised and the data sent downstream for customers.

How to cite: Spelman, M.: Cloudburst: A Platform for Running Post-Processing Workflows at the Met Office, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5870, https://doi.org/10.5194/egusphere-egu25-5870, 2025.

EGU25-6014 | ECS | Orals | AS1.1

Data-driven dynamic motion field generation for rainfall nowcasting 

Ruben Imhoff, Daniel A. Blázquez Martín, Riccardo Taormina, and Marc Schleiss

Rainfall nowcasting algorithms rely primarily on extrapolation, where recent radar rainfall observations are projected forward in time based on a motion field that is determined with past data. While additional (stochastic) processes may be incorporated, as is for example done in the pySTEPS models, extrapolation remains the fundamental mechanism. Although the motion field estimates are robust, they assume a steady state in the motion field for the future. This assumption can face significant challenges in maintaining accuracy over time, especially during convective weather events characterized by rapid changes in precipitation patterns and their movement.

In this study, we focus on three objectives: 1) identifying the current errors and uncertainties in the steady-state motion field derivation using pySTEPS, 2) the construction of a dynamic motion field derivation approach using a new deep-learning model, MotioNNet, and 3) the development of ensemble motion fields for MotioNNet. MotioNNet is a U-Net based deep-learning architecture, which uses the past radar images (five in this study) in combination with the estimated static motion field from pySTEPS to estimate the deviation from the provided static motion field per grid cell with increasing lead time. For the ensemble generation in MotioNNet, we tested probabilistic techniques such as SpatialDropout and Monte Carlo dropout.

We trained and tested our model on C-band weather radar data from the Royal Netherlands Meteorological Institute (KNMI), using 10,000 rainfall events. These events were selected to include cases with both intense precipitation and significant motion errors. Our results show that the static motion field approach results in average motion field errors of 1 – 3 km h-1 at the start of the forecast and increases to 4 – 8 km h-1 (on average, and locally sometimes much higher) at a lead time of 90 minutes. The dynamic motion field estimates of MotioNNet improve the motion prediction accuracy by approximately 13%. The improvement is much higher for structured and stable events (up to 45%), but almost negligible for localized thunderstorm events. The results of the ensemble construction in MotioNNet indicate that MotioNNet is capable of adding perturbations in space where most uncertainty takes place, especially for structured and stable events. This is an advantage compared to the spatially uniform approach of pySTEPS. However, the spread of the ensembles is still underestimated, even more so than with pySTEPS, indicating that the uncertainty in the forecast is not yet well represented.

We conclude that the hybrid MotioNNet approach can substitute and enhance parts of the motion field module in pySTEPS. MotioNNet refines initial motion field estimates, rather than replacing them, which leads to a modular approach that fits well in the overall pySTEPS framework. We expect that the dynamic motion field approach from MotioNNet will aid in further enhancing the predictability of (high-intensity) rainfall events for short lead times, especially for structured events where motion errors currently play a role in the forecast error.

How to cite: Imhoff, R., Blázquez Martín, D. A., Taormina, R., and Schleiss, M.: Data-driven dynamic motion field generation for rainfall nowcasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6014, https://doi.org/10.5194/egusphere-egu25-6014, 2025.

EGU25-6937 | ECS | Posters on site | AS1.1

Lead time-dependent postprocessing of 2-meter temperature forecast using a multivariate generative machine learning model  

Sameer Balaji Uttarwar, Jieyu Chen, Sebastian Lerch, and Bruno Majone

The spatiotemporal dependence structure in postprocessed weather forecast variables is essential for reliable hydrological and socio-economic applications. However, in univariate postprocessing, where statistical or advanced machine learning techniques are applied independently in each margin, the multivariate dependence structure present in the raw ensemble forecasts is lost. To restore the disrupted spatial or temporal dependence structure of univariately postprocessed forecasts, copula-based methods are traditionally applied as an additional step that utilizes dependency information from raw ensemble forecasts or historical observations. However, such a two-step framework faces difficulty incorporating exogenous variables to model the dependence structure. To overcome these limitations, a multivariate non-parametric data-driven distributional regression postprocessing technique based on a generative neural network is employed to draw samples directly from multivariate predictive distribution as output [1]. This study focuses on preserving temporal dependency and investigates the performance of a multivariate generative model against two-step approaches to postprocess a 2-meter temperature forecast with a one-month lead time over the Trentino-South Tyrol region in the northeastern Italian Alps. The forecast dataset is a fifth-generation seasonal weather forecast system (SEAS5) generated by the European Centre for Medium-Range Weather Forecasts (ECMWF), which has a 0.125° x 0.125° horizontal grid resolution with 25 ensemble members over a reforecast period from 1981 to 2016. The reference dataset is the high-resolution (250 m x 250 m) gridded observational data over the region. The results are presented using multivariate proper scoring rules (i.e., energy and variogram scores) to measure the overall discrepancy and dependence structure in the postprocessed forecast. The performance analysis reveals that the multivariate generative postprocessing model outperforms the two-step approach over the entire region.

 

References:

[1] Chen, J., Janke, T., Steinke, F. & Lerch, S. Generative Machine Learning Methods for Multivariate Ensemble Postprocessing. Ann. Appl. Stat. 18, 159–183 (2024).

How to cite: Uttarwar, S. B., Chen, J., Lerch, S., and Majone, B.: Lead time-dependent postprocessing of 2-meter temperature forecast using a multivariate generative machine learning model , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6937, https://doi.org/10.5194/egusphere-egu25-6937, 2025.

EGU25-7540 | Posters on site | AS1.1

A Study on Catenary Icing Prediction Method Integrating Physical Modeling and Transformer-Based Deep Learning 

Xiaowei Huai, Wenjun Kang, Bo Li, Jing Luo, Wen Dai, and Rongtao Liu

This paper proposes a novel method for predicting icing on overhead contact lines by integrating physical modeling with Transformer-based deep learning, addressing the limitations of traditional meteorological models in complex weather conditions and terrains. The method combines physical factors such as meteorological data (e.g., temperature, humidity, wind speed) and topographic features to construct a physical model for initial predictions, while leveraging the Transformer model's robust capability in processing time-series data to capture the nonlinear dynamics of the icing process. Experimental results demonstrate that the proposed method significantly outperforms traditional single meteorological models in prediction accuracy across various weather conditions, particularly excelling in extreme weather and complex terrain scenarios. This approach provides reliable technical support for disaster prevention, mitigation, and early warning systems in the transportation sector, offering substantial practical value for engineering applications.

How to cite: Huai, X., Kang, W., Li, B., Luo, J., Dai, W., and Liu, R.: A Study on Catenary Icing Prediction Method Integrating Physical Modeling and Transformer-Based Deep Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7540, https://doi.org/10.5194/egusphere-egu25-7540, 2025.

EGU25-7697 | Posters on site | AS1.1

Characteristics of the Macro- and Micro-Structures of Different Grades of Fog in Jiangsu, China 

Hongbin Wang, Zhiwei Zhang, and Duanyang Liu

Based on the minute-resolution meteorological elements data observed at 70 automatic weather stations in Jiangsu, the second-resolution sounding data of 3 sounding stations and the fog droplet spectrum data of 21 dense fog events, from January 1, 2013 to December 31, 2023, the spatial and temporal distribution, boundary layer structure and microphysical structure characteristics of the fog at different grades in Jiangsu were analyzed. The results show that in recent years, the number of fog hours in Jiangsu are distributed along the Yangtze River and to the north along the Huaihe River. The average annual fogging time at each station is 318.5h, the strong dense fog and extremely dense fog were mainly concentrated along the Huaihe River and its north, accounting for 16.4% of the total fog hours. The probability of occurrence of fog in Jiangsu is the highest at 05:50, and the probability of occurrence of fog in winter, spring, summer and autumn is the highest at 07:10, 05:50, 05:20 and 05:50, respectively. The temperature structure of fog at different grades between 0 and 1500 m has inversion layer, and with the increase of fog intensity, the inversion intensity increases. And the relative humidity is saturated in the lower layer, but with the increase of fog intensity, the relative humidity of upper layer decreases. With the increase of fog intensity, the number of fog drops of different sizes all increase, and the spectrum of fog drops expands obviously when strong dense fog or extremely dense fog occurs.

How to cite: Wang, H., Zhang, Z., and Liu, D.: Characteristics of the Macro- and Micro-Structures of Different Grades of Fog in Jiangsu, China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7697, https://doi.org/10.5194/egusphere-egu25-7697, 2025.

EGU25-7761 | Orals | AS1.1

Future Satellite Observations of the Dynamics and Microphysics of Convection from the NASA Atmosphere Observing System (AOS) 

Scott Braun, Pavlos Kollias, Jie Gong, Yuli Liu, Nobuhiro Takahashi, Takuji Kubota, Helene Brogniez, Thierry Amiot, John Yorks, and Daniel Cecil

Atmospheric convection plays a fundamental role in the vertical redistribution of atmospheric constituents, in driving atmospheric circulation, and in creating severe weather conditions that put life and property at risk. Cloud and precipitation processes in convection and their related release of latent heat are coupled to the rate of vertical air motion in convective updrafts and downdrafts. Observations of vertical air motion in convection have generally been confined to suborbital observations of limited areas and periods of time, but understanding the global distribution of convection is very much needed.

 

The NASA Atmosphere Observing System (AOS) was formulated based on the NASA 2017 Earth Science Decadal Survey to address key objectives tied to aerosols, clouds, convection, and precipitation. As of March 2024, the AOS constellation consists of four individual projects: 1) AOS-Storm, in partnership with JAXA and CNES, flying in a 55° inclined orbit and focusing on convective precipitation, vertical air motions, and convective ice cloud properties; 2) AOS-Sky, a satellite carrying a suite of passive sensors including a multi-angle polarimeter, passive microwave radiometer, and thin ice cloud far infrared imaging radiometer flying in tandem with a CSA-provided spacecraft (called HAWCsat) carrying aerosol and moisture limb imagers; 3) an Italian Space Agency led mission, in partnership with NASA, carrying a multi-frequency elastic backscatter lidar with Raman channels for measurement of aerosol, cloud, ocean, and land properties; and 4) an expected cloud profiling radar to be competed as part of an announcement of opportunity.

 

This talk will focus on the AOS-Storm project consisting of the JAXA Precipitation Measuring Mission (PMM) and the CNES Convective Core Observations through MicrOwave Derivatives in the trOpics (C2OMODO) mission, with NASA providing a spacecraft bus for one of the CNES radiometers and launch of both satellites.  The PMM mission includes a JAXA-provided spacecraft and Ku-band Doppler radar that will provide radar reflectivity across a 255-km swath (similar to TRMM and GPM) and Doppler velocity measurements at nadir in moderate to strong convective systems. The CNES C2OMODO mission consists of two identical passive microwave radiometers (channels near 89, 183, and 325 GHz) flying in tandem with a temporal spacing expected to be in the 30-120 second range. The time-differenced passive microwave brightness temperatures will characterize the rate of change of ice water path and anvil size as well as the vertical flux of ice mass. We will highlight recent simulations of expected performance for measurements of vertical air motions and ice water path in convective clouds.

How to cite: Braun, S., Kollias, P., Gong, J., Liu, Y., Takahashi, N., Kubota, T., Brogniez, H., Amiot, T., Yorks, J., and Cecil, D.: Future Satellite Observations of the Dynamics and Microphysics of Convection from the NASA Atmosphere Observing System (AOS), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7761, https://doi.org/10.5194/egusphere-egu25-7761, 2025.

EGU abstract 2025

NP5.2 EDI: Advances in statistical post-processing, blending, and verification of deterministic and probabilistic forecasts

The challenge of uncertain observations: Probabilistic verification of decadal predictions with high temporal resolution

Verification plays an important role in the evaluation and the development of climate predictions. With new developments in the field and ever larger availability of computational resources, temporal high resolutions become an option. But we often do not make use of the full temporal distribution and much too often we still rely on temporal averages to reduce the dimensionality of the data to make a verification with common metrics manageable. One of the reasons is the challenge how to verify in an understandable manner probabilistic model predictions with probabilistic, uncertain observations.

Tools for probabilistic verification are available, like the Continuous Rank Probability Score (CRPS), but are often defined for perfect observations. Furthermore, many tools are for the wider community hard to comprehend and are as such often not applied. This poses the question on how to verify predictions on the basis of current imperfect usage of metrics within the field and how to communicate prediction skill in general. 

This contribution will address two main approaches and apply it to the comparison between a decadal prediction and the associated projection (historical simulation), with an assimilation simulation as an observational reference. In the first we will ask how to communicate verification results for a wider community. For this we will look at framing the skill as yearly matchups between the two model results. Basing on the Integrated Quadratic Distance each year determines which model result is closer to the observations and the years how often one result was better than the other leads to our verification result. In a second approach it will be discussed to find modifications of some of the most applied metrics in our field, Anomaly Correlation (ACC) and Root-Mean Square (RMS), towards uncertain observations. While these metrics are imperfect, they allow an easy communication for people already applying them. Differences in their interpretation will be discussed, giving us insights about how uncertain observations change our understanding of a good prediction. We address also significance estimation and it will be highlighted why we need to find easy comprehendible approaches to handle uncertain observations in the future.

How to cite: Düsterhus, A.: The challenge of uncertain observations: Probabilistic verification of decadal predictions with high temporal resolution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8034, https://doi.org/10.5194/egusphere-egu25-8034, 2025.

EGU25-8427 | Orals | AS1.1

A multi-criteria evaluation of the performance of bias correction using Delta Quantile Mapping for simulated precipitation over Germany 

Edgar Espitia, Yanet Díaz Esteban, Moritz Haupt, Muralidhar Adakudlu, Odysseas Vlachopoulos, and Elena Xoplaki

Bias correction techniques are often used as effective and reliable approaches to improve the representation of current and past conditions in climate models. This study aims to evaluate the performance of Quantile Delta Mapping (QDM) as a bias correction method for daily precipitation simulations from climate models: the Icosahedral Nonhydrostatic Model (ICON), the Regional Climate Model COSMO-CLM (CCLM), and the Regional Climate Model (REMO) at a spatial resolution of 3 km over Germany. The dataset consists of historical observations from HYRAS and climate model simulations between 1961 and 1990, split into a calibration period (1961–1980) and an independent validation period (1981–1990). To assess performance, we considered four aspects: 1) sequence of events, 2) distribution of values, 3) spatial structure, and 4) visual inspection of distance metrics, ultimately providing an integrative qualitative ranking across these aspects. Performance metrics included correlation, Nash-Sutcliffe efficiency (NSE), Kling-Gupta efficiency (KGE), and error metrics such as BIAS, mean square error (MSE), and root mean squared error (RMSE). Additional metrics considered were the Kolmogorov-Smirnov (KS) statistic, Perkins Skill Score (Sscore), probability density function (PDF), 80th, 90th, and 95th percentiles, and spatial autocorrelation. As a preliminary assessment of the simulated precipitation from ICON, results show only slight improvements in the time and spatial distribution of precipitation metrics. For example, the KS statistic improved from 0.0314 to 0.0190, while the Sscore improved from 0.0314 to 0.0195 when comparing HYRAS vs. ICON raw and HYRAS vs. ICON bias-corrected using QDM, respectively. Therefore, limited improvement is expected from bias correction when the climate model already performs well, whereas significant improvements can be achieved when the climate models perform only acceptably.

How to cite: Espitia, E., Díaz Esteban, Y., Haupt, M., Adakudlu, M., Vlachopoulos, O., and Xoplaki, E.: A multi-criteria evaluation of the performance of bias correction using Delta Quantile Mapping for simulated precipitation over Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8427, https://doi.org/10.5194/egusphere-egu25-8427, 2025.

EGU25-8449 | Posters on site | AS1.1

The crossing-point quantile: an optimal point-forecast in terms of ROC areas.  

Zied Ben Bouallegue and Maxime Taillardat

A point-forecast is defined as a single-value forecast expressed in the unit of a variable of interest. A deterministic forecast for 2m temperature at Vienna tomorrow is a point-forecast. Point-forecasts are required by some forecast users and for various applications. When an ensemble prediction system is at hand, a point-forecast can take the form of a distribution functional such as the ensemble mean or an ensemble quantile. In this context, we introduce a new type of point-forecast based on the concept of crossing-point forecast (Ben Bouallègue, 2021). We argue that this self-adaptive forecast should be better suited for some users than other point-forecasts. More precisely, we demonstrate that the so-called crossing-point quantile is an optimal forecast in terms of Pierce Skill Score (or equivalently in terms of area under the ROC curve) for any event of interest.  

Ben Bouallègue Z (2021), On the verification of the crossing-point forecast, Tellus A. DOI:10.1080/16000870.2021.1913007 

How to cite: Ben Bouallegue, Z. and Taillardat, M.: The crossing-point quantile: an optimal point-forecast in terms of ROC areas. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8449, https://doi.org/10.5194/egusphere-egu25-8449, 2025.

EGU25-9468 | Posters on site | AS1.1

Improvements to NWP visibility forecasts using statistical post-processing 

Katharine Hurst and Gavin Evans

Accurate visibility forecasting is essential for aviation, road safety, and maritime operations as well as communicating the weather on a daily basis to the public. Despite advancements in Numerical Weather Prediction (NWP) models, it is well understood in the forecasting community that NWP visibility forecasts are inherently poor, often suffering from calibration issues and systematic biases. In post-processing we can enhance skill, however, it is very difficult to add skill when the input data are particularly poor, so this diagnostic remains a known problem. 

This study explores the application of different parametric and non-parametric statistical post-processing techniques to enhance the accuracy and reliability of visibility forecasts. The chosen method will build upon a new visibility scheme at the Met Office, VERA (Visibility Employing Realistic Aerosol), which uses a more physically realistic representation of the condensation nuclei required to form fog and therefore produces a better distribution of visibility for statistical post-processing to work with. 

The calibration methods included in this study include Quantile Regression Random Forests, Reliability Calibration, Bayesian Additive Regression Trees, and finally Distributional Regression Networks using truncated normal and log normal Continuous Ranked Probability Score loss functions, as well as threshold weighted variants of these loss functions. These methods are tailored, where appropriate, to better support the characteristics of visibility data. 

The methodology is tested on an extensive training dataset from the European Centre for Medium-Range Weather Forecasts (ECMWF), which spans 20 years of reforecasts and several European countries capturing a wide range of visibility conditions, including the rarer low visibility events which are most impactful. 

Initial results demonstrate that Quantile Regression Random Forests post-processed forecasts show a marked reduction in Root Mean Square Error compared to raw NWP outputs, and work is in progress to compare this to other methods. These improvements, so far, highlight the great potential of statistical post-processing in refining visibility predictions and supporting decision-making in weather-sensitive sectors. 

How to cite: Hurst, K. and Evans, G.: Improvements to NWP visibility forecasts using statistical post-processing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9468, https://doi.org/10.5194/egusphere-egu25-9468, 2025.

Lightning, hail, severe turbulence and severe icing associated with cumulonimbus clouds (Cb) present a significant safety hazard to air traffic and can impact the comfort and timeliness of a flight. The World Area Forecast System (WAFS) facilitates safe and efficient flight planning by providing global forecasts of key meteorological hazards. The next generation of WAFS will provide probabilistic forecasts of these hazards, including cumulonimbus clouds.

At the Met Office, these forecasts are currently made using three simple threshold tests applied to parameters from MOGREPS-G, a global NWP ensemble. These thresholds are used as a proxy for the occurrence of cumulonimbus clouds in the NWP data.

In this work, a series of deep learning models have been trained to predict the occurrence of cumulonimbus in global satellite observations using a wider set of parameters from the control member of MOGREPS-G. The purpose of the training is for the deep learning model to learn the representation of a cumulonimbus in the NWP data in a supervised manner. The model predictions are then applied to the whole ensemble to produce a probability forecast of cumulonimbus occurrence.

A range of loss functions were used during model training and verification to account for spatial information at a range of scales. Different loss functions were also used to enhance the reward for correct forecasts of the relatively rare cumulonimbus clouds.

Some of the trained models are shown to have greater skill than a baseline using the threshold test method. The model characteristics change depending on the choice of loss function used during training.

Further work is needed to explore how to make predictions at a range of lead times and how to use inputs from the whole ensemble.

How to cite: Creswick, A.: A deep learning approach for probabilistic forecasts of cumulonimbus clouds from NWP data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9783, https://doi.org/10.5194/egusphere-egu25-9783, 2025.

EGU25-9837 | Orals | AS1.1

Probabilistic Postprocessing of Hourly Precipitation Ensemble Forecasts Using UNet 

Marcos Esquivel González, Albano González, Juan Carlos Pérez, Juan Pedro Díaz, and Pierre Simon Tondreau

Title: Probabilistic Postprocessing of Hourly Precipitation Ensemble Forecasts Using UNet 

Authors: Marcos Esquivel-González, Albano González, Juan Carlos Pérez, Juan Pedro Díaz, Pierre Simon Tondreau

Affiliation of authors: Grupo de Observación de la Tierra y la Atmósfera (GOTA), Avenida Astrofísico Francisco Sánchez, s/n, La Laguna, 38200, Canary Islands, Spain

Abstract: Reliable precipitation forecasting is crucial in sectors like public safety, agriculture and water management. Numerical Weather Prediction (NWP) models, which form the backbone of modern forecasting, are prone to errors due to their limitations and the chaotic behavior of equations, requiring postprocessing to improve accuracy and quantify uncertainties. Thus, this study evaluates probabilistic postprocessing models tailored for the Canary Islands, with the aim of enhancing Weather Research and Forecasting (WRF) ensemble forecasting accuracy in hourly precipitation forecast. UNet-based models were explored using two approaches,  one incorporating  the full set of km-scale convection-permitting ensemble forecast simulations (25) and another applying dimensionality reduction via Principal Component Analysis (PCA) and feature selection methods. These models were compared to traditional benchmarks like the Censored Shifted Gamma Distribution (CSGD) with Ensemble Model Output Statistics (EMOS) and the Analog Ensemble method. In the analysis of the results, not only the reliability of the predictions for the set of available meteorological stations was considered, but also the generalization capacity of the UNet models to obtain precipitation predictions for the whole region.

In general, UNet models outperformed traditional approaches. The UNet with PCA excelled in probabilistic and deterministic metrics but struggled in regions without weather station data. Conversely, the UNet with feature selection, while slightly less accurate overall station locations, showed better generalization to unseen locations, maintaining consistent performance across the region and reducing computational demand. Additionally, the Integrated Gradients technique, an interpretability method that quantifies the contribution of each input feature to a model’s predictions by analyzing gradients, was employed to evaluate the impact of input variables on model performance. This analysis revealed that the integration of digital terrain elevation data significantly contributed to the UNet's outputs, underscoring the importance of topographic data in rainfall prediction.

How to cite: Esquivel González, M., González, A., Pérez, J. C., Díaz, J. P., and Tondreau, P. S.: Probabilistic Postprocessing of Hourly Precipitation Ensemble Forecasts Using UNet, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9837, https://doi.org/10.5194/egusphere-egu25-9837, 2025.

EGU25-10090 | Posters on site | AS1.1

Precipitation Downscaling Using Dynamical and Neural Network Approaches. 

Bijan Fallah and Masoud Rostami

High-resolution climate projections are crucial for assessing the future impacts of climate change. Statistical, dynamic, or hybrid climate data downscaling is often employed to create the datasets required for impact modelling. In this study, we utilize the COSMO-CLM (CCLM) version 6.0, a regional climate model, to investigate the advantages of dynamically downscaling a general circulation model (GCM) from CMIP6, with a focus on Central Asia (CA). The CCLM, running at a 0.22° horizontal resolution, is driven by the MPI-ESM1-2-HR GCM (at 1° spatial resolution) for the historical period 1985–2014 and projections for 2019–2100 under three shared socioeconomic pathways (SSPs): SSP1-2.6, SSP3-7.0, and SSP5-8.5 (Fallah et al., 2025). Using the CHIRPS gridded observation dataset for evaluation, we assess the performance of the CCLM driven by ERA-Interim reanalysis over the historical period.

The added value of CCLM, particularly over mountainous areas in CA, is evident, with a reduction in mean absolute error and bias of climatological precipitation by 5 mm/day for summer and 3 mm/day for annual values (Fallah et al., 2024). While no error reduction is achieved for winter, the frequency of extreme precipitation events improves in the CCLM simulations. Future projections indicate an increase in the intensity and frequency of extreme precipitation events in CA by the century’s end, particularly under the SSP3-7.0 and SSP5-8.5 scenarios. The number of days with more than 20 mm of precipitation increases by more than 90, and the annual 99th percentile of total precipitation increases by over 9 mm/day in mountainous areas.

A convolutional neural network (CNN) is also trained to map GCM simulations to their dynamically downscaled CCLM counterparts. The CNN successfully emulates the GCM-CCLM chain across large areas of CA but demonstrates reduced skill when applied to other GCM-CCLM chains. This downscaling approach and CNN architecture provide an alternative to traditional methods and could be a valuable tool for the scientific community involved in downscaling CMIP6 models (Harder et al., 2023).

In future work, we aim to extend this approach by training a neural network model to map the available GCM-RCM model chains for CORDEX-EU and applying the trained model to decadal prediction ICON simulations. This will enable the production of CORDEX-EU-like regional ICON simulations, bridging the gap between global and regional climate information on decadal timescales. By integrating decadal predictions into the framework, we aim to enhance the usability of regionalized climate data for short-term climate planning and decision-making.

References:

  • Fallah, B., Russo, E., Menz, C., Hoffmann, P., Didovets, I., and Hattermann, F. F.: Anthropogenic influence on extreme temperature and precipitation in Central Asia, Sci. Rep., 13, 6854, https://doi.org/10.1038/s41598-023-33921-6, 2023.
  • Fallah, B., Menz, C., Russo, E., Harder, P., Hoffmann, P., Didovets, I., and Hattermann, F. F.: Climate Model Downscaling in Central Asia: A Dynamical and a Neural Network Approach, Geosci. Model Dev. Discuss. [preprint], https://doi.org/10.5194/gmd-2023-227, accepted, 2025.
  • Harder, P., Hernandez-Garcia, A., Ramesh, V., Yang, Q., Sattegeri, P., Szwarcman, D., Watson, C., and Rolnick, D.: Hard-Constrained Deep Learning for Climate Downscaling, J. Mach. Learn. Res., 24, 1–40, 2023.

How to cite: Fallah, B. and Rostami, M.: Precipitation Downscaling Using Dynamical and Neural Network Approaches., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10090, https://doi.org/10.5194/egusphere-egu25-10090, 2025.

EGU25-10119 | ECS | Posters on site | AS1.1

Pavement Temperature Forecasts Based on Model Output Statistics: Experiments for Highways in Jiangsu, China 

Shoupeng Zhu, Yang Lyu, Hongbin Wang, Linyi Zhou, and Chengying Zhu

Forecasts on transportation meteorology, such as pavement temperature, are becoming increasingly important in the face of global warming and frequent disruptions from extreme weather and climate events. In this study, we propose a pavement temperature forecast model based on stepwise regression—model output statistics (SRMOS) at the short-term timescale, using highways in Jiangsu, China, as examples. Experiments demonstrate that the SRMOS model effectively calibrates against the benchmark of the linear regression model based on surface air temperature (LRT). The SRMOS model shows a reduction in mean absolute errors by 0.7–1.6 °C, with larger magnitudes observed for larger biases in the LRT forecasts. Both forecasts exhibit higher accuracy in predicting minimum nighttime temperatures compared to maximum daytime temperatures. Additionally, it overall shows increasing biases from the north to the south, and the SRMOS superiority is greater over the south with larger initial LRT biases. Predictor importance analysis indicates that temperature, moisture, and larger-scale background are basically the key predictors in the SRMOS model for pavement temperature forecasts, of which the air temperature is the most crucial factor in the model’s construction. Although larger-scale circulation backgrounds are generally characterized by relatively low importance, their significance increases with longer lead times. The presented results demonstrate the considerable skill of the SRMOS model in predicting pavement temperatures, highlighting its potential in disaster prevention for extreme transportation meteorology events.

How to cite: Zhu, S., Lyu, Y., Wang, H., Zhou, L., and Zhu, C.: Pavement Temperature Forecasts Based on Model Output Statistics: Experiments for Highways in Jiangsu, China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10119, https://doi.org/10.5194/egusphere-egu25-10119, 2025.

Raw forecasts, be they weather or hydrological, suffer from the inevitable errors stemming from either model structures or initial conditions estimation. With forecasting being a critical component in addressing challenges in flood control, reservoir and hydropower operation, and other fields related to the environment, energy and public safety, improving forecasting skill is increasingly necessary. Post-processing methods can help in this regard and can help improve forecast accuracy and reliability. Non-Homogeneous Gaussian Regression (NGR) and Bayesian Model Averaging (BMA) are the two most commonly used methods when it comes to post-processing probabilistic forecasts, and they have shown to be similarly efficient in many studies. For case studies where there are several distinct forecasts for one single observation, NGR risks losing information on uncertainty by aggregating the forecasts even though it accounts for heteroscedasticity. BMA, on the other hand, evaluates distinct model components and utilizes them accordingly, while assuming all the forecasts are alike in their under/overdispersion. This work introduces a mixed NGR-BMA approach for calibrating air temperature forecasts with lead-times of 1-10 days where the forecasts are first processed with NGR and then corrected once more by BMA according to a priori information on the skill of model components. This way, the upsides of each method is maintained through post-processing. The results generally show that the higher the lead-time, the more the proposed method outperforms either BMA or NGR taken individually. 

How to cite: Oghbaei, B. and Arsenault, R.: Using Non-Homogeneous Gaussian Regression to incorporate heteroscedasticity when post-processing air temperature forecasts by Bayesian Model Averaging, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10245, https://doi.org/10.5194/egusphere-egu25-10245, 2025.

EGU25-10701 | Orals | AS1.1

Leveraging Data-Driven Weather Forecasting for Improving Numerical Weather Prediction Skill Through Large-Scale Spectral Nudging 

Leo Separovic, Syed Husain, Jean-François Caron, Rabah Aider, Mark Buehner, Stéphane Chamberland, Charles Creese, Ervig Lapalme, Ron McTaggart-Cowan, Christopher Subich, Paul Vaillancourt, Jing Yang, and Ayrton Zadra

Operational weather forecasting has traditionally relied on physics-based numerical weather prediction (NWP) models, but the rise of AI-based weather emulators is reshaping this paradigm. However, most data-driven models for medium-range forecasting still face limitations, such as a narrow range of predicted variables and low effective spatiotemporal resolution. This presentation will compare the strengths and weaknesses of these two approaches, using Environment and Climate Change Canada’s Global Environmental Multiscale (GEM) model and Google DeepMind’s GraphCast model. It will demonstrate that GraphCast outperforms GEM in predicting large-scale features, particularly for longer lead times.

Building on these findings, we propose a new hybrid NWP-AI system, in which GEM’s large-scale state variables are spectrally nudged towards GraphCast’s inferences, while GEM continues to generate fine-scale details critical for weather extremes. Results show that this hybrid system improves GEM’s forecast accuracy, reducing RMSE for the 500-hPa geopotential height by 5-10% and extending predictability by 6-12 hours in the extratropics, peaking at day 7 of the forecast. It also yields significant improvements in tropical cyclone trajectory prediction without degrading intensity forecasts. Unlike state-of-the-art AI-based models, the hybrid system ensures meteorologists retain access to all forecast variables, including those critical for high-impact weather. Preparations are currently well underway for the operationalization of this hybrid system at the Canadian Meteorological Centre. 

How to cite: Separovic, L., Husain, S., Caron, J.-F., Aider, R., Buehner, M., Chamberland, S., Creese, C., Lapalme, E., McTaggart-Cowan, R., Subich, C., Vaillancourt, P., Yang, J., and Zadra, A.: Leveraging Data-Driven Weather Forecasting for Improving Numerical Weather Prediction Skill Through Large-Scale Spectral Nudging, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10701, https://doi.org/10.5194/egusphere-egu25-10701, 2025.

EGU25-11378 | Orals | AS1.1

The Role of Water Vapour in Shaping Mediterranean Summer Climate: Findings from MESSA-DIN 2021 measurement campaing in southern Italy 

Fabio Madonna, Ilaria Gandolfi, Marco Rosoldi, Faezeh Karimian Saracks, Yassmina Hesham Essa, and Giada Salicone

Water vapour fluxes, originating mainly from the Atlantic, North Africa, and the Mediterranean region, play a critical role in shaping the climate dynamics of the Mediterranean Basin, especially during the summer months. These fluxes significantly influence relative humidity levels in the troposphere, affecting both local and regional weather patterns, such as intense rainfall events and prolonged droughts, while also contributing to the amplification of heatwaves through enhanced surface radiation trapping. This study uses observational data collected during the Mediterranean Experiment for Sea Salt and Dust Ice Nuclei (MESSA-DIN) from July to September 2021 in Soverato, southern Italy, to characterise the synoptic conditions of the severe summer of 2021.

A combination of ground-based remote sensing instruments revealed intense and persistent water vapour transport in the mid-troposphere. ERA5 data were used to identify the moisture dynamics over the Mediterranean Basin. The comparison between ERA5 reanalysis data and ground-based measurements further highlighted discrepancies in the representation of water vapour, particularly a dry bias in relative humidity in the range between 500 hPa and 300 hPa. While ERA5 provided a coherent and detailed representation of synoptic patterns and showed general agreement in the time evolution of the atmospheric vertical structure with observations, it exhibited a dry bias in relative humidity (RH) values compared to a ground-based microwave profiler (MWP). However, the magnitude of the bias also depends on the bias affecting the MWP retrieval, typically within 10-15% RH in the mid-troposphere. ERA5 also overestimates the presence of both cold and warm clouds, while ground instruments detected much less frequent cloud cover. This emphasizes the need for improving reanalysis performance in complex coastal and orographic settings. The bias in ERA5 was further assessed using GRUAN data from the Potenza station and regular upper-air data from Mediterranean stations.

The study underscores the importance of ground-based measurements, such as those from microwave radiometers, in improving weather forecasts for extreme events. Despite their lower vertical resolution, these instruments—both on their own and when combined with higher-resolution measurement techniques such as Raman lidars and upper-air soundings—provide continuous, real-time measurements of atmospheric water vapour. These measurements are essential for enhancing our understanding of water vapour fluxes and their impact on cloud formation, as well as for improving the accuracy of high-resolution forecasting models, especially in the representation of extreme weather events in the Mediterranean and Central Europe.

How to cite: Madonna, F., Gandolfi, I., Rosoldi, M., Karimian Saracks, F., Hesham Essa, Y., and Salicone, G.: The Role of Water Vapour in Shaping Mediterranean Summer Climate: Findings from MESSA-DIN 2021 measurement campaing in southern Italy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11378, https://doi.org/10.5194/egusphere-egu25-11378, 2025.

EGU25-12077 | ECS | Orals | AS1.1 | Highlight

The AIFS: ECMWF’s data-driven weather forecasting system 

Sara Hahner and the AIFS-Team

Machine learning-based models are rapidly transforming medium-range weather forecasting. The European Centre for Medium-Range Weather Forecasts (ECMWF) has developed the Artificial Intelligence Forecasting System (AIFS), a state-of-the-art data-driven model combining a graph neural network encoder-decoder with a sliding window transformer processor. Trained on ECMWF's ERA5 re-analysis and operational numerical weather prediction analyses, AIFS demonstrates exceptional deterministic forecast skill across upper-air variables, surface weather parameters, and tropical cyclone tracks.

Building on this foundation, ECMWF has introduced AIFS-CRPS, a probabilistic extension of AIFS designed for ensemble forecasting. AIFS-CRPS is obtained by training a stochastic model with the Continuous Ranked Probability Score (CRPS) as its loss function. It addresses uncertainties and generates highly skilful probabilistic forecasts. For medium-range timescales, AIFS-CRPS matches or outperforms ECMWF’s physics-based Integrated Forecasting System ensemble across key variables and lead times.

This presentation will highlight recent advancements in deterministic and probabilistic forecasting with AIFS, showcasing its operational readiness and its potential to redefine medium-range forecasting at ECMWF.

How to cite: Hahner, S. and the AIFS-Team: The AIFS: ECMWF’s data-driven weather forecasting system, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12077, https://doi.org/10.5194/egusphere-egu25-12077, 2025.

EGU25-13191 | ECS | Orals | AS1.1

Using VIL density for identification of storm nuclei, tracking and nowcasting in the Barcelona Metropolitan Area 

Laura Esbri, Tomeu Rigo, Montserrat Llasat-Botija, and María Carmen Llasat

Urban resilience to extreme weather events is increasingly threatened by the intensification of short-duration rainfall, often leading to urban flooding. This study focuses on improving the prediction of heavy rainfall in the Metropolitan Area of Barcelona, located on the Catalan Mediterranean coast in the northeast of the Iberian Peninsula, using high-resolution radar products and rain gauge data. Despite the decrease in average of annual rainfall in the AMB over recent decades, the intensity rates of some storm events are among the highest of the existing series, with occasional convective events causing urban flooding and severe disruptions for the urban region. The latest climate change reports (IPCC 2022) point towards an increase in frequency and intensity of heavy rainfall events in the region.

An extensive dataset of rainfall days spanning from 2014 to 2022 is analysed, including volumetric radar products (VIL, Echo Top), surface rainfall measurements, and incident reports. A bottom-up approach is used to identify 45 intense convective days with significant impacts in the study region. A radar-based nowcasting approach is introduced, utilizing a two-dimensional radar product with three-dimensional atmospheric information to enhance early warnings in the urban region, with high spatial resolution. This approach focuses on the convective parts of storms through Vertical Integrated Liquid (VIL) density-based tracking and nowcasting with six-minute temporal updates to characterize storm centroids and their evolution. The density of VIL (DVIL), derived from radar composites, provides vertical storm structure information in a two-dimensional format, enabling faster data processing without losing volumetric capabilities.

The findings reveal spatial coherence between maximum DVIL intensities and maximum rainfall locations, with all events exceeding the 2.5 g/m³ DVIL threshold coinciding with high-intensity rainfall. Centroid trajectories show seasonal patterns, with some summer events originating from scattered sources and moving more slowly, while some autumn ones align along the coast and propagating inland. The time lag between initial DVIL detection and peak precipitation for the analysed days ranges from 30 minutes to over two hours, offering critical lead times for early warnings.

This study demonstrates the strengths and limitations of DVIL as a predictor of heavy rainfall in urban areas. The RaNDeVIL module shows promise for operational nowcasting, with necessary improvements to address complex interactions of the storm dynamics and more complex modelling to nowcast longer timescales. These advancements aim to enhance resilience to intense precipitation in the Metropolitan Area of Barcelona under changing climatic conditions.

 

This project has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement 101037193.

How to cite: Esbri, L., Rigo, T., Llasat-Botija, M., and Llasat, M. C.: Using VIL density for identification of storm nuclei, tracking and nowcasting in the Barcelona Metropolitan Area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13191, https://doi.org/10.5194/egusphere-egu25-13191, 2025.

EGU25-13477 | Posters on site | AS1.1

Impact of climate change on ERA5 cloud cover and convective parameters in Central Europe (1983-2022) 

Virág Soós and Breuer Hajnalka

In discussions about climate change, the focus is usually on rising temperatures. However, it is important to understand the significant impact of climate change on the entire weather system. The cloud feedback mechanism is one of the most complex factors in the climate system. This is because clouds can have a heating and cooling effect at the same time, and this balance has a significant influence on the global radiation balance. To understand how all the different factors work together to create a complex system, we need to look closely at how these factors have changed over time.

The aim of this research is to examine changes in cloud cover and convective parameters, as well as the background, causes and effects of these changes in Central Europe between 1983 and 2022. The research uses data from the ERA5 reanalysis database. Aside from the analysis of environmental conditions, an objective cyclone identifying method is used to determine regions under low- or high-pressure weather system influence.  

The statistical analysis shows that in general, the decrease in ERA5 low-level cloud cover is associated with an increase in cloud base. Medium- and high-level cloud cover, however, is influenced by changes in large-scale circulation systems.

Low-level cloud cover decrease in the northern regions of the study area is likely due to increasing temperatures and decreasing boundary layer humidity. Though temperatures in the Mediterranean region also have risen, the increase in the frequency of negative NAO situations, and an increase in Mediterranean cyclone and low-pressure system activity - the latter of which is likely induced by the higher evaporation of the Mediterranean Sea - resulted in the increase in cloud cover over the central Mediterranean region. We have also observed an increase in the CAPE (convective area pressure energy) in the Mediterranean during the summer months, which leads to an increase in the frequency of heavy thunderstorms and extreme precipitation events in this area, contributing to the intensification of weather extremes in the region. Changes over the study area are not linear but show a region dependent 10-20 years periodical pattern which is also investigated.

How to cite: Soós, V. and Hajnalka, B.: Impact of climate change on ERA5 cloud cover and convective parameters in Central Europe (1983-2022), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13477, https://doi.org/10.5194/egusphere-egu25-13477, 2025.

Based on hourly precipitation data, the warm-sector rainfall events in Beijing-Tianjin-Hebei region are selected and classified using objective methods. There are 33 warm-sector rainfall events in this region from 2010 to 2023. They mainly occur during June and August with the most in July. The average lifetime of these warm-sector rainfall events is 5.44 h. The warm-sector rainfall events are mainly concentrated in the center of the Beijing-Tianjin-Hebei region, and the frequency of occurrence in the east is higher than that in the west. The frequency of occurrence in Beijing is much higher than that in other regions, and it is mainly concentrated in the terrain bell mouth of northeast Beijing. According to the circulation situation that generates warm-sector rainfall, three types of precipitation are obtained: low-vortex type, shear-line type and southerly-wind type. The occurrence months, starting times and locations of warm-sector rainfall events in different types are slightly different. Based on the analysis of the synthetic circulation situation, the dynamic, water vapor and low-level vertical motion conditions of the low-vortex type is most favorable for warm-sector rainfall. The vertical upward movement of shear line warm-sector rainfall events is strong in Beijing; The dynamic condition of southerly-wind type is the weakest, but the water vapor condition is more favorable and the occurrence is related to the topographic distribution of  Beijing-Tianjin-Hebei.

How to cite: Liu, R.: Selection and Classification of Warm-Sector Rainfall Events in Beijing-Tianjin-Hebei, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14147, https://doi.org/10.5194/egusphere-egu25-14147, 2025.

Precipitation nowcasting, which entails high-resolution forecasting of precipitation events within 1–2 hours, is significant to daily life and professional activities. Nevertheless, accurate short-term precipitation forecasting remains a considerable challenge at present. Traditional numerical weather prediction, which relies on intricate physical equations to simulate the Earth's atmospheric state, necessitates substantial computational resources and frequently yields lower accuracy for small-scale forecasts, thereby failing to meet the demands of precipitation prediction in complex regions. Most deep learning methodologies concentrate exclusively on the spatiotemporal prediction of a singular precipitation variable, thereby neglecting the dynamic spatiotemporal relationships between precipitation and other meteorological data within the meteorological system. Moreover, due to the rapid pace of climate change, long-term time series data is often inadequate for accurately addressing precipitation forecasting for extreme weather events, since past meteorological time series data may not accurately reflect the current atmospheric conditions. There is an urgent need to rely on short-term time series for prediction tasks. However, most current methods that rely on short-term time series for prediction perform poorly in forecasting moderate to heavy precipitation events. Inspired by spatiotemporal information transformation schemes, we introduce a spatiotemporal information(STI) transformation equation from chaotic dynamics into the field of computer vision and develop a neural network model framework based on spatiotemporal information transformation. This framework maps high-dimensional spatial information to the temporal information of future precipitation information, thereby facilitating the integration of dynamic spatiotemporal relationships between various meteorological data and precipitation, and enabling the mutual transformation of spatiotemporal information for enhanced forecasting accuracy. Furthermore, we propose an adaptive gradient loss function designed to improve the model's sensitivity to learning moderate-intensity precipitation. This research utilizes the US SEVIR dataset for training and testing, which encompasses data such as satellite visible light, infrared temperature, humidity, and cloud precipitation while employing multiple meteorological data for precipitation forecasting over the subsequent hour. We selected the Structural Similarity Index, Peak Signal-to-Noise Ratio, False Alarm Rate, Critical Success Index, and Heidke Skill Score as both quantitative and qualitative evaluation metrics. Experimental results demonstrate that the STI framework reduces the model's error in moderate to heavy precipitation events, making the model more sensitive to severe rainfall events. Furthermore, when the STI framework is integrated into other deep learning models and retrained, it further enhances their precipitation prediction accuracy. This finding indicates that the STI framework effectively captures the dynamic spatiotemporal relationships between various meteorological and precipitation data.

How to cite: Hu, J., Liu, D., Huang, X., and Wu, X.:  Spatiotemporal Information Transformation for Precipitation Nowcasting Using Multi-Meteorological Factors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14517, https://doi.org/10.5194/egusphere-egu25-14517, 2025.

Moist convection in the Maritime Continent (MC) is typically driven by synoptic disturbances: Northerly Cold Surge (NCS), Borneo Vortex, and Madden-Julian Oscillation (MJO). One or more of these tropical disturbances can control the convective behaviour in the MC, resulting in changes in the diurnally forced convection, cloud populations and diurnal precipitation. This investigation analyses a record extreme rainfall event on Java Island around New Year's Eve 2020, the highest amount of rainfall recorded in the capital city of Indonesia, Jakarta. We use reanalysis data from ECMWF Reanalysis v5 (ERA5) to identify and analyse the southward propagation of the NCS. Satellite measurements from the Himawari-8 Advanced Himawari Imager and satellite-derived cloud physical properties reveal the cloud signatures of the NCS. High-resolution Weather Research & Forecasting Model (WRF) simulations were performed to understand the mesoscale dynamic process of the NCS's interaction with the enhanced precipitation at the diurnal scale.

Our results suggest that this extreme event resulted from the interaction of an NCS event and the diurnally forced convection. A persistent northwesterly wind near the surface over the Java Sea induced an intense low-level wind convergence from the meridional moisture transport associated with the NCS and the equatorial trough over Java. This promoted the necessary unstable conditions for organised convection during the afternoon-evening. The cloud populations and diurnal cycle of heavy rainfall in western Java were affected by the frontal region of the NCS with the offshore propagating land breeze from Java and Sumatra, as well as the intense convergence of moisture air in the internal seas of the MC. Our analysis also suggests that the presence of this strong cross-equatorial flow in the MC induced moisture transport from the southern part of Sumatra to the western region of Java. The findings outlined here could be utilised to enhance our understanding of severe weather in the MC.

How to cite: Lopez-Bravo, C.: A high-resolution modelling and observational analysis of an extreme rainfall event driven by the Northerly Cold Surge and intraseasonal tropical variability in Jakarta: January 2020, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14567, https://doi.org/10.5194/egusphere-egu25-14567, 2025.

EGU25-15060 | Orals | AS1.1

Fair Box ordinate transform for multivariate Gaussian forecasts 

Sándor Baran and Martin Leutbecher

In evaluating multivariate probabilistic forecasts predicting vector quantities such as a weather variable at multiple locations or a wind vector, an important step is the assessment of their calibration and reliability. Here, we focus on the Gaussian Box ordinate transform (BOT), which is appropriate if the forecasts and observations are multivariate normal. The BOT is based on the Mahalanobis distance of the observation vector and the estimated Gaussian mean and asymptotically standard uniform if the forecasts and the observation are drawn from the same multivariate Gaussian law. However, for small ensemble sizes combined with high dimensionality, deviation from uniformity is substantial even for reliable forecasts, resulting in hump-shaped or triangular BOT histograms. To circumvent this problem, we derive an ensemble size and dimension-dependent fair version of the Gaussian BOT, where the uniformity holds for any combination of these parameters. With the help of a simulation study, first, we assess the behaviour of the fair BOT for various dimensions, ensemble sizes, and types of calibration misspecification. Then, using ensemble forecasts of vectors consisting of multiple combinations of upper-air weather variables, we demonstrate the usefulness of the fair BOT when multivariate normality is only an approximation.

*Research was supported by the Hungarian National Research, Development and Innovation Office under Grant No. K142849.

How to cite: Baran, S. and Leutbecher, M.: Fair Box ordinate transform for multivariate Gaussian forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15060, https://doi.org/10.5194/egusphere-egu25-15060, 2025.

EGU25-15639 | Posters on site | AS1.1

Ensemble Convective Rainfall Nowcasting by integrating Numerical Weather Prediction models and Neural Networks: the ICREN project 

Giovanna Venuti, Xiangyang Song, Stefano Federico, Giorgio Guariso, Matteo Sangiorgio, Claudia Pasquero, Seyed Hossein Hassantabar Bozroudi, Ali Badr Eldin Ali Mohamed, Ruken Dilara Zaf, Lorenzo Luini, Roberto Nebuloni, and Eugenio Realini

Convective events pose a significant threat to society due to the associated heavy rainfall, large hail, strong winds, and lightning. Location and timing determination of convective precipitation is still a challenge for modern meteorology. Despite the good skills of current weather forecasting tools in the prediction of the large-scale environment facilitating the onset of convective phenomena, the multitude of spatial scales involved in such events makes their characterization, observation, and forecast a difficult task. The problem is further complicated by their rapid temporal development, which lasts from minutes to a few hours depending on the specific case.

Recent research indicates that the predictability of these events can be strongly improved accounting for local meteorological observations. 

The goal of the ICREN (Intense Convective Rainfall Events Nowcasting) project is to enhance the nowcasting of convective events by:

  • exploiting the information made available by local standard and non-conventional observations of meteorological variables
  • integrating physically based Numerical Weather Prediction (NWP) models with data-driven black box Neural Networks (NNs). 

The NWP model is used to support the NN by means of pseudo-observations (forecasted variables); while the fast computational speed of the NN enables advancing predictions in time and generating ensemble forecasts of convective phenomena.

The project is carried out in the Seveso River basin (almost 300 km2) in Northern Italy. In this region, convective events trigger floods and flash floods heavily impacting the large urban area of Milan.

Within the project, the Weather Research and Forecasting (WRF) NWP model is employed. By using three nested grids, the model achieves a 2 kkm x 2 km spatial resolution over the test area. To optimize the prediction of meteorological variables required by the NN, the model assimilates lightning observations and GNSS-derived Zenith Tropospheric Delays (ZTDs), both of which enhance the representation of local atmospheric humidity.

Several NN models have been trained on standard meteorological data, GNSS ZTDs, and radar-derived parameters—including the position, velocity, and attenuation of convective cells—to identify the architecture best suited for predicting 10-minute accumulated rainfall from 10 minutes up to 1 hour following the detection of a convective event in the test area.

The best-performing models are used to generate ensemble predictions of rainfall events by suitably perturbing the input variables.

Results from the WRF model, the NN predictions and the ensemble forecasts will be presented along with initial integration outcomes for selected convective events occurring in the test area in 2019.

 

This work is supported by the ICREN-PRIN project (MUR- CUP: D53D23004770006). 



How to cite: Venuti, G., Song, X., Federico, S., Guariso, G., Sangiorgio, M., Pasquero, C., Hassantabar Bozroudi, S. H., Mohamed, A. B. E. A., Zaf, R. D., Luini, L., Nebuloni, R., and Realini, E.: Ensemble Convective Rainfall Nowcasting by integrating Numerical Weather Prediction models and Neural Networks: the ICREN project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15639, https://doi.org/10.5194/egusphere-egu25-15639, 2025.

Mesoscale vortices in the boundary layer are characterized by short lifespans, small spatial scales, and difficulty in prediction, leading to their frequent oversight in operational forecasting. This oversight often results in lower accuracy for precipitation forecasting associated with these vortices. From April 2 to April 3 2023, a squall line event triggered by vortices extending from the lower troposphere to the boundary layer occurred across eastern Hubei to western Anhui. This event developed ahead of a shallow mid-tropospheric trough, while the lower levels were influenced by southwest flow. High-resolution numerical simulations successfully reproduced the evolution of the vortex and the organizational development of the squall line. Dynamic diagnosis revealed that the nocturnal boundary layer vortex (925 hPa) was initiated by the intensification of the nocturnal jet and the blocking effect of terrain. Subsequently, through vertical advection of horizontal vorticity from boundary layer to lower level, the vortex at the lower troposphere (850 hPa) developed and intensified. Later, under the combined influence of horizontal divergence and horizontal advection, the vortex rapidly strengthened, creating favorable convergence conditions for the squall line's development due to the northerly flow west of the vortex and the southwest flow south of it.

How to cite: Zhang, Y., Xi, X., and Sun, J.: The formation and evolution mechanism of the boundary layer vortex east of thesecond-step terrain along the middle reaches of the Yangtze River, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15786, https://doi.org/10.5194/egusphere-egu25-15786, 2025.

EGU25-15861 | ECS | Orals | AS1.1

Improving seasonal forecasts for early warning systems in Germany 

Yanet Díaz Esteban, Qing Lin, Fatemeh Heidari, Edgar Fabián Espitia Sarmiento, and Elena Xoplaki

Climate forecasts at seasonal timescales are critical for various sectors, and play a key role in decision-making processes, helping to mitigate risks associated with climate variability and extreme events. However, model outputs are typically insufficient for many practical applications due to coarse resolution and systematic biases, requiring the employment of post-processing techniques to enhance their usability and target stakeholders’ interest such as early warning systems. Post-processing techniques such as downscaling and bias correction can translate model outputs into higher-resolution, bias-corrected forecasts that are more relevant and best appropriate for local applications. We present a physics-informed CNN-based framework for downscaling and bias correction of ECMWF SEAS5.1 seasonal temperature and precipitation forecasts over Europe from 1° to ~1.2km, which represents a downscaling factor of ~60. The approach considers several climate drivers of atmospheric surface variables from SEAS5.1 as input and takes European Meteorological Observations at 1.2 km as ground truth data. We use an analog-based approach to account for the mismatch between long-range model outputs and observations due to model drifting, which is a problem for supervised neural networks algorithms running on climate datasets. Finally, we present a detailed evaluation of the performance for the period 2017-2022, by comparing our results to the raw output. In most cases, the post-processed forecasts outperform the raw predictions in terms of bias reduction, spatial representation and capturing the extremes. This work has potential implications for reducing uncertainties, improving spatial representation, and addressing systematic biases present in raw ECMWF seasonal products.

How to cite: Díaz Esteban, Y., Lin, Q., Heidari, F., Espitia Sarmiento, E. F., and Xoplaki, E.: Improving seasonal forecasts for early warning systems in Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15861, https://doi.org/10.5194/egusphere-egu25-15861, 2025.

EGU25-16130 | Posters on site | AS1.1

Enhancing Radar-Based Precipitation Nowcasting Model with AI-Predicted Precipitation Intensity Change Rates 

Kwang-Ho Kim, Kyeongyeon Ko, and Kyung-Yeub Nam

The importance of precipitation nowcasting is gradually expanding due to the increasing frequency and intensity of localized rainfall caused by climate change. The growth and decay processes of precipitation are critical factors influencing the accuracy of precipitation nowcasting, necessitating advanced modeling approaches. This study proposes a novel methodology that integrates artificial intelligence (AI) with high-resolution radar data to predict the growth and decay processes of precipitation, incorporating these predictions into a radar-based nowcasting model. In this study, AI was applied to predict radar-based precipitation intensity change rates up to two hours ahead, and these predictions were integrated into a precipitation nowcasting model. The AI effectively learned the spatiotemporal patterns of nonlinear precipitation evolution using the RainNet architecture. The AI was trained on three years (2021 – 2023) of radar-derived precipitation intensity change rates, with one year (2020) used for validation to evaluate its performance. The nowcasting model was developed using cross-correlation techniques to calculate motion vectors of the precipitation system at different spatial scales, and a semi-Lagrangian backward extrapolation method was employed for precipitation prediction. Integrating AI-predicted precipitation intensity change rates into the nowcasting model resulted in significant improvements in prediction performance. The results showed a 10% improvement in precipitation prediction accuracy compared to the baseline nowcasting model that did not incorporate AI-based precipitation intensity change rate predictions. The model effectively captured rapid changes in precipitation intensity, demonstrating the utility of AI-based predictions for short-term nowcasting. This study highlights the potential of combining traditional nowcasting models with AI techniques, presenting a promising approach for enhancing precipitation prediction accuracy.

This research was supported by the "Development of radar based severe weather nowcasting technology (KMA2021-03122)" of "Development of integrated application technology for Korea weather radar" project funded by the Weather Radar Center, Korea Meteorological Administration.

How to cite: Kim, K.-H., Ko, K., and Nam, K.-Y.: Enhancing Radar-Based Precipitation Nowcasting Model with AI-Predicted Precipitation Intensity Change Rates, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16130, https://doi.org/10.5194/egusphere-egu25-16130, 2025.

EGU25-16651 | Orals | AS1.1

RUSH: A Novel Fully AI-driven Framework for Seamless Integration of Observations and Global AI Forecasts in Short-term Weather Prediction 

Gabriele Franch, Elena Tomasi, Simon de Kock, Matteo Angelinelli, and Marco Cristoforetti

Short-term weather forecasting, especially for extreme events, remains challenging due to the need to effectively combine recent observations with numerical weather predictions. To tackle this challenge, we present RUSH (Rapid Update Short-term High-resolution forecast), an innovative framework designed to provide high-resolution (1 km) precipitation forecasts on a national scale with lead times up to 24 hours. RUSH follows the recent attempts to create fully AI-driven kilometer-scale forecasting systems that completely replace traditional numerical modeling with a combination of machine learning and observational data. Our system employs a Latent Diffusion Model architecture to seamlessly blend information from multiple data sources, including radar composites, satellite observations (SEVIRI bands), and ECMWF's AI-based global forecasting system (AIFS). 

The model is conceptually designed to transition from observation-driven predictions in the first few hours to a sophisticated spatial and temporal downscaling of AIFS forecasts at longer lead times. This approach aims to leverage the strengths of both data sources: the high spatial and temporal resolution of observational data for immediate forecasts, and the physically consistent evolution provided by AIFS for longer horizons. By utilizing an end-to-end AI architecture from global to local scale, RUSH not only addresses the computational constraints typically associated with traditional numerical weather predictions but also explores the potential for a new generation of fully data-driven weather forecasting systems. 

Our framework processes multi-source input data at different spatial and temporal scales, including radar-derived 30-minute precipitation accumulations, key SEVIRI channels, and selected AIFS forecast fields at 25km resolution. The model's sequence-to-sequence architecture allows for flexible spatial domain handling and probabilistic precipitation forecasting through multiple realizations. 

We will present preliminary results from two experimental implementations over different European domains (Italy and Belgium), demonstrating the model's capability to generate rapid-update forecasts and discussing its potential for operational implementation in weather services. The evaluation will focus on precipitation prediction skills across different intensity thresholds and temporal scales, with particular attention to extreme event forecasting. A preliminary comparison with operational limited area models (COSMO-2I and ALARO-AROME) over selected case studies will assess the competitiveness of this fully AI-driven approach against high-resolution numerical weather prediction systems. 

How to cite: Franch, G., Tomasi, E., de Kock, S., Angelinelli, M., and Cristoforetti, M.: RUSH: A Novel Fully AI-driven Framework for Seamless Integration of Observations and Global AI Forecasts in Short-term Weather Prediction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16651, https://doi.org/10.5194/egusphere-egu25-16651, 2025.

EGU25-16934 | ECS | Posters on site | AS1.1

Clustering-based spatial interpolation of parametric post-processing models 

Mária Nagy-Lakatos and Sándor Baran

Parametric approaches to post-processing methods are widely used today, as they provide full predictive distributions for the weather variable of interest. These methods rely on training data consisting of historical forecast-observation pairs to estimate their parameters. Consequently, post- processed forecasts are generally restricted to locations with accessible training data. To overcome this limitation, we introduce a general clustering-based interpolation technique that extends calibrated predictive distributions from observation stations to any location within the ensemble domain where ensemble forecasts are available. Using the ensemble model output statistics (EMOS) post-processing technique, we conduct a case study based on 10-m wind speed ensemble forecasts from the European Centre for Medium-Range Weather Forecasts.  The results illustrate the effectiveness of the proposed method, demonstrating its advantages over both regionally estimated and interpolated EMOS models as well as raw ensemble forecasts.

Reference:  Baran, S. and Lakatos, M. (2024) Clustering-based spatial interpolation of parametric post-processing models. Wea. Forecasting  9, 1591-1604.

Research was supported by the Hungarian National Research, Development and Innovation Office under Grant No. K142849.

How to cite: Nagy-Lakatos, M. and Baran, S.: Clustering-based spatial interpolation of parametric post-processing models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16934, https://doi.org/10.5194/egusphere-egu25-16934, 2025.

EGU25-17194 | ECS | Orals | AS1.1

Exploring spatiotemporal vector autoregressive models for radar nowcasting 

Viv Atureta, Stefan Siegert, and Peter Challenor

Radar nowcasting methodologies have evolved from traditional optical flow and extrapolation techniques to advanced deep learning algorithms. However, accurately modeling growth and decay processes remains a significant challenge. This study explores spatio-temporal statistical models inspired by physics-based stochastic partial differential equations (SPDEs). Specifically, the solution to the advection-diffusion PDE is framed as a vector autoregressive process with coloured noise, characterized by non-uniform spectral properties.

We investigate the stochastic component using Gaussian Processes (GPs) and Gauss Markov Random Fields (GMRFs), evaluating covariance structures such as exponential, squared exponential, and dynamically weighted covariance and precision matrices. Nowcasts employing state-dependent GPs and GMRFs are assessed over lead times ranging from 15 minutes to 2 hours. The approach is tested on simulated data and UK precipitation events from the Met Office Nimrod system, focusing on a 200 km × 200 km region. Training data spans January 2014 to December 2020, with observational dimensions on the order of 10^4. To enable computationally efficient Bayesian inference, we utilize sparse matrix methods and Laplace approximations.

How to cite: Atureta, V., Siegert, S., and Challenor, P.: Exploring spatiotemporal vector autoregressive models for radar nowcasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17194, https://doi.org/10.5194/egusphere-egu25-17194, 2025.

EGU25-17279 | ECS | Posters on site | AS1.1

Nowcasting precipitation events from mesoscale convective systems for Dakar, Senegal  

Mai-Britt Berghöfer, Diana L. Monroy, and Jan O. Härter

Senegal, located in the West Sahel region, frequently experiences flooding driven by mesoscale convective systems (MCSs), which contribute 90% of the region’s rainfall. Current early warning systems for hydrological extremes struggle with timely and accurate predictions, necessitating advancements in precipitation nowcasting. Nowcasting describes short-term weather forecasts with a lead time of typically less than two hours. In this region traditional numerical weather models have limited accuracy in predicting short-term events, and nowcasting models therefore outperform numerical weather prediction in this time frame. Precipitation nowcasts can be helpful in supporting and informing decision makers on time to adapt to the risk and protect society from hydrological extremes.

A major challenge in developing warning systems for this region is the lack of radar data coverage, which is typically used in nowcasting models, compounded by a sparse ground-based observational network. Increasing the data availability and understanding the properties of MCSs could enhance the predictability of regional weather conditions, which is a primary objective of the High-resolution weather observations East of Dakar (DakE)-project. During the project, 14 automated weather stations have already been installed east of Dakar.

The objective of this study, which is part of the DakE-project, is to integrate the in-situ station data with satellite data to develop a precipitation nowcasting model that is optimally adapted to local conditions considering different spatial and temporal scales. An optical flow routine, based on statistical extrapolation of the current state of the atmosphere, is used for this purpose. To incorporate a stochastic term, which represents the unpredictable component, the STEPS (short-term ensemble prediction system) approach is applied. The skill of the forecast depends, among other things, on the geographical location, the spatial and temporal scales and the meteorological conditions, since developments that do not fulfil the steady-state assumption, such as the initiation, growth and termination of convective systems, are not resolved. The next step is to investigate whether these shortcomings can be compensated by implementing machine learning approaches.

 

References:

 

Anderson, Seonaid R., et al. "Nowcasting convective activity for the Sahel: A simple probabilistic approach using real‐time and historical satellite data on cloud‐top temperature." Quarterly Journal of the Royal Meteorological Society150.759 (2024): 597-617.

Mathon, V., Laurent, H., & Lebel, T. (2002). Mesoscale convective system rainfall in the Sahel. Journal of Applied Meteorology and Climatology41(11), 1081-1092.

Pulkkinen, S., Nerini, D., Pérez Hortal, A. A., Velasco-Forero, C., Seed, A., Germann, U., & Foresti, L. (2019). Pysteps: An open-source Python library for probabilistic precipitation nowcasting (v1. 0). Geoscientific Model Development12(10), 4185-4219.

Taylor, Christopher M., et al. "Nowcasting tracks of severe convective storms in West Africa from observations of land surface state." Environmental Research Letters 17.3 (2022): 034016.

 

 

Keywords: Nowcasting, Senegal, Mesoscale Convective System, Precipitation

How to cite: Berghöfer, M.-B., Monroy, D. L., and Härter, J. O.: Nowcasting precipitation events from mesoscale convective systems for Dakar, Senegal , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17279, https://doi.org/10.5194/egusphere-egu25-17279, 2025.

EGU25-17282 | ECS | Orals | AS1.1

Hybrid Post-Processing for Solar Power: Bridging Nowcasting to Short-Range   

Petrina Papazek, Pascal Gfäller, and Irene Schicker

Accurate forecasting of solar power generation is crucial for grid operators, as location-dependent photovoltaic (PV) installations exhibit diverse production patterns. The need for high temporal and spatial resolution, combined with the inherent variability of PV outputs, presents significant challenges for forecasting and post-processing across different time horizons. This study addresses these challenges in post-processing optimal point forecasts for PV sites across multiple forecasting ranges, with the aim of providing seamless output for end-users in the energy sector. Specifically, we focus on two-day-ahead PV site forecasts, with an emphasis on a highly resolved nowcasting range (from minutes to hours ahead) and a smooth transition to short-range forecasts. Advanced machine learning techniques, gridded meteorological models, and a variety of location-specific data sources are employed to enhance our post-processing approach for optimal site forecasts.

Focusing on an Austrian case study, we develop a post-processing framework based on machine learning approaches for time-series forecasting, with particular emphasis on Long Short-Term Memory (LSTM) models compared to more classical methods such as Random Forest (RF) and Multiple Linear Regression (MLR). Our primary objective is to smoothly post-process and identify transitions among a set of range-specific, mostly gridded background models spanning various spatial and temporal resolutions. The post-processed models used as input primarily represent irradiance and related parameters. Our work integrates IrradPhyD-Net, a high-resolution AI-based nowcasting model, with AROME, a limited-area Numerical Weather Prediction (NWP) model for the alpine region, providing valuable physical information extending into the short- and medium-range. To exploit the location-specific characteristics of the site, we incorporate additional time-series models that capture the climatology and trends of PV, irradiance, and strongly correlated parameters identified during pre-processing. Given the substantial and growing input data needs of AI and machine learning, we build on our previous contributions by integrating semi-synthetic data to address challenges posed by limited or inconsistent historical PV data, thereby improving model stability. In this context, additional data sources, such as satellite-based CAMS radiation time-series and ERA-5 reanalysis, are essential.

By leveraging skillful input models, supported by synthetic data, our post-processing framework demonstrates strong forecast skill across the studied ranges. Thus, sourcing and transforming data from multiple inputs proves to be an effective way to achieve seamless, high-skill forecasts while maintaining high temporal resolution for nowcasting.

How to cite: Papazek, P., Gfäller, P., and Schicker, I.: Hybrid Post-Processing for Solar Power: Bridging Nowcasting to Short-Range  , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17282, https://doi.org/10.5194/egusphere-egu25-17282, 2025.

Gridscale forecasts of surface weather delivered by operational global NWP suffer from biases which depend strongly on the weather situation and on geographical factors. Such biases also plague re-analyses, such as ECMWF’s ERA5, as operational models are the engines of those re-analyses. This presentation will itemise a number of different gridscale biases identified through a conditional verification exercise in which millions of station measurements were compared with short range Control run forecasts of the ECMWF operational ensemble. We will postulate what physical reasons might underpin these biases. There is for example a strong dependence of rainfall forecast bias on model near surface relative humidity, which seems to relate to the handling of droplet evaporation and other cloud physics processes. All such errors can in principle be addressed via ECMWF’s “ecPoint” post-processing approach; indeed the conditional verification activity here was managed via ecPoint calibration software. The resulting corrections will be illustrated.

Whilst data-driven AI models are currently delivering better predictions of the synoptic pattern than classical physics-based global NWP, the fact remains that those AI models are generally using unadjusted re-analyses for training, and so the situation-dependant biases will clearly put a cap on skill attainable by them for surface weather parameters, even when the forecast synoptic pattern is ‘perfect’. Some ECMWF views on how to overcome this barrier, to deliver even better predictions, will be very briefly presented.

How to cite: Hewson, T.: Using Conditional Verification to describe Situation-dependant Model Biases for Surface Weather – Applications and Implications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18177, https://doi.org/10.5194/egusphere-egu25-18177, 2025.

This research aims to examine the evolution of the large-scale localized buoyancy anomalies in mid-latitude regions, investigating the adjustments in the atmosphere for moist-convective environments. For the global dynamical simulation, the two-layer moist-convective thermal rotating shallow water (mcTRSW) model Aeolus2.0 with intermediate complexity was employed. The concept of two interacting layers enabled the study of the dynamics of localized extreme heatwaves in baroclinic and barotropic situations. The model initialization comprises daily averaged velocity and potential temperature variables from ERA5 data. The results reveal the presence of a circular positive buoyancy anomaly in the lower layer, while the upper layer shows opposite circular rotation wind movement for some of the cases analyzed. The condensed liquid water content anomaly evolution shows that baroclinic localized buoyancy perturbation should play an important role for increased cloud formation and condensation, as a result of the heatwave propagation in the atmosphere for those extreme forcings. Comparing the strong and weak buoyancy anomalies results, we can notice the prolonged effects of baroclinic initial condition over the barotropic case.

How to cite: Oliveira Guimarães, S., Rostami, M., and Petri, S.: An Intermediate Complexity Approach to the Dynamics of Localized Extreme Heatwaves in the Mid-Latitude Atmosphere for moist-convective environments using Aeolus2.0, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18630, https://doi.org/10.5194/egusphere-egu25-18630, 2025.

EGU25-19296 | ECS | Posters on site | AS1.1

Assessing the Performance of Convection-Permitting Regional Climate Models in Simulating the 2002 Extreme Rainfall Event Over Central Europe 

Shruti Verma, Natalia Machado Crespo, Michal Belda, Tomas Halenka, Peter Huszar, and Eva Holtanova

Extreme rainfall events represent a substantial risk to regions across the globe, including the Central Europe. The 2002 Central European flood was a devastating natural disaster affecting countries like Germany, Austria, the Czech Republic, and Hungary. Intense rainfall, saturated soils, and overflowing rivers caused severe flooding, displacing many and leading to significant loss of life. With damages exceeding €20 billion, it remains one of Europe’s most costly flood events, heavily impacting historic cities such as Prague and Dresden (Chorynski et al., 2012).

The spatial and temporal resolution of climate models can present challenges when simulating extreme rainfall events at regional or local scales in term of both the intensity and spatial distribution of precipitation. Therefore, In this study the implementation of high-resolution RCMs with "explicit" convection has been applied which directly resolves deep convection on the model grid without relying on parameterization schemes, known as convection-permitting (CP) models (Prein et al., 2013a,b). This study evaluates the performance of RegCM5 in simulating two consecutive extreme rainfall events (6–7 and 11–13 August 2002) over Central Europe and the Czech Republic, comparing 12 km and 3 km i.e. CP-RCM simulations along with sensitivity of planetary boundary layer (PBL) scheme Holtslag and UW. The results reveal significant discrepancies in the 12km RCM simulations, particularly in Czech Republic, where they struggle to capture the rainfall patterns of both events. The model configurations with UW PBL closely follow the observed extreme rainfall patterns, demonstrating improved alignment with the events. While CP simulations improve the representation of small-scale processes, accurately capturing localized extreme events, particularly the first spell, remains challenging. These findings highlight the potential of CP-RCM simulations for extreme precipitation in terms of climate adaptation, infrastructure development, and policy planning to mitigate the potential risks

How to cite: Verma, S., Crespo, N. M., Belda, M., Halenka, T., Huszar, P., and Holtanova, E.: Assessing the Performance of Convection-Permitting Regional Climate Models in Simulating the 2002 Extreme Rainfall Event Over Central Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19296, https://doi.org/10.5194/egusphere-egu25-19296, 2025.

EGU25-19431 | ECS | Orals | AS1.1

Anemoi: A New Collaborative Framework for Data-driven Weather Forecasting 

Ana Prieto Nemesio, Daniele Nerini, Jasper Wijnands, Thomas Nipen, and Matthew Chantry

Anemoi is an open-source framework co-developed by ECMWF and several European national meteorological services to build, train, and run data-driven weather forecasts. Its primary goal is to empower meteorological organisations to train machine learning (ML) models using their data, simplifying the process with shared tools and workflows.
Designed for modularity and flexibility, Anemoi offers key components for efficient data-driven forecasting. The framework is organised into distinct Python packages covering the entire machine learning lifecycle—from the creation of customised datasets from diverse meteorological sources to the development and training of advanced deep learning graph models. Once a model is trained, Anemoi enables users to run it for inference, using the outputs of physics-based NWP analyses or ensembles as initial conditions, while maintaining comprehensive lineage tracking.
Anemoi has already been applied in experimental operational forecasting, including ECMWF’s Artificial Intelligence Forecasting System (AIFS). It has supported models utilising stretched grid and limited-area configurations. These applications demonstrate Anemoi’s potential to enhance forecasting accuracy by integrating ML techniques into existing systems.
More than just a technical framework, Anemoi represents a collaborative effort among meteorological services, researchers, and technologists, fostering knowledge exchange and innovation.

How to cite: Prieto Nemesio, A., Nerini, D., Wijnands, J., Nipen, T., and Chantry, M.: Anemoi: A New Collaborative Framework for Data-driven Weather Forecasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19431, https://doi.org/10.5194/egusphere-egu25-19431, 2025.

EGU25-19706 | Posters on site | AS1.1

Advances in Project IMA, the Seamless Prediction Programme of the Royal Meteorological Institute of Belgium 

Lesley De Cruz, Simon De Kock, Michiel Van Ginderachter, Maarten Reyniers, Alex Deckmyn, Idir Dehmous, Wout Dewettinck, Felix Erdmann, Ruben Imhoff, Arthur Moraux, Ricardo Reinoso-Rondinel, Mats Veldhuizen, Joseph James Casey, Loic Faleu Kemajou, Anshul Kumar, and Viktor Van Nieuwenhuize

Seamless prediction systems provide frequently updated forecasts across different timescales by combining observations, such as weather radar data, with numerical weather prediction (NWP) models. These systems are increasingly needed by users like hydrological services, local authorities, renewable energy operators, and smartphone apps to make better and earlier decisions. This is especially true for precipitation, which is highly variable in space and time and strongly influences downstream models like (urban) hydrology. To achieve this, forecasts must not only be fast and accurate but also come with calibrated ensembles to estimate uncertainty and propagate errors properly.
In Belgium, Project IMA (inspired by the Japanese word for "now" or "soon") is the seamless prediction system developed by the Royal Meteorological Institute (RMI). It uses RMI’s observation network, including RADQPE for gauge-corrected precipitation estimates, the pysteps-be probabilistic rainfall nowcasting system, the INCA-BE nowcasting system, and the ACCORD NWP models ALARO and AROME. Unlike many other systems, Project IMA offers seamless ensemble precipitation nowcasts for lead times up to 6 hours, updated every 5 minutes, designed to improve flash flood predictions and quantify their uncertainty.
This presentation will showcase recent developments in Project IMA, including updates to the open-source pysteps framework, such as an improved runtime efficiency, code structure and better representation of extremes. We will discuss new deep learning-based methods for blending forecasts to extend their lead time and improve accuracy, calibration, and usefulness for end users such as hydrologists, crisis managers and water authorities.
Project IMA aims to ensure a rapid transfer from research to operations and encourages open-source contributions to ensure transparency and reproducibility. It supports the United Nations’ “Early Warnings for All” initiative, which strives to make forecasts more accessible and actionable by 2027.

How to cite: De Cruz, L., De Kock, S., Van Ginderachter, M., Reyniers, M., Deckmyn, A., Dehmous, I., Dewettinck, W., Erdmann, F., Imhoff, R., Moraux, A., Reinoso-Rondinel, R., Veldhuizen, M., Casey, J. J., Faleu Kemajou, L., Kumar, A., and Van Nieuwenhuize, V.: Advances in Project IMA, the Seamless Prediction Programme of the Royal Meteorological Institute of Belgium, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19706, https://doi.org/10.5194/egusphere-egu25-19706, 2025.

Accurate weather forecasting is vital for societal decision-making in sectors such as renewable energy, agriculture, and disaster management. Statistical post-processing techniques play a critical role in calibrating forecasts and addressing issues of model bias and ensemble dispersion. However, many post-processing methods rely on complete and high-quality datasets, and the presence of missing data can significantly undermine their effectiveness. This study presents a comparative analysis of imputation methods aimed at bridging data gaps to enhance the performance of statistical post-processing techniques.
The evaluation process focuses on a selection of widely used imputation approaches, including ensemble member mean substitution, persistence, Fourier fit, and Neural Networks. These methods are assessed using the forecasts and observations from the EUPPBench dataset by introducing randomly selected missing data, focusing on metrics such as imputation accuracy and their impact on post-processing performance. To quantify the benefit of missing data imputation the study compares different post-processing techniques, ranging from the simpler EMOS to the more advanced Neural Networks, where the latter is known to be more affected by incomplete data. 

How to cite: Lakatos-Szabó, M.: A comparative study of imputation methods for improving statistical post-processing of weather forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19873, https://doi.org/10.5194/egusphere-egu25-19873, 2025.

The Asian Summer Monsoon Anticyclone (ASMA) plays a critical role in trapping, transporting, and redistributing water vapour in the upper troposphere and lower stratosphere, particularly into the extratropical lower stratosphere. Comparison of ERA5 reanalysis data with remote sensing data and simulations with the model ICON-CLM in convection-parameterized (12 km grid spacing) and convection-permitting (3.3 km) setups indicate that the transport into the ASMA is overestimated in ERA5 over the Tibetan plateau (Singh & Ahrens 2023). This presentation critically discusses the water vapour transport into the upper-troposphere/lower-stratosphere by deep convective events over the Tibetan plateau and the Himalayas – an area identified as hotspot for troposphere-stratosphere exchange (Škerlak et al. 2014) using convection-parameterized reanalysis data. Our investigations use a decade-long ICON-CLM climate-like simulation (Collier et al. 2024) performed as a contribution to the CORDEX flagship pilot study Convection-Permitting Third Pole (CPTP).

References

Collier, E., N. Ban, N. Richter, B. Ahrens, D. Chen, X. Chen, H-W. Lai, R. Leung, L. Li, T. Ou, P.K. Pothapakula, E. Potter, A. F. Prein, K. Sakaguchi, M. Schroeder, P. Singh, S. Sobolowski, S. Sugimoto, J. Tang, H. Yu, C. Ziska: The First Ensemble of Kilometre-Scale Simulations of a Hydrological Year over the Third Pole. Clim Dyn. https://doi.org/10.1007/s00382-024-07291-2, 2024

Singh, P., B. Ahrens: Modeling Lightning Activity in the Third Pole Region: Performance of a km-Scale ICON-CLM Simulation. Atmosphere, 14(11), 1655, DOI: 10.3390/atmos14111655, 2023

Škerlak, B., M. Sprenger, and H. Wernli: A global climatology of stratosphere–troposphere exchange using the ERA-Interim data set from 1979 to 2011. English. Atmospheric Chemistry and Physics 14 (2), 913–937. doi: 10.5194/acp-14-913-2014, 2014

How to cite: Ahrens, B. and Singh, P.: Moist convection and tracer transport in and out of the Asian Summer Monsoon Anticyclone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20360, https://doi.org/10.5194/egusphere-egu25-20360, 2025.

EGU25-21081 | ECS | Posters on site | AS1.1

Spatial and Temporal Verification of High-Resolution Modelled Rainfall Data for Urban Flood Risk Assessment 

Markus Pichler and Dirk Muschalla

Reliable climate forecasts are crucial for adapting to future challenges, particularly in urban flood management, where pluvial flooding poses a significant threat. This study focuses on the verification and enhancement of rainfall data for urban flood modelling by analysing critical aspects such as total depth, intensities, seasonality, dry weather periods, and spatial distribution during extreme storm events.

In Graz, Austria, a network of 23 high-resolution precipitation measurement stations covering 120 km², including 13 stations with over a decade of data, was utilized to calibrate a regional climate model through a downscaling approach. This provided minute-level rainfall data for each station, enabling a detailed comparison of historical measurements from the past 10 years with climate model outputs for the current state of the climate. Subsequently, changes in key rainfall characteristics were assessed for the near future (2040–2050) and far future (2090–2100).

Our analysis evaluated yearly precipitation totals, spatial rainfall distribution, intensity-duration-frequency (IDF) functions, and the seasonality of extreme rainfall events. The results revealed promising alignment with historical data, though discrepancies were noted for shorter durations and seasonal shifts. Specifically, heavy rainfall events were projected to occur more frequently in autumn in the future, a trend absent in historical observations.

This study underscores the importance of statistically robust downscaling and verification techniques in blending observational and model-based forecasts to enhance the reliability of climate predictions. These advancements provide critical insights for urban flood resilience planning and illustrate the evolving nature of extreme rainfall under changing climatic conditions.

How to cite: Pichler, M. and Muschalla, D.: Spatial and Temporal Verification of High-Resolution Modelled Rainfall Data for Urban Flood Risk Assessment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21081, https://doi.org/10.5194/egusphere-egu25-21081, 2025.

EGU25-2643 | Posters on site | AS1.2

Initializing the Taiwan WRF-based Regional Ensemble Prediction System with an Ensemble Partial Cycling Strategy 

Yi-Jui Su, Ting-Chi Wu, Chih-Hsin Li, Guo-Yuan Lien, and Chia-Hong Hsieh

A 20-member WRF-based regional Ensemble Prediction System (WEPS) is operationally run at the Central Weather Administration (CWA) to provide up to 5-day ensemble forecasts over the East Asian region with a 15-km grid spacing and a 3-km nest centered over Taiwan. Since becoming operational in 2011, WEPS has been under continuous development that aims to improve the construction of its perturbations in initial conditions (IC), boundary conditions (BC), as well as model uncertainties due to numerical approximations and physical parameterizations. Among these uncertainties, construction of IC perturbations for WEPS is the focus of this study.

 

An initialization method named ensemble partial cycling (EnPC) is proposed for the WEPS. The EnPC method combines partial cycling data assimilation (DA) and the ensemble of DA approach with an additional blending procedure that merges large-scale global features with small-scale regional information, leveraging the DA efforts from the deterministic system of CWA. EnPC is compared with three other initialization methods that are popularly used for regional ensemble forecasting, including dynamic downscaling from a global EPS, Ensemble Adjustment Kalman Filter (EAKF) based regional ensemble DA, and a blended version of the two, the last of which is equivalent to the current operational configuration of WEPS. Among all 4 methods, EnPC is the only method that allows separate initializations for the parent and the nested domains while the initialization for the nested domain in the other three methods is simply a downscale-interpolation from the corresponding parent grid.

 

Several sets of WEPS experiments are conducted over a 5-week period, including five typhoons. EnPC-initialized WEPS forecasts are found to be comparable to the dynamically downscaled forecasts in many evaluation metrics and have more accurate near-surface forecasts over the first 12 h and better precipitation forecast discrimination ability for typhoon events. Compared to the EAKF and the blended methods, forecasts initialized from EnPC have overall smaller errors in most of the evaluation metrics by both deterministic and probabilistic measures and better spread-to-error ratios. As an alternative initialization method, EnPC not only adds some regional benefits on top of downscaling, but also shows some advantages over the operational method. With the planned retirement of EAKF and the anticipation of a more unified production suite at CWA, EnPC will replace the current operational method.

How to cite: Su, Y.-J., Wu, T.-C., Li, C.-H., Lien, G.-Y., and Hsieh, C.-H.: Initializing the Taiwan WRF-based Regional Ensemble Prediction System with an Ensemble Partial Cycling Strategy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2643, https://doi.org/10.5194/egusphere-egu25-2643, 2025.

EGU25-3280 | Posters on site | AS1.2

Sensing the Wind with Hot-air Balloons and their Application in an NWP model 

Evert I. F. (Cisco) de Bruijn

 

Numerical Weather Prediction (NWP) models with a horizontal resolution of 2 km or finer need detailed information for estimating the initial state of the atmosphere. Ground-based remote-sensing instruments like Sodars, Doppler lidars and Profilers provide already meteorological information of the Atmospheric Boundary Layer (ABL). Although observational networks have been extended over the years, there are still gaps in data gathering particular on the finer scales. Therefore we have commenced research to investigate data from third parties. Here we focus on wind-information in the ABL from recreational Hot-air Balloon (HaB) flights. In the basic equipment of a HaB pilot there is a professional navigation device, which is compulsory for safety reasons. Similarly to routinely launched weather balloons, the Global Navigation Satellite System (GNSS)-data from consecutive positions and the elapsed time are the basis of the calculation of the horizontal wind vector. Yearly about 6000 flights take place in the Netherlands, mainly during the morning- and evening transition. As soon as the surface is covered with snow and when convection is strongly reduced, flights may also occur during the day. The HaB data are validated with observations from the meteorological site of Cabauw and we compare the HaB winds with mast data and other available observations like a RASS wind profiler. To explore the possibilities of this new type of wind observations in more complex terrain, we will present the results of an intriguing HaB flight in  Austria, revealing a striking mountain-valley circulation. We also compare the HaB data with the results of an NWP model and we will report about a first attempt to assimilate the HaB data in a NWP model. 

How to cite: de Bruijn, E. I. F. (.: Sensing the Wind with Hot-air Balloons and their Application in an NWP model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3280, https://doi.org/10.5194/egusphere-egu25-3280, 2025.

EGU25-3327 | Orals | AS1.2

Development of NASA’s Earth Science Modeling Strategy 

Ivanka Stajner

NASA is developing an Earth Science Modeling Strategy. This is motivated by recommendation 4.2 from the United States National Academies of Sciences, Engineering, and Medicine, Thriving on Our Changing Planet: A Midterm Assessment of Progress Toward Implementation of the Decadal Survey (2024, https://doi.org/10.17226/27743): “To ensure continued advances in modeling in conjunction with Earth observation: NASA should develop a long-term strategic plan for a strong sustained commitment to Earth system modeling in concert with observations. Success in observation-driven modeling holds the key for maintaining the end-to-end capability that has served NASA well in its effectiveness and service to society.” Moreover, one of the main objectives of NASA’s Earth Science to Action Strategy (https://science.nasa.gov/earth-science/earth-science-to-action/) is to Deliver Trusted Information to Drive Earth Resilience Activities. This Objective will rely on comprehensive Earth system modeling as a key result that will enable NASA to advance and integrate Earth science knowledge to empower humanity to create a more resilient world.

 

In this presentation we will overview the approach being taken to develop the Earth Science Modeling Strategy, within NASA and with the broader community.  Some of the key aspects being considered include comprehensive state-of-science modeling representation of the coupled Earth system, from global to local scales, analyses and predictions at different lead times, from short term predictions to climate projections, and using ensembles. Another key facet is data assimilation into Earth system models and improved utilization and demonstration of the value of Earth observations.  It is envisioned that bold innovation, new disruptive technologies, including artificial intelligence and machine learning, and utilization of large Earth science datasets will be key enablers for cutting edge research, increased understanding of the Earth system, and improved ability to provide actionable Earth science information for societal applications to meet broad user needs. Modeling underpins NASA’s Earth Science to Action strategy as a key capability for advancing foundational knowledge, Earth system science and applied research, as well as increasing societal value of NASA’s data and information leading to improved public understanding. 

How to cite: Stajner, I.: Development of NASA’s Earth Science Modeling Strategy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3327, https://doi.org/10.5194/egusphere-egu25-3327, 2025.

Super typhoons can pose severe threats to coastal cities. For instance, Typhoon Yagi caused hundreds of fatalities and extensive property damages while sweeping across southern China and Southeast Asia in 2024. Accurately predicting the dynamic motion and intensity of super typhoons in high resolution is critical for effective disaster prevention and mitigation. Over the past few decades, the accuracy of typhoon track predictions has notably improved due to the advancements in global numerical weather prediction models. However, their capability to assess typhoon intensity and dynamic structure is still limited by coarse spatiotemporal resolution. The application of physics-based regional models, such as the Weather Research and Forecasting (WRF) model, presents a promising solution to this challenge.

To simulate high-resolution wind fields during super typhoons through WRF, it is essential to determine optimal and robust physical parameterization schemes. In previous studies, sensitivity analysis is often carried out solely based on the error criteria related to typhoon track and intensity, which are inadequate for the performance evaluation of local wind simulation. Additionally, there is a lack of consistent physical parameterization settings for different super typhoons. Furthermore, due to the inherent biases and model errors, a dynamic bias correction strategy is required for local wind forecasting. To this end, we aim to develop an integrated framework in this study that combines typhoon simulation, multi-metric evaluation, and dynamic bias correction.

The super typhoons that have significantly impacted Hong Kong over the past two decades have been chosen as study cases, i.e. Hato, Mangkhut, and Saola. A series of numerical experiments were designed to assess the impact of various physical models. By comparing simulation results with best track data and field observations from the Hong Kong Observatory and the Shenzhen Meteorological Gradient Mast, the multi-metric evaluation method provides a comprehensive understanding of both global and local wind field simulation performance. The best-performing physical models were thereby identified, achieving consistent typhoon tracks (MAE < 30 km), relatively accurate typhoon intensity predictions (RMSE < 5 m/s), and highly correlated wind fields (r > 0.9) between simulation and observation results. To further reduce the effects of systematic biases, a dynamic linear bias correction strategy was introduced to adjust local wind predictions dynamically based on real-time observations. Given the time-evolving local wind data, the linear bias correction factor can reach convergence and provide reliable forecast corrections with a lead time of approximately 15 hours. The proposed framework shows great potential to enhance disaster warning systems and improve local wind prediction accuracy in typhoon-prone regions.

How to cite: Wang, F. and Wang, L.: A multi-metric evaluation and dynamic correction framework for local wind field prediction during super typhoons, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3638, https://doi.org/10.5194/egusphere-egu25-3638, 2025.

Reconstructing historical weather and climate at the daily scale during the early 19th century (1806–1821) is crucial for understanding variability and predictability in this data-scarce period. This study assimilates additional historical pressure and temperature observations into the 20th Century Reanalysis Version 3 (20CRv3) to improve the reliability of daily reconstructions over Europe. 

We use state-of-the-art data assimilation methods, with the Ensemble Kalman Filter as the primary framework for integrating historical series. Alternative techniques, including the Ensemble Square Root Filter and the Iterative Ensemble Smoother, are also investigated to study their performance in capturing daily weather. 

We assess the impact of these methods using evaluation metrics, probabilistic measures, and comparisons to independent observations. Our results reduce the ensemble spread and uncertainty of 20CRv3, providing insights into internal variability at the daily scale and short-term climate dynamics. 

How to cite: Corbella, C.: Reconstructing Daily Weather in the Early 19th Century: New Insights from Data Assimilation , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3762, https://doi.org/10.5194/egusphere-egu25-3762, 2025.

EGU25-3809 | ECS | Posters on site | AS1.2

Development of a Ocean Surface Albedo Scheme with Wave Breaking Factor 

Xueyi Jing and Lanning Wang

Ocean surface albedo (OSA) plays a important role in the energy balance of the climate systems. In climate models, it is typically treated as a constant or represented by a simplistic function of Solar Zenith Angle (SZA). However, research by Jin (2011) indicates that OSA can be significantly influenced by whitecaps under moderate to high surface wind conditions (denoted as Jin11 scheme). Whitecap coverage is a key factor in this parameterization, often expressed as a power function of surface wind speed. Given that water depth and wave height are associated with wave breaking—of which whitecaps are the primary manifestation—the ratio of theoretical wave height to water depth has been incorporated into the Jin11 scheme for adjustment. This modification reflects the characteristic that certain areas are more prone to whitecaps under identical wind conditions.

In this study, we incorporated this improved OSA parameterization scheme into the Community Earth System Model Version 2 (CESM2) and conducted coupled simulation experiments. The numerical results show an alleviation of the excessive reduction in sea surface temperature in the equatorial ocean, the North Pacific subtropical gyre circulation, and the southern westerly wind belt as simulated by the Jin11 scheme. Additionally, longwave radiative heating in the tropical regions is significantly altered after accounting for the wave breaking factor. Precipitation simulations over the northwest Pacific, the tropical Indian Ocean, and the Indo-Pacific Convergence Zone show improvements, while the induced substantial changes in latent heating have further affected vertical motion and convective activity.

How to cite: Jing, X. and Wang, L.: Development of a Ocean Surface Albedo Scheme with Wave Breaking Factor, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3809, https://doi.org/10.5194/egusphere-egu25-3809, 2025.

In this study, a latent heat nudging lightning data assimilation (LDA) method independent of the flash rate was developed and tested with data from the Lightning Mapping Imager (LMI) onboard the Feng-Yun-4A (FY-4A) satellite based on the Weather Research and Forecasting (WRF) model. In this LDA method, the positive temperature perturbations at the lightning location are first calculated by the difference between the moist adiabatic temperature of a lifted air parcel and the model temperature. The positive temperature perturbations in the mixed-phase region are then assimilated by a nudging method to adjust the latent heat within the convective system. Meanwhile, the water vapor mixing ratio is adapted to the temperature perturbations accordingly to constrain the relative humidity to remain unchanged. This method considers the physical nature of the convective system, in contrast with other LDA methods that establish an empirical or statistical relationship between the lightning flash rates and model variables.

The impact of this LDA method on short-term (≤6 h) forecasts was evaluated using two severe convective events in eastern China: a multi-region heavy rainfall event and a thunderstorm high-wind event. The results showed that LDA could add thermodynamic information associated with the convective system to the WRF model during the nudging period, leading to a more reasonable storm environment. In the forecast fields, the simulations with LDA produced more realistic convective structures, resulting in an improvement in forecasts of precipitation and high winds.

How to cite: Gao, Y. and Wang, X.: Impact of Assimilating FY-4A Lightning Data with a Latent Heat Nudging Method on Short-Term Forecasts of Severe Convective Events in Eastern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3879, https://doi.org/10.5194/egusphere-egu25-3879, 2025.

    The level of uncertainty of reanalysis datasets varies greatly based on the quality and amount of available observations and the uncertainty of physical parameterizations used in the background forecast model. Ensemble data assimilation (EDA) schemes are used to quantifiy this combined uncertainty. However, isolating the effects of observational and model uncertainties based on a given ensemble reanalysis is not straightforward. Here, we use the 9 member EDA ensemble produced for the ECMWF 5th Generation Reanalysis product (ERA5) to investigate synoptic scale model uncertainty and its connection to the occurrence of specific weather regimes.

    To control for ensemble spread caused by observation uncertainty - especially on long time scales - we devise grid-point-wise statistical models for the logarithmic ensemble variance with temporal predictors. We use a binary segmentation algorithm to objectively identify change points in ensemble spread time-series caused by abrupt changes in the observation system.

    The set of statistical models allows for statements about the relative impact of changes in the observation system on the total background forecast uncertainty between different grid-points. After filtering out the impact of changes in the observation uncertainty, we obtain a long time series of model uncertainty estimates, which we analyze climatologically with respect to flow characteristics, regime structure and impact of physical parameterizations. This provides regions of high model uncertainty for the respective regimes as well as differences in the role of model uncertainty among the regimes.

How to cite: Schoeller, H. and Pfahl, S.: Isolating the effects of model uncertainty on ensemble reanalysis data and their relation to North Atlantic flow regimes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4243, https://doi.org/10.5194/egusphere-egu25-4243, 2025.

EGU25-5157 | Posters on site | AS1.2

Enhancing Precipitation Predictions in the WRF Model: The Role of Convection Schemes and Increased Spatial Resolution in the Convective Gray Zone 

Rafaella - Eleni P. Sotiropoulou, Ioannis Stergiou, Nektaria Traka, Dimitris G. Kaskaoutis, and Efthimios Tagaris

The Numerical Weather Prediction (NWP) gray zone (GZ) represents a critical challenge in modeling, occurring at spatial resolutions typically ranging from approximately 500 m to 5 km, depending on factors such as the modeling framework, the prevailing atmospheric conditions, and the geographical context where neither full parameterization nor explicit simulation of physical processes is feasible. Within this range, convection parameterizations often become unreliable, particularly for cumulus clouds and turbulence, leading to uncertainties in weather forecasts. High-resolution models (below 4 km) assume explicitly resolved convection, yet this approach does not consistently improve prediction accuracy. Recent advancements in scale-aware parameterizations offer a promising solution, enabling a gradual transition from parameterized to resolved convection, enhancing model performance and reducing biases within the GZ. To explore these challenges, the Weather Research and Forecasting (WRF) model was employed to simulate eight precipitation events across Schleswig-Holstein and Baden-Württemberg in Germany, all exceeding the severe weather threshold of 40 mm/h (warning level 3) set by the German Weather Service. A comprehensive suite of 1,440 simulations was conducted, combining 10 microphysics schemes, 6 cumulus schemes, 8 event cases, and 3 spatial setups. The model setups included a single domain with a 9 km grid size and two two-way nesting configurations with spatial resolutions of 9 km and 3 km. To investigate the role of convection schemes in the convective GZ and the benefits of higher spatial resolution, simulations at 3 km resolution were run both with and without active convection schemes. Initial and boundary conditions were provided by the ERA5 dataset at a spatial resolution of 0.25°. A detailed performance analysis was carried out using pairwise comparisons and the Technique for Order of Preference by Similarity to Ideal Solution (TOPSIS), which ranked the parameterization combinations based on multiple criteria. Results revealed that non-convection-permitting setups performed better during summer precipitation events, where convection is more localized and intense. On the other hand, winter events, influenced by larger-scale processes, showed similar accuracy between convection-permitting and non-convection-permitting configurations. Interestingly, increasing resolution from 9 km to 3 km did not consistently improve model performance. Furthermore, the best-performing parameterizations at 9 km resolution outperformed those at 3 km across all configurations, challenging the common assumption that higher resolution inherently improves model accuracy. These findings emphasize the need to carefully balance resolution and parameterization choices in severe weather forecasting, particularly for convective systems. The study underscores the critical influence of model physics and nesting configurations on simulation outcomes, offering valuable insights for future research and operational modeling efforts.

How to cite: Sotiropoulou, R.-E. P., Stergiou, I., Traka, N., Kaskaoutis, D. G., and Tagaris, E.: Enhancing Precipitation Predictions in the WRF Model: The Role of Convection Schemes and Increased Spatial Resolution in the Convective Gray Zone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5157, https://doi.org/10.5194/egusphere-egu25-5157, 2025.

The Geostationary Interferometric Infrared Sounder (GIIRS) on board the Fengyun 4B (FY-4B) satellite is the first hyperspectral interferometer flying in geostationary orbit. It can provide atmospheric information with high spatial and temporal resolution, which has significant potential for application in regional numerical weather prediction (NWP) models. Due to the high correlation between the infrared hyperspectral channels, it is critical to accurately characterize the inter-channel observational error correlation (IOEC) for assimilating the GIIRS radiance data effectively. This study firstly constructed an observation error covariance matrix for considering the inter-channel correlation of FY-4B GIIRS radiance data based on the NWP system developed by the China Meteorological Administration Beijing Urban Meteorological Institute (CMA-BJ). There was a strong error correlation between adjacent channels and channels with similar detection for the GIIRS radiances. Single-point observation assimilation experiments indicated that the IOEC had a significant impact on the magnitude and structure of temperature and humidity analysis increments. Two groups of assimilation experiments over a 10-day period were carried out and compared. The results showed that an average improvement of 1.5% could be obtained in the RMSE of the temperature and humidity forecasts within the first 12 hours incorporated the IOEC. With the IOEC, a positive impact was also achieved on the precipitation forecast skill, although it was not significant.

How to cite: Xie, Y.: Assimilation and Impact of FY-4B GIIRS Radiances in CMA-BJ Numerical Weather Prediction System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5543, https://doi.org/10.5194/egusphere-egu25-5543, 2025.

        An ensemble down-selection method is proposed to improve the analysis and forecast with a small ensemble,  reducing computational needs. A usual problem with ensemble down-selection is that, despite of the reduction of forecast error, ensemble spread sharply decrease. To limit ensemble spread collapse, this study introduces two variations of a novel down-selection method seeking to minimize the sub-ensemble’s Continuous Ranked Probability Score (CRPS), thereby preserving ensemble spread while minimizing forecast error. The approaches are then tested with a regional-scale model whose precipitation forecast we seek to improve. The precipitation forecast performance of sub-ensembles obtained by these CRPS-based methods is evaluated against the full ensemble, and 100 randomly down-selected sets using various verification metrics measuring precipitation forecast skill. Results demonstrate that the CRPS-based sub-ensembles improve probabilistic forecast accuracy by achieving lower CRPS with the lowest Root Mean Square Error (RMSE) value, especially for short forecasts, without increasing false alarms. Additionally, the Brier Score shows improved forecasts, while Fraction Skill Score (FSS) confirms the improved spatial accuracy in light precipitation. These findings suggest that CRPS-based methods are viable sub-ensembling approaches for balancing accuracy, reliability, and computational efficiency in operational forecasting. By preserving ensemble spread, they improve the sub-ensemble's capacity to represent uncertainty, offering a practical and robust solution for ensemble down-selection.

How to cite: Lee, M.-T., Yau, M.-K., Jacques, D., and Fabry, F.: Ensemble precipitation down-selection methods using Continuous Ranked Probability Score (CRPS): Balancing accuracy and spread under computational constraints, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6903, https://doi.org/10.5194/egusphere-egu25-6903, 2025.

EGU25-7206 | ECS | Orals | AS1.2

Precipitation rate, convective diagnostics and spin-up compared across physics suites in the model uncertainty model intercomparison project (MUMIP)  

Edward Groot, Hannah Christensen, Xia Sun, Kathryn Newman, Wahiba Lfarh, Romain Roehrig, Kasturi Singh, Hugo Lambert, Jeff Beck, Keith Williams, Ligia Bernadet, and Judith Berner

A parameterisation suite is the combination of all parameterisation schemes that is used by a numerical model of the atmosphere. These parameterisation (or “physics”) suites are widely seen as the most uncertain components of atmospheric models.  

In MUMIP we compare deterministic parameterisation suites from across different modelling centres under common prescribed large-scale dynamics. In the first MUMIP experiment, these dynamical tendencies have been derived by coarse-graining the convection-permitting ICON DYAMOND simulation to 0.2 degree resolution. We use these realistic spatiotemporal dynamical patterns to drive millions  of single column model simulations over the tropical Indian Ocean with prescribed SSTs. We use this data to estimate the uncertainty from their physics across four models, each using their default convection-parametrised physics suites. The models are: IFS, GFS, RAP and ARPEGE.

The distributions of precipitation rate, convective available potential energy (CAPE), convective inhibition (CIN) and level of neutral buoyancy are analysed, as well as individual model tendencies and rate of change of CAPE and CIN as a function of lead time and, for instance, the diurnal cycle . We find notable differences across the physics suites and even more strongly between convection-parameterised physics suites and the convection-permitting ICON DYAMOND benchmark. Furthermore, we relate these diagnostics to biases in temperature and specific humidity. We also develop a framework for the detection of statistical relations among diagnostics and/or their change. The framework may for instance be used to quantify the impact of spin-up compared to persistence ("memory") and randomness within a dataset and to identify similarity in the physics across modelling centres.

In this contribution some of the early results of the international MUMIP project will be presented and we hope to encourage other researchers to use and/or complement the data of MUMIP. Please refer to https://mumip.web.ox.ac.uk for details of how to get involved.   

How to cite: Groot, E., Christensen, H., Sun, X., Newman, K., Lfarh, W., Roehrig, R., Singh, K., Lambert, H., Beck, J., Williams, K., Bernadet, L., and Berner, J.: Precipitation rate, convective diagnostics and spin-up compared across physics suites in the model uncertainty model intercomparison project (MUMIP) , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7206, https://doi.org/10.5194/egusphere-egu25-7206, 2025.

FengYun-3E (FY-3E), the fifth satellite in China's second-generation polar-orbiting satellite FY-3 series, was launched on 5 July 2021. FY-3E carries a third-generation microwave temperature sounder (MWTS-3) and a second-generation microwave humidity Sounder (MWHS-2). In this study, the influence of assimilating FY-3E MWTS-3 and MWHS-2 clear-sky radiance data on tropical cyclone forecasts in a regional model is investigated through a series of data assimilation experiments. More than five typhoons from the northwest Pacific Ocean during 2024 typhoon season are selected for the numerical experiments of assimilation and forecasts, and the assimilation effects of FY-3E MWTS-3 and MWTS-2 are carefully evaluated. The results show that assimilation of MWTS-3 and MWTS-2 has positive impact on typhoon track forecasts, especially for forecasts beyond 12 hours, in terms of intensity forecasts, the impact of the data is neutral or slightly positive.

How to cite: Zhang, L., Niu, Z., Weng, F., and Huang, W.: Direct Assimilation of FY-3E Microwave Sounding Channel Data in a Regional Model to Improve Typhoon Forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7592, https://doi.org/10.5194/egusphere-egu25-7592, 2025.

EGU25-7684 | Posters on site | AS1.2

Application of Gridless Method in Data Assimilation 

Xinpeng Yuan

In general, data assimilation systems analyze values on regularly distributed grids according to the irregularly distributed observations. As long as a data assimilation system was established on a certain grid, it cannot adapt to another grid. In this study, the gridless method was introduced into the three-dimensional variation (3DVar) system. Compared with grid-based method, the gridless method uses discrete points for calculation and does not require grid division, thus being immune to grid distribution. Therefore, the data assimilation system based on gridless method can adapt to most model grid structures without the need to write new code. In the data assimilation system based on gridless method, the Cressman analysis technique is adopted as observation operator and the physical transformation matrix is handled using the Taylor expansion method. The idealized experiments based on the Rankine vortex demonstrate that the 3DVar system based on gridless method can handle structured grid, unstructured grid, and mixed (structured and unstructured) grid. Furthermore, the study showed that data assimilation can be performed simultaneously for different grid resolutions, resulting in higher consistency between the grids than when data assimilation is performed separately. 

How to cite: Yuan, X.: Application of Gridless Method in Data Assimilation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7684, https://doi.org/10.5194/egusphere-egu25-7684, 2025.

EGU25-9393 | ECS | Orals | AS1.2

Performance Evaluation of High-Resolution Numerical Weather Prediction Models Using MSG Brightness Temperatures 

Giuseppe Giugliano, Giusy Fedele, Alessandro Bonfiglio, Angelo Campanale, Mario Raffa, Paolo Antonelli, and Paola Mercogliano

This study has been inspired by the activities developed within the IRIDE project in the service chain on “Hydro-meteorological mapping and monitoring atmospheric structure”. The work presents a preliminary evaluation of three numerical weather prediction models, WRF (Weather Research and Forecasting), ICON (ICOsahedral Non-hydrostatic), and COSMO (COnsortium for Small-scale MOdelling), by comparing synthetic and observed brightness temperatures (BTs) from the Meteosat Second Generation geostationary satellite. Synthetic satellite images were generated using the Radiative Transfer for TOVS (RTTOV) model, version 13.2. The analysis spans a verification period of over one month, with all models operating at a horizontal resolution of approximately 2 km and a temporal resolution of 1 hour.

A special focus of the study is the evaluation of the models' ability to reconstruct the intense weather events that struck some Italian regions during the recent years. This severe event caused widespread damage and highlighted the critical need for accurate and timely forecasting capabilities. By analyzing the models' performance during this extreme weather event, we aim to identify strengths and limitations in their ability to simulate localized and high-impact phenomena.

To assess the performance of the models, key verification metrics were calculated to provide a quantitative basis for understanding the accuracy and reliability of the models in predicting atmospheric conditions as represented by BTs.

The results of the verification are thoroughly discussed, with particular emphasis placed on their broader implications for both the development and refinement of numerical weather prediction models. This discussion delves into how these findings can inform improvements in various aspects of model design, from enhancing their ability to simulate complex physical processes to addressing persistent biases and inaccuracies. Differences in model performance are meticulously analyzed to identify potential sources of error, which may arise from a range of factors such as deficiencies in physical parameterizations, limitations in boundary condition specifications, or inaccuracies stemming from radiative transfer assumptions. 

These analyses aim to provide a deeper understanding of the underlying causes of discrepancies, paving the way for more targeted adjustments. This work represents a significant contribution to the ongoing evolution of high-resolution numerical weather prediction models, offering a wealth of valuable insights for both researchers striving to push the boundaries of modeling capabilities and operational forecasters seeking to improve real-time prediction accuracy. By shedding light on the intricate interplay between model dynamics and observational data, it underscores the importance of continuous innovation and refinement in the pursuit of more reliable and precise forecasting tools.

How to cite: Giugliano, G., Fedele, G., Bonfiglio, A., Campanale, A., Raffa, M., Antonelli, P., and Mercogliano, P.: Performance Evaluation of High-Resolution Numerical Weather Prediction Models Using MSG Brightness Temperatures, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9393, https://doi.org/10.5194/egusphere-egu25-9393, 2025.

EGU25-9428 | ECS | Orals | AS1.2

Potential of error-evolving tracer forecasts for operational assimilation of PM2.5 during wildfire smoke episodes 

Annika Vogel, Richard Ménard, James Abu, and Jack Chen

2023 was record-breaking for wildfires in Canada with unprecedented impacts on local ecosystems as well as large scale smoke hazards. These exceptional fire impacts rose the public demand for accurate forecasts of smoke plumes as well as analysis of air quality impacts. However, fire smoke plumes are extreme air quality events with exceptionally high concentrations and related uncertainties fall outside statistical ranges. These particular conditions induce specific challenges for data assimilation algorithms, because error estimates need to capture the high uncertainties and spatial gradients. At the same time, operational forecast systems require high computational efficiency to deliver fast, yet accurate forecasts to the public.

This study explores the potential of a novel assimilation approach, called parametric Kalman filter (PKF), for operational air quality forecasting during extreme air quality events. By explicitly evolving the main error parameters, the PKF has been proven to provide accurate uncertainty estimates at very low computational costs. In this work, a dynamical propagation of error standard deviations is implemented in the Canadian atmospheric-chemical forecast model GEM-MACH. This extended forecast model is applied to a case study of Quebec wildfires in early July 2023. First results indicate that the forecast error distributions during this events can be sufficiently approximated by a passive error-tracer. It is demonstrated that vertical diffusion is a critical component for dynamical error forecasting of extreme air quality events. The error standard-deviation forecasts are used in the current objective analysis (OA) for surface air quality at ECCC (Environment and Climate Change Canada) and compared to operational OA results.

How to cite: Vogel, A., Ménard, R., Abu, J., and Chen, J.: Potential of error-evolving tracer forecasts for operational assimilation of PM2.5 during wildfire smoke episodes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9428, https://doi.org/10.5194/egusphere-egu25-9428, 2025.

EGU25-9643 | ECS | Posters on site | AS1.2

Performance Assessment of CRA40 and ERA5 Precipitation Products over China 

Zelan Zhou, sheng Chen, Zhi Li, Yanping Li, and Chunxia Wei

Precipitation datasets derived from reanalysis products play a critical role in weather forecasting and hydrological applications. This study aims to assess the performance of two distinct reanalysis precipitation products, i.e., the first-generation Chinese global land-surface reanalysis precipitation product (CRA40) and the fifth-generation European reanalysis precipitation product (ERA5), over mainland China. The assessment is conducted with daily-scale gridded-point rain gauge data obtained from Chinese surface meteorological stations as reference, and the continuous and categorical statistical indicators as assessment metrics. The findings of this study are as follows: 1) CRA40 outperforms ERA5 in terms of the 13-year daily mean precipitation and seasonal daily precipitation. CRA40 shows better correlation coefficients (0.97), relative biases (5.25%), root mean square errors (0.34 mm), and fractional standard errors (0.05). 2) Both CRA40 and ERA5 generally exhibit an overestimation of precipitation over mainland China. The degree of overestimation is particularly pronounced in dry climatic regions (e.g., Xizang-Qinghai plateau, Xinjiang province), while wet regions (e.g., the middle and lower reaches of Changjiang River, and South China) demonstrate relatively less overestimation. 3) ERA5 shows better performance in the detection of daily precipitation than CRA40. Neither CRA40 nor ERA5 can well capture heavy precipitation events. These findings are expected to advance our understanding of the strengths and limitations of the reanalysis precipitation products, CRA40 and ERA5, over China.

How to cite: Zhou, Z., Chen, S., Li, Z., Li, Y., and Wei, C.: Performance Assessment of CRA40 and ERA5 Precipitation Products over China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9643, https://doi.org/10.5194/egusphere-egu25-9643, 2025.

EGU25-10029 | Orals | AS1.2

Development and Application of KIM-based Local Ensemble Model 

Hyuncheol Shin, Eun Jung Kim, Sug-gyeong Yun, Jong-Im Park, Jong-Chul Ha, and Dong-Joon Kim

The KIM(Korean Integrated Model)-based local ensemble model, which has a 3km horizontal resolution and 13 members, was developed to improve the prediction of heavy rainfall. The members of the local ensemble model were generated by downloading the KIM global ensemble model. The initial and boundary fields for the members were provided by the KIM global ensemble model. The local ensemble model covers the Korean Peninsula and surrounding areas and produces a 5-day forecast twice a day.
With the introduction of the KIM local ensemble model, the CSI score for precipitation were improved alleviating the underestimation of precipitation in the KIM global model.  In summer, the 75% and 90% percentiles of the local ensemble model show the best performance in heavy rainfall forecasting, while in winter, the median provides the best results.
The analysis verification(RMSE) results also showed that the KIM local ensemble model generally provided improved outcomes compared to the KIM regional model and exhibited similar performance to the UM (Met Office Unified Model)-based local ensemble.

The summer season on the Korean Peninsula is characterized by frequent extreme rainfall events, and this extreme rainfall presents a major challenge for forecasters in producing accurate forecasts. Therefore, various strategies using local ensembles have been developed to predict these extreme rainfall events. Probability matching and percentiles are representative methods, and by employing these techniques, many of the issues associated with the underestimation of extreme rainfall in numerical weather prediction have been largely addressed.

Keywords: local ensemble model, regional model, member, RMSE, CSI, underestimation, extreme rainfall, probability matching, percentiles

How to cite: Shin, H., Kim, E. J., Yun, S., Park, J.-I., Ha, J.-C., and Kim, D.-J.: Development and Application of KIM-based Local Ensemble Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10029, https://doi.org/10.5194/egusphere-egu25-10029, 2025.

EGU25-10218 | Posters on site | AS1.2

Optimizing parameterization schemes with ensemble-based parameter estimation 

Stefano Serafin and Martin Weissmann

State augmentation in a data assimilation cycle can be used as an objective method to estimate uncertain empirical constants in parameterization schemes. In this approach, empirical parameters are appended to the model state vector. They cannot be observed, but, like any other unobserved state variable, they can be updated based on their correlations with the model equivalents of observable quantities. State-parameter correlations are likely flow-dependent, therefore they are best estimated with an ensemble of simulations.

Despite its potential usefulness in parameterization design, ensemble-based parameter estimation has been used so far as a way of accounting for model errors in the assimilation process, and as a method to increase ensemble spread. In this study, we discuss if and how it can aid parameterization optimization. As a case study, we consider a simple first-order parameterization of turbulence in the atmospheric boundary layer. We run several idealized assimilation experiments, partly in a perfect-model scenario (the forecast ensemble and the nature run providing the assimilated observations are instances of the same model), partly in a more realistic imperfect-model scenario (the models providing the forecast ensemble and the nature run the have different formulations).

We demonstrate that, in our case, sensible parameter estimation results are obtained only under restrictive conditions. First, initial conditions must be very accurate, so that the spread of the forecast ensemble is determined primarily by the uncertain parameter. Second, the error variance of the assimilated observations must be low enough for the state perturbations induced by the estimated parameter to be accurately sampled. We show that, when these conditions are met, optimized parameters can compensate for sources of model error, and argue that this property can be used to extend the flexibility of parameterization schemes. For instance, this could be achieved by using parameter estimation experiments to populate lookup tables for adaptive parameters.

How to cite: Serafin, S. and Weissmann, M.: Optimizing parameterization schemes with ensemble-based parameter estimation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10218, https://doi.org/10.5194/egusphere-egu25-10218, 2025.

EGU25-10827 | Posters on site | AS1.2

Analysis of an incorrect forecast of a torrential rain event in the UAE 

Haraldur Ólafsson and Ólafur Rögnvaldsson

On 16 April 2024, the United Arab Emirates experienced torrential rain, with values exceeding 200 mm in less than a day.  In this study the WRF-based forecasting system Weather On Demand (WOD), developed by the Belgingur consortium in Iceland, is employed to explore the medium-range forecasts of the event, by simulations with initial values at different times.  A simulation of the event with 120h lead time was very bad, while a 72h simulation was quite accurate in terms of reproducing an extreme precipitation event.  A comparison of the simulations corresponding to the two forecasts reveals that the error in the 120h simulation is related to incorrect advection of dry air from the desert into the path of the convective storm across the Persian Gulf. The incorrect advection is associated with a wrong perturbation in the atmospheric flow, extending throughout the troposphere.  This perturbation error is associated with an erroneous simulation of a mesoscale convective complex occurring in the vicinity of Bahrain a day before the 16 April event. 

How to cite: Ólafsson, H. and Rögnvaldsson, Ó.: Analysis of an incorrect forecast of a torrential rain event in the UAE, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10827, https://doi.org/10.5194/egusphere-egu25-10827, 2025.

EGU25-10861 | Orals | AS1.2

Recent progress and outlook for the ECMWF Integrated Forecasting System  

Chris Roberts, Florence Rabier, Johannes Flemming, and Stephen English

This presentation will provide an overview of recent scientific and technological developments at ECMWF, including the 2024 upgrade of the Integrated Forecasting System (IFS).

IFS Cycle 49r1 was implemented operationally on 12 November 2024 and substantially improved near surface wind and temperature predictions, especially in the Northern Hemisphere winter season. Key changes to the forecast model in Cycle 49r1 included the introduction of the Stochastically Perturbed Parametrisations (SPP) scheme for model uncertainty, improvements in wave and convective physics, and updates to land surface and atmospheric composition models.

Updates to data assimilation and observation usage in Cycle 49r1 included the assimilation of 2m temperature observations, assimilation of additional satellite data over sea ice, improved modelling of ocean emission and reflection and all-sky assimilation of AMSU-A, several changes to the land data assimilation system, and the introduction of version 13.2 of the radiative transfer model, RTTOV. The grid spacing of the Ensemble of Data Assimilations (EDA) was also reduced from 18 km to 9 km, with the inner loop minimisation grid reduced from 100 km to 40 km.

The impacts of Cycle 49r1 include substantial improvements to 2m temperature and 10m wind speed forecasts, increased spread for tropical cyclones intensity forecasts, a slight reduction of extreme wind forecast errors, and changes to representation of snow cover and snow density. The land data assimilation and model changes lead to a systematic reduction of soil moisture and higher spatial variability in soil moisture levels. At sub-seasonal lead times, Cycle 49r1 has small but statistically robust impacts on ensemble spread, which are driven by the switch to SPP scheme for model uncertainty. These changes are most evident in the tropics, where ensemble spread in the free atmosphere is reduced by several per cent, which represents a slight improvement in ensemble reliability relative to Cycle 48r1. In addition, Cycle 49r1 slightly improves the skill of Madden–Julian Oscillation (MJO) forecasts during weeks 3-4.

Cycle 49r1 is also the foundation for Cycle 49r2, a non-operational IFS cycle that will introduce new versions of the NEMO4/SI3 ocean and sea-ice model and underpin the 6th generation atmosphere and ocean reanalyses (ERA6/OCEAN6), the new version of the atmospheric composition reanalysis (EAC5), and the next seasonal prediction system (SEAS6).  

In parallel to ongoing development of the IFS, ECMWF has developed the Anemoi machine learning toolbox to facilitate the development of data-driven weather prediction models, including deterministic and ensemble variants of the ECMWF AIFS. Real-time evaluation of pre-operational AIFS configurations has demonstrated that they are capable of very skilful medium-range forecasts for a range of upper-atmosphere variables, surface weather variables, and tropical cyclone tracks. The first operational version of the AIFS will be implemented later this year.

Finally, higher-resolution modelling capabilities are being accelerated by Digital Twin developments under the European Commission Destination Earth programme, which is building km-scale capability for a range of potential future HPC architectures. Major efforts are being invested in the code scalability of the Integrated Forecasting System to be able to run on GPUs and investigate alternative dynamical core options.

How to cite: Roberts, C., Rabier, F., Flemming, J., and English, S.: Recent progress and outlook for the ECMWF Integrated Forecasting System , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10861, https://doi.org/10.5194/egusphere-egu25-10861, 2025.

EGU25-11144 | Orals | AS1.2

Assimilation of WIVERN Doppler Data in Weather Research and Forecasting (WRF) Model for the Medicane Ianos: A Comparison with Alternative Data Sources 

Stefano Federico, Rosa Claudia Torcasio, Claudio Transerici, Mario Montopoli, Maryam Pourshamsi, and Alessandro Battaglia

Improving the representation of the initial state of the atmosphere in the Numerical Weather Prediction (NWP) model is critical for advancing the quality of weather forecasts which are vital for our daily life. Wind, cloud and precipitation are driving factors for Earth’s water and energy cycles and sometimes they can represent weather-related threats. Uncertain measurements of these variables present challenges for NWP models.

The WIVERN (Wind Velocity Radar Nephoscope) mission (Illingworth et al., 2018) is one of two candidate missions in Phase A studies for potential selection as the Earth Explorer 11 mission under the European Space Agency’s FutureEO programme. WIVERN would be the first-ever satellite to measure global in-cloud winds. The data from WIVERN is expected to provide significant benefits across multiple sectors, including advancing our understanding of weather phenomena, validating climate statistics, and improving the NWP models performance.

We focus on the NWP performance after assimilating WIVERN Doppler data, specifically Line of Sight (LoS) winds, for the high-impact case study of the Medicane Ianos, occurred in mid-September 2020 in the central Mediterranean. The experimental results of WIVERN Doppler assimilation are compared with those obtained from the output of similar experiments assimilating other data types: the Advanced SCATterometer (ASCAT) radar data, radiosoundings, and Atmospheric Motion Vectors (AMV).

WIVERN pseudo-observations were generated by running an ensemble of WRF at a 4 km horizontal resolution, using the European Centre for Medium range Weather Forecast – Ensemble Prediction System (ECMWF-EPS) analysis/forecast cycle issued at 12 UTC on 16 September 2020 as initial and boundary conditions. The approach consisted of the following steps:

  • The WRF model was run using the initial and boundary conditions from all 51 ECMWF-EPS members.
  • The forecast trajectories of Medicane Ianos from the 51 WRF ensemble members were compared to the observed trajectory.
  • The best WRF member, i.e., the one with the closest agreement between the simulated and observed trajectories, was selected.
  • Pseudo-observations were generated from the output of the selected WRF best member.
  • These pseudo-observations were assimilated into all other members of the WRF ensemble.

For consistency, all observations in this study were pseudo-observations. Assimilation and forecast were performed at 12 UTC on 17 September, followed by a 24-hour forecast.

The trajectories followed by the Medicane are evaluated considering the assimilation of different data sources. Results show marginal improvement of the Ianos’ trajectory when radio-soundings or Atmospheric Motion Vector (AMV) are assimilated, while the trajectory forecast is substantially improved by ASCAT data assimilation (20% improvement). The assimilation of WIVERN data is very important, as the trajectory forecast was improved by over 40%.

A similar positive impact is shown when WIVERN data are assimilated together with other data sources. Specifically, two additional experiments were conducted: in the first, all data sources except WIVERN were assimilated, while in the second, WIVERN data were included. The results show an important improvement of over 10% in the trajectory forecast of Medicane Ianos when WIVERN data are used in combination with ASCAT, AMV and radio-soundings observations.

 

References

Battaglia, A., et al., 2022, https://doi.org/10.5194/amt-15-3011-2022.

Illingworth, A. J., et al., 2018, DOI: 10.1175/BAMS-D-16-0047.1, 1669-1687.

How to cite: Federico, S., Torcasio, R. C., Transerici, C., Montopoli, M., Pourshamsi, M., and Battaglia, A.: Assimilation of WIVERN Doppler Data in Weather Research and Forecasting (WRF) Model for the Medicane Ianos: A Comparison with Alternative Data Sources, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11144, https://doi.org/10.5194/egusphere-egu25-11144, 2025.

EGU25-11527 | Orals | AS1.2

NOAA’s Environmental Modeling Center Update: Transitioning to Unified Forecast System Applications for Operations: Accomplishments till date and Future Plans 

Vijay Tallapragada, Daryl Kleist, Fanglin Yang, Neil Barton, Jacob Carley, and Jason Levit

National Oceanic and Atmospheric Administration’s (NOAA’s) Environmental Modeling Center (EMC) is a lead developer of operational Numerical Weather Prediction (NWP) systems at the National Weather Service (NWS), which are used for the protection of life and property and the enhancement of the economy. EMC transitions to operations and maintains more than 20 numerical prediction systems that are used by NWS, NOAA, other United States (U.S.) federal agencies, and various other stakeholders. These systems are developed through a close collaboration with academic, federal and commercial sector partners. EMC maintains, enhances and transitions-to-operations numerical forecast systems for weather, ocean, climate, land surface and hydrology, hurricanes, and air quality for the U.S. and global domains.

NOAA’s operational predictions are transitioning to the Unified Forecast System (UFS) framework in order to simplify the operational prediction suite of modeling systems. The UFS is being designed as a community-based, comprehensive atmosphere-ocean-sea-ice-wave- aerosol-land coupled Earth modeling system with coupled data assimilation and ensemble capabilities, organized around applications spanning from local to global domains and predictive time scales ranging from sub-hourly analyses to seasonal predictions.  Disparate legacy operational applications that have been developed and maintained by EMC in support of various stakeholder requirements are being transitioned to the UFS framework. The transition started several years ago and is planned to continue over the next few years. Fewer resulting applications will consolidate NCEP’s Production Suite that shares a set of common scientific components and technical infrastructure.  This streamlined suite is expected to accelerate the transition of research into operations and simplify maintenance of operational systems.

There is also a major development effort in the area of AI/ML for NWP, and EMC has stepped up its efforts in adopting and testing the new technologies that show significant promise in revolutionizing operational NWP for NOAA.  

This talk describes major development and operational implementation projects at EMC over the last couple of years, and progress in advancing UFS applications for operations. We will also present EMC plans for AI/ML for NWP, within the overall NOAA strategy, and how planned efforts link with other modeling efforts within NOAA, in the broader U.S. and international community.

How to cite: Tallapragada, V., Kleist, D., Yang, F., Barton, N., Carley, J., and Levit, J.: NOAA’s Environmental Modeling Center Update: Transitioning to Unified Forecast System Applications for Operations: Accomplishments till date and Future Plans, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11527, https://doi.org/10.5194/egusphere-egu25-11527, 2025.

EGU25-12320 | Posters on site | AS1.2

Assimilation of High-volume commercial GNSS Radio Occultation (RO) Observations during ROMEX in NASA’s Global Earth Observing System 

Michael J. Murphy, Jr, Mohar Chattopadhyay, Amal El Akkraoui, Ronald Gelaro, Richard A. Anthes, and Jianjun Jin

The GNSS Radio Occultation (RO) Modeling Experiment (ROMEX) seeks to quantify the benefit of the increasing quantity of RO observations available for use in operational numerical weather prediction (NWP) systems and products.  ROMEX includes participation from multiple operational NWP centers and NWP models, among them are NASA’s Global Earth Observing System (GEOS) model produced and run at the Global Modeling and Assimilation Office (GMAO).  The design of the numerical experiments core to ROMEX include:  1) a control experiment that includes all the RO observations currently used operationally with the sole exception of those from commercial sources and 2) a ROMEX experiment that adds to the control over 25 thousand additional RO profiles per day from commercial RO providers, with both experiments run over the three-month period of September through November 2022.  The ROMEX experiment greatly augments the relatively small subset of the currently available commercial RO profiles which have been purchased for routine use in operational NWP by the various NWP centers.  While this smaller subset of commercial RO profiles currently used in operations has been shown to have a positive impact on NWP forecasts, the additional impact from the ROMEX RO dataset has yet to be determined and is the focus of ROMEX.  Results from GEOS are presented, including the impact on both analyses and forecasts over the study period and statistics using the forecast sensitivity-based observation impact (FSOI) method.

 

How to cite: Murphy, Jr, M. J., Chattopadhyay, M., El Akkraoui, A., Gelaro, R., Anthes, R. A., and Jin, J.: Assimilation of High-volume commercial GNSS Radio Occultation (RO) Observations during ROMEX in NASA’s Global Earth Observing System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12320, https://doi.org/10.5194/egusphere-egu25-12320, 2025.

EGU25-12631 | ECS | Orals | AS1.2

Applying a Genetic Algorithm to Optimize Hail Prediction Using the Weather Research and Forecasting Model 

Iciar Guerrero-Calzas, Lorenzo Rossetto, Ana Cortés Fité, Mauricio Hanzich, and Josep Ramón Miró

Hailstorms are highly localized severe weather events that can cause extensive damage to agriculture, infrastructure, and property, necessitating accurate forecasting for effective risk mitigation. The Weather Research and Forecasting (WRF) model, a numerical model which is able to simulate features from a wide range of scales, offers a range of physics parameterizations to simulate sub-grid scale processes which are essential for hail storm forecast. However, the vast number of possible configurations complicates the identification of an optimal setup for hail simulation. This study leverages a genetic algorithm (GA) to systematically optimize WRF physics parameterizations for hail prediction over Central Europe, focusing on the severe hail events of June 2022.

The GA framework encodes WRF physical parameterizations configurationsas individuals within a population, evolving through selection, crossover, and mutation across multiple generations. Fitness is evaluated using the F2 score, prioritizing recall to address the imbalance between observed hail and non-hail events. By exploring over 2.4 million potential configurations, the GA provides the best combinations of physical parametrizations to capture the spatial and temporal characteristics of hailstorms. The results show that this methodology enables the exploration of a wide range of possible configurations, demonstrating its potential to optimize parameterizations for high-impact weather events effectively. This novel methodology represents a substantial step toward advancing hail forecasting capabilities using high-resolution NWP models.

How to cite: Guerrero-Calzas, I., Rossetto, L., Cortés Fité, A., Hanzich, M., and Miró, J. R.: Applying a Genetic Algorithm to Optimize Hail Prediction Using the Weather Research and Forecasting Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12631, https://doi.org/10.5194/egusphere-egu25-12631, 2025.

EGU25-12777 | Posters on site | AS1.2

A Prototype High-Resolution Data-Assimilation System for Israel 

Ehud Strobach, Offer Rozenstein, and Dorita Rostkier-Edelstein

Climate change is already here, but our understanding of its local impacts in Israel is still lacking. Although large networks of in-situ observations cover Israel, and there is an increasing amount of information coming from satellites, there are still spatial and temporal gaps that are not expected to be solved in the coming decades. The problem is more pronounced in Israel than in other locations due to its complex terrain and high climate variability. These characteristics necessitate more observations (relative to other regions) to reliably sample the regional variability and allow for regular temporal and spatial data interpolation. Reanalysis datasets have become more popular in the last few decades due to their regularity in space and time, which is achieved by combining observations with model outputs using a predefined data assimilation method. However, current reanalysis products are still too coarse to represent the high climate variability in Israel, and therefore, their use is limited. In this presentation, we will describe our effort to generate a prototype high-resolution convection-permitting ensemble-based data-assimilation system and a reanalysis product for Israel.

How to cite: Strobach, E., Rozenstein, O., and Rostkier-Edelstein, D.: A Prototype High-Resolution Data-Assimilation System for Israel, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12777, https://doi.org/10.5194/egusphere-egu25-12777, 2025.

EGU25-13971 | ECS | Posters on site | AS1.2

Improvement of Impact-based Forecast Using Multi Model Ensemble in 2024 

Sug-gyeong Yun, Hyun-Cheol Shin, Jong-Chul Ha, and Dong-joon Kim

 The Korea Meteorological Administration(KMA) is producing an impact-based forecast data based on Multi-Model Ensemble(MME) system which integrates Unified Model(global, global ensemble, local, and local ensemble models), ECMWF(global and global ensemble models) and KIM(Korean Integrated Model) global model for heat waves (HW) and cold waves (CW). MME-based impact forecast(MEPS) determines the impact(safe, concern, caution, warning, alarm) by using the probability of occurrence of maximum feels-like temperature for HW and lowest temperature for CW in Korea. 
   The distribution from 93 MME members was converted to a GEV(Generalized Extreme Value) distribution until 2023, but there is a problem that only the daily temperature can be considered. Definition of HW and CW should take into account the 2-day duration/falling temperature compared to the previous day. Therefore, the probability calculation method was modified with the ratio of the number of members satisfying the HW and CW condition among all members and its performance was compared with the previous method. 
  Verification was conducted by evaluating how well impact-based forecast was matched to the observed impact in 177 regions about 1~9 forecast day. HW was verified for August and September 2023, and CW was verified for December 2023 and January 2024.
  As a result, in the case of HW forecasting, impact-based forecast with new method showed a little better performance than previous method with GEV. New method has better Bias at concern(4-9day), warning(3-9day), alarm, and Equitable Thread Score at safe(2-9day), concern(2-9day), alarm. In addition, there are cases in which the definition of guidance is more accurately satisfied compared to the previous MEPS guidance, which was overestimated. Also, new method required much less calculation time than previous method. On the other hand, new method are not applied to CW MEPS due to its overall low performance. 
  It is presumed that the reason for the degration of performance of new method for CW is that the probability table for determining the impact in the probability distribution has not been tuned. If this table is optimized, it is expected that the performance can be improved in CW case, too.

How to cite: Yun, S., Shin, H.-C., Ha, J.-C., and Kim, D.: Improvement of Impact-based Forecast Using Multi Model Ensemble in 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13971, https://doi.org/10.5194/egusphere-egu25-13971, 2025.

EGU25-14710 | Orals | AS1.2

Sensitivity analysis of severe weather events to different background error covariances in meteorological aircraft data assimilation 

Seung-Beom Han, Tae-Young Goo, Sueng-Pil Jung, Min-Seong Kim, Deok-Du Kang, and Chulkyu Lee

Aircraft data are considered one of the best platforms for obtaining atmospheric spatial information in the observation gap over the ocean. The National Institute of Meteorological Sciences (NIMS) has operated an atmospheric research aircraft to mitigate this observation gap. In particular, the dropsonde and AIMMS-20 systems installed on the aircraft generate vertical distributions of meteorological variables over the ocean, and these specialized observation data enhance the accuracy of the initial model fields. These aircraft observation data provide continuous distributions of meteorological variables and significantly contribute to improving the performance of numerical predictions. In this study, we evaluated the effectiveness of data assimilation (DA) on the prediction of severe meteorological phenomena affecting the Korean Peninsula using high-resolution numerical modeling using atmospheric research aircraft observation data. To analyze the sensitivity of the difference in the background error covariance in the data assimilation method, three sets of simulation experiments were performed. First, an experiment was conducted using the background error covariance option CV3 based on the NMC method, which is suitable for simple settings or when the computational resources are limited. Second, an experiment using option CV5 is suitable for studying more complex situations or high-accuracy forecasts. This option generates a covariance structure that adapts to atmospheric conditions by using an ensemble-based method. The last is an experiment using the CV7 option, which is a hybrid background error covariance option that combines static methods (such as CV3) and ensemble-based methods (such as CV5), and has the advantage of combining climate statistics and flow-dependent features to improve model prediction performance.

How to cite: Han, S.-B., Goo, T.-Y., Jung, S.-P., Kim, M.-S., Kang, D.-D., and Lee, C.: Sensitivity analysis of severe weather events to different background error covariances in meteorological aircraft data assimilation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14710, https://doi.org/10.5194/egusphere-egu25-14710, 2025.

Extreme rainfall events often lead to significantly heavier rainfall over urban areas compared to their surrounding regions. Predicting these positive urban precipitation anomalies during heavy rainfall remains a critical challenge in numerical weather modeling. This study explores the sensitivity of the Weather Research and Forecasting (WRF) model to approximately 70 combinations of parameterization schemes, including microphysics, cumulus convection, planetary boundary layer options, and urban canopy model schemes, focusing on urban precipitation anomalies.

The analysis is based on two significant heavy rainfall events over Chennai, India: October 22, 2006, and November 8, 2015. Model simulations are validated against Integrated Multi-satellite Retrievals for GPM (IMERG) precipitation data to evaluate their ability to capture urban anomalies. High-resolution simulations demonstrate that specific combinations of parameterization schemes, particularly those incorporating multi-level urban canopy models, enhance the model’s capacity to predict significant positive anomalies during intense rainfall events.

The findings underscore the critical role of urban canopy models in shaping precipitation intensity and spatial distribution and the interplay between cumulus convection and boundary layer processes in driving urban precipitation dynamics. These insights provide practical guidance for optimizing WRF parameterization settings, advancing the accuracy of urban-scale weather prediction, and deepening the understanding of urban hydrometeorological processes.

How to cite: Kalamalla, L. and Satyanarayana, A.: Sensitivity Analysis of Parameterization Schemes in the WRF Model for Predicting Urban Precipitation Anomalies Over Chennai, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15854, https://doi.org/10.5194/egusphere-egu25-15854, 2025.

EGU25-17036 | Posters on site | AS1.2

Land surface temperature trends in Iceland 

Iman Rousta and Haraldur Ólafsson

Land surface temperature (LST) on Iceland has been retrieved by means of remote sensing for the period 2001-2023.  The trend in the data shows substantial geographical variability on different scales and is partly very different from the general upward trend in the 2 m temperatures.  There are areas with strong negative trend and other areas with strong positive trend.  The variability may be attributed to changes in snow cover and vegetation.  Impact of volcanic eruptions and retreat of glaciers are also detected.  The results suggest that using data decades back in time to train forecasting models may lead to systematic errors in surface temperature forecasts.        

How to cite: Rousta, I. and Ólafsson, H.: Land surface temperature trends in Iceland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17036, https://doi.org/10.5194/egusphere-egu25-17036, 2025.

EGU25-17466 | ECS | Posters on site | AS1.2

Arctic Temperature Persistence in Summer and Autumn and Seasonal Forecasting 

Negar ekrami and Haraldur Olafsson

Persistence is the first approximation to seasonal and sub-seasonal temperature forecasting.  In the present study, summer and autumn temperature persistence in mean monthly temperatures in the circumpolar Arctic is explored in time-series of monthly mean data.The temperature correlations extend from being negative to very high. 

The spatial variability of temperature persistence may be linked to the Bowen ratio, static atmospheric stability, snow cover and sea-ice extent.  The variability in these factors may contribute directly to seasonal variability in the radiation budget as well as in surface fluxes.  In some regions there are also detectable impacts that can be associated with regional circulation patterns.

How to cite: ekrami, N. and Olafsson, H.: Arctic Temperature Persistence in Summer and Autumn and Seasonal Forecasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17466, https://doi.org/10.5194/egusphere-egu25-17466, 2025.

EGU25-18433 | ECS | Posters on site | AS1.2

The Impact of Ground-based Microwave Radiometer Data Assimilation: A Case Study 

Changliang Shao, Yakai Guo, and Yuting Dong

Atmospheric profiles are indispensable for operational weather forecasting across a wide range of scales and latitudes. Despite their importance, the assimilation of tropospheric wind and temperature profiles remains a complex task with considerable potential to markedly improve weather predictions. This research investigates the impact of Ground-based Microwave Radiometer profile measurements on Numerical Weather Prediction (NWP) using a real rainfall case study. Employing the Local Error-Subspace Transform Kalman filter (LESTKF), we assimilate temperature and wind profiles derived from the Ground-based Microwave Radiometer observation network. The coupled WRF-PDAF (Parallel Data Assimilation Framework) system is utilized to conduct twin experiments. These experiments, which vary observation variables and localization distances, offer valuable insights into the assimilation process. The study evaluates potential configurations for future profile measurements and discusses recommended localization distances. The results demonstrate that incorporating multiple observation variables leads to substantial forecast improvements compared to using individual variables alone. The research culminates in a recommendation for an optimal localization distance, which has the potential to enhance the accuracy and reliability of weather forecasting.

How to cite: Shao, C., Guo, Y., and Dong, Y.: The Impact of Ground-based Microwave Radiometer Data Assimilation: A Case Study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18433, https://doi.org/10.5194/egusphere-egu25-18433, 2025.

EGU25-18692 | Orals | AS1.2

Numerical Weather Prediction meets Machine Learning - a synergy for better forecasts 

Olafur Rognvaldsson and Karolina Stanislawska

Numerical Weather Prediction (NWP) has recently lost its hegemony in weather forecasting, as more machine-learning-based models achieve results comparable to NWP. It turns out that data-driven models are capable of identifying patterns and distilling physical laws that, until now, have only been formulated by atmospheric physics specialists. Although ML-based models are already being used by meteorological institutes alongside NWP-based models, this does not mean that NWP will fade into irrelevance. In this talk, we will show how NWP and ML can interoperate to achieve the shared goal of providing more accurate weather forecasts. From NWP providing high-quality training data for ML models to ML models replacing specific parameterizations, the spectrum of collaboration is vast. ML models cannot succeed without high-quality training data provided by NWP, and NWP can benefit from this new technology by incorporating ML models in places where conventional physics parameterizations are found lacking. None of the currently successful ML-based models would exist without the high-quality reanalysis data generated through numerical models. Decades of expertise and extensive research in numerical modelling now serve as a solid foundation for the remarkable achievements of data-driven applications. The future of weather forecasting is built on this synergy — numerical modelling and machine learning working together to achieve what neither could accomplish on its own.

How to cite: Rognvaldsson, O. and Stanislawska, K.: Numerical Weather Prediction meets Machine Learning - a synergy for better forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18692, https://doi.org/10.5194/egusphere-egu25-18692, 2025.

EGU25-19128 | ECS | Orals | AS1.2

Multi-model high resolution analysis of Mediterranean Hurricane Daniel with WRF and ICON 

Piero Serafini, Antonio Ricchi, Chiara Marsigli, and Rossella Ferretti

Medicanes are very dangerous meteorological phenomena with large uncertainty on genesis and intensification usually case dependent. The peculiarity of medicane Daniel analyzed in this study is the long life and strong tropical-like characteristics even on land with baroclinic atmosphere. It is essential to deepen the knowledge of these events to improve operational forecasts and waring systems. In this perspective, the models used in this analysis have reported results sufficiently close to observations. In particular, the WRF model performed better in terms of temporal synchronization of the phenomenon, internal structure of the cyclone and spatial distribution of precipitations; while ICON better modeled lower layers and highlighted different feature on track and tropical transition.
For both the models the tracks obtained from the simple algorithm used are discrete, with major errors in the initial phase. The landfall was simulated with acceptable errors. Minimum Mean Sea Level Pressure values are modeled as lower than the observed one, with WRF simulating a most intense cyclone. Wind speed data correctly passed the threshold for classification as a Category 1 hurricane, although WRF overestimated the mid-tropospheric wind. The Hart's Cyclone Phase Space diagram consistently highlighted the tropical phase of the medicane with a symmetric deep warm core at its most intense period, but the values of the parameters differ from simulation to simulation. Finally, the point values of precipitation are not satisfactory in any model even if the field of cumulated precipitation is consistent with the observations.

How to cite: Serafini, P., Ricchi, A., Marsigli, C., and Ferretti, R.: Multi-model high resolution analysis of Mediterranean Hurricane Daniel with WRF and ICON, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19128, https://doi.org/10.5194/egusphere-egu25-19128, 2025.

The evaluation of two reanalysis precipitation datasets, CRA40 and ERA5, was conducted over the Ganjiang River Basin, utilizing precipitation records from 37 ground rainfall gauges and surface-observed stream flow data spanning from January 1998 to December 2008. Both CRA40 and ERA5 were found to effectively capture the spatial and temporal precipitation characteristics at the basin scale. However, significant differences in precipitation quality were observed between the two. ERA5 demonstrated superior accuracy in depicting short-term precipitation changes, particularly on a daily basis. In contrast, CRA40 exhibited better performance on a monthly scale, offering more stable and long-term precipitation trends. Simulations of stream flow using the VIC hydrological model driven by these two precipitation products revealed that (1) CRA40 outperformed ERA5 in both daily and monthly stream flow simulations, with a higher Nash-Sutcliffe Efficiency (NSE, 0.65 for CRA40 vs. 0.6 for ERA5) and a greater correlation coefficient (CC, 0.96 for CRA40 vs. 0.91 for ERA5). Although ERA5 had a relatively good CC (0.86 and 0.93 respectively), its NSE was notably poor (0.29 and 0.30 respectively); (2) both CRA40 and ERA5 tended to overestimate stream flows in the basin, especially during the flood season (April-September), with ERA5's overestimation being more evident. This study is anticipated to offer a foundation for selecting reliable reanalysis products for precipitation and hydrological simulations in the Ganjiang River Basin.

How to cite: li, Z., Zhou, Z., and Chen, S.: Hydrological Evaluation of CRA40 and ERA5 Reanalysis Precipitation Products over Ganjiang River Basin in Humid Southeastern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20414, https://doi.org/10.5194/egusphere-egu25-20414, 2025.

EGU25-20640 | Posters on site | AS1.2

A paradigm shift for developing parameterizations of subgrid motion in NWP models 

Jian-Wen Bao and Sara Michelson

We introduce a paradigm shift for developing parameterizations of subgrid motion in numerical weather prediction (NWP) models, which is based on recent developments in the theory of computational fluid dynamics.  The governing equations of an NWP model are based on the same Navier-Stokes (N-S) equations used in computational fluid dynamics.  They must be averaged over a grid-cell volume before transforming into discrete forms in order to be solved numerically.  Consequently, extra terms of turbulent subgrid motion appear in these governing equations that must be approximated or parameterized.  The recent development of the formal theory on the N-S equations filtered via numerical discretization concludes that such parametrizations cannot be exact for the equations to be solvable numerically.  Approximation in these parameterizations is necessary for the N-S equations to be solvable as a well-posed problem.  Practically, this has two implications for parameterizing subgrid motion in NWP models.  First, the development of the parameterizations of subgrid motion is required to be driven by improving the accuracy of the parameterizations to address specific prominent performance issues of an NWP model, and the improvement should be based on observations of forecast variables and subgrid processes for it to be physically relevant.  Second, the parameterizations should be as simple as possible for feasible performance tuning based on observations and for computational efficiency.  In this presentation, we will use two examples to discuss what the problem-driven and observation-based approach means in developing subgrid convection and turbulent mixing parameterizations in NWP models.  We will use the two examples to advocate that the problem-driven and observation-based approach should be used to develop all subgrid physics parameterizations in weather and climate models for developing parameterizations of subgrid motion.

How to cite: Bao, J.-W. and Michelson, S.: A paradigm shift for developing parameterizations of subgrid motion in NWP models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20640, https://doi.org/10.5194/egusphere-egu25-20640, 2025.

EGU25-20650 | Posters on site | AS1.2

A process-level comparison of two PBL schemes in the Unified Forecast System in a fog case study 

Evelyn Grell, Sara Michelson, and Jian-Wen Bao

We present an investigation in which two planetary boundary layer (PBL) schemes are compared at the parameterized physical process level in a fog simulation case study.  The two PBL schemes in question are two options in the Unified Forecast System (UFS) for global and regional applications.  We investigated the difference between the two schemes using both 3-D regional and single-column configurations of the UFS.  We found that there are no significant differences in terms of parameterized physical processes.  The two schemes differ mainly in the closure assumptions and the magnitudes of parameters used in the parameterization formulations, resulting in more or less success in simulating the development of the observed fog layer.  Both schemes have their own error characteristics in representing essential processes for fog formation and dissipation, pointing to the uncertainty in PBL process parameterizations when observations and realistic large-eddy simulations are insufficient for process evaluation.

How to cite: Grell, E., Michelson, S., and Bao, J.-W.: A process-level comparison of two PBL schemes in the Unified Forecast System in a fog case study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20650, https://doi.org/10.5194/egusphere-egu25-20650, 2025.

EGU25-20960 | Orals | AS1.2 | Highlight

Implications of AI for Atmospheric Predictability of Convection and Winter Storms 

Steven Greybush and Christian Spallone

Recent advances in artificial intelligence (AI), specifically with applications of deep learning, have brought paradigm-shifting changes to Numerical Weather Prediction.  Recent AI-based NWP systems have rivaled traditional physics-based global NWP systems according to some verification metrics.  However, the performance of these systems for extreme events, and their implications for atmospheric predictability, has not yet been fully explored.    In this study, the practical predictability for winter storms in eastern North America will be compared using forecasts generated by several traditional NWP and AI-NWP systems.   In addition to domain-wide verification statistics, the realism of cyclone structure and evolution will be evaluated at different forecast lead times.  We plan to discuss the ensemble predictability of events, evaluating the sensitivity of the AI-NWP systems to initial condition perturbations, with implications for data assimilation.  Finally, at the mesoscale, we will demonstrate a convection initiation nowcasting system that utilizes deep learning to generate probabilities of new convection forming at lead times under one hour, which we interpret using explainable AI and uncertainty quantification.

How to cite: Greybush, S. and Spallone, C.: Implications of AI for Atmospheric Predictability of Convection and Winter Storms, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20960, https://doi.org/10.5194/egusphere-egu25-20960, 2025.

Traditional ensemble forecasting based on numerical weather prediction (NWP) models, is constrained by the need for massive computational resources, resulting in limited ensemble sizes. Although emerging artificial intelligence (AI)-based weather models offer high forecast accuracy and improved computational efficiency, they still face considerable challenges in ensemble forecasting applications.

In this study, we propose a fast, physics-constrained perturbation scheme through self-evolution dynamics of AI-based weather model for ensemble forecasting of tropical cyclones (TCs). These initial perturbations are conditioned on specific amplitude and spatial characteristics, exhibiting physically reasonable dynamical growth and spatial covariance. Based on this perturbation scheme, the TC track ensemble forecasts within the AI-based model significantly outperform those from the European Centre for Medium-Range Weather Forecasts (ECMWF) in both deterministic and probability metrics. Notably, we conduct TC track forecasts with 2000 members for the first time, achieving further enhanced forecast skill in probability distribution and extreme scenario of TC movement.

How to cite: Pu, J., Mu, M., Feng, J., Zhong, X., and Li, H.: A Fast Physics-based Perturbation Generator of Machine Learning Weather Model for Efficient Ensemble Forecasts of Tropical Cyclone Track, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2160, https://doi.org/10.5194/egusphere-egu25-2160, 2025.

Incorporating appropriate physical constraints to data assimilation is of great significance for the assimilation of disastrous weather data assimilation and numerical forecasting. Generally, model constraints are often difficult to describe complex sub-grid physical processes with strong nonlinearity and discontinuity, due to difficulties in developing the tangent linear and adjoint. In 4DVar, simplified physical process schemes are often used instead. With the development of artificial intelligence (AI) technology, complex sub-grid physical processes can be probably considered in variational constraints. On the basis of momentum equation constraints, this study introduces sub-grid boundary layer turbulent friction effects through machine learning (ML) and adds them into momentum equation constraints. Firstly, a deep neural network model is used to train the horizontal momentum tendency simulated by the YSU boundary layer parameterization scheme of WRF model. Secondly, under the Ensemble-Var framework of WRFDA, the momentum tendency of the boundary layer is introduced into the weak constraint of the horizontal momentum equation of variational method. The boundary layer turbulent friction term is implemented by embedding a deep neural network model, and its tangent and adjoint operators are developed to construct a ML-DA scheme. Finally, a physical constraint scheme considering the turbulent friction effect of boundary layer is established for data assimilation. The new assimilation scheme is applied to the radial wind assimilation of coastal radar. Numerical simulation experiments on different typical landing typhoons show that the new scheme better described the boundary layer four-force balance during the data assimilation process. Assimilating the direct-observed wind field, the thermal fields such as pressure and temperature are also improved. The new scheme plays a positive role in typhoon intensity and structure forecasting.

How to cite: Li, X.: Implementing the sub-grid boundary layer turbulent effects into variational constraints trough machine learning and its impact on typhoon assimilation , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2217, https://doi.org/10.5194/egusphere-egu25-2217, 2025.

This study investigates the uncertainties of two AI-driven meteorological models, Pangu-Weather and Fuxi, in the forecasts of tropical cyclones (TCs) from perspective of target observations. The conditional nonlinear optimal perturbation (CNOP) method is used to identify the sensitive areas for target observations, and the TCs in the Northwest Pacific and Bay of Bengal (BoB), with the latter being often referred as “BoB storms”, are investigated. The results suggest that the predictability of the “Pangu-Weather” model with respect to the BoB storm tracks is limited within 24 hours, and model error effects dominate the uncertainty of the forecasts after 24 hours; while for the TCs in the Northwest Pacific, the Fuxi model is shown to be strongly sensitive to initial perturbations and provide much accurate sensitive areas for target observations associated with TC track forecasts. These results illustrate the uncertainties of the two AI models and provide a theoretical basis for implementing field campaigns for target observations using AI models.

How to cite: Duan, W.: Uncertainty of AI models in tropical cyclone forecasts: target observation perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2261, https://doi.org/10.5194/egusphere-egu25-2261, 2025.

EGU25-3579 | ECS | Posters on site | AS1.3

Multivariate adjustment in the IAU-based tropical cyclone initialization scheme  in TRAMS model 

Shaojing Zhang, Daosheng Xu, Wenshou Tian, and Banglin Zhang

The operational Tropical Regional Atmospheric Model System (TRAMS) model often underestimates the initial typhoon intensity when using the global analysis field as the initial condition. The tropical cyclone (TC) initialization scheme developed based on incremental analysis updates (IAU) technique can help reduce the initial bias. However, the IAU-based TC initialization scheme only adjusted the wind field at the analysis moment, with other variables adjusted implicitly under the constraints of the model according to the gradually inserted wind increment (named “univariate adjustment scheme” hereafter). The univariate adjustment scheme required approximately 3  to reach a dynamic equilibrium state, limiting the use of hourly TC observation information and dissipating too much meaningful short-wave information of the adjustment increment. To reduce the equilibrium adjustment time, this study constructed a multivariate adjustment IAU-based TC initialization scheme by introducing the gradient wind balance and hydrostatic balance as large-scale constraints. The case sensitivity tests of TC Hato (1713) demonstrated that the multivariate adjustment scheme can reduce the IAU relaxation time to 1  and slightly improve TC forecasts. By incorporating the equilibrium assumption as a strong constraint for the TC axisymmetric component, the multivariate adjustment scheme achieved a faster convergence of the model to its equilibrium state, reducing the loss of useful observed information. This conclusion was further confirmed with 12 other TCs. The IAU-based multivariate adjustment initialization scheme developed in this study provides a foundation for 4-D initialization with hourly TC observations.

How to cite: Zhang, S., Xu, D., Tian, W., and Zhang, B.: Multivariate adjustment in the IAU-based tropical cyclone initialization scheme  in TRAMS model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3579, https://doi.org/10.5194/egusphere-egu25-3579, 2025.

EGU25-4099 | Orals | AS1.3 | Highlight

RIKEN’s activities to integrate data assimilation and AI/ML 

Takemasa Miyoshi, Shigenori Otsuka, Jianyu Liang, Michael Goodliff, Gwendal Saliou, Said Ouala, and Pierre Tandeo

At RIKEN, the Japan’s national flagship research institute for all sciences, we have been exploring several attempts to integrate data assimilation (DA) and AI/ML. DA integrates the (usually process-driven) model and data, while AI/ML is purely data driven and is proven to be very powerful in many applications. An example is to integrate data-driven AI/ML-based precipitation nowcasting with process-driven numerical weather prediction (NWP). We developed a nowcasting system based on a convolutional long short term memory (LSTM) which takes several time steps of 2-D precipitation image data to predict future images. NWP with radar DA produces future precipitation images, which can be input to the data-driven LSTM to further improve the predicted images. Another example is to develop ML’ed observation operators for satellite radiances. We obtained an improvement by purely ML’ed observation operators without any information from a physically based radiative transfer model. The third example is to use DA with an ML’ed surrogate model for producing more accurate analyses for further training the ML’ed surrogate model. We found that DA with flow-independent background error covariance could produce more accurate ML’ed surrogate model, but ensemble-based DA resulted in a mixed situation probably because the ensemble forecasts by the ML’ed surrogate model may not produce proper error covariance. We also explored developing a limited-area ML’ed surrogate NWP model in collaboration with IMT-Atlantique. In this presentation, we will share the most recent activities of integrating DA and AI/ML at RIKEN.

How to cite: Miyoshi, T., Otsuka, S., Liang, J., Goodliff, M., Saliou, G., Ouala, S., and Tandeo, P.: RIKEN’s activities to integrate data assimilation and AI/ML, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4099, https://doi.org/10.5194/egusphere-egu25-4099, 2025.

Recently, artificial intelligence (AI) models have upended numerical weather prediction (NWP) by achieving performance comparable to or even surpassing that of physics-based NWP models while also significantly reducing computational costs. However, these AI solutions generally operate with initial conditions produced by NWP data assimilation, which remains costly and can suffer from approximations. We introduce OMG-HD, an end-to-end AI weather forecasting model designed to make predictions directly from observational data, including surface observations, radar, and satellite, thus bypassing the data assimilation step. OMG-HD provides kilometer-scale, 12-hour forecasts across the contiguous United States (CONUS) that exhibit greater skill than the leading operational NWP models. Compared to the High-Resolution Rapid Refresh (HRRR), we achieve a 13-48% improvement in RMSE for 2-meter temperature, 10-meter wind speed, 2-meter specific humidity, and surface pressure. These results demonstrate the feasibility of AI-driven end-to-end approaches for operational weather forecasting free of NWP data, offering a promising step towards faster and more accurate weather forecasts to support weather-dependent decision-making.

How to cite: Dong, H.: OMG-HD: A High-Resolution AI Weather Model for End-to-End Forecasts from Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4604, https://doi.org/10.5194/egusphere-egu25-4604, 2025.

EGU25-5156 | Posters on site | AS1.3

Ensemble Sensitivity Analysis in the Operational Met Office in the UK Ensemble System 

Brian Ancell, Steve Willington, Helen Titley, Caroline Jones, Brent Walker, Adrian Semple, Rebekah Hicks, Phil Relton, Rosa Barciela, Daniel Etheridge, and Nigel Roberts

The Met Office in the UK is exploring the use of ensemble sensitivity analysis (ESA) as an operational tool to support its upcoming focus on its global ensemble system. Ensemble sensitivity analysis is a technique that identifies atmospheric flow features throughout a forecast period that are relevant to high-impact forecast aspects such as high winds, heavy precipitation, and extreme temperatures (known as response functions). ESA typically highlights the importance of the position or magnitude of features like upper-level troughs, ridges, and wind maxima/minima in the jet stream, as well as structure in low-level pressure and moisture fields, to the response function. Since ESA also identifies specifically how features are associated with differences in high-impact response functions (e.g., an eastward shift of a 300hPa geopotential height trough off the U.S. east coast might be associated with heavier precipitation two days later in the UK), it can add substantial value to the forecasting process through forecaster awareness. This value can be realized through both improved dynamical understanding of high-impact flows and ensemble subsetting, a method that weights ensemble members more if they are more skillful in sensitive areas.

 

The Met Office in the UK has created a real-time ESA tool for initial evaluation to understand its value in the forecasting process. Wind, precipitation, temperature, and visibility response functions to seven-day forecast time over the UK, both coverage and maximum values, serve as the response functions. Sensitivities to geopotential height and wind speed aloft, surface pressure, and simulated water vapor imagery are produced every six hours from the response function backward to initial forecast time. This presentation involves what operational forecasters and research personnel have learned from day-to-day ensemble sensitivity fields, the use of ESA in the forecasting process, and the climatological nature of sensitivity. Future plans for the Met Office in the UK ESA tool will also be discussed.

How to cite: Ancell, B., Willington, S., Titley, H., Jones, C., Walker, B., Semple, A., Hicks, R., Relton, P., Barciela, R., Etheridge, D., and Roberts, N.: Ensemble Sensitivity Analysis in the Operational Met Office in the UK Ensemble System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5156, https://doi.org/10.5194/egusphere-egu25-5156, 2025.

The occurrence of severe weather events has shown increasing frequency and intensity due to global climate change. The Korean Peninsula, characterized by complex inland orography and surrounded by seas on three sides, exhibits diverse meteorological phenomena significantly influenced by seasonal wind regimes. While forecasters traditionally analyze synoptic conditions using locally available observations, the irregular spatial and temporal distribution of these observations limits their ability to conduct comprehensive three-dimensional analyses. Furthermore, although global model analysis fields have been widely used for operational forecasting, their coarse spatial and temporal resolutions constrain the real-time analysis of localized severe weather events. To address these limitations and enhance nowcasting capabilities, the Korea Meteorological Administration (KMA) has implemented the Korea Analysis System (KAS) since May 2024, a real-time analysis system that utilizes a high-resolution regional model to provide rapid updates of current atmospheric conditions essential for monitoring and predicting mesoscale weather phenomena.

This study evaluates KAS's effectiveness in reproducing real-time atmospheric phenomena and its practical utility for severe weather analysis through extensive synoptic case studies. KAS generates hourly three-dimensional nowcast analysis fields at 3 km resolution by integrating 15 categories of synoptic and non-synoptic observational data with the operational Korean Integrated Model-regional (KIM-regional) forecast fields, assimilating observations up to 15 minutes past each hour to provide near real-time atmospheric conditions. The system demonstrated remarkable capability in capturing critical meteorological features across various weather regimes. During summer, KAS effectively identified precursors of convective precipitation by analyzing real-time low-level convergence zones, dewpoint depression fields, high equivalent potential temperature areas, and vertical p-velocity distributions. The system's skew T-log P diagrams revealed significant Convective Available Potential Energy (CAPE) values, providing quantitative measures of atmospheric instability and potential for convective cloud development and subsequent precipitation in specific regions. In winter scenarios, KAS accurately depicted strong wind variations, including northwesterly cold air flows and easterly winds associated with orographic precipitation. Notably, the system's thermal advection analysis fields effectively identified regions of warm air advection and their interaction with cold air masses, providing crucial indicators for potential snowfall accumulation zones, particularly in areas where warm maritime air masses encounter pre-existing cold air.

The results validate KAS's capability to provide forecasters with coherent three-dimensional nowcast analyses, overcoming the limitations of traditional forecasting methods based on irregularly distributed observations and coarse-resolution global model analyses. This advancement establishes a foundation for improved real-time severe weather detection and forecast accuracy across the Korean Peninsula and East Asia region.

Acknowledgement: This work was supported by Development of Numerical Weather Prediction and Data Application Techniques (KMA2018-00721).

How to cite: Kim, M., Lee, E., Kang, Y., and Lee, Y.: A case study on synoptic analysis using the Korea Analysis System (KAS) to enhance severe weather monitoring over the Korean Peninsula, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5510, https://doi.org/10.5194/egusphere-egu25-5510, 2025.

Cold waves are one of the most frequent extreme weather events in the winter mid- and high-latitude regions of the Northern Hemisphere. Due to their sudden onset, persistence, and wide-ranging effects, they often cause significant economic and social losses. Although progress has been made in short-term cold wave forecasting, sub-seasonal (3-4 weeks) forecasting remains a major challenge due to the loss of initial condition information, and the complex and nonlinear external forcings. Current numerical models, which dominate operational cold wave forecasting, are computationally expensive and difficult to run large-scale simulations. In contrast, machine learning models, particularly FuXi-S2S developed by Fudan University, offer significant potential due to their efficiency and accuracy in sub-seasonal forecasting.

In the preliminary work, the researcher identified the spatiotemporal characteristics and circulation evolution of cold events in Eurasia, proposing the "Cold Arctic-Warm Continent" mode and its interaction with tropical Pacific signals. Despite improvements in understanding the mechanisms of cold waves, predicting their occurrence at the sub-seasonal scale remains difficult due to uncertainties and complex nonlinear processes. Therefore, exploring new machine learning-based forecasting methods is essential to improve prediction accuracy.

The goal of this study is to: 1) identify key pre-cold wave factors at the sub-seasonal scale in China; 2) develop a probabilistic forecasting scheme based on FuXi-S2S with physically constrained perturbations. The research methodology includes composite analysis and the design of initial perturbations for the FuXi-S2S model with physical constraints, aimed at improving forecast accuracy. By comparing ensemble and deterministic forecasts, this study will evaluate the effectiveness of the proposed scheme and contribute to early warning strategies for cold wave events.

How to cite: Liu, Q.: Research on Subseasonal Ensemble Forecasting of Cold Surges over China Based on Physically-Constrained Perturbations in AI-based Weather Prediction Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7063, https://doi.org/10.5194/egusphere-egu25-7063, 2025.

EGU25-7596 | ECS | Orals | AS1.3 | Highlight

WeatherReal: A Benchmark Based on In-Situ Observations for Evaluating Weather Models 

Weixin Jin, Jonathan Weyn, and Haiyu Dong

In recent years, AI-based weather forecasting models have matched or even outperformed numerical weather prediction systems. However, most of these models have been trained and evaluated on reanalysis datasets like ERA5. These datasets, being products of numerical models, often diverge substantially from actual observations in some crucial variables like near-surface temperature, wind, precipitation and clouds - parameters that hold significant public interest. To address this divergence, we introduce WeatherReal, a novel benchmark dataset for weather forecasting, derived from global near-surface in-situ observations. WeatherReal also features a publicly accessible quality control and evaluation framework. This paper details the sources and processing methodologies underlying the dataset, and further illustrates the advantage of in-situ observations in capturing hyper-local and extreme weather through comparative analyses and case studies. Using WeatherReal, we evaluated several data-driven models and compared them with leading numerical models. Our work aims to advance the AI-based weather forecasting research towards a more application-focused and operationready approach.

How to cite: Jin, W., Weyn, J., and Dong, H.: WeatherReal: A Benchmark Based on In-Situ Observations for Evaluating Weather Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7596, https://doi.org/10.5194/egusphere-egu25-7596, 2025.

EGU25-7652 | ECS | Orals | AS1.3

A hybrid deep learning and data assimilation method for model error estimation 

Ziyi Peng, Lili Lei, and Zhe-Min Tan

Forecast errors of numerical weather prediction consist of model errors and the growth of initial condition errors, while the initial condition is often optimized based on short-term forecasts. Thus it is difficult to untangle the initial condition error and model error, but it is essential to infer model errors not just for prediction but also for data assimilation (DA). A hybrid deep learning (DL) and DA method is proposed here, aiming to correct model errors. It uses a convolutional neural network (CNN) to extract characteristics of initial conditions and forecast errors, and then provides estimations for model errors. The CNN-based model error estimation method can consider the model error resulted from inaccurate model parameters, or simultaneously consider the model error and initial condition error. Based on the Lorenz05 model, offline and online experiments demonstrate that the CNN-based model error estimation method can effectively correct model errors resulted from inaccurate model parameters, including the forcing F, coupling coefficient c, and relative scale b. For both online and offline model error estimations, simultaneously considering model errors and initial condition errors are beneficial to infer the model errors, compared to considering model errors only. Moreover, using the observations to verify the forecasts has advantages over using the analyses, to estimate the model errors. Using observations can also achieve a faster convergence of model error estimation with online DA than using analyses.

How to cite: Peng, Z., Lei, L., and Tan, Z.-M.: A hybrid deep learning and data assimilation method for model error estimation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7652, https://doi.org/10.5194/egusphere-egu25-7652, 2025.

EGU25-7911 | Orals | AS1.3 | Highlight

A data-to-forecast machine learning system for global weather 

Xiuyu Sun

Operational numerical weather prediction (NWP) systems consist of three fundamental components: the global observing system for data collection, data assimilation (DA) for generating initial conditions (referred to as analysis), and the forecasting model to predict future weather conditions. While NWP have undergone a quiet revolution, with forecast skills progressively improving over the past few decades, their advancement has slowed due to challenges such as high computational costs and the complexities associated with assimilating an increasing volume of observational data and managing finer spatial grids. Advances in machine learning offer an alternative path towards more efficient and accurate weather forecasts. The rise of machine learning based weather forecasting models has also spurred the development of machine learning based DA models or even purely machine learning based weather forecasting systems. This paper introduces FuXi Weather, an end-to-end machine learning based weather forecasting system. FuXi Weather employs specialized data preprocessing and multi-modal data fusion techniques to integrate information from diverse sources under all-sky conditions, including microwave sounders from 3 polar-orbiting satellites and radio occultation data from Global Navigation Satellite System. Operating on a 6-hourly DA and forecasting cycle, FuXi Weather independently generates robust and accurate 10-day global weather forecasts at a spatial resolution of 0.25°. It surpasses the European Centre for Mediumrange Weather Forecasts (ECMWF) high-resolution forecasts (HRES) in terms of predictability, extending the skillful forecast lead times for several key weather variables such as the geopotential height at 500 hPa from 9.25 days to 9.5 days. The system’s high computational efficiency and robust performance, even with limited observations, demonstrates its potential as a promising alternative to traditional NWP systems.

How to cite: Sun, X.: A data-to-forecast machine learning system for global weather, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7911, https://doi.org/10.5194/egusphere-egu25-7911, 2025.

EGU25-11811 | Posters on site | AS1.3

Assimilation of water vapor lidar data from the WaLiNeAs experiment to decrease false positives and negatives in heavy precipitation forecasts 

Thomas Schwitalla, Diego Lange, Andreas Behrendt, Volker Wulfmeyer, Patrick Chazette, Paolo Di Girolamo, Jeremy Lagarrigue, Frédéric Laly, Marco Di Paolantonio, Donato Summa, and Julien Totems

Southern France is often affected by heavy-precipitation events (HPEs) leading to severe flooding in the regions of Occitanie, Provence-Alpes-Côte d'Azur, and Corsica. In many cases, these HPEs are triggered by a strong south-easterly moisture transport from the Mediterranean lower atmosphere (below 850 hPa). To date forecasting the magnitude and location of HPEs is challenging for numerical weather prediction models (NWP): forecasting false positive alarms as well as false negative HPEs need to be minimized. We hypothesize that an accurate distribution of water vapor is hypothesized to be a key for improvements.

During the WaLiNeAs experiment (Flamant et al., 2021), which took place in fall-winter of 2022, water-vapor measurements of eight Raman lidar systems were performed over Southern France, Spain and Corsica. From this unique data set, we use the data of the two lidar systems operated by the Universita della Basilicata (Toulon and Camargue), the lidar data from the Institut Pierre-Simon Laplace (IPSL) at Montpellier and the ARTHUS lidar system (Lange et al., 2019) operated by the University of Hohenheim on the island of Corsica (Ajaccio). The first three systems were aligned along the Coast with an average distance of 100 km between each other.

The water vapor lidar data applied in our simulation experiment were collected during a strong precipitation event between 14-16 November 2022. Observed rainfall near the coast was between 100 and 150 mm/24h, however over the sea extreme precipitation with up to 300 mm/24h was observed.

To investigate the impact of additionally assimilating water vapor data of the four lidar systems on the prediction of this challenging to forecast precipitation event, the Weather Research and Forecasting (WRF)-NOAHMP 3DEnVar system is used on a convection permitting resolution with 10 ensemble members. The assimilation follows the setup of Thundathil et al. (2021) with a rapid update cycle length of 42 h with hourly update intervals. The results show an analysis increment of up to 2 g/kg in the lowest 2000 m. We present further results of the spatial-temporal impact of the assimilation of the water-vapor lidar data on the analysis and the forecasts up to 24 h.

References

Flamant, C., et al. (2021): A network of water vapor Raman lidars for improving heavy precipitation forecasting in southern France: introducing the WaLiNeAs initiative. Bulletin of Atmospheric Science and Technology (2021) 2: 10. https://doi.org/10.1007/s42865-021-00037-6

Lange, D., Behrendt, A., & Wulfmeyer, V. (2019). Compact operational tropospheric water vapor and temperature Raman lidar with turbulence resolution. Geophysical Research Letters, 46, 14844–14853. https://doi.org/10.1029/2019GL085774

Thundathil, R., Schwitalla, T., Behrendt, A. & Wulfmeyer, V. (2021) Impact of assimilating lidar water vapour and temperature profiles with a hybrid ensemble transform Kalman filter: Three-dimensional variational analysis on the convection-permitting scale. Q J R Meteorol Soc, 147(741, 4163–4185. Available from: https://doi.org/10.1002/qj.4173

How to cite: Schwitalla, T., Lange, D., Behrendt, A., Wulfmeyer, V., Chazette, P., Di Girolamo, P., Lagarrigue, J., Laly, F., Di Paolantonio, M., Summa, D., and Totems, J.: Assimilation of water vapor lidar data from the WaLiNeAs experiment to decrease false positives and negatives in heavy precipitation forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11811, https://doi.org/10.5194/egusphere-egu25-11811, 2025.

EGU25-12662 | ECS | Orals | AS1.3 | Highlight

The PREVENIR rapid-update data assimilation and short-range numerical weather prediction system prototype: an urban flood case study over Buenos Aires.  

Paula Maldonado, Arata Amemiya, Maria Eugenia Dillon, Jorge Gacitua Gutierrez, Federico Cutraro, Gimena Casaretto, Juan Ruiz, Manuel Pulido, Yanina Garcia Skabar, and Takemasa Miyoshi

One of the most critical tools to mitigate the impact of urban flash floods is having an effective and timely early-warning system. The Argentine National Meteorological Service (SMN) is actively working in this direction through the PREVENIR Argentina-Japan cooperation project, which aims to develop an impact-based early-warning and emergency management system for urban flash floods in two Argentine target basins by 2027. As the current SMN operational system consists of 4-km resolution deterministic and warm-start probabilistic forecasts, to provide a more accurate and timely precipitation forecast, under PREVENIR, we are developing a higher-resolution (2-km), rapid-update data assimilation and numerical weather forecasting system coupling the Local Ensemble Transform Kalman Filter (LETKF) with the Weather Research and Forecasting (WRF) model. The system ingests local data from automated surface weather stations and C-band Doppler weather radars to obtain a 40-member analysis ensemble every 5 minutes, and 10-h 20-member extended forecasts every 30 minutes. This work aims to evaluate the performance of the WRF-LETKF prototype system based on a 4-day case study of almost continuous precipitation over the Buenos Aires region in March 2024, which led to urban floods in one of the pilot basins. A preliminary comparison with Radar Quantitative Precipitation Estimation (RQPE) indicates a good performance of the precipitation forecasts and added value for early warning and decision-making.

How to cite: Maldonado, P., Amemiya, A., Dillon, M. E., Gacitua Gutierrez, J., Cutraro, F., Casaretto, G., Ruiz, J., Pulido, M., Garcia Skabar, Y., and Miyoshi, T.: The PREVENIR rapid-update data assimilation and short-range numerical weather prediction system prototype: an urban flood case study over Buenos Aires. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12662, https://doi.org/10.5194/egusphere-egu25-12662, 2025.

EGU25-14520 | ECS | Posters on site | AS1.3 | Highlight

Variational Autoencoder-Enhanced Variational Methods for Data Assimilation 

Yi Xiao, Qilong Jia, Kun Chen, Wei Xue, and Lei Bai

Data assimilation (DA) is a statistical approach used to estimate the states of physical systems by integrating prior model predictions (background states xb​) with observational data (y). This integration produces an accurate estimate, called analysis states (​xa), by sampling or maximizing the posterior likelihood p(xxb, y). In weather forecasting, background states are generated by imperfect models, and the likelihood p(xxb) is often unknown. Observations, sourced from diverse instruments, are mapped to model space using observation operators (H). Effective DA algorithms must accurately estimate p(xxb) while accommodating various observation operators, including those involving sparse, noisy or irregular data.

Traditional DA methods, such as variational assimilation, assume that the background error (​x - xb) follows a Gaussian distribution independent of xb​. This allows explicit computation of p(xxb, y) and optimization via techniques like gradient descent. While robust to various observation operators, these methods depend heavily on expert knowledge to construct error correlations and are limited by their Gaussian assumptions.

Generative neural networks, particularly diffusion models, have emerged as alternatives for modeling p(xxb). Notable examples include SDA and DiffDA, which use diffusion models to learn background distributions. SDA incorporates observations via diffusion posterior sampling, while DiffDA employs the repaint technique. These approaches improve on traditional methods by capturing more complex distributions but often struggle with sparse, irregular observations. For instance, DiffDA assumes grid-aligned data, while SDA relies on assumptions that can reduce accuracy in real-world scenarios.

In this research, we aim to develop a neural network-based data assimilation algorithm that not only captures the non-Gaussian characteristics of the conditional background distribution for enhanced accuracy but also effectively assimilates data under real-world observations (sparse, noisy and outside of the grid). We introduce VAE-Var, a novel data assimilation algorithm in which a variational autoencoder is first employed to learn the conditional background distribution and then the decoder component is utilized to construct a variational cost function, which, when optimized, yields the analysis states.

Key advantages of VAE-Var include:

  • This algorithm inherits the framework of traditional variational assimilation by explicitly modeling the posterior probability function p(xxb, y) and maximizing it to derive the analysis states. As a result, compared to other neural network data assimilation methods such as SDA and DiffDA, VAE-Var can better handle different types of observation operators, particularly irregular observations that do not fall on the grid points of the physical field.
  • Unlike traditional variational assimilation algorithms, VAE-Var alleviates the dependence on expert knowledge for constructing the conditional background distribution, enabling the model to effectively capture non-Gaussian structures. This makes VAE-Var perform better in sparse observational settings.

Experiments with the FengWu weather forecasting system at 0.25° resolution show that VAE-Var achieves higher accuracy than DiffDA and traditional algorithms (interpolation and 3DVar) in sparse observational settings. When integrated with FengWu, VAE-Var reliably assimilates real-world GDAS prepbufr observations over a one-year period.

How to cite: Xiao, Y., Jia, Q., Chen, K., Xue, W., and Bai, L.: Variational Autoencoder-Enhanced Variational Methods for Data Assimilation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14520, https://doi.org/10.5194/egusphere-egu25-14520, 2025.

EGU25-14682 | Posters on site | AS1.3

Skillful Precipitation Nowcasting Based on Multi-scale fusion and Radar Observations 

Sheng Chen, Qiqiao Huang, and Jinkai Tan

Accurate and reliable precipitation nowcasting plays a critical role in disaster prevention and mitigation. The heavy precipitation forecast is a challenging task for most deep learning (DL)-based models. To address this challenge, we develop a novel DL architecture called “multi-scale feature fusion” (MFF) that can give skillful precipitation forecast with a lead time of up to 3 h. The MFF model uses convolution kernels with varying sizes to create multi-scale receptive fields. This helps to capture the movement features of precipitation systems, such as their shape, movement direction, and speed. Additionally, the architecture makes use of the mechanism of discrete probability to reduce uncertainties and forecast errors, enabling it to predict heavy precipitation even at longer lead times. Four-year radar observation data from 2018 to 2021 are used for model training, and the data of 2022 for model testing. The MFF model is compared with three existing extrapolative models: time series residual convolution (TSRC), optical flow (OF), and UNet. The results show that MFF achieves superior forecast skills with high probability of detection (POD), low false alarm rate (FAR), small mean absolute error (MAE), and high structural similarity index (SSIM). Particularly, MFF can predict high-intensity precipitation fields at 3 h lead time, while the other three models cannot. Furthermore, MFF shows improvement in the smoothing effect of the forecast field, as observed from the results of radially averaged power spectral (RAPS).   

How to cite: Chen, S., Huang, Q., and Tan, J.: Skillful Precipitation Nowcasting Based on Multi-scale fusion and Radar Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14682, https://doi.org/10.5194/egusphere-egu25-14682, 2025.

EGU25-14792 | ECS | Posters on site | AS1.3

Improved Model Prediction with Dual-polarimetric Radar Operator in Ensemble Data Assimilation 

Ji-Won Lee, Ki-Hong Min, and Gyuwon Lee

 Dual-polarimetric (dual-pol) radar variables, such as differential reflectivity (ZDR) and specific differential phase (KDP), provide valuable information about hydrometeor types, sizes, and water content. A dual-pol radar operator that applies scattering calculations using the T-matrix method for rain and the Rayleigh scattering approximation for snow and graupel can more accurately translate model variables into observed variables. Assimilating dual-pol radar variables in numerical weather prediction models enhances the forecast accuracy for evolving mesoscale precipitation events. Therefore, developing advanced radar observation operators capable of calculating dual-pol radar variables using microphysical variables is crucial.

In this study, an improved observation operator (K-DROP; KNU dual-pol radar observation operator) is developed. The K-DROP restricts the distribution of mixed-phase hydrometeors in regions with strong vertical motions, thereby reducing overestimation of radar variables near the melting layer. Additionally, by incorporating the observed snow axis ratios for cold rain process, the calculation of  as a constant value in subfreezing regions is corrected. Observed maximum hydrometeor radius data are also applied, reducing overestimations of  and in warm regions. Experiments using LETKF are conducted for both convective and stratiform precipitation cases and compared with the previous observation operator without modifications. While the previous operator improved forecast accuracy compared to control experiments without DA, it showed limited improvements near the melting layer due to reduced hydrometeor mixing ratios and increased downdrafts. In contrast, K-DROP produced more realistic radar variables, stronger updrafts, and higher correlations with observations. These improvements are particularly effective for convective precipitation with localized heavy rainfall, demonstrating the importance of assimilating dual-pol radar variables containing water content information.

Key words: Dual-polarization radar operator, Radar data assimilation, Observation operator, Precipitation forecasting.

Acknowledgments: This work was supported by the National Research Foundation (NRF) grant funded by the Korea government (MSIT) (No. 2022R1A2C1012361), the Korea Meteorological Administration Research and Development Program under Grant RS-2023-00237740 and the Brain Korea 21 program.

How to cite: Lee, J.-W., Min, K.-H., and Lee, G.: Improved Model Prediction with Dual-polarimetric Radar Operator in Ensemble Data Assimilation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14792, https://doi.org/10.5194/egusphere-egu25-14792, 2025.

El Niño-Southern Oscillation (ENSO) is the dominant atmosphere-ocean coupled mode of year-to-year variations in the tropical Pacific. It shows diverse spatiotemporal characteristics and casts major influences on seasonal predictions of global weather-climate extrema. Despite numerous dynamical and statistical models for ENSO prediction and predictability studies, they are commonly subjected to one-to-three issues among less skillful simulation of El Niño diversity, huge requirements of computational resources and a low robustness in statistics. Here, an efficient deep-learning model involving nonlinear coupling of multiple variables is independently developed to study the predictability of two types of El Niño events related to initial uncertainty, which is the first kind of predictability problem. The model can skillfully simulate statistically robust features of observed El Niño diversity in terms of periodicity, amplitude, and seasonal phase-locking. Using this model, we have revealed mathematically several new types of fastest-growing initial errors in two types of El Niño predictions based on a novel concept of conditional nonlinear optimal perturbation (CNOP), especially including one that can strengthen central Pacific types of events, which is rarely investigated before. Moreover, CNOPs are superimposed into a numerical model, GFDL CM2p1, for comprehensive validation and growth mechanism mining, which demonstrates the consistent dynamical evolutions of initial errors in both numerical and AI models. Our study represents the first attempt to explore the first kind of ENSO predictability problem from perspectives of nonlinear error evolving dynamics using a data-driven model. This is of great importance as it offers us sufficient confidence to perform ENSO-related (such as the Madden-Julian Oscillation, etc.) mechanisms and predictability studies for future data assimilations and observation programs without strongly relying on dynamical numerical models.

How to cite: Qin, B. and Mu, M.: The First Kind of Predictability Problem of El Niño Predictions in a Multivariate Coupled Data-driven Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14917, https://doi.org/10.5194/egusphere-egu25-14917, 2025.

In this paper, we explore the prevalent issue of underestimation of extreme precipitation values in deep learning models utilized for precipitation forecasting. We emphasize that this challenge arises from the double penalty phenomenon, which is exacerbated by the joint effect of the commonly adopted mean squared error (MSE) loss function and the intrinsic uncertainty of forecasting tasks. Drawing inspiration from probability-matching ensemble forecasting, we introduce Sort Loss, a straightforward yet highly effective deep learning loss function. By leveraging the ordinal relationships within meteorological data, Sort Loss circumvents the positional information-related double penalty problem. Experimental results from precipitation nowcasting and short-term forecasting tasks demonstrate that Sort Loss effectively diminishes the distributional discrepancies between model forecasts and actual observations. Consequently, it significantly enhances forecasting performance in heavy rainfall scenarios, while simultaneously maintaining stability across other weather conditions. This study offers a novel perspective on optimizing deep learning models for weather forecasting and showcases the potential of applying Sort Loss to improve the accuracy of extreme weather predictions.

How to cite: Cao, Y., Chen, L., and Feng, J.: Imroving Extreme Precipitation Prediction Accuracy: A Novel Probability-Matching-Based Loss Function for Deep Learning Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15517, https://doi.org/10.5194/egusphere-egu25-15517, 2025.

Data assimilation (DA) is the best tool for assessing the state of time-evolving chaotic systems. An estimate (analysis) is derived by combining Information from the most recent and previous batches of observations, the latter of which are carried forward by first guess forecasts started from previous analyses. Error variance in successful DA cycles fluctuate around an expected value. What factors determine this value?

Three parameters are found to describe the level of analysis error variance ( ), or the amount of Information in state estimates: the level of Information extracted from a recent set of observations by a DA system at analysis time ( ), the growth rate of error in the first guess ( ), and the relative weight used for combining Information from the latest set of observations and the first guess ( ). A key recognition of this study is that in DA systems with stationary performance, the gain of Information from the most recent observations, and the loss of Information due to chaotic error growth, in an expected sense, must be equal.

Exploiting this equilibrium relationship, error variance or Information in a state estimate can be expressed as a function of the three driving parameters. Analysis Information linearly and exponentially depend on  and alpha, respectively, while the optimal weight  is found to be a simple function of the rate of error growth. An evaluation of four operational DA systems reveals that their quality is driven by the amount of observational Information they each extract from the a virtually common set of globally available observations. The ECMWF analysis performs best, with two and a half times lower error variance than in any other system. A simple global adjustment of the relative weight between observations and the first guess may yield an 11-43% reduction in error variance.

How to cite: Feng, J.: An Equilibrium Between the Observational Gain and Chaotic Loss of Information, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20424, https://doi.org/10.5194/egusphere-egu25-20424, 2025.

EGU25-21364 | ECS | Orals | AS1.3 | Highlight

A Multi-Modal Observation-Driven Foundation Model for Global Data Assimilation 

Thomas Vandal, Kate Duffy, and Yoni Nachmany

Accurate characterization of meteorological conditions across urban regions is crucial for developing equitable energy and climate solutions. However, this task faces significant challenges: observational data often lacks spatial and temporal continuity, while numerical weather prediction models can struggle to localize severe weather events due to substantial latency between observation collection and forecast production. To address these challenges we introduce a multi-modal foundation model that rapidly integrates heterogeneous in situ and satellite data to produce a gap-filled global state. Our results show that the atmospheric structures predicted by our model are consistent with observed phenomena such as liquid and frozen precipitation and convection. Further, we apply our model to produce reanalysis and forecast datasets of solar irradiance for renewable energy applications. We also discuss ongoing work to connect global and local systems through a regional high-resolution foundation model, which is driven by multi-modal observations and the dynamics captured by the global model. This research aims to build predictive understanding of environmental systems and their interactions with built environments by improving our ability to forecast phenomena such as cold and warm fronts, convective weather, and their impacts on health, safety, and energy supply and demand.

How to cite: Vandal, T., Duffy, K., and Nachmany, Y.: A Multi-Modal Observation-Driven Foundation Model for Global Data Assimilation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21364, https://doi.org/10.5194/egusphere-egu25-21364, 2025.

EGU25-100 | Orals | AS1.4

Impacts of Assimilating GPS-PWV in Convective-permitting Model on Forecasting Monsoon Precipitation over Arizona Complex Terrain 

Christoforus Bayu Risanto, Avelino F. Arellano, Jr., Steven Koch, Christopher L. Castro, Samkeyat Shohan, and David K. Adams

Forecasting monsoon precipitation over Arizona is challenging due to its complex terrain since the model grid structure may misrepresent topographic details and the sparse observation network is insufficient for initialization of the model at the scale of the topography, particularly the spatial distribution of moisture. Our study aims to evaluate the monsoon precipitation forecast skill over Arizona by conducting an Observing System Experiment (OSE), or “data denial study” using the Data Assimilation Research Testbed (DART) to assimilate Global Positioning System precipitable water vapor (GPS-PWV) into the advanced version of the Weather Research and Forecast (WRF) model. The High-Resolution Rapid Refresh (HRRR) model is used as the initial and boundary conditions. The hourly GPS-PWV data were collected from 30 sites across Arizona characterized by a very nonuniform distribution with clusters of observations separated by large spatial gaps.

The precipitation event of interest occurred on 16 August 2021 with convective initiation developing over the Mogollon Rim in the afternoon and precipitation occurring over Flagstaff, Sedona, and Prescott as the increasingly well-organized mesoscale convective system propagated southwestward to the Arizona-California border. The amount of total precipitation recorded by NOAA’s MRMS (Multi Radar – Multi Sensor) system was 25 - 60 mm within the 12- hour period of 00 UTC 16 August to 12 UTC 16 August. In this study we initiated the forecast at 06 UTC 15 August with 40 ensemble members and assimilated the hourly GPS-PWV data over the 6h period from 1200-1800 UTC, after which we ran a deterministic forecast using the mean ensemble data assimilation analysis at 18 UTC as the initial condition for this “free forecast”.

We discovered that this forecast and assimilation system was sensitive to the specification of the initial state of the atmosphere, the radius of influence in the Ensemble Kalman Filter data assimilation system, and the model physics. Therefore, we tested the simulation using a variety of horizontal and vertical localizations and microphysics schemes to find a configuration resulting in the least-bias PWV. We used this optimal configuration to forecast 24 other precipitation events occurring in the 2021 monsoon season.

Our results show: 1) GPS-PWV data assimilation reduced forecast PWV errors across the model domain. 2) GPS-PWV data assimilation increased instability (due to moistening) of the pre-convective atmosphere over the Mogollon Rim and southeastern Arizona by as much as 1000 J/kg. 3) GPS-PWV data assimilation maintained these more favorable atmospheric conditions for convection and improved precipitation forecasts for at least 6 hours into the free forecast period but became too moist afterward. 4) The results revealed a surprising dry bias of 3-4 mm PWV in the HRRR model (used for initial conditions) compared to the actual GPS-PWV values, and this bias was maintained in the WRF model control run without GPS-PWV data assimilation for at least 18h. 

How to cite: Risanto, C. B., Arellano, Jr., A. F., Koch, S., Castro, C. L., Shohan, S., and Adams, D. K.: Impacts of Assimilating GPS-PWV in Convective-permitting Model on Forecasting Monsoon Precipitation over Arizona Complex Terrain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-100, https://doi.org/10.5194/egusphere-egu25-100, 2025.

EGU25-420 | ECS | Orals | AS1.4

A neural network-based observation operator for weather radar data assimilation 

Marco Stefanelli, Ziga Zaplotnik, and Gregor Skok

Forecasting convective storms is one of the most challenging tasks in Numerical Weather Prediction (NWP). Data Assimilation (DA) methods improve the initial condition and subsequent forecasts by combining observations and previous model forecasts (background). Weather radar provides a dense source of observations in storm monitoring. Therefore, assimilating radar data should significantly improve storm forecasting skills. However, extrapolating rainfall patterns (nowcasting) from radar data is often better than numerical model-based forecasting with DA in the first 2 or 3 hours (Fabry and Meunier, 2020). This is related to the fact that the radar data only provides information on the precipitation pattern and intensity in the area affected by the storm. Furthermore, it does not directly provide information on other variables that are strongly linked with the storm, such as temperature, wind, and humidity, either within the precipitation region or in the areas far from the storm. One potential solution to this problem is to use machine learning (ML) techniques to construct the DA observations operator to generate a model-equivalent of the radar data. In this approach, NWP model fields (temperature, wind components, relative humidity, precipitation) would serve as input, and radar observations would be the output of an encoder-decoder neural network. The constructed observation operator describes a non-linear relationship between the NWP model storm-related variables and radar observations, spreading radar information to other variables and potentially enhancing storm forecasting skills.

How to cite: Stefanelli, M., Zaplotnik, Z., and Skok, G.: A neural network-based observation operator for weather radar data assimilation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-420, https://doi.org/10.5194/egusphere-egu25-420, 2025.

EGU25-2686 | ECS | Posters on site | AS1.4

Validation of Rainfall Data Analysis Using Disdrometer Data Under Wet-Bulb Temperature Conditions 

Hyeon-Joon Kim, Sung-Ho Suh, Jongyun Byun, and Changhyun Jun

Abstract

To enhance the accuracy of rainfall estimation using remote sensing data, such as radar and satellite, it is crucial to improve the accuracy of the estimation relationships. Rainfall estimation is influenced by various factors, including rainfall type, geographical characteristics (e.g., inland and oceanic rainfall), and orographic rainfall features. Developing estimation formulas that account for variations in rainfall characteristics based on topography (elevation) and seasonal temperature changes is essential. Ensuring the reliability of observation data used in deriving these formulas is a top priority for achieving accurate rainfall estimation. This study evaluates the effectiveness of utilizing rain gauge data under varying wet-bulb temperature conditions to improve the reliability of rainfall analysis. The analysis employed disdrometer data collected over five years (2020–2024), applying channel-based particle diameter information and number concentration-based variable calculation methods to enhance the generalizability of the findings. Quantitative comparisons of rain gauge observation accuracy under different wet-bulb temperature conditions were conducted, alongside an analysis of the temperature ranges in which two types of rain gauges (tipping-bucket and weighing gauges) could be effectively utilized. Furthermore, we assessed the quality management of rain gauge data preprocessing for raindrops across various temperature conditions. The results indicate that when the wet-bulb temperature exceeded 2°C, the difference (RMSE) in rainfall between disdrometer and rain gauge observation data was less than 0.2 mm. However, this difference increased significantly to over 0.4 mm when the wet-bulb temperature was below 2°C, with particularly large differences exceeding 1.0 mm when disdrometer data were not preprocessed. These discrepancies reflect variations in hydrometeor characteristics and particle fall velocities due to temperature changes. This study underscores the necessity of establishing meteorological conditions for rainfall analysis.

 

Keywords: Disdrometer, Wet-bulb temperature, Long-term observation, Hydrometeor

 

Acknowledgement

This research was supported by Basic Science Research Program through the National Research Foundation of Korea(NRF) funded by the Ministry of Education (RS-2022-NR071182).

How to cite: Kim, H.-J., Suh, S.-H., Byun, J., and Jun, C.: Validation of Rainfall Data Analysis Using Disdrometer Data Under Wet-Bulb Temperature Conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2686, https://doi.org/10.5194/egusphere-egu25-2686, 2025.

In the wake of the continuous expansion and refinement of the ground automatic meteorological observation network in China, the development of an effective quality control system for ground automatic station observation data has become an urgent task of great significance in the field of meteorology. Although extensive research has been conducted on quality control techniques for traditional ground observation meteorological variables such as precipitation, temperature, and pressure both domestically and abroad, the exploration of quality control strategies for precipitation phase observation data remains relatively limited.This research endeavor undertakes the utilization of upper-air and manual ground observation datasets covering the period from 2000 to 2014. Through a comprehensive analysis and selection process, meteorological factors that exert a pronounced influence on precipitation phase are identified and optimized. Subsequently, the random forest algorithm is applied to establish a quality control model for the automatic observation data of three primary precipitation phases: rain, snow, and sleet. Employing this meticulously constructed quality control model, an in-depth quality assessment is carried out on the ground automatic precipitation phase observation data collected during the period from 2015 to 2023, after the discontinuation of manual observations. A total of 15,806 station-records are flagged as suspicious or incorrect. It is observed that the stations with such data anomalies are preponderantly located in regions with sparse human habitation and challenging maintenance conditions, such as the Qinghai-Tibet Plateau, the Tianshan Mountains, and the mountainous areas in northern Heilongjiang. In contrast, regions like Guangdong, Guangxi, Yunnan, Fujian, and Hainan exhibit relatively high data quality, with the eastern regions generally outperforming the western ones (Figure 1).For the identified suspicious data, a rigorous manual verification procedure is implemented. For example, at 14:00 on January 31, 2019, the quality control results for Wuqia, Akto, and Kashgar stations in Xinjiang indicated snowfall, yet the automatic observations registered precipitation. With the ground temperatures of these stations being -10°C, -6°C, and -6°C respectively, it is meteorologically implausible for rain to occur in Xinjiang during winter. Hence, the automatic precipitation observations at these stations are deemed incorrect. After conducting a substantial amount of manual verification on other suspicious and incorrect data, it is determined that the identification accuracy rate of this quality control method surpasses 98.5%. Presently, this research outcome has been successfully incorporated into the operational quality control framework for ground automatic precipitation phase observation.

Figure 1 Frequency Diagram of Stations with Suspected or Incorrect Precipitation Phase Quality Control from 2015 to 2023

 

How to cite: Ou, X., Lin, H., and Huang, X.: Research on Quality Control Methodology of Automatic Precipitation Phase Observation Data Based on Machine Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3384, https://doi.org/10.5194/egusphere-egu25-3384, 2025.

Variational data assimilation theoretically assumes Gaussian-distributed observational errors, yet actual data often deviates from this assumption. Traditional quality control methods have limitations when dealing with nonlinear and non-Gaussian-distributed data. To address this issue, our study innovatively applies two advanced machine learning (ML) based quality control (QC) methods, Minimum Covariance Determinant (MCD), and Isolation Forest to process precipitable water (PW) data derived from satellite FengYun-2E (FY2E). We assimilated the ML QC-processed TPW data using the Gridpoint Statistical Interpolation (GSI) system and evaluated its impact on heavy precipitation forecasts with the Weather Research and Forecasting (WRF) v4.2 model. Both methods notably enhanced data quality, leading to more Gaussian-like distributions and marked improvements in the model’s simulation of precipitation intensity, spatial distribution, and large-scale circulation structures. During key precipitation phases, the Fraction Skill Score (FSS) for moderate to heavy rainfall generally increased to above 0.4. Quantitative analysis showed that both methods substantially reduced Root Mean Square Error (RMSE) and bias in precipitation forecasting, with the MCD method achieving RMSE reductions of up to 58% in early forecast hours. Notably, the MCD method improved forecasts of heavy and extremely heavy rainfall, whereas the Isolation Forest method demonstrated superior performance in predicting moderate to heavy rainfall intensities. This research not only provides a basis for method selection in forecasting various precipitation intensities, but also offers an innovative solution for enhancing the accuracy of extreme weather event predictions.

How to cite: Shen, W., Chen, S., Xu, J., Zhang, Y., Liang, X., and Zhang, Y.: Enhancing Extreme Precipitation Forecasts through Machine Learning Quality Control of Precipitable Water Data from Satellite FengYun-2E: A Comparative Study of Minimum Covariance Determinant and Isolation Forest Methods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3931, https://doi.org/10.5194/egusphere-egu25-3931, 2025.

EGU25-4163 | ECS | Posters on site | AS1.4

Direct assimilation of  dual-polarization radar data in the idealized setup 

Tatsiana Bardachova, Maryam Ramezani Ziarani, and Tijana Janjic

The accuracy of numerical weather prediction models is highly dependent on the precision of the initial conditions, especially for forecasting storms and convective-scale weather events. Radars, with their ability to capture the internal structure and important microphysical and dynamical processes within convective systems, play a crucial role in improving weather forecasts at convective scales. Unlike conventional single-polarization radar, dual-polarization radar additionally provides information on the types and sizes of hydrometeor particles. As a result, polarimetric radar data (PRD) is a valuable data source for data assimilation (DA). Despite its potential, PRD is not yet directly assimilated into operational convection-permitting numerical models. This limitation arises from several challenges, including the highly non-linear nature of observation operators for polarimetric variables and the difficulty of estimating model error at convective scales, which require further research.

Our study primarily aims to directly assimilate PRD within an idealized setup. To accomplish this, Observation System Simulation Experiments (OSSEs) were conducted to simulate the evolution of a long-lived supercell using the ICOsahedral Nonhydrostatic (ICON) model with a two-moment microphysics scheme. For the assimilation of PRD data, the Kilometer-scale Ensemble Data Assimilation (KENDA) system was utilized, which incorporates the Local Ensemble Transform Kalman Filter (LETKF), along with the polarimetric radar forward operator EMVORADO-POL developed at the Deutscher Wetterdienst (DWD). In the current idealized setup, two types of DA experiments were conducted: a reference experiment that assimilated only non-polarimetric variables, such as reflectivity and radial velocity, and an experiment that assimilated differential reflectivity (ZDR) in addition to the non-polarimetric variables. The results from both experiments were compared, and appropriate thresholds and equivalents of noreflectivity data for polarimetric data were examined. Additionally, the sensitivity to DA settings, such as localization radius and the number of ensemble members, was also tested.

How to cite: Bardachova, T., Ramezani Ziarani, M., and Janjic, T.: Direct assimilation of  dual-polarization radar data in the idealized setup, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4163, https://doi.org/10.5194/egusphere-egu25-4163, 2025.

EGU25-4313 | ECS | Posters on site | AS1.4

Enhancing Tropical Weather Forecasts with Constrained Data Assimilation 

Maryam Ramezani Ziarani, Yvonne Ruckstuhl, and Tijana Janjic

Forecasting precipitation in tropical regions is challenging because of substantial errors in both the models and the initial conditions. The interaction between tropical waves and convection suggests possible predictability. Therefore, an accurate representation of these waves in the models and initial conditions is important for increasing the accuracy of precipitation forecasts. This study intends to improve the predictive reliability of the ICON (Icosahedral Nonhydrostatic) global model for tropical weather events, such as tropical waves and the Madden-Julian Oscillation (MJO). We initially analyze the ability of data assimilation (DA) to conserve total energy, enstrophy, moist static energy, and other physical properties. Then, we implement an advanced DA technique, the Quadratic Programming Ensemble (QPEns), with a moist static energy constraint. Preliminary findings show that the moist static energy constraint, together with accurate wind and humidity data, decreases forecast errors and improves tropical wave representation. This induces more reliable long-term precipitation forecasts.

How to cite: Ramezani Ziarani, M., Ruckstuhl, Y., and Janjic, T.: Enhancing Tropical Weather Forecasts with Constrained Data Assimilation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4313, https://doi.org/10.5194/egusphere-egu25-4313, 2025.

This research investigates the dynamics of the Sea Breeze Front (SBF) in the southwestern Caspian Sea, specifically focusing on Bandar Anzali, Iran. Utilizing two years of observational data alongside Weather Research and Forecasting (WRF) model simulations, the study examines the meteorological characteristics and behaviors associated with SBF events. SBF days were identified by analyzing land-sea temperature contrasts, supported by wind shifts, temperature decreases, increases in humidity, and cloud formation.

In-depth analysis reveals consistent atmospheric patterns during SBF events, such as temperature variations and notable wind shifts. The intensity of the land-sea thermal contrast is influenced by both local topography and atmospheric stability. A detailed case study of March 4, 2022, highlighted key meteorological changes, including temperature drops and wind direction shifts. While the WRF model accurately captured temperature and pressure variations, it slightly underestimated humidity and dew point.

Machine learning techniques, particularly K-means clustering, were employed to classify distinct atmospheric regimes linked to SBF occurrences. The clustering analysis identified two primary atmospheric patterns: cold, humid air masses favorable to SBF development, emphasizing the significant role of land-sea temperature gradients and local wind dynamics.

This study highlights the value of combining observational data, numerical simulations, and machine learning techniques to better understand coastal mesoscale processes. The findings provide fresh insights into SBF behavior in the Caspian region, with implications for enhancing coastal weather forecasting and management. Future work should focus on improving the accuracy of WRF model simulations and further examining the impact of regional topography on SBF dynamics.

 

 

Keywords: Sea Breeze Front, Machine Learning, WRF, K-means Clustering, Temperature Gradient, Caspian Sea,.

 

 

How to cite: Sepehri, J.: Exploring the Dynamics of Sea Breeze Fronts in the Southwestern Caspian Sea: Analysis Using Observational Data, WRF Simulations, and Machine Learning Approaches, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7413, https://doi.org/10.5194/egusphere-egu25-7413, 2025.

EGU25-7546 | Orals | AS1.4

Investigations of Tropical Cyclone Thermodynamic Structure using NASA TROPICS Observations 

William Blackwell and the TROPICS Science Team

New constellations to provide high-resolution atmospheric observations from microwave sounders operating in low-earth orbit are now coming online and are demonstrating the potential to provide operationally useful data. The first of these missions, the NASA TROPICS (Time-Resolved Observations of Precipitation structure and storm Intensity with a Constellation of Smallsats) Earth Venture (EVI-3) mission, was successfully launched into orbit on May 8 and May 25, 2023 (two CubeSats in each of the two launches).  TROPICS is now providing nearly all-weather observations of 3-D temperature and humidity, as well as cloud ice and precipitation horizontal structure, at high temporal resolution to conduct high-value science investigations of tropical cyclones. TROPICS is providing rapid-refresh microwave measurements (median refresh rate of better than 60 minutes early in the mission with four functional CubeSats, and now approximately 70-90 minutes with three functional CubeSats) over the tropics that can be used to observe the thermodynamics of the troposphere and precipitation structure for storm systems at the mesoscale and synoptic scale over the entire storm lifecycle. Hundreds of high-resolution images of tropical cyclones have been captured thus far by the TROPICS mission, revealing detailed structure of the eyewall and surrounding rain bands.  The new 205-GHz channel in particular (together with a traditional channel near 92 GHz) is providing new information on the inner storm structure, and, coupled with the relatively frequent revisit and low downlink latency, is already informing tropical cyclone analysis at operational centers.  A neural network algorithm to retrieve the atmospheric temperature and moisture vertical profiles has recently been developed and validated, with retrieval uncertainties approaching those of state-of-the-art microwave sounders, but with much better revisit rate. In this presentation, we highlight the use of these high-revisit thermodynamic data from TROPICS to better characterize storm structure and environmental conditions over a variety of cases over the nearly two-year mission lifetime to date.

How to cite: Blackwell, W. and the TROPICS Science Team: Investigations of Tropical Cyclone Thermodynamic Structure using NASA TROPICS Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7546, https://doi.org/10.5194/egusphere-egu25-7546, 2025.

EGU25-8227 | Orals | AS1.4

Study on representation error of radar data in convective scale data assimilation 

Yuefei Zeng, Alberto de Lozar, Yuxuan Feng, Ulrich Blahak, Kobra Khosravianghadikolaei, and Tijana Janjic

 The current study utilizes the operational data assimilation system of Deutscher Wetterdienst (DWD) to investigate the impacts of improved radar forward operator. First of all, it is shown that for experiments in which both conventional and radar data are assimilated and the latent heat nudging (LHN) is applied, the one with improved operator (i.e., with improved Mie-scattering scheme and accounting for beam broadening effect and etc.) exhibits neutral impacts on short-term forecasts. However, in subsequent experiments, in which conventional data are not assimilated and the LHN is switched off, the one with improved operator not just reduces representation error during data assimilation cycles but also enhances the short-term forecast skills. In addition, it is found that the subsequent experiments result in much shorter observation error correlation length scales for radar reflectivity data, indicating that the application of the LHN or assimilation of conventional data may increase the length scales. 

How to cite: Zeng, Y., de Lozar, A., Feng, Y., Blahak, U., Khosravianghadikolaei, K., and Janjic, T.: Study on representation error of radar data in convective scale data assimilation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8227, https://doi.org/10.5194/egusphere-egu25-8227, 2025.

EGU25-10275 | ECS | Posters on site | AS1.4

Dealing with unresolved scales of motion and systematic errors in the assimilation of cloud-affected satellite radiances 

Lukas Kugler, Stefano Serafin, and Martin Weissmann

Hydrometeor formation and cloud processes occur at very small spatial scales and cannot be explicitly resolved on the numerical grids of weather prediction models. Parameterizations of these processes are a necessary component of forecast models and are known to be a major source of forecast error. Two main challenges arise. First, the mismatch between the effective resolution of prediction models and the resolution of satellite observations leads to representativeness errors. Second, sub-optimal parameterizations induce systematic errors in hydrometeor fields and cloud properties. In the presence of such model biases, the assimilation of cloud-scale observations can be detrimental to the analysis. It remains an open question how to properly account for the scale mismatch and for systematic errors when assimilating small-scale observations into a larger-scale numerical model.

In this work, we compare different approaches for assimilating radiance observations that contain unresolved scales, such as data thinning, use of superobservations, and a multi-scale decomposition of the two-dimensional cloud field. We study the problem using observing system simulation experiments (OSSEs) performed with the WRF model and the DART EAKF assimilation system. The nature run is a high-resolution large eddy simulation (dx=250 m) of deep moist convection developing in moderate wind shear, which supports organization into multicell storms. Synthetic satellite imagery is computed from the nature run using operators available through RTTOV. Several 40-member km-scale ensemble experiments (dx=2 km) evaluate the impact of assimilating thinned, averaged, or multi-scale radiance observations.

How to cite: Kugler, L., Serafin, S., and Weissmann, M.: Dealing with unresolved scales of motion and systematic errors in the assimilation of cloud-affected satellite radiances, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10275, https://doi.org/10.5194/egusphere-egu25-10275, 2025.

EGU25-10874 | Orals | AS1.4

Assimilating multi-platform observations to improve severe convection forecasting in the ICON model 

Marcello Grenzi, Thomas Gastaldo, Virginia Poli, Chiara Marsigli, Tijana Janjic, Carlo Cacciamani, and Alberto Carrassi

Accurate representation of atmospheric dynamics at convection scale still represents a major challenge for numerical models and a critical aspect in operational weather predictions. Reliable forecast initial conditions, generated by the data assimilation cycle using new observations coming from different platforms, are crucial to improve the forecast accuracy in deep convection environments. In this work, the ICOsahedral Non-hydrostatic (ICON) model is run at convection-permitting scale over the Italian domain, in combination with the Kilometre-scale Ensemble Data Assimilation (KENDA) system, to test the model performance on a poorly-predicted extreme convective storm in the Marche region, Italy, on 15 September 2022. We show here the positive impact of data assimilation at convection scale on the forecast of this event, which allows to improve the localization and the intensity of the storm although substantial underestimation of precipitation still persists. The relative impact of different observations datasets is evaluated, starting from conventional and radar data operationally assimilated for numerical weather predictions over Italy. After pointing out the importance of low-level moisture convergence in the process of convection initiation and the significant undersampling of humidity field in conventional data, the added value of humidity-sensitive microwave radiances from polar satellites is analyzed. Observations sensitive to mid-lower tropospheric humidity in clear-sky conditions are employed, taken from the Microwave Humidity Sounder instrument, still little investigated in limited-area models at many numerical weather prediction centers. In order to better exploit the information content of microwave satellite observations, the preliminary development towards all-sky assimilation is presented.

How to cite: Grenzi, M., Gastaldo, T., Poli, V., Marsigli, C., Janjic, T., Cacciamani, C., and Carrassi, A.: Assimilating multi-platform observations to improve severe convection forecasting in the ICON model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10874, https://doi.org/10.5194/egusphere-egu25-10874, 2025.

EGU25-10945 | Orals | AS1.4

Diffusion Model Data Assimilation of Sparse Weather Station Observations at Kilometer Scales 

Peter Manshausen, Yair Cohen, Jaideep Pathak, Mike Pritchard, Piyush Garg, Morteza Mardani, Karthik Kashinath, Simon Byrne, and Noah Brenowitz

Data assimilation of observational data into full atmospheric states is essential for weather forecast model initialization. Recently, methods for deep generative data assimilation have been proposed which allow for using new input data without retraining the model. They could also dramatically accelerate the costly data assimilation process used in operational regional weather models. Here, in a central US testbed, we demonstrate the viability of score-based data assimilation in the context of realistically complex km-scale weather. We train an unconditional diffusion model to generate snapshots of a state-of-the-art km-scale analysis product, the High Resolution Rapid Refresh. Then, using score-based data assimilation to incorporate sparse weather station data, the model produces maps of precipitation and surface winds. The generated fields display physically plausible structures, such as gust fronts, and sensitivity tests confirm learnt physics through multivariate relationships. Preliminary skill analysis shows the approach already outperforms a naive baseline of the High-Resolution Rapid Refresh system itself. By incorporating observations from 40 weather stations, 10% lower RMSEs on left-out stations are attained. Despite some lingering imperfections such as insufficiently disperse ensemble DA estimates, we find the results overall an encouraging proof of concept, and the first at km-scale. It is a ripe time to explore extensions that combine increasingly ambitious regional state generators with an increasing set of in situ, ground-based, and satellite remote sensing data streams.

How to cite: Manshausen, P., Cohen, Y., Pathak, J., Pritchard, M., Garg, P., Mardani, M., Kashinath, K., Byrne, S., and Brenowitz, N.: Diffusion Model Data Assimilation of Sparse Weather Station Observations at Kilometer Scales, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10945, https://doi.org/10.5194/egusphere-egu25-10945, 2025.

EGU25-11180 | ECS | Posters on site | AS1.4

Comparison of Hybrid-3DEnVar against 3DVar for the assimilation of surface observations over the Alpine terrain in AROME-Austria 

Kaushambi Jyoti, Philipp Griewank, Florian Meier, and Martin Weissmann

Surface observations can provide crucial information for NWP models. If not assimilated carefully, however, they can degrade forecast accuracy, especially in complex terrains like the Alps. The horizontal and vertical covariances of climatological background error covariances used in the three-dimensional variational (3DVar) data assimilation (DA) method can produce unrealistic increments over sloped terrain. For instance, an observation from a valley station can still generate increments at the mountaintop, even though the valley observation may not accurately represent the mountaintop's weather conditions. 
We used a hybrid three-dimensional ensemble variational (Hybrid-3DEnVar) DA method to address this issue, incorporating a 50-member convection-permitting ensemble. This method was recently tested in Geosphere Austria's convective scale limited-area NWP model AROME at a 2.5 km horizontal resolution. We assimilated 2-meter temperature, 2-meter relative humidity, geopotential, and 10-meter wind components from 680 surface stations, including the Austrian TAWES network and SYNOP observations from neighbouring countries. 400 stations were actively assimilated from the observation dataset, and the rest were used to verify the analysis.  
Our results present the effectiveness of this newly tested Hybrid-3DEnVar against GeoSphere Austria's operational 3DVar in assimilating surface observations over complex Alpine terrain.

How to cite: Jyoti, K., Griewank, P., Meier, F., and Weissmann, M.: Comparison of Hybrid-3DEnVar against 3DVar for the assimilation of surface observations over the Alpine terrain in AROME-Austria, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11180, https://doi.org/10.5194/egusphere-egu25-11180, 2025.

EGU25-12280 | Orals | AS1.4

Convective-scale ensemble data assimilation using unstructured meshes 

Soyoung Ha and Jun Park

In an effort to enhance storm-scale data assimilation and prediction, we have recently updated the atmospheric Model for Prediction Across Scales (MPAS-A; Skamarock et al. 2012), coupled to the Ensemble Kalman Filter (EnKF) Data Assimilation Research Testbed (DART) system (Ha et al., 2017), for regional analysis using variable-resolution capabilities. In this talk, we will introduce unique features of the interface, leveraging the model's native coordinate both horizontally (e.g., unstructured meshes) and vertically (e.g., terrain-following height), and demonstrate its suitability for storm-scale DA. As its robustness was demonstrated in the U. S. National Severe Storms Laboratory (NSSL)'s Warn-On-Forecast framework during tornado watches in 2024, the performance of regional ensemble analysis incorporating storm-scale data assimilation using radars and cloud water path from the GOES-R satellite will be presented.

How to cite: Ha, S. and Park, J.: Convective-scale ensemble data assimilation using unstructured meshes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12280, https://doi.org/10.5194/egusphere-egu25-12280, 2025.

EGU25-12711 | ECS | Posters on site | AS1.4

Evaluation of visible satellite images from AROME-Austria as preparation for assimilating visible observations 

Sandy Chkeir, Philipp Griewank, Leonhard Scheck, Florian Meier, Christoph Wittmann, and Martin Weissmann

Assimilating visible satellite observations has become an increasingly active research topic and has been shown to provide valuable information for improving weather forecasts. The assimilation of these observations, however, is challenging due to operator deficiencies and model deficiencies in the representation of clouds. Our work focuses on evaluating the potential of the RTTOV observation operator to simulate visible satellite images in the convection-permitting AROME-Austria model, which is operational at Geosphere Austria. Specifically, we examine the systematic deviations caused by operator and model errors in all-sky conditions. In cloudy conditions, we build on findings from preceding studies and conduct sensitivity tests to evaluate model equivalents with modified operator settings. In clear-sky conditions, we aim to evaluate and mitigate the systematic deviations caused by orographic shadowing and high-albedo surfaces with the help of an advanced visible operator developed by DWD. A summer month of 3-hourly forecasts from 6 UTC to 18 UTC provides the basis for this analysis. Our findings aim to address operator deficiencies and model inconsistencies, laying the groundwork for integrating visible observations as a new observation type into the AROME-Austria model.

How to cite: Chkeir, S., Griewank, P., Scheck, L., Meier, F., Wittmann, C., and Weissmann, M.: Evaluation of visible satellite images from AROME-Austria as preparation for assimilating visible observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12711, https://doi.org/10.5194/egusphere-egu25-12711, 2025.

EGU25-12910 | ECS | Posters on site | AS1.4

Tempered local ensemble transform kalmann filter: simple model experiments 

Jorge Gacitua Gutierrez, Juan Jose Ruiz, Manuel Pulido, Maria Eugenia Dillon, Yanina García Skabar, Paula Maldonado, Shigenori Otsuka, Arata Amemiya, Takemasa Miyoshi, and Renato Pajarola

Extreme weather events associated with deep moist convection pose significant social risks, requiring advanced technologies for anticipatory measures. Numerical forecasting, particularly at convection-resolving scales, relies heavily on high-quality initial conditions obtained through the assimilation of complex remote-sensing-based observations. Integrating these observations into assimilation systems presents challenges due to the nonlinear relationships between observed quantities and model variables. This research explores an iterative implementation of the Local Ensemble Transform Kalman Filter based on the tempering of the observation likelihood (tempered LETKF), which can partially handle these non-linearities.

In this work, we use an N-variable Lorenz model for its simplicity and low computational cost to evaluate the performance of the method against the traditional implementation of the LETKF. We conducted comparisons under various levels of uncertainty concerning both the model and the observations. Additionally, we tested the behavior of the system for different ensemble sizes and for varying degrees of tempering. The initial findings show notable enhancements in the estimation of initial conditions and the stability of the data assimilation cycle, indicating potential benefits in more realistic model applications. The encouraging results motivate further research on tempering methods in mesoscale modeling systems, especially for predicting severe weather events linked to deep moist convection.

How to cite: Gacitua Gutierrez, J., Ruiz, J. J., Pulido, M., Dillon, M. E., García Skabar, Y., Maldonado, P., Otsuka, S., Amemiya, A., Miyoshi, T., and Pajarola, R.: Tempered local ensemble transform kalmann filter: simple model experiments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12910, https://doi.org/10.5194/egusphere-egu25-12910, 2025.

EGU25-16093 | Posters on site | AS1.4

Sensitivity of convection to environment within local neighborhoods 

Tomislava Vukicevic, Sai Prasanth, Ziad Haddad, Derek Posselt, and Svetla Hristova-Veleva

This study investigates sensitivity of convection to coincident atmospheric environment at meso-gamma spatial scales. The data used for the study comprise a large ensemble of three-dimensional high-resolution local domains that were extracted from cloud-resolving model simulations of different cases of subtropical and tropical convection over land and ocean.  The simulations were produces as part of the NASA (National Aeronautics and Space Administration) INCUS (Investigation of Convective Updrafts) mission (van den Heever, 2021). The simulations include a diverse set of convective morphologies associated with different synoptic environments (Marinesku et al., 2024 ).  Each neighborhood domain of dimensions 25.6 x 25.6 x 18 km, respectively in latitudinal, longitudinal and vertical direction, is centered on a deep convection core vertical profile that was selected for tracking convective cloud evolutions for the purpose of investigations within the INCUS mission  (Sokolowsky et al. 2024 ). The ensemble of neighborhoods used in this study therefore represent a distribution of local convective states and the associated environments embedded in a wide range of larger scales environments. 

To capture relationships between convection and environment states over a range of spatial scales contained within the neighborhoods in a concise manner, the analysis was performed in a phase space of two-dimensional horizontal scales spectral powers that are associated with leading vertical principal components of the physical variables representing the convection and environment. The convection state  was represented by vertical velocity and total condensate, and the environment by temperature, humidity, divergence and vorticity. 

The main finding is that the variability of vertical velocity and total condensate states at the convective scales (< 10 km)  exhibits high insensitivity to the variability of the neighborhood domain average environment states.   In contrast, notable co-variance was found between the vertical velocity and environment states at the convective scales, especially with the temperature mid-to-upper tropospheric warming variability and the variability of divergence in mid-troposphere and above 10 km.  For the total condensate, significant co-variance was exhibited also between its neighborhood domain average and the the convection scale environment.  This relationship reflects impact of the convective processed on the environment states including coupling between the convection dynamics and microphysics.

In the context of convective scale data assimilation the findings suggest that for representation of the convection state variability at the convective scales would be weekly constrained  in the absence of convective scale observations of the environment states. 

References

Marinescu, P.J., van den Heever, S.C., Grant, L.D., Bukowski, J. and Singh, I., 2024. How Much Convective Environment Subgrid Spatial Variability Is Missing Within Atmospheric Reanalysis Data Sets?. Geophysical Research Letters, 51(24), p.e2024GL111856.

Sokolowsky, G.A., Freeman, S.W., Jones, W.K., Kukulies, J., Senf, F., Marinescu, P.J., Heikenfeld, M., Brunner, K.N., Bruning, E.C., Collis, S.M. and Jackson, R.C., 2024. tobac v1. 5: introducing fast 3D tracking, splits and mergers, and other enhancements for identifying and analysing meteorological phenomena. Geoscientific Model Development, 17(13), pp.5309-5330.

van den Heever, S. C. (2021). NASA selects new mission to study storms, impacts on climate models. NASA Earth (https://www.nasa.gov/press‐release/nasa‐selects‐new‐mission‐to‐study‐storms‐impacts‐on‐climate‐models)

 

How to cite: Vukicevic, T., Prasanth, S., Haddad, Z., Posselt, D., and Hristova-Veleva, S.: Sensitivity of convection to environment within local neighborhoods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16093, https://doi.org/10.5194/egusphere-egu25-16093, 2025.

EGU25-16990 | Posters on site | AS1.4

Optimal vertical localization for the assimilation of cloud-affected satellite observations 

Philipp Griewank, Martin Parker, Tobias Necker, Takemasa Miyoshi, Annika Schomburg, Theresa Diefenbach, and Martin Weissmann

Localization is essential for any ensemble-based data-assimilation system for numerical weather prediction, and most localization approaches are distance-based. For example, in the observation-space localization used by the Deutscher Wetterdienst (DWD), the localization is a function of the distance between a model grid point and an observation location. Observation-space localization for satellite observations is especially challenging because they do not have a constant or well-defined observation location. Instead, the observed signal may originate from various vertical levels and is affected by the presence of clouds. We derive an optimal localization for all-sky visible and infrared satellite observations over Germany by minimizing the difference between the DWD operational analysis and radiosonde profiles in a 1-month cycled assimilation experiment that excluded radiosondes. We use reconstructed partial analysis increments (PAI) to approximate a wide range of localization settings without needing to rerun the costly month-long experiment. We find that visible satellite observations require no localization, but that infrared observations deteriorate the analysis if they are not localized carefully.

How to cite: Griewank, P., Parker, M., Necker, T., Miyoshi, T., Schomburg, A., Diefenbach, T., and Weissmann, M.: Optimal vertical localization for the assimilation of cloud-affected satellite observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16990, https://doi.org/10.5194/egusphere-egu25-16990, 2025.

The Global-to-Regional ICON (GLORI) Digital Twin is a configurable on-demand global-to-regional short-range high-resolution digital twin based on ICON. It is developed in a tri-lateral cooperation between Germany, Italy and Switzerland.

GLORI provides short-range global predictions down to the storm-scale (~3 km horizontal) and on-demand high resolution (~ 500 m) predictions for selected regions, like the Alpine domain or the Italian peninsula. It includes an uncertainty estimation through ensemble forecasts for global and regional scales. The data assimilation system is ensemble-based, both for the global and the regional components. The GLORI Digital Twin aims at providing forecasts down to the application level, for a range of use cases including flood forecasting, urban heat island and urban flooding events, mineral dust predictions for energy applications and pollen predictions.

Moving to higher resolution requires improvements both in the model and in the data assimilation system. We test the ICON model in complex topography and highlight its behaviour in dependence of conditions like stable boundary layer, flow interacting with the orography, convection development, different soil textures and urban areas. In that, GLORI can also be seen as testing environment for the development of hectometric scale modeling. The research focuses also on data assimilation at higher resolution, both for the global and for the regional runs, and on the usage of high-resolution observations. The assimilation of the radar data of the three partner countries is tested over the Alpine domain, aiming at the improvement of the prediction of convective events. Dedicated studies focus on direct assimilation at 1 km resolution. This goal demands a rigorous evaluation of the entire assimilation workflow, including observation thinning, averaging strategies, localization, and observation error quantification. The impact of performing data assimilation at 2 km resolution with nesting at 1 km is then compared with direct assimilation in the 1km domain. The performance of the Digital Twin is assessed on high-impact weather events, considering in particular convective development leading to severe weather and the recent flood events.

How to cite: Marsigli, C. and the GLORI Team: The GLObal-to-Regional ICON (GLORI) Digital Twin: towards hectometric scale predictions for high-impact weather, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17981, https://doi.org/10.5194/egusphere-egu25-17981, 2025.

EGU25-18449 | ECS | Orals | AS1.4

Optimizing all-sky infrared radiance assimilation with dynamic cloud-dependent error modeling  

Adhithiyan Neduncheran, Florian Meier, Christoph Wittmann, Martin Weissmann, and Philipp Griewank

Satellite data assimilation is progressing beyond the conventional “clear-sky” approach towards the “all-sky” approach. While the former eliminates observations affected by clouds, the latter assimilates all observations including clear-sky, cloudy and precipitation conditions. The exploitation of cloud affected radiances is a promising endeavour as these observations are directly related to particularly challenging weather phenomena (e. g. convection, frontal systems, low stratus, and fog). This study focuses on the assimilation of clear and cloud affected (all-sky) radiances, from the 6.2 μm and 7.3 μm channel sensitive to water vapour in the upper troposphere using satellite data from SEVIRI, an instrument onboard Meteosat-10. The goal is to describe the improvements in short range forecasts in the high-resolution limited area Numerical Weather Prediction Model (NWP), AROME (Application of Research to Operations at MEsoscale) used at GeoSphere Austria. 3D-Var data assimilation experiments were performed to study the impact of all-sky vs clear-sky. A significant challenge is accurately representing observation errors, which are influenced by the complex and variable nature of clouds. This work implements an observation error model that dynamically adjusts error values based on cloud amount. The model addresses the increased uncertainties in cloud-dense regions by assigning higher observation errors, while clearer areas receive lower error values, in alignment with the need for spatially adaptive error characterization in all-sky conditions. Results demonstrate that the cloud-dependent error model leads to more Gaussian departures which can be expected to improve the assimilation of cloud-affected radiances, leading to better initial conditions and refined representations of atmospheric states and consequently the forecast.   

How to cite: Neduncheran, A., Meier, F., Wittmann, C., Weissmann, M., and Griewank, P.: Optimizing all-sky infrared radiance assimilation with dynamic cloud-dependent error modeling , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18449, https://doi.org/10.5194/egusphere-egu25-18449, 2025.

EGU25-168 | Posters on site | CL5.9

Deep Learning Postprocessing to Enhance Subseasonal Soil Moisture Forecasts Across Europe 

Noelia Otero Felipe, Atahan Özer, and Jackie Ma

Flash droughts are a unique natural hazard characterized by their sudden onset and rapid intensification. Accurate and reliable forecasts on subseasonal-to-seasonal (S2S) timescales are crucial for effective preparation and mitigation of the impacts of these events. To enhance the accuracy of soil moisture predictions—a key factor in identifying flash droughts—we propose a hybrid modeling approach that integrates state-of-the-art dynamical forecasts from the European Centre for Medium-Range Weather Forecasts (ECMWF) with deep learning techniques (DL).

We use a set of DL models of different complexity for post-processing soil moisture forecasts to not only improve S2S forecasts by correcting systematic errors inherent in numerical weather prediction models, but also to enhance the spatial resolution of the forecasts.  This downscaling process is crucial as it addresses a common limitation in S2S forecasts, the coarse spatial resolution that can overlook some variations in soil moisture at a higher spatial scale. By using deterministic inputs, such as the mean and spread from the ensemble forecasting system, we further assess forecast uncertainty through dropout neural networks via Monte Carlo (MC) sampling. This technique allows us to generate probabilistic forecasts by applying MC dropout during the testing phase, thereby generating probabilistic forecasts. Our results show that the DL models outperform the S2S forecasts and lead to skillful S2S forecasts. This advanced modeling framework aims to deliver skillful soil moisture S2S forecasts, ultimately contributing to more effective strategies for managing and mitigating the effects of flash drought events.

How to cite: Otero Felipe, N., Özer, A., and Ma, J.: Deep Learning Postprocessing to Enhance Subseasonal Soil Moisture Forecasts Across Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-168, https://doi.org/10.5194/egusphere-egu25-168, 2025.

EGU25-369 | ECS | Orals | CL5.9

A machine learning-based backward extension of IMERG daily precipitation over the Greater Alpine Region 

Iman Goudarzi, Davide Fazzini, Claudia Pasquero, Agostino N Meroni, and Matteo Borgnino

An accurate knowledge of precipitation data at high spatio-temporal resolution is crucial for hydrological forecasting, meteorological analysis, and climate studies. This is especially true in  mountainous areas, where traditional climate models struggle to accurately predict precipitation due to factors such as low spatial resolution and where rain gauges are sparse. High-elevation areas are particularly relevant as they act as reservoirs of water resources and are characterized by elevation-dependent climate change signals (Pepin et al., 2022). By leveraging the good performances of the satellite-based IMERG (Integrated Multi-satellitE Retrievals for GPM) rainfall product and the realism of the ERA5 atmospheric reanalysis, we aim to produce a multi-decadal daily rainfall product at the IMERG spatial resolution (roughly 8 km) over the Greater Alpine Region (GAR). To achieve this, we employ advanced machine learning techniques designed to capture the complex, non-linear relationships inherent in atmospheric processes.  

Twenty years of IMERG data (from 2001 to 2020) are used to train and test various types of machine learning algorithms to estimate daily precipitation maps starting from some ERA5 atmospheric fields including mid-tropospheric temperature and winds; vertically integrated ice, liquid water and water vapour contents; total precipitation, and other relevant variables. In addition to these atmospheric fields, a high-resolution elevation dataset (ETOPO) is used to represent the intricate terrain of the Alps. The Recursive Feature Elimination (RFE) technique is employed to select key input variables, introducing effective predictors and enhancing the understanding of the influence of physical atmospheric variables and their inter-relationships in mountainous regions. ERA5 total precipitation, vertically integrated ice and water vapour content appear to be the three most relevant input fields for an optimal estimate of IMERG precipitation. Among the algorithms tested (XGBoost, Random Forest, Convolutional Neural Networks, Deep Neural Networks), XGBoost (XGB) is found to be the most reliable and computationally efficient.

The results show a spatiotemporal RMSE improvement of approximately 15 percent, decreasing from 5.18 mm/day (between ERA5 and IMERG) to 4.37 mm/day (between XGB and IMERG). On a seasonal basis, the RMSE is higher in summer and fall, where higher mean precipitation intensities are observed. Also, in terms of changes with the terrain height, the RMSE follows quite tightly the mean precipitation elevation dependence. The XGB model is used to backward extend the IMERG dataset so that precipitation biases and trends can be computed over a multi-decadal time range. These findings demonstrate the potential of machine learning to improve the accuracy of ERA5 rainfall data, which can be exploited to advance our understanding of the emerging elevation-dependent climate change signal. 

How to cite: Goudarzi, I., Fazzini, D., Pasquero, C., Meroni, A. N., and Borgnino, M.: A machine learning-based backward extension of IMERG daily precipitation over the Greater Alpine Region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-369, https://doi.org/10.5194/egusphere-egu25-369, 2025.

EGU25-1037 | ECS | Posters on site | CL5.9

Enhancing Hyperlocal 3-Hourly Rainfall Forecasting for Mumbai Using a Hybrid CNN-LSTM Model. 

Puja Tripathy, Raghu Murtugudde, Subhankar Karmakar, and Subimal Ghosh

The increasing frequency and severity of extreme weather events, such as heavy rainfall and flooding, emphasize the urgent need for advanced early warning systems. Short-duration rainfall extremes, exacerbated by climate change, significantly increase flood risks, particularly in urban coastal cities like Mumbai. Mumbai's vulnerability arises from rapid urbanization, its coastal location, and variable topography, which contribute to significant spatial variability in rainfall. We have used Global Forecast System (GFS) data to identify key predictors for high-resolution, 3-hour rainfall forecasts for Mumbai. The GFS variables were selected using a correlation matrix. We have used past 3-hour observed rainfall data from Automatic Weather Stations (AWS) across 15 locations in Mumbai (2015–2023) along with selected GFS variables, which include Precipitable Water, Precipitation Rate, Relative Humidity, and Total Cloud Cover, to forecast rainfall for one timestep ahead. The dataset was divided into 80% for training and 20% for testing. We employed a hybrid Convolutional Neural Network-Long Short-Term Memory (CNN-LSTM) model to enhance forecast accuracy. The CNN captures spatial features, while the LSTM models temporal dependencies, effectively addressing the challenges of hyperlocal rainfall forecasting. Further, we incorporated a weighted Mean Squared Error (MSE) loss function to prioritize extreme rainfall events (≥95th percentile). The results indicate that using CNN-LSTM models reduced the Root Mean Square Error (RMSE) by 9.41% -12.38% and increased the Correlation Coefficient (CC) by 70.4%-113% compared to GFS models. At the 95th percentile, the Hit Rate (HR) improved by 233% -483.3%, while the False Alarm Rate (FAR) decreased by 7%-16.2%. Using weighted MSE also enhanced performance, increasing the HR by 255.5%-583.3% at the 95th percentile and reducing the FAR by 7% -13.2%. Implementing weighted MSE as a loss function resulted in a reduction in RMSE by 9.94% -12.86% and an increase in CC by 85.2%-126%. This study highlights that the hybrid CNN-LSTM model, combined with a weighted MSE loss function, demonstrates superior capability in accurately forecasting 3-hourly extreme rainfall events in Mumbai, providing critical advancements for early warning systems and flood risk mitigation.

How to cite: Tripathy, P., Murtugudde, R., Karmakar, S., and Ghosh, S.: Enhancing Hyperlocal 3-Hourly Rainfall Forecasting for Mumbai Using a Hybrid CNN-LSTM Model., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1037, https://doi.org/10.5194/egusphere-egu25-1037, 2025.

We present Prithvi-Typhoon, an innovative adaptation of the Prithvi WxC weather foundation model for tropical cyclone intensity prediction. Through a novel three-stage progressive fine-tuning framework, we bridge the gap between general weather forecasting and specialized tropical cyclone prediction. The model integrates multi-source data from tropical cyclones (1987-2023), incorporating satellite observations, reanalysis products, and historical records. Our architecture features domain-specific feature extraction and multi-scale integration, enabling adaptive balance between local storm features and global atmospheric patterns.

Evaluation results demonstrate substantial improvements over existing methods. Notably, Prithvi-Typhoon shows enhanced skill in predicting rapid intensification events, outperforming both traditional numerical models and existing deep learning approaches. This work represents a advancement in applying foundation models to extreme weather prediction, offering a computationally efficient solution while maintaining physical consistency.

How to cite: Meng, F.: Prithvi-Typhoon: A Foundation Model Approach for Enhanced Tropical Cyclone Intensity Prediction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1738, https://doi.org/10.5194/egusphere-egu25-1738, 2025.

EGU25-1879 | ECS | Posters on site | CL5.9

Regional High-Resolution Weather Forecasting over the Arabian Peninsula: A Data-Driven Approach 

Sofien Resifi, Elissar Al Aawar, Hari Dasari, Hatem Jebari, and Ibrahim Hoteit

Accurate high-resolution spatio-temporal weather forecasting is vital for advancing our understanding of regional weather dynamics and improving meteorological applications. Traditional forecasting relies on numerical weather prediction (NWP) models, which are computationally demanding, particularly when implemented for large domains and high-resolution grids. Recently, Deep Learning (DL) has emerged as a powerful alternative, leveraging historical data to identify patterns and predict future atmospheric conditions. In this work, we develop a regional DL-based forecasting system tailored for the Arabian Peninsula (AP), a region with unique climatic conditions characterized by extreme temperatures and high wind energy potential. Therefore, it serves as an ideal case study for regional weather forecasting. The developed system forecasts hourly meteorological variables such as wind speed, wind direction, and temperature at a 5 km spatial resolution up to 48 hours ahead, with a focus on key vertical levels relevant to wind energy applications. Two forecasting approaches are explored: recursive forecasting, which iteratively advances fine-scale spatio-temporal states over time, and downscaling, which refines coarse-resolution forecasts of the meteorological variables into their high-resolution counterparts.  Additionally, we propose a combined approach that integrates these methods by combining fine-scale dynamics propagation with coarse-scale to fine-scale refinement. The frameworks were evaluated both qualitatively and quantitatively, demonstrating that while recursive forecasting accumulates errors over time, the downscaling approach effectively produces high-resolution forecasts. The combined approach significantly improves the forecasting precision, offering robust performance at early time steps and reduced error accumulation over extended forecasting horizons.

How to cite: Resifi, S., Al Aawar, E., Dasari, H., Jebari, H., and Hoteit, I.: Regional High-Resolution Weather Forecasting over the Arabian Peninsula: A Data-Driven Approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1879, https://doi.org/10.5194/egusphere-egu25-1879, 2025.

EGU25-2013 | Orals | CL5.9

Addressing the US Tropical Cyclone-Storm Surge risk using RAFT-DeepSurge, an advanced AI-based approach  

Karthik Balaguru, Julian Rice, David Judi, Ning Sun, and Brent Daniel

Extreme climate events or tails of natural hazard distributions tend to be the most damaging in terms of societal impacts. While traditional physics-based approaches are suitable for gaining mechanistic understanding and for process-based studies, they may not be adequate for characterizing probabilistic risk from extreme events. Here, we demonstrate a ML/AI-based approach for estimating probabilistic risk from tropical cyclones (TCs) and the associated coastal flooding. First, we simulate nearly one million TCs for the current and future climates using the Risk Analysis Framework for Tropical Cyclones (RAFT), a hybrid model that combines physics with deep neural networks. Subsequently, we apply RAFT-simulated TC tracks to DeepSurge, an AI-based storm surge model that is trained on a large number of ADCIRC simulations in the North Atlantic. Our results suggest a significant increase in storm surge risk for the northern Gulf Coast, Florida and some areas near the mid-Atlantic. Also importantly, we show that ML/AI can be leveraged effectively to address the potential issue of ‘Grey Swan’ TCs and their impacts.

How to cite: Balaguru, K., Rice, J., Judi, D., Sun, N., and Daniel, B.: Addressing the US Tropical Cyclone-Storm Surge risk using RAFT-DeepSurge, an advanced AI-based approach , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2013, https://doi.org/10.5194/egusphere-egu25-2013, 2025.

EGU25-3286 | Posters on site | CL5.9

Emulation and S2S probabilistic prediction of 2-m temperature and precipitation over the global domain using linear inverse modeling 

Sergey Kravtsov, Andrew Robertson, Jing Yuan, and Mohammad Ghadamidehno

We developed a data-driven system for joint prediction of daily precipitation (Pr) and near-surface temperature (T2m) over the global domain by utilizing NASA’s satellite observations and the associated reanalysis products, with the focus on S2S hydrologic forecasting. Our approach is based on a well-established methodology of linear inverse modeling modified and adapted by our science team for high-resolution modeling of precipitation. The key element of this new methodology is the usage of a so-called pseudo-precipitation (PP) variable, equal to the actual Pr where precipitation is occurring and, otherwise, equal to the (negative) air-column integrated water-vapor saturation deficit — the amount of water vapor to be added to the air column to achieve saturation at each vertical level. The model’s jointly obtained Pr and T2m forecasts are then validated against the observed fields as usual.

The above model is shown to be an efficient tool for emulating daily sequences of global coupled T2m and Pr fields with spatiotemporal characteristics strikingly similar to the observed characteristics. We used a large (100-member) ensemble of our statistical model’s hindcasts of precipitation over global domain to predict probabilities of weekly and biweekly precipitation amounts in one of the three categories (below normal, normal, and above normal) and compared these hindcasts with those based on the NASA GEOSS2S v2p1 model (4-member ensemble), calibrated using extended logistic regression. While the statistical model’s S2S precipitation forecast skill is somewhat lower than that of the reference NASA state-of-the-art system, it exhibits similar geographical and seasonal distributions, which warrants further research. We are currently looking into incorporating automated ML/AI feature identification techniques into our existing set up (with a linear activation function), to fine-tune the model learning and improve its predictive potential.

How to cite: Kravtsov, S., Robertson, A., Yuan, J., and Ghadamidehno, M.: Emulation and S2S probabilistic prediction of 2-m temperature and precipitation over the global domain using linear inverse modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3286, https://doi.org/10.5194/egusphere-egu25-3286, 2025.

EGU25-4576 | ECS | Posters on site | CL5.9

On the robustness of AI model forecast skill and initial condition uncertainty of the 2021 Pacific Northwest Heatwave 

Osamu Miyawaki, Cuiyi Fei, Siyu Li, Dhruvit Patel, Giorgio Sarro, Huan Zhang, Adam Marchakitus, Pedram Hassanzadeh, Dorian Abbot, Jonathan Weare, Noboru Nakamura, and Tiffany Shaw

AI weather models are becoming valuable tools for predicting the weather. While AI models’ general forecasts are known to be skillful, their forecast skill of extreme events is not fully understood. The 2021 Pacific Northwest (PNW) heatwave is a good case study for AI models because it falls outside of the distribution of heat waves in AI model training datasets.

Here, we investigate the forecast performance of 8 AI models (AIFS, Gencast, NeuralGCM, Graphcast, Fuxi, Pangu, Fourcastnet, FourcastnetV2) of the 2021 PNW heatwave. Despite the event being out of the training dataset distribution, their forecast performance is comparable to that of a state-of-the-art numerical weather prediction model (IFS). Specifically, AI models and IFS can accurately forecast the heatwave for lead times less than 7 days.

Two recent studies suggest the predictability barrier of the PNW heatwave may be due to an initial condition observation error. Leach et al. (2024) found that the 26th ensemble member of a 250 member IFS forecast accurately forecasts the heatwave 12 days in advance. Vonich and Hakim (2024) used backpropagation in Graphcast to find an optimal initial condition that leads to an accurate forecast 10 days in advance. Are these initial conditions robust across an ensemble of AI models? And do these initial conditions point to a unique solution?

We find a large spread in forecast accuracy when running the 8 AI models with the Leach et al. (2024) and Vonich & Hakim (2024) initial conditions. Furthermore we ran 1000 member ensembles in NeuralGCM and find initial conditions that lead to an accurate long-term forecast are not unique. These results suggest that the improvement in forecast accuracty to certain initial conditions may not necessarily be due to the initial conditions being closer to ground truth but rather they are due to cancelation of model error.

How to cite: Miyawaki, O., Fei, C., Li, S., Patel, D., Sarro, G., Zhang, H., Marchakitus, A., Hassanzadeh, P., Abbot, D., Weare, J., Nakamura, N., and Shaw, T.: On the robustness of AI model forecast skill and initial condition uncertainty of the 2021 Pacific Northwest Heatwave, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4576, https://doi.org/10.5194/egusphere-egu25-4576, 2025.

EGU25-4735 | ECS | Orals | CL5.9

Application of a novel deep learning model for precipitation nowcasting  

Fereshteh Taromideh, Giovanni Francesco Santonastaso, and Roberto Greco

In recent decades, the prediction of precipitation has become a central focus for atmospheric scientists and weather forecasters. In particular, improving the predictability of rapidly forming rainfall events is critical for protecting lives and property. The island of Ischia, located in the Campania region of Italy, has experienced several landslides and flash floods in recent years with catastrophic effects. To mitigate these geohydrological hazards on this island, we propose a method for short-term rainfall forecasting, with "short-term" defined as a time frame up to six hours. Accurate predictions are essential, as they enable timely implementation of protective measures to safeguard the population.

Accurately predicting rainfall is a complex task influenced by numerous factors, including humidity, temperature, pressure, and wind speed. Historically, rainfall nowcasting has primarily relied on numerical weather prediction (NWP) models. However, this approach has notable limitations, such as high computational requirements and significant processing time, which make NWP models less practical for short-term forecasts.

In the past decade, machine learning (ML) models have revolutionized the way complex problems are addressed and solved, offering solutions that are both fast and highly efficient. Within this domain, deep neural networks (DNNs) a subset of ML have become increasingly prevalent for tackling complex problems using large datasets. Among these, U-Net, a specific DNNs architecture, has proven to be one of the most effective and accurate models for prediction tasks when the input data is image-based. However, achieving high accuracy with such models requires careful preprocessing of the dataset to enhance the model’s ability to effectively learn from the data. Additionally, properly tuning the model's hyperparameters is crucial for optimizing its performance.

In this study, we propose an enhanced U-Net model for nowcasting rainfall with a 120-minute lead time. The input data consists of rainfall radar data and rain gauge measurements. Furthermore, the study evaluates the model's performance under different training scenarios, comparing its efficacy when using only rainfall radar data versus an integrated dataset combining radar and rain gauge data. It is worth noting that the model operates in a regression framework, where the labels or outputs are the rain gauge readings with a 120-minute lead time.

 

How to cite: Taromideh, F., Santonastaso, G. F., and Greco, R.: Application of a novel deep learning model for precipitation nowcasting , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4735, https://doi.org/10.5194/egusphere-egu25-4735, 2025.

Accurate air temperature (Ta)  forecasting in urban areas is crucial for various socio-economic aspects, including risk warning and optimization of electricity systems. However, forecasting within urban environments faces substantial challenges due to the coarse spatial resolution and inadequate urban representation in numerical weather prediction (NWP) models. In this study, we present a novel multimodal deep learning framework that learns local dynamics from ground-level weather stations while effectively informing large-scale weather patterns for short-range (1- 24  hour lead time) Ta forecasting. The framework first employs graph neural networks (GNNs) to model intra-city spatiotemporal dynamics across 35 weather stations, achieving over 12% forecast improvement compared to modeling individual time series, primarily through mean state regularization. We further develop an end-to-end multimodal framework by integrating the GNN with synoptic weather patterns, achieving an additional 23% improvement, with particular expertise in winter and capturing cold spell events. Our study demonstrates the effectiveness of incorporating multi-scale information from diverse data sources and reveals that weather patterns within approximately 2000 km are critical for local city-scale forecasting. This framework can be readily adapted to other urban areas and will benefit significantly from the increasing deployment of smart IoT sensors to effectively address intra-city temperature heterogeneity.

How to cite: Wang, H. and Yang, J.: Multimodal Deep Learning Framework for Urban Air Temperature Forecasting: Bridging Local and Synoptic Scales, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4940, https://doi.org/10.5194/egusphere-egu25-4940, 2025.

EGU25-5319 | ECS | Posters on site | CL5.9

Precipitation nowcasting diffusion model based on turbulence theory and multi-source data 

Dawei Li, Kefeng Deng, Di Zhang, Hongze Leng, Kaijun Ren, and Junqiang Song

Precipitation nowcasting is a long-standing challenge due to the inherent unpredictability, which often lead to significant risks and damage. While traditional approaches focus on modeling the nonlinear relationship between initial precipitation states and future states, these methods often fail to capture accurate precipitation dynamics, such as its distribution and intensity. The absence of guidance from physical theory limits data-driven methods in disclosing the chaotic nature of precipitation. To address this, we integrate Prandtl’s mixing length theory from fluid dynamics with diffusion models commonly used in computer vision to enhance the prediction of precipitation distributions and details over the next 200 minutes. This integration accounts for the turbulent properties of precipitation, improving both accuracy and granularity in forecasts. Additionally, we leverage multi-source data, particularly lightning observations, to train a control network for our diffusion model. This enhancement allows for more accurate and controllable predictions of precipitation initiation, decay, and overall spatial-temporal patterns. Our approach advances the state of the art in precipitation nowcasting, offering a robust framework that bridges physical theory with modern deep learning techniques.

How to cite: Li, D., Deng, K., Zhang, D., Leng, H., Ren, K., and Song, J.: Precipitation nowcasting diffusion model based on turbulence theory and multi-source data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5319, https://doi.org/10.5194/egusphere-egu25-5319, 2025.

EGU25-7021 | ECS | Posters on site | CL5.9

Uncertainty-aware precipitation generation for Earth system models with diffusion models 

Michael Aich, Sebastian Bathiany, Philipp Hess, Yu Huang, and Niklas Boers

Earth system models (ESMs) play a vital role in understanding and forecasting the dynamics of the Earth's climate system. Accurate simulation of precipitation is especially critical for evaluating the impacts of anthropogenic climate change, anticipating extreme weather events, and devising sustainable strategies to manage water resources and mitigate related risks. However, ESMs often exhibit significant biases in precipitation simulation due to the wide range of scales involved in these processes and the substantial uncertainties they encompass. Moreover, due to computational constraints, ESM simulations still have low horizontal resolution compared to the scales relevant for precipitation.
    In this work, we present a novel framework to improve the representation of precipitation in ESMs by integrating physically modeled circulation variables with state-of-the-art generative diffusion models. Based on large-scale (1 degree) circulation fields, our method produces accurate high-resolution (0.25 degree) precipitation estimates at global scale. Our approach introduces stochasticity into the precipitation field, significantly improving the representation of extreme events and fine-scale variability while maintaining the fidelity of large-scale patterns. Our proposed methods thus provides an alternative to traditional column-based parameterization, avoiding the need for a posteriori bias correction and downscaling.
    Preliminary results highlight the ability of our generative model to produce precipitation fields with substantially smaller biases compared to those derived from classical parameterizations of the GFDL model, while achieving higher spatial resolution. In future climate scenarios, precipitation derived from parameterizations often becomes increasingly uncertain, whereas circulation variables, being more directly tied to large-scale dynamics, may provide a more stable foundation for generating high-resolution precipitation fields. Building on this, we demonstrate the application of our framework to generate daily high-resolution precipitation maps for future climate projections, offering an improved and robust tool to address critical challenges in climate impact studies.

How to cite: Aich, M., Bathiany, S., Hess, P., Huang, Y., and Boers, N.: Uncertainty-aware precipitation generation for Earth system models with diffusion models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7021, https://doi.org/10.5194/egusphere-egu25-7021, 2025.

EGU25-7075 | Posters on site | CL5.9

Use of NVIDIA FourCastNet model to improve tropical cyclones risk modelling.  

Remi Meynadier, Xavier Renard, Marius Koch, Hugo Rakotoarimanga, Georg Ertl, Jussi Leinonen, and Marcin Detyniecki

AXA is developing in-house Natural Hazard models (or Natural Catastrophe models) in order to gain a deeper understanding of, evaluate, and monitor the climate risks underpinning (re)insurance portfolios. Such models simulate large numbers of synthetic weather events to estimate the probability of rare and extreme events, enabling more robust risk management and informed decision-making.

AI-driven weather models offer the capability to rapidly produce thousands of unique ensemble scenarios of low-likelihood high-impact weather events such as tropical cyclones. This study specifically utilizes tropical cyclones (TCs) as a primary illustration of the potential of AI-based weather models for risk management.

In this study we use FourCastNet SFNO, the global data-driven weather forecasting model developed by NVIDIA available on the NVIDIA Earth-2 platform to simulate historical but also synthetic (i.e. never observed) hurricanes. SFNO trained on ECMWF ERA5 reanalysis data provides short to medium-range global predictions at 0.25° resolution. A large ensemble of hurricane simulations is performed using the HENS method, developed at Berkeley, the NVIDIA leveraging Earth2Studio from NVIDIA’s Earth-2 platform.

HENS-SFNO performance is first assessed by evaluating the model's ability to reproduce post-2017 historical hurricanes (intensity, track, landfall location). HENS-SFNO capabilities in simulating synthetic hurricanes are then assessed in a second step by evaluating track density and landfall frequencies by categories of hurricanes against the historical tropical cyclone IBTrACS database.

How to cite: Meynadier, R., Renard, X., Koch, M., Rakotoarimanga, H., Ertl, G., Leinonen, J., and Detyniecki, M.: Use of NVIDIA FourCastNet model to improve tropical cyclones risk modelling. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7075, https://doi.org/10.5194/egusphere-egu25-7075, 2025.

EGU25-7861 | Posters on site | CL5.9

Subseasonal to Seasonal Forecast Using Neural Ordinary Differential Equations 

Jonghan Lee and Woosok Moon

While short-term weather forecasting has benefited from extensive data and research, leading to high predictive accuracy, long-term forecasts, particularly medium-range predictions, lag significantly due to data scarcity. This research aims to bridge this gap by leveraging the advancements in Artificial Intelligence (AI), particularly Deep Learning. We propose a novel approach using Neural Ordinary Differential Equations (NODEs), which represents a transformative step in dynamic systems modeling. Neural ODEs offer a flexible and powerful framework for continuous-time models, which is particularly beneficial for handling sparse or irregularly sampled data prevalent in climate studies. Our methodology utilizes the Empirical Orthogonal Function (EOF) to extract principal component time series from limited climate data. These components serve as inputs for NODEs to predict future climatic conditions. This approach is innovative in its ability to handle non-linearities and temporal dependencies in climatic data, making it highly suitable for medium-range weather forecasting. The potential of NODEs in this context is significant, as they provide a means to accurately predict weather patterns with less data, a common limitation in long-term forecasting. By enhancing the precision of medium-range forecasts, this research contributes to more effective climate change adaptation and mitigation strategies, ultimately aiding in the safeguarding of ecosystems and human societies against the adverse effects of extreme weather conditions.

How to cite: Lee, J. and Moon, W.: Subseasonal to Seasonal Forecast Using Neural Ordinary Differential Equations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7861, https://doi.org/10.5194/egusphere-egu25-7861, 2025.

EGU25-8890 | ECS | Orals | CL5.9

Using deep neural networks for thunderstorm risk prediction. 

Mélanie Bosc, Adrien Chan Hon Tong, Aurélie Bouchard, and Dominique Béréziat

Airliners, struck by lightnings on average once a year, sometimes sustain structural or electrical damage. Even if these incidents generally do not compromise safety onboard due to existing certifications, they lead to costly downtimes and mandatory maintenance operations for the aviation industry. Anticipating the presence of thunderstorm risk areas could help minimize these impacts. Nowadays, predict the exact location of electrical activity in the atmosphere is a complex task because lightning is a non-linear phenomenon which is related to chaotic stormy environments. Numerous variables influence the initiation of electrical discharges, making their modeling using physical equation very challenging. This motivates the use of neural networks to establish relationships between various atmospheric parameters and electrical activity. In the context of aviation safety, this study focuses on the development of a very short term (less than one hour and every five minutes) thunderstorm risk forecasting method above oceans. The proposed methodology is based on computer vision techniques such as neural networks to generate lightning occurrence’s probability maps in the following hour. An encoder-decoder network named ED-DRAP (Che, H et al. 2022) is employed and adapted to the data. In addition to integrating convolutional operations, it also uses spatial and temporal attention mechanisms to process spatio-temporal sequences. Input data come from NOAA’s geostationary GOES-R satellite, including brightness temperature measured by the Advanced Baseline Imager sensor and past electrical activity detected by the Geostationary Lightning Mapper sensor. Outputs from the Numerical Weather Prediction model, Global Forecasting System, are also employed to complement the information provided by satellite imagery. Finally, the model’s outputs are calibrated to produce lightning risk probability maps which are representative of the physical reality, enabling better risk interpretation.

How to cite: Bosc, M., Chan Hon Tong, A., Bouchard, A., and Béréziat, D.: Using deep neural networks for thunderstorm risk prediction., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8890, https://doi.org/10.5194/egusphere-egu25-8890, 2025.

EGU25-9087 | ECS | Orals | CL5.9

Coupling AI Emulators and Rare Event Algorithms to Sample Extreme Heatwaves 

Amaury Lancelin, Alex Wikner, Pedram Hassanzadeh, Dorian Abbot, Freddy Bouchet, Laurent Dubus, and Jonathan Weare

Heatwaves are among the most impactful extreme weather events, posing significant risks to human health, ecosystems, and energy systems. Understanding the return times of these events and assessing how climate change alters their frequency and intensity are critical for effective adaptation strategies. However, the rarity of record-breaking heatwaves in observational datasets makes this task highly challenging. Climate models, while capable of simulating such rare events, require prohibitively long simulations to generate robust statistics for events with return times on the order of centuries.

Our study addresses these challenges by leveraging a dual approach combining rare event simulation algorithms and AI-driven climate model emulators. Rare event algorithms, such as genetic algorithms, efficiently target the extreme trajectories leading to heatwaves while avoiding typical weather conditions, allowing for a more focused exploration of the event space. Although effective for long-duration events, these approaches are less suited to capturing shorter-term phenomena, necessitating novel methodologies for finer temporal scales.

In parallel, we leverage the advancements of deep learning in climate science by training neural networks-based climate model emulators based on Vision Transformers. These emulators drastically reduce computational costs and generate realistic climate simulations, including heatwave dynamics. Here, we explore coupling emulators with a new rare event algorithm specifically designed to sample short and extreme heatwaves. We demonstrate the efficiency of this method by calculating return times for unprecedented heatwave events.

In this work, we use data from PlaSim, a cheap-to-run climate model of intermediate complexity, which enables the verification of return periods spanning up to thousands of years. The next steps involve utilizing more state-of-the-art climate models at finer spatial resolutions and evaluating how the statistics of heatwaves may evolve under various climate change scenarios.

How to cite: Lancelin, A., Wikner, A., Hassanzadeh, P., Abbot, D., Bouchet, F., Dubus, L., and Weare, J.: Coupling AI Emulators and Rare Event Algorithms to Sample Extreme Heatwaves, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9087, https://doi.org/10.5194/egusphere-egu25-9087, 2025.

EGU25-9541 * | ECS | Posters on site | CL5.9 | Highlight

Benchmarking Deep Learning Models for Probabilistic Subseasonal Forecasting of Heat Extremes 

Cas Decancq, Thomas Mortier, Daniel Hagan, Victoria Deman, Damián Insua Costa, Gustau Camps-Valls, Dim Coumou, and Diego Miralles

Predicting climate extremes such as droughts, heatwaves, and heat stress episodes remains a critical challenge in Earth system sciences. Current state-of-the-art methods often fail to deliver reliable forecasts, especially at subseasonal-to-seasonal (S2S) timescales (i.e., from two weeks to two months in advance). As global climate variability continues evolving, the need for advanced, trustworthy, data-driven forecasting methodologies has never been more pressing.

Extended numerical weather prediction systems, such as those led by the European Centre for Medium-Range Weather Forecasts (ECMWF), remain the primary method for S2S prediction (Vitart & Robertson, 2018). While recent deep learning approaches have demonstrated remarkable competitive performance (e.g. Olivetti & Messori, 2024), proposed models predominantly focus on global-scale average weather predictions, overlooking critical local-scale extreme events (Pasche et al., 2024). Moreover, creating accurate probabilistic forecasts conditioned on the initial state remains a significant challenge within the scientific community. In the context of weather forecasting, traditional statistical methods, such as ensemble-based techniques that generate multiple forecasts to estimate uncertainty, are commonly used. These approaches include techniques such as introducing noise into initial states, varying neural network parameters, or training generative models. While generative models offer the most robust solutions, they demand substantial computational resources and extensive data availability.

Here, we evaluate several state-of-the-art dynamical weather forecasting systems, such as those of ECMWF and the National Centers for Environmental Prediction (NCEP), together with recently-proposed deep learning models on their ability to predict extreme heatwaves across all continents at S2S timescales. Since uncertainty quantification is essential for supporting practical decision-making, we focus on deep learning models that provide probabilistic forecasts and have publicly available source code. These include FourCastNet, proposed by Kurth et al. (2023), as well as ArchesWeather and ArchesWeatherGen, developed by Couairon et al. (2024). This analysis underscores the limitations of contemporary deep learning and dynamical weather forecasting systems in reliably and probabilistically predicting S2S extremes, while also providing a valuable benchmark to guide future research efforts.

 

References:

Couairon, G., Singh, R., Charantonis, A., Lessig, C., & Monteleoni, C. (2024). ArchesWeather & ArchesWeatherGen: a deterministic and generative model for efficient ML weather forecasting. arXiv preprint arXiv:2412.12971.

Kurth, T., Subramanian, S., Harrington, P., Pathak, J., Mardani, M., Hall, D., Miele, A., Kashinath, K., & Anandkumar, A. (2023). FourCastNet: Accelerating global high-resolution weather forecasting using adaptive Fourier neural operators. Proceedings of the Platform for Advanced Scientific Computing Conference (PASC '23), Article 13, 1–11. https://doi.org/10.1145/3592979.3593412

Olivetti, L., & Messori, G. (2024). Do data-driven models beat numerical models in forecasting weather extremes? A comparison of IFS HRES, Pangu-Weather, and GraphCast. Geoscientific Model Development17(21), 7915-7962.

Pasche, O. C., Wider, J., Zhang, Z., Zscheischler, J., & Engelke, S. (2025). Validating Deep Learning Weather Forecast Models on Recent High-Impact Extreme Events. Artificial Intelligence for the Earth Systems4(1), e240033. https://doi.org/10.1175/AIES-D-24-0033.1

Vitart, F., & Robertson, A. W. (2018). The sub-seasonal to seasonal prediction project (S2S) and the prediction of extreme events. npj climate and atmospheric science1(1), 3.

How to cite: Decancq, C., Mortier, T., Hagan, D., Deman, V., Insua Costa, D., Camps-Valls, G., Coumou, D., and Miralles, D.: Benchmarking Deep Learning Models for Probabilistic Subseasonal Forecasting of Heat Extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9541, https://doi.org/10.5194/egusphere-egu25-9541, 2025.

EGU25-11549 | ECS | Orals | CL5.9

Improving Spatial Uncertainty Representation in Sub-seasonal Wind Speed Forecasts Using Quantile Regression, VAE and Diffusion 

Ganglin Tian, Anastase Alexandre Charantonis, Camille Le Coz, Alexis Tantet, and Riwal Plougonven

The uncertainty quantification in sub-seasonal wind speed forecasting is important for risk assessment and decision-making. One way to improve dynamical forecast skills is to regress information from forecasts of large-scale fields to surface fields by a supervised learning model. For such a statistical downscaling approach, Tian et al. (2024) demonstrated that spatially independent stochastic perturbations based on model residuals can improve the representation of ensemble dispersion. However, this method is limited in fully representing complex spatial correlations and maintaining physical consistency across meteorological fields. Recent advances in probabilistic deep learning models offer promising new approaches for uncertainty quantification, particularly in capturing spatial dependencies.

 

This study investigates how different statistical downscaling methods can better represent dynamic spatial uncertainty in sub-seasonal ensemble forecasts compared to the independent stochastic perturbation approach. We examine three probabilistic deep learning methods with distinct uncertainty quantification mechanisms: the Quantile Regression for direct modeling of distribution quantiles, the Variational Autoencoders (VAE) for latent space sampling, and the Diffusion model for iterative denoising-based distribution modeling. Our two-stage framework first trains these regression models on the ERA5 reanalysis to establish their capacity for spatial uncertainty representation from the 500hPa geopotential height (Z500) to the surface wind speeds (U100), then applies these probabilistic models to the ECMWF Z500 hindcasts to regress U100 ensembles.

 

Comprehensive verification reveals distinct characteristics of each method. First, in terms of grid point-wise metrics (the MSE and the CRPS), all these probabilistic methods achieve comparable forecasting skills to independent stochastic perturbations, despite their different approaches to uncertainty representation. Second, spatial structure analysis through Empirical Orthogonal Functions (EOF) analysis and zonal energy spectra demonstrates notable differences: while all methods effectively capture large- and medium-scale features, they differ significantly in representing small-scale spatial correlations. The grid-independent nature of independent stochastic perturbations leads to over-representation of small-scale variations, whereas the Diffusion model shows superior performance across all spatial scales. The Quantile Regression and the VAE show relatively limited skill in capturing small-scale spatial features. These findings suggest that probabilistic downscaling methods, particularly the Diffusion model, can better reconstruct spatial characteristics while maintaining comparable forecasting skills.

 

Our results indicate that probabilistic downscaling methods can provide more realistic representations of spatial uncertainty compared to the independent stochastic approach, particularly in reconstructing spatial correlations and maintaining physical consistency. This study advances our understanding of how deep learning methods can improve uncertainty quantification in sub-seasonal forecasting.

 

Tian, Ganglin, et al. "Improving sub-seasonal wind-speed forecasts in Europe with a non-linear model." arXiv preprint arXiv:2411.19077 (2024).

How to cite: Tian, G., Charantonis, A. A., Le Coz, C., Tantet, A., and Plougonven, R.: Improving Spatial Uncertainty Representation in Sub-seasonal Wind Speed Forecasts Using Quantile Regression, VAE and Diffusion, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11549, https://doi.org/10.5194/egusphere-egu25-11549, 2025.

EGU25-11905 | ECS | Orals | CL5.9

Feature selection for data-driven seasonal forecasts of European heatwaves 

Ronan McAdam, Jorge Pérez-Aracil, Antonello Squintu, Cesar Peláez-Rodríguez, Felicitas Hansen, Verónica Torralba, Harilaos Loukos, Eduardo Zorita, Matteo Giuliani, Leone Cavicchia, Sancho Salcedo-Sanz, and Enrico Scoccimarro

The early-warning of heatwaves using seasonal forecasting systems has the potential to mitigate economic losses and loss of life. Because of the limited reliability and computational expense of dynamical forecast systems, efforts in recent years have turned to exploiting the power of Machine Learning. Recent years have seen data-driven methods of forecasting deliver added-value for short-term forecasting, yet work on the seasonal scale is not yet as mature. Within the framework of the European Horizon project “CLINT - Climate Intelligence”, a purely data-driven approach to forecasting summer heatwaves on seasonal timescales has been developed. This approach is based on a novel optimisation-based feature selection framework that detects the optimal combination of variables, domains and lag times used to predict heatwaves. The feature selection is performed on multi-millennial paleo-simulation, ensuring sufficient training data, and it is demonstrated that predictors in the model-world are relevant to predictions of the recent past (1993-2016). For forecasts of summer heatwave propensity initialised in May, the data-driven approach matches the skill of the state-of-the-art dynamical multi-model product over Europe, and even outperforms individual systems, at a considerably lower cost. Moreover, low skill over Scandinavia and northern Europe, a long-term issue common to most dynamical systems, is improved in the data-driven approach. Besides forecasts, the data-driven approach also provides insight into the key predictors of European summer heatwave tendency; in particular most-commonly selected predictors correspond to 1-2 months prior to the start of summer (i.e., March) and some have not yet been discussed in existing literature. 

How to cite: McAdam, R., Pérez-Aracil, J., Squintu, A., Peláez-Rodríguez, C., Hansen, F., Torralba, V., Loukos, H., Zorita, E., Giuliani, M., Cavicchia, L., Salcedo-Sanz, S., and Scoccimarro, E.: Feature selection for data-driven seasonal forecasts of European heatwaves, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11905, https://doi.org/10.5194/egusphere-egu25-11905, 2025.

EGU25-11955 | ECS | Orals | CL5.9

Enhancing Subseasonal Precipitation Forecasting with Foundation Models: A Performance-Driven Study 

Francesco Bosso, Riccardo Musto, and Loris Panza

Sub-seasonal to seasonal (S2S) precipitation forecasting, the forecasting of precipitation from 2 weeks up to 1 month in advance, is crucial to support early warning and decision-making operations in real-world scenarios. To correctly allocate water resources or plan mitigation strategies at sub-seasonal lead times, high-quality precipitation forecasting can be game-changing to prevent phenomena such as droughts or floods. One of the main sources of uncertainty affecting state-of-the-art models comes from the overlapping of phenomena at different spatiotemporal scales. At sub-seasonal lead-time, the timeframe is short enough for the atmosphere to retain some influence from its initial state but also long enough for oceanic variability to affect atmospheric circulation. This turns into an overlapping of different effects that state-of-the-art models struggle to relate.

Foundation Models (FMs) are emerging as a transformative paradigm in artificial intelligence, revolutionising remote sensing and Earth observation through their ability to build general and high-level representations from large-scale datasets. These models leverage Self-Supervised Learning (SSL) techniques to address fundamental challenges in Earth observation, most notably the scarcity of labelled data and the dynamic nature of environmental phenomena. By employing pre-training on vast amounts of unlabeled geospatial data, FMs generate informative representations that can be effectively adapted to multiple downstream tasks with minimal supervised fine-tuning. Once trained, FMs can achieve high performance across diverse applications while adapting to various spatial and temporal contexts with minimal additional training.

In this study, we aim to perform sub-seasonal precipitation prediction by leveraging the general climatic data representations derivable from FMs, augmented with region-specific fine-tuning. The approach focuses on adapting the global-level representation encoded within the model to a specific region, enabling a blending effect in the model’s parameters that captures information across multiple spatial scales and generates a more informed view to predict S2S precipitation. The process is currently focused on model training and calibration, with insights to be shared upon achieving stable performance.

How to cite: Bosso, F., Musto, R., and Panza, L.: Enhancing Subseasonal Precipitation Forecasting with Foundation Models: A Performance-Driven Study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11955, https://doi.org/10.5194/egusphere-egu25-11955, 2025.

The rise of deep learning weather prediction (DLWP) models promises to improve short- to mid-ranged weather forecasts out to 14 days. Deep learning models, however, are known in general to perform poorly in conditions that are represented sparsely in the training data and to generalize poorly out of the distribution of the training data. Translated to weather forecasting, this suggests that DLWP models are inaccurate when predicting extreme events that occur only rarely. These extreme events, however, are of highest interest when preventing danger and damage to societies. Here, we therefore inspect how state-of-the-art DLWP models compare to the numerical weather prediction (NWP) model from the European Center for Medium-Ranged Weather Forecasts (ECMWF) on extreme cold and hot spells over North America and Europe. Our results speak not only for DLWP forecasts under normal conditions, but also promise significant skill improvements when forecasting extreme events with DLWP models, emphasized most stongly on cold spells over North America. Similar but weaker trends are observed in cold spell conditions over Europe, as well as in hot spells over North America and Europe. In general, our findings encourage further research in data driven models, such as Pangu-Weather, GraphCast, Aurora, and ECMWF's AIFS. Notably, the advances in DLWP is directly related to decades of research on NWP models. In future research, we will explore the response of DLWP models to warmer climate scenarios that are expected in the later 21st century.

How to cite: Schaible, A., Karlbauer, M., and Butz, M. V.: Deep Learning Weather Prediction Models Exhibit Outstanding Accuracy when Predicting Cold and Hot Spells over North America and Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11969, https://doi.org/10.5194/egusphere-egu25-11969, 2025.

EGU25-12021 | ECS | Posters on site | CL5.9

Meteorological Analysis and Prediction of Gusts at Istanbul Airport Using Machine Learning Algorithms 

ibrahim akbayır, veli yavuz, Deniz Demirhan, and Berk Münci İnanç

Wind gust is a sudden meteorological weather phenomenon. It can cause many material and moral accidents, especially if it occurs during aircraft take-off and landing at airports. In this study, gust analysis and gust prediction for Istanbul Airport were performed using machine learning algorithms. Metar data of Istanbul Airport between 01.11.2018 and 31.12.2024 were used in the study. When this Metar data was analysed, it was found that on average between 250 and 300 Gust events were reported annually.  Gust values were found to vary between 11 and 65 knots. It was reported that the highest number of gust events was reported in November with 179 times and the lowest number was reported in August with 38 times. When the gust intensities are analyzed, it is seen that the strongest gusts occurred in February. When the gusts were analyzed hourly, it was found that most gusts occurred between 01.00 and 03.00 hours. The most severe gusts occurred between 15.00 and 20.00. In the study, the relationship between gusts and other meteorological variables such as temperature, pressure, dew point temperature was analyzed. In the other part of the study, three different machine learning methods Random Forest (RF), long-short term memory (LSTM) and extreme gradient boosting (XGB) were used to predict gusts. In these methods, models were derived and evaluated on 1000 different randomly selected subsets, 70% for training and 30% for testing. It was observed that the prediction success of the three different models used in the study increased at times of high wind gust values (≥ 30 knots), while the prediction success was lower at times of low wind gust values.

 

How to cite: akbayır, I., yavuz, V., Demirhan, D., and İnanç, B. M.: Meteorological Analysis and Prediction of Gusts at Istanbul Airport Using Machine Learning Algorithms, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12021, https://doi.org/10.5194/egusphere-egu25-12021, 2025.

We present a machine learning based method for predicting extreme precipitation events. This method uses dynamical and thermodynamical variables at coarse resolution as input and the probability of extreme precipitation at higher resolution as the ground truth. Preliminary results show that our detection method, trained on historical EC-Earth3 global climate data and an extreme precipitation mask calculated from the 99th percentile of precipitation from the HCLIM regional model, achieves an accuracy of over 90% for the 2050–2100 period under the SSP126 and SSP370 scenarios within the European domain.
We are working on further improving the method, testing its performance on reanalysis datasets (e.g., ERA5 and CERRA), and adapting it for statistical downscaling and regional climate model emulation.

How to cite: Ivanov, M. and Fuentes Franco, R.: DETEX – Detection of Extreme Precipitation Events in Present and Future Climates at High Resolution Using Machine Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12676, https://doi.org/10.5194/egusphere-egu25-12676, 2025.

EGU25-12774 | ECS | Orals | CL5.9

From Weather Data to River Runoff: Using Spatiotemporal Convolutional Networks for Discharge Forecasting 

Florian Börgel, Sven Karsten, Karoline Rummel, and Ulf Gräwe

The quality of the river runoff determines the quality of regional climate projections for coastal oceans or other estuaries. This study presents a novel approach to river runoff forecasting using Convolutional Long Short-Term Memory (ConvLSTM) networks. Our method accurately predicts daily runoff for 97 rivers within the Baltic Sea catchment by modeling runoff as a spatiotemporal sequence defined by atmospheric forcing. The ConvLSTM model predicts river runoff with an accuracy of ±5% when compared to the hydrological model. Compared to more complex process-based hydrological models, ConvLSTM offers fast processing times and easy integration into climate models, demonstrating its potential as a powerful tool for climate simulation and water resource management.

How to cite: Börgel, F., Karsten, S., Rummel, K., and Gräwe, U.: From Weather Data to River Runoff: Using Spatiotemporal Convolutional Networks for Discharge Forecasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12774, https://doi.org/10.5194/egusphere-egu25-12774, 2025.

EGU25-13004 | ECS | Orals | CL5.9

Analysis of optimal atmospheric predictability using machine learning-based forecasting models 

Robert Brunstein, Christian Lessig, Thomas Rackow, and Jakob Schlör

With the development of highly skillful, machine learning-based weather prediction models over the last 2-3 years, many new possibilities have emerged. These include applications, such as downscaling, temporal interpolation, or generating climate storylines, but also a wide range of scientific questions can be (re)examined with the models. One of these is the study of predictability limits by leveraging the full differentiability of the models. For instance, Vonich and Hakim (2024) demonstrated that optimizing initial conditions using the pre-trained GraphCast model significantly reduces forecasting error, even when used with another machine learning-based forecasting model. While this suggests that the improvement in the initial conditions is not only due to compensation in model error, it remains currently unclear to which extent the initial conditions are enhanced by physically meaningful features.

In our work, we aim to address this shortcoming. As a first step, we analyze whether optimized initial conditions can be identified for a broad range of cases by assessing the forecast skill of the model for a larger set of examples. We evaluate the improvement of the forecasts for several variables dependent on the number of optimization steps, the forecast lead time, and for different models. Subsequently, we consider case studies over Europe and compare the optimized initial conditions with data from independent, high quality datasets, in particular local reanalyses and conventional observations. In this way, we examine if the optimized states are physically better aligned with reference data than the original ERA5 initial conditions. To better understand which of the features in the optimized initial conditions lead to the improved forecast, we analyze the null space of the given machine learning-based weather prediction models. This allows us to obtain insight into the information that is exploited by the models for a forecast. 

Our work will shed light on the intrinsic predictability limits of weather forecasts and also how MLWP can provide forecasts that outperform equation-based weather prediction models.

How to cite: Brunstein, R., Lessig, C., Rackow, T., and Schlör, J.: Analysis of optimal atmospheric predictability using machine learning-based forecasting models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13004, https://doi.org/10.5194/egusphere-egu25-13004, 2025.

EGU25-13581 | Posters on site | CL5.9

Enhancing European heatwave characterization: deep learning-based downscaling of global climate data 

Tian Tian, Hortense Ronzani, Maxime Beauchamp, Jian Su, Kristofer Krus, Shuting Yang, and Ramon Fuentes-Franco

As part of the OptimESM project, this work aims to prototype a framework for downscaling post-CMIP6 Earth System Models (ESMs) to refine long-term projections up to 2300. This effort focuses on understanding regional climate impacts and extreme events, including heatwaves, droughts, and precipitation extremes, with the goal of supporting robust regional climate projections and informing adaptation strategies across Europe. Within this broader context, our study investigates the application of deep learning techniques to downscale daily temperature fields, enhancing the detection and characterization of European heatwaves through improved spatial resolution. Utilizing the open-source DeepR library based on Transformer architecture, we obtained a five-fold downscaling from ERA5 to CERRA datasets. Performance evaluation highlighted significant improvements in detecting heatwaves, particularly in mountainous areas. Integrating high-resolution orography data increases accuracy by 53%, improving the detection rates of heatwave days from 18% (ERA5) to 27% (DeepR) in regions like southern Norway during the validation period 2015-2020. Despite some perceptual improvement, challenges remain in generalizing across spatial domains and accurately modeling temperature distribution tails, which are critical for extreme events. To address these limitations, we explore advanced architectures such as UNet and Diffusion Models, alongside high-resolution land-cover data and enhanced land-sea masks.

How to cite: Tian, T., Ronzani, H., Beauchamp, M., Su, J., Krus, K., Yang, S., and Fuentes-Franco, R.: Enhancing European heatwave characterization: deep learning-based downscaling of global climate data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13581, https://doi.org/10.5194/egusphere-egu25-13581, 2025.

EGU25-14049 | Orals | CL5.9

Application and Evaluation of Data-Driven Weather Prediction (DWP) Model for Climate Modeling 

Chia-Ying Tu, Yu-Chi Wang, Chung-Cheh Chou, and Zheng-Yu Yan

Recent advancements in AI/ML weather prediction models have attracted significant attention for their innovative approaches to forecasting. These models, leveraging deep learning techniques applied to the European Centre for Medium-Range Weather Forecasts (ECMWF) ERA5 reanalysis data, predict future states of meteorological variables iteratively over specific time steps to generate forecasts. Known as Data-Driven Weather Prediction (DWP), this methodology has demonstrated comparable accuracy to Numerical Weather Prediction (NWP) models for certain variables while requiring substantially less computational effort. Despite its advantages, DWP’s reliance on historical data patterns limits its ability to predict extreme or evolving weather phenomena influenced by global warming and climate change. These limitations present challenges for its application in climate simulations and projections.

To address these limitations, this study explored the application of the GraphCast DWP model in climate research, focusing on global climate downscaling and bias correction. Preliminary experiments with 24-hour GraphCast integrations spanning 36 years (1979–2014) demonstrated that GraphCast’s climate integrations closely align with the mean state and trends of the HiRAM climate simulation. Additionally, the model demonstrates variance in precipitation and surface temperature comparable to ERA5. The primary objective of this study is to demonstrate that this innovative approach to global climate modeling provides both computational efficiency and robust performance, effectively capturing climate phenomena while preserving critical information from climate simulations. Furthermore, the proposed methodology underscores the potential of GraphCast to advance global climate modeling, indicating its suitability for future projections conducted by low-resolution climate models.

How to cite: Tu, C.-Y., Wang, Y.-C., Chou, C.-C., and Yan, Z.-Y.: Application and Evaluation of Data-Driven Weather Prediction (DWP) Model for Climate Modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14049, https://doi.org/10.5194/egusphere-egu25-14049, 2025.

EGU25-14190 | Posters on site | CL5.9

Development of a Deep Learning-Based Weather Forecasting Model Using Short-Term Neighborhood Forecast Data 

Sangbeom Jang, Ju-Young Shin, Jiyeon Park, Seoyoung Kim, and Gayoung Lee

Weather forecasting plays a critical role in preventing natural disasters and improving convenience in daily life. However, traditional physics-based numerical weather prediction models have limitations in real-time and high-resolution predictions due to computational complexity and restricted computational resources. This study aims to enhance the predict skill of short-term weather forecasting by utilizing deep learning technologies. Particularly, this study attempts to seek developing methodologies to improve the skill of short-term rainfall forecasts produced by the Korea Meteorological Administration through artificial intelligence. By addressing systemic biases and errors in rainfall prediction data, this research aims to enhance predictive performance. Weather forecast data collected at 1-hour intervals—including temperature, wind speed, humidity, and precipitation—was preprocessed and used as input for the deep learning model. A deep neural network-based architecture was designed for building the forecast model. The model was trained, validated, and evaluated using data spanning the past three years. This study is expected to improve the skill of short-term weather forecasts while enhancing computational efficiency compared to conventional physics-based numerical weather prediction models. Furthermore, the proposed model demonstrates high potential for application in various fields, including disaster management, agriculture, and energy management.

How to cite: Jang, S., Shin, J.-Y., Park, J., Kim, S., and Lee, G.: Development of a Deep Learning-Based Weather Forecasting Model Using Short-Term Neighborhood Forecast Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14190, https://doi.org/10.5194/egusphere-egu25-14190, 2025.

EGU25-14537 | Orals | CL5.9

Developing Extreme Weather Event training datasets to accelerate Machine Learning Applications 

Adrian McDonald and Gokul Vishwanathan

Climate change is increasing the frequency and intensity of Extreme Weather Events (EWEs), which causes widespread disruption globally. As these events intensify, the need for better hazard identification becomes critical. While machine learning (ML) is already enhancing forecasts, and has huge potential for identifying future hazards. To unlock this potential, we need comprehensive training datasets of historic EWEs that integrate and harmonize diverse datasets, account for data collection discrepancies, and address gaps in temporal and spatial records.

This presentation initially discusses the development of an Aotearoa New Zealand EWE database from 1996 to 2021, which currently includes occurrence data derived from subjective classifications from the national weather service, research organizations, and insurance information. Careful analysis of that database and ancillary reanalyses output can successfully characterise rainfall extreme intensities by deriving duration, peak rainfall, and total accumulation.

Building on that work, this presentation will discuss the development and testing of a methodology to integrate extreme weather event (EWE) occurrence, intensity, and storm track data into a unified database. By processing this combined dataset, we aim to harmonise data from the disparate sources and improve data accuracy and reliability, making it robust for future ML analyses. We also use our experience of applying ML classification schemes in climate research to provide proof-of-concept applications demonstrating the value of our harmonisation methodology.

How to cite: McDonald, A. and Vishwanathan, G.: Developing Extreme Weather Event training datasets to accelerate Machine Learning Applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14537, https://doi.org/10.5194/egusphere-egu25-14537, 2025.

EGU25-15547 | Orals | CL5.9

AI- enhanced seasonal predictions of Mediterranean cyclones 

Leone Cavicchia, Guido Ascenso, Luca Proserpio, Enrico Scoccimarro, Silvio Gualdi, Matteo Giuliani, and Andrea Castelletti

Intense cyclones form frequently in the Mediterranean region, with the potential to cause damage to life and property when they hit highly populated coastal areas. Cyclone impacts are caused by the associated strong winds, flash flooding and storm surge. The social and economic impacts are not limited to the Mediterranean area, as cyclones forming in the region can affect Central Europe. While the skill of weather models to forecast such events has dramatically improved over the last decade, the seasonal predictability of Mediterranean cyclones lags behind due to the limitations on horizontal resolution in probabilistic forecasts requiring a large ensemble of simulations. Improving the prediction at a seasonal scale of those extreme events would be of great benefit for society, enabling better disaster risk management and reducing the economic losses they cause. A better prediction of climate extremes would also directly benefit a number of economic sectors such as the insurance and re-insurance industry.

The goal of this work, within the CLINT Horizon project, is to use Artificial Intelligence techniques to enhance the skill of a state-of-the-art seasonal prediction system for predicting Mediterranean cyclones. Here we present results making use of a hybrid AI approach linking the occurrence of those extreme events to their large-scale drivers. The training and validation of different machine learning models is performed using ERA5 reanalysis data. The trained models are then applied to the output of the CMCC operational seasonal forecasts in hindcast mode, and the skill of the modelling chain is assessed. The performance of machine learning models of varying complexity (e.g. random forest, gradient boosting, convolutional neural networks) is evaluated.

How to cite: Cavicchia, L., Ascenso, G., Proserpio, L., Scoccimarro, E., Gualdi, S., Giuliani, M., and Castelletti, A.: AI- enhanced seasonal predictions of Mediterranean cyclones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15547, https://doi.org/10.5194/egusphere-egu25-15547, 2025.

EGU25-15750 | ECS | Posters on site | CL5.9

Sub-seasonal Prediction of Agricultural Drought in India Using Long-Short-Term Memory Networks 

Saurabh Verma and Karthikeyan Lanka

Agricultural drought (AGD), defined by a deficit in soil moisture, is a complex natural hazard phenomenon that causes extreme damage to water supply, food production, and socio-economic loss at different time scales. India is a developing country, and 60% of its population depends on agriculture. India has experienced frequent extreme drought conditions in the last few decades, for example, the 2015-16 North Indian and 2017-18 Southern Indian drought, where more than 330 million people were affected due to food unavailability and shortage in groundwater resources. The spatial patterns of AGD vary significantly in India due to uncertainty in regional climatic conditions caused by the immense increase in global warming. The prediction of agricultural drought at a sub-seasonal scale would help the farming community to plan appropriate crops for the season and conserve water for irrigation.

This study proposes a statistical framework to predict the agricultural drought with 1-, 2-, and 3-month lead times over the Indian subcontinent. Soil moisture percentiles (SMP) are utilised as a drought index where values less than 20th percentiles represent drought conditions. SMP is a widely used drought index in research because it directly represents the water content in the soil and responds relatively quickly to changes in soil water content due to variations in rainfall and irrigation. The variation of SMP depends on various hydroclimatic parameters at local and non-local scales. Thus, this study has considered the air temperature (max. and min.), Potential Evapotranspiration, Vapour Pressure Deficit, Rainfall, soil moisture percentile, Normalised Difference Vegetation Index, El-Nino southern oscillation, North Atlantic Oscillation, Indian Ocean Dipole, Pacific Decadal Oscillation, and Madden Julian Oscillation as a predictor (or feature) from the various satellite (NOAA-19, 20, and AVHRR) and observational (IMD – Indian Meteorological Department) data sources. The Long-Short-Term Memory (LSTM) model, with an MSE custom loss function, is used to forecast agricultural drought. The model was trained from June 1981 to May 2015 and tested at each grid point cell between June 2015 and May 2022. The model performance is examined using Pearson’s correlation > 0.6 for a 1-month lead and further decreased for a 2 and 3-month lead. The forecasting matrices such as percentage porrect, POD, FAR, and ETS indicated that the predictability of AGD is comparably high over northern, southern, and north-eastern India. At last, the trained models are used to discover variables that, depending on feature relevance, influence agricultural drought predictability on a sub-seasonal scale. The result shows that vapour pressure deficit followed by maximum temperature, Pacific decadal oscillation, and soil moisture percentile are the primary features that control drought predictability.

How to cite: Verma, S. and Lanka, K.: Sub-seasonal Prediction of Agricultural Drought in India Using Long-Short-Term Memory Networks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15750, https://doi.org/10.5194/egusphere-egu25-15750, 2025.

EGU25-17884 | ECS | Orals | CL5.9

Predicting Hot Spell Duration with Random Forests 

Duncan Pappert, Mathieu Vrac, Dim Coumou, Alexandre Tuel, and Olivia Martius

High summer temperatures place significant stress on human and natural systems, often leading to severe impacts. Summer hot spells vary widely in terms of intensity and duration, yet event duration is often overlooked or considered a secondary aspect when it comes to studying and predicting such extremes. Different sectors in society, the economy, and the environment are vulnerable to extreme heat on different timescales; therefore, knowing  the likelihood of a heat event lasting only a few days or surviving over many weeks is crucial for developing more effective adaptation strategies.

In the last decade, machine learning (ML) techniques have increasingly been used to tackle extreme weather forecasting. Among these, Random Forests (RF) have emerged as an effective tool proven to have some skill in predicting the occurrence and mean amplitude of extreme near-surface temperature events. To the best of our knowledge, such statistical models have yet to be used for the purpose of predicting hot spell duration. This study aims to fill that gap.

The objective of this research is to assess whether a random forest (RF) model can predict the duration of a hot spell from its first day. Specifically, we aim to determine if the model can distinguish between short and long durations, covering both synoptic and subseasonal timescales. To achieve this, we develop a statistical model using data from the Community Earth System Model version 2 Large Ensemble (CESM2-LE) historical runs. For two regions in Western Europe, hot spells are defined as periods when the region-averaged deseasonalised and detrended anomalies exceed 1.5 standard deviations. The model is trained with a number of local and remote predictors, incorporating variables from the land, sea, and atmosphere. These features are provided for the days, weeks and months leading up to the event, as well as for the first day of the event itself.

We perform both a RF classification to predict different duration cohorts (short, medium, long) and a Quantile Random Forest (QRF) to model the full conditional distribution of the response variable (event duration). A key challenge is handling a highly imbalanced dataset, with 3-day events far outnumbering events lasting beyond 10 days.

In addition to shedding light on the statistical and dynamical relationships that drive the persistence of hot spells, the results could be relevant for climate adaptation and policy planning.

How to cite: Pappert, D., Vrac, M., Coumou, D., Tuel, A., and Martius, O.: Predicting Hot Spell Duration with Random Forests, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17884, https://doi.org/10.5194/egusphere-egu25-17884, 2025.

EGU25-18929 | ECS | Posters on site | CL5.9

Sphere Fusion Forecast (SFF): A Neural Operator–Based Model for Global Weather Forecasting 

Qilong Jia, Zhixiang Dai, Chenyu Wang, Ivan Au Yeung, Hao Jing, Rita Zhang, Jian Sun, and Wei Xue

Weather forecasting is crucial for human activities, yet traditional numerical models often face limitations due to complex physical processes and high computational cost. Deep learning–based neural networks offer a promising alternative. The Spherical Fourier Neural Operator (SFNO) model introduces the Spherical Harmonic Transform to maintain SO(3) rotational invariance, ensuring long-term stability in forecasts and preventing early collapse. However, we have identified two key shortcomings in SFNO: high memory consumption and limited ability to capture high-frequency information due to the truncated of spectrum.

To address these issues, we propose the SFF model, which improves upon the well-known SFNO model primarily in the following ways:

  • a) U-Structure: We add up-sampling and down-sampling operators between SFNO blocks, allowing the initial and final stages of the SFNO block chain to handle broader frequency spectra, while the middle layers focus on relatively low-frequency information. Under a limited memory budget, this design enables us to increase the number of SFNO blocks or enlarge the embedding dimension, thereby enhancing forecast accuracy.
  • b) Vision Transformer-like Residual Connection: We introduce a Vision Transformer–like architecture between the encoder and decoder as the skip connection, and specialize it to focus on local features. This strengthens the model's ability to capture high-frequency information, enhances its capacity for local feature learning, and leads to more robust and accurate predictions.

 

Considering the discontinuous occurrence and development of precipitation, SFF employs an independent precipitation model which can be easier to learn the physical processes of precipitation and leverages classification weighting to improve the detection and prediction accuracy of heavy rainfall, further extending the effective lead time of precipitation forecasts through joint training.

 

We conducted experiments on ERA5 dataset, using data from 1979–2017 for training, 2018 for validation, and 2020 for testing. The experiment results demonstrate that SFF can generate  stable 30-day forecasts cost-effectively on a single NVIDIA H20 GPU, with key metrics—such as the root mean square error (RMSE) and anomaly correlation coefficient (ACC) for Z500/t2m/t850 comparable to the well-established IFS model, and better than the SFNO model. Meanwhile, for precipitation predictions, SFF also exhibits a forecast skill level comparable to that of the IFS model. Moreover, for heavy rainfall prediction, SFF achieves a Threat Score (TS) of over 0.25 in single-step forecasts for 70 mm of precipitation. After joint training of SFF and the precipitation model, the precipitation score within 10-day forecasts can be improved by 5% compared to direct coupling. This study underscores the potential of Neural Operator–Based AI models in advancing weather forecasting and extreme weather prediction.

How to cite: Jia, Q., Dai, Z., Wang, C., Au Yeung, I., Jing, H., Zhang, R., Sun, J., and Xue, W.: Sphere Fusion Forecast (SFF): A Neural Operator–Based Model for Global Weather Forecasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18929, https://doi.org/10.5194/egusphere-egu25-18929, 2025.

EGU25-19014 | Orals | CL5.9

Building a high-resolution machine learning weather model 

Karolina Stanisławska and Olafur Rognvaldsson

After numerous successful applications of machine-learning-based global weather models, a new interesting direction of application is to seek high-resolution regional ML-based models that could complement high resolution numerical models serving day-to-day purposes. Development of such a model would combine speed and resource efficiency of ML models with high-resolution capabilities available so far only in the numerical models. Most ML-based models created so far are restricted to the resolution of underlying ERA5 data, often further downsampled due to various constraints, leaving substantial room for further research. With the objective of building a high-resolution ML model for Iceland and equipped with 30 years of 2-km reanalysis data covering Iceland and the surrounding ocean, we are exploring possibilities of the applications of existing ML architectures to our domain. The model we are currently building is based on ClimaX architecture from Microsoft, which we are modifying to best serve our objectives. Understanding the unique needs of regional models during training is one of the key factors in generating a successful regional model. While some of the architectures of the available global models can be applied directly to build a local model, many questions arise: do we need to adjust the cost function during training to handle domain boundaries? Which model levels should we prioritize during training — would it be better to focus on lower levels if the resolution is high and the timescale is short? To what extent can we use transfer learning (leveraging pre-trained weights from the global experiment) and how much will it guide the model toward the optimum? In this talk, we will discuss some of the above considerations for successfully running a regional model and present our high-resolution model for Iceland. The successful development of large machine-learning-based weather models has given weather and climate scientists confidence that models and reanalysis data built over decades are capable of capturing enough variability for ML-based inference. This now opens a new world of possibilities for model improvements and scientific advancements.

How to cite: Stanisławska, K. and Rognvaldsson, O.: Building a high-resolution machine learning weather model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19014, https://doi.org/10.5194/egusphere-egu25-19014, 2025.

EGU25-19963 | Posters on site | CL5.9

AI-based Short-Term Wind Speed Forecasting for Real-Time Applications. 

Marcos Martínez-Roig, Nuria P. Plaza-Martín, César Azorín-Molina, Kevin Monsalvez-Pozo, Miguel Andrés-Martin, Deliang Chen, Zhengzhong Zeng, Sergio M. Vicente-Serrano, Tim R. McVicar, Jose A. Guijarro, and Amir Ali Safaei-Pirooz

The generation of accurate and reliable short-term forecasts (<12 hours) of near-surface (~10 m above ground level) gridded wind speed data, hereinafter called NSWS, are crucial for various socioeconomic and environmental applications. For instance, in the face of climate change, accurate wind speed predictions can contribute to the decarbonization of the electricity grid by optimizing the wind energy generation

Traditional NSWS forecasting methods relies on Numerical Weather Prediction (NWP) models, which require significant computational resources, particularly when high spatial and temporal resolution are required. Moreover, these models often yield inaccurate results, especially in regions with complex topography. As a more efficient alternative to this pressing issue, the Climatoc-Lab, as part of the PTI+Clima, is exploring Artificial Intelligence (AI) methods to enhance the efficiency and accuracy of short-term NSWS predictions. We propose the use of two deep learning methods:

  • A U-Net architecture based on Partial Convolutions to generate high-resolution hourly NSWS maps from station-based observations.

  • An encoder-decoder architecture based on mixed convolutional and recurrent (ConvLSTM) layers to predict short-term NSWS maps using the generated infilled data as input.

This AI-based product, designed as an early warning system, generate high-resolution (~3/9-km) short-term (12 h; 1-h resolution) NSWS forecasts in near real-time (seconds) using a GPU.

Measurements from meteorological station networks provide accurate site-specific observations, capturing local wind effects, but with limited spatial coverage, being sparse and almost absent in mountainous and remote areas. Conversely, reanalysis and simulation products offer complete spatial coverage at low resolution but fail to accurately reproduce local NSWS. Our AI-based tool combine the strenghts of both worlds, as it is trained using both, observation and simulation data. The observations are provided by the Spanish Meteorological State Agency (AEMET), while the simulation data comes from reanalysis like ERA5-Land (9-km).

The AI-based tool achieves a high correlation of 0,96 for Infilling and 0,849 for Prediction for the year 2020 of ERA5-Land data used for validation, with potential for further improvements. This also shows a reasonably high correlation of 0,84 with the AEMET meteorological observations. This scalable AI-based approach promises to enhance short-term NSWS forecasting for AEMET and other meteorological services, highlighting the promising role of AI to improve both forecast precision and operational efficiency in meteorology applications.

How to cite: Martínez-Roig, M., Plaza-Martín, N. P., Azorín-Molina, C., Monsalvez-Pozo, K., Andrés-Martin, M., Chen, D., Zeng, Z., Vicente-Serrano, S. M., McVicar, T. R., Guijarro, J. A., and Safaei-Pirooz, A. A.: AI-based Short-Term Wind Speed Forecasting for Real-Time Applications., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19963, https://doi.org/10.5194/egusphere-egu25-19963, 2025.

EGU25-20607 | ECS | Orals | CL5.9

Beyond the Unseen: Assessing AI Climate Emulators’ Capacity to Simulate Very Rare Events 

Alexander Wikner, Troy Arcomano, Amaury Lancelin, Karan Jakhar, Dhruvit Patel, Freddy Bouchet, and Pedram Hassanzadeh

The risk of extreme weather under climate change is of paramount importance, but remains one of the most difficult problems to study using conventional physics-based global climate models (GCMs). This is due to the high uncertainty in estimates of extreme weather return times owing to the computational cost of evolving these models for long enough to observe very rare events. AI models trained on historical reanalysis to emulate the dynamics of the global atmosphere have demonstrated both high forecast accuracy and greatly reduced computational cost. Some of these AI emulators can generate stable, decades-long trajectories, which, in conjunction with their affordability, have the potential to greatly reduce extreme weather uncertainties. However, it is impossible to validate if AI emulations can accurately estimate the risk of extreme weather events with return times longer than the historical record. In a first-of-its-kind experiment to assess this capability, we simulate 100,000 years of a stationary climate using PlaSim, a coarse resolution GCM. We then train a selection of stable AI emulators using only 100 years of data, and compare the emulated and true return times of extreme heat waves over Western Europe and the Pacific Northwest. We finally assess how the addition of a land moisture component to these AI emulators improves the accuracy of return time estimates.

How to cite: Wikner, A., Arcomano, T., Lancelin, A., Jakhar, K., Patel, D., Bouchet, F., and Hassanzadeh, P.: Beyond the Unseen: Assessing AI Climate Emulators’ Capacity to Simulate Very Rare Events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20607, https://doi.org/10.5194/egusphere-egu25-20607, 2025.

EGU25-2679 | ECS | Posters on site | AS1.7

Improving Subseasonal Prediction of Summer Extreme Precipitation Over Southern China Based on a Deep Learning Method 

Yang Lyu, Xiefei Zhi, and Shoupeng Zhu

The reliable Subseasonal-to-Seasonal (S2S) forecast of precipitation, particularly extreme precipitation, is critical for disaster prevention and mitigation, which however remains a great challenge for mission agencies and research communities. In this study, a deep learning method based on U-Net with additional atmospheric factor forecasts (e.g., wind and specific humidity at multiple levels) included is proposed to correct the S2S forecasts of summer precipitation derived from European Centre for Medium-range Weather Forecasts (ECMWF) over Southern China. The weighted loss function integrated by mean square error and threat score is introduced to capture extreme precipitation more precisely. Generally, the U-Net model improves forecast skills in terms of both general statistics and extreme events, showing prominent superiorities to the ECMWF and quantile mapping (QM) forecasts. Importantly, it shows pronounced calibrations on extreme precipitation forecasts at lead times of 3-4 weeks with the averaged HSS increased by ~5%, which shows higher improvement magnitudes than those at lead times of 1-2 weeks. For all lead times, the greatest forecast skills are mainly distributed over the middle and lower reaches of the Yangtze River basin, presenting HSS of greater than 30% even for the 4-week lead time. Predictor importance analyses show that at the 1-week lead time, the U-Net forecast skills are mainly derived from the synchronous precipitation forecasts. With the increasing lead times, the contributions from the atmospheric variables (especially those associated with moisture flux) rise rapidly. Therefore, the channel combining numerical weather prediction model and deep learning framework is demonstrated promising in S2S precipitation forecasts. Thus, combining numerical models and deep learning is very promising in subseasonal precipitation forecasts and can also be applied to the routine forecast of other atmospheric and ocean phenomena in the future.

How to cite: Lyu, Y., Zhi, X., and Zhu, S.: Improving Subseasonal Prediction of Summer Extreme Precipitation Over Southern China Based on a Deep Learning Method, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2679, https://doi.org/10.5194/egusphere-egu25-2679, 2025.

Based on an elliptic orbit representation of the yearly varying annual cycles of the Northern Hemisphere stratospheric polar vortex (SPV) from 1979 to 2021, we develop a statistical model to predict the parameters of the SPV’s elliptic orbit on a yearly basis. The predictors include indices describing the phase of key climate modes, such as ENSO and the quasi-biennial oscillation (QBO), as well as the initial state of the polar stratosphere, all derived from prior seasons. Our results demonstrate that the predicted annual SPV evolution, initialized on October 1, provides skillful forecasts with anomaly correlation skill exceeding 0.7 throughout the November-to-March period. In particular, our forecasts can accurately predict the timing and magnitude of peak vortex strength, the timing of the final warming, as well as providing insights into the sub-seasonal evolution of the vortex.

How to cite: Secor, M.: Long-Lead Forecasts of the Yearly Varying Annual Evolution of the Northern Hemisphere Stratospheric Polar Vortex, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3789, https://doi.org/10.5194/egusphere-egu25-3789, 2025.

Subseasonal-to-seasonal (S2S) precipitation forecast skill is critical for sectors that depend on medium-range forecasts, such as energy grid management, irrigated agriculture, drought and flood mitigation, and long-term water supply planning. Reliable S2S forecasting models are essential for adapting water resource management practices to shifts in hydroclimatology. To improve these forecasts, it is important to understand the factors that influence S2S precipitation. While short and long-range forecasts are relatively accurate, the skill of S2S forecasts—ranging from 15 to 90 days—is often less reliable. Understanding the current skill of S2S precipitation forecasts and identifying the factors that contribute to this skill is key to operationalizing these models. Known influences on S2S precipitation across the Conterminous United States (CONUS) include large-scale atmospheric circulation patterns and climate oscillations, such as the El Niño-Southern Oscillation (ENSO), Madden-Julian Oscillation (MJO), Pacific Decadal Oscillation (PDO), and Atlantic Multidecadal Oscillation (AMO). This study investigates the contribution of several different hydroclimatic indices on S2S precipitation forecast skill of the European Centre for Medium-Range Weather Forecast (ECMWF) Model.  The attribution analysis considers the correlation of the absolute error between forecast and observed precipitation values with each of the indices including Niño-3.4, MJO, PDO, AMO, Pacific North American Pattern (PNA), and North Atlantic Oscillation (NAO) for lead times of 15-90 days and for four forecast-initialized seasons: a) JFM, b) AMJ, c) JAS, and d) OND. Additionally, feature importance is evaluated using lasso regression for feature selection and principal component analysis. As climate change exacerbates hydroclimatic extremes, developing accurate forecasting models is essential for preparing for future uncertainties.

How to cite: Levey, J.: Subseasonal-to-Seasonal (S2S) Forecast Skill Attribution across the United States, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3926, https://doi.org/10.5194/egusphere-egu25-3926, 2025.

EGU25-4253 | ECS | Orals | AS1.7

Unraveling the sources of subseasonal predictability with machine learning 

Ana-Cristina Mârza, Daniela I.V. Domeisen, Lorenzo Ramella-Pralungo, and Angela Meyer

Actionable weather information at the subseasonal timescale informs decision-makers in many societally relevant sectors, including energy demand and supply. However, the predictive skill of subseasonal forecasts varies widely: from forecast ‘busts’ with low predictive skill, to windows of opportunity yielding exceptionally skillful forecasts. It is therefore useful to know ahead of time if a given forecast will be skillful enough to form the basis of operational planning: i.e., along with the forecast itself, users wish to have an a priori estimate of the forecast uncertainty. We propose to achieve this with machine learning (ML). In our study, an ML model trained on historical weather data learns to relate the forecast initial conditions to the probabilistic forecast error at subseasonal lead times. As opposed to ensemble forecasting, this is a computationally cheaper approach to estimate the forecast skill. Moreover, explainability techniques allow us to rank the sources of subseasonal predictability in hindcast data by their importance; a first to our knowledge.

Building on studies that examine the link between the forecast skill of the European Centre for Medium-range Weather Forecasts (ECMWF) subseasonal ensemble model, and the atmospheric conditions at forecast initialization time (weather regime, season, phase of the Madden-Julian Oscillation), we propose a decision-tree-based approach to predicting future forecast skill from past observations. Concretely, a gradient boosted decision tree model is trained to predict the Continuous Ranked Probability Score (CRPS) of ECMWF hindcasts at lead times 0-46 days, by leveraging initial conditions (geopotential height, sea surface temperature, zonal wind speed) extracted from the Earth System Reanalysis 5 (ERA5) dataset. The ERA5 data undergo dimensionality reduction (e.g., principal component analysis) before being fed to the ML model, and are supplemented with pre-computed indices like the El Niño-Southern Oscillation Index. Forecast skill is computed for the 500 hPa geopotential height field in the European region with respect to ERA5 ground truth.

The ML model outperforms a climatological baseline (averaged CRPS by calendar date and lead time) at the task of predicting European forecast skill out to week 7. We find the most important predictor of skill to be the strength of the stratospheric polar vortex, in addition to lead time and calendar date. Training separate models by lead time reveals clear differences in feature importance, such that, for example, lead time contributes the most predictability in the first 2 weeks, while the seasonal cycle is a strong predictor in weeks 3-4. Different teleconnections become important at different lead times, but their predictive potential also fluctuates throughout the year. We will provide an in-depth breakdown of the feature importances by lead time and season in our presentation.

In conclusion, machine learning provides a novel way to estimate a priori the forecast skill of numerical weather prediction models. The presented method enables us for the first time to rank the relative contributions of the sources of forecast skill, as deduced from hindcast data, thereby advancing our understanding of subseasonal predictability.

How to cite: Mârza, A.-C., Domeisen, D. I. V., Ramella-Pralungo, L., and Meyer, A.: Unraveling the sources of subseasonal predictability with machine learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4253, https://doi.org/10.5194/egusphere-egu25-4253, 2025.

EGU25-4325 | ECS | Posters on site | AS1.7

The coupling of MJO with oceanic Kelvin waves in the three major oceanic basins 

Fernando Belinchón Martín

The Madden-Julian Oscillation (MJO) is a critical component of tropical intraseasonal variability, influencing global weather patterns. This study investigates the interaction between the MJO and oceanic waves, specifically Kelvin waves, using indices from Wheeler and Hendon (2004) for the MJO and Rydbeck (2019) for sea surface height (SSH) anomalies. Our methodology involves cross-referencing the phases of the MJO with the phases of the Kelvin Index. We contrast the MJO days with significant oceanic Kelvin wave activity with those when the Kelvin wave signal is weak. By analyzing these intersections, we aim to elucidate the coupling of oceanic waves and the MJO across the three major ocean basins.

Our findings indicate that during significant Kelvin wave activity, there is enhanced convection and more clearly defined oceanic wave structures within the MJO phases in the Pacific basin. This suggests a strong coupling between atmospheric and oceanic processes, where the presence of Kelvin waves can amplify convective activity associated with the MJO. Additionally, we observed that during periods of weak Kelvin wave signals, the MJO tends to be weaker, with more diffuse wave structures. Conversely, in the Atlantic basin, MJO’s impact on ocean Kelvin waves involves episodes of atmospheric convective anomalies over the Amazon, which tend to be related with stronger MJO previous activity in the western Pacific. For the Indian basin, the methodology is able to discriminate the oceanic Kelvin waves triggered by equatorial wind stress anomalies associated with MJO.

We also evaluate 30-yr long simulations from storm-resolving coupled models performed in the framework of EU-NextGEMS project to evaluate their performance in simulating MJO’s footprint on the ocean.

This study provides new insights into the complex dynamics of the MJO and its interaction with oceanic waves, highlighting the importance of considering both atmospheric and oceanic components in understanding tropical variability. The results have significant implications for improving the predictability of the MJO and its associated weather impacts, offering potential advancements in climate modeling and forecasting.

How to cite: Belinchón Martín, F.: The coupling of MJO with oceanic Kelvin waves in the three major oceanic basins, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4325, https://doi.org/10.5194/egusphere-egu25-4325, 2025.

EGU25-4729 | ECS | Orals | AS1.7

Seasonal AFNOCast: A Deep Learning Approach for Enhanced Regional Seasonal Predictions 

Rebecca Wiegels, Julius Polz, Luca Glawion, Jan Niklas Weber, Tanja Schober, Christof Lorenz, Christian Chwala, and Harald Kunstmann

Regionalized seasonal forecasts allow improved decision making, particularly when applying the meteorological forecasts to sectors such as agriculture or water management. In regions like the Blue Nile Basin, a transboundary catchment in East Africa, reliable seasonal predictions are crucial for addressing local needs due to the complex topography combined with high dependency on water resources.

In this study, we introduce Seasonal AFNOCast, a Deep Learning (DL) approach designed to bias-correct and downscale global seasonal forecasts (SEAS5). The objective is to provide a computational efficient approach that provides reliable ensembles, realistic and skillful predictions at a daily and monthly scale. The regionalized forecast provides 51 ensemble members with a 215 day forecast horizon of a spatial resolution of approximately 9 km.

Seasonal AFNOCast is a DL network that applies a specific type of transformer, called the Adapted Fourier Neural Operator (AFNO), in combination with an ensemble-member-specific architecture. The network is trained with the ERA5-Land reanalysis product as reference using an ensemble specific loss function. Its performance is evaluated against Bias-Correction and Spatial Disaggregation (BCSD), a well-established statistical baseline method for post-processing global seasonal forecasts. The evaluation includes comprehensive skill metrics such as the continuous ranked probability score (CRPS), normalized rank histograms, and precipitation-specific metrics, along with qualitative analyses.

Our analysis demonstrates that Seasonal AFNOCast delivers skillful regionalized seasonal predictions that are comparable to, and in specific cases outperform, state-of-the-art statistical methods. These findings underscore the potential of DL-based post-processing of seasonal forecasts, particularly in challenging regions like the Blue Nile Basin.

How to cite: Wiegels, R., Polz, J., Glawion, L., Weber, J. N., Schober, T., Lorenz, C., Chwala, C., and Kunstmann, H.: Seasonal AFNOCast: A Deep Learning Approach for Enhanced Regional Seasonal Predictions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4729, https://doi.org/10.5194/egusphere-egu25-4729, 2025.

EGU25-5407 | ECS | Orals | AS1.7

Convectively Coupled Tropical Waves and Their Influence on Rainfall in Tropical Australia: Observations and Predictability 

Fadhlil Rizki Muhammad, Claire Vincent, Andrew King, and Sandro W. Lubis

Convectively coupled tropical waves (CCTWs) are modes of intra-seasonal variability that affect circulation and rainfall in the tropics. Here, we specifically examine their impact on Australian rainfall and circulation, as well as their representation in sub-seasonal-to-seasonal (S2S) models, and their predictability. Our findings reveal that CCTWs with off-equatorial convective centres, such as equatorial Rossby waves (ER), mixed Rossby-gravity waves (MRG), and tropical depression-type waves (TD-type), significantly increase the likelihood of extreme rainfall (above the 90th percentile) during austral summer. Specifically, ER waves enhance the probability by approximately 1.5 to 2.4 times, while MRG and TD-type waves increase it by 1.4 to 1.6 times relative to the seasonal average. These effects are comparable with the Madden-Julian Oscillation (MJO), which increases the probability of extreme rainfall by around 1.3 – 2.7 times compared to the seasonal probability. The increased likelihood of extreme rainfall is attributed to the increase in moisture convergence and advection driven by wave activity. These findings highlight the potential to improve S2S predictions by incorporating CCTWs, thereby increasing the accuracy of extreme event forecasts in tropical Australia.

                  The representation of CCTWs is then assessed in the operational Australian S2S model, ACCESS-S2, a coupled atmosphere-ocean model. We use a 38-year seasonal hindcast period to evaluate representation of CCTWs. We show that the predictability of ER waves and MJO in the filtered outgoing longwave radiation (OLR) field during austral summer extends out to around 9 and 16 days, respectively (r > 0.5). Meanwhile, other CCTWs have shorter skill forecast periods. Space-time spectral analysis also shows that the representation of CCTWs in the OLR field is underestimated. In particular, the relative OLR spectral power of ER waves, Kelvin waves, and the MJO are 20 – 30% less than observations. Moreover, the MRG waves are nearly non-existent in the model. More skill is identified using the filtered lower-level zonal wind (U850), both in terms of predictability and spectral amplitude. For example, considering the U850 only, predictability extends to around 11 days for ER waves and 18 days for the MJO, and the U850-spectra of ER waves mostly indicates less than 10% difference compared to observations, while Kelvin waves and the MJO show less than around 20% differences. However, the MRG is still non-existent in the U850 field. Further cross-spectral analysis demonstrates that there is a weak convection-circulation coupling bias in the model. Overall, this study highlights the role of CCTWs in driving extreme rainfall in tropical Australia through their coupling with convection and circulation. This also identifies current limitations and emphasizes the need to improve the representation of CCTW variability in S2S models to ultimately enhance extreme rainfall prediction in this region.

How to cite: Muhammad, F. R., Vincent, C., King, A., and Lubis, S. W.: Convectively Coupled Tropical Waves and Their Influence on Rainfall in Tropical Australia: Observations and Predictability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5407, https://doi.org/10.5194/egusphere-egu25-5407, 2025.

EGU25-6102 | ECS | Posters on site | AS1.7

Investigating the role of the Madden-Julian Oscillation in Antarctic sea ice variability 

Arnab Sen, Pranab Deb, Adrian Matthews, and Manoj Joshi

In the tropics, deep convection triggers upper-level quasi-stationary Rossby waves that propagate to higher latitudes and influence local climate patterns. This study examines the teleconnection between the Madden-Julian Oscillation (MJO), the dominant mode of tropical intraseasonal variability, and Antarctica, using daily gridded observational datasets (precipitation from CMAP, 250-hPa geopotential height, 2 m air temperature, and 10 m winds from ERA5, and sea ice concentration from NSIDC) and the Linear Response Theory Method (LRTM) across all southern seasons during 1979-2014. Our results reveal that MJO-driven variations in surface temperature and winds substantially affect Antarctic sea ice concentration throughout the year. In austral summer and autumn, significant sea ice responses are evident in both the eastern (Lazarev Sea to Somov Sea) and western Antarctic sectors (Ross Sea, Amundsen Sea, and Weddell Sea). During summer, the most notable sea ice changes occur in MJO phases 1 and 5, while in autumn, the most potent responses are associated with phases 1–3. Conversely, in winter and spring, the sea ice responses are primarily restricted to the western Antarctic sectors (Ross Sea, Amundsen Sea, Bellingshausen Sea, and Weddell Sea). All MJO phases exert a pronounced influence on sea ice in winter, whereas in spring, phases 1 and 5 dominate. The LRTM effectively elucidates the mechanisms underlying these changes, attributing the observed sea ice variability to wind-driven forcing, thermal advection, or their combined effects.

How to cite: Sen, A., Deb, P., Matthews, A., and Joshi, M.: Investigating the role of the Madden-Julian Oscillation in Antarctic sea ice variability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6102, https://doi.org/10.5194/egusphere-egu25-6102, 2025.

EGU25-7776 | Posters on site | AS1.7

Effect of Parameter Variation in the BMJ Scheme on the Simulation of MJO Propagation and Structure 

Xiaoyu Zhu, Zhong Zhong, and Wei Lu

In this study, the Betts-Miller-Janjić (BMJ) convective adjustment scheme in the Weather Research and Forecasting (WRF) model version 4.0 was used to investigate the effect of its α-parameter, which influences the first-guess potential temperature reference profile on the Madden‒Julian oscillation (MJO) propagation and structure. This study diagnosed the MJO active phase composites of the MJO-filtered outgoing longwave radiation (OLR) during the December-to-January (DJF) period of 2006–2016 over the Indian Ocean (IO), Maritime Continent (MC), and western Pacific (WP). The results show that the MJO-filtered OLR intensity, propagation pattern, and MJO classification (standing, jumping, and propagating clusters) are sensitive to the α-value, but the phase speeds of propagating MJOs are not. Overall, with an increasing α-value, the simulated MJO-filtered OLR intensity increases, and the simulated propagation pattern is improved. Results also show that the intensity and propagation pattern of an eastward-propagating MJO are associated with MJO circulation structures and thermodynamic structures. As α increases, the front Walker cell and the low-level easterly anomaly are enhanced, which premoistens the lower troposphere and triggers more active shallow and congestus clouds. The enhanced shallow and congestus convection preconditions the lower to middle troposphere, accelerating the transition from congestus to deep convection, thereby facilitating eastward propagation of the MJO. Therefore, the simulated MJO tends to transfer from standing to eastward propagating as α increases. In summary, increasing the α-value is a possible way to improve the simulation of the structure and propagation of the MJO.

How to cite: Zhu, X., Zhong, Z., and Lu, W.: Effect of Parameter Variation in the BMJ Scheme on the Simulation of MJO Propagation and Structure, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7776, https://doi.org/10.5194/egusphere-egu25-7776, 2025.

EGU25-7926 | Posters on site | AS1.7

Subseasonal activities of tropical cyclones over the western North Pacific in GloSea6 

Eunji Kim, Taehyung Kim, and Dong-Hyun Cha

Tropical cyclones (TCs), which often form over the western North Pacific (WNP), have a large socioeconomic impact and result in destructive damage in East Asian countries. Therefore, it is crucial to estimate TCs characteristics and predict TCs using the model. This study analyzed the subseasonal predictability of TC activities over the WNP region from June to September, using 24 years (1993–2016) of 21-member ensemble hindcasts generated by the Global Seasonal Forecast System version 6 (GloSea6). We analyzed TC activities using dynamic genesis potential index (DGPI) developed by Wang and Murakami, and tracking algorithm (i.e., TempestExtremes (TE)). Compared to IBTrACS best track data, these two methods captured TC genesis points well and showed high correlation in TC genesis density. However, particularly in the South China Sea (SCS), a negative bias was observed in TE, while GPI exhibited a positive or zero bias. Despite using the same input data, different results were observed in this region, and we analyzed the reasons for this discrepancy in two parts. First, why does such a bias occur in DGPI? Second, what causes the differences between DGPI and TE? We used ERA5 data to analyze the relative error and bias of DGPI and examined how westerly wind biases in GloSea6 influenced wind shear and omega errors. In conclusion, one of the key reasons for the differences between the two methods was attributed to the wind shear error induced by the westerly wind bias.

How to cite: Kim, E., Kim, T., and Cha, D.-H.: Subseasonal activities of tropical cyclones over the western North Pacific in GloSea6, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7926, https://doi.org/10.5194/egusphere-egu25-7926, 2025.

EGU25-9206 | ECS | Posters on site | AS1.7

AI-based reconstruction of European temperature and precipitation anomalies from the Euro-Atlantic weather regimes 

Alessandro Camilletti, Elena Tomasi, Gabriele Franch, and Marco Cristoforetti

Despite recent advances, forecasting European weather on a seasonal timescale remains challenging for both numerical and statistical methods. Weather regimes (WRs), which represent recurrent, quasi-stationary, and persistent states of the atmospheric circulation, are well known to exert considerable influence over the European weather, offering a promising window of opportunity for sub-seasonal to seasonal forecasting. However, while much research has focused on the study of the correlation and the impacts of the WRs on the European weather, the estimation of ground-level climate variables, such as temperature and precipitation, from Euro-Atlantic WRs remains largely unexplored and limited to linear methods.

In this study, we present an AI model designed to reconstruct monthly mean anomalies of the European temperature and precipitation based on the dominant WRs. The model can capture and introduce complex non-linearities in the relation between multiple WRs, describing the state of the Euro-Atlantic atmospheric circulation, and the corresponding surface temperature and precipitation anomalies in Europe. The ability to reconstruct anomalies from WRs constitutes only a portion of the overall challenge. Predicting WRs on a monthly timescale is inherently difficult, and such forecasts are inevitably affected by errors, which can propagate and influence the quality of the reconstructed anomalies. In view of future developments, we examine the effect of inaccuracies in the WRs estimation on the anomalies reconstruction, establishing a lower bound on the WRs prediction accuracy required to outperform the ECMWF seasonal forecast system, SEAS5.

The model utilizes the monthly averages of weather regimes (WRs) to reconstruct the monthly averages of two-meter temperature and total precipitation anomalies during winter (DJF) and summer (JJA). ERA5 and NOAA-CIRES-DOE Twentieth Century Reanalysis datasets are used to compute the WRs and train the AI framework. Using ERA5 as the ground truth, the reconstruction performance is assessed through commonly used metrics, including mean squared error (MSE), anomaly correlation coefficient (ACC), and coefficient of efficiency (CE).

The results presented underline the importance of developing reliable WRs forecasting methods alongside reconstruction models to fully realize the potential of WRs-based forecasting systems. Our findings demonstrate that WRs-based anomaly reconstruction powered by AI-tools offers a viable pathway to better understand and predict seasonal variations.

How to cite: Camilletti, A., Tomasi, E., Franch, G., and Cristoforetti, M.: AI-based reconstruction of European temperature and precipitation anomalies from the Euro-Atlantic weather regimes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9206, https://doi.org/10.5194/egusphere-egu25-9206, 2025.

EGU25-9459 | ECS | Orals | AS1.7

Seamless Climate Information for climate extremes through merging of forecasts across seasonal to multi-annual timescales 

Muhammad Adnan Abid, Beena Balan Sarojini, and Antje Weisheimer

Predicting tailored climate extreme events seamlessly from seasons to multi-annual timescales is one of the challenges in the forecasting community. Novel post processing methodologies are required to address this issue, which is discussed in the present study. A new climate application is designed in co-production framework with the agriculture sector to develop the climate information for them on season to two-years timescale using seasonal to the extended seasonal forecast dataset available from the European Centre for Medium-Range Weather Forecasts (ECMWF) Seasonal Forecasting System (SEAS5) for the period 1981-2022. A temporal merging technique is developed to combine the forecasts on season to multi-annual timescale for the actionable climate information for the Frost risk, which affects the vineyard industry in southwestern Europe, in particular focus over Spain, during Spring (March-April) season. We noted a varying level of forecast skill for the Frequency of Frost Days (FFDs) during spring season (target season) in different start dates from lead month-0 (i.e., March start date) to lead month-23 (i.e., May start date). No Forecast Skill is noted for spring FFDs at lead month-2 (i.e., January start date), while a prominent skill is noted at lead month-11 (i.e., May start date). Temporally merging from lead month-23 to month-0 provide a large ensemble size, which have positive feedback onto the FFD’s forecast skill during the spring season. We also noted most of the forecast skill is mainly modulated by the long-term trends in most of the start dates, except for lead month-11 (May start date), while a combination of long-term trends as well as of internal variability (about 60%) is noted to the forecast skill for the FFDs in spring season. This post-processed seamless climate information will be useful for the local vineyard community to take some preventive measures well in advance from the frost risk, which may help to minimize the losses.

How to cite: Abid, M. A., Sarojini, B. B., and Weisheimer, A.: Seamless Climate Information for climate extremes through merging of forecasts across seasonal to multi-annual timescales, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9459, https://doi.org/10.5194/egusphere-egu25-9459, 2025.

EGU25-10659 | Posters on site | AS1.7

Probabilistic Load Forecasting for the City of Milan based on Subseasonal Predictions 

Riccardo Bonanno and Elena Collino

Summer heatwaves are a major concern for electricity distribution companies due to the high electrical loads they can place on urban distribution networks. These load peaks, driven by increased cooling demand, pose a serious threat to network infrastructure by accelerating the deterioration of underground components. During the summer, these components are prone to failure, resulting in cascading blackouts across multiple urban areas. In addition to meteorological forecasting of heat waves, it is therefore crucial to accurately estimate the probability that the electrical load in urban areas will exceed pre-defined thresholds.

In this study, temperature outputs from sub-seasonal forecasts are used to derive probabilistic forecasts of the expected electrical load. A machine learning approach is used, focusing on a single grid point representing the urban area of Milan. The chosen algorithm is Random Forest, where the target variable is the daily electrical load in Milan. The period used to train and validate the algorithm ranges from 2013 to 2023, and the predictors include the Degree Days (DD) and the "week of the year", since the electrical load shows strong seasonal variations.

The time series of the daily load in Milan, used to train the model, shows a significant shift from 2020 onwards due to the pandemic and the associated lockdowns, resulting in lower load values on average with respect to the 2013-2019 period. To ensure comparability between the pre-pandemic and the post-pandemic period (2021-2023), the historical series were detrended using a seasonal trend decomposition (STL) based on LOESS (Locally Estimated Scatterplot Smoothing), making the series almost stationary over the period analysed.

With the detrended electricity load time series, two forecasting models, both based on Random Forest, were implemented and tested. The first, called the Ensemble Model, trains the Random Forest with the Degree Days (DD) derived from ERA5 temperatures for 2013-2019 and applies the learned relationship to each of the bias-corrected seasonal S2S ensemble members for 2021-2023 to predict the electric load in the test period. The final load prediction in this case is the ensemble mean load.

The second approach, called the Quantile-Based model, uses the quantiles of the DD distribution derived from the bias-corrected S2S temperatures as predictors, providing greater flexibility for different ensemble configurations (e.g. 50 or 100 members). It is also tailored to specific forecast lead times and includes a simplified version based on the DD median.

The models have been evaluated using both deterministic and probabilistic metrics. The results indicate that while both models provide more reliable load forecasts than climatology, the Quantile-Based model outperforms the Ensemble Model beyond the third forecast week. It provides probability distributions that are more centred on the observed load, thereby improving forecast reliability.

These forecasting methods can help distribution system operators to address critical peak demand issues with preventive or more timely interventions.

How to cite: Bonanno, R. and Collino, E.: Probabilistic Load Forecasting for the City of Milan based on Subseasonal Predictions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10659, https://doi.org/10.5194/egusphere-egu25-10659, 2025.

EGU25-11278 | Posters on site | AS1.7

Distinct dynamic processes in 10–25-day and 25–70-day variability of the Siberian High 

Hongchang Ren and Fang Zhou

Focusing on the intraseasonal variability (ISV) of the Siberian high (SH), this study found that the SH presents two main periods of 10–25 and 25–70 days, which dominated the cold waves in the winter of 1995/96 and 2005/06 over eastern China (EC), respectively. The influence of these two ISV on East Asian climate is reflected in the evaluation of the East Asian winter monsoon and surface air temperature. The southeastward and downward Rossby wave activity indicates that the upper-level Ural anticyclone is the key to the SH ISV. By utilizing a transformed vorticity budget analysis, distinct dynamic processes in 10–25-day and 25–70-day variability of the SH were further revealed. Forcing from the mean flow acts as a guiding role in both 10–25-day and 25–70-day variability that induces the Ural anticyclone to propagate westward and eastward, respectively. Forcing from the ISV flow is similar to that from the mean flow with a smaller intensity. The dynamic synoptic eddy feedback positively contributes to both the 10–25-day and 25–70-day variability. It promotes (restrains) the westward (eastward) propagation of the Ural anticyclone in the 10–25-day (25–70-day) variability, which may be the main reason for these two distinct ISV of the SH.

How to cite: Ren, H. and Zhou, F.: Distinct dynamic processes in 10–25-day and 25–70-day variability of the Siberian High, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11278, https://doi.org/10.5194/egusphere-egu25-11278, 2025.

Outlooks of drier or wetter condition few weeks ahead has significant societal applications. Skillfully forecasting such conditions can enhance the climate prediction services for the agricultural sectors, provide drought outlooks and identify potential windows of wildfire risk. However, conventional numerical weather prediction (NWP) and emerging artificial intelligence (AI) methods have shown limited skill at this lead time, particularly for water-related variables. Hybrid methods, which blends observational data and numerical model using data-driven approach, have demonstrated potential to improve the skill of the forecast at these timescales. Additionally, identifying flow regime is also a widely used method to provide an outlook of temperature and precipitation in the extended range.

In this study, we combine both hybrid and flow regime approach to predict consecutive days without rain within a week. We first use machine learning to identify large-scale flow regimes that modulates weekly precipitation. Subsequently, a Bayesian Framework is employed to infer the posterior distribution of the predictand. This is done by updating the per-grid prior distribution of the predictand using two likelihood components: one derived from preceding large-scale regimes and another based on instantaneous flow regimes provided by extended-range forecasts from the Integrated Forecasting System (IFS).

 

How to cite: Chu, H. Y.: Subseasonal Prediction of Consecutive Dry Days in Southern Norway using Flow Regimes within a Bayesian Framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13640, https://doi.org/10.5194/egusphere-egu25-13640, 2025.

EGU25-14025 | Orals | AS1.7

Quantifying sources of subseasonal prediction skill in CESM2 in a perfect modeling framework 

Abigail Jaye, Judith Berner, Anne Sasha Glanville, and Jadwiga H. Richter

Recently, Richter at al. 2024 investigated the sources of predictability from initializing the ocean, atmosphere and land components and verifying S2S predictions against observations. They find that ocean initialization adds little skill in weeks 4-6 and land initializations deteriorate skill in week 1-2. These results point to possible problems with spin-up and coupled model drift. Here we will revisit these results, but in a perfect modeling framework which eliminates model error. For the perfect model, we find that land initializations do contribute to skill, especially in the summer hemisphere. By studying the evolution of the lead-time dependent bias in the actual and perfect predictions, we attempt to disentangle initialization error from coupled model drift.

 

Richter, J.H., Glanville, A.A., King, T. et al. Quantifying sources of subseasonal prediction skill in CESM2. npj Clim Atmos Sci 7, 59 (2024). https://doi.org/10.1038/s41612-024-00595-4

How to cite: Jaye, A., Berner, J., Glanville, A. S., and Richter, J. H.: Quantifying sources of subseasonal prediction skill in CESM2 in a perfect modeling framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14025, https://doi.org/10.5194/egusphere-egu25-14025, 2025.

EGU25-14345 | Orals | AS1.7

Benefits of online bias-correction versus postproessing methods 

Judith Berner, Abby Jaye, and William E. Chapman

Recently, there has been pronoued interest in predictability on the

subseasonal-to-seasonal (S2S) timescale. Skill at this forecast range is

only positive, if the lead-time dependent forecast bias is removed.

Recently, Chapman and Berner, 2024, developed an online bias-correction

from nudging tendencies and saw a bias reduction for surface and

free-atmosphere variables of up to 60% in climate simulations. Here, we

quantify the performance of this model-error scheme against

post-processing in S2S-forecasts. We find that the online bias-correction

reduces the bias, but less so than removing the lead-time dependent bias.

Together, they perform better than reducing the lead-time dependent bias

alone.

How to cite: Berner, J., Jaye, A., and Chapman, W. E.: Benefits of online bias-correction versus postproessing methods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14345, https://doi.org/10.5194/egusphere-egu25-14345, 2025.

A major sudden stratospheric warming (SSW) occurred in the Northern Hemisphere in early 2021, which caused extreme cold events across East Asia and North America, with record-breaking cold temperatures, notably 151 deaths in Texas. A better understanding of the SSW predictability for an improved surface seasonal to subseasonal (S2S) forecast is a pressing issue. Here we quantify the practical local predictability limit and find sensitive areas of forecast errors of 2021 SSW event within ERA5 reanalysis data and subseasonal to seasonal (S2S) reforecasts. A novel nonlinear method, Backward Searching for the Initial Condition (BaSIC), is used to estimate the local predictability of the SSW. This method is advanced because the nature of SSW is chaotic system with intrinsic properties, making it difficult to measure its predictability with traditional linear methods. The local predictability limit of this 2021 SSW event is estimated to be 17 days using BaSIC method.

We also trace the sensitive areas of forecast errors of this SSW. At the beginning, the overall forecast errors are relatively small, but with increase of time, errors increased more in the high altitude over central Eurasia (30°E-60°E). This indicates that this area is sensitive to forecast error growth, which limits the forecast skills of the 2021 SSW event. And it suggests that the central Eurasia is a key area for the improvements of the SSW forecast.

How to cite: Zhou, X., Zhang, G., Li, X., and Li, Y.: Quantifying the practical local predictability of the January 2021 sudden stratospheric warming using a novel nonlinear method, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14531, https://doi.org/10.5194/egusphere-egu25-14531, 2025.

EGU25-14935 | Orals | AS1.7

Skillful seasonal predictions of extended summer drought and fire risk from southern Europe to the Middle East 

Swen Brands, Óscar Mirones, Maialen Iturbide, José Manuel Gutiérrez, and Joaquín Bedia

The present study uncovers the capability of the ECMWF SEAS5 seasonal forecasting system to skillfully forecast the May-to-September Standardized Precipitation Evapotranspiration and Fire Weather indices (SPEI, FWI) in southern Europe and the Middle East, considering the unique verification period available for this system (1981-presence). This capability is visible in essentially all standard skill metrics (deterministic and probabilistic) up to a lead-time of six months and is particularly strong over the Iberian Peninsula, western France, northern Africa, the Near and Middle East, and in the regions surrounding the Black and Caspian Seas. Although the skill mainly resides on the correct reproduction of the long-term trend caused by anthropogenic warming, there is some skill for the detrended inter-annual time series pointing to the model’s capability to forecast internal climate variability. We also explore possible low-frequency skill modulations associated with distinct ENSO phases and model deficiencies diagnosed with the Ratio of Predictable Components, the latter measuring whether the ensemble’s spread and/or signal strength are realistic.

How to cite: Brands, S., Mirones, Ó., Iturbide, M., Gutiérrez, J. M., and Bedia, J.: Skillful seasonal predictions of extended summer drought and fire risk from southern Europe to the Middle East, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14935, https://doi.org/10.5194/egusphere-egu25-14935, 2025.

EGU25-15260 | Posters on site | AS1.7

Predicting the Power Load of a Market Area in Italy at the Seasonal Scale 

Simone Sperati and Stefano Alessandrini

Estimating power load, a crucial variable, is essential for optimizing power grid management, especially when forecasts are made months in advance. Weather conditions significantly influence power load; for example, high temperatures lead to increased energy demand for cooling during the summer. Utilizing seasonal weather forecasts to predict future power load represents a promising research direction in this field.

This study utilizes the European Centre for Medium-Range Weather Forecasts (ECMWF) SEAS5 model, which is currently one of the most advanced in seasonal forecasting, to predict power load in a large region of Italy. Given the coarse spatial resolution (~30 km) of SEAS5, developing an application that forecasts the monthly aggregated power load for a large region such as the North Italy market area was appropriate. The method involves calculating degree-days from the predicted temperature and other predictors and then employing a multiple linear regression model to estimate the power load.

The monthly aggregated power load for North Italy is estimated using seasonal forecast data from the ECMWF SEAS5 model at a 0.25° resolution, covering the period from July 2017 to June 2024. The ECMWF SEAS5 system has been providing operational forecasts since 2017, and forecasts are made for horizons ranging from 2 to 7 months ahead. The earlier period (1993-2016) is used for bias correction of the SEAS5 forecasts by comparing them with the ERA5 reanalysis dataset.

Measured load data are retrieved from the European Network of Transmission System Operators for Electricity (ENTSO-E) portal. The data from 2020 are excluded, as they are considered an anomaly, to avoid negatively impacting the training of the forecasting system.

Daily forecast data, predicted 2 to 7 months in advance, are used to calculate degree days and other predictors, which are then translated into predicted power load on a seasonal scale by the multi-linear regression. While daily forecasts at the seasonal scale typically exhibit very low or no skill, we managed to retain some skill by aggregating them over a one-month period. Specifically, this application used forecasts with daily time resolution to estimate monthly cumulative degree days derived from the SEAS5 model data.

The meteorological variables considered include daily maximum and minimum temperatures as well as daily cumulative solar irradiance, spatially aggregated for the area of interest (Northern Italy). To calculate Heating Degree Days (HDD) and Cooling Degree Days (CDD), thresholds of 18°C and 21°C, respectively, were used, reflecting the characteristics of the selected region.

The load forecasting system was evaluated using commonly used metrics, including the mean absolute percentage error (MAPE), mean error, and correlation. The system demonstrates highly promising results, proving to be more skillful up to 7 months ahead compared to climatology and persistency approaches. In these alternative methods, mean meteorological data are used as predictors instead of SEAS5 data (climatology), or the previous year's monthly load observations are directly used as load predictions (persistency).

How to cite: Sperati, S. and Alessandrini, S.: Predicting the Power Load of a Market Area in Italy at the Seasonal Scale, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15260, https://doi.org/10.5194/egusphere-egu25-15260, 2025.

EGU25-17591 | ECS | Orals | AS1.7

Enhancing Seasonal Predictions with Machine Learning: A Global Perspective on SST Influence in Early Winter 

Víctor Galván Fraile, Marta Martín-Rey, Irene Polo, Belén Rodríguez-Fonseca, Magdalena Alonso Balmaseda, Esteban Rodríguez-Guisado, and María N. Moreno-García

Seasonal predictability of early winter (November-December) atmospheric patterns is determined, to a large extent, by the anomalous ocean surface thermal conditions. Globally, sea surface temperatures (SSTs) serve as a key driver of wintertime atmospheric patterns, with their predictive importance varying across different regions and time lags. The extratropical regions  present greater challenges for seasonal predictability due to the complexity of their atmospheric processes and interaction of signals from different sources of predictability. Globally, sea surface temperatures (SSTs) serve as a key driver of wintertime atmospheric patterns, with their predictive importance varying across different regions and time lags. In the North Atlantic region,  seasonal predictability of early winter (November-December) atmospheric patterns can be determined, to a large extent, by the anomalous ocean surface thermal conditions.  Nevertheless, current seasonal prediction systems, which rely significantly on the well known interannual phenomenon known as the El Niño-Southern Oscillation (ENSO), develop large biases in the extratropical SSTs, leading to poor performances in other key variables in those regions, such as the Euro-Atlantic region (EAR). Thus, it is important to develop alternative statistical models to overcome these problems.

This study assesses the predictive capability of global SST anomalies with lead times ranging from 1 to 10 months to forecast November-December sea level pressure (SLP) anomalies. For such purpose, we use three different statistical approaches: a Maximum Covariance Analysis (MCA) to identify dominant patterns of co-variability between SSTs and atmospheric conditions; a neural network-based method (NN) designed to capture non-linear teleconnections; and a hybrid methodology that combines the strengths of the MCA and NN techniques.

Our results highlight regions of high predictive skill across the globe, with a focus on understanding how the different initializations impact the predictability. By comparing traditional statistical methods (MCA) with advanced non-linear approaches (NN and Hybrid), this study provides a comprehensive understanding of global atmospheric predictability during early winter. In particular, significant skill in terms of anomaly correlation coefficient is found for the neural network-based methods in the EAR from 7 to 10 months in advance. Additionally, analysis of the non-stationarity of these teleconnections is found and analyzed throughout the period ranging from 1940 to 2019. Furthermore, the non-stationarity of these teleconnections over the whole period is identified and analysed, detecting windows of opportunity for more accurate seasonal forecasts. The findings aim to improve our understanding of oceanic forced atmospheric teleconnections, not only by establishing windows of opportunity for seasonal forecasts, but also by means of analysing possible drivers of these teleconnections. All of these aid in the development of more accurate and robust prediction models for managing climate-related risks worldwide.

How to cite: Galván Fraile, V., Martín-Rey, M., Polo, I., Rodríguez-Fonseca, B., Alonso Balmaseda, M., Rodríguez-Guisado, E., and Moreno-García, M. N.: Enhancing Seasonal Predictions with Machine Learning: A Global Perspective on SST Influence in Early Winter, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17591, https://doi.org/10.5194/egusphere-egu25-17591, 2025.

EGU25-17667 | ECS | Orals | AS1.7

Subseasonal and seasonal windows of forecast opportunity of extreme European winter weather 

Marlene Kretschmer, Fiona Spuler, and Ted Shepherd

At subseasonal to seasonal lead times, the forecast skill of extreme events is known to be intermittent and dependent on specific phenomena or conditions, such as a strong El Niño event or sudden stratospheric warming. These states of enhanced predictability in the climate system are termed windows of forecast opportunity. Although this concept is widely recognised, diagnosing windows of opportunity remains an issue and often relies on evaluating conditional model skill, thereby conflating the window of opportunity with the ability of the model to represent it. Furthermore, identifying suitable representations of the dynamical drivers that provide enhanced predictability of a specific extreme event remains a challenge. Here, we propose an information-theoretic diagnostic of windows of forecast opportunity, which can be evaluated in a causal inference framework based on reanalysis data. We apply this diagnostic to characterise the seasonal modulation of subseasonal teleconnections relevant to weather extremes over Europe. Furthermore, we demonstrate the ability of a novel targeted clustering approach based on variational autoencoders to identify circulation regimes that disentangle the drivers of a specific extreme while maintaining their own predictability and physical teleconnections at S2S lead times. Combining the novel diagnostic with the improved representation of dynamical drivers provides a way forward to addressing the challenge of identifying windows of opportunity at subseasonal to seasonal lead times.

How to cite: Kretschmer, M., Spuler, F., and Shepherd, T.: Subseasonal and seasonal windows of forecast opportunity of extreme European winter weather, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17667, https://doi.org/10.5194/egusphere-egu25-17667, 2025.

EGU25-19590 | Posters on site | AS1.7

Subseasonal predictability of European winters using a weather regimes approach 

Ignazio Giuntoli and Daniele Mastrangelo

The ability of predicting winter anomalies of surface variables like surface temperature (t2m) is important for economic sectors like energy production and trade. Sub-seasonal predictions can provide a useful basis for the early detection of these anomalies. However, the skill varies considerably depending on the season and the location, and identifying periods of increased predictability is nontrivial. This study aims to work in this direction targeting atmospheric patterns leading to skillful winter predictions at S2S lead times using a weather regime (WR) approach with the overall goal to build confidence in the forecast. With a focus on Europe, we explore extended range t2m predictability (up to week 5) over 20 extended winters (1999-2018) in the ECMWF reforecasts with ERA5 reanalysis as the reference. Using the Euro Atlantic weather regimes, computed with 500 hPa geopotential height daily data, we identify the predominant WR weekly in both reanalysis and reforecast data. We propose a framework that allows for quantifying the degree of similarity between the reanalysis and the forecast WRs and assess whether higher similarity brings about improved skill. This is done by considering the difference in skill between all of the start dates with a predominant WR at week 1 and a subset made of occurrences with a degree of similarity that is higher than the climatology (i.e., the forecast system predicted the reanalysis WR better than the climatology did).  Results indicate that the framework proposed helps identifying more skillful forecasts making use of the WR similarity, particularly during NAO+ and NAO- conditions. This study constitutes an important step in the direction of exploiting flow dependent predictability to improve confidence in the forecast and can be considered as a preparatory step to the use of the more comprehensive real-time ensemble forecasts.

How to cite: Giuntoli, I. and Mastrangelo, D.: Subseasonal predictability of European winters using a weather regimes approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19590, https://doi.org/10.5194/egusphere-egu25-19590, 2025.

EGU25-21170 | Posters on site | AS1.7

Global Impacts of MJO Large-Scale Precipitation on Tropical Cyclones, Atmospheric Rivers, and Extreme Rainfall 

Shuyi Chen, Brandon Kerns, Edoardo Mazza, and Yakelyn Jauregui

The Madden-Julian Oscillation (MJO) is the most dominate mode of subseasonal-to-seasonal (S2S) variability, which bridges global weather and climate (Zhang, 2013). The MJO has been recognized as a source of predictability of the global weather on the S2S time scales and can influence onset of the El Nino (e.g., Kerns and Chen, 2021, Jauregui and Chen 2024a, 2024b). We developed a new capability by tracking the multiscale systems like the MJO, atmospheric rivers (ARs), jet stream, the ITCZ, easterly waves, tropical cyclones (TCs), and mesoscale convective systems (MCSs) using Multiscale Objects-Tracking and AI Climate Modeling for Extremes (Mosaic4E). One of the unique capabilities of Mosaic4E is the MJO Large-scale Precipitation Tracking (LPT, Kerns and Chen 2016, 2022) that can identify the MJO large-scale convective heating over the Northern Hemisphere (NH) and Southern Hemisphere (SH) can be used to study teleconnection patterns that are fundamental to extreme rainfall, heat waves and drought, which is not possible with the traditional MJO RMM index. When the MJO convection/precipitation is in the NH, it has a direct impact on the blocking patterns influencing the heatwaves and flooding and drought events. The MJO influence on the global high-impact weather involving heavy rainfall and flooding such as tropical cyclones (TCs) and the atmospheric rivers (ARs) are investigated using Mosaci4E. It is found that the number of TC activities increases 50-100% when MJO LPTs ended up over NH than when is in SH. Similar results are found for the MJO LPTs impacts on the ARs and extreme rainfall over the CONUS. The MJO-LPT represents the S2S time scale bridging the weather and climate and is a key for better understanding and predicting extreme events. The multiscale tracking capability will be enhanced by AI/ML tools in Mosaic4E for identifying, understanding, and predicting the extreme events. Mosaic4E is developed and tested using satellite and in situ observations as well as the ERA5 reanalysis data from 1979-2024. Mosaic4E has shown high skills in coastal flooding over the US and is currently tested globally. The satellite observation and reanalysis data are used to evaluate global weather and climate models.  Results show that most models overproduce precipitation over land in non-LPTs and underestimate large-scale precipitation over the oceans compared with the observations. For example, the MJO contributes up to 40-50% of the observed annual precipitation over the Indio-Pacific warm pool region, which are usually much less in the models because of models’ inability to represent the MJO dynamics. Furthermore, the spatial variability of precipitation ENSO is more pronounced in the observations than models.

How to cite: Chen, S., Kerns, B., Mazza, E., and Jauregui, Y.: Global Impacts of MJO Large-Scale Precipitation on Tropical Cyclones, Atmospheric Rivers, and Extreme Rainfall, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21170, https://doi.org/10.5194/egusphere-egu25-21170, 2025.

EGU25-21268 | Posters on site | AS1.7

Advancing March-May seasonal rainfall prediction for the East Africa region through Machine Learning to facilitate agriculture management 

Sinclair Chinyoka, Gert-Jan Steeneveld, Jordi Vila-Guerau de Arellano, Masilin Gudoshava, Hussen Seid Endris, and Zachary Atheru

Accurate weather and climate predictions are crucial for agriculture, water management, and disaster preparedness across Africa. However, several studies have highlighted the need to improve rainfall prediction at short-range, medium-range, sub-seasonal, and seasonal timescales. The inability of numerical weather prediction models to reliably capture probabilities of near-normal rainfall, coupled with their overconfidence, poses a significant challenge for many operational weather and climate prediction centers in Africa.

To address these challenges, we developed a machine learning (ML)-based framework for March–May (MAM) seasonal rainfall forecasting within East Africa Region, utilizing Random Forest (RF) and Extreme Gradient Boosting (XGB) models. These models leverage key climatic indicators, including the Indian Ocean Dipole (IOD), Mozambique Channel Trough (MOZ), and Oceanic Niño Index (ONI), computed as lagged indices (December–January) to capture antecedent conditions driving seasonal rainfall. About fifteen climate drivers computed from winds, soil moisture and sea surface temperatures were used as inputs for the machine learning models outputting MAM seasonal total rainfall.

Feature selection using mutual information scoring identified predictors with the strongest relationships to rainfall variability. Separate ML models were developed for each IGAD country to account for the spatial heterogeneity of climatic drivers, ensuring localized precision. A fair forecast performance of the RF and XGB models was achieved so far and also offering advantages in handling complex non-linear relationships.

This study demonstrates the potential of integrating ML with traditional forecasting methods to address the limitations of current model products, providing improved predictions to inform disaster risk reduction and climate adaptation strategies. By advancing the understanding of rainfall drivers, this work supports actionable decision-making for climate resilience within the East Africa region.

How to cite: Chinyoka, S., Steeneveld, G.-J., Vila-Guerau de Arellano, J., Gudoshava, M., Seid Endris, H., and Atheru, Z.: Advancing March-May seasonal rainfall prediction for the East Africa region through Machine Learning to facilitate agriculture management, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21268, https://doi.org/10.5194/egusphere-egu25-21268, 2025.

EGU25-1846 | Posters on site | AS1.8

A Robust Control Framework for Precipitation Regulation under NWP Model Uncertainty 

Yang Bai, Masaki Ogura, and Shunji Kotsuki

    Severe rainfall events can cause significant harm to individuals, damage infrastructure, and result in substantial economic losses. If precipitation regulation could be realized, it could help mitigate the risks of disasters. However, controlling precipitation remains a formidable challenge due to the highly complex and uncertain dynamics of weather systems. To address this, we propose a novel control framework for precipitation management based on a numerical weather prediction (NWP) model and applied the framework for a series of warm bubble experiments, where the direction and amplitude of regional wind serve as the input and precipitation as the output. This approach investigates the potential of modifying regional wind patterns to effectively influence and regulate precipitation intensity and distribution.

    The proposed framework integrates a Sampling-Based Model Predictive Control (SBMPC) module to generate ideal control inputs for precipitation reduction and a novel Control Barrier Function (CBF) module to refine these inputs when discrepancies between the model and real weather systems are detected. The SBMPC combines the strengths of model predictive control and random sampling techniques to efficiently solve high-dimensional and nonlinear optimization problems. Inspired by ensemble prediction methods in numerical weather forecasting, the developed SBMPC module uses sampled control inputs to simulate potential system responses with a numerical weather prediction model and selects the input, whose corresponding output most closely aligned with the desired one, as the nominal control input. However, the effectiveness of the SBMPC module depends heavily on the accuracy of the NWP model, making it vulnerable to discrepancies between the simulated and real weather systems.

    To mitigate this limitation, our control framework incorporates a CBF module to ensure safety by enforcing constraints, such as maintaining precipitation intensities within predefined boundaries to prevent extreme weather events. Unlike conventional CBF methods, which rely on precise system dynamics, the CBF controller developed in this work reduces dependency on detailed models, making it particularly effective for managing the complexity and uncertainty inherent in weather systems.    

    The feasibility of the proposed framework is validated through simulations using the SCALE Regional Model (SCALE-RM), which emulates real-world weather systems. Results demonstrate that the proposed control framework effectively regulates precipitation to a safe level and maintains computational efficiency, offering a robust and practical solution for managing precipitation.

How to cite: Bai, Y., Ogura, M., and Kotsuki, S.: A Robust Control Framework for Precipitation Regulation under NWP Model Uncertainty, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1846, https://doi.org/10.5194/egusphere-egu25-1846, 2025.

If the error growth of initial conditions in numerical weather systems is scale-dependent, then micro or mesoscale significantly affects the accuracy of a cyclonic weather system prediction. Thus, as the forecast skill improves (by including smaller-scale phenomena and reducing the error of the initial conditions), we would reach an intrinsic limit of predictability that we have set for the forecast of mid-latitude synoptic phenomena (geopotential height 500 hPa) at about three weeks. For scale-dependent initial error growth, it may turn out that small-scale phenomena that contribute little to the forecast product significantly affect the ability to predict that product. It is reasonable to study whether omitting these atmospheric phenomena will improve the predictability of the final value. The topic is studied in the extended system of Lorenz (2005). This system shows that omitting small spatiotemporal scales will reduce predictability more than modeling it. In other words, a system with model error (omitting phenomena) will not improve predictability. Orrell's hypothesis is extended to explain and describe this behavior, whereby the difference between systems (model error) produced at each time step is treated as an error in the initial conditions. The resulting model error is then defined as the sum of the time evolution increments of the initial conditions so defined. The theory is compared to the fit parameters that define the model error in certain approximations of the average forecast error growth. Parameters are interpreted in this context, and the hypotheses are used to estimate the errors described in the theory. The results of the annual averages of the prediction error growth (geopotential height 500 hPa) of the ECMWF system from 1987 to 2011 are discussed. 

How to cite: Bednar, H. and Kantz, H.: Analysis of initial and model error in forecast errors of extended atmospheric Lorenz' 05 systems and the ECMWF system, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2014, https://doi.org/10.5194/egusphere-egu25-2014, 2025.

EGU25-7791 | Posters on site | AS1.8

Detection of Separation Scenarios in Extreme Weather Events Using Regional Ensemble Prediction Data 

Pascal Oettli, Keita Tokuda, Yusuke Imoto, and Shunji Kotsuki

To support disaster prevention, it is essential to know in advance when scenarios start to distinguish one from the others, thus requiring the development of early detection methods of such separations. Ensemble prediction systems has been developed to provide scenarios of evolutions via their ensemble members, because the future state of the atmosphere predicted by a single ensemble member is less meaningful than the estimate of the future probability density from all the ensemble members. By construction, the primary function of an ensemble prediction system is to provide forecasters with a degree of uncertainty and level of confidence. For the last couple of years, we have developed different approaches which take advantage of the information provided by different ensemble prediction systems.

Tropical cyclone tracks forecasted by a prediction system sometimes group together into trajectories parting away from each other. An objective method, based on a robust clustering approach, has been created to detect such separation scenarios in the Mesoscale Ensemble Prediction System developed by the Japan Meteorological Agency. At each initialization time, when the number of clusters is greater than 1, local separation scenarios exist. Separations are related to different steering environments predicted by the different ensemble members.

On the same data used for the clustering, we also applied biological concepts such as the Waddington’s epigenetic landscape, and bioinformatics techniques like the graph-Hodge decomposition, to produce “MeteoScape”, an innovative way to characterize the evolution of a tropical cyclone. Particularly, “MeteoScape” can detect the possible paths and their associated probabilities of realization, as well as the regional separatrix, i.e., the spatial boundary between paths/scenarios, regardless of the initialization time (as in the clustering approach).

Using the cases of intense precipitations that occurred in western Japan in July 2018 and August 2021, we introduce a way to detect separation scenarios in a n-dimensional space. A dimensionality reduction technique is applied to the geopotential height at 500 hPa extracted from two different ensemble prediction systems (the Japanese Mesoscale Ensemble Prediction System and the North American National Centers for Environmental Prediction). In the resulting 3-dimensional latent space, trajectories of ensemble members at different initialization times can also part away. We show that these separations are linked to attracting atmospheric trajectories.

Further, the different techniques developed provide information on controllability, particularly where and when a manipulation could be performed.

How to cite: Oettli, P., Tokuda, K., Imoto, Y., and Kotsuki, S.: Detection of Separation Scenarios in Extreme Weather Events Using Regional Ensemble Prediction Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7791, https://doi.org/10.5194/egusphere-egu25-7791, 2025.

EGU25-8594 | Posters on site | AS1.8

Mitigating extreme events through multi-scenario ensemble forecasts and local interventions in the Lorenz 96 model 

Takahito Mitsui, Shunji Kotsuki, Naoya Fujiwara, Atsushi Okazaki, and Keita Tokuda

The prediction and mitigation of extreme weather events are important challenges in science and society. Recently, Miyoshi and colleagues introduced the control simulation experiment framework to examine the controllability of chaotic systems under observational uncertainty. Using this framework, they developed a method to reduce extreme events in the Lorenz 96 model by exploiting the system’s sensitivity to initial conditions, guiding trajectories toward desired outcomes with small control inputs (Sun et al., Nonlin. Processes Geophys., 30, 117-128, 2023). Their method is primarily designed to apply control inputs to all grid variables, reducing the success rate of extreme event mitigation to approximately 60% when the control input is applied to only one site. In this study, we propose a new approach to mitigate extreme events in the Lorenz 96 model through local interventions based on multi-scenario ensemble forecasts. Specifically, we explore effective intervention scenarios by computing the system’s responses to a limited number of feasible interventions. Our method achieves a success rate of 94%, even when interventions are applied to only one site per step. This represents a significant improvement over the ~60% success rate of the previous study, albeit at a moderately higher intervention cost. Furthermore, the success rate increases to 99.4% when interventions are applied to two sites.

How to cite: Mitsui, T., Kotsuki, S., Fujiwara, N., Okazaki, A., and Tokuda, K.: Mitigating extreme events through multi-scenario ensemble forecasts and local interventions in the Lorenz 96 model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8594, https://doi.org/10.5194/egusphere-egu25-8594, 2025.

Tropical cyclones are highly destructive natural disasters that pose a grave threat to society. As a result, the Moonshot Project of the Typhoon Control Research Aiming for a Safe and Prosperous Society is working towards finding artificial means to reduce an approaching typhoon. Therefore, making it less destructive. To achieve this less destructive storm, we initiate a cold pool, a natural feature of convective storms, to suppress convection by cooling the sub-cloud layer of an approaching typhoon thereby reducing the amount of heat energy being fed to the storm. To test if this approach is feasible, we conduct a series of experiments using the stretched version of the non-hydrostatic icosahedral atmospheric model (NICAM) with a minimum grid spacing of 1.4km. The artificial cold pool is generated by simulated rain which we produce by pumping seawater continuously through 1km high cylindrical stacks and then ejecting it at the top. The stacks have a radius of 5km and 50km and are on a moving platform that is positioned at the centre of the Typhoon. Typhoon Jebi we use as our test case. Our generated cold pool has an intensity that is a constant cooling source of 1K/hr and 10K/hr each for each radius making a total of 4 experiments. The experiments run for 48 hours prior to landfall in Japan. Overall, the tracks of the four experiments are not affected, only minor shifts in the location of the centre. The time evolution of the sea level pressure (slp) shows that the presence of the cold pool affects the slp for all experiments where the experiment with an intensity of 10K/hr at a 50 km radius experiences the greatest increase in minimum slp, signaling a weakening of the cyclone. Snapshots at 6, 12, 24 and 48hr time intervals of the slp, 10m-windspeed, the 2m-temperature, and the total precipitation reveal that the presence of the cold pool varies in the degree it affects these parameters for each experiment. A pattern where areas of weakening and areas of strengthening encircle the cooling source emerged in the differences in the 10m-windspeed and slp snapshots. The experiment 10K/hr at 50km radius tends to show the only discernible cold pool in the 2m-temperature difference snapshot. However, this experiment was proven to be difficult to reproduce in reality so our focus is on the 10K/hr at 5km radius experiment. After zooming in on the 2m-temperature difference between the experiment and the control, we notice that the drop in temperature (evidence of the cold pool) for the 10K/hr at 5km radius, is very small therefore indicating that the cold pool is very weak. This initiated a new group of experiments where we are testing different locations to find the most suitable area in a tropical cyclone to position our moving platform with the cooling source. The preliminary results suggest that the best location lies somewhere in the inner eyewall region where the winds are no more than 20m/s. Further testing is being conducted.

How to cite: Lee, M. and Satoh, M.: Understanding the Impact an Artificial Cold Pool has on an Approaching Typhoon using The Nonhydrostatic Icosahedral Atmospheric Model (NICAM), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14252, https://doi.org/10.5194/egusphere-egu25-14252, 2025.

EGU25-14879 | Posters on site | AS1.8

Transient low dimensional distribution of ensemble prediction in high dimensional chaos and control using the low dimensional latent representation 

Keita Tokuda, Takahito Mitsui, Shunji Kotsuki, and Naoya Fujiwara

We report that in several chaotic, high-dimensional nonlinear systems, the evolution of multiple ensembles starting from nearby initial conditions exhibits a transient low-dimensional distribution in phase space. This low-dimensional distribution of the ensembles is primarily achieved by stretching the ensemble distribution along the unstable directions of the system's trajectories. Furthermore, we discuss the potential of using this transient low-dimensional distribution to significantly reduce the search space when controlling the system's future states. As a concrete example of a high-dimensional nonlinear system, we use the Lorenz 96 model under a parameter setting that produces chaotic behaviors. We generate ensembles by adding small random perturbations to the initial conditions and compute the trajectories starting from each initial condition. By applying principal component analysis (PCA) to the ensemble distributions at each time step, we evaluate the dimension of the ensemble spread using a statistics that we call PCA dimension. Our results demonstrate that the PCA dimension initially decreases to values much smaller than the number of ensembles or the system's dimension, before increasing and converging to a value approximately equal to the Kaplan-Yorke dimension of the attractor. This phenomenon is considered to correspond to the asymmetry of the local Lyapunov exponents. Moreover, we show that at times when the PCA dimension of the ensemble distribution transiently decreases, it is possible to accurately regress the system's state at the time of a future extreme event using the scores of the first two principal components of the ensemble distribution. Additionally, using a regression model trained in this low-dimensional latent space, we succeed in identifying an optimal perturbation to the initial conditions to demonstrate the possibility of avoiding extreme events. Since meteorological phenomena are ultra-high-dimensional systems, attempts to reduce the dimensionality of the control search space may contribute to the feasibility of implementing such control measures. This presentation includes the most recent progress, such as using a weather prediction model, at the time of the conference.

How to cite: Tokuda, K., Mitsui, T., Kotsuki, S., and Fujiwara, N.: Transient low dimensional distribution of ensemble prediction in high dimensional chaos and control using the low dimensional latent representation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14879, https://doi.org/10.5194/egusphere-egu25-14879, 2025.

Sea surface temperature anomalies (SSTAs) over the North Atlantic (NA) have a significant impact on the weather and climate in both local and remote regions. This study first evaluated the seasonal prediction skill of NA SSTA using the North American multi-model ensemble and found that its performance is limited across various regions and seasons. Therefore, this study constructs models based on the long short-term memory (LSTM) network machine learning method to improve the seasonal prediction of NA SSTA. Results show that the seasonal prediction skill can be significantly improved by LSTM models since they show higher capability to capture nonlinear processes such as the impact of El Nin ̃o-Southern Oscillation on NA SSTA. This study shows the great potential of the LSTM model on the seasonal prediction of NA SSTA and provides new clues to improve the seasonal predictions of SSTA in other regions.

How to cite: Yan, X. and Tang, Y.: Seasonal prediction of North Atlantic sea surface temperature anomalies using the LSTM machine learning method , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-153, https://doi.org/10.5194/egusphere-egu25-153, 2025.

EGU25-3747 | Orals | CL4.6

Bridging paleoclimate and seasonal climate prediction: The case of European summer climate 

Martin Wegmann and Stefan Brönnimann

Understanding monthly-to-annual climate variability is essential for improving climate forecast products as well as adapting to future climate extremes. Previous studies show, that European summer climate, including temperature and precipitation extremes, is modulated by hemispheric large-scale circulation patterns, which themselves are connected to Earth system components such as sea surface temperature across temporal scales. Nevertheless, it remains unclear as to how stationary these teleconnections are and if their predictive power is potent across multiple centuries and background climates. By combining d18O isotopes from a European tree ring network with independent paleo-climate reanalyses, we highlight precursors and atmospheric dynamics behind European summer climate over the last 400 years.

We further present evidence that centennial ensemble seasonal climate forecasts capture the causality of the atmospheric
dynamics behind these teleconnections in the 20th century. Our results suggest that tropical sea surface temperature anomalies trigger specific precipitation and diabatic heating patterns which are dynamically connected to extratropical Rossby wave trains and the formation of a circumglobal teleconnection pattern weeks later.

How to cite: Wegmann, M. and Brönnimann, S.: Bridging paleoclimate and seasonal climate prediction: The case of European summer climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3747, https://doi.org/10.5194/egusphere-egu25-3747, 2025.

EGU25-3839 | ECS | Posters on site | CL4.6

Causal Links Between North Atlantic SSTs and Summer East Atlantic Pattern Predictability: Implications for Seasonal Forecasting 

Julianna Carvalho Oliveira, Giorgia Di Capua, Leonard F. Borchert, Reik V. Donner, and Johanna Baehr

We use causal effect networks to assess the influence of spring North Atlantic sea surface temperatures (NA-SSTs) on summer East Atlantic (EA) pattern predictability during 1908–2008. In the ERA-20C reanalysis, a robust causal link is identified for 1958–2008, where the spring meridional SST gradient causes a 0.2 standard deviation change in the summer EA. Additionally, the spring meridional SST index has an estimated negative causal effect (~−0.2) on summer 2m air temperatures over northwestern Europe. However, both links are absent when analysing the full period and are sensitive to interannual variability.

Analysis of the Max Planck Institute Earth System Model in mixed resolution (MPI-ESM-MR) shows that historical simulations fail to reproduce the observed causal links, while initialised ensembles occasionally capture them but underestimate their strength. Predictive skill assessments conditioned on these causal links indicate limited overall impact but suggest potential local improvements for European summer climate forecasts. These findings underscore the value of causal approaches for refining seasonal predictability.

How to cite: Carvalho Oliveira, J., Di Capua, G., Borchert, L. F., Donner, R. V., and Baehr, J.: Causal Links Between North Atlantic SSTs and Summer East Atlantic Pattern Predictability: Implications for Seasonal Forecasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3839, https://doi.org/10.5194/egusphere-egu25-3839, 2025.

EGU25-5880 | Orals | CL4.6

Intermittency of seasonal forecast skill for the wintertime North Atlantic Oscillation and East Atlantic Pattern  

Laura Baker, Len Shaffrey, Antje Weisheimer, and Stephanie Johnson

The wintertime North Atlantic Oscillation (NAO) and East Atlantic Pattern (EA) are the two leading modes of North Atlantic pressure variability and have a substantial impact on winter weather in Europe. The year-to-year contributions to multi-model seasonal forecast skill in the Copernicus C3S ensemble of seven prediction systems are assessed for the wintertime NAO and EA, and well-forecast and poorly-forecast years are identified. Years with high NAO predictability are associated with substantial tropical forcing, generally from the El Niño Southern Oscillation (ENSO), while poor forecasts of the NAO occur when ENSO forcing is weak. Well-forecast EA winters also generally occurred when there was substantial tropical forcing, although the relationship was less robust than for the NAO. These results support previous findings of the impacts of tropical forcing on the North Atlantic and show this is important from a multi-model seasonal forecasting perspective.

How to cite: Baker, L., Shaffrey, L., Weisheimer, A., and Johnson, S.: Intermittency of seasonal forecast skill for the wintertime North Atlantic Oscillation and East Atlantic Pattern , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5880, https://doi.org/10.5194/egusphere-egu25-5880, 2025.

EGU25-6006 | ECS | Orals | CL4.6

 Investigating the sensitivity of 20th century seasonal hindcasts to tropospheric aerosol forcing 

Matthew Wright, Antje Weisheimer, Tim Woollings, Retish Senan, and Timothy Stockdale

Previous studies have identified multi-decadal variations in the skill of winter seasonal forecasts of large-scale climate indices, including ENSO, the PNA, and NAO. Forecast skill is significantly lower in the middle of the 20th century (1940—1960) than at the start or end of the century. We hypothesise that tropospheric aerosol forcing, which is spatially and temporally heterogeneous and poorly constrained in the hindcasts used in previous studies, contributes to this low skill mid-century period.

This study assesses the sensitivity of ECMWF’s state-of-the-art seasonal forecasting model to tropospheric aerosol forcing, using a newly developed aerosol forcing dataset based on CEDS emissions data. We analyse DJF hindcasts initialised every November from 1925—2010, each with 21 ensemble members. For each year, we run hindcasts with ‘best guess’, doubled, and halved aerosol forcing (perturbing both anthropogenic and natural aerosols). All experiments exhibit similar multi-decadal variability in skill for large-scale climate indices. Aerosol forcing has no significant impact on forecast skill but some impacts on mean biases, suggesting other factors drive the mid-century skill minimum.

Aerosol forcing has large regional impacts. Increasing aerosol forcing leads to cooler 2m temperature and SSTs globally, with amplified cooling in regions with large aerosol forcings, such as northern India and North Africa. Dynamical responses include an ‘anti-monsoon’ circulation over Africa, with a weakening of the trade winds and Atlantic Walker circulation, and local southwards shift of the ITCZ. The magnitude of the response increases when ocean initial conditions are perturbed to represent the cumulative impact of aerosol forcing, suggesting that coupling enhances the atmospheric response.

These results highlight the model’s sensitivity to tropospheric aerosols, with large differences in bias and mean state after four months, despite limited impact on skill. The circulation changes over Africa warrant further investigation, with implications for future aerosol scenarios. Planned experiments will explore the impact in summer and quantify the timescale of the response to aerosols.

How to cite: Wright, M., Weisheimer, A., Woollings, T., Senan, R., and Stockdale, T.:  Investigating the sensitivity of 20th century seasonal hindcasts to tropospheric aerosol forcing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6006, https://doi.org/10.5194/egusphere-egu25-6006, 2025.

This study shows a close relationship between winter Arctic sea ice concentration (WASIC) anomalies in the Barents-Greenland Seas and the subsequent autumn Indian Ocean Dipole (IOD) based on the observational analysis and numerical simulations. Particularly, more (less) WASIC in the Barents-Greenland Seas tends to lead to a positive (negative) IOD in the following autumn. Above-normal WASIC in the Barents-Greenland Seas results in reduction of the upward turbulent heat flux and induces tropospheric cooling over the Arctic. This tropospheric cooling triggers an atmospheric teleconnection extending from the Eurasian Arctic to the subtropical North Pacific. Numerical experiments with both the linear barotropic model and atmospheric general circulation model can well capture the atmospheric teleconnection associated with the WASIC anomalies. The subtropical atmospheric anomalies generated by the WASIC anomalies then result in subtropical sea surface temperature (SST) warming, which sustains and expands southward to the equatorial central Pacific during the following summer via a wind-evaporation-SST feedback. The resulting equatorial central Pacific SST warming anomalies induce local atmospheric heating and trigger an anomalous Walker circulation with descending motion and low-level anomalous southeasterly winds over the southeastern tropical Indian Ocean. These anomalous southeasterly winds trigger positive air-sea interaction in the tropical Indian Ocean and contribute to the development of the IOD. The close connection of the WASIC anomalies with the subsequent IOD and the underlying physical processes can be reproduced by the coupled climate models participated in the CMIP6. These results indicate that the condition of WASIC is a potential effective precursor of IOD events.

How to cite: Xin, C.: Influence of winter Arctic sea ice anomalies on the following autumn Indian Ocean Dipole development, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6176, https://doi.org/10.5194/egusphere-egu25-6176, 2025.

EGU25-7163 | Orals | CL4.6

Robust decadal predictability of cold surge frequency in Taiwan and East Asia through teleconnection of North Atlantic Oscillation 

Wan-Ling Tseng, Yi-Chi Wang, Ying-Ting Chen, Yi-Hui Wang, Huang-Hsiung Hsu, and Chi-Cherng Hong

This study investigates the decadal predictability of cold surge frequency (CSF) in East Asia, including Korea, Japan, and Taiwan, through the lens of the North Atlantic Oscillation (NAO) index. The findings suggest that extreme events such as cold surges can be predicted on decadal timescales when the teleconnection mechanism is robustly established. The study revisits and consolidates the dynamical mechanisms underlying wave propagation and the teleconnection between the NAO and the East Asian trough, highlighting their role in creating a winter environment conducive to cold surges in Taiwan and East Asia. The study demonstrates the skill of climate models in capturing the NAO's decadal variability, and develops a statistical-dynamical hybrid approach. This method integrates decadal prediction datasets with a statistical model to enhance the prediction of extreme cold surge occurrences on a multi-annual timescale. The results of the study underscore the scientific significance of merging climate dynamical mechanisms with decadal prediction systems for extreme events, and introduce a hybrid framework that combines numerical decadal climate predictions with statistical regression models. This addresses the challenges posed by biases in climate prediction models and advances the capability to predict regional extreme events such as cold surges.

How to cite: Tseng, W.-L., Wang, Y.-C., Chen, Y.-T., Wang, Y.-H., Hsu, H.-H., and Hong, C.-C.: Robust decadal predictability of cold surge frequency in Taiwan and East Asia through teleconnection of North Atlantic Oscillation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7163, https://doi.org/10.5194/egusphere-egu25-7163, 2025.

EGU25-8693 | ECS | Orals | CL4.6

Decadal prediction for the European Energy Sector 

Benjamin Hutchins, David Brayshaw, Len Shaffrey, Hazel Thornton, and Doug Smith

The timescale of decadal climate predictions, from a year-ahead up to a decade, is an important planning horizon for stakeholders in the energy sector. With power systems transitioning towards a greater share of renewables, these systems become more vulnerable to the impacts of both climate variability and climate change. As decadal predictions sample both the internal variability of the climate and the externally forced response, these forecasts can provide useful information for the upcoming decade. 

There are two main ways in which decadal predictions can benefit the energy sector. Firstly, they can be used to try to predict how a variable of interest, such as average temperature, may evolve over the coming year or decade. Secondly, a large ensemble of decadal predictions can be aggregated into a large synthetic event set to explore physically plausible extremes, such as winter wind droughts. 

We find predictive skill at decadal timescales for surface variables over Europe during both winter (ONDJFM) and summer (AMJJAS). Although this skill is patchy, there are regions of relevance to the energy sector, such as over the UK for temperature, where this skill emerges. We find significant skill when using pattern-based (e.g., NAO) approaches to make predictions of European energy indicators during the extended winter, including Northern Europe offshore wind generation, Spanish solar generation, and Scandinavian precipitation. For predicting UK electricity demand, we find significant skill when directly using the model predictions of surface temperature. Our results highlight the potential for operational decadal predictions for the energy system, with potential benefits for both the planning and operation of the future power system. 

How to cite: Hutchins, B., Brayshaw, D., Shaffrey, L., Thornton, H., and Smith, D.: Decadal prediction for the European Energy Sector, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8693, https://doi.org/10.5194/egusphere-egu25-8693, 2025.

EGU25-8904 | Orals | CL4.6

On the predictive skill for warm spells in Germany across seasons  

Fabiana Castino, Tobias Geiger, Alexander Pasternack, Andreas Paxian, Clementine Dalelane, and Frank Kreienkamp

Intense warm spells, such as heatwaves, can significantly impact human health, the environment, and socio-economic systems. Although heatwaves are typically associated with summer, the occurrence of warm spells during cold seasons can also have profound effects on various sectors. While some effects, such as reduced cold-related mortality, can be considered beneficial, the long-term consequences, e.g. on ecosystems, forests, and agriculture, are concerning. Warm spells during the cold seasons can alter the natural dormancy cycles of plants, causing premature sprouting, flowering, or growth and negatively affecting crop yield and quality. In addition, cold season warm spells can reduce snow accumulation in mountainous regions, potentially affecting downstream water availability. As climate change drives increases in the frequency, intensity, and duration of warm spells, their impacts are becoming more severe and far-reaching. This makes predicting such events a key priority for climate science and risk management.

Climate forecast models offer the potential to predict extreme events like warm spells weeks to months in advance, becoming increasingly relevant for decision-making across various socio-economic sectors. This study examines the predictive skill of the downscaled German Climate Forecast System Version 2.1 (GCFS2.1) for warm spells in Germany on a seasonal scale, encompassing both warm seasons (spring and summer) and cold seasons (autumn and winter).  The analysis relies on hindcast data from the 1991-2020 base period, statistically downscaled to 5 km resolution. It evaluates multiple extreme temperature climate indices, as for example the Warm Spells Duration index, and applies various statistical metrics to assess the predictive skill. The findings reveal high heterogeneity in the ability of the (downscaled) GCFS2.1 to forecast warm spells across seasons, with higher predictive skill during the cold seasons but more limited for the warm seasons.

How to cite: Castino, F., Geiger, T., Pasternack, A., Paxian, A., Dalelane, C., and Kreienkamp, F.: On the predictive skill for warm spells in Germany across seasons , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8904, https://doi.org/10.5194/egusphere-egu25-8904, 2025.

EGU25-8980 | ECS | Orals | CL4.6

Predicting North Atlantic Temperature Trends with the Analogue Method using the MPI CMIP6 Grand Ensemble 

Lara Heyl, Sebastian Brune, and Johanna Baehr

The analogue method is a powerful and efficient tool for climate predictions, particularly in regions like the North Atlantic, where impacts of climate change have been relatively modest. While climate projections effectively estimate global mean surface temperature trends over a century, decadal trends in the North Atlantic diverge from the global trend. Here, we leverage on the similar evolution of analogous patterns on a decadal time scale by comparing SST patterns in observed data with patterns from an existing simulation ensemble. We apply this method to ten-year SST trend reconstructions in the North Atlantic using the MPI CMIP6 grand ensemble. In addition, we assess the impact of volcanic eruptions on the quality of the SST trend reconstruction for the time period 1960-2019. We also provide a prediction for 2020–2029. We find that the analogue method delivers high correlation of SST trend reconstructions with observed trends for the MPI CMIP6 grand ensemble. Volcanic influence can be accounted for by trimming the time series to those times unaffected by volcanic eruptions, which results in a higher correlation. Our results suggest that the decadal predictions of SST trends might also be achieved without the need for new, computationally expensive simulations.

How to cite: Heyl, L., Brune, S., and Baehr, J.: Predicting North Atlantic Temperature Trends with the Analogue Method using the MPI CMIP6 Grand Ensemble, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8980, https://doi.org/10.5194/egusphere-egu25-8980, 2025.

EGU25-9006 | Posters on site | CL4.6

Is the winter mean NAO white noise? Models and observations. 

Bo Christiansen and Shuting Yang

The NAO is a dominant mode of variability in the Northern Hemisphere with strong impacts on temperature, precipitation, and storminess. The predictive skill of the NAO on annual to decadal scales is therefore an important topic, which is often studied using, e.g., (initialized) climate models. The temporal structure is closely related to the predictability, and on inter-annual time scales the observed NAO is frequently described to have power at 2-7 years and sometimes with a distinct peak around 7 or 8 years.  However, the observational record is brief, and such estimations have high uncertainty.

Here, we present a thorough study to answer the questions: is the winter mean NAO different from white noise and is the observed NAO different from the NAO in historical experiments with contemporary climate models (CMIP6)? To this end we use a range of statistical tools in both the temporal and spectral domain: Power-spectra, wavelet-spectra, autoregressive models, and various well-known time-series statistics.

Overall, we find little evidence to reject that the NAO is white noise. For observations, the peak in the power-spectrum at 8 years is, taken individually, significant in the period after 1950 but not before. However, considering the complete spectrum, significant peaks will often occur at some frequency, even for white noise.  The large CMIP6 multi-model ensemble is statistically very similar to an ensemble of similar size of white noise, e.g., the ensemble averages of the power spectrum and the wavelet spectra are completely flat.  Furthermore, for both observations and the model ensemble the tests based on autoregressive modelling and time-series statistics do not reject the null-hypothesis of white noise.

How to cite: Christiansen, B. and Yang, S.: Is the winter mean NAO white noise? Models and observations., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9006, https://doi.org/10.5194/egusphere-egu25-9006, 2025.

EGU25-10305 | ECS | Posters on site | CL4.6

Towards improved forecast initialisations with an observation-informed ocean grid 

Marlene Klockmann, Kai Logemann, Sebastian Brune, and Johanna Baehr

For climate forecasts it is crucial to initialise the ocean state from observations because they rely on the memory of the ocean. If, however, the initialised ocean state is far away from the model’s own preferred mean state, predictive skill will suffer due to model drift. We are testing whether an ocean grid with variable resolution - designed to represent sparse and well-observed regions with appropriate resolution - has advantages over an ordinary grid with uniform resolution. The locally high resolution could lead to an improved mean ocean state through a better representation of mesoscale processes. The observation-informed grid will allow for high-resolution data assimilation in well-observed areas, which will potentially lead to improved initial conditions and predictive skill.  

We developed such a grid for the ocean component of the coupled ICON model designed for seamless predictions (ICON-XPP). The grid resolution varies from 40 to 10km, depending on the observation density in the EN4 database from 1960 to 2023. The local refinement in well-observed areas leads to a better representation of ocean features such as fronts and western boundary currents. We assess the effect of these improvements on the mean climate state by comparing to a reference simulation with a uniform 20km ocean resolution. 

 

How to cite: Klockmann, M., Logemann, K., Brune, S., and Baehr, J.: Towards improved forecast initialisations with an observation-informed ocean grid, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10305, https://doi.org/10.5194/egusphere-egu25-10305, 2025.

EGU25-10747 | Posters on site | CL4.6

Ocean–atmosphere feedbacks key to NAO decadal predictability 

Panos J. Athanasiadis, Casey Patrizio, Doug M. Smith, and Dario Nicolì

Recent studies using initialised large-ensemble re-forecasts have shown that the North Atlantic Oscillation (NAO) exhibits significant decadal predictability, which is of great importance to society given the significant climate anomalies that accompany the NAO. However, the key physical processes underlying this predictability, including the role of ocean–atmosphere interactions, have not yet been pinned down. Also, a critical deficiency in the representation of the associated predictable signal by climate models has been identified in recent studies (the signal-to-noise problem), still lacking an explanation.

In this study, the decadal prediction skill for the NAO and the interactions of the associated atmospheric circulation anomalies with the underlying ocean are assessed using retrospective forecasts from eight decadal prediction systems and observation-based data. We find considerable spread in the NAO skill across these systems and critically, that this is linked to differences in the representation of ocean–NAO interactions across the systems. Evidence is presented that the NAO skill depends on a direct positive feedback between subpolar sea surface temperature anomalies and the NAO, which varies in strength across the prediction systems, yet may still be too weak even in the most skillful systems compared to the observational estimate. This positive feedback is opposed by a delayed negative feedback between the NAO and the ocean circulation that also contributes to disparities in the NAO skill across systems. Our findings therefore suggest that North Atlantic ocean–atmosphere interactions are central to NAO decadal predictability. Finally, it is suggested that errors in the representation of these interactions may be contributing significantly to the signal-to-noise problem.

How to cite: Athanasiadis, P. J., Patrizio, C., Smith, D. M., and Nicolì, D.: Ocean–atmosphere feedbacks key to NAO decadal predictability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10747, https://doi.org/10.5194/egusphere-egu25-10747, 2025.

EGU25-10815 | Posters on site | CL4.6

Planktonic foraminifera as a tool of past seasonality reconstruction 

Zhoufei Yu, Baohua Li, and Shuai Zhang

Seasonal changes in seawater temperature leave large imprints on the stable oxygen isotope composition (δ18O) of planktonic foraminiferal tests, based on which the past seasonal changes can be reconstructed. However, there are still problems needed to be figured out in regard to this new method, to improve the reliability of seasonality reconstruction. For example, the selected foraminiferal species, the used size fraction, and the sample area. As a result, by analyzing planktonic foraminiferal test δ18O from the sediment trap samples deployed in the South China Sea, we found that foraminiferal seasonal δ18O signal is strongly distorted (amplified or damped) by seasonal variations in their habitat depth, particularly for the species living in low latitude. Furthermore, Globigerinoides ruber of 300-355 um can record the most comprehensive seawater seasonality information. This study provides strong support to the reconstruction of past seawater seasonal temperature by using individual planktonic foraminifera.

How to cite: Yu, Z., Li, B., and Zhang, S.: Planktonic foraminifera as a tool of past seasonality reconstruction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10815, https://doi.org/10.5194/egusphere-egu25-10815, 2025.

EGU25-11024 | ECS | Orals | CL4.6

Skill assessment of a multi-system ensemble of initialized 20-year predictions 

Dario Nicolì, Sebastiano Roncoroni, Wolfgang A. Mueller, Holger Pohlmann, Sebastian Brune, Markus Donat, Rashed Mahmood, Steve Yeager, William J. Merryfield, Reinel Sospedra-Alfonso, and Panos J. Athanasiadis

Decadal predictions have advanced greatly in recent years: not only have they become operational worldwide and have been demonstrated to be skillful in various aspects of climate variability, including predicting changes in the atmospheric circulation and in the occurrence of extremes several years ahead, but —as such— they are also being used increasingly in climate services. Climate adaptation and policy making, however, also require climate predictions that go beyond the 10-year horizon. For climate information beyond 10 years into the future, uninitialized climate projections, which completely miss any predictability stemming from internal variability, have been the only available product. Trying to account for this lack of information in climate projections regarding any predictable components of internal variability, methods to constrain climate projections using information from large ensembles of initialized decadal predictions have been developed and have been shown to reduce the uncertainty and increase the skill of climate projections, even beyond the 10-year horizon. The demonstrated benefits of such indirect methods to account for predictable internal variability indicate that the latter remains significant beyond the 10-year limit of decadal predictions. Hence, directly harnessing this predictability through running initialized 20-year predictions emerges as a strategic endeavour.
In this study a novel, multi-system ensemble of initialized extended-decadal predictions is assessed. These predictions consist of a grand ensemble of 71 members derived from 6 forecast systems. They are initialized every 5 years from 1960 onward and run ahead for 20 years. Our analysis uses an elaborate drift- and bias-correction method that accounts for the correct representation of trends. Importantly, we show significant skill against observations for a number of variables (fields and indices), even in the second decade of the forecasts. The origin of such predictability is discussed together with the limitations of these 20-year predictions. The respective experimental protocol was defined in the framework of the ASPECT EU project and has been proposed as a tier-2 Decadal Climate Prediction Project (DCPP) protocol for the Coupled Model Intercomparison Project phase 7 (CMIP7).

How to cite: Nicolì, D., Roncoroni, S., Mueller, W. A., Pohlmann, H., Brune, S., Donat, M., Mahmood, R., Yeager, S., Merryfield, W. J., Sospedra-Alfonso, R., and Athanasiadis, P. J.: Skill assessment of a multi-system ensemble of initialized 20-year predictions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11024, https://doi.org/10.5194/egusphere-egu25-11024, 2025.

EGU25-11166 | ECS | Orals | CL4.6

Multidecadal variability of the ENSO teleconnection to Europe in early-winter and implications for seasonal forecasting 

Pablo Fernández-Castillo, Teresa Losada, Belén Rodríguez-Fonseca, Diego García-Maroto, Elsa Mohino, and Luis Durán

El Niño-Southern Oscillation (ENSO) is the leading mode of global climate variability. Through its associated teleconnections, ENSO can impact the climate of numerous regions worldwide at seasonal timescales, highlighting its role as the main source of seasonal predictability. Numerous studies have demonstrated a significant influence of ENSO on the climate of the Euro-Atlantic sector, but the impacts and mechanisms of the teleconnection in early-winter (November-December) remain unclear. Besides, in early-winter, ENSO teleconnections involve tropospheric pathways, which may change in response to different background states of the ocean. Thus, a crucial research question to address is whether the early-winter teleconnection to the Euro-Atlantic sector has changed under the different background states of sea surface temperature (SST) over the Pacific Ocean. 

 

This work aims to analyse the ENSO early-winter teleconnection to the Euro-Atlantic sector from a nonstationary perspective. Specifically, the teleconnection is analysed under different background states of SST over the Pacific Ocean, related to changes in the phase of the Pacific Decadal Oscillation (PDO). Using observational and reanalysis datasets for the period 1950-2022, results reveal that the tropospheric pathways of the teleconnection change under the different Pacific SST background states, leading to distinct responses of the North Atlantic atmospheric circulation to ENSO. We also confirm that these distinct responses in the North Atlantic entail significantly different impacts of ENSO on the surface climate across Europe, particularly on surface air temperature. Furthermore, the teleconnection is analysed in the SEAS5 state-of-the-art dynamical seasonal prediction model. The analysis within the model is also conducted from a nonstationary perspective, and aims to determine whether the model successfully reproduces a shift in the teleconnection in the late 1990s identified in reanalysis and observations. Results show that the model accurately captures the spatial pattern of the teleconnection impacts across Europe after the late 1990s, but not before. In turn, significant changes in the skill of seasonal forecasts are observed between before and after the late 1990s. However, skill after the late 1990s is just moderate due to a significant underestimation of the teleconnection impacts. 

 

The results of this study shed light on the nonstationary behaviour of the early-winter teleconnection to the Euro-Atlantic sector and have important implications on seasonal predictability in Europe. Particularly, the nonstationarity of the teleconnection gives rise to the emergence of windows of opportunity for seasonal forecasting, in which forecast skill may be greater than initially expected from a stationary analysis.

How to cite: Fernández-Castillo, P., Losada, T., Rodríguez-Fonseca, B., García-Maroto, D., Mohino, E., and Durán, L.: Multidecadal variability of the ENSO teleconnection to Europe in early-winter and implications for seasonal forecasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11166, https://doi.org/10.5194/egusphere-egu25-11166, 2025.

EGU25-11511 | Orals | CL4.6

Constraining near-term climate projections by combining observations with decadal predictions 

Rémy Bonnet, Julien Boé, and Emilia Sanchez

Reducing the uncertainty associated with internal climate variability over the coming decades is crucial, as this time frame aligns with the strategic planning needs of stakeholders in climate-vulnerable sectors. Three sources of information are available: non-initialized ensembles of climate projections, initialized decadal predictions, and observations. Non-initialized ensembles of climate projections span seamlessly from the historical period to the end of the 21st century, encompassing the full range of uncertainty linked to internal climate variability. Initialized decadal predictions aim to reduce uncertainty from internal climate variability by initializing model simulations with observed oceanic states, phasing the simulated and observed climate variability modes. However, they are usually limited to 5 to 10 years, with small added value after a few years, and they are also subject to drift due to the shock from the initialization. Finally, we can also use observations that can provide information to constrain the climate evolution over the next decades. Providing the best climate information at regional scale over the next decades is therefore challenging. Previous methods addressed this challenge by using information from either the observations or the decadal predictions to constrain uninitialized projections. In this study, we propose a new method to make use of the different sources of information available to provide relevant information about near-term climate change with reduced uncertainty related to internal climate variability. First, we select a sub-ensemble of non-initialized climate simulations based on their similarity to observed predictors with multi-decadal signal potential over Europe, such as Atlantic multi-decadal variability (AMV). Then, we further refine this sub-ensemble of trajectories by selecting a subset based on its consistency with decadal predictions. We present a case study focused on predicting near-term future surface temperatures over Europe. To evaluate the effectiveness of this method in providing reliable climate information, we conduct a retrospective analysis over the historical period.

How to cite: Bonnet, R., Boé, J., and Sanchez, E.: Constraining near-term climate projections by combining observations with decadal predictions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11511, https://doi.org/10.5194/egusphere-egu25-11511, 2025.

EGU25-12107 | Orals | CL4.6

Overcoming the spring predictability barrier with a supermodel 

Noel Keenlyside, Tarkeshwar Singh, Ping-Gin Chiu, Francois Counillon, and Francine Schevenhoven

Climate models suffer from long-standing biases that degrade climate prediction skills. While radically increasing resolution offers promise, we are still many years away from being able to perform operational climate predictions with models that can explicitly resolve the most important physical processes. Here we demonstrate that supermodelling can enhance climate predictions through better using the current generation of models. A supermodel connects different models interactively so that their systematic errors compensate. It differs from the standard non-interactive multi-model ensembles, which combines model outputs a-posteriori. We have developed an ocean-connected Earth System model using NorESM, CESM, and MPIESM in their CMIP5 versions. The model radically improves the simulation of tropical climate, strongly reducing SST and double ITCZ biases. We perform seasonal predictions for the period 1990-2020, initialized through (EnOI) data assimilation of SST. We have performed one forecast per season but are currently extending the ensemble size to ten members. The supermodel shows marked improvement in prediction skill for forecasts started before boreal spring, significantly overcoming the spring predictability barrier. Initial investigation indicates the skill enhancement is connected to better simulation of ocean-atmosphere interaction during the first part of the year, which also leads to improved initial conditions. Our results indicate the importance of better representing the signal-to-noise in the western and central Pacific during boreal spring.

How to cite: Keenlyside, N., Singh, T., Chiu, P.-G., Counillon, F., and Schevenhoven, F.: Overcoming the spring predictability barrier with a supermodel, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12107, https://doi.org/10.5194/egusphere-egu25-12107, 2025.

EGU25-12143 | Posters on site | CL4.6

Probabilistic climate outcomes from prediction aggregation 

Robin Lamboll, Sofia Palazzo Corner, and Moritz Schwarz

Currently, much of the literature around the Paris Agreement, Paris Compliance and manging the transition to net zero requires heavy use of integrated assessment models (IAMs). IAMs provide economic projections of future emissions, conditional on idealised scenarios. However, for most adaptation and cost-benefit analysis, policymakers require predictions, which IAMs do not even attempt to provide. How can we use aggregated estimates of emissions and resulting climate change to give probability distributions of climate impacts? We outline why human computation likely out-performs other prediction methods and present a flexible method to collect intended predictions from a variety of people to effectively estimate future emissions, temperatures and climate impacts via prediction aggregation platforms. These can subsequently be used to inform estimates of climate impacts. It can also highlight deficiencies in the IAM scenarios literature and indicate relative probabilities of scenarios. We estimate all-uncertainty temperatures in 2050 and outline extensions of the work.

How to cite: Lamboll, R., Palazzo Corner, S., and Schwarz, M.: Probabilistic climate outcomes from prediction aggregation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12143, https://doi.org/10.5194/egusphere-egu25-12143, 2025.

EGU25-12247 | ECS | Orals | CL4.6

Forecasting monthly-to-seasonal sea surface temperatures and marine heatwaves with graph neural networks and diffusion methods 

Varvara Vetrova, Ding Ning, Karin Bryan, and Yun Sing Koh

Knowing future sea surface temperature (SST) patterns play a crucial role not only in industries such as fisheries, shipping and tourism but also in conservation of marine species . For example, DNA of endangered species can be sampled prior to anticipated marine heatwaves to preserve marine biodiversity. Overall, availability of SST forecasts allows to mitigate potential adverse impacts of extreme events such as marine heatwaves. 

There is a strong interest in accurate forecasts of SST and their anomalies on various time scales. The commonly used approaches include physics-based models and machine learning (ML) methods. The first approach is computationally intensive and limited to shorter time scales. While several attempts have been made by the community to adapt ML models to SST forecasts several challenges still remain. These challenges include improving accuracy for longer lead SST anomaly forecasts. 

Here we present an integrated deep-learning based approach to the problem of SST anomalies and MHW forecasting. On one hand, we capitalise both on inherent climate data structure and recent advances in the field of geometric deep learning. We base our approach on a flexible architecture of graph neural networks, well suited for representing teleconnections. From another hand, we adapt the diffusion method to increase lead time of the forecasts.  Our integrated approach allows marine heatwave forecasts up to six months in advance.

How to cite: Vetrova, V., Ning, D., Bryan, K., and Koh, Y. S.: Forecasting monthly-to-seasonal sea surface temperatures and marine heatwaves with graph neural networks and diffusion methods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12247, https://doi.org/10.5194/egusphere-egu25-12247, 2025.

The expansion of and increasing dependency on renewable energy that exploit climate variables, such as wind and precipitation, are highly sensitive to climate variability and weather extremes. Climate Futures is a Center of Research-based Innovation that aims to “co-produce new and innovative solutions for predicting and managing climate risks from sub-seasonal-to-seasonal (S2S) and seasonal-to-decadal (S2D) time scales with a cluster of partners in climate- and weather-sensitive sectors, including the renewable energy sector, through long-term cooperation between businesses, public organizations and research groups.

The aim of the cross-sectoral collaboration is for renewable energy companies to integrate improved climate predictions into their decision making. The long-term implications are a more resilient energy sector and stable power production. Examples of ongoing projects within the center include (1) using large ensemble climate model simulations to estimate near-future changes in precipitation variability, and (2) estimating future wind power production and variability using state-of-the-art decadal climate predictions. These results are important for future wind- and hydropower operations and infrastructure planning.

How to cite: Svendsen, L.: Climate services for and with the renewable energy sector in Norway, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12574, https://doi.org/10.5194/egusphere-egu25-12574, 2025.

EGU25-13076 | Posters on site | CL4.6

Usage of seasonal forecasts in Tropical Cyclone risk models 

Rudy Mustafa, Ulysse Naepels, Hugo Rakotoarimanga, Rémi Meynadier, and Clément Houdard

Tropical cyclones (TCs) pose significant risks to lives, infrastructure and economies, especially in coastal areas.

AXA has been developing stochastic natural hazard models (also called natural catastrophe or NatCat models) to quantify the impact of events such as TCs on its portfolios. However, NatCat models tend to model the average annual risk for a given peril. NatCat models do not consider the present state of the atmosphere and therefore are not conditioned with respect to the current tropical cyclone season.

Information about the TC risk in the upcoming weeks or months of a season could be crucial for an insurer, especially regarding its reinsurance coverage, but also for better risk mitigation through reinforced and more efficient prevention systems.

Previous studies have demonstrated that ensemble seasonal forecasts have skill in predicting TC occurrence several weeks in advance. We explore the ability of ensemble seasonal forecasts to provided skilled information on the general activity of the season to come for various lead-times (number of occurrences, number of landfalls, ACE…) and how can NatCat models be adapted to provide a more dynamic vision of the TC risk.

How to cite: Mustafa, R., Naepels, U., Rakotoarimanga, H., Meynadier, R., and Houdard, C.: Usage of seasonal forecasts in Tropical Cyclone risk models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13076, https://doi.org/10.5194/egusphere-egu25-13076, 2025.

EGU25-13668 | Orals | CL4.6

Forecasting the annual CO2 rise at Mauna Loa 

Richard Betts, Chris Jones, Jeff Knight, John Kennedy, Ralph Keeling, Yuming Jin, James Pope, and Caroline Sandford

For the last 9 years, the Met Office has issued forecasts of the annual increment in atmospheric carbon dioxide measured at Mauna Loa, accounting for both anthropogenic emissions and the effects of El Niño Southern Oscillation (ENSO) on natural carbon sinks and sources. The first forecast was produced when the 2015-2016 El Niño was emerging, and correctly predicted the largest annual CO2 increment on record at the time. In most years, the inclusion of ENSO provides a more skilful forecast than just considering emissions alone, except for 2022-2023 when La Niña conditions in late 2022 were followed by an early emergence of El Niño conditions in the second quarter of 2023. The impacts of interannual differences in emissions on the CO2 rise are usually smaller than those of ENSO variability, except in 2020 when the emergence of an unexpected large drop in global emissions due to societal responses to the COVID-19 pandemic required the forecast to be re-issued with a new estimate of the annual profile of emissions. Our forecast methodology also provides a simple means of tracking the changes in anthropogenic contributions to the annual atmospheric CO2 rise against policy-relevant scenarios. The Met Office forecast for 2023-2024 predicted a relatively large annual CO2 rise, but the observed rise was even larger, with exceptional wildfires in the Americas a likely contributor to the additional increase. Even without the effects of El Niño and other climatic influences on carbon sinks, the human-driven rise in CO2 in 2023-2024 would have been too fast to remain compatible with IPCC AR6 scenarios that limit global warming to 1.5°C with little or no overshoot. While the 2024-2025 rise is predicted to be smaller than 2023-2024, it will still be above these 1.5°C scenarios.

How to cite: Betts, R., Jones, C., Knight, J., Kennedy, J., Keeling, R., Jin, Y., Pope, J., and Sandford, C.: Forecasting the annual CO2 rise at Mauna Loa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13668, https://doi.org/10.5194/egusphere-egu25-13668, 2025.

EGU25-13771 | Posters on site | CL4.6

Seasonal forecasting of East African short rains 

Giovanni Liguori, Agumase Kindie Tefera, William Cabos, and Antonio Navarra

The variability of East African Short Rains (October-December) has profound socioeconomic and environmental impacts on the region, making accurate seasonal rainfall predictions essential. We evaluated the predictability of East African short rains using model ensembles from the multi-system seasonal retrospective forecasts from the Copernicus Climate Change Service (C3S). We assess the prediction skill for 1- to 5-month lead times using forecasts initialized in September for each year from 1993 to 2016. Although most models exhibit significant mean rainfall biases, they generally show skill in predicting OND (October-December) precipitation anomalies across much of East Africa. However, skill is low or absent in some northern and western parts of the focus area. Along the East African coasts near Somalia and over parts of the western Indian Ocean, models demonstrate skill throughout the late winter (up to December-February), likely due to the persistence of sea surface temperature anomalies in the western Indian Ocean. Years when models consistently outperform persistence forecasts typically align with the mature phases of El Niño Southern Oscillation (ENSO) and/or Indian Ocean Dipole (IOD). This latter mode, when tracked using the Dipole Mode Index, is generally able to predict the sign of the rainfall anomaly in all models. Despite East Africa's proximity to the west pole of the IOD, the correlation between short rains and IOD maximizes when both east and west are considered. This finding confirms previous studies based on observational datasets, which indicate that broader-scale IOD variability associated with changes in the Walker Circulation, rather than local SST fluctuations, is the primary driver behind East African rainfall.     

How to cite: Liguori, G., Tefera, A. K., Cabos, W., and Navarra, A.: Seasonal forecasting of East African short rains, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13771, https://doi.org/10.5194/egusphere-egu25-13771, 2025.

EGU25-13847 | ECS | Posters on site | CL4.6

Decadal Predictions with Diffusion Models: Combining Machine Learning and Earth System Modelling 

Simon Lentz, Johanna Baehr, Christopher Kadow, Johannes Meuer, Felix Oertel, and Bijan Fallah

In the past years, decadal prediction systems have started to fill the gap between seasonal forecasts and long-term climate projections. Despite huge progress in predictive skill and decadal predictions outperforming climate projections in almost all forecast tasks, decadal predictions still possess large rooms for improvement. Machine learning based forecast systems have already outperformed traditional weather forecast systems in recent years. Similarly, machine learning has successfully transformed or assisted in data assimilation or climate data reconstruction tasks. Despite its success in the climate sciences, machine learning methods have not yet been successfully integrated in decadal prediction systems.

Combining machine learning and numerical modeling, we attempt to produce decadal climate predictions utilizing Diffusion Models, essentially probabilistic neural networks. We use such a neural network to predict global 2m-air temperatures by training it on the historical MPI-ESM-LR Grand Ensemble and finetuning it on the MPI-ESM-LR decadal predictions and on ERA5 reanalyses. The resulting predictions are qualitatively comparable to the standard MPI-ESM-LR decadal prediction system, surpassing their predictive skill for leadyears 1 and 2. With diffusion models still new to climate predictions, we expect this result to stand only at the beginning of further machine learning integration into climate predictions in general and decadal predictions in particular.

How to cite: Lentz, S., Baehr, J., Kadow, C., Meuer, J., Oertel, F., and Fallah, B.: Decadal Predictions with Diffusion Models: Combining Machine Learning and Earth System Modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13847, https://doi.org/10.5194/egusphere-egu25-13847, 2025.

EGU25-15772 | Orals | CL4.6

A perfect-model perspective on the signal-to-noise paradox in initialized decadal climate predictions 

Markus G. Donat, Rashed Mahmood, Francisco J. Doblas-Reyes, and Etienne Tourigny

Initialized climate predictions are skillful in predicting regional climate conditions in several parts of the globe, but also suffer from different issues arising from imperfect initializations and inconsistencies between the model and the real world climate and processes. In particular, a so-called signal-to-noise paradox has been identified in recent years. This ‘paradox’ implies that the models can predict observations with higher skill than they predict themselves, despite some physical inconsistencies between modeled and real world climate. This is often interpreted as an indicator of model deficiencies.

Here we present a perfect-model decadal prediction experiment, where the predictions have been initialized using climate states from the model's own transient simulation. This experiment therefore avoids issues related to model inconsistencies, initialization shock and the climate drift that affect real-world initialized climate predictions. We find that the perfect-model decadal predictions are highly skillful in predicting the near-surface air temperature and sea level pressure of the reference run on decadal timescales. Interestingly, we also find signal-to-noise issues, meaning that the perfect-model reference run is predicted with higher skill than any of the initialized prediction members with the same model. This suggests that the signal-to-noise paradox may not be due just to model deficiencies in representing the observed climate in initialized predictions, but other issues that affect the statistical properties of the predictions. We illustrate that this signal-to-noise problem is related to analysis practices that concatenate time series from different discontinuous initialized simulations, which introduces inconsistencies compared to the continuous transient climate realizations and the observations. In particular, the concatenation of predictions initialized independently into a single time series breaks the auto-correlation of the time series.

How to cite: Donat, M. G., Mahmood, R., Doblas-Reyes, F. J., and Tourigny, E.: A perfect-model perspective on the signal-to-noise paradox in initialized decadal climate predictions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15772, https://doi.org/10.5194/egusphere-egu25-15772, 2025.

EGU25-18643 | Orals | CL4.6

Extending the Lead Time for European Winterstorm Activity Predictions 

Gregor C. Leckebusch, Kelvin S. Ng, Ryan Sriver, Lisa Degenhardt, Eleanor Barrie, and Elisa Spreitzer

The most dangerous and costly meteorological hazards in Europe are extreme extra-tropical cyclones and associated windstorms (EUWS) in winter. Recent studies have shown that seasonal prediction systems can skilfully predict the seasonal frequency of EUWS with a one-month lead time using November initialisations. Given that many seasonal prediction systems produce seasonal forecasts at the start of each month, this raises the question whether pre-November initialised seasonal forecasts could provide usable information in predicting seasonal activity of EUWS.

In this study, we will present preliminary results of an approach aimed at extending the predictive horizon of seasonal EUWS activity. While the direct outputs of the pre-November initialised seasonal predictions of EUWS do not have the sufficient skill, skilful predictions of seasonal EUWS activity can be obtained by an approach that utilises the information of the upper ocean mean potential temperature from seasonal prediction systems. Based on our approach, skilful predictions of seasonal EUWS activity becomes possible as early as October.

How to cite: Leckebusch, G. C., Ng, K. S., Sriver, R., Degenhardt, L., Barrie, E., and Spreitzer, E.: Extending the Lead Time for European Winterstorm Activity Predictions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18643, https://doi.org/10.5194/egusphere-egu25-18643, 2025.

Long-range winter predictions over the Euro-Atlantic sector have demonstrated significant skill but suffer from systematic signal-to-noise errors. Here, we examine sources of early winter seasonal predictability in across state-of-the-art seasonal forecasting systems. As in previous studies, these systems demonstrate skill in the hindcasts of the large-scale atmospheric circulation in early winter, associated with the East Atlantic pattern. The predictability is strongly tied to the ENSO teleconnection to the North Atlantic, though the systems' response to ENSO is systematically too weak. The hindcasts of the East Atlantic index exhibit a substantial signal-to-noise errors, with the systems' predicted signal generally being smaller than would be expected for the observed level of skill, though there is substantial spread across systems. The signal-to-noise errors are found to be strongly linked to the strength of the ENSO teleconnection in the systems, those with a weaker teleconnection exhibit a larger signal-to-noise problem. The dependency on modelled ENSO teleconnection strength closely follows a simple scaling relationship derived from a toy model. Further analysis reveals that the strength of the ENSO teleconnection in the systems is linked to climatological biases in the behaviour of the North Atlantic jet. 

How to cite: O'Reilly, C.: Signal-to-noise errors in early winter Euro-Atlantic predictions linked to weak ENSO teleconnections and pervasive North Atlantic jet biases, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18821, https://doi.org/10.5194/egusphere-egu25-18821, 2025.

EGU25-21570 | ECS | Posters on site | CL4.6

Predicting climate indicators at the decadal scale using a hybrid prediction system: application to SUEZ water management plans over France 

Joanne Couallier, Ramdane Alkama, Charlotte Sakarovitch, and Didier Swingedouw

As climate change reshapes hydrological cycles, workers in water management face unprecedented challenges in ensuring resource availability, mitigating flood risks, and maintaining resilient infrastructure. Nowadays, water utilities and authorities rely on long-term climate projections to plan for challenges extending through the end of the century. However, critical gaps persist in actionable information for shorter timescales, such as the decadal scale, which better aligns with political and operational decision-making. In this context, decadal climate predictions can be pivotal to address the needs of the water management sector and develop efficient climate services. However, their added values as compared to projections remained limited up to now.
To better understand user requirements, we collaborate with various teams from SUEZ, a company specializing in water management. Through interviews, we have identified the demand for specific indicators based on climate variables (e.g., precipitation, temperature) and corresponding spatio-temporal scales. Building on this understanding, we also develop in IPSL-EPOC decadal prediction team a new hybrid approach to improve our forecasts. This approach includes identifying a climate index (e.g., NAO, WEPA) derived from Sea Level Pressure (SLP) that correlates with the climate variable of interest. Using all the available decadal climate predictions from the DCPP project, we evaluate the predictability of this index, which is usually high for NAO and WEPA. This index is then employed to subsample a few of member CMIP6 climate projections that are in phase with the prediction of the DCPP ensemble. This latter step allows to inflate the amplitude of the predictable signal, resolving the limitation coming from the signal-to-noise paradox. It is also allowing to perform a proper statistical downscaling, used to refine these forecasts, ensuring their usability for identified needs. The resulting forecasts are designed to integrate seamlessly into SUEZ’s water sector models.
Preliminary work has identified diverse parameters of interest for water management, such as daily precipitation (resource availability forecasting), extreme precipitation events at fine temporal resolution (Combined Sewer Overflows modeling), and the number of very cold or very hot days (linked to risks of water mains and service lines failures, respectively). Early findings also suggest that, for the average precipitation over France, the WEPA index exhibits the largest correlations, unlike the NAO, which has greater influence for other European regions. The production of forecasts is currently underway, and their performance regarding the initially identified parameters will be presented.

How to cite: Couallier, J., Alkama, R., Sakarovitch, C., and Swingedouw, D.: Predicting climate indicators at the decadal scale using a hybrid prediction system: application to SUEZ water management plans over France, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21570, https://doi.org/10.5194/egusphere-egu25-21570, 2025.

Predicting the diurnal cycle of deep convection is valuable for applications ranging from day-to-day weather forecasting and aviation safety to climate modelling and resource management. However, current weather and climate models often struggle to accurately capture the timing of deep convective events, frequently predicting the peak of convective precipitation and the onset of storm formation too early. This study suggests that these timing inaccuracies stem from the absence of cloud-convection interactions in many models. Such interactions represent rapid feedback mechanisms with timescales similar to the transition from shallow to deep convection within a diurnal cycle (Vraciu et al., 2024). By contrast, the typical convective parameterization schemes used by the weather prediction and climate models only incorporate interactions between convection and a uniform environment, which produces feedback mechanisms too slow to align with the diurnal cycle's timing.

To address this gap, this work introduces a unified cloud-convection model that includes both cloud-convection and convection-environment interactions, applicable to both shallow and deep convection. The proposed model comprises a set of prognostic equations for the fractional areas of different cloud types and the convective updraft velocity at varying levels. In addition, following the framework of Arakawa and Schubert (1974), a prognostic equation is included to account for the cloud feedback on the large-scale environment for each cloud type. The model is tested using idealized large-eddy simulations of the shallow-to-deep transition in a diurnal cycle, yielding promising results. Furthermore, the role of cold pools is discussed in the new proposed model, based on simulations where cold pool effects are suppressed. The prognostic model presented here may form the basis for a new class of cumulus parameterization schemes with unified cloud-convection representation and unified shallow and deep treatment.

 

References:

Arakawa, A., & Schubert, W. H. (1974). Interaction of a cumulus cloud ensemble with the large-scale environment, Part I. Journal of the Atmospheric Sciences, 31(3), 674-701.

Vraciu, C. V., Savre, J., & Colin, M. (2024). The rapid transition from shallow to precipitating convection as a predator-prey process. ESS Open Archive, DOI: 10.22541/au.170964875.54219458/v2.

How to cite: Vraciu, C.-V.: A unified cloud-convection prognostic model for the diurnal cycle of deep convection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-42, https://doi.org/10.5194/egusphere-egu25-42, 2025.

EGU25-1221 | Orals | AS1.10

Investigating the effects of orography and ambient wind on deep convection over tropical islands 

Frank Robinson, Daniel Kirshbaum, Steven Sherwood, Lucinda Cahill, Erica Juliano, and Chuntao Liu

Examination of the Tropical Rainfall Measuring Mission (TRMM) satellite database (1994-2015) of 272 tropical and subtropical islands reveals a modest weakening of convective intensity with increased terrain height,h or ambient wind,U (for a given island area, A), and a strengthening with increasing A. Quasi-idealized, convection-permitting simulations broadly reproduce these sensitivities to h and A, but not that to U. In both observations and simulations, intensity increases with the island-averaged convective available potential energy (CAPE). Because CAPE generally decreases over taller islands that protrude deeper into the free troposphere, convective intensity varies inversely with h. The frequency of convective events increases with total island area over which both large CAPE and strong near-surface horizontal convergence coincide. This trend favors higher frequencies over larger islands with complex (but shallow) terrain. The model's inability to reproduce the observed decrease of convective intensity with U stems from a negative observed correlation between CAPE and U that was neglected in the simulations. Thus, as with h, the negative observed trend between intensity and U ultimately stems from the impacts of CAPE on convective intensity.

How to cite: Robinson, F., Kirshbaum, D., Sherwood, S., Cahill, L., Juliano, E., and Liu, C.: Investigating the effects of orography and ambient wind on deep convection over tropical islands, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1221, https://doi.org/10.5194/egusphere-egu25-1221, 2025.

EGU25-1228 | ECS | Orals | AS1.10

A robust constraint on the response of convective mass fluxes to warming 

Andrew I. L. Williams and Nadir Jeevanjee

A fundamental quantity in tropical dynamics is the `convective mass flux', which measures the rate at which mass is transported upwards, per unit area, in convective updrafts. Convective mass flux encodes information about the frequency and intensity of thunderstorms, and has been linked to the strength of the large-scale tropical circulation. Changes in convective mass flux under warming are thus an important, but uncertain, aspect of climate change. Here we build off recent work linking changes in mass flux to the clear-sky energy budget to show that convective mass fluxes decrease along isotherms at around 3-5 \% K$^{-1}$ under warming. We show that this constraint holds throughout the free-troposphere and across a hierarchy of models; from idealized radiative-convective equilibrium simulations to CMIP6 models. This decrease in convective mass flux with warming is driven by a stabilization of the lapse rate and can be captured with a simple analytical model. We also revisit previous work by Held and Soden (2006), who proposed a scaling for changes in the convective mass flux with warming. We show that the Held and Soden scaling does not capture inter-model spread in cloud-base mass flux changes under warming in cloud-resolving models, and that their original verification is not robust across GCMs. Altogether, this work provides a quantitative constraint on changes in convective mass flux throughout the troposphere which can be derived from first principles, and which is verified across a hierarchy of models. 

How to cite: Williams, A. I. L. and Jeevanjee, N.: A robust constraint on the response of convective mass fluxes to warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1228, https://doi.org/10.5194/egusphere-egu25-1228, 2025.

EGU25-1540 | Posters on site | AS1.10

Using observations from the new ATTO-Campina site and LES modeling to study cloud organization and the shallow-to-deep transition 

Micael Amore Cecchini, Rachel Ifanger Albrecht, Luiz A. T. Machado, Paulo Artaxo, Gabriel G. Balestra, Amábile S. Bighetto, and Marina C. S. Neofiti

We first present a summary of results from ATTO-Campina, a new permanent observational site deployed in central Amazon, about 4 km from the ATTO towers. Those results are then complemented by preliminary modeling studies about shallow cumulus clouds organization. Operational since 2020, ATTO-Campina focuses on characterizing atmospheric, cloud and rainfall properties through remote sensing. The overarching goal is to provide continuous, complementary measurements to the ATTO towers, addressing the rainforest’s complex and unique gas-aerosol-cloud-precipitation dynamics. Previous studies have highlighted the critical role of convective clouds in the new particle formation (NPF) process, driven by the vertical transport of gasses and aerosol particles. Using a 3.5-year dataset, we classified convective clouds into three types: shallow cumulus (ShCu), congestus (Con) or (Deep) clouds. The shallow-to-deep transition takes about three hours, starting with ShCu formation at 11:00 local time. The accumulated rainfall peak follows at about 16:00 local time. Only weak downdrafts are present in the upper troposphere where NPF takes place, while strong downdrafts are mostly limited to heights below 5 km. Con and Deep convective days have higher concentrations of ultrafine aerosol and lower concentration of accumulation-mode particles compared to ShCu. Convective clouds also significantly modify gas mixing ratios, with a distinct background concentration of CO2 for different cloud types. In addition, deep convective clouds considerably increase the O3 mixing ratio close to the surface. Our results showcase the added detail achieved by integrating data from the ATTO towers and ATTO-Campina sites. Together, these sites support a better understanding of the interconnected gas-aerosol-cloud-precipitation processes in the Amazon and their evolution under the influence of climate change. On the modeling side, we provide preliminary results from 100-m resolution simulations of shallow cumulus cloud fields. The cloud fields are analyzed in terms of their organization indexes and the role of aerosols is quantified on changes of those indexes. Overall, we will discuss the characteristcs of shallow and deep convection in the Amazon, as well as how the organization indexes can be used to quantify the shallow-to-deep transition.

How to cite: Cecchini, M. A., Albrecht, R. I., Machado, L. A. T., Artaxo, P., Balestra, G. G., Bighetto, A. S., and Neofiti, M. C. S.: Using observations from the new ATTO-Campina site and LES modeling to study cloud organization and the shallow-to-deep transition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1540, https://doi.org/10.5194/egusphere-egu25-1540, 2025.

EGU25-2141 | Posters on site | AS1.10

Lifecycle Of Convective Precipitation Systems over the Arabian Peninsula Using Object Tracking 

Ahmed Homoudi, Klemens Barfus, Christian Bernhofer, and Matthias Mauder

The Arabian Peninsula (AP) is one of the most arid regions, and precipitation is scarce; it occurs as sporadic and localised convective events (Loung et al., 2020). Numerous studies have focused on studying precipitation in the AP using pixel-wise methods. However, these methods fail to scrutinise the development of precipitation systems from a Lagrangian perspective. A Lagrangian framework can provide valuable insights such as the lifecycle of convective cells and their response to climate change. To address this gap, precipitation in the AP needs to be examined using object-based methods.

We utilise the IMERG V07 data and apply a modified version of the tracking algorithm developed by Seelig et al. (2021, 2023) to obtain precipitation systems (a sequence of object tracks with the possibility of merging and splitting). The tracking algorithm combines overlapping and centroid projection methods, with the centroid projection technique utilising motion vectors derived from particle imaging velocimetry. We use a threshold of 0.5 mm/h to delineate the objects and a threshold of 3 mm/h to filter non-convective systems. Furthermore, we classify the systems into different types using hierarchical agglomerative clustering.

The results show three distinct types of precipitation systems over the AP: a) summer systems (T1), occurring over the southern AP and reaching their peak frequency in August, influenced by the Indian monsoon; b) spring systems (T2), observed over the middle to southern areas of the AP with a peak in April, modulated by extratropical-tropical moisture transport; and c) winter systems (T3), located over the northern AP and peaking in December, impacted by extratropical cyclones entering the AP. The typical life cycle of these systems involves reaching their peak intensity first, followed by maximum precipitation volume, and finally, their largest extent. Nevertheless, T2 systems living longer than 24 hours show varying behaviour. The early afternoon is the most favourable time for rain initiation for T1 and T2 systems, whereas it is the late evening for T3 systems. Most T1 systems cease to rain in the late afternoon. However, both T2 and T3 systems stop around midnight. Generally, systems with merging/splitting objects show higher growth and decay rates than those without merging/splitting.

References:

Luong, T. M., Dasari, H. P., & Hoteit, I. (2020). Extreme precipitation events are becoming less frequent but more intense over Jeddah, Saudi Arabia. Are shifting weather regimes the cause? Atmospheric Science Letters, 21(8), e981. https://doi.org/10.1002/asl.981

Seelig, T., Deneke, H., Quaas, J., & Tesche, M. (2021). Life Cycle of Shallow Marine Cumulus Clouds from Geostationary Satellite Observations. Journal of Geophysical Research: Atmospheres, 126(22). https://doi.org/10.1029/2021JD035577

Seelig, T., Müller, F., & Tesche, M. (2023). Do Optically Denser Trade-Wind Cumuli Live Longer? Geophysical Research Letters, 50(13), 1–8. https://doi.org/10.1029/2023GL103339

How to cite: Homoudi, A., Barfus, K., Bernhofer, C., and Mauder, M.: Lifecycle Of Convective Precipitation Systems over the Arabian Peninsula Using Object Tracking, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2141, https://doi.org/10.5194/egusphere-egu25-2141, 2025.

EGU25-2257 | ECS | Orals | AS1.10

The Gill and non-Gill equatorial wave circulations associated with convective variability over the subtropical western North Pacific 

Peishan Chen, Nedjeljka Žagar, Frank Lunkeit, Katharina Holube, Yuan-Bing Zhao, and Riyu Lu

Atmospheric convection over the subtropical western North Pacific (SWNP) varies on time scales around 2 weeks with significant effects on local and remote circulation. Among unknown effects, coupling between the SWNP convection variability and equatorial wave circulation is poorly understood. This paper quantifies equatorial wave perturbations using a global, wave space regression between the 43-year outgoing longwave radiation data over the SWNP region and spectral expansion coefficients of tropospheric circulation from ERA5 reanalyses. The resulting tropical wave flow is divided between the Rossby and Kelvin waves, which constitute the Gill pattern of tropical wave response to heating, and mixed Rossby-gravity (MRG) and inertia-gravity (IG) waves, which are named non-Gill pattern. The non-Gill part in the upper tropical troposphere is shown to have as large amplitude as the Gill part of the response. In particular, the IG and MRG waves contribute most of the cross-equatorial circulation and the MRG wave signals have about 25% greater amplitude than the IG wave signals. As SWNP convection intensifies, the MRG wave northerly winds across the equator strengthen whereas the IG waves represent strengthening outflow over the SWNP region. The combined effect of the Kelvin and Rossby waves enhance the circulation on the equatorward side of the anticyclone over the SWNP region, with the three times stronger Rossby wave than Kelvin wave easterlies in the upper troposphere. In the weakening phase of the SWNP convection, the northerly IG flow in the southern Indian ocean is coupled with developing anticylonic circulation of Rossby waves, suggesting the effects on extratropics in austral winter. The results suggest a caution when using Gill solution for the interpretation of circulation associated with asymmetric heating sources in real atmosphere or its models.

How to cite: Chen, P., Žagar, N., Lunkeit, F., Holube, K., Zhao, Y.-B., and Lu, R.: The Gill and non-Gill equatorial wave circulations associated with convective variability over the subtropical western North Pacific, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2257, https://doi.org/10.5194/egusphere-egu25-2257, 2025.

EGU25-4833 | ECS | Orals | AS1.10

Environmental Drivers and Dynamics of Downdrafts in Simulations of Convection 

Quinlan Mulhern and John Peters

Downdrafts play an essential role in the feedback between deep convective clouds and their surrounding environment, and they must be properly accounted for in climate model parameterization schemes. Such downdrafts found near and in-cloud, such as subsiding shells and hydrometeor-loaded downdrafts, significantly contribute to downward mass flux in the lower and middle troposphere. However, environmental links to driving mechanisms and characteristics of downdrafts must be understood for proper implementation in parameterization schemes. Using CM1, simulations modeling convection were performed utilizing weakly-sheared dry and wet season composite soundings compiled during the Green Ocean Amazon Campaign, as well as similar thermodynamic soundings with a prescribed increase of vertical wind shear. The soundings in this study were adapted to isolate relative humidity and shear effects on convective downdrafts. All deep convective updrafts in the simulations that met a required vertical velocity threshold were analyzed, along with their near-cloud environments and associated downdrafts. Magnitude differences of subsidence in the matrix of environments encouraged a parcel trajectory analysis, which showed that downward accelerations were primarily driven by negative buoyancy accelerations and were aided by cloud-top pressure perturbations. Compared to other near-cloud downdrafts, subsiding shell accelerations relied heavily on strongly negative thermal buoyancy for downward accelerations but were also moderated by upward vertical perturbation pressure gradient accelerations away from cloud top, ultimately making them weaker than all other downdrafts. Future work aims to increase understanding of and improve mass transport processes found in near-cloud downdrafts and apply such understanding to climate model cumulus and convective parameterization schemes.

How to cite: Mulhern, Q. and Peters, J.: Environmental Drivers and Dynamics of Downdrafts in Simulations of Convection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4833, https://doi.org/10.5194/egusphere-egu25-4833, 2025.

EGU25-5932 | Orals | AS1.10

Strengthening of Mesoscale Convective Systems by Soil Moisture Gradients in ICON  

Emma Barton, Cornelia Klein, Christopher Taylor, John Marsham, Douglas Parker, Ben Maybee, Zhe Feng, L. Ruby Leung, and Cathy Hohenegger

Mesoscale convective systems (MCSs) are large, organised storms that threaten communities in multiple regions around the world with extreme rainfall, lightning and strong winds that can lead to flooding, mudslides, destruction of property and loss of life. Improving predictability of these storms is vital for reducing their impact on the population and requires understanding of processes that favour their growth.

Our recent observation-based analysis of thousands of MCSs across seven storm “hot-spots” (West Africa, South Africa, India, China, South America, Great Plains and Australia) revealed a new mechanism of storm enhancement by mesoscale (~500 km) soil moisture gradients via vertical wind shear, a key ingredient for MCS growth. Specifically, a 10-30% increase in extreme (90th percentile) precipitation feature size and rainfall was observed on days with favourable surface conditions, compared to days with unfavourable conditions.

In the current work we exploit multidecadal global convection permitting high-resolution (10 km) ICON simulation to analyse surface driven MCS enhancement under climate change. For the seven regions considered in the observational analysis, in ICON we find precipitating mature storms to be favoured in the vicinity of mesoscale soil moisture gradients and a strong relationship between vertical wind shear and storm size and rainfall, consistent with the observations. For an SSP370 type scenario (7 W/m² forcing by the year 2100) we show the impact of changing surface conditions on MCS enhancement linked to our identified mechanism.

How to cite: Barton, E., Klein, C., Taylor, C., Marsham, J., Parker, D., Maybee, B., Feng, Z., Leung, L. R., and Hohenegger, C.: Strengthening of Mesoscale Convective Systems by Soil Moisture Gradients in ICON , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5932, https://doi.org/10.5194/egusphere-egu25-5932, 2025.

EGU25-6495 | ECS | Posters on site | AS1.10

Response of Microphysical and Rainfall Characteristics to Cloud Seeding: A case study of widespread cloud seeding operations over Saudi Arabia 

Raja Boragapu, ioannis Matsangarous, Stavros A Logothetis, and Ayman Mohmmed Albar

The Kingdom of Saudi Arabia (KSA) consists of arid and semi-arid climates with extremely low levels of daily rainfall. Cloud seeding is an exemplary alternative to enhance rainfall and thus increase the water resources in the region. The Regional Cloud Seeding Program of the National Center for Meteorology was initiated in 2022 to address this issue through glaciogenic and hygroscopic seeding of convective clouds over the southwest and central parts of KSA. However, to understand and improve the effectiveness of cloud seeding, it is essential to analyse the rainfall characteristics and cloud microphysical processes in the region. Given the unique combination of dry and hot background conditions, analysing their response is particularly important due to their sensitivity to any seeding activity in the region. High resolution numerical simulations are performed using the Weather Research and Forecasting model (WRF4.6) to investigate the microphysical and rainfall characteristics of convective clouds. Valuable data derived from research aircraft used for validating the simulations and understanding cloud microphysical process. The study emphasizes the sensitivity of rainfall enhancement to model configurations on microphysics schemes during a widespread seeding activity over the southwest and central parts of KSA. 

How to cite: Boragapu, R., Matsangarous, I., A Logothetis, S., and Mohmmed Albar, A.: Response of Microphysical and Rainfall Characteristics to Cloud Seeding: A case study of widespread cloud seeding operations over Saudi Arabia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6495, https://doi.org/10.5194/egusphere-egu25-6495, 2025.

EGU25-6542 | ECS | Orals | AS1.10

Diabatic heating of mesoscale convective cloud systems from synergistic satellite data  

Xiaoting Chen, Claudia Stubenrauch, and Giulio Mandorli

Upper tropospheric clouds are most abundant in the tropics and often form as cirrus anvils from convective outflow, building mesoscale systems (MCS). While latent heating is released into the atmosphere by the precipitating parts of these MCSs, the long-lasting anvils play a crucial role in modulating the Earth’s energy budget and heat transport. Convective organization may change the relationship between latent and radiative heating within the MCSs.

We present a coherent long-term dataset which describes tropical UT cloud systems for process and climate studies. In order to investigate also the cirrus surrounding these anvils, we used CIRS (Clouds from IR Sounders) data, retrieved from AIRS (Atmospheric InfraRed Sounder) and IASI (Infrared Atmospheric Sounding Inferometer) measurements, together with atmospheric and surface properties from the meteorological ERA reanalyses as input to artificial neural network (ANN) models to simulate the cloud vertical structure and radiative heating rates derived from CloudSat radar – CALIPSO lidar measurements, available only along narrow nadir tracks. In this way, we could expand this sparse sampling in space and in time. Furthermore, a rain rate classification, with an accuracy of about 70%, allows us to build objects of strong precipitation to identify convective organization. This dataset is now available at https://gewex-utcc-proes.aeris-data.fr/data/.

We could demonstrate that this rain intensity classification is more efficient than cold brightness temperatures to detect large latent heating, the latter derived from radar measurements of the Tropical Rainfall Measuring Mission (TRMM). While TRMM provides a diurnal sampling over a month, the spatial coverage within a time window of one hour is only about 7%. Therefore, we also expanded these latent heating profiles over the whole tropics, using ANN regression. The zonal averages of vertically integrated latent heating (LP) align well with those from the full diurnal sampling of TRMM–SLH over ocean.

In combination with a cloud system analysis we found that deeper convection leads to larger heavy rain areas, with a slightly smaller thick anvil emissivity. Convective organization enhances the mean atmospheric cloud radiative effect (ACRE) of the MCSs, in particular at small rain intensity. The projection of different MCS properties in the LP-ACRE plane can be further used for a process-oriented evaluation of parameterizations in climate models.

How to cite: Chen, X., Stubenrauch, C., and Mandorli, G.: Diabatic heating of mesoscale convective cloud systems from synergistic satellite data , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6542, https://doi.org/10.5194/egusphere-egu25-6542, 2025.

EGU25-6843 | ECS | Posters on site | AS1.10

Evaluation of eddy dissipation rate within a regional atmospheric model (MetUM) using radar retrievals 

Chun Hay Brian Lo and Thorwald H. M. Stein

Turbulent processes are important for cloud evolution and their morphology. Turbulent mixing is partly parametrised in sub-km numerical weather prediction models, whose simulations of convection are sensitive to the configuration of sub-grid turbulence schemes. Past studies have used large-eddy simulations and aircraft observations to characterise turbulence generated by clouds and thunderstorms in Germany and Australia. However, characteristics of in-cloud turbulence and especially its spatial distribution remain poorly understood.

Here, we present an evaluation of sub-km simulations of convective storms with the Met Office Unified Model against turbulence estimates derived from radar measurements collected as part of the 2023 Wessex convection (WesCon) field campaign over the southern United Kingdom. Turbulence intensity is expressed as an eddy dissipation rate, ε and retrieved by isolating the turbulent component of the Doppler velocity spectrum width observed by the Chilbolton Advanced Meteorological Radar.

In a WesCon deep convection case, median in-cloud values of retrieved ε range from 3 × 10-3 to 2 × 10-2 m2s-3, with values increasing with height. Results are compared with equivalent statistics derived from 300-m, 100-m and 55-m grid-length Met Office Unified Model simulations of the observed cases to evaluate the model’s blended sub-filter mixing scheme. More intense turbulence was found near the tops of simulated reflectivity cores with regions of high ε co-located with regions of strong horizontal shear around updrafts. The 95th and 99th percentiles of 300-m grid length model ε are comparable with observations, while simulated ε values within finer grid resolutions are up to half an order of magnitude lower. In contrast to observations, turbulence intensity within simulations peaks in the mid-levels of the convective clouds before decreasing with height.

How to cite: Lo, C. H. B. and Stein, T. H. M.: Evaluation of eddy dissipation rate within a regional atmospheric model (MetUM) using radar retrievals, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6843, https://doi.org/10.5194/egusphere-egu25-6843, 2025.

We develop a novel approach to detect cloud-subcloud coupling during the cloud life cycle and analyze a large eddy simulation of marine shallow cumulus based on the Barbados oceanographic and meteorological experiment campaign. Our results demonstrate how the activity of sub-cloud coherent updrafts (SCUs) affect the evolution of shallow cloud properties during their life cycles, from triggering to development, and through to dissipation. Most clouds (~80%) are related to SCUs during their lifetime but not every SCU (~20% for short-lived ones) leads to cloud formation. The fastest growing SCUs in a relatively moist region are most likely to initiate clouds. The evolution of cloud base mass-flux depends on cloud lifetime. Compared with short-lived clouds, longer lived clouds have longer periods of development, even normalized by the full lifetime, and tend to increase their cloud base mass-flux to a stronger maximum. This is consistent with the evolution of mass flux near the top of SCU, indicating that the development of clouds is closely related to the sub-cloud activity. When the SCUs decay and detach from the lifting condensation level, the corresponding cloud base starts to rise, signifying the start of cloud dissipation, during which the cloud top lowers to approach the rising cloud base. Previous studies have described similar conceptual pieces of this relationship but here we provide a continuous framework to cover all the stages of cloud-subcloud coupling. Our findings provide quantitative evidence to supplement the conceptual model of the shallow cloud life cycle and could help to improve the steady-state assumption in parameterization.

How to cite: Holloway, C. E., Gu, J.-F., and Plant, R. S.: Connections Between Sub-Cloud Coherent Updrafts and the Life Cycle of Maritime Shallow Cumulus Clouds in Large Eddy Simulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7055, https://doi.org/10.5194/egusphere-egu25-7055, 2025.

Shallow cumulus clouds (SCC) play a vital role in regulating the Earth’s energy and water cycles, yet their accurate representation in numerical weather prediction and climate models remains a significant challenge. This study employs realistic large-eddy simulations (LES) using the ICON model to analyze both instantaneous and lifetime-averaged statistics of SCC observed on three different days during the FESSTVaL campaign. The excess of virtual potential temperature within the cloud is used to categorize the clouds into active and passive states. The estimated cloud mass flux follows the Weibull distribution, with distinct shape parameters for active and passive clouds, reflecting the memory of the random process. The unity shape parameter for passive clouds indicates memorylessness, while a shape parameter less than unity for active clouds highlights the role of convective memory, where past convection influences the current convective state.

Additionally, the mass flux distribution varies significantly across different cases. These differences can be explained in terms of efficiency, which depends on energy partitioning, the Bowen ratio, and large-scale forcing, and is conceptually linked to approximating moist atmospheric convection as a moist heat engine. This further highlights the role of turbulent fluxes and boundary layer dynamics in shaping the efficiency, which governs the estimation of moist static energy under varying environmental conditions. These findings enhance our understanding of SCC dynamics and offer valuable insights for improving cloud parameterizations in weather and climate models. This study underscores the crucial role of realistic numerical simulations in addressing the challenges of atmospheric convection and turbulence, particularly at the gray-zone scale.

How to cite: Singh, J., Sakradzija, M., and Schmidli, J.: Investigating the Cloud Base Mass Flux and Its Controlling Factors in Shallow Cumulus: Insights from Realistic Large-Eddy Simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7335, https://doi.org/10.5194/egusphere-egu25-7335, 2025.

EGU25-8288 | Orals | AS1.10

How does a convection cluster respond to a large-scale mean wind? 

Bidyut Bikash Goswami, Alexis Aubel, and Caroline Muller

Atmospheric convection can spontaneously cluster and confine within an envelope. These clusters of convection often propagate under the influence of a large-scale mean wind, such as the Madden-Julian oscillation (MJO). The motivation of this study is to understand how a large-scale mean wind influences the propagation of a convection clusterTo this end, we investigate the response of convective self-aggregation, a model depiction of a convection cluster in radiative-convective equilibrium (RCE), to a wind perturbation. We impose a constant mean wind on aaggregated convective system (obtained through a simulation without mean windand observe its evolution in a three-dimensional cloud-resolving model. We note in our modeling experiments that convection clusters exhibit a propagating behavior under a large-scale mean windalbeit with a speed that is less than the prescribed forcing. We find that surface fluxes are critical in slowing down the convection clusters. Enthalpy and momentum fluxes slow down the convection cluster with comparable effects through different mechanisms. Enthalpy fluxes favor convection upwind through the wind-induced surface heat exchange (WISHE) feedback, opposing the convection cluster movement. Momentum flux acts aa negative feedback on surface winds in places of strongest near-surface winds.

How to cite: Goswami, B. B., Aubel, A., and Muller, C.: How does a convection cluster respond to a large-scale mean wind?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8288, https://doi.org/10.5194/egusphere-egu25-8288, 2025.

This work describes the study of the influence of vertical wind shear (hereafter "shear") on deep convective clouds. Using a set of high-resolution Large-Eddy Simulations (LES) produced by the research model Meso-NH with varying shear, tendencies in the relationship between shear magnitude and the organisation and intensity of the storms are drawn. Increasing shear is associated with higher precipitations, stronger ascent in the updraft, and more intense cold pools under the convective cells. When the shear becomes strong enough, the convective cells evolve into supercells, drastically changing the regime of the event and highlighting a non-linearity in the behaviour of convective systems. Turbulent quantities are affected, with higher subgrid and resolved turbulent kinetic energy (TKE) for higher intensity storms. Moreover, the upwind TKE is higher than the downwind TKE, although the ratio for all simulations is not affected. Using four different indicators of organisation, a clear trend towards increasing organisation is diagnosed, with the supercell regime diverging from the other simulations. Vertical wind shear, via its effect on the organisation of convective cells, significantly alters the effect of convective storms, and should be taken into account by parametrization schemes.

How to cite: Bidou, G., Ricard, D., and Lac, C.:  Influence of vertical wind shear on organisation and decametric-scale turbulence in convective clouds using large-eddy simulations., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8868, https://doi.org/10.5194/egusphere-egu25-8868, 2025.

EGU25-9530 | ECS | Posters on site | AS1.10

The response of deep convection to solar geoengineering 

Alzbeta Pechacova, Lokahith Agasthya, and Caroline Muller

Solar geoengineering proposes to reduce the surface warming caused by increased concentrations of greenhouse gases through a manipulation of the incoming solar radiation. The response of the climate system to various geoengineering scenarios has been investigated using Global Climate Models (Kravitz, Caldeira, et al. 2013, Kravitz, Rasch, et al. 2013), including the impacts on tropical precipitation, stability and radiative fluxes. However, similar simulations in high-resolution limited domain models are largely limited to shallow convection (Schneider, Kaul, and Pressel 2020).

This study focuses on the effect of solar geoengineering on tropical deep convection. We performed a set of idealized simulations in a cloud-resolving model (Khairoutdinov and Randall 2003) with increasing CO2 concentrations. Solar geoengineering was represented simply by fixing the sea surface temperature to 300 K across all experiments. This setup resulted in the expected decrease in radiative cooling, and thus reduced evaporation and precipitation. A slight decrease in anvil cloud cover was observed, but cloud top temperature remained nearly constant, supporting the fixed anvil temperature (FAT) hypothesis (Hartmann and Larson 2002), more so than the tropopause temperature. The shortwave and longwave cloud radiative effects both decreased in magnitude due to the reduced cloud fraction. Additionally, the longwave heating effect was reduced further due to a lower effective emission temperature of the clear sky, resulting in a smaller difference between the radiation emitted by clear and cloudy sky.

These results partially agree with results from GCMs and they offer insight into how tropical clouds might respond to solar geoengineering. Plans for future work include a more realistic representation of solar geoengineering (e.g. interactive SST with a reduced solar constant) as well as improved high cloud microphysics.

How to cite: Pechacova, A., Agasthya, L., and Muller, C.: The response of deep convection to solar geoengineering, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9530, https://doi.org/10.5194/egusphere-egu25-9530, 2025.

EGU25-10136 | ECS | Orals | AS1.10

Multiscale oceanic precipitation extremes are determined by the morphology of rain events throughout the lifecycle of deep convective systems. 

Maxime Carenso, Benjamin Fildier, Rémy Roca, and Thomas Fiolleau

Extreme precipitation intensities in the tropics depend strongly on the spatiotemporal scale at which they are calculated, potentially introducing biases when assessing their physical drivers, impacts, and climate sensitivities. Furthermore, the contribution of Mesoscale Convective Systems (MCSs) to these extremes remains loosely constrained, especially on kilometer scales. Here, we use a new analysis framework for the co-occurrence of oceanic precipitation extremes at both convective (km) and mesoscale levels, and we compare their regional prevalence and rainfall morphology. We apply a storm tracking algorithm to ten global storm-resolving models (GSRMs) and one multi-year geostationary satellite product, focusing on various convective system types.

Our results reveal that the two scales of precipitation extremes are largely statistically independent, occurring in distinct regions with large model disagreement. Heavy km-scale events predominantly appear at the edges of convective zones, with 40% of such extremes in the satellite observations produced by MCSs. Their peak intensity is not correlated with the total area of precipitation features. In contrast, intense mesoscale events scale with the precipitating area, and are generated by MCSs in about a third of cases. We also observe a continuum of extreme precipitation features, spanning deep (DCS), very-deep (vDCS), and mesoscale convective systems.

We finally discuss the relative importance of cloud and rain morphology and life cycle parameters for understanding rain extremes on multiple scales, and we comment on relationships between environmental conditions and extreme-contributing DCS that emerge in our new multiscale analysis framework.When compared to observations, the models typically underestimate the precipitating surface and show substantial variability in the fraction of extreme rainfall attributable to different convective systems. These diagnostics highlight the need for further refining GSRMs to more accurately capture the relationship between convective organization and heavy rainfall.

How to cite: Carenso, M., Fildier, B., Roca, R., and Fiolleau, T.: Multiscale oceanic precipitation extremes are determined by the morphology of rain events throughout the lifecycle of deep convective systems., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10136, https://doi.org/10.5194/egusphere-egu25-10136, 2025.

Abstract:A review was conducted of the subjective and objective forecasts and their biases for the extreme thunderstorm and gale event in Beijing on May 30, 2024. Additionally, using multi-source observational data such as Beijing's S-band dual-polarization radar and automatic weather stations, an analysis was performed on the convective characteristics, causes, and mechanisms of the gale. The results indicate: (1) This thunderstorm and gale event was influenced by a cold vortex, characterized by significant temperature differences between the upper and lower troposphere and moderate-to-strong vertical wind shear conditions, but with extremely poor humidity. The gale exhibited extreme characteristics. (2) Scattered convection rapidly intensified into a squall line as it moved downslope. Radar monitoring revealed widespread velocity aliasing, rear inflow jet (RIJ), and local small-scale vortices, all indicating straight-line strong winds at the surface and locally possible vortex-induced strong winds. (3) The primary reason for the forecast bias was inadequate consideration of the intensity of convection downslope in a dry environment. In conditions of poor humidity unfavorable for convection enhancement downslope, the coupling of thermodynamic processes can rapidly saturate the relative humidity near the storm, thereby enhancing convection downslope in conjunction with strong thermodynamic instability and dynamic processes. (4) The RIJ forms as a compensation for the intense downward divergent airflow within the storm, which subsequently further entrains dry air into the cloud. The evaporation, cooling, and temperature decrease processes of cloud and rain particles within the storm result in the formation of strong dry convective available potential energy (DCAPE), which enhances surface winds. This is the reason for the intensification of winds leading to extreme thunderstorm and gale events.

Keywords:Extreme Gale, Cold Vortex, Dry Environment, Enhanced Downslope Convection , Rear Inflow Jet(RIJ)

How to cite: Lei, L.: The Characteristic and Mechanism of an Extreme Gale in Beijing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11259, https://doi.org/10.5194/egusphere-egu25-11259, 2025.

In the tropics, a significant portion of precipitation originates from deep convective systems (DCS), which are composed of convective cells organized in both space and time. These systems are characterized by upper-level cloud shields made up of high-altitude, ice-topped clouds that form cohesive and recognizable structures, easily identifiable in satellite imagery. These cloud shields vary widely in spatial and temporal scales, ranging from a few dozen to millions of square kilometers and lasting from a few hours to several days. Due to their ubiquity over tropical oceans, these cloud shields play a critical role in the Earth's radiation budget and influence related climatic feedbacks. However, their potential morphological changes in response to climate change remain poorly understood.

In this study, we analyze the sensitivity of the cloud shield morphology to environmental conditions using a comprehensive dataset spanning nine years of satellite observations over the entire tropical ocean. By combining this dataset with the recent ECMWF reanalysis, we build robust statistics to explore the relationship between cloud shield morphology and environmental factors. Our focus is on a specific dimension of this complex problem: investigating how the thermodynamic and dynamic environment influences the morphology of the cloud shield. This work advances previous studies by encompassing the full spectrum of deep convective systems (DCS), rather than focusing solely on mesoscale convective systems (MCS). Moreover, we emphasize the cloud shield characteristics of these systems, going beyond the traditional focus on precipitation features morphology. Multilinear regression between DCS morphology and environment is used in a 2D phase space linked to the life cycle of the systems, namely the time to reach the maximum extension and the associated maximum area.

In this presentation, we will show that dynamical drivers exert stronger morphological control than the thermodynamic factors. The result reveals an overwhelming role for wind shear over a deep tropospheric layer in explaining the scale dependence of cloud shield morphology. In particular, the variability of the shield growth rate is very well explained by deep layer shear. The depth of the systems is also strongly related to dynamics and secondly to water vapor loading. These results feed the debate on the relative role of deep- vs. low-level shear in influencing deep convection.

How to cite: Fiolleau, T., Roca, R., and Netz, L.: Scale-dependence of tropical oceanic deep convective systems’ cloud shield morphology to environmental conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11683, https://doi.org/10.5194/egusphere-egu25-11683, 2025.

EGU25-12076 | ECS | Orals | AS1.10

Investigating the Future Evolution of Extreme Convective Wind Gusts Using Pseudo-Global Warming Experiments.  

Greeshma Surendran, Alejandra Isaza Uribe, Steven Sherwood, Jason Evans, Moutassem El Rafei, Andrew Dowdy, and Fei Ji

Extreme convective wind gusts (≥ 25 m/s) primarily occur when a thunderstorm downdraft sinks with high momentum to the ground level and diverges. Rising global temperatures and increased atmospheric moisture (as per the Clausius-Clapeyron relation) are expected to alter convective processes in a future climate. Atmospheric instability diagnostics (MUCAPE, DCP, K-Index, and Total-totals index) demonstrate some, but limited, skill in predicting extreme convective winds; Idealized model studies indicate that convection and severe weather will likely intensify due to higher CAPE, possibly intensifying extreme gusts. We employ a Pseudo-Global Warming (PGW) approach to investigate how an observed warm-season extreme wind gust event in New South Wales (NSW), Australia would have evolved if it occurred in a warmer climate. The event was simulated using the Weather Research and Forecasting (WRF) model run in a three-nested domain configuration ranging from 5 kilometers to 200 meters horizontal grid resolution, using initial and lateral boundary conditions from ERA-5 reanalysis. An ensemble of 13 Coupled Model Intercomparison Project Phase 6 (CMIP6) Global Climate Models (GCMs) was used to calculate the climate delta considering the SSP370 scenario, between the future (2070–2100) and historical (1984–2014) period, which is then added to the ERA-5 data to produce the PGW perturbed simulations. This presentation will explore whether the gust is indeed stronger in warmer climates, and what thermodynamic and dynamical mechanisms are at play.

How to cite: Surendran, G., Isaza Uribe, A., Sherwood, S., Evans, J., El Rafei, M., Dowdy, A., and Ji, F.: Investigating the Future Evolution of Extreme Convective Wind Gusts Using Pseudo-Global Warming Experiments. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12076, https://doi.org/10.5194/egusphere-egu25-12076, 2025.

EGU25-12161 | ECS | Posters on site | AS1.10

A Gravity Wave-Driven Toy Model to Study Convective Organization  

Ashly Wilson

The interaction between convection and geophysical flows is an open dynamic area of
research. Organized convection plays a critical role in driving extreme weather events such as
thunderstorms and tropical cyclones, with far-reaching implications for lives and livelihoods.
In this study, we present a gravity wave-driven toy model to mimic the feedback mechanisms
that evolve into convective aggregation.
Our model is based on the framework of convection-generated atmospheric oscillations.
A convective ”kick” initiates gravity waves, which subsequently interact with one another.
When these oscillations constructively interfere and reach a critical amplitude, they provide
an additional convective boost. This enhanced convection, in turn, generates new oscilla-
tions, perpetuating the feedback cycle. The interplay of these processes is proposed as a
mechanism of self-organization of tropical convection. Boussinesq equations in the absence
of Earth’s rotation are used. Convection is modeled as a triggered function (Dirac Delta).
Preliminary results suggest that the interaction between convection and atmospheric os-
cillations can give rise to a feedback mechanism that can reproduce a behavior qualitatively
similar to convective self-organization. This approach opens avenues for future investigations
into the role of gravity waves in modulating large-scale atmospheric patterns and extreme
weather phenomena.
Keywords: Convective Organization, Convectively Coupled Gravity Waves, Triggered Con-
vection

How to cite: Wilson, A.: A Gravity Wave-Driven Toy Model to Study Convective Organization , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12161, https://doi.org/10.5194/egusphere-egu25-12161, 2025.

EGU25-12394 | Posters on site | AS1.10

Observational Insights into Humidity Evolution during Cold Pool Passages 

Anja Rapmund, Marco Clemens, and Felix Ament

Cold pools are formed by convective clouds as precipitation evaporates below the cloud base, generating cool and dense air. The air descends rapidly, creating downdrafts that extend outward across the surface. These events generate gust fronts that lift ambient air and trigger secondary convection. The temperature structure of cold pools has been studied more extensively than their moisture dynamics. Simulations often suggest “moisture rings”, which are regions with increased water vapor content at the cold pool edge. However, these are rarely confirmed by observations.

To address this gap, data from the FESSTVaL (Field Experiment on Sub-mesoscale Spatio-Temporal Variability in Lindenberg) campaign, conducted during the summer of 2021, were analyzed. A dense network of surface stations was strategically positioned over an area of 30 km in diameter to provide high-resolution measurements. In total, 99 stations were deployed, including 19 Vaisala WXTs capable of measuring relative humidity every 10 seconds.

High-resolution temperature time series were used to detect the timing of more than 300 cold pool passages at individual stations. All these events were compiled into one composite using a common time axis relative to the time of the passage. This analysis of the average humidity evolution reveals that the median specific humidity is about 1 g/kg higher after a cold pool passage compared to before, indicating a post-cold-pool moisture rise. When distinguishing between stronger and weaker cold pools, weaker cold pools exhibited a short decrease in specific humidity – a “dry dip” – shortly after a cold pool passage, followed by an increase in humidity. This pattern was not observed in stronger cold pools. However, there is a large spread in humidity evolution, and individual cold pool passages might deviate significantly – even in sign – from the aforementioned patterns.

In addition, the impact of measurement uncertainty in terms of calibration and inertia of sensors will also be discussed. All these findings contribute to the upcoming VITAL II (Vertical profiling of the troposphere: Innovation, opTimization, and AppLication) campaign in 2026, which will further expand the observational basis to describe the moisture structure of cold pools.

 

How to cite: Rapmund, A., Clemens, M., and Ament, F.: Observational Insights into Humidity Evolution during Cold Pool Passages, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12394, https://doi.org/10.5194/egusphere-egu25-12394, 2025.

EGU25-12680 | ECS | Orals | AS1.10

Getting a single tropical rainbelt in a global storm-resolving model 

Hans Segura, Clara Bayley, Romain Fiévet, Helene Glöckner, Moritz Günther, Lukas Kluft, Ann-Kristin Naumann, Sebastián Ortega, Divya Sri Praturi, Marius Rixen, Hauke Schmidt, Marius Winkler, Cathy Hohenegger, and Bjorn Stevens

Resolving deep convection using a horizontal grid spacing of 10 km or finer was supposed to produce a correct representation of tropical precipitation. Global coupled or uncoupled storm-resolving simulations using the ICOsahedral Non-hydrostatic model (ICON) show a proper representation of the tropical rainbelt over land. However, the tropical rainbelt over the western Pacific shows a double structure, and the uncoupled simulation relates this bias to the lack of precipitation over the warm pool. We test three hypotheses based on an energetic framework to explain the lack of precipitation over the warm pool, 1) the radiative effect of high clouds, 2) too-frequent or efficient shallow precipitating clouds, and 3) surface heat fluxes in light near-surface winds. Experiments show that in ICON, increasing surface heat fluxes over light near-surface winds produces more precipitation over the warm pool, giving a single tropical rainbelt over the Western Pacific. An increased radiative effect of high clouds did not increase warm pool precipitation due to compensation with reduced surface heat fluxes and changes in circulation. Moreover, the representation of precipitating shallow convection does not affect warm pool precipitation. Thus, our experiments indicate the role of surface heat fluxes in light near-surface winds to trigger precipitation, as over the warm pool.

How to cite: Segura, H., Bayley, C., Fiévet, R., Glöckner, H., Günther, M., Kluft, L., Naumann, A.-K., Ortega, S., Praturi, D. S., Rixen, M., Schmidt, H., Winkler, M., Hohenegger, C., and Stevens, B.: Getting a single tropical rainbelt in a global storm-resolving model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12680, https://doi.org/10.5194/egusphere-egu25-12680, 2025.

EGU25-12737 | ECS | Posters on site | AS1.10

A method for characterizing the spatial organization of convection in deep convective systems’ cloud shield 

Louis Netz, Thomas Fiolleau, and Rémy Roca

Deep convective systems (DCSs) play a major role in the radiative budget and the water cycle over the tropics, as they are responsible for a significant part of the tropical precipitation and represents the major contributors to extreme rain rates. The spatial arrangement of deep convection within the convective system’s cloud shield exerts a strong influence on the morphology of the systems shield yet difficult to quantify objectively.

A new method is introduced that aims to evaluate this spatial arrangement of convective areas in the cloud shield. The method is based on 2D autocorrelation metrics and a stochastic approach to generate randomly organized scenes. A bootstrap technique permits to compare each scene with respect to these stochastic distributions. The technique is applied on a large satellite-based dataset and a non-supervised classification of spatial arrangement is performed. The classification reveals well separated classes corresponding to well identified organization of convection. The method is further applied onto idealized km scale simulations and is shown to hold also for the model. A comparison of the results of our approach with existing metrics will also be shown at the conference to highlight the added value of the present effort.

How to cite: Netz, L., Fiolleau, T., and Roca, R.: A method for characterizing the spatial organization of convection in deep convective systems’ cloud shield, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12737, https://doi.org/10.5194/egusphere-egu25-12737, 2025.

EGU25-13678 | ECS | Orals | AS1.10

What causes faster and slower diurnal offshore rainfall propagation in New Guinea? 

Zijian Chen, Yu Du, Claire Vincent, Ewan Short, and Hongpei Yang

Twenty-year satellite observations of rainfall have shown offshore propagation of diurnal rainfall signals in northern coastal areas of New Guinea, with propagation speed varying from 8 m s-1 to 12 m s-1 even under similar weak offshore background wind conditions. This study investigates the mechanisms behind this variability in propagation speed using the Maritime Continent Austral summer climatology v1.0 (MCASClimate), a 10-year high resolution model simulations dataset. By calculating the rainfall propagation speed on days with pronounced propagation, we classify the top 30% and bottom 30% of propagation speeds as faster and slower groups, respectively.

 

The faster group exhibits a more widespread rainfall pattern, suggesting that inertial-gravity waves driven by land-sea thermal contrast is the dominant factor. Conversely, the slower group displays more concentrated rainfall, indicating the dominance of cold pool dynamics far offshore. The faster group is associated with clearer skies, allowing more shortwave radiation to be absorbed during the daytime, which enhances land-based convection and cold pools in the evening. This results in stronger land-sea temperature contrasts, driving more intense inertial-gravity waves that govern the rainfall propagation. In contrast, the slower group is influenced by stronger low level wind shear, which leads to convection initiation primarily at the cold pool leading edges, yielding slower propagation speeds. An interesting finding of this study is that, either cold pools or inertial-gravity waves can govern rainfall propagation over distances greater than 600 km in New Guinea, albeit with different propagation speed.

How to cite: Chen, Z., Du, Y., Vincent, C., Short, E., and Yang, H.: What causes faster and slower diurnal offshore rainfall propagation in New Guinea?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13678, https://doi.org/10.5194/egusphere-egu25-13678, 2025.

EGU25-13914 | ECS | Posters on site | AS1.10

Mesoscale Convective Systems and Their Atmospheric Drivers Over South America 

Amanda Rehbein, Andreas Prein, and Tercio Ambrizzi

Understanding the atmospheric conditions that favor the development of Mesoscale Convective Systems (MCSs) is critical for improving convection-permitting models, particularly in regions with sparse observational data. This study investigates the environmental drivers of MCSs over South America using 20 years of simulations from the Weather Research and Forecasting (WRF) model version 4.1.5. These simulations, conducted within the South America Affinity Group (NSF NCAR), provide high spatial and temporal resolution, downscaling three-hourly ERA5 reanalysis data to produce 4 km and hourly outputs. By focusing on the atmospheric conditions, we aim to identify the key factors that promote MCS formation in South America. We specifically examine the role of cold pools in MCSs, investigating how they interact with surface temperature, precipitation, Convective Available Potential Energy (CAPE), Convective Inhibition (CIN), equivalent potential temperature (θe), and wind shear at varying altitudes above the surface. The results are presented for five South American regions (NWS, NSA, SAM, NES, SES) and analyzed by season, revealing significant spatial and temporal variability. This work contributes to our understanding of convection organization in the region and offers insights into improving the representation of MCSs in weather prediction models. The findings also provide valuable information to help fill observational gaps, particularly in remote or data-scarce areas of South America.

How to cite: Rehbein, A., Prein, A., and Ambrizzi, T.: Mesoscale Convective Systems and Their Atmospheric Drivers Over South America, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13914, https://doi.org/10.5194/egusphere-egu25-13914, 2025.

EGU25-15340 | ECS | Orals | AS1.10

Convective Cold Pools and Their Influence on Hurricane Intensification: A Case Study of Hurricane Helene (2024) 

Sasanka Talukdar, Alejandro Casallas, Sundararaman Gopalakrishnan, Caroline Muller, and Dev Niyogi

Convective cold pools—regions of cooled, dense air formed by evaporating rainfall—play a pivotal role in modulating atmospheric convection, yet their influence on hurricane dynamics remains insufficiently explored, especially in real-world simulations. In this study, we investigate the role of convective cold pools in the evolution of Hurricane Helene (2024) using a modified version of the Hurricane Weather Research and Forecasting model (HWRFxUT). Hurricane Helene formed in the Caribbean and intensified to become one of the deadliest hurricanes in recent history, offering a unique opportunity to study cold pool–hurricane interactions. The model setup includes nested domains at 9 km, 3 km, and 1 km resolution over the contiguous United States and employs a set of sensitivity experiments. Specifically, the rainfall evaporation rate in the Ferrier–Aligo microphysics scheme is altered by 20%, 50%, 150%, and 180% relative to a control run to assess how changes in cold pool characteristics affect the storm.

Cold pools are identified using a watershed algorithm, enabling systematic comparisons of their spatial extent and thermodynamic properties across all experiments. Analyses show that modifications to the rainfall evaporation rate significantly influence the development and distribution of cold pools in the vicinity of Hurricane Helene, with consequent impacts on storm rainfall, intensity, and track. The results underscore how changes in cold pool strength can yield marked differences in hurricane structure and evolution. These findings highlight the importance of accurately representing cold pool processes in numerical models to enhance tropical cyclone forecasts and underscore the need for continued research into this critical yet under examined aspect of hurricane physics.

How to cite: Talukdar, S., Casallas, A., Gopalakrishnan, S., Muller, C., and Niyogi, D.: Convective Cold Pools and Their Influence on Hurricane Intensification: A Case Study of Hurricane Helene (2024), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15340, https://doi.org/10.5194/egusphere-egu25-15340, 2025.

EGU25-15829 | ECS | Orals | AS1.10

The influence of convective organization on tropical free-tropospheric temperature 

Jiawei Bao, Caroline Muller, and Martin Singh

Idealised simulations under the assumption of radiative-convective equilibrium (RCE) demonstrate that the spatial aggregation of convection can significantly influence the domain-mean climate. One notable implication is the warming of the free troposphere with increased convective organisation, resulting in greater atmospheric stability. However, atmospheric temperature is also closely tied to surface temperature in regions of deep convection. The interplay between convective organisation and surface temperature in modulating free-tropospheric temperature remains unclear.

To address this question, we conduct idealised cloud-resolving simulations incorporating a diurnal cycle and prescribed sea surface temperatures (SSTs). The SST is spatially fixed with temperature gradients: a warmer ocean hotspot surrounded by cooler ocean regions. We vary the temperature of the ocean hotspot to modify the temperature gradients between the hotspot and the surrounding oceans. Additionally, we introduce an island away from the hotspot by coupling the atmosphere to a 0.05-meter deep slab ocean model. The latent heat flux calculation in the slab ocean model is rescaled by a factor of 0.1 to represent the reduced latent heat fluxes typically observed over land. The presence of temperature gradients enables continuous convection over the hotspot, whereas convection over land occurs only in the afternoon, after being heated by incoming radiation. Consequently, the model successfully simulates a diurnal cycle, characterised by enhanced precipitation over land in the late afternoon and early evening, and increased precipitation over the ocean in the early morning.

We find that daily variations in atmospheric temperature are closely related to the daily evolution of convective organisation. Additionally, enhanced temperature gradients between the hotspot and the surrounding ocean further promote convective organisation. Consequently, convection is most organised, and the free troposphere is warmest, in the simulation with the highest hotspot temperature (and the largest temperature gradients). We test the modelling results with ERA5 reanalysis data and confirm that the degree of organisation plays a crucial role in modulating the tropical free-tropospheric temperature. However, organisation appears to be primarily important for daily variations in atmospheric temperature on timescales shorter than 20 days, while surface temperature in the deep convective region becomes more significant on longer timescales (greater than 20 days).

How to cite: Bao, J., Muller, C., and Singh, M.: The influence of convective organization on tropical free-tropospheric temperature, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15829, https://doi.org/10.5194/egusphere-egu25-15829, 2025.

Turbulence in unstable atmospheres often self-organize into cellular structures. While many studies have examined their shape, size, flux characteristics, and implications for observations and boundary layer parameterization, the mechanisms driving their formation remain inadequately understood, e.g., why their horizontal dimensions are roughly one boundary layer height? This study aims to address this gap by investigating the dynamics of cellular structures in an idealized dry, surface-homogeneous free convective atmosphere boundary layers, using large eddy simulation for obtaining data. Key content include: (1) modifying subgrid parameters to simulate idealized conditions and investigating their influence on self-organized structures; (2) analyzing velocity and temperature budget within updrafts and downdrafts to identify the factors driving cellular structures and their interrelations; and (3) modeling the process by which downdrafts reach the surface, are heated, and rise as updrafts. Preliminary results suggest that the surface heating process plays a critical role in determining the horizontal shape of cellular structures. This study provides new insights into the fundamental dynamics of turbulent self-organization, potentially contributing to improved parameterizations and understanding of convective boundary layers.

How to cite: Liu, H. and Cai, X.: How is turbulence organized in the dry convective atmosphere? A study utilizing large-eddy simulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16031, https://doi.org/10.5194/egusphere-egu25-16031, 2025.

EGU25-16247 | Posters on site | AS1.10

Synoptic-Scale Forcing and its Role in a Rare Severe Rainfall Event over the UAE: A Case Study of 15–16 April 2024  

Noor AlShamsi, Ahmed Al Kaabi, Abdulla Al Mandous, Omar Al Yazeedi, Alya Al Mazrouei, Micheal Weston, Andrew VanderMerwe, Mahmoud Hussein, Esra AlNaqbi, Ahmad Al Kamali, Sufian Farah, Mahra Al Ghafli, and Brandt Maxwell

Between 15 and 16 April 2024, an intense rainfall event affected the United Arab Emirates (UAE). This study investigates the atmospheric conditions responsible for the formation of large convective storms during this period. Specifically, we analyze the atmospheric dynamics and large-scale flow that led to the development of a cut-off low-pressure (COL) system over the Arabian Peninsula on 15 April 2024, triggering a two-day period of intense precipitation over the UAE. Our findings indicate that the storms were driven by upper-air instability, a prolonged moisture influx from the monsoon system into the UAE, and the presence of a surface front. Some regions recorded over 200 mm of precipitation within this period, resulting in flash floods, infrastructure disruptions, and significant impacts on the local population. The unusual development of the rainfall event was linked to the displacement of the subtropical jet, which facilitated the formation and intensification of a COL system traversing the region.

How to cite: AlShamsi, N., Al Kaabi, A., Al Mandous, A., Al Yazeedi, O., Al Mazrouei, A., Weston, M., VanderMerwe, A., Hussein, M., AlNaqbi, E., Al Kamali, A., Farah, S., Al Ghafli, M., and Maxwell, B.: Synoptic-Scale Forcing and its Role in a Rare Severe Rainfall Event over the UAE: A Case Study of 15–16 April 2024 , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16247, https://doi.org/10.5194/egusphere-egu25-16247, 2025.

EGU25-16721 | ECS | Posters on site | AS1.10

Modeling the dynamics of Pockets of Open Cells on Marine Stratocumulus: A complexity approach 

Diana L. Monroy and Jan Haerter

More of Earth’s surface is covered by Stratocumulus clouds (Sc) than by any other cloud
type making them extremely important for Earth’s energy balance, mostly due to reflection of
solar radiation. However, representing Sc and their radiative impact is one of the largest chal-
lenges for global climate models because these cannot resolve the length scales of the processes
involve in its formation and evolution. For this reason, Sc clouds represent a large uncertainty
for climate projections [1].
The challenge becomes more intricate due to the organizational complexity that Sc clouds
present in a broad range of spatial scales. In particular, Sc fields over the oceans display
characteristic mesoscale patterns that can present both organized and unorganized structures.
Between these morphological types, cellular convection receives particular attention given than
cloud decks self-organize into honeycomb-like hexagonal patterns composed by closed and
open convective cells fields.
The purpose of this project is to model a particular tendency of Sc to organize into spatially
compact, cellular-patterned, low-reflectivity regions of open cells embedded in closed cellular
cloud fields called as pockets of open cells (POCs) [2].
First, an observational analysis of the time and spatial dynamics of POCs is made to under-
stand their creation, evolution and extinction. Then, using existing data of precipitation from
in-situ measurements on Sc clouds fields and Large eddy simulation (LES) models, a simplified
physical mechanism of the formation of POCs is proposed. Based on the previous results, an
heuristic model is developed using a statistical physics approach to capture the dynamics of
POCs and their relation with other atmospheric phenomena as cold pools and self-organized
convection.


[1] Wood, R., 2012: Stratocumulus Clouds. Mon. Wea. Rev., 140, 2373–2423,
https://doi.org/10.1175/MWR-D-11-00121.1https://doi.org/10.1175/MWR-D-11-00121.1.
[2] Stevens, B., G. Vali, K. Comstock, R. Wood, M. C. van Zanten, P. H. Austin, C. S. Brether-
ton, and D. H. Lenschow, 2005: POCKETS OF OPEN CELLS AND DRIZZLE IN MARINE
STRATOCUMULUS. Bull. Amer. Meteor. Soc., 86, 51–58, https://doi.org/10.1175/BAMS-86-1-
51https://doi.org/10.1175/BAMS-86-1-51.

How to cite: Monroy, D. L. and Haerter, J.: Modeling the dynamics of Pockets of Open Cells on Marine Stratocumulus: A complexity approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16721, https://doi.org/10.5194/egusphere-egu25-16721, 2025.

EGU25-17637 | Posters on site | AS1.10

Advancing Spaceborne Observations of Atmospheric Convection: Addressing Sampling Challenges with the WIVERN Mission 

Maryam Pourshamsi, Cathy Hohenegger, Pavlos Kollias, Alessandro Battaglia, Remy Roca, and Maximilian Maahn

Convective storms occur globally, especially over the tropical oceans, and span a wide range of scales influenced by diverse environmental factors. Advancing our understanding of convective storms requires unraveling the complex relationships between convective dynamics, microphysical processes, and environmental forcing. These critical relationships demand statistically significant observations to inform model development and enable robust verification.

Satellite observations along with reanalysis have provided a wealth of information on the relationship between the environment and the mesoscale organization of convection, however, no such comprehensive global dataset exist for convective dynamics. Key attributes of such a dataset (e.g. capturing updrafts, mass fluxes, and storm three-dimensional structure) remain undefined, particularly for exploring the relationship between convective dynamics and the near-storm environment.

In this research, we use kilometer-scale simulations from diverse tropical oceanic basins, to explore the attributes of a global convective dynamics dataset, including sampling size, sensitivity to updraft magnitude, and associated uncertainties. By under-sampling the model, we define the minimum sampling size required for a statistically significant dataset capable of mapping the relationship between updrafts and environmental conditions. The analysis will allow us to specify the sampling characteristics needed for a satellite-based observing system to provide such data globally.

Our findings support the case for the Wind Velocity Radar Nephoscope (WIVERN) mission which is one of two candidate missions currently in Phase A studies for potential selection as the Earth Explorer 11 mission under the European Space Agency’s FutureEO programme.  WIVERN proposes a conically scanning Doppler radar in polar orbit, offering a swath of approximately 800 km at a viewing angle of 42o. We demonstrate how these measurements, offered by WIVERN’s unprecedented spatiotemporal sampling, facilitate the reconstruction of vertical motions and the three-dimensional vertical distribution of ice mass in mesoscale systems. Additionally, we examine the robustness of the relationship between the convective updrafts dataset and the environment, focusing on the sensitivity to the updraft magnitude detection limit.

How to cite: Pourshamsi, M., Hohenegger, C., Kollias, P., Battaglia, A., Roca, R., and Maahn, M.: Advancing Spaceborne Observations of Atmospheric Convection: Addressing Sampling Challenges with the WIVERN Mission, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17637, https://doi.org/10.5194/egusphere-egu25-17637, 2025.

EGU25-19005 | ECS | Posters on site | AS1.10

Conceptual model of organized thunderstorm clusters under wind shear 

Lotta Bergfeld and Jan O. Haerter

Mesoscale convective systems (MCSs) are organized thunderstorm clusters which span over 100 km horizontally. They are responsible for producing the majority of rainfall in the tropics and can cause extreme precipitation events. Over the tropical ocean, MCSs can develop into tropical cyclones.

Recent work found that including a diurnal cycle -  to mimic surface temperature variations between night and day over land - enables convective self-aggregation (CSA) in idealised cloud-resolving atmospheric simulations, which means that there is a persistent spatial separation into dry patches and patches with a lot of rainfall. In simulations with a constant surface temperature – which mimic the situation over the ocean – no strong aggregation is observed (Jensen et al., JAMES, 2022).  

This study investigates the effects of wind shear in simulations with and without a diurnal cycle. Including wind shear as an imposed idealised wind profile that was derived from ERA5 data makes the simulations more realistic. Similar to the simulations without wind shear, in the case of a diurnal cycle and wind shear, self-aggregation is observed. For the constant surface temperature simulation, the aggregation stays low in comparison to the diurnal case but including wind shear increases the reached normalized spatial variance level by one order of magnitude (Kruse, University of Copenhagen, 2024).

We observe that in the simulation with wind shear and a diurnal cycle (DIU Wind), stripes with either abundant or no precipitation form along the imposed wind direction. In contrast, in the simulation with wind shear and constant surface temperature (OCEAN Wind), the clouds - less pronounced - tend to form stripes perpendicular to the wind direction which are advected by the wind.  In the DIU Wind simulation, the advection velocity of the outgoing longwave radiation at the top of the atmosphere slows down simultaneously with the formation of CSA, and converges with the wind velocity and advection velocity of the moisture field at 3500 m, indicating that the onset of CSA and the slowdown are related.  We also observe multi-day oscillations in the advection velocities in the DIU Wind simulation that will be further explored.

Our work has implications for the understanding of the organization of the convectively-driven moisture field over continent and its advection over the ocean - where it can pre-condition tropical cyclogenesis. 

How to cite: Bergfeld, L. and Haerter, J. O.: Conceptual model of organized thunderstorm clusters under wind shear, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19005, https://doi.org/10.5194/egusphere-egu25-19005, 2025.

EGU25-19398 | ECS | Posters on site | AS1.10

CIN and stable layers in the pre-convective environment 

Jake Bland, Sue Gray, Thorwald Stein, and Chris Holloway

In convection permitting models there is a bias towards earlier convection initiation, and a problem with the generation of small showers which are not seen in observations. A possible cause for this is the misrepresentation of the pre-convective environment, with insufficient convective inhibition (CIN) and stable layers in the models. To assess this systematically we compare three years of radiosonde ascents from 14 sites in and around Britain to profiles taken from the UK Met Office UM analysis and forecasts for both the global and limited area configurations. This comparison shows that larger values of CIN are underrepresented in model analyses, but that this problem is reduced in forecasts. When considering stable layers as defined by high values of the vertical gradient of virtual potential temperature it is also found that stable layers observed by radiosondes are more likely to be deeper than those identified in model profiles. These statistical results are put into context by considering the evolution of case studies from the 2023 Wessex Convection (WesCon) field campaign. For these cases a higher spatial and temporal density of radiosonde launches allows us to illustrate the impacts of the misrepresentation of atmospheric stability on the representation of convection in the model.

How to cite: Bland, J., Gray, S., Stein, T., and Holloway, C.: CIN and stable layers in the pre-convective environment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19398, https://doi.org/10.5194/egusphere-egu25-19398, 2025.

EGU25-19471 | Orals | AS1.10

The energy efficiency of tropical circulations 

Martin Singh

In 1987, Neelin & Held introduced the concept of the "gross moist stability" (GMS) to quantify how efficiently the tropical circulation transports energy. They constructed a simple model in which the spatial pattern of the GMS plays a leading role in determining the time-mean distribution of precipitation in the tropics. Since then, further work has revealed the importance of the GMS in theories of the Hadley Cell, the width of the intertropical convergence zone, and convectively coupled circulations, but a theory for the GMS itself remains elusive.

Here, I show that the atmospheric energy balance places strong constraints on the spatial distribution of the GMS, specifically, that the GMS must be uncorrelated with large-scale upward motion. This is contrary to the conventional view that convergence zones coincide with minima in the GMS. The importance of this result for convectively coupled circulations is explored using a series of convection-permitting simulations of a Mock-Walker cell in an idealised channel geometry. By varying an imposed radiative cooling profile, the vertical structure of the circulation is changed, allowing for large variations in the GMS. The results are then interpreted through a modified version of the theory of slow convectively coupled processes of Emanuel (2019).

How to cite: Singh, M.: The energy efficiency of tropical circulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19471, https://doi.org/10.5194/egusphere-egu25-19471, 2025.

EGU25-19575 | ECS | Posters on site | AS1.10

Convective mass flux and cloud anvil development in km-scale climate models 

Mathilde Ritman, William Jones, and Philip Stier

Understanding the interactions between convective processes and anvil cloud properties is increasingly important for future climate feedbacks. However, gaps remain in our understanding of how convection and convective mass flux control deep convective cloud development, and the amount and opacity of anvil cloud.

Progress has been challenged by the lack of a global-scale view of cloud convection and vertical dynamics. Until recently, cloud vertical motion was not observable by geostationary or orbiting satellites, and global climate models represented convection and clouds implicitly only through parameterisations. Now, new opportunities arise from the development of global km-scale climate models which simulate convective dynamics as part of the large scale circulation.

We seek a process-level understanding of the relationship between cloud convective mass flux and anvil cloud at regional scales using the Icosahedral Nonhydrostatic (ICON) global non-hydrostatic km-scale climate model. By tracking convective updrafts and anvil clouds in 3D at 15-minute time resolution using the tobac algorithm cloud properties can be assessed over the cloud lifetime, and simplified physical models can be used to analyse the results. We address the relationship between convective mass flux and key cloud anvil properties in the tracked clouds, as well as when, where and why these relationships vary at regional and global scales.

How to cite: Ritman, M., Jones, W., and Stier, P.: Convective mass flux and cloud anvil development in km-scale climate models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19575, https://doi.org/10.5194/egusphere-egu25-19575, 2025.

EGU25-20304 | Orals | AS1.10

Convective self-aggregation as a dual-phase damped gravity wave 

Gilles Bellon, Aurélien Ribes, Benoit Meyssignac, and Olivier Geoffroy

We propose a simple, piecewise linear model for self-aggregation based on primitive equations. In this model, each atmospheric column is in one with two possible convective regimes: deep-convective or convectively inhibited, and the thermodynamics in each regime is linearised. The model simulates aggregated and non-aggregated stationary states, reproducing many properties of self-aggregation as simulated by kilometre-resolution models, in particular an hysteresis with multiple equilibria, aggregated and non-aggregated, and a similar sensitivity to convective triggering, domain size, and boundary-layer radiative cooling in the convectively-inhibited region. These results suggest that a self-aggregated state can be considered as a gravity wave with two phases: one convective and one convectively inhibited. 

How to cite: Bellon, G., Ribes, A., Meyssignac, B., and Geoffroy, O.: Convective self-aggregation as a dual-phase damped gravity wave, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20304, https://doi.org/10.5194/egusphere-egu25-20304, 2025.

EGU25-1319 | Posters on site | AS1.11

Impacts of an upper tropospheric cold low on the extreme precipitation in Henan Province, China in July 2021 

Liangliang Li, Wenshou Tian, Jian Li, Jinlong Huang, Rui Wang, and Jiali Luo

From 19 to 21 July 2021, Henan province of China experienced an extreme precipitation event that caused massive flooding and great loss of lives. This event is thus far the second heaviest precipitation event observed by rain gauges in this region. Based on the ERA5 reanalysis data, the ECMWF operational global ensemble forecasts and numerical simulations using the ARW-WRF model, impacts of an upper tropospheric cold low (UTCL) on the extreme precipitation are examined. It is found that due to the influence of the persistent intrusion of stratospheric high potential vorticity (PV) air, a long-lived UTCL was detached from the upper level flow a week prior to the extreme precipitation event. The UTCL then moved westward, reaching the Yellow Sea and the East China Sea and maintaining there until the precipitation event ended. During this event, a broad northeast-southwest oriented area of ascending motion associated with the UTCL could be observed in front of the UTCL and strong ascending motions developed in the upper troposphere above Henan province. Analysis of the ECMWF operational global ensemble forecasts reveals that the amount of precipitation over Henan is positively correlated with the UTCL intensity. The UTCL impact on the extreme precipitation and the underlying mechanisms are further investigated based on results of numerical experiments. The control experiment reasonably reproduces the UTCL location as well as the distribution and evolution of the extreme precipitation. When the UTCL intensity is reduced in the initial condition using the piecewise PV inversion for sensitivity experiment, the upper tropospheric divergence reduces correspondingly and the dynamical ascending motion weakens in the second precipitation stage. As a result, the amount and intensity of precipitation both decrease. When the UTCL is completely removed from the initial condition, the sensitivity experiment indicates that the upper tropospheric divergence and dynamical ascending motion further weaken, resulting in a large decrease in precipitation intensity during the whole precipitation period. These findings highlight that the occurrence of the long-lived UTCL is a crucial factor that affects the intensity of the extreme precipitation event.

How to cite: Li, L., Tian, W., Li, J., Huang, J., Wang, R., and Luo, J.: Impacts of an upper tropospheric cold low on the extreme precipitation in Henan Province, China in July 2021, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1319, https://doi.org/10.5194/egusphere-egu25-1319, 2025.

EGU25-1567 | ECS | Orals | AS1.11

How does the spatial scale of surface flux variability affect MCS properties? 

Ben Maybee, Cornelia Klein, Christopher Taylor, Helen Burns, John Marsham, Douglas Parker, and Emma Barton

Understanding drivers and controls on Mesoscale Convective Systems (MCSs) is critical for predicting rainfall extremes and its impacts across time scales, from nowcasting to climate change. For MCSs over land, heterogeneity in surface fluxes across length scales presents a primary influence on storms. In West Africa, for example, MCS initiation is enhanced by ~20km scale gradients in soil moisture [1]; mature MCS cores are favoured over ~200km scale dry soil anomalies [2]; and the regional circulation responds to ~2000km scale soil moisture gradients [3], with this response explaining an observed intensification in MCSs over the last 30 years [4].

To better understand how MCSs respond to this spectrum of surface flux gradients, here we present a novel sensitivity experiment framework in which a convection-permitting Control simulation is reinitialised daily from a soil moisture field where we have modified the spectrum of surface variability using wavelet filtering. We conduct two scale experiments: one in which all sub-1000km scale soil moisture variability is suppressed; and one in which we return sub-mesoscale variability. The Control simulation is run at 1.5km over West Africa for 40 days using the Met Office Unified Model and features realistic land-surface and radiation schemes and a full suite of moisture tracers. Combining results from this simulation and outputs from 2-day long sensitivity experiments gives 200 days of CP data, enabling investigation of the impact of land-surface heterogeneity on MCSs in unprecedented detail.

We hereby elucidate the chain of mechanisms through which variability in mesoscale soil moisture anomalies propagates through surface fluxes to planetary boundary layer (PBL) fields and the regional circulation, and crucially, the effect on MCS lifecycles and intensities. We find a substantial reduction in MCSs when all sub-1000km soil moisture variability is suppressed, with numbers recovering when <100km scale variability is reintroduced. Precursor PBL fields found at MCS core locations in all experiments are consistent with those about relatively dry mesoscale soil moisture anomalies. However, the relative control of soil moisture and insolation on heat fluxes is modified in the sensitivity experiments, indicating that PBL conditions preferential for mature MCS cores are achieved via different controls and at different frequencies, affecting storm populations.

References

  • Taylor et al, Frequency of Sahelian storm initiation enhanced over mesoscale soil-moisture patterns. Nature Geoscience 4, 430-433 (2011)
  • Klein and Taylor, Dry soils can intensify mesoscale convective systems. Proceedings of the National Academy of Sciences, 202007998, (2020)
  • Cook, Generation of the African Easterly Jet and Its Role in Determining West African Precipitation, Journal of Climate 12(5), 1165–1184 (1999)
  • Taylor et al, Frequency of extreme Sahelian storms tripled since 1982 in satellite observations. Nature 544, 475-478, (2017).

How to cite: Maybee, B., Klein, C., Taylor, C., Burns, H., Marsham, J., Parker, D., and Barton, E.: How does the spatial scale of surface flux variability affect MCS properties?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1567, https://doi.org/10.5194/egusphere-egu25-1567, 2025.

EGU25-2340 | ECS | Posters on site | AS1.11

Comprehending the Attributes and Strengthening of Mesoscale Convective Systems over South Asia 

Debjit Paul and Sarvesh Kumar Dubey

Mesoscale Convective Systems (MCSs) account for over 50% of annual rainfall across the tropics and many regions of the subtropics and midlatitudes. They are often associated with strong lightning and extremely heavy rainfall, which can lead to floods. Consequently, comprehending the spatio-temporal attributes and long-term trends of MCSs is crucial for better preparedness to avoid natural hazards in current and future climatic conditions. In contrast to other MCS hotspots around the globe, investigations on the long-term alterations of MCSs in South Asia are still scarce. Our work employs high-resolution satellite brightness temperature and precipitation data, together with a novel MCS tracking method (PyFLEXTRKR), to generate a database of MCS occurrences in South Asia during the last two decades (2001-2020), and then perform a detailed analysis to understand their climatological characteristics, the environmental conditions favouring them and the long term trend. Bay of Bengal, Western Ghats, and Southern Peninsula of India are the sites where the highest number of MCSs develop. Additionally, there is a distinct seasonality in MCS activity, with the summer monsoon season seeing the highest formation of convective systems. During this season, especially over the Bay of Bengal, we observe the strong characteristics of the MCS, such as its larger area, longer duration, and greater rain rate. To a certain degree, the formation of small (<104 km2) and medium-sized (104 km2–4.4 x 104 km2) MCSs is equally dispersed between the ocean and land, whereas the large (4.4 x 104 km2–1.6 x 105 km2) MCSs form mostly across the oceans. On the other hand, the Super (> 1.6x105 km2) MCSs are exclusively found over the Bay of Bengal, primarily during the monsoon season. The percentage of rainfall contributed by MCSs over South Asia varies with the seasons, and the highest amount is received during the monsoon season. There is also a disparity over land and ocean, with land areas receiving 40%-50% and oceans receiving 55%-65% of their annual mean rainfall. Compared to the other types of convections, the MCSs contribute to the major fraction of total rainfall produced over both land and ocean, especially towards the higher magnitudes of rainfall. The ability to produce strong rainfall by any MCS strongly depends on its spatial extent (rcorr = 0.83 (0.88) over land (ocean)), followed by lifetime (rcorr = 0.48 (0.65) over land (ocean)), whereas the brightness temperature is negatively correlated weakly (rcorr = -0.24 (-0.37) over land (ocean)). The analysis of the large-scale environmental conditions reveals a gradual build-up of favorable conditions six hours before the initiation, with a noticeable increase within a 100-kilometer radius just three hours before the initiation. Our analysis shows that within the last 20 years, MCSs have increased in frequency and spatial extent. Furthermore, the precipitation associated with MCS has shown a notable upward trend. The rising frequency and severity of MCSs are propelled by increasingly conducive water vapor rich environment, which are expected to escalate with global warming. This could significantly impact the hydroclimate of South Asia, particularly the probability of severe events.

How to cite: Paul, D. and Dubey, S. K.: Comprehending the Attributes and Strengthening of Mesoscale Convective Systems over South Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2340, https://doi.org/10.5194/egusphere-egu25-2340, 2025.

The North American Monsoon (NAM) contributes the most significant amount of annual precipitation from July to September over northwestern Mexico. The increase in deep convection during the NAM is due to the emergence of extensive cumulonimbus cloud agglomerations, known as Mesoscale Convective Systems (MCSs). Previous studies suggest that upper tropospheric inverted troughs (IVs) (200 hPa), which occur over the NAM region, induce favorable environmental conditions for the development and intensification of MCSs. This talk shows the relationship of VIs with the organization of MCSs that occur over the NAM region. GOES-13 infrared satellite images (2010-2013) and the CLAUS database (1984-2008) are used to identify the trajectory of MCSs. ERA5 reanalysis data (1984–2008) characterize the atmospheric and thermodynamic conditions induced by VIs and upwellings. The results show that MCSs developed mainly in July and August, beginning to decline during September. A similar behavior is observed in the VIs, as most  of them originate from tropical upper tropospheric trough (TUTT) detachments. It is concluded that 22.8% of all MCSs formed during the study period interacted with VIs and produced more intense precipitation, unlike MCSs that did not interact. Although this percentage is small, MCSs that interacted with VIs induced more moisture to be transported to mid-atmospheric levels (500 hPa), compared to those that did not interact. Therefore, detecting these systems is essential to determine the existence of intense precipitation events over the NAM region.

How to cite: Dominguez, C.: The influence of inverted troughs on the formation of mesoscale convective systems during the North American Monsoon, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2623, https://doi.org/10.5194/egusphere-egu25-2623, 2025.

EGU25-5357 | ECS | Posters on site | AS1.11

The Influence of South China Sea Summer Monsoon Onset on Mesoscale Convective Systems in Southern China 

Wenyi Li, Riyu Lu, and Lin Wang

Mesoscale convective systems (MCSs) frequently occur over southern China during early summer, often leading to significant precipitation and associated socioeconomic impacts. This study investigates the differences in MCS frequency and related precipitation in southern China before and after the onset of the South China Sea summer monsoon (SCSSM) during 2001-2020, using high-resolution satellite data from the Global Precipitation Measurement mission and iterative rain cell tracking (IRT) method that combines cloud and precipitation criteria.

Our analysis indicates that during two pentads after the SCSSM breaks out, the frequency of MCSs significantly decreases in southern China, especially over the middle and lower reaches of Yangtze River basin (MLYRB). Accordingly, the heavy rainfall amounts decrease sharply. For instance, the number of grids with hourly precipitation between 10 and 30 mm drops by over 40% over MLYRB after the monsoon onset. It is found that the remarkable weakening of lower-level vertical wind shear and abnormal descending motion over southern China are unfavorable for the formation of MCSs. Corresponding to the SCSSM onset, on the one hand, atmosphere warms much less over the tropical oceans, including the SCS, than over the extratropical lands, resulting in smaller magnitude of meridional air temperature gradient and a subsequent decrease in vertical wind shear. On the other hand, the lower-level northerly winds induced by the SCSSM onset result in the suppressed ascent flows over southern China.

How to cite: Li, W., Lu, R., and Wang, L.: The Influence of South China Sea Summer Monsoon Onset on Mesoscale Convective Systems in Southern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5357, https://doi.org/10.5194/egusphere-egu25-5357, 2025.

EGU25-5421 | Posters on site | AS1.11

The Interaction Between Low-level Jets and Cold Pools and Their Impacts on Convection Initiation 

Yu Du, Dong Fu, and Hongpei Yang

Previous studies have investigated the optimal configuration of squall lines affected by linear vertical wind shear and cold pools, as described by the RKW theory. However, the interaction dynamics between low-level jets (LLJs) with nonlinear vertical wind shear, and cold pools remain insufficiently understood. This study utilizes idealized numerical simulations to examine the impacts of LLJs on cold pools and their subsequent role in initiating convection, focusing on the sensitivity to LLJ height and strength. The simulations reveal that, under the influence of an LLJ, a cold pool typically evolves into a two-step structure with two distinct heads, and its intensity diminishes more rapidly compared to scenarios with quasi-linear shear or no wind. Two prominent regions of vertical velocity are identified near these heads, with oneassociated with the elevated cold pool head and elevated convection initiation. Variations in parcel lifting above and below the jet core arise from differences in horizontal vorticity induced by LLJ shear, resulting in two distinct clusters of parcel trajectories. A lower or weaker LLJ leads to earlier convection initiation due to larger initial vertical velocity driven by LLJ-cold pool interactions. Convection intensity peaks when the LLJ height aligns with levels of high CAPE and when vorticity pairing above the jet core reaches its optimal state, consistent with RKW theory.

How to cite: Du, Y., Fu, D., and Yang, H.: The Interaction Between Low-level Jets and Cold Pools and Their Impacts on Convection Initiation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5421, https://doi.org/10.5194/egusphere-egu25-5421, 2025.

Secondary convective initiation (SCI) ahead of mesoscale convective systems, such as squall lines, is a globally observed phenomenon. This study employs idealized numerical simulations to investigate the spatiotemporal characteristics of SCI and its connection to squall line evolution. In a typical mid-latitude environment, SCI frequently develops ahead of the squall line, subsequently modifying squall line’s morphology and intensity through processes like merging or shifting the leading edge, depending on their relative distance.

Over an 8-hour simulation, SCI becomes increasingly frequent and exhibits periodic explosive growth (outbreaks), primarily driven by distant SCI events (≥ 5 km from the leading edge), while the number of close SCI events (< 5 km) remains stable. Distant SCIs also extend progressively farther over time, with some forming over 100 km ahead. These SCIs are more likely to occur ahead of regions with locally stronger cold pools and higher radar reflectivity within the squall line. In contrast to close SCI events governed by spatial cold pool variability, SCI outbreaks consistently lag behind recurrent surges in cold pool intensity and are closely linked to the passage of n=2 gravity waves. These waves are characterized by upward motion in the lower troposphere and downward motion aloft. Their formation is primarily driven by strong evaporative cooling and the melting of hydrometeors within the squall line, which concurrently enhances the cold pool. As each n=2 wave propagates forward, its ascent induces adiabatic cooling and enhances low-level moisture, significantly humidifying and destabilizing the lower troposphere, thereby promoting each SCI outbreak. Moreover, the repeated wave generation and long-distance wave propagation (>300 km) amplify these effects, increasing SCI frequency and expanding its reach.

How to cite: Yang, H. and Du, Y.: Cold pool and Gravity Waves Drive Secondary Convective Initiation Ahead of Squall Lines, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5461, https://doi.org/10.5194/egusphere-egu25-5461, 2025.

EGU25-5635 | Posters on site | AS1.11

Simulations of selective seeding of hailstorms over Switzerland: impacts for precipitation and lightning 

Ulrike Lohmann, Nikolaos Papaevangelou, and Manuel Brülisauer

Hailstorms can cause a lot of damage for agriculture and property. Therefore, efforts exist to mitigate hail damage by means of seeding a developing hailstorm with ice nucleating particles. Motivated by the Swiss hail mitigation campaign, we examined the impact of silver iodide (AgI) perturbations on a convective storm observed over northern Switzerland on July 6, 2019. We evaluated the effectiveness of an early seeding strategy and investigated the concept of beneficial competition, where increased number of INPs lead to the formation of smaller, less damaging hailstones. We used the Consortium for Small-Scale Modeling Regional Weather and Climate Model (COSMO) to simulate this case. AgI particles were added as a prognostic variable to the hailstorm during its cumulus stage and were released in the updraft region near the cloud base with concentrations ranging from 0.2/cm3 to 2000/cm3 in ensemble simulations. While seeding delayed the onset of precipitation, increased the graupel concentration and reduced supercooled liquid water, especially in the upper part of the convective cloud, no systematic change in the overall hail size has been found.

The lightning potential index (LPI) depends both on simultaneous occurrence of liquid water and ice species, as well as on the updraft strength. LPI increased in all seeding simulations in terms of intensity and spatial extent, because seeding increased the updraft strength and the graupel weighted ice mixing ratio.

How to cite: Lohmann, U., Papaevangelou, N., and Brülisauer, M.: Simulations of selective seeding of hailstorms over Switzerland: impacts for precipitation and lightning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5635, https://doi.org/10.5194/egusphere-egu25-5635, 2025.

EGU25-5857 | ECS | Orals | AS1.11

Controls on the convective environment in the Lake Victoria region and their interactions with large-scale climate variability 

Eliza Karlowska, Andrew G. Turner, and Steven Woolnough

The Lake Victoria region is inhabited by over 40 million people and is a major source of food, water and economic activity in East Africa. As the intertropical convergence zone passes by, this region experiences two rainy seasons that result in extreme precipitation events and flash flooding. Over 80% of extreme rainfall around Lake Victoria is produced by mesoscale convective systems (MCSs), which are characterised by organised convection spanning a few hundred kilometres, and often lasting several hours. Here, we tracked 4,811 MCSs between 2014 and 2019 that moved over Lake Victoria and lasted longer than 3 hours. A clustering algorithm was applied to identify different types of MCSs crossing this region: cross-lake storms that initiate overnight East Africa time, lake-to-land storms that initiate in the morning, and land-to-lake storms that initiate in the afternoon. We examined conditions of the local environment leading to the development of these storms to link them to larger scale climate variability, such as the Madden-Julian Oscillation (MJO). The MJO is an eastward-propagating envelope of suppressed and enhanced convection that originates over the western Indian Ocean. Active MJO convection over the western Indian Ocean (MJO phase 2) creates favourable zonal wind anomalies for the formation of lake-to-land and land-to-lake storms. In addition, MJO phase 2 is also likely to influence specific humidity and temperature anomalies prior to and during the formation of land-to-lake storms. Conditions over the Lake Victoria region during days when no storms occur are similar to the conditions created during active MJO phase 6, i.e., when active MJO convection is over the Maritime Continent. Our analysis is used to inform a machine learning model that will predict the probability of a given storm type occurring over this region in order to improve predictions of high-impact weather over the lake.

How to cite: Karlowska, E., Turner, A. G., and Woolnough, S.: Controls on the convective environment in the Lake Victoria region and their interactions with large-scale climate variability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5857, https://doi.org/10.5194/egusphere-egu25-5857, 2025.

EGU25-7625 | ECS | Posters on site | AS1.11

Analysis on the Causes and Forecast Deviation of Rainstorm on the Eastern Foot of Qinling Mountains 

Xiao Yiqing, Li Ming, and Ma Yongyong

Doppler radar, FY-4B satellite data, wind profile radar, ERA-5 reanalysis data, automatic weather station and other multi-source observation data are used to analyze the causes and forecast deviation of a rainstorm on the eastern foot of Qinling mountains in Shaanxi province of China on 19th July 2024, and the results indicated that the rainstorm had strong suddenness, locality and convection. The main water vapor and energy for the rainstorm were provided by the southwest low-level jet at 700 hPa, and the strengthening of the jet stream and the decrease in the height of the jet stream core had a good correlation with the occurrence of heavy precipitation. The mesoscale convective system(MCS) causing rainstorm was formed by the the merging and strengthening of locally generated cold clouds in the convergence and upward movement zone of 700 hPa jet stream front and mesoscale convective clouds moving from southwest to east. And the convective system continued to develop along the mountain direction, forming a "train effect" that strengthens local heavy rainfall. Topography played an important role in this rainstorm.  On the one hand, the Qinling Mountains block the low-level jet stream at 700hPa, causing water vapor to strongly accumulate on the windward slope and converge and rise. On the other hand, the Qinling Mountains produced a significant topographic uplift movement on the ground and southerly winds at 850 hPa, thereby strengthening precipitation together. The 24-hour precipitation forecast was significantly missed by several numerical models because of deviation of 700 hPa jet location and intensity, but the CMA-BJ model had good prediction on the falling area and intensity of heavy rainfall for 3 h. Conducting analysis of similar rainstorm events, summarizing the deviation characteristics of the numerical models, considering the triggering and maintenance mechanisms of convection, and the important role of terrain would help improve the forecasting and early warning capabilities of such rainstorm.

 

How to cite: Yiqing, X., Ming, L., and Yongyong, M.: Analysis on the Causes and Forecast Deviation of Rainstorm on the Eastern Foot of Qinling Mountains, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7625, https://doi.org/10.5194/egusphere-egu25-7625, 2025.

Using a convection initiation (CI) identification method designed for isolated convection, 11,646 CI events (CIEs) were identified based on composite reflectivity (CR) in the middle reaches of the Yangtze River Basin from May to September of 2016–2020. CIEs occur more frequently in July and August (62.7%) and from 11 BJT to 16 BJT (62.2%) with a diurnal peak at 12 BJT. CI area (area of the connected region with CR  40 dBZ at CI time) has a diurnal peak at 16 BJT, which is related to the frequent occurrence of large-area CIEs (LACIEs, 1%) with a CI area larger than 62 km². Most LACIEs occur under stronger atmospheric instability and higher vertical wind shear with the rapid intensification and expansion of convective regions after CI. Regions with high-frequency CIEs correspond well with mountain terrains. Mountain CIEs, which are under the weak unstable stratification and low vertical wind shear, occur about twice (5,831) as frequently as foothill or plain CIEs. Compared to other terrains, the local heterogeneity of soil moisture (SM) near CI locations is the strongest over the mountains. Mountain CIEs occur at the center of a high SM region located in the transition zone between the positive and negative SM gradients, with the highest SM gradient magnitude located to the north side of CI locations.

How to cite: Wei, Q., Sun, J., Zhang, Y., and Zheng, L.: Statistical Characteristics of Convection Initiation over Different Terrains in the Middle Reaches of the Yangtze River Basin Based on the Doppler Weather Radar Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7928, https://doi.org/10.5194/egusphere-egu25-7928, 2025.

EGU25-9414 | Orals | AS1.11

Grid Spacing Sensitivity of Simulated Convective Drafts in Tropical and Mid-Latitude Mesoscale Convective Systems 

Andreas F. Prein, Die Wang, Ming Ge, Alexandra Ramos Valle, and Manda Chasteen

Organized deep convection plays a critical role in the global water cycle and drives extreme precipitation events in tropical and mid-latitude regions. However, simulating deep convection remains challenging for modern weather forecasts and climate models due to the complex interactions of processes from microscales to mesoscales. Recent models with kilometer-scale (km-scale) horizontal grid spacings (∆x) offer notable improvements in simulating deep convection compared to coarser-resolution models. Still, deficiencies in representing key physical processes, such as entrainment, lead to systematic biases. Additionally, evaluating model outputs using process-oriented observational data remains difficult. In this study, we present an ensemble of MCS simulations with ∆x spanning the deep convective grey zone (∆x from 12 km to 125 m) in the Southern Great Plains of the U.S. and the Amazon Basin. Comparing these simulations with Atmospheric Radiation Measurement (ARM) wind profiler observations, we find greater ∆x sensitivity in the Amazon Basin compared to the Great Plains. Convective drafts converge structurally at sub-kilometer scales, but some discrepancies, such as too-deep up- and down-drafts and too-weak peak downdrafts in both regions or too-strong updrafts in Amazo- nian storms remain. Overall, we observe higher ∆x sensitivity in the tropics, including an artificial buildup in vertical velocities at five times the ∆x, suggesting a need for ∆x≤250 m. Nevertheless, bulk convergence – agreement of storm average statistics – is achievable with km-scale simulations within a ±10 % error margin, with ∆x=1 km providing a good balance between accuracy and computational cost.

How to cite: Prein, A. F., Wang, D., Ge, M., Ramos Valle, A., and Chasteen, M.: Grid Spacing Sensitivity of Simulated Convective Drafts in Tropical and Mid-Latitude Mesoscale Convective Systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9414, https://doi.org/10.5194/egusphere-egu25-9414, 2025.

Mesoscale convective systems (MCSs), as major contributors to extreme precipitation events, have garnered significant attention in the context of global warming. In 2020, vast areas of East Asia—downstream of the Tibetan Plateau (TP) and home to over 30% of the global population—experienced an anomalously wet rainy season, marked by intense MCS-induced precipitation that resulted in severe socio-economic impacts and extensive losses.

This study leverages the first ensemble run of kilometer-scale (~4 km) WRF simulations for the Water Year 2020 (WY2020) under the CORDEX-FPS-CPTP framework. The performance of these simulations in representing MCS precipitation characteristics has been assessed using the GPM-IMERG precipitation product and the CMA Multi-Source Merged Precipitation Analysis (CMPA).

The results demonstrate that while all ensemble members can generally capture the spatial distribution of MCS precipitation downstream of the TP, notable differences arise among the simulations with single-physics perturbations. Specifically, simulations using the Morrison and WSM5 microphysics schemes exhibit strong agreement with observations. In contrast, simulations employing the SBU_YLin or WDM6 microphysics schemes significantly underestimate MCS precipitation in the region. Regarding planetary boundary layer (PBL) scheme sensitivity, simulations utilizing the YSU and Shin-Hong schemes outperform those employing the MYNN3 scheme.

Despite these variations, a common bias emerges across all seven kilometer-scale WRF simulations: they collectively underestimate the rainfall area of MCSs by 30.9% to 43.0%, while simultaneously overestimating precipitation intensity of MCSs by 59.4% to 64.1%. These results suggest a consistent tendency for K-scale WRF simulated MCS precipitation to exhibit smaller spatial extents yet greater magnitudes compared to observations.

To explore potential improvements, we expanded the model domain from [15.0°N–50.0°N; 65.0°E–125.0°E] to [5.0°N–55.0°N; 45.0°E–160.0°E; almost doubled] and conducted additional WY2020 simulations. Preliminary results indicate that the expanded domain not only enhances the model’s ability to capture heavy MCS rainfall centers during Mei-yu season, particularly over the Western North Pacific Ocean (south to Japan), but also better reproduces MCS precipitation features than other K-scale WRF runs. Remarkably, the expanded domain simulation even outperforms the GPM data in representing MCS precipitation over the middle and lower reaches of the Yangtze River basin in eastern China, compared to CMPA.

The K-scale WY2020 ensemble run represents a valuable resource for advancing our understanding of the K-scale model uncertainties on MCS and the hydrological cycle over the TP and its downstream regions.

How to cite: Li, P.: Simulating Mesoscale Convective Systems Downstream of the Tibetan Plateau at Kilometer-Scale: Insights from the First Ensemble Run of ‘WY2020’ in CORDEX-FPS-CPTP, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9830, https://doi.org/10.5194/egusphere-egu25-9830, 2025.

EGU25-10450 | ECS | Orals | AS1.11

Mesoscale convective systems over South America: Representation in km-scale climate simulations and future change 

Harriet Gilmour, Robin Chadwick, Jennifer Catto, Kate Halladay, and Neil Hart

South America is highly vulnerable to storms and extreme precipitation. Mesoscale Convective Systems (MCSs), a prevalent storm type in tropical and subtropical South America, can be particularly damaging due to the organised, deep convection that fuels heavy precipitation over wide areas. Future warming will likely bring changes to MCS characteristics and precipitation extremes across the region. However, the relatively coarse spatial resolution of current regional climate models fails to explicitly resolve convective processes, making future changes to MCSs uncertain. Here, the representation of modelled MCSs is investigated in decade-long convection-permitting climate simulations over South America run by the UK Met Office. Changes to MCSs under global warming are then assessed using a future climate simulation. Simulated MCSs are tracked using a cloud tracking algorithm (tobac) and compared with those in satellite observations for seasonality, storm characteristics and regional differences. The simulations perform well at capturing the observed MCS climatology, including spatial frequency and seasonal cycle. However, the simulations overestimate MCS frequency over the Amazon Basin by a factor of 2 and underestimate MCS frequency over the La Plata Basin, likely due to a weak bias in the simulated South American Low-Level Jet.  In general, regional variations in MCS characteristics are also well simulated, but precipitation-related characteristics show larger model-observed differences. Simulated MCSs overestimate precipitation intensity and underestimate precipitation area. This results in an underestimation of the MCS contribution to total rainfall of 20-30% in the model, particularly in subtropical South America. The results from this work suggest that MCSs are generally well-captured by the CPM and have been used to inform results for future changes to MCSs over South America under climate change.

How to cite: Gilmour, H., Chadwick, R., Catto, J., Halladay, K., and Hart, N.: Mesoscale convective systems over South America: Representation in km-scale climate simulations and future change, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10450, https://doi.org/10.5194/egusphere-egu25-10450, 2025.

EGU25-11230 | Orals | AS1.11

Quasi-Linear Convective Systems and Derechos across Europe: Climatology, Accompanying Hazards, and Societal Impacts 

Artur Surowiecki, Natalia Pilguj, Mateusz Taszarek, Krzysztof Piasecki, Tomáš Púčik, and Harold Brooks

In this work, we use 8 years (2014–2021) of Operational Programme for the Exchange of Weather Radar Information (OPERA) radar data, lightning detection network (ATDnet) data, and severe weather reports to create a climatology of quasi-linear convective systems (QLCSs) in Europe. In the first step, 15-min OPERA radar scans were used to identify 1475 QLCS cases. The manual investigation of each individual led to the recognition of QLCS morphological and precipitation archetypes, areal extent, width, length, duration, speed, forward motion, accompanying hazards, injuries, and fatalities. Severe weather reports, lightning data, and morphological properties were used to classify QLCSs according to their intensity into 1151 marginal (78.0%), 272 moderate (18.5%), and 52 derecho (3.5%) events. Spatio-temporal analysis indicate that QLCSs are the most frequent during summer in Central Europe, while in southern part of Europe their occurrence is extended to late autumn. A bow echo morphological archetype occurred in around 29% of QLCS cases, while a mesoscale convective vortex occurred in almost 9%. Among precipitation modes, trailing and embedded stratiform types accounted for around 50% of QLCSs. Based on ESWD Database we found that the most frequent QLCS-related hazard was lightning (taking up on average 94.4% of the area impacted by QLCS), followed by severe wind gusts (7.9%), excessive precipitation (6.1%), large hail (2.9%), and tornadoes (0.5%). Derechos had the largest coverage of severe wind reports (49.8%), while back-building QLCSs were mostly associated with excessive precipitation events (13.5%). QLCSs caused 104 fatalities and 886 injuries. Nearly half of all fatalities and injuries were associated with only the 10 most impactful QLCS events, mostly warm-season derechos producing severe to extreme widespread wind gusts.

How to cite: Surowiecki, A., Pilguj, N., Taszarek, M., Piasecki, K., Púčik, T., and Brooks, H.: Quasi-Linear Convective Systems and Derechos across Europe: Climatology, Accompanying Hazards, and Societal Impacts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11230, https://doi.org/10.5194/egusphere-egu25-11230, 2025.

EGU25-13858 | Orals | AS1.11

Global projections of hail hazard frequency under climate change 

Timothy Raupach, Raphael Portmann, Christian Siderius, and Steven Sherwood

Hail can injure people and damage infrastructure, with hailstorms a driving cause of insured losses. Hailstorms are expected to be affected by global warming, primarily via changes to atmospheric instability, wind shear, and the height of the melting level. However, the nuances of expected changes remain uncertain and are generally only studied regionally, partly because global climate models typically lack the fine grid spacing required to explicitly resolve hailstorms. Here, we show global projections using an ensemble of four hail proxies to estimate hail-prone conditions occurrence frequency in eight global climate models. We use a temperature-based framework and show projected changes in global hail hazard frequency in scenarios with two and three degrees of warming over a recent historical period. By analysing changes in the "ingredients" for the proxies we can determine which factors are most pertinent to the changes in hail-prone conditions. Under global warming, the multi-model multi-proxy results show general poleward shifts in hail-prone condition frequency, and shifts from the warm season to the cool season in many regions. The results reinforce the benefit of using proxies designed specifically for hail for such studies, since some more general thunderstorm proxies neglect the effects of temperature and can show significantly different results. Finally, we use our results to analyse changes in hail exposure to various crops worldwide. This work encompasses the first global projections for severe storms using proxies specifically designed for hailstorms.

How to cite: Raupach, T., Portmann, R., Siderius, C., and Sherwood, S.: Global projections of hail hazard frequency under climate change, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13858, https://doi.org/10.5194/egusphere-egu25-13858, 2025.

EGU25-15921 | Posters on site | AS1.11

A case study of hailstorm dynamics during mountain ridge crossing 

Kateřina Skripniková and Zbyněk Sokol

Data from lightning detection sensors and dual-polarized weather radars are used for high-resolution analysis of hailstorms developing around the Ore Mountains ridge. Measured radar and lightning parameters provide information on storm dynamics and are indicative of severe hailfall occurrence. Our case study deals with a multicellular hailstorm that developed during a summer afternoon near the ridge of the Ore Mountains from Germany to Czechia.

On 27 June 2022, hailstorms formed on both the windward and leeward sides of the Ore Mountains ridge. The multicellular storm evolved in warm air ahead a warm front advancing to the east. Severe hail was reported in many places, with hailstones up to 5 cm in diameter. And high lightning activity was detected.

Both radar and lightning detection data were used to study the hailstorm evolution thoroughly. Lightning data from the ENTLN network provide lightning activity parameters from the entire area of interest. Radar data from the Czech weather service C-band radar network are covering the area of interest as well. Data from the X-band radar situated on the Milesovka hill are used in the radar range, which is 30 km from the Milesovka observatory. This measurement does not cover the entire study area of the storms, but provides more detailed information, also due to the frequent RHI scanning in the scanning strategy.

How to cite: Skripniková, K. and Sokol, Z.: A case study of hailstorm dynamics during mountain ridge crossing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15921, https://doi.org/10.5194/egusphere-egu25-15921, 2025.

EGU25-16917 | ECS | Posters on site | AS1.11

Comparison of future hail trends across Europe based on the HAILCAST diagnostic and hail proxies 

Iris Thurnherr, Lena Wilhelm, Ruoyi Cui, Monika Feldmann, Sandro Beer, Christoph Schär, and Heini Wernli

Thunderstorm-related severe weather, particularly hail, causes extensive damage to life and infrastructure across Europe. However, the effect of a warmer climate on the occurrence of hail is still not fully understood. To date, most projections of hail occurrence under future climate scenarios have relied on hail proxies derived from global and regional climate models that use parameterized representations of convection. Recently, convection-permitting regional climate simulations with a high computational resolution of 2 km, using the COSMO model with the online hail diagnostic HAILCAST, have provided new insights. The simulations revealed spatially contrasting changes in hail frequency under a 3°C global warming scenario, showing a substantial decrease in summer hail frequency in southwestern Europe and an even larger increase in central and eastern Europe. In this study, we leverage these high-resolution model outputs to assess future projections of hail occurrence. Specifically, we compare differences in hail day frequencies between a warmer future climate and the present day climate as derived from (i) traditional hail proxies using environmental variables (e.g. CAPE and wind shear) and (ii) the HAILCAST online diagnostic. Through this comparison, we aim to better understand two key questions: (1) how accurately hail proxies capture the spatial and temporal patterns of hail occurrence in comparison to HAILCAST, and (2) whether the relationship between environmental variables and hail occurrence remains stationary under changing climatic conditions.

How to cite: Thurnherr, I., Wilhelm, L., Cui, R., Feldmann, M., Beer, S., Schär, C., and Wernli, H.: Comparison of future hail trends across Europe based on the HAILCAST diagnostic and hail proxies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16917, https://doi.org/10.5194/egusphere-egu25-16917, 2025.

EGU25-17755 | Posters on site | AS1.11

A Local Terrain Smoothing Approach for Stabilizing Microscale and High-Resolution Mesoscale Simulations: Application to FastEddy® and WRF 

Juan Pedro Montávez, Eloisa Raluy-López, Domingo Muñoz-Esparza, and Jeremy Sauer

High-resolution simulations, both at mesoscale and microscale, have become increasingly prevalent, often leveraging high-resolution terrain datasets. However, terrain-following coordinate models can encounter numerical instabilities in regions where terrain slopes exceed critical thresholds, generally around 35º. To address this issue, terrain smoothing is typically required. Current approaches usually involve applying global smoothing methods across the entire domain, which inevitably results in a loss of terrain detail and resolution to prevent numerical instabilities in regions where it is not necessary. Moreover, as the model resolution increases, the number of grid points with steep slopes grows, underscoring the need for alternative terrain smoothing strategies.

This study presents the development and implementation of a local terrain smoothing approach designed to mitigate numerical instabilities in a mesoscale model (the WRF model) and a microscale model (NCAR-RAL’s GPU-accelerated FastEddy® LES model). Various smoothing techniques were evaluated, including both simultaneous and sequential approaches. Following a thorough performance analysis—considering the number of iterations required for convergence, computational cost, and, most importantly, the degree of terrain distortion—the most effective method was selected and implemented. The final approach applies a Gaussian filter (σ = 25) over a 3x3 grid centered on each steep-slope point, with a blending factor of 0.2 at the edges. This ensures that the central point is smoothed while the surrounding points retain 80% of their original terrain characteristics. Each steep slope is addressed individually but processed simultaneously across iterations. A higher blending factor results in greater terrain distortion, while a lower blending factor significantly increases computational time, often preventing convergence within the imposed iteration limit.

This terrain smoothing method has been fully implemented in FastEddy® and is now used operationally and routinely within the model. This implementation will be made publicly available in the next release of FastEddy®, hosted on GitHub (https:// github.com/NCAR/FastEddy-model, starting with version 3.0). For WRF, the method has been integrated as an additional step in the WPS workflow, following the execution of the geogrid program. The proposed local smoothing approach helps preventing the occurrence of CFL errors in high-resolution simulations over complex terrain without relying on excessively high values of the time off-centering parameter (epssm) to dampen vertically propagating sound waves, which can lead to excessive high-frequency damping, negatively impacting the accuracy of the simulations.

In conclusion, this study presents a simple yet effective method for avoiding terrain-driven numerical instabilities in high-resolution simulations, ensuring the maximal preservation of terrain resolution in both microscale and mesoscale models. This approach can be easily applied to other models, offering a straightforward solution to enhance numerical stability while maintaining high-resolution terrain features in diverse simulation environments.

Acknowledgements: The authors acknowledge the ECCE project (PID2020-115693RB-I00) of the Ministerio de Ciencia e Innovación/Agencia Estatal de Investigación (MCIN/AEI/10.13039/501100011033). ERL thanks her predoctoral contract FPU (FPU21/02464) to the Ministerio de Universidades of Spain.

How to cite: Montávez, J. P., Raluy-López, E., Muñoz-Esparza, D., and Sauer, J.: A Local Terrain Smoothing Approach for Stabilizing Microscale and High-Resolution Mesoscale Simulations: Application to FastEddy® and WRF, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17755, https://doi.org/10.5194/egusphere-egu25-17755, 2025.

EGU25-18567 | ECS | Posters on site | AS1.11

Spatio-temporal aggregation of convective cell clusters in European MCSs 

Nicolas Da Silva, Diana Monroy, Ashly Wilson, and Jan Haerter

Mesoscale Convective Systems (MCSs) are organized collections of thunderstorms that typically consist of narrow, intense regions of convective precipitation alongside broader, lighter areas of stratiform precipitation. These systems are the primary contributors to extreme precipitation events across Europe (Da Silva & Haerter, 2023). While both convective and stratiform precipitation rates are expected to increase with temperature according to thermodynamic expectations (the Clausius-Clapeyron relationship), their statistical superposition may intensify at an even faster rate due to increased proportion of convective-type precipitation within MCSs under warmer conditions (Da Silva & Haerter, 2025, accepted).

Both the intensity and proportion of convective-type precipitation in MCSs play a critical role in determining flood risks, but the spatial and temporal organization of convection is equally significant for shaping the characteristics and severity of flooding. Larger, long-lived clusters of convection within MCSs are indeed more likely to trigger severe flooding compared to smaller, isolated clusters.

In this study, we analyze the spatio-temporal characteristics of convective clusters within MCSs. MCSs are identified and tracked using both radar precipitation data (RADOLAN radar; Bartels et al., 2004) and lightning records from the EUropean Cooperation for LIghtning Detection (EUCLID; Schulz et al., 2016) network over Germany. Convective-type precipitation is classified based on its proximity to lightning strikes. To explore links between these clusters and local environmental conditions, we incorporate data from German Weather Service (Deutscher Wetterdienst, DWD) weather stations and the ERA5 reanalysis dataset (Hersbach et al., 2020).

We measure the spatial clustering of convection within MCSs using two novel spatial organization indices that quantify deviations from random distributions. Our preliminary findings suggest that convective clusters within MCSs become wider at higher temperatures, consistent with observations of larger CAPE (Convective Available Potential Energy) environments. Additionally, we observe a geographic trend in the location of convective clusters: they are more frequently concentrated in the southern portions of MCSs. However, under warmer conditions, a larger fraction of MCSs exhibit convective clusters on their northern edges. We hypothesize that this shift is driven by stronger convective instability ahead of the northern flanks of MCSs at higher temperatures. This effect may be linked to increased near-surface baroclinicity and horizontal temperature gradients at warmer temperatures.

The temporal evolution of these convective clusters is further analyzed through the framework of directed percolation, a statistical physics approach that allows us to investigate the growth and connectivity of convective cells over time. Through this lens, we aim to better understand the lifecycle of convective clusters within MCSs, including their formation, propagation, and eventual dissipation. By combining spatial and temporal analyses, this study provides critical insights into how environmental conditions influence the organization of convection within MCSs, thereby advancing our ability to predict and mitigate flood risks in a warming climate.

How to cite: Da Silva, N., Monroy, D., Wilson, A., and Haerter, J.: Spatio-temporal aggregation of convective cell clusters in European MCSs, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18567, https://doi.org/10.5194/egusphere-egu25-18567, 2025.

EGU25-20189 | Posters on site | AS1.11

Effects on urbanization on a WRF-simulated heavy precipitation over the Maceió city 

Maria Cristina Lemos da Silva, Helber Gomes, Matheus José Arruda Lyra, Dirceu Herdies, Fabricio Daniel dos Santos Silva, Heliofábio Barros Gomes, and Hakki Baltaci

Land use in the city of Maceió is rapidly changing from its natural state to accommodate a growing population and tourism. These changes include increased urbanization. There has been a significant increase in the frequency and intensity of extreme events occurring in recent years in the Northeast region of Brazil (NEB), especially in its metropolitan areas. It is believed that this may be associated with the exacerbated land use (LU) in these areas. Therefore, the objective of this work is to evaluate how an intense simulation event using the WRF model would be affected if the size of the Maceió metropolitan region were increased. Furthermore, the study will investigate the effects that the LU has on the intensity of this extreme event and its structure. To achieve this, the land use around the metropolitan region of Maceió was changed to a slightly larger urban area in the input files and then re-executed under the same parameters. Control and experimental simulation were compared using vertical profiles, flow fields and instability indices. The heavy rains that occurred on March 17, 2020 over Maceió were caused by an intense confluence of air at low levels (1000 hPa) observed on the state's coast in the early hours of the day. This conference occurred due to a small low pressure center that was present near the coast of Bahia, which could also be observed in the Sea Level Pressure field. The Convective Available Potential Energy (CAPE) field also indicated intense instability over the region, with values above 1000 J/Kg after 16 UTC over a large part of the north/east sector of Alagoas. Skew T Log-P thermodynamic profiles demonstrated high levels of instability throughout the 17th, gaining more strength between 16-21 UTC, with a maximum CAPE of 1864 J/Kg at 18 UTC. Throughboth simulations, it was reported that in the LU experiment there was an increase in the intensity and spatial distribution of the occurrence over the city of Maceió, as well as being associated with an increase in instability. Impacts were also identified on sensible and latent heat fluxes, and vertical shear. These results, despite being initial, show that there is a sensitivity in the use of land in convection and, consequently, in the intensity of learning.

How to cite: Silva, M. C. L. D., Gomes, H., Lyra, M. J. A., Herdies, D., Silva, F. D. D. S., Gomes, H. B., and Baltaci, H.: Effects on urbanization on a WRF-simulated heavy precipitation over the Maceió city, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20189, https://doi.org/10.5194/egusphere-egu25-20189, 2025.

EGU25-3571 | ECS | Orals | AS1.13

Cloud-circulation coupling in convection-permitting simulations 

Anna Mackie, Michael P. Byrne, and Chris J. Short

Understanding of cloud-circulation coupling in a warming world is underpinned by global climate models (GCMs) with coarse horizontal resolutions necessitating the use of convective parameterizations. Global convection-permitting models are now emerging, but their high computational cost is a barrier to their use for studies of climate change. 

Here, we present results from 2-year atmosphere-only, limited domain simulations at a horizontal resolution of ~4.5km over a region of the west Pacific using the Met Office Unified Model. The limited-area model is driven at the lateral boundaries by an existing ~25km global model. Two simulations are analysed: a control run with present-day SSTs and a perturbed run with a prescribed SST warming of approximately 4K. 

There are substantial differences in cloud-circulation coupling between the high-resolution simulations and the global driving model. In particular, we find – on average – large cloud radiative effects (CREs) associated with strongly subsiding gridpoints, in comparison to the relatively small CREs for this circulation regime as expected from previous GCM studies and indeed in the global driving model. We demonstrate that this systematic difference in subsiding CRE between models arises from the existence of complex circulation structures in the high-resolution simulations, which are absent in the global simulations. For the highest (>80%) percentiles of column relative humidity, subsiding gridpoints have O(5 Wm-2) weaker cooling compared to ascending gridpoints with similar column relative humidity. We discuss how this strong subsidence regime responds to warming, and potential implications for cloud feedbacks.

How to cite: Mackie, A., Byrne, M. P., and Short, C. J.: Cloud-circulation coupling in convection-permitting simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3571, https://doi.org/10.5194/egusphere-egu25-3571, 2025.

EGU25-4547 | Orals | AS1.13

Sensitivity of Warm Rain Rates to Lower PBL Structure as Observed by Synthetic Aperture Radar over the Subtropical Ocean 

Ryan Eastman, Justin Stopa, Ralph Foster, Doug Vandemark, and Hauke Schulz

Synthetic Aperture Radar (SAR) is capable of detecting wind and rain signatures at a 5-meter resolution on the ocean surface without interference from overlying cloud cover. Here, wind signatures represent the spatial distributions of capillary waves produced by gusts and lulls in the surface winds. These distinct wind signatures vary based on the 3-dimensional structure of the lower boundary layer and fall into two dominant categories: mesoscale convective (MC), and wind streaks (WS). MC boundary layers tend to be associated with gentler motions and lighter winds while WS are associated with stronger overturning “rolls” and heavier winds. SAR can detect rain columns as drops disturb the ocean surface and can also discern cold pools and atmospheric boundaries associated with precipitation. A machine learning routine has been developed to classify SAR images based on these signatures.

 

SAR images classified as MC, WS, or containing boundaries or rain columns are compared to a variety of satellite cloud data in order to independently verify the classification system, and to gain insight into whether these classified PBL states have an effect on cloud and precipitation processes. Randomly spaced and located SAR images taken only at sunrise and sunset during the year 2018 are linked to polar orbiting A-Train satellite observations. Observations are linked by using Lagrangian PBL trajectories, following the cloud-level winds forward and backward from the SAR image to the 1:30 and 13:30 A-Train observation times. This “brackets” the SAR image with satellite data observed 12-hours apart, or in the case of daytime-only data, 24-hours apart. Comparisons are made in four marine subtropical stratocumulus regions.

 

Results show that SAR-observed rain columns and cold pools are associated with higher rain rates as seen by AMSR/2 89 GHz rain rate estimates tuned by CloudSat. PBLs with wind streaks are associated with stronger rain rates and greater cloud liquid water path compared with mesoscale convective PBLs, even after controlling for wind speed. Further analysis shows that WS PBLs tend to be cloudier, shallower, and contain fewer cloud drops. This work highlights the importance of small-scale turbulent boundary layer processes in controlling cloud processes on sub-daily timescales, and motivates investment in future SAR observations over the ocean.

How to cite: Eastman, R., Stopa, J., Foster, R., Vandemark, D., and Schulz, H.: Sensitivity of Warm Rain Rates to Lower PBL Structure as Observed by Synthetic Aperture Radar over the Subtropical Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4547, https://doi.org/10.5194/egusphere-egu25-4547, 2025.

EGU25-5370 | Orals | AS1.13

Ship-borne radar observations of organized convection during the ORCESTRA/PICCOLO field campaign 

Allison Wing, Michael Bell, James Ruppert, Sarah Kennison, Wei-Ting Hsiao, Delián Colón-Burgos, Daniel Klocke, Chaehyeon Chelsea Nam, and Morgan O'Neill

The ORganized Convection and Earthcare Studies over the TRopical Atlantic (ORCESTRA) field campaign occurred in the tropical Atlantic in August and September 2024. ORCESTRA is an international initiative that combined eight different sub-campaigns utilizing seven different ship, aircraft, ground-based, and satellite platforms. Here we focus on preliminary results from PICCOLO (Process Investigation of Clouds and Convective Organization over the atLantic Ocean), the NSF-funded sub-campaign that deployed the CSU SEA-POL radar on the RV Meteor in coordination with the BOWTIE ship campaign to study the nature, governing mechanisms, and impact of mesoscale convective organization within the Atlantic ITCZ. SEA-POL is a ship-stabilized scanning C-band radar that measures dual-polarization and provides advanced retrievals of precipitation and its spatial pattern. PICCOLO has four objectives: (1) evaluate process relationships between precipitation, humidity, and organization; (2) use advanced polarimetric radar retrievals to investigate microphysical, dynamical, and radiative characteristics of convection; (3) investigate the importance of radiative processes in driving mesoscale organization; and (4) use novel observational approaches to compute the entropy budget to advance understanding of the impacts of convection on climate. 

The 40-day cruise primarily sampled within the moist tropics and observed a wide variety of convective states. There was a significant longitudinal contrast, in which conditions east of 40W were rainier and moister with cooler sea surface temperatures, stronger surface winds, and stronger vertical wind shear than areas west of 40W. We use the SEA-POL retrievals to examine the variability of convective structures within the ITCZ including variability in the prevalence of congestus versus deep convection. We also present initial classifications of the spatial organization of convection, its variability, and its influence on precipitation amount and intensity.

How to cite: Wing, A., Bell, M., Ruppert, J., Kennison, S., Hsiao, W.-T., Colón-Burgos, D., Klocke, D., Nam, C. C., and O'Neill, M.: Ship-borne radar observations of organized convection during the ORCESTRA/PICCOLO field campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5370, https://doi.org/10.5194/egusphere-egu25-5370, 2025.

EGU25-6335 | ECS | Posters on site | AS1.13

First insights into the diverse remote sensing observations of convection during BOW-TIE 

Anna Trosits, Andreas Foth, and Heike Kalesse-Los

Convection, which influences cloud and precipitation properties as well as, the radiative effects of clouds, needs to be better understood for a comprehensive picture of interconnected climate processes all over the globe and requires a better representation for accurate climate projections. Meanwhile, the modelling of these phenomena is already a challenge itself, the quality and quantity of high-resolution observational data of convective clouds are limited, especially over the (tropical) oceans. The recent measurement campaign BOW-TIE (“Beobachtung von Ozean und Wolken – das Trans ITCZ Experiment”) on board the research vessel Meteor in August and September 2024 focussed on atmospheric and oceanic measurements inside the Atlantic ITCZ (intertropical convergence zone), between Mindelo (Cabo Verde) and Bridgetown (Barbados). Our working group from the Leipzig Institute for Meteorology concentrated on the investigation of the microphysical properties of clouds and precipitation by deploying a continuously measuring remote sensing suite mainly consisting of a motion-stabilized, vertically-pointing 94 GHz cloud radar and a microwave radiometer (MWR; to derive liquid water path (LWP) and integrated water vapor (IWV)) on the research vessel. In combination with data obtained with the ceilometer deployed by the MPI for Meteorology Hamburg, the synergetic Cloudnet processing chain can be employed. Cloudnet products include a hydrometeor target classification as well as cloud microphysical properties like the effective radius of cloud droplets and ice crystals, the hydrometeors phase, ice water content (IWC), and liquid water content (LWC). All observed and derived cloud and precipitation characteristics are contrasted between the Eastern and Western Atlantic. A first insight reveals the dominance of shallow convective clouds in the Eastern Atlantic, while the Western Atlantic also evinces convective clouds with a height up to six kilometers and cirrus clouds more frequently. Related to the frequency of occurrence of the different cumulus cloud types, the distribution of the microphysical properties like the effective radius of hydrometeors, IWC, and LWC allows for a more detailed glimpse into differences of the processes in the Eastern and Western ITCZ. With that, the convective processes above the tropical Atlantic Ocean are studied concerning microphysics and their distribution and contribute to an improved understanding of cloud-affecting processes.

How to cite: Trosits, A., Foth, A., and Kalesse-Los, H.: First insights into the diverse remote sensing observations of convection during BOW-TIE, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6335, https://doi.org/10.5194/egusphere-egu25-6335, 2025.

EGU25-7132 | ECS | Posters on site | AS1.13

Interaction between cloud-radiative effects and convective systems measured during the ORCESTRA field campaign in Aug-Sep 2024 

Wei-Ting Hsiao, Allison Wing, Sarah Kennison, Michael Bell, and James Ruppert

As convective aggregation has been found to be supported by radiative heating in idealized simulations, this study seeks to answer whether such a property of convection exists in the observed convective organization. Data was collected during the ORCESTRA field campaign over the tropical Atlantic in August and September 2024. Cloud properties, precipitation, atmospheric radiative fluxes, and the derived degree of convective organization are measured by the Sea-Pol radar and other instruments on a shipborne platform (RV Meteor) supported by sub-campaigns including PICCOLO and BOW-TIE. We analyze how atmospheric radiative effects support the spatial organization of tropical deep convection, and also inversely, how the convective organization affects the strength of convective-radiative feedback. In particular, the strength of convective-radiative feedback is assessed by the temporal covariance between atmospheric radiative heatings and either moist static energy tendency or precipitation rate. We will show the observed dependency of convective-radiative feedback on the occurrence of various convective organization phenomena, including mesoscale convective organization and the passage of tropical waves. The effect of radiative heating and its induced circulation on the state of convective organization during the field campaign will also be derived from mechanism-denial numerical simulations.

How to cite: Hsiao, W.-T., Wing, A., Kennison, S., Bell, M., and Ruppert, J.: Interaction between cloud-radiative effects and convective systems measured during the ORCESTRA field campaign in Aug-Sep 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7132, https://doi.org/10.5194/egusphere-egu25-7132, 2025.

EGU25-7235 | Posters on site | AS1.13

Mesoscale controls on trade-wind inversion structure and cloudiness during EUREC4A 

Raphaela Vogel and Martin Janssens

Two thirds of variability in cloud cover in the trade-wind regions is associated with cloudiness near the top of the cloud layer, which mostly occurs in the form of stratiform layers. Stratiform inversion cloud is also the cloud component that changes most across different patterns of cloud organization and potentially also under climate change. Unfortunately, our understanding of the factors controlling the occurrence and lifetime of stratiform layers and how they link to the structure of the trade inversion is limited. Because the trade inversion can be as thin as 10-100m, even high-resolution large-eddy simulations have serious issues in accurately representing the sharpness of the inversion and its associated cloudiness. The EUREC4A field campaign released >850 dropsondes from the HALO aircraft upstream Barbados in January-February 2020 in 200 km diameter circles, constituting a sounding dataset which lends itself particularly well to investigate the structure and variability of the trade inversion. Here we use the dropsonde data in conjunction with lidar-retrieved cloud-top height distributions and high resolution large-eddy simulations (the cloud botany ensemble) to investigate controls on inversion strength and height, document their variability at different scales, and assess their connection with cloudiness.    

How to cite: Vogel, R. and Janssens, M.: Mesoscale controls on trade-wind inversion structure and cloudiness during EUREC4A, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7235, https://doi.org/10.5194/egusphere-egu25-7235, 2025.

EGU25-9024 | ECS | Orals | AS1.13

Rain Evaporation Below Shallow Tropical Trade-Wind Cumuli as Predicted by a New Super-Droplet Model 

Nils Niebaum, Clara Bayley, Mampi Sarkar, Ann Kristin Naumann, and Raphaela Vogel

How much rain evaporation occurs below shallow cumuli is a crucial determinant of the organisation of such clouds, yet both modelling studies and observations which can robustly quantify the amount of evaporation are in short supply. In this study we combine observations of a diverse population of precipitating cumuli from the EUREC4A field campaign with a simple 1-D rain-shaft model, in order to predict the amount of rain evaporation in the sub-cloud layer and the relative influence on it of microphysical vs environmental controls. The rain-shaft uses superdroplet model microphysics so that our analysis benefits from its detailed and yet comprehensible depiction of the droplet size distribution and microphysical processes involved. Surprisingly, we find that evaporated fractions are usually low, below 20%, and that collisional processes between droplets have a very minor influence on rain evaporation, meanwhile dominant roles are played by the droplet size distribution at cloud base and the sub-cloud layer relative humidity profile. The evaporated mass fraction can vary substantially between clouds and even when clouds’ liquid water contents are comparable, evaporated fraction can be upto 50% larger because of small differences to mean cloud droplet radius. These results stress the importance or accurately measuring/modelling droplet size distributions rather than microphysical processes in order to study rain evaporation. We find too that the vertical profile of evaporation rate is above all controlled by the vertical relative humidity profile, which suggests the sub-cloud layer could be highly sensitive to the feedback between evaporation and relative humidity.

How to cite: Niebaum, N., Bayley, C., Sarkar, M., Naumann, A. K., and Vogel, R.: Rain Evaporation Below Shallow Tropical Trade-Wind Cumuli as Predicted by a New Super-Droplet Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9024, https://doi.org/10.5194/egusphere-egu25-9024, 2025.

EGU25-13564 | ECS | Posters on site | AS1.13

Examining Downstream Impacts of Mesoscale Sea Surface Temperature Anomalies on Trade Cumulus Clouds in Satellite Observations 

Xuanyu Chen, Isabel McCoy, Ryan Eastman, Martin Janssens, Hauke Schulz, Geet George, and Juliana Dias

Trade-wind cumuli play a key role in the earth’s radiative budget and are at the heart of the longstanding uncertainty in climate sensitivity estimates. Understanding the mesoscale spatial organization (20 to 2000 km) of trade cumuli is at the forefront of addressing this uncertainty. Recent observations have shown that trade cumulus cloudiness is locally modulated by the weak yet ubiquitous sea surface temperature anomalies (SSTAs) over O(10-100) km in the Northwest Tropical Atlantic trade wind region. Specifically, the daily cloud fraction is increased above daily warm SSTAs. We hypothesize that the associated condensation heating anomalies can trigger convective aggregation downwind of warm SSTAs through an inherent convective instability for nonprecipitating shallow cumulus shown in Janssens et al. 2023. To test this hypothesis, we employ a Lagrangian framework where trade cumulus trajectories are estimated using ERA5 wind fields at 925 hPa. These Lagrangian cloud trajectories are initiated over the daily centroids of warm and cold mesoscale SST anomalies identified from the NOAA GOES-POES blended SST analysis at different local times. Cloud properties and cloud organization metrics are obtained and computed from the NASA SatCORPS CERES GEO Edition 4 GOES-16 Northern Hemisphere V1.2 product. Our preliminary composite analysis on ~400 Lagrangian trajectories passing warm and cold SSTAs, respectively, in the EUREC4A/ATOMIC region suggests that there is likely a downstream response in trade cumulus cloud fraction within 6 hours (~170 km) after an air parcel passes through a warm or cold SSTA. For trajectories initiated over the daily centers of SSTAs at 1:30am LT, we found that cloud fraction reduces after experiencing warm SSTAs and increases after experiencing cold SSTAs, similar to stratocumulus cloud responses to large-scale SST perturbations. The outcome of this study will help clarify the role of mesoscale air-sea interaction in trade cumulus cloud organization.

How to cite: Chen, X., McCoy, I., Eastman, R., Janssens, M., Schulz, H., George, G., and Dias, J.: Examining Downstream Impacts of Mesoscale Sea Surface Temperature Anomalies on Trade Cumulus Clouds in Satellite Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13564, https://doi.org/10.5194/egusphere-egu25-13564, 2025.

EGU25-13654 | Orals | AS1.13

The active role of stratiform and anvil clouds through longwave radiative feedback 

James Ruppert, Emily Luschen, Rosimar Rios-Berrios, Shun-Nan Wu, and Yunji Zhang

Our emphasis on distinct tropical convective cloud modes has evolved over the decades in step with advancements in our understanding of tropical convection, its governing dynamics, and its role in large-scale weather and climate. While an early undilute plume view of tropical convection emphasized the role of latent heating from deep cumulonimbi in tropical ascending motion, a later emphasis on shallow to congestus clouds came with our improved grasp of water vapor’s essential role as governor to convective cloud development and organization. Here I discuss the unique role of stratiform and anvil clouds in this context, which play a surprisingly active role in the mesoscale organization of deep convection. While stratiform and anvil clouds are the biproducts of deep convection, consuming remnant buoyancy from their parent cumulonimbi, their much larger spatial and temporal footprints cause radiative forcing that fosters the upscale growth of moist convection and its coupling with the larger-scale environment. These clouds are therefore uniquely capable of coupling convection with the larger scale owing to their very long inherent lifecycles, compared to the fundamental scales of deep convection. In this presentation, I first motivate these arguments through consideration of scales. I next present the results from numerical model experiments and observations of tropical convection supporting the argument that longwave forcing by stratiform and anvil clouds actively promote convective upscale development and intensification. This forcing acts by reducing downdraft mass flux in stratiform regions, which in turn yields more upward motion per unit precipitation in the overall convective system. This constitutes a destabilization of the moist convective system, fostering its intensification, compared to if cloud–radiative forcing was absent. The results of this study imply that stratiform and anvil clouds and their radiative forcing are essential elements to any realistic conceptual model of tropical moist convection, and hence, to the tropical hydrologic cycle.

How to cite: Ruppert, J., Luschen, E., Rios-Berrios, R., Wu, S.-N., and Zhang, Y.: The active role of stratiform and anvil clouds through longwave radiative feedback, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13654, https://doi.org/10.5194/egusphere-egu25-13654, 2025.

We analyze the CERES solar radiative balance trends of the past 23 years, with the objective to separate the contribution to the solar absorption trends of shifts in the atmospheric general circulation and changes in cloud controlling processes. Regimes of large cloud cover and strong cloud radiative cooling are defined in the low latitude and the high latitude zones, representing the tropical rainy zone and the midlatitude storm zones respectively, and the trends in the areal coverage of those regimes over the past 23 years are examined along with the trends in the cloud solar radiative effect within each regime. This allows the decomposition of the global solar cloud radiative trends into circulation induced changes and those induced by cloud controlling processes. The results show that the general circulation component of the cloud solar radiative changes, which manifests itself as a contraction of the midlatitude storm zones and the tropical rainy zone, is the largest term in the solar absorption trend, causing decreased sunlight reflection of 0.37 W/m2 per decade. We explore the relationship between the cloud regime contraction and the main atmospheric circulation indices, including the width of the Hadley circulation and the location of the midlatitude jet, in order to understand the processes responsible for the cloud regime changes.

How to cite: Tselioudis, G. and Kelly, J.:  Contraction of the world’s storm-cloud zones and the relationship to atmospheric circulation changes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13780, https://doi.org/10.5194/egusphere-egu25-13780, 2025.

EGU25-14463 | Orals | AS1.13

Understanding drivers of local lower tropospheric stability 

Maria Rugenstein and Senne Van Loon

The radiative effect of shallow clouds, especially in the subtropical ocean upwelling regions, is very efficient and mostly controlled by local sea surface temperatures and the lower tropospheric inversion strength. The latter caused the radiative feedback of shallow clouds to switch from positive to negative over the last couple of decades and likely controls cloud feedbacks in the future. Drivers of lower tropospheric inversion strength are not well understood theoretically and vary strongly between reanalyses. We employ convolutional neural networks and explainable artificial intelligence to create maps of drivers of lower tropospheric inversion strength in the subtropical ocean upwelling regions. We quantify the relative relevance of local and remote surface temperatures and find that the edges of regions of deep convection matter much more than their center. The West Pacific Warm Pool is much less and the subtropical Atlantic more relevant than expected. Our results quantify how the theories of tropospheric weak temperature gradient and the convection circus tent play out for setting local free tropospheric temperatures and the local tropospheric inversion stength. Currently, our method is based on large ensemble climate model simulations and the results are robust across models. Applying this framework to observations, it might be possible to constrain the spread of this cloud controlling factor across reanalyses and constrain its future evolution, hence improving projections of the radiative effect of shallow clouds.

How to cite: Rugenstein, M. and Van Loon, S.: Understanding drivers of local lower tropospheric stability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14463, https://doi.org/10.5194/egusphere-egu25-14463, 2025.

EGU25-16165 | Posters on site | AS1.13

BOWTIE: A ship-based field campaign to explore the inner life of the Atlantic ITCZ 

Daniel Klocke, Allison Wing, Marcus Dengler, Hans Segura, Geet Georges, Louise Nuijens, Micheal Bell, Heike Kalesse-Los, James Ruppert, and Hauke Schmidt

The BOWTIE ship-based field experiment explored the influence of convective storm processes and their oceanic interactions on the Atlantic Inter-Tropical Convergence Zone (ITCZ) in August and September 2024. This research is driven by evidence suggesting that storm-scale dynamics is pivotal for shaping the broader structure of the ITCZ and its connection to global circulation patterns and energy transport. Utilizing the German research vessel METEOR, the expedition involved extensive sampling within the ITCZ from its Northern to Southern edge - while transiting the tropical Atlantic from East to West - with detailed atmospheric and oceanic vertical profiling. The research focuses on obtaining vertically resolved cross-sections of the ITCZ and its surrounding conditions, with an emphasis on the atmosphere-ocean boundary layers. Key measurements include precipitation, cloud and humidity profiles, wind, sea-surface temperature, as well as physical and biogeochemical upper ocean characteristics with state-of-the-art instrumentation. BOWTIE is embedded within the international initiative ORCESTRA that combines eight different sub-campaigns. During BOWTIE the research vessel METEOR also served as a platform for two additional subcampaigns of ORCESTRA, which contributed UAVs (STRINQS) and a dual-polarization C-band radar (CSU’s SEA-POL, through PICCOLO) to the ship’s instrumentation. We will present an overview of BOWTIE and first results from the comprehensive measurments.

How to cite: Klocke, D., Wing, A., Dengler, M., Segura, H., Georges, G., Nuijens, L., Bell, M., Kalesse-Los, H., Ruppert, J., and Schmidt, H.: BOWTIE: A ship-based field campaign to explore the inner life of the Atlantic ITCZ, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16165, https://doi.org/10.5194/egusphere-egu25-16165, 2025.

EGU25-16875 | Posters on site | AS1.13

Track ‘n’ Type: Do tracked clouds show a realistic behavior with respect to cloud type? 

Matthias Tesche, Felix Müller, and Torsten Seelig

The temporal development of cloud properties along the trajectory of a tracked clouds can show a behavior that is clearly unrealistic. For instance, a low-level cloud that is partly obscured by faint high-level clouds above can show development of cloud-top temperature with jumps of 40 K or more. To assess the general development of clouds tracked over central Europe, we have applied the ISCCP cloud classification to those clouds. It is found that the majority of the tracked clouds shows transitions between time steps that are either between identical cloud types (e.g. cumulus to cumulus) or represent reasonable development (e.g. stratus to stratocumulus or vice versa). The additional consideration of objective weather types enables an assessment of the large-scale conditions under which different cloud types are most abundant.

How to cite: Tesche, M., Müller, F., and Seelig, T.: Track ‘n’ Type: Do tracked clouds show a realistic behavior with respect to cloud type?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16875, https://doi.org/10.5194/egusphere-egu25-16875, 2025.

EGU25-17353 | ECS | Posters on site | AS1.13

Tracking Clouds: Assessing the representation of mesoscale cloud patterns in the EUREC4A model data 

Felix Müller, Torsten Seelig, Hauke Schulz, Diego Villanueva, and Matthias Tesche

We compare satellite data from the EUREC4A campaign (observed by the Advanced Baseline Image onboard the GOES-16 satellite) and model output from ICON-LEM tailored for the EUREC4A campaign [1]. All datasets are located east of Barbados in the Caribbean Sea. We build on previous cloud tracking analyses for the GOES satellite dataset [2].

We use a cloud tracking algorithm [2] to find lifetime and cloud size distributions. The trajectories can be classified into the four mesoscale cloud patterns “sugar” to “fish” based on C3ONTEXT data which makes it possible to investigate how well these patterns are represented in the model data. We compare the distributions of cloud sizes, lifetimes and the average development of cloud size over the cloud’s lifetimes.

Cloud modelling is a very important tool for climate research. However, it is not an easy task to validate model data and assess a model’s performance. The cloud tracking enables us to provide a unique quality assessment of the model data. Lifetime information is interesting because it encompasses multiple dynamic scales from micro to planetary regimes, while cloud size and cloud cover are important factors for the radiative properties of the clouds in a region and characterise the clouds’ general behavior.

 

[1] Schulz, Hauke & Stevens, Bjorn (2023) “Evaluating Large-Domain, Hecto-Meter, Large-Eddy Simulations of Trade-Wind Clouds Using EUREC4A Data” in Journal of Advances in Modeling Earth Systems, doi: 10.1029/2023MS003648

[2] Seelig et al. (2023) “Do optically denser trade-wind cumuli live longer?”, in Geophysical Research Letters, doi: 10.1029/2023GL103339

How to cite: Müller, F., Seelig, T., Schulz, H., Villanueva, D., and Tesche, M.: Tracking Clouds: Assessing the representation of mesoscale cloud patterns in the EUREC4A model data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17353, https://doi.org/10.5194/egusphere-egu25-17353, 2025.

EGU25-17730 | ECS | Posters on site | AS1.13

Boundary-layer measurements of the ITCZ with meteorological quadcopters off a trans-Atlantic ship expedition 

Geet George, Robert Mackenzie, Owen O'Driscoll, Daniel Klocke, Louise Nuijens, Pier Siebesma, and Team Menapia

STRINQS stands for Soundings and TuRbulent eddy measurements in the ITCZ with a Network of QuadcopterS and is one of the sub-campaigns under the umbrella of ORCESTRA, an international collaboration of measurement campaigns with the larger goal of understanding mesoscale organization of convection in the tropical Atlantic. STRINQS made measurements of the ITCZ boundary layer by employing four meteorological quadcopters, designed and developed by Menapia. Co-ordinated flights were conducted with the German research vessel Meteor as base, a part of the BOWTIE subcampaign in ORCESTRA. The quadcopters, designed to sustain performance in heavy rain and strong wind, provide high-resolution atmospheric soundings of temperature, humidity, pressure, and winds while allowing for high flight ceilings. There are two sets of meteorological sensors in each quadcopter, with a sampling frequency of 10 Hz. Additionally, a sonic anemometer configured on a 1 m arm above the quadcopter body helps provide wind measurements without disturbances due to the wake of the propellers during non-descending trajectories. The team had to initially overcome multiple logistical and technical challenges, unfortunately including mishaps. However eventually, between the period of 30th August and 9th September, the team successfully conducted around 45 vertical profiles reaching altitudes of up to 1500 m (the permitted flight ceiling for STRINQS) in addition to flying horizontal hexagonal patterns that traversed distances between 2 and 4 km horizontally. Some flights recorded intriguing case-studies such as profiling the boundary-layer thrice in a span of 40 minutes as an organized squall-line rain event passed over the ship, thus providing contrasting conditions before, during and after the storm. The meteorological sensors' data show promising results in the drone's capability to sample the boundary layer, but some corrections still need to be made to the retrieval of wind measurements, particularly vertical wind, which is known to be a challenging measurement from UAV (uncrewed aerial vehicle) platforms. Post data-processing and preliminary analyses, the data will be made publicly available in state of the art data formats. Although STRINQS only partially achieved its scientific goal of statistical sampling, the learnings on the measurement capabilities of such methods have been significant. With this demonstration of using a ship as a launchpad for coordinated flights of heavyduty quadcopters even in heavy rain events, STRINQS signals the possibilities of such strategies in future campaigns to provide a rich spatial characterization of the boundary layer.

How to cite: George, G., Mackenzie, R., O'Driscoll, O., Klocke, D., Nuijens, L., Siebesma, P., and Menapia, T.: Boundary-layer measurements of the ITCZ with meteorological quadcopters off a trans-Atlantic ship expedition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17730, https://doi.org/10.5194/egusphere-egu25-17730, 2025.

EGU25-18395 | Orals | AS1.13 | Highlight

Revisiting the Doldrums: New Insights from the ORCESTRA Campaign 

Julia Windmiller, Romain Fiévet, Helene Glöckner, and Bjorn Stevens

The Intertropical Convergence Zone (ITCZ) is a central component of the atmospheric general circulation and is traditionally described as a region of mean surface convergence and high precipitation rates. The ITCZ is also associated with the doldrums, regions of low wind speeds and variable wind directions, although the exact relationship between the two remains unclear. Reexamining this relationship, we show that the doldrums are largely confined to the area between the edges of the ITCZ, which are characterised by enhanced surface convergence. Although this is a region of high time-averaged precipitation, low wind speed events only occur in the absence of precipitation. This suggests that the traditional explanation of the doldrums being the result of ascending air motion is incorrect. We therefore investigate the vertical structure of the doldrums using data collected during the ORCESTRA (Organized Convection and EarthCARE Studies over the Tropical Atlantic) field campaign. ORCESTRA took place in the tropical Atlantic in August and September 2024 and consisted of eight sub-campaigns. Here, we focus on the sampling of vertical air motion that we measured with dropsondes in the deep tropics in general and in the doldrums in particular. In combination with limited-area simulations that provide daily hindcasts of atmospheric conditions in the campaign region, we use these data to characterise for the first time the vertical structure of vertical air motion within regions of low wind speeds. This study can also be seen as an example of a more fundamental goal of the ORCESTRA campaign, which is to gain a better understanding of the mesoscale structure of the ITCZ and the importance of its significant day-to-day variability.

How to cite: Windmiller, J., Fiévet, R., Glöckner, H., and Stevens, B.: Revisiting the Doldrums: New Insights from the ORCESTRA Campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18395, https://doi.org/10.5194/egusphere-egu25-18395, 2025.

Clouds and convection play a key role in structuring atmospheric circulation and in determining the climate sensitivity. However, it is still not understood how clouds and convection will respond to warming of the atmosphere. This is due to an insufficient representation of clouds and moist convection in climate models. A better understanding of the coupling between water vapor, convection, cloud formation and circulation is needed. Shallow marine convection shows the largest frequency of occurrence amongst clouds. But besides being uniform clouds of similar structure, they can occur in different larger scale patterns of organization. The trade wind region is characterized by a complex structure of water vapor, aerosols and clouds. Depending on the season and larger scale circulation, it was found, that lofted layers of water vapor and aerosols can have a quite significant impact on the atmospheric stability, and with that on cloud structure and evolution.

Airborne lidar measurements with the combined water vapor differential absorption and high spectral resolution lidar system WALES provide simultaneous measurements of the water vapor mixing ratio and of aerosol properties. The WALES instrument was deployed in a series of airborne experiments aiming to better understand the coupling of clouds and convection over the sub-tropical and tropical Atlantic Ocean. The first campaign of this series, the NARVAL experiment, was conducted in wintertime out of Barbados. It was followed by the NARVAL-II experiment in August 2016, the EUREC4A experiment in January/February 2020 and the PERCUSION campaign in August and September 2024. The latter especially focused on the transition of shallow to deep convection and the ITCZ. Another add on of this campaign was the contrasting measurements over the east and west Atlantic Ocean. We used these measurements to investigate how the complex structure of water vapor and aerosol impact the stability of the atmosphere and with that the evolution and structure of clouds. We found that the impact is different, if the water vapor and aerosol are within distinct layers. During summertime, when they are well separated from the marine boundary layer, the radiative effect of the layers dominates. The evolution of shallow marine clouds below the SAL is suppressed. In wintertime, the e.g. dust is transported at lower altitudes and the dust layer is frequently mixed into the marine boundary layer. During this time of the year the effect of the layer on the evolution and lifetime of marine trade wind convection is much more complex, as the dust particles within the SAL might additionally act as cloud or ice nuclei.

In our presentation we will give an overview of the performed measurements and the radiative transfer calculations that were performed based on our findings. Those calculations together with the observations better help to understand the impact of lofted layers on cloud evolution and structure.

How to cite: Gross, S., Gutleben, M., Wirth, M., and Ewald, F.: Impact of elevated water vapor and aerosol layers on the stability of the sub-tropical atmosphere and the structure and evolution of shallow marine clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18408, https://doi.org/10.5194/egusphere-egu25-18408, 2025.

EGU25-18477 | ECS | Orals | AS1.13

How does the cloud fraction response to aerosol change over the diurnal cycle? 

Geoffrey Pugsley, Edward Gryspeerdt, and Vishnu Nair

Stratocumulus clouds play an important role in the Earth’s energy balance due to their widespread spatial coverage and radiative properties. However, the impact of aerosol on stratocumulus cloud fraction (CF) remains poorly constrained resulting in large uncertainties for the effective radiative forcing due to aerosol cloud interactions (ERFaci). Stratocumuli undergo a strong diurnal cycle driven by variations in cloud top radiative cooling, which alters the processes sustaining the cloud. Despite this, many previous observational studies have only considered the state of the cloud field during the daytime due to the availability of satellite data.

In this work we use a Lagrangian tracking method, combined with geostationary satellite data, to investigate the CF response to aerosol over the entire
diurnal cycle. Strong variations in the cloud response to aerosol are found with the diurnal cycle. This brings satellite-based studies into closer alignment with ground- and insitu-based measurement campaigns, emphasising the importance of nighttime cloud processes for understanding aerosol cloud interactions and constraining the ERFaci.

How to cite: Pugsley, G., Gryspeerdt, E., and Nair, V.: How does the cloud fraction response to aerosol change over the diurnal cycle?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18477, https://doi.org/10.5194/egusphere-egu25-18477, 2025.

Tropical anvil clouds have significant impacts on the atmosphere due to their cloud radiative effect (CRE), and their response to warming remains one of the largest uncertainties in future climate projections. Recent research has highlighted both the importance of changes in anvil cloud structure and changes in convective mass flux in a warmer climate to CRE feedbacks. However, understanding of these processes is limited due to a lack of observations linking convective processes to anvil cloud properties across their entire lifetimes. We apply the tobac-flow algorithm to a year of Meteosat SEVIRI observations over Africa and the tropical Atlantic to detect and track convective cores and their subsequent anvil clouds to investigate the impact of convective dynamics on anvil clouds. By combining this cloud tracking dataset with retrieved cloud properties and broadband fluxes, changes in the intensity and organisation of convection can be linked to changes in anvil CRE. Overall, both more intense and more organised convection tends to result in anvils with positive CRE, as these storms produce higher, colder anvil clouds and, over land, anvils that exist for longer at night. However, when controlling for the anvil temperature and time of day, more intense convection tends to result in positive CRE, while more organised convection results in a negative CRE. We attribute these differences to changes in anvil structure, as we observe that more organised convection tends to produce thicker anvils, while more intense convection results in thinner anvils. The contrasting effects of different convective processes on anvil CRE highlight the importance of understanding the mechanisms through which convective dynamics affect anvil structure, and indicate that different changes in convective processes may lead to regional differences in anvil cloud feedbacks.

How to cite: Jones, W. and Stier, P.: Contrasting effects of convective intensity and organisation on anvil cloud radiative effect observed using cloud tracking, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19918, https://doi.org/10.5194/egusphere-egu25-19918, 2025.

EGU25-20029 | ECS | Orals | AS1.13

Shallow convection modulation of wind stress patterns in marine atmospheric boundary layer 

Edoardo Foschi, Louise Nuijens, Paco Lopez-Dekker, and Owen O'Driscoll

Shallow convection and precipitation in the marine atmospheric boundary layer can modulate near-surface winds on scales from 100 m - 100 km. This may substantially influence the exchange of heat and momentum across the air-sea interface and turbulent mixing on either side of the interface. Here we analyze spatial patterns of near-surface wind and momentum flux down to a 100 m scale as a function of Richardson number and as a function of the development in moist precipitating convection in many large-domain large eddy simulations (DALES) as part of the BOTANY ensemble. To assess the modulation effect that convection has on surface momentum fluxes, we decompose the LES wind stress across the simulations into contributions from different scales and processes, and answer how these dependencies change as simulations develop deeper moist convection and consequently precipitation. At the ocean surface, DALES currently uses a rough-wall boundary condition with a bulk flux formulation that relates surface fluxes to resolved-scale variables at the first grid level, consistent with Monin-Obukhov similarity theory. Knowing that the representation of wind stress in LES is likely flawed, we reflect on the largest uncertainties given the model assumptions and how observations from space and from the recent ORCESTRA/BOWTIE campaigns can help validate and improve the formulation of wind stress. 

How to cite: Foschi, E., Nuijens, L., Lopez-Dekker, P., and O'Driscoll, O.: Shallow convection modulation of wind stress patterns in marine atmospheric boundary layer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20029, https://doi.org/10.5194/egusphere-egu25-20029, 2025.

EGU25-20399 | ECS | Posters on site | AS1.13

Development of a surface wind retrieval by analysing sunglint geometry from specMACS radiance measurements 

Anja Stallmach, Anna Weber, and Bernhard Mayer

Near-surface winds are a key component for the coupling of the atmosphere- ocean system. Convergence and divergence patterns can be inferred from measurements of the surface wind vector, enabling the characterization of meso- and synoptic-scale atmospheric dynamics. Observations over remote areas, such as the Atlantic ocean, are mostly limited to satellites and buoys. Geostationary satellites derive wind data primarily from cloud tracking and thus do not measure surface winds. In contrast, polar-orbiting satellites can provide surface wind data predominantly using active remote sensing instruments, such as scatterometers, wind-lidars or synthetic aperture radars, providing better spatial but certainly lower temporal resolution. Finally, buoy measurements are point-observations and cannot be employed for large-scale wind field analyses. This work aims to explore an alternative approach for quantifying surface wind fields over the ocean by analysing high-spatial resolution imagery from airborne observations.


Measurements of specularly reflected solar radiation (sunglint) by the hyperspectral and polarized imager specMACS aboard the German research aircraft HALO are employed for the development of a surface wind retrieval. Size and shape of the sunglint are predetermined by wind speed and direction: With ocean surface roughness directly corresponding to near-surface wind speed, the specMACS retrieval makes use of the relationship between ocean wave slope distribution and angular variation of sunglint radiance. SpecMACS measurements of spectral radiances are evaluated against simulated spectral radiances for different solar zenith and azimuth angles, as well as surface wind speeds and directions. The radiative transfer simulations are done with the Monte Carlo (MYSTIC) solver of the libRadtran radiative transfer package.


The overarching goal of this work is the development of an operational surface wind retrieval after analysing selected cases as an initial step. The retrieval requires a view of the ocean surface from the aircraft. We aim to explore to what extent the wind retrieval can be employed for (a) partially cloud-covered scenes or (b) scenes with an optically thin cirrus layer above or below the aircraft. A first application will be the analysis of data acquired during the recent ’Persistent EarthCare underflight studies of the ITCZ and organized convection’ (PERCUSION) sub-campaign in the tropical Atlantic. Research concerned with the horizontal wind field structure of atmospheric phenomena, e.g. the doldrums in the deep tropics, will benefit from along flight-track surface wind observations. Continuous surface wind data also further supplement dropsonde point-measurements.

How to cite: Stallmach, A., Weber, A., and Mayer, B.: Development of a surface wind retrieval by analysing sunglint geometry from specMACS radiance measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20399, https://doi.org/10.5194/egusphere-egu25-20399, 2025.

EGU25-393 | ECS | Posters on site | AS1.14

Quantifying the Relative Contributions of CCN and IN to Extreme Monsoon Rainfall 

Rituparna Chowdhury

The Indian summer monsoon, marked by extreme rainfall events during June–September, often triggers severe natural hazards such as floods. Accurate prediction of heavy rainfall is crucial to minimizing loss of life and property damage. While the roles of large-scale circulation, water vapor, and topography in monsoon convection have been studied, aerosol-cloud interactions remain poorly understood in this context. Aerosols, acting as cloud condensation nuclei (CCN) and ice nuclei (IN), influence cloud microphysics, precipitation mechanisms, and the hydrological cycle, intensifying weather and climate variability. Mixed-phase clouds, sensitive to aerosol effects, play a key role in regulating the Earth's radiation budget but are challenging to model due to complex processes like ice nucleation and particle growth. However, how uncertainty in aerosol data contributes to errors in quantitative precipitation forecasts (QPF) has yet to be thoroughly investigated. Understanding these interactions is critical for unraveling monsoon rainfall variability and enhancing forecast accuracy. To address this gap, this study uses the Weather Research and Forecasting (WRF) model with a triple-moment microphysics scheme to assess aerosol-cloud interactions in Indian summer monsoon precipitation. High-resolution simulations of monsoon depression events are performed under clean continental and urban (polluted) aerosol conditions, with model results compared to observations. Results of sensitivity simulations show that the microphysics can capture the observed rainfall pattern. However, in model performance it differs due to variations in mixing ratios of microphysics categories and associated dynamic and thermodynamic parameters. Polluted conditions significantly enhance extreme precipitation and updraft intensities, driven by increased ice-phase processes and larger snow and graupel hydrometeor sizes. These findings emphasize the pivotal role of aerosol concentrations in modulating extreme rainfall through intricate microphysical, thermodynamic, and dynamical interactions, offering new insights into improving the predictability of monsoon precipitation extremes.

 

How to cite: Chowdhury, R.: Quantifying the Relative Contributions of CCN and IN to Extreme Monsoon Rainfall, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-393, https://doi.org/10.5194/egusphere-egu25-393, 2025.

EGU25-583 | ECS | Posters on site | AS1.14

 Improving Precipitation Simulations in Regional Climate Models over the Yucatan Peninsula: The Role of Ice-Nucleating Particles in Cloud Microphysics Parameterizations 

Salvador Castillo-Liñan, Ruth Cerezo-Mota, Luis Antonio Ladino-Moreno, José Abraham Torres-Alavez, and María Eugenia Allende-Arandía

This study aims to enhance the precipitation simulations of regional climate models (RCMs) over the Yucatan Peninsula by implementing a cloud microphysics parameterization based on observational data of ice-nucleating particles (INPs) collected in the region.

Cloud microphysics parameterizations derived from observational INP data enable RCMs to more accurately represent heterogeneous nucleation, a critical process in the formation of ice crystals in clouds, which plays a key role in modulating both the duration and amount of precipitation.

Preliminary analyses with the RegCM model suggest that simulated precipitation is highly sensitive to modifications in cumulus and microphysics parameterizations. These findings provide valuable insights for advancing the understanding of INPs’ role in simulations over tropical regions. Nonetheless, further detailed analyses are required to comprehensively assess their influence and scope in these settings.

How to cite: Castillo-Liñan, S., Cerezo-Mota, R., Ladino-Moreno, L. A., Torres-Alavez, J. A., and Allende-Arandía, M. E.:  Improving Precipitation Simulations in Regional Climate Models over the Yucatan Peninsula: The Role of Ice-Nucleating Particles in Cloud Microphysics Parameterizations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-583, https://doi.org/10.5194/egusphere-egu25-583, 2025.

EGU25-2195 | ECS | Orals | AS1.14

Using SST as a proxy for cloud phase biases over the Southern Ocean 

Joaquin Blanco, Rodrigo Caballero, Steven Sherwood, and Lisa Alexander

The 50˚–65˚ latitude band exhibits the largest hemispheric asymmetry of cloud albedo over the oceans as well as the largest negative Southern Ocean (SO) cloud albedo biases in CMIP models. In this study, we show that cloud albedo regressed against sea-surface temperatures (SSTs) highlights essential differences between the observed Northern and Southern hemisphere climatologies, and between the SO’s simulated and observed albedos. The threshold 4˚–5˚C stands out as a regime separator in both comparisons.

By linking our empirical findings with the extensive evidence that model errors are related to the unique microphysical characteristics of the SO environment, we hypothesize that cloud albedo as a function of SST may act as a predictor of the presence/absence of supercooled liquid water cloud content.

Using satellite-retrieved cloud optical thickness (COT) and cloud top temperature (CTT), we verify that a regime separation of COT as a function of CTT exists between the Northern and Southern hemispheres (for CTT< -12˚C), which becomes more noticeable under midlevel subsidence conditions (i.e., low, boundary layer clouds).

Our simple and straightforward method using macrophysical variables can be easily applied in model evaluation with an insight in microphysics performance, especially given the scarcity of archived cloud-specific variables by the participating CMIP models. For example, it is well known that models tend to produce glaciated rather than supercooled liquid water clouds, and we show that in many cases models are simulating Northern Hemisphere clouds for the SO. We also detect that some of the CMIP models produce the right climatological cloud albedo over the SO but for the wrong reasons.

How to cite: Blanco, J., Caballero, R., Sherwood, S., and Alexander, L.: Using SST as a proxy for cloud phase biases over the Southern Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2195, https://doi.org/10.5194/egusphere-egu25-2195, 2025.

EGU25-3449 | ECS | Posters on site | AS1.14

First evaluation of Greenland clouds in RACMO2.4 using EarthCARE observations 

Thirza Feenstra, Willem Jan van de Berg, and Gerd-Jan van Zadelhoff

Clouds present one of the major challenges for climate modeling and cause large uncertainties in climate projections. This results from the complexity involved in representing small-scale cloud microphysics in coarse-gridded climate models. Over the Greenland Ice Sheet, clouds modulate melt, but with sharply contrasting impacts for snow and ice surfaces. Therefore, accurate representation of cloud processes and cloud occurrence is essential for reliable melt projections over the ice sheet.

The recently launched Earth Cloud, Aerosol and Radiation Explorer (EarthCARE) will provide cloud, precipitation and radiation profiles in unprecedented detail. We use these novel observations to evaluate cloud representation over Greenland in the latest version of the Regional Atmospheric Climate Model (RACMO2.4). Along-track atmospheric profiles of RACMO2.4 model output are compared with EarthCARE Level 2 cloud retrievals, as well as with Level 1 lidar and radar data, using derived backscatter and reflectivity profiles from the RACMO2.4 model output. The latter will help to explain which of the differences between observed and modeled cloud properties are due to model inaccuracies, and which are due to sensor limitations and data processing choices.

Using a selected number of case studies, our first comparison indicates that RACMO2.4 represents ice clouds reasonably well. However, we find large discrepancies regarding the representation of liquid clouds. Our analysis of cloud microphysical properties and aerosol representation will provide insights into the processes underlying these differences and will guide model development.

How to cite: Feenstra, T., van de Berg, W. J., and van Zadelhoff, G.-J.: First evaluation of Greenland clouds in RACMO2.4 using EarthCARE observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3449, https://doi.org/10.5194/egusphere-egu25-3449, 2025.

EGU25-4261 | ECS | Orals | AS1.14

How does Model Grid Resolution Influence Mixed-Phase Processes and UTLS Moisture Transport by a WCB? 

Cornelis Schwenk and Annette Miltenberger

Warm conveyor belts (WBCs) are large-scale ascending airstreams found in extratopical cyclones. They constitute a major source of upper tropospheric/lower stratospheric (UTLS) water vapor—a potent greenhouse gas—and hydrometeors, which can form cirrus clouds. Therefore, WCBs play an important role for Earth’s radiative budget. Additionally, WCBs transport large amounts of heat across latitudes and can influence large scale upper tropospheric circulation after their dissipation, underscoring their significance for Earth’s weather and climate.

Recent studies using high-resolution, convection-permitting simulations have shown that convection is a prominent feature of WCBs, with convective air parcels transporting significantly more hydrometeors into the UTLS than their slower-ascending counterparts. Furthermore, the cloud and precipitation development in convective air parcels is dominated by different processes than in slower ascending air. However, the global numerical weather prediction and climate models commonly used to assess the climatological and future impacts of WCBs operate at coarse grid resolutions (15–50 km) that are not convection-permitting, relying instead on convection parametrization schemes. The widely used Tiedtke-Bechtold convection parameterization scheme is designed to simulate heat, moisture, and momentum transport in convective systems but includes only basic representations of cloud microphysics. This raises the question of whether low-resolution simulations fail to accurately represent the transport of hydrometeors into the UTLS by WCBs when compared to high-resolution, convection-permitting simulations.

To address this, we analyze two simulations of the same WCB—one convection-permitting and one using convection parameterization—with a specific focus on vapor and hydrometeor transport. Our results show that the WCB in the high-resolution simulation transports substantially larger amounts of hydrometeors into the UTLS, while UTLS vapor conditions remain comparable between the two simulations. Microphysics processes also shift from liquid-dominated to frozen-dominated depending on the grid-scale.

How to cite: Schwenk, C. and Miltenberger, A.: How does Model Grid Resolution Influence Mixed-Phase Processes and UTLS Moisture Transport by a WCB?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4261, https://doi.org/10.5194/egusphere-egu25-4261, 2025.

EGU25-4385 | Orals | AS1.14

Simulation of satellite observations with RTTOV for ice clouds from deep convection using in-situ observations and a mesoscale model 

Romain Joseph, Emmanuel Fontaine, Alfons Schwarzenboeck, Julien Delanoe, Gaëlle Kerdraon, Tony Le Bastard, Helena Gonthier, Pierre Tulet, Christelle Barthe, and Jérôme Vidot

As part of the NWCSAF project (Nowcasting Satellite Application Facility), the CNRM participates in the retrieval of cloud properties from geostationary satellite observations. These retrievals include the Cloud Mask and Cloud Types classification, thermodynamics properties at the macroscopic scales (Cloud Top Temperature and Height) as well as microphysical cloud properties (effective radius, optical thickness, liquid and ice water path). Radiative transfer simulations are mandatory to retrieve these properties. In this study, I performed simulations of observations from the Meteosat Second Generation satellite based on in-situ measurements taken on board an airborne campaign and mesoscale models using the radiative transfer model RTTOV.In order to compare the differences between simulation and observations for the case of ice clouds formed by deep convective systems, in the infrared and visible. Then discuss the sensitivity of the simulations to the physical and optical properties of the clouds, for example, how a misrepresentation of the ice water content at the top of clouds can be highlighted using simulations.

How to cite: Joseph, R., Fontaine, E., Schwarzenboeck, A., Delanoe, J., Kerdraon, G., Le Bastard, T., Gonthier, H., Tulet, P., Barthe, C., and Vidot, J.: Simulation of satellite observations with RTTOV for ice clouds from deep convection using in-situ observations and a mesoscale model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4385, https://doi.org/10.5194/egusphere-egu25-4385, 2025.

EGU25-5713 | ECS | Posters on site | AS1.14

Riming-dependent Snowfall Rate and Ice Water Content Retrievals for W-band cloud radar 

Nina Maherndl, Alessandro Battaglia, Anton Kötsche, and Maximilan Maahn

Accurate measurements of snowfall in mid- and high-latitudes are particularly important, because snow provides a vital freshwater source, and impacts glacier mass balances as well as surface albedo. However, ice water content (IWC) and snowfall rates (SR) are hard to measure due to their high spatial variability and the remoteness of polar regions.

Here, we present novel ice water content - equivalent radar reflectivity (IWC-Ze) and snowfall rate - equivalent radar reflectivity (SR-Ze) relations for 40° slanted and vertically pointing W-band cloud radar. The relations are derived from joint in situ snowfall and remote sensing (radar and radiometer) data from the SAIL site (Colorado, USA) and validated for sites in Hyytiälä (Finland), Ny-Ålesund (Svalbard, Norway), and Eriswil (Switzerland). In addition, gauge measurements from SAIL and Hyytiälä are used as an independent reference for validation. We show the dependence of IWC-Ze and SR-Ze on riming, which we utilize to reduce the spread in the IWC-Ze and SR-Ze spaces. Normalized root mean square errors (NRMSE) are below 25% for IWC>0.1 gm⁻³. For SR, the NRMSE is below 70% over the whole SR range. We also present relations using liquid water path (LWP) as a proxy for the occurrence of riming, which can be applied to both ground-based and space-borne radar-radiometer instruments. The latter is demonstrated using the example of the proposed ESA Earth Explorer 11 candidate mission WIVERN, which consists of a conical scanning 94 GHz radar and a passive 94 GHz radiometer. With this approach, NRMSE are below 75% for IWC>0.1 gm⁻³ and below 80% for SR>0.2 mmhr⁻¹.

The proposed IWC and SR relations provide a novel way to reduce uncertainties of IWC and SR estimates for W-band radar by accounting for particle riming. Advantages to current literature relations are the flexibility in terms of viewing angle and the inclusion of LWP, allowing the application to ground-based and space-borne radar-radiometer combinations like EarthCARE or the proposed WIVERN mission.

How to cite: Maherndl, N., Battaglia, A., Kötsche, A., and Maahn, M.: Riming-dependent Snowfall Rate and Ice Water Content Retrievals for W-band cloud radar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5713, https://doi.org/10.5194/egusphere-egu25-5713, 2025.

EGU25-6543 | ECS | Orals | AS1.14

Chasing ice crystals: Lagrangian trajectories in ICON-LES for investigating liquid and ice phase interactions 

Nadja Omanovic, Sylvaine Ferrachat, Christopher Fuchs, Fabiola Ramelli, Jan Henneberger, Anna J. Miller, Robert Spirig, Huiying Zhang, and Ulrike Lohmann

The ice phase is a major contributor to precipitation formation over continents, as ice hydrometeors efficiently grow to large enough sizes for them to sediment. Several mechanisms underlie the growth of ice crystals, with one being the growth through vapor deposition onto the ice crystal. The speed of this growth depends next to temperature also on the availability of water vapor, one source being cloud droplets in mixed-phase clouds that locally may experience water-subsaturated conditions. This is referred to as the Wegener-Bergeron-Findeisen (WBF) process and describes the ability of ice crystals to grow at the expense of cloud droplets. While the presence of the WBF process is established, the actual growth rates of ice crystals in such conditions remain ambiguous. We conducted field experiments within the CLOUDLAB project with the goal to infer ice crystal growth rates in naturally occurring supercooled clouds through local perturbations from cloud seeding. A unique dataset was collected describing the characteristics of cloud droplets and ice crystals in the probed clouds, including their sizes, number concentrations, and ice and water contents.

Here, we combine large-eddy simulations (LES) in 65 m horizontal resolution with online Lagrangian trajectories to achieve a more straightforward comparison to our observations. We show that the model simulations can reproduce the field experiments in terms of ice crystal number concentrations. However, both the simulated changes in the liquid phase as a consequence of the WBF process and the ice crystal growth rates are underestimated compared to the observations. We perform a series of sensitivity studies on the vapor depositional growth equation of ice crystals given the uncertainty and simplification of two parameters of that equation.  We find that an increase of the vapor deposition efficiency up to a factor of three achieves comparable growth rates. However, matching growth rates in the model and observations does not lead to coinciding changes in the liquid phase, i.e., the WBF process remains too slow. We identify two limitations of our approach: (i) the simulated and actual water vapor fields may differ and (ii) our LES are still too coarse to fully capture the small-scale interactions between the liquid and ice phases. This study highlights the synergy of high-resolution model simulations and field observations for investigating a fundamental cloud process. Our results provide insights for future mixed-phase cloud modeling studies. 

How to cite: Omanovic, N., Ferrachat, S., Fuchs, C., Ramelli, F., Henneberger, J., Miller, A. J., Spirig, R., Zhang, H., and Lohmann, U.: Chasing ice crystals: Lagrangian trajectories in ICON-LES for investigating liquid and ice phase interactions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6543, https://doi.org/10.5194/egusphere-egu25-6543, 2025.

EGU25-6792 | Orals | AS1.14

Detection of Linear Contrails with a Morphological Algorithm and with Deep Neural Networks 

Nicolas Gourgue, Olivier Boucher, and Laurent Barthes

The climate impact of aviation can be separated into CO2 and non-CO2 effects, with the latter being potentially larger than the former. In this context we are more specifically interested in condensation trails (hereafter contrails) and induced cirrus. Monitoring contrail formation and evolution is necessary to understand their radiative effects and help the aviation industry to transition towards a more sustainable activity. 
Current research aimed at detecting contrails is mostly based on geostationary satellite images because they allow to follow the contrail over a long period of time. However a major shortcoming of this approach, due to the current spatial resolution of geostationary imagers, is that the contrail formation phase cannot be detected and larger, but older, contrails cannot always be attributed to the flights that produced them. To circumvent this problem and observe the contrail formation phase, we use a ground-based hemispheric camera with a two-minute sampling rate as a complementary source of information. 
As a first step, we have developed a traditional morphological algorithm that will help preparing a sufficiently large labelled database as required to train a deep-learning algorithm. This algorithm aims to detect whether each aircraft that passes in the field of view of the camera (as monitored from an ADSB radar) produces a contrail or not and, whenever possible, track the contrail across successive images. 
We are thus able to relate contrail formation and evolution with aircraft type, flight altitude and weather conditions.  We consider all weather conditions except completely cloudy conditions that prevent contrails from being observed. The performance of this algorithm is evaluated against a database that was manually annotated consisting of 400 images with 407 contrails. We find a specificity of 97\%, i.e. there are few false detections, but a sensitivity of about 55\%, i.e. it is missing a significant fraction of contrail that were annotated manually. An analysis of several years of contrail detection will be presented to determine precisely the fraction of contrail-producing flights and the  weather conditions associated with short-lived (less than 2 min) and longer-lived(more than 2 min) contrails. 
Additionally to this approach, which misses part of the young contrails and does not detect contrails formed outside the field of view of the camera, we have trained deep neural networks such as Unet and DeeplabV3, on a database of 1600 images in order to overcome those limits. Our preliminary results show a good performance on young contrails, with an improved detection capability, in particular for contrails formed outside of the camera field of view. The deep neural networks also work better for old contrails but may confuse very old contrails with background cloud features. 

How to cite: Gourgue, N., Boucher, O., and Barthes, L.: Detection of Linear Contrails with a Morphological Algorithm and with Deep Neural Networks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6792, https://doi.org/10.5194/egusphere-egu25-6792, 2025.

EGU25-6928 | ECS | Orals | AS1.14

Observations and Analysis of Cirrus Clouds in the Arctic during Warm Air Intrusions 

Georgios Dekoutsidis, Silke Groß, Martin Wirth, Christian Rolf, Martina Krämer, Andreas Schäfler, and Florian Ewald

Cirrus clouds permit much of the incoming solar shortwave radiation to pass through while trapping and reemitting the Earth's outgoing longwave thermal radiation. This results in a net warming effect globally at the top of the atmosphere. They are found almost over every region, but their impact can differ depending on latitude. The arctic is a unique and fascinating area. Over the last few decades, scientists have shown that its average temperature is increasing at an accelerated rate compared to global warming. This phenomenon has been labeled Arctic Amplification and cirrus clouds are considered a potential contributor. Another arctic-specific phenomenon linked to arctic amplification are Warm Air Intrusions (WAI). During such events, warm, water-vapor- and aerosol-rich airmasses are meridionally transported into the arctic from the midlatitudes. Apart from the transport of sensible heat and water vapor, a strong greenhouse gas, these events can potentially alter properties and effects of the cirrus clouds that form in the arctic. The positive trend found in the frequency and longevity of these events further highlights the importance to understand how they affect the macrophysical and optical properties of cirrus clouds in the arctic.

In March and April of 2022, the HALO-(AC)3 field campaign was conducted. The main goal of this campaign was to investigate WAI events and airmass transformations in the arctic. One of the platforms employed during this campaign was the German research aircraft HALO. It was used to perform remote sensing measurements at high altitudes over cirrus clouds. Among the instruments aboard HALO, were the combined water vapor differential absorption and high spectral resolution lidar system WALES and the HAMP package including a cloud radar and radiometers. Measurements from these two instruments form the basic dataset analyzed in this study. The cirrus clouds detected during this campaign are classified as either WAI cirrus or AC cirrus depending on if they were measured during an active WAI or during undisturbed arctic conditions. In order to better classify the clouds and provide a more in-depth analysis their backwards trajectories were calculated using the Lagrangian analysis tool LAGRANTO and the CLaMS-Ice model, which combines the Chemical Lagrangian Model of the Stratosphere (CLaMS) with two-moment ice microphysics.

In this presentation we are comparing the geometrical and optical depths of WAI and AC cirrus as measured by WALES. From the same instrument we also calculate the supersaturations with respect to ice and get a first insight into the probable nucleation processes. The backwards trajectories reveal more details regarding the origin, formation process, nucleation pathway and microphysical properties of the two cloud types. The analysis of the microphysical properties is further strengthened by analyzing the combined radar-lidar products.

How to cite: Dekoutsidis, G., Groß, S., Wirth, M., Rolf, C., Krämer, M., Schäfler, A., and Ewald, F.: Observations and Analysis of Cirrus Clouds in the Arctic during Warm Air Intrusions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6928, https://doi.org/10.5194/egusphere-egu25-6928, 2025.

EGU25-7011 | ECS | Posters on site | AS1.14

Cirrus formation in particle-based aerosol-cloud microphysics 

Tim Lüttmer, Sylwester Arabas, and Peter Spichtinger

We developed an ice phase extension for the PySDM Python package. PySDM is used for simulating the microphysics of population of particles, e.g. for modeling liquid droplets and their interactions with aerosol in clouds. PySDM uses the particle-based approach (‘super droplet method’) and features Monte-Carlo type solvers for processes such as collisions, coagulation, breakup, and freezing.

Our aim is to adapt that framework for the simulation of (pure) ice clouds in the cirrus temperature regime. Ice super particles are affected by homogeneous freezing of solution droplets, deposition nucleation, growth by vapor deposition and sedimentation. The main research question is the investigation of in-situ ice formation and sedimentation rates of in-situ formed ice into lower cloud layers. We present some early results for prescribed flow.

How to cite: Lüttmer, T., Arabas, S., and Spichtinger, P.: Cirrus formation in particle-based aerosol-cloud microphysics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7011, https://doi.org/10.5194/egusphere-egu25-7011, 2025.

EGU25-7218 | ECS | Posters on site | AS1.14

In-situ characterisation of graupel in deep convective cloud 

Ezri Alkilani-Brown, Alan Blyth, Declan Finney, Chetan Deva, Paul Field, and Jonathan Crosier

Graupel continues to be the least well constrained and understood hydrometeor in numerical models. Playing an important role in cloud electrification and precipitation in cumulonimbus, graupel is critical to model correctly. New observations from the Deep Convective Microphysics Experiment1 (DCMEX) have been used to evaluate a recently developed machine-learning algorithm, which categorises hydrometeor images. An overview of the overarching ice habit distribution from DCMEX cumulonimbus will be presented, alongside preliminary analysis of the observed graupel formation and its corresponding environmental conditions.

DCMEX presents a unique opportunity of complementary in-situ and radar observations. The project was conducted in the Magdalena Mountains of New Mexico during the summer of 2022. The airborne sampling strategy involved repeated sampling of cloud turrets as convection strengthened through the day, allowing for evolving in-situ observations as the cloud deepened. The campaign was able to successfully sample convective cloud on 17 out of 19 flight days.

To understand the microphysical processes within a developing cloud, ice images from the 2D Stereo Probe and High Volume Precipitation Spectrometer have been analysed. These images have been categorised into habit, using the supervised machine learning algorithms from Jaffeux et al.2,3. Independent evaluation of the algorithms has been conducted, to test the generalisation capabilities under different cloud conditions.

This work aims to strengthen our understanding of graupel in deep convective cloud, whilst evaluating a novel machine learning approach to process data. Ultimately, this will contribute to the assessment of ice microphysics in regional forecasts.

References:

(1)        Finney, D.L. et al. (2024). Earth Syst. Sci. Data, 16(5), 2141-2163.

(2)        Jaffeux, L. et al. (2022). Atmos. Meas. Tech., 15(17), 5141-5157.

(3)        Jaffeux, L. et al. (2024). EGUsphere (Preprint).

How to cite: Alkilani-Brown, E., Blyth, A., Finney, D., Deva, C., Field, P., and Crosier, J.: In-situ characterisation of graupel in deep convective cloud, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7218, https://doi.org/10.5194/egusphere-egu25-7218, 2025.

EGU25-7821 | ECS | Posters on site | AS1.14

 Cloud microphysics in Arctic and Antarctic environments derived from infrared emission spectroscopy 

Joseph Hung, Penny Rowe, Emily McCullough, Liam Kroll, Raia Ottenheimer, Rachel Chang, and Kimberly Strong

Climate models struggle to accurately represent polar regions, particularly during polar night, when cloud cover is especially prevalent. The uncertainty budget is dominated by cloud and cloud-aerosol interactions, but the difficulty in maintaining robust field observations means a lack of long-term validation datasets for key cloud parameters. Long-term measurements of the downwelling thermal infrared (400 - 3000 cm-1) have been recorded since 2008 with an Atmosphere Emitted Radiance Interferometer (AERI) at the Polar Environment Atmospheric Research Laboratory (PEARL) in Eureka, Nunavut, Canada (80°N, 86°W) and operated by the Canadian Network for the Detection of Atmospheric Change (CANDAC), while a similar instrument was deployed at McMurdo Station for 2016 as part of the ARM [Atmosphere Radiation Measurement] West Antarctic Radiation Experiment (AWARE) program. We analyse the downwelling infrared emission of the polar atmosphere recorded by these AERI instruments, with supplementary data from observations and models, to derive a climatology of microphysical and optical properties of clouds at Eureka (since 2008) and McMurdo (2016), including optical depth, thermodynamic phase, and liquid droplet and ice crystal effective scattering radii. A comparison of these Arctic and Antarctic cloud properties reveals an abundance of cloud morphological states at these two polar locations. This presentation will also describe the temperature dependence of cloud microphysics, seasonality in the timeseries, and the effect of inversions on cloud boundaries, as well as challenges in performing these retrievals.

How to cite: Hung, J., Rowe, P., McCullough, E., Kroll, L., Ottenheimer, R., Chang, R., and Strong, K.:  Cloud microphysics in Arctic and Antarctic environments derived from infrared emission spectroscopy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7821, https://doi.org/10.5194/egusphere-egu25-7821, 2025.

EGU25-8032 | Orals | AS1.14

Quantifying ice crystal growth rates in natural clouds from glaciogenic cloud seeding experiments 

Christopher Fuchs, Fabiola Ramelli, Ulrike Lohmann, Anna J. Miller, Nadja Omanovic, Robert Spirig, Huiying Zhang, and Jan Henneberger

Ice crystals in mixed-phase clouds (MPCs) can grow rapidly to large sizes by vapor deposition via the Wegener-Bergeron-Findeisen (WBF) process, i.e., growth of ice crystals at the expense of cloud droplets. This rapid growth can trigger subsequent processes such as riming and aggregation, which often initiate precipitation, making MPCs the major source of precipitation over continents. The growth of ice crystals has been thoroughly studied in the laboratory for many decades and several theoretical models were developed on their basis. However, in situ measurements of growth rates to confirm laboratory studies are still sparse due to the lack of controllability of experiments in natural clouds.

In the CLOUDLAB project, we conducted confined, controlled, and repeatable glaciogenic cloud seeding experiments to study ice crystal growth in natural clouds. A drone released seeding particles in supercooled low stratus clouds to initiate the formation of ice crystals. The freshly formed ice crystals were observed 5-10 minutes downwind of the seeding location using cloud radars and holographic imager for in situ observations. The holographic imager obtains phase-resolved information on cloud droplets > 6 µm and ice crystals > 25 µm with a high spatio-temporal resolution, which allows us to quantify accurate ice crystal growth rates.

In this study, we present ice crystal growth rates obtained from in-situ observations from 14 seeding experiments in the temperature range between -5.1°C and -8.3°C. During the seeding experiments, ice crystal number concentrations (ICNC) increased by several orders of magnitude, accompanied by a strong reduction in cloud droplet number concentration, a clear indicator of the WBF process.  We also observed that high ICNCs limit or inhibit ice growth due to the competition of the ice crystals for the available water vapor.  The obtained ice crystal growth rates are compared with laboratory studies and show on average slightly lower values. We also observed the expected variation in growth rates across our temperature range agreeing with laboratory findings. These findings can connect laboratory studies and in situ observations and provide valuable insights into vapor depositional growth of ice crystals in natural clouds.

How to cite: Fuchs, C., Ramelli, F., Lohmann, U., Miller, A. J., Omanovic, N., Spirig, R., Zhang, H., and Henneberger, J.: Quantifying ice crystal growth rates in natural clouds from glaciogenic cloud seeding experiments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8032, https://doi.org/10.5194/egusphere-egu25-8032, 2025.

EGU25-8666 | Posters on site | AS1.14

Cirrus cloud median microphysical and optical properties in the IWC-temperature space from a comprehensive airborne size distribution database  

Reinhold Spang, Martina Krämer, Irene Bartolome Garcia, and Nicole Spelten

The detailed information on the particle size distributions (PSDs) of ice clouds is essential for various topics of radiative transport in a cloudy atmosphere. The new composite of in-situ PSD measurements, including 9 airborne campaigns with in total 137 flight hours in cirrus cloud conditions, is currently the most comprehensive data set for studying PSD parameters. The PSDs cover for all campaigns particle diameters down to 3 microns and are not affected by the so-called shattering effect. The database covers the complete cirrus cloud temperature range (185 - 235 K) and IWC from 10−6 to 1 g/m3 and and is thus especially well-suited to investigate optically thinnest clouds hitherto not included in PSD data bases.

Here, the database is used for detailed analysis of PSDs of cirrus clouds for two size modes, as Bartolomé García et al. (2023) have shown that ice cloud PSDs are better represented by bimodal PSDs. To this end, two log-normal functions are derived for the measured PSDs, one for small and one for large ice particles. An iterative approach for fitting the bimodal log-normal functions to the measured PSD by minimizing a cost function have been applied to the data with overall good fitting results.

Next, microphysical and optical properties such as ice water content (IWC), mean mass diameter (D), effective radius (Reff) and extinction are determined for the total cirrus particle size range and also for each of the two size modes. For each parameter, median values are then computed at predefined IWC - temperature intervals.

Characteristics of the total size range as well as of the small and large size modes in the IWC-temperature space in terms of microphysical and optical properties will be presented for mid-latitudes and the tropics. The potential imprint of the results on currently applied cloud modules and cloud parameterization in global climate models will be investigated.

 

References: Bartolomé García, I., Sourdeval, O., Spang, R., and Krämer, M.: Technical note: Bimodal parameterizations of in situ ice cloud particle size distributions, Atmos. Chem. Phys., 24, 1699–1716, https://doi.org/10.5194/acp-24-1699-2024, 2024.

How to cite: Spang, R., Krämer, M., Bartolome Garcia, I., and Spelten, N.: Cirrus cloud median microphysical and optical properties in the IWC-temperature space from a comprehensive airborne size distribution database , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8666, https://doi.org/10.5194/egusphere-egu25-8666, 2025.

EGU25-9155 | Orals | AS1.14

Aerosol effects on Secondary Ice Production in Deep ConvectiveClouds: exploiting the synergistic benefit of observations andaerosol-aware cloud simulations 

Sami Romakkaniemi, Tomi Raatikainen, Harri Kokkola, Paul Lawson, and Silvia Calderón

Secondary ice production (SIP) refers to a series of physical mechanisms that significantly increase ice number concentrations above those from primary ice production (PIP) via ice nucleating particles (INP). In-cloud observations have provided increasing evidence of SIP in mixed-phase stratiform and convective clouds at different latitudes. The presence of fragmented frozen drops and small columnar particles in measurements from holographic particle imaging systems is consistent with findings of laboratory experiments focused on rime splintering (RS), droplet shattering (DS), and ice-ice collisional breakup (IIBR) mechanisms. Since SIP rates are driven by the relative size of interacting hydrometeors, there is a need to understand which microphysical conditions trigger which mechanism in realistic atmospheric conditions where cloud micro physics are constrained by aerosols. Without describing aerosol-hydrometeor interactions, the majority of cloud modelling tools are limited to prescribed size distributions and process rates that may fail giving proper description of ice formation via primary and secondary pathways missing important links to others such as secondary activation and aerosol invigoration.
In this study we offer insights on aerosol-induced effects on SIP rates by coupling results from aerosol-aware large-eddy- simulations and in-cloud observations of a deep convective cloud case studied in the SPICULE campaign in the Southern Great Plains (USA) on June 05 2021. We employed UCLALES-SALSA, an LES model with sectional representation of aerosol microphysics to resolve rates for PIP via immersion freezing with time evolving contact angle distribution and SIP via droplet shattering (DS), and ice-ice collisional breakup (IIBR). After model initialization with observed atmospheric soundings and aerosol concentrations, we were able to reproduce observed trends in cloud properties including boundaries and vertical profiles of droplet and ice particle size distributions. The model was able to emulate the observed ice multiplication in the rising cloud tower indicating a positive feedback between SIP-DS and SIP-IIBR processes which in turn increased convection intensity through mixed-phase invigoration at the upper level and finally lead to glaciation and precipitation via seeder-feeder mechanism. Both, the convective available energy (CAPE) and the level of neutral buoyancy (LNB), were adjusted to reach model closure in the cloud tower. We also compared simulations differing in the aerosol number concentration in the accumulation mode used for model initialization and found that increasing fine particle concentrations increase ice formation and updraft strength above freezing level suggesting that mixed-phase invigoration has an role in cloud phase structure and glaciation of convective clouds.

How to cite: Romakkaniemi, S., Raatikainen, T., Kokkola, H., Lawson, P., and Calderón, S.: Aerosol effects on Secondary Ice Production in Deep ConvectiveClouds: exploiting the synergistic benefit of observations andaerosol-aware cloud simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9155, https://doi.org/10.5194/egusphere-egu25-9155, 2025.

EGU25-10410 | ECS | Posters on site | AS1.14

Impacts of Entrainment and Mixing on Ice Growth in Mixed-Phase Clouds 

Benjamin Ascher and Fabian Hoffmann

Shallow mixed-phase clouds, in which ice and liquid particles co-exist, occur frequently in the middle and high latitudes of Earth. Yet despite their frequency and importance for local precipitation and radiative balance, our understanding of these clouds is limited. Especially the interaction of small-scale turbulence and mixed-phase microphysics has received little attention so far. To address this knowledge gap, we conducted large-eddy simulations with a highly detailed Lagrangian cloud microphysics parameterization. We simulate a shallow mixed-phase cloud observed during the Indirect and Semi-Direct Aerosol Campaign (ISDAC). We focus on the processes occurring in regions of mixing and entrainment near the cloud edges, with particular focus on the Wegener-Bergeron-Findeisen (WBF) process. We also investigate the effect on cloud properties, lifetime, and radiative balance from using a kinetically-limited ice crystal growth parameterization as opposed to a traditional capacitance-based growth parameterization. 

How to cite: Ascher, B. and Hoffmann, F.: Impacts of Entrainment and Mixing on Ice Growth in Mixed-Phase Clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10410, https://doi.org/10.5194/egusphere-egu25-10410, 2025.

EGU25-11239 | ECS | Posters on site | AS1.14 | Highlight

Impacts of Wildfire Smoke on Cirrus Cloud Formation 

Paraskevi Georgakaki, Christina-Anna Papanikolaou, Odran Sourdeval, and Johannes Quaas

The increasing prevalence of wildfire smoke layers in the upper troposphere and lower stratosphere, likely driven by climate change, highlights their growing influence on the climate system. These smoke plumes travel across continents affecting climate through multiple pathways, emphasizing the need for their accurate representation in global climate models (GCMs). Among these pathways, this study focuses on the role of wildfire smoke particles in cirrus cloud formation by acting as efficient ice-nucleating particles (INPs).

The mechanisms governing cirrus cloud formation—whether dominated by homogeneous freezing or a competition with heterogeneous ice nucleation—determine their microphysical and optical properties, as well as their role in seeder-feeder and precipitation processes. Recent ground-based lidar and radar studies (e.g., Mamouri et al., 2023; Ansmann et al., 2024) provide evidence that aged wildfire smoke particles can trigger heterogeneous ice nucleation. However, their limited temporal and spatial coverage constrains our understanding of the broader-scale impacts of wildfire-induced cirrus, thereby complicating the development of reliable parameterizations for GCMs.

In this study, we seek to address this limitation by leveraging spaceborne observations to investigate the relationship between wildfire smoke and cirrus cloud formation. Potential smoke INPs are retrieved using the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) level 2 V4.51 data products, while in-cloud ice crystal number concentrations (ICNCs) are derived from the DARDAR-Nice (liDAR–raDAR-Number concentration of ICE particles) product. By integrating these datasets with global reanalysis data, we analyze multiple large wildfire events across both hemispheres, which help uncover the large-scale and seasonal characteristics of wildfire-induced cirrus. With wildfires becoming increasingly frequent and intense under a warming climate, understanding how smoke influences the occurrence and properties of cirrus clouds is critical for improving the accuracy of future climate projections.

 

Ansmann, A., Jimenez, C., Roschke, J., Bühl, J., Ohneiser, K., Engelmann, R., Radenz, M., Griesche, H., Hofer, J., Althausen, D., Knopf, D. A., Dahlke, S., Gaudek, T., Seifert, P., and Wandinger, U.: Impact of wildfire smoke on Arctic cirrus formation, part 1: analysis of MOSAiC 2019–2020 observations, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2024-2008, 2024

Mamouri, R.-E., Ansmann, A., Ohneiser, K., Knopf, D. A., Nisantzi, A., Bühl, J., Engelmann, R., Skupin, A., Seifert, P., Baars, H., Ene, D., Wandinger, U., and Hadjimitsis, D.: Wildfire smoke triggers cirrus formation: lidar observations over the eastern Mediterranean, Atmos. Chem. Phys., 23, 14097–14114, https://doi.org/10.5194/acp-23-14097-2023, 2023

How to cite: Georgakaki, P., Papanikolaou, C.-A., Sourdeval, O., and Quaas, J.: Impacts of Wildfire Smoke on Cirrus Cloud Formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11239, https://doi.org/10.5194/egusphere-egu25-11239, 2025.

EGU25-11347 | ECS | Orals | AS1.14

Detailed coupled approach to ice particles nucleation induced by gravity waves in a global NWP model 

Alena Kosareva, Stamen Dolaptchiev, Axel Seifert, Peter Spichtinger, and Ulrich Achatz

One of the sources of uncertainties in climate models and numerical weather prediction (NWP) models is cirrus clouds. They are highly sensitive to subgrid-scale dynamics, such as gravity waves (GWs) and turbulence, making them challenging to model in detail within coarse-resolution settings.  Additionally, their net radiative effect remains poorly understood, highlighting the importance of accurately representing their microphysical properties as one of the main areas of focus for research and model refinement.

The current work focuses on a coupled approach to GW–ice microphysics interactions and its application in the global NWP model ICON. The ice scheme, developed by Dolaptchiev et al. (J. Atmos. Sci., 2023), describes GW-induced homogeneous nucleation of ice crystals and proposes a prototype parameterization used in this study. The representation of a local GW field is diagnosed using the Multi-Scale Gravity Wave Model (MS-GWaM) parameterization. MS-GWaM parameterization supports multiple GW source types, and allows for 3D GW propagation, enhancing its physical realism. The full coupling of GW forcing, along with feedback from the new scheme into the overall microphysics and radiation schemes, has been implemented in a test regime in ICON model.

To validate the approach and assess the impact of GWs, several global ICON simulations were conducted. The results show a significant influence of GWs on ice number density, indicating higher concentrations of ice crystals in tropical regions. These findings highlight the potential of the coupled approach to improve predictions of cloud microphysics and their radiative impacts. Further investigations will explore the role of different GW sources and account for the superposition of GWs, offering deeper insights into the broader effects of GW representation on global atmospheric processes.

How to cite: Kosareva, A., Dolaptchiev, S., Seifert, A., Spichtinger, P., and Achatz, U.: Detailed coupled approach to ice particles nucleation induced by gravity waves in a global NWP model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11347, https://doi.org/10.5194/egusphere-egu25-11347, 2025.

EGU25-12739 | ECS | Orals | AS1.14

Combined Remote-Sensing, In-Situ and Modelling of Cloud Microphysical Perturbations in Supercooled Stratus Clouds 

Willi Schimmel, Fabian Senf, Jens Stoll, Kevin Ohneiser, Patric Seifert, Jan Henneberger, Ulrike Lohmann, Rober Spirig, Fabiola Ramelli, Christopher Fuchs, Anna Miller, Huiying Zhang, and Nadja Omanovic
Aerosol-cloud interactions in mixed-phase clouds still present major challenges for weather and climate models. The PolarCAP project (Polarimetric Radar Signatures of Ice Formation Pathways from Controlled Aerosol Perturbations) investigates how aerosols influence cloud-microphysical processes via cold cloud seeding experiments. Ice formation and evolution is studied under slightly supercooled conditions (T > -10°C) within a thermodynamically and aerosol-controlled environment, employing radar polarimetry, holographic imagery and spectral-bin modeling. In collaboration with the CLOUDLAB project at the ETH Zurich, PolarCAP investigates the development of an artificially initiated ice phase within supercooled stratus clouds. Utilizing cloud seeding with silver iodide, the freezing process of super-cooled cloud droplets is initiated. The subsequent evolution is monitored using in-situ measurements and ground-based cloud remote sensing tools. The collaboration has yielded a unique dataset, incorporating observations from the Leipzig Aerosol and Cloud Remote Observing System (LACROS) and in-situ data from CLOUDLAB in tandem with data from the cloud-resolving spectral-bin microphysics model COSMO-SPECS.

We present a comparative evaluation between observational and model data, complemented by a Lagrangian analysis that tracks ice formation and growth processes within the seeded cloud to provide detailed insights into the evolution of the ice phase. A multitude of ensemble model runs were performed on two different mesh sizes, with horizontal resolution of ~400m and ~100m, varying the flare INP injection rate and initial cloud condensation nuclei (CCN) number concentrations. First, we show the model's ability to replicate observed cloud responses, providing insights into primary ice growth processes, particularly the Wegener-Bergeron-Findeisen (WBF) process. During the seeding experiments, observations show simultaneous decreases in cloud droplet concentrations alongside increases in ice crystal concentrations, including periods where cloud droplets were entirely depleted. Second, the measured ice crystal sizes and growth rates, are compared to the model output. This comparison revealed discrepancies in ice crystal size distributions, highlighting potential model biases in parameterizations of ice nucleation and growth rates for columnar ice crystals.

How to cite: Schimmel, W., Senf, F., Stoll, J., Ohneiser, K., Seifert, P., Henneberger, J., Lohmann, U., Spirig, R., Ramelli, F., Fuchs, C., Miller, A., Zhang, H., and Omanovic, N.: Combined Remote-Sensing, In-Situ and Modelling of Cloud Microphysical Perturbations in Supercooled Stratus Clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12739, https://doi.org/10.5194/egusphere-egu25-12739, 2025.

EGU25-12954 | Orals | AS1.14

Distribution of RHice inside thin and thick cirrus clouds over the Northern Mid-latitudes and in a Subtropical Region 

Andreas Petzold, Neelam F. Khan, Yun Li, Susanne Rohs, Susanne Crewell, and Martina Krämer

In-situ based information on the distribution of RHice inside cirrus clouds is still retrieved mainly from focused research aircraft campaigns for dedicated regions and seasons, but a long-term and seasonal perspective is missing. We report on the distribution of RHice in clear sky as well as inside thin and thick cirrus clouds for the North Atlantic region and over subtropical Southeast Asia, with the focus on the occurrence of ice-supersaturated air masses.

The underlying data base builds on more than 7 years of continuous in-situ observations by the European research infrastructure IAGOS (www.iagos.org) which measures, among others, temperature, RHice and ice cloud particles, on instrumented passenger aircraft. Information on cloud coverage and cloud thickness were taken from ERA5 global reanalysis by means of the cloud ice water content (CIWC). The separation of clear-sky and in-cloud flight sequences was achieved by applying a novel ERA5 CIWC based cloud index validated by IAGOS in-situ RHice observations.

The analysed data set covers the period from June 2014 to December 2021. Four regions were identified for in-depth statistical analyses, with three of them located in the Northern midlatitudes (30–60°N), namely Eastern North America (105–65°W), the North Atlantic flight corridor (65–5°W), and Western Europe (5°W–30°E), and one in the Southeast Asian subtropics (0–30°N, 45–120°E).

We will present the novel cloud index and discuss the features of the resulting RHice probability distribution functions of the analysed regions, including seasonal variations, and potential implications for the underlying cirrus cloud formation processes.

How to cite: Petzold, A., Khan, N. F., Li, Y., Rohs, S., Crewell, S., and Krämer, M.: Distribution of RHice inside thin and thick cirrus clouds over the Northern Mid-latitudes and in a Subtropical Region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12954, https://doi.org/10.5194/egusphere-egu25-12954, 2025.

EGU25-14507 | Posters on site | AS1.14

Improved Simulation of Arctic Mixed-Phase Clouds with Modified Ice Microphysics in the WDM6 Scheme 

Hyun-Joon Sung, Kyo-Sun Sunny Lim, Song-You Hong, JiHoon Shin, Baek-Min Kim, and Ji-Hun Choi

In this study, we evaluated the simulation performance of Arctic mixed-phase clouds using the Weather Research and Forecasting (WRF) Double-Moment 6-class (WDM6) scheme and its improved version (WDM6_ICE). WDM6_ICE prognoses the cloud ice number concentrations and incorporates the enhanced cloud ice shape parameters and cloud ice formation processes. Sensitivity experiments were conducted during the Mixed-Phase Arctic Cloud Experiment (M-PACE) period of October 9–10, 2004.

WDM6_ICE significantly improved cloud simulation, showing the enhanced low-level cloud fraction and more realistic radiation effects compared to WDM6. The vertical structure analysis revealed that WDM6_ICE more effectively maintained supercooled cloud liquid by reducing ice deposition and enhancing condensation processes and reduced efficiency of Wegener-Bergeron-Findeisen (WBF) process. Through the sensitivity experiments involving changes in cloud ice shape (SP) and ice nucleation processes (IN) (WDM6_SP and WDM6_SP_IN), we demonstrated how these changes contributed to the improved phase partitioning in mixed-phase clouds. However, our analysis also revealed limitations in the representation of total water content and boundary layer structure, suggesting the need for further improvements in surface-atmosphere interactions under stable Arctic conditions. Our findings provide insights for improving the representation of cloud microphysics and their interaction with boundary layer processes in Arctic mixed-phase clouds.

How to cite: Sung, H.-J., Lim, K.-S. S., Hong, S.-Y., Shin, J., Kim, B.-M., and Choi, J.-H.: Improved Simulation of Arctic Mixed-Phase Clouds with Modified Ice Microphysics in the WDM6 Scheme, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14507, https://doi.org/10.5194/egusphere-egu25-14507, 2025.

EGU25-14979 | ECS | Posters on site | AS1.14

Orientation dynamics of the ice crystal in a cloud: Effects of Turbulence and Electric Field 

Himanshu Mishra, Pijush Patra, and Anubhab Roy

We investigate the orientation dynamics of an ice crystal in homogeneous isotropic turbulence and in the presence of an external electric field in a cloud. At the scale of the ice crystal, we assume that viscous effects dominate the flow, and thus, the dynamics can be studied in the Stokesian regime. Further, when the size of the ice crystal is smaller than the Kolmogorov scale, the flow field around the particle can be modeled locally as a stochastic linear flow. This approximation becomes particularly useful when studying the orientation dynamics of an ice crystal in homogeneous isotropic turbulence and when the orientation dynamics of the ice crystal is governed by the Jeffery equation, which involves the local fluctuating velocity gradient. The turbulent velocity gradient is obtained from the stochastic model given by Girimaji and Pope. The model uses the log-normal distribution of the pseudo-dissipation rate. In the presence of an external electric field, experiments performed in a laboratory cold chamber have revealed that the ice crystal aligns in the direction of the electric field. We study the competition due to the torque induced by the turbulent velocity gradient and the electric field. The orientation dynamics is analyzed by varying a non-dimensional parameter Σ, which is defined as a ratio of the Kolmogorov time scale and the electric relaxation time scale. For lower values of Σ, we show that the ice crystal exhibits an isotropic orientational distribution, whereas it fluctuates along the direction of the electric field at higher values of Σ. We calculate moments of the orientation distribution at large electric field limits using asymptotic methods and compare them with numerical calculations. A second-order moment in the orientation, which quantifies the fluctuations in the orientation, depends on Σ and the shape of an ice crystal. The fourth-order moment of the orientation, a measure of the non-Gaussian statistics of the orientation distribution, increases from its Gaussian value with the increase in Taylor-scale Reynolds number.

How to cite: Mishra, H., Patra, P., and Roy, A.: Orientation dynamics of the ice crystal in a cloud: Effects of Turbulence and Electric Field, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14979, https://doi.org/10.5194/egusphere-egu25-14979, 2025.

EGU25-15500 | Orals | AS1.14

Does small-scale turbulence matter for ice growth in mixed-phase clouds? 

Bernhard Mehlig, Grigory Sarnitsky, Gaetano Sardina, Gunilla Svensson, Alain Pumir, and Fabian Hoffmann

Representing the glaciation of mixed-phase clouds in terms of the Wegener-Bergeron-Findeisen process is a challenge for many weather and climate models, which tend to overestimate this process because cloud dynamics and microphysics are not accurately represented. As turbulence is essential for the transport of water vapour from evaporating liquid droplets to ice crystals, we developed a statistical model using established closures to assess the role of small-scale turbulence. The model successfully captures results of direct numerical simulations, and we use it to assess the role of small-scale turbulence. We find that small-scale turbulence broadens the droplet-size distribution somewhat, but it does not significantly affect the glaciation time on submetre scales. However, our analysis indicates that  turbulence on larger spatial scales is likely to affect ice growth. While the model must be amended to describe larger scales, the present work facilitates a path forward to understanding the role of turbulence in the Wegener-Bergeron-Findeisen process. This talk is based on  arXiv:2410.06724 which is joint work with G. Sarnitsky, G. Sardina, G. Svensson, A. Pumir, and F. Hoffmann.

How to cite: Mehlig, B., Sarnitsky, G., Sardina, G., Svensson, G., Pumir, A., and Hoffmann, F.: Does small-scale turbulence matter for ice growth in mixed-phase clouds?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15500, https://doi.org/10.5194/egusphere-egu25-15500, 2025.

EGU25-16830 | Orals | AS1.14

Aerosol-Driven Parameterization of Ice Nucleation and Secondary Ice Processes in EC-Earth3: Evaluation and Climate Impacts 

Montserrat Costa-Surós, María Gonçalves, Marios Chatziparaschos, Paraskevi Georgakaki, Stelios Myriokefalitakis, Twan Van Noije, Philippe Le Sager, Maria Kanakidou, Athanasios Nenes, and Carlos Pérez García-Pando

Clouds remain a major source of uncertainty in climate projections, particularly due to complexities in aerosol-cloud interactions. To improve the representation of mixed-phase clouds in EC-Earth3, the model's heterogeneous ice nucleation scheme has been updated. The previous temperature-based parameterization has been replaced with aerosol- and temperature-sensitive immersion freezing schemes for mixed-phase clouds that consider ice-active desert dust minerals (K-feldspar and quartz) and marine organic aerosols, both explicitly tracked in EC-Earth3. Additionally, a secondary ice production scheme based on a random forest regressor further enhances the ice crystal concentrations.

The updated model is evaluated against an extensive observational dataset of ice-nucleating particle (INP) concentrations, satellite observations of cloud properties (MODIS and CALIPSO), and both Top of the Atmosphere (TOA) and surface radiative Cloud Radiative Effect (CRE) flux components from CERES-EBAF. The impact of the updates is analysed relative to the previous temperature dependent parameterization.

Results from 12-year (2009-2020) nudged simulations show improved agreement with INP observations using the updated aerosol-aware scheme compared to the earlier approach. The ice nucleation parameterization clearly links simulated ice crystal number concentrations with aerosol emission sources and transported pathways. Despite remaining biases largely attributed to other processes, this update improves consistency with MODIS and CALIPSO retrieved data, including total cloud cover, low/mid/high cloud area percentages, liquid and ice cloud fractions, and water paths. Sensitivity analyses reveal that the new scheme impacts global cloud cover, liquid and ice water content, temperature, and radiative balances. Evaluation with CERES-EBAF indicates that the new parameterization reduces surface net CRE bias at mid-to-high latitudes while slightly increasing bias at low latitudes, despite no specific model tuning for this configuration.

Our approach offers potential enhancements in future climate projections using EC-Earth3-AerChem and future generations of the model.

How to cite: Costa-Surós, M., Gonçalves, M., Chatziparaschos, M., Georgakaki, P., Myriokefalitakis, S., Van Noije, T., Le Sager, P., Kanakidou, M., Nenes, A., and Pérez García-Pando, C.: Aerosol-Driven Parameterization of Ice Nucleation and Secondary Ice Processes in EC-Earth3: Evaluation and Climate Impacts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16830, https://doi.org/10.5194/egusphere-egu25-16830, 2025.

EGU25-16983 | Posters on site | AS1.14

Global analysis of cirrus origins using satellite observations and Lagrangian trajectories 

Odran Sourdeval, Silvia Bucci, and Athulya Saiprakash

In addition to their formation mechanisms, the origin of cirrus clouds (liquid-origin or in situ) can significantly influence their microphysical and radiative properties. Liquid-origin cirrus, which form through the freezing of water droplets from the mixed-phase region upon reaching cirrus temperatures (below -38°C), are typically characterized by high ice crystal concentrations and are associated with a strong cooling effect. In contrast, in situ-origin cirrus consist of ice crystals that form directly within the cirrus regime via homogeneous or heterogeneous freezing. Large cloud systems often comprise a mixture of both types. However, the global occurrence, distribution, and environmental conditions associated with these cirrus types remain poorly understood.

This study investigates cirrus clouds by integrating satellite observations with reanalysis data. Observations from lidar-radar satellite instruments (DARDAR-Nice) provide detailed retrievals of cirrus microphysical properties, including ice water content and ice crystal number concentration. To trace the origins of cirrus clouds, we employ Lagrangian air mass trajectories based on ERA5 reanalyses, using the FLEXPART Lagrangian model. This analysis is conducted for every satellite retrieval pixel, with a horizontal resolution of 1.7 km and a vertical resolution of 60 m. Environmental conditions at and preceding cirrus formation, as well as those in the mixed-phase regime for liquid-origin cirrus, are examined along the trajectories. Aerosol data from CAMS reanalyses are also included to assess their influence.

A combined cloud-aerosol dataset, derived from satellite observations and reanalysis tools, is compiled for one year of global data. The global occurrence of liquid-origin cirrus is analyzed in relation to ice crystal formation drivers and the resulting microphysical and radiative properties of these clouds, as retrieved by the DARDAR-Nice product. The relative occurence of insitu- and liquid-origin ice in cirrus is also assessed. The role of aerosols in cirrus formation processes will briefly be explored.

How to cite: Sourdeval, O., Bucci, S., and Saiprakash, A.: Global analysis of cirrus origins using satellite observations and Lagrangian trajectories, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16983, https://doi.org/10.5194/egusphere-egu25-16983, 2025.

EGU25-17170 | ECS | Orals | AS1.14

First estimates of Tropical Tropopause Cirrus lifetimes using balloon-borne lidar observations 

Thomas Lesigne, Aurélien Podglajen, and François Ravetta

Tropical tropopause layer (TTL) cirrus clouds play a key role in the Earth climate system, yet the relative role of the various processes shaping them remains poorly known. Characterizing the temporal evolution of cloudy structures from observations is essential to address this issue, but represents a challenge. Indeed, space- and air-borne platform are not well-suited for this task: moving much faster than the air, they only provide instantaneous snapshots. In boreal winter 2021-2022, two balloon-borne lidars flew over the Equatorial Pacific Ocean, slowly drifting above the clouds. We use those unique observations of truncated (nighttime only) lifetime distribution to quantify the underlying continuous distribution of cloud lifetime above this homogeneous region. While most clouds are short-lived (mean lifetime estimated at about 6 h, a median value of 1 h), the temporal cloud cover is still dominated by the few long-lived ones (24 h or more). These results are compared to cirrus lifetimes in ERA5 reanalysis, showing a fair agreement between the reanalysis and the observations, and demonstrating the value of our approach to evaluate cirrus representation in global models.

How to cite: Lesigne, T., Podglajen, A., and Ravetta, F.: First estimates of Tropical Tropopause Cirrus lifetimes using balloon-borne lidar observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17170, https://doi.org/10.5194/egusphere-egu25-17170, 2025.

EGU25-17522 | ECS | Orals | AS1.14

Clouds Decoded: Understanding Mixed-Phase Clouds with High Resolution Multispectral Data 

Alistair Francis, Jacqueline Campbell, and Mikolaj Czerkawski

Clouds and their radiative effects remain one of the most pernicious unknowns in  our predictions of the climate. Climate models are particularly affected by uncertainties around mixed-phase clouds (MPCs) consisting of both super-cooled liquid droplets and ice crystals. Inaccurate measurements of the liquid water content can lead to an under or overestimation of the warming properties of these clouds. Moreover, we lack adequate constraints and parameterisations of the spatial heterogeneity of water/ice mixtures, and the distribution of ice crystal sizes within MPCs. 

Traditional cloud-monitoring satellites are able to retrieve physical cloud properties pertinent to these unknowns via, for example, LIDAR and radar sensors, but must necessarily treat MPCs as homogeneously mixed at scales below their resolution, which is on the order of 100s of metres to kilometres per pixel. Meanwhile, cloudy imagery from multispectral satellites with high spatial resolution, such as Sentinel-2, is treated as a waste product, with the ~60% of cloudy pixels left to gather dust in the archive. Multiple barriers exist that make these multispectral satellites difficult to use for ice cloud property retrievals, including their lack of thermal information, their tendency to mostly observe over land and not the ocean, their infrequent revisit times, and their sun-synchronous orbits which mean they only observe at 10 am local time. Nevertheless, these sensors offer a unique angle from which to study clouds, which can complement existing and future cloud-specialised sensors.

Here, we present early results of the Clouds Decoded project, funded by the Advanced Research + Invention Agency (ARIA), which seeks to help the community to tackle some of the key unknowns related to MPCs and ice clouds. Clouds Decoded aims to retrieve several physical cloud properties including cloud top height, optical depth (for optically thin clouds), ice/water ratio and ice particle effective radius, all at very fine resolution. This is being done at a massive scale, with the goal of processing several hundred terabytes of Sentinel-2 data from across the globe during the project. In this presentation, we will focus on a handful of case-studies which demonstrate how our data can be of use to the community. In particular, statistical relationships between cloud top temperature (inferred from height) and ice properties, alongside spatial frequency analyses, will be leveraged to describe the complex processes occurring in MPCs.

How to cite: Francis, A., Campbell, J., and Czerkawski, M.: Clouds Decoded: Understanding Mixed-Phase Clouds with High Resolution Multispectral Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17522, https://doi.org/10.5194/egusphere-egu25-17522, 2025.

EGU25-17818 | ECS | Posters on site | AS1.14

A lattice Boltzmann method to study light scattering by hydrometeors 

Mohd. Meraj Khan, Sumesh P. Thampi, and Anubhab Roy

We present lattice Boltzmann method (LBM) for simulating light scattering by hydrometeors, addressing the limitations of existing techniques. The accurate modelling of light scattering by hydrometeors, which include raindrops, hailstones, graupel, snowflakes, and ice crystals, is essential for remote sensing, climate modelling, and atmospheric studies. Current methods, such as the Finite-Difference Time-Domain (FDTD) method, are limited by computational cost and accuracy issues, particularly for larger particle sizes; for example, FDTD is generally restricted to size parameters smaller than about 20. This restriction arises from the method's need for fine grid resolution, where the number of numerical operations increases rapidly with particle size, scaling approximately with the fourth power of the size parameter. These limitations make FDTD impractical for many hydrometeor simulations, which often require larger size parameters. The T-matrix method and the Discrete Dipole Approximation (DDA) are alternative approaches, but they, too, have limitations. Therefore, a more efficient and accurate numerical method is needed to overcome these challenges. The LBM aims to overcome these limitations by exploring an alternative numerical approach; the goal is to provide a more computationally efficient and accurate approach. By addressing the computational challenges associated with existing numerical methods, this work enables more realistic and detailed simulations of light scattering by hydrometeors across a wider range of sizes and shapes. This has significant implications for improving remote sensing retrievals of cloud and precipitation properties, as well as advancing our understanding of the role of hydrometeors in the Earth's climate system.

How to cite: Khan, M. M., Thampi, S. P., and Roy, A.: A lattice Boltzmann method to study light scattering by hydrometeors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17818, https://doi.org/10.5194/egusphere-egu25-17818, 2025.

EGU25-18125 | Orals | AS1.14

Visualizing the Spatial Structure of Strong Riming Events using Scanning Cloud Radars 

Paul Ockenfuss, Gregor Köcher, and Stefan Kneifel

The coexistence of liquid water and ice crystals in mixed phase clouds allows for collisions and subsequent freezing of droplets on ice crystals and aggregates, which is called riming. Because riming fills air cavities in aggregates and makes particles more round, rimed snow has a higher fall speed compared to unrimed crystals and aggregates. Therefore, a reliable method to detect riming are fall speed measurements based on the Doppler shift of cloud radar echos. For this, the cloud radar has to be oriented vertically, otherwise the Doppler shift is dominated by the horizontal wind advection of the hydrometeors. Limited to vertical observations, one of the key strengths of atmospheric radar is missing: To probe the atmosphere in 3D. In this contribution, we present the results from a winter measurement campaign, where we performed elevation scans through strong riming events. Assuming a model for the horizontal wind speed, we can remove the horizontal wind contribution from the Doppler signal. This reveals the underlying riming signatures from the measurements, allowing us to create snapshots in time of the actual spatial organization of strongly rimed particles in mixed phase clouds. By choosing the scanning plane into the main wind direction, we are able to track spatial features over multiple snapshots. A better characterization of the spatial picture can enhance our conceptual understanding of the structure and organization of strong riming in mixed phase clouds. Since supercooled liquid water is a precondition for riming and aircraft icing alike, our results could also proof helpful to design aircraft icing hazard warning products.

How to cite: Ockenfuss, P., Köcher, G., and Kneifel, S.: Visualizing the Spatial Structure of Strong Riming Events using Scanning Cloud Radars, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18125, https://doi.org/10.5194/egusphere-egu25-18125, 2025.

EGU25-18152 | Orals | AS1.14

Early Ice Particles in Growing Convective Clouds over a New Mexico Mountain Range during DCMEX 

Gary Lloyd, Alan Blyth, Martin Gallagher, Thomas Choularton, Keith Bower, Kezhen Hu, Benjamin Murray, and Martin Daily

The formation of the first ice particles in developing convective clouds is a critical event in cloud evolution. The timing, location and amount of the initial ice has potentially significant implications for the eventual micro and macro scale properties as the cloud evolves. Here we present in-situ measurements of the first ice particles observed in growing convective clouds during the DCMEX project over the Magdalena mountains in New Mexico, USA. The Facility for Airborne Atmospheric (FAAM) Bae-146 research aircraft was used to make penetrations of the convective clouds below the freezing level, following the cloud top upwards. We used an Optical Array probe with a large sample volume suitable for detecting the earliest ice particles as they developed. We often observed no ice particles initially at only slightly supercooled temperatures before the eventual appearance of small irregular ice particles in low concentrations around the -8°C level. We will present the characteristics of the particles observed and compare their concentrations with Ice Nucleating Particle (INP) data analysed during the same project.

How to cite: Lloyd, G., Blyth, A., Gallagher, M., Choularton, T., Bower, K., Hu, K., Murray, B., and Daily, M.: Early Ice Particles in Growing Convective Clouds over a New Mexico Mountain Range during DCMEX, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18152, https://doi.org/10.5194/egusphere-egu25-18152, 2025.

EGU25-18946 | ECS | Posters on site | AS1.14

How does the change from sea ice to open ocean alter Arctic mixed-phase clouds? 

Nina Elisabeth Larsgård, Rob O. David, Tim Carlsen, Alfons Schwarzenboeck, Harald Sodemann, and Trude Storelvmo

Mixed-phase clouds consist of both liquid water and ice crystals, which affect their radiative properties. The amount of ice in the clouds is also important for the formation of precipitation and the lifetime of the clouds. Mixed-phase clouds are abundant in the Arctic, which through Arctic amplification is experiencing the largest and fastest changes in climate. Clouds, including Mixed-phase clouds, remain one of the biggest causes of uncertainty in climate models. The clouds' radiative effects depend on the composition, location, amount, and longevity of the clouds, which are complex properties both to measure and to model.

So how will the Arctic mixed-phase clouds change in a warming world? We expect warmer temperatures to lead to more liquid clouds, with smaller and more abundant cloud particles and thereby more reflective clouds. Ultimately resulting in surface cooling (temperature effect). However, increased warming also leads to a decrease in sea ice. Less sea ice will lead to changes in the available aerosols, making more locally emitted aerosols available to act as ice-nucleating particles (INPs), possibly resulting in ice forming at higher temperatures. Less sea ice can then lead to more ice in the clouds, resulting in less reflective clouds and surface warming (aerosol effect). 

The focus of this study is to investigate the changes in microphysical properties of the mixed-phase clouds over different surface conditions: How do the microphysical properties change as the sea ice disappears?

Aircraft measurements from the spring 2022 field campaign of the Isotopic Links to Atmospheric water's Sources (ISLAS) project are used to investigate the microphysical properties of Arctic mixed-phase clouds during Cold Air Outbreaks. These Cold air outbreaks act like a natural laboratory, which makes them ideal for studying the effect of the clouds from the same airmass over different surfaces such as sea ice and open ocean. 

The ISLAS flights from April 3rd, 2022 passed over both sea ice and open ocean and are used as a case study. We focus on cloud microphysical properties such as cloud droplet number concentration, size distribution, and the supercooled liquid fraction (SLF: liquid water content/ total water content), measured by in-situ cloud probes. We compare the results for the clouds encountered over sea ice vs. over open ocean, and at different heights within the clouds. Whether or not we see any differences for the clouds above sea ice vs. open ocean indicates which of the two processes, the temperature effect or the aerosol effect, dominates as the sea ice disappears in a warming climate.

How to cite: Larsgård, N. E., David, R. O., Carlsen, T., Schwarzenboeck, A., Sodemann, H., and Storelvmo, T.: How does the change from sea ice to open ocean alter Arctic mixed-phase clouds?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18946, https://doi.org/10.5194/egusphere-egu25-18946, 2025.

EGU25-18983 | ECS | Posters on site | AS1.14

Investigating ice formation pathways in satellite-observed cirrus clouds using Lagrangian microphysical modelling 

Athulya Saiprakash, Martina Krämer, Christian Rolf, Patrick Konjari, Jérôme Riedi, and Odran Sourdeval

Understanding the formation mechanisms of ice clouds is challenging due to their complex composition and diverse growth processes. Observational constraints have historically been limited, resulting in significant gaps in our understanding and representation of ice clouds. Satellite measurements are particularly limited by the absence of critical environmental context information needed to identify cloud formation mechanisms and evolution. These observations provide only a snapshot of cloud states and their microphysical properties at a single moment. This study seeks to overcome these limitations by incorporating additional metrics on ice cloud history and origin alongside operational satellite products.

We introduce a novel framework that combines satellite observations with Lagrangian transport and ice microphysical modelling to provide insights into the history and origin of air parcels contributing to ice cloud formation. The Chemical LAgrangian Model of the Stratosphere (CLaMS) is employed to trace air parcel trajectories along the DARDAR-Nice track. Additionally, the CLaMS-Ice model is used to simulate cirrus clouds along these trajectories, offering metrics on cirrus age, origin (in situ vs. liquid-origin), and ice formation pathways (heterogeneous vs. homogeneous nucleation) that can be associated with satellite observations.

To illustrate this approach, we present three case studies representative of distinct mid-latitude synoptic conditions: fast updraft, slow updraft, and orographically driven ice clouds. These cases demonstrate an in-depth analysis of air parcel evolution since cirrus formation, followed by a statistical examination of the relationship between microphysical properties and the origin-based metrics. Furthermore, the method is evaluated by comparing modeled microphysics with satellite retrievals. A sensitivity analysis is conducted to assess the impact of input parameters in CLaMS-Ice, including small-scale temperature fluctuations, environmental ice-nucleating particle (INP) concentrations, and sedimentation parameterizations. Overall, this comprehensive approach enhances our understanding of ice cloud processes, provides valuable context for interpreting satellite observations, and contributes to refining the representation of cirrus clouds in atmospheric models.

How to cite: Saiprakash, A., Krämer, M., Rolf, C., Konjari, P., Riedi, J., and Sourdeval, O.: Investigating ice formation pathways in satellite-observed cirrus clouds using Lagrangian microphysical modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18983, https://doi.org/10.5194/egusphere-egu25-18983, 2025.

EGU25-19056 | Posters on site | AS1.14

Early results from EarthCARE cloud microphysics and Doppler Velocity products 

Kaori Sato and Hajime Okamoto

This paper introduces the early results obtained from the active sensor-based EarthCARE JAXA Level 2 cloud and precipitation microphysics products (Sato et al., 2024, Sato and Okamoto, 2023). In the microphysics retrievals, a maximum of two size modes in each vertical grid are considered to treat coexistence of cloud liquid particles and ice/snow in the mixed phase, transition from cloud ice to snow and cloud liquid to precipitation in the ice phase and liquid phase, respectively. Ice and snow are classified into five different habit categories, and their vertical resolved geographical distributions are investigated together with their microphysical properties, Doppler velocity-related products such as hydrometeor fall speeds and air vertical velocities, and environmental conditions.

How to cite: Sato, K. and Okamoto, H.: Early results from EarthCARE cloud microphysics and Doppler Velocity products, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19056, https://doi.org/10.5194/egusphere-egu25-19056, 2025.

EGU25-20471 | Orals | AS1.14

An Overview of the Cold-Air outbrEaks over the Sub-Arctic Region (CAESAR) campaign 

Paquita Zuidema, Bart Geerts, and Greg McFarquhar

In the spring of 2024, the US National Science Foundation sponsored the Cold-Air outbrEaks in the Sub-Arctic Region (CAESAR) aircraft campaign, with the simple goal of characterizing cold-air outbreak (CAO) clouds coming off of the Arctic sea ice as comprehensively as possible. A strength of the CAESAR strategy is a comprehensive aerosol, cloud and remote sensing instrumentation suite and early development of a close connection to modeling spanning a range of scales, in part by building on prior DOE-sponsored activity through the Cold-Air Outbreaks in the Marine Boundary Layer (COMBLE) campaign. The higher-level motivation for CAESAR is to better understand how clouds participate and feedback upon the changing Arctic. New technologies, improved data integration and modeling frameworks that are increasingly comparable to the observations hold promise that both the numerical weather prediction and  global modeling of the super-cooled liquid, mixed-phase and ice clouds can be improved through the focus provided by the field campaign. In this presentation we provide an overview of the NCAR C-130 aircraft campaign, and its approach to the problem of improving understanding of the cold-air outbreak cloud evolution, microphysical processes including their relationship to aerosol, and cloud mesoscale organization including the development of CAO clouds into polar lows. Initial highlights will be included.

How to cite: Zuidema, P., Geerts, B., and McFarquhar, G.: An Overview of the Cold-Air outbrEaks over the Sub-Arctic Region (CAESAR) campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20471, https://doi.org/10.5194/egusphere-egu25-20471, 2025.

EGU25-20620 | Posters on site | AS1.14

Dominant microphysical processes for mixed-phase clouds across climate models 

Luisa Ickes, Hannah Frostenberg, Montserrat Costa Surós, Paraskevi Georgakaki, Ulrike Proske, Georgia Sotiropoulou, Eleanor May, Maria Gonçalves Ageitos, Patrick Eriksson, Anna Lewinschall, Athanasios Nenes, David Neubauer, Carlos Pérez García-Pando, and Øyvind Sedland

Global climate models poorly represent mixed-phase clouds in a realistic way, which leads to uncertainties in cloud radiative forcing and precipitation. In the FORCeS ice experiment (FOR-ICE) we compare three global climate models (ECHAM-HAM, NorESM, EC-Earth) and show which processes are crucial for a realistic representation of cloud ice and supercooled water in each global climate model framework using the factorial method as a statistical approach. A specific focus of the experiments is on secondary ice production (SIP) - which apart from one mechanism (rime splintering) is not represented in models, even if observations of ice crystal concentrations of ice crystal number in warm mixed-phase clouds often exceed available ice nuclei by orders of magnitude. We evaluate the importance of three SIP mechanisms combined (rime splintering, ice-ice collisions, and droplet shattering) compared to all other processes that can modulate ice mass and number in mixed-phase clouds: ice nucleation, sedimentation, and transport of ice crystals. Satellite observations are used to evaluate the representation of mixed-phase clouds. We found large discrepancies in dominant microphysical processes for mixed-phase clouds across the investigated climate models.

How to cite: Ickes, L., Frostenberg, H., Costa Surós, M., Georgakaki, P., Proske, U., Sotiropoulou, G., May, E., Gonçalves Ageitos, M., Eriksson, P., Lewinschall, A., Nenes, A., Neubauer, D., Pérez García-Pando, C., and Sedland, Ø.: Dominant microphysical processes for mixed-phase clouds across climate models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20620, https://doi.org/10.5194/egusphere-egu25-20620, 2025.

Terrestrial gamma-ray flashes (TGFs) are bursts of energetic X- and gamma-rays which are emitted from thunderstorms as the Bremsstrahlung radiation of relativistic electrons. Recently, the ALOFT (Airborne Lightning Observatory for FEGS and TGFs) mission has shown that the emission of such energetic radiation, also including gamma-ray glows and flickering gamma-ray flashes, is more abundant than previously thought. This raises the question how the relativistic electrons and photons interact with the atmosphere and whether they have an impact on the chemical composition while propagating through the atmosphere, potentially relevant for the production of greenhouse gases. The propagation and interaction of relativistic particles with the atmosphere can be studied with particle Monte Carlo collision models requiring cross sections as an input. Whilst there are well established data for photoionization, Compton scattering and pair production, we lack cross sections for photoexcitation, photodissociation or the excitation of air molecules through relativistic electrons which contribute to the chemical activation of the atmosphere. In order to fill this gap of data, we here present a novel numerical tool calculating cross sections for energetic particles propagating in air. We provide an overview of the code structure and present benchmarking cases against well-known cross sections. Additionally, we will present a first application by calculating cross sections for photodissociation for a wide range of energies. In the end, we will give an outlook how this will allow to pave the path for more realistic simulations of energetic phenomena in our atmosphere, relevant for chemical processes.

How to cite: Köhn, C. and van Gemert, H.: Towards the investigation of chemical effects of energetic electrons and photons in the atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1217, https://doi.org/10.5194/egusphere-egu25-1217, 2025.

EGU25-1630 | Posters on site | NH1.6

On the influence of lightning distance on the atmospheric electric field 

Konstantinos Kourtidis, Athanassios Karagioras, Ioannis Kosmadakis, and Vassiliki Kotroni

The influence of lightning on the atmospheric electric field (potential gradient, PG) is examined at Xanthi, NE Greece. The data span one year, 01/06/2011 - 31/05/2012. The influence of lightning distance on PG is large, and is evident up to distances of 50 km. At distances shorter than 1 km, the 1-min absolute PG values mean increase is 10 kV/m, while 1-sec values may increase above 20 kV/m for lightning distances below 10 km. It appears that PG increases linearly with decreasing lightning distance. Lightning can cause both positive and negative PG values. It is found that negative PG values increase faster than positive ones as the lightning distance decreases, and mean negative values are at any distance up to 50 km 20% higher than the mean positive ones. It is also examined how synoptic weather types influence lightning frequency and PG values. Circulation Weather Types (CWT) that produce more lightning near Xanthi are ones associated with high 500 hPa geopotential heights over the area and high thickness of the 850-500 hPa isobaric surfaces. Thgey are encountered predominantly during summer, and to a lower extend during spring and autumn. During such systems, when lightning was detected at distances shorter than 100 km from the site, the mean absolute values of PG were 1-1.2 kV/m.

How to cite: Kourtidis, K., Karagioras, A., Kosmadakis, I., and Kotroni, V.: On the influence of lightning distance on the atmospheric electric field, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1630, https://doi.org/10.5194/egusphere-egu25-1630, 2025.

The appearance of transient luminous events (TLEs) in the mesosphere is known to be associated with strong (almost exclusively) positive cloud-to-ground (+CG) strokes with large charge moment change (CMC) values in tropospheric thunderstorms. Nevertheless, despite numerous observational campaigns from ground and space-based platforms, robust theoretical models, and laboratory experiments, there are lingering open questions concerning the exact circumstances for the appearance of sprites, among which is the cause for the observed delay in sprite appearance relative to the onset of the current in the parent stroke. Curiously, seemingly identical +CG discharges with the same CMC that should lead to a mesospheric discharge do not initiate sprites, while sometimes even weaker +CG discharges are able to do so. Previous studies aiming to resolve this issue have investigated different effects, such as mesospheric inhomogeneities, the presence of meteoritic ablation products, discharges in neighboring cloud cells, associative detachment of electrons from atomic oxygen ions, and long continuing currents. Here, we investigate the properties of the parent +CG's continuing current by suggesting piecewise-varying discharge time dependence. We present the results of simulations using a 3D quasi-electrostatic model (Haspel and Yair, 2024) with various patterns of the parent flash discharge current. We show how short, moderate, and long delayed sprites can be incepted due to piecewise-varying discharge current time dependence, and how discharges possessing low iCMC values can still produce electric fields in the mesosphere with magnitudes above the conventional electrical breakdown field. The model is validated by simulating two sprite events observed from the International Space Station during the ILAN-ES campaigns in April 2022 (on AX-1) and February 2024 (on AX-3), showing how a delayed sprite is incepted by a prolonged piecewise pattern of the current in the parent +CG flash.

 

Haspel, C. and Y. Yair (2024), Numerical Simulations of the region of possible sprite inception in the mesosphere above winter thunderstorms under windshear. Ad. Spa. Res.., 74, 11, 5548-4468, doi:10.1016/j.asr.2024.08.050

How to cite: Yair, Y. and Haspel, C.: Simulating the possible regions of delayed sprite inception above thunderstorms using piecewise-varying lightning current time dependence , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2357, https://doi.org/10.5194/egusphere-egu25-2357, 2025.

EGU25-3614 | ECS | Orals | NH1.6

Enhancing Lightning Resilience: Predictive Models and Infrastructure Protection for UK Electric Power Systems 

Xue Bai, Xinyuan He, Martin Fullekrug, Chenghong Gu, Mingyi Xu, Bohan Li, Laiz Souto, Tinashe Chikohora, and Douglas Dodds

The UK’s goal of achieving net zero emissions by 2050 requires the construction of extensive new power infrastructure to accommodate low carbon energy technologies (e.g., offshore wind, nuclear) while mitigating climate risks. Lightning activity poses severe risks to power system security and can result in significant economic losses (Ofgem, 2019; Bialek, 2020). These risks must be mitigated as effectively as possible as new power grid infrastructure is built in the coming years and climate scenarios.

To represent lightning activity, this study employs a newly developed thunder hour dataset from Earth Networks, with a spatial resolution of approximately 5.5 km, specifically designed for climate research (DiGangi et al., 2022). Ten years of monthly historical UK thunder hour data from Earth Networks are analysed to identify lightning climatology trends and support the development of a long-term predictive lightning model. This study differentiates itself from previous UK lightning research by focusing directly on lightning risks impacting the UK’s power grid infrastructure, aiming to offer actionable insights for risk mitigation during the planning of future power assets for National Grid Electricity Transmission (NGET).

Historical lightning damage hotspots are identified by linking power system fault records with spatiotemporal lightning activity characteristics such as peak current and lightning duration from lightning detection and location networks. Analysing lightning activity’s impact on power system line trippings helps improve the grid’s reliability and safety (Li et al., 2024). The novelty of this research lies in its integration of lightning hotspot analysis, informed by lightning climatology trends, with asset distribution to pinpoint high-risk areas for electrical infrastructure, validated through power system failure case studies. These findings offer a basis for improved disaster prevention and mitigation strategies, enhancing grid resilience and safety.

 

Acknowledgement:

The authors acknowledge the support for the KERAUNIC project (ref: NIA2_NGET0055, National Grid Electricity Transmission, 2024), which focuses on improving the understanding of lightning-induced damage to UK power systems. This research is part of an innovation effort funded through the Network Innovation Allowance (NIA).

References:

Bialek, J. (2020). What does the GB power outage on 9 August 2019 tell us about the current state of decarbonised power systems? Energy Policy, 146, 111821.

DiGangi, E., Stock, M., & Lapierre, J. (2022). Thunder Hours: How Old Methods Offer New Insights into Thunderstorm Climatology. Bulletin of the American Meteorological Society, 103, E548-E569. https://doi.org/10.1175/BAMS-D-20-0198.1.

Li, M., Cheng, S., Wang, J., Cai, L., Fan, Y., Cao, J., & Zhou, M. (2024). Thunderstorm total lightning activity behaviour associated with transmission line trip events of power systems. npj Climate and Atmospheric Science, 7(1), 148.

National Grid Electricity Transmission. (2024). Knowledge Elicitation of Risks to Assets Under LightNing Impulse Conditions (KERAUnIC). https://smarter.energynetworks.org/projects/nia2_nget0055/.

Ofgem. (2019). Investigation into 9 August 2019 Power Outage. Retrieved from https://www.ofgem.gov.uk/publications/investigation-9-august-2019-power-outage.

How to cite: Bai, X., He, X., Fullekrug, M., Gu, C., Xu, M., Li, B., Souto, L., Chikohora, T., and Dodds, D.: Enhancing Lightning Resilience: Predictive Models and Infrastructure Protection for UK Electric Power Systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3614, https://doi.org/10.5194/egusphere-egu25-3614, 2025.

EGU25-4072 | Orals | NH1.6

Upcoming broadband electromagnetic balloon measurements related to terrestrial gamma ray flashes and gamma glows  

Ivana Kolmasova, Ondrej Santolik, Sébastien Celestin, Eric Defer, and Radek Lan

Thunderclouds and lightning produce high-energy radiation over a wide range of time scales. Terrestrial gamma-ray flashes (TGFs) are brief emissions lasting ~100 µs, consisting of photons with energies ranging from 20 keV to 40 MeV. Simultaneous ground-based measurements of electromagnetic fields and gamma-ray emissions have found TGFs to be associated with the evolutionary phases of both intracloud and cloud-to-ground lightning discharges.

Gamma-ray glows, on the other hand, last from a few seconds to several tens of minutes, typically coincide with the passage of thunderclouds, and are sometimes abruptly terminated by nearby lightning. Photons emitted during gamma-ray glows share the same energy spectrum as TGFs but are less intense. It was recently discovered that thundercloud regions can glow for hours and that gamma glows are more dynamic phenomena than originally thought.

Both types of gamma-ray emissions are believed to be generated via bremsstrahlung by energetic runaway electrons accelerated in the strong electric fields within thunderclouds. However, the connection between TGFs and gamma-ray glows remains not fully understood.

Until now, the only simultaneous gamma ray and radio wave measurements were conducted onboard an airplane during the ALOFT campaign. The TARANIS mission, which was intended to carry a unique set of electromagnetic, particle, gamma ray, and optical instruments, was unfortunately lost due to the failure of the Vega launcher in 2020.

The STRATELEC balloon project (part of the French-US STRATEOLE-2 project of long-duration balloon flights at the tropical tropopause), with precise synchronization of broadband electric field measurements and a gamma-ray detector, will provide a unique opportunity to correlate individual photon detections with electromagnetic pulses emitted by various lightning processes. These coordinated measurements could help answer the following questions:

  • a) At which stage of the evolution of lightning discharges are TGFs produced?
  • b) Which types of intracloud discharges produce detectable high-energy radiation?
  • c) What are the differences in the electromagnetic signatures of lightning processes associated with TGFs and gamma glows?
  • d) What are the temporal variations in electromagnetic emissions associated with gamma glows?
  • e) Are flickering TGFs truly radio silent?

In this presentation, we introduce the FPGA-based radio receiver RIP (Radio Instrument Package), developed for the STRATELEC balloon project. The receiver is designed to capture and analyze the electromagnetic signatures of various lightning phenomena associated with gamma-ray production, including leader pulses, initial breakdown pulses, compact intracloud discharges, and dart-stepped leader pulses. The anticipated launch is late 2026.

How to cite: Kolmasova, I., Santolik, O., Celestin, S., Defer, E., and Lan, R.: Upcoming broadband electromagnetic balloon measurements related to terrestrial gamma ray flashes and gamma glows , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4072, https://doi.org/10.5194/egusphere-egu25-4072, 2025.

EGU25-4688 | ECS | Posters on site | NH1.6

Correction of Parallax Shift Effect Based on Cloud Top Height for FY-4A LMI 

Yuansheng Zhang, Xiushu Qie, Dongjie Cao, Jing Yang, and Dongfang Wang

The Lightning Mapping Imager (LMI) onboard the Fengyun-4A (FY-4A) satellite is the first independently developed satellite-borne lightning imager in China. It enables continuous lightning detection in China and surrounding areas, regardless of weather conditions. The FY-4A LMI uses a Charge-Coupled Device (CCD) array for lightning detection, and the accuracy of lightning positioning is influenced by cloud top height (CTH). In this study, we proposed an ellipsoid CTH parallax correction (ECPC) model for lightning positioning applicable to FY-4A LMI. The model utilizes CTH data from the Advanced Geosynchronous Radiation Imager (AGRI) on FY-4A to correct the light-ning positioning data. According to the model, when the CTH is 12 km, the maximum deviation in lightning positioning caused by CTH in Beijing is approximately 0.1177° in the east–west direction and 0.0530° in the north–south direction, corresponding to a horizontal deviation of 13.1558 km, which exceeds the size of a single ground detection unit of the geostationary satellite lightning imager. Therefore, it is necessary to be corrected. A comparison with data from the Beijing Broadband Lightning Network (BLNET) and radar data shows that the corrected LMI data exhibit spatial distribution that is closer to the simultaneous BLNET lightning positioning data. The coordinate differences between the two datasets are significantly reduced, indicating higher consistency with radar data. The correction algorithm decreases the LMI lightning location deviation caused by CTH, thereby improving the accuracy and reliability of satellite lightning positioning data. The proposed ECPC model can be used for the real-time correction of lightning data when CTH is obtained at the same time, and it can be also used for the post-correction of space-based lightning detection with other cloud top height data.

How to cite: Zhang, Y., Qie, X., Cao, D., Yang, J., and Wang, D.: Correction of Parallax Shift Effect Based on Cloud Top Height for FY-4A LMI, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4688, https://doi.org/10.5194/egusphere-egu25-4688, 2025.

EGU25-4814 | Posters on site | NH1.6

The STRATELEC (STRatéole-2 ATmospheric ELECtricity) project 

Eric Defer, Serge Soula, Sébastien Célestin, Yanis Hazem, François Trompier, Ivana Kolmašová, Ondrej Santolík, Radek Lán, Jean-Jacques Berthelier, Elena Seran, Michel Godefroy, Albert Hertzog, and Stéphanie Venel

About 45 lightning flashes occur per second all around the Earth with a predominant distribution over the continents and along the inter-tropical band. While different types of Transient Luminous Events (TLEs) induced by lightning flashes can be produced above the thunderstorms, Terrestrial Gamma Ray Flashes (TGFs) are bursts of high-energy photons originating from the Earth’s atmosphere in association with thunderstorm activity with a great majority of TGFs occurring in the inter-tropical region. In addition to those radiation bursts, another type of high-energy emission, so-called gamma ray glows, has been observed inside thunderstorms corresponding to significant enhancements of background radiation that last for more than a few seconds. All these connected phenomena remain to be documented both remotely and on an in-situ manner. Balloon-borne missions offer the required in-situ close-range high-altitude measurements of the ambient electrostatic field, conductivity, TGF radiation and lightning occurrence for a better understanding and modeling of these complex phenomena and of their effects on the Earth atmosphere and the global atmospheric electrical circuit.

The STRATELEC (STRatéole-2 ATmospheric ELECtricity) project (Defer et al., 2022), funded by CNES, aims at deploying within the Stratéole-2 framework (Hertzog and Plougonven, 2020) new atmospheric electricity instrumentation on several stratospheric balloons to:

  • Document the electrical state of the atmosphere and the production of high-energy radiation through in-situ and remote sensing measurements to reach better understanding and better modeling capabilities of the processes occurring during thunderstorms,
  • Identify state-of-the-art and emerging technologies to populate the STRATELEC instrumentation package with new sensors in the perspective of their operation on stratospheric balloons, high altitude aircraft and even low-level drones to eventually propose new balloon and/or space mission concepts,
  • Contribute to additional scientific returns on any space mission dedicated to lightning detection (e.g. MTG-LI, GOES-GLM) and more generally to the study of the convection in the Tropics and of electrodynamic couplings in the terrestrial atmosphere-ionosphere-magnetosphere system.

First, we will remind the scientific objectives of the STRATELEC project. Then we will provide an update on the different scientific and technical activities, including the development and the testing of STRATELEC instruments, but also the data analysis méthodology. Finally, we will discuss the way forward for the upcoming and final Stratéole-2 campaign (winter 2026-2027), as well as some initial thoughts on future balloon campaigns.

 

Hertzog A., and R. Plougonven (2020), Stratéole-2 : des ballons longue durée pour étudier la tropopause tropicale, La Météorologie - n° 108 - février 2020.

Defer, E., et al. (2022), An Overview of the STRATELEC (STRatéole-2 ATmospheric ELECtricity) Project, 25th ESA Symposium on European Rocket and Balloon Programmes and Related Research, 1-5 May 2022, Biarritz, France.

 

How to cite: Defer, E., Soula, S., Célestin, S., Hazem, Y., Trompier, F., Kolmašová, I., Santolík, O., Lán, R., Berthelier, J.-J., Seran, E., Godefroy, M., Hertzog, A., and Venel, S.: The STRATELEC (STRatéole-2 ATmospheric ELECtricity) project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4814, https://doi.org/10.5194/egusphere-egu25-4814, 2025.

EGU25-5416 | ECS | Posters on site | NH1.6

Lightning statistics and spatial distribution in South Korea in 2023 

Kyeongyeon Ko, Sunwoo Chu, Kyung-Yeub Nam, and Kwang-Ho Kim

An analysis of lightning strike statistics and spatial distributions in South Korea was conducted throughout 2023 to archive records and to support weather research through the use of radar data. The annual lightning strikes reached 73,341, demonstrating a twofold increase from 36,750 in the previous year but still below the 10-year (2014-2023) average of 93,380. Temporal analysis shows summer recorded the highest number of lightning strikes at 55,258, accounting for 75.35% of annual occurrences, a pattern consistent with the 10-year average. June, October, and December exhibited higher strikes than the 10-year average, while February, March, and August showed significantly lower activity. Spatial distribution examination identified Gyeongsangbuk-do as the dominant region with 12,892 strikes constituting 17.58% of the total. In contrast, Daejeon Metropolitan City recorded the lowest count with 270 strikes, equivalent to 0.37%. The grid investigation revealed high activity zones over the West Sea and around Seoul and Busan, representing increased strikes compared to the 10-year average. Ground-to-cloud discharges prevailed, with high intensities recorded over the South Sea relative to other regions. The five days with the highest number of lightning strikes were identified as 27 June, 11 July, 12 July, 26 July, and 26 October, followed by an analysis of regional strike distribution for each date. This study contributes to an improved understanding of lightning climatology in South Korea, enhancing meteorological forecasting capabilities.

This research was supported by the "Development of radar based severe weather monitoring technology (KMA2021-03121)" of "Development of integrated application technology for Korea weather radar" project funded by the Weather Radar Center, Korea Meteorological Administration.

How to cite: Ko, K., Chu, S., Nam, K.-Y., and Kim, K.-H.: Lightning statistics and spatial distribution in South Korea in 2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5416, https://doi.org/10.5194/egusphere-egu25-5416, 2025.

EGU25-5624 | ECS | Posters on site | NH1.6

Characterizing continuing current lightning using multi instrument observations 

Pablo Antonio Camino-Faillace, Francisco José Gordillo-Vazquez, Francisco Javier Pérez-Invernón, Joan Montanya, Janusz Mlynarczyk, Neubert Torsten, Olivier Chanrion, and Nikolai Østgaard

Lightning flashes with continuing current (CC) are a type of cloud-to-ground (CG) flash that pose significant risks, including air quality degradation, damage to electrical systems and the igniting of wildfires.  Understanding CC lightning is important for mitigating its effects and assessing its potential connection to climate change.

In this study, we used a combination of space-based instruments (ASIM and GLM) and ground-based networks (ENTLN and ELF) to systematically identify CC lightning across the Contiguous United States (CONUS) from June 1, 2018, to December 31, 2021.

ASIM, aboard the International Space Station, provides high-resolution optical measurements at dual wavelengths (337.0 nm and 777.4 nm), while GLM offers continuous geostationary monitoring of optical emissions at 777 nm. Ground-based systems like ENTLN and ELF provide complementary radio data.

We utilized two distinct methods to classify lightning flashes as CC or no CC. The first relied on the predictive models of Fairman and Bitzer (2022), based on the optical signal of GLM, while the second utilized a metric derived from Extreme Low Frequency (ELF) magnetic signals.

We found clear differences between optical properties in ASIM dual-wavelength (337.0~nm, 777.4~nm) light curves associated with CC and no CC lightning, indicating potential for identifying CC flashes using ASIM optical recordings.

Results reveal optical and electromagnetic differences between CC and no CC lightning. First, CC flashes have longer-lasting optical emissions, higher power densities, and elevated total energy levels compared to no CC flashes. Second, the processed ELF radio signal can sense the presence of CC and the electrical polarity of lightning flashes. These findings highlight the value of combining space-based optical and ground-based ELF measurements to improve detection and classification of CC lightning.

How to cite: Camino-Faillace, P. A., Gordillo-Vazquez, F. J., Pérez-Invernón, F. J., Montanya, J., Mlynarczyk, J., Torsten, N., Chanrion, O., and Østgaard, N.: Characterizing continuing current lightning using multi instrument observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5624, https://doi.org/10.5194/egusphere-egu25-5624, 2025.

EGU25-5745 | Orals | NH1.6

Search for in situ signatures of electric activity on Mars 

Baptiste Chide, Ralph Lorenz, Franck Montmessin, Sylvestre Maurice, Yann Parot, Ricardo Hueso, German Martinez, Alvaro de Vicente-Retortillo, Xavier Jacob, Mark Lemmon, Bruno Dubois, Pierre-Yves Meslin, Claire Newman, Tanguy Bertrand, Agnès Cousin, and Roger Wiens

Electrical discharges such as lightning are among the most energetic and remarkable phenomena in planetary atmospheres. Both laboratory experiments and modeling studies have predicted that triboelectric charging of wind-blown particles in dust events on Mars should lead to significant electrification. However, there have been no direct measurements of a Martian electric field or observations of discharges. Here, using acoustic recordings from the SuperCam microphone onboard the Perseverance rover, we report evidence for an atmospheric discharge in a dust devil, based on the electromagnetic and acoustic signatures observed in the microphone signal. This is the first direct detection of a triboelectric discharge in the Mars atmosphere. It shows that the electric field in a dust devil can reach 25 kV/m, which is the expected breakdown threshold of the Mars atmosphere. Electrical discharges on Mars may have implications for dust dynamics, the chemistry of oxidants and methane in the atmosphere, and ultimately robotic and human exploration.

How to cite: Chide, B., Lorenz, R., Montmessin, F., Maurice, S., Parot, Y., Hueso, R., Martinez, G., de Vicente-Retortillo, A., Jacob, X., Lemmon, M., Dubois, B., Meslin, P.-Y., Newman, C., Bertrand, T., Cousin, A., and Wiens, R.: Search for in situ signatures of electric activity on Mars, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5745, https://doi.org/10.5194/egusphere-egu25-5745, 2025.

EGU25-5799 | Orals | NH1.6 | Highlight

Characterisation and localisation of lightning by a flotilla of stratospheric balloons. 

Thomas Farges, Gael Burgos, Daniel C. Bowman, Olaf Gainville, Sarah A. Albert, and Alexis Le Pichon

On 3 August 2021, Sandia launched a flotilla of four Heliotrope solar hot air balloons (Bowman et al., 2020) from Belen regional airport in New Mexico (USA) to coincide with the launch of the Boeing Starliner rocket. These Heliotrope balloons allow level flights between 15 and 25 km altitude for several hours from sunrise to sunset. Despite the cancellation of the rocket launch, the microbarometers on board these balloons were able to record in the stratosphere the acoustic signals emitted by eight chemical explosions and the lightning that occurred in a thunderstorm cell. This storm cell was located between 10 and 40 km from three of the four balloons.

In this presentation, we first identify the individual signals that may be due to lightning. For this we use the method proposed by Farges and Blanc (2010) for ground-based thunder measurements and by Lamb et al. (2018) for the first stratospheric balloon lightning measurements. Signal analysis has enabled us to (i) confirm that the acoustic energy of thunder decreases as the inverse square of the distance, and (ii) identify that the electrostatic mechanism of thunder production in the infrasonic range (Wilson, 1921; Dessler, 1973; Pasko, 2009) is indeed present when the observer is located just above or just below the thundercloud. One of the balloons was equipped with two microbarometers separated vertically by around 30 m. The time difference between the two microbarometers for the arrival of signals from a flash of lightning is characteristic of the angle of incidence of the wave. It can be seen that this time difference evolves as expected as the balloon moves away from the storm cell.

Finally, we show for the first time that with a network of three sensors located in the stratosphere, it is possible to give a 3D localization of the first arrival of lightning signals. An equivalent acoustic source inside the cloud is clearly identified when the discharge is of the intranuage type, whereas the acoustic source is located between the ground and the cloud when the discharge is of the cloud-to-ground type.

SNL is managed and operated by NTESS under DOE NNSA contract DE-NA0003525.

How to cite: Farges, T., Burgos, G., Bowman, D. C., Gainville, O., Albert, S. A., and Le Pichon, A.: Characterisation and localisation of lightning by a flotilla of stratospheric balloons., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5799, https://doi.org/10.5194/egusphere-egu25-5799, 2025.

EGU25-5994 | Posters on site | NH1.6

UHU - another experiment to observe lightning and TLEs from the ISS 

József Bór, Yoav Yair, Tibor Hegedüs, and Zoltán Jäger

Several successful attempts have been made so far to utilize the uninterrupted view on the atmosphere from space and discover yet undocumented features of lightning activity and transient luminous events (TLEs), most recently THOR and ILAN-ES (2022-2024). As Hungary is considering sending an astronaut to the International Space Station (ISS) in 2025, an experiment has been proposed that aims at further enriching the existing set of space-borne targeted observations of nighttime electrical phenomena in the atmosphere. This is to be accomplished by an optical camera which is directed to preselected thunderstorm targets by the astronaut. This would be the UHU experiment which has been named after the Eurasian eagle-owl, a nighttime predator bird known for its extremely silent flight and exceptionally sharp eyes. The experiment is planned to be supported by a ground-based global observation and data collection campaign. One utterly desired achievement of the experiment and the accompanying observation campaign would be obtaining optical records of one or more TLEs taken simultaneously from the ISS and from a ground location. The experiment would also serve to elevate public awareness about the benefits of monitoring atmospheric electric parameters in studying the atmosphere and the near-Earth space environment. In this contribution, the motivation and the scientific aims behind organizing yet another TLE observation experiment from the ISS are presented and planning of the experiment as well as the supporting observation campaign are described.

How to cite: Bór, J., Yair, Y., Hegedüs, T., and Jäger, Z.: UHU - another experiment to observe lightning and TLEs from the ISS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5994, https://doi.org/10.5194/egusphere-egu25-5994, 2025.

EGU25-6249 | Orals | NH1.6

Electromagnetic model of M-components 

Petr Kaspar, Ivana Kolmasova, Thomas Marshall, Maribeth Stolzenburg, and Ondrej Santolik

M-components are transient enhancements of the channel luminosity occurring simultaneously with the continuing current phase of the cloud-to-ground lightning. They are initiated by the connection of the in-cloud channel to the grounded channel. We have developed a new model of M-component processes, which is based on the numerical solution of the Maxwell’s equations together with the Poisson’s equation for a given thundercloud charge structure. We compute the radiated electric and magnetic fields at various distances from the lightning channel. We model a microsecond-scale electric field pulse emitted during the connection of the in-cloud channel to the grounded channel and compare its waveform with measurements conducted in Florida. The modeled current waveforms at various heights above the ground are the outputs of our model and we compare them with measured luminosity curves. We also show how the M-component simulation results depend on the parameters of the model.

How to cite: Kaspar, P., Kolmasova, I., Marshall, T., Stolzenburg, M., and Santolik, O.: Electromagnetic model of M-components, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6249, https://doi.org/10.5194/egusphere-egu25-6249, 2025.

EGU25-6293 | Orals | NH1.6

Total lightning for the early warning: Severe weather signatures from the real-time Lightning Mapping Array network in Catalonia 

Nicolau Pineda, Ferran Fabró, Oriol Rodríguez, David Romero, Oscar van der Velde, Jesús Alberto López, and Joan Montanyà

Lightning Mapping Array (LMA) networks detect very-high-frequency (VHF, 60–66 MHz) emissions from lightning channels inside clouds. This enables the mapping of lightning in three dimensions. The use of real-time LMA data has proven beneficial for forecasting and warning about impending severe weather. Beyond the standard analysis of cloud-to-ground lightning information, the ability to visualize 3D total lightning has provided forecasters with greater knowledge of storm-scale processes.

A network of more than 20 LMA stations has been established in Catalonia (northeastern Iberian Peninsula) thanks to a partnership between the Meteorological Service of Catalonia (SMC) and the Technical University of Catalonia (UPC). Since it began real-time operations during the summer of 2023, it has grown to become Europe's largest LMA network.

To complement classic severe weather signatures observed in weather radar (e.g., storm splitting, BWER, TBSS) and in satellite imagery (e.g., overshooting tops, v-shape), we put our focus here on severe weather signatures observed with the LMA network during the thunderstorm seasons of 2023 and 2024 in Catalonia. Indeed, lightning distribution and evolution can portray complementary information in real-time surveillance, adding confidence to the forecaster and therefore reinforcing the decision-making when issuing alerts for imminent severe weather.

How to cite: Pineda, N., Fabró, F., Rodríguez, O., Romero, D., van der Velde, O., López, J. A., and Montanyà, J.: Total lightning for the early warning: Severe weather signatures from the real-time Lightning Mapping Array network in Catalonia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6293, https://doi.org/10.5194/egusphere-egu25-6293, 2025.

EGU25-7039 | ECS | Orals | NH1.6

Assessing the Role of Continuing Current in Fire-Igniting Lightning Strokes with Space-Based Measurements 

Francisco Javier Perez-Invernon, Jose V. Moris, Francisco J. Gordillo-Vázquez, Yanan Zhu, and Jeff Lapierre

Lightning is a primary driver of natural wildfires globally. In mid- and high-latitude regions, summer thunderstorms are key precursors of lightning-ignited wildfires, contributing substantially to the total burned area. While the influence of meteorological conditions and fuel availability on wildfire occurrence is relatively well understood, the role of the electrical characteristics of lightning in ignition probability remains uncertain. In particular, it is unclear whether the presence of a continuing current lasting tens to hundreds of milliseconds is essential for ignition or whether it significantly affects ignition probability compared to meteorological factors and fuel availability.

In this study, we investigate the factors that increase the probability of wildfire ignition in Contiguous United States (CONUS). We investigate the meteorological conditions during the occurrence of fire-igniting flashes, the value of fire danger indices, the presence of continuing currents detected from space by the Geostationary Lightning Mapper (GLM), and the polarity of the strokes provided by the Earth Networks Lightning Total Network (ENTLN). We found that the lightning ignition efficiency of fire-igniting strokes with continuing current is slightly higher than that of lightning without continuing current. In particular, we report that strokes with continuing currents may have a higher potential to produce wildfires than cloud-to-ground strokes without continuing currents when the conditions for fire ignition and spread are less favorable. Additionally, we find that lightning strokes with continuing currents are associated with smaller burned areas, likely due to less favorable conditions for fire spread.

How to cite: Perez-Invernon, F. J., Moris, J. V., Gordillo-Vázquez, F. J., Zhu, Y., and Lapierre, J.: Assessing the Role of Continuing Current in Fire-Igniting Lightning Strokes with Space-Based Measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7039, https://doi.org/10.5194/egusphere-egu25-7039, 2025.

EGU25-7073 | ECS | Orals | NH1.6

Space-Based Observations of Lightning Initiation: A Multisystem Case Study Combining Optical and Electromagnetic Data 

Andrea Kolínská, Ivana Kolmašová, and Ondřej Santolík

By combining space-based data from the Lightning Imaging Sensor (LIS) aboard the International Space Station (ISS) with broadband ground-based electromagnetic measurements, we investigate the relationship between electromagnetic emissions from lightning processes and their optical signatures, focusing on the lightning initiation phase. Our case study is based on data from the SLAVIA (Shielded Loop Antenna with Versatile Integrated Amplifier) magnetic detectors at various European locations, as well as on data from the lightning location systems ENTLN (Earth Networks Total Lightning Network), WWLLN (World Wide Lightning Location Network), EUCLID (European Cooperation for Lightning Detection), and from the SAETTA Lightning Mapping Array. Our analysis of 11 lightning flashes from 2020-2023 reveals that the light emitted during the preliminary breakdown stage can be clearly observable from the low Earth orbit, highlighting the potential for space-based systems to detect and study the lightning initiation processes.

How to cite: Kolínská, A., Kolmašová, I., and Santolík, O.: Space-Based Observations of Lightning Initiation: A Multisystem Case Study Combining Optical and Electromagnetic Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7073, https://doi.org/10.5194/egusphere-egu25-7073, 2025.

EGU25-8351 | Orals | NH1.6

A new global gridded lightning dataset with high spatial and temporal resolution 

Yuquan Qu, Matthew W. Jones, Esther Brambleby, Hugh G.P. Hunt, Francisco J. Pérez-Invernón, Marta Yebra, Li Zhao, Jose V. Moris, Thomas Janssen, and Sander Veraverbeke

Lightning is a key atmospheric phenomenon that modulates atmospheric chemistry and impacts terrestrial carbon dynamics through the ignition of wildfires and direct tree mortality. Despite its importance, there is a data gap in publicly available global lightning datasets with high spatial and temporal resolution for scientific use. In this study, we present our progress towards creating a global gridded lightning dataset derived from Vaisala’s Global Lightning Detection Network (GLD360), covering the period from 2019 to 2024, with potential annual updates thereafter. This dataset is produced through a systematic gridding procedure that converts raw GLD360 lightning event data into 0.1º hourly, 0.25º daily, and 0.5º monthly gridded values. It includes key variables such as positive and negative cloud-to-ground and intra-cloud stroke count/density, stroke peak current, stroke location uncertainty, and flash count/density, making it valuable for a wide range of scientific applications. We are evaluating the gridded dataset using local lightning detection networks in Alaska (USA), Spain, South Africa, and the New South Wales and Australian Capital Territory (Australia). Meanwhile, we are comparing stroke density with the Global Lightning Climatology (WGLC) dataset derived from the World Wide Lightning Location Network (WWLLN) and flash density with the Lightning Imaging Sensor/Optical Transient Detector (LIS/OTD). The dataset could be particularly useful for advancing studies on lightning climatology, the role of lightning in wildfire ignition, thunderstorm identification, and other related topics. Its high spatial and temporal resolution also supports regional studies of lightning-related hazards and ecosystem impacts. Our goal is to make this dataset publicly available to the scientific community to facilitate new insights into the role of lightning in the Earth system.

How to cite: Qu, Y., Jones, M. W., Brambleby, E., Hunt, H. G. P., Pérez-Invernón, F. J., Yebra, M., Zhao, L., Moris, J. V., Janssen, T., and Veraverbeke, S.: A new global gridded lightning dataset with high spatial and temporal resolution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8351, https://doi.org/10.5194/egusphere-egu25-8351, 2025.

EGU25-8563 | ECS | Orals | NH1.6

ASTRAPÉ: Atmospheric STReamer And relativistic Particle Engine – a GPU-based particle code for pre-exascale supercomputing  

Elloïse Fangel-Lloyd, Pierre Gourbin, Saša Dujko, Mathias Gammelmark, Sven Karlsson, Angel Ricardo Jara Jimenez, and Christoph Köhn

While thunderstorm processes, such as the acceleration of electrons to relativistic energies, are widely studied, the computational challenges involved have made definitive proofs difficult to acquire. High precision in electric discharge simulations is achieved by resolving particles individually, via for example Monte Carlo methods, rather than by applying a fluid approximation; however, this is computationally expensive, and the multiscale nature of thunderstorm processes incurs additional difficulties. To address these challenges, we have developed the Atmospheric STReamer And Relativistic Particle Engine (ASTRAPÉ), a fully 3D GPU-based Monte Carlo particle-in-cell code capable of tracing approximately 109 computational particles, modeling all relevant electron-molecule collisions and solving the Poisson equation to include space charge effects. We will present the particulars of the GPU implementation, along with benchmarking against existing data and performance metrics. Additionally, we will discuss code optimization for LUMI (Large Unified Modern Infrastructure), Europe’s first pre-exascale supercomputer, which allows for exceptionally fast streamer simulations. Finally, we will discuss how ASTRAPÉ  can be used to study the generation of relativistic electrons in thunderclouds. 

How to cite: Fangel-Lloyd, E., Gourbin, P., Dujko, S., Gammelmark, M., Karlsson, S., Jara Jimenez, A. R., and Köhn, C.: ASTRAPÉ: Atmospheric STReamer And relativistic Particle Engine – a GPU-based particle code for pre-exascale supercomputing , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8563, https://doi.org/10.5194/egusphere-egu25-8563, 2025.

EGU25-8887 | ECS | Orals | NH1.6

Towards a hybrid model to simulate lightning and associated energetic events in various atmospheres 

Pierre Gourbin, Elloise Fangel-Lloyd, Saša Dujko, Mathias Gammelmark, Sven Karlsson, Angel Ricardo Jara Jimenez, Hannah van Gemert, and Christoph Köhn

Thunderstorm processes represent a challenge for numerical models, as they involve numerous processes of various scales, and explosive events producing exponentially increasing numbers of particles in a very short span of time. A phenomenon called a Relativistic Runaway Electron Avalanche can occur under the right conditions, and lead to the production of a Terrestrial Gamma-Ray Flash (TGF), spanning over tens of microseconds, and during which up to 1017 electrons and photons are produced for the most intense ones, the weaker ones still producing 1012 to 1015 energetic photons. While Monte Carlo models are often used to simulate such processes, runtime typically scales with particle number, which leads to poor performance without a way to limit the number of particles computed. On the other hand, a fluid model may be adapted to deal with large particle densities, but it will struggle to deal with the extreme energies and electric fields, and will lose track of the physics of individual particles, which becomes relevant when submitted to such extreme parameters.

In order to accurately and efficiently simulate all these processes, we are developing a fully parallelized 3-D hybrid model. The code is optimised for massively parallel usage on Graphics Processing Units (GPUs), and uses the AMReX library, a software framework for massively parallel, block-structured codes, allowing us to run in parallel with implemented adaptive mesh refinement (AMR), which further improves the accuracy of the model.

With this model, we are aiming at obtaining a better understanding of lightning processes and TGFs, not only in the current Earth atmosphere, but also in the atmosphere of other celestial bodies, and in mixtures likely to have existed in the environment of Primordial Earth.

How to cite: Gourbin, P., Fangel-Lloyd, E., Dujko, S., Gammelmark, M., Karlsson, S., Jara Jimenez, A. R., van Gemert, H., and Köhn, C.: Towards a hybrid model to simulate lightning and associated energetic events in various atmospheres, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8887, https://doi.org/10.5194/egusphere-egu25-8887, 2025.

EGU25-8909 | Orals | NH1.6

LOFAR Observations of Dart Leader Starts 

Brian Hare, Olaf Scholten, Martin Lourens, Paulina Turekova, Steve Cummer, Joseph Dwyer, Ningyu Liu, John Pantuso, Caitano Da Silva, Chris Sterpka, and Sander ter Veen

Dart leaders are a poorly understood lightning phenomenon where a current pulse propagates quickly (~10^7 m/s) along a previously established, now decayed, plasma channel, resulting in a re-heating of the channel. It is not understood how dart leaders propagate or how they get started. Therefore, in this work we have imaged the beginning of multiple dart leaders with the LOFAR radio telescope. We have observed two interesting phenomena related to the start of dart leaders. Firstly, we regularly observe other discharges, such as needles or `mini’ dart leaders, hundreds of microseconds before the start of the dart leader. The `mini’ dart leaders are particularly fascinating, as they propagate up side branches over a few hundred meters (towards the positive leader branch tip) before stopping. The main dart leader then initiates after the `mini’ dart leader. The exact connection between these preceding discharges (needles and mini-darts) and the main dart leaders, if one triggers the other, or why mini-darts ought to occur at all, are difficult to understand. In addition, previous work has shown that dart leaders tend to start with an exponential rise in VHF power and speed. In this work we find that some dart leaders have a period at their beginning where they propagate relatively slowly with weak VHF emission before a period of exponential growth. In one particular case, a dart leader initiated on a side branch, propagated slowly (~5x10^6 m/s) and weakly for about for about 100 µs until it connected with the main leader branch, and only then accelerated to a high speed (~ 1.7x10^7 m/s) over a period of about 50 µs. Finally, we will attempt to relate our measurements to recent hypothesis that dart leaders are a new kind of propagation that essentially amounts to a heating wave; the dart leader charge pushes a weak current in-front of it that heats up the plasma channel which in turn allows the current to increase further and the main charge packet to move forward.

How to cite: Hare, B., Scholten, O., Lourens, M., Turekova, P., Cummer, S., Dwyer, J., Liu, N., Pantuso, J., Da Silva, C., Sterpka, C., and ter Veen, S.: LOFAR Observations of Dart Leader Starts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8909, https://doi.org/10.5194/egusphere-egu25-8909, 2025.

EGU25-9121 | ECS | Posters on site | NH1.6 | Highlight

Nowcasting Thunderstorms to Protect Lives in Africa 

Vlad Landa, Colin Price, and Yuval Reuveni

Central Africa is widely recognized as the most active region for thunderstorms globally, with the highest frequency of lightning strikes occurring near Kifuka in the Democratic Republic of Congo, where over 150 lightning flashes per square kilometer are recorded annually. The absence of accessible early warning systems in many developing countries significantly amplifies the risks associated with lightning. For instance, on August 28, 2020, a catastrophic lightning strike near the Uganda-Democratic Republic of Congo border resulted in the deaths of nine children, with a tenth succumbing while being transported to the hospital. Moreover, the detrimental effects of lightning on critical sectors—such as livestock, forestry, power utilities, aviation, high-tech industries, and public safety—are increasingly evident. A discernible rise in lightning-related fatalities has been observed, potentially attributable to population growth, which increases exposure to thunderstorms, or to changes in thunderstorm frequency driven by climate change. Regardless of the underlying causes, the risk posed to the African population remains significant and appears to be intensifying.

Building on the recent advancements of Denoising Diffusion Probabilistic Models (DDPMs)—which have demonstrated superior performance over adversarial and autoencoder-based frameworks in applications such as image generation, text-to-image synthesis, precipitation nowcasting, and weather forecasting—this research introduces an innovative nowcasting system. The proposed system predicts lightning probabilities up to six hours in advance, with 30-minute intervals, offering a probabilistic and life-saving early warning mechanism tailored for Central Africa.

Specifically, we investigate the potential of DDPMs for lightning nowcasting by adapting spatiotemporal frameworks originally developed for precipitation nowcasting. In essence, diffusion models learn the underlying data distribution Ρ(Χ), where Χ represents the spatiotemporal probability density function of lightning. This is achieved by training the model to reverse a predefined noising process that progressively corrupts the target data with Gaussian noise. Here, the diffusion process has been extended to condition on auxiliary data Υ, such as satellite-derived wavelength imagery, constituting the approach suitable for spatiotemporal conditional nowcasting Ρ(ΧΥ).

As a data source, we leverage recent datasets from the Meteosat Third Generation (MTG) Lightning Imager (LI) over Africa and the Earth Networks Total Lightning Network (ENTLN) to train the model that locally characterizes the stochastic nature of lightning events.

How to cite: Landa, V., Price, C., and Reuveni, Y.: Nowcasting Thunderstorms to Protect Lives in Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9121, https://doi.org/10.5194/egusphere-egu25-9121, 2025.

EGU25-9498 | ECS | Orals | NH1.6

A Nowcasting Method for Severe Convective Weather Based on Array Radar and Lightning Jumps 

Mingyi Xu, Xiushu Qie, Ye Tian, Martin Fullekrug, Chenghong Gu, Xue Bai, Shuqing Ma, Yan Liu, Chenxi Zhao, Xinyuan He, Bohan Li, Laiz Souto, Tinashe Chikohora, and Douglas Dodds

Convective weather, often associated with heavy precipitation, hail, lightning, and other hazardous phenomena, is highly unpredictable, short-lived, and localized, making forecasting and early warning particularly challenging. The formation of lightning is closely tied to the thermodynamic and microphysical processes within severe convective weather systems (e.g., Qie et al., 2021). Not only does it pose a significant threat to human life and properties, but it has also been recognized by the International Electrotechnical Commission (IEC) as a major hazard to power systems, communication networks, buildings, and electronic devices.

Since the mid-20th century, Doppler weather radars have been widely used to monitor hazardous weather by identifying precipitation, storm structures, and movement. Advances in radar technology, especially the introduction of array weather radar, have further enhanced the precision and timeliness of severe weather nowcasting. Unlike traditional single-antenna radars, array radars use multiple small antennas to form a large, flexible antenna array for rapid and precise beam control. This distributed phased-array system excels in detecting fine-scale flow and intensity fields, offering powerful tools for studying small-scale convective phenomena (e.g., Adachi et al., 2016).

This study utilizes array radar data from Foshan, Guangdong, China, high-precision lightning location data, and ground-based meteorological observation data to identify, track, and forecast severe convective weather. Based on a radar dual-threshold convective storm tracking and identification algorithm (e.g., Tian et al., 2019), combined with a lightning jump algorithm (e.g., Schultz et al., 2017), this nowcasting method monitors the lightning variation characteristics within strong convective cells (CCs), providing indices for severe convective weather. By comparing results with observations and optimizing algorithm parameters, the method improves hit rates, reduces false alarms, and achieves an average lead time of ~22 minutes with a hit rate over 80%, as demonstrated by case studies. This method can be effectively applied to enhance the monitoring and early warning capabilities for severe convective weather, thereby mitigating the impact of lightning and reducing lightning-related disasters for critical infrastructure, particularly power systems.

 

Acknowledgment

This work was jointly supported by the KERAUNIC project (ref: NIA2_NGET0055, National Grid Electricity Transmission, 2024) under the Network Innovation Allowance (NIA), the Arctic Pavilion Open Research Fund of Nanjing Joint Institute for Atmospheric Sciences under Grant BJG202410 and the China Scholarship Council program under Grant 202305330027.

 

References

Adachi, T., Kusunoki, K., Yoshida, S., et al. (2016). High-speed volumetric observation of a wet microburst using X-band phased array weather radar in Japan. Monthly Weather Review144(10), 3749-3765.

National Grid Electricity Transmission. (2024). Knowledge Elicitation of Risks to Assets Under LightNing Impulse Conditions (KERAUnIC). https://smarter.energynetworks.org/projects/nia2_nget0055

Qie, X., Yuan, S., Chen, Z., et al. (2021). Understanding the dynamical-microphysical-electrical processes associated with severe thunderstorms over the Beijing metropolitan region. Science China Earth Sciences, 64, 10-26.

Schultz, C. J., Carey, L. D., Schultz, E. V., & Blakeslee, R. J. (2017). Kinematic and microphysical significance of lightning jumps versus nonjump increases in total flash rate. Weather and forecasting32(1), 275-288.

Tian, Y., Qie, X., Sun, Y., et al. (2019). Total lightning signatures of thunderstorms and lightning jumps in hailfall nowcasting in the Beijing area. Atmospheric Research230, 104646.

How to cite: Xu, M., Qie, X., Tian, Y., Fullekrug, M., Gu, C., Bai, X., Ma, S., Liu, Y., Zhao, C., He, X., Li, B., Souto, L., Chikohora, T., and Dodds, D.: A Nowcasting Method for Severe Convective Weather Based on Array Radar and Lightning Jumps, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9498, https://doi.org/10.5194/egusphere-egu25-9498, 2025.

EGU25-9659 | Orals | NH1.6

Measuring self-induced corona discharges of individual aerosol particles in an optical trap  

Andrea Stoellner, Isaac Lenton, Caroline Muller, and Scott Waitukaitis

            Although cloud electrification and lightning have been studied for hundreds of years, the field still deals with many open questions [1]. One of the most puzzling examples is that of lightning inititation – neither the mechanism by which a cloud generates enough charge to cause lightning nor the process by which lightning itself is triggered are well understood. In our experiment we aim to gain insight into both questions on the scale of a single particle. We utilize optical tweezers to levitate individual aerosol particles and observe their charging and discharging dynamics over days-to-weeks time periods and with elementary-charge resolution. Our approach allows us to study these processes without losing information to ensemble averages or external interference from other particles or substrates [2], and is applicable to solid and liquid particles in the micrometer size range. Using multi-photon absorption from the trapping laser [3] we can charge the trapped particle at different rates and to different values, observing every charging and discharging event along the way. Additionally, the experiment allows us to control the relative humidity around the particle and to fully discharge the particle using air ions. By studying the charging behavior of the particle and the spontaneous discharges it experiences, we hope to contribute to a better understanding of the microphysical processes involved in lightning initiation and adjacent electrical phenomena in the atmosphere.

This project has received funding from the European Research Council (ERC) under the European Union’s Starting Grant (A. Stoellner, I. Lenton & S. Waitukaitis received funding from ERC No. 949120, C. Muller received funding from ERC No. 805041).

[1] J. R. Dwyer and M. A. Uman, Physics Reports 534, 147 (2014).
[2] F. Ricci, M. T. Cuairan, G. P. Conangla, A. W. Schell, and R. Quidant, Nano Letters 19, 6711 (2019).
[3] A. Ashkin and J. M. Dziedzic, Physical Review Letters 36, 267 (1976).

How to cite: Stoellner, A., Lenton, I., Muller, C., and Waitukaitis, S.: Measuring self-induced corona discharges of individual aerosol particles in an optical trap , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9659, https://doi.org/10.5194/egusphere-egu25-9659, 2025.

EGU25-9775 | Orals | NH1.6

Prediction of Lightning-Ignited Wildfires On A Global Scale based on Explainable Machine Learning Model 

Colin Price, Assaf Shmuel, Oren Glickman, Teddy Lazebnik, and Eyal Heifetz

Wildfires pose a significant natural disaster risk to populations and contribute to accelerated climate change. As wildfires are also affected by climate change, extreme wildfires are becoming increasingly frequent. Although they occur less frequently globally than those sparked by human activities, lightning-ignited wildfires play a substantial role in carbon emissions and account for the majority of burned areas in certain regions. While existing computational models, especially those based on machine learning, aim to predict lightning-ignited wildfires, they are typically tailored to specific regions with unique characteristics, limiting their global applicability. In this study, we present machine learning models designed to characterize and predict lightning-ignited wildfires on a global scale. Our approach involves classifying lightning-ignited versus anthropogenic wildfires globally over a long timespan, and estimating with high accuracy of over 91% the probability of lightning to ignite a fire based on a wide spectrum of factors such as meteorological conditions and vegetation. Utilizing these models, we analyze seasonal and spatial trends in lightning-ignited wildfires shedding light on the impact of climate change on this phenomenon. Our findings highlight significant global differences between anthropogenic and lightning-ignited wildfires. Moreover, we demonstrate that, even over a short time span of less than a decade, climate change has steadily increased the global risk of lightning-ignited wildfires. We also find that models trained to predict lightning-ignited wildfires and models trained to predict anthropogenic wildfires are very different. This dramatically reduces the predictive performance of models trained on anthropogenic wildfires when applied to lightning-ignited ignitions, and vice versa. This distinction underscores the imperative need for dedicated predictive models and fire weather indices tailored specifically to each type of wildfire.

How to cite: Price, C., Shmuel, A., Glickman, O., Lazebnik, T., and Heifetz, E.: Prediction of Lightning-Ignited Wildfires On A Global Scale based on Explainable Machine Learning Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9775, https://doi.org/10.5194/egusphere-egu25-9775, 2025.

EGU25-10228 | ECS | Orals | NH1.6

Investigating vertical distribution of charge in fog through tethered balloon measurements and modelling 

Caleb Miller, Keri Nicoll, Chris Westbrook, and R. Giles Harrison

Fog, a reduction in visibility caused by water droplets suspended in the atmosphere, is a weather phenomenon which is linked to atmospheric electrical changes. Measurements of the potential gradient (PG) in particular have been shown to be useful for predicting fog, which has important applications for the aviation industry. The underlying theory behind these changes in PG during and before fog events is still an area of active research. Previously, in many studies of fog and atmospheric electricity, it has been assumed that fog droplets are neutral, for simplicity. However, it is well known that many clouds contain significant layers of space charge, and it is likely that fog droplets may also be charged. In this work, the distribution of charge in fog is studied using both numerical modelling and real-world measurements.

Numerical investigations use an earth-electrode model, in which it is assumed that the earth is a negatively charged surface and that there is a vertical electric field in the atmosphere above the surface. Using a system of 1D electrostatic equations, the steady-state distribution of vertical charge can be found, both in clear air and in a foggy air with prescribed aerosol. The results of these simulations provide the expected electrical charge in an idealised setup, which show appreciable space charge near the surface of the earth, as well as a rapidly decreasing PG with height.

Real-world measurements of the vertical charge distribution in fog up to 55m are made using a miniature electrode sensor and battery powered datalogger which is attached to a tethered balloon. The electrode current is amplified, and changes are apparent if the balloon passes through a sharp vertical gradient in space charge. As a result, vertical profiles of the magnitude and polarity of space charge in the fog layer can be measured and then compared with the modelled ideal case. In this presentation, we will show the measurements made during several fog cases with this setup.

A better understanding through modelling and measurements of the space charge in fog will help to identify cases where PG is especially well suited to fog prediction.

How to cite: Miller, C., Nicoll, K., Westbrook, C., and Harrison, R. G.: Investigating vertical distribution of charge in fog through tethered balloon measurements and modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10228, https://doi.org/10.5194/egusphere-egu25-10228, 2025.

EGU25-10264 | Orals | NH1.6

Trend-based scaling for high-resolution lightning in climate projections  

Enrico Arnone, Nicola Cortesi, Sara Rubinetti, Stefano Dietrich, and Marco Petracca

New geostationary satellites, together with ground networks, now provide high-resolution, continuous lightning observations, offering unprecedented insights into lightning activity across vast areas of the globe. In contrast, global climate models (GCMs) lack the spatial resolution and physical processes required to simulate lightning directly, leading to the need for parameterizations and scaling methods. In this study, we present a novel trend-based scaling approach that bridges the gap between coarse-resolution GCM output and high-resolution lightning flash rates to improve projections of lightning activity by the end of the century. The scaling method employs machine learning techniques to identify the atmospheric parameters that best reproduce observed current lightning activity, which are then combined with coarser GCM trends (individually for each quantile of the distribution) to project future lightning changes.

Italy was selected as a case study, using the past 15 years of lightning observations from the LINET network to identify lightning predictors among atmospheric parameters from the ERA5 reanalysis. The best predictors identified include a combination of convective available potential energy, relative humidity, temperature gradients, wind velocity and shear, geopotential height, and freezing level. This model accurately reproduces the spatial distribution and temporal variability of current lightning activity. Trend scaling from multiple future climate scenarios was then applied using CMIP6 projections to evaluate changes in lightning activity across different regions and time periods. 

Our results show that trend-based scaling significantly improves the spatial distribution and intensity of projected lightning flash rates compared to traditional parameterizations. This work provides a practical framework for integrating lightning projections into climate impact studies, enhancing the reliability of lightning future changes under various climate scenarios. The main advantage of the proposed method is that it can be applied to reanalysis datasets of any resolution, offering a flexible tool for assessing lightning-related risks in a warming world.

How to cite: Arnone, E., Cortesi, N., Rubinetti, S., Dietrich, S., and Petracca, M.: Trend-based scaling for high-resolution lightning in climate projections , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10264, https://doi.org/10.5194/egusphere-egu25-10264, 2025.

EGU25-10378 | ECS | Orals | NH1.6

A parameter-space exploration of the Relativistic Discharge Model mapping for which conditions ALOFT’s Flickering Gamma-ray Flashes are produced 

Øystein Håvard Færder, Nikolai Lehtinen, David Sarria, Martino Marisaldi, and Nikolai Østgaard

During the ALOFT flight campaign, July 2023, a novel type of multi-pulse gamma-ray emission from thunderclouds was systematically recorded. Referred to as flickering gamma-ray flashes (FGFs), this type of emission is not linked with lightning leaders and does not coincide with detectable radio emissions [1].

A promising candidate theory for explaining this phenomenon is the relativistic feedback discharge (RFD) developed by Dr. J. Dwyer and his group [2]. Fully self-consistent 3D Monte-Carlo calculations of RFD [3], which take the field quenching by produced currents into account, are quite computationally intensive. In fact, the full physics of RFD has barely been explored outside Dwyer’s group.

Therefore, we developed an independent numerical model especially made to evaluate the capability of the RFD theory to reproduce FGFs. Despite its simplification into a set of spatially-independent ordinary differential equations (ODEs), it applies the most relevant physics: ionisation, electron dynamics, attachment processes, relativistic runaway electron avalanche (RREA), and feedback akin to Dwyer’s theory. The ODEs that we end up solving are analogous to a complexified Lotka-Volterra model which describes a system with oscillations.

In this presentation, we introduce a 0.5D model (i.e., with indirect account of the spatial size of the RREA region) and demonstrate its ability to reproduce emission light curves very alike FGFs under realistic conditions, given the right set of parameters (see below). Furthermore, we show that the same model also reproduces light curves alike terrestrial gamma-ray flashes (TGFs, both single and multiple pulses) and gamma-ray glows (GRGs) for different sets of parameters but still under realistic conditions, hence proving this model to be even more general than originally intended.

With this, we performed a parameter-space exploration, using our model and systematically applying different values for 1) the initial (background) internal electric field strength of the cloud, 2) the characteristic growth time of the external electric field, 3) the vertical size of the high-field region in the cloud, and 4) the maximum change of the external field. The results, as shown in parameter-space diagrams, are qualitatively as expected. TGFs tend to occur for relatively small high-field regions. For larger high-field regions, the model reproduces GRGs in the case of slowly increasing external fields while FGFs and weak TGFs in the case of rapidly increasing external fields. The amplitude and the number of pulses typically scale with the maximum change of the external field. Finally, increasing the value of the initial internal electric field leads to a decrease in the minimum required change in the external field needed to reproduce FGFs, multi-pulse TGFs and GRGs.

 

References:

[1] Østgaard, N., Mezentsev, A., Marisaldi, M., Grove, J. E., Quick, M., Christian, H., Cummer, S., Pazos, M., Pu, Y., Stanley, M., et al., “Flickering gamma-ray flashes, the missing link between gamma glows and TGFs”, Nature (2023).

[2] Dwyer, J. R., “Relativistic breakdown in planetary atmospheres,” Physics of Plasmas, vol. 14, no. 4, p. 042901 (2007).

[3] Liu, N., Dwyer, D., “Modeling terrestrial gamma ray flashes produced by relativistic feedback discharges”, Journal of Geophysical Research (Space Physics), Vol. 118, no. 5, p. 2359-2376 (2013)

How to cite: Færder, Ø. H., Lehtinen, N., Sarria, D., Marisaldi, M., and Østgaard, N.: A parameter-space exploration of the Relativistic Discharge Model mapping for which conditions ALOFT’s Flickering Gamma-ray Flashes are produced, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10378, https://doi.org/10.5194/egusphere-egu25-10378, 2025.

From rubbing a balloon on one's hair to the dramatic display of volcanic lightning, the triboelectric effect is a widespread phenomenon where contact between objects leads to an exchange of electric charge. Despite its ubiquity, our understanding of the underlying physics remains largely phenomenological. Among the many open questions, one is particularly relevant to earth science and astrophysics: why do objects made of the same material continually exchange electric charge? This effect is especially pronounced in systems involving grains or powders, where frequent collisions can result in a significant buildup of electrostatic potential energy. Such processes can influence the dispersal range of aerosols in the atmosphere, determine whether protoplanetary dust will coalesce, and even trigger thunderstorms during volcanic eruptions or forest fires. Using acoustic levitation, we isolate individual grains and conduct controlled collisions with a substrate, measuring the charge by observing the grain's behavior in electric fields. This method can accurately resolve individual collision events, allowing us to investigate various proposed charging mechanisms and explore in detail what causes the breaking of symmetry between positively and negatively charging samples. We determine that slight variations in surface composition due to molecules recruited from the atmosphere can lead to drastic changes in the charging behavior.

How to cite: Grosjean, G. and Waitukaitis, S.: Investigating the origins of static charge in granular systems of silica and other oxides using acoustic traps, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10837, https://doi.org/10.5194/egusphere-egu25-10837, 2025.

EGU25-10850 | ECS | Orals | NH1.6

LOFAR Lightning Data: Accuracy in Polarization Reconstruction 

Paulina Turekova, Brian Hare, Olaf Scholten, Marten Lourens, Steven Cummer, Joseph Dwyer, Ningyu Liu, Chris Sterpka, and Sander ter Veen

The polarization of VHF radio signals emitted by lightning can help shed light on the intricate science of lighting propagation, through the direction of the corona VHF emission. However, this lightning radio polarization is not easily measured and, thus, understood. Employing the LOFAR radio telescope, we use a near-field beamforming algorithm (TRI-D) that coherently sums antenna voltages while accounting for the antenna function. This allows us to reconstruct VHF source location and polarization in 3 dimensions. In this work, we evaluate the accuracy of these unparalleled results. Performing a Monte Carlo error analysis, we simulate the antenna voltage signal resulting from a point-like dipole, which is then reconstructed with the imager. The difference between the input and the reconstructed source parameters gives us an approximation of the polarization error bars. We find that the polarization error is at maximum 12 degrees. This value fluctuates with varying source location and angle suspended between the polarization vector and the radial vector. We are testing the polarization reconstruction accuracy for radio point-like sources, background noise, and extended sources. We will present a comprehensive report on these results and their interpretation, our technique, and the imaging algorithm.

How to cite: Turekova, P., Hare, B., Scholten, O., Lourens, M., Cummer, S., Dwyer, J., Liu, N., Sterpka, C., and ter Veen, S.: LOFAR Lightning Data: Accuracy in Polarization Reconstruction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10850, https://doi.org/10.5194/egusphere-egu25-10850, 2025.

EGU25-11142 | ECS | Orals | NH1.6

Lightning Assimilation based on a 2D-to-3D Bayesian method for Vertical Velocity and Water Vapor 

Di Shaoxuan, Qie Xiushu, and Han Wei

Lightning can indicate the location of strong convection in thunderstorms. We develop a lightning data assimilation observational operator based on a 2D-to-3D Bayesian method, which converts the 2D lightning distribution into vertical velocity profiles and RH profiles for each grid point in the plane. The new lightning observational operator provides a good representation of the shape and peak height of the instantaneous vertical velocity profiles in thunderstorms, rather than using a fixed or long-term averaged profile distribution. After 1-hour forecasting, experiments that assimilated both vertical velocity and water vapor still maintained a close vertical distribution to the observations in the lower layers. It also shows significant improvement in heavy rainfall forecasting within 1 hour, with a notable increase in precipitation scores. The improvement in heavy rainfall prediction primarily lies in the positive adjustment of the location of intense rainfall and the enhancement of rainfall intensity.

How to cite: Shaoxuan, D., Xiushu, Q., and Wei, H.: Lightning Assimilation based on a 2D-to-3D Bayesian method for Vertical Velocity and Water Vapor, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11142, https://doi.org/10.5194/egusphere-egu25-11142, 2025.

EGU25-11832 | ECS | Posters on site | NH1.6

High resolution imaging of negative leader propagation with LOFAR 

Marten Lourens, Brian Hare, Olaf Scholten, Paulina Turekova, Steve Cummer, Joe Dwyer, Ningyu Liu, Chris Sterpka, and Sander ter Veen
The propagation of negative leaders is poorly understood and one of the top questions in lightning research. In the optical, negative leaders are observed to propagate in steps similar to those seen in laboratory experiments, with an average velocity between 105 and 106 m/s. Step formation occurs via a luminous section formed in front of the leader tip, referred to as a “space stem”. This space stem grows bi-directionally and eventually connects with the leader channel, resulting in a surge of current, a luminosity wave traversing back up the channel, and a burst of negative corona streamers emitted from the new tip.
In the VHF, stepping is also observed, but emission associated with space stems has so-far not been identified. Instead, a propagating front of VHF pulse sources is observed, which exhibits a filametary structure at high altitudes.
In this work, we leverage the high tempo-spatial resolution of the LOFAR radio telescope and the high sensitivity and completeness of a new near-field beamforming algorithm (TRI-D) to construct detailed three-dimensional images of negative leader propagation. The spatial resolution of the resulting images is better than 1 m and the time resolution is 100 ns. Studying the distribution of VHF pulse sources, we hope to improve our conceptual understanding of negative leader stepping. Specifically, we want to show whether there is any evidence for space stems and better understand the distribution and interaction of streamers. Here, I present the initial findings of this research.

How to cite: Lourens, M., Hare, B., Scholten, O., Turekova, P., Cummer, S., Dwyer, J., Liu, N., Sterpka, C., and ter Veen, S.: High resolution imaging of negative leader propagation with LOFAR, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11832, https://doi.org/10.5194/egusphere-egu25-11832, 2025.

EGU25-12324 | ECS | Orals | NH1.6

Simulating Electric and Magnetic Fields from Dust Devils 

David Reid, Karen Aplin, and Nicholas Teanby

Dust storms have been observed to generate significant DC electric fields. Dust devils specifically are a subset of dust storm, with an ordered sense of rotation about a central axis. Observations in Arizona and Nevada have recorded both electric and magnetic fields associated with dust devils. These electromagnetic signatures are important for future space exploration, with charged dust presenting issues for solar power generation and optics as well as the possibility of communication disruption. The likelihood of lightning from dust devils also has implications for the origin of life, and the chemical composition of the Martian surface and atmosphere.

Building upon terrestrial observations of dust devils, and other properties of triboelectrically charged particles, a lumped particle methodology for the generation of electromagnetic fields based on fundamental laws of physics is presented. In this model, the particle motion is constrained to a simple harmonic motion, tracing a circle in 2D, with parameterised relationships for the height variation of the dust devil, the charge profile with grain height and the velocity of the rotational motion determined.

Results from the simulation of a dust devil with 3.5 metre radius are compared to the measurements from a terrestrial dust devil of the same size. With a tuned surface electron density input to an event-driven tribocharging model, calculated electrical and magnetic fields are within a factor of two of the measured values. An idealised 3.5 m radius dust devil with its centre passing directly over magnetic and electric field sensors, has an electric field approaching the terrestrial breakdown field strength. This is consistent with recent observations of electric discharge in the vicinity of a dust devil in the UAE. The vertical and horizontal variation of the electric and magnetic field in the vicinity of the dust devil can now be predicted, and the model can readibly be used to interpret field observations on Earth, lander measurements on Mars, and predict signals in future instrument deployments to inform sensor design.

How to cite: Reid, D., Aplin, K., and Teanby, N.: Simulating Electric and Magnetic Fields from Dust Devils, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12324, https://doi.org/10.5194/egusphere-egu25-12324, 2025.

EGU25-12365 | ECS | Posters on site | NH1.6

Comparing lightning Superbolts detected independently in the optical and VLF ranges 

Navot Yehieli, Colin Price, and Yoav Yair

This study investigates the phenomenon of “Superbolts”, High-intensity lightning flashes – by examining their occurrence and correlations across multiple lightning monitoring networks. Given inconsistencies in Superbolt definitions in prior research, this study addresses the feasibility of establishing a universal definition for Superbolts and analyzes the inherent challenges to do so.

 

A statistical methodology was used to study Superbolts occurrence across three datasets: the ISS Lightning Imaging Sensor (LIS), the World-Wide Lightning Localization Network (WWLLN), and the Earth Networks Total Lightning Networks (ENTLN). This study employed current peak power and energy thresholds to propose statistical-based thresholds for Superbolts radiance and used spatial and temporal matching criteria to examine the correlation between the occurrence of Superbolts in different detection methods.

 

This study identified notable divergences between spatial and temporal distributions of Superbolts across different systems. Both LIS and WWLLN datasets show high-density regions of superbolts over the Maritime Continent of Asia, South America, and South Africa, but disparities appear around Australia, Central America, and northern regions. Moreover, temporal analysis shows a seasonal dependency, with LIS data indicating higher Superbolt incidence in summer, contrasting with WWLLN's peak during winter. While WWLLN data partially align with Kirkland's "three Superbolt chimneys" (1999), the observed high-density regions differ substantially from those presented in Holzworth et al. (2019). Correlation analysis between ENTLN and LIS datasets showed insignificant matching in Superbolts occurrence.

 

These findings underscore the inherent challenges to establish a universal definition for Superbolts, especially when comparing data from optical-based and RF-based monitoring networks. Challenges include differences in temporal and spatial coverage, detection biases due to atmospheric conditions, and non-unique matching of flashes. Hence, system-specific or statistical based thresholds may provide a more feasible alternative. Future research should include meteorological data, such as clouds cover and optical-depth, and explore the relationships between global lightning distribution and Superbolts formation.

How to cite: Yehieli, N., Price, C., and Yair, Y.: Comparing lightning Superbolts detected independently in the optical and VLF ranges, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12365, https://doi.org/10.5194/egusphere-egu25-12365, 2025.

EGU25-12436 | ECS | Orals | NH1.6

A new multi-year data set of Potential Gradient variations at a suburban site in Northeastern Germany  

Gayane Karapetyan, Reik V. Donner, Keri Nicoll, and Hripsime Mkrtchyan

We report the characteristics of a new multi-year atmospheric electricity data set obtained in a suburban area in Northeastern Germany, a region where comparable measurements have been missing so far. Specifically, a CS110 electric field mill (Campbell Scientific) operates since March 2021 as part of a small weather station located at the Herrenkrug campus of Magdeburg-Stendal University of Applied Sciences in Magdeburg, Germany (52.13939°N, 11.67628°E) at an altitude of approximately 50 m a.s.l. Continuous measurements have since been undertaken at 1-minute temporal resolution, providing valuable data on local atmospheric Potential Gradient (PG) variability and their linkages with Global Electric Circuit (GEC) characteristics.

PG values recorded at the site range from -1 to 1 kV/m. Typically, during undisturbed weather conditions, diurnal variation of the PG  shows a single maximum and ranges between 5 and 20 V/m. On most days, there is a noticeable drop around 6-7 UTC, followed by a maximum around 14-15 UTC. Measurements from Magdeburg demonstrate an unusually small range of daily variations compared to other sites. While theoretically expected PG values under fair weather conditions should be around 100 V/m, the local instrument has never reached such values. Recent PG measurements performed at three different stations of the GLOCAEM network with an identical instrument showed median PG values in a range between 60 and 240 V/m during unperturbed conditions (Nicoll et al. 2019), while our measurements exhibited a median value of only 13.5 V/m, demonstrating that both PG median amplitude and variability obtained at the site are smaller than would be expected. 

To further investigate this issue, a short campaign with parallel measurements using an identical reference instrument has been undertaken during summer and fall of 2024. Since the original field mill is located inside a fenced area, it might be expected that the surrounding metallic fence negatively affects the measurements. By conducting parallel measurements with the reference field mill also being placed inside the fenced area, we however did not find significant systematic effects of the fence on the measured PG values. 

A second series of measurements was conducted at about 200 m distance from the original field mill, where the surrounding area was relatively clear from any trees and built infrastructure. Measurements at this site have been obtained under different weather conditions. While there exists considerable co-variability between both sites during most of the day, we found much larger, even qualitative differences between both instruments arising during sunrise and sunset. 

The results of our parallel measurements contribute to identifying discrepancies between co-located electric field measurements, which have also been reported in other previous studies, and clarifying the underlying root causes. To this end, the reference measurements during daytime have been used to determine a statistical correction for the values obtained with our primary instrument, which will be further employed for calibrating our ongoing measurements. The thus obtained long-term time series of local PG variations provides a new dataset allowing further detailed studies of atmospheric electricity variations in suburban areas of Central Europe.

How to cite: Karapetyan, G., Donner, R. V., Nicoll, K., and Mkrtchyan, H.: A new multi-year data set of Potential Gradient variations at a suburban site in Northeastern Germany , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12436, https://doi.org/10.5194/egusphere-egu25-12436, 2025.

EGU25-13218 | Posters on site | NH1.6

Thermodynamic-Aerosol Relationships of Thunderstorm Environments in the Bangkok Metropolitan Region 

Mace Bentley, Jo-Jinda Sae-jung, Zhuojun Duan, and Tobias Gerken
Bangkok, Thailand is a tropical asian megacity with high aerosol concentrations and frequent thunderstorm activity. This investigation examines relationships between thermodynamics, aerosols, and thunderstorms using lightning stroke counts as a metric of intensity. The investigation incorporates data from the aerosol robotic network (AERONET), ERA-5 reanalysis, ground-based air quality stations, and total lighting stroke data from Vaisala Inc.’s GLD360 network.
 
Results indicate that aerosol relationships with thunderstorm intensity are robust and, when examined in concert with instability, evidence suggests aerosols can augment lightning. Thermodynamic instability is also positively correlated with stroke counts in thunderstorms. Particulate matter (PM10) concentration is significantly higher in thunderstorms containing more than 100 strokes, supporting the potential role of aerosols in promoting non-inductive charge processes. The emergence of a “boomerang” effect appears as aerosol optical depth (AOD)  increases. Evidence suggests that higher AOD initially promotes, then limits, instability and thunderstorm intensity. 

How to cite: Bentley, M., Sae-jung, J.-J., Duan, Z., and Gerken, T.: Thermodynamic-Aerosol Relationships of Thunderstorm Environments in the Bangkok Metropolitan Region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13218, https://doi.org/10.5194/egusphere-egu25-13218, 2025.

EGU25-13547 | Orals | NH1.6

Understanding variability in atmospheric electricity measurements at Sodankyla, Finland 

Keri Nicoll, Owen O'Neill, Caleb Miller, Jussi Paatero, and Thomas Ulich

High latitude measurements of the atmospheric Potential Gradient (PG) can provide valuable information on understanding sources of variability in the Global Electric Circuit (GEC).  The influence of solar activity on electrical processes (such as ionisation) is much greater at high latitudes, allowing the mechanisms by which space weather affects atmospheric electricity to be studied. The often cleaner environment, which means that PG measurements are not dominated by variations in local aerosol concentrations, also means that processes related to changes in near surface ionisation (e.g. from radon) can be studied.

Measurements of PG have been made at a high latitude site in Sodankyla, Finland (67°22' N, 26°38' E) since 2017 using a Campbell Scientific CS110 Electric Field Mill.  Sodankyla is a heavily instrumented site for meteorological, geophysical and auroral research and so a wealth of additional observations are available to support PG analysis.   This research provides an overview of 7 years of PG measurements at Sodankyla, including analysis of the typical fair weather diurnal variation, which demonstrates clear evidence of the GEC signal, with a morning minimum and evening maximum,  with significantly larger PG values during summer months than winter.  This work will also analyse the diurnal and seasonal variability in PG at Sodankyla alongside the variability in co-located ionisation measurements, comprising observations of Radon222, as well as “external” radiation from a gamma ray spectrometer which is sensitive to gamma emission from natural radioactivity as well as galactic cosmic rays.  This work will contribute to understanding around how conductivity variations resulting from changes in local ionisation rate contribute to diurnal and seasonal variability in PG at clean air sites.

How to cite: Nicoll, K., O'Neill, O., Miller, C., Paatero, J., and Ulich, T.: Understanding variability in atmospheric electricity measurements at Sodankyla, Finland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13547, https://doi.org/10.5194/egusphere-egu25-13547, 2025.

        Most tropical cyclones (TCs) landfalling Southern China originated from the Northwest Pacific (NWP) and tracked over the South China Sea (SCS) before landfall. The internal structures such as convective characteristics of the tropical cyclones may change as the TCs translate from the open ocean (NWP) to the enclosed sea (SCS) due likely to the impacts from nearby landmass. This study compares the lightning activity and convective structures, as well as the large-scale environments, of TCs over the NWP and SCS to better understand the structural changes and underlying physical mechanisms. It is interesting that TCs over SCS are much more electrically active than NWP TCs (especially in the outer rainbands), even though the NWP TCs precipitate heavier. Multi-satellite observations suggest that the NWP TCs have a deeper layer of ice particles, producing heavier surface rainfall; however, the SCS TCs own more large ice particles or supercool liquid in the mixed-phase region, which is essential for charge separation thus lightning production. It is surprising that the thermodynamic conditions (e.g., SST and atmospheric instability) of the NWP are more favorable for convective development than SCS. A few factors may contribute to higher lightning activity in SCS TCs, including stronger vertical wind shear, thinner warm cloud depth and higher aerosol optical depth, all may help to produce asymmetric intense convection and active mixed-phase processes. Furthermore, SCS TCs display a marked lightning maximum in the front quadrants of the moving direction, but NWP TCs are less so, likely because the thermodynamic and aerosol impacts from land are stronger in the SCS. Lightning in the SCS TCs is also more asymmetric relative to the vertical wind shear than the NWP TCs, which is featured by a maximum in the right of the downshear region of the outer rainband (opposite to the precipitation pattern). 

How to cite: Xu, W. and Xie, Y.: Contrasting Lightning Activity and Convective Structures between Tropical Cyclones over Open Ocean and Enclosed Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14349, https://doi.org/10.5194/egusphere-egu25-14349, 2025.

EGU25-14876 | ECS | Orals | NH1.6

Evaluating Microphysics, Cumulus, and Lightning Parameterization Schemes in WRF Model for Thunderstorm Simulation Over East India 

Vn Rinuragavi, Rupraj Biswasharma, Nandivada Umakanth, and Sunil Pawar

   Lightning originates from electrical discharges driven by the non-inductive charging mechanism within thunderstorms. The charge separation in these regions is governed by the surrounding convective environment, storm dynamics, and microphysical processes, including updraft velocity and ice content, which intensify the storm's electric field. In recent decades, advances in understanding cloud microphysics, charge separation mechanisms, and thundercloud electrical structure have significantly improved lightning forecasting. The selection and tuning of parameterization schemes, particularly for microphysics (MP), cumulus (Cu), and lightning (LP) processes, play a critical role in enhancing model performance and accuracy.

   This study uses various parameterization schemes to evaluate the performance of the Weather Research and Forecasting (WRF) model in simulating lightning and thunderstorm events. A severe thunderstorm event on May 14, 2022, over eastern India (West Bengal and Jharkhand), which recorded a peak 30-minute flash count of ~8000 flashes observed by the Indian Lightning Location Network (ILLN) was simulated in the WRF model. A total of 57 combinations of MP, Cu, and LP schemes were tested, using three nested domains (27 km, 9 km, 3 km) and analyzed the output of the inner domain (3 km). Seven MP schemes (WSM-6, Goddard, Thompson, Milbrandt, Morrison, WDM-5, WDM-6), two Cu schemes (Kain-Fritsch, Multi Kain-Fritsch), and two LP schemes (LP1: vertical velocity-based; LP2: 20 dBZ reflectivity-based) were assessed. 

   Results show better performance of LP2 over LP1 with higher correlation and lower standard deviation with the observed flash counts. For cumulus parameterization, Kain-Fritsch (KF) turned off for the inner domain, and achieved strong performance (correlation: 0.75–0.95) with lower RMSE and standard deviation. Among MP schemes, Morrison, Goddard, and WDM-6 consistently performed well across different combinations. The best-performing simulations included Goddard (LP2, KF on), Morrison (LP2, KF on), WDM-6 (LP2, KF off), and WDM-5 (LP2, KF on), achieving correlations of 0.94, 0.93, 0.91, and 0.91 with observed flash counts, respectively. This study underscores the WRF model's capability in simulating lightning activity with optimal parameterization combinations, particularly LP2 and KF schemes. These findings provide promising results for real-time lightning forecasting, aiding in mitigating lightning-related hazards.

How to cite: Rinuragavi, V., Biswasharma, R., Umakanth, N., and Pawar, S.: Evaluating Microphysics, Cumulus, and Lightning Parameterization Schemes in WRF Model for Thunderstorm Simulation Over East India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14876, https://doi.org/10.5194/egusphere-egu25-14876, 2025.

EGU25-14901 | Orals | NH1.6

Characterization of thunderstorms in South China that produced gigantic jets in a burst manner 

Gaopeng Lu, Hailiang Huang, and Yiwei Zhao

 

Since the summer season of 2020, with the contributions from amateurs sited at different places mainly in the southern part of China, we have obtained the optical observations (most in colorful mode with relatively high image resolution) for nearly 1000 transient luminous events (TLEs). One of the major findings is that the coastal thunderstorms typically originating from somewhere in South China Sea could produce a burst of gigantic jets (GJs) during a special stage of its lifetime. We selected three thunderstorm cases of this situation and combine all available observational datasets (such as satellite brightness temperature, lightning detection, and radar reflectivity, etc.) to characterize the parent thunderstorms from several different perspectives. The general results regarding the features of thunderstorms in South China capable of producing GJs including a burst of overshooting thundercloud top penetrating the local tropopause, active lightning activity between the major charge regions, and also the elevated bottom of the thunderstorms. More detailed analyses regarding the genesis of GJ outbreak during a short time period of these thunderstorms are being implemented.

How to cite: Lu, G., Huang, H., and Zhao, Y.: Characterization of thunderstorms in South China that produced gigantic jets in a burst manner, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14901, https://doi.org/10.5194/egusphere-egu25-14901, 2025.

EGU25-15529 | ECS | Orals | NH1.6

Towards predicting lightning and TLE’s in exoplanetary atmospheres  

Marrick Braam, Assaf Hochman, Thaddeus Komacek, Denis Sergeev, Yoav Yair, Roy Yaniv, Meirion Hills, and Daniel Mitchard

Electrical processes such as lightning and transient luminous events (TLEs) are important drivers of chemical processes in planetary atmospheres, including potentially facilitating the formation of important prebiotic molecules. The numerous extrasolar planets discovered present a huge diversity in environmental conditions to explore the possible emergence of electrical processes. To this end, we adapt general circulation models to simulate these exoplanet atmospheres and study the potential emergence of electrical processes. Here, we present results from simulations of tidally locked rocky exoplanets with the Met Office Unified Model. Lightning parameterisations that use bulk cloud properties - such as cloud-top height, frozen water content, and graupel flux - are initially used to infer lightning flash rates. For tidally locked exoplanets, we find that lightning is limited to the permanent dayside hemisphere, with substantial spatial and temporal variations. We then discuss methods to determine the charge structure and thus electric field strengths in the atmospheres, that can be used to infer whether lightning flashes can be followed by TLEs. Finally, we put the electrical processes into context of the atmospheric chemistry and potential observational consequences.

How to cite: Braam, M., Hochman, A., Komacek, T., Sergeev, D., Yair, Y., Yaniv, R., Hills, M., and Mitchard, D.: Towards predicting lightning and TLE’s in exoplanetary atmospheres , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15529, https://doi.org/10.5194/egusphere-egu25-15529, 2025.

EGU25-15628 | Posters on site | NH1.6

The difference between multiple TGFs and FGFs 

Nikolai Ostgaard, Anders Fuglestad, Andrey Mezentsev, Martino Marisaldi, David Sarria, Torsten Neubert, Olivier Chanrion, Freddy Christiansen, Frencisco Gordillo-Vazques, and Alejandro Luque

Atmosphere Space Interaction Monitor (ASIM) has been in operation since 2018 to observe Terrestrial Gamma-ray flashes (TGFs) and optical signals from lightning. ASIM has two payloads, the Modular X- and Gamma-ray Sensor (MXGS) and the Modular Multi-Spectral Imaging Assembly (MMIA). MXGS consists of two detector layers, one pixelated detector in the low energy range (50 keV to 400 keV) and another in the high energy range (300 keV to >30 MeV), with temporal resolution of 1µs and 28 ns, respectively.  MMIA has three photometers (337 nm, 180-230 nm, 777 nm) and two cameras (337 nm and 777 nm). During nighttime we observe both the TGFs and the lightning that produced them.

 

Multiple and double TGFs  separated by 1-2 ms have frequently been observed by ASIM. Here we present double TGFs, which  were all associated with  optical pulses from a hot leader (777 nm). Furthermore the first and second pulses come from the same location, indicating that the double TGFs are produced by the same leader as it propagates upward.

 

A related but different gamma-ray phenomenon was observed during the ALOFT campaign in 2023, when more than 25 Flickering Gamma.ray Flashes were observed. The FGFs are trains of pulsed gamma-ray emissions, each pulse lasting typically 1-2 ms and the entire FGF last about 50-100 ms. The FGFs have no associated detectable optical or radio signal, which differentiate them from the multi-TGFs. The FGFs observed during the ALOFT campaign were all too weak to be seen from space.

 

However, in May 2024 ASIM passed over pulsed gamma-ray emissions which was identical to the FGFs seen by ALOFT, but contrary to the ones observed by ALOFT,  this FGF was bright enough to be seen from space.

Unfortunately, the FGF occurred  during day-time over the coast of West Africa, so no optical data were available - and radio coverage is also very poor in this region.

How to cite: Ostgaard, N., Fuglestad, A., Mezentsev, A., Marisaldi, M., Sarria, D., Neubert, T., Chanrion, O., Christiansen, F., Gordillo-Vazques, F., and Luque, A.: The difference between multiple TGFs and FGFs, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15628, https://doi.org/10.5194/egusphere-egu25-15628, 2025.

EGU25-15696 | Orals | NH1.6

A statistical study of lighting-induced electron precipitation (LEP) events observed by the CSES-01 satellite 

Coralie Neubüser, Roberto Battiston, William Jerome Burger, Francesco Maria Follega, Emanuele Papini, Alessio Perinelli, Mirko Piersanti, and Dario Recchiuti

The CSES-01 satellite, with its versatile set of payloads, is able to detect short bursts of lightning-induced electron precipitation (LEP) simultaneously with injected up-going whistler waves. The electron bursts are identified individually for each telescope of the low-energy detector of the high-energy particle package (HEPP-L) within the energy range from 100 to 250 keV. The whistler wave detection is based on the power spectral density of the magnetic field in the frequency range from 1 to 10 kHz, measured by the search coil magnetometer (SCM). The wave and particle observations of CSES-01 are complemented by the ground-based lightning network of the World Wide Lightning Location Network (WWLLN). The found LEP events occur within ≤120 ms of the causative lightning discharge. A statistical study of the LEP events has been performed, which includes a background estimation for the wave-particle correlation. The identified LEP events are found to be shifted significantly polewards of the initial lightning and extend over some 1000 km longitudinally. In addition, it was found that the distance from the LEP event to the lightning decreases as the absolute lightning latitude increases. This finding is in agreement with models of electron interaction with obliquely propagating lightning-generated whistlers and observations from previous missions.

How to cite: Neubüser, C., Battiston, R., Burger, W. J., Follega, F. M., Papini, E., Perinelli, A., Piersanti, M., and Recchiuti, D.: A statistical study of lighting-induced electron precipitation (LEP) events observed by the CSES-01 satellite, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15696, https://doi.org/10.5194/egusphere-egu25-15696, 2025.

EGU25-15838 | Orals | NH1.6

New Class of Gamma-Ray Flashes Indicate Gamma Glow Reset through Fast Streamer Discharge. 

Andrey Mezentsev, Nikolai Østgaard, Martino Marisaldi, Steven Cummer, Yunjiao Pu, Eric Grove, Mason Quick, Hugh Christian, Marni Pazos, Mark Stanley, David Sarria, Timothy Lang, Cristopher Schultz, and Richard Blakeslee

Recent aircraft campaign over the Caribbean region in July 2023, called ALOFT, resulted in several discoveries that significantly improved our understanding of atmospheric gamma-ray phenomena. It was demonstrated that strong convective systems produce strong, long lasting electric fields that generate highly dynamic gamma-ray glow emissions. About 600 individual glows, arranged in tens of glowing episodes were recorded, a certain part of which show abrupt decrease in photon flux due to some electrical discharge leading to reduction of the electric field in the active region. Many of those abruptly reset glows bear a bright terrestrial gamma-ray flash (TGF) at the very apex of the gamma-ray glow. All these TGFs are closely followed by a fast streamer discharge recorded as a positive narrow bipolar event (NBE) in radio and as a strong optical pulse in the 337 nm blue light emission with very little contribution in the 777.4 nm red light emission. This indicates that the +IC leader is not involved in this process, contrary to “conventional” leader-related TGFs usually observed from space. The partial discharge of the active volume and the gamma glow reset is achieved through the fast streamer discharge. The TGFs associated with this gamma glow reset process have very short rise time, short duration peak phase, and low fluence, which makes them undetectable from space and kept them undiscovered until the ALOFT campaign.

How to cite: Mezentsev, A., Østgaard, N., Marisaldi, M., Cummer, S., Pu, Y., Grove, E., Quick, M., Christian, H., Pazos, M., Stanley, M., Sarria, D., Lang, T., Schultz, C., and Blakeslee, R.: New Class of Gamma-Ray Flashes Indicate Gamma Glow Reset through Fast Streamer Discharge., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15838, https://doi.org/10.5194/egusphere-egu25-15838, 2025.

EGU25-16145 | Posters on site | NH1.6

Optical and radio emissions from different high-energy electron acceleration mechanisms 

Nikolai Lehtinen, Øystein Håvard Færder, David Sarria, Andrey Mezentsev, Martino Marisaldi, and Nikolai Østgaard

Electric fields in thunderclouds can accelerate electrons to relativistic energies, which leads to bremsstrahlung production of gamma radiation. This radiation was recently recorded by the ALOFT experimental aircraft campaign [1], and may be classified into various types according to their lightcurve shapes, for example, flickering gamma flashes (FGF), single and multiple terrestrial gamma flashes (TGF), and extended gamma-ray glows (GRG). Electromagnetic field in radio and optical range was also recorded, and has different features for the enumerated gamma radiation types.

The relativistic runaway electrons may be produced in various ways. We consider two different mechanisms: (1) electrons are accelerated from low energies in high fields at the tips of long streamers, and (2) runaway electrons grow in large-scale (km-size) avalanches sustained by relativistic feedback mechanism [2].

The first mechanism (long streamers) is analyzed using the novel Streamer Parameter Model (SPM) [3]. This model had been shown to agree with experiments for laboratory-size streamers, and here it is applied to streamers exceeding several meters in length. Such long streamers may describe the fast positive and negative breakdown (FPB/FNB), experimentally observed in thunderstorms. The long streamers, compared to regular laboratory-observed streamer, are predicted to have higher (subluminal) velocities, higher electric fields at the tip, and wider tips. These factors all facilitate production of large quantities of relativistic runaway electrons and, therefore, efficient radiation of x-rays in the form of short pulses, which may be observed as TGF. The currents radiate a short electromagnetic pulse similar to the observed narrow bipolar events (NBE).

The second mechanism (large-scale feedback) is analyzed using the recently developed 0.5D FGF model [4] which is a dynamic model of electric field and cloud conductivity connected through production of relativistic runaway electrons, secondary electrons and ions. This model describes a system in which oscillations may be excited by changing external field [2]. For various set of parameters (such as the system size, and time scale and strength of the external field change), as analyzed by [4], one may obtain gamma radiation lightcurves similar to all the observed types listed above. Charge redistributions and electric currents, for certain sets of parameters, may produce detectable electromagnetic fields.

For both mechanisms, we also calculate optical radiation excited by secondary electrons and estimate its detectability.

[1] N. Østgaard et al, Flickering gamma-ray flashes, the missing link between gamma glows and TGFs. Nature, 634, p. 53-56, 2024. doi:10.1038/s41586-024-07893-0.

[2] N. Liu and J. R. Dwyer. Modeling terrestrial gamma ray flashes produced by relativistic feedback discharges. J. Geophys. Res.–Space, 118 (5), p. 2359-2376, 2013. doi:10.1002/jgra.50232.

[3] N. G. Lehtinen (2021). Physics and Mathematics of Electric Streamers, Radiophys Quantum El, 64, p. 11-25, doi:10.1007/s11141-021-10108-5.

[4] Færder et al, this session.

How to cite: Lehtinen, N., Færder, Ø. H., Sarria, D., Mezentsev, A., Marisaldi, M., and Østgaard, N.: Optical and radio emissions from different high-energy electron acceleration mechanisms, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16145, https://doi.org/10.5194/egusphere-egu25-16145, 2025.

EGU25-16240 | Posters on site | NH1.6

Evidence of gamma-ray glows observed in the relativistic feedback regime during the ALOFT 2023 flight campaign 

David Sarria, Nikolai Østgaard, Martino Marisaldi, Andrey Mezentsev, Nikolai Lehtinen, Ingrid Bjørge-Engeland, Anders Fuglestad, Timothy J. Lang, and Mark A. Stanley and the The ALOFT Team

In July 2023, the ALOFT flight campaign deployed an ER-2 research aircraft that flew at 20 km altitude above thunderstorms, carrying an extensive suite of instruments. The campaign observed numerous gamma-ray glows exhibiting complex and highly dynamic morphologies (Marisaldi et al. 2024). This study focuses on two specific glow events recorded on July 29th, 2023, between 20:30:20 and 20:31:40 UTC over Florida. By combining Monte Carlo simulations with observations from hard-radiation instruments and ground-based interferometers, we can estimate the multiplication factor required, based on cosmic-ray secondary electrons, to produce gamma-ray glows of the observed magnitude (exceeding 7 times the background level on the ALOFT-BGO detector).

Our analysis reveals multiplication factors of seed electrons (cosmic-ray secondaries) significantly exceeding a factor 5000, occurring multiple times and persisting for periods of several seconds. According to previous studies (Dwyer et al. 2007; Kelley et al. 2015), such high multiplication factors indicate substantial contribution from the Relativistic Feedback Discharge mechanism. Using the methodology established by Kelley et al. (2015), we estimated that the discharge currents resulting from the relativistic process during high-intensity phases of the glow could range in the tens to hundreds of amperes. These values substantially exceed those previously reported by Kelley et al. (2015) and could be large enough to significantly influence the thunderstorm's charging rate.

This study provides evidence that the Relativistic Runaway Electron Avalanche process, amplified by the relativistic feedback mechanism, could compete with conventional discharge mechanisms in certain thunderstorm conditions.

References:

  • Marisaldi, M., Østgaard, N., Mezentsev, A., Lang, T., Grove, J. E., Shy, D., Heymsfield, G. M., Krehbiel, P., Thomas, R. J., Stanley, M., Sarria, D., Schultz, C., Blakeslee, R., Quick, M. G., Christian, H., Adams, I., Kroodsma, R., Lehtinen, N., Ullaland, K., Yang, S., Qureshi, B. H., Søndergaard, J., Husa, B., Walker, D., et al. (2024). Highly dynamic gamma-ray emissions are common in tropical thunderclouds. Nature. https://doi.org/10.1038/s41586-024-07936-6
  • Kelley, N. A., Smith, D. M., Dwyer, J. R., Splitt, M., Lazarus, S., Martinez-McKinney, F., Hazelton, B., Grefenstette, B., Lowell, A., & Rassoul, H. K. (2015). Relativistic electron avalanches as a thunderstorm discharge competing with lightning. Nature Communications.  https://doi.org/10.1038/ncomms8845
  • Dwyer, J. R. (2007). Relativistic breakdown in planetary atmospheres. Physics of Plasmas. https://doi.org/10.1063/1.2709652

How to cite: Sarria, D., Østgaard, N., Marisaldi, M., Mezentsev, A., Lehtinen, N., Bjørge-Engeland, I., Fuglestad, A., Lang, T. J., and Stanley, M. A. and the The ALOFT Team: Evidence of gamma-ray glows observed in the relativistic feedback regime during the ALOFT 2023 flight campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16240, https://doi.org/10.5194/egusphere-egu25-16240, 2025.

EGU25-16451 | ECS | Posters on site | NH1.6

Investigating the termination mechanisms of gamma-ray glows observed during the ALOFT aircraft campaign 

Ingrid Bjørge-Engeland, Nikolai Østgaard, Martino Marisaldi, Andrey Mezentsev, Anders N. Fuglestad, David Sarria, Nikolai Lehtinen, Timothy J. Lang, Christopher Schultz, Hugh Christian, and Mason G. Quick

During the Airborne Lightning Observatory for FEGS and TGFs (ALOFT) campaign conducted in the summer of 2023, hundreds of gamma-ray glows were observed. Numerous glow regions, each consisting of several individual glows, were observed as the aircraft passed over active thunderstorms (Marisaldi et al. 2024). We will investigate the mechanisms behind the termination of the individual glows, focusing on whether specific types of discharges are responsible or if the glows terminate themselves. We will combine observations from different instruments onboard the aircraft, including gamma-ray detectors, electric field change meters and photometers. Lightning discharges will be characterized by optical emissions and data from on-board electric field change meters. We also couple this with detections by the ground-based lightning location network GLD360.

 

References:

  • Marisaldi, M., Østgaard, N., Mezentsev, A., Lang, T., Grove, J. E., Shy, D., Heymsfield, G. M., Krehbiel, P., Thomas, R. J., Stanley, M., Sarria, D., Schultz, C., Blakeslee, R., Quick, M. G., Christian, H., Adams, I., Kroodsma, R., Lehtinen, N., Ullaland, K., Yang, S., Qureshi, B. H., Søndergaard, J., Husa, B., Walker, D., et al. (2024). Highly dynamic gamma-ray emissions are common in tropical thunderclouds. Nature. https://doi.org/10.1038/s41586-024-07936-6

 

How to cite: Bjørge-Engeland, I., Østgaard, N., Marisaldi, M., Mezentsev, A., Fuglestad, A. N., Sarria, D., Lehtinen, N., Lang, T. J., Schultz, C., Christian, H., and Quick, M. G.: Investigating the termination mechanisms of gamma-ray glows observed during the ALOFT aircraft campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16451, https://doi.org/10.5194/egusphere-egu25-16451, 2025.

EGU25-17913 | ECS | Posters on site | NH1.6

Tree and Forest Traits Influencing Lightning Strike Probability 

Bianca Zoletto, Masha Van der Sande, Peter Van der Sleen, Dennis Babaasa, Aventino Nkwasibwe, Evan Gora, Martin Sullivan, and Aida Cuni-Sanchez

Lightning is a significant disturbance agent in tropical forests, with ecological impacts including tree mortality and influencing forest structure and carbon dynamics. Our research explores the environmental and tree-specific factors affecting the probability of a tree being struck by lightning in Afromontane forests. We surveyed 89 kilometers of transects across ridges, slopes, and valleys in Bwindi Impenetrable National Park, Uganda, and recorded 94 lightning strikes.

Our findings reveal that topography significantly influences strike probability, with ridges experiencing the highest strike density (2.0 strikes/km) compared to slopes (1.4 strikes/km) and valleys (0.25 strikes/km). Elevation alone was not a significant predictor when topography was included, suggesting that a tree's relative position in the landscape plays a crucial role.

At the individual tree level, struck trees were not always the tallest within a 20-meter radius plot. Only 30% of struck trees had the largest diameter at breast height (DBH), and 19.5% were the tallest, highlighting the influence of factors beyond size. However, struck trees exhibited a higher median DBH and a greater proportion of emergent canopy trees compared to controls. Generalized Linear Mixed Models (GLMM) identified DBH (Estimate = 0.025, p < 2.39e-06) and canopy exposure (Estimate = 1.20, p = 2.04e-08) as significant predictors of strike probability.

These results suggest that lightning strikes are influenced by a combination of environmental and tree-specific traits, including topographical context, DBH, and canopy exposure. Our findings contribute to understanding lightning as a selective agent in tropical forests, with implications for forest dynamics and carbon storage.

How to cite: Zoletto, B., Van der Sande, M., Van der Sleen, P., Babaasa, D., Nkwasibwe, A., Gora, E., Sullivan, M., and Cuni-Sanchez, A.: Tree and Forest Traits Influencing Lightning Strike Probability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17913, https://doi.org/10.5194/egusphere-egu25-17913, 2025.

EGU25-18036 | Posters on site | NH1.6

Testing the hypothesis of lightning initiation by runaway air breakdown with ALOFT data 

Martino Marisaldi, Nikolai Østgaard, Andrey Mezentsev, David Sarria, Nikolai Lehtinen, Ingrid Bjørge-Engeland, Anders Fuglestad, Øystein Færder, Timothy J. Lang, Mason Quick, Richard Blakeslee, Hugh Christian, J. Eric Grove, Daniel Shy, Steven A. Cummer, Yunjiao Pu, and Marni Pazos

Lightning initiation is one of the top unsolved problems in atmospheric electricity. Runaway electron breakdown of air has been suggested to play a key role in lightning initiation, by locally enhancing the ambient electric field above the conventional breakdown threshold. The recent results from the ALOFT flight campaign have shown a tight interconnection between highly convective cores, lightning activity, and high-energy particle acceleration observed as a wide range of gamma-ray phenomena (gamma-ray glows, Terrestrial Gamma-ray Flashes, and the recently reported Flickering Gamma-ray Flashes). Thanks to the combination of simultaneous, high-sensitivity gamma-ray, optical and radio measurements, the ALOFT dataset provides a unique opportunity to investigate the lightning initiation problem and test the runaway breakdown hypothesis. Here we focus on the lightning discharges observed within the field of view of the gamma-ray instrument and not associated to any detectable gamma-ray enhancement. We will try to answer the following questions: how many discharges are there unambiguously not associated to gamma-rays? What are the characteristics of these discharges? What can we infer about the hypothesis of lightning initiation triggered by runaway air breakdown?

How to cite: Marisaldi, M., Østgaard, N., Mezentsev, A., Sarria, D., Lehtinen, N., Bjørge-Engeland, I., Fuglestad, A., Færder, Ø., Lang, T. J., Quick, M., Blakeslee, R., Christian, H., Grove, J. E., Shy, D., Cummer, S. A., Pu, Y., and Pazos, M.: Testing the hypothesis of lightning initiation by runaway air breakdown with ALOFT data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18036, https://doi.org/10.5194/egusphere-egu25-18036, 2025.

EGU25-18046 | ECS | Orals | NH1.6

Comparing Upward Negative Stepped Leader and Preliminary Breakdown Pulses 

Toma Oregel-Chaumont, Mohammad Azadifar, Antonio Šunjerga, Marcos Rubinstein, and Farhad Rachidi

The study explores the characteristics of upward negative stepped leader pulses recorded at the Säntis Tower in Switzerland. Analysis of simultaneous channel-base current and 14.7-km vertical electric field data revealed two distinct types of pulses associated with upward negative stepped leaders [2].
Category A pulses were characterized by bipolar electric field signatures with initial positive half-cycles, correlated with negative unipolar current pulses. The E-field pulses had an average duration of 23.7 (± 11.7) μs and exhibited time-dependent characteristics, including increased frequency and slower risetimes.
Category B pulses were characterized by unipolar (positive or negative) or bipolar field signatures that lacked correlation with any major current pulses. These had narrower temporal widths compared to Category A pulses.
As discussed in Azadifar et al. 2018 [3], notable similarities exist between these two categories and, respectively, “Classical” and “Narrow” Preliminary Breakdown Pulses (PBPs) observed in the initial stages of downward negative leaders [6].
Herein, we present a statistical analysis of 45 Category A pulses from 5 Type-II upward positive flashes, which confirms their similarity to Classical PBPs, particularly in regards to key characteristic timescales reported in the literature, such as the aforementioned pulse duration [1,4,5,6,10], 10-90% risetime (6.1 ± 3.6 μs) [1,9], and zero-crossing time (11.9 ± 6.1 μs) [1,9]. In this dataset, 7 (~16%) of these bipolar pulses were observed to be inverted (with a negative initial half-cycle), and were excluded from this preliminary analysis, though it is of note that a similar phenomenon has been observed in downward stepped leaders as well [8].
The temporal widths of the initial and second half-cycles were observed to be linearly correlated (with correlation coefficient ρ = 0.77), as were their peak amplitudes (ρ = -0.80). Further linear correlations were found to exist between the peak E-field and current amplitudes (R2 = 0.74), as well as their risetimes (R2 = 0.73), with E-field pulses generally rising faster than current pulses. To the best of our knowledge, these specific relationships have not been reported in the literature, though correlations between PBP amplitude and: duration [7], and return stroke peak current [10] have been observed.
These findings enhance our understanding of upward lightning phenomena and associated electromagnetic radiation, revealing parallels with the Breakdown, Intermediate, and Leader stages of downward negative flashes. This study contributes to the ongoing debate about the underlying physical mechanisms of lightning initiation and propagation, and highlights the need for further research in this area. Observational studies are specifically recommended to validate these correlations and refine proposed modeling frameworks.

 

References:


[1] Adhikari & Adhikari (2021). Scientific World Journal, 2021, 1–9.


[2] Azadifar et al. (2015). XIII SIPDA, 32–36.


[3] Azadifar et al. (2018). 34th ICLP, 1–6.


[4] Cai et al. (2022). Atmospheric Research, 271, 106126.


[5] Granados et al. (2022). TecnoLógicas, 25(55), e2343.


[6] Nag & Rakov (2008). JGR: Atmospheres, 113(D1).


[7] Nag et al. (2009). Atmospheric Research, 91(2–4), 316–325.

[8] Ogawa (1993). Journal of Atmospheric Electricity, 13(2), 121–132.

[9] Shi et al. (2024). Remote Sensing, 16(20), 3899.


[10] Zhu et al. (2016). Atmosphere, 7(10), 130.

How to cite: Oregel-Chaumont, T., Azadifar, M., Šunjerga, A., Rubinstein, M., and Rachidi, F.: Comparing Upward Negative Stepped Leader and Preliminary Breakdown Pulses, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18046, https://doi.org/10.5194/egusphere-egu25-18046, 2025.

EGU25-18235 | ECS | Orals | NH1.6

Assimilation of Rainfall and Total Lightning Data for Nowcasting Torrential Rainfall During Summer Thunderstorms in Japan 

Debrupa Mondal, Yasuhide Hobara, Hiroshi Kikuchi, and Jeff Lapierre

Recently, detailed spatio-temporal analysis, using X-band multi-parameter radar-derived 3D volume scan and total lightning data in Japan, have revealed the peak in-cloud (IC) lightning occurs ~10 mins before maximum ground precipitation for individual cells of a summer thunderstorm (TS) producing torrential rain. This study investigates the potential of utilizing the total lightning data for monitoring and short-term prediction of torrential rain during three summer TS events causing heavy rainfall over Japan: an isolated TS, a TS possessing a merging of two cells, and a splitting TS cell. We construct simple linear regression models using (1) only ground precipitation volume (PV) and (2) a combination of ground PV and IC pulse rate. These models are continuously updated with the latest observations of IC and ground PV values to predict the one-step and multi-step ahead values of ground rainfall. We demonstrate a promising approach for short-term prediction of ground rainfall, by simultaneous application of the current and historical data of IC pulse rate and PV, which showed high accuracy (cross-correlation coefficient between observed and predicted PV was 0.84~0.94).

How to cite: Mondal, D., Hobara, Y., Kikuchi, H., and Lapierre, J.: Assimilation of Rainfall and Total Lightning Data for Nowcasting Torrential Rainfall During Summer Thunderstorms in Japan, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18235, https://doi.org/10.5194/egusphere-egu25-18235, 2025.

EGU25-19743 | ECS | Posters on site | NH1.6

First Simulations of Lighthing Optical Observations during Daytime in the Context of the C³IEL Mission 

Antoine Rimboud, Eric Defer, Céline Cornet, François Thieuleux, and Didier Ricard

For over two decades, optical observations from low Earth orbit satellites have enabled the creation of the first global map of lightning activity. Today, the latest generation of geostationary meteorological satellites, such as the European Meteosat Third Generation (MTG) Lightning Imager (LI), is equipped with lightning imagers. Additionally, instruments like the Lightning Imaging Sensor (LIS) and the Atmosphere-Space Interactions Monitor (ASIM) on board the International Space Station detect optical lightning signals across various wavelengths, ranging from near-UV to near-IR, with cameras and photometers.

Understanding the radiative transfer of light generated by lightning discharges within clouds is crucial for interpreting detected optical signals. In this work, the three-dimensional radiative transfer code 3DMCPOL (Cornet et al., 2010) is adapted to simulate realistic lightning waveforms and images. The 3DMCPOL code simulates light propagation through three-dimensional atmospheres using the Monte Carlo method, originally for solar or thermal sources. A realistic four-dimensional (time and space) lightning source was implemented (Rimboud et al., 2024), and its detection by ground-based or space-borne photometers and cameras.

The methodology will first be detailed, focusing on how realistic imagery observations are simulated using geometric models of the Lightning Optical Imager (LOI) developed by the French space agency for the French-Israeli C³IEL (Cluster for Cloud Evolution, Climate, and Lightning) mission currently under development. Then, simulations of realistic daytime LOI observations will be presented using the microphysical outputs of the French cloud-resolving model Meso-NH for the cloud description. First results on the necessary acquisition frequency for background scenes and the impact of tilted observations on lightning detection, will be discussed from these simulations.

How to cite: Rimboud, A., Defer, E., Cornet, C., Thieuleux, F., and Ricard, D.: First Simulations of Lighthing Optical Observations during Daytime in the Context of the C³IEL Mission, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19743, https://doi.org/10.5194/egusphere-egu25-19743, 2025.

EGU25-20073 | ECS | Orals | NH1.6

High-Speed Ultraviolet and Visible Optical Emission Spectroscopy of High-Voltage Impulses Representing Lightning 

Meirion Hills, Daniel Mitchard, and Nicolas Peretto

To better understand lightning interactions with the atmosphere, a high-speed (streak) spectrograph was used to characterise various high voltage impulses representing lightning. A Marx generator was used to produce 1.2/50 μs high voltage impulses, according to the IEC 60060 standard, ranging from 60 kV to 160 kV. The atomic emission spectrum was captured using a high-speed streak system at resolutions of 0.35 μs/pixel to 0.14 μs/pixel. Spectral data were first recorded over a broad range of 250 to 990 nm, covering a part of the ultraviolet spectrum, full visible spectrum and into near-infrared. Then three smaller bands were chosen for high resolution spectral data to enable the identification of key atomic emission lines such as Oxygen-I, Nitrogen-I and II, and Argon-I from the atmosphere, as well as Tungsten-I from the experiment electrodes. It was observed that an increase in high voltage lead to greater spectral intensity with more prominent lines, as expected, indicating an increase in energy transfer into the surrounding atmosphere. Subsequent analysis of the data resulted in both temperature and energy measurements of these arcs. Such spectral signatures have important implications for refining atmospheric electricity models and better understanding risks associated with lightning, particularly for built infrastructure, such as struck power lines and wind turbines, but also natural features, like forests and woodland. It is the intention that this work will progress onto the study of spectra from laboratory generated lightning arcs.

How to cite: Hills, M., Mitchard, D., and Peretto, N.: High-Speed Ultraviolet and Visible Optical Emission Spectroscopy of High-Voltage Impulses Representing Lightning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20073, https://doi.org/10.5194/egusphere-egu25-20073, 2025.

EGU25-21014 | ECS | Orals | NH1.6

Exploring the Effect of Wind Farms on Lightning and Storm Development 

Jacquelyn Ringhausen, Elizabeth DiGangi, Jeff Lapierre, and Yanan Zhu

With the growing use of alternative energy generation such as wind turbines, it is important to understand their effect on the environment and, in turn, on storms. One environmental parameter that could be directly impacted by wind turbines is lightning, since tall objects can enhance lightning development. Additionally, wind turbines can potentially alter the boundary layer of storms, which can cause changes in the low-level winds within the storms and affect their evolution. Several studies have been performed focusing on the lightning trends directly over specific wind farms, the attachment and upward development of lightning from turbines, and the protection of wind turbines from lightning in general; however, few studies have performed large-scale analysis of the effect turbines have on lightning and storms. This study analyzes the trends in lightning not only occurring over the wind farms but surrounding the wind farms on both a storm level, and at larger temporal and spatial scales. For this analysis, the Earth Networks Total Lightning Network (ENTLN) and the Geostationary Lightning Mapper (GLM) provide extensive lightning datasets covering CONUS, while radar data from the Multi Radar Multi Sensor (MRMS) platform offers information on storm development.  Preliminary results show a potential change in both the lightning patterns and characteristics, as well as radar echoes with storm passage over wind farms, indicating some effect may be present.

How to cite: Ringhausen, J., DiGangi, E., Lapierre, J., and Zhu, Y.: Exploring the Effect of Wind Farms on Lightning and Storm Development, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21014, https://doi.org/10.5194/egusphere-egu25-21014, 2025.

EGU25-21146 | Orals | NH1.6

TOTEM: The Top of Thunderstorms Experimental Module 

Torsten Neubert, Olivier Chanrion, and Francisco J. Gordillo-Vazquez

TOTEM is a payload for observation of the fast processes of electrical activity at the top of thunderstorm clouds and for evaluation of a new camera technology with high time resolution and dynamic range, yet with low weight, data rate and power consumption. The Atmosphere-Space Interactions Module (ASIM) on the International Space Station (2018- ) discovered high levels of blue electrical corona activity in thunderstorm cloud tops reaching into the stratosphere. The discharges represent a new pathway of perturbations to greenhouse gas concentrations at high altitudes, which affect the atmosphere's radiative properties up to 5 times more than in the lower troposphere.  However, the altitude of events and clouds are poorly resolved with the nadir-pointing instruments of ASIM. With instruments pointing at a slanted angle, TOTEM will measure the activity – and the cloud structure where they are found – with < 300 m altitude resolution to understand their regional and global impact on greenhouse gas concentrations. The instruments include neuromorphic cameras that allow image reconstruction at up to 100.000 frames per second. TOTEM is developed by an international network of scientists and engineers. It is studied under a contract with ESA. TOTEM can be implemented on the International Space Station (ISS) or other low-Earth Orbit platforms.

 

How to cite: Neubert, T., Chanrion, O., and J. Gordillo-Vazquez, F.: TOTEM: The Top of Thunderstorms Experimental Module, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21146, https://doi.org/10.5194/egusphere-egu25-21146, 2025.

Thunderstorms are components of typhoons, linear precipitation bands and supercells, which cause severe wind and flood damage and lightning strikes. Observationally tracking the time variation in their development and decay, which is directly linked to precipitation, is important for understanding and predicting precipitation and lightning discharge activity. However, general C-band radars for meteorological use cannot observe cloud particles, and Ka-band radars require a large amount of money for maintenance because the consumable parts are expensive, and there are also limits to high-resolution observations in the vertical direction because it takes time for spatial scanning. Furthermore, it is difficult to track the occurrence and initial growth of cumulonimbus clouds from the horizontal resolution problem because the cloud top altitude cannot be geometrically obtained from geostationary meteorological satellites. The central Tokyo area is facing the risk of flooding due to the limits of its drainage capacity, and it is an urgent issue to accurately grasp the movement of thunderstorms.

Our research group has achieved results in the measurement of electrostatic fields and lightning discharge radio waves associated with thunderstorm activity in the Metro Manila, as well as in 3D cloud measurement using aircraft and satellites. In this study, we will make use of this experience to construct a system that monitors the charge separation within thunderstorm and the time-dependent changes in the three-dimensional shape of clouds. We will do this by deploying three sets of cloud stereo imaging equipment that combines field-mil electric field sensors and multiple digital cameras to surround an area with a diameter of approximately 20 km in the center of Tokyo.

How to cite: Takahashi, Y.: Development of a thunderstorm monitoring system based on atmospheric electric fields and 3D cloud imaging on the ground, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21153, https://doi.org/10.5194/egusphere-egu25-21153, 2025.

EGU25-21157 | Posters on site | NH1.6

Bottom-dominated negative dipole charge structure in thunderstorms over Tibetan Plateau    

Xiushu Qie, Dongxia Liu, Fengquan Li, Zhuling Sun, Shanfeng Yuan, and Rubin Jiang

The Tibetan Plateau stands as the highest plateau globally, showcasing distinct geological and climatic characteristics. Thunderstorms there usually shows unique structural and spatiotemporal features compared to those in low-altitude plains, and they typically exhibited small size, short duration, lower charging and flash rate. Using the data from the accurate lightning VHF interferometer, electric field mill, fast/slow antenna and C-band radar, evolution of charge structure of thunderstorms involved in lightning discharge are investigated. Different from the lower-altitude thunderstorm usually starting from a positive dipole charge structure in the middle upper portion of cloud, the charge structure inside thunderstorm usually evolves from an initial inverted dipole charge structure. In the mature stage, it may keep the inverted dipole in the whole life cycle of the thunderstorm, or exhibit a bottom heavy tripole charge structure with a large lower positive charge center (LPCC). Under different magnitudes of the LPCC, various lightning discharges including -IC, +IC, -CG and bolt-from-blue flashes are generated, indicating the crucial effects of LPCC on the lightning discharge types.

How to cite: Qie, X., Liu, D., Li, F., Sun, Z., Yuan, S., and Jiang, R.: Bottom-dominated negative dipole charge structure in thunderstorms over Tibetan Plateau   , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21157, https://doi.org/10.5194/egusphere-egu25-21157, 2025.

EGU25-21881 | ECS | Orals | NH1.6

Comprehensive Lightning Observation Using VHF Interferometer and LHAASO

Shanfeng Yuan, Xiushu Qie, Zhuling Sun, Jizhou Feng, Zhengqi Wang, Zifan Huang, and Shaoxuan Di

EGU25-530 | ECS | Orals | HS7.2

Improving Precipitation Merging: A Generalized Two-Stage Framework Using the Signal-to-Noise Ratio Optimization (SNR-opt) 

Seokhyeon Kim, Suraj Shah, Yi Liu, and Ashish Sharma

Gauge-independent, multi-source precipitation merging methods are well-established approach for improving precipitation estimates. These methods predominantly aim to minimise uncertainty in precipitation magnitude, yet they frequently neglect errors in distinguishing between rain and no-rain events. This oversight often leads to biased merging weights and suboptimal precipitation estimates. In this study, we introduce an innovative two-stage framework called the Generalised Signal-to-Noise Ratio Optimisation (G-SNR) framework, specifically designed to address these limitations. The first stage employs the Categorical Triple Collocation-Merging (CTC-M) method for binary merging, effectively mitigating errors in rain/no-rain classification. The second stage applies Signal-to-Noise Ratio Optimisation (SNR-opt) to enhance precipitation magnitude estimates, leveraging the improved classification outcomes. Evaluation results demonstrate that G-SNR consistently surpasses both input data and existing methods in terms of binary classification and magnitude estimation. Importantly, it achieves error reductions across all percentiles, delivering robust performance for both low and extreme precipitation events. This framework provides a comprehensive and reliable solution to longstanding challenges in precipitation merging, significantly enhancing both accuracy and dependability.

How to cite: Kim, S., Shah, S., Liu, Y., and Sharma, A.: Improving Precipitation Merging: A Generalized Two-Stage Framework Using the Signal-to-Noise Ratio Optimization (SNR-opt), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-530, https://doi.org/10.5194/egusphere-egu25-530, 2025.

Reliable precipitation data from in-situ stations is often limited by inconsistent quality, resolution, and spatial coverage. This is particularly true in regions like the West Bank, where ground-based observations are scarce. This hampers hydrological and environmental studies where accurate precipitation estimates are vital.  Therefore, satellite-based rainfall products are an appealing alternative due to their broad spatial and consistent temporal coverage. However, the accuracy of these products in complex terrain is questionable due to sensor and retrieval errors, necessitating adjustment to improve their reliability. This study evaluates various adjustment methods for four satellite precipitation products (IMERG Final Run, PDIR-Now, CCS-CDR, and CMORPH) across the study area of Historical Palestine (West Bank and Israel). Daily satellite precipitation estimates were compared to observations from 316 in-situ stations (256 in Israel and 58 in the Palestinian territories). Adjustment methods included traditional bias correction techniques (Linear Scaling, Daily Translation, and Annual Sums), more advanced approaches (Empirical Quantile Mapping, Robust Quantile Mapping, Gaussian Distribution Mapping, and Local Intensity Scaling), and machine learning models (Random Forest and Artificial Neural Networks). Results show that, among the non-machine learning approaches, Daily Translation (DT) achieved the greatest improvement in accuracy followed by Power Bias adjustment. DT applied to IMERG resulted in an improvement of 24% and 17% in R2 and Mean Absolute Error (MAE) respectively. All machine learning approaches outperformed non-machine learning methods, with a two-step Random Forest (RF2) method delivering the best results. RF2, which leverages data from multiple satellites, had a 109% improvement in R2 and a 54% improvement in MAE. Additionally, the global RFG model showcased excellent results in producing a unified model that can be generalized for the entirety of the study area. The findings are globally applicable and evaluate multiple adjustment methods which opens the opportunity for easily accessible remotely sensed precipitation products to be used in many hydrological applications.

How to cite: Jayousi, F. and O'Loughlin, F.: Precision in Precipitation:  Bias Corrections and Machine Learning for Reliable Satellite Precipitation in The Levant, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-722, https://doi.org/10.5194/egusphere-egu25-722, 2025.

EGU25-841 | ECS | Orals | HS7.2

Urban runoff response to climate-change-driven heavy precipitation and urbanization 

Raz Nussbaum, Moshe Armon, and Efrat Morin

Excess runoff from heavy precipitation events (HPEs) in urban environments often leads to urban flooding, a severe hazard with significant implications for human life, property, and infrastructure. Modeling runoff response in complex and heterogeneous urban areas, while accounting for rainstorm and surface characteristics, remains a significant challenge. Climate change and urbanization are key drivers of increased future urban runoff intensity. Research on the interaction between these factors and urban runoff in the eastern Mediterranean region is particularly limited. Previous studies using high-resolution models have projected an increase in short-duration rainfall intensities, alongside a decrease in long-duration intensities, rainfall coverage area, and total event rainfall during HPEs in the eastern Mediterranean under the RCP8.5 scenario. The current study examines the implications of these changes on peak discharge and volume of urban runoff by the end of the 21st century and evaluates the influence of varying urbanization scenarios, providing insights into the interplay between climate change and urban development. Using high-resolution radar-rainfall and surface data, we developed and calibrated a SWMM-based urban rainfall-runoff model for the Nahal Ra'anana basin (13 km²) on Israel's coastal plane. This Mediterranean-climate region encompasses most of the city of Ra'anana and has approximately 40% impervious surfaces. The model was developed using 23 runoff events utilizing leave-one-out cross-validation and a multi-objective optimization approach, and demonstrated robust performance with KGE values of 0.80 for runoff peak discharge and 0.83 for total runoff volume. A variance-based sensitivity analysis identified three primary factors influencing urban runoff: rainstorm intensity distribution, impervious surface coverage, and basin water storage. Analysis of HPEs under historical and future climatic conditions revealed that, at the current urbanization level of the city, climate change alone is unlikely to alter peak or total runoff discharge significantly. This is attributed to the decrease in total event rainfall and coverage area, alongside an increase in short-duration rainfall intensities. However, with substantial urbanization (e.g., increasing impervious surface to 52% or more), future climate HPEs are expected to exhibit a noticeable shift in the trend, leading to increased peak discharge. Further analysis indicates the elevated importance of rainfall intensities in determining runoff peaks in future climate conditions. In historical HPEs the maximum rainfall intensities over a 60-minute duration strongly correlate with peak runoff discharge (R2=0.75), where in future climate HPEs, correlations of shorter and longer rainfall durations are improved compared to historical HPEs with the maximum obtained for 60–120-minute durations (R2=0.81). The non-linear discharge response to climate change underscores the importance of integrating climate projections into urban planning to mitigate future flooding risks and highlight the potential for short-term peak discharge forecasting under both current and future climatic conditions.

 

How to cite: Nussbaum, R., Armon, M., and Morin, E.: Urban runoff response to climate-change-driven heavy precipitation and urbanization, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-841, https://doi.org/10.5194/egusphere-egu25-841, 2025.

EGU25-1018 | ECS | Posters on site | HS7.2

Statistical Downscaling Techniques and Projection of Future Climate Extremes in the Sudano Sahelian Environment 

Ibrahim Njouenwet and Jérémy Lavarenne

The Sudano-Sahelian Region of Cameroon (SSRC) faces significant challenges due to high rainfall variability and rapid population growth. Despite long-standing adaptation strategies, the region's vulnerability to climate variability and change remains a critical concern, prompting extensive research and calls for greater adaptation funding. In Sahelian West Africa, the decline in rainfall stations has significantly reduced data availability, hindering the calibration and evaluation of climate models and limiting their ability to accurately represent the region's climate. However, there are notable discrepancies between global and regional models regarding projected changes in precipitation patterns across specific regions and seasons, particularly in areas like the Eastern Sahel region, which includes the SSRC. Bias correction (BC) and downscaling (DS) are crucial, as these bias can be propagated into impact models. This study aims to fill the gap of localized and reliable information for climate services in the Sudano Sahelian region.

Using high-resolution rainfall data from NoCORA—daily interpolated rainfall maps for Northern Cameroon based on 418 stations (1948–2022) at 0.01° resolution (Jérémy et al., 2023)—the 25-km resolution regional climate models derived from a CMIP5 model are employed to better capture the climatology of extreme precipitation events, with kilometer-scale bias correction applied to outputs over the study area. Additionally, a subset of CMIP6 simulations is statistically downscaled to evaluate local-scale model uncertainties and compare the effectiveness of statistical and dynamical downscaling methods.

This study evaluates the performance of four state-of-the-art statistical downscaling techniques namely Linear Scaling, CDF-t, Quantile Mapping and Quantile DeltaMapping using different metrics and compares extreme precipitation changes under climate change scenarios to identify a suitable method for correcting bias in climate models projections for the period 2005-2100. The findings of this study will help impact modelers by enhancing the application of bias adjustment methods, thereby supporting the development of robust local climate change impact assessments in agriculture and hydrology domains.

Keywords : extreme precipitation, biais correction, Statistical downscaling, climate models

How to cite: Njouenwet, I. and Lavarenne, J.: Statistical Downscaling Techniques and Projection of Future Climate Extremes in the Sudano Sahelian Environment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1018, https://doi.org/10.5194/egusphere-egu25-1018, 2025.

EGU25-2058 | ECS | Posters on site | HS7.2

Refining Rainfall Erosivity Estimation: Methodological improvements towards more accurate soil erosion assessments 

Athanasios Serafeim, Roberto Deidda, Paolo Nasta, Nunzio Romano, Dario Pumo, and Andreas Langousis

Rainfall erosivity is a fundamental parameter in estimating soil erosion as it quantifies the potential of raindrops to detach soil particles and make them available for subsequent transport by surface runoff. Erosivity depends mainly on the intensity, duration, and energy of precipitation events, which directly affect the impact of raindrops on the soil surfaces and runoff. The most common methods for identifying erosive events emphasize short-duration, high-intensity rainfall events, while introducing critical thresholds for characterizing erosive events, such as the 30-minute maximum rainfall intensity (I30) and storm separation criteria (see e.g. Wischmeier and Smith, 1978, Foster et al., 1981 and Renard et al., 1997).

Nevertheless, both historical and recently proposed frameworks occasionally consolidate rainfall events that should be disaggregated according to the established six-hour dry period threshold, leading to overestimation of rainfall event durations and erosivity factors. The present study aims at refining the identification and analysis of erosive rainfall events, a key component of soil erosion prediction, by introducing an alternative approach that strictly adheres to the original criteria introduced by Wischmeier and Smith (1978) and Renard et al. (1997), ensuring precise segmentation of rainfall events when rainfall accumulation is below the 1.27 mm threshold over a six-hour period.

The proposed method classifies rainfall events as erosive when total rainfall exceeds 12.7 mm or meets intensity thresholds of 6.4 mm in 15 minutes or 12.7 mm in 30 minutes. Comparative analysis with existing approaches demonstrates improved alignment with fundamental criteria while addressing modern computational challenges, contributing to the advancement of soil erosion prediction by bridging historical methodologies with contemporary analytical precision.

References

Wischmeier, W.H., Smith, D. D. (1978) Predicting rainfall erosion losses: A guide to conservation planning. Agric. Handb. 537. US Gov. Print. Office, Washington, DC.

Foster, G.R., McCool, D.K., Renard, K.G., Moldenhauer, W.C. (1981) Conversion of the universal soil loss equation to SI metric units. J. Soil Water Conserv. 36, 355–359.

Renard, K., Foster, G., Weesies, G., McCool, D. and Yoder, D. (1997) Predicting Soil Erosion by Water: A Guide to Conservation Planning with the Revised Universal Soil Loss Equation (RUSLE). US Department of Agriculture, Agriculture Handbook No.703USDA, USDA, Washington DC.

How to cite: Serafeim, A., Deidda, R., Nasta, P., Romano, N., Pumo, D., and Langousis, A.: Refining Rainfall Erosivity Estimation: Methodological improvements towards more accurate soil erosion assessments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2058, https://doi.org/10.5194/egusphere-egu25-2058, 2025.

EGU25-2770 | Posters on site | HS7.2

A new tool for correcting the spatial and temporal pattern of global precipitation products across mountainous catchments: EcoProbSet Product 

Shima Azimi, Christian Massari, Gaia Roati, Silvia Barbetta, and Riccardo Rigon

This study aims at integrating global precipitation data into hydrological models at the catchment scale, a common practice in hydrological research. Specifically, the study investigates how biased spatial and temporal patterns in precipitation data affect model performance and uncertainty. The European Meteorological Observations (EMO) and Climate Hazards Group InfraRed Precipitation with Station data (CHIRPS) global datasets are utilized as inputs for the GEOframe-NewAGE hydrological model to simulate the hydrological processes of the mountainous Aosta Valley catchment in northwestern Italy. Subsequently, the uncertainty of the hydrological model forced with global precipitation data is assessed using a proposed method called Empirical Conditional Probability (EcoProb). The results show that, although traditional performance metrics suggest similar outcomes for the model forced with EMO and CHIRPS, the proposed uncertainty analysis reveals higher uncertainty when CHIRPS is used as the precipitation input. To leverage all useful information in the global precipitation data, the spatial correlation of CHIRPS is combined with a subset of raingauges using the EcoProb method to modify the EMO precipitation data. This approach enables the integration of the advantages of EMO and CHIRPS, which offer higher temporal and spatial correlation with ground observation, respectively, into a unified precipitation product. The combined dataset, referred to as the EcoProbSet product in this study, outperforms both the CHIRPS and EMO products, reducing the uncertainty introduced into hydrological models compared to the original global datasets.

How to cite: Azimi, S., Massari, C., Roati, G., Barbetta, S., and Rigon, R.: A new tool for correcting the spatial and temporal pattern of global precipitation products across mountainous catchments: EcoProbSet Product, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2770, https://doi.org/10.5194/egusphere-egu25-2770, 2025.

EGU25-3254 | ECS | Posters on site | HS7.2

Exploring Hourly Rainfall Extremes in a Changing Climate 

Marc Lennartz and Benjamin Poschlod

Previous research shows that for limited sample sizes applying the simplified metastatistical extreme value (sMEV) distribution instead of the more commonly used general extreme value (GEV) distribution can significantly reduce the associated uncertainty in rainfall return levels. Recent literature has also highlighted the possibility to analyze the effects of climate change using the non-stationary version of the sMEV distribution. Thus, the objective of this study is to test the performance of the sMEV and GEV for hourly precipitation using a convection-permitting regional climate model. The global climate model MIROC5 is employed to drive the regional climate model COSMO over the greater Germany area for the past, near future, and distant future. It is set up at a high temporal and spatial resolution allowing it to explicitly resolve deep convection, which is important when assessing extreme hourly precipitation. No comparable time series from a convection-permitting model has previously been analyzed using the sMEV distribution. The results show that the sMEV performs much better than the GEV in terms of the uncertainty for almost all return periods regardless of the observational years available. In addition, there is a north-south gradient in the return level difference, the uncertainty difference and the adequacy of the left-censoring threshold chosen for the sMEV. Investigating non-stationary versions of the sMEV and GEV shows that the non-stationary sMEV is more suitable to describing the change in return levels. However, both implemented versions of the non-stationary distributions are limited by the complexity of the temperature dependency. Therefore, we recommend a careful application for the prediction of return levels under higher temperatures. 

How to cite: Lennartz, M. and Poschlod, B.: Exploring Hourly Rainfall Extremes in a Changing Climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3254, https://doi.org/10.5194/egusphere-egu25-3254, 2025.

EGU25-3262 | ECS | Orals | HS7.2

How IDF Relations Changed in the Past and How They Will Change in the Future 

Felix Fauer and Henning Rust

We investigate intensity-duration-frequency (IDF) relations. They describe the major statistical characteristics of extreme precipitation events (return level, return period, time scale) and provide information on the probability of exceedance of certain precipitation intensities. IDF relations help to visualize either how extreme (in terms of probability/frequency/return period) a specific event is or which intensity is expected for a given probability. We model the distribution of extreme precipitation in an extreme-value statistics setting. To increase model efficiency, we include the duration and model a duration-dependent GEV. The durations range from minutes to days and are modeled in one single model in order to prevent quantile-crossing and to assure that estimated quantiles are consistent. This way, we are capable of considering large-scale influences by using covariates for the GEV parameters.

The influence of climate change is included by letting the GEV parameters (covariates) depend on the covariates NAO, temperature, humidity, blocking and year (as a proxy for climate change). We found an increase in probability of extreme precipitation with year and temperature, while the effect of the other variables depends on the season. We present a downscaling approach under the perfect-prognosis assumption as a proof-of-concept, where we use future values of large-scale covariates from climate projections to derive future GEV distributions. This poses some challenges because the polynomial dependencies of the past might not hold for an extrapolation into the future. Right now, our model is based on measurement stations, but we will give an outlook how we plan to include gridded datasets of precipitation observations or reanalyses.

How to cite: Fauer, F. and Rust, H.: How IDF Relations Changed in the Past and How They Will Change in the Future, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3262, https://doi.org/10.5194/egusphere-egu25-3262, 2025.

EGU25-4086 | ECS | Orals | HS7.2

Can discharge be used to inversely correct precipitation? 

Ashish Manoj J, Ralf Loritz, Hoshin Gupta, and Erwin Zehe

This study explores the feasibility of using the information contained in observed streamflow discharge measurements to inversely correct catchment-average precipitation time series provided by reanalysis products. We explore this possibility by training LSTM models to predict precipitation. The first model uses discharge as an input feature along with other meteorological factors, while the second model uses only the meteorological factors. Although the model provided with discharge information showed better mean performance, a detailed analysis of various time series measures across the continental scale revealed underestimation biases when compared with the original reanalysis product used for training. However, an out-of-sample test showed that the inversely estimated precipitation is better able to reproduce small-scale, high-impact events that are poorly represented in the original reanalysis product. Further, using the inversely generated precipitation time series for classical hydrological “forward” modeling resulted in improved estimates for streamflow and soil moisture. Given the notable disconnect between reanalysis products and extreme events, particularly in data-scarce regions worldwide, our findings have implications for achieving better estimates of precipitation associated with high-impact events.

How to cite: Manoj J, A., Loritz, R., Gupta, H., and Zehe, E.: Can discharge be used to inversely correct precipitation?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4086, https://doi.org/10.5194/egusphere-egu25-4086, 2025.

EGU25-4684 | ECS | Orals | HS7.2

Precipitation-driven storm types and their climatology across the Alpine range 

Georgia Papacharalampous, Eleonora Dallan, Moshe Armon, Joydeb Saha, Colin Price, Marco Borga, and Francesco Marra

The separation of storms into physically meaningful classes, including the key distinction between convective and non-convective events, is crucial for advancing precipitation science. Indeed, each of these classes may necessitate different modelling strategies, or distinct bias adjustment procedures for climate model simulations. Here, we present a large-scale study that aimed at achieving this separation only based on information from precipitation timeseries. We focused on a vast set of sub-hourly rain gauge records collected from four countries across the Alpine region and extracted hundreds of thousands of storms. We used an unsupervised clustering algorithm based on a small set of features to organize the storms into storm types. Despite the simplicity of the clustering approach, we successfully distinguished convective storms from other types, as validated using independent features that were not involved in the clustering, such as lightning counts. We analyzed the climatology of the storm types, including investigations of their spatial coherence and temporal changes in their occurrence. Overall, we believe that the storm clusters we provide can be used for several purposes, ranging from developing stochastic models tailored on the storm types of interests to improving bias adjustment methods for climate simulations. Given its simplicity and versatility, the framework can be transferred to other regions globally, with marginal adjustments based on the prior knowledge of the regional climatology and on the research objectives.

Our study was carried out within the RETURN Extended Partnership and received funding from the European Union Next-GenerationEU (National Recovery and Resilience Plan – NRRP, Mission 4, Component 2, Investment 1.3 – D.D. 1243 2/8/2022, PE0000005).

How to cite: Papacharalampous, G., Dallan, E., Armon, M., Saha, J., Price, C., Borga, M., and Marra, F.: Precipitation-driven storm types and their climatology across the Alpine range, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4684, https://doi.org/10.5194/egusphere-egu25-4684, 2025.

EGU25-4866 | Orals | HS7.2

Toward the stochastic modelling of extreme precipitation probability with thermodynamic and dynamic covariates 

Francesco Marra, Riccardo Ciceri, Samuele Stante, and Cinzia Sada

To properly adapt to climate change, we need to estimate extreme precipitation probability in future climate scenarios. The task is particularly challenging for sub-daily and sub-hourly extremes, as they are hardly represented by most of the available climate models. As an alternative to explicit model simulations, one can use stochastic models trained on physical covariates. For example, it was recently shown that we can predict changes in sub-daily and sub-hourly extreme precipitation only based on shifts in wet-day daily temperatures. With the aim of extending the applicability of such stochastic models, we examine here the use of covariates representing both thermodynamic and dynamic processes.

We focus on a set of ~300 stations in the Alps (from France, Switzerland, Austria, Italy) for which we have sub-daily precipitation and temperature observations. First, we assess the importance of statistical independence of the events on the identification of the scaling relationships between extreme precipitation and temperature that are commonly used to quantify the thermodynamic component. Then, we evaluate the relative importance of the thermodynamic and dynamic components for durations ranging between 10 minutes and 24 hours using as covariates dew point, vertical velocity at 500 hPa, and divergence at 300 hPa from ERA5 reanalysis simulations.

Our results show that (1) evaluating extreme precipitation-temperature scaling relations using all the wet time intervals (as done in several studies) leads to biased estimates of the scaling rates relevant for extreme sub-daily precipitation projections. (2) The scaling rates between extreme precipitation and dew point tend to decrease logarithmically with duration, an information that can be used to extract the scaling rate at sub-hourly durations from hourly observations. (3) The importance of the thermodynamic component decreases with duration (rank correlation decreases from ~0.55 at 10 minutes to ~0.2 at 24 hours), while the importance of the dynamic component that can be appreciated at the ERA5 resolution (~30 km) tends to increase with duration (rank correlation increases from ~0.2 at 10 minutes to ~0.45 at 24 hours). (4) From a stochastic simulation perspective, temperatures and dew point during precipitation events in the Alps can be simulated using generalized normal distributions (or normal distributions in case of seasonal data), while vertical velocities and divergence need to be simulated using skewed models such as a generalized extreme value distribution. 

How to cite: Marra, F., Ciceri, R., Stante, S., and Sada, C.: Toward the stochastic modelling of extreme precipitation probability with thermodynamic and dynamic covariates, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4866, https://doi.org/10.5194/egusphere-egu25-4866, 2025.

EGU25-5084 | ECS | Orals | HS7.2

Development of Rainfall Scenario with Transition Probability Reflecting on Temporal Distribution of Heavy Rainstorm Events 

Hoyoung Cha, Jongjin Baik, Jinwook Lee, Wooyoung Na, and Changhyun Jun

  This study proposes a method utilizing Rainfall Transition Probability (RTP) to create rainfall scenarios that consider the temporal distribution of heavy rainstorm events. RTP refers to the probability of rainfall amount at time t occurring after a specific rainfall amount at time t+1. The method consists of a temporal distribution that builds region-specific RTPs using rainfall data observed at 1-minute interval, a function that users define the desired conditions for the rainfall scenario, and a processing module that generates scenarios based on the RTP. To develop the RTP, the rainfall data about 1-minute interval used for separating Independent Rainstorm Events (IREs) according to each region. Among the identified IREs, those exhibiting high-intensity rainfall (above 15 mm/hour) are used to calculate and establish the RTP. Afterward, users define the conditions for the rainfall scenario in the function with conditions such as region, total rainfall, and rainfall duration. The generator then utilizes the RTP for the selected region to generate various rainfall scenarios with different temporal distributions and presents them to the user. By extracting the temporal distribution from regional IREs, the generator reflects local rainfall patterns and can be applied to regional hydrological modelling.

Keywords: Rainfall Generator, Rainfall Transition Probability, 1-minute Rainfall Data, Temporal Distribution, Heavy Rainstorm Events

 

Acknowledgment

This work was supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIT) (RS-2024-00334564).

 

How to cite: Cha, H., Baik, J., Lee, J., Na, W., and Jun, C.: Development of Rainfall Scenario with Transition Probability Reflecting on Temporal Distribution of Heavy Rainstorm Events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5084, https://doi.org/10.5194/egusphere-egu25-5084, 2025.

Abstract

In this study was investigated three different microphysics schemes on the rainfall patterns over Kuwait on 02 January 2022. The primary objective is to improve precipitation predictions using the Weather Research and Forecasting (WRF) high resolution 4 km model, which has been dynamically downscaled from the Community Climate Model version 4 (CCM4). The performance of three selected microphysics schemes—Lin, WSM6, and Thompson was evaluated using the ERA5 reanalysis dataset. ERA5 has been previously validated in this region and has consistently provided reliable results, making it a suitable dataset for such studies. Three numerical simulations were conducted using the WRF model, each incorporating one of the three microphysics schemes. The simulations were assessed by comparing the model outputs against the ERA5 data to determine the accuracy of the rainfall forecasts. The results revealed that the WRF Single-Moment 6-class microphysics scheme (WSM6) outperformed the other microphysics schemes, including Lin and Thompson, in forecasting rainfall patterns during the storm. The Lin scheme was found to be the least reliable, providing less accurate rainfall predictions compared to the Thompson and WSM6 schemes. This study highlights the critical role of selecting appropriate microphysics schemes for accurate precipitation prediction, particularly in extreme weather events like the 2022 storm in Kuwait. The findings suggest that the WSM6 scheme is a more effective choice for rainfall forecasting in this region, whereas the Lin scheme may not be as suitable for this particular type of storm event. Further research is recommended to extend this analysis to different regions and storms for more comprehensive results.

How to cite: Alsarraf, H.: Evaluation of WRF Microphysics Schemes for Precipitation Forecasting in an Arid Region: A Case Study Over Kuwait, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5123, https://doi.org/10.5194/egusphere-egu25-5123, 2025.

EGU25-6812 | ECS | Orals | HS7.2

Comparison and evaluation of different precipitation products in capturing climate extremes in Kamp Catchment, Austria 

Zryab Babker, Morteza Zagar, Tim G. Reichenau, Mohammed Basheer, and Karl Schneider

The availability of accurate long-term gap-free precipitation data at high spatiotemporal resolutions is crucial for hydroclimatic extremes assessment, water resources management, infrastructure design, hydrological modeling, and evaluation of climate change impacts. However, many ground precipitation data contain gaps, which can hinder accurate assessments and analyses. Therefore, different gridded precipitation products (PPs) are promising alternatives to overcome this deficiency, especially in heterogeneous regions with different terrains where ground observations are sparse or non-existent. This study evaluates four daily precipitation products, i.e., SPARTACUS, IMERG-V07, CHIRPS-V2.0, and ERA5-land, to determine their performance in representing observed patterns, the intensity, and frequency of extreme precipitation events in Kamp Catchment in Austria for the period 1998-2020 at different temporal scales. The Kamp River is the longest in the “Waldviertel” region and has key ecological, societal, and economic functions, with many popular leisure and excursion destinations for tourism. The catchment also frequently experiences severe floods, causing adverse socioeconomic impacts. Ground-based precipitation data from 33 stations distributed within and around the catchment are used to conduct point-to-pixel evaluation for the four products. To measure the disparity between the products and the ground observations, six performance metrics were used: the Root Mean Square Error (RMSE), Mean Absolute Error (MAE), Mean Bias Error (MBE), Nash-Sutcliffe Efficiency (NSE), Correlation coefficient (r), and Willmott index of agreement (d). The intensity and frequency of extreme precipitation reflected by the four evaluated PPs are assessed using selected extreme climate indices defined by the Expert Team on Climate Change Detection and Indices (ETCCDI). The PPs were ranked to select the best-performing product in the study area. The ranking results of the performance metrics revealed that SPARTACUS is the top-performing product on a daily and monthly scale and in capturing the frequency and intensity of precipitation extremes, followed by IMERG-V07 and ERA5-land, whereas CHIRPS-V2.0 ranked the lowest. SPARTACUS showed superior performance across the catchment with the highest correlation with the observed data and lowest bias (on daily and monthly scales, mean r values are 0.92 and 0.96 and mean MBE values are -0.02 and -0.81, respectively). Other products exhibit systematic precipitation underestimation. Regarding capturing precipitation extremes, all products show low skills and overestimate the daily extreme precipitation events, with the highest NSE of -0.32 shown in SPARTACUS. CHIRPS-V2.0 and ERA5-land presented different performances for detecting the longest wet and dry spells in the catchment. CHIRPS-V2.0 overestimated the consecutive dry days (CDD) and underestimated the consecutive wet days (CWD), whereas ERA5-land shows the opposite pattern. SPARTACUS shows minor overestimation of CDD and underestimation of CWD (MBE = -0.09 and 0.13 mm, respectively). Accordingly, a simple drought assessment was performed in the catchment using SPARTACUS data and the Standardized Precipitation Index (SPI). Our results highlight the importance of site-specific validation before using any precipitation products.

This study is conducted within the frame of the DISTENDER project (EU Horizon-ID 101056836), where climate extremes and climate change impacts upon several European catchments are analyzed and robust adaptation strategies are developed.

 

Keywords: Precipitation extremes, Precipitation products, Point-to-pixel evaluation, SPI, Kamp catchment, Austria

How to cite: Babker, Z., Zagar, M., G. Reichenau, T., Basheer, M., and Schneider, K.: Comparison and evaluation of different precipitation products in capturing climate extremes in Kamp Catchment, Austria, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6812, https://doi.org/10.5194/egusphere-egu25-6812, 2025.

EGU25-7599 | ECS | Orals | HS7.2

Prior knowledge-constrained deep learning for probabilistic precipitation downscaling 

Dayang Li, Long Yang, Baoxiang Pan, Yuan Liu, and Yan Zhou

Precipitation downscaling, particularly at convection-permitting scales (less than 4 km), is highly uncertain. This is especially pronounced in mountainous regions due to the interplay of complex topography and atmospheric dynamics. It impedes reliable estimation of variability and risks in localized extreme rainstorms. Deep learning-based downscaling methods have gained increasing attention but have primarily focused on deterministic prediction, which fails to capture uncertainty. Here we developed a novel Probabilistic High-resolution Precipitation Downscaling Network (P-HRDNet) with prior knowledge of key precipitation characteristics to design its loss function and model architecture. This knowledge includes data imbalance, skewed distribution, heteroscedasticity, and spatial and temporal dependencies of precipitation. P-HRDNet was tested in the southeastern Tibetan Plateau, a mountainous region lacking high-resolution precipitation data. Ten-year WRF simulations with nested domains provided coarse (9 km) and fine resolution (1 km) daily precipitation to train P-HRDNet. Compared with a baseline model SRCNN, P-HRDNet achieved greater accuracy in terms of root mean square error, mean absolute error, and Pearson correlation coefficient. Besides, it offers better uncertainty coverage and narrower uncertainty widths. This superiority is particularly evident in the extreme values. Our study highlights the importance of incorporating prior knowledge of precipitation characteristics into deep learning, and has a potential to physically constrain Artitifical-Intelligience (AI) based weather forecasting models. Furthermore, our WRF-AI framework offers an efficient solution for obtaining reliable high-resolution precipitation estimates in poorly gauged regions.

How to cite: Li, D., Yang, L., Pan, B., Liu, Y., and Zhou, Y.: Prior knowledge-constrained deep learning for probabilistic precipitation downscaling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7599, https://doi.org/10.5194/egusphere-egu25-7599, 2025.

Summer precipitation over High Mountain Asia (HMA) has exhibited a dipolar trend over the past 50 years. Understanding its future changes and underlying mechanisms relies heavily on climate models. However, the impact and mechanisms of model resolution on the simulation of long-term precipitation trends over the HMA remain underexplored. In this study, we use six pairs of models with high- and low-resolution comparisons from the CMIP6 all-forcing experiments to investigate the resolution-dependent differences in the long-term trends of summer precipitation from 1951 to 2024. The results show that compared to low-resolution models, the simulations from high-resolution models are closer to observations, with the largest improvement in the southern margin of the HMA and surrounding areas (STP), where the wet bias is reduced by approximately 65%.  The moisture budget, moist static energy budget, and mixed-layer heat budget are used to explore the mechanism behind this reduction in wet bias. High-resolution models, with their enhanced ability to simulate oceanic advection and mixing, can capture the central-warm and eastern-cool tropical Indian Ocean SST pattern better. This SST pattern suppresses precipitation over Malaysia and the South China Sea, triggering Rossby waves that generate an anomalous anticyclone over the northern Bay of Bengal. The anticyclone then transports dry air to the STP, suppressing local convection and reducing wet bias. Our study emphasizes the importance of simulating Indian Ocean warming for accurately representing long-term precipitation trends over HMA.

How to cite: li, L.: Precipitation Trends over southern High Mountain Asia affected by Indian Ocean warming: Insights from high- and low-resolution versions of CMIP6 models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7737, https://doi.org/10.5194/egusphere-egu25-7737, 2025.

EGU25-7792 | Posters on site | HS7.2

Statistical downscaling of hourly precipitation in South Korea using the MS-PRISM method 

Maeng-Ki Kim, Sang Jeong, and Youngseok Lee

In this study, we developed a grid climate dataset with a horizontal resolution of 500m × 500m for South Korea, utilizing observational station data from the Korea Meteorological Administration (KMA). The high-resolution 500m data were calculated using a newly developed Multi-Step (MS) PRISM (Parameter-elevation Regressions on Independent Slopes Model) method, which enhances the Modified Korean (MK) PRISM—a statistical downscaling technique for estimating high-resolution gridded data from observational data. First, to produce high-resolution hourly precipitation data, we performed quality control on the hourly precipitation observation data to select valid entries. Next, we created geographic information data, including Digital Elevation Model (DEM), aspect, and coastal proximity, all at a resolution of 500m. This geographic data was then applied to the MS-PRISM method to calculate hourly precipitation data at the same resolution. To confirm the reliability of the 500m resolution hourly precipitation produced, we conducted a verification of the final estimated data. We compared and analyzed the daily precipitation estimation errors as well as the hourly precipitation estimation errors at the same spatial resolution. Additionally, we evaluated the estimation results based on changes in spatiotemporal resolution by comparing the estimation errors associated with different spatial resolutions while maintaining the same temporal resolution.

How to cite: Kim, M.-K., Jeong, S., and Lee, Y.: Statistical downscaling of hourly precipitation in South Korea using the MS-PRISM method, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7792, https://doi.org/10.5194/egusphere-egu25-7792, 2025.

EGU25-8629 | ECS | Orals | HS7.2

Correction of Precipitation Bias from Convection-Permitting Models at the Station Scale in Switzerland 

Lauren Cook, Trang Nguyen, Andreas Dietzel, and Patricio Velasquez

Unlike regional climate models, convection-permitting models (CPMs) are able to resolve convection-scale processes and therefore better estimate short-duration, extreme precipitation events, particularly useful for the urban drainage community. Despite their state-of-the-art capabilities, bias correction of CPMs is still required to ensure their output is representative of the station scale, a resolution needed by many urban drainage models. Due to its simplicity, quantile-mapping is commonly used for bias-correction and downscaling, but does come with limitations that have not yet been evaluated for CPMs. This study tests five variations of empirical quantile-mapping to bias-correct and downscale the 2.2 km simulations of COSMO-CLM (a CPM) for over 70 weather stations in Switzerland. Ten years of simulation data are corrected using ten years of observations at the 30-minute interval. Traditional QM and several advanced versions are evaluated, including: using a 91-day moving window to account for temporal variability, spatial pooling of surrounding grid cells for spatial variability, and extending the observational record (to 30 years) for data variability. These techniques are validated using cross-validation and through evaluation of historical rainfall indices (e.g., consecutive dry days) and the climate change signal. Findings show that wet biases in raw CPM output remain (up to 30-35 mm/hour above the 98th quantile) and only the moving window technique (and its combination with spatial pooling) is able to reduce biases in quantiles above the 98th. All QM methods do reduce remaining biases, but can distort the climate change signal, particularly in indices related to frequency of rainfall. Despite the additional computational burden, the moving window technique is highly recommended to the urban drainage community as a robust technique for CPM downscaling. As more CPM simulations become available, future work will reexamine these aspects for a range of CPMs, time periods, and simulation domains.

How to cite: Cook, L., Nguyen, T., Dietzel, A., and Velasquez, P.: Correction of Precipitation Bias from Convection-Permitting Models at the Station Scale in Switzerland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8629, https://doi.org/10.5194/egusphere-egu25-8629, 2025.

EGU25-9341 | ECS | Orals | HS7.2

Decadal climatology and trends in global oceanic precipitation from 27 satellite and reanalysis datasets 

Si Cheng, Lisa Alexander, and Steven Sherwood

Understanding changes in global oceanic precipitation remains challenging due to limitations in current observational datasets and model deficiencies, particularly in the representation of cloud and precipitation properties within oceanic regions. To address this, we examined climatologies and trends in oceanic precipitation between 2001 and 2020 using a collection of 27 state-of-the-art satellite and reanalysis datasets available on a uniform daily 1°×1° resolution from the Frequent Rainfall Observations on Grids (FROGS) database. The results showed that reanalysis datasets generally report higher annual mean daily precipitation than satellite datasets. The tropical region exhibits the greatest absolute discrepancies in precipitation rates, while arid regions such as the southeast Pacific and Atlantic show significant relative differences among products. An increasing trend is primarily observed in satellite products, whereas reanalyses suggest strong declines. Taken together, reanalyses show pronounced decreases over the Intertropical Convergence Zone (ITCZ) and North Atlantic, contradicting the “wet gets wetter, dry gets drier” (WWDD) pattern. In contrast, the satellites better align with the WWDD pattern, with over half of oceanic regions meeting this expectation. The precipitation trend in the combined reanalysis products also exhibits the weakest consistency with sea surface temperature (SST) trends in wet regions (34.2%), compared with dry regions in the reanalysis cluster (53.4%) and both wet (59.6%) and dry (58.5%) regions in the satellite cluster. We recommend using an ensemble of satellite products for investigating global oceanic precipitation while exercising greater caution when utilizing reanalysis datasets.

How to cite: Cheng, S., Alexander, L., and Sherwood, S.: Decadal climatology and trends in global oceanic precipitation from 27 satellite and reanalysis datasets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9341, https://doi.org/10.5194/egusphere-egu25-9341, 2025.

EGU25-9859 | ECS | Posters on site | HS7.2

Drizzle Bias adjustment in climate models: A simple two-step downscaling approach 

Matteo Sangiorgio, Roberto Caspani, Lorenzo Scarpellini, Matteo Giuliani, and Andrea Castelletti

Precipitation is a key variable for assessing the impacts of climate change across diverse sectors, from hydrology to ecology. However, climate models frequently overestimate the occurrence of light precipitation events—days or hours that should be dry are instead assigned a low rainfall rate. This pervasive issue, known as the “drizzle bias” or “drizzle problem” in climate science, undermines the reliability of climate impact assessments.

Traditional bias correction methods, such as linear scaling or empirical quantile mapping, address overall precipitation distributions but often fail to properly account for the frequency and duration of wet and dry periods. As a result, these methods may improve precipitation totals but fail to correct the skewed distribution of rainy events.

In this study, we propose a simple yet effective two-step statistical downscaling approach to address the drizzle bias. The first step aligns the frequency of wet and dry periods by assuming equivalence between observed and simulated rain frequencies. The second step corrects the precipitation distribution exclusively for wet samples.

We apply this methodology to a range of climate data products, including ERA5 Land reanalyses, as well as simulations from global circulation models (GCMs), regional circulation models (RCMs), and convection-permitting models (CPMs). Our analysis focuses on multiple measurement stations in Northern Italy, encompassing urban contexts such as Milan and mountainous contexts in the Italian Alps. Results reveal that drizzle bias is a widespread issue across these datasets, regardless of the modeling framework.

The findings demonstrate that our two-step downscaling approach effectively adjusts for drizzle bias, significantly improving the statistical fidelity of precipitation projections. This approach offers a straightforward and practical solution for enhancing the reliability of climate model outputs, enabling more robust assessments of climate change impacts across sectors sensitive to precipitation variability.

How to cite: Sangiorgio, M., Caspani, R., Scarpellini, L., Giuliani, M., and Castelletti, A.: Drizzle Bias adjustment in climate models: A simple two-step downscaling approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9859, https://doi.org/10.5194/egusphere-egu25-9859, 2025.

EGU25-10165 | ECS | Posters on site | HS7.2

Removal of interfering RLAN signals from C-band weather radar data 

Krystian Specht, Katarzyna Ośródka, Jan Szturc, and Włodzimierz Freda

The algorithm of removing interfering RLAN signals (so called spikes) in weather radar data is implemented in the Institute of Meteorology and Water Management – National Research Institute (IMGW) as a component of the RADVOL-QC system for the radar data quality control. Eliminating the interfering signals in C-band (5 GHz) radars is important for accurate weather monitoring. The main difficulty in spike removal are their unique shapes, and the task is especially challenging while they overlap the precipitation.

The process of detecting interference caused by signals from the RLAN network is carried out by evaluating the variability of echoes along and across the beam for each bin at various elevation angles. Such echoes are considered potential spikes. For each azimuth, the number of bins containing potential spike echoes is determined. If this count exceeds the established threshold for a given azimuth, the echoes are treated as real spikes.

The spike correction process consists of analyzing each bin with detected real spike and its surroundings. The analysis extends to bins in adjacent and further azimuths on left and right until bins without detected spikes are encountered. Depending on the specific case, these echoes may be replaced with an arithmetic mean if classified as precipitation or removed entirely. While removing spikes, the analysis extends to adjacent azimuths within a range of 3 to 4 bins on either side to ensure accurate identification and removal of false echoes. This extended analysis considers potential anomalies in adjacent data that may have been overlooked during the detection process.

Examples of applied techniques are presented using the weather radar product maximum reflectivity (CMAX). The examples illustrate the enhancement of the radar data, where the extended analysis effectively eliminates RLAN interference that was not identified by the detection algorithm but falls within the analysis area. This improvement is crucial from a meteorological perspective, as high-quality radar data significantly impacts meteorological and hydrological models, leading to more accurate forecasts.

How to cite: Specht, K., Ośródka, K., Szturc, J., and Freda, W.: Removal of interfering RLAN signals from C-band weather radar data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10165, https://doi.org/10.5194/egusphere-egu25-10165, 2025.

The increasing frequency and intensity of extreme events due to global warming, such as heavy rainfall and consequent floods, underline the need for research on the driving factors of these extremes. Accurate simulations of meteorological extremes at convection-permitting scale are crucial for understanding their spatial and temporal characteristics. Recently, various studies have demonstrated the added value of using convection-permitting regional climate models to simulate extreme precipitation. Further improvements of these regional models can therefore lay the foundation for better impact assessment, as well as for developing adaptation measures to tackle climate change. 

In this study, we investigate the optimal model configuration for the regional climate model REMO2020-iMOVE to capture extreme precipitation events, using the heavy rainfall that led to the devastating Ahr valley flood of July 2021 as a case study. Our simulations are performed with the non-hydrostatic version of REMO with ERA5 reanalysis data as forcing at a horizontal resolution of 3 km. By including the vegetation module iMOVE, we aim to improve the representation of vegetation-atmosphere interactions and, in a future step, investigate the effects of land use and land cover changes on extreme events. Here, we explore the impact of different model setups such as different domain sizes and initialization times on the simulation results. Furthermore, we validate our findings against observations and assess uncertainty within the model. This research provides insight into optimizing regional climate models to improve our understanding of extreme weather events. 

How to cite: Detjen, L., Rechid, D., and Böhner, J.: Optimizing convection-permitting model configurations for accurate simulation of extreme precipitation events with the regional climate model REMO-iMOVE, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11604, https://doi.org/10.5194/egusphere-egu25-11604, 2025.

EGU25-12783 | Orals | HS7.2

Using LOCA to downscale precipitation over Europe 

Bridget Thrasher

Localized Constructed Analogs (LOCA) is a statistical downscaling technique that uses a multiple scale approach to determine appropriate local analogs from historical data. It was developed with a particular focus on the preservation of extreme events that were dampened or lost altogether when employing earlier analog methods. The LOCA method has been used to produce relatively high-resolution projections of precipitation over the coterminous United States for use in hydrologic applications but has never been applied over Europe. In this presentation we will describe the method in detail and show how it is being utilized to downscale CMIP6 precipitation to 1 arcmin x 1 arcmin horizontal resolution over the continent using the European Meteorological Observations (EMO-1) gridded dataset as the analog pool. Lastly, we will compare the LOCA output to that from other downscaled products. 

How to cite: Thrasher, B.: Using LOCA to downscale precipitation over Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12783, https://doi.org/10.5194/egusphere-egu25-12783, 2025.

EGU25-12929 | ECS | Posters on site | HS7.2

Reanalysis Data in Hydrological Applications: A Case Study from Georgia 

Andrea Nobile, Francesca Zanello, Francesco Lubrano, Matteo Nicolini, and Elisa Arnone

Reanalysis data have proven to be a valuable support for hydrologic modeling and calculation of standardized climate indices, useful tools for characterizing local climate regimes and improving water resource management in areas with limited availability of observational data.

This study examines the use of ERA5 dataset emphasizing bias correction techniques to enhance their applicability and understanding their limits in a case study in Georgia. The work assesses the effectiveness of five bias correction techniques - Linear Scaling (LS), Empirical Quantile Mapping (QM-EMP), Quantile Mapping Spline Bias Correction (QM-SBC), Mean Bias Subtraction (MBS), and Simple Linear Regression (SLR) - each examined through two different bias correction approaches: classical and sliding window, applied to daily and monthly reanalysis time series. Observational climate data are scarce in Georgia, therefore the opportunity of using reanalysis data for hydrological studies is of great interest for engineering applications.

In this study, performed in collaboration with Idrostudi S.r.l., one of the foremost European engineering professional services consulting firms, the extraction of ERA5 data for the entire nation of Georgia was performed automatically by developed algorithms that also allowed to do bias correction. The algorithms, developed using the open-source programming language R, employ observed data collected by five meteorological stations across diverse climatic zones of Georgia to test and compare different bias correction methodologies. The aim is to validate the performance of bias correction methods to improve the accuracy of rainfall data generated by ERA5 reanalysis model at daily and monthly scales. The techniques were evaluated carrying out two experiments, i.e. using (i) the complete datasets and (ii) the series that were split into a calibration and validation subset; metrics such as Root Mean Square Error (RMSE) and Nash-Sutcliffe Efficiency (NSE) were used to assess the performance. The dataset undergoes a calibration phase using 70% of the data to tune the bias correction methods, followed by a validation phase with the remaining 30% to test their effectiveness.

Results demonstrate that bias correction improves the quality of reanalysis data, dealing to enhanced reliability for hydrological modelling and climate index computation. The LS method has emerged as the most effective among classical techniques for bias correction in daily-scale reanalysis data when all data are available. The introduction of the Sliding Window approach has further enhanced the performance of all techniques, adapting the correction to local variations and improving accuracy for daily precipitation events. It is important to note, however, that at a monthly scale, the classic approach to bias correction already proves to be sufficiently reliable. Therefore, further enhancements through the sliding window approach are not deemed necessary for monthly corrections. In the experiment (ii), techniques such as QM-EMP, QM-SBC, and SLR proved to be more suitable for applications in climatic contexts with high variability and fragmentation. This underlines the importance of selecting the appropriate bias correction technique based on the quality and availability of data, as well as the specific objectives of the analysis. Further studies are needed for a further optimization of bias correction approaches.

How to cite: Nobile, A., Zanello, F., Lubrano, F., Nicolini, M., and Arnone, E.: Reanalysis Data in Hydrological Applications: A Case Study from Georgia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12929, https://doi.org/10.5194/egusphere-egu25-12929, 2025.

EGU25-13830 | Posters on site | HS7.2

Considerations in multifractal downscaling of rainfall: canonical vs. microcanonical cascades 

Alin Andrei Carsteanu, Stergios Emmanouil, Andreas Langousis, and Roberto Deidda

Disaggregation of rainfall time series focuses on preserving the statistical properties of those small-scale intensities, which are being downscaled from measured large-scale values. Multifractal scaling properties have offered, for a few decades already, a parsimonious framework for simulating the joint statistics observed in the small-scale values, and recent work emphasizes the use of more sophisticated cascading processes, in order to better capture all statistical requirements imposed (Cappelli et al., Stoch Environ Res Risk Assess 2024, https://doi.org/10.1007/s00477-024-02827-8). Comparisons between downscaling models based on canonical vs. microcanonical cascades have been presented already more than two decades ago (see e.g. Molnar and Burlando, Atmos Res 77, 2005, https://doi.org/10.1016/j.atmosres.2004.10.024), but recent theoretical results (Aguilar-Flores and Carsteanu, Fractals 32, 2024, https://doi.org/10.1142/S0218348X24500725) have prompted us to consider the importance of taking into account the asymptotic properties of the measures generated by canonical and microcanonical cascades, respectively, for downscaling purposes. The reflection of such properties in real-life rainfall data is being analyzed in the work communicated herein.

How to cite: Carsteanu, A. A., Emmanouil, S., Langousis, A., and Deidda, R.: Considerations in multifractal downscaling of rainfall: canonical vs. microcanonical cascades, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13830, https://doi.org/10.5194/egusphere-egu25-13830, 2025.

EGU25-13869 | Posters on site | HS7.2

MET Nordic Reanalysis data improves the performance of catchment-level hydrological models 

Csilla Farkas, Moritz Shore, Jessica Fennell, and Mojtaba Shafiei

High-quality input data is the foundation for good model performance, including catchment level hydrological models. The resolution and quality of meteorological data has a direct impact on modelling results and as such strongly influences the outcomes of scenario analyses of different types. Nowadays one can choose between different meteorological products when setting up a mathematical model, including direct measurements and reanalyses. The goal of this study was to test the ability of MET Nordic data, a reanalysis product from Met Norway, on improving the simulations of hydrological models.  The MET Nordic Reanalysis Dataset consists of post-processed products that (a) describe the current and past weather (reanalysis), and (b) gives a best estimate of the weather in the short-term future (forecasts). The products integrate output from MetCoOp Ensemble Prediction System (MEPS) as well as measurements from various observational sources, including crowdsourced weather stations. 

Two different catchment models were set up and calibrated against measured discharge data. The SWAT+ model was applied in two Norwegian and one Danish catchment, while the CWatM model was tested in one Norwegian catchment. The model’s performance was compared when using input datasets from measuring stations and MET Nordic reanalysis data. We concluded that applying reanalysis data can significantly improve the performance of the tested models, therefore the use of these data in hydrological modelling is highly recommended.  

How to cite: Farkas, C., Shore, M., Fennell, J., and Shafiei, M.: MET Nordic Reanalysis data improves the performance of catchment-level hydrological models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13869, https://doi.org/10.5194/egusphere-egu25-13869, 2025.

Probabilistic radar-based precipitation nowcasting has become increasingly crucial for real-time hydrological applications due to its high accuracy at short lead time. However, its reliability for hydrological usage is limited by two major sources of error and uncertainty, both of which tend to exacerbate quickly with lead time. The first source lies in the limitations of nowcasting algorithms, including inaccuracies in rainfield advection and inadequate modeling of rain cell evolution. The second arises from discrepancies in precipitation measurements, referring to the differences between radar-derived estimates and rain gauge observations. Aligning these estimates with actual ground-level precipitation is vital for practical hydrological applications.

This study focuses on addressing the errors and uncertainties inherent in precipitation 'measurements', aiming to enhance the reliability of original nowcasts. Here, uncertainty refers to the range within which the true value is expected to fall at a given confidence level, while error denotes to the systematic bias between estimated and true values. The proposed methodologies utilise rain gauge data as the ground truth and employs the Short-Term Ensemble Prediction System (STEPS) to generate radar-based ensemble nowcasts. To deal with these issues, an initial attempt was conducted with the Censored Shifted Gamma Distribution (CSGD) model. However, the model faces challenges in selecting an appropriate metric as the adjusted value, limiting the potential reduction in RMSE to approximately 5–10%. To overcome this limitation, a random forest (RF) regression model is proposed, as it can avoid predefined assumptions about rainfall intensity distribution. This model incorporates variables such as nowcasted rainfall intensity, orographic features, and meteorological parameters such as wind speed, wind direction, humidity, cloud type, and cloud base height (CBH), to estimate corresponding rain gauge measurements. At each rain gauge location, the error distribution is parametrised by comparing the original and adjusted rainfall intensities and fitting them to various probability functions. These parameters are then spatially interpolated using geostatistical techniques to generate an error map. The resulting error map is applied to correct the original nowcasts across the study area, enhancing their overall accuracy and reliability.

The United Kingdom, benefiting from its comprehensive and high-quality meteorological data, was selected as the study area. The 1-km UK C-band radar composite, derived from the Met Office Nimrod System, serve as the radar rainfall dataset for generating ensemble nowcasts. Rain gauge data and additional meteorological variables are sourced from the Met Office Integrated Data Archive System (MIDAS) and the Met Office LIDARNET ceilometer network. Rainfall events from 2016 to 2022 are analysed, with events from 2016 to 2020 designated as the training period for developing random forest models and error maps. For validation, 20 events from 2021 to 2022 are selected to assess the performance of both the original and adjusted nowcasts. Preliminary results indicate that the adjusted ensemble nowcasts exhibit significantly improved alignment with rain gauge measurements compared to the original nowcasts. These findings highlight the potential of the proposed methodology to reduce both error and uncertainty in radar-based precipitation nowcasting, particularly for hydrological applications such as flood and landslide forecasting.

How to cite: Lin, H.-M. and Wang, L.-P.: Enhancing the applicability of radar-based precipitation nowcasting to hydrological applications with a machine-learning based error modelling method, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14377, https://doi.org/10.5194/egusphere-egu25-14377, 2025.

EGU25-14564 | ECS | Posters on site | HS7.2

Blunt Extension and Dynamic Generation of Multifractal Cascade Fields Tree for Rainfall Drop Trajectories Simulations 

Chi-Ling Wei, Auguste Gires, and Li-Pen Wang

Precipitation variability at small space-time scales significantly influences hydrological processes, particularly in heterogeneous environments such as urban areas. Building on established methodologies for generating universal multifractal cascade fields, we propose an alternative approach that optimizes memory efficiency while maintaining the fidelity and flexibility of high-resolution simulations. Our method generates cascade fields dynamically, we call it Cascade Tree, which reduces memory usage by over 100 times compared to precomputing and storing full datasets. This improvement complements existing techniques by offering a scalable option for real-time applications.

 

To further enhance the realism of the simulated fields, we integrate the blunt extension of universal multifractals, which smooths transitions between far branches in Cascade Tree and addresses non-conservativeness in a computationally efficient manner. By leveraging GPU acceleration, we achieve rapid computation of cascade fields, enabling their use in simulating complex phenomena such as rainfall dynamics in turbulent wind fields.

 

The method is applied to simulate 3D trajectories and velocities of raindrops in a high-resolution multifractal turbulent wind field, using real wind field data to improve the applicability of the results. Our simulations capture the spatial and temporal variability of rainfall and demonstrate the dispersion of over 100,000 raindrops across scales relevant to radar pixels and urban catchment hydrology.

 

This work provides new tools for exploring rainfall-driven processes, with applications ranging from downscaling radar precipitation data to refining hydrological response models. By complementing established methods with a memory-efficient and GPU-accelerated framework, our approach bridges the gap between drop-scale dynamics and catchment-scale impacts.

How to cite: Wei, C.-L., Gires, A., and Wang, L.-P.: Blunt Extension and Dynamic Generation of Multifractal Cascade Fields Tree for Rainfall Drop Trajectories Simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14564, https://doi.org/10.5194/egusphere-egu25-14564, 2025.

EGU25-14679 | ECS | Orals | HS7.2

Bartlett-Lewis based stochastic rainfall model: An improvement to effectively reproduce sub-hourly rainfall extremes 

Chi Vuong Tai, Jeongha Park, Li-Pen Wang, and Dongkyun Kim

Despite significant advancements in the Poisson cluster-based Bartlett-Lewis model for effectively reproducing rainfall extremes, there is still room for further refinement. This study proposes a refined model, referred to as RBL7, introducing module k with a modified equation for rainfall disaggregation. This adjustment allows the power of the sine function to vary inversely with rain cell duration, thereby capturing the realistic characteristics of rainfall extremes, which often come with high intensity over short durations. Furthermore, an improved calibration approach is also proposed for the first module of the RBL7 model. This involves a hybrid optimization technique combining Particle Swarm Optimization (PSO) and fmincon methods, iterately executed until the objective function reaches the pre-assigned threshold. While the calibration of the RBL7 model relies solely on observed rainfall aggregated at hourly and longer timescales, it effectively reproduces rainfall extremes from uncalibrated sub-hourly to supra-hourly aggregation intervals, outperforming existing models using sine-2 and rectangular pulse shapes. Additionally, this refined model maintains its capability to capture rainfall standard statistics, i.e., mean, variance, covariance, skewness, and proportion of wet period, at various timescales ranging from 5 minutes to a month. These findings highlight the robustness of the RBL7 model in simulating rainfall characteristics, especially extreme values at sub-hourly aggregation intervals.

 

Acknowledgement

This study was supported by Korea Environment Industry & Technology Institute (KEITI) through R&D Program for Innovative Flood Protection Technologies against Climate Crisis Program (or Project), funded by Korea Ministry of Environment(MOE)(RS-2023-00218873).

How to cite: Vuong Tai, C., Park, J., Wang, L.-P., and Kim, D.: Bartlett-Lewis based stochastic rainfall model: An improvement to effectively reproduce sub-hourly rainfall extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14679, https://doi.org/10.5194/egusphere-egu25-14679, 2025.

EGU25-14931 | ECS | Posters on site | HS7.2

Quantifying Future Shifts in Intensity–Duration–Frequency (IDF) in Singapore: A comparison of methods 

Mengzhu Chen, Nadav Peleg, and Simone Fatichi

Intensity-Duration-Frequency (IDF) curves are critical for urban drainage design and flood risk mitigation, particularly in highly urbanized regions like Singapore, where short-duration extreme rainfall events pose significant challenges. This study quantifies future changes in IDF curves and their associated uncertainties under two representative emission scenarios: SSP 2-4.5 and SSP 5-8.5. To construct future IDF curves, we compare two methods. First, we use a stochastic downscaling methodology that makes use of the AWE-GEN weather generator, to downscale precipitation projections from 25 Global Climate Models (GCMs) to the local point scale. The results show that the magnitude of future extreme precipitation quantiles is expected to get higher toward the end of the 21st century under both future scenarios. Higher-emission scenarios lead to substantial intensification of rare precipitation events, accompanied by a large uncertainty. However, internal climate variability is the dominant source of uncertainty, with climate model and emission scenario uncertainties being less relevant. Second, the results are compared with outputs of the TENAX (Temperature dependent Non-Asymptotic statistical model for eXtreme return levels) model, a novel framework that incorporates temperature as a covariate in a physically consistent manner to project rainfall return levels in a warmer climate using fewer inputs. This study compares state-of-the-art methodologies for computing IDF representative of future climates and provides actionable insights for engineers and policymakers to update urban stormwater design guidelines and enhance resilience against future rainfall extremes.

How to cite: Chen, M., Peleg, N., and Fatichi, S.: Quantifying Future Shifts in Intensity–Duration–Frequency (IDF) in Singapore: A comparison of methods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14931, https://doi.org/10.5194/egusphere-egu25-14931, 2025.

Climate change is an essential part of sustainable development challenges in developing countries. Climate change represents one of the greatest environmental, social, and economic threats facing the world today. Accurate meteorological and hydrological projections are vital for effective climate adaptation and resource management, particularly under changing climate scenarios. However, the coarse spatial resolution of General Circulation Models (GCMs) limits their applicability for localized impact assessments. This study proposes a deep learning-based super-resolution approach combined with an advanced hydrological model to downscale and enhance the spatial resolution of three GCM datasets—GFDL-CM4, GISS-E2-1-G, and IPSL-CM6A-LR—to approximately 0.01°. The performance of the method is evaluated based on mean square error (RMSE), mean absolute error (MAE), Peak signal-to-noise ratio (PSNR), and Pearson correlation coefficient (R). This study hypothesizes to have more precise and accurate meteorological and hydrological predictions and projections under this framework. The model is conducted on historical climate data and compared with high-resolution observational datasets, showcasing its ability to capture fine-scale climatic and hydrological variability. This approach bridges the resolution gap in climate projections and provides a robust framework for better-informed decision-making in climate change adaptation and mitigation strategies.

Funding

This research was supported by Disaster-Safety Platform Technology Development Program of the National Research Foundation of Korea (NRF) funded by the Ministry of Science and ICT. (No. 2022M3D7A1090338).

How to cite: Huong, O. S. and Lee, G.: Improving Climate Change  Data through Deep Learning Super-Resolution Downscaling of GCMs for Precise Hydrological Projections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15576, https://doi.org/10.5194/egusphere-egu25-15576, 2025.

EGU25-15818 | ECS | Orals | HS7.2

Hourly Precipitation Biases and Clausius-Clapeyron Scaling in Convection-Resolving and Convection-Parameterizing Regional Climate Models 

Alzbeta Medvedova, Isabella Kohlhauser, Douglas Maraun, Mathias W. Rotach, and Nikolina Ban

Regional climate models (RCMs) are crucial tools for understanding and predicting climate change and its impacts, such as precipitation extremes. We investigate the characteristics of hourly precipitation and the associated extremes in RCM ensembles with two resolutions: km-scale (the CORDEX-FPS Convection ensemble with ~3 km grid spacing, where deep convection is represented explicitly), and coarser-scale (~12 km grid spacing, with parameterized convection). The km-scale ensemble is downscaled from the coarser one, and both cover three time periods: evaluation, historical, and end-of-the-century period under the RCP8.5 warming scenario (2000-2009, 1996-2005, and 2090-2099, respectively). Evaluating the model ensembles against data from 179 weather stations in Austria, we study how the intensity, duration, and the time of onset of precipitation depend on mean daily temperature. We then examine how these characteristics change under warming conditions.

It is well established that over the Alps the coarser RCMs produce too much light and persistent precipitation which is triggered too early in the day. We find that these shortcomings in models with parameterized convection become more pronounced with rising temperatures. We show that the km-scale ensemble closely matches observations and greatly outperforms the coarser ensemble in capturing the investigated hourly precipitation characteristics, especially at higher temperatures and on days with heavy rainfall. As high temperatures are expected to become more common in future climates, our results imply that coarser RCMs suffer from more severe biases in hourly precipitation in the future than under present climate conditions, especially for short-duration extremes. 

In this light, we also assess the ability of both km-scale and coarser RCM ensembles to capture the Clausius-Clapeyron scaling of extreme precipitation with temperature, and discuss how model deficiencies in the coarser ensemble affect this relationship.

In summary, our findings highlight the importance of km-scale RCMs for accurate simulations of hourly precipitation and its extremes, particularly in the warming climate.

How to cite: Medvedova, A., Kohlhauser, I., Maraun, D., Rotach, M. W., and Ban, N.: Hourly Precipitation Biases and Clausius-Clapeyron Scaling in Convection-Resolving and Convection-Parameterizing Regional Climate Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15818, https://doi.org/10.5194/egusphere-egu25-15818, 2025.

EGU25-15936 | Posters on site | HS7.2

A Framework for Convection-Permitting Climate Downscaling over Southern Italy 

Giuseppe Mendicino, Luca Furnari, Elnaz Hatami Bahman Beygloo, Thomas Rummler, Harald Kunstmann, and Alfonso Senatore

Projecting climate change impact in southern Italy is particularly challenging because this region is located in the center of the Mediterranean basin, which is a recognized climate change hotspot, and is characterized by steep and complex orography requiring analysis at high spatial resolution. Therefore, climate models at the convection-permitting scale considerably improve the ability to simulate water cycle trends in that region, especially severe events.

This note introduces the modeling framework on which climate simulations are being carried out for southern Italy using CMIP6 projections and presents the first results related to the comparison of the historical simulation with observational datasets. A preliminary analysis revealed that the best CMIP6 global climate model (GCM) for reproducing the interannual cycle of precipitation and temperature over the study area is the High-Resolution MPI-ESM-1-2 model (1°x1° as horizontal resolution). Such a GCM was chosen to provide 6-hour boundary conditions for dynamic downscaling with the WRF (Weather Research and Forecasting) limited-area model with two domains one-way nested: the external one D01, with a horizontal resolution of about 20km, covering the entire Mediterranean area (209x214 grid points), and the internal one D02, with a horizontal resolution of about 4km, centered on southern Italy (285x265 grid points). The historical simulation extends from 1995 to 2014. The future simulations cover the period 2025 to 2045. The first future simulation employs the SSP 5-8.5 scenario.

Total precipitation and near-surface air temperature resulting from the historical simulation are compared with both observational datasets (namely, the spatially distributed products BigBang, SCIA, E-OBS, and validated weather station time series) and reliable downscaled reanalyses (e.g., ERA5-Land, MERIDA, MERIDA HRES, SPHERA, CERRA, VHREA_IT), which are increasingly available for the Italian peninsula. The results highlight that the evaluation of the performance of the historical simulation is partially affected by the selection of the reference dataset.

 

 

Acknowledgments: This study was funded by the Next Generation EU - Italian NRRP, Mission 4, Component 2, Investment 1.3, project WaterWISE - Water Management Strategies and Climate Change Adaptation in Southern Italy, n. PE00000005, CUP D43C22003030002; and by the Next Generation EU - Italian NRRP, Mission 4 ‘Education and Research’ - Component C2, Investment 1.1, Research Project of National Interest (PRIN 2022 PNRR) ­- An integrated modeling approach for mitigating climate CHANge effects through enhanCEd weathering in Southern Italy (CHANCES, CUP H53D23011260001), Italian Ministry of University and Research.

How to cite: Mendicino, G., Furnari, L., Hatami Bahman Beygloo, E., Rummler, T., Kunstmann, H., and Senatore, A.: A Framework for Convection-Permitting Climate Downscaling over Southern Italy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15936, https://doi.org/10.5194/egusphere-egu25-15936, 2025.

Precipitation time series are used as input for hydrological modeling. As the main driver of the hydrological cycle, they directly influence soil moisture, runoff, river flows, and groundwater recharge. High-resolution precipitation data is required to obtain accurate hydrological models. In addition, data should be available from different locations to reflect spatial dependencies in these models. As precipitation is measured only at selected locations, the simulated series can be used for design purposes.

In recent years, various models have been developed based on the Fourier Transform because of its ability to preserve desirable statistical properties. The concept is to transform the time series from the time domain to the frequency domain and calculate the two main components of the transformed series: the power spectrum (the square of the absolute values of the Fourier frequencies) and the phase spectrum (phase angle of the frequencies). The main idea behind all the Fourier-based models is to preserve the power spectrum because it relates to the autocorrelation function and overall structure.

This study compares the most common Fourier-based time series generators using different measures. As most spectral methods are iterative, this can be challenging for the precipitation time series, especially for the hourly resolution. In this regard, a non-iterative method is introduced. This method takes advantage of the Wiener–Khinchin theorem for the transformation between the autocorrelation function and the power spectrum. Another method, the Phase Annealing method, is introduced for precipitation time series generation and keeping the spatial and temporal properties. The results have been compared for the developed models and the most common Fourier-based methods.

How to cite: Mehrvand, M. and Bárdossy, A.: Comparative study of spectral methods for precipitation time series generators based on the conserving observed spatial and temporal properties, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16085, https://doi.org/10.5194/egusphere-egu25-16085, 2025.

EGU25-17581 | ECS | Posters on site | HS7.2

Daily precipitation dataset (1991-2021) at 1 km resolution over the Po river basin area using Kriging 

Sohaib Baig, Gaia Roatti, Marco Brian, Francesco Tornatore, Giuseppe Formetta, and Riccardo Rigon

The Po river basin, in the north of Italy, is the lifeline of the economic and ecology of the North of Italy. The 661 km long river covers an area of 71327 km2 and replenishes the water demands of agriculture, industry and domestic consumers. The topography is diverse  with alps mountains in the north and fertile plains in the south. The annual precipitation is 1200 mm which varies between ~2000 mm in the Alps to ~700 mm in the downstream. This study presents the estimates the precipitation on daily resolution over a grid of 1 km across the Po river basin for the period from 1991 to 2021, thus providing a consistent datasets for analyses of the recent climatology of the area. Total 1511 number of observed precipitation stations were included in the study along with topographic information. The statistical technique of kriging was employed to produce the grid data cube. The workflow of the study is summarized in the following steps:

  • obtain the meteorological data from the data providers
  • estimate the empirical semivariogram
  • fit theoretical models to the empirical semivariogram and analyses of the statistical correlation
  • use the theoretical model for solving the kriging system
  • produce continuous surface maps or time series of the quantity desired in any gridded point of the domain
  • calculate estimation errors.

For the estimation of errors Leave-one-out (LOO) is adopted which consists of removing a single station at a time and performing the interpolation for the location of the removed point by using the remaining stations. The approach is repeated until every station has been, in turn, removed and estimates are calculated for each station.

The results have shown that the average precipitation in the basin is 1131 mm with significant spatial patterns, some of which are reported for example. The northern subbasins have shown annual precipitation up to 2500 mm while the downstream planes receives up to 550 mm. The results show clear spatial and temporal patterns across the basin which  are reported in the study.

How to cite: Baig, S., Roatti, G., Brian, M., Tornatore, F., Formetta, G., and Rigon, R.: Daily precipitation dataset (1991-2021) at 1 km resolution over the Po river basin area using Kriging, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17581, https://doi.org/10.5194/egusphere-egu25-17581, 2025.

EGU25-19416 | ECS | Orals | HS7.2

Enhancing Extreme Rainfall Nowcasting with Weighted Loss Functions in Deep Learning Models 

Hyojeong Choi, Yongchan Kim, and Dongkyun Kim

With the increasing frequency and intensity of extreme rainfall events, the importance of nowcasting to minimize damage from disasters such as flash floods is becoming ever more prominent. However, most nowcasting models use loss functions aimed at minimizing the average prediction error. As a result, they tend to underestimate extreme rainfall—which has relatively low occurrence frequency but significant impact. In this study, we applied various types of weighted loss functions to a ConvLSTM-based nowcasting model to more accurately predict extreme rainfall. In particular, we varied parameters within these weighted loss functions and conducted sensitivity analyses to identify the optimal weighting strategies. We also categorized extreme rainfall types and evaluated the models’ predictive performance with weighted loss functions, thereby examining both the accuracy and stability of the model’s forecasts under extreme conditions from multiple perspectives. The results showed that the model employing a weighted loss function achieved significantly improved accuracy in predicting extreme rainfall, compared to an unweighted model. Furthermore, depending on the type of weighted loss function and parameter settings, the model demonstrated notably strong performance for specific types of extreme rainfall. This finding suggests that, in a rainfall environment characterized by high variability, dynamically selecting weighted loss functions according to forecasting objectives and conditions can enhance both the efficiency and reliability of extreme rainfall prediction. The approach presented in this study can be applied to flood forecasting and is anticipated to contribute to the advancement of deep learning–based disaster response systems, reducing the potential damage caused by natural disasters.

 

Acknowledgements

This work was supported by Korea Environment Industry & Technology Institute(KEITI) through R&D Program for Innovative Flood Protection Technologies against Climate Crisis Program(or Project), funded by Korea Ministry of Environment(MOE)(RS-2023-00218873).

How to cite: Choi, H., Kim, Y., and Kim, D.: Enhancing Extreme Rainfall Nowcasting with Weighted Loss Functions in Deep Learning Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19416, https://doi.org/10.5194/egusphere-egu25-19416, 2025.

EGU25-19913 | Orals | HS7.2

Postprocessing of rainfall forecasts over East Africa 

Fenwick Cooper, Shruti Nath, Masilin Gudoshava, Nishadh Kalladath, Ahmed Amdihun, Jason Kinyua, Hannah Kimani, David Koros, Zacharia Mwai, Christine Maswi, Asaminew Teshome, Samrawit Abebe, Isaac Obai, Jesse Mason, Florian Pappenberger, Matthew Chantry, Antje Weisheimer, and Tim Palmer

We test methods of postprocessing rainfall forecasts out to 7 days over East Africa.

Using the physical forecast models, IFS from ECMWF and GFS from NCEP, we apply several combinations of post-processing techniques to empirically correct the predicted rainfall towards IMERG blended satellite rainfall data. The techniques we apply include a generative adversarial neural network (GAN) model (Harris et al. 2022), isotonic distributional regression (EasyUQ, Walz et al. 2024), EMOS (Gneiting et al. 2005), linear regression, and the kernel density estimate. Other approaches are also considered, however for the purposes of practical operational forecasts, we mainly focus on computationally cheap methods. Because we are comparing against IMERG, our results compare favourably against fully empirical models, such as FuXi and Graphcast, that have been trained to predict ERA5.

Being computationally cheap, in an operational forecast cycle on a standard desktop computer, the GAN model can produce spatially correlated 1000 member ensembles from the input forecast data. from which we can display the distribution using a histogram. The other techniques also cheaply produce rainfall distributions. We compare the quality of these distributions using the CRPS, variogram score and reliability diagrams. Biases in the raw rainfall forecasts are most notably reduced over the large lakes, for example Lake Victoria, over mountains, Indian ocean, and other places of high rainfall. We find it difficult to reduce biases in dry regions and over the Congo rainforest.

Different empirical modelling methods are optimal for different physical phenomena, and there is no theory for the most accurate model without physical insight. We also observe that it is often possible to improve each of the models with various tweaks. Each of the tested approaches might improve in the future, and the question we are trying to answer is “what is the best practical model available today?”

How to cite: Cooper, F., Nath, S., Gudoshava, M., Kalladath, N., Amdihun, A., Kinyua, J., Kimani, H., Koros, D., Mwai, Z., Maswi, C., Teshome, A., Abebe, S., Obai, I., Mason, J., Pappenberger, F., Chantry, M., Weisheimer, A., and Palmer, T.: Postprocessing of rainfall forecasts over East Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19913, https://doi.org/10.5194/egusphere-egu25-19913, 2025.

 Accurate precipitation estimation is crucial for hydrological modeling and flood forecasting in the Yangtze River Basin (YRB), China. This study explores the use of machine learning (ML) and deep learning (DL) methods to fuse multi-source precipitation data, including satellite, radar, and ground-based observations. We apply models such as Random Forest (RF), Support Vector Machines (SVM), Convolutional Neural Networks (CNN), and Long Short-Term Memory (LSTM) networks to improve precipitation estimation accuracy. Performance is evaluated using metrics like Mean Absolute Error (MAE) and Root Mean Square Error (RMSE). Our results demonstrate that deep learning models, particularly CNNs and LSTMs, outperform traditional ML methods in terms of accuracy and spatial consistency. This work provides a robust approach to multi-source data fusion, enhancing precipitation monitoring and hydrological applications in the YRB.

How to cite: Chen, T.: Machine Learning and Deep Learning for Multi-Source Precipitation Integration in the Yangtze River Basin, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1507, https://doi.org/10.5194/egusphere-egu25-1507, 2025.

EGU25-3311 | PICO | HS7.1

A novel algorithm for remote sensing rainfall retrieval 

Massimiliano Ignaccolo and Carlo De Michele

Dual-polarization radar rainfall rate estimates are based on scaling laws involving the horizontal reflectivity Zh and the ratio between horizontal and vertical reflectivity ZDR. Scaling law parameters obtained from disdrometric observations are highly dependent on the data set used. As a consequence ZR scaling laws do not generalize well. Using the jargon of data science, a ZR scaling law has an accpetable training accuracy and a poor validation accuracy. 

To overcome this limitation, we propose the Formula-R algorithm based on the adoption of the data science parametrization of drop size distributions and its universal shape factors [https://doi.org/10.1175/JHM-D-21-0211.1]. We show, using a worldwide catalog of disdrometric observations, how the Formula-R outperforms the ZR scaling law both in training and validation accuracy. 

The Formula-R algorithm could be used as the foundation of a universal remote sensing retrieval algorithm making the question "which ZR-relationship should we use?" a question of the past.

 

How to cite: Ignaccolo, M. and De Michele, C.: A novel algorithm for remote sensing rainfall retrieval, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3311, https://doi.org/10.5194/egusphere-egu25-3311, 2025.

High resolution rainfall data are essential to quantify small scale and fast hydrological processes. The objective of the paper is to determine temporal variability and spatial patterns of precipitation statistic of one-minute resolution rainfall across Germany. The German Weather Service (DWD) started in 1993 to deploy rain gauges that achieve 1 minute temporal and 0.01 mm volumetric resolution by combining tipping buckets with weigthing (rain[e]H3 by LAMBRECHT meteo GmbH and OTT Pluvio by OTT Hydromet). 345 of those stations all over Germany have data with more than 10 years. For each station empirical cumulative distribution functions (eCDF) of precipitation intensity and dry periods were derived. Data were then aggregated to lower resolutions ranging from 2 min to 4 months. For all aggregation levels we fitted power law, log-normal and Weibull distribution functions and compared the goodness of fit. To determine spatial correlations between stations we extracted intensity and dry period duration at a given frequency from the empirical distribution function and applied a correlation analysis with station longitude, latitude, elevation and total rainfall. Annual and diurnal variations were analysed by fitting a power law to a moving window of data. A 60d segment of the yearly cycle (combining data of all years) and a 4h segment of the daily cycle (combining data of all days) were used. Similar the dependence of the power-law coefficient on temperature was analysed with a moving window of 2.5K width, shifted between -10 to 30°C.

We show that rainfall intensity measured at 1 minute resolution shows a distinct power-law distribution for all stations. The dry period durations instead are not purely power-law distributed. When aggregated, the distribution of the data transitions to lognormal distribution at 15 min aggregation level and to a Weibull distribution from 6 hours onwards. This has significant implication for estimating flood risk and deriving design storm properties as each temporal resolution requires a different statistical distribution to be fitted. We conclude that the mixing of the intensity and dry-period statistic creates this effect. While total rainfall in Germany clearly varies, with high totals in the north-west and lower values in the east, the intensity distribution does not reflect that. We find no significant correlation with longitude, latitude, elevation nor total station rainfall. But the dry-period statistic correlates well. This leads to the conclusion that rainfall intensity statistic is very similar in all of Germany and the difference in recurrence intervals and total rainfall is mostly defined by the dry periods between rain events. The power-law exponent varies annually with a sine curve from -1 to -2 in phase with the annual temperature cycle. It also shows a clear diurnal cycle. It can be expected that those cycles are driven by a strong dependence on temperature. The power-law exponent is close to -3 at 0°C and -1 at 25°C, creating higher intensities at higher temperatures.

How to cite: Frechen, N. and Hinz, C.: One-minute rainfall data reveal temperature dependend seasonal and diurnal variability of the power-law distribution for Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6463, https://doi.org/10.5194/egusphere-egu25-6463, 2025.

EGU25-6983 | ECS | PICO | HS7.1

Multifractal analysis of Liquid Water Content vertical and temporal variability 

Emna Chikhaoui and Auguste Gires

Driven by complex mechanisms, precipitation exhibits extreme variability across scales both in space and time. A clearer insight into this variability can be obtained by exploring multiple parameters, such as the Liquid Water Content (LWC). It is a measurement that quantifies the amount of liquid water available in the atmosphere and as such it provides valuable information about precipitation variability across space and time. While extensive research has focused on analyzing LWC variability at the surface level, studies addressing the vertical variability remain relatively limited. However, it contributes to better understanding of rainfall dynamics, and notably the variability occurring at scales smaller than radar gate.

Within this scope, six months of a Micro Rain Radar PRO (MRR-PRO) observations were gathered in Ecole nationale des ponts et chaussées, Institut Polytechnique de Paris, which is located next to Paris, France. The MRR-PRO is a K-band weather radar that measures hydrometeors fall velocity up to more than 4 kilometers of altitude above its position with a 35 meters spatial resolution and a 10 seconds time step. From collected data and simple assumptions, various quantities related to rainfall drop size distribution including LWC can be derived. The generated data were analyzed to study the spatial and temporal variations of LWC using Universal Multifractals (UM); which is a physically based framework that assesses the variability of geophysical fields across wide ranges of scales with the help of only three parameters with physical interpretation.

In this study, two types of UM analysis are implemented. As a first step, the time series of  LWC at  each altitude is studied. As a second step, vertical profiles of LWC are analyzed and UM parameters characterizing vertical variability are derived. Obtained results and their interpretation in a space-time framework will be presented and discussed.

Authors acknowledge the France-Taiwan Ra2DW project for financial support (grant number by the French National Research Agency – ANR-23-CE01-0019-01).

How to cite: Chikhaoui, E. and Gires, A.: Multifractal analysis of Liquid Water Content vertical and temporal variability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6983, https://doi.org/10.5194/egusphere-egu25-6983, 2025.

The abstraction of precipitation can be defined as the difference between precipitation and runoff. Understanding the dynamics behind water abstraction could provide new insights into hydrological processes and contributes to improved water resource management strategies. This research aims to investigate the phenomenon of water abstraction and critically examine the widely acknowledged assumption that near-surface air temperature is the primary factor influencing the magnitude of water abstraction. The study employs a simplified water balance equation to quantify water abstraction, using observed data from dam catchments in Taiwan, Japan, and South Korea, which span a range of climate types. Data mining techniques, including linear regression and related statistical analyses, are applied to explore the relationship between precipitation and water abstraction across various timescales. Preliminary results indicate that, on a monthly timescale, there is generally a positive correlation between precipitation and water abstraction during the flood season (January–May and November–December) across all catchments. However, the relationship during the dry season (June–October) remains ambiguous. Among the three regions, Japan experiences the highest water abstraction during all seasons, whereas the lowest water abstraction is observed in South Korea during the dry season and in Taiwan during the flood season. On an annual timescale, Japan shows the relative highest water abstraction, while South Korea records the lowest. Notably, our findings diverge from previous research. In Taiwan, particularly during the flood season, an increased incidence of negative water abstraction has been observed. This phenomenon suggests that runoff processes in Taiwan are more influenced by groundwater dynamics than by precipitation.

How to cite: Lu, C. and You, J.-Y.: Observation and Comparison of Precipitation and Water Abstraction Data in Taiwan, Japan, and South Korea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7906, https://doi.org/10.5194/egusphere-egu25-7906, 2025.

EGU25-11476 | ECS | PICO | HS7.1

Retrieval of the hail size number distribution from polarimetric C-band weather radar using double-moment normalization 

Matteo Guidicelli, Alfonso Ferrone, Gionata Ghiggi, Marco Gabella, Urs Germann, and Alexis Berne

Estimating the distribution of hail sizes is crucial for assessing related weather hazards and potential damage to buildings, vehicles and agriculture. In this study, we present a novel technique for estimating the hail size number distribution (HSND) using polarimetric C-band radar data. A generalized additive model (GAM) is employed to estimate two empirical moments of the HSND, which is then reconstructed using double-moment normalization. This approach capitalizes on the relative invariance of the double-moment normalized HSND. The model is trained on data from the Swiss network of automatic hail sensors, spanning from September 2018 to August 2024 and covering three regions of Switzerland particularly prone to hail. Several polarimetric features are extracted from a 3D radar composite that combines observations from all operational Swiss radars. Among the various extracted features, the model selects the echo-top height of 50 dBZ reflectivity value at vertical polarization and the volume of the region with a cross-correlation coefficient rhoHV below 0.97, as these provided the best predictive performance. Radar-derived HSND estimates show good agreement with independent hail sensor observations. Additionally, the model is evaluated through comparisons with photogrammetric drone surveys and crowd-sourced reports of hail. This technique enables high spatio-temporal resolution (1 km and 5 minutes) retrievals of HSND and related metrics, such as kinetic energy. Further ground observations, particularly drone-based, are essential for more comprehensive evaluation of the retrieved HSND.

How to cite: Guidicelli, M., Ferrone, A., Ghiggi, G., Gabella, M., Germann, U., and Berne, A.: Retrieval of the hail size number distribution from polarimetric C-band weather radar using double-moment normalization, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11476, https://doi.org/10.5194/egusphere-egu25-11476, 2025.

Spatial and temporal interpolation methods are generally used for estimation of missing data. Objective selection of control points (sites) with available data in a region for use in spatial interpolation to estimate missing data in space and time is always a challenge. The numerical weights derived through spatial and temporal interpolation approaches attached to data available at different sites have an impact of the estimation of missing data. Parsimonious and robust interpolation models can be developed using schemes that objectively select optimal number of sites and methodologies that eliminate redundant sites and regulate the weights. In this study regularization schemes, mathematical programming model formulations and different feature selection methods used in machine learning field are developed and evaluated for optimal and objective selection of sites for estimation of missing precipitation records. Variants of regularization schemes such as ridge regression, lease absolute shrinkage selection operator (LASSO) and elastic net are experimented. Mixed integer nonlinear optimization programming (MINLP) models with binary variables and multiple feature selection methods are adopted in this work. A case study using precipitation data at several rain gauges in a temperate climatic region of Kentucky, USA is used to demonstrate the benefits of using regularization schemes and optimization with binary variables to select an optimal subset of control points. Results point to improved estimations when these approaches are used for estimation of missing precipitation data.

How to cite: Teegavarapu, R.: Objective and Optimal Spatial Interpolation Approaches for Imputing Missing Precipitation Records, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13245, https://doi.org/10.5194/egusphere-egu25-13245, 2025.

EGU25-13674 | ECS | PICO | HS7.1

 A decade-long analysis of rainfall in Rome based on disdrometer: Rain patterns and Intermittency  

Ravi Shankar Pandey, Natale Alberto Carrassi, Federico Porcù, and Elisa Adirosi

The study presents the first analysis of the rain structure based on 11 years (2013-2023) of continuous 1-min disdrometer data collected by the TC-Clima disdrometer located nearby Rome (Italy). The investigation employs various techniques, including delineating rainfall events based on different minimum inter-event times (MITs), calculating rain rate, mass-weighted mean diameter (Dm), as well as stratiform and convective precipitation classification. The dataset has been pre-processed to filter/remove missing/erroneous information and to ensure unbiased measurements. Seasonal variations showed that autumn had the highest rainfall accumulation (38.8%, 3126.8 mm), despite shorter rain durations (1116.5 hours) compared to winter (1446.5 hours). Winter contributed 28.2% (1986.65 mm) with prolonged rain events of smaller droplets (Dm = 0.98), while summer had the lowest total rainfall (10%, 1329.6 mm) but the highest average rain rate (3.4 mm/h) and largest drops (Dm = 1.39). The difference in drop sizes and rain types across seasons is important, as stratiform clouds, linked to steady rain, were more common in autumn and winter, while convective clouds, associated with intense, short-duration rain, dominated summer. We then focus on rainfall intermittency: the abrupt onset or interruptions of rainfall events. We quantify intermittency by using the intermittency fraction (IFr), i.e., the proportion of time with no rain during an event. Diurnal analysis of IFr revealed significant seasonal differences. Intermittency Fraction peaked between 9am and 2pm, with summer seeing sharp peaks before noon, followed by a rapid decrease in the afternoon. Winter maintained more consistent IFr throughout the day. Rain interruptions have been more frequent in winter, but these breaks were generally short, indicating long-duration, low-intensity rainfall. In contrast, summer had fewer interruptions, but they lasted longer due to intense, short-lived rain. These seasonal differences are robust and appear also by varying the fixed-time averages of the rainfall intermittency. Overall, the longest continuous rain event lasted 19.4hrs, while the longest dry spell was 534.4hrs. The rainfall is an intermittent natural phenomenon whose start and end are defined by rainless intervals referred to as minimum inter-event time, MIT. Intra event rainfall intermittency across various MITs shows higher IFrs at shorter MITs, particularly during summer. Our research also shows that disdrometer measures higher rain amount than conventional rain gauge with highest contrast in summer season. This further underscores the importance of high-resolution rainfall data for accurate predictions. Disdrometers confirmed to be a unique source of reliable and detailed rainfall measurements, which are essential for enhancing resilience against hydro-meteorological challenges such as flooding.

How to cite: Pandey, R. S., Carrassi, N. A., Porcù, F., and Adirosi, E.:  A decade-long analysis of rainfall in Rome based on disdrometer: Rain patterns and Intermittency , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13674, https://doi.org/10.5194/egusphere-egu25-13674, 2025.

Rainfall is known to exhibit extreme variability over wide range of space and time scale, which makes it challenging to characterize, model and even measure. Rainfall measurement devices have observation scales very different from one another ranging from roughly 20 cm in space and few tens seconds (or few minutes) in time for punctual measurement such as disdrometers (or rain gauge), to few hundreds meters in space and few minutes in time for operational weather radars, and up to few kilometres in space and few tens of minutes for satellite data. This very significant observation scale gap between these devices creates a challenge in the comparion simply because of the intrinsic variability of rainfall, even without considering instrumental biases associated to each device.

This work focuses on the impact of the intrinsic rainfall variability on the comparison between punctual (disdrometer or rain gauge) and weather radar rainfall measurement. In order to achieve this, the physically based and mathematically robust framework of Universal Multifractals will be used. It relies on the assumption that rainfall is generated through an underlying multiplicative process. In such framework, the rain rate field can be written as the resolution (defined as the ratio between the outer scale of the phenomenon and the observation scale) to the power of a singularity. This singularity is preserved through scales.

Rainfall data collected in UK and Taiwan are used. These include high-resolution radar composite products and ground gauge records. In the UK, C-band radar composite, Nimrod, at 5-min and 1-km resolutions is used to compare with 1-min rainfall records derived from tipping bucket gauge records, while, in Taiwan, S-band radar composite, QPESUM, at 10-min and 1-km resolutions is used to compare with 10-second disdrometer rainfall records.

The concept of singularity is used to suggest an innovative comparison approach between rainfall measurement devices. More precisely, the local singularity along with the associated uncertainty is assessed using radar data on the range of available space time scales and then compared with the one of disdrometer or rain gauge accounting for the ratio between the observation scales. Results and interpretation of this novel comparison method on the available data will be discussed.

Authors acknowledge the France-Taiwan Ra2DW project (supported by the French National Research Agency – ANR-23-CE01-0019-01 and Taiwan’s National Science and Technology Council – 113-2923-M-002-001-MY4) for partial financial support.

How to cite: Gires, A. and Wang, L.-P.: Multifractal singularity to bridge the scale gap between various rainfall measurement devices, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13715, https://doi.org/10.5194/egusphere-egu25-13715, 2025.

EGU25-15409 | PICO | HS7.1

The wind effects on disdrometer and rain gauges measurements: results from a 4-year long rain series data-set in Pescara and a 10-year long rain series data-set in Calabria (Italy) 

Elisa Adirosi, Leone Parasporo, Luca Baldini, Arianna Cauretuccio, Enrico Chinchella, Tommaso Caloiero, and Luca Lanza

Disdrometers are in-situ, non-catching devices capable of measuring the size and fall velocity (for most models) of each individual hydrometeor (solid or liquid) that enters their measurement volume. These devices are primarily used for research purposes, and their data have applications in fields such as meteorology, climatology, and hydrology. However, their measurements can be influenced by the presence of wind. In this context, one of the objectives of the PRIN project titled “Fostering innovation in precipitation measurements: from drop size to hydrological and climatic scales” is to quantify the accuracy of disdrometers. In this regard, data collected from a Thies Clima disdrometer and wind sensors installed in the city of Pescara serve as a valuable resource for: i) characterizing precipitation, ii) conducting a joint analysis of atmospheric conditions, including wind directionand speed, and iii) evaluating the effect of wind on disdrometer measurements. The dataset covers the period from July 2021 to August 2024, although it includes significant interruptions. This study presents the main characteristics of the site in terms of wind and rain distributions, as well as their joint distributions. Additionally, the effects of wind on disdrometer measurements are quantified in terms of the associated bias on on DSD (Drop Size Distribution) estimation. Results indicate that wind-corrected DSDs differ, on average, by 136.41m−3 ·mm−1 in terms of root mean square error compared to uncorrected DSDs. Subsequently, since we do not have a DSD from the rain gauge, we hypothesize that it has the form of an exponential αeβ, and we interpolate these parameters from the disdrometer data. Then this parametrs are used to apply corrections to nearby rain gauge measurements, and the corrected and uncorrected values are compared. These differences are found to be statistically significant. Furthermore, twenty-six stations in Calabria, equipped with rain gauges and anemometers, are analyzed using the same DSD parameters derived from the Pescara dataset. Precipitation amounts obtained from corrected and uncorrected DSDs are compared with corresponding corrected and uncorrected rain gauge data, revealing statistically significant differences. These findings provide insight into the effects of the applied correction on rain rate measurements.
Acknowledgments
This work was carried out within the framework of the ongoing Italian national project PRIN2022MYTKP4 “Fostering innovation in precipitation measurements: from drop size to hydrological and climatic scales”.

How to cite: Adirosi, E., Parasporo, L., Baldini, L., Cauretuccio, A., Chinchella, E., Caloiero, T., and Lanza, L.: The wind effects on disdrometer and rain gauges measurements: results from a 4-year long rain series data-set in Pescara and a 10-year long rain series data-set in Calabria (Italy), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15409, https://doi.org/10.5194/egusphere-egu25-15409, 2025.

EGU25-15697 | ECS | PICO | HS7.1

Rain scintillation spectra from microwave links: A potential source of information for raindrop size distributions 

Peiyuan Wang, Arjan Droste, Marc Schleiss, and Remko Uijlenhoet

Rainfall has been monitored with microwave links opportunistically for nearly 20 years. So far, most studies have focused on retrieving rainfall rates using the mean received signal, based on the power-law relation between specific attenuation and rainfall rate. However, theories and measurements have indicated that the power spectral density (PSD) of received signal contains extra information about rainfall. The drop size distribution (DSD) and the motion of raindrops both play a role in determining the scintillation spectrum of rain. To evaluate the feasibility of making use of rain spectra for retrieving information about DSDs, measurements from different experimental datasets are investigated. Initial results indicate that some information about rainfall (e.g. rainfall rate) is indeed retained in the spectra measured by a radio link at 26 GHz and a scintillometer at 160 GHz. Furthermore, a simulation of the PSD of the received voltage during rain is made to gain understandings of its behavior. The simulation, based on Ishimaru’s work (1978), allows for the customization of various settings (e.g., wavelength, geometry, antenna gain functions) of radio links, as well as the DSD at different locations along the links. It is shown that large raindrops have more influence on the PSD of received voltage than smaller raindrops. A theoretical method to retrieve DSD from the PSD of the received voltage is proposed and its performance is assessed by simulation. Results show that the concentration of the tiniest raindrops is hard to retrieve because of their minor impacts on PSD. In the simulation, the concentration of larger raindrops can be relatively reliably retrieved, even when a large variation of DSDs is present along the microwave link.

How to cite: Wang, P., Droste, A., Schleiss, M., and Uijlenhoet, R.: Rain scintillation spectra from microwave links: A potential source of information for raindrop size distributions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15697, https://doi.org/10.5194/egusphere-egu25-15697, 2025.

EGU25-15743 | ECS | PICO | HS7.1

Small-scale spatial rainfall variability during the extreme convective rain event of June 11th, 2018, over the city of Lausanne 

Adrien Liernur, Lionel Peyraud, Marco Gabella, Urs Germann, and Alexis Berne

Localized and Intense Rainfall Events (LIREs) can cause significant societal and economic damages. Typically developing over very small spatial and temporal scales, the accurate characterization and forecasting of such events remains, however, particularly challenging. By collecting distributed space-time observations, weather radars can provide useful information for the analysis of such events. In this study we take advantage of the experimental high-resolution radar data from the MeteoSwiss operational radar network available at 83 m radial resolution, every 5 minutes, over 20 different elevations to analyze the small-scale spatial variability associated with the extreme Lausanne LIRE of June 11th, 2018, leading to the largest ever recorded 10-min rain gauge accumulation in Switzerland (41 mm). First, investigating the large-scale processes associated with this extreme event, a synoptic and dynamic analysis was conducted. This revealed the presence of a moderately unstable maritime tropical airmass which aided in the formation of a multicell thunderstorm which produced a wet microburst right over the city of Lausanne pouring an enormous quantity of water over very small spatial and temporal scales and leading to considerable localized flood and wind damage. Then, relying on the high-resolution radar data, the variability at small scale was measured by comparing rain rate values derived at different resolutions. More specifically, starting from the 83 m radar data, different existing hydrometeor-specific Z-R / Z-S relationships were used to compute an equivalent rain rate value at the gate level. Those were then compared against the corresponding rain rate values integrated at coarser radial resolutions of 500 m and 1000 m, and the difference across resolutions was derived as an indicator of small-scale spatial variability. With 1.5%, 0.41% and 0.18% of the total extracted and pre-processed gate volume showing differences larger than 25, 50 and 75 mm/hr between the 83 m and the 500 m data, a few but extreme small-scale rainfall variability peaks were observed, mostly associated with intensity peaks. Although most of these peaks were located above or within the melting layer, several of them were still observed below the melting layer, at proximity to the ground, and potentially decisive for hydrological applications. Converting this 3D information into 2D maps of sub-grid variability, a significant variability at the 5 min / 1km2 resolution was observed highlighting not only the highly dynamic evolution of this event but also and the added value of high-resolution radar data to capture small-scale peaks associated with this extreme LIRE. By providing complementary insights on rainfall variability peaks, the retrieved sub-grid information can help improve the characterization of LIRE and enrich existing rainfall products.

How to cite: Liernur, A., Peyraud, L., Gabella, M., Germann, U., and Berne, A.: Small-scale spatial rainfall variability during the extreme convective rain event of June 11th, 2018, over the city of Lausanne, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15743, https://doi.org/10.5194/egusphere-egu25-15743, 2025.

EGU25-17651 | PICO | HS7.1

Wind tunnel experiments to evaluate the wind-induced bias on disdrometer measurements 

Luca G. Lanza, Enrico Chinchella, Filippo Calamelli, Arianna Cauteruccio, and Daniele Rocchi

Wind has a significant impact on precipitation measurement instruments, including disdrometers, by inducing aerodynamic disturbances around their bodies. These airflow features divert trajectories of falling hydrometeors, often reducing the amount of precipitation detected when compared to  windless conditions. Furthermore, the shape of disdrometers, which is non-radially symmetric, makes the wind-induced bias dependent on wind direction. Traditionally, field experiments have been used to develop corrections for the wind-induced bias. However, Computational Fluid Dynamics (CFD) simulations offer a more versatile approach for studying wind-induced bias on different instrument designs under varying climatic conditions. In this work a wind tunnel experimental campaign was conducted to show the interaction between wind and disdrometers and to validate a suitable CFD model by providing detailed data on drop trajectories. Full-scale tests were conducted in the high-speed test section of the Wind Tunnel facility available at Politecnico di Milano. The chamber (4m wide, 3.8m high and 6m long) is characterized by a nearly laminar flow and a narrow boundary layer. The disdrometers were fixed to the ground on a rotating plate to facilitate alignment with the flow direction. Furthermore, a specially designed drop generator – attached to a moving gantry – was used to release water drops into the wind flow, allowing precise control of drop diameter, release height and timing. Finally, a high-speed camera, operating at 1000 fps, recorded the trajectories of the drops approaching the sensing areas of the disdrometers. Images were processed to identify each drop, calculate their velocity and track their movement through the camera field of view. The study focused on two disdrometer models, the Thies CLIMA LPM and the OTT Parsivel2, which use an optical method to measure drop size and velocity. The experiments were conducted for wind speeds of 10 m/s, drop diameters ranging from 1.0 to 1.2 mm, and three wind directions (0°, 45°, and 90°). Results showed that wind significantly alters drop trajectories, often diverting them away from the sensing area or causing them to collide with the instrument body. A numerical model - already used in e.g., Chinchella et al., (2024) – was validated by simulating the experimental conditions and comparing the results against observations. Validation shows that the numerical approach is suitable for developing adjustment curves to correct disdrometer measurements under windy conditions. This work further highlights the importance of addressing wind effects in precipitation measurements, by applying correction curves (see e.g., Chinchella et al., 2024) to enhance the accuracy of rainfall measurements obtained from disdrometers like the Thies CLIMA LPM or the OTT Parsivel2.

ACKNOWLEDGMENTS

The wind tunnel campaign on disdrometers was carried out within the framework of the Italian national projects PRIN2022MYTKP4 “Fostering innovation in precipitation measurements: from drop size to hydrological and climatic scales”.

References:

Chinchella E., Cauteruccio, A., & Lanza, L. G. (2024). Quantifying the wind-induced bias of rainfall measurements for the Thies CLIMA optical disdrometer. Water Resources Research, 60(10), e2024WR037366. https://doi.org/10.1029/2024WR037366   

How to cite: Lanza, L. G., Chinchella, E., Calamelli, F., Cauteruccio, A., and Rocchi, D.: Wind tunnel experiments to evaluate the wind-induced bias on disdrometer measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17651, https://doi.org/10.5194/egusphere-egu25-17651, 2025.

EGU25-17854 | PICO | HS7.1

Assessing the Impact of Weather Conditions on Radar-Based Rainfall Estimation in the Tropics: A Case Study in Thailand 

Narongrit Luangdilok, Ruben Imhoff, Claudia Brauer, and Albrecht Weerts

In hydrological modeling and forecasting, rainfall data is a key factor in determining the model’s accuracy. The higher the accuracy of the estimated rainfall, the more accurate the model’s predictions can be. Rain gauges can be utilized to estimate the amount of rainfall within a catchment area but their effectiveness is often limited by the sparse distribution of rain gauges and the lack of sufficient spatial information they provide for comprehensive distributed hydrological simulations. Weather radar serves as an alternative source of rainfall data, capable of providing remotely sensed rainfall estimates with high temporal and spatial resolution. However, conventional radar quantitative precipitation estimation (QPE) is subject to uncertainties, primarily arising from variations in the drop size distribution (DSD) of hydrometeors and variations in vertical profile reflectivity (VPR). Those variations are typically influenced by the local climate and weather conditions and their impacts on the performance of QPE remains a subject of research especially in tropical regions. Therefore, this study aims to investigate relationships between weather conditions and the performance of radar QPE using statistical and machine learning approaches at different time scales. In Thailand, the radar-based rainfall data is derived with a standard fixed power law relationship between radar reflectivity and rain rate, from three weather radars located in different parts of the country. The rainfall estimates from this radar rainfall product are investigated with weather conditions from ERA5 reanalysis datasets and local observations in the period of 2022-2024. The findings help us to identify the key factors influencing the accuracy of radar rainfall estimation, which can be used to improve radar rainfall estimation, for example through finding adequate predictors for the construction of a dynamic Z-R relationship in tropical conditions. Future studies could expand this analysis by integrating these impact factors into radar QPEs and implementing improved estimated rainfall products in hydrological models.

How to cite: Luangdilok, N., Imhoff, R., Brauer, C., and Weerts, A.: Assessing the Impact of Weather Conditions on Radar-Based Rainfall Estimation in the Tropics: A Case Study in Thailand, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17854, https://doi.org/10.5194/egusphere-egu25-17854, 2025.

The Advanced Quantitative Precipitation Information Project (AQPI) provides supplemental radar observations across the Greater San Francisco Bay Area – specifically, 4 X-band radars (3 already installed) and 1 C-band radar, by the end of 2025. These new radars complement the existing radar network by filling horizontal and vertical gaps in coverage caused by terrain blockage and distance from the existing radars. Additionally, the new radars operate at a much higher spatial and temporal resolution than the existing network. Together, these aspects provide for much more accurate estimation of rainfall rates and improved short-term forecast capability across the area. Local stakeholders and emergency managers can make direct use of the rainfall estimations, both in real time and integrated over various historical periods, as well as the improved forecasts to optimize any number of operations. These include emergency response, water and wastewater management, flood response, aquifer recharge, transportation efficiencies, and more. The data from AQPI radars can also be assimilated into short-range forecast models and used as an improved forcing dataset for hydrology models, especially those predicting streamflow for small and flashy basins across the area. A robust user interface provides data visualization and delivery, and will continue to mature as the program grows. Notably, AQPI represents a unique collaboration amongst local, state, and federal level entities from the academic, governmental, and private sectors.

This presentation will focus on key aspects of the program including an overview of system hardware, software, and the user interface that ties it all together. It will also highlight a case study that demonstrates the value of the AQPI radar precipitation estimates with respect to those of the existing network. And finally, it will describe a vision of the future of this important effort.

How to cite: Rutz, J., Vilela, R., Steen, M., Chandrasekaran, V., and Ralph, M.: The Advanced Quantitative Precipitation Information (AQPI) Project: Building a State-of-the-Art Precipitation Observation and Forecast System for the Greater San Francisco Bay Area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-71, https://doi.org/10.5194/egusphere-egu25-71, 2025.

EGU25-162 | Orals | AS1.18

The V07B Near-realtime (NRT) update of IMERG and extension of record to January 1998 

Erich Franz Stocker, Jason West, Yi Song, and Owen Kelley

During 2024 two important events impacted the processing of the IMERG near-realtime product. On 1 June 2024 the NRT was converted to use the RedHat RHEL 8 operating system.  Equally importantly the system was converted to use python 3. Coupled with these system updates, the IMERG NRT algorithms were updated to V07B. This update had been implemented almost a year earlier for the Final IMERG product (appx. 3 months latency from realtime). This much improved algorithm corrected some issues with V06 and added features some of which are discussed in this paper. In October 2024 IMERG products were extended back to January of 1998. Until V07 IMERG only extended back to May 2000. This restriction was due to IR products used as part of IMERG processing not being available before 2000. This paper will provide information about this early phase processing and provide images that illuminate processing for this period. The paper will also discuss the plans and status of availability of NRT version of the 1998-2000 data for early and late versions of IMERG V07B.

How to cite: Stocker, E. F., West, J., Song, Y., and Kelley, O.: The V07B Near-realtime (NRT) update of IMERG and extension of record to January 1998, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-162, https://doi.org/10.5194/egusphere-egu25-162, 2025.

EGU25-356 | Posters on site | AS1.18

Study of freezing rain in Belgrade from 1949 to 2022 

Nemanja Kovačević, Katarina Veljović Koračin, and Suzana Putniković

A paper examines the climatology of freezing rain events in Belgrade (Serbia) in the period from 1949 to 2022. This phenomenon occurs from October to March, most frequently in January and December, mostly at night (00–07 local time), and lasts up to 2 hours in 62% of cases. The onset of freezing rain events occurs most frequently between 00 and 01 local time (~ 16 %). The second maximum of these events is between 06 and 07 local time (~ 11 %). The vertical temperature profiles for days with freezing rain show that 60.42 % of all events have a characteristic “warm nose” at altitude (near the 850 hPa level), below which there is usually a temperature inversion and a supercooled layer of air near the ground. This result is consistent with the study [1], which found that in 30–40% of all vertical soundings there was no “warm nose” above the supercooled air layer on the ground. This study shows that the number of freezing rain events has decreased over time, which can be attributed to climate change. The analysis of the surface maps shows that freezing rain occurs under the same conditions as the local Košava wind: with almost meridional isobars and a typical southeasterly flow with strong pressure gradients between the low pressure area in the western Mediterranean and the anticyclone in the east. The analysis of the upper-level maps shows a wind shear with an almost westerly flow, which also indicates warm air advection in the analyzed layer.

[1] Carrière, J.-M., Lainard, C., Le Bot, C., Robart, F. 2000. A climatological study of surface freezing precipitation in Europe, Meteorol. Appl., 7, 229–238.

Keywords: freezing rain, climatology, Košava 

Acknowledgement: This research was supported by the Science Fund of the Republic of Serbia, No. 7389, Project: "Extreme weather events in Serbia - analysis, modelling and impacts” - EXTREMES

How to cite: Kovačević, N., Veljović Koračin, K., and Putniković, S.: Study of freezing rain in Belgrade from 1949 to 2022, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-356, https://doi.org/10.5194/egusphere-egu25-356, 2025.

This study focuses on the development of a new high-resolution gridded rainfall dataset for Senegal, which is essential for rainfed agriculture, which is sensitive to climate variability. Given the limited number of rain gauges, the research will evaluate 17 publicly available gridded rainfall datasets (P-datasets) against data from 21 stations of the Senegalese National Meteorological Service (ANACIM) over a 17-year period (2005-2021). The evaluation uses several agroclimatic indices, including rainfall onset and cessation, rainy season duration, and extreme events. The results show that the reliability of the P-datasets varies significantly depending on the metrics used. For total precipitation, ARC2, CHIRPS, ERA5 and RFEv2 were found to be the most reliable datasets. ERA5 achieved the highest Kling-Gupta Efficiency (KGE) value of 0.81 at the daily scale. In terms of agroclimatic parameters, ARC2, CHIRPS and RFEv2 excelled in accurately representing the start (KGE ≥ 0.45) and end (KGE ≥ 0.39) dates of the rainy season. However, the P datasets generally overestimate rainfall events and struggle to identify dry spells. The newly constructed merged dataset (M-dataset) showed over 100% improvement in correlation for daily estimates and a significant reduction in bias of 99.19% for ARC2, 80% for CHIRPS and 90.57% for RFEv2. This research provides critical insight into the selection of appropriate datasets to improve climate information for agricultural decision making in Senegal.

How to cite: Asse, M.: Reliability assessment of 17 gridded rainfall dataset for the construction of a daily high-resolution reanalysis (4km) across Senegal for agroclimatic applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-539, https://doi.org/10.5194/egusphere-egu25-539, 2025.

EGU25-836 | ECS | Orals | AS1.18

Vertical profiles of precipitating clouds in Monsoon Regions using the GPM satellite  

Amit Kumar and Dushmanta Ranjan Pattanaik

The vertical structure of precipitating clouds plays a vital role in shaping the rainfall characteristics of the surrounding region. Based on the dual-frequency space-borne precipitation radar observation placed on the Global Precipitation Measurement (GPM) satellite for the years 2014-2023, we examined the vertical profiles of precipitating clouds over three different regions of India (Western Ghats, Central India, and Arabian Sea), based on the dual-frequency space-borne precipitation radar observation placed on the Global Precipitation Measurement (GPM) satellite for the years 2014-2023. Vertical distribution of radar reflectivity (Z), rain rate (R), mass-weighted mean diameter (Dm), and normalized intercept parameter (Nw) with altitude for the convective and stratiform clouds for each region is determined. The distribution shows considerable variation with altitude due to the difference in microphysical properties of precipitating clouds with cloud type and topography. Intense convective cloud formation is dominated over the Western Ghats region with high echo tops (>10 km), near-surface Z > 40 dBZ, large R and bigger rain droplets (high Dm) due to strong orographic lifting and enhanced collision-coalescence process in the precipitating clouds. Over the Central India region, deep convective precipitating clouds often form during the monsoon depression, exhibiting echo top above 12 km and considerable variation in rain droplet diameter due to intense updrafts with increased concentration of ice particles. However, relatively weak marine convective clouds were observed over the Arabian Sea, having echo tops of up to 8 km, small R, low near-surface Z, and significant concentrations of smaller rain droplets (low Dm). Stratiform cloud vertical profiles are uniform with little variation. Regional comparison showing the domination of different microphysical processes for stratiform and convective precipitation in all three regions.

How to cite: Kumar, A. and Pattanaik, D. R.: Vertical profiles of precipitating clouds in Monsoon Regions using the GPM satellite , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-836, https://doi.org/10.5194/egusphere-egu25-836, 2025.

EGU25-1549 | Posters on site | AS1.18

Annual and seasonal extreme precipitation events in Novi Sad 

Ivana Tosic, Antonio Samuel Alves da Silva, Suzana Putniković, Lazar Filipović, Vladimir Djurdjević, Borko Stosic, and Tatijana Stosic

Serbia is located in the central part of the Balkan Peninsula, and is characterized by a continental climate in the north, a temperate continental climate in the central part and a modified Mediterranean climate in the south. The average annual precipitation is between 500 and 700 mm in the lowlands and over 1000 mm in the mountains. Novi Sad (45°20’ north latitude, 19°51’ east longitude, 84 m altitude) is located in the south of the Pannonian Plain and is the capital of the autonomous province of Vojvodina in northern Serbia. The average annual precipitation in the period 1961-2020 amounted to 655.5 mm.

The following extreme precipitation events were analysed based on daily precipitation data from 1961 to 2020 in Novi Sad: very heavy precipitation days (RR20), highest 1-day precipitation amount (Rx1d) and highest 3-day precipitation amount (Rx3d). The modified Mann-Kendall test (MMK) and the Sen’s slope method are used to examine the possible trends and their magnitudes. The generalised extreme value distribution (GEV) and the generalised Pareto distribution (GPD) were used for the analysis of extreme precipitation.

A small number of RR20 was observed in all seasons except summer. The lowest number of heavy precipitation days was recorded in winter. The mean value of RR20 was 2.4 from 1961 to 1990 and 3.2 from 1991 to 2020 in summer, with a maximum value of 9 and 8, respectively. The highest 1-day and 3-day precipitation values were measured in summer. The highest values of Rx1d (121.9 mm) and Rx3d (149.4 mm) were observed in spring 2015. A significant positive trend was observed for Rx3d in all seasons, for Rx1d in spring, summer and fall and for RR20 in spring and fall. A positive but non-significant trend was observed for Rx1d in winter and for RR20 in summer. A significant positive trend was observed for all indices on an annual basis.

The GPD distribution was fitted to the daily precipitation series with a threshold of 20 mm in Novi Sad. The maximum likelihood estimates of the location and scale parameters were 30.36 and 197.7, respectively. Maximising the GEV log-likelihood for Rx1d and Rx3d leads to the estimation of the shape parameter 0.31 for Rx1d and 0.17 for Rx3d, respectively. The positive values of the shape parameter indicate that the Fréchet distribution was fitted to the highest 1-day and 3-day precipitation amounts in Novi Sad.

How to cite: Tosic, I., Alves da Silva, A. S., Putniković, S., Filipović, L., Djurdjević, V., Stosic, B., and Stosic, T.: Annual and seasonal extreme precipitation events in Novi Sad, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1549, https://doi.org/10.5194/egusphere-egu25-1549, 2025.

EGU25-1657 | Orals | AS1.18

Precipitation Uncertainties at Climate Time Scales  

Christian Kummerow

The Global Precipitation Measurement (GPM) mission was launched in February 2014 as a joint mission between JAXA from Japan and NASA from the United States.  By applying the insight provided by the GPM radars, the program has contributed enormously to the quality of the passive microwave radiometer time series that now spans almost 40 years.  This talk will examine the long time series of precipitation from 3 approaches.  The first is an uncertainty analysis based upon first principles.  It shows that time series can be homogenized, but that potential changes in convective organization over annual time scale must be included as a source of uncertainty in order to homogenize the time series of different satellites.  This is verified with the second approach that focuses on closing the water budget on regional scales.  While not as direct, it also hints strongly at the fact that our current time series overestimate precipitation when convection is better organized into large Mesoscale Convective Complexes.  The final approach seeks to correlate biases with large scale meteorological conditions to also show that biases due to convective organization are predictable.  While not applied in any product yet, this insight may serve as a blueprint for gaining confidence in our time series of precipitation where even a 1% change/decade in global precipitation is more than currently expected from observed warming trends.

How to cite: Kummerow, C.: Precipitation Uncertainties at Climate Time Scales , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1657, https://doi.org/10.5194/egusphere-egu25-1657, 2025.

Snowfall significantly affects regional climate and water resources across mountainous and high-elevation regions, where it determines seasonal water availability and influences local hydrological processes. The high spatial and temporal heterogeneity of snowfall in complex terrain regions poses considerable challenges for conventional observation networks Satellite-based precipitation products provide an effective approach to monitor snowfall from regional to global scales. However, validating these products against ground observations remains essential for quantifying their uncertainties.

The Global Precipitation Measurement (GPM) mission's latest IMERG algorithm has been updated to improve its snowfall retrieval capabilities, incorporating enhanced detection methods and refined quantification procedures. However, comprehensive evaluation across different monitoring networks remains crucial for understanding its performance in various environmental conditions. This study examines IMERG V07B's snowfall estimation accuracy through systematic comparison with diverse ground-based monitoring networks over mainland China, including standard meteorological stations, automatic weather stations, and specialized snowfall observation sites.

By leveraging these multi-source observations, we investigate IMERG's performance not only in terms of snowfall amount but also in capturing the temporal characteristics of snowfall events, including intensity distribution and duration patterns. The evaluation is stratified by elevation zones and network density to assess the impact of topographic complexity and observation capability on validation results. Initial findings reveal varying degrees of estimation accuracy across different network types, with notable challenges in regions with complex terrain and sparse monitoring coverage. We also compare the differences in snowfall estimation between IMERG V06B and IMERG V07B.

Our comprehensive assessment provides valuable insights into the strengths and limitations of IMERG V07B's snowfall estimates across different monitoring environments, offering essential guidance for both algorithm refinement and product applications in various research and operational contexts.

How to cite: Li, X. and wang, N.: Evaluation of satellite-based snowfall estimates: A comprehensive assessment of IMERG V07B across diverse monitoring networks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2362, https://doi.org/10.5194/egusphere-egu25-2362, 2025.

One of the primary challenges in satellite infrared (IR) quantitative precipitation estimates (QPEs) is accurately characterizing the nonlinear relationship between cloud properties and rainfall rates. This research proposes a deep neural network (DNN) method to classify clouds as rainy or non-rainy using brightness temperatures (BTs), reflectances (Refs), and cloud microphysical properties derived from the Advanced Himawari Imager (AHI) aboard the Himawari-8/9 satellite. The study incorporates cloud microphysical properties with BTs and Refs in the DNN model training process and conducts a comprehensive assessment of these features to elucidate their physical properties. The DNN-trained QPE models are validated by ground-based radar observation and compared to operational satellite-derived precipitation products like GSMaP and IMERG. The results indicate that including cloud microphysical properties enhances QPE model performance, with promising implications for real-time precipitation monitoring in East Asia.

How to cite: Liu, C.-Y. and Lin, M.-Y.: Application of Machine Learning Techniques in Satellite Precipitation Detection Using Himawari Spectral and Cloud Data , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2485, https://doi.org/10.5194/egusphere-egu25-2485, 2025.

It has been widely reported that precipitation tends to occur more in the form of rainfall rather than snowfall under global warming, as expected from theory. However, the observed data across China from 1961 to 2022 show that the rainfall to total precipitation rate decreased, especially in Northwest and Northeast China. This study investigates this paradox from perspective of the time-variable observational errors in the precipitation observation. The national standard gauge without a wind shield has long been used in China. There is an undercatch issue with the gauge caused by the turbulence generated when wind blows over it. This issue is more severe for snow and is exacerbated during strong winds. To improve the accuracy of snowfall measurement, new weighing gauges with one-layer wind shield have been deployed since 2009 in China. The authors conducted wind-induced error corrections for rainfall and snowfall at approximately 2300 national weather stations. It was found that the national mean annual precipitation, rainfall, snowfall were 794 mm, 763 mm, and 27 mm before correction and were 854 mm, 810 mm, and 40 mm after correction. After correction, the national mean rainfall to total precipitation rate showed an increasing trend (0.17 %/decade) from 1961 to 2022 instead of a decreasing trend (-0.04 %/decade) in the raw data. Especially, the trend of rainfall proportions in the Northwest China and the Northeast China changed from significant negative to positive. The key reason for this change is that wind-induced error decreased due to a reduction in surface wind speed, which is amplified by the instrument replacement. This is more obvious for snowfall.

How to cite: Li, Y. and Wang, K.: Time-variable observational errors explain the spurious rainfall and snowfall proportion trend in China under global warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2830, https://doi.org/10.5194/egusphere-egu25-2830, 2025.

EGU25-3399 | Posters on site | AS1.18

Convective and stratiform rainfall characteristics from ground-based observations 

Xinxin Xie and Xiaofeng Li

This study investigates precipitation observed by collocated ground-based instruments at the rooftop observatory in Zhuhai, a coastal city located at the southern tip of the Pearl River Delta of Guangdong Province in South China. Two-year ground-based observations collected from a tipping-bucket rain gauge (RG), two laser disdrometers (PARSIVEL and Present Weather Sensor 100 (PWS)), and a vertically pointing Doppler Micro Rain Radar-2 (MRR), are analyzed in this study. The precipitation from January 2022 to December 2023 is classified into convective, stratiform, and undetermined rainfall categories with the PARSIVEL observations. Statistics are conducted to provide an overview of the rainfall at the coastal city after quality control. An insight into raindrop size distributions indicates that under stratiform rainfall events, measurement discrepancies between the observation instruments can be alleviated, and good consistency are found for the collocated deployment which mitigates uncertainties originating from spatial/temporal variabilities. The rainfall microphysics for convective and stratiform events are further characterized with the two-year dataset.

How to cite: Xie, X. and Li, X.: Convective and stratiform rainfall characteristics from ground-based observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3399, https://doi.org/10.5194/egusphere-egu25-3399, 2025.

EGU25-3492 | ECS | Orals | AS1.18

Machine Learning-based Precipitation Merging: Selection of Input Features and Evaluation Benchmarks 

Yue Xu, Guoqiang Tang, Lingjie Li, Wentao Xiong, and Wei Wan

Multi-source merging is essential for creating high-quality gridded precipitation datasets. Machine learning (ML) and/or deep learning (DL) algorithms have achieved inspiring success in this area. This study aims to explore two critical yet underexplored issues in ML-based precipitation merging, i.e., the selection of input features and evaluation benchmarks.

The first issue is about input features of ML models, which often include precipitation products such as satellite and reanalysis datasets, along with auxiliary features like topographical and meteorological variables. One major concern is data independence. Many precipitation products, particularly satellite datasets, are calibrated using similar gauge data, yet the impact of this interdependence on ML-based merging performance is largely unknown. Another challenge is the interaction between input features and regional characteristics, such as climatic regimes, topographical features and gauge density, which affects model generalization across regions or scales but receives little attention in current research.

The second issue relates to benchmark selection. Processes like merging, bias correction, downscaling, and interpolation often employ similar supervised learning frameworks: utilizing high-accuracy reference data (e.g., gauge observations) as training labels with various static or dynamic variables (e.g., latitude and longitude, low-accuracy precipitation products) as features. The ambiguous boundaries between these techniques leads to diverse benchmark choices, ranging from original datasets to sophisticated methods such as geographically weighted regression (GWR). This inconsistency fosters subjective and potentially misleading evaluations, impeding progress in merging precipitation datasets with ML methods.

We investigate these issues through a series of experiments merging five precipitation datasets and high-density gauge data in mainland China, using multiple ML methods including random forest, convolutional neural network and artificial neural network with self-attention modules. The experiments involve varying degrees of data dependence, across eight sub-regions with diverse geographical conditions and gauge densities, and are compared against several benchmark datasets and methods.

By controlling the data dependence, our findings highlight its impact on spatial estimation. Additionally, we identify optimal feature selections across different regions and gauge densities. Interestingly, in areas with low gauge density, simple feature sets without auxiliary environmental variables often outperform those with complex predictors. Moreover, our results show that the ML models function more as interpolation rather than merging, suggesting that complex interpolation algorithms such as GWR might serve as more fitting benchmarks. Our work offers critical insights not only for precipitation datasets but also applicable to a wide range of geoscience data, emphasizing the importance of comprehensive evaluations beyond simplistic comparisons and hasty conclusions.

How to cite: Xu, Y., Tang, G., Li, L., Xiong, W., and Wan, W.: Machine Learning-based Precipitation Merging: Selection of Input Features and Evaluation Benchmarks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3492, https://doi.org/10.5194/egusphere-egu25-3492, 2025.

EGU25-3513 | Posters on site | AS1.18

Change in the distribution of precipitation events due to the temperature increase 

Zbyněk Sokol, Daniela Řezáčová, and Kateřina Skripniková

We investigated the dependence of several characteristics of precipitation events on ground temperature. We defined the precipitation events as a time-continuous events based on hourly precipitation data, using a threshold of 0.2 mm/h for the rain / non-rain distribution. We considered ground temperature before the start of precipitation to ensure that the temperature was not affected by precipitation. We investigated the precipitation events for the warm half of the year (from April to September) and compared their characteristics for (i) precipitation events obtained from ground measurements for the period 1998-2019 from 97 precipitation stations, (ii) precipitation events based on reanalyses for a 25-year long period (1990-2014) and (iii) precipitation events using climate projections for three future periods (2026-2050, 2051-2075 and 2076-2100). The reanalyses and climate projections were calculated using a modified ALADIN NWP model with a horizontal resolution of 2.3 km.The results show a difference in the precipitation events determined from measured data as compared to those determined by the model. This is likely related to the significantly different number of the data and the fact that the model precipitation is smoother than the measured precipitation. The characteristics of precipitation events based on reanalyses and climate projections are similar in structure, but the projections show an increase in precipitation with increasing temperature in future to a certain temperature threshold. 

How to cite: Sokol, Z., Řezáčová, D., and Skripniková, K.: Change in the distribution of precipitation events due to the temperature increase, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3513, https://doi.org/10.5194/egusphere-egu25-3513, 2025.

EGU25-4014 | ECS | Posters on site | AS1.18

Modeling the Impact of Land Use Dynamics on Flooding: A Case Study of Hafr Al-Batin, Saudi Arabia 

Ahmed Al-Areeq and Abdirizak Dirie

Land use and land cover (LULC) changes are known to significantly affect hydrological processes, directly influencing the frequency, magnitude, and spatial distribution of flood events. This study focuses on understanding the impact of LULC changes on flood dynamics in Hafr Al-Batin, Saudi Arabia, a region highly susceptible to flooding due to a combination of natural and anthropogenic factors. Remote sensing data, acquired from satellite imagery for multiple time periods, will be utilized to map and analyze changes in LULC using supervised classification techniques. These analyses will focus on key drivers of land use change, such as urban expansion, deforestation, agricultural intensification, and their role in altering watershed characteristics. To assess the hydrological implications of these changes, the Hydrologic Modeling System (HEC-HMS) will be used to simulate critical processes such as surface runoff, infiltration, and stream discharge to evaluate how LULC transitions influence flood patterns over time. Integrating historical flood data with HEC-HMS outputs will provide a comprehensive understanding of how LULC changes exacerbate or mitigate flood risks. The study aims to bridge gaps in knowledge regarding the interplay between land use dynamics and flood risks in arid and semi-arid regions like Hafr Al-Batin. The findings are expected to support the development of evidence-based land management strategies, sustainable watershed planning, and flood risk mitigation measures tailored to the region’s unique environmental and socio-economic context. Ultimately, this research seeks to contribute to disaster risk reduction efforts, helping to safeguard communities and infrastructure from the increasing threats posed by floods in the face of changing land use patterns.

How to cite: Al-Areeq, A. and Dirie, A.: Modeling the Impact of Land Use Dynamics on Flooding: A Case Study of Hafr Al-Batin, Saudi Arabia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4014, https://doi.org/10.5194/egusphere-egu25-4014, 2025.

Several studies demonstrated the importance of snowfall regime identification when retrieving snowfall rate from Passive Microwave (PMW) observations. Whether a precipitation algorithm is based on a-priori or training references, it is crucial to build complete and representative datasets to correctly detect and quantify snowfall from spaceborne sensors. Within the Global Precipitation Measurement (GPM) mission, the Goddard PROFiling (GPROF) algorithm snowfall retrieval is investigated. A combined CloudSat-GPM dataset is used to build a training dataset for an eXtreme Gradient Boost (XGB) model in which the GPM Microwave Imager (GMI) brightness temperatures are associated with a Cloud Profiling Radar (CPR) snowfall regime, classifying the observed scene into ‘dry’ (no precipitation detected), ‘shallow convective’, ‘deep stratiform’ or ‘other’ snowfall class. The Machine Learning (ML) approach is crucial to interpret strong but complex relationships between PMW signals within the atmosphere and snowfall regimes at the surface. The ML classifier training is performed using a CloudSat classifying technique, based on snowing profiles and cloud classification, and applied to GPROF. A couple of case studies will be presented to show the benefits of classifying the snowfall regime for PMW snowfall retrievals.

How to cite: Milani, L. and Petkovic, V.: Snowfall Regime Classification: Application of a Machine Learning Classifier to Passive Microwave Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4405, https://doi.org/10.5194/egusphere-egu25-4405, 2025.

Temperature and humidity are extremely important physical parameters of the atmosphere that can directly constrain atmospheric state variables, form the basis for data assimilation and are routine indicators for weather forecasting. Temperature and humidity parameters directly affect the interaction of solar shortwave radiation with longwave radiation in the earth-air system, which in turn affects the global balance of radiative energy. Therefore, accurate and rapid acquisition of temperature and humidity profiles in the atmosphere is of great significance for human production and life, climate and environmental monitoring and ecosystem assessment. Since the particles in the atmosphere, such as ice, clouds, rain and snow, have a certain attenuation effect on the surface microwave radiation, based on the high vertical resolution and high spectral resolution observation radiation in the test area obtained by the aircraft platform, the Fine Spectrum Microwave Atmospheric Sounder (FSMAS) can obtain different atmospheric information from different channels, so as to obtain more accurate information on the distribution of water vapour and its changes, and invert the atmospheric water vapour contours and precipitation information.

 

 

How to cite: He, J.: Detection and mining of water vapour and precipitation information based on microwave hyperspectral techniques, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4412, https://doi.org/10.5194/egusphere-egu25-4412, 2025.

Wet downbursts are commonly associated with heavy rain. Because the precipitation flux is proportional to the summed product of the mass and downward velocity of precipitating hydrometeors, the rain rate within downbursts can be significantly amplified due to the increased fall velocities. All existing radar methodologies for rainfall estimation assume that the fall velocity of raindrops is equal to their terminal velocity in still air. This results in a strong underestimation of precipitation in the presence of downbursts or microbursts.

Hail and graupel play an important role in generating downbursts via precipitation loading and negative buoyancy caused by melting of ice hydrometeors. These effects are quantified in the framework of our 1D cloud model with spectral bin microphysics that explicitly treats melting, sublimation, and evaporation for various size distributions of ice particles aloft and vertical thermodynamic profiles. The cloud model is coupled with an advanced polarimetric radar forward operator and generates vertical profiles of radar variables such as radar reflectivity Z, specific differential phase KDP, and specific attenuation A used in modern radar QPE methods.

KDP is the primary radar variable used for rain rate (R) estimation when rain is mixed with hail. However, the parameters of the power-law R(KDP) relation may vary depending on the predominant hail size. For example, storms producing a large amount of small hail (SPLASH storms) in high concentration are frequently characterized by anomalously high values of KDP. On the other hand, the effects of diabatic cooling that determine the strength of the downdraft (along with precipitation loading) are stronger for SPLASH storms.

The major points of this study will be illustrated by the results of model simulations and polarimetric radar observations of hail-bearing storms.

 

How to cite: Ryzhkov, A. and Carlin, J.: The impact of downburst and hail on the accuracy of polarimetric radar rainfall estimation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4467, https://doi.org/10.5194/egusphere-egu25-4467, 2025.

EGU25-4886 | Orals | AS1.18

The latest GPCP Daily and Monthly Products: Current Status, Assessments, and the Future Plans 

Ali Behrangi, George J. Huffman, Robert F. Adler, Yang Song, David T. Bolvin, Eric J. Nelkin, and Guojun Gu

The Global Precipitation Climatology Project (GPCP) is a popular combined satellite-gauge precipitation dataset in which the long-term CDR standards of consistency and homogeneity are emphasized. This presentation is composed of four major parts: (1) a brief overview of the latest GPCP Daily and Monthly products (V3.2) and satellite-gauge input data sets used in them; (2) comparison of the GPCP V3.2 products with the previous version of GPCP Daily (V1.3) and Monthly (V2.3) products and highlighting major changes; (3) assessment of the GPCP V3.2 products over the oceans using Passive Aquatic Listeners (PALs), over sea ice using snow depth data from a combination of ICESat-2 and Cryosat-2 observations plus ERA5 estimates, and over Antarctica using CloudSat; (4) insights from the latest GPM (V07) products as they are related to GPCP and the update of GPCP to GPCP V3.3. Several major changes occurred in GPCP V3.2, including: (1) moving from Monthly 2.5°x2.5° and Daily 1.0°x 1.0° spatial resolution in V2.3 to 0.5°x0.5° for both Monthly and Daily products; (2) calibrations to climatologies based on high-accuracy satellite missions, including TRMM, CloudSat, GPM, and GRACE; and (3) use of new precipitation retrieval and calibration methods. Compared to V2.3, GPCP V3.2 shows about a 6.5% increase in global oceanic and about a 4.5% increase in global (land and ocean) precipitation rates with some major changes over the ocean between 40°S and 60°S. Similar to V2.3, near-zero global precipitation trend is observed in V3.2.  However, regional trends, which are substantial, remain generally similar between V2.3 and V3.2. Evaluations over the oceans using PALs showed that GPCP V3.2 substantially outperforms GPCP V2.3 in representing rain occurrence and rain intensity at daily scale, likely due to the use of IMERG in the GPCP V3.2 Daily product. Our study suggests that GPCP V3.2 generally captures the snowfall accumulation pattern over sea ice, compared to that obtained from the combined ICESat-2 and Cryosat-2 observations, as well as that from ERA5. However, this set of products shows considerable differences in the amount of snowfall accumulation, with ERA5 often showing the highest values. We will end the presentation by briefly discussing our plans for further improvement of GPCP, including higher spatial and temporal resolution, lower latency, and the use of more-advanced gauge analysis and precipitation retrieval methods.

How to cite: Behrangi, A., Huffman, G. J., Adler, R. F., Song, Y., Bolvin, D. T., Nelkin, E. J., and Gu, G.: The latest GPCP Daily and Monthly Products: Current Status, Assessments, and the Future Plans, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4886, https://doi.org/10.5194/egusphere-egu25-4886, 2025.

EGU25-4982 | ECS | Posters on site | AS1.18

Ground validation of GPM-IMERG precipitation products across the Kingdom of Saudi Arabia  

Stavros-Andreas Logothetis, Ioannis Matsangouras, Mariya Ibrahim Alhmoud, Amani Ahmed Badrous, Muath Abdullatif Alkhalaf, Nojood Adel Aalismail, Ioannis Basiakos, and Ayman Mohammed Albar

Accurate precipitation estimation is vital for understanding hydrological processes, managing water resources, and mitigating climate-related risks. In arid regions such as the Kingdom of Saudi Arabia (KSA), where ground-based rainfall measurement networks are sparse, satellite-based precipitation products provide a valuable alternative. Since 2022, the National Center for Meteorology (NCM) has launched a cloud seeding program to increase rainfall across the KSA. Therefore, it is crucial to have a quality-assured precipitation dataset that covers the KSA both spatially and regionally, in order to monitor the precipitation patterns across the cloud seeding area of interest.

This study evaluates the performance of the latest Global Precipitation Measurement (GPM) Integrated Multi-satellite Retrievals for GPM (IMERG) Version 07 (V07) precipitation products over KSA. The accuracy of IMERG V07 precipitation products (Early, Late, and Final) was evaluated on multiple temporal scales (daily and monthly) by using reference precipitation measurements from NCM’s ground-based rainfall measurement networks during 2001−2023. The error analysis was conducted using key performance metrics, including mean bias error (MBE), root mean square error (RMSE), correlation coefficient (CC), and categorical statistics such as the probability of detection (POD), false alarm ratio (FAR), and frequency bias index (FBI).

The performance of IMERG products compared to the ground-based rain gauge measurements indicated an adequately high correlation among all three products (daily: 0.74−0.85, monthly: 0.85−0.97), with the final product presenting the best performance. The three IMERG products suffer from systematic overestimation of daily and monthly precipitation (20.4−34.1%) across KSA. The two indices of precipitation detection ability, POD and FAR, presented records around 93−95% and 45−48%, respectively. The findings highlight the strengths and limitations of IMERG V07 for capturing precipitation patterns in arid environments and provide valuable insights for improving its application in hydrological modeling, climate, and cloud seeding studies in KSA.

How to cite: Logothetis, S.-A., Matsangouras, I., Alhmoud, M. I., Badrous, A. A., Alkhalaf, M. A., Aalismail, N. A., Basiakos, I., and Albar, A. M.: Ground validation of GPM-IMERG precipitation products across the Kingdom of Saudi Arabia , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4982, https://doi.org/10.5194/egusphere-egu25-4982, 2025.

Due to the limitation of remote sensing observation, the research on the three-dimensional precipitation in Northwest China is insufficient. However, the launch of GPM provides convenience for the study of precipitation structures and types in Northwest China. In this work, the spatio-temporal distributions of convective and stratiform precipitation and corresponding thermal structures are analyzed during summer of 2014-2019 in Northwest China based on GPM observations, EAR5 reanalysis and IGRA2 datasets. The result shows that the stratiform precipitation is dominant in Northwest China and four representative sub-regions are divided to further discuss (Tianshan Mountain, Tarim Basin, Qilian Mountain and eastern part of Northwest China). The storm tops of convective precipitation are generally 2-3 km higher than those of stratiform precipitation, and the storm top reaches the maximum in the Tianshan Mountain (16 km) and the lowest in the Tarim Basin (10 km). Moreover, the maximum rain rate of convective precipitation below 4 km occurs in the Tianshan Mountain, while maximum rain rate of stratiform precipitation occurs in the eastern part of Northwest China. The maximum latent heating of both precipitation types occurs at 4-6 km. The peak frequency of convective precipitation mainly appears in the afternoon, whereas the diurnal variation of stratiform precipitation displays a bimodal peak (in the early morning and evening). Furthermore, the intensities of both precipitation types vary with the total column water vapor and follow an approximate quadratic function relationship. The precipitation conversion of convective precipitation and CAPE are obviously larger than those of stratiform precipitation. There is convergence in the lower troposphere and divergence in the upper troposphere, which is favorable to occurrence of precipitation (except for Tarim Basin). Additionally, the positive temperature and humidification are significant in the lower-middle troposphere during process of both precipitation types. This study aims to reveal the features of convective and stratiform precipitation from the perspective of GPM remote sensing observation and provide reference for numerical simulation in arid-semiarid regions.

How to cite: Wang, R.: Characteristics of different precipitation types and corresponding thermal structures in Northwest China in summer derived from GPM observation, ERA5 and IGRA2, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5351, https://doi.org/10.5194/egusphere-egu25-5351, 2025.

EGU25-6647 | Orals | AS1.18

Evaluating the sensitivity of GNSS-PRO to different microphysical assumptions 

Antía Paz, Ramon Padullés, and Estel Cardellach

The Polarimetric Radio Occultation (PRO) technique involves tracking signals emitted by navigation satellites (GPS, Galileo, Beidou…) from a Low Earth Orbit (LEO) satellite as it rises or sets behind the Earth’s limb. This method extends the capabilities of the standard Radio Occultation (RO) technique by employing two orthogonal linear polarizations—horizontal (H) and vertical (V)—thereby providing relevant information about atmospheric hydrometeors. Furthermore, the traditional RO products (vertical profiles of thermodynamic variables) are simultaneously measured, becoming the first technique to provide both type of observations.

This technique has been under testing since 2018 aboard the Spanish PAZ satellite, a mission that successfully demonstrated the GNSS-PRO concept. Moreover, since 2023, it has been implemented on three Spire global commercial CubeSats and one PlanetiQ satellite. The polarimetric capability of PRO enables to retrieve the observable called differential phase shift, defined as the difference between the phase delays associated with the horizontal and vertical polarizations. Intense precipitation events, characterized by non-spherically symmetric hydrometeors, exhibit a positive differential phase shift when these observations pass through such phenomena, showing sensitivity to microphysical properties related to these events.

The primary hypothesis, that PRO is sensitive to oblate raindrops, has already been validated. Unexpectedly, the technique also demonstrated sensitivity to frozen hydrometeors, further expanding its potential applications. The validation of PRO has been successfully achieved through comparisons with both two-dimensional datasets, such as IMERG-GPM products, and three-dimensional datasets, including observations from NEXRAD polarimetric radars.

Current analyses focus on evaluating the sensitivity of PRO to various microphysical parameterizations obtained from the Weather Research and Forecasting (WRF) model. Additionally, its sensitivity to specific particle habits is being examined using the Atmospheric Radiative Transfer Simulator (ARTS) database. The study is centered on Atmospheric Rivers (AR) to investigate how variations in microphysical parameterizations influence the ability of PRO to detect and characterize hydrometeors. Preliminary results indicate that some specific parameterizations and particle habits better compare to PRO actual observations. These findings aim to enhance our understanding of the processes associated with extreme weather systems and advance the application of PRO in atmospheric science.

How to cite: Paz, A., Padullés, R., and Cardellach, E.: Evaluating the sensitivity of GNSS-PRO to different microphysical assumptions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6647, https://doi.org/10.5194/egusphere-egu25-6647, 2025.

EGU25-6682 | ECS | Posters on site | AS1.18

Enhancing IR-Based Satellite Precipitation Estimates Using Machine Learning. 

Matthieu Meignin, Nicolas Viltard, Laurent Barthès, and Cécile Mallet

Abstract: Accurate precipitation estimation is essential for various applications, including hydrological modelling, climate studies, and disaster management. Satellite-derived precipitation estimates are particularly valuable in regions with limited ground-based measurements, such as oceans and remote areas. However, challenges persist in improving the accuracy of these estimates, especially when relying solely on infrared (IR) satellite data. While microwave (MW) data has traditionally been favoured for precipitation estimation due to its strong correlation with precipitation[1], infrared (IR) data has become increasingly important, offering superior spatio-temporal coverage and resolution, essential for global observations.

This study explores the application of machine learning techniques to enhance IR-based precipitation estimates. Specifically, we employ U-Net, a convolutional neural network, known for its ability to capture spatial dependencies and local patterns in data, making it ideal for improving the spatial resolution and accuracy of precipitation estimates using only IR channels[2]. We leverage IR data from the MSG satellite to develop a model that enhances precipitation extraction from IR imagery alone

To achieve this, we utilise a database of IR brightness temperatures from three distinct IR channels (87, 108, and 120 μm). These channels capture a broad spectrum of thermal emissions, from cloud tops to deeper atmospheric layers, enabling the model to estimate precipitation rates more effectively[3]. These data are co-located with a radar mosaic from Météo-France, gauge-corrected for improved accuracy, which serves as a reference to evaluate the performance of the U-Net model and ensure alignment with actual measurements.

Our dataset spans 13 years, providing a diverse range of scenarios, including varying weather patterns and seasonal fluctuations. Initial results indicate that the U-Net model enhances precipitation estimation by accurately capturing spatial patterns, even with the inherent limitations of IR channels. In evaluating this approach, we consider a range of metrics specifically designed to address the unique characteristics of precipitation, such as intensity and spatial distribution. This targeted evaluation ensures a comprehensive assessment of the model's ability to account for the variability and intensity of precipitation, key challenges in accurate satellite-based Precipitation estimation.

These promising results highlight the potential of deep learning techniques to improve satellite-derived precipitation estimates from IR data. Looking ahead, we will explore the integration of microwave and IR satellite data to further refine the consistency and accuracy of these estimates. Additionally, we plan to investigate cutting-edge deep learning architectures tailored to this specific use case, aiming to optimise model performance and address the complexities of satellite-based precipitation retrieval.

References:

[1] Viltard, N., Sambath, V., Lepetit, P., Martini, A., Barthes, L., & Mallet, C. (2023). Evaluation of DRAIN, a deep-learning approach to rain retrieval from GPM passive microwave radiometer. IEEE Transactions on Geoscience and Remote Sensing. https://doi.org/10.1109/TGRS.2023.3293932

[2] Wang, C., Tang, G., Xiong, W., Ma, Z., & Zhu, S. (2021). Infrared precipitation estimation using convolutional neural network for FengYun satellites. Journal of Hydrology, 603(C), 127113. https://doi.org/10.1016/j.jhydrol.2021.127113

[3]Sadeghi, Mojtaba, Nguyen, Phu, Hsu, Kuolin, & Sorooshian, Soroosh (2020). Improving near real-time precipitation estimation using a U-Net convolutional neural network and geographical information. Environmental Modelling and Software, 134(C). https://doi.org/10.1016/j.envsoft.2020.104856.

How to cite: Meignin, M., Viltard, N., Barthès, L., and Mallet, C.: Enhancing IR-Based Satellite Precipitation Estimates Using Machine Learning., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6682, https://doi.org/10.5194/egusphere-egu25-6682, 2025.

The Global Precipitation Measurement Mission (GPM) is nearing 10 years in operation, building a legacy of unprecedented advances in understanding the global distribution and characteristics of rain and snow. The GPM core satellite, with coincident active dual-frequency radar and passive microwave radiometer ranging from 10-183 GHz, acts as the cornerstone of this mission, providing a calibration source for radiometers of opportunity and allowing for a consistent global precipitation product every 30 minutes. The resulting 10-year dataset offers unique applications for optimization of global passive microwave retrievals, using the coincident radar as a local comparison. Considering precipitation mapping in the 2030 timeframe, a key future issue will be the character of the constellation members.  To date, smaller radiometers such as TROPICS and the upcoming AOS mission have been limited to the higher frequency microwave channels.  While these PMW channels present excellent opportunities for understanding clouds, ice, and snow, the relationships to precipitation are more indirect than for lower-frequency channels, and therefore more uncertain, which will have an effect on global precipitation mapping as well as applications value. In this work we quantify how lower-frequency window channels (particularly 19, 37, and 90 GHz) provide key information that underpins accurate retrievals across a range of global climatic zones, using the GPM core satellite. A Bayesian retrieval scheme is employed and results computed using variable channel selection. These are then compared as a function of surface type, meteorology, intensity, and other environmental parameters, as well as for specific events such as a tropical storm. This work aims to provide information to aid in planning for the future constellation in a way that emphasizes climate study and applications continuity.

How to cite: Ringerud, S. and Kidd, C.: Optimizing Channel Selection for Passive Microwave Precipitation Measurement: A GPM Study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6684, https://doi.org/10.5194/egusphere-egu25-6684, 2025.

EGU25-7237 | Orals | AS1.18

Plans for IMERG V08 and Future Perspectives for Global Satellite Precipitation 

George Huffman, David Bolvin, Robert Joyce, Eric Nelkin, and Jackson Tan

The Integrated Multi-satellitE Retrievals for GPM (IMERG) dataset is computed by the U.S. Science Team of the NASA-JAXA Global Precipitation Measurement (GPM) mission.  It provides global satellite precipitation estimates for a wide range of scientific research and societal applications.  Using a constellation of low-Earth orbit passive microwave and geosynchronous-orbit infrared satellites of opportunity provided by domestic and international partners, IMERG supplies precipitation estimates at high spatial and temporal resolution globally (0.1° every half hour),  Three separate Runs, with increasing latencies, are generated to fit the diverse needs of the scientific and applications communities.  

The presentation focuses on the future of IMERG for the upcoming V08 and thereafter.  This includes issues remaining from V07 development, new issues identified in analysis of the V07 time series, calibration shifts due to the GPM Core Observatory (GPM-CO) orbit boost (and in retrospect the Tropical Rainfall Measuring Mission [TRMM] orbit boost and the TRMM Precipitation Radar’s A/B electronics switch), the advent of SmallSats capable of observing precipitation, the advent of machine learning algorithms, and priorities stemming from the approaching end of the GPM-CO satellite (circa 2032).  The complete retrospective processing that will accompany the introduction of Version 08 is planned as the last upgrade before the end of mission.

The goal of this work is to continue the progress that the GPM mission and the IMERG products have realized over the past decade, especially over regions with limited ground observations. We emphasize our continuing goal of providing the scientific and applications communities with a long record of reliable high-resolution precipitation observations, and invite discussion on the next generation of sustained observations and algorithms for global satellite precipitation.

How to cite: Huffman, G., Bolvin, D., Joyce, R., Nelkin, E., and Tan, J.: Plans for IMERG V08 and Future Perspectives for Global Satellite Precipitation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7237, https://doi.org/10.5194/egusphere-egu25-7237, 2025.

EGU25-7426 | Posters on site | AS1.18

Extending and enhancing the satellite precipitation data record from passive microwave sensors 

Chris Kidd, Rachael Kroodsma, Veljko Petkovic, and Linda Bogerd

Passive microwave (PMW) observations form the backbone of global precipitation measurements due to their relative directness of precipitation retrievals compared to those in the visible/infrared. The NASA/JAXA Tropical Rainfall Measuring Mission (TRMM) and Global Precipitation Measurement (GPM) missions have been central to advancing satellite precipitation measurements since TRMM was launched in 1997. Prior to TRMM, PMW estimates were derived primarily using observations from the US Defense Meteorological Satellite Program (DMSP) Special Sensor Microwave/Imager (SSM/I) sensors, first launched in 1987. The PMW data records preceding the SSM/I era are extremely important for providing long term precipitation measurements. Data from earlier missions could potentially extend the satellite precipitation data record back to 1973 and is therefore highly desirable, although these precipitation-capable sensors have not been fully exploited. Furthermore, while current PMW precipitation retrievals utilize a range of observations from both cross-track ‘sounders’ and conically scanning ‘imaging’ sensors, not all the available observations from these sensors are presently exploited.

This poster outlines the fundamental requirements of improving our measurements of global precipitation through exploiting and enhancing current and past precipitation-capable missions and their data using conventional and new methodologies. In particular, the different channel availability is shown to significantly affect the ability to provide accurate precipitation retrievals which impacts the generation of a consistent climate precipitation record. Extending the precipitation data record and fully exploiting the available observations has the potential to improve our knowledge of the Earth System and its’ water cycle, provide a greater understanding of our changing global climate, and gain better insights into the naturally occurring and human-induced changes.

How to cite: Kidd, C., Kroodsma, R., Petkovic, V., and Bogerd, L.: Extending and enhancing the satellite precipitation data record from passive microwave sensors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7426, https://doi.org/10.5194/egusphere-egu25-7426, 2025.

EGU25-7635 | ECS | Orals | AS1.18

Development of EarthCARE - GPM coincidence dataset with combination of spaceborne cloud and precipitation radars 

Shunsuke Aoki, Takuji Kubota, and F. Joseph Turk

The Global Precipitation Measurement (GPM) Dual-Frequency Precipitation Radar (DPR) (Ku- and Ka-band) provides vertically resolved information on rain and ice water under moderate to heavy precipitation conditions across the tropics and mid-latitudes (Hou et al. 2014, Skofronick-Jackson et al. 2017). Owing to the unique asynchronous orbit of the GPM Core Observatory with the DPR and the GPM Microwave Imager (GMI), its orbital ground tracks intersect with those of many other sun-synchronous satellites. The CloudSat - GPM coincidence dataset (CSATGPM; Turk et al. 2021), focusing on intersections with the W-band cloud radar onboard CloudSat, which excels at observing clouds and light precipitation, offers "pseudo three-frequency" radar profiles of near-coincident observations. In addition, simultaneous observations by CloudSat and the Tropical Rainfall Measuring Mission (TRMM; Kummerow et al. 1998) satellite, the predecessor of GPM, are also available (CSATTRMM; Turk et al. 2021), which includes a larger number of cases compared to CSATGPM, as it covers the period before CloudSat transitioned to day-time only operation in 2011. These datasets have been utilized for many scientific purposes, such as studies of cold-season precipitation, ice microphysics, and light rainfall.

The Earth Clouds, Aerosols and Radiation Explorer (EarthCARE) satellite (Illingworth et al., 2015; Wehr et al., 2023), launched in May 2024, is equipped with four sensors employing different observation methods: radar, lidar, imager, and radiometer. In particular, the Cloud-Profiling Radar (CPR), developed by the Japan Aerospace Exploration Agency (JAXA) and the National Institute of Information and Communications Technology (NICT), is the first spaceborne W-band radar with Doppler capability. It continues the cloud and precipitation observations performed by the CloudSat while introducing the novel measurements of vertical cloud motion from space. Building on the CSATGPM dataset, we are constructing a coincident observation dataset for the EarthCARE era.

From August to December 2024, the two satellites recorded several hundred coincident observation events per month, with approximately one-third of these events detecting precipitation on both satellites. An examination of the vertical profiles of radar reflectivity revealed that while the DPR detected large raindrops and snow particles in advanced stages of growth, the CPR captured detailed features within clouds at higher altitudes. In stratiform precipitation cases, Doppler velocity observations from the CPR showed slower downward motion at altitudes above the bright band detected by the DPR, and faster downward motion at lower altitudes. Furthermore, in addition to using DFR from three-frequency observations during the CloudSat era to classify solid precipitation particles, the incorporation of Doppler velocity as a new constraint suggests the potential for more advanced microphysical analysis of ice particles.

The combination of active observations from the W-band radar and 13-channel (10–183 GHz) GMI is also useful for algorithm development and evaluation, sensitivity studies of snow and light rain, cloud process studies, and radiative transfer simulations. In this presentation, we will also introduce preliminary results from coincident observations of the EarthCARE/CPR and the GMI radiometer.

How to cite: Aoki, S., Kubota, T., and Turk, F. J.: Development of EarthCARE - GPM coincidence dataset with combination of spaceborne cloud and precipitation radars, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7635, https://doi.org/10.5194/egusphere-egu25-7635, 2025.

EGU25-7962 | Posters on site | AS1.18

Temporal Trends and Climate Variability Impacts on Precipitation over Saudi Arabia 

Sara Vanessa C. R. Da Silva, Stavros-Andreas Logothesis, Ioannis Matsangouras, and Ayman Mohammed A-Albar

Saudi Arabia, classified under Koppen’s climate classification as an arid to semi-arid region, faces persistent water scarcity conditions exacerbated by desertification that further diminish water availability. In response, a Regional Cloud Seeding Program has been implemented to enhance precipitation over the southwestern and central regions since 2022.

This study investigates the spatiotemporal distribution of precipitation and rainy days focusing on annual, monthly and seasonal variability using a comprehensive statistical framework. Key analyses include long term trends, five years moving averages, change point detection and sub long term trends evaluations using the non-parametric Mann Kendal test and Sen’s slope detection method. Furthermore, the Tau statistics test was used to assess the significance of trends. The influence of major climatic variability phenomena such as ENSO, IOD and PDO was examined through seasonal Pearson, Spearman and Tau correlation coefficients.

The findings reveal strong dependence (> 0.70) between precipitation and rainy days across all seasons and regions. Seasonal and regional correlations analysis identified weak to moderate (<0.60) dependence correlation between precipitation, rainy days and climate variability, ENSO, IOD and PDO, but significant linear, nonlinear and especially monotonic correlations. Moving correlation coefficients analysis shows that correlation coefficients are not static in time but rather dynamic. Moving correlation coefficients show periods of weak correlation and others of moderate and significant linear, nonlinear and monotonic correlation between precipitation and rainy days’ number to each one of the climate variability phenomena. The findings of this study provide valuable insights into precipitation variability and climatic influences, which are essential for guiding effective, data-driven water resource management, optimizing rainfall enhancement programs, and mitigating the risks associated with water scarcity in Saudi Arabia.

Keywords= Arid Climate, Saudi Arabia, Precipitation, Rainy Days, Cloud Seeding, Climate Variability, ENSO, IOD, PDO

How to cite: C. R. Da Silva, S. V., Logothesis, S.-A., Matsangouras, I., and A-Albar, A. M.: Temporal Trends and Climate Variability Impacts on Precipitation over Saudi Arabia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7962, https://doi.org/10.5194/egusphere-egu25-7962, 2025.

EGU25-8738 | Posters on site | AS1.18

Regional frequency analysis of maximum 2-day precipitation in Slovakia 

Pavel Fasko, Ladislav Markovič, and Milan Onderka

Ongoing climate change continues to accelerate, significantly altering climatic conditions across the globe. These changes are evident not only in the rising mean global temperature but also in the increasing frequency and intensity of extreme weather events (IPCC, 2021). Extreme precipitation events, characterized by high multi-day precipitation totals, pose a severe risk to infrastructure, public safety, and property, even in the absence of climate change. This study presents a comprehensive seasonal regional frequency analysis (RFA) of maximum 2-day precipitation totals (Rx2D) in Slovakia using the L-moment approach (Hosking and Wallis, 1997). We analyzed 70 years (1951–2020) of precipitation data from 419 stations. The stations were grouped into homogeneous regions using a multi-regression approach and distance matrices, enabling the development of regional frequency curves. The L-moments ratio diagrams, 𝑍𝐷𝑖𝑠𝑡 measure, and Anderson-Darling goodness-of-fit tests were applied to identify the most suitable theoretical extreme-value distributions. The analysis identified nine distinct regions, with the generalized extreme value (GEV) distribution providing the best fit for Rx2D in eight of the nine clusters. The resulting regional frequency curves offer reliable estimates of extreme 2-day precipitation return values at any location within the study area. These findings are crucial for improving flood risk management, guiding infrastructure design, and supporting climate adaptation planning.

How to cite: Fasko, P., Markovič, L., and Onderka, M.: Regional frequency analysis of maximum 2-day precipitation in Slovakia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8738, https://doi.org/10.5194/egusphere-egu25-8738, 2025.

In this study, we produced surface precipitation data at a high spatial resolution of 0.1° by integrating observations from two spaceborne radars, TRMM PR and GPM DPR KuPR, spanning a 25-year period. This dataset allowed us to analyze the seasonal variation in diurnal peaks, enhancing our understanding of spatiotemporal precipitation patterns and their detectability. The precipitation data were classified based on the horizontal scale for the individual precipitation systems, represented by the area-equivalent diameter of consecutive precipitation regions. Certain grid points in the equatorial and mid-latitude zones lacked sufficient long-term, time-resolved samples due to limited satellite overpasses. For example, in mid-latitude regions such as Europe, observations by DPR alone provided fewer than 10 passes under the current conditions for averaging time.
To address these limitations, we applied a running average technique and imputed missing values to minimize outlier impacts. Seasonal changes in the timing of maximum precipitation were then categorized into distinct clusters, revealing key spatiotemporal patterns. On the Tibetan Plateau, small-scale precipitation systems predominantly generate early afternoon peaks throughout the year, while in winter, morning rain frequently occurs in certain valleys. In the southern foothills of the Himalayas, precipitation peaks in the morning, whereas evening showers are observed in the southernmost regions during summer. In the southwestern part of Japan, which is heavily influenced by the ocean, large-scale precipitation dominates during the rainy season, with morning rainfall prevailing, while midsummer shows a shift toward afternoon peaks. Additionally, medium-scale precipitation systems tend to follow small-scale systems by a few hours, while large-scale systems exceeding 100 km in diameter exhibit distinct timing patterns. 
These findings underscore the diverse precipitation regimes shaped by geographical features and prevailing winds, highlighting the need to assess the value and challenges of leveraging high-resolution precipitation climate datasets.

How to cite: Hirose, M. and Mantas, V.: Detecting seasonal differences in the variations in diurnal precipitation using spaceborne Ku-band radars, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9231, https://doi.org/10.5194/egusphere-egu25-9231, 2025.

EGU25-9513 | ECS | Posters on site | AS1.18

Evaluation of Satellite-Based Precipitation Products in the 2023 Summer Extreme Precipitation Events Over North China 

Haixia Liang, Zhi Li, Sheng Chen, Xiaoyu Li, Yanping Li, and Chunxia Wei

In the summer of 2023, North China was hit by an exceptionally intense precipitation storm caused by Typhoons Doksuri and Khanun, resulting in significant secondary disasters and underscoring the critical need for accurate rainfall forecasting. Satellite-based quantitative precipitation estimation (QPE) products, such as Integrated Multi-Satellite Retrievals for GPM (IMERG) and Global Satellite Mapping of Precipitation (GSMaP) from the Global Precipitation Measurement (GPM) Mission, show great merits for enhancing forecasts. This study uses a dense rain gauge network as a benchmark to evaluate the performance of the latest version 7B IMERG and version 8 GSMaP satellite-based QPE products during the 2023 summer extreme precipitation event in North China. The satellite-based QPE products include four satellite-only products, namely IMERG early run (IMERG_ER), IMERG late run (IMERG_LR), GSMaP near-real-time (GSMaP_NRT), and GSMaP microwave-infrared reanalyzed (GSMaP_MVK), as well as two gauge-corrected products IMERG final run (IMERG_FR) and GSMaP gauge-adjusted (GSMaP_Gauge). The results show that the satellite-based QPE products, particularly IMERG_LR and GSMaP_MVK, show good performance in capturing the spatial distribution and overall rainfall amounts during the extreme precipitation event. However, they have significant under-detect high-intensity precipitation events in this region. The IMERG products generally outperform the GSMaP products, especially in terms of temporal rainfall measurement, but all products tend to underestimate rainfall. At high rainfall rates, while the detection ability is high, the false alarm ratios are also significantly elevated for all satellite-based QPE products. These findings highlight the need for further improvement of satellite-based QPE products for more accurate and reliable rainfall estimation.

How to cite: Liang, H., Li, Z., Chen, S., Li, X., Li, Y., and Wei, C.: Evaluation of Satellite-Based Precipitation Products in the 2023 Summer Extreme Precipitation Events Over North China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9513, https://doi.org/10.5194/egusphere-egu25-9513, 2025.

EGU25-9781 | ECS | Posters on site | AS1.18

Improving Quantitative Precipitation Estimation with Solid-State X-Band Radar 

Nicolás Andrés Chaves González, Alessandro Ceppi, Carlo De Michele, Giovanni Ravazzani, and Orietta Cazzuli

Radar-based measurements are crucial for accurately estimating precipitation and capturing the spatial variability of rainfall, which enhances both precipitation forecasting and hydrological modeling. This study focuses on quantitative precipitation estimation (QPE) using radar data in the Lombardy Region of northern Italy, examining the limitations of radar measurements and identifying optimal configurations. Specifically, data from two newly installed X-band radars with solid-state transmitters, operated by the Regional Environmental Protection Agency (ARPA Lombardia), were analyzed.

The goal of this research is to determine radar settings that maximize QPE performance at an operational level and explore post-processing methods to address radar limitations, particularly during extreme precipitation events that could lead to flooding. The methodology is twofold: first, to identify radar configurations that accurately correlate rainfall intensity with radar data, and second, to address radar challenges during severe events, focusing on attenuation correction, signal extinction, and the integration of third-party data sources.

Extreme and non-extreme precipitation events affecting the Milan hydraulic node were analyzed, highlighting opportunities to enhance the radar network through post-processing techniques that could aid future hydrological modeling. The study compares different QPE methods, including basic Z-R relationships and Z-R matching techniques based on previous research.

This work provides a foundation for optimizing operational QPE and proposes strategies for overcoming radar limitations during extreme weather events. Additionally, it supports future improvements, such as integrating real-time rain gauge data to enhance flood forecasting accuracy.

How to cite: Chaves González, N. A., Ceppi, A., De Michele, C., Ravazzani, G., and Cazzuli, O.: Improving Quantitative Precipitation Estimation with Solid-State X-Band Radar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9781, https://doi.org/10.5194/egusphere-egu25-9781, 2025.

EGU25-10031 | ECS | Posters on site | AS1.18

Intercomparison of gauge based, reanalysis and satellite gridded precipitation datasets in High Mountain Asia: insights from observations and runoff data. 

Alessia Spezza, Guglielmina Adele Diolaiuti, Davide Fugazza, Veronica Manara, and Maurizio Maugeri

The Tibetan Plateau and the adjacent mountain ranges are known as the "Asian Water Tower" (AWT) because they hold the third largest frozen water reserve in the world after the polar regions. This region plays a vital role in supplying water to nearly 2 billion people through rivers like the Indus, Ganges, Brahmaputra, Yangtze, and Yellow River. 
Accurate precipitation data are essential for understanding hydrological processes in high mountain basins. However, in many mountainous areas, precipitation gauges are either sparse or absent due to the challenging environmental conditions. Moreover, the available precipitation gauges are often located in valleys and they are not adequate to represent the diverse topography of the territory. This underlines a significant gap in the existing precipitation datasets, since precipitation at high elevations is likely considerably underestimated.
In this study, we aim to address these challenges by analyzing an extensive area of High Mountain Asia (70°-100°E for longitude and 25°-40° N for latitude). Specifically, we examined two reanalysis datasets (ERA5 and HAR), two gauge-based datasets (GPCC and Aphrodite), and one satellite-derived dataset (PERSIANN) to evaluate their performance in capturing precipitation patterns. 
At first, we compared the different datasets over the common period (1983-2007) evaluating their ability to reproduce the precipitation spatial distribution both at annual and seasonal level.
Then, due to the discrepancies in precipitation values over the area, particularly influenced by the complex orography, we decided to compare the datasets with the observational data available from the Copernicus Data Store (Global Land Surface Atmospheric Variables dataset, 1755–2020) and the runoff data provided by the GRDC (Global Runoff Data Centre) dataset as a reference.
When comparing gauge-based datasets with the observational data, there is consistency, whereas the other datasets tend to exhibit higher precipitation especially in areas with greater topographic complexity.
To compare precipitation values with the measured river flow, the total evaporation from the ERA5-Land dataset was taken into account to improve the estimates. The results indicate that reanalysis datasets are the most effective in simulating the hydrological balance while the gauge-based and the satellite datasets significantly underestimate precipitation.

How to cite: Spezza, A., Diolaiuti, G. A., Fugazza, D., Manara, V., and Maugeri, M.: Intercomparison of gauge based, reanalysis and satellite gridded precipitation datasets in High Mountain Asia: insights from observations and runoff data., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10031, https://doi.org/10.5194/egusphere-egu25-10031, 2025.

EGU25-10789 | Posters on site | AS1.18

Validation of satellite estimates of precipitation over Italy 

Tommaso Caloiero, Francesco Chiaravalloti, Roberto Coscarelli, and Gaetano Pellicone

Precipitation is a critical variable for hydrological studies and water resource management. However, while rain gauges generally produce the most reliable observational results, their often-sparse distribution causes them not to be fully representative of some regions, especially large ones. In fact, in regions with a complex orography and scarce human settlements, rain gauges are usually not sufficient to provide data to resolve precipitation processes in simulation studies. Satellite retrievals have thus been used to create regular data grids, in order to fill in on lacking observations and to address the scarcity of stations in ungauged regions.

This study aimed to evaluate the skills of five satellite precipitation products in reproducing precipitation across three temporal scales (daily, seasonal, and annual) over Italy. These are the Integrated Multi-satellitE Retrievals for GPM (IMERG) Final Run, the PERSIANN Dynamic Infrared–Rain Rate (PDIR-Now), the EUMETSAT Satellite Application Facility on Support to Operational Hydrology and Water Management (HSAF H05), and the Soil Moisture to Rain (SM2Rain). To this purpose, precipitation data for the period 2000-2021 have been extracted from the National System for collection and processing of climate data (SCIA) gridded observational rainfall dataset provided by the Italian Environmental Protection Agency (ISPRA). After resampling all the different datasets to a common grid with spatial resolutions of 0.1°, the performance of the satellite products was then assessed using two distinct sets of statistical metrics. In particular, the accuracy of satellite products at a daily temporal resolution has been evaluated using performance metrics such as the Probability of Detection (POD), the False Alarm Ratio (FAR), the Success Ratio (1-FAR), the BIAS, and the Critical Success Index (CSI). Conversely, at annual and seasonal scales, the Root Mean Square Error (RMSE), the coefficient of determination (R²), and the standard deviation (SD), have been applied.

Results showed that GPM-IMERG Final Run satellite data performed better at a daily resolution both in capability (POD) and reliability (SR), except during the summer season, when the HSAF H05 demonstrates a better overall performance. Conversely, the PDIR-Now tends to overestimate rainfall events. As regards the annual and seasonal time scales,  HSAF H05, GPM-IMERG, and SM2Rain demonstrate strong correlations with observed data at annual scale, with high R2 values (≥0.88) and generally low errors (SD and RMSE).

The procedure applied in this work is general and easily applicable where gridded data are available and might help scientists and policy makers to select among available datasets those best suited for further applications, even in areas with a complex orography and an inadequate amount of representative stations.

This work was funded by the Next Generation EU - Italian NRRP, Mission 4, Component 2, Investment 1.5, call for the creation and strengthening of Innovation Ecosystems', building 'Territorial R&D Leaders' (Directorial Decree n. 2021/3277) - project Tech4You – Technologies for climate change adaptation and quality of life improvement, n. ECS0000009. This work reflects only the authors’ views and opinions, neither the Ministry for University and Research nor the European Commission can be considered responsible for them.

How to cite: Caloiero, T., Chiaravalloti, F., Coscarelli, R., and Pellicone, G.: Validation of satellite estimates of precipitation over Italy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10789, https://doi.org/10.5194/egusphere-egu25-10789, 2025.

In Dual-frequency Precipitation Radar (DPR), the observed radar reflectivity factor cannot be used near the ground surface because of the main lobe clutter. Therefore, the standard algorithm V07 estimates the precipitation rate in the main-lobe clutter region, assuming that the attenuation-corrected radar reflectivity factor does not change in the beam direction. On the other hand, Hirose et al. (2021) produced a database of vertical profiles of precipitation rate (DB21) using observations near the nadir, where the effect of main lobe clutter is relatively small, and applied it to observations outside the nadir to estimate precipitation rate at ground surface level. This estimation method extrapolates precipitation rate profiles estimated by the standard algorithm, and its consistency with other estimates, such as path-integrated attenuation, is not guaranteed.
In this study, we improved the precipitation rate estimation method in the standard algorithm using DB21 and its updated database (DB24). When the standard algorithm estimates using different parameters, the precipitation rate profile in the main lobe clutter region changes in the beam direction according to DB21 or DB24. The precipitation rate estimates obtained in this manner were consistent with those of the other estimates.
Experiments conducted for all orbits in June 2018 showed that the surface altitude precipitation rate of the dual-frequency algorithm increased by 6.6% (10.5%) compared with V07 when using DB21 (DB24). For DB24, the database classification by precipitation rate at the reference altitude (2.25 km or 3.25 km) was added. In addition, the classification of the database by precipitation rate gradient between the reference altitude and 0.5 km higher was subdivided. As a result, the downward increase in precipitation rate, especially in heavy precipitation, can be more easily expressed. The estimated precipitation rate at the clutter-free bottom was 1.2% lower for DB24 than for V07. This is due to the need to compensate for the general increase in precipitation rate in the main lobe clutter region, because the conditions of the surface reference technique remain the same.

How to cite: Seto, S. and Hirose, M.: Improved Precipitation Rate Profile Estimation Method for the Main-lobe Clutter Region in GPM/DPR, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10838, https://doi.org/10.5194/egusphere-egu25-10838, 2025.

EGU25-11059 | ECS | Posters on site | AS1.18

A Critical Assessment of Precipitation Datasets Over Italy 

Benedetta Moccia, Luca Buonora, Claudia Bertini, Elena Ridolfi, Fabio Russo, and Francesco Napolitano

Italy, because of its complex orography and geography, is prone to extreme precipitation events, which may result in enormous damages and losses. It is therefore fundamental to monitor precipitation across the Italian territory and across time. Even though Italy has been a pioneer in developing meteorological observations, its rain gauge network – as those of many other countries in the World –is characterised by an uneven density and with records not always freely available online. Satellite and reanalysis precipitation datasets have the potential to overcome some of the issues characterising ground-based monitoring networks, but their performances vary widely across climate, topography and time scale. In this work we assess the performance of six remote sensing and reanalysis datasets (ERA5-Land, CERRA-Land, CHIRPS, CMORPH, IMERG, PERSIANN-CCS-CDR) in observing precipitation across the entire Italian peninsula, using the ground-based national records of the SCIA dataset as ground-truth. For our analysis, we compute common continuous and categorical metrics across different time scales (daily, monthly, annual). We then provide the best performing dataset at different spatial scales (i.e. watershed, administrative province, administrative region, nation-wide, Köppen-Geiger climate zone), providing useful insights for hydrological studies of various purposes. Our results show that at the national level, the two reanalysis datasets (CERRA-Land and ERA5-Land) outperform the satellite-based observations, having overall higher and consistent performances across the different climatic zones. Among the satellite datasets analysed, the most-performing is IMERG, while the least-performing in all the Italian climatic regions are CMORPH and PERSIANN-CCS-CDR, with the worst performances in the alpine and cold semi-arid climates, respectively.

How to cite: Moccia, B., Buonora, L., Bertini, C., Ridolfi, E., Russo, F., and Napolitano, F.: A Critical Assessment of Precipitation Datasets Over Italy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11059, https://doi.org/10.5194/egusphere-egu25-11059, 2025.

EGU25-11151 | Posters on site | AS1.18

Preliminary results of the assimilation of GNSS delays along slant paths 

Rosa Claudia Torcasio, Claudio Transerici, Eugenio Realini, Mattia Crespi, and Stefano Federico

A reliable Numerical Weather Prediction (NWP) is useful to guide responsive actions for mitigating the impact of severe weather. The accuracy of the forecast given by NWP models depends also on the knowledge of the initial conditions, which can be improved by data assimilation.

In the last three decades, there has been a significant advancement of GNSS technology, which has broadened its range of applications, especially within the realm of the meteorology. GNSS-ZTD has proven to be an important source of water vapor data, which can be used to improve the weather forecast, in general, including intense precipitation events (Torcasio et al., 2023).

However, a relevant part of the information related to water vapor distribution remains still unexploited. In fact, routinely zenith tropospheric delays (ZTDs) are estimated off-line generally on an hourly basis at each GNSS site only, introducing the hypothesis of azimuthal isotropy of the troposphere.

The objective of the NEW-ARGENT (Improvement of NumErical Weather prediction through data Assimilation of Real-time GNSS-Estimated Non-isotropic Troposphere) project, funded by the Ministry of University and Research, is to assimilate the GNSS delay along slant path, to recover the local directional anisotropy. A possible way to recover, at least, part of the directional information given by GNSS observations, is through the assimilation of the gradients in the East and North directions (Zus et al., 2023). While for GNSS-ZTD data assimilation the WRFDA offers a specific tool, gradients assimilation has been recently added in a version of the WRFDA distributed by the link https://doi.org/10.5281/zenodo.10276429 and presented in the paper (Thundathil et al., 2024). 

In this work we show the impact of GNSS gradient data assimilation in the WRF model for the month of September 2022 when several convective and intense storms occurred over Italy. Specifically, we compared the precipitation forecast at the short-range in four different experiments set-up: CTRL (control), without GNSS data assimilation, GNSS-ZTD, with the assimilation of GNSS zenith delay, GNSS-GRA, in which the gradients are assimilated, and GNSS-ZTD-GRA, in which both the gradients and the zenith total delay are assimilated. Simulations, lasting 12 each, are performed in a Very Short-term Forecast (VSF) approach. The first six hours are for spin-up and data assimilation (one analysis per hour), while the last six hours are considered as forecast phase. 

Results show that the assimilation of the gradients, both alone and with the GNSS-ZTD, is beneficial for the improvement of precipitation forecast of convective events over Italy.

 

References

Thundathil, R. et al., 2024, https://doi.org/10.5194/gmd-17-3599-2024

Torcasio, R. C. et al., 2023, https://doi.org/10.5194/nhess-23-3319-2023

Zus, F. et al., 2023, https://doi.org/10.3390/rs15215114 

 

Acknowledgments

This work has been realized in the project PRIN-PNRR NEW-ARGENT (Improvement of NumErical Weather prediction through data Assimilation of Real-time GNSS-Estimated Non-isotropic Troposphere) funded by the Ministry of University and Research contract number: P20228LMA2.

How to cite: Torcasio, R. C., Transerici, C., Realini, E., Crespi, M., and Federico, S.: Preliminary results of the assimilation of GNSS delays along slant paths, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11151, https://doi.org/10.5194/egusphere-egu25-11151, 2025.

EGU25-11337 | Posters on site | AS1.18

Regional Cloud Seeding and Rainfall Enhancement in Saudi Arabia: Preliminary Observations and Insights from 2022 Using EUMETSAT CMSAF GIRAFEv1 CDR 

Ioannis Matsangouras, Stavros Andreas Logothetis, and Ayman Mohammed Albar

The Kingdom of Saudi Arabia (KSA) initiated a Regional Cloud Seeding Program (RCSP) in 2022 to enhance precipitation over the southwestern and central parts of the country. This study presents an overview of RCSP cloud seeding operations conducted from 2022 to 2024, along with preliminary results on precipitation enhancement during the autumn season of 2022.

Precipitation data from the Global Interpolated Rainfall Estimation (GIRAFE) dataset, provided by EUMETSAT Climate Monitoring Satellite Application Facility (CM SAF), were used to investigate the relationship between precipitation anomalies and cloud seeding operations. The analysis focused on identifying spatial patterns where high precipitation anomalies coincided with regions of elevated cloud seeding flare density. These regions were categorized to evaluate the potential influence of cloud seeding activities.

This exploratory study highlights spatial correlations between cloud seeding operations and rainfall patterns, without accounting for additional meteorological or synoptic variables. The findings contribute to understanding the spatial dynamics of cloud seeding operations and their potential role in enhancing precipitation in arid regions, offering valuable insights for the optimization of weather modification strategies.

How to cite: Matsangouras, I., Logothetis, S. A., and Albar, A. M.: Regional Cloud Seeding and Rainfall Enhancement in Saudi Arabia: Preliminary Observations and Insights from 2022 Using EUMETSAT CMSAF GIRAFEv1 CDR, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11337, https://doi.org/10.5194/egusphere-egu25-11337, 2025.

EGU25-12347 | Posters on site | AS1.18

Projected Changes in the CORDEX-Central Asia’s Precipitation Extremes Using the NEX-GDDP-CMIP6 Models 

M. Tufan Turp, Nazan An, Zekican Demiralay, B. Cem Avci, and M. Levent Kurnaz

In this study, future projections of changes in precipitation extremes over the CORDEX-Central Asia domain were analyzed using high-resolution (0.25° x 0.25°) outputs from NEX-GDDP-CMIP6 models under SSP1-2.6, SSP2-4.5, SSP3-7.0, and SSP5-8.5 scenarios. Initially, 17 models were compared against ERA5 reanalysis data, and the five models with the best statistical performance (i.e., IPSL-CM6A-LR, GFDL-ESM4, MRI-ESM2-0, ACCESS-CM2, and BCC-CSM2-MR) were selected. These models were employed to analyze various precipitation indices, including consecutive dry and wet days, heavy and very heavy precipitation days, maximum of annual maximum precipitation, annual 5-day maximum precipitation, wet and very wet days, and simple daily intensity for the periods of 2026–2050, 2051–2075, and 2076–2100 with respect to the reference period of 1981-2010. The findings indicate an overall decrease in the average number of consecutive dry days across the region. Similarly, a slight average increase in the number of consecutive wet days is expected, which could have significant implications for regional water resource management and agricultural activities. Furthermore, the number of heavy precipitation days is projected to increase on average, highlighting the risk of flooding. These analyses underscore significant changes in precipitation extremes due to future climate change in the CORDEX-Central Asia domain. These findings are critical for shaping regional climate adaptation strategies, offering valuable insights for policymakers in water resource management, agricultural planning, and disaster mitigation. By understanding these projected changes, regional resilience to climate impacts can be enhanced, reducing future risks and fostering sustainable development.

Acknowledgement: This research has been supported by Boğaziçi University Research Fund Grant Number 19367. 

How to cite: Turp, M. T., An, N., Demiralay, Z., Avci, B. C., and Kurnaz, M. L.: Projected Changes in the CORDEX-Central Asia’s Precipitation Extremes Using the NEX-GDDP-CMIP6 Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12347, https://doi.org/10.5194/egusphere-egu25-12347, 2025.

EGU25-12666 | Orals | AS1.18

Recent Progress On Hydrometeor Identification Product For GPM DPR 

Chandra V Chandrasekar and Minda Le

A vertical description of the profiles of precipitation is a long-term goal of atmospheric research and precipitation science. The detailed hydrometeor identification products have great potential for constraining four-dimensional distributions of bulk hydrometeors and thus microphysical conversion processes for evaluating cloud-resolving models (CRMs), which is an important tool in the weather and climate research community. New three-dimensional hydrometeor type product will be available in the classification module in the next version (V8) of GPM DPR level 2 algorithm. This is a unique advantage for the space borne radar to provide a three-dimensional hydrometeor type over the globe while ground based observations are limited to the regions of deployment. The products developed by our team in the classification module allow us to have the potential to take a big step forward adding vertical profile of hydrometeors for DPR full swath data. Although GPM DPR has fine vertical resolutions in dual-frequency observations, most of the algorithms or products developed are 2 dimensional with either a “flag” or “type” (or etc.) on a 2-dimentional surface. These products include 1) Stratiform, convective rain separation; 2) detection of melting regions; 3) Developing a surface snowfall identification algorithm; (4) Developing a graupel and hail identification algorithm; and 5) the hail identification algorithm. 

 

How to cite: Chandrasekar, C. V. and Le, M.: Recent Progress On Hydrometeor Identification Product For GPM DPR, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12666, https://doi.org/10.5194/egusphere-egu25-12666, 2025.

EGU25-12874 | Posters on site | AS1.18

Application of ergodicity in regional rainfall frequency analysis  

Milan Onderka

Accurate estimation of rainfall quantiles at ungauged locations is critical for designing hydraulic infrastructure that can withstand extreme rainfall events over a broad range of timescales. However, short rainfall series often fail to capture the full variability and distribution of rainfall, leading to sampling bias. Geographical and climatological factors further complicate the estimation of rainfall frequencies in ungauged locations. To address these challenges, the concept of ergodicity in spatio-temporal patterns of rainfall extremes has been revisited. Ergodicity, in the context of stochastic processes, ensures that long-term time averages converge to the ensemble mean. This principle enables the pooling of rainfall data from multiple rain gauges within homogeneous regions to construct "regional" intensity-duration-frequency (IDF) curves. This mathematical framework has been investigated using normalized data from 100 rain gauges in Slovakia, with rainfall aggregated over time intervals ranging from 5 to 240 minutes. The analysis focused on low-probability rainfall events (p = 10-2 – 10-3) corresponding to recurrence intervals far exceeding the length of available records (approx. 15 years). Homogeneous regions were identified using fuzzy C-means clustering, revealing two homogenous clusters of rain gauges. Each cluster was assessed for ergodic behavior. To estimate the rainfall quantile for each cluster, the GEV distribution was applied to annual maximum series with parameters inferred using a Bayesian approach. Unique IDF curves were generated for each cluster, satisfying the criteria of ergodicity. These findings demonstrate the potential of the ergodicity-based approach to improve regional rainfall frequency estimates.

 

Acknowledgment: This work was supported by the Slovak Research and Development Agency under Contract No. APVV-23-0332.

How to cite: Onderka, M.: Application of ergodicity in regional rainfall frequency analysis , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12874, https://doi.org/10.5194/egusphere-egu25-12874, 2025.

EGU25-12943 | ECS | Orals | AS1.18

GPM DPR-Based Calibration of two Ground-based Weather Radars 

Eleni Loulli, Silas Michaelides, Johannes Bühl, Athanasios Loukas, and Diofantos G. Hadjimitsis

In the past decades, ground-based weather radars gained popularity for enhancing the understanding of precipitation systems, the accuracy of the Quantitative Precipitation Estimation (QPE) and for serving as input in numerical weather models. Nevertheless, they are prone to errors from various sources, including significant calibration errors. Previous research showed that the Ku-band precipitation radar aboard the Global Precipitation Measurement Mission Dual-Precipitation Radar (GPM DPR) is effective for calibrating ground-based radars. Several studies proposed the alignment of ground-based radar reflectivities with those from the GPM DPR to achieve their absolute calibration. This study performs the absolute calibration of the Rizoelia (LCA) and Nata (PFO) radars in Cyprus for approximately six years of observations (October 2017 to May 2023), assessing and comparing volume-matching thresholds and data filtering techniques. The results indicate that excluding reflectivities within the melting layer and adding a 250 m buffer consistently improved calibration for both radars. The selected calibration schemes were combined, and the resulting offsets were compared against stable radar parameters to identify stable calibration periods. Future work will include disdrometer data and expand the analysis to quantitative precipitation estimation.

Acknowledgements

The authors acknowledge the ‘EXCELSIOR’: ERATOSTHENES: EΧcellence Research Centre for Earth Surveillance and Space-Based Monitoring of the Environment H2020 Widespread Teaming project (www.excelsior2020.eu). The ‘EXCELSIOR’ project has received funding from the European Union’s Horizon 2020 research and innovation programme under Grant Agreement No 857510, from the Government of the Republic of Cyprus through the Directorate General for the European Programmes, Coordination and Development and the Cyprus University of Technology.

The authors also acknowledge the Department of Meteorology of the Republic of Cyprus for providing the X-band radar data.

 

How to cite: Loulli, E., Michaelides, S., Bühl, J., Loukas, A., and Hadjimitsis, D. G.: GPM DPR-Based Calibration of two Ground-based Weather Radars, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12943, https://doi.org/10.5194/egusphere-egu25-12943, 2025.

EGU25-13256 | Orals | AS1.18

Innovative improvements supporting version 3 of the Climate Hazard Center Infrared Precipitation with Stations 

Chris Funk, Pete Peterson, Laura Harrison, Robert Saldivar, Martin Landsfeld, Frank Davenport, Seth Peterson, William Turner, Daniella Alaso, Austin Sonnier, Shraddhanand Shukla, Enbo Zhou, Andreas H. Fink, Michael Budde, Diego Pedreros, James Verdin, and Gregory Husak

In the latest improvements to the Climate Hazards Infrared Precipitation with Stations dataset, CHIRPS3 (version 3), we address key shortcomings and validate the results against high gauge density datasets. The Climate Hazards Infrared Precipitation with Stations version 2 (CHIRPS2) is a widely-used 1981-present quasi-global 0.05° dataset that combines thermal infrared (TIR) geostationary satellite observations, a high-resolution climatology, and in situ rainfall gauge observations. While many studies have shown that CHIRPS2 performs well, we have identified and addressed an important shortcoming — a tendency to underestimate temporal precipitation variance. We also update and improve version 2 of the Climate Hazards Precipitation Climatology (CHPclimv2), and extend CHIRPS to 60°N/S. Finally, thousands of additional new time-varying stations are now included in CHIRPS3. Several countries in Africa, Central America and South America routinely contribute stations monthly.

We validate estimates using the high quality ‘Rainfall on a Gridded Network’ (REGEN) data set, comparing the performance of the CHIRP2 and CHIRP3 and similar products in 12 regions with high gauge densities. We also perform a validation study in Ethiopia. The usage section contrasts CHIRP2 and CHIRP3 performance in East Africa, during recent seasons associated with severe drought or extreme precipitation, to illustrate the value of the advancements made in the CHIRPS precipitation data product.

 

How to cite: Funk, C., Peterson, P., Harrison, L., Saldivar, R., Landsfeld, M., Davenport, F., Peterson, S., Turner, W., Alaso, D., Sonnier, A., Shukla, S., Zhou, E., Fink, A. H., Budde, M., Pedreros, D., Verdin, J., and Husak, G.: Innovative improvements supporting version 3 of the Climate Hazard Center Infrared Precipitation with Stations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13256, https://doi.org/10.5194/egusphere-egu25-13256, 2025.

EGU25-13282 | Posters on site | AS1.18

Development of a high-resolution database for daily precipitation in Greece 

Panagiotis T. Nastos, George Ntagkounakis, John Kapsomenakis, and Angelos Chasiotis

The accurate assessment of precipitation is a critical challenge in meteorology due to the non-normal distribution characteristics commonly associated with precipitation data. This distribution can lead to significant errors in forecasting models, particularly concerning extreme precipitation events, which are both infrequent and increasingly influenced by climate change. The implications of climate change on the frequency and intensity of these extreme events further complicate the task of accurate prediction, necessitating improved methodologies for rainfall estimation.

In the context of Greece, the challenge is intensified by a sparse network of precipitation observation stations. This limited data availability, coupled with the region's inherent geographical variability—characterized by diverse topographic features such as mountains and valleys—creates additional hurdles in the generation of reliable precipitation datasets. Consequently, the objective of this study is not only to address these challenges but also to create a high-resolution precipitation database specifically for Greece, employing advanced statistical interpolation techniques.

To achieve this, we systematically investigate a range of interpolation techniques aimed at generating high-resolution gridded daily precipitation datasets across the Greek territory. Our approach utilizes a comprehensive dataset of meteorological stations, which forms the backbone of our analysis. In addition, we incorporate geographical variables derived from satellite-based elevation data and integrate precipitation data sourced from the ERA5 atmospheric reanalysis, a product known for its high spatial and temporal resolution.

Three distinct modeling approaches are developed throughout this research.

  • General Additive Model and Indicator Kriging: In the first approach, we employ a General Additive Model combined with an Indicator Kriging methodology, relying predominantly on the station data and a limited selection of geographical variables. This foundational model serves as the baseline for understanding the initial relationships between observed precipitation and geographical factors.
  • Incorporation of ERA5 Data: The second iteration enriches the interpolation methodology by blending ERA5 reanalysis data with the observational datasets. In this stage, we expand the geographical variables used, allowing for a more nuanced understanding of precipitation patterns in relation to the diverse topography of Greece.
  • Multi-Model Interpolation Framework: Lastly, we introduce a novel modeling framework that not only integrates ERA5 data and an array of geographical datasets but also employs a multi-model interpolation process. This strategic approach utilizes different models tailored to predict precipitation during distinct thresholds. By addressing various precipitation intensity levels, this model enhances the ability to accurately forecast both average and extreme precipitation events.

The results of this study demonstrate that the inclusion of ERA5 data can significantly enhance the accuracy of the interpolated precipitation, particularly in regions where the observational station dataset is sparse. Moreover, the implementation of multi-model interpolation techniques—where distinct models are utilized for different precipitation thresholds—offers substantial improvements in the accuracy of both total precipitation forecasting and the modeling of extreme precipitation events. This multi-faceted approach effectively addresses crucial limitations exhibited in previous modeling efforts, thereby contributing valuable insights and robust methodologies to the field of meteorological research in Greece.

How to cite: Nastos, P. T., Ntagkounakis, G., Kapsomenakis, J., and Chasiotis, A.: Development of a high-resolution database for daily precipitation in Greece, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13282, https://doi.org/10.5194/egusphere-egu25-13282, 2025.

EGU25-13347 | ECS | Orals | AS1.18

Numerical evaluation of the wind-induced bias for the OTT Parsivel2 optical disdrometer 

Enrico Chinchella, Arianna Cauteruccio, and Luca G. Lanza

Non-Catching Gauges (NCGs) are increasingly employed to study precipitation microphysics and often serve as ground-based references for validating radar and satellite measurements. Their growing popularity is also due to their minimal maintenance requirements, that counterbalance their higher costs. However, wind-induced biases significantly affect NCG measurements by potentially diverting hydrometeors away from the instrument sensing area. This bias, already a concern for traditional catching gauges, is even more pronounced for NCGs due to their complex shapes, usually not radially symmetric (see e.g. Chinchella et al. 2024). This study investigates the wind-induced bias of measurements taken by the OTT Parsivel2 disdrometer using Computational Fluid Dynamics (CFD) simulations coupled with a Lagrangian particle tracking model implemented in the OpenFOAM software. CFD simulations provide the wind velocity field around the instrument body for different combinations of wind speed and direction by numerically solving the Unsteady Reynolds-Averaged Navier-Stokes equations, using a k-ω SST turbulence model and a local time-stepping approach. Results show that wind parallel to the laser beam causes maximum disturbance on the instrument sensing area, while wind perpendicular to the laser beam minimizes the disturbance. Hydrometeor trajectories are modelled starting from the simulated velocity fields, by releasing drops ranging from 0.25 mm to 8 mm in diameter within the computational domain. The trajectories are tracked until the drops either reach the gauge, exit the domain, or fall below the sensing area. From these simulations, the Catch Ratio (CR) is calculated, representing the ratio of the number of droplets reaching the instrument sensing area in the presence of wind and their number in undisturbed conditions. For wind parallel to the laser beam, limited overcatch is shown at low wind speed (1–2.5 m/s), while severe undercatch occurs at high wind speed. For wind perpendicular to the laser beam, the bias is limited, with minor overcatch observed at high wind speed. By fitting the CR, adjustments to the measurements can be applied, provided the wind speed and direction are known at the installation site. Since the CRs strongly depend on the hydrometeors diameter, wind also affects the measured Drop Size Distribution (DSD), with small drops often missed entirely in certain wind conditions. Similar results are shown when integrating the CRs over the full range of drop sizes, obtaining the Collection Efficiency, that represent the ratio of the precipitation volume sensed by the instrument to the actual precipitation volume. The effect of free stream turbulence is also being tested by superimposing turbulent vortexes over the free stream flow at the inlet of the simulation domain. In conclusion, wind significantly affects the measurement of precipitation microphysical and integral properties, including the derived DSD and rainfall volume, when using the OTT Parsivel2 disdrometer. These biases can be mitigated by applying adjustments as a function of wind speed and direction, thereby improving the reliability of NCG measurements in windy conditions.

References:

Chinchella E., Cauteruccio, A., & Lanza, L. G. (2024). Quantifying the wind-induced bias of rainfall measurements for the Thies CLIMA optical disdrometer. Water Resources Research, 60(10), e2024WR037366. https://doi.org/10.1029/2024WR037366

How to cite: Chinchella, E., Cauteruccio, A., and Lanza, L. G.: Numerical evaluation of the wind-induced bias for the OTT Parsivel2 optical disdrometer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13347, https://doi.org/10.5194/egusphere-egu25-13347, 2025.

EGU25-13507 | ECS | Orals | AS1.18

Kriging-variance based multi-member ensembles of radar-raingauge precipitation estimates: application in Switzerland  

Athanasios Ntoumos, Ioannis Sideris, Marco Gabella, Marco Boscacci, Lorenzo Clementi, Urs Germann, and Alexis Berne

CombiPrecip is an operational algorithm of MeteoSwiss that combines in real-time raingauge measurements with radar precipitation estimates across a domain of 710x640km2, covering Switzerland and extending beyond the Swiss borders. The system utilizes a geostatistical approach known as kriging with external drift as an interpolation technique, offering probabilistic outcomes that provide both a mean value and a variance at each interpolated point. The purpose of our study is two-fold: (i) We investigate to what extent the kriging variance of CombiPrecip is a satisfactory measure of uncertainty of the kriging expected value. We answer this question through a probabilistic verification of a seven-year dataset against raingauge measurements. (ii) We present an algorithm which integrates the kriging expected value and variance of the CombiPrecip output with spatially autocorrelated noise fields to generate ensembles of N realistic members. The verification suggests that the probabilistic CombiPrecip output has skill, which remains satisfactory even for high precipitation intensities. The ensembles generated by this method can serve as valuable initial conditions for precipitation nowcasting systems. Moreover, the proposed ensemble-generation technique is not restricted to geostatistics-based applications and can be readily adapted to other approaches that produce probabilistic outputs.

 

 

How to cite: Ntoumos, A., Sideris, I., Gabella, M., Boscacci, M., Clementi, L., Germann, U., and Berne, A.: Kriging-variance based multi-member ensembles of radar-raingauge precipitation estimates: application in Switzerland , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13507, https://doi.org/10.5194/egusphere-egu25-13507, 2025.

EGU25-13676 | Orals | AS1.18

A Generative Diffusion Model for Probabilistic Ensembles of Precipitation Maps Conditioned on Multisensor Satellite Observations 

Efi Foufoula-Georgiou, Clement Guilloteau, Gavin Kerrigan, Kai Nelson, Giosue Migliorini, Padhraic Smyth, Runze Li, and Neda Dolatabadi

Uncertainty quantification is an important component of satellite-derived precipitation products, yet most current methodologies lack the ability to provide such estimates. Here we use a  generative diffusion model to produce probabilistic ensembles of precipitation intensity maps at the 1-hour 5-km resolution, conditional on infrared and microwave radiometric measurements from the GOES and DMSP satellites. The model is trained with merged ground radar and gauge data over the southeastern United States. We show that the generated precipitation maps accurately reproduce the magnitude and location of precipitation features, and the spatial autocovariance and higher order statistics of the gauge-radar reference fields over a range of scales.  The 128-member ensemble is evaluated to assess whether it provides an accurate estimate of the precipitation uncertainty. We show that on average, the spectral coherence between any two ensemble members is approximately the same as that between any ensemble member and the ground reference, attesting that the ensemble dispersion is a proper measure of the estimation uncertainty across a range of scales.  We also evaluate the ensemble in terms of reproducing the probability of exceedance of any desired intensity threshold, at the 5-km resolution of the generation up to 80-km aggregation scale and show impressive agreement. Finally, generalization of the model to “unseen domains” is pursued by applying the trained model to the Western US and the challenges and opportunities in this generalization will be discussed.

How to cite: Foufoula-Georgiou, E., Guilloteau, C., Kerrigan, G., Nelson, K., Migliorini, G., Smyth, P., Li, R., and Dolatabadi, N.: A Generative Diffusion Model for Probabilistic Ensembles of Precipitation Maps Conditioned on Multisensor Satellite Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13676, https://doi.org/10.5194/egusphere-egu25-13676, 2025.

EGU25-14175 | Orals | AS1.18

The Fengyun rainfall mission FY3G: the scientific products and validation progress 

Lin Chen and Peng Zhang and the FY3G product technology team

Precipitation is one of the most important parameters in the earth system. China began to develop satellites dedicated to precipitation measurements in the second generation of the FENGYUN polar-orbiting meteorological satellite program (FY-3). The first of total two rainfall missions scheduled, FY-3G, was successfully launched on 16 April 2023 and became the world’s third satellite to measure precipitation with space-borne radar after the TRMM in 1997 and GPM in 2014. In this presentation, we will illustrate the scientific products and validation program.

The instruments on the FY-3G satellite can produce important geophysical parameters, including precipitation, atmospheric profiles, various clouds products and so on. As the core remote sensing instrument on the Fengyun rainfall mission, PMR(Precipitation Measurement Radar) can provide the 3D structure of precipitation, invert to obtain accurate information such as precipitation intensity and precipitation type, and improve the space-based precipitation measurement capability. Products such as bright band detection, precipitation type, precipitation phase state, precipitation rate, and latent heating will be processed to generate.19 kinds of scientific products have been publicly released and can be obtained through the dedicated website, FENGYUN Satellite Data Center (http://satellite.nsmc.org.cn/portalsite/default.aspx)..

The FY-3G Precipitation Measurement Radar (PMR) are comparable to Global Precipitation Measurement Dual-frequency Precipitation Radar (GPM DPR). Ground-based weather radar (GR) data are used to perform a comparative analysis of the reflectivity consistency between PMR and DPR satellite-ground radar observations. The results indicate that PMR and DPR are all systematic higher than GR. PMR and DPR are 1.15 dB and 1.56 dB higher than CINRAD reflectivity respectively, while 1.73 dB and 2.85 dB higher with NEXRAD with uncertainty round 2 dB. Stratiform samples exhibits the smallest biases, with reflectivity differences further reduced below the bright band (BB). PMR precipitation classification result aligns well with DPR. Through ground-based comparisons with CINRAD and NEXRAD, the FY-3G PMR exhibits relatively small differences. This makes it well-suited for joint global precipitation observations alongside the DPR.

As a pioneer of China's rainfall missions, FY-3G will greatly improves our ability to provide global precipitation measurements, understand Earth's water and energy cycle, and forecast extreme events for the benefit of society.

How to cite: Chen, L. and Zhang, P. and the FY3G product technology team: The Fengyun rainfall mission FY3G: the scientific products and validation progress, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14175, https://doi.org/10.5194/egusphere-egu25-14175, 2025.

EGU25-14218 | Orals | AS1.18

The Airborne Phased Array Radar (APAR) Observing Simulation, Processing, and Research Environment (AOSPRE) 

Wen-Chau Lee, Brad Klotz, Kevin Manning, and Jothiram Vivekanandan

The National Science Foundation (NSF) of the United States approved the Airborne Phased Array Radar (APAR) Mid-scale Research Infrastructure-2 proposal in 2023 to develop the next generation airborne polarimetric, Doppler weather radar mounted on the NSF/National Center for Atmospheric Research (NCAR) C-130 aircraft. Development of anew observing system is critical for the advancement of scientific understanding of weather phenomena. These instruments establish a proving ground for future operational transition while also providing tools for the research community. One of the issues with developing new instrumentation is the unknown performance characteristics of the instrument and the subsequent unknowns in uncertainty in measurements.

 

The APAR Observing Simulation, Processing, and Research Environment (AOSPRE) was developed to simulate APAR's measurement capabilities for heavy precipitation and high-impact weather events. Using Cloud Model 1 (CM1) and Weather Research and Forecasting (WRF) model output to provide various storms of interest and their surrounding environments, simulated NCAR C-130 flights are operated within the model space. Radar moments and dual-Pol variables are determined using the Cloud Resolving Model Radar Simulator (CR-SIM). Three-dimensional dual-Doppler radar winds can be retrieved from the Spline Analysis at Mesoscale Utilizing Radar and Aircraft Instrumentation (SAMURAI). The output can be examined directly or passed through additional tools to analyze various aspects of the data collected during each flight.

 

AOSPRE is linked to a NSF NCAR wide INtegrating Field Observations and Research Models (INFORM) to (1) establish and support best practices and methods for comparisons between models and observations, (2) exploit, assess and quantify the impacts of integrating observations and models to improve understanding of the prediction and predictability of the Earth system, and (3) improve the design, planning, deployment strategy of field programs and instrument development. The AOSPRE will be expanded into a field program planning tools as wells as a post campaign re-analysis tool with DA capability.

 

AOSPRE is developed as an open-source software. The first version of AOSPRE software has been released to the research and operational community in the last quarter of 2024. This paper will provide an overview of the AOSPRE and report the recent development of the AOS to better simulate the characteristics of a phased array radar on a moving platform. In addition, the authors will outline how AOSPRE will be used as a component in the future APAR data analysis software system.

How to cite: Lee, W.-C., Klotz, B., Manning, K., and Vivekanandan, J.: The Airborne Phased Array Radar (APAR) Observing Simulation, Processing, and Research Environment (AOSPRE), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14218, https://doi.org/10.5194/egusphere-egu25-14218, 2025.

EGU25-14491 | ECS | Posters on site | AS1.18

Precipitation observations using snow weight gauges and lysimeters 

Takashi Yamada, Shigeru Mizugaki, and Tomohito Yamada

Precipitation is a critical physical quantity in a variety of disciplines and is observed globally. Ground-based observations of precipitation typically use precipitation gauges; however, various losses must be considered. Of particular note is the importance of wind-induced undercatch in the context of solid precipitation. In addition, climate change may change snowfall to rainfall, increasing the importance of accurate precipitation observations.

The objective of this study is to evaluate the accuracy of precipitation observations, including snowfall, and to provide basic information for precipitation correction methods.
The present study focuses on wind-induced undercatch loss and estimates the capture rate of precipitation gauges by comparing them with observations from snow-weight gauges and lysimeters. This approach differs from the commonly used double-fence intercomparison reference.

These observations were made in a mountainous area of Japan (Hokkaido, 439 m above sea level) and included observations other than precipitation.
In addition, observations were made during the summer season to estimate the capture rate for precipitation.

Precipitation was verified by careful comparison of precipitation gauge readings with lysimeter readings and snow weight meter increments.
The study site is located in one of the snowiest regions of the world.
The region's water resources are primarily derived from the snowpack, underscoring the need for accurate snowpack estimates.
The measurement period began in November 2023 and data through mid-April 2025 are used in the following presentation.

The effectiveness of the lysimeter in capturing precipitation was found to be approximately 95%, a result consistent with previous studies conducted in Japan.
The cumulative capture rate (for the entire winter) for snowfall was about 60%, which is reasonable.
The presentation will also include a comparison with the capture rate estimate by Yokoyama (2003).

How to cite: Yamada, T., Mizugaki, S., and Yamada, T.: Precipitation observations using snow weight gauges and lysimeters, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14491, https://doi.org/10.5194/egusphere-egu25-14491, 2025.

EGU25-14561 | Orals | AS1.18

Progress Toward Addressing the Challenge of Mixed-phase Precipitation for the GPM Combined Algorithms  

Kwo-Sen Kuo, Ines Fenni, and Hélène Roussel

Available evidence indicates that accurate electromagnetic (EM) single scattering properties (SSPs) obtained from hydrometeors with realistic morphology are crucial for simulated signals to align with radar and radiometer observations (across all frequencies). Melting hydrometeors are of particular interest. Although they are confined to the melting layer, occupying only a few radar range gates, their greatly enhanced reflectivity and extinction obscure the EM signal of rainfall from below when observed from space, increasing uncertainty in surface precipitation estimates.
All recent efforts to enhance the realism of melting hydrometeor models and their SSPs have been constrained by computational costs and uncertainties in the scattering solutions. The Discrete Dipole Approximation (DDA) method, for its versatility with target geometry, has been applied to realistic solid hydrometeors, achieving unprecedented consistency in active (radar) and passive (radiometer) retrievals of snowfall. However, when applied to melting hydrometeors of mixed liquid-solid composition with high refractive contrast, DDA methods reveal their limitations, producing significant and varying uncertainties depending on dipole resolution and liquid mass fraction. 
To tackle these challenges in the relevant microwave spectrum for the full range of hydrometeors, we developed MIDAS, a numerically efficient 3D full-wave model for scattering by complexly shaped scatterers. Its core concept involves devising a direct-solver-based domain decomposition for the Method of Moment based on the volume integral equation to solve the EM scattering of electrically large and arbitrarily shaped scatterers. MIDAS has demonstrated not only a significant computational advantage over DDA-based codes when applied to realistic solid snow particles but also a greater potential to overcome DDA’s limitations concerning melting hydrometeors 
Indeed, promising initial results indicate that MIDAS outperforms the DDA code ADDA in calculating the SSPs of heterogeneous particles. We observe a good agreement, with relative differences below 2%, among MIDAS, ADDA, and Mie solutions for the scattering by heterogeneous (ice and water) 2-layer spheres and melting hydrometeors, provided the dipole size for MIDAS and ADDA is 5 times smaller than required by the normal criterion. However, MIDAS is 30 times faster than ADDA when SSPs are computed for 703 particle orientations. 
Furthermore, as we understand the need to economize further to meet the demands and constraints of melting hydrometeors, we have implemented adaptive mesh in MIDAS. The concept involves using a cell size inversely proportional to the material’s (i.e., water or ice) refractive index and ensuring compliance with the stricter validity criterion for liquid water without over-meshing the solid ice components of the melting hydrometeor. Initial results obtained with a mixed-resolution mesh where the finer mesh's cell size is half that of the coarser mesh are promising. The mere reduction in cell size by a factor of two for the liquid water portion significantly decreases computation costs, shortening the total computing time from 13.75 hours to 6.15 hours for the entire melting process (25 melting stages). The outcomes of this ongoing research will directly enhance the accuracy of SSPs for melting hydrometeors and provide a robust characterization of the uncertainties related to hydrometeor scattering in precipitation retrievals.

How to cite: Kuo, K.-S., Fenni, I., and Roussel, H.: Progress Toward Addressing the Challenge of Mixed-phase Precipitation for the GPM Combined Algorithms , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14561, https://doi.org/10.5194/egusphere-egu25-14561, 2025.

EGU25-14578 | ECS | Posters on site | AS1.18

Enhancing Flood Resilience through Developed Intensity Duration Frequency (IDF) Curves for Makkah, Saudi Arabia 

Abdirizak Dirie and Ahmed Al-Areeq

Developing Intensity-Duration-Frequency (IDF) curves is critical for effective water resource management, infrastructure design, and flood risk mitigation, particularly in arid and semi-arid regions where rainfall events are infrequent but intense. This study focuses on the development of IDF curves for Makkah, Saudi Arabia, an arid region characterized by limited ground rainfall station coverage. To address the data scarcity, a hybrid approach combining ground-based rainfall records and remote sensing data from the Integrated Multi-satellite Retrievals for GPM (IMERG) was employed. Ground station data provided localized accuracy, while IMERG data offered spatial and temporal completeness, compensating for the sparse ground observations. The analysis involved statistical techniques to calibrate and validate remote sensing data against ground measurements, followed by the derivation of IDF relationships through probabilistic modeling. The resulting IDF curves provide insights into extreme rainfall events, enhancing the understanding of hydrological patterns in arid regions and supporting climate resilience initiatives. This methodology underscores the utility of integrating remote sensing with traditional ground-based observations to overcome data limitations in resource-constrained environments.

How to cite: Dirie, A. and Al-Areeq, A.: Enhancing Flood Resilience through Developed Intensity Duration Frequency (IDF) Curves for Makkah, Saudi Arabia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14578, https://doi.org/10.5194/egusphere-egu25-14578, 2025.

EGU25-14923 | Orals | AS1.18

Potential for Remote Sensing of Precipitation using the Dynamic Microwave Radiometer on the NASA INCUS Mission based on the Heritage of TEMPEST Scientific Results 

Steven C Reising, Venkatachalam Chandrasekar, Chandrasekar Radhakrishnan, Shannon T. Brown, and Susan van den Heever

The INvestigation of Convective UpdraftS (INCUS) is a NASA Earth Venture mission (EVM-3) that will provide the first global systematic investigation into convective mass flux, the vertical transport of air and water, and its evolution within deep tropical convection.  The overarching goal of the INCUS mission is to understand why, when and where tropical convective storms form, and why only some storms produce extreme weather.  INCUS is led by PI Susan van den Heever of Colorado State University (CSU), in collaboration with NASA/Jet Propulsion Laboratory (JPL), Blue Canyon Technologies, and Tendeg Systems.  INCUS consists of a series of three small satellites flying in formation, each carrying a Ka-band radar based on RainCube and one cross-track scanning radiometer based on TEMPEST. A novel time-differencing approach among the three satellites flown in close succession (30, and 90, and 120 seconds apart) will provide the first estimates of convective mass flux across the tropics.

The success of the INCUS EVM-3 proposal to NASA relied on the prior success of two pathfinder CubeSat missions: RainCube, the first weather radar on a CubeSat, led by NASA/JPL, and the Temporal Experiment for Storms and Tropical Systems – Demonstration (TEMPEST-D) mission, led by CSU, producing the first global (up to 58 degrees latitude) observations from a multi-frequency microwave radiometer on a CubeSat, operating for nearly three years in LEO.

TEMPEST-D, a NASA Earth Venture Technology mission, produced global atmospheric science data, a well-calibrated, highly stable radiometer over three years of operations. TEMPEST-D brightness temperatures were validated using scientific and operational microwave sensors, including GPM/GMI and four MHS sensors, operating at similar frequencies to TEMPEST-D channels at 87, 164, 174, 178 and 181 GHz. Using the double-difference approach, TEMPEST-D performance was shown to be comparable to or better than much larger scientific and operational sensors, in calibration accuracy, precision, stability and instrument noise, during its nearly 3-year mission.

A duplicate TEMPEST sensor produced alongside TEMPEST-D was integrated with the Compact Ocean Wind Vector Radiometer (COWVR) from NASA/JPL and launched by the U.S. Space Force to demonstrate low-cost space technologies to improve global weather forecasting. COWVR/TEMPEST were launched on the STP-H8 mission on December 21, 2021, and have performed coordinated observations of Earth’s oceans and atmosphere from the ISS since January 7, 2022.  Retrievals of water vapor profiles, clouds, and precipitation from COWVR/TEMPEST-H8 are being performed in collaboration between JPL and CSU.

Previous studies have validated the accuracy and precision of TEMPEST-D brightness temperatures using clear-sky oceanic observations.  Recent advances extended the validation of TEMPEST-D and TEMPEST-H8 brightness temperature observations over tropical cyclones using GPM/GMI brightness temperatures and GPM/DPR vertical cumulative reflectivity. 

Prior studies demonstrated accurate quantitative precipitation estimation using machine learning over CONUS.  Recent advances expanded this capability to a global basis using GPM/GMI and AMSR-2 datasets for training and validation and IMERG rain rates for cross comparison.  The heritage of TEMPEST-D and TEMPEST-H8 will be used to demonstrate the potential for remote sensing of precipitation from the Dynamic Microwave Radiometer on the INCUS mission.

How to cite: Reising, S. C., Chandrasekar, V., Radhakrishnan, C., Brown, S. T., and van den Heever, S.: Potential for Remote Sensing of Precipitation using the Dynamic Microwave Radiometer on the NASA INCUS Mission based on the Heritage of TEMPEST Scientific Results, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14923, https://doi.org/10.5194/egusphere-egu25-14923, 2025.

EGU25-15261 | Orals | AS1.18

How can global snowfall estimates be improved by ESA's proposed Earth Explorer 11 WIVERN mission? 

Maximilian Maahn, Alessandro Battaglia, Marco Coppola, Sabine Hörnig, Pavlos Kollias, Stef Lhermitte, Nina Maherndl, Mario Montopoli, Filippo Scarsi, Frederic Tridon, and Anthony Illingworth

Snowfall is an important indicator of climate change, affecting surface albedo, glaciers, sea ice, freshwater storage, cloud lifetime, and ecosystems. Accurate measurements of snowfall at high latitudes are particularly important for estimating the mass balance of ice sheets; however, snowfall is difficult to quantify from both in situ and remotely sensed measurements.

Today, global snowfall products are mostly based on space-borne cloud radar observations such as CloudSat and now EarthCARE. However, these products suffer from systematic and random errors due to poor spatio-temporal sampling, the inability to observe snowfall near the surface due to ground clutter, and retrieval uncertainties due to insufficient information content of the observations.

WIVERN (WInd VElocity Radar Nephoscope) is one of the two remaining ESA Earth Explorer 11 candidate missions, with the final selection in July 2025. It is equipped with a 94 GHz conical scanning polarimetric Doppler radar and a 94 GHz passive radiometer. The main objective of the mission is to measure global horizontal winds in clouds, but it will also quantify cloud water content and precipitation rate.

Here we analyze WIVERN's potential to improve global snowfall products through the mission's unique design. Compared to CloudSat, WIVERN's 800 km swath provides 70 times better coverage including sampling closer to the poles and its 42 off-zenith angle significantly reduces the radar blind zone near the surface (especially over the ocean). In addition, WIVERN's radar includes polarimetric measurements and is accompanied by a radiometric mode, which can further improve the estimation of snowfall rates. Our results show that the WIVERN sampling strategy significantly reduces the uncertainty in polar snowfall estimates, making it a valuable product for climate model evaluation and as an input to surface mass balance models of the major ice sheets at the regional and seasonal spatio-temporal scales.

How to cite: Maahn, M., Battaglia, A., Coppola, M., Hörnig, S., Kollias, P., Lhermitte, S., Maherndl, N., Montopoli, M., Scarsi, F., Tridon, F., and Illingworth, A.: How can global snowfall estimates be improved by ESA's proposed Earth Explorer 11 WIVERN mission?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15261, https://doi.org/10.5194/egusphere-egu25-15261, 2025.

EGU25-15581 | ECS | Posters on site | AS1.18

Assessing climatological trends in daily precipitation extremes in Berlin-Brandenburg, Germany, using 43 years of station-based and reanalysis-based data 

Frederik Bart, Benjamin Schmidt, Fred Meier, Henning Rust, Daniel Fenner, and Dieter Scherer

Precipitation extremes have caused considerable damages in the Berlin-Brandenburg metropolitan region (Germany) during recent decades. To assess the climatological trends in intensity and probability of occurrence of these events, long-term precipitation data sets are an important prerequisite. Often, such investigations are based on measurements or interpolations of ground station networks. However, due to the high spatial variability of precipitation and its extremes, even relatively dense station networks may not be sufficient to accurately represent small-scale events. The utilization of long-term data, derived from numerical model simulations, has the potential to facilitate an area-wide evaluation. Therefore, we analyzed the spatial distribution of precipitation extremes in Berlin-Brandenburg based on observations by ground measurements and the capabilities of a gridded, reanalysis-based data set for assessment of spatial patterns in changes in seasonal return levels.

The data used consists of 43 years of daily rain gauge measurements by 227 stations of the German Weather Service (DWD) and precipitation data of the Central Europe Refined Analysis version 2 (CER v2, Bart et al., 2024). The CER v2 is a WRF-based dynamical downscaling of ERA-5 for the Berlin-Brandenburg region with a maximum spatial resolution of 2 km. For both data sets we fitted a Generalized Pareto Distribution using a time-dependent seasonal threshold and scale parameter to estimate the 2-, 5- and 10-year return levels at each location (station, grid point). After evaluating the goodness-of-fit at each station the magnitude and change in return levels was compared between both data sets.

The estimated changes in return levels for the CER v2 data correspond relatively well to changes estimated from the DWD stations. However, the CER v2 return levels themselves were on average 10-18% higher. The spatial patterns show an increase in the intensity of the 2-, 5- and 10-year events during summer months in both data sets and a decrease across the region during spring. The spatial variability of the rates of change is particularly high in winter and fall. Overall, the results show that reanalysis-based data could provide an important complement in the assessment of changes in regional precipitation extremes.

Bart, F., Schmidt, B., Wang, X., Holtmann, A., Meier, F., Otto, M., Scherer, D., 2024. The Central Europe Refined analysis version 2 (CER v2): evaluating three decades of high-resolution precipitation data for the Berlin-Brandenburg metropolitan region. metz. https://doi.org/10.1127/metz/2024/1233

How to cite: Bart, F., Schmidt, B., Meier, F., Rust, H., Fenner, D., and Scherer, D.: Assessing climatological trends in daily precipitation extremes in Berlin-Brandenburg, Germany, using 43 years of station-based and reanalysis-based data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15581, https://doi.org/10.5194/egusphere-egu25-15581, 2025.

EGU25-15807 | ECS | Posters on site | AS1.18

Investigating the Potential for Rimed Mass Retrieval Using Polarimetric Cloud Radar Observations 

Sabine Hörnig, Alessandro Battaglia, Maximilian Maahn, Nina Maherndl, and Mario Montopoli

Ice-related microphysical processes play a central role in global precipitation formation, but remain complex and difficult to quantify. Among these, riming, a mechanism by which supercooled liquid droplets freeze onto falling ice particles, significantly influences precipitation properties (essentially particle’s mass and fall speed). However, accurate measurements of riming remain difficult to obtain due to the limitations of remote sensing.

Current radar-based riming retrievals mostly rely on the higher fall velocity of rimed particles of the vertically-pointing radar Doppler spectrum. However, these retrievals are easily disturbed by vertical air motions and turbulence limiting their applicability in e.g. complex terrain.

Here, we explore the potential of slanted polarimetric W-band cloud radar observations for quantifying riming. Slanted view gives the opportunity to extend the retrieval capability over larger areas and more importantly enables the potential of polarimetry in case of horizontally aligned hydrometeros. As a reference, we use a normalized rime mass retrieval approach combining a 94 GHz Doppler cloud radar and in situ snowfall measurements from the Video In Situ Snowfall Sensor (VISSS). The instrument was deployed during the Surface Atmosphere Integrated Field Laboratory (SAIL) campaign.

Our analysis shows a strong relation between the normalized rime mass, column-integrated radar reflectivity (Ze), and the differential phase shift (ΦDP) from slanted polarimetric W-band radar observations. This suggests that polarimetric radar measurements, particularly the combination of Ze and ΦDP, can be used to estimate rimed mass with comparable performances than the joint use of radar and direct in-situ measurements.

This finding is particularly relevant in view of the forthcoming selection of ESA's Earth Explorer 11 mission, with WIVERN (WInd VElocity Radar Nephoscope) as one of the final candidates. WIVERN includes a conically scanning 94 GHz Doppler radar with polarimetric capabilities. Our results indicate that the correlation between ΦDP and Ze could potentially be used to retrieve rimed mass from spaceborne observations, opening a new way to study ice-related microphysical processes on a global scale.

How to cite: Hörnig, S., Battaglia, A., Maahn, M., Maherndl, N., and Montopoli, M.: Investigating the Potential for Rimed Mass Retrieval Using Polarimetric Cloud Radar Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15807, https://doi.org/10.5194/egusphere-egu25-15807, 2025.

EGU25-17837 | Posters on site | AS1.18

AQUAS - A quality control tool at GeoSphere Austria 

Niko Filipovic

Rain gauge measurement network of the Austrian national weather service operated by GeoSphere Austria comprises about 270 weather stations equipped with weighing rain gauges and, at a smaller part, with tipping bucket rain gauges. Each gauge is additionally equipped with a precipitation monitor that detects the beginning and the end of precipitation events. Precipitation data are checked for plausibility and completeness in several steps within a framework of an automated quality control tool called AQUAS (short for Austria Quality Service). The software was developed in 2016 at ZAMG (now GeoSphere Austria) in Vienna as part of the quality management in the area of real-time processing of near-surface observation data.
The basis for quality control procedure is formed by standard methods for checking meteorological and climatological data in accordance with the WMO recommendation (e.g. plausibility check, temporal, spatial and internal consistency check, etc.); in addition, test procedures are developed that take into account the specific errors in the measuring devices.  The test methods are continuously improved and further developed within the framework of AQUAS. Individual system components are designed to test the incoming observation parameters in real time - at the time resolution of 10 minutes, for example, for wind or temperature data and down to 1 minute time resolution for precipitation data. In AQUAS, each parameter can be processed independently of the other measured variables of a weather station. In addition, data from other sources are implemented in AQUAS, such as radar and satellite data. Data from numerical weather prediction models and data from other measurement networks, such as hydrological network or another third-party network, can also be integrated.

Some examples for the operational use of AQUAS and the current state of research on quality control of precipitation data will be presented. As an example, a novel method for real-time quality control of 1-minute weighing gauge precipitation data is demonstrated, which detects missing gauge precipitation based on the observation of the precipitation monitor and the total weight changes of the rain gauge.   

How to cite: Filipovic, N.: AQUAS - A quality control tool at GeoSphere Austria, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17837, https://doi.org/10.5194/egusphere-egu25-17837, 2025.

EGU25-18722 | ECS | Posters on site | AS1.18

Evaluation of GPM DPR products after orbit boost using disdrometers over Italy 

Sabina Angeloni, Elisa Adirosi, Federico Porcù, Mario Montopoli, Luca Baldini, Alessandro Bracci, Vincenzo Capozzi, Clizia Annella, Giorgio Budillon, Orietta Cazzuli, Gian Paolo Minardi, Renzo Bechini, Valentina Campana, Roberto Cremonini, Lorenzo Luini, Roberto Nebuloni, Vincenzo Rizi, Paolo Valisa, Simone Scapin, and Wolff David B. and the Sabina Angeloni

Precipitation monitoring plays a key role in understanding Earth's climate system and its effects on sectors such as hydrology, water resource management, and agriculture. Satellite-based measurements, particularly through missions like the Global Precipitation Measurement (GPM), have significantly enhanced our ability to observe precipitation patterns globally. Onboard the GPM Core Observatory, the Dual-frequency Precipitation Radar (DPR), consisting of the Ku-band Precipitation Radar (KuPR), which operates at 13.6 GHz, and the Ka-band precipitation radar (KaPR) at 35.5 GHz. The DPR has proven to be an indispensable instrument for characterizing water cycle study applications. To extend the life of a satellite, in order to guarantee the continuity of observations, a common strategy is to increase the orbit altitude. For this reason, on November 7 and 8, 2023, the GPM Core Observatory performed two orbit boost maneuvers that raised its altitude from 407 km to 442 km. As a result of this orbital elevation, the observing parameters of the GPM DPR instruments underwent some changes, such as the increase of spatial resolution and of the minimum detectable rain rate, which has had an impact on some geophysical products. To ensure the accuracy and reliability of satellite data over time, the GPM mission supported a Ground Validation program, which aims to verify and improve precipitation retrieval algorithms over time using multiple ground based instruments. This study focuses on GPM DPR Level 2 Version 7, which is the first to incorporate a modified scan pattern for the KaPR, introduced on May 21, 2018. This adjustment enables the dual-frequency radar to operate across the full observation swath. This study compares the GPM DPR Version 7 products, specifically the earlier Version 7A (before the orbit boost) with Version 7C (after the orbit boost), over Italy, using data from a network of ground-based laser disdrometers networked by the GID (Gruppo Italiano Disdrometria, in Italian). The dual-frequency-based 2ADPR-FS, as well as the single-frequency-based 2AKa-FS and 2AKu-FS Version 7 Level 2 DPR products are used. GPM data from May 22, 2018, to November 30, 2024, were analyzed. The following variables have been investigated: reflectivity factors at the Ku and Ka bands corrected for attenuation, rainfall rate, and DSD parameters Dm and Nw. Statistical indices are used to assess the agreement between satellite observations and disdrometer data. After the orbit boost, dual frequency still presents a slightly better agreement with disdrometers with respect to single frequency products. Discrepancies, however, were noted in the performance of rainfall and microphysical parameters, especially in areas with complex terrain and disdrometers located at high altitudes. In general, the comparison of Version 7A and Version 7C products with disdrometers helped reveal the limited influence of the orbit boost on the quality of DPR products. The results suggest that an orbital adjustment, similar to those implemented for the GPM mission, can be effectively adopted by other missions aimed at reconstructing the 3D structure of clouds and precipitation, since extending the satellite's operational life results in only a negligible impact on the quality of the data products.

How to cite: Angeloni, S., Adirosi, E., Porcù, F., Montopoli, M., Baldini, L., Bracci, A., Capozzi, V., Annella, C., Budillon, G., Cazzuli, O., Minardi, G. P., Bechini, R., Campana, V., Cremonini, R., Luini, L., Nebuloni, R., Rizi, V., Valisa, P., Scapin, S., and David B., W. and the Sabina Angeloni: Evaluation of GPM DPR products after orbit boost using disdrometers over Italy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18722, https://doi.org/10.5194/egusphere-egu25-18722, 2025.

EGU25-18724 | Posters on site | AS1.18

On validating EarthCARE CPR precipitation products with different instruments  at ground 

Luca Baldini, Sabina Angeloni, Elisa Adirosi, Mario Montopoli, Alessandro Bracci, Giandomenico Pace, Daniela Meloni, Claudio Scarchilli, Virginia Ciardini, and Matteo Picchiani

Satellite-based measurements are necessary to provide reliable measurements of clouds and  precipitation on global scale. Starting from the NASA/JAXA TRMM and NASA CloudSat missions, and consolidated by the NASA/JAXA GPM (Global Precipitation Measurement) mission, radars on satellite are playing a growing important role allowing to cover remote and oceanic areas and to reveal the vertical structure of clouds and precipitation systems. The ESA/JAXA EarthCARE (Clouds, Aerosol and Radiation Explorer) satellite, in orbit since 28 May 2024, has on board a 94 GHz Cloud Profiling Radar (CPR) provided by JAXA and NICT, with Doppler capability that provides information on vertical cloud profiles and precipitation properties through complex algorithms that require physical assumptions. It is there important to validate both satellite quantitative products with independent measurements and the physical assumptions underlying the retrieval algorithms.  Missions addressing clouds and precipitation have relied on field campaigns, using suborbital flights seeking for coincidence in locations of aircraft and satellite measurements, networks of instruments for long-term statistical validation, or supersites with multiple instruments capable of collecting high quality measurements correlative to satellite measurement.

Unlike other atmospheric parameters, clouds and even more, precipitation are significantly affected by spatial variability, even within a few kilometers and have an intrinsic intermittent nature. This fact poses specific challenges in obtaining an adequate quantity of significant correlative measurements during satellite overpasses from fixed installation. Satellite radar observations are validated with ground-based measurement devices, including raingauges and disdrometers (although the satellite measurement unaffected by ground clutter are several hundred meters above) or radars. Ground-based profiling radars operating at vertical incidence have adequate vertical resolution for matching satellite radar measurements but, depending on the wavelengths adopted on satellite and at ground, could differ in sensitivity and wavelengths. The spatial coincidence of individual satellite and ground-based profiles is unlikely. The GPM-GV program includes scanning weather radars, including operational ones, to match observations, considering the different sampling volume. They have a wider vertical resolution compared to radar profilers for most distances and lack sensitivity for clouds parameters. This study  part of the project “Contribution to EarthCARE products VALidation during the commissioning phase from atmospheric observatories in Central MEDiterranean in Italy (EC-VALMED.it)“ funded by ASI consider available data collected from satellite along with datasets available in the two validation sites of Rome and Lampedusa. The evaluation of the influence of spatial variability of observed precipitation phenomena at small scale is the aim of this study, crucial to understand the representativeness of the two validation sites and to define the validation strategy to be followed to validate geophysical products of EarthCARE CPR. An experimental approach based on operational weather radar and satellite radar profiles, aims at pointing out the effect of non-coincident measurements, along effects of difference of wavelength between satellite and ground sensors, and the effect of blind zone close to the surface. To this purpose, L2 CPR data will be considered, together with measurements collected from the instruments at ground available in the validation sites (disdrometer, radar profilers) and quasi-coincident data from operational scanning radars.

How to cite: Baldini, L., Angeloni, S., Adirosi, E., Montopoli, M., Bracci, A., Pace, G., Meloni, D., Scarchilli, C., Ciardini, V., and Picchiani, M.: On validating EarthCARE CPR precipitation products with different instruments  at ground, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18724, https://doi.org/10.5194/egusphere-egu25-18724, 2025.

EGU25-19080 | ECS | Posters on site | AS1.18

An evaluation of the uncertainty of precipitation measurements from optical sensors at a Norwegian mountainous site. 

Renaud Gaban, Mareile Wolff, and Bikas Chandra Bhattarai

In remote areas with high mountains or challenging weather conditions, ground-based precipitation measurements cannot be performed by instruments that require extensive maintenance. Still, in-situ measurements are essential to validate model predictions or remote sensing measurement methods. Optical sensors (disdrometers and present weather sensors) constitute a good alternative to traditional methods, requiring little maintenance and having no moving parts that could deteriorate. However, these devices are calibrated in laboratory conditions that can be very different from the ones they experience in the field. Therefore, it is essential to improve our understanding of the reliability of these instruments when they operate in a challenging environment.

Users who rely on optical instruments are primarily interested in high-frequency reports of precipitation type (e.g. public road management, aviation) and precipitation rate (e.g. hydropower systems, agriculture). These variables are derived from semi-empirical knowledge together with measurements of hydrometeors’ sizes and fall velocities, that can both be affected by the wind or other instrumental systematic biases. 

In this work, we analyze data collected at the former WMO-SPICE site of Haukeliseter in Telemark, Norway. This station is operated by MET Norway. Two to three models of different popular optical instruments (OTT Parsivel2, Thies Clima LPM, Vaisala PWD12 and PWD22), unevenly exposed to the wind, have been deployed there since September 2023, providing two winters of precipitation data to analyze. Haukeliseter is located in a mountainous area commonly experiencing strong winds and is covered with snow for about 6 months a year, making it an excellent location to study solid precipitation.

We perform a systematic intercomparison of these instruments to evaluate their level of agreement and, in turn, quantify their accuracy. A reference for the precipitation rates consisting of a Geonor rain gauge placed in a standard WMO-defined DFAR (double fence automated reference) setup is available. There exists no similar standard field reference for precipitation type detection. Where possible, human observations are used as a benchmark, but they are often available at a much lower time resolution than automatic measurements. To compensate for the lack of such long-term observations at Haukeliseter, a campaign of on-site high-frequency human observations of the precipitation type performed in early 2025 is used as a comparison reference. Preliminary results of the intercomparison and analysis from this winter’s measurement campaign will be presented.

How to cite: Gaban, R., Wolff, M., and Bhattarai, B. C.: An evaluation of the uncertainty of precipitation measurements from optical sensors at a Norwegian mountainous site., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19080, https://doi.org/10.5194/egusphere-egu25-19080, 2025.

The Middle East, characterized by dry climates and water scarcity, has seen significant changes in precipitation patterns over the past few decades. This research investigated the temporal and spatial changes of precipitation during the statistical period of 1981-2023 in the Middle East using CHIRPS satellite images. Analysis of average monthly rainfall in the Middle East showed that January, January, March, and December were the wettest months, and June, July, August, and September were the driest months. An upward trend of rainfall was observed in all months except February. This trend was especially significant in June, September, July, and August. The months of January, April, May, and June showed the highest annual increase in rainfall. Also, based on the results of seasonal rainfall, the winter season had the highest average rainfall, followed by spring and summer, which showed the highest slope of rainfall changes. Based on the results of the visual trend of precipitation in summer, regions such as southeast and eastern Anatolia in Turkey, Basra, and various regions of Iraq and Iran experienced a significant decrease in rainfall with a trend of approximately 0.25 mm. Likewise, during the fall, this trend continued in the northern regions of Iran, Yemen, Oman, and parts of Türkiye, Iraq, Egypt, and Syria. Parts of Lebanon and northern Iraq have experienced a significant decrease in some places during the winter season. A part of the north of Matrouh province in Egypt, southwest (Khuzestan), and north (Mazandaran, Gilan, and Ardabil) of Iran have experienced an increase in rainfall up to .5 mm in the winter season. In general, according to the picture of the annual changes in precipitation, the northern half of the Middle East in the countries of Iran, Turkey, Syria, and northern Iraq has seen a decrease in precipitation, and the southern half of the Middle East and northern Turkey in the Black Sea geographical region have seen an increase in precipitation over 43 years. have experienced in the past.

How to cite: Rousta, I. and Ólafsson, H.: Assessing Spatio-Temporal Precipitation Variations in the Middle East (1981-2023) Using Remote Sensing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19134, https://doi.org/10.5194/egusphere-egu25-19134, 2025.

EGU25-20148 | Orals | AS1.18

MSWEP V3: Enhancing Global Precipitation Estimates with Machine Learning 

Hylke Beck, Xuetong Wang, Hayley Fowler, Raied Alharbi, and Diego Miralles

We introduce Version 3 (V3) of the gridded near real-time Multi-Source Weighted-Ensemble Precipitation (MSWEP) product — the first fully global, machine learning-based precipitation (P) product, developed to address the growing demand for accurate precipitation data amid escalating climate challenges. MSWEP V3 provides hourly 0.1° resolution data from 1979 to the present, updated continuously with a latency of less than two hours. The development involves a two-stage process: first, baseline P fields are generated using machine learning model stacks that integrate satellite and (re)analysis P and air temperature products alongside static P-related variables, trained with hourly and daily observations from nearly 18,000 global gauges. Second, these fields are corrected using available daily gauge observations, accounting for gauge reporting times. To assess MSWEP V3's performance, we conducted an extensive evaluation of 19 gridded P products, using independent observations from almost 18,000 gauges excluded from training. MSWEP V3 (prior to gauge corrections) achieved a mean daily Kling-Gupta Efficiency (KGE) value of 0.69, outperforming all 18 other products evaluated. For comparison, other non-gauge-corrected products such as CHIRP, ERA5, GSMaP V8, and IMERG-L V7 achieved mean KGE values of 0.31, 0.61, 0.38, and 0.46, respectively. MSWEP V3 consistently ranked first or second across multiple metrics, including correlation, overall bias, peak bias, wet days bias, and the critical success index. Notably, MSWEP V3 (without gauge corrections) also outperformed several products that directly incorporate gauge observations, such as CHIRPS, CPC Unified, and IMERG-F V7, which achieved mean KGE values of 0.36, 0.54, and 0.62, respectively. Set for release in early 2025, we anticipate that MSWEP V3 will support climate research, water resource assessments, flood management, and numerous other applications.

How to cite: Beck, H., Wang, X., Fowler, H., Alharbi, R., and Miralles, D.: MSWEP V3: Enhancing Global Precipitation Estimates with Machine Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20148, https://doi.org/10.5194/egusphere-egu25-20148, 2025.

EGU25-20488 | Orals | AS1.18

Event-based Precipitation Features from GPM IMERG Data Product 

Michael Bauer, Kwo-Sen Kuo, and Dai-Hai Ton-That

We extract statistical precipitation features from precipitation events tracked in both space (two-dimensional, 2D) and time (one-dimensional, 1D) using NASA Global Precipitation Mission’s IMERG data product. These features can be used to ensure IMERG product consistencies (since the combination of instruments and algorithms used to derive this product evolves with time) and study decadal precipitation variations. They may even reveal climate change signals.

We use connected component labeling (CCL) for tracking. Two-dimensional (2D) connected precipitating components (with precipitation rate ≥ 0.1 mm/hr and an area coverage ≥ 25 grid cells, i.e., ~2500 km2) are identified first in each half-hour (spatial) slice of IMERG data. We consider the components touching the space or time boundary incomplete and discard them from temporal tracking. Spatially overlapping 2D connected components in adjacent half-hour time slices are considered to be of the same precipitating events and are given unique labels. A precipitation event thus may start as disjoint 2D components, experience merging and splitting, and eventually disappear.

We extract event-based precipitation features based on tracked events instead of spatially connected 2D components. This is a significant departure from previous precipitation feature studies ( e.g., Liu et al., 2008; Hayden et al., 2021), in which precipitation features are based on 2D connected components in a half-hour IMERG slice, i.e., in space only. Hayden et al. (2021) perform tracking based on the overlap in adjacent IMERG time slices of equivalent-area circular discs derived from these 2D connected components, which may or may not have overlapping precipitating cells.

We report in this presentation statistical precipitation features extracted from 10 years of Northern Hemisphere IMERG data (2014-2023). Such features include distributions of event duration, maximum area coverage, maximum precipitation rate, event-integrated precipitation volume, etc. We also report these features filtered by season and geographical region for more detailed analysis.

References

Hayden, L., Liu, C., and Liu, N.: Properties of Mesoscale Convective Systems Throughout Their Lifetimes Using IMERG, GPM, WWLLN, and a Simplified Tracking Algorithm, Journal of Geophysical Research: Atmospheres, 126, e2021JD035264, https://doi.org/10.1029/2021JD035264, 2021.

Liu, C., Zipser, E. J., Cecil, D. J., Nesbitt, S. W., and Sherwood, S.: A Cloud and Precipitation Feature Database from Nine Years of TRMM Observations, Journal of Applied Meteorology and Climatology, 47, 2712–2728, https://doi.org/10.1175/2008JAMC1890.1, 2008.

How to cite: Bauer, M., Kuo, K.-S., and Ton-That, D.-H.: Event-based Precipitation Features from GPM IMERG Data Product, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20488, https://doi.org/10.5194/egusphere-egu25-20488, 2025.

EGU25-45 | ECS | Orals | CR5.1

Improvement of the CLASSIC Snow Model to Better Simulate Arctic Snowpacks 

Mickaël Lalande, Christophe Kinnard, and Alexandre Roy

Current snow models – including the most sophisticated ones, such as CROCUS and SNOWPACK – struggle to properly simulate Arctic snowpack characteristics such as density profiles. Indeed, those models have been developed and designed for Alpine snowpacks, which evolve differently from Arctic ones due to higher wind speeds, increasing the compaction of the upper snowpack layers, and stronger temperature gradients, inducing upward water vapor fluxes within the snowpack and influencing the compaction and metamorphism. Both phenomena – combined with complex interactions with the vegetation – are at the origin of the wind-slab and depth hoar formation in Arctic snowpacks. The Canadian Land Surface Scheme including Biogeochemical Cycles (CLASSIC) – being the Canadian Earth System Model (CanESM) land surface component – uses a medium-complexity single-layer snow scheme. Whether correctly representing Arctic snowpack bulk characteristics requires a multilayer approach over a single-layer snow scheme is still an open question. To assess the model skills, 1D simulations were performed at ten sites – including three Arctic sites. Improvements in the snow model scheme were carried out, including three new parameterizations to better represent Arctic snow: (1) blowing snow sublimation losses, (2) wind inclusion in the computation of fresh snow density, and (3) increased wind compaction. Those improvements allow most of the current model skills to be improved at the Arctic sites. Uncertainties related to the meteorological forcing, variable measurements, snow drift, and model bias compensations are a perpetual challenge in those model assessments. Future studies will involve spatial evaluation of those model developments in addition to implementing new snow cover fraction parameterization in CLASSIC. The influence of these new developments will be assessed against the ESA Snow CCI variables for different land types and for the simulated surface energy and carbon fluxes.

How to cite: Lalande, M., Kinnard, C., and Roy, A.: Improvement of the CLASSIC Snow Model to Better Simulate Arctic Snowpacks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-45, https://doi.org/10.5194/egusphere-egu25-45, 2025.

Snow cover and seasonally frozen ground (SFG) are the key cryospheric elements on the southern edge of Altai Mountains (SEAM). Quantifying the thermal effect of snow cover on the frozen ground remains challenging. Utilizing the datasets observed at Altai Kuwei Snow Station (AKSS) and by National Meteorological Stations of China Meteorological Administration (CMA), we evaluated the thermal effect of snow cover on SFG regime. The results observed by AKSS indicated that the energy exchange between the ground and atmosphere was significantly insulated by snow cover, resulting in a considerable temperature offset between the snow surface and the ground below. This offset reached a maximum of 12.8 °C for a snow depth of 50 cm, but decreased for snowpack depths of >70 cm, whereas the snow temperature lapse rate was systematically steeper in the upper snowpack than at depth. Snow cover was the dominating driver of inter-annual differences in the SFG regime, as represented by the annual maximum freezing depth and soil heat flux. The observed average soil heat loss rate increased from 2.68 to 5.86 W/m2 on two occasions when the average snow depth decreased from 61.2 cm to 13.7 cm, resulting in an increase in maximum freezing depth of SFG from 69 cm to >250 cm soil depth. The results observed by CMA also demonstrate how snow cover controlled the SFG regime by warming the ground and inhibiting freezing of the soil column. Snow cover caused a 44.5-cm decline of annual maximum freezing depth during 1961-2015 period. SFG degradation between 1961 and 2015 was accompanied by increases in both air temperature and snow cover, with the former playing the dominant role. The correlation between snow cover and the ground–atmosphere temperature offset provides a new empirical method of evaluating the effective thermal effect of snow cover on SFG.

How to cite: zhang, W.: Observations on snow cover and frozen ground in the Chinese Altai Mountains, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2196, https://doi.org/10.5194/egusphere-egu25-2196, 2025.

EGU25-3069 | ECS | Orals | CR5.1

Drifting Snow Particle Fragmentation Enhances Blowing Snow Sublimation 

Guang Li, Jiacheng Bao, Hongxiang Yu, and Ning Huang

Snowflakes usually have different shapes for different formation environments. When drifting snow happens, fragmentation makes snowflakes transform into rounder shapes and releases more small particles. This is important because it changes airborne snow particles' size distribution(SPSD) and concentration, affecting blowing snow mass flux and sublimation rate. However, current drifting and blowing snow models ignore this, increasing uncertainty in predicting snow mass and energy balance. Here, we develop a drifting and blowing snow model considering the snow fragmentation process during particle-bed interaction and investigate the effects of fragmentation on drifting and blowing snow. The results show that compared to not considering fragmentation, fragmentation changes the SPSD, resulting in an enhancement of mass flux and sublimation rate. The sublimation rate of blowing snow increases by 75% on average under a moderate wind speed ( with a friction velocity between 0.3 and 0.5 m/s). Initial SPSD also affects the final sublimation rate, which indicates that SPSD is an important factor for blowing snow modeling.

How to cite: Li, G., Bao, J., Yu, H., and Huang, N.: Drifting Snow Particle Fragmentation Enhances Blowing Snow Sublimation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3069, https://doi.org/10.5194/egusphere-egu25-3069, 2025.

EGU25-3774 | ECS | Posters on site | CR5.1

Dry snow densification over ice sheets in the ORCHIDEE land surface model  

Philippe Conesa, Cécile Agosta, Sylvie Charbit, Simon Beylat, and Christophe Dumas

The Antarctic and Greenland ice sheets are particularly vulnerable to global warming. Surface melt and runoff are increasing over Greenland, inducing a decrease in surface mass balance. Projections suggest that this process will accelerate in the future and could also affect the Antarctic ice sheet. Over ice sheets, snowpacks can reach several tens of meters and have the capacity to store and refreeze liquid water. This process directly impacts the amount of runoff and is strongly dependent on the physical characteristics of the snowpack, particularly the snow density governed by metamorphism and overburden pressure. Consequently, understanding and modelling the evolution of ice sheets requires an accurate representation of surface and internal snowpack processes.  However, many Earth system models have simplified snowpack schemes, often evaluated and adapted for seasonal snow but not for polar snow conditions.

Here we present an automatic method for initialization and calibration of densification in snowpack models, applied  to the ORCHIDEE model, the land surface scheme of the IPSL-CM Earth system model. ORCHIDEE includes an intermediate complexity representation of the snowpack with 12 snow layers and 8 ice layers. In this work, we use ORCHIDEE in offline conditions with atmospheric forcings from the polar-oriented regional atmospheric model MAR. We develop a snowpack initialization method adaptable to any snowpack thickness and model. To address the limitations of densification parameterizations for polar regions identified in ORCHIDEE, we use  an automatic tuning method known as History Matching to calibrate free parameters of the densification formulations. Calibration of 1D simulations over two characteristic dry-snow locations in Greenland and Antarctica enable us to improve densification across the rest of the ice sheets. We apply this method for two different types of density parameterizations and obtain similar good agreement with observed density profiles from the SUMup database. In the future, this methodology can be extended to other free parameters of the model, such as those associated with the albedo parameterization.

How to cite: Conesa, P., Agosta, C., Charbit, S., Beylat, S., and Dumas, C.: Dry snow densification over ice sheets in the ORCHIDEE land surface model , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3774, https://doi.org/10.5194/egusphere-egu25-3774, 2025.

EGU25-3784 | Orals | CR5.1

Characterizing and Predicting Watershed-Wide Snowpack Ripening Patterns with Machine Learning Methods 

Joel Harper, Clément Cherblanc, Javier Pérez Álvaro, and Jesse Johnson

A melting snowpack initiates runoff production after cold content has been eliminated and the pore liquid water content has grown to overcome capillary resistance, a process called ripening. Here, we quantify the time-space distribution of ripening within a 4341 km² mountain basin in Montana, USA. Using model output for a 19 year period we compute a time-series of the energy needed for ripening, termed the Runoff Energy Hurdle (REH). The REH is associated with snowpack mass but is variably influenced by cold content, peaks earlier than mass, and is typically eliminated in days. We show that individual locations have complex year-to-year histories of REH growth and loss. Through K-means clustering, we identify four distinct ripening behaviors across high year-to-year variability. One cluster has ripening events throughout the snow season and can include 7-92 % of the basin depending on the year. Three additional clusters ripen progressively later in the spring season within narrowing time windows. We test machine learning methods for predicting the major spring ripening event at each location, based solely on snowpack state. The predictability is proportional to the magnitude of REH, with runoff activation of the highest REH locations predictable within an 18-day window eight weeks in advance. 

How to cite: Harper, J., Cherblanc, C., Pérez Álvaro, J., and Johnson, J.: Characterizing and Predicting Watershed-Wide Snowpack Ripening Patterns with Machine Learning Methods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3784, https://doi.org/10.5194/egusphere-egu25-3784, 2025.

EGU25-5827 | ECS | Orals | CR5.1

Some insights from the second principle for snow modelling 

Kevin Fourteau, Kaoane Jondeau, and Clement Cances

As snowpacks are largely governed by thermodynamics, special care is usually given as to ensure the first principle, i.e. energy conservation, in their mathematical and numerical descriptions. On the other hand, the second principle, i.e. entropy production, has received less attention. However, the second principle, and its numerical translation, has proven to be a powerful tool in applied mathematics to ensure the stability of mathematical and numerical models. The goal of this work is thus to present the derivation of thermodynamically consistent numerical snowpack models. This rigorous approach restricts the number of acceptable numerical schemes that unconditionally comply with the second principle, and which are thus free of spurious oscillations, overshoots, or divergence. As examples, we consider some regularly encountered cases of numerical instabilities in snowpack models, and re-visit them based on the second principle point of view.

How to cite: Fourteau, K., Jondeau, K., and Cances, C.: Some insights from the second principle for snow modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5827, https://doi.org/10.5194/egusphere-egu25-5827, 2025.

As a form of solid precipitation, snow plays a crucial role in climate regulation by reflecting solar radiation and insulating the ground. Additionally, it serves as a vital water resource, influencing hydrological cycles through its seasonal melting process. So, accurate predictions of snowfall and the subsequent evolution of the snowpack are essential. In this study, some investigations are made to reveal the impact of multi-strategically assimilating Global Precipitation Measurement (GPM) precipitation and Himawari-8/Advanced Himawari Imager (AHI) water vapor radiances (WVR) on forecasting a heavy snowfall event and snow properties on the ground over the Eastern Qinghai-Tibet Plateau employing the Weather Research and Forecast model (WRF) and the Four-Dimensional Variational assimilation system. DA strategies includes two aspects: the initial time of Reg_NWPs runs and the type of observations used. The initial times of Reg_NWPs are 0000 UTC, 0600 UTC, and 1200 UTC on October 28, 2022. Separate and combined DA tests are conducted to forecast. For the process of snowfall, the joint assimilation of the two not only yields multi-dimensional atmospheric insights but also addresses the limitations of individual assimilation. Assimilation GPM and AHI are respective sensitivity to the lower layers (about 800hpa) and upper layers (about 400hpa) of model. The individual assimilation GPM has the greatest effect on near-surface humidity field, and AHI plays a dominant role in the joint assimilation. In addition, we further compare the 12-hourly cumulative snowfall with in-situ meteorological station observations. The predictions of snowfall from DA_G&A perform much better with the correlation coefficient and root-mean-square error 0.36 and 3.14mm, respectively. As for different initial times of NWPs, the best snowfall forecast is 0600 UTC on October 28, 2022, and the CC is 0.4. For the snow properties on theground, the results indicate that the predictions of snow properties, such as snow depth (SD), snow cover fraction (SCF) and snow albedo (SAL), are influenced by both the initial time of Reg_NWPs and the type of observations. DA_G&A showed a significant increase in deep snow area (SD >15cm), and a decrease in shallow snow area (SD<5cm). Comparing with some reanalyzed and remote sensing inversion datasets, the predictions exhibit good physical consistency between snow parameters and fine temporal-spatial resolution. However, the land surface scheme of Reg_NWPs tends to overestimate SCF and SAL. So, in the future, the integration of a land surface DA system (LDAS) into Reg_NWPs will be considered for on-line coupling.

 

How to cite: Ren, J. and Huang, C.: Impact of the Snowfall and Snow Properties Predictions with Multiple Data Assimilation Strategies Digesting GPM Precipitation and Himawari-8/AHI water vapor radiance into Reg_NWPs over TP plateau , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6026, https://doi.org/10.5194/egusphere-egu25-6026, 2025.

EGU25-8377 | ECS | Posters on site | CR5.1

Evaluation of simulated snow inside forests using measured ground temperature 

Brage Storebakken, Erwin Rottler, Michael Warscher, and Ulrich Strasser

Forests influence the inside-canopy snow dynamics in various ways depending on topography and the prevailing climate. Understanding how forest effects on snow change with climate variability and climate change is essential for predicting the future role of forests for seasonal snow dynamics. Thereby location-specific studies, such as the one presented here, provide valuable insights into forest-snow interactions within particular regions. In this study, the physically-based and fully distributed snow model openAMUNDSEN, was used to simulate the seasonal snow cover evolution in the Berchtesgaden National Park, Bavaria, Germany. This area is characterized by significant elevation differences (ranging up to 2000 meters within a 3.5 km distance) and offers an ideal setting to examine how forest-snow interactions vary across complex mountain terrain. The model is forced with meteorological data collected from 20 automatic weather stations located in open areas and distributed across different elevations. Simulations were conducted at a spatial resolution of 50 x 50 meters. The temperature at 10 cm ground was measured by 150 temperature-moisture sensors positioned within the forest. These sensors are deployed across various elevations and forest densities. Using these measurements, snow cover duration and snow disappearance date were derived for forested plots and used to evaluate the simulated snow cover. The results indicate that observed and simulated snow metrics generally show consistent patterns within the forested regions of the study area, though some deviations were observed at specific locations. The presented investigations contribute to a more detailed understanding of forest-snow interactions in mountainous environments.

How to cite: Storebakken, B., Rottler, E., Warscher, M., and Strasser, U.: Evaluation of simulated snow inside forests using measured ground temperature, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8377, https://doi.org/10.5194/egusphere-egu25-8377, 2025.

EGU25-9709 | ECS | Orals | CR5.1

Modelling Meltwater Infiltration and Refreezing in Snow under Non-Isothermal Conditions 

Camilla Crippa, Alessio Fumagalli, Anna Scotti, Monica Papini, and Laura Longoni

The flow of meltwater through snow, acknowledged as a porous medium, is a crucial hydrological process essential for predicting the cryosphere’s response to climate change. This work aims to model the intricate coupling between meltwater infiltration and the non-equilibrium thermodynamics of ice-melt phase change at the Darcy scale. The proposed model consists of the Richards’ equation for infiltration, and evolution equations for ice and water temperature fields, which account for the thermal budget resulting from melt refreezing. Additionally, the model takes into account variations in porosity within the ice structure. The study presents numerical results from simulations conducted on 2D models of snowpacks with distinct initial levels of dryness and varying physical setups, which examine the mechanics of infiltration and alteration of the porosity structure due to refreezing. The implementation employs the PorePy and PyGeoN Python libraries.

How to cite: Crippa, C., Fumagalli, A., Scotti, A., Papini, M., and Longoni, L.: Modelling Meltwater Infiltration and Refreezing in Snow under Non-Isothermal Conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9709, https://doi.org/10.5194/egusphere-egu25-9709, 2025.

EGU25-9995 | ECS | Posters on site | CR5.1

Insights of the seasonal evolution of an arctic snowpack from an intensive field campaign 

Lisa Bouvet, Neige Calonne, Pascal Hagenmuller, Laurent Arnaud, Oscar Dick, Kévin Fourteau, Mathieu Fructus, Daniel Kramer, Alexandre Langlois, Yves Lejeune, Julien Meloche, Jacques Roulle, Arvids Silis, Louis Védrine, Vincent Vionnet, and Marie Dumont

The Arctic snowpack covers a large portion of the Earth’s surface, yet detailed snow observations in these areas are sparse compared to observations in alpine environments. The Arctic presents unique environmental conditions, leading to thin snowpacks undergoing high-temperature gradients. These conditions lead to specific evolutions of the snow microstructure, which results in peculiar snowpack properties. To improve our understanding and description of the Arctic snowpack, an eight-month-long field campaign (IVORI) was conducted in Cambridge Bay at the Canadian High Arctic Research Station, Nunavut, Canada (69°N) during the 2023-2024 winter. The campaign is based on daily acquisitions of the 3D snow microstructure at 10 μm using a cold laboratory X-ray tomograph located next to the field site, along with extensive monitoring of the meteorological conditions and traditional snow characterizations. This dataset notably contains 200 tomographic samples and 50 snow stratigraphic profiles covering the full snow depth.

Here we present the specific climatic context of the 2023-2024 winter at Cambridge Bay, along with an analysis of the evolution of the vertical profiles of density and specific surface area. Finally, a preliminary overview of the performance of snow models at this Arctic location is given, highlighting potential areas for improvement.

How to cite: Bouvet, L., Calonne, N., Hagenmuller, P., Arnaud, L., Dick, O., Fourteau, K., Fructus, M., Kramer, D., Langlois, A., Lejeune, Y., Meloche, J., Roulle, J., Silis, A., Védrine, L., Vionnet, V., and Dumont, M.: Insights of the seasonal evolution of an arctic snowpack from an intensive field campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9995, https://doi.org/10.5194/egusphere-egu25-9995, 2025.

EGU25-10482 | Posters on site | CR5.1

Intensive field campaign on snow microstructure evolution at a low-elevation alpine site 

Neige Calonne, Pascal Hagenmuller, Rémi Granger, Lisa Bouvet, Kévin Fourteau, Julien Brondex, François Tuzet, Yves Lejeune, Anne Dufour, Mathieu Fructus, and Marie Dumont

Dataset of snowpack properties combined with atmospheric forcing are necessary to evaluate snow models. Here, we followed the evolution of the snowpack at Col de Porte, a regular snow observation site located near Grenoble at 1350 m, with detailed measurements of the snow microstructure and related properties. The goals were 1/ to test the feasibility of using X-ray tomography for regular snowpack monitoring, 2/ to carry out an inter-comparison of different instruments for density and specific surface area (SSA) measurements, and 3/ to provide new dataset of snow properties including snow microstructure and meteorological forcing for model driving and evaluation for a low-elevation alpine environment. Over the winters 2021-2022 and 2022-2023, the standard observation program was complemented by SnowMicroPen measurements, SSA measurements with two optical instruments (DUFISSS and HISSGraS), and 3D imaging using a cold laboratory X-ray tomograph located next to the snow field. Measurements were performed weekly to bi-weekly. For tomography, snow were collected in cylinders of 4 cm diameter and 15 cm height. The scans were performed at two resolutions: 10 microns (50 min scan per cm) and 42 microns (3 min scan per cm). We present the evolution of the snowpack in relation to the weather conditions. Snow heights were well below average for the second winter, with several total snowpack disappearances, from mid-February on. Both winters showed regular rain-on-snow and melt events throughout the winter, offering suited data to evaluate wet snow and liquid water flow in models, especially. An inter-comparison of density and SSA estimates from tomography, SnowMicroPen and optical instruments is provided. Finally, we present a preliminary comparison of the snowpack evolution between measurements and the snowpack model Crocus.

How to cite: Calonne, N., Hagenmuller, P., Granger, R., Bouvet, L., Fourteau, K., Brondex, J., Tuzet, F., Lejeune, Y., Dufour, A., Fructus, M., and Dumont, M.: Intensive field campaign on snow microstructure evolution at a low-elevation alpine site, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10482, https://doi.org/10.5194/egusphere-egu25-10482, 2025.

EGU25-10619 | ECS | Posters on site | CR5.1

Simulating snow properties and Ku-band backscatter across the forest-tundra ecotone 

Georgina Woolley, Nick Rutter, Leanne Wake, Vincent Vionnet, Chris Derksen, Julien Meloche, Benoit Montpetit, Gabriel Hould Gosselin, Richard Essery, and Philip Marsh

Sophisticated snowpack models are required to provide accurate estimation of snowpack properties across the forest-tundra ecotone where in situ measurements are rare. As snowpack properties strongly influence radar scattering signals, accurate simulation is crucial for the success of spaceborne radar missions to retrieve snow water equivalent (SWE). In this study, we evaluate the ability of default and Arctic Crocus embedded within the Soil, Vegetation and Snow version 2 (SVS2-Crocus) land surface model to simulate snowpack properties (e.g. depth, density, SWE, specific surface area) across a 40-km transect of the Northwest Territories, Canada, using two winter seasons (2021-22 & 2022-23) of in situ measurements. An ensemble of simulated snowpack properties (120 members from default and Arctic SVS2-Crocus) were used in the Snow Microwave Radiative Transfer (SMRT) model to simulate Ku-band (13.5 GHz) backscatter. SMRT backscatter using multi-layer SVS2-Crocus snowpack simulations were compared to backscatter using a simplified 3-layer radar-equivalent snowpack. Results highlight that Arctic SVS2-Crocus wind-induced compaction modifications were spatially transferable across the forest-tundra ecotone and lead to an improvement in the simulation of surface snow density at all sites, reducing the RMSE of surface density by an average of 29%. The parameterisation of below-canopy wind speed limits the ability of SVS2-Crocus to increase surface density to match measurements, despite the inclusion of Arctic modifications and should be revised for sparse (e.g. canopy densities < 15 %) canopy environments. Basal vegetation modifications were less effective in simulating low-density basal snow layers at all sites (default RMSE: 67 kg m-3; Arctic RMSE: 69 kg m-3) but were necessary to simulate a physically representative Arctic density profile. SVS2-Crocus underestimated snow specific surface area (SSA) leading to high errors in the simulation of snow backscatter (default RMSE: 3.5 dB; Arctic RMSE: 5.3 dB). RMSE of backscatter was reduced by implementing a minimum SSA value (8.7 m2 kg-1; default RMSE: 1.4 dB; Arctic RMSE: 1.3 dB) or by scaling the scattering effects of the snowpack (polydispersity: 0.63; default RMSE: 1.6 dB; Arctic RMSE: 2.6 dB). Utilising a radar-equivalent snowpack was effective in retaining the scattering behaviour of the multi-layer snowpack (RMSE < 1 dB) providing a means to monitor SWE with reduced computational complexity.

How to cite: Woolley, G., Rutter, N., Wake, L., Vionnet, V., Derksen, C., Meloche, J., Montpetit, B., Hould Gosselin, G., Essery, R., and Marsh, P.: Simulating snow properties and Ku-band backscatter across the forest-tundra ecotone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10619, https://doi.org/10.5194/egusphere-egu25-10619, 2025.

Precipitation and snowmelt from the Andes Cordillera are vital water resources for downstream communities and ecosystems, particularly in Central Chile, where agricultural water demands peak during hot, dry summers—out of sync with the winter precipitation regime. The snowpack serves as a natural reservoir, delaying water release; however, warmer temperatures are shifting precipitation patterns from snow to rain and accelerating snowmelt, potentially undermining the snowpack’snatural storage capacity. Understanding the vulnerability of this natural reservoir to climate warming is critical. In this study, we employ the Weather Research and Forecasting (WRF) model, configured for convective-permitting simulations over South America (WRF-SAAG), to analyze snowpack dynamics under current and future climate conditions. We simulate a moderate-to-high socioeconomic scenario (SSP3.7.0) over a 22-year period and compare model outputs with observations from high-elevation hydrometeorological stations in Chile and Argentina. Results show reasonable agreement in snow water equivalent (SWE) timing and magnitude, though mean monthly precipitation is overestimated by ~20%. We calculate the Snow Storage Index (Hale et al., 2023) for both historical (2000–2021) and future (2060–2080) periods, assessing its temporal and spatial variability at both grid (4 km) and catchment scales. We also analyze key snowpack characteristics, including peak SWE, duration, and melt rates, highlighting projected reductions in natural storage capacity across the Southern Andes. This research enhances our understanding of snow dynamics in a region with complex topography and varying climatic conditions. Findings are crucial for policymakers and water managers, providing essential insights for developing climate adaptation strategies in the Southern Andes foothills, an area of growing societal importance yet relatively understudied.

How to cite: Scaff, L. and Krogh, S.: Quantifying the vulnerability of the natural storage capacity of the Andes Cordillera snowpack using a 4-km convection-permitting regional climate model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14003, https://doi.org/10.5194/egusphere-egu25-14003, 2025.

We investigated the effect of formed snowdrifts in advance on the turbulent flow and subsequent snowdrift distribution in a numerical simulation. We conducted an ideal numerical simulation for snowdrift distribution around three types of snow fences: two-dimensional fence, three-dimensional fence, and two-dimensional fence with a bottom gap. Snowdrifts resulting from an 8-hour drifting snow event were estimated by dynamically updating the bottom boundary conditions every 2 hours to reflect the developed snowdrift structures. Compared to simulation without boundary updates, snowdrift height on windward side of the two-dimensional fence was higher in the updated simulation. This increase was attributed to the weakened wind speed and modified snow particle trajectories around the previous snowdrifts. For the three-dimensional and bottom-gap fences, significant differences of snowdrift height were observed on the leeward areas between the updated and no-updated simulations. Snowdrifts on the leeward side of these fences were formed further downstream in the no-updated simulation. In contrast, the updated simulations generated snowdrifts closer to the fence on the leeward side. These findings suggested that neglecting the impact of the previous snowdrift structures in numerical simulation could lead to an overestimation of snowdrift development on the leeward side of obstacles.

How to cite: Tanji, S.: Estimating the effect of pre-existing snowdrift on turbulent airflow and subsequent snowdrift in the numerical simulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14098, https://doi.org/10.5194/egusphere-egu25-14098, 2025.

EGU25-15329 | ECS | Posters on site | CR5.1

Investigating the potential of snow liquid water content retrieval from near-infrared reflectance measurements 

Valentin Philippe, Lars Mewes, and Benjamin Walter

Assessing snow melt and the liquid water content (LWC) of snow is crucial for understanding the hydrological cycle for predicting water resources, hydroelectric power generation, runoff, and potential flooding. It is also essential for correcting remote sensing signals (RADAR) and forecasting wet snow avalanches, for which snow stability is closely linked to its water content. Various methods exist to measure snow LWC, including calorimetry techniques, centrifugal separation, and dielectric methods based on permittivity differences between ice, air, and water. While these methods are well established, they are limited to low sampling resolutions and do not capture the typically high spatial variability of liquid water within the snowpack. However, Donahue et al. recently (2022) demonstrated the potential of near-infrared (NIR) spectral imaging for visualizing the 2D spatial variability of snow wetness in their study, Mapping Liquid Water Content in Snow at the Millimeter Scale: An Intercomparison of Mixed-Phase Optical Property Models Using Hyperspectral Imaging and In Situ Measurements (The Cryosphere).

The SnowImager instrument (snowimager.ch), recently developed at the Institute for Snow and Avalanche Research (WSL/SLF) together with a local start-up (Davos Instruments), allows for measuring the 2D spatial NIR diffuse-reflectance of snow stratigraphies at wavelengths of 850 nm and 940 nm. Leveraging the fact that reflectance at 850 nm is less influenced by liquid water than at 940 nm, we explore the application of NIR diffuse-reflectance imaging for measuring 2D LWC distribution with the SnowImager. As a first step, we developed a wetness index based on the reflectance measurements, and which is proportional to the LWC. Because the NIR diffuse-reflectance also depends on the optical equivalent grain diameter, a baseline dry reflectance ratio was determined using dry snow samples collected over the winter season 2023/2024. In addition, field measurements (in Weissfluhjoch test site and in Tschuggen during the melt season) were carried out to compare the wetness index against conventional liquid water content measurements obtained with a capacitive sensor.

Results from the Tschuggen campaign exhibit good agreement between the wetness index and the LWC measurements with the capacitive sensor for the snowpack wetness evolution. Furthermore, the imaging approach demonstrates the ability of capturing high resolution 2D variability of the LWC within a snowpack. Although the findings are promising, limitations were identified at snow microstructure regions of high textural contrasts. Further research is required to validate the wetness index method comprehensively, particularly concerning the characterization of the baseline reflectance ratio.

How to cite: Philippe, V., Mewes, L., and Walter, B.: Investigating the potential of snow liquid water content retrieval from near-infrared reflectance measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15329, https://doi.org/10.5194/egusphere-egu25-15329, 2025.

EGU25-16197 | ECS | Orals | CR5.1 | Highlight

Drifting Snow around Icebergs: Understanding the Role of Iceberg Size and Shape Through Modeling and Observational Data 

Océane Hames, Iolène Bouzdine, Christian Haas, and Michael Lehning

The state of research on snow mass balance over sea ice has advanced in recent years, with significant progress in understanding the complex snow-ice interactions. However, challenges remain in accurately assessing the snow depth variability over sea ice in both space and time, particularly when considering the effect of snow transport by wind. In Antarctica, the calving of ice shelves generates icebergs that get trapped in landfast sea ice and act as obstacles to drifting snow. By accumulating snow around them, icebergs may influence the dynamics of land-fast ice in coastal areas but their precise impact on the mass balance and spatial distribution of snow remains uncertain. Drifting snow models are valuable for isolating the geometric properties of obstacles and independently examining their impact on snowdrifts. In our study, we investigate the effect of iceberg geometry on snowdrift quantities by combining aerial laser scanner observations and numerical Euler-Lagrange simulations. Properties such as iceberg size, roundness and elongation were evaluated and the model outcome was compared to the observations. Results show that the size of icebergs governs the snowdrift quantities, while other shape characteristics mostly affect the snow distribution across the iceberg sides. A new scaling law has been discovered, revealing a clear power-law relationship between the size of snowdrifts and icebergs. Our work improves the understanding of drifting snow processes over Antarctic land-fast ice, particularly the impact of large-scale features on the snow distribution. It can offer deeper insights into the comparison of regions with small and large icebergs, along with their associated land-fast ice characteristics and help to quantitatively predict sea ice dynamics.

How to cite: Hames, O., Bouzdine, I., Haas, C., and Lehning, M.: Drifting Snow around Icebergs: Understanding the Role of Iceberg Size and Shape Through Modeling and Observational Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16197, https://doi.org/10.5194/egusphere-egu25-16197, 2025.

EGU25-16255 | ECS | Orals | CR5.1

Monitoring dry snow metamorphism from in-situ tomographic measurements 

Oscar Dick, Neige Calonne, Pascal Hagenmuller, and Benoît Laurent

Snow physical properties result from the complex 3D arrangement of ice and air at the micrometre scale, referred to as snow microstructure. Describing snow microstructure and predicting its temporal evolution are keys for snowpack models, such as CROCUS or SNOWPACK. Currently, the evolution laws of density and SSA in both models are not fully satisfactory, as shown by some model errors when compared to observations. For example, SSA of new snow simulated on CROCUS tends to decrease faster than what is observed experimentally, while the inverted density profile due to strong gradient metamorphism observed in arctic snowpacks is not captured by CROCUS. These limitations result partly from the fact that evolution laws were empirically derived from experimental time series covering a limited number of snow evolution scenarios, and whose temporal and spatial resolutions could be enhanced.

X-ray tomography has brought new insights into snow microstructure observation, enabling a quantitative assessment of its variations and a deeper understanding of the physical processes at the micrometer scale. While first measurements were made at room temperature and required to fix the microstructure evolution with impregnation, the use of micro-CT directly inside a cold lab offers the possibility to conduct extensive measurements of snow samples in a cold environment. In this work, we use micro-CT measurements to characterize the temporal evolution of microstructural properties of snow under dry snow metamorphism. To do so, we designed a snow-metamorphism cell to control the temperature at the upper and lower boundaries of a cylindrical snow sample of size 1.8 cm x 2 cm2. This cell can operate directly inside the tomograph and offers the possibility to conduct in-situ monitoring under various experimental conditions. We explored temporal evolutions for different initial snow types, mean temperatures, and temperature gradients ranging from isothermal condition up to 200 K/m. From the micro-CT measurements, we calculate the microstructure properties and analyze their temporal evolution. We also explore the relationships between characteristic lengths, such as ssa, correlation length, mean chord length, and curvature length. In this work, we present the preliminary results from a selection of experiments. The long-term objective is to produce highly resolved time-series with systematic variations of the experimental conditions, and to monitor the evolution of the snow microstructural properties in order to compare them to existing evolution laws and suggest improvements if needed.

How to cite: Dick, O., Calonne, N., Hagenmuller, P., and Laurent, B.: Monitoring dry snow metamorphism from in-situ tomographic measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16255, https://doi.org/10.5194/egusphere-egu25-16255, 2025.

In mountains, wind- and gravity-driven transport of snow affects the overall distribution of snow and can have a significant effect on snowmelt dynamics. In the context of the Swiss operational snow melt forecasting, a compromise must be found to enable the representation of such small-scale processes over the entire Swiss Alps while maintaining viable computational costs.

To this end, the snow redistribution modules SNOWTRAN-3D and SnowSlide were implemented and adapted within the FSM2oshd physics-based snow cover model. In an earlier study we showed the added value of snow redistribution representations on a 1180 km2 domain within the Eastern Swiss Alps when running simulations at 25, 50 and 100 m spatial resolutions. Here, we present the challenges and developments that are needed to apply this research model successfully over the whole Swiss Alps at 100 m resolution in an operational setting. In particular, we discuss the following issues:

- The Swiss Alps include very high elevations, with summits above 4000 m.a.s.l. and glaciers. Transport parameters that were shown to be suitable for terrain at 2500 m.a.s.l. are not applicable in more extreme conditions and need diversification.

- Wind fields, although dynamically downscaled, need further post-processing to mitigate biases that became evident in comparison to wind station measurements, particularly on exposed ridges.

- The representation of snow redistribution and of forest snow processes have to be integrated as both types of processes coexist wherever open alpine terrain interfaces with subalpine forest.

- The snow cover fraction scheme has to be adapted to better account for snow transport processes and sub-grid variability in simulations at high spatial resolution.

How to cite: Quéno, L., Jonas, T., Mazzotti, G., and Magnusson, J.: Including snow redistribution in snow hydrology modelling: challenges and developments to make a research model operational at nation-scale , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17090, https://doi.org/10.5194/egusphere-egu25-17090, 2025.

EGU25-17427 | ECS | Posters on site | CR5.1

Learning to filter: Snow data assimilation using a Long Short-Term Memory network 

Giulia Blandini, Francesco Avanzi, Lorenzo Campo, Simone Gabellani, Kristoffer Aalstad, Manuela Girotto, Satoru Yamaguchi, Hiroyuki Hirashima, and Luca Ferraris

In snow-dominated regions, today’s snow is tomorrow’s water, making reliable estimates of snow water equivalent (SWE) and snow depth crucial for water resource management. In this context, data assimilation is a powerful tool to optimally combine models and measurements, enhancing accuracy and reliability. Ensemble-based techniques like the Ensemble Kalman Filter (EnKF) and Particle Filter (PF) are often used but their deployment in real-time applications can make it challenging to ensure timely and accurate results. To address these challenges, we propose an innovative data assimilation framework for snow hydrology that leverages Long Short-Term Memory (LSTM) networks. Using data from seven diverse study sites across the Northern Hemisphere, our framework is trained on the outputs of an EnKF, persuing a balance between computational efficiency and model complexity to advance data assimilation applications in snow hydrology. This LSTM-based framework achieves performance comparable to the EnKF in improving open-loop estimates, with only minor increases in root-mean-square error (RMSE): +6 mm for SWE and +6 cm for snow depth on average. Adding a memory component enhances stability and accuracy, especially under sparse data conditions. When trained on long-term datasets spanning 25 years, the LSTM framework demonstrated promising spatial transferability, with accuracy reductions of less than 20% for snow water equivalent and snow depth estimation. After training, the LSTM approach significantly outperformed a parallelized EnKF in computational efficiency, reducing runtime by 70% while maintaining comparable accuracy. Training on multi-site data further ensured robust performance across diverse climate regimes and during both dry and average water years, with a modest RMSE increase compared to the EnKF (+6 mm for SWE and +18 cm for snow depth). By combining the strengths of traditional ensemble methods and modern machine learning, this framework offers a scalable, computationally efficient, and reliable alternative for operational snow hydrology data assimilation.

 

How to cite: Blandini, G., Avanzi, F., Campo, L., Gabellani, S., Aalstad, K., Girotto, M., Yamaguchi, S., Hirashima, H., and Ferraris, L.: Learning to filter: Snow data assimilation using a Long Short-Term Memory network, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17427, https://doi.org/10.5194/egusphere-egu25-17427, 2025.

EGU25-17643 | Orals | CR5.1

Calibrating a compressible firn rheology and application to firn in shear zones 

Aslak Grinsted, Nicholas Mossor Rathmann, and Christine Hvidberg
Most existing firn densification models are one-dimensional and empirical, limiting their ability to accurately represent complex stress regimes. For instance, they fail to account for enhanced densification in shear zones. In contrast, the Gagliardini and Meysonnier 1997 (GM97) model offers a more comprehensive approach by incorporating a compressible firn rheology. This allows modelling densification under arbitrarily complex stress regimes. Unfortunately this model not as constrained empirically, and less practical to implement in a typical one dimensional use case. Here we report on progress on bridging the gap in the firn model hierarchy. How can the GM97 model be reformulated so that it can be used in 1D models, such as the Community Firn Model, while still accounting for horizontal shear? How can we calibrate the model so that it performs as well as simpler models without case by case tuning?

How to cite: Grinsted, A., Rathmann, N. M., and Hvidberg, C.: Calibrating a compressible firn rheology and application to firn in shear zones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17643, https://doi.org/10.5194/egusphere-egu25-17643, 2025.

EGU25-18277 | ECS | Posters on site | CR5.1

Spatial-variability of snow surface and snowpack properties characterized by near-infrared diffuse reflectance imaging 

Lars Mewes, Valentin Philippe, Martin Schneebeli, Henning Löwe, and Benjamin Walter
Near-infrared diffuse reflectance imaging is well-suited to accurately characterize macro- and microscopic properties of snow.1 The technique's versatility and capability to resolve details down to the millimeter-scale, while simultaneously capturing areas up to a few square-meters, renders it ideal for ground-truth observations of snow surfaces and its stratigraphic structure. Specific surface area, density, as well as liquid water content properties are readily derived from the measured reflectance data using snow-optical theory.2-6
 
We present recent results of surface and snowpack measurements obtained during field-campaigns in the Swiss Alps, the Arctic and the Antarctic, focusing on spatial-variability on the centimeter to meter scale. These insights provide valuable information to established measurement techniques that sample one-dimensional profiles only and thus lack the additional spatial information. Moreover, especially the surface measurements provide small scale details that are averaged-out in remote sensing data from drones, planes and satellites.
 
Using near-infrared diffuse reflectance imaging enables us to observe spatio-temporal variations of snow properties on the centimeter to meter scale, providing important ground-truth observations to better gauge the snow's role within the climate system.
 
1. Matzl, M. & Schneebeli, M., J. Glaciol. 52, 558–564 (2006).
2. Mewes, L. et al., under review.
3. Donahue, C. et al., The Cryosphere 16, 43-59 (2022).
4. Bohren, C. F. & Barkstrom, B. R., J. Geophys. Res. 79, 4527–4535 (1974).
5. Warren, S. G., Rev. Geophys. 20, 67 (1982).
6. Kokhanovsky, A. A. & Zege, E. P., Appl. Opt. 43, 1589 (2004).

How to cite: Mewes, L., Philippe, V., Schneebeli, M., Löwe, H., and Walter, B.: Spatial-variability of snow surface and snowpack properties characterized by near-infrared diffuse reflectance imaging, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18277, https://doi.org/10.5194/egusphere-egu25-18277, 2025.

The snow depth and the increase of snow depth after three consecutive days of snowfall, hereinafter referred to as ds and DH3gg, respectively, are typically chosen for avalanche protection and avalanche hazard assessment purposes. With specific reference to the Central Apennines (Central Italy), the preferable provider of observations for avalanche related applications is MeteoMont, which supplies ds observations at 34 manual stations, measured between 1978 and 2023. The area of interest is also covered by ERA5-Land, over a period of 73 years, from 1950 to 2023. In terms of temporal, spatial and quantitative availability of snow information, ERA5-Land consists in a more appealing choice as most manual weather stations set up in the Central Apennines are located at lower altitudes compared to where avalanches are likely to occur. Moreover, data recorded at manual stations appears to be incomplete, especially during extreme snowfall events. However, it is necessary to stress that ERA5-Land is affected by biases (e.g. underestimation or overestimation of extremes) and the use of uncorrected data in all applications might lead to unreasonable results. Therefore, in order to overcome the listed limitations, the suggested approach consists in the regionalisation of both ERA5-Land and MeteoMont ds and DH3gg and in the subsequent bias correction and downscaling of the regionalised ERA5-Land variables by means of the regionalised MeteoMont ones. With regards to ERA5-Land, 51 nodes have been considered as their grids intersect recorded and reconstructed avalanche paths in the Abruzzo Region (extracted from the Avalanche Record and the Map of Probabilistic Location of Avalanches provided by the Abruzzo Region). This ensures that the selected nodes are solely representative of areas where avalanches are most likely to occur. The regionalisation of both ERA5-Land and MeteoMont ds and DH3gg is performed by applying the index value regional method before the bias correction and the downscaling of ERA5-Land data as, in terms of computational efforts, only 2 bias corrections and downscalings for each couple of best-matched ERA5-Land and MeteoMont homogeneous areas would be required instead of 102 (2 for each couple of nodes and stations). The bias correction and downscaling of the ERA5-Land regionalised variables are then performed by means of a statistical transformation based on the assumption that said variables are described by one of the distributions belonging to the GEV family. This work is of particular relevance as, on the one hand, it overcomes the limited availability of snow information in the Central Apennines, especially in relation to avalanche related applications. In fact, it provides a tool that quantifies ds and DH3gg quantiles at elevations and sites that are not supplied with observations. On the other hand, it provides realistic initial and boundary conditions for simulating avalanche dynamics, drawing up hazard and risk maps, and designing active and/or passive defence structures. 

How to cite: Fontana, S., Pasquali, D., and Di Risio, M.: Regionalisation, Bias Correction and Downscaling of ERA5-Land Snow Variables by Means of Local Observations Recorded in Central Italy , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19323, https://doi.org/10.5194/egusphere-egu25-19323, 2025.

EGU25-20052 | Posters on site | CR5.1

Snow Microstructure over Antarctic Landfast Ice 

Ruzica Dadic, Julia Martin, Roberta Pirazzini, Brian Anderson, Martin Schneebeli, Matthias Jaggi, Amy Macfarlane, Michael Lehning, Nander Wever, and Petra Heil
Landfast ice plays a significant role in climate and ecosystems in Antarctic coastal regions. From October to December 2022, we investigated the physical properties of snow and sea ice on Antarctic landfast ice in McMurdo Sound, following the protocols from the MSOAiC expedition. Our measurements confirmed some findings from MOSAiC (e.g. the potential mass transfer from the sea ice surface to snow , the high spatial variability of snow depth}, and the discrepancy between meteorological snowfall and snow accumulation),  but we also had observations that were contrasting our MOSAiC data, for example: 1) presence of salt up to 15 cm of snow height (as opposed to MOSAiC's 5 cm for a relatively similar total snow height), 2) the lack of the surface scattering layer on melting sea ice, which caused significantly lower albedos of bare sea ice (0.45, as opposed to MOSAiC's 0.65), 3) average densities of non-melting snow of 450 kg/m3 (as opposed to MOSAIC'S 350 kg/m3 ). Here, we will discuss the microCT measurements from our samples and relate them to the macroscale obervations of parameters like snow density, snow height, snow surface roughness, salinity or stable water isotopes. The main focus in this study in on the prevalance of a prominent depth hoar layer at the snow-ice interface, which we to be caused by the mass transfer between snow and ice because of the large vertical temperature gradients. This is also visible by the microscale roughness of the interface. Additionally, we will discuss the microstructure of the extremely dense wind slab that dominates most of the snow profile and the implications of these findings for modelling and remote sensing of snow on sea ice. 
 
 

How to cite: Dadic, R., Martin, J., Pirazzini, R., Anderson, B., Schneebeli, M., Jaggi, M., Macfarlane, A., Lehning, M., Wever, N., and Heil, P.: Snow Microstructure over Antarctic Landfast Ice, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20052, https://doi.org/10.5194/egusphere-egu25-20052, 2025.

EGU25-21697 | ECS | Posters on site | CR5.1

Firn densification across the Greenland Ice Sheet from the IMAU-FDM (1940-2023) 

Elizabeth Case, Peter Kuipers-Munneke, Max Brils, Willem-Jan van de Berg, Carleen Tijm-Reijmer, and Michiel van den Broeke

The IMAU Firn Densification Model (IMAU-FDM) is a 1D, semi-empirical model that simulates the evolution of snow grain size, firn density, firn air content, temperature, and liquid water content. It has been used primarily to investigate future surface changes over both Greenland and Antarctica, as well as for continent-wide estimates of mass change from satellite altimetry. Here, we will present a streamlined, updated IMAU-FDM with results for the Greenland Ice Sheet extended back to 1940 and through to 2023. IMAU-FDM is driven by ERA5, dynamically downscaled by the regional climate model RACMO 2.3p2 to 5.5 km^2 resolution. We will present timeseries of firn air content, liquid water content, and ice slab presence across the Greenland Ice Sheet, and initial results of future runs through 2100.

How to cite: Case, E., Kuipers-Munneke, P., Brils, M., van de Berg, W.-J., Tijm-Reijmer, C., and van den Broeke, M.: Firn densification across the Greenland Ice Sheet from the IMAU-FDM (1940-2023), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21697, https://doi.org/10.5194/egusphere-egu25-21697, 2025.

Determination of the reliable estimate of risk associated with hydrometeorological extremes over a region requires discerning information on spatial variability of the associated at-site statistics/parameters. Extreme rainfall at finer spatio-temporal resolution allows for improved analysis of spatial variability, as local-scale statistical similarities (LSS) and heterogeneities are disclosed. The knowledge of LSS facilitates the use of information on regional spatial variability (in lieu of complex at-site spatial variability) for risk analysis. In addition, it is established in literature that geographical features influence the occurrence of extreme rainfall over an area. For a subcontinent with complex non-uniform patterns of geographical features, the regional spatial variability may be influenced by the geographic composition. To quantify this regional spatial variability, statistically homogenous regions need to be deciphered. Most studies on the regionalization of sub-daily extreme rainfall (SDER) are limited to a smaller spatial extent, and none was focused on a subcontinent. Furthermore, there are no prior studies focused on the analysis of regional spatial variability of SDER. To study the role of geography in modulation of the regional spatial variability of mesoscale SDER, the present study proposes a framework. It involves (i) dividing the study area into subareas based on geographical features, as they are deemed to influence the occurrence of extreme rainfall, (ii) the delineation of each subarea into statistically homogenous SDER regions using a novel regionalization technique, (iii) quantification of the regional spatial variability of SDER in each subarea using the delineated regions and a proposed novel index, and (iv) identifying the role of geographic features in modulating the regional spatial variability. The efficacy of the proposed framework is demonstrated by application to Indian subcontinent (66.5-100o E, 6.5-38.5o N) considering 0.12o resolution SDER data corresponding to different durations (1,2,3,6 and 12-hour) for the period 1981-2020. The data were prepared by bias correcting the 0.12o resolution NCMRWF IMDAA hourly gridded rainfall (at 20,717 grids) to be consistent with the widely used 0.25o resolution IMD (India Meteorological Department) daily rainfall. The Indian subcontinent is divided into seven subareas based on geographic features. On application of the framework, it has been found that the regional spatial variability of SDER in a subarea is regulated by its geography and that of its neighbouring subareas. Insights are obtained on the effect of factors such as orography and coastal width on regional spatial variability of SDER. The study is of significance as the knowledge discerned on potential covariates/attributes has wide applications including identification of similar extreme rainfall sites for regional frequency analysis for extreme rainfall and risk assessment of consequent floods at ungauged/sparsely gauged hotspots such as water control (e.g., dams, barrages, levees) and conveyance infrastructure (culverts) in river basins under various climate change scenarios. The inherent physio-geographic features of the catchment may not be enough to analyze the similarity with neighbouring catchments. The boundary conditions around the catchment also plays a role. 

How to cite: Varshney, A. and Srinivas, V. V.: A New Framework for Quantification of Regional Spatial Variability of Mesoscale Sub-daily Extreme Rainfall for Subcontinent , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1068, https://doi.org/10.5194/egusphere-egu25-1068, 2025.

Climate change intensifies the global hydrological cycle, altering hydrometeorological variables and amplifying flood risks, with significant social, economic, and environmental consequences. Reliable flood estimates are crucial for designing cost-effective flood protection structures. The assessment often focusses only on peak discharge, overlooking vital factors like flood wave frequency, duration, and time to peak, which are key elements for preparedness and resilience. Although. the use of general circulation models (GCMs) for future simulations has advanced our understanding of catastrophic floods under climate change. Yet, the socio-economic impacts of these events remain insufficiently explored, leaving crucial vulnerabilities inadequately addressed. This study therefore evaluates the flood characteristics and socio-economic vulnerabilities in a large river basin using downscaled GCMs of CMIP6. The hydrological and hydrodynamic models were used for determining the flood wave characteristics considering non stationarity. We also examine the benefits of limiting global warming to 1.5°C, aligned with COP28 goals, by assessing global warming levels of 1.5°C, 2°C, and 3°C and the EF (2021–2050) and FF (2071–2100).

The flood peaks in major cities are projected to rise by 10–14% during pre-monsoon and monsoon seasons, with high-warming scenarios causing a ~35% increase in high flow by 2100. However, limiting the warming to 1.5°C could reduce the return flood discharge by 9,000 m³/s in FF. The projections indicate a paradigm shift in the flood wave characteristics of the basin, with a notable increase in both flood wave duration (~0.31 days per year) and frequency (~3 more flood waves) during the pre-monsoon and monsoon seasons. Socio-economic vulnerability assessments reveal heightened risks under high-warming scenarios, driven by population growth and intensified hydroclimatic extremes, leading to greater inundation extents, depths, and displacement risks. These findings underscore the urgent need for global and regional cooperation, evidence-based policies, and climate-resilient infrastructure to mitigate flood risks and adapt to evolving hydroclimatic extremes in vulnerable transboundary basins.

How to cite: Gupta, R. and Chembolu, V.: Flood Vulnerability under High-Warming Scenarios: Insights from flood wave Projections and Socio-Economic Assessment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1079, https://doi.org/10.5194/egusphere-egu25-1079, 2025.

EGU25-1255 | ECS | Posters on site | HS7.5

Sources and characteristics of short-duration heavy convective precipitation events in the southeastern Alpine forelands 

Stephanie Haas, Nadav Peleg, Gottfried Kirchengast, and Jürgen Fuchsberger

Severe short-duration thunderstorms are a characteristic part of summer rainfall in the southeastern Alpine forelands. These heavy convective precipitation events (HCPEs) pose a severe risk to the region in the form of flash floods and landslides. Despite their crucial role in summer rainfall and natural hazards, the moisture sources and spatial structure of such HCPEs are still largely unknown.

The presented study links these highly localized events to large-scale processes to identify possible moisture source regions through backward trajectories obtained from Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model runs with ERA5 data. To complement this large-scale analysis, we use high-resolution data from the dense WegenerNet climate station network in southeastern Austria, to investigate the local characteristics and spatial structure of HCPEs.

The combination of large- and local-scale analysis results in a multi-faceted picture of HCPEs and their characteristics. We find that temperature is a key driver of HCPEs and that moisture from the Mediterranean region is a key influencing factor on the occurrence, magnitude, and spatial extent of such events in the study region. Furthermore, we find differences in the storm characteristics depending on the season and region of moisture source.

From a more general perspective, our findings imply that rises in temperature and humidity will likely result in more intense HCPEs with larger spatial extents, which potentially will increase the severity of floods and other natural hazards and hence also the damage risks in the southeastern Alpine forelands.

How to cite: Haas, S., Peleg, N., Kirchengast, G., and Fuchsberger, J.: Sources and characteristics of short-duration heavy convective precipitation events in the southeastern Alpine forelands, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1255, https://doi.org/10.5194/egusphere-egu25-1255, 2025.

EGU25-1636 | ECS | Posters on site | HS7.5

Regional Disparities in Hydro-climatic Extremes Across Central Asia: Insights from the Tienshan Mountains 

Xueqi Zhang, Yaning Chen, Zhi Li, Fan Sun, Yupeng Li, and Yifeng Hou

The Tienshan Mountains of Central Asia, a key region in global arid and semi-arid zones, faces highly uneven precipitation distribution due to its unique topography and climate. Precipitation variations significantly affect the region’s ecosystems, agriculture, and hydrological security. While extreme heavy precipitation has been widely studied, research on extreme light precipitation is limited. Additionally, spatial distribution patterns and driving mechanisms of extreme events under varying climatic and geomorphic conditions remain underexplored. This study systematically examines the spatial-temporal trends of extreme hydro-climatic events in the Tienshan Mountains, focusing on both heavy and light precipitation, to provide insights for water resource management and disaster prevention.

The Tienshan Mountains have experienced significant changes in extreme hydro-climatic events since 2000. The frequency anomaly of extreme light precipitation events (R1p) shifted from positive to negative, indicating a marked decline compared to the historical average, while extreme heavy precipitation events (R99p) shifted from negative to positive, reflecting a substantial increase in frequency. The intensity of both events has also risen notably during this period. Spatially, the intensity variations of extreme events show consistent signals across the Tienshan region, while frequency exhibits strong spatial heterogeneity. Around 80°E, extreme heavy precipitation frequency increases eastward and decreases westward. Vertically, mid-altitudes exhibit the most pronounced changes. The frequency of extreme light precipitation declines at 0.471 days/year in mid-altitudes compared to 0.356 days/year at high altitudes. Similarly, extreme heavy precipitation intensity increases at 0.106 mm/year in mid-altitudes, much higher than 0.014 mm/year at high altitudes. These patterns result from the combined effects of Tibetan Plateau thermal dynamics and monsoon-driven moisture transport, creating distinct differences in extreme precipitation between the eastern and western Tienshan. Future studies should explore the interactions between the plateau and atmospheric circulation to improve the prediction and mitigation of extreme events, aiding water resource management and disaster preparedness.

How to cite: Zhang, X., Chen, Y., Li, Z., Sun, F., Li, Y., and Hou, Y.: Regional Disparities in Hydro-climatic Extremes Across Central Asia: Insights from the Tienshan Mountains, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1636, https://doi.org/10.5194/egusphere-egu25-1636, 2025.

EGU25-1794 | ECS | Orals | HS7.5

Increasing typhoon risks in Shanghai under the effect of urbanization and sea surface temperature warming 

Qi Zhuang, Marika Koukoula, Shuguang Liu, Zhengzheng Zhou, and Nadav Peleg

Tropical cyclones, also known as typhoons in the western North Pacific, are one of the most devastating natural disasters in the world, especially when they strike highly urbanized regions with large populations. For instance, in September 2024, two typhoons, Bebinca and Pulasan, directly affected Shanghai within 4 days, resulting in severe floods, widespread power outages, and the evacuation of more than 500,000 residents. However, there is limited knowledge about the variability and mechanism of typhoon activities in this region under the effect of climate change and urbanization. In light of these facts, we use the Weather Research and Forecasting (WRF) convection-permitting model to simulate five typhoon events that made landfall along the southeastern coast of China and severely impacted Shanghai between 2018 and 2022. By comparing with various scenarios, including the current and projected expansion of Shanghai's urban area and the 1, 2, and 3 °C rise in sea surface temperature (SST), the effects of urbanization and climate change are estimated. The results find that typhoon tracks are significantly shifted southerly away from the city by higher SST, but the typhoon risk continues to increase due to substantial enhancement of rainfall intensity and wind velocity. Warmer SST increases air temperature and decreases sea level pressure, thereby facilitating the formation and development of typhoon sizes and their dynamic systems. The southward shift of the typhoon tracks is linked to the Fujiwhara effect when two typhoons exist and interact, causing an intensified mutual counterclockwise rotation with SST increase. Urbanization further intensifies the local rainfall intensity within Shanghai due to the increase in urban surface roughness. In the future, the risk of typhoons under the compound effects of urbanization and climate warming in Shanghai and other megacities in typhoon-affected regions should be raised to attention.

How to cite: Zhuang, Q., Koukoula, M., Liu, S., Zhou, Z., and Peleg, N.: Increasing typhoon risks in Shanghai under the effect of urbanization and sea surface temperature warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1794, https://doi.org/10.5194/egusphere-egu25-1794, 2025.

EGU25-1877 | ECS | Posters on site | HS7.5

Analysis of extreme precipitation timeseries in Serbia based on station data 

Lazar Filipovic, Ivana Tosic, Antonio Samuel Alves de Silva, Borko Stosic, Tatijana Stosic, and Vladimir Djudjevic

Serbia lies between Central and Southern Europe and is characterised by a complex topography, with the Pannonian Plain in the north and the Dinaric Alps in the west and southwest. Three climate types characterise Serbia: continental climate in the north, temperate continental climate in the central part and modified Mediterranean climate in the south. Precipitation in Serbia is generally the result of passing cyclones and associated atmospheric fronts as part of the general circulation of the atmosphere in the mid-latitudes (Tošić et al., 2017). In recent decades, flash flooding resulting from extreme precipitation events has proven to be a great threat to human life and a great cause of economic strife (an estimate of 1.7 billion euros in damages in 2014 alone when catastrophic flooding occurred in Bosnia, Croatia and Serbia).

The highest yearly 1-day precipitation (Rx1day) was analyzed on an annual and seasonal basis at ten stations in Serbia in the period 1961-2020. The modified Mann-Kendall test was used to examine the significance of the trend. An increase was observed in all annual time series of Rx1day. A significant positive trend was observed at 9 out of 10 stations. The Rx1day time series increased in Niš in southern Serbia, but not significantly. In addition, all fall and spring time series showed a positive trend, of which 8 and 5, respectively, were significant. In summer, 5 stations (Zrenjanin, Novi Sad, Veliko Gradište, Kragujevac and Zaječar) showed a significant positive trend, while 4 stations (Sremska Mitrovica, Belgrade, Loznica and Kragujevac) showed a positive trend and one (Niš) showed a negative but non-significant trend. In winter, a significant increase in Rx1day was observed at two stations (Kragujevac and Zaječar) and a negative trend at Veliko Gradište. The generalised extreme value function was calculated and analyzed for all of the available stations, for the periods of 1961-1990, 1990-2020 and 1961-2020 with the inclusion of return periods.

The highest increase of Rx1day was observed in Novi Sad, both on an annual and seasonal basis. The highest summer value of Rx1day (116.6 mm) was measured in Novi Sad in 2018, which led to flooding in the city (Savić et al., 2020). This precipitation episode was determined to be caused by convective rainfall.

Tošić, I., Unkašević, M., Putniković, S., 2017: Extreme daily precipitation: the case of Serbia in 2014. Theor. Appl. Climatol. 128, 785–794. doi:10.1007/s00704-016-1749-2

Savić, S.; Kalfayan, M.; Dolinaj, D. Precipitation Spatial Patterns in Cities with Different Urbanisation Types: Case Study of Novi Sad (Serbia) as a Medium-sized City. Geogr. Pannon. 2020, 24 (2), 88–99. https://doi.org/10.5937/gp24-25202

How to cite: Filipovic, L., Tosic, I., de Silva, A. S. A., Stosic, B., Stosic, T., and Djudjevic, V.: Analysis of extreme precipitation timeseries in Serbia based on station data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1877, https://doi.org/10.5194/egusphere-egu25-1877, 2025.

EGU25-2722 | ECS | Posters on site | HS7.5

Sensitivity of pluvial flood exposure to the selection of intensity-duration-frequency data 

Jannis Hoch, Anthony Cooper, and Conor Lamb

Pluvial floods are and will remain an important driver of flood risk, especially in an urban context. Recently, several floods triggered by extreme rainfall made the news and led to many casualties, such as those in Valencia and Nepal in 2024. To better prepare for such disasters, urban planners may use pluvial flood maps to assess flood risk and plan accordingly. Typically, such maps are produced by distributing rainfall over topography using a hydraulic model which solves some variation of the shallow water equations. While the decision for a specific hydraulic model may impact pluvial flood maps, here we will focus on the role of pluvial input data.

Typically, intensity-duration-frequency (IDF) data is used to drive these models, yet these data are highly uncertain due to, for instance, the absence of accurate rainfall observations or the application of extreme value statistics.

Here, we present results of a sensitivity analysis in which we employed a range of global and national IDF data sets, such as NOAA Atlas 14, KOSTRA-DWD, BURGER, GPEX, PPDIST and PXR. Each data set is unique in the amount of data it was produced with, the spatial extent, the spatial regionalization of point-based estimates, the extreme value distribution used, and so forth. All IDF datasets were fed into a hydraulic model (LISFLOOD-FP) using the Chicago Design Storm (CDS) method to produce consistent and comparable maps of pluvial flood hazard for several test cases. Subsequently, the (dis-)agreement of the flood maps obtained is assessed.

To convert flood maps into impact, they are intersected with exposure data to obtain an estimate of average annual exposure (AAE) to pluvial floods, which is a better measure for assessing the impact of these floods.

While we expect that intensities extracted from the different IDF data sets will differ markedly, this study will shed light on the impact these differences may have on flood hazard and flood exposure estimates.

How to cite: Hoch, J., Cooper, A., and Lamb, C.: Sensitivity of pluvial flood exposure to the selection of intensity-duration-frequency data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2722, https://doi.org/10.5194/egusphere-egu25-2722, 2025.

EGU25-3385 | ECS | Orals | HS7.5

Integrating natural hazards and social vulnerability to estimate lightning-related mortality risk in Mexico 

Alejandro Jaramillo and Christian Dominguez

Lightning poses a significant threat to life, infrastructure, and economic sectors worldwide. This study evaluates lightning risk at the municipal level in Mexico by integrating the interplay of natural hazards and social vulnerability into a comprehensive risk estimation. Although lightning-related fatalities have declined in Mexico, likely driven by demographic shifts and improved urban infrastructure, significant social vulnerability persists, particularly in rural areas where labor-intensive agriculture and lower education levels are prevalent. Using this integrated approach, we develop a lightning fatality risk map that identifies high-risk regions in Mexico. These regions are characterized by high lightning occurrence and elevated social vulnerability. By providing detailed municipal-level insights, this research contributes to advancing local resilience and informing policy and disaster risk mitigation efforts, ultimately enhancing public safety in the face of natural hazards.

How to cite: Jaramillo, A. and Dominguez, C.: Integrating natural hazards and social vulnerability to estimate lightning-related mortality risk in Mexico, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3385, https://doi.org/10.5194/egusphere-egu25-3385, 2025.

Sardinia Island, situated in the Mediterranean Sea, is a water-scarce region frequently affected by severe multi-year droughts. This study investigates the dynamics of two distinct reservoir systems on the island—Bau Pressiu, a single reservoir with a small basin and limited storage capacity, and Flumendosa, a complex system of four interconnected reservoirs. By analyzing their monthly reservoir storage dynamics alongside the basin’s average monthly precipitation, we aim to understand their response to drought and its propagation. We employed the n-month Standardized Precipitation Index (SPI) and 1-month Standardized Storage Dynamics Index (SSDI), calculated using non-parametric fitting methods, to characterize precipitation and storage variability. Correlation analyses using Pearson and Kendall’s tau identified the precipitation accumulation period (propagation time) strongly correlated with storage dynamics. Contrasting operational rules and societal demands led to markedly different responses during droughts between the two systems. Continuous Wavelet Transform (CWT) and Cross Wavelet Transform (XWT) analyses revealed multiscale correlations between precipitation and reservoir storage. While precipitation exhibited independent multiscale power, reservoir signals displayed consistent annual-scale power linked to societal demand during summers and broader-scale patterns during severe droughts. Additionally, cross-wavelet analyses between SPI and large-scale climatic indicators, such as the Niño 3.4 index and Atlantic Multidecadal Oscillation (AMO), highlighted their significant but contrasting influences during multiyear droughts. Our findings confirm that both systems effectively mitigate short-term drought impacts. However, multiyear droughts, driven predominantly by large-scale climatic oscillations, severely strain reservoir systems and societal resilience, underscoring the so-called "reservoir effects". These insights are critical for improving water resource management strategies in drought-prone regions like Sardinia.

Keywords: multiyear drought, storage dynamics, wavelet analysis, climatic drivers, reservoir effect

How to cite: Majhi, A., Deidda, R., and Viola, F.: Unveiling the Climatic Drivers of Multi-Year Droughts in Sardinia: A Study of Reservoir Storage and Precipitation Dynamics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4161, https://doi.org/10.5194/egusphere-egu25-4161, 2025.

EGU25-5145 | Orals | HS7.5

Identifying trends in extreme hydro-meteorological events to assess water-related hazards in urban-rural areas in South Africa 

Torsten Weber, Sophie Biskop, Fabian Schreiter, Muhammad Fraz Ismail, Hubert Lohr, Deborah Schaudt, Christine Fürst, and Francois Engelbrecht

Building resilience in urban-rural areas against hydro-meteorological hazards such as prolonged droughts and floods is crucial for economic development and safeguarding vulnerable people in Africa. Extreme hydro-meteorological events are projected to become more frequent and intense under climate change, leading to human, material, economic and environmental losses and impacts. In particular, southern Africa exhibits pronounced hydro-meteorological extreme events in response to El Niño and La Niña events, with El Niño Southern Oscillation (ENSO) impacts projected to intensify in southern Africa in a warmer world. Two of South Africa’s major river systems have been identified as hot spots of water-related hazards, in the context of major risks of water insecurity and flood disasters in a warmer world.

The Integrated Vaal River System (IVRS), a large, complex water system comprising water resources of different river basins, and several mega-dams within, serves as a water lifeline of the Gauteng Province, the economic hub in South Africa. The IVRS is vulnerable to the occurrence of multi-year droughts. Although a drought so severe that the IVRS can no longer supply the Gauteng Province with water (a ‘day-zero drought’) has never occurred before in the historical record, a four-year drought culminating in the El Niño drought of 2015/2016 resulted in the level of the Vaal Dam falling to about 25% (a dam level below 20% would have implied the presence of a day-zero drought). East of the Lesotho highlands, major rivers such as the Umgeni drain eastwards towards the KwaZulu-Natal coastal plain. These rivers are prone to flooding, especially during La Niña years. In April 2022, South Africa experienced its worst flood disaster when more than 544 people died during flash flooding in the Umgeni, Mlazi and Mbokodweni rivers in the greater Durban area. Present analysis focuses on changes in trends and characteristics of drought and extreme precipitation events in both study regions for the past 40-years using the ERA5-Land reanalysis and observational datasets such as CHIRPS. The ERA5-Land dataset has a spatial resolution of 0.1°x0.1° (~11 km) and goes back to 1950, making it possible to analyse long-term trends of meteorological drought and extreme precipitation. Results will highlight changes in frequency, duration and intensity of hydro-meteorological extreme events.

The research is part of the “Water security in Africa – WASA” programme, project WaRisCo, which deals with water risks and resilience in urban-rural areas in southern Africa and the co-production of hydro-climate services for an adaptive and sustainable disaster risk management.

How to cite: Weber, T., Biskop, S., Schreiter, F., Ismail, M. F., Lohr, H., Schaudt, D., Fürst, C., and Engelbrecht, F.: Identifying trends in extreme hydro-meteorological events to assess water-related hazards in urban-rural areas in South Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5145, https://doi.org/10.5194/egusphere-egu25-5145, 2025.

EGU25-5363 | ECS | Posters on site | HS7.5

An Improved DP-POA Method for Optimal Operation of Reservoir Flood Control 

Yawei Ning, Minglei Ren, Junbin Zhang, Rong Tang, Liping Zhao, and Gang Wang

The consuming-time of the algorithm for solving the reservoir optimal operation model is crucial to real-time flood control. The traditional DP-POA (Dynamic Programmin-Progressive Optimization Algorithm) has better solutions but takes a long time. This study proposed an improved DP-POA method, which effectively reduces the amount of calculation and improves the calculation speed by simplifying the objective function. Taking Yuecheng Reservoir in China as an example, this study conducted a comparative analysis of five algorithms, including improved DP-POA, traditional DP-POA, improved POA, traditional POA and PSO (Particle Swarm Optimization). The results show that the improved DP-POA exhibits significant advantages in both consuming-time and solution quality. In the 2021 flood case, compared with the traditional DP-POA, the consuming-time of the improved DP-POA is shortened from about half an hour to less than 5 minutes; meanwhile, the solution of the improved DP-POA is better than or basically equal to other comparative methods.

How to cite: Ning, Y., Ren, M., Zhang, J., Tang, R., Zhao, L., and Wang, G.: An Improved DP-POA Method for Optimal Operation of Reservoir Flood Control, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5363, https://doi.org/10.5194/egusphere-egu25-5363, 2025.

EGU25-5958 | Posters on site | HS7.5

StoryMaps: Advancing Public Awareness, Preparedness, and Resilience to Flood Risks 

Peter Fischer-Stabel, Jaqueline Hoffmann, and Joshua Azvedo

Floods count as some of the most devastating natural disasters, inflicting extensive damage on infrastructure, disrupting communities, and posing serious threats to human lives. The flooding in Germany’s Ahr Valley in 2021 is a strong reminder of the devastating consequences. The increasing intensity of such events, driven by climate change, underscores the urgency of enhanced prevention and preparedness strategies (Deumlich & Gericke, 2020).

Fluvial (river) floods, which often occur at regular intervals, tend to remain in the collective memory of affected populations. However, when sufficient time passes without an event, a phenomenon referred to as "flood dementia" can emerge. This leads to diminished public awareness and preparedness, increasing vulnerability during future disasters. The issue is even more pronounced with pluvial (rainfall-induced) floods, which are harder to predict and therefore require robust preventive measures.

Effective flood risk management demands targeted approaches to engage diverse demographic groups. A survey conducted as part of the BMBF-FloReST project revealed significant disparities in awareness across age groups. While individuals aged 50 and older were well-represented in the survey, those aged 20 and younger were notably underrepresented. This younger age group often lacks the life experience needed to fully comprehend the impacts of pluvial flooding, underscoring the importance of targeted educational initiatives.

StoryMaps have emerged as a valuable tool for addressing this gap, particularly among younger audiences. By integrating geospatial data visualization with storytelling elements such as maps, images, videos, and narratives, StoryMaps transform complex environmental information into an engaging and accessible format. Young people, who are more responsive to interactive and visually rich content, benefit from enhanced comprehension and retention. For example, StoryMaps can depict flood-prone areas, recount historical flood events, and simulate potential outcomes of mitigation strategies, thus bridging technical concepts with tangible, real-world examples.

Furthermore, StoryMaps help young people connect local flood risks to broader global challenges. By exploring the links between climate change and flooding, students can better understand the interconnectedness of environmental issues. This fosters a sense of accountability and encourages proactive participation in community resilience initiatives. Additionally, StoryMaps promote critical thinking by enabling users to explore “what-if” scenarios, such as the impacts of improved drainage systems or reforestation on flood dynamics.

Their digital accessibility makes StoryMaps particularly effective for engaging tech-savvy younger generations. They can be seamlessly incorporated into school curricula, workshops, and community outreach programs, equipping young people with practical knowledge about sustainable water management and disaster preparedness.

In conclusion, StoryMaps represent a forward-thinking approach to flood risk awareness and education, particularly for younger audiences. By blending education with engagement, they empower a generation to better understand and address the challenges of climate-related disasters. Our presentation will showcase two StoryMaps—focused on the 2021 Ahr Valley flood and the 2024 Saarland Pentecost flood—developed as part of the FloReST project and introduced in schools to foster awareness and resilience among young learners.

How to cite: Fischer-Stabel, P., Hoffmann, J., and Azvedo, J.: StoryMaps: Advancing Public Awareness, Preparedness, and Resilience to Flood Risks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5958, https://doi.org/10.5194/egusphere-egu25-5958, 2025.

EGU25-6246 | Posters on site | HS7.5

Adaptation to flood risk on Reunion Island (France): A historical perspective from photographic evidence 

Gilles Arnaud-Fassetta, Jean Larive, François Taglioni, David Lorion, Salem Dahech, and Alizé Méchain

Reunion Island, situated in the Indian Ocean, has faced significant flood risks since its early settlement in the 17th century. Currently, the island comprises six territories identified as flood-risk areas (TRI). Understanding the historical context of this risk is crucial for effective management and adaptation strategies. To explore the evolution of flood risk, we examined a collection of historical postcards from the late 19th to early 20th centuries, archived at the Archives Départementales in Saint-Denis. We selected approximately fifty postcards based on specific criteria: the relationship between habitats and rivers, the need for a comprehensive spatial perspective, and the representation of diverse watersheds across the island. Field missions conducted in 2024 and 2025 allowed us to replicate the photographs at the same locations as depicted on the ancient postcards, facilitating a direct comparison of changes in land use and hydromorphological structures (including “planèzes”, slopes, and valley floors). Our findings reveal significant insights comparing land use from the late 19th century to the present day (2024-2025). We observed new housing developments on planèzes, which have heightened risks of urban runoff and flooding associated with small rivers. Certain regions remain unchanged, indicating that the original placement of habitats was appropriate, situated on alluvial terraces and slopes protected from landslides and debris flows. In contrast, urban encroachment into the active channels of large rivers (“ravines”) has created substantial risks for local populations. These findings align with the analyses of D. Lorion (2013), who characterizes the rise in flood-risk areas during the 1970s and 1980s as a manifestation of the 'security utopia' created by river embankment systems.

 

References

 

Lorion D. (2013) – From a utopia of security to the integrated management of drainage basins: The example of Reunion Island (France). In Arnaud-Fassetta G., Masson E., Reynard E. (Eds.) European continental hydrosystems under changing water policy. Friedrich Pfeil Verlag, München, 87-98.

How to cite: Arnaud-Fassetta, G., Larive, J., Taglioni, F., Lorion, D., Dahech, S., and Méchain, A.: Adaptation to flood risk on Reunion Island (France): A historical perspective from photographic evidence, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6246, https://doi.org/10.5194/egusphere-egu25-6246, 2025.

EGU25-6432 | Orals | HS7.5 | Highlight

Large-Sample Machine Learning Models for Estimation, Attribution, and Projection of Hydrometeorological Extremes 

Louise Slater, Michel Wortmann, Simon Moulds, Yinxue Liu, Boen Zhang, Laurence Hawker, Liangkun Deng, and Emma Ford

The estimation, attribution or projection of hydro-meteorological extremes in individual locations is constrained by the limited number of observations of extreme events. Recent advances in large-sample machine learning (ML) models, however, have demonstrated significant potential to mitigate the impact of data scarcity on the quantification of hydrological risks. These models integrate hundreds to thousands of time-series records alongside local descriptors of climate and catchment characteristics, enabling them to learn relationships across diverse environments and provide accurate estimations of hydro-meteorological extremes. This presentation will highlight our recent advancements and challenges in developing large-sample ML models for estimating, attributing, and projecting hydro-meteorological extremes.

At the core of our ML models is the GRIT river network, a new global bifurcating network which includes multi-threaded rivers, canals, and deltas. Unlike conventional single-threaded global river networks, GRIT incorporates bifurcations derived from the 30m Landsat-based river mask from GRWL and elevation-based streams from the FABDEM digital terrain model. This realistic depiction is critical, as 98% of floods identified in the Global Flood Database occur within 10 km of a river bifurcation. Individual river reaches in GRIT are assigned a broad range of static and time-varying variables describing the local meteorology, climate, geology, soils, geomorphology, Earth observation, terrestrial water storage, land cover time series, socio-economic data, and a novel archive of historical river discharge records from approximately 60,000 gauges.

This novel dataset enables us to tackle three key challenges: (1) Flood estimation: We estimate flood hazards globally, such as bankfull river discharge, the mean annual flood, and return periods, and assess the ability of the models to produce spatially-consistent hazard estimates. By leveraging an expanded training envelope, the ML models generate reliable estimates in data-sparse regions. (2) Flood attribution: Leveraging a range of explainability methods such as model probes, sensitivity testing, SHAP, ALE, PDP, and gradient-based methods, we investigate flood-generating mechanisms across diverse catchment types. Explainable AI (XAI) tools enable us to interrogate the models to enhance our understanding of the physical and anthropogenic drivers of flooding. (3) Flood prediction and projection: We assess the utility of hybrid large-sample ML models trained directly on subseasonal to seasonal forecasts or Earth system model (ESM) outputs for future flood projections. We show how large-sample models can implicitly correct spatio-temporal biases in forecasts or ESM outputs and deliver reliable predictions, bypassing traditional modelling steps such as downscaling and bias-correction.

Finally, we discuss key challenges in large-sample modelling, such as systematic biases in training data, inconsistencies in XAI results, causality, and the relative strengths and weaknesses of simple ML models versus deep learning. These challenges underscore the need for continued innovation in large-sample model design and application. By integrating diverse datasets and advanced ML techniques, large-sample models present transformative opportunities for flood estimation, attribution, and projection, enabling informed decision-making for management of hydro-meteorological extremes.

 

How to cite: Slater, L., Wortmann, M., Moulds, S., Liu, Y., Zhang, B., Hawker, L., Deng, L., and Ford, E.: Large-Sample Machine Learning Models for Estimation, Attribution, and Projection of Hydrometeorological Extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6432, https://doi.org/10.5194/egusphere-egu25-6432, 2025.

EGU25-6777 | Orals | HS7.5

The Risk of Negatively Biased and Overconfident Return Level Estimates: A Critique of the Metastatistical Approach to Extremes 

Torben Schmith, Karsten Arnbjerg-Nielsen, and Bo Christiansen

Classical extreme value analysis (EVA) often give large uncertainties on estimated return levels due to the limited length of real-world hydrological time series. The metastatistical extreme value (MEV) approach (Marani and Ignaccolo 2015) aims to overcome these limitations by describing all data using a common distribution, treating extremes as large ordinary data values. The above authors perform Monte Carlo simulations with synthetic time series generated from a Weibull distribution and fit a Weibull distribution to each series, as prescribed in the MEV approach. These simulations show that the MEV give unbiased estimates with smaller confidence intervals, compared with the GEV and Gumbel methods from classical EVA.

However, the MEV method neglects that physical mechanisms producing extremes often differ from those for ordinary events. Therefore, the ordinary and extreme events should in general be described by a mixture distribution and this may influence the results of MEV. To test this, we replicated their work and added a variant using synthetic time series from a Weibull mixture distribution, formed by mixing the original Weibull distribution with a tiny fraction of another Weibull distribution with a longer tail. This mimics the shift in distribution between ordinary and extreme events. When applying the Weibull-based MEV to the Weibull mixture samples, the MEV method produced systematically biased estimates, which are outside the confidence intervals provided by MEV. In contrast, GEV produced unbiased estimates that are inside the confidence interval.

Finally, goodness-of-fit tests are not able to distinguish between time series distributed according to Weibull and Weibull mixture, and can therefore provide no guidance on when to use MEV. In summary, we find the MEV approach unreliable for real-world applications and strongly caution against using it.

How to cite: Schmith, T., Arnbjerg-Nielsen, K., and Christiansen, B.: The Risk of Negatively Biased and Overconfident Return Level Estimates: A Critique of the Metastatistical Approach to Extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6777, https://doi.org/10.5194/egusphere-egu25-6777, 2025.

EGU25-6994 | ECS | Orals | HS7.5

Subjective and Objective Methods in Multi-Criteria Decision-Making (MCDM) for Flood Mitigation: Implications on Policymaking 

Hassan Sabeh, Chadi Abdallah, Nanée Chahinian, Marie-George Tournoud, Rouya Hdeib, and Roger Moussa

Flood risk management comprises risk assessment through robust modeling and mitigation through measure implementation. Decision-making on mitigation measures is complicated by the plethora of criteria, stakeholder influence, implementation scale and financial constraints. Multi-criteria decision-making (MCDM) methods have emerged as valuable tools in this context, allowing for the systematic integration of diverse factors and perspectives. Nonetheless, MCDM applications in mitigation measure ranking remain challenged by the lack of informed evaluation of criteria and the diversity of measures at local reach-scale. This work aims to develop a comprehensive methodology for prioritizing flood mitigation measures. An application is conducted on a Mediterranean catchment, the Ostouane River (144 km2), Northern Lebanon. The approach involves identifying 11 intervention reaches, proposing 38 mitigation measures, and evaluating a set of 7 primary criteria decomposed into 19 multidimensional secondary criteria. We introduce criteria of effectiveness, technical, exposure and vulnerability in addition to the commonly used criteria of environmental impact, socio-economic impact, and cost. The criteria are evaluated based on qualitative and quantitative inputs derived from the literature, surveys, questionnaires, hydrological and hydraulic modelling. The TOPSIS model is employed using 6 subjective stakeholder-driven weighting methods and 6 data-driven objective weighting methods. The methodology is evaluated through a sensitivity analysis that emphasizes on the importance of measure effectiveness, environmental impact, and cost criteria in the model. Results show that subjective weighting methods tend to prioritize structural measures at downstream areas with high-value assets, while objective methods show a more balanced distribution of measures, including green solutions and upstream reaches. The total cost of the 10 prioritized measures using subjective methods is 20% higher than that of objective methods. However, the specific choice of a weighting method can imply a substantial variation in total implementation and maintenance cost. Essentially, the choice of weighting method in MCDM can significantly alter the resulting strategies and management of risk. This contrast highlights the need for policymakers to develop flexible, adaptive strategies that balance immediate protection needs with long-term sustainability goals. Overall, this work provides a novel approach for integrated flood risk management based on adapted local-scale and informed decision-making.

How to cite: Sabeh, H., Abdallah, C., Chahinian, N., Tournoud, M.-G., Hdeib, R., and Moussa, R.: Subjective and Objective Methods in Multi-Criteria Decision-Making (MCDM) for Flood Mitigation: Implications on Policymaking, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6994, https://doi.org/10.5194/egusphere-egu25-6994, 2025.

Landslides, predominantly triggered by intense and prolonged rainfall, pose a critical hazard in the Himalayan region, with Indian Himalayas contributing approximately 15% of global rainfall-triggered landslides. Despite advances in landslide prediction, existing thresholds often fail to account for the diverse climatic and geophysical conditions across the Himalayas. To address these gaps, this study establishes both at-site and regional rainfall thresholds for landslide prediction by integrating advanced statistical techniques and environmental analyses. Seasonal rainfall thresholds were established to define rainy days, revealing higher winter thresholds in the Northwestern Himalayas (NWH) due to snowmelt contributions and elevated monsoon thresholds in the Northeastern Himalayas (NEH), driven by prolonged rainfall and antecedent moisture saturation. Building on this, we derived empirical event-duration (E-D) thresholds using a novel non-crossing quantile regression approach to ensure robustness against lower quantile crossing issues. The derived regional thresholds for NEH (E = -11.10 + 0.62D) and NWH (E = -12.00 + 0.63D) fits within global bounds . Land use/land cover (LULC) analysis and probabilistic mutual information ─ based analysis further identified critical environmental controls shaping these thresholds. In the NWH, built-up areas, elevation, and vegetation emerged as key factors playing significant roles in shaping rainfall thresholds to trigger landslides, while elevation, rangeland, and the Standardized Precipitation Index (SPI) were significant in the NEH. These insights underscore the need for region-specific E-D thresholds for landslide prediction and disaster management in the Himalayan region. By integrating environmental controls into a 'physics-based statistical learning' framework, this study overcomes limitations of conventional empirical rainfall threshold for landslide prediction models, delivering region-specific thresholds, thereby enhancing disaster preparedness, a step towards developing a climate-resilient landslide early warning system in the Himalayas.

How to cite: Monga, D. and Ganguli, P.: Developing Site-Specific Rainfall Thresholds for Landslide Prediction in the Himalayas: A Comparative Assessment between Northwestern and Northeastern Himalayas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7120, https://doi.org/10.5194/egusphere-egu25-7120, 2025.

EGU25-7334 | Posters on site | HS7.5

Rainfall extremes and their impacts: from the local to the National Scale. The INTENSE project.  

Elisa Arnone, Marco Marani, Leonardo V. Noto, Roberta Paranunzio, Matteo Darienzo, Antonio Francipane, Cesar Arturo Sanchez Pena, Juby Thomas, Dario Treppiedi, and Francesco Marra

This study describes the activities developed within the project “raINfall exTremEs and their impacts: from the local to the National ScalE (INTENSE)”, funded by the Italian Ministry of University and Research (MUR) and by the EU. INTENSE will provide a novel assessment of hazards related to extreme rainfall and landslides, to aid risk management at the local and national scales.

The long historical rainfall records available from rain gauges allow us to derive extreme precipitation probabilities in gauged locations, but they hardly represent ungauged areas and cannot adequately sample the spatial variability of extreme rainfall in areas with strong climatological gradients, such as orographic and coastal regions. To overcome these limitations, we collect national-scale observations from rain gauges, weather radars and satellites and we use state-of-the-art statistical approaches, stochastic weather generators, and physically based landslide models.

In particular, a novel statistical approach for the analysis of extreme values from remotely sensed rainfall is used to produce national scale maps of extreme rainfall at multiple scales. The INTENSE approach allows us to link local rainfall climatology (i.e. frequency of rainstorms; intensity of ordinary and extreme rainstorms; rainstorms temporal structure) to the probability of initiation of shallow mass movements, a long standing challenge in rainfall-related hazards assessment. This is done feeding physically based landslide initiation models with long simulations of climate variables able to adequately represent the statistics and properties of both ordinary and extreme rainstorms.

We present here the preliminary results of the project with a particular focus on (i) rainfall frequency analysis, (ii) downscaling of extreme precipitation, and (iii) of the critical soil moisture maps needed to trigger shallow movements in a selected case study.

 

This research received funding from European Union NextGenerationEU – National Recovery and Resilience Plan (PNRR), Mission 4, Component 2, Investiment 1.1 -PRIN 2022 – 2022ZC2522 - CUP G53D23001400006

How to cite: Arnone, E., Marani, M., Noto, L. V., Paranunzio, R., Darienzo, M., Francipane, A., Sanchez Pena, C. A., Thomas, J., Treppiedi, D., and Marra, F.: Rainfall extremes and their impacts: from the local to the National Scale. The INTENSE project. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7334, https://doi.org/10.5194/egusphere-egu25-7334, 2025.

EGU25-7484 | ECS | Posters on site | HS7.5

Evolving Dependence Structures Between Compound Flood Drivers Under Future Climate Scenarios: A case study over Greater Boston 

Stergios Emmanouil, Andreas Langousis, Elizabeth Perry, Joshua P. Hacker, and Emmanouil N. Anagnostou

The assessment of compound flood risk often relies on the assumption that the dependence structure between flood drivers (e.g., rainfall intensity, coastal water levels, and streamflow) remains stationary under changing climatic conditions. Yet, traditional approaches that inherently assume stationary dependencies, or rely solely on historical relationships, may misrepresent flood risk and fail to identify hotspots of emerging infrastructure vulnerabilities. This study aims to (a) characterize the dependence structure between compound flood drivers using a parsimonious parametric framework, and (b) explore potential changes in this structure under future climate scenarios, by leveraging outputs from the Coupled Model Intercomparison Project Phase 6 (CMIP6) regional climate projections. An ensemble of synthetic and historical storms is employed to simulate flood impacts across the Greater Boston region, forming the basis for statistically modeling the conditional dependence of the main flood drivers. Changes in the marginal distributions of these drivers, informed by CMIP6 simulations under various Representative Concentration Pathways (RCPs), are also integrated into the dependence framework to evaluate future trajectories of compound flood risk. The findings focus on determining whether shifts in the dependence structure offer a more nuanced understanding of evolving flood risk profiles, as well as identifying areas where traditional stationary assumptions may result in systematic errors. Ultimately, the study advances understanding of the dynamic interplay between flood drivers under future climate scenarios, and supports the development of adaptation strategies for regions vulnerable to compound flooding.

How to cite: Emmanouil, S., Langousis, A., Perry, E., Hacker, J. P., and Anagnostou, E. N.: Evolving Dependence Structures Between Compound Flood Drivers Under Future Climate Scenarios: A case study over Greater Boston, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7484, https://doi.org/10.5194/egusphere-egu25-7484, 2025.

The floods that hit wide parts of Central Europe in July 2021 demonstrate the impact that extreme precipitation events can have on our continent. Heavy continuous rainfall from 12th to 15th of July 2021, caused by low-pressure system "Bernd", resulted in widespread flooding. In Germany, the federal states of Rhineland-Palatinate and North Rhine-Westphalia were particularly affected, experiencing the most fatalities and material damage. The rapid surge of rivers and creeks in these areas overwhelmed residents and authorities. After the flood, criticisms arose over inadequate crisis management and early warning systems. This raises the question of the extent to which the population was prepared for such an event and what lessons were learned to be better prepared for future climate-related hazards.

This research focuses on the question of how the experience of a highly disruptive disaster, such as the 2021 floods, affects the population's risk perception towards multiple natural hazards. Further, it assesses if severe affectedness and experiences with natural hazards trigger better preparedness and behavioural knowledge. To answer these questions, an online survey (n= >282) assesses risk perception and preparedness towards natural hazards. The survey was spread in Opladen and Schlebusch, two districts of the city of Leverkusen that were affected by the 2021 flood. Data from the survey underwent statistical analysis, including Pearson Correlation and linear regression.

Early results show that risk perception is highest for heavy rainfall, followed by river floods in both districts. However, the perception of heatwaves and drought differs in the two study areas. In Opladen, where the Urban Heat Island (UHI) effect is more pronounced, the risk of heat and drought is perceived more strongly compared to Schlebusch. We also analysed how the 2021 flood affected people's perception of natural hazard risk. Results reveal that more than 75% of respondents in Opladen and more than 60% of respondents in Schlebusch reported an altered risk perception after the 2021 floods. Before this event, the risk perception towards extreme precipitation and river flooding was notably lower. Of all natural hazards mentioned in the questionnaire, heat was perceived as the greatest threat in Opladen, while in Schlebusch it was storms.

The findings of this study will be used in the BMBF project Co-Site to design risk communication strategies and workshops aimed at enhancing the public’s preparedness for natural hazards. Understanding people’s risk perception and preparedness for natural hazards can help identify training needs for better preparedness and foster appropriate communication about disaster risk.

Keywords: Risk Perception, Natural Hazards, Preparedness, Germany

How to cite: Könsgen, I., Braun, B., and Nehren, U.: How do disruptive events influence risk perception and preparedness towards natural hazards? An empirical study in Leverkusen, Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8371, https://doi.org/10.5194/egusphere-egu25-8371, 2025.

EGU25-8795 | Posters on site | HS7.5

Nowcasting Radar for Hydrological Flood Prediction: applications in the Marche Region, Italy 

Barbara Tomassetti, Francesco Iocca, Francesca Sini, Gabriella Speranza, Valentino Giordano, Mario Montopoli, Saverio Di Fabio, Lorenzo Giorgio Didimi, Marco Lazzeri, Marco Tedeschini, Marco Pellegrini, and Annalina Lombardi

Accurate flood forecasting is essential to mitigate the impacts of extreme rainfall on communities and infrastructure. Traditional hydrological prediction methods often rely on rain gauge data and numerical models, which can be limited in capturing precipitation's spatial and temporal dynamics, particularly during intense or rapid-onset events. X-band polarimetric radar provides a valuable alternative for quantitative rainfall estimation, offering finer spatial and temporal resolution crucial for hydrological applications.

This study investigates the integration of radar nowcasting into flood forecasting workflows, focusing on data from an X-band polarimetric radar operated by the Civil Protection Service of the Marche Region, Italy. Several case studies have been analyzed considering different precipitation regimes: convective events with a short-time peak of intense rainfall and stratiform events, characterized by several hours of persistent precipitation associated with frontal systems.

The Cetemps Hydrological Model (CHyM) is used to simulate river discharge and assess hydrological stress indices under three scenarios: (1) rain gauge data alone, (2) radar data alone, and (3) radar data integrated with nowcasting outputs to generate 1-hour forecasted rainfall fields. Results demonstrate that radar-based nowcasting significantly improves flood prediction accuracy and lead time, particularly in flash flood scenarios driven by convective systems.

This study highlights the importance of radar nowcasting techniques in improving flood forecasting capabilities for enhancing flood prediction in regions prone to extreme rainfall, emphasizing its role in building more resilient and proactive flood management systems.

How to cite: Tomassetti, B., Iocca, F., Sini, F., Speranza, G., Giordano, V., Montopoli, M., Di Fabio, S., Didimi, L. G., Lazzeri, M., Tedeschini, M., Pellegrini, M., and Lombardi, A.: Nowcasting Radar for Hydrological Flood Prediction: applications in the Marche Region, Italy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8795, https://doi.org/10.5194/egusphere-egu25-8795, 2025.

EGU25-9425 | Orals | HS7.5

Recent European floods from a (re)insurance market perspective 

Francesco Zuccarello, Christopher Masafu, Brian Kerschner, Sumeet Kulkarni, and Laurence Taylor

A nearly stationary low-pressure system generated significant rainfall across central Europe in September 2024 resulting in life-threatening and costly flooding in Central and Eastern Europe. Catastrophic floods also struck southern Spain in October and southern Germany from late May to early June. These events marked an escalation in severity compared to 2023, which saw major flood events impacting Italy and Greece in June and September, respectively. This escalating pattern of widespread, severe flooding, coupled with rising financial losses and risks, has drawn significant attention from (re)insurers.

We present a retrospective on these events using the Gallagher Re Europe Flood Model, a pan-European flood catastrophe model designed to assess the potential financial impact of floods in terms of their magnitude and likelihood. By using quantitative indexes to compare observed flooding with thousands of stochastic event footprints included in the model, we show that a complementary qualitative analysis is necessary to identify the most representative events. This hazard-based analysis is than complemented by the estimation of financial losses. The results reveal a range of losses for near-similar events, reflecting the complexities involved in modelling the financial impact of flooding. These complexities include, but are not limited to, the granularity of the peril, the geo-localization of the exposure and the impact of flood defences. For example, by leveraging the flexibility of our model, we show an estimate of the financial implications for a (re)insurer should the defences have failed during the development of major events.    

In conclusion, while there is no control on the meteorological drivers of such events, our  analyses shows the relevance and importance of catastrophe models to support (re)insurers in targeted exposure management and improved risk assessment.

How to cite: Zuccarello, F., Masafu, C., Kerschner, B., Kulkarni, S., and Taylor, L.: Recent European floods from a (re)insurance market perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9425, https://doi.org/10.5194/egusphere-egu25-9425, 2025.

EGU25-9751 | ECS | Orals | HS7.5

Thunderstorm in Taiwan and Its Impact on Railway 

Chi-June Jung, Ben Jong-Dao Jou, Ko Pak Tin Boaz, Yi-Hsi Lee, and Kai-Shiang Yang

Severe convective storms frequently occur in Taiwan, bringing heavy rainfall, strong winds, and lightning. These events significantly disrupt critical infrastructure, including railways, by causing operational delays and damage to facilities. The proximity of the railway network to high-frequency thunderstorm zones highlights the need for tailored meteorological applications to mitigate these risks. 

Heavy rainfall and wind gust are key characteristics of severe convective storms. Analysis of a thunderstorm event in Taipei Basin demonstrates that merged convective cells can produce extreme rain rates exceeding 60 mm in 20 minutes, which is closely tied to urban flash flood occurrences. Microbursts, identified through radar signatures like descending precipitation cores and strong near-ground divergent outflows, further exacerbate railway hazards, generating wind gusts exceeding 10 m/s. 

To address these challenges, the Central Weather Administration issues real-time severe thunderstorm warnings based on radar observations, such as radar echoes > 55 dBZ and 60-minute rainfall > 40 mm. Since 2024, National Taiwan University has collaborated with Taiwan Railway Company to implement targeted warnings. These alerts, distributed via the LINE app, provide real-time updates on affected railway sections, improving disaster preparedness and operational resilience. 

Between April and October 2024, alerts were issued for various disasters, including flooding, fallen trees, and landslides. However, the actual occurrence rate was only 2%. To reduce false alarms and enhance the accuracy of warnings, radar-based quantitative precipitation forecast (QPF) thresholds are being introduced. These efforts aim to strengthen railway safety and minimize disruptions caused by severe weather events.

How to cite: Jung, C.-J., Jou, B. J.-D., Boaz, K. P. T., Lee, Y.-H., and Yang, K.-S.: Thunderstorm in Taiwan and Its Impact on Railway, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9751, https://doi.org/10.5194/egusphere-egu25-9751, 2025.

EGU25-10315 | ECS | Posters on site | HS7.5

Atmospheric drivers of extreme precipitation events in the Indian sub-continent 

Nandana Dilip K and Vimal Mishra

Extreme precipitation events in the Indian sub-continent have profound socio-economic and environmental impacts, particularly due to their role in triggering flash floods. These events are driven by a combination of atmospheric conditions, moisture sources and pathways, geomorphology, and hydrometeorology. However, while the hydrometeorological and geomorphological factors have been extensively studied, the role of atmospheric drivers and moisture pathways remains underexplored, creating a significant research gap. To address this gap, we analyzed the atmospheric processes and moisture sources contributing to widespread extreme hourly precipitation events across the Indian subcontinent during the period 1981–2020. Using a combination of reanalysis datasets, event detection algorithms, and moisture tracking methods, we identified the spatial and temporal distribution of these events. We find the Himalayas as a major hotspot, with most extreme events occurring during the Indian summer monsoon season. We find recycled moisture from land surfaces is the dominant source of moisture in the Himalayas, whereas moisture from the Arabian Sea and the Bay of Bengal primarily drives precipitation extremes in peninsular India. Our findings highlight the interconnected dynamics between the atmosphere, land, and ocean in driving extreme precipitation. The study underscores the importance of incorporating atmospheric drivers into disaster management frameworks and early warning systems to enhance preparedness and mitigate impacts effectively.

How to cite: Dilip K, N. and Mishra, V.: Atmospheric drivers of extreme precipitation events in the Indian sub-continent, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10315, https://doi.org/10.5194/egusphere-egu25-10315, 2025.

EGU25-10418 | Orals | HS7.5

  Are rainfall warning levels ready for climate change? A case study from Catalonia, Spain 

Erika Meléndez-Landaverde, Daniel Sempere-Torres, Víctor González, and Carles Corral

Extreme precipitation events, characterised by significant rainfall amounts over short periods, are projected to intensify and occur more frequently under the influence of climate change. These projected changes, combined with rapid urbanisation, will likely lead to more frequent and extreme pluvial flood events (urban and flash floods) due to the precipitation intensity rapidly and easily exceeding the current capacity of natural and artificial drainage systems. Assessing the impact of future climate scenarios on extreme precipitation is therefore critical for identifying and designing sustainable adaptation and mitigation actions for at-risk communities and their citizens.

As part of the EU Horizon 2020 project CLIMAAX, an extreme precipitation workflow has been developed to provide step-by-step guidelines for communities and regions to identify and assess how their critical rainfall thresholds could shift in both magnitude and frequency under climate projections. In this work, a critical rainfall threshold is defined as the precipitation intensity necessary to trigger unsustainable or unacceptable impacts in a specific location or area. These thresholds are commonly used in designing drainage systems and flood protection infrastructure and serve as decision support values for triggering rainfall warnings or advisory information during emergencies. By employing the workflow to assess how these critical rainfall thresholds are projected to change, communities can make informed decisions about the most appropriate long-term adaptation measures to enhance their overall climate resilience. Moreover, the flexible workflow structure facilitates the integration of diverse hazard, exposure and vulnerability datasets at multiple scales (e.g., CORDEX, WorldPoP), making it adaptable to specific regional needs.

The extreme precipitation workflow has been applied in the Catalonia Region, Spain, to evaluate how the current rainfall thresholds used for triggering rainfall warnings for Dangerous Meteorological Situations will vary due to the influence of climate change. Model combinations of EURO-CORDEX climate projections at a 12km spatial resolution for the different Representative Concentration Pathways (RCPs) were employed for assessing future rainfall projections. Considering the increased number of extreme precipitation events in the region over the past years, the impacts associated with these and the number of triggered warnings per year, the results are expected to provide authorities with valuable insights into the frequency and magnitude shifts of these extreme events in the region.

How to cite: Meléndez-Landaverde, E., Sempere-Torres, D., González, V., and Corral, C.:   Are rainfall warning levels ready for climate change? A case study from Catalonia, Spain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10418, https://doi.org/10.5194/egusphere-egu25-10418, 2025.

Disaster monitoring and early warning systems are typically associated with the detection of extreme events capable of causing significant social impacts, particularly in cases of rain-related disasters such as floods, flash floods, and landslides. However, this traditional approach—focused solely on assessing the likelihood of threats materializing—proves insufficient when monitoring areas with high heterogeneity in terms of exposure and population vulnerability. In such cases, less extreme but more frequent events can result in recurring impacts that, when analyzed historically, surpass those of extreme events. In Brazil, approximately 90% of landslide occurrences are associated with low magnitude impact. Low magnitude events cannot be neglected because even though they cause low-severity losses, their high-frequency and cumulative effect adds up to a large number of losses and affected people. Understanding the impacts of low magnitude events can aid in defining risk scenarios as part of the potential impact dimension within a risk matrix. Thus, this study uses a database developed by the Brazilian National Center for Monitoring and Early Warning of Natural Disasters (CEMADEN) to better understand these relationships. Furthermore, it proposes an approach to develop a potential impact indicator based on retrospective risk analyses, linking average impact levels over time to extreme rainfall frequency data. The study focuses on Santa Catarina state (Southern Brazil), analyzing impact data from 80 municipalities between 2016 and 2024. During this time period, the monitored municipalities in the state reported 568 landslide/related impact events, affecting over 8,000 individuals. The analyzed data indicate 548 events with low magnitude impacts, which can be classified as extensive risk events (high frequency, low severity), typically characterized by situations that had 1 to 2 small landslides. On the other hand, 18 events were identified with medium magnitude impacts, where 3 to 10 landslides were generally recorded. Only 2 large magnitude events (>10 landslides) were recorded in the analyzed period, which can be classified as intensive risk events (low frequency, high severity). The results reveal distinct municipal profiles, highlighting two key scenarios: i) areas where the combination of frequent heavy rainfall events and a high potential impact indicator result in very high climate risk and, ii) contrasting situations where significant impact occur despite of low frequency of heavy rainfall suggesting a bigger weight of social vulnerability and exposure of human systems. In addition to providing critical insights for enhancing CEMADEN's decision-making in disaster early warning issuance, the study offers valuable information for prioritizing risk reduction measures and climate adaptation actions.

How to cite: Bernardes, T. and Camarinha, P.: Comparative analysis between impact data related to landslides and extreme rainfall events in Southern Brazil: a proposal to establish potential impact indicators, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11982, https://doi.org/10.5194/egusphere-egu25-11982, 2025.

EGU25-14504 | Orals | HS7.5

Global Insight into Extreme Events and Land Subsidence: Understanding Drivers, Interplay, and Impacts 

Laurie Huning, Charlotte Love, Hassan Anjileli, Farshid Vahedifard, Yunxia Zhao, Pedro Chaffe, Kevin Cooper, Aneseh Alborzi, Edward Pleitez, Alexandre Martinez, Samaneh Ashraf, Iman Mallakpour, Hamed Moftakhari, and Amir AghaKouchak

Land subsidence (LS) or the relative lowering of the Earth’s ground surface is a critical concern that warrants global attention. LS is a chronic hazard in many areas that has adverse effects on built infrastructure, people, and natural systems. As global atmospheric temperatures rise and the water cycle intensifies, climatic extreme events (e.g., droughts, wildfires, heatwaves, floods) are expected to become more severe. We must therefore better understand the impact of interactions and feedbacks among extreme events, LS, human activities, and their effects around the world. Notably, our global study highlights that LS can alter the potential impacts of extreme events, and extreme events can contribute to LS. We also identify a variety of LS drivers, both natural and anthropogenic (e.g., natural compaction, urbanization, extraction of fossil fuels and groundwater from the subsurface), and corresponding LS rates throughout a variety of climatic zones and environments from the coastline inland. This study presents analysis of anthropogenic-related activities and natural processes that cause LS, but can also enhance climate change as greenhouse gases are released from the soil into the atmosphere (e.g., via permafrost thawing or peatland and wetland removal). Through our synthesis of process-driven relationships and examples, we underscore the interplay of climatic extremes and LS that damages infrastructure and enhances the vulnerability of large populations to floods and other natural hazards. Our study provides guidance for future policies and adaptation and mitigation approaches that account for the critical connections between the land surface, environmental change, and extreme events.

How to cite: Huning, L., Love, C., Anjileli, H., Vahedifard, F., Zhao, Y., Chaffe, P., Cooper, K., Alborzi, A., Pleitez, E., Martinez, A., Ashraf, S., Mallakpour, I., Moftakhari, H., and AghaKouchak, A.: Global Insight into Extreme Events and Land Subsidence: Understanding Drivers, Interplay, and Impacts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14504, https://doi.org/10.5194/egusphere-egu25-14504, 2025.

EGU25-14685 | ECS | Posters on site | HS7.5

Role of moisture transport in extreme flood events in the Brahmaputra basin 

Gayathri Vangala and Vimal Mishra

The Brahmaputra River basin, a complex hydrological system in South Asia, is among the most flood-prone regions in the world. It frequently experiences severe and devastating flood events. The floods are closely linked to the region’s complex atmospheric moisture dynamics, which govern the spatiotemporal distribution of precipitation. However, the mechanisms driving extreme precipitation events, especially their connection to large-scale moisture transport, remain poorly understood. We investigate the role of Integrated Vapor Transport (IVT) in the initiation and intensification of extreme flood events within the Brahmaputra basin.  We analyzed the spatial and temporal patterns of IVT and their correlation with changes in patterns of precipitation. Our findings indicate that IVT, characterized by strong moisture flux convergence, is closely associated with significant increases in rainfall intensity, particularly during the summer monsoon season. The improved understanding of the physical mechanisms behind precipitation intensification can significantly improve forecasting and early warning systems for extreme flood events. These advancements are crucial for mitigating the impacts of extreme floods and enhancing the actionable strategies in one of the world’s most vulnerable regions.

How to cite: Vangala, G. and Mishra, V.: Role of moisture transport in extreme flood events in the Brahmaputra basin, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14685, https://doi.org/10.5194/egusphere-egu25-14685, 2025.

Maharashtra is India’s second-largest state in population and third-largest in area. It faces escalating environmental challenges from diverse hydroclimatic extremes, including droughts, floods, and cyclones. IPCC reports underscore the need for a comprehensive understanding of socioeconomic vulnerability (SEV) to address the inequality and differential impacts of these hazards within a robust risk assessment framework. Several national and regional vulnerability assessments have been conducted in India and Maharashtra. These studies lack a finer-resolution assessment of socioeconomic vulnerability (SEV), limiting the understanding of localised variations. They also fall short of incorporating a broad range of SEV indicators, which hinders comprehensive vulnerability analysis. The major drivers contributing to vulnerability need to be identified.

The current study advances local adaptation planning by thoroughly evaluating socioeconomic vulnerability (SEV) at Maharashtra's finest resolution of sub-district (talukas/tehsils) level based on the availability of the demographic data. The study utilised composite indicators, which were procured and derived from the latest available Census of India (CoI, 2011) data. This method offers a thorough grasp of susceptibility patterns by concentrating on the finest possible spatial resolution based on the limited availability of the resource for socioeconomic indicator information. The subjectivity constraints of weighing these socioeconomic indicators have been addressed using the non-parametric Data Envelopment Analysis (DEA) optimisation technique. The study also utilised variance-based factor analysis to identify the major contributing drivers of the SEV for Maharashtra. Additionally, a localised cluster-level SEV analysis is also performed based on multiple administrative divisions to identify the local-level significant indicators. Applying this methodology to 357 sub-districts of Maharashtra reveals a concentration of highly vulnerable sub-districts in the Central and Eastern Vidarbha Zone, moderately vulnerable districts in the Central Maharashtra Plateau Zone, and less vulnerable districts in the North Konkan Coastal. The factor analysis results also highlight agricultural labourers, marginal working populations, and marginal female working populations as the most critical drivers influencing vulnerability for the entire Maharashtra State.

This proposed framework is generic and comprehensive and can be applied to any other state or spatial scale. The results of this study can assist policymakers and stakeholders in identifying vulnerable hotspots and developing proper social and economic policies to better understand and improve the socioeconomic situations of Maharashtra at the sub-district scale.

Keywords: Data envelopment analysis, Principal component analysis, Socioeconomic indicators, Sub-district level, Vulnerability analysis.

How to cite: Dev, I., Chakraborty, A., and Karmakar, S.: A Comprehensive Socioeconomic Vulnerability Analysis Using Robust DEA Technique at the Finest Resolution of Sub-District Scale in Entire Maharashtra State of India: Identifying Significant Vulnerability Drivers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14777, https://doi.org/10.5194/egusphere-egu25-14777, 2025.

EGU25-14945 | ECS | Posters on site | HS7.5

Multi-day extreme precipitation caused major floods in India during summer monsoon of 2024 

Dipesh Singh Chuphal, Iqura Malik, Rajesh Singh, Gayathri Vangala, M Niranjan Naik, Urmin Vegad, Nandana Dilip K, Parthsarathi Mukhopadhyay, J Parvathy Selvan, Vivek Kapadia, and Vimal Mishra

Climate change has increased the risk of extreme precipitation and flooding in India. During the 2024 summer monsoon season, three major extreme precipitation events occurred across the western, southern, and northern states of India, leading to widespread flooding in these regions. We examine the causes and impacts of extreme precipitation and flood events using a combination of observational data, reanalysis datasets, and hydrological models. In all the three regions, extreme rainfall occurred immediately after multiday continuous precipitation, resulting in catastrophic flooding. The 3-day extreme precipitation that caused flooding in the three regions had return periods of more than 75 years, 100 years, and 200 years, respectively. The primary moisture source for the Gujarat floods (western India) was the Arabian Sea, while the floods in Andhra Pradesh and Telangana (southern India) were driven by dual moisture advection from both the Arabian Sea and the Bay of Bengal. For the floods in northern India, the dominant moisture sources were recycled land moisture and southwest moisture transport from the Arabian Sea. These moisture inflows, combined with favorable atmospheric conditions and pre-existing saturated soils, resulted in severe flooding across all regions. Our findings underscore the escalating challenge of managing such extreme events as their frequency and intensity rise with global warming.

How to cite: Singh Chuphal, D., Malik, I., Singh, R., Vangala, G., Naik, M. N., Vegad, U., Dilip K, N., Mukhopadhyay, P., Selvan, J. P., Kapadia, V., and Mishra, V.: Multi-day extreme precipitation caused major floods in India during summer monsoon of 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14945, https://doi.org/10.5194/egusphere-egu25-14945, 2025.

EGU25-16503 | Orals | HS7.5

Living with floods: strengthening adaptation and preparedness through better risk communication 

Serena Ceola, Irene Palazzoli, Chiara Binelli, Chiara Puglisi, and Raya Muttarak

Europe has been experiencing catastrophic floods. On October 19, 2024, the city of Bologna located in the Emilia-Romagna region, in central-northern Italy received 180 mm of rainfall – its average for September and October – within just 24 hours, with an intensity typical of summer thunderstorms. The region has yet barely recovered from severe flooding and landslides caused by the Storm Boris in September 18-19, 2024. These recent events followed the worst Emilia-Romagna's flood in a century, in May 2023, which resulted in 17 deaths and an estimated 8.5 billion euro in damages cost. With severe storms and their accompanying devastating floods projected to become more frequent and intense, and with an increasing concentration of people living close to rivers, Europe must urgently scale up its adaptation efforts. Understanding the preparedness of flood-prone regions and their populations is therefore crucial. 

A recent survey among 1,795 residents of Emilia-Romagna conducted in July 2024 (after the devastating flood events in May 2023) investigated their flood risk awareness and preparedness to face such crises. The survey reveals that most respondents were unprepared for flood event and that providing accessible information on local flood risk can play a vital role in bolstering personal adaptation measures. Respondents reported that providing educational resources on flood preparedness and the provision of guidance on flood prevention and management are also fundamental to effective flood responses and enhanced citizens’ resilience. Effective risk communication can also generate a spillover effect, fostering broader climate awareness and a commitment to mitigation. We therefore envisage that adaptation initiatives must prioritize citizen involvement and access to reliable flood risk information. Engaging citizens as active participants in adaptation planning ensures that strategies align with local needs and are more likely to gain public support. In this way Europe can create more resilient communities and stimulate meaningful climate action. 

 

How to cite: Ceola, S., Palazzoli, I., Binelli, C., Puglisi, C., and Muttarak, R.: Living with floods: strengthening adaptation and preparedness through better risk communication, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16503, https://doi.org/10.5194/egusphere-egu25-16503, 2025.

EGU25-17944 | ECS | Posters on site | HS7.5

Socio-economic vulnerability assessment at building scale: A case study in Youngsan watershed, South Korea 

Hung Vu Quoc, Dongkyun Kim, and Chi Vuong Tai

Despite the growing efforts in quantifying disaster vulnerability, its assessment at the building scale remains a challenge. In this study, we aim to quantify the socio-economic vulnerability index (SEVI) for every building by combining its housing price data with SEVI values at sub-district level. The methodology consists of three main steps. First, the latest social and economic data from Gwangju and Jeollanam provinces of Youngsan watershed were collected at sub-district and district levels. These data served as inputs for the Principal Component Analysis (PCA) algorithm to compute SEVI at sub-districts level. Second, housing price data were gathered for as many residential buildings as possible and combined with the SEVI values of their associated sub-districts. This combination was conducted with an assumption that households with more expensive housing are less vulnerable to natural disasters. Finally, a geocoding technique was adopted to tranform physical addresses into geospatial locations, enabling the assignment of vulnerability values into building polygons for further analysis and visualization. The outcome of this study is a map detailing the vulnerability levels of individual buildings. The main findings reveal that (1) the Southeastern part of Youngsan watershed tends to be more vulnerable to disaster, with sub-districts exhibiting high SEVI levels mostly located near the Youngsan River; (2) sub-districts with the highest number of highly vulnerable buildings tend to have only medium SEVI levels. By integrating these insights into disaster risk mitigation efforts, policymakers can develop more detailed and effective strategies for both short and long term, focusing on each building individually.

 

Acknowledgement

This study was supported by Korea Environment Industry & Technology Institute (KEITI) through R&D Program for Innovative Flood Protection Technologies against Climate Crisis Program (or Project), funded by Korea Ministry of Environment(MOE)(RS-2023-00218873).

How to cite: Vu Quoc, H., Kim, D., and Vuong Tai, C.: Socio-economic vulnerability assessment at building scale: A case study in Youngsan watershed, South Korea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17944, https://doi.org/10.5194/egusphere-egu25-17944, 2025.

This study uses catchment-level statistical characterization of reanalysis and precipitation datasets to create a typology of the evolution atmospheric conditions associated with hydrologic dam incidents in the eastern United States. Extreme precipitation elevates the risk of dam overtopping, which is the main cause of a third of US dam failures. As the intensity of precipitation is predicted to increase in future climates, understanding the evolution of precipitation-generating features within the atmospheric system, alongside the hydrologic conditions leading up to the failure, is a crucial initial step in properly characterizing and predicting the risk of dam failures during a range of weather events.

This analysis divides the US eastern seaboard into four regions to examine the meteorological events within a 30-day period prior to a dam’s hydrologic incident. Initial analysis of the northeast sub-region found that although quasi-stationary fronts (frontal) or tropical cyclones (TC) present their own risk, compound events combining the two were most immediately associated with numerous dam failures over a broad region. However, catchment-level precipitation analysis further highlighted that the basins that had failures during these TC/frontal events also had numerous smaller precipitation events in the timeframe leading up to the incident. This longer tendency towards higher precipitation is associated with persistent large-scale patterns within the 14 days prior to the event. Ongoing analysis of the other sub-regions within the study area will further characterize variations across the region, as well as provide deeper insight into processes that determine how precipitation is distributed within the catchment.  

How to cite: Hence, D. and Orok, H.: Characterizing the Atmospheric Conditions Leading to Dam Overtopping in the Eastern United States, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18032, https://doi.org/10.5194/egusphere-egu25-18032, 2025.

EGU25-18771 | Posters on site | HS7.5

Comparative Analysis of Flash Flood Vulnerability and Resilience through Multidimensional Indices 

Jose María Bodoque, Estefania Aroca, and Juan Antonio García

This research examines the relationships between vulnerability and resilience concerning flash flood risk in the Castilla y León region (Spain). The study compares vulnerability and resilience indices and investigates the relationships between their elements and flash flood risk variables. It discusses the necessity of enhancing vulnerability and resilience evaluations by integrating diverse aspects, encompassing social, economic, ecosystem, physical, institutional, and cultural dimensions. The methodology incorporates statistical and spatial approaches, such as Spearman correlation, bivariate choropleth maps, and regression models. The study reveals that vulnerability and resilience are related but represent distinct constructs. Despite a weak correlation between the vulnerability and resilience indices (r = 0.06), significant correlations exist among various elements within these indices. This underscores the need for a multidimensional approach that combines theoretical frameworks with practical implementation, providing insights for policy makers and guiding future research efforts. For example, the resilience index and the vulnerability index's exposure component are strongly correlated (r = 0.40). The spatial relationships are more evident between the vulnerability and resilience indices, with a local R2 of 0.74 between the resilience index and the different dimensions within the vulnerability index. The study also finds significant correlations between specific vulnerability elements and flash flood risk variables, particularly in the exposure component (r = 0.59 for the population at risk) and the institutional dimension (r = -0.48 for the total flood indemnities provided by the insurance company). Notably, the vulnerability and resilience indices show a strong spatial relationship with critical infrastructure at risk, with a local R2 of 0.85.  This research highlights the need for more research to improve vulnerability and resilience assessments and tailor them to specific local contexts. This underscores the need for a multidimensional approach that combines theoretical frameworks with practical implementation, providing insights for policy makers and guiding future research efforts. 

How to cite: Bodoque, J. M., Aroca, E., and García, J. A.: Comparative Analysis of Flash Flood Vulnerability and Resilience through Multidimensional Indices, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18771, https://doi.org/10.5194/egusphere-egu25-18771, 2025.

EGU25-19293 | Posters on site | HS7.5

Large scale atmospheric cross-peril stochastic catastrophe models 

Martin Kadlec and Anežka Švandová

Impact Forecasting, a catastrophe model development branch of Aon, develops catastrophe models for various countries and perils, including floods, windstorms, earthquakes, wildfires, hurricanes, and typhoons. These models are crucial for the insurance and reinsurance industry to estimate losses in terms of severity and frequency.

To address the increasing demand for evaluating losses across multiple countries and perils, Impact Forecasting has started using large ensembles of global climate models (GCM) and regional climate models (RCM). These models serve as a common forcing input for catastrophe models related to atmospheric perils such as flooding (fluvial, pluvial, and coastal), summer storms, windstorms, and wildfires.

The use of GCM/RCM as common forcing input offers two main advantages:

  • Spatial Consistency: The data are spatially consistent at a global or continental scale, which helps in addressing the issue of cross-country correlations.
  • Variability: The large number of available ensembles provides sufficient variability to build a representative stochastic catalogue of potential catastrophes.

We will present several examples of this approach (Pan-European flood model, the Canadian flood and wildfire models), where common GCM/RCM inputs are used to provide a consistent view of losses across large regions and various perils. We will also show how we adress the issue of low resolution of GCM/RCM models using machine learning.

How to cite: Kadlec, M. and Švandová, A.: Large scale atmospheric cross-peril stochastic catastrophe models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19293, https://doi.org/10.5194/egusphere-egu25-19293, 2025.

EGU25-19347 | Orals | HS7.5

 Compound, Cascading, and Multihazard Perils: Lessons Learnt from Hurricanes Helene and Milton 

Jose Luis Salinas Illarena, Sacha Khoury, Jessica Williams, and Sarah Hartley

The 2024 hurricane season presented unique challenges in hydrological and risk modeling with the consecutive landfalls of Hurricanes Helene and Milton in Florida, USA. This study investigates the compounded, cascading, and multihazard perils associated with these events, focusing on the interplay of antecedent conditions, vulnerability, and exposure.

One of the factors considered was the influence of antecedent soil moisture and river storages on hydrological modeling. Hurricane Helene, which made landfall in early September, saturated the soil and filled river systems to near capacity. These conditions significantly altered the hydrological response to Hurricane Milton, which struck just two weeks later. Hydrological models had to account for the already saturated soils and high river levels, which exacerbated flooding and runoff, leading locally to more extensive inundation than would have been predicted for Hurricane Milton in isolation.

Another point of focus is the impact on vulnerability, particularly the presence of debris from Hurricane Helene affecting the region's resilience. Debris obstructed drainage systems, increased the potential for secondary flooding, and complicated emergency response efforts. Additionally, the weakened infrastructure and partially damaged buildings from the first hurricane heightened the susceptibility of the population to the subsequent event, resulting in higher overall damage and more prolonged recovery periods.

Finally, the study examines the effect on exposure, including the "build-back-better" phenomenon observed in even previously to the aftermath of Hurricane Helene. While some structures were rebuilt to higher standards, providing increased resilience against Hurricane Milton, many areas remained in a state of recovery, with temporary shelters and makeshift repairs that were less able to withstand the impact of the second hurricane. This mixed state of exposure created a complex landscape for risk assessment and emergency planning.

Overall, the lessons learnt from Hurricanes Helene and Milton underscore the importance of incorporating antecedent conditions into hydrological models, considering the cumulative impacts on vulnerability, and recognizing the dynamic nature of exposure in multihazard scenarios. These insights are crucial for improving predictive models and enhancing resilience strategies in regions prone to sequential natural disasters.

How to cite: Salinas Illarena, J. L., Khoury, S., Williams, J., and Hartley, S.:  Compound, Cascading, and Multihazard Perils: Lessons Learnt from Hurricanes Helene and Milton, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19347, https://doi.org/10.5194/egusphere-egu25-19347, 2025.

EGU25-19638 | ECS | Orals | HS7.5

Quantitative fluvial and coastal flood risk assessments for European coastal cities considering various climate scenarios and ecosystem-based approaches for hazard mitigation 

Rui Figueiredo, Raymundo Rangel-Parra, Gianbattista Bussi, Paola Ceresa, Rossella Mocali, Michele Bendoni, Carlo Brandini, Luís Campos Rodrigues, Mar Riera-Spiegelhalder, Juan Iglesias, Jokin Etxebarria, and Sara Soloaga

Coastal cities, due to their geographic location, are particularly exposed to hydro-meteorological and climate-related natural hazards. The EU-funded Horizon 2020 project SCORE (Smart Control of the Climate Resilience in European Coastal Cities), within its various activities, aims to provide a better understanding of how to mitigate and manage the effects of extreme events, particularly floods, in European coastal cities. Achieving this objective requires adequate knowledge about the probabilities and potential consequences of flood events based on a probabilistic risk assessment framework encompassing models of flood hazard for different climate scenarios, exposed elements, and vulnerability.

In this context, the present work describes the methodology and presents the results of quantitative risk assessments developed for fluvial and coastal flooding for three of SCORE’s coastal city living labs (CCLLs): Massa (Italy), Oarsoaldea (Spain) and Vilanova i la Geltrú (Spain). The risk assessments cover four types of exposed elements, i.e., population, buildings, roads, and railways, and a number of flood scenarios, both in terms of different climate conditions and considering the absence or presence of ecosystem-based approaches (EBAs) for the mitigation of fluvial flood hazard. This allows understanding both the impact that climate change is expected to have on flood risk in these CCLLs, and the influence that specific EBAs can have in reducing fluvial flood risk from a baseline to an improved infrastructural condition (i.e., residual risk).

The results of the assessments provide invaluable information to support flood risk management activities, such as gridded maps of losses for each hazard scenario and type of exposed element, maps of estimated average annual losses (AAL), and aggregate loss metrics at urban scale. In addition, they serve as input for subsequent tasks of the SCORE project, such as the development of cost-benefit analyses of specific EBA solutions and the development of financial resilience strategies for the flood risk management of the three CCLLs.

How to cite: Figueiredo, R., Rangel-Parra, R., Bussi, G., Ceresa, P., Mocali, R., Bendoni, M., Brandini, C., Campos Rodrigues, L., Riera-Spiegelhalder, M., Iglesias, J., Etxebarria, J., and Soloaga, S.: Quantitative fluvial and coastal flood risk assessments for European coastal cities considering various climate scenarios and ecosystem-based approaches for hazard mitigation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19638, https://doi.org/10.5194/egusphere-egu25-19638, 2025.

EGU25-20548 | ECS | Posters on site | HS7.5

Investigating the impact of considering hazard preconditions in scenario-based risk estimation 

Amelie Hoffmann and Daniel Straub

Scenarios are commonly used in alpine hazard risk management. They can serve different purposes such as design of structures and mitigation measures, risk analysis for the prioritization of measures and the allocation of resources, and in preparing for the unexpected. In scenario-based quantitative risk analysis, few scenarios are used to obtain an estimate of risk, i.e., the annual expected losses, by approximating the loss exceedance curve. The scenarios are frequently selected from a range of plausible hazard intensities, such as discharges for hydrologic hazards or volumes for gravitational hazards and evaluated in terms of their expected consequences.

In the absence of long event records and lack of comprehensive data collection (e.g., from measurement stations or field investigations), as is often the case in alpine catchments, it can be difficult to assign occurrence probabilities to the specified hazard intensities. The recurrence of the scenarios (and thereby the expected consequences) is frequently equated with the recurrence of meteorological trigger conditions, thereby neglecting the effects of necessary preconditions for hazards to occur. In turn, to consider preconditions as additional parameters in evaluating the recurrence of expected consequences, it is required to adapt the development of the loss exceedance curve. For that purpose, we derive the unconditional probability distribution of the expected consequences from the distributions of damages conditional on the preconditions.

Using the example of an alpine catchment, we illustrate how considering preconditions invalidate the assumption of equating the recurrence frequency of the triggering conditions with the recurrence frequency of the consequences. We investigate the impact of considering different preconditions on the risk estimates by modelling the physical response of the natural environment to these trigger conditions. The information about frequency and magnitude of hazard scenarios is combined with the probability of different preconditions to derive scenarios that are representative of consequences with given recurrence frequency, hence better reflect the overall risk.

How to cite: Hoffmann, A. and Straub, D.: Investigating the impact of considering hazard preconditions in scenario-based risk estimation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20548, https://doi.org/10.5194/egusphere-egu25-20548, 2025.

EGU25-1331 | PICO | HS7.9

Balancing Benefits and Challenges of Regreening in Semi-Arid Climates. 

Mokhammad suleiman Mostamandi, Sergey Osipov, Georgiy Stenchikov, and Yoshihide Wada

Land surface characteristics significantly influence regional weather patterns, with the surface heat budget being governed by factors such as surface albedo, emissivity, heat fluxes, and evaporation.  In this study, we investigate the impact of regreening on regional temperature regimes and livability factors in the semi-arid NEOM region in northern Saudi Arabia. We conduct numerical experiments using a high-resolution (1.5x1.5 km grid spacing) Weather Research and Forecast (WRF) regional model to study the effect of converting the surface type from desert to savanna trees with 45% density across a 3.2E5-hectare area. We evaluate the effects of regreening using simulations over three summer months.

Our results indicate that regreening reduces surface temperature by approximately 0.6°C, primarily due to enhanced evapotranspiration. However, irrigation and increased moisture fluxes contribute to a rise in wet-bulb temperature, an important metric for heat stress. Specifically, the wet-bulb temperature increased by 0.7°C, potentially exacerbating heat stress in the region. Notably, maintaining this regreened area requires about 1.2 billion tons of water for irrigation during the summer period.

In semi-arid regions used in this study, where natural water sources are absent, irrigation relies on desalinated water. Although desalination ensures a reliable water supply, it requires substantial energy and generates emissions that contribute to atmospheric warming and negatively impact regional air quality.

These findings highlight the trade-offs associated with regreening in semi-arid regions, where reductions in surface temperature due to evapotranspiration may be offset by increased heat stress, energy demands, and environmental costs of desalination. This emphasizes the need for integrated and sustainable approaches to such interventions.

How to cite: Mostamandi, M. S., Osipov, S., Stenchikov, G., and Wada, Y.: Balancing Benefits and Challenges of Regreening in Semi-Arid Climates., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1331, https://doi.org/10.5194/egusphere-egu25-1331, 2025.

EGU25-2201 | ECS | PICO | HS7.9

Impacts of South-to-North Water Diversion Project  Continuous Water Diversions on Increased Precipitation and Decreased Temperature in Water-Receiving Areas 

Haodong Deng, Qingming Wang, Yongnan Zhu, Yunpeng Gui, Yong Zhao, and Xiaoxue Chen

Climate impacts of the South-to-North water diversion project in China on water-receiving areas (WRA) is simulated by the Weather Research and Forecasting (WRF) model. The results show that during the 2015—2022 water diversion period, the WRA experiences increased precipitation and decreased temperature. Annual precipitation increased by 2.8 mm, mainly dominated by non-convective precipitation (1.92 mm), Although the upwind region receives more water, the increase in water vapor flux is more dramatic in the downwind region due to the spring northwest monsoon; The decreased temperature effect is most pronounced in spring (over 0.15 °C), and over 10 mm of evaporation increase in the downwind region. The sensible heat flux decrease is less pronounced than the latent heat flux increase, mainly because of the insulating effect, which prevented evaporative cooling reduction. This study advances our understanding of the mechanisms by which large-scale water diversion affects WRA climates.

How to cite: Deng, H., Wang, Q., Zhu, Y., Gui, Y., Zhao, Y., and Chen, X.: Impacts of South-to-North Water Diversion Project  Continuous Water Diversions on Increased Precipitation and Decreased Temperature in Water-Receiving Areas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2201, https://doi.org/10.5194/egusphere-egu25-2201, 2025.

EGU25-4645 | ECS | PICO | HS7.9 | Highlight

Irrigation indirectly sustains rainfed crops in India and China through atmospheric recycling 

Akash Koppa, Francesca Bassani, Victoria Deman, Damián Insua-Costa, Jessica Keune, Diego Miralles, and Sara Bonetti

India and China host ~45% of the world’s irrigated area, with irrigation accounting for 65–75% of the total water usage in these countries. The impact of intense irrigation on regional precipitation and even monsoonal dynamics is well acknowledged. However, the degree to which recycled irrigation water helps sustain rainfed crops, acting as an indirect source of water supply, remains unknown. This is especially important in India and China, where irrigated crops are grown in close proximity to rainfed ones. In this study, we quantify (a) the contribution of atmospherically recycled irrigation water to rainfall over rainfed regions, and (b) the importance of this contribution for satisfying the water demand of rainfed crops. 

The methodology involves 20 years of global Lagrangian atmospheric model (FLEXPART) simulations tracking 10 million air parcels. These simulations were constrained by ERA5 reanalysis data and satellite-based terrestrial evaporation data from GLEAM4. Evaporation from irrigated and rainfed crops was computed using the FAO-Penman method. Air parcels that contribute to rainfall over rainfed crops were tracked backward in time for a period of 15 days. Subsequently, the contribution of evaporation from irrigated crops to rainfall over rainfed crop regions was computed. 

Preliminary results show that, on average, ~15% of the rainfall over rainfed crops can be attributed to irrigation evaporation in upwind regions. The irrigation contribution to rainfall reaches as high as 50% in parts of the intensively irrigated Indo-Gangetic plain. Stark differences are observed between India and China, with irrigation contribution to rainfall over rainfed regions being substantially higher in India. Removal of this irrigation contribution would result in an average increase in evaporative stress of ~10%, with a maximum increase of 25%. With irrigation projected to expand to sustain crop production in a changing climate, it is likely to play an indirect yet significant role in supporting rainfed crops as well. Our results highlight the relevance of considering recycled irrigation as an essential source of water supply for rainfed crops. 

How to cite: Koppa, A., Bassani, F., Deman, V., Insua-Costa, D., Keune, J., Miralles, D., and Bonetti, S.: Irrigation indirectly sustains rainfed crops in India and China through atmospheric recycling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4645, https://doi.org/10.5194/egusphere-egu25-4645, 2025.

Northwest China is a typical arid and semi-arid region and an important climate-sensitive and vulnerable area. In recent decades, this region has experienced a notable trend toward humidification. Understanding the characteristics and trends of precipitation and the atmospheric water vapor cycle in this area is essential for predicting the future evolution of this phenomenon. Using observational and reanalysis data, this study classified precipitation in Northwest China from 1961 to 2020 into 20 levels, ranging from light to heavy events. The analysis shows that the overall increase in precipitation is largely driven by extreme precipitation events exceeding the 90th percentile, with the rising frequency of heavy precipitation accounting for most of the observed changes. Precipitation intensity across different levels is positively correlated with both external moisture transport and regional moisture contributions. Heavy precipitation events are closely linked to stronger moisture inflows and more active regional recycling processes. Enhanced precipitation efficiency and shorter moisture residence times further facilitate the occurrence of intense precipitation in the region. The increasing trend in heavy precipitation is primarily associated with greater moisture contributions from cross-equatorial flows over the Indian Ocean and increased local evaporation. These factors enhance land-atmosphere interactions and precipitation efficiency, thereby driving the frequency and intensity of extreme precipitation events.

How to cite: Hua, L.: Extreme precipitation driven humidification in Northwest China: Changes in precipitation characteristics and atmospheric water vapor transport in Northwest China, 1961-2020, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5660, https://doi.org/10.5194/egusphere-egu25-5660, 2025.

EGU25-6217 | ECS | PICO | HS7.9

Non-local impacts of upwind vegetation on soil moisture across South America 

Shijie Jiang, Feini Huang, and Wei Shangguan

Soil moisture variability and drought severity in South America are increasingly pressing challenges, driven by global climate change and extensive land use change. In particular, the biophysical effects of vegetation not only influence local water availability, but also have non-local impacts through atmospheric moisture transport. Understanding how upwind vegetation dynamics affect downwind soil moisture anomalies (SMA) is critical to addressing these challenges. In this study, we investigate the role of upwind vegetation in modulating SMA from 2001 to 2018 using a deep learning framework. We identified a pronounced sensitivity of downwind SMA to Amazonian vegetation, with water transport dominating during more than half of the drought events. Hotspots in the eastern Amazon were found where increased vegetation could significantly enhance atmospheric moisture supply to downwind regions, thereby buffering soil moisture variability in Brazilian agricultural zones. Overall, our results highlight the critical role of atmospheric moisture transport in shaping regional hydrology and emphasize the interconnectedness of land use change and hydrological processes. By integrating vegetation dynamics and non-local moisture transport into hydrological and land management strategies, this research provides actionable insights for improving drought resilience and managing the hydrological impacts of vegetation in a changing climate.

How to cite: Jiang, S., Huang, F., and Shangguan, W.: Non-local impacts of upwind vegetation on soil moisture across South America, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6217, https://doi.org/10.5194/egusphere-egu25-6217, 2025.

EGU25-6823 | ECS | PICO | HS7.9

Simulating Precipitation Reductions from Land-Use Changes in South America: A Novel Emulator Approach 

Luis Gustavo Cattelan, Marina Hirota, Jess Baker, Stephen Sitch, Chris Huntingford, Jefferson Goncalves De Souza, and Emanuel Gloor

The Amazon rainforest faces mounting pressure from deforestation, resource extraction, and infrastructure development, with approximately 20% of its forest cover lost in recent decades. These changes, alongside rising temperatures and shifting precipitation patterns, are severely impacting the forest’s resilience Deforestation not only reduces local evapotranspiration and alters surface energy balance—leading to declines in precipitation and increases in temperature—but also disrupts downstream rainfall through changes in water vapor transport, affecting regions dependent on Amazonian moisture.

While Earth System Models (ESMs) offer critical insights into these impacts, their high computational demands limit the range of scenarios they can assess. To overcome this, ESM emulators such as the IMOGEN system provide efficient, pattern-scaled projections. However, existing emulators often fail to incorporate essential local climate feedbacks, which are critical for understanding the Amazon’s resilience to climate change and land-use shifts.

This study enhances the IMOGEN/PRIME emulator to account for localized rainfall changes driven by upstream land-use alterations and deforestation. Using the WAM-2layers model with ERA5 data, we generate sensitivity matrices to quantify how evapotranspiration (ET) from different Amazon regions contributes to precipitation elsewhere. These are combined with ET anomalies simulated by the JULES land-surface model under various land-use scenarios. Scenarios are derived from the LuccME framework (Aguiar et al., 2016) and include: Sustainability, reflecting socio-economic and environmental advancements; Fragmentation, representing resource depletion and inequity.; Middle of the Road, a mix of both; Extreme cases, such as total South American deforestation, are also assessed.

By combining ET anomalies with water vapor transport sensitivities, precipitation change patterns are spatially mapped for each scenario and incorporated into IMOGEN. This integration allows for simulations of cascading effects from land-use changes on regional precipitation and climate.

The enhanced emulator offers a powerful framework to assess deforestation-driven climate impacts, including their effects on forest resilience and biogeochemical cycles. This approach provides a comprehensive evaluation of Amazon forest dieback risks under diverse CMIP6-aligned scenarios, delivering critical insights for conservation and sustainable land management strategies.

 

How to cite: Cattelan, L. G., Hirota, M., Baker, J., Sitch, S., Huntingford, C., Goncalves De Souza, J., and Gloor, E.: Simulating Precipitation Reductions from Land-Use Changes in South America: A Novel Emulator Approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6823, https://doi.org/10.5194/egusphere-egu25-6823, 2025.

Located in the Congo River basin, the Cuvette Centrale is a densely forested peatland containing billions of tons of carbon. Past work has shown that this peatland is susceptible to large-scale drying trends, which could lead to substantial carbon release to the atmosphere. Understanding the sources of atmospheric water that sustain the Cuvette Centrale, as well as changes to these sources, is essential for characterizing current and future vulnerability. In this presentation, I will share recent work that examines the sources of moisture for the Cuvette Centrale over the first two decades of the 21st century. The results indicate that a substantial fraction of mean annual precipitation falling in the Cuvette Centrale arises as both local evaporation and evaporation from elsewhere in the Congo Basin. An analysis of annual anomalies reveals a multi-decadal drying trend occurring in the Cuvette Centrale, which may be associated with changes occurring throughout key evaporation source areas. Likewise, important links are shown between key ecohydrologic dynamics and moisture recycling to the Cuvette Centrale, such as changes in upwind evaporative stress. This work provides an approach for examining and interpreting changing hydroclimatic vulnerability of critical, global carbon stocks, such as in tropical peatlands. Furthermore, this work underlines the importance of monitoring land-surface changes that could affect moisture recycling to the Cuvette Centrale, such as expanding deforestation across the Congo Basin.

How to cite: Keys, P.: Moisture recycling and vulnerability of Congo's peatlands, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7817, https://doi.org/10.5194/egusphere-egu25-7817, 2025.

EGU25-10508 | ECS | PICO | HS7.9

Evapotranspiration and Feedback Effects with Climate and Land Use Change in the Eastern German Lowlands 

Somayeh Ahmadpour, Yasin Bayzidi, and Katja Trachte

Evapotranspiration (ET) is a vital component of the hydrological cycle, mediating energy, water, and carbon exchanges on land surfaces and the atmosphere, which are critical for agricultural water availability. Understanding the spatiotemporal variability of ET and its relationship with atmospheric drivers and land use/land cover change (LUCC)  is crucial for assessing environmental impacts on regional water cycles and improving water resource management.

This study focuses on the lowlands in eastern Germany. It is a predominantly agricultural region with a continental climate. Despite being one of the driest areas in Germany, 45% of its land is used for agriculture. Using environmental data obtained by MODIS (ET, temperature, solar radiation, and LUCC) and the German Weather Service (relative humidity, precipitation, wind speed, soil moisture, and vapor pressure deficit), ET trends and drivers are analyzed from 2000 to 2020. The objectives are to (i) identify key factors influencing ET and (ii) estimate the effects of climate change and LUCC on ET. 

Results reveal a slight increase in annual ET (taking into account the European vegetation period), with spatial trends showing increases of up to 7.17%, particularly in the southern and southeastern regions. Over the same period, Temp and VPD rose by 37% in the western and eastern areas, while RH decreased by more than 55% in areas experiencing higher Temp and VPD levels. Significant LUCC was observed, including a 22.24% decrease in cropland-to-grassland conversion and a 14.75% increase in grassland-to-cropland conversion, leading to a 21% decline and a 10% increase in ET, respectively.

Among climatic factors, VPD, Temp, RH, and SR had the most substantial influence on ET variability, contributing 28.24%, 27.68%, and 26.84%, respectively. Overall, climate change accounted for 97% of ET variation, underscoring its dominant role. Notably, discrepancies between ET and climatic drivers in western, eastern, and southeastern regions align with drought periods documented in this study. Our findings highlight the important role of Temp and RH in agricultural and water resources management, particularly in the context of climate change.

How to cite: Ahmadpour, S., Bayzidi, Y., and Trachte, K.: Evapotranspiration and Feedback Effects with Climate and Land Use Change in the Eastern German Lowlands, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10508, https://doi.org/10.5194/egusphere-egu25-10508, 2025.

EGU25-12170 | ECS | PICO | HS7.9

Hydroclimatic simulations sensitivity to land use changes  

Mariana Castañeda-Gonzalez, Siavash Pouryousefi Markhali, Annie Poulin, Jean-Luc Martel, Richard Arsenault, François Brissette, Béatrice Turcotte, Olivier Asselin, and Richard Turcotte

Historical changes in land use have shown different effects on climatic and hydrological processes across spatial and temporal scales. Among these, snow accumulation, snowmelt, and evapotranspiration are key processes sensitive to land use changes that can directly influence streamflow production at the catchment scale. The potential future effects of land use changes on streamflow production highlight the importance of assessing the sensitivity of modelling tools commonly used to produce hydrological projections, such as hydrological models (HMs) and regional climate models (RCMs). Therefore, this study aims to assess the individual and combined effects of RCM- and HM-simulated land use changes on the streamflow simulations of five North American catchments. To assess RCM-simulated land use change impacts, three simulations from the Canadian RCM version 5 (CRCM5) were used: a reference simulation (current land uses), a forested scenario (100% forest land use), and a grass scenario (100% grass land use), following the Land-Use and Climate Across Scales (LUCAS) protocol. Two distributed HMs, WASIM and HYDROTEL, were used to evaluate HM-simulated land use change effects on streamflow under the same reference, forest and grass scenarios. Results indicated that RCM-simulated land use changes had a greater impact on streamflow than those simulated by HMs alone. Regarding the differences between hydrological models, HYDROTEL showed higher sensitivity to land use changes in snow processes, while WASIM showed greater sensitivity in modelling evapotranspiration. Further comparisons with a modified version of the GR4J hydrological model provided additional insights into how model structures influence the level of sensitivity to land use, highlighting the importance of each hydrological model internal formulations. Moreover, this study underscores the need for further research into how HMs represent complex land use changes and emphasizes the importance of selecting appropriate tools for specific local hydroclimatic conditions and land use dynamics to improve hydrological modelling and water resources management.

How to cite: Castañeda-Gonzalez, M., Pouryousefi Markhali, S., Poulin, A., Martel, J.-L., Arsenault, R., Brissette, F., Turcotte, B., Asselin, O., and Turcotte, R.: Hydroclimatic simulations sensitivity to land use changes , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12170, https://doi.org/10.5194/egusphere-egu25-12170, 2025.

EGU25-14837 | ECS | PICO | HS7.9

On the Link Between Physical Aridity and Rainfall Intermittency 

Mijael Rodrigo Vargas Godoy, Annalisa Molini, Yannis Markonis, and Gabriele Villarini

Rainfall intermittency is a defining characteristic of the hydrology in arid and semi-arid regions. These climates experience prolonged droughts interrupted by brief, intense rainfall events, which have substantial effects on landforms, ecosystems, and water resources. Under climate change, intermittent precipitation patterns are expected to become more prevalent across a wider range of climates. Despite this, there is limited research on the link between rainfall intermittency and physical aridity. Furthermore, high-resolution representation of rainfall variability remains a significant source of uncertainty in rainfall modeling and downscaling. Herein, we investigate the relationship between rainfall intermittency, its temporal scaling behavior, and aridity from a climatological standpoint. We hypothesize that intermittency is shaped by fine-scale processes, such as land-atmosphere interactions and local water and energy dynamics, alongside large-scale atmospheric forces. By analyzing extensive hourly and sub-hourly precipitation datasets from the Contiguous United States (NOAA US-HPD) and Australia (Australian Bureau of Meteorology), we uncover a clear functional relationship between intermittency and aridity metrics across diverse water-limited climates. These findings offer a foundation for enhancing precipitation downscaling techniques and understanding future precipitation regimes in regions with limited water availability.

How to cite: Vargas Godoy, M. R., Molini, A., Markonis, Y., and Villarini, G.: On the Link Between Physical Aridity and Rainfall Intermittency, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14837, https://doi.org/10.5194/egusphere-egu25-14837, 2025.

EGU25-15031 | PICO | HS7.9

Observational Evidence of Increased Afternoon Rainfall Downwind of Irrigated Areas 

Peter Greve, Amelie U. Schmitt, Diego G. Miralles, Sonali McDermid, Kirsten L. Findell, Almudena Garcia-Garcia, and Jian Peng

Irrigation plays a vital role in addressing the growing food demand of an increasing global population. About 70% of worldwide freshwater withdrawals are used for irrigation, and of the ca. 16 million km2 of global cropland, about 20% are irrigated. Due to the massive redistribution of water across the land surface and pumping of groundwater resources, irrigation represents one of the most critical and direct human interventions on the coupled water and energy cycles. As irrigated farmland continues to expand, understanding the climate impact of extensive irrigation becomes increasingly important. Yet, the effect on rainfall patterns near irrigated areas remains less clear. Here, we detect a systematic impact of extensive irrigation at the global scale on the location and downwind rainfall amount of afternoon rain. Using two global, high-resolution, sub-daily precipitation datasets, we show that afternoon rain events occur more often 10 km to 50 km downwind and less often upwind of extensively irrigated land. However, we also find that the total amount of heavy afternoon rain downwind of irrigated areas is lower than upwind. Our results provide large-scale observational evidence of the local precipitation dynamics and land-atmosphere interactions surrounding irrigated areas to provide new insights for regional water management and help constrain the representation of these processes in next-generation climate and weather forecasting models.

How to cite: Greve, P., Schmitt, A. U., Miralles, D. G., McDermid, S., Findell, K. L., Garcia-Garcia, A., and Peng, J.: Observational Evidence of Increased Afternoon Rainfall Downwind of Irrigated Areas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15031, https://doi.org/10.5194/egusphere-egu25-15031, 2025.

EGU25-18802 | ECS | PICO | HS7.9

Revisiting global oceanic and terrestrial moisture sources based on state-of-the-art Lagrangian transport simulations  

Victoria M. H. Deman, Damián Insua-Costa, and Diego G. Miralles

Understanding atmospheric moisture sources and their transport pathways is essential for advancing our knowledge of hydrological processes, regional precipitation patterns, and climate variability. In this study, we analyze continental and oceanic moisture sources with a focus on climatological patterns and long-term trends. To revisit our understanding of global moisture sources, we leverage a new global, open-source dataset spanning 45 years (1979–2024), derived from Lagrangian transport modeling with FLEXPART (Bakels et al, 2024). It contains 3-hourly information on the position of the air parcels which are distributed globally according to density as well as different associated state variables such as temperature or specific humidity. 

The outputs from the Lagrangian model are fed to HAMSTER, a tool for source attribution that is constrained by observational data of both precipitation and evaporation (Keune et al., 2022). Notably, we analyze the moisture sources for each continent separately in addition to the sources for the global land area as a whole, which enables us to: (1) assess intra-continental precipitation and evaporation recycling ratios, (2) investigate the inter-continental transport of moisture, and (3) analyze the role of different ocean basins in providing moisture to specific terrestrial regions. Moreover, the dataset’s longer record and its higher spatial and temporal resolution compared to their predecessors allow for an up-to-date investigation of the change in moisture source contributions over the past four decades. This includes exploring the impact of climate change and land use alterations on the hydrological cycle and how these changes affect the balance between oceanic and terrestrial moisture sources per continent. Overall, this study refines our understanding of atmospheric moisture transport dynamics in a changing climate, highlighting ongoing shifts in our global hydrological cycle.  

 

References

Bakels, L., Tatsii, D., Tipka, A., Thompson, R., Dütsch, M., Blaschek, M., Seibert, P., Baier, K., Bucci, S., Cassiani, M., Eckhardt, S., Groot Zwaaftink, C., Henne, S., Kaufmann, P., Lechner, V., Maurer, C., Mulder, M. D., Pisso, I., Plach, A., Subramanian, R., Vojta, M., and Stohl, A.: FLEXPART version 11: improved accuracy, efficiency, and flexibility, Geosci. Model Dev., 17, 7595–7627, https://doi.org/10.5194/gmd-17-7595-2024, 2024. 

Keune, J., Schumacher, D. L., and Miralles, D. G.: A unified framework to estimate the origins of atmospheric moisture and heat using Lagrangian models, Geosci. Model Dev., 15, 1875–1898, https://doi.org/10.5194/gmd-15-1875-2022, 2022. 

How to cite: Deman, V. M. H., Insua-Costa, D., and G. Miralles, D.: Revisiting global oceanic and terrestrial moisture sources based on state-of-the-art Lagrangian transport simulations , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18802, https://doi.org/10.5194/egusphere-egu25-18802, 2025.

EGU25-19822 | ECS | PICO | HS7.9

Water Use in Agroecosystems: An Extended Budyko Framework 

Sara Cerasoli, Giulia Vico, and Amilcare Porporato

Climate change and human activities are rapidly altering watershed dynamics, with agricultural management being a key protagonist in modifying water partitioning within watersheds. The Budyko framework relates precipitation partitioning to climatic conditions through fundamental constraints of water and energy availability. However, managed watersheds deviate from the natural Budyko curve due to their modified water balance, particularly through irrigation inputs.
This study develops a process-based extension of the Budyko framework by explicitly incorporating irrigation into the water balance equations. Our approach accounts for both stochastic rainfall and irrigation inputs, considering different management methods, climatic conditions, and crop parameters. This allows us to predict and explain the shifts in water partitioning observed in managed watersheds within the Budyko space.
We validate our theoretical predictions using real-world basins that span diverse climates and management practices - from rainfed to fully irrigated agriculture. The framework successfully captures the transitions between different agricultural strategies through their modified evaporative patterns, showing good agreement with observed data across various irrigation methods and crop types, demonstrating how these interventions have altered hydrological patterns on a global scale.
This framework advances our understanding of agricultural feedbacks on the water cycle through modified evapotranspiration patterns. The ability to characterize these changes using minimal parameters makes it valuable for improving hydrological models and detecting irrigation practices through their distinctive signatures in the Budyko space.

How to cite: Cerasoli, S., Vico, G., and Porporato, A.: Water Use in Agroecosystems: An Extended Budyko Framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19822, https://doi.org/10.5194/egusphere-egu25-19822, 2025.

EGU25-20298 | ECS | PICO | HS7.9

Simulating moisture-vegetation feedbacks in the Amazon under drought and deforestation scenarios 

Caterina Vanelli, Lauren Seaby Andersen, Simon Felix Fahrländer, Arie Staal, Werner von Bloh, Nico Wunderling, and Boris Sakschewski

The Amazon rainforest, a global biodiversity hotspot and home to over 40 million people—2.2 million of whom are Indigenous—plays a critical role in the global regulation of water and carbon cycles. However, its unique biocultural diversity is increasingly threatened by climate and land-use changes, which could shift vegetation in multi-stable forest areas to savannah- or grassland-like states. Satellite-based observations, Earth system models, and rainfall exclusion experiments provide evidence of the rainforest's critical dependency on precipitation and seasonality. Additionally, complex systems approaches suggest that forests in bistable areas are maintained by cascading moisture recycling, a process that is significantly reduced by regional deforestation.

This research employs  the dynamic global vegetation model LPJmL (version 5.9), incorporating variable tree rooting strategies and coupled with moisture network data derived from the Lagrangian moisture transport model UTrack. The observation-based monthly moisture networks for the period 2003–2014 proportionally redistribute evapotranspiration from LPJmL over the Amazon basin as precipitation, providing a partially dynamic representation of the moisture-vegetation feedback. Future scenarios, including increased drought frequencies (based on the major droughts of 2005 and 2010 as analogs for future extremes)and two deforestation projections (based on the Governance and Business as Usual scenarios from Soares-Filho et al. (2006)), are implemented to analyse rainfall changes and the forest's local and telecoupled moisture response in LPJmL. We also provide a first estimate of the collective contribution of Indigenous Peoples’ Lands to terrestrial precipitation in the Amazon, by explicitly accounting for atmospheric water flows originating from Indigenous territories as in the data provided by Garnett et al. (2018). 

These findings add to our understanding of forest-water interactions from a moisture recycling perspective, assessing the impacts of drought and deforestation while highlighting the role of Indigenous land management. Advances in modelling could support future assessments of forest resilience and tipping risks, providing critical inputs for forest management and underscoring the urgency of effective climate mitigation.

How to cite: Vanelli, C., Andersen, L. S., Fahrländer, S. F., Staal, A., von Bloh, W., Wunderling, N., and Sakschewski, B.: Simulating moisture-vegetation feedbacks in the Amazon under drought and deforestation scenarios, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20298, https://doi.org/10.5194/egusphere-egu25-20298, 2025.

EGU25-21892 | ECS | PICO | HS7.9

Vegetation and Wind Speed Dominate Precipitation-Evaporation Recycling Processes during 1980–2021 

Yiying Wang, Chiyuan Miao, Qi Zhang, Jiajia Su, Jiaojiao Gou, Qingyun Duan, and Alistair GL Borthwick

Atmospheric moisture plays a crucial role in connecting global water and energy exchanges within the water cycle. Using a water recycling model, this study examines the spatiotemporal characteristics of precipitation and evaporation recycling ratios (PRR and ERR) across 200 river basins worldwide from 1980 to 2021, with data fused from three reanalysis datasets. The results reveal that regions near the equator exhibit higher PRR values, signifying strong moisture self-sufficiency, whereas arid, high-latitude, and inland regions show lower PRR values, indicating a higher dependence on external water vapor. Temporal trends indicate a decline in PRR and ERR in regions such as North America, South Africa, and Australia, while some areas in Central Asia and Europe have experienced increases. Structural Equation Modeling reveals that land cover, especially the Leaf Area Index (LAI), and wind speed are key drivers of spatial and temporal variability in water recycling ratios. The study classifies river basins into four categories based on their water recycling trends: ‘Enhanced Exchange Basins,’ ‘Beneficial Basins,’ ‘Shrinkage Basins,’ and ‘Reduced Exchange Basins.’ These classifications provide valuable insights into regional water cycles and can inform targeted water resource management strategies, crucial for addressing challenges like water scarcity and ecosystem restoration.

How to cite: Wang, Y., Miao, C., Zhang, Q., Su, J., Gou, J., Duan, Q., and Borthwick, A. G.: Vegetation and Wind Speed Dominate Precipitation-Evaporation Recycling Processes during 1980–2021, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21892, https://doi.org/10.5194/egusphere-egu25-21892, 2025.

EGU25-736 | Orals | AS1.22

Isotopic Signatures of Precipitation: Linking Tropospheric and Surface Processes in India's Core Monsoon Zone 

Supriya Chakraborty, Neha Trivedi, and Rajendra Trivedi

The monsoon system is a dynamic and complex component of the atmospheric water cycle, profoundly impacting weather, climate, and human activities. A variety of meteorological observations are used to understand the monsoon system. The isotopic technique provides a unique perspective on moisture dynamics, enhancing our understanding of the monsoon system. The isotopic signature of precipitation is shaped by numerous geographical and environmental variables, making only select regions suitable for in-depth monsoon isotopic studies. The central Indian region, a pivotal monsoon zone, exhibits distinct characteristics ideal for studying monsoon dynamics. Key features include the passage of the monsoon trough- a modified Intertropical Convergence Zone, and frequent low-pressure systems (LPS) from the northern Bay of Bengal, contributing significantly to summer monsoon rainfall. Notably, rainfall variability in central India shows an out-of-phase relationship with northeastern India. Furthermore, central Indian rainfall strongly correlates with the All-India Summer Monsoon Rainfall, serving as a reliable proxy. Despite its potential, the isotopic technique remains underutilized in this core monsoon zone (CMZ: approximately defined by an area 18-28oN, 65-88oE) for monsoon research.

We report a multi-year (2016-2021) precipitation isotopic record obtained from Sagar, a site in the CMZ of India. We explore the relationship between isotopic signatures and regional-scale atmospheric processes mediated by diabatic heating and its vertical distribution pattern, the LPSs, moisture source dynamics, monsoon trough variability, and other meteorological conditions. We also examine the role of recycled rainfall in modulating the precipitation isotopic variability.

We have computed the diabatic heating profiles over India's CMZ. The calculated heating profiles are strongly associated with the monsoon rainfall variability expressed through a precipitation index over the CMZ. We observed a strong association between precipitation isotopic depletion and tropospheric heating. Our analysis reveals that LPSs significantly influence rainfall isotopic values through their origin, trajectory, and intensity. These systems and associated convective activity yield depleted isotopic signatures. A strong inverse relationship exists between LPS intensity and corresponding precipitation isotopic values.

Terrestrial evaporation, leading to substantial recycled rainfall, plays a pivotal role in modulating precipitation isotopic variability. A notable inverse correlation exists between precipitation isotopes and recycled rainfall. The isotopic depletions resulting from diabatic heating, LPSs, and recycled rainfall collectively manifest the amount effect, highlighting a common link among these processes.

The out-of-phase isotopic patterns observed in central and northeastern India mirror the region's dipolar rainfall variability, rendering the CMZ an optimal location for proxy-based reconstructions of past rainfall variability.

How to cite: Chakraborty, S., Trivedi, N., and Trivedi, R.: Isotopic Signatures of Precipitation: Linking Tropospheric and Surface Processes in India's Core Monsoon Zone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-736, https://doi.org/10.5194/egusphere-egu25-736, 2025.

EGU25-1423 | Posters on site | AS1.22

Comparison of local and remote controlling factors on the precipitation isotopic variation in northwestern Ethiopia 

Shuang-Ye Wu, Zhaojun Zhan, Zelalem Bedaso, and Yonas Hagos

Investigating the mechanisms of precipitation isotope variation is essential for interpreting hydrological processes and reconstructing isotope-based paleoclimate records, especially in arid regions with complex precipitation patterns like Ethiopia. This study analyzed the seasonal and interannual variations of stable isotopes in precipitation at Addis Ababa, northwestern Ethiopia, using observed and simulated monthly δ18O data from GNIP and IsoGSM2, respectively. Results show a significant 18Op depletion during the rainy season (June to September, JJAS) compared to the dry season. Locally enhanced convection, intensified convective and large-scale precipitation, and higher relative humidity may contribute to this depletion. These local meteorological variables explained nearly half of the JJAS δ18Op variation. In addition, moisture contribution and rainout process along the path from the Southern Indian Ocean (SIO) to the western Ethiopian Highland also contribute to the JJAS 18Op depletion. This study also demonstrates the relationship between El Niño and the Southern Oscillation (ENSO) and the interannual variation of JJAS δ18Op in Ethiopia: the warm (cold) phase of ENSO modulates the enrichment (depletion) of JJAS 18Op via the less (more) JJAS rainfall. Warm SST anomalies in the Central Pacific weaken the intensity of the Indian Summer Monsoon (ISM), suppress the convective activities, and reduce the amount and intensity of JJAS rainfall over Ethiopia, causing significant 18Op enrichment during El Niño years. Our study provides insights into understanding hydrological processes and interpreting paleoclimate δ18Op records in East Africa.

How to cite: Wu, S.-Y., Zhan, Z., Bedaso, Z., and Hagos, Y.: Comparison of local and remote controlling factors on the precipitation isotopic variation in northwestern Ethiopia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1423, https://doi.org/10.5194/egusphere-egu25-1423, 2025.

EGU25-2539 | ECS | Orals | AS1.22

The Water Vapor Origin of a Rainstorm Event in the Taklamakan Desert 

Yongqi Gong and Haipeng Yu

In July 2021, the Taklamakan Desert (TD) experienced an unprecedented rainstorm with daily precipitation exceeding 61.1 mm, triggering mudslides and landslides, highlighting the increasing frequency of extreme precipitation events even in arid regions under global warming. The water vapor sources and transport paths of this rainstorm are still puzzling due to the insufficient representation of physical processes in previous analytical models, leading to possible deviations from reality. Here, using the online Eulerian Weather Research and Forecasting model with water vapor tracer (WRF-WVT), we aim for an improved understanding of water vapor sources of the rainfall event. Results demonstrate that the most important water source for this event is water vapor from local evapotranspiration, contributing to 32.77% of the rainstorm moisture. Water vapor from Upstream Westerlies (28.95%) and East Asian Drylands (28.54%) are transported over the precipitation area by the westerlies owing to the strong lower-level low-pressure system, being the second-most important precipitation source. These sources contribute significantly more than other regions, including the Arabian Sea (5.56%), the Tibetan Plateau (2.16%), and the South Asian Monsoon (0.77%). External moisture sources collectively provide over 65.98% of the precipitation, underscoring their important role. Notably, local evapotranspiration significantly influences precipitation, exceeding the contributions from other individual sources. By comparing with the 2016 precipitation event, it is found that a low-pressure trough extending southward to the west of the TD plays a significant role in the 2021 rainstorm event. The presence of the trough significantly enhances the moisture transport of the westerlies and the upward motion, contributing to the occurrence of extreme precipitation events.

How to cite: Gong, Y. and Yu, H.: The Water Vapor Origin of a Rainstorm Event in the Taklamakan Desert, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2539, https://doi.org/10.5194/egusphere-egu25-2539, 2025.

EGU25-3310 | Orals | AS1.22

High-Frequency Isotopic Analysis Unveils the Complexity of Convective Rainfall Dynamics in the Central Amazon 

Didier Gastmans, Vinícius Santos, Shujiro Komiya, Ricardo Sánchez-Murillo, Sam Jones, Zayra Christine Sátyro Santos, Rafaela Rodrigues Gomes, Susan Trumbore, Gerd Gleixner, and Ana Maria Duran-Quesada

The Amazon region is recognized as one of the world's most significant active convective areas, generating precipitation systems that regulate the climate and weather across the region. Climate projections indicate increased convection over South America, expected to intensify extreme events and amplify their impacts on society. Stable water isotopes are a valuable tool for investigating the formation and evolution of extreme rainfall events in tropical regions. This study presents high-frequency (5-30 minutes) isotope data for rainfall (n=115) and vapor (Picarro Inc., USA L2140i analyzer) from 19 convective events at the ATTO tower site (25/Jan-08/Feb 2024), coupled with various meteorological data (Rain Micro Radar, ATTO tower, Reanalysis, GOES-16). Rainfall and vapor exhibited distinct isotopic signatures with similar temporal trends, with vapor being more depleted in 𝛿18O (-13.78 to -8.92‰) than rainfall (-6.28 to +1.03‰).  Rainfall events were short-lived (< 1 hour) and associated with lower cloud top temperature (-33ºC to +9°C). The averaged 𝛿18O variability within (intra-) and between events (intra: -6.28 to -4.03‰, between: -5.13‰ and +1.03‰), suggests a complex interplay of factors influencing precipitation formation. These factors likely include moisture transport, limited vertical development, and the incorporation of forest evapotranspiration. This study provides valuable insights into the intricate relationship between the Amazon rainforest and rainfall formation. The generated knowledge and data can contribute to improving atmospheric models and understanding the potential impacts of climate change on the Amazon's hydroclimatic system.

How to cite: Gastmans, D., Santos, V., Komiya, S., Sánchez-Murillo, R., Jones, S., Santos, Z. C. S., Gomes, R. R., Trumbore, S., Gleixner, G., and Duran-Quesada, A. M.: High-Frequency Isotopic Analysis Unveils the Complexity of Convective Rainfall Dynamics in the Central Amazon, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3310, https://doi.org/10.5194/egusphere-egu25-3310, 2025.

EGU25-4013 | Orals | AS1.22

Acceleration of the Hydrological Cycle under Global Warming for the Poyang Lake Basin in Southeast China: An Age-Weighted Regional Water Tagging Approach 

Jianhui Wei, Joel Arnault, Thomas Rummler, Benjamin Fersch, Zhenyu Zhang, Patrick Laux, and Harald Kunstmann

Global warming is accelerating the global water cycle. However, quantification of the acceleration and regional analyses remain open. Accordingly, in this study we address the fundamental hydrological question: Is the water cycle regionally accelerating/decelerating under global warming? For our investigation we have implemented the age-weighted regional water tagging approach into the Weather Research and Forecasting WRF model, namely WRF-age, to follow the atmospheric water pathways and to derive atmospheric water residence times defined as the age of tagged water since its source. We apply a three-dimensional online budget analysis of the total, tagged, and aged atmospheric water into WRF-age to provide a prognostic equation of the atmospheric water residence times and to derive atmospheric water transit times defined as the age of tagged water since its source originating from a particular physical or dynamical process. The newly developed, physics-based WRF-age model is used to regionally downscale the reanalysis of ERA-Interim and the MPI-ESM Representative Concentration Pathway 8.5 scenario exemplarily for an East Asian monsoon region, i.e., the Poyang Lake basin (the tagged water source area), for historical (1980-1989) and future (2040-2049) times. In the warmer (+1.9 °C for temperature and +2% for evaporation) and drier (-21% for precipitation) future, the residence time for the tagged water vapor will regionally decrease by 1.8 hours (from 14.3 hours) due to enhanced local evaporation contributions, but the transit time for the tagged precipitation will increase by 1.8 hours (from 12.9 hours) partly due to slower fallout of precipitating moisture components. These findings reveal the physical mechanisms behind dry-getting-dryer at regional scales.

How to cite: Wei, J., Arnault, J., Rummler, T., Fersch, B., Zhang, Z., Laux, P., and Kunstmann, H.: Acceleration of the Hydrological Cycle under Global Warming for the Poyang Lake Basin in Southeast China: An Age-Weighted Regional Water Tagging Approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4013, https://doi.org/10.5194/egusphere-egu25-4013, 2025.

The Ganga Basin, a region vital for agriculture and water resources, is heavily influenced by monsoonal rainfall patterns. Understanding the sources of this rainfall and their role in extreme weather events is critical. This study investigates the transport and contribution of moisture from two major sources the Bay of Bengal and the Arabian Sea on extreme rainfall events in the Ganga Basin from 2012 to 2023. We focus on analyzing the dynamics of moisture flow and the contributions of these sources during periods of heightened rainfall caused by cyclonic systems and other meteorological factors. Using a Lagrangian trajectory model, we track moisture fluxes and quantify water vapor transport from both the Bay of Bengal and the Arabian Sea. Our findings highlight the pivotal role of the Bay of Bengal in the Ganga Basin's rainfall, particularly during monsoon extremes. The Bay of Bengal's proximity to the Ganga Basin and its larger surface area make it the primary moisture source. The moisture generated in the Bay, aided by the monsoon winds, moves inland, directly influencing the seasonal and extreme rainfall patterns over the region. Additionally, cyclonic activity such as tropical storms and depressions further intensifies moisture transport, causing localized flooding and extreme rainfall events that alter the regular monsoon cycle. While the Arabian Sea does contribute to the Ganga Basin’s rainfall, especially during specific monsoonal periods, its influence is more intermittent and weaker compared to the Bay of Bengal. Moisture transport from the Arabian Sea is less direct, with its contributions more noticeable during particular timeframes, outside the peak monsoon season. This study provides a comprehensive understanding of how moisture recycling within the Ganga Basin interacts with moisture fluxes from the Bay of Bengal and the Arabian Sea. We assess how much each of these moisture sources influences extreme rainfall events, revealing the interconnectedness between the Ganga Basin’s moisture recycling processes and the external moisture inputs. This analysis is crucial in understanding the dependency of the Ganga Basin’s rainfall on these external moisture sources, as well as their combined contribution to extreme rainfall events. By examining these dynamics, the study contributes to a more precise understanding of the mechanisms that drive extreme rainfall in the Ganga Basin. It highlights the critical role of the Bay of Bengal in sustaining rainfall, especially during periods of heightened rainfall intensity, and offers insights into how these moisture sources affect the region’s water availability and agricultural productivity.

How to cite: Kumar, R. and Pathak, A.: Tracing Moisture Flow from the Bay of Bengal and Arabian Sea with its Impact on Ganga Basin during Monsoonal Extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4531, https://doi.org/10.5194/egusphere-egu25-4531, 2025.

EGU25-11440 | ECS | Posters on site | AS1.22

Bridging the Scale Gap: Leveraging EOF and Non-Parametric Correlation to Connect Meteorological Fields and Precipitation Isotopes 

Harsh Oza, Ludvig Löwemark, George Kontsevich, Akkaneewut Jirapinyakul, Sakonvan Chawchai, Helmut Duerrast, Mao-Chang Liang, Midhun Madhavan, and Chung-Ho Wang

In the fields of atmospheric and climate science, there is growing use of machine learning and global circulation models. These approaches are becoming increasingly sophisticated with the availability of extensive ground-based and remotely sensed datasets. However, both approaches rely on the availability of large spatial and temporal datasets. For over half a century, stable isotopes of oxygen and hydrogen have been used as robust proxies for understanding hydrometeorological processes, acting as conservative tracers of land-ocean-atmosphere interactions. However, these isotopic measurements are non-continuous and highly discreet. Although satellites such as ACE, TES, Aura, and SCIMACHY do measure the isotopic composition of atmospheric vapour, they carry high uncertainties, making them less reliable. Therefore, despite their promise, these approaches are not readily applicable for deciphering local hydrometeorological processes, primarily due to limited data availability and relatively coarser spatial resolution.

Here, we introduce a simple yet robust approach to link meteorological and atmospheric data with discreet and limited isotopic measurements, aiming to understand how large-scale ocean-atmosphere processes govern local hydrometeorology. We employed Empirical Orthogonal Function (EOF) to identify prominent oceanic and atmospheric patterns over large spatial domains and to reduce dimensionality, thus converting the 3D climate datasets (e.g., ECMWF reanalysis) into 2D representations. We then applied non-parametric correlation technique, specifically Spearman‘s rank correlation, to link the meteorological data with localized, discreet precipitation isotope measurements. Adopting a non-parametric correlation avoids strict assumptions about data distributions. This approach offers significant benefits over traditional and more complex, modern methods by handling non-linearity and spatial heterogeneity. It also provides an effective means of identifying and interpreting local hydroclimatic processes and their linkages to broader atmospheric and oceanic drivers, thereby bridging the gap between large-scale atmospheric factors and local hydrological responses. Consequently, it offers deeper insight into the complex interplay among numerous processes operating at varied spatiotemporal scales.

Our preliminary findings quantitatively highlight the roles of sea surface temperature gradient between the eastern Indian Ocean and the South China Sea, pressure, potential vorticity, boundary layer height, vertical transport, wind speeds, and specific humidity in driving precipitation isotope variability in the Malaya peninsula. These linkages were previously unknown or qualitatively estimated by traditional methods, highlighting the value of this synergistic approach in bridging the spatial data disparities and improving our understanding of the regional drivers in the local hydrological cycle.

How to cite: Oza, H., Löwemark, L., Kontsevich, G., Jirapinyakul, A., Chawchai, S., Duerrast, H., Liang, M.-C., Madhavan, M., and Wang, C.-H.: Bridging the Scale Gap: Leveraging EOF and Non-Parametric Correlation to Connect Meteorological Fields and Precipitation Isotopes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11440, https://doi.org/10.5194/egusphere-egu25-11440, 2025.

EGU25-12038 | ECS | Orals | AS1.22

Long-term isotopic monitoring in Southeast region of Brazil 

Amanda Soares, Didier Gastmans, and Vinicius dos Santos

Observations on the variability of the isotopic composition of rainfall have been used to understand the effects of climate change, but there is a gap in this type of analysis in tropical regions. Studies in tropical regions are extremely important to assess the influence of meteorological parameters on the isotopic composition of rainfall, as these regions have a unique climate that greatly influences the distribution of rainfall regimes. The aim of this study is to evaluate the historical series of isotopic data from the GNIP station at Rio Claro, located in Southeast region of Brazil, since the climate in this area is directly influenced by a variety of atmospheric systems that impact the variation in isotopic composition of rainfall. This study presents the analysis of a 10-year dataset of daily isotopic precipitation data (δ¹⁸O, δ²H, and d-excess). The isotopic signatures for δ¹⁸O ranged from -21.74‰ to 9.09‰ VSMOW, and for δ²H the variation was from -158.45‰ to 44.9‰ VSMOW, determining the Local Meteoric Water Line (LMWL) of Rio Claro as δ²H = 7.76 * δ¹⁸O + 10.97. The values of the LMWL are close to the Global Meteoric Water Line (GMWL), demonstrating a balance between evaporation and vapor recirculation processes. The rainy season LMWL (δ²H = 7.72 * δ¹⁸O + 10.3) is also close to the LMWL for Rio Claro. However, when considering data from the dry season, which represents 24% of the rainfall data, the LMWL indicates stronger vapor recirculation processes (δ²H = 7.7 * δ¹⁸O + 12.12), caused by rainfall initiated by cold fronts. Trend analysis using the Mann-Kendall test revealed a decreasing trend for δ²H and d-excess, while rainfall showed an increasing trend over the study period. These findings highlight the significance of determining the LMWL for Rio Claro, as it provides a valuable reference for isotopic studies in the region. Moreover, the analysis offers a comprehensive overview of the isotopic dataset, which can be further expanded and refined through the integration of synoptic meteorological data.

How to cite: Soares, A., Gastmans, D., and dos Santos, V.: Long-term isotopic monitoring in Southeast region of Brazil, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12038, https://doi.org/10.5194/egusphere-egu25-12038, 2025.

Northern India receives rainfall from dual precipitation systems: Indian Summer Monsoon (ISM) and the Westerlies. Isotopic analysis of precipitation water and water vapor isotopes from the region can serve as a tracer to identify the moisture source and atmospheric phenomenon associated with the advection of moisture-laden air parcel. Water isotopic ratios (δ17O, δ18O) and secondary parameters (d-excess and 17O-excess) provide critical insights in understanding the monsoon dynamics of the region. 17O-excess enables us to estimate relative humidity conditions at the source region. This study presents the first continuous record of triple oxygen isotopes in the North Indian region (a low-latitude region but still having high heat exchange capacity due to extensive glacial mass).

Event based rainwater samples have been collected using a standard rain collector and high-resolution isotopic data of atmospheric vapor has been acquired using Picarro-L2140i installed at Manali station for June-July-August-September (JJAS) 2024. Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) back trajectory analysis suggests that moisture responsible for rainfall in Manali originates from Bay of Bengal, Arabian Sea, Westerlies and some local moisture sources. Specific humidity changes plotted along the back trajectories carry vital information regarding moisture percentage calculations from various sources. Local Meteoric Water Line (LMWL) have also been generated for the region which suggests significant influence of continental recycling and evaporative enrichment. Quantitative estimation of moisture contribution from various sources and effects of local meteorological parameters (e.g. wind speed & direction, relative humidity, temperature, rainfall amount) on isotopic values of atmospheric water observed in this study will be discussed at the time of presentation.

How to cite: Singh, A. and Dixit, Y.: Understanding summer monsoon variability in Northern India through isotopic signatures of precipitation water and water vapor isotopes , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12645, https://doi.org/10.5194/egusphere-egu25-12645, 2025.

EGU25-12738 | Posters on site | AS1.22

Water Isotopologue Time Series across Tropical Sites during ENSO extremes 

Lucinda Bryce, Kim Cobb, Jessica Conroy, Samantha Levin, Manlin Xu, Germain Hernández, Ricardo Sánchez-Murillo, Madeleine Hardt, Nicole Murray, Elisabeth Holland, Wendy-Jane Powell, Xi-Kai Wang, and Syria Lejau

Potential anthropogenic shifts in the hydroclimate impacts of El Niño Southern Oscillation (ENSO) extremes are poorly resolved by available data. Water isotopologues provide valuable tracers of hydroclimatic processes, including the balance of precipitation versus evaporation and the relative importance of regional versus local drivers of hydroclimate variability  (Dee et al., 2023 and references therein; Moerman et al., 2013). However, very few water isotopologue datasets exist in the tropical Pacific, and those that do fail to resolve a full ENSO cycle. In this study, we present oxygen isotope (δ18O) and deuterium (δ2H) time series for precipitation, seawater, as well as sea-surface salinity time series from 5 sites spanning the tropical Pacific across the 2023/24 El Niño event and 2024/25 La Nina event.. Weekly seawater and daily rainwater δ18O time series from the Galapagos, Fiji, Hawaii, and Kiritimati Island, as well as rainwater δ18O time series from northern Borneo and Costa Rica reveal a distinct signature of the 2023/24 El Niño event. Preliminary analyses indicate that seawater δ18O values reflect both local and remote processes, with the relative balance being largely site-dependent. This study provides quantitative estimates of rainfall and seawater δ18O anomalies through a cycle of ENSO extremes, and investigates regional drivers of hydrologic circulation across space and time. Taken together, our results provide the first empirical dataset of ENSO-related δ18O anomalies spanning the tropical Pacific across a complete ENSO cycle, with applications to data-model intercomparison studies and investigations of tropical Pacific hydroclimatic processes. 

How to cite: Bryce, L., Cobb, K., Conroy, J., Levin, S., Xu, M., Hernández, G., Sánchez-Murillo, R., Hardt, M., Murray, N., Holland, E., Powell, W.-J., Wang, X.-K., and Lejau, S.: Water Isotopologue Time Series across Tropical Sites during ENSO extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12738, https://doi.org/10.5194/egusphere-egu25-12738, 2025.

EGU25-12895 | ECS | Posters on site | AS1.22

Understanding the environmental characteristics of frontal precipitation 

Hongsheng Wang and Jennifer Catto

Climatological studies have marked the important role of atmospheric fronts in the hydroclimate and water cycle of the Earth system, especially in the mid-latitudes. Precipitation associated with fronts is highly affected by the (spatially and temporally) co-existing weather systems with fronts such as atmospheric rivers (ARs) and mesoscale convective systems (MCSs) proved by previous studies. Current work discloses the environmental characteristics of frontal precipitation, which is less discussed, through analyzing the environmental variables including frontogenesis, moisture flux convergence (MFC), and convective available potential energy (CAPE) within the frontal zone. Results show that the extreme-precipitating fronts have higher mean positive frontogenesis and mean positive MFC than non-extreme-precipitating fronts. The study attempts to explicate the role of ARs and MCSs in frontal precipitation by analyzing the statistical distribution and cross-section in the cross-front direction of environmental variables of categorized fronts (co-occurring with ARs, MCSs, and both). There is a distinguishable shift of mean positive MFC distribution towards the high end when fronts co-occur with ARs (including both ARs and MCSs) compared with these with MCSs only, indicating the critical role of ARs in moisture transport to facilitate precipitation within the frontal zone. This work aims to highlight the environmental characteristics of fronts, especially those producing extreme precipitation, contributing to the theoretical understanding of precipitation from the perspective of weather phenomenon.

How to cite: Wang, H. and Catto, J.: Understanding the environmental characteristics of frontal precipitation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12895, https://doi.org/10.5194/egusphere-egu25-12895, 2025.

EGU25-12908 | Posters on site | AS1.22

The NISBO data set – high altitude daily precipitation stable isotope data since 2016 

Johannes Christoph Haas, Giorgio Höfer-Öllinger, and Elke Ludewig

Since August of 2016, daily precipitation samples for stable isotope analysis are collected at the Sonnblick Observatory (SBO). The SBO is located on the peak of Mt. Hoher Sonnblick, at an elevation of 3106 m above sea level, on the main ridge of the Alps in Austrias Hohe Tauern Region [1, 2]. These samples are analyzed using laser absorption spectroscopy (OA-ICOS, LGR T-LWIA-45-EP) at ISOLAB Salzburg, geoconsults in-house laboratory, producing data for the precipitations δ2H, δ18O and δ17O stable isotope composition.

To our knowledge, this data set, both in location (highly alpine) as well as in temporal resolution (daily data) and length of the data (multiple, full years) is unique. The aim of this Poster is to raise awareness about this data set and to discuss preliminary findings, before publishing the data for further work.

As expected, the data show pronounced seasonal variations (up to approx. 25 ‰ for δ18O, 10 ‰ for δ17O and 120 ‰ for δ2H) and notable differences between the various years in the data set, which compares well to the longterm observation from the nearby Böckstein Station of the Austrian Network of Isotopes in Precipitation and Surface Waters (ANIP) [3, 4]. However, the ANIP station, located in a valley, at 1014 m a s l, is collected in monthly intervals only.

Besides these seasonal and annual variations, significant differences in isotopy between single precipitation events can be observed. At a maximum, from December 27. to December 28. 2017 (21,6 mm of precipitation) δ18O and δ2H drop from ‑8.07 and ‑85.89 ‰ VSMOW to ‑30.14 and ‑224.60 ‰ VSMOW, a difference of -22.07 and -138.71 ‰ respectively, within a day. Similarly, from March 04. to March 05. 2020 (2.5 mm of precipitation), δ18O and δ2H rise from ‑22.10 and -172.04 ‰ VSMOW to ‑2.22 and ‑47.05 ‰ VSMOW, a difference of +19.88 and +124.99 ‰.

Such changes, reflecting a multitude of possible causes, such as for example altitude effect or different sources of the precipitating moisture (Mediterranean vs. Atlantic in case of the Sonnblick) are generally not seen in the prevailing monthly data and pose an interesting field for further research.

In general, most of the data follow both, the global mean water line (GMWL [5]) and the Austrian mean water line (AMWL [6]); but a trend towards higher δ18O and δ2H values, resulting in a local, daily, water line of approx. δ2H = 6.3 δ18O – 18.1 for this high-alpine environment can be distinguished.

[1] https://www.sonnblick.net/en/about-us/

[2] https://www.sonnblick.net/en/the-observatory/location/

[3] KRALIK, PAPESCH, & STICHLER (2003): Austrian Network of Isotopes in Precipitation (ANIP): Quality assurance and climatological phenomenon in one of the oldest and densest networks in the world. Isotope hydrology and integrated water resources management: 146-149.

[4] https://www.umweltbundesamt.at/wasser/informationen/isotope/isotopenmessnetz-anip

[5] CRAIG, H. (1961): Isotopic Variations in Meteoric Waters. Science, 133: 1072-1073

[6] HAGER, B. & FOELSCHE, U. (2015): Stable isotope composition of precipitation in Austria. AJES, 108: 2-13

How to cite: Haas, J. C., Höfer-Öllinger, G., and Ludewig, E.: The NISBO data set – high altitude daily precipitation stable isotope data since 2016, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12908, https://doi.org/10.5194/egusphere-egu25-12908, 2025.

The age of water vapor in the atmosphere is often invoked to explain a well known discrepancy in the change of the hydrologic cycle with global warming. Although moisture increases at a rate of 7% per degree of global warming, precipitation increases only at a rate of 2% per degree of global warming. The difference between these rates can be explained by a 5% increase in water vapor age per degree of global warming. Although this explanation works on a global scale, it does not explain the spatial distribution in the increase of the age, or the dynamical mechanisms which are responsible for this increase in age.

In this project, we demonstrate the potential of a 3D Eulerian age tracking system for the age of water vapor in a simplified atmospheric general circulation model. The age tracking system works by computing the moments of the age distribution, which form a recursive system. The moments themselves exist as passive tracers, so they can be transported with the water vapor using a consistent transport calculation. This method allows us to track the age of water vapor online in any configuration where the model can be run, including both control and climate change simulations. Our intial tests with an aquaplanet model show a relative increase with age with height and towards the poles, with a decrease over the midlatitude eddies and an increase in the updraft of the Hadley cell. Additionally by resolving the standard deviation of the age distribution we can calculate the shape parameter of the distribution (raio of mean to standard deviation), which shows which regions of the atmosphere are affected by transport from a single pathway and which regions are affected by transport from multiple pathways. We further demonstrate the ability of our age tracking system in more realistic model configurations and climate change scenarios. 

How to cite: Fajber, R. and Boulanger, P.: 3D Eulerian Calculation of water vapor age moments for climate change and atmospheric dynamics studies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14470, https://doi.org/10.5194/egusphere-egu25-14470, 2025.

EGU25-14484 | ECS | Orals | AS1.22

Temporal Evolution of Diurnal Cycle of Rainfall Using Rain Gauge Data Over India 

Thanangka Chutia and Arindam Chakraborty

Hourly rainfall data from 81 Self Recording Rain Gauge stations were analyzed to study the temporal change of the diurnal cycle of rainfall across India between the two periods: 1969-1991 (past) and 1992-2014 (recent). Except east and northeast (ENE) and west India (WI), majority of the stations showed delayed phase of the diurnal cycle of rainfall in recent period.Both frequency and intensity diurnal cycle contributes to the delayed phase over central India (CI) whereas only the intensity diurnal cycle is responsible for advanced phase over WI. Decrease in the number of heavy rainfall events in the past phase contributes most to the delayed phase in CI while increase in the intensity of heavy rainfall events in the recent phase primarily contributes to the advanced phase over WI. Besides, increase in the number of break days over CI is also responsible its delayed phase. The decrease (increase) in CAPE over WI (CI) is responsible for advanced (delayed) phase.

How to cite: Chutia, T. and Chakraborty, A.: Temporal Evolution of Diurnal Cycle of Rainfall Using Rain Gauge Data Over India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14484, https://doi.org/10.5194/egusphere-egu25-14484, 2025.

EGU25-16758 | Posters on site | AS1.22

Dual-Isotope Eddy Covariance Measurements: Insights and Challenges in Ecosystem Water Flux Measurements Over Winter Wheat in Central Germany 

Anas Emad, Leo Oskar Franke, Gökben Demir, Christian Markwitz, Maren Dubbert, and Alexander Knohl

Dual-isotope eddy covariance measurements offer a novel approach for studying water fluxes in ecosystems, providing detailed insights into evapotranspiration (ET) and its components, evaporation (E) and transpiration (T). During the 2024 growing season, a dual-isotope eddy covariance system was deployed over a winter wheat cropland in central Germany, integrating a Los Gatos Research (LGR) Water Vapor Isotope Analyzer with a conventional eddy covariance setup. This system continuously measured isotopic fluxes (δD and δ18O) alongside water vapor, carbon dioxide, and energy fluxes at high temporal resolution. These measurements were supplemented by soil water profiles, biometeorological observations, and vegetation indices.

The isotopic flux data revealed diurnal and seasonal dynamics of water vapor isotopes, linked to environmental drivers such as vapor pressure deficit, soil moisture, and crop phenology. Preliminary results show a diurnal cycle of isotope fluxes of ET, characterized by isotopic enrichment during the middle of the day, with δ18OET reaching -12‰ and δDET reaching -110‰ (both against VSMOW). The results suggest that transpiration dominates ET during peak growth stages, while evaporation increases following precipitation events or during early crop development.

Key challenges include correcting for high-frequency dampening effects and addressing the analyzer’s sensitivity to water vapor concentration under different conditions, particularly during low-flux periods. Despite these challenges, dual-isotope techniques give valuable insights into crop water use strategies and responses to environmental drivers, offer the opportunity for isotope-based flux partitioning, and give a unique dataset for validating isotope-enabled land surface models.

How to cite: Emad, A., Franke, L. O., Demir, G., Markwitz, C., Dubbert, M., and Knohl, A.: Dual-Isotope Eddy Covariance Measurements: Insights and Challenges in Ecosystem Water Flux Measurements Over Winter Wheat in Central Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16758, https://doi.org/10.5194/egusphere-egu25-16758, 2025.

EGU25-18111 | Orals | AS1.22

Moisture sources and transport pathways of summertime intense extratropical cyclones in the North-Atlantic 

Frank Selten, Rikke Stoffels, Chris Weijenborg, and Imme Benedict

Extratropical cyclones are essential for the redistribution of energy, moisture, and momentum from the equator to the poles. Although wintertime extratropical cyclones are relatively well studied, less is known about summertime cyclones. Therefore, this research aims to improve our understanding of how summertime extratropical cyclones in the Northern Atlantic shape the global water cycle. More specifically, we focused on determining the moisture sources of these cyclones and analysed how precipitating air parcels were transported to the cyclone center. Changes in the moisture uptake and transport characteristics during the cyclone life cycle were also evaluated. To this end, 8-day backward trajectories were computed for the 20% most intense storms for three different stages in their life cycle: intensification, time of maximum intensity, and decay. Trajectory calculations were performed for all precipitating air parcels in a 500 km radius surrounding the cyclone center using the Lagrangian analysis tool LAGRANTO. Subsequently, moisture uptakes along the trajectories of only precipitating parcels were identified using the moisture source diagnostic WaterSip. We find that the bulk of the precipitation falls close to the cyclone center and along the fronts, mostly during the intensification phase. The origins of this moisture correspond to areas of high evaporation, with hotspots over the Gulf Stream region and its northeastern extension, and continental sources for cyclones in the Labrador Sea. The source distance is large during intensification, while local evaporation becomes more important during decay. Finally, we discuss the differences between summer and winter, as they have different dependencies on preceding "parent" cyclones for moisture supply.

How to cite: Selten, F., Stoffels, R., Weijenborg, C., and Benedict, I.: Moisture sources and transport pathways of summertime intense extratropical cyclones in the North-Atlantic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18111, https://doi.org/10.5194/egusphere-egu25-18111, 2025.

EGU25-18530 | ECS | Orals | AS1.22

Water vapour isotope anomalies during an atmospheric river event at Dome C, East Antarctica 

Niels Dutrievoz, Cécile Agosta, Amaëlle Landais, Cécile Davrinche, Camille Risi, Sébastien Nguyen, Christophe Leroy-Dos Santos, Inès Ollivier, Elise Fourré, Antoine Berchet, and Jonathan Wille

On December 19-21 2018, an atmospheric river hit the French-Italian Concordia station, located at Dome C, East Antarctic Plateau, 3 269 m above sea level. It induced a significant surface warming (+ 15°C in 3 days), combined with high specific humidity (multiplied by 3 in 3 days) and a strong isotopic anomaly in water vapour (+ 15 ‰ for δ18O). The isotopic composition of water vapour monitored during the event may be explained by (1) the isotopic signature of long-range water transport, and by (2) local moisture uptake during the event. In this study, we use continuous meteorological and isotopic water vapour observations, together with the atmospheric general circulation model LMDZ6iso, to describe this event and to quantify the influence of each of these processes. The presence of mixed-phase clouds during the event induced a significant increase in downward longwave radiative fluxes, which led to high turbulent mixing in the boundary layer. These fluxes are well represented by LMDZ6iso, as are the near-surface temperature and specific humidity. The surface vapour δ18O is accurately simulated during the event, despite an overestimated amplitude in the diurnal cycle outside of the event. Using this LMDZ6iso simulation, we perform a water vapour mass budget in the boundary layer and we show that the primary driver of the positive δ18O anomaly in vapour is surface sublimation, which becomes significantly stronger during the event compared to typical diurnal cycles. The second contribution arises from large-scale moisture advection associated with the atmospheric river. Consequently, the isotopic signal monitored in water vapour during this atmospheric river event reflects both long-range moisture advection and interactions between the boundary layer and the snowpack. Only specific meteorological conditions driven by the atmospheric river can explain these strong interactions. Enhancing the representation of local processes in climate models, especially by incorporating isotopic fractionation during sublimation, could substantially improve the simulation of the isotopic signal over Antarctica. Given the importance of air-snow vapour exchanges at the surface and in the atmosphere and their influence on the isotopic composition of surface snow, such simulations could provide valuable insights into how moisture advection events might affect the climate-scale isotope signal in ice cores.

 

How to cite: Dutrievoz, N., Agosta, C., Landais, A., Davrinche, C., Risi, C., Nguyen, S., Leroy-Dos Santos, C., Ollivier, I., Fourré, E., Berchet, A., and Wille, J.: Water vapour isotope anomalies during an atmospheric river event at Dome C, East Antarctica, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18530, https://doi.org/10.5194/egusphere-egu25-18530, 2025.

EGU25-21252 | Posters on site | AS1.22

Dry periods amplify the Amazon and Congo forests’ rainfall self-reliance 

Lucie Bakels, Lan Wang-Erlandsson, Ruud van der Ent, Arie Staal, Patrick Keys, Delphine Clara Zemp, Ingo Fetz, Makoto Taniguchi, and Line J. Gordon

Moisture recycling is an important source of precipitation in the tropical forests of South America and Africa. Moisture is partly recycled from the tropical forests themselves (forest rainfall self-reliance) and is therefore subject to deforestation, which reduces evaporation. During the dry season, when water is already scarce, a further reduction in precipitation due to decreasing moisture recycling rates could potentially be fatal for already vulnerable ecosystems. It is therefore important to better understand the self-reliance of precipitation in tropical forests. For this reason, we present climatologies of precipitation dependence on evaporation in and from tropical forests using WAM2layers driven by ERA5 data. We find that forest rainfall self-reliance increases during the dry season in both the Amazon and Congo rain forests.

How to cite: Bakels, L., Wang-Erlandsson, L., van der Ent, R., Staal, A., Keys, P., Zemp, D. C., Fetz, I., Taniguchi, M., and Gordon, L. J.: Dry periods amplify the Amazon and Congo forests’ rainfall self-reliance, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21252, https://doi.org/10.5194/egusphere-egu25-21252, 2025.

EGU25-192 | Orals | AS1.23

Global coupled dynamics of tropical easterly waves and tropical cyclone genesis 

Xueqing Du, Jung-Eun Chu, Fei-Fei Jin, and Hung Ming Cheung

Tropical easterly waves (TEWs) are westward-moving waves often within trade winds but occurs ubiquitously in tropics and play a significant role in the genesis of tropical cyclones (TCs). They are well-known as primary precursors of TCs in the Atlantic, yet their global relationship with TCs has been less explored. This study, for the first time, presents the global distribution of TEW activity using a combined thermodynamic and dynamic framework, based on 6-hourly Outgoing Longwave Radiation and curvature vorticity. We then demonstrate that TEWs play a dominant role in approximately 23–71% of global TC genesis, with their highest impacts in the North Atlantic (71%) and Western Pacific (54%). We further identify that TEWs, in its general coupling with TC genesis dynamics, act to intensify TC convection and vorticity in all TC main development regions, albeit the vorticity enhancement is relatively weaker in the North Atlantic. To understand the basin differences in this general TEW-TC relationship, we further investigated background conditions for TC genesis in each basin and found an additional dry environment constraint in the Atlantic TC genesis, yet still delineating the critical role of TEWs in TC development.

How to cite: Du, X., Chu, J.-E., Jin, F.-F., and Cheung, H. M.: Global coupled dynamics of tropical easterly waves and tropical cyclone genesis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-192, https://doi.org/10.5194/egusphere-egu25-192, 2025.

EGU25-559 | ECS | Posters on site | AS1.23

Intraseasonal Oscillations and hydroclimate of Northern South America, Central America and Mexico (Part II: Effects on precipitation) 

Johanna Yepes, Alejandro Builes, Hernan Salas, Juliana Valencia, Paris Rivera, Alejandra Carmona, and Mauricio Bedoya

This work is a second part contribution of the effect of intraseasonal oscillations on precipitation over the study region. The index generated for each wave (Part I) allow to classify events like convection inhibiting (dry) and convection favoring (wet) days and correlate with precipitation data from ERA5 and CHIRPS. Results show positive and negative precipitation anomalies across the region associated with each oscillatory process, which can be linked to anomalies in moisture transport and convection within the atmospheric column. During wet days, the Tropical Easterly Waves contribute up to 20% of precipitation over Caribbean Sea and eastern Pacific (and western Mexico), while the Kelvin waves accounts for 15% over the tropical eastern Pacific. On the other hand, Mixed Rossby-Gravity waves accounts for 15% of precipitation over the eastern Pacific (10°N - and western Mexico) during wet days and, 12% of precipitation on the Pacific coast of Central America during dry days. Finally, the Madden-Julian Oscillation contributes nearly 15% of precipitation over the Pacific coast of Mexico and Central America during wet days. These findings offer new insights into the spatial and temporal patterns within the region related to these intraseasonal oscillations.

How to cite: Yepes, J., Builes, A., Salas, H., Valencia, J., Rivera, P., Carmona, A., and Bedoya, M.: Intraseasonal Oscillations and hydroclimate of Northern South America, Central America and Mexico (Part II: Effects on precipitation), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-559, https://doi.org/10.5194/egusphere-egu25-559, 2025.

EGU25-587 | Orals | AS1.23

The relationship between TC wind profile and TC rainfall profile in DYMOND-NICAM dataset 

Gufeng Bian, Satoh Masaki, and Jianping Tang

Dynamics of the Atmospheric general circulation Modeled On Nonhydrostatic Domains (DYAMOND) dataset which contains nine global models that were all initialized on 1 August 2016 with the analysis from the European Centre for Medium-Range Weather Forecasts (ECMWF) and integrated for 40 days (1 August – 10 September 2016) in convection-permitting resolution. In this study, we choose one of the global models Nonhydrostatic Icosahedral Atmospheric Model (NICAMS) to study TC characteristics further.
To identify TCs in the model output, suitable TC tracking methods were attempted and adopted. It was agreed with the observation that the Western Pacific is the most TC active basin. Although the total number of TCs in DYAMOND-NICAM is similar as the observation, the fewer and more simulated TCs in Eastern Pacific and North Atlantic separately. Then, in order to study the TC structure, we fit the observation surface wind profile using Modified Rankine Vortex (MRV) wind model and get the rainfall profile from GSMAP. Compared with the observation, we found that the model simulated smaller radius of maximum wind (RMW) and rainfall (RMR) and higher peak precipitation.
Further, to study possible relationship between TC wind profile and rainfall profile, some dynamic and thermodynamic variables in the model boundary layer were used. The TC wind model in Chavas et al.(2015) was used to fit the surface wind in order to get more reseasonable TC wind profile.  Then the simulated Ekman pumping transportation (TC vertical mass flux and radial mass flux) was also estimated which could be used to evaluated the precipitation transition efficiency in the model and construct the connection with TC surface wind and precipitation. We found that the accumulated Ekman pumping transportation has a great relationship (correlation efficiency nearly 0.85) with the accumulated precipitation within the TC inner core region. The results might provide some new insights to study and predict realistic and reliable TC precipitation.

How to cite: Bian, G., Masaki, S., and Tang, J.: The relationship between TC wind profile and TC rainfall profile in DYMOND-NICAM dataset, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-587, https://doi.org/10.5194/egusphere-egu25-587, 2025.

Extratropical disturbances are known to impact the genesis and intensification of Mixed Rossby-Gravity waves (MRGW) in the Western Hemisphere (WH). The study provides observational evidence supporting the wave resonance (WR) theory which attempts to explain the intensification of MRGW by extratropical forcing. Wavenumber-frequency cospectral analysis and a bulk measure of growth of MRGW estimated using reanalysis data reveal that the extratropical forcing manifested in the form of eddy momentum flux convergence can create eddy kinetic energy (EKE) and aid the intensification of MRGW via WR mechanism during boreal winter season. However, the WR mechanism does not hold during boreal summer season as the extratropical forcing tends to dampen the MRGW. The analysis also reveals that the Doppler-shifted eastward propagating MRGW in the WH during boreal winter season are not maintained by extratropical forcing, marking another highlight of this study.

How to cite: Mehak, M. and Ettammal, S.: Wave Resonance Induced Intensification of Mixed Rossby-Gravity Waves by Extratropical Forcing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-589, https://doi.org/10.5194/egusphere-egu25-589, 2025.

EGU25-657 | ECS | Orals | AS1.23

Rain Microphysical Characteristics of Rapidly and Slowly Intensifying Tropical Cyclones over North Indian Ocean 

Surya Pramod Jalakam, Pay-Liam Lin, Wei-Yu Chang, Balaji Kumar Seela, and Jayalakshmi Janapati

This study investigates the rain microphysics of tropical cyclones (TCs) that underwent rapid (RI) and slow intensification (SI). TCs that formed in the North Indian Ocean (NIO) are considered, particularly over the Arabian Sea (AS) and Bay of Bengal (BOB) regions for years 2014-2023. Among the 114 TCs recorded in NIO, 42 underwent intensification (RI-22; SI-20). The probability density functions (PDFs) of rain microphysics parameters vary with the intensification mode (RI and SI) and the type of rain (total, stratiform, and convective). The storm height is slightly taller in RI than SI TCs, most notably in convective systems, which underscores the structural difference between the two intensification categories. The contour frequency by altitude diagrams, as well as the vertical mean profiles, reveal that for all rain types, RI TCs have higher rain rates (R), stronger reflectivity (𝑍), larger drop size diameters (𝐷𝑚), and lower drop concentrations (𝑁𝑤) as compared to SI TCs. Results from this study may be used to delineate an impending RI from SI.

How to cite: Jalakam, S. P., Lin, P.-L., Chang, W.-Y., Seela, B. K., and Janapati, J.: Rain Microphysical Characteristics of Rapidly and Slowly Intensifying Tropical Cyclones over North Indian Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-657, https://doi.org/10.5194/egusphere-egu25-657, 2025.

EGU25-663 | ECS | Posters on site | AS1.23

Intraseasonal Oscillations and hydroclimate of Northern South America, Central America and Mexico (Part I: The identification process) 

Alejandro Builes-Jaramillo, Johanna Yepes, Hernán D. Salas, Juan M. Bedoya-Soto, Paris Rivera, Juliana Valencia, and Alejandra M. Carmona

The contribution of intraseasonal variability (10- 90 days) in OLR data across Northern South America, Central America, and Mexico was studied. This variability is driven by planetary and tropical oscillations, including Kelvin waves, Tropical Easterly Waves, Mixed Rossby-Gravity Waves, and the Madden-Julian Oscillation, which display distinct signals in the wavenumber—frequency power spectra. Using the Wheeler-Kiladis methodology (1999) and the spatial EOF analysis for local activity index and composites by Mounier (2007), our findings reveal that intraseasonal variability accounts for 10% to 35% of the total variance, depending on the specific location, with Kelvin waves being the largest contributors to the OLR variance in the study region. This methodology allows to propose a local index for each coupled convective wave aiming to classify as convection inhibiting (dry) and convection favoring (wet) days events. The annual cycle of these dry and wet events for each wave show interesting patterns like a predominance of Tropical Easterly Waves and Mixed Rossby-Gravity Waves during the boreal summer and major Kelvin waves occurring during May and April.

How to cite: Builes-Jaramillo, A., Yepes, J., Salas, H. D., Bedoya-Soto, J. M., Rivera, P., Valencia, J., and Carmona, A. M.: Intraseasonal Oscillations and hydroclimate of Northern South America, Central America and Mexico (Part I: The identification process), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-663, https://doi.org/10.5194/egusphere-egu25-663, 2025.

This research investigates the complex dynamics of tropical cyclone (TC) formation over the North Indian Ocean (NIO), focusing on equatorial wave influences, cyclogenesis mechanisms, barotropic energy conversion, and pre-genesis evolution through high-resolution modeling. Using the severe cyclonic storm Mora (2017) as a primary case study, the research demonstrates that tropical waves play a crucial role in cyclogenesis, particularly through the interaction between Madden-Julian Oscillation (MJO) and Equatorial Rossby (ER) waves. Analysis reveals that MJO provides essential mid-level moisture while ER waves initiate low-level circulation, leading to low formation. A comprehensive composite analysis of tropical cyclones from 2017-2022 further establishes that cyclogenesis predominantly occurs during the interaction of MJO phases 2-3 and ER phases 5-7, while non-developing systems typically involve single wave or no wave interaction. The study investigates the barotropic energy conversion processes within the wave interactions, revealing how eddy kinetic energy is transferred from the mean flow to the disturbances during cyclogenesis. This energy conversion analysis provides crucial insights into why some systems develop into tropical cyclones while others remain as non-developing lows. It is observed that developing systems exhibit stronger barotropic energy conversion rates, particularly during the interaction of MJO and ER waves, contributing to the intensification of the initial disturbance.

Further, to address the challenges in early detection of tropical cyclones, this study introduces a novel stream function-based methodology for tracking quasi-closed circulation (QCC) systems before low formation. Traditional approaches using mean sea level pressure have proven insufficient for early detection. The newly developed method successfully tracked the evolution of cyclone Mora and was subsequently automated and validated across multiple seasons from 2017 onwards. This tracking algorithm demonstrates remarkable accuracy in distinguishing between developing and non-developing lows based on stream function values and amplitude differences, along with total precipitable water, achieving high accuracy. Machine learning approach is further addressed to distinguish between developing and non-developing tropical lows to tropical cyclones irrespective of different numerical model’s data.

The research extends into high-resolution numerical modeling simulation using the Model for Prediction Across Scales (MPAS-A) at 3km spatial resolution. Utilizing ERA5 initial conditions and NOAA interpolated SST data, simulations were conducted for SCS Mora over Bay of Bengal, Indian ocean. The non-hydrostatic model successfully captured pre-vortex formations and accurately simulated wind speeds and reflectivity patterns prior to low formation, providing valuable insights into the pre-genesis phase of tropical cyclones.

This comprehensive study advances our understanding of tropical cyclone formation over the NIO by establishing the critical role of wave interactions and barotropic energy conversion in cyclogenesis, developing an innovative tracking methodology, and validating high-resolution modeling approaches. The findings have significant implications for improving tropical cyclone forecasting and early warning systems in the region, particularly in identifying and tracking potential cyclonic developments prior to low pressure area formation.

How to cite: Rongmie, E., Deshpande, M., Ahire, P., and Mano Kranthi, G.: Investigation of Physical Processes Leading to the Genesis of Tropical Cyclones over the North Indian Ocean: An Integrated Study of Wave Dynamics, Energy Conversion, and Advanced Tracking Methods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-844, https://doi.org/10.5194/egusphere-egu25-844, 2025.

Understanding precipitation variability and extremes in Equatorial East Africa is vital for ensuring water and food security and mitigating the socioeconomic consequences of extreme events. Previous research has shown that sub-seasonal precipitation variability in this region is closely related to the wind direction, with precipitation more probable on days where the wind blows anomalously from the west, advecting moisture from the Congo basin. However, the exact nature of the westerly circulation and the conditions under which it forms are not fully understood. Here, we present a multi-decadal analysis of East African westerly winds. We use methods developed from studies of atmospheric rivers to objectively identify “westerly moisture transport events” (WMTEs), facilitating new insights into the seasonal distribution and importance of these westerlies, the regions within Eastern Africa where they occur, and the role of both the Madden-Julian Oscillation and tropical cyclones in their development. Finally, we also investigate the role of WMTEs as drivers of regional sub-seasonal precipitation variability.

How to cite: Peal, R. and Collier, E.: A multi-decadal analysis of westerly moisture transport events (WMTEs) in Equatorial East Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-877, https://doi.org/10.5194/egusphere-egu25-877, 2025.

EGU25-1450 | ECS | Orals | AS1.23

Synoptic variability in the moist margin and its connection to tropical and extratropical weather systems 

Corey Robinson, Sugata Narsey, Christian Jakob, and Hanh Nguyen

The moist margin is a sharp gradient of humidity that separates the moist deep tropics from the drier subtropics, and as such its movement is important for describing rainfall variability. In this work, we investigate how weather systems are related to synoptic variability in the moist margin. We use an object-based approach to relate moist margin perturbations to convectively coupled equatorial waves, the Madden-Julian Oscillation (MJO) and monsoon low-pressure systems (LPS). We also consider extratropical interactions with the moist margin, which are defined through upper-level potential vorticity (PV) anomalies. The results indicate that the MJO and equatorial Rossby waves have significant modulating effects on the moist margin. In comparison, monsoon LPS are infrequent but strongly influence the moist margin when they occur. The largest and longest-lived perturbations are commonly related to PV anomalies, and their composite structure reveals a clear wave-like signal, often with anticyclonic PV anomalies near the perturbed margin and cyclonic PV anomalies remotely. Open questions remain regarding the potential two-way interactions and feedback mechanisms between extratropical PV anomalies and the moist margin, which are examined here in some detail.

How to cite: Robinson, C., Narsey, S., Jakob, C., and Nguyen, H.: Synoptic variability in the moist margin and its connection to tropical and extratropical weather systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1450, https://doi.org/10.5194/egusphere-egu25-1450, 2025.

EGU25-1453 | Orals | AS1.23

Asymmetry Analysis of ERA5 Reanalysis Data in the Context of Tropical Cyclones 

Yibin Chen, Xiaofeng Zhao, Chunshan Wei, Yuxing Wang, and Pinglv Yang

A detailed analysis of temperature and relative humidity biases in the ERA5 reanalysis under tropical cyclone (TC) conditions is conducted using a composite analysis approach. This study incorporates the influences of TC movement and vertical wind shear (VWS). The results show that the temperature bias in the ERA5 data is more pronounced in the core region of TCs than in the outer regions. A similar pattern is observed for relative humidity, but it is most evident in the middle and upper troposphere. Additionally, the temperature bias exhibits a strong asymmetry, particularly in the core region of the TC, where larger errors are observed on the right-front side in the direction of motion and on the front side of the VWS at higher altitudes. This asymmetry is likely associated with more intense convection in these two directions.

How to cite: Chen, Y., Zhao, X., Wei, C., Wang, Y., and Yang, P.: Asymmetry Analysis of ERA5 Reanalysis Data in the Context of Tropical Cyclones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1453, https://doi.org/10.5194/egusphere-egu25-1453, 2025.

EGU25-1771 | ECS | Orals | AS1.23

 Complex networks to identify the merging of patches of coherent vorticity dynamics during tropical cyclones in the Bay of Bengal  

Shruti Tandon, Apoorva Singh, Bhupendra Nath Goswami, and Raman I Sujith

Predicting the intensity of cyclones a few days in advance during the formation as well as intensification of the cyclone is an open challenge. Heating from moist convection within the cyclone is considered the primary driver for the large-scale cyclonic vortex. However, the effect of interactions between small-scale vortices within the cyclone environment on the intensification of the cyclone vortex and its event-to-event variability are poorly considered. To enable skilful cyclone predictions, it is essential to first understand the local interactions in the atmosphere that facilitate self-sustained rotation and updraft of moist air.

We present a novel approach using complex networks to study atmospheric interactions and identify vortical perturbations that influence the formation of a depression and eventually a cyclone. We analyze the atmospheric flow over the Bay of Bengal (BoB) during different category-5 cyclones, namely, Amphan (2020), Sidr (2007) and Bangladesh (1991). Relative vorticity is obtained at hourly temporal resolution from the ERA5 reanalysis dataset (ECMWF reanalysis project). Nodes are locations between the equator to 30°N and 75°E to 105°E with a spatial resolution of 0.5°. We construct time-varying networks where each network corresponds to a short time period of 29 hours. Consecutive networks are separated by a difference of three hours. In each network, links are established between two nodes if (i) the time series of relative vorticity at both locations are correlated in a 24-hour window with a maximum of five-hour lag, and (ii) the two nodes are in spatial proximity of 2° latitude-longitude width centred at any one of the nodes. Note that, the spatial proximity is approximately 200 km that is comparable to the gale force wind radius of category-5 cyclones in BoB.

Through this approach, we decipher the relation between the local flow interactions and the global emergence of order in the form of a cyclone in the atmosphere. Regions of high connectivity in the network represent patches of locally coherent vorticity dynamics. Multiple such patches emerge throughout the life of a cyclone. Initially, these patches revolve around a developing low-pressure system, merging and intensifying the low-pressure system into a tropical depression and eventually into a tropical cyclone. Our approach helps identify prominent mesoscale convective systems that can form away from the low-pressure system but are entrained towards the depression and help intensify the storm at different stages. 

Next, we use Broadcast Mode Analysis (BMA), an advanced tool to identify the critical nodes that influence information propagation in time-varying networks. The analysis reveals nodes (locations) from where the most influential patch of coherent vorticity dynamics emerges that will eventually propagate, merge with and intensify the storm. We find the most influential region (the broadcast mode) and the most influenced region (receiving mode) in every 56-hour period corresponding to 10 networks. The receiving mode of one 56-hour period is approximately similar to the broadcast mode of the next 56-hour period. Broadcast mode analysis highlights the potential of tracking local interactions and mesoscale patches of coherent vorticity dynamics to improve the prediction of cyclone intensity.

How to cite: Tandon, S., Singh, A., Goswami, B. N., and Sujith, R. I.:  Complex networks to identify the merging of patches of coherent vorticity dynamics during tropical cyclones in the Bay of Bengal , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1771, https://doi.org/10.5194/egusphere-egu25-1771, 2025.

EGU25-2162 | ECS | Orals | AS1.23

Cold pool contribution to the development of convective storms over southwest Sumatra: insights from sub-km modelling 

Jack Mustafa, Cathryn Birch, John Marsham, Helen Burns, and Simon Peatman

The large islands of the Maritime Continent experience a strong diurnal cycle, with enhanced convection and precipitation over land through the afternoon and evening. Convective storms that initiate over land may then propagate out over surrounding coastal waters overnight; the land breeze is typically assumed to drive the overnight convergence of moisture offshore, however some of the offshore moisture convergence may also be attributed to other density current drivers, such as cold pools.

A regional configuration of the MetUM over southwest Sumatra has been used to isolate the influence of cold pool dynamics on the development of the diurnal cycle for three case study days by switching off precipitation re-evaporation (thereby preventing cold pool formation), and these results are compared with control runs with precipitation re-evaporation enabled.

This presentation will offer insight into the contribution of cold pools to offshore propagation of convective storms under different large-scale conditions, and into the influence of model resolution on how well this contribution is resolved.

How to cite: Mustafa, J., Birch, C., Marsham, J., Burns, H., and Peatman, S.: Cold pool contribution to the development of convective storms over southwest Sumatra: insights from sub-km modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2162, https://doi.org/10.5194/egusphere-egu25-2162, 2025.

Currently, the Monte Carlo Method is commonly used to estimate the uncertainty of tropical cyclone (TC) track forecasts. By performing random sampling of both along-track and cross-track errors, the potential range of official forecast errors is estimated (DeMaria et al. 2009; Tsai et al. 2011).

This study utilizes a Recurrent Neural Network (RNN) with an Encoder-Decoder architecture to represent situation-dependent track forecast uncertainty and the spatiotemporal correlations of forecast errors. The datasets used in this study include the Central Weather Administration’s (CWA) official TC track forecasts from 2018 to 2022, as well as deterministic and ensemble track forecasts from global numerical weather prediction models, specifically ECMWF and NCEP models.

Preliminary results indicate that the RNN-based approach reasonably reflects potential error ranges under different scenarios. For instance, TCs located at mid-to-high latitudes with higher translation speeds usually exhibit smaller cross-track forecast errors. Additionally, the prediction intervals (PIs) derived in this study can reasonably cover the proportion of observed data: the uncertainty ranges of the mean +/- one (two)  standard deviations encompass approximately 70% (95%) of observed data. Furthermore, large-scale environmental indices (e.g., steering flow and monsoon circulation) are considered to further reduce the uncertainty of TC track forecasts. More detailed findings will be presented during the meeting.

How to cite: Lin, F.-Y. and Tsai, H.-C.: Improving Situation-Dependent Uncertainty Estimation in Tropical Cyclone Track Forecasts Using Encoder-Decoder Neural Networks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2416, https://doi.org/10.5194/egusphere-egu25-2416, 2025.

Recent research highlights the influence of the Atlantic Niño on the likelihood of strong hurricanes forming in the tropical Atlantic. This phenomenon increases the risk of hurricanes impacting the Caribbean islands and the United States. A recent study distinguishes two variants of the Atlantic Niño, characterized by warming concentrated in the central (CA) and eastern (EA) equatorial Atlantic, respectively. Through an analysis of observational and reanalysis data, we investigated how these two types of Atlantic Niño affect hurricane activity. The findings reveal that the CA Niño enhances hurricane frequency south of 20°N, while the CA Niña promotes hurricanes north of 20°N. The CA Niño exerts a more significant influence on hurricanes than the EA Niño, primarily by affecting wind shear, relative vorticity, and vertical velocity. In contrast, the EA Niño mainly impacts relative humidity and African Easterly Waves. These insights could improve the accuracy of seasonal hurricane forecasts.

How to cite: Wang, H., Wang, C., and Zhang, L.: Differentiated Impacts of Central and Eastern Atlantic Niño on Hurricane Activity in the Tropical North Atlantic , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2717, https://doi.org/10.5194/egusphere-egu25-2717, 2025.

EGU25-3022 | Posters on site | AS1.23

Probabilistic Predictions on TC Rapid Intensification 

Hyemin Lee, Jihee Kim, Seonghee Won, and Hyunsoo Lee

Some of Tropical Cyclones undergo a rapid intensification process, which causes them to become stronger typhoons. Rapid Intensification (RI) is defined as the increase in maximum sustained winds to 30 kt (15 m/s) or more within a 24-hour period (Kaplan and DeMaria, 2003). Typhoons that have undergone RI mainly strengthen into strong LMIs, which can cause significant damage in a relatively short period of time. The recent increase in the number of cases of RI of Tropical Cyclones has highlighted the importance of advanced forecasting. However, achieving accuracy in these forecasts remains a significant challenge. In general, the intensity of typhoons is highly dependent on thermal conditions, such as ocean temperatures. However, the process of rapid intensity development is complex and influenced by dynamic factors, such as upper-level divergence and vertical wind shear. In this study, we developed a guidance for predicting the probability of rapid intensity development in a typhoon using environmental prediction factors at the time of its occurrence. For the purpose of supporting KMA's typhoon forecasting, a statistical based prediction model for the probability of RI was developed and evaluated from 2023 to 2024. It uses logistic regression to provide RI predictions up to the next 24 hours and 48 hours. The predictor variables included upper-level divergence, relative humidity, equivalent potential temperature (EPT), depth-averaged temperature (DAT), tropical cyclone heat potential (TCHP), thermodynamic net energy gain rate (NGR) (Lee et al., 2019), and 30 kt wind radius. To evaluate the accuracy of predictions for typhoons that occurred between June and November 2021-2023, 12 cases of RI and 42 cases of non-RI were analyzed. The POD was 0.78 and 0.76 for the 24-hour and 48-hour prediction accuracy, respectively, with corresponding FAR of 0.32 and 0.38. Predictive models showed good results during the validation period, but predicting favorable conditions for RI is still complex and challenging.

How to cite: Lee, H., Kim, J., Won, S., and Lee, H.: Probabilistic Predictions on TC Rapid Intensification, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3022, https://doi.org/10.5194/egusphere-egu25-3022, 2025.

EGU25-3055 | ECS | Posters on site | AS1.23

A ML-based perspective on spatio-temporal patterns of convective organisation 

Sarah Brüning and Holger Tost

Convective clouds play a vital role in Earth's hydrological cycle. In the tropics, these clouds often form extensive, spatially connected structures known as mesoscale convective systems (MCSs). MCSs are significant contributors to severe weather and are linked to potential changes in precipitation extremes. However, they are still connected to uncertainties, particularly regarding the intensity and variability of their spatio-temporal clustering (convective organisation).

This study aims to characterise regional patterns of convective organisation and explore their connections to convective cloud microphysics. The analysis covers a region in tropical Africa between 30° W – 30° E and 30° N – 30° S with a focus on the spring-to-summer period. Convective clouds and the intensity of their organisation are detected using 3D radar reflectivities. These spatio-temporal contiguous predictions are derived through a machine learning (ML) based extrapolation of observations from passive (MSG SEVIRI) and active (CloudSat) 2D remote sensing sensors. Furthermore, three organisation indices are used to quantify the organisational state of the atmosphere. They are leveraged to examine the relationship between convective cloud development and large-scale organisation. Using an object-based algorithm, we identify convective core and anvil regions in the predicted 3D radar reflectivities at each time step. These cloud objects are tracked over time to construct seamless 4D trajectories that capture cloud movement in three dimensions. Then, we calculate the indices to characterise the degree of organisation at each time point. The study evaluates regional statistics for convective organisation and analyses the key features of the observed systems.

Our findings highlight regional hotspots of convective organisation over the Gulf of Guinea, continental West Africa, and the Atlantic Ocean. These areas frequently host long-lasting, highly active cloud systems, such as MCSs. We observe seasonal variations in convective cloud development lead to a modest 5 % increase in organisation during summer. For example, differences in landmass distribution and the influence of extratropical dynamics in the southern hemisphere contribute to greater variability compared to the northern hemisphere. Over the ocean, organisation indices are approximately 5–10 % higher than over land. Overall, the results highlight the importance of regional characteristics in assessing convective organisation. Integrating data from multiple remote sensing instruments offers valuable insights, potentially enhancing climate risk assessments. However, our study emphasises that the overlapping effects of isolated and clustered convection may impact the statistical analysis. Addressing this issue requires an adapted organisation index.

How to cite: Brüning, S. and Tost, H.: A ML-based perspective on spatio-temporal patterns of convective organisation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3055, https://doi.org/10.5194/egusphere-egu25-3055, 2025.

Accurate forecasting of tropical cyclones is crucial for safeguarding coastal areas against the loss of life and property. Near-real-time analysis data, such as the Cross-Calibrated Multi-Platform Ocean Surface Wind Vector (CCMP), is widely utilized for predicting tropical cyclones due to its comprehensive coverage and consistent temporal and spatial measurements. However, CCMP has a limited resolution of 25 kilometers and frequently underestimates wind speeds during tropical cyclones because of rain interference. In contrast, Synthetic Aperture Radar (SAR) can measure ocean surface winds under all weather conditions with a significantly higher resolution of approximately 0.5 kilometers, though it lacks extensive area and temporal coverage. We developed a novel deep learning approach that leverages the strengths of both CCMP and SAR data. By using SAR wind measurements for tropical cyclones globally as the ground truth, we trained our deep learning model on the corresponding CCMP data to enhance its accuracy and spatial resolution. We evaluated various deep learning architectures, including U-Net, DeepLabV3+, and TransUNet. Our results indicate that TransUNet performs the best, improving CCMP's accuracy by 45% for wind speeds over 20 m/s, 20% for overall wind field, 56% for the maximum wind speeds, and 64% for the radius of the maximum wind speed. Our method can create gap-free, high-resolution, and accurate ocean surface wind data for tropical cyclones.

How to cite: Zhang, E., Su, H., and Chan, P.-W.: Deep Learning-based Fusion of Analysis and Satellite Measurements for Ocean Surface Wind Downscaling for Tropical Cyclones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3457, https://doi.org/10.5194/egusphere-egu25-3457, 2025.

Estimating the typhoon sizes, including the radius of maximum wind (RMW) and the wind radii, is a challenging aspect of typhoon monitoring and forecasting. Currently, methods for estimating typhoon sizes include ground-based pressure and wind measurements, airborne Stepped Frequency Microwave Radiometer (SFMR) measurements, satellite-based infrared (IR) and microwave instrument retrievals, etc. Retrievals of sea surface winds based on the microwave scatterometers/radiometers suffer from coarse spatial resolution (40-50 km) and susceptibility to heavy rainfall; meanwhile, IR brightness temperatures lack a direct physical correlation with sea surface winds at the pixel level.

Due to the lack of regular aircraft reconnaissance, the determination of typhoon sizes in the western North Pacific relies solely on IR and microwave retrievals. Our assessment based on synthetic aperture radar (SAR) wind products indicates that the Joint Typhoon Warning Center's (JTWC) best track dataset has a better estimation of typhoon intensities than inner sizes, with an uncertainty within 15% for maximum sustained wind (Vmax) estimation, but as high as 30-60% for RMW estimation, which is above the global average of 25-40%.

This study establishes an RMW estimation algorithm for eyed typhoons based on geostationary satellite IR observations, with key steps including: (a) determining the typhoon center; (b) distinguishing clear-eye cases from unclear-eye cases; (c) estimating the eyewall radius (Reye) separately for clear- and unclear-eye cases; (d) estimating the RMW.

A TC-red-green-blue (TC-RGB) composite was designed by using satellite multichannel observations (reflectance, brightness temperature, and brightness temperature differences), which can effectively differentiate convective clouds, cirrus clouds, and low clouds, proving very effective in identifying exposed low-level circulation centers. Combining the TC-RGB composite image with 10-min atmospheric motion vectors products, a precise typhoon center location can be obtained through interactive human-computer methods. Using SAR positioning results as a reference, the root mean square difference (RMSD) for eyed typhoon positioning results was calculated, with the JTWC dataset direct interpolation result being ~8.6 km, and the interactive method being ~6.6 km, reducing by over 20%.

Subsequently, an objective method to differentiate between clear- and unclear-eye typhoons was established, along with an IR-based method for measuring Reye. For clear-eye typhoons, the calculated Reye has a correlation coefficient as high as 0.89 with the SAR observed RMW (RMW_SAR); for unclear-eye typhoons, the correlation coefficient between Reye and RMW_SAR also reaches 0.82.

Ultimately, an RMW regression equation for eyewall typhoons was established based on Reye and RMW_SAR, with a mean absolute error (MAE) of 5.46 km and a root mean square error (RMSE) of 7.35 km, nearly 40% less than the JTWC dataset.

How to cite: Zhuge, X.: Geostationary Satellite-based Estimation Method for Typhoon Radius of Maximum Wind, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3650, https://doi.org/10.5194/egusphere-egu25-3650, 2025.

The classic theories on tropical cyclone (TC) intensification (i.e., CISK, WISHE) are based on the assumption of an axisymmetric and vertically aligned TC circulation. However, how the TC vortices align at various altitudes within a sheared environment is a challenging topic in the TC intensity change research. This study investigates vortex alignment in tropical cyclones (TCs) through two idealized experiments conducted under easterly vertical wind shears (VWS) of 6 m s⁻¹ and 10 m s⁻¹. Both experiments simulate TCs that  exhibit intensification simultaneously. While the onset of intensification hinges on the achievement of a vertically aligned vortex structure, the evolution of vortex tilt displays significant differences between the two cases. We find the crucial role of convective asymmetry, predominantly intensified on the downtilt side of the simulated TCs, in driving vortex alignment.On one hand, diabatic heating associated with the asymmetric convection directly aids in reducing the vortex tilt. On the other hand, this convective asymmetry generates counter-rotating gyres within the inner-core region. These gyres produce cyclonic vorticity downstream of the heating zone and anticyclonic vorticity downstream of the cooling zone, which obstructs vertical structure coupling. The interplay between these processes ultimately dictates the evolution of vortex tilt. This research emphasizes the importance of capturing convective processes to improve the  TC intensification prediction.

How to cite: Feng, Y. and Wu, L.: Influences of Asymmetric Convection on Vortex Alignment of  Tropical Cyclones: Idealized Experiments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3660, https://doi.org/10.5194/egusphere-egu25-3660, 2025.

EGU25-3781 | Posters on site | AS1.23

Radiative feedbacks in the Madden-Julian oscillation 

Eric Maloney and Wei-Ting Hsiao

The organization of tropical deep convection is supported by radiative feedbacks, in which high clouds and moisture anomalies associated with convection imposes anomalous longwave (LW) radiative heating in the atmosphere, further supporting convection. Despite an abundance of studies with numerical simulations, the interactions between tropical convective organization, radiative feedbacks, and the large-scale atmospheric environment have not been examined comprehensively using observations. This presentation examines such interactions among tropical mesoscale organized convection, radiative feedbacks, and the Madden-Julian oscillation (MJO) using a set of observation-derived data products, including retrievals using spaceborne satellites, ground-based precipitation radar, and reanalyses.  The results of this analysis demonstrate that: (1) Higher sea surface temperature and stronger low-level wind shear strength enhance tropical mesoscale convective activity, increasing cirrus cloud cover and LW heating generated per unit precipitation. (2) The estimation of LW cloud-radiative feedback (LW CRF), defined as the LW cloud-radiative heating produced per unit precipitation, is sensitive to the precipitation data set used. (3) Radiatively driven circulations and the associated moistening effects in the MJO can be derived in a weak-temperature-gradient framework and a linear baroclinic model. LW heating moistens the MJO more efficiently than the total apparent heat source, while shortwave (SW) radiative effects dry the MJO. (4) The LW CRF of the MJO is spatially inhomogeneous, with stronger feedbacks over the tropical Indian ocean and to the northwest of Australia, but weaker feedbacks over the tropical western and central Pacific. The spatial pattern may be determined by the spatial distribution of preferred convective types and precipitation efficiency.

How to cite: Maloney, E. and Hsiao, W.-T.: Radiative feedbacks in the Madden-Julian oscillation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3781, https://doi.org/10.5194/egusphere-egu25-3781, 2025.

The formation of a vertically aligned vortex is essential for the intensification of tropical cyclones (TCs), particularly under conditions of environmental vertical wind shear (VWS). This study investigates the physical mechanisms driving vortex tilt evolution in two simulated TCs subjected to environmental shears of 6 m s⁻¹ and 10 m s⁻¹. Our findings indicate that balanced dynamics play a pivotal role in governing vortex tilt. Specifically, the tilt-induced distortion of isentropic surfaces generates negative virtual potential temperature anomalies on the downtilt side and positive anomalies on the uptilt side of the vortex. As air parcels undergo cyclonic rotation along these distorted isentropic surfaces, they ascend on the right side of the tilt vector, resulting in increased relative humidity and eventual saturation. This leads to diabatic ascent and enhanced convection in the downtilt and downtilt-left quadrants, which amplifies the wavenumber-1 circulation through convectively coupled vortex Rossby waves, further modifying the vortex tilt. This study underscores the importance of balanced dynamics in understanding the interplay between vortex tilt, wavenumber-1 structures (Rossby waves), and convective asymmetries in the intensification of tropical cyclones under vertical wind shear. 

How to cite: Wu, L. and Zhou, X.: Balanced Evolution of the Vertical Tilt of Simulated Tropical Cyclone Vortices in a Sheared Environment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3913, https://doi.org/10.5194/egusphere-egu25-3913, 2025.

EGU25-4145 | ECS | Orals | AS1.23

Impact of tropical waves on the atmospheric structure and composition above Cabo Verde during the CADDIWA campaign  

Tanguy Jonville, Maurus Borne, Cyrille Flamant, Juan Cuesta, Olivier Bock, Pierre Bosser, Christophe Lavaysse, Andreas Fink, and Peter Knippertz

The Cabo Verde region is subject to the activity of many tropical waves during the boreal summer. They are known to favour or inhibit convective activity, and to play a role in the formation of Tropical Cyclones. A frequency-wavenumber filtering method is used to identify the different waves. A novel tracking protocol is used to distinguish African Easterly Waves propagating north and south of the African Easterly Jet based on their frequencies within the Mixed-Rossby Gravity - Tropical Disturbance (MRG-TD) domain, labeled MRG-TD1 and MRG-TD2, respectively. Based on in-situ and satellite measurements from the Cloud Atmospheric Dynamics Dust Interactions in West Africa (CADDIWA) campaign which took place in Cape Verde in September 201, the impact of each tropical type on the atmosphere vertical structure and dust content is discussed. Our results show that Equatorial Rossby waves mainly impact thermodynamics above 750 hPa, while MRG-TD1 affect jet-level thermodynamics, and MRG-TD2 modulate moisture in the lower troposphere. Dust event are mainly driven by MRG-TD2. The importance of the interaction between waves for tropical cyclogenesis is also highlighted which provides new outlooks for improving tropical cyclogenesis forecasting in the region. 

How to cite: Jonville, T., Borne, M., Flamant, C., Cuesta, J., Bock, O., Bosser, P., Lavaysse, C., Fink, A., and Knippertz, P.: Impact of tropical waves on the atmospheric structure and composition above Cabo Verde during the CADDIWA campaign , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4145, https://doi.org/10.5194/egusphere-egu25-4145, 2025.

EGU25-4206 | ECS | Posters on site | AS1.23

China coasts facing more tropical cyclone risks during the second decaying summer of double-year La Niña events 

Xi Luo, Lei Yang, Johnny.C.L. Chan, Sheng Chen, Qihua Peng, and Dongxiao Wang

Long-lasting La Niña events (including double-year and triple-year La Niña events) have become more frequent in recent years. How the multi-year La Niña events affect tropical cyclone (TC) activities in the western North Pacific (WNP) and whether they differ from single-year La Niña events are unknown. Here we show that TCs are more active over the far-WNP (FWNP, 110°–150°E), leading to marked high risks at China coasts during the second decaying summer of double-year La Niña events. The anomalous TC activities are directly related to the enhanced cyclonic anomaly over the FWNP, possibly a result of large-scale remote forcing initiated by the tropical North Atlantic (TNA) cooling. The persistent TNA cooling from the decaying winter to summer of double-year La Niña events drives westerlies over the Indo-western Pacific through Kelvin waves, which induce the cooling over the north Indian Ocean via the wind-evaporation-sea surface temperature effect, favoring the asymmetric heat distribution pattern and stimulating an anomalous vertical circulation over the eastern Indian Ocean to FWNP. The cooling over the north Indian Ocean also excites Gill responses, magnifying the TNAinduced westerlies and boosting the anomalous vertical circulation, and thus gives rise to the strong cyclonic circulation anomaly over the FWNP in summer. We suggest that the key point of the process is the strong TNA cooling related to the persistent negative Pacific-North American pattern (PNA) and positive North Atlantic Oscillation (NAO) while double-year La Niña events decay, distinct from the rapid decline of PNA and NAO during single-year La Niña events. The work provides a unique perspective on understanding TC activities over the WNP related to the El Niño-Southern Oscillation.

How to cite: Luo, X., Yang, L., Chan, J. C. L., Chen, S., Peng, Q., and Wang, D.: China coasts facing more tropical cyclone risks during the second decaying summer of double-year La Niña events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4206, https://doi.org/10.5194/egusphere-egu25-4206, 2025.

Tropical cyclones (TCs) are modulated by El Niño-Southern Oscillation (ENSO) on interannual timescales as ENSO impacts local Sea Surface Temperatures (SST) and atmospheric conditions, especially in the Pacific basin. The frequency, intensity, startup SST, windshear and life cycle of TCs vary between ENSO phases and TC seasons. Previous research focused on the Southwest Pacific (SWP) Basin has consistently shown that during El Niño phases TCs tend to form more towards the central Pacific, while during La Niña, their formation shifts towards the northeast coast of Australia. Also, TCs form more frequently during the late TC seasons than during the early TC seasons. Here, TC genesis is assessed using a Coupled ENSO index (using Niño 3.4 SST and the Southern Oscillation Index (SOI)) and a grouping into early (Oct-Jan) and late (Feb-May) TC seasons, in the decades from 1971 to 2020. We find that though the number of TCs in SWP are decreasing over the years, their SST at genesis and maximum wind speed are increasing, generating more intense TCs over the SWP basin. TCs formed during El Niño are more intense than those formed during La Niña even though there is no significant difference in their SST at genesis. We find that the threshold of environmental factors responsible for cyclogenesis in SWP are gradually changing, leading to more severe TC events in the region. 

How to cite: Oginni, T., Renwick, J., and Behrens, E.: Impact of El Niño-Southern Oscillation Phases on Tropical Cyclone Genesis in the Southwest Pacific: A Study of Seasonal and Decadal Changes (1971-2020, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5295, https://doi.org/10.5194/egusphere-egu25-5295, 2025.

Using dynamic-balanced data in which tropical cyclones (TCs) are removed by the potential vorticity inversion technique, Arakane and Hsu (2021) showed that TCs significantly modulated the long-term mean state of the summer monsoon in the western North Pacific (WNP), and increased its intraseasonal variability by 50% to 70%. In order to investigate the TC impact on the global climate field, not just over the WNP, we have newly created TC removal data in which all TCs in all ocean basins are removed, rather than limiting it to TCs over the WNP region as in the previous version. In the process, improvements were also made to the potential vorticity inversion formulation to make it more suitable for removing TCs. In this presentation, we will report on the details of creating this new TC-removed data, and TC impacts on the mean fields and variability of global climate as revealed by the analysis using this data.

How to cite: Arakane, S. and Hsu, H.-H.: Dynamic-balanced global tropical cyclone removal dataset and tropical cyclone impacts on the global climate mean field and variability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5455, https://doi.org/10.5194/egusphere-egu25-5455, 2025.

EGU25-5779 | ECS | Posters on site | AS1.23

Tropical Cyclone Dynamics Shaped by Aerosol-Cloud-Interactions: A Composite Perspective Using ICON Ensemble Simulations. 

Andrina Caratsch, Sylvaine Ferrachat, and Ulrike Lohmann

Tropical cyclones (TCs) pose a significant threat to coastal populations and ecosystems. To effectively mitigate TC risk, it is essential to understand their evolution under current and future climate conditions. One aspect of their development that remains unclear is the role of aerosol-cloud interactions (ACI). Satellite observations indicate that aerosols can invigorate convection in tropical deep convective clouds (Jiang et al., 2018). However, observations of ACI in TCs remain limited. In contrast, numerical simulations indicate that aerosol-induced convective invigoration can either weaken or strengthen TCs, depending on where the aerosols enter the storm (Lin et al., 2023; Hoarau et al., 2018).

In the future, aerosol concentrations are expected to decrease due to reductions in anthropogenic emissions (Riahi et al., 2017). The impact of this overall aerosol decline on TCs remains unclear. As part of the EU-funded CleanCloud project, our goal is to investigate TC dynamics in cleaner aerosol conditions to refine our understanding of ACI in TCs and improve future TC risk assessments.

We use the numerical weather prediction and climate model ICON (Zängl et al., 2015) in limited area mode using a 10 km horizontal resolution to run ensemble simulations of the North Atlantic TC season in 2020. Cloud processes are parameterized with a two-moment microphysics scheme (Seifert and Beheng, 2006) while deep convection parametrisation is disabled. Aerosols are uniformly prescribed in varying concentrations, allowing TCs to evolve in both clean and polluted conditions. By implementing a novel cyclone composite method that normalizes the storms by their eyewall location and extent, we evaluate the clean and polluted cyclone populations in terms of their circulation and structure. Our study compares TC activity on the storm scale in the 2020 TC season under both clean and polluted aerosol conditions, offering insights into how TC dynamics might be shaped by ACI.

 

Literature

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  • Lin, Y., Wang, Y., Hsieh, J.-S., Jiang, J. H., Su, Q., Zhao, L., Lavallee, M., & Zhang, R. (2023). Atmospheric Chemistry and Physics, 23(21), 13835–13852. https://doi.org/10.5194/acp-23-13835-2023
  • Riahi, K., van Vuuren, D. P., Kriegler, E., Edmonds, J., O’Neill, B. C., Fujimori, S., Bauer, N., Calvin, K., Dellink, R., Fricko, O., Lutz, W., Popp, A., Cuaresma, J. C., Kc, S., Leimbach, M., Jiang, L., Kram, T., Rao, S., Emmerling, J., Tavoni, M. (2017). Global Environmental Change, 42, 153–168. https://doi.org/10.1016/j.gloenvcha.2016.05.009
  • Seifert, A., & Beheng, K. D. (2006). Meteorology and Atmospheric Physics, 92(1), 45–66. https://doi.org/10.1007/s00703-005-0112-4
  • Zängl, G., Reinert, D., Rípodas, P., & Baldauf, M. (2015). Quarterly Journal of the Royal Meteorological Society, 141(687), 563–579. https://doi.org/10.1002/qj.2378

 

 

 

How to cite: Caratsch, A., Ferrachat, S., and Lohmann, U.: Tropical Cyclone Dynamics Shaped by Aerosol-Cloud-Interactions: A Composite Perspective Using ICON Ensemble Simulations., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5779, https://doi.org/10.5194/egusphere-egu25-5779, 2025.

EGU25-6210 | ECS | Orals | AS1.23

On the temporal decay of tropical cyclones over the ocean 

Min Li and Ralf Toumi

It is important to understand how tropical cyclones (TCs) decay over the ocean as this is a critical pre-landfall stage. A modified exponential decay model ($\beta$ model) with two parameters $\alpha$ and $\beta$ is proposed. The scale parameter $\alpha$ defines the decay scale, while the shape parameter $\beta$ determines whether the decay rate decelerates or accelerates over time. Global fittings indicate that around 40\% of TCs exhibit decelerating decay ($\beta \leq 1$), while the majority (about 60\%) show accelerating decay ($\beta > 1$). Correlation analysis reveals a strong negative correlation between the scale parameter $\alpha$ and the initial Coriolis parameter ($r=-0.96$) and a positive correlation between the shape parameter $\beta$ and the meridional component of the initial translation velocity ($r=0.75$). The $\beta$ model provides a comprehensive understanding of how TCs decay with time and how environmental conditions affect the decay scale and evolution.

How to cite: Li, M. and Toumi, R.: On the temporal decay of tropical cyclones over the ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6210, https://doi.org/10.5194/egusphere-egu25-6210, 2025.

EGU25-6232 | Orals | AS1.23

Effects on the dynamical and microphysical structures of tropical storms in ICON 

Roxana S. Cremer and Fabian Senf

Tropical cyclones are impressive phenomena of tropical meteorology and form spatially highly organised structures. To shed more light on microphysical sensitivities and dynamical structure when modelling these storms, we selected the hurricane Paulette to simulate one week of the storm’s evolution with the German weather and climate model ICON in a limited area mode.

Hurricane Paulette occurred in the North-Atlantic basin in September 2020 and is the longest-lasting tropical cyclone of that year (7-22nd September).

In our experiments perturbations in the Cloud Condensation Nuclei (CCN) type and concentration are explored as well as the vertical resolution of the model. Additionally, the horizontal grid spacing is reduced to hectometre scale (300m) to get a more detailed look into the hurricane.

Here we present some key findings for the wind speed, surface pressure and cloud related variables along the hurricane track, next to how accurate the track is compared to NOAA observational data. Lastly, the influence of the introduced perturbations and reduction in resolution, horizontal and vertical, on radiation fluxes at the top-of-the-atmosphere in the simulated area is assessed. It can be stated that in most simulations the strength of Paulette is underestimated compared to the observations and the model produces to little ice to accurately represent the hurricane clouds in comparison to satellite observations. 

How to cite: Cremer, R. S. and Senf, F.: Effects on the dynamical and microphysical structures of tropical storms in ICON, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6232, https://doi.org/10.5194/egusphere-egu25-6232, 2025.

EGU25-6289 | ECS | Orals | AS1.23

Synoptic drivers of humid heatwaves in West Africa 

Jack Law, Cathryn Birch, Lawrence Jackson, Dominique Bouniol, Massimo Bollasina, and John Marsham

Humid heatwaves (HHWs) can cause heat stress in humans by reducing the ability to sweat in higher humidity. West Africa is an area of high interest due to its rapid population growth, high vulnerability, and latitudinal variation in HHW drivers. There is little understanding in how HHWs are triggered at synoptic scales. Using reanalysis and satellite-derived rainfall, we find different drivers in the three key regions of the Guinean coast, Sahel and Sahara. HHWs are associated with elevated near-surface specific humidity in all three regions. Near-surface temperature is also elevated in the Guinean Coast and Sahel regions while the Sahara region experiences a decrease during events. The rise in both temperature and humidity can be explained by the combination of increased near-surface downward shortwave radiation and trapping of moisture in the lower troposphere. The main moisture source is rainfall two days prior. After rainfall, clearer skies brought by dry mid-tropospheric northeasterly winds drive increased shortwave radiation, providing energy for surface evaporation and increasing temperature. In the Sahara region, the background air temperature is already very high, so there is enough energy for surface evaporation despite the mitigating impact of rain on temperature, indicated by the increase of surface latent heat flux to the atmosphere by as much as 118%. African Easterly Waves (AEWs) are a key driver of rainfall in Sahel and Sahara regions, and, therefore, are also a source of HHW predictability. The probability of a HHW increases during an AEW passage by as much as 24% in Western Sahara, which contains major population centres of over 1 million people. We also find most HHW events occur south of the intertropical discontinuity, which moves north and south with the onset and cessation of the African monsoon. While the majority of HHW events occur during the African Monsoon season in the Sahara, most events occur immediately before and after the start of the monsoon season further south. In addition, we analyse vertical profiles of cloud from CloudSat and CALIPSO, and show a clear anomaly from climatology during HHWs, with reduced cloud in the moister Guinean coast and Sahel to the south and increased cloud associated with rain in the more arid region of the Sahara. Understanding of the drivers and predictability of HHWs is important for risk management and adaptation measures such as the development of early warning systems.

How to cite: Law, J., Birch, C., Jackson, L., Bouniol, D., Bollasina, M., and Marsham, J.: Synoptic drivers of humid heatwaves in West Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6289, https://doi.org/10.5194/egusphere-egu25-6289, 2025.

EGU25-6646 | ECS | Posters on site | AS1.23

Upper level processes in simple models for tropical cyclones in high resolution simulations 

Giousef Alexandros Charinti, Andrea Polesello, Caroline Muller, Andrea Davin, and Claudia Pasquero

Estimating the intensity of tropical cyclones has been a critical research topic in the field.
Theoretical models such as the potential intensity (PI), first introduced by Emanuel 1986 [1],
provide an upper bound for the intensity a tropical cyclone can achieve based on pre-storm
conditions. However, PI and other similar models are based on idealized settings that may
not always match real-world conditions, such as assuming a neutral atmosphere to moist
convection. Using simulations from the high resolution cloud resolving model SAM [3] in
rotating radiative-convective equilibrium settings, we assess the validity of the idealiza-
tions of the PI theory. We find that upper level processes are responsible for the intensity
oscillations of the tropical cyclone in the simulations, as confirmed by a recent study [5]. We
further show that when accounting for the upper level processes, it is possible to modify
PI such that it approximately follows the observed intensity evolution.

[1] K. A. Emanuel, J. Atmos. Sci. 43, 6 (1986).
[2] K. A. Emanuel et al., Annu. Rev. Earth Planet Sci. 31, 1 (2003).
[3] M. F. Khairoutdinov, D. A. Randall, J. Atmos. Sci. 60, 4 (2003).
[4] C. J. Muller, D. M. Romps, PNAS 115, 12 (2018).
[5] A. Polesello, G. A. Charinti,  A. N. Meroni, C. J. Muller, C. Pasquero (submitted, 2025).
[6] A. A. Wing, K. A. Emanuel, J. Adv. Model. Earth Syst. 6, 1 (2014).

How to cite: Charinti, G. A., Polesello, A., Muller, C., Davin, A., and Pasquero, C.: Upper level processes in simple models for tropical cyclones in high resolution simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6646, https://doi.org/10.5194/egusphere-egu25-6646, 2025.

In early June 2023, New York City (NYC) and other cities in the northeastern US experienced a severe air pollution event. Although reports associated this hazardous pollution event with the smoke from Canadian wildfires, the factors triggering the southward waft of the smoke remain unclear. We found the northerly anomaly that transported the smoke was linked to the Rossby wave train excited by the Madden–Julian Oscillation (MJO) over the Philippine Sea, which led to the formation of an enhanced northerly at the western edge of the cyclonic anomaly over the East Coast–North Atlantic. When the MJO convection left the western Pacific, the disorganized teleconnection caused the pollution to dissipate. Observational findings were further supported by model simulations and predictions. These results suggest that monitoring and predictions of MJO activity may help mitigate air pollution events over the northeastern US during Canadian wildfire seasons.

 

How to cite: Zhu, Y., Hsu, P., and Qian, Y.: Influence of Western Pacific Madden–Julian Oscillation on New York City's Record‐Breaking Air Pollution in Early June 2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6698, https://doi.org/10.5194/egusphere-egu25-6698, 2025.

EGU25-6816 | Orals | AS1.23

Diurnal Cycle Effects over the Maritime Continent on Tropical Waves Using a Simple Linear Model 

Scott Hottovy, Moira Camacho, and Maria Flatau
The diurnal cycle plays a large role in convective activity in the tropical atmosphere. It is estimated that the diurnal cycle contributes as large as 70% of the tropical variability and spans across multiple scales in time and space. A challenge to modeling is incorporating interactions between the diurnal cycle and the various convectively coupled atmospheric waves. These interactions can be complex especially over the Maritime Continent. This paper aims to model these interactions using a simple unified model of the tropical power spectrum from Stechmann & Hottovy 2017. In this model a simple source/sink of lower tropospheric moisture captures the diurnal cycle effects over two islands in the Maritime Continent (Sumatra and Borneo). Using this model, theoretical results are presented to show all modes of the model are excited by the diurnal forcing, the strongest effects are the resonant effect to the small scale Kelvin and Western Inertial Gravity waves, and the effects on each mode depend on how big of a factor lower tropospheric moisture is in an individual mode.
 

How to cite: Hottovy, S., Camacho, M., and Flatau, M.: Diurnal Cycle Effects over the Maritime Continent on Tropical Waves Using a Simple Linear Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6816, https://doi.org/10.5194/egusphere-egu25-6816, 2025.

EGU25-6831 | ECS | Orals | AS1.23

TOPIM – Modelling hurricane Intensity in the Caribbean Region 

Samantha Hallam, Jake Hallam, Mark Guishard, Randy Aird, and Donovan Campbell

Tropical cyclones are one of the most frequent and costly disasters affecting the Small Island Developing States (SIDS) in the Caribbean.

Historical analysis of tropical cyclones in the Caribbean Region (10-30°N 55-90°W), using HURDAT data, shows that the mean Maximum Sustained Wind (MSW) has increased significantly by 30kts since 1965, a rate of 5.3kts per decade with a corresponding significant decrease in the minimum pressure of 2.3mb per decade. The increasing MSW observed is significantly correlated with the August, September and October (ASO) ocean temperatures, which are rising at 0.2ºC per decade in the Caribbean.

TOPIM - Tropical cyclone Ocean-coupled Potential Intensity Model has been developed to better predict tropical cyclone intensity in the Caribbean. TOPIM is an ocean-coupled dynamical and statistical model which has been developed for the Caribbean and already has proof of concept, having been working experimentally for Bermuda since 2021. TOPIMuses subsurface ocean temperature from Argo floats and atmospheric sounding data to improve the prediction of tropical cyclone intensity (wind strength and minimum pressure) in near real-time, using little computing requirements. The model calculates the expected TC potential intensity based on; the average temperature over the top 100m ocean layer in the Caribbean, the local atmospheric sounding data, and local wind pressure relationship for past hurricanes in the area since 1965. The top 100m layer is chosen as it provides the closest prediction of hurricane intensity in the Caribbean region on a hindcast basis since 1990. Results show the prediction better forecasts actual tropical cyclone potential intensity than models using sea surface temperature alone.

TOPIM can also be used for future scenario planning. Past storms can be placed in a warmer ocean environment, to understand the expected increase in maximum sustained wind - an ocean sensitivity analysis. The analysis assumes the atmospheric sounding conditions remain the same. Analysis of historical Caribbean storms suggests a 27kt increase in intensity on average for a 1°C rise in ocean temperature over the top 100m layer.

(Hallam et al. Modelling hurricane Intensity in the Caribbean Region, in prep.)

https://www.topim.org

 

How to cite: Hallam, S., Hallam, J., Guishard, M., Aird, R., and Campbell, D.: TOPIM – Modelling hurricane Intensity in the Caribbean Region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6831, https://doi.org/10.5194/egusphere-egu25-6831, 2025.

EGU25-7183 | ECS | Orals | AS1.23

Adiabatic and diabatic energy tendencies of the equatorial Kelvin wave 

Katharina Meike Holube, Frank Lunkeit, Sergiy Vasylkevych, and Nedjeljka Žagar

Kelvin waves play an important role in tropical circulation variability. Previous research has shown that the tropospheric Kelvin wave activity is associated with both tropical convection and dry dynamics, which can be connected to the extratropics. The relative importance of the adiabatic and diabatic processes for Kelvin wave energy tendencies has not yet been consistently evaluated in reanalysis data.
In this study, we investigate the Kelvin wave energy budget focusing on the relative contributions of physical and dynamical processes in ERA5 reanalysis data. Kelvin waves and their energy tendencies are identified by applying three-dimensional normal-mode function decomposition. A novel aspect of our method is that momentum and temperature tendencies are computed directly from the complex normal-mode function expansion coefficients. This allows to quantify the adiabatic energy tendencies as nonlinear interactions of Rossby and inertia-gravity waves and the zonal mean flow. The diabatic energy tendencies are determined from the momentum and temperature tendencies due to parametrizations in the short-term ERA5 forecasts. 
The most relevant results are that the advection of zonal momentum is on average a source of Kelvin wave energy, whereas Kelvin wave energy variability on diurnal and submonthly scales is mainly due to heating by shortwave radiation and latent heat forcing, respectively. The 3D normal-mode decomposition allows to reveal the roles of wave-wave and wave-mean flow interactions in dynamical processes, in particular in the tropics.

How to cite: Holube, K. M., Lunkeit, F., Vasylkevych, S., and Žagar, N.: Adiabatic and diabatic energy tendencies of the equatorial Kelvin wave, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7183, https://doi.org/10.5194/egusphere-egu25-7183, 2025.

EGU25-7847 | ECS | Posters on site | AS1.23

Analyzing long term Spatial Changes of Parameters Affecting Cyclonic Activity over the North Indian Ocean 

Akshay Kumar Sagar and Arun Chakraborty

This study undertakes a thorough analysis of the elements that influence the variability of tropical cyclones (TC) in the North Indian Ocean (NIO) from 1960 to 2020, with a specific focus on the periods before and after the monsoon season. The study utilizes historical satellite data to investigate the factors that impact the formation, strength, and trajectories of cyclones. The primary method for evaluating cyclone strength is by calculating the Accumulated Cyclone Energy (ACE). The study observes a decreasing trend in ACE levels during 1991–2005, which started increasing just after from 2006 to 2020. The Bay of Bengal (BoB) has a more uniform distribution of ACE in comparison to the Arabian Sea (AS), with higher average values and more variability over the Main Development Region (MDR), which is the area where cyclone development occurs most frequently. Cyclones of greater intensity generally occur following the monsoon season. Examination of storm paths reveals that cyclones with greater intensity frequently hit the northeastern and southeastern coastal regions of India. The study emphasizes notable discrepancies in parameters within the MDR, which impact cyclone strength and ACE values throughout various periods.

 

Keywords: ACE; Tropical Cyclone; Bay of Bengal; Variability

How to cite: Kumar Sagar, A. and Chakraborty, A.: Analyzing long term Spatial Changes of Parameters Affecting Cyclonic Activity over the North Indian Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7847, https://doi.org/10.5194/egusphere-egu25-7847, 2025.

EGU25-8947 | ECS | Orals | AS1.23

A novel algorithm for detecting Lake Victoria's lake-breeze fronts from station observations 

Musa Ssemujju, Marlon Maranan, and Andreas H. Fink

Due to its vast size, Lake Victoria in East Africa significantly impacts the region’s climate through lake breezes, which influence convective activity, and thus precipitation, as well as air pollution and quality in coastal cities. These breezes, with their leading edges known as lake-breeze fronts (LBF), affect local and regional weather by initiating deep moist convection, even during the dry months of December-February (DJF) and June-August (JJA). This can lead to heavy precipitation inland or over the lake, resulting in weather-related disasters and losses. Despite their importance, there is limited research on LBFs linked with Lake Victoria. To address this gap, we developed a novel algorithm to detect LBF passages, mainly focusing on the shorelines of Uganda. We leveraged 15-minute observations from 44 automatic weather stations from the Trans-African Hydrometeorological Observatory (TAHMO) and Uganda National Meteorological Authority (UNMA) over six years (2017-2022).

Our objective observation-based lake breeze detection algorithm (OLBDA) identifies LBF passages using wind speed and direction, temperature, dew point, and precipitation measurements from stations. We focused on daytime periods (0900 – 1900LT) when the coastal land-lake temperature contrast is strongest, specifically during the dry months. The algorithm employs three criteria to detect LBF passages at any given station. First, OLBDA checks for a rapid wind reversal from offshore (relative to the nearest coastline) to onshore, or a rapid increase in wind speed within defined onshore directions. If the wind criterion is met, the data are then tested for a drop in air temperature and an increase in dew point. Here, percentile-based thresholds for temperature and dew point criteria are applied to account for regional variabilities. Lastly, to avoid false detections caused by precipitation-induced temperature drops and wind shifts, a 3-hour precipitation amount < 0.1mm at a station before the LBF passage is required. If all criteria are met, that day is considered a lake-breeze day at that station.

To test the performance, we compared the OLBDA-detected lake-breeze days with manually identified lake-breeze days (“ground truth”) within the study period from NASA’s satellite visible spectrum (Terra- and Aqua-MODIS, and NOAA-20). The algorithm detected more than 70% and 60% of the total cases identified from satellite images for coastal (within 2 km) and semi-coastal (2-10km) stations respectively, indicating good performance.

Preliminary results show that most LBF passages occur from afternoon to late evening, peaking at 1300LT for coastal stations and shifting with the station's distance from the coastline. The majority of detected lake-breeze days occur during the DJF months, with January having the most detected days. Other lake breeze characteristics including the onset and cessation time, strength, duration, propagation speed and time, and inland penetration depth, are being examined.

Finally, we aim to develop a detailed year-round observed Lake Victoria breeze climatology over Uganda. Our findings can serve as an observational benchmark to (a) improve understanding of this phenomenon’s impact on the local climate and communities along the northern shores of Lake Victoria, and (b) validate numerical simulations of lake breezes over the region.

How to cite: Ssemujju, M., Maranan, M., and Fink, A. H.: A novel algorithm for detecting Lake Victoria's lake-breeze fronts from station observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8947, https://doi.org/10.5194/egusphere-egu25-8947, 2025.

EGU25-9467 | ECS | Orals | AS1.23

Global and Regional Characteristics of Tropical Cyclone Rapidly Intensifying Events 

Mulin Li, Weixin Xu, and Xinyan Zhang

Accurate prediction of tropical cyclone (TC) intensity still faces great challenges, and rapid intensification (RI) imposes the largest uncertainty in forecasting the TC intensity change. TC RI has been extensively studied, but most studies considered RI during an 24h period, but not the whole life cycle of the RI event. This study investigates the characteristics and environmental factors of ~1500 full lifecycle RI events from 1980 to 2020 in global TCs and compare their regional difference. Our results show that most RI events actually initiate at the tropical storm stage (30-40 kts) preferentially in the early morning, which is consistent across basins. The  locations of RI onsets in the southern hemisphere are generally limited  between 9°S and 20°S, while in the northern hemisphere, they occur at higher latitudes, particularly in the North Atlantic, reaching above 30°N. Nearly half of the RIs last longer than 42h, and RIs in the western North Pacific last significantly longer than RIs in the North Atlantic and South Indian. It is interesting that no matter the initial intensity, RI events with longer duration have higher intensification rate (INTRATE), except for extremely lasted events. Also, the total intensification amplitudes of RIs are more determined by the duration than the INTRATE. Overall, the duration and INTRATE of RIs have a positive relationship with maximum potential intensity (MPI), SST and mid-level relative humidity, and a negative relationship with vertical wind shear. Of course, the initial environmental conditions for RIs are more favorable than regularly intensifying events. It is intriguing whether environments of extreme RIs (extremely high INTRATE) differ from normal RIs, which will be further investigated.

How to cite: Li, M., Xu, W., and Zhang, X.: Global and Regional Characteristics of Tropical Cyclone Rapidly Intensifying Events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9467, https://doi.org/10.5194/egusphere-egu25-9467, 2025.

Modern tropical cyclones (TCs), which originate in the tropics, feature deep warm-core symmetric structures. However, the characteristics of TCs in the early Eocene remain unclear. Here, we showed evidence from proxy data, climate modeling, and cyclone phase space that cyclones with deep warm-core symmetric structures appeared at high latitudes during the early Eocene. Under the favorable conditions of warm sea surface temperature and weak baroclinicity, most of these cyclones originated from the transition of extratropical cyclones. Meanwhile, in the tropics, only 36.91% of symmetric cyclones had a deep warm core, while 49.86% had a warm core at lower levels. These shallow cyclones tend to induce more intense rainfall than modern TCs. Our results provide unique insights into TC changes under high carbon dioxide levels and highlight the growing threat of extreme rainfall and winds associated with TCs at high latitudes.

How to cite: Zhang, T.: Contrast change of cyclogenesis over tropical and extratropical in the Eocene , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9532, https://doi.org/10.5194/egusphere-egu25-9532, 2025.

EGU25-9790 | ECS | Orals | AS1.23

Intensity oscillations of tropical cyclones: surface versus mid and upper tropospheric processes 

Andrea Polesello, Giousef Alexandros Charinti, Agostino Niyonkuru Meroni, Caroline Muller, and Claudia Pasquero

Classical models of tropical cyclone intensification often predict that cyclones will intensify to a steady-state intensity determined primarily by surface fluxes, while convection maintains the atmosphere close to a neutrally stable state (Emanuel et al. (2003); Emanuel (1995)). However, simulations using the non-hydrostatic, high-resolution SAM model under idealized conditions (rotating radiative-convective equilibrium in a doubly-periodic domain) reveal a more complex intensity evolution.
While the early intensification aligns with theoretical predictions, later in its evolution, the cyclone exhibits oscillations in wind speed. This oscillation can be linked to feedbacks between the cyclone intensity and air buoyancy: convective heating and mixing with warm low stratospheric air warm the mid and upper troposphere of the cyclone, stabilizing the air column and thus reducing its intensity. After the intensity decay phase, mid and upper tropospheric cooling, due to both local longwave radiation emission and cold advection from the surroundings, rebuilds CAPE, that peaks just before a new intensification phase. These idealized simulations highlight the potentially important interactions between a tropical cyclone, its environment and radiation.

 

 

References


Kerry Emanuel et al. Tropical cyclones. Annual review of earth and planetary sciences, 31(1):
75–104, 2003.


Kerry A. Emanuel. The behavior of a simple hurricane model using a convective
scheme based on subcloud-layer entropy equilibrium. Journal of Atmospheric Sci-
ences, 52(22):3960 – 3968, 1995. doi: 10.1175/1520-0469(1995)052⟨3960:TBOASH⟩2.0.CO;
2. URL https://journals.ametsoc.org/view/journals/atsc/52/22/1520-0469_1995_
052_3960_tboash_2_0_co_2.xml.

 

How to cite: Polesello, A., Charinti, G. A., Meroni, A. N., Muller, C., and Pasquero, C.: Intensity oscillations of tropical cyclones: surface versus mid and upper tropospheric processes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9790, https://doi.org/10.5194/egusphere-egu25-9790, 2025.

Tropical Cyclones (TCs) are devastating natural disasters. Ocean thermal stratification and TC attributes (e.g., translation speed and intensity) have been demonstrated to affect TC intensification via modulating sea surface temperature (SST) cooling effect. Here, we found that both ocean internal tides and storm size could affect TC intensification. Analyzing decades of global TC data, here we explore the modulating role of ocean internal tides and storm size on TC-induced sea surface temperature anomalies (SSTA) and TC intensification in global TC-active oceans. Originating from complex interplays between astronomic tides and the SCS topography, gigantic ocean internal tides in the South China Sea (SCS) interact with TC-generated oceanic near-inertial waves and induce a strong ocean cooling effect, effectively suppressing the TC intensification. Consequently, among all global TC-active basins, the SCS stands out as a particularly difficult ocean for TCs to intensify, despite favorable atmosphere and ocean conditions. Over the SCS, TC intensification rate and its probability for a rapid intensification are only 1/2 and 1/3, respectively, of those for the rest of the world ocean. Moreover, as a typical TC attribute, storm size can also modulate TC intensification through ocean cooling effect. Large TCs induce stronger and more widespread SSTA, which reduces ocean’s enthalpy flux supply and thus suppresses TC intensification globally, as compared to small TCs. This modulating effect emerges in each basin, suggesting a globally consistent effect of storm size on TC intensification through an oceanic pathway. Small TCs, occupying weaker SST cooling and larger enthalpy flux, are more likely to undergo rapid intensification, with the probability of 1.1–1.8 times larger than large TCs in global TC-active oceans. Inclusion of this interaction between internal tides and storm size and TC in operational weather prediction systems is expected to improve forecast of TC intensity in TC-active basins.

How to cite: Guan, S. and Tian, J.: TC-Ocean interaction: modulating roles of ocean internal tides and storm size, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9891, https://doi.org/10.5194/egusphere-egu25-9891, 2025.

EGU25-9984 | Posters on site | AS1.23

Tropical Cyclogenesis Microphysics : modeling the impact of dust on Tropical Storm Rose (2021) development over the Atlantic 

Cyrille Flamant, Tanguy Jonville, Pierre Tulet, Guillaume Feger, Jean-Pierre Chaboureau, Héléna Gonthier, and Christophe Lavaysse

According to the marsupial paradigm, some African Easterly Waves exhibit a pouch structure that shields convective systems from lateral intrusion of dry air. This protective mechanism also influences dust transport from the Saharan Air Layer, preventing its intrusion at mid to high altitudes. A Meso-NH model based simulation of the life cycle of Tropical Storm Rose (2021) is presented and validated against ECMWF ERA5 reanalyses as well as ground-based and airborne CADDIWA campaign data. The sensitivity of the model simulations to the concentration of dust is discussed. By modifying initial conditions, the impact of dust on the storm development and intensification is investigated with a specific focus on microphysics. 

How to cite: Flamant, C., Jonville, T., Tulet, P., Feger, G., Chaboureau, J.-P., Gonthier, H., and Lavaysse, C.: Tropical Cyclogenesis Microphysics : modeling the impact of dust on Tropical Storm Rose (2021) development over the Atlantic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9984, https://doi.org/10.5194/egusphere-egu25-9984, 2025.

EGU25-10201 | Posters on site | AS1.23

The impact of changes of atmospheric water mass ontropical cyclone intensification in ICON-A 

Janina Tschirschwitz, Marco Giorgetta, and Bjorn Stevens

For many modelling applications, the total mass of the atmosphere and hence the global mean surface pressure can be considered constant and invariant under precipitation and evaporation. This is also the case for the atmosphere model ICON-A: Changes to the atmospheric water mass are compensated by changes in dry air composition, hence the mass of an atmospheric layer is constant and only its physical properties change. However, there are limits to this simplification, especially when it comes to modelling very moist environments or atmospheres. In moist environments, water becomes a major contributor to atmospheric mass and surface pressure, thus changes in water mass from evaporation and precipitation can affect the surface pressure. 

By separating the atmospheric mass in ICON-A into contributions from dry air and from water constituents and by allowing the water component to vary with precipitation and evaporation, we are adding a simplified precipitation mass sink / evaporation mass source to the ICON-A model (for simplicity only referred to as ‘precipitation mass sink’).

The impact of this precipitation mass sink on atmospheric dynamics is investigated in a tropical cyclone test case: A vortex is initialised on a rotating aquaplanet and evolves into a tropical cyclone over the period of ten simulation days. Simulations with and without the precipitation mass sink are compared. The effect of the precipitation mass sink on cyclone development and, in particular, its strength are investigated. 

How to cite: Tschirschwitz, J., Giorgetta, M., and Stevens, B.: The impact of changes of atmospheric water mass ontropical cyclone intensification in ICON-A, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10201, https://doi.org/10.5194/egusphere-egu25-10201, 2025.

We investigate the projected changes to the location, width and intensity of the intertropical convergence zone (ITCZ) in two global 30-year coupled storm resolving simulations, evolving under the shared socioeconomic pathway 3.7-0 forcing. The first simulation performed using the storm resolving version of the ICOsahedral Nonhydrostatic model, ICON-Sapphire, resolves convection explicitly and employs a horizontal resolution of 10 km in the atmosphere and 5 km in the ocean. The second simulation performed using the Integrated Forecasting System coupled to the Finite-volumE Sea ice-Ocean Model (IFS-FESOM), utilizes a convective parameterization with reduced cloud base mass flux and has a similar horizontal resolution as the ICON-Sapphire simulation (9 km in the atmosphere and 5 km in the ocean). 

The magnitude of warming over 30 years is about 1K in ICON-Sapphire and 2K in IFS-FESOM. Changes in the seasonal mean ITCZ positions, determined from the latitude of maximum precipitable water in [30°S, 30°N], are not substantial in both the models, except in IFS-FESOM during boreal spring where a southward shift is seen in the Central Pacific basin. Monthly anomalies in the ITCZ latitude also show a southward shift in IFS-FESOM. Trends in the ITCZ width, computed based on the moist margins of the tropics, and ITCZ intensity, determined using precipitation in the ITCZ latitudes, are also analyzed.

How to cite: Praturi, D. S. and Hohenegger, C.: Projected changes to the intertropical convergence zone in warming scenario global storm resolving simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10328, https://doi.org/10.5194/egusphere-egu25-10328, 2025.

EGU25-11740 | ECS | Posters on site | AS1.23

Comparison of Three Cloud Microphysical Schemes on the Rapid Intensification of Typhoon Hagupit (2020) 

Guiling Ye, Wentao Zhang, Jeremy Cheuk-Hin Leung, Wenjie Dong, and Banling Zhang

A typhoon Hagupit (2020) that intensifies rapidly near the coast is simulated by using the Weather Research and Forecasting (WRF V4.2.1) model. The typhoon track, intensification, and precipitation simulated by WSM6, Morrison, and Goddard 4-ice cloud microphysics schemes were evaluated based on observations. The simulation biases during the typhoon’s Rapid intensification process were analyzed. The results showed that all three schemes effectively simulated the typhoon's track and precipitation, but their simulations of intensity varied significantly. The Morrison scheme better reproduced the typhoon's intensity, whereas WSM6 underestimated it and Goddard 4-ice overestimated it. Differences in the simulated typhoon intensity corresponded well with variations in the mass mixing ratio of ice-phase particles. During the intensification process, Goddard 4-ice exhibited the highest rate of ice particle formation through vapor deposition, while WSM6 had the lowest. Sensitivity experiments further demonstrated that latent heat release from the deposition of ice-phase particles warmed the air, which enhanced the typhoon's warm-core structure and strengthened the upward outflow in the eyewall. This process accelerated the inflow of low-level air toward the typhoon center, increasing the pressure gradient and maintaining the extremely low central pressure. This study proposes that the process of ice-phase hydrometeor deposition plays a critical role in simulating typhoon rapid intensification.

How to cite: Ye, G., Zhang, W., Leung, J. C.-H., Dong, W., and Zhang, B.: Comparison of Three Cloud Microphysical Schemes on the Rapid Intensification of Typhoon Hagupit (2020), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11740, https://doi.org/10.5194/egusphere-egu25-11740, 2025.

EGU25-12499 | ECS | Orals | AS1.23

Convective-to-Stratiform Transition of MCSs off Western Africa and its Relationship to the Diurnal Offshore Precipitation Maximum 

Rosimar Rios-Berrios, Naoko Sakaeda, Elinor Martin, and Shun-Nan Wu

Satellite-based climatological analyses show a sharp contrast between the fractional convective and stratiform rainfall over Africa and its neighboring eastern Atlantic water. While convective rainfall dominates over continental Africa, stratiform precipitation dominates the rainfall totals over the eastern Atlantic. The convective maximum over land is mainly contributed by numerous mesoscale convective systems (MCSs). At the same time, the diurnal peak of precipitation exhibits a maximum just offshore from western Africa. To this end, the objective of this study is to use a phenomenon-based approach to investigate the sharp rainfall morphology contrast between continental Africa and the eastern Atlantic while also relating that contrast to the climatological precipitation maximum off western Africa. We hypothesize that MCSs coming off Africa structurally change as they move off continental Africa and into the maritime environment over the Atlantic. To test this hypothesis, we use primarily hindcasts produced during NASA’s Convective Processes Experiment - Cabo Verde (CPEX-CV) field campaign using the Model for Prediction Across Scales - Atmosphere (MPAS-A). This model was configured with a convection-permitting mesh extending from eastern Africa to the western Atlantic, thus covering the extensive tracks of multiple MCSs as they propagated offshore into the Atlantic. Results show that MCSs in MPAS-A transition from mature trailing stratiform systems over land to decaying stratiform systems over water. Further analysis will investigate if shear-cold pool dynamics can explain this behavior, and how such dynamics change with the time of day. 

How to cite: Rios-Berrios, R., Sakaeda, N., Martin, E., and Wu, S.-N.: Convective-to-Stratiform Transition of MCSs off Western Africa and its Relationship to the Diurnal Offshore Precipitation Maximum, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12499, https://doi.org/10.5194/egusphere-egu25-12499, 2025.

EGU25-13846 | Posters on site | AS1.23

Introducing synthetic convectively coupled Kelvin waves into the Met Office Unified Model 

Natasha Senior, Adrian Matthews, Benjamin Webber, Claudio Sanchez, Richard Jones, and Mohamed Husein Nurrahmat

The Maritime Continent (MC) is the rainiest region on Earth, where extreme precipitation constitutes a major hazard. Convectively coupled Kelvin waves (CCKWs) are weather systems that travel eastwards across the equatorial waveguide and can trigger convection in their convergent phase. CCKWs are linked to up to a fourfold increase in precipitation rates across the equatorial Maritime Continent (Ferrett et al., 2020). However, not all CCKWs produce precipitation extremes. Recent studies reveal that CCKWs arriving in phase with the local diurnal cycle of convection may be more likely to cause high impact weather events or when part of a multiscale interaction with the MJO, organising the large-scale precipitation on a more localised scale (Baranowski et al., 2016; Baranowski et al., 2020; Latos et al., 2021; Senior et al., 2023).

Current methods for studying these mechanisms have some limitations. For example, composite studies of CCKWs are useful for revealing statistical links but smooth out key interactions. Case studies are useful for identifying mechanisms in particular high-impact weather events but are difficult to generalise. Modelling such high-impact weather events provides additional insights; however, lacks the capability for fine-tuning.

Hence, we have developed a methodology for introducing synthetic CCKWs into convection-permitting Met Office Unified Model (MetUM) forecasts. This involves generating 3D CCKW structures on key dynamical fields using ERA5 data and adding these to the model’s initial conditions. The methodology will be presented, and a comparison of diagnostics from control and perturbation experiments will be provided. We will then discuss how the methodology will be applied to studying the mechanisms through which CCKWs cause precipitation extremes across various locations in the MC. Since CCKWs are an important dynamical predictor of extreme precipitation, understanding these mechanisms is crucial for providing accurate forecasts of hazardous weather in the MC.

Baranowski, D.B. et al., (2016Phase locking between atmospheric convectively coupled equatorial Kelvin waves and the diurnal cycle of precipitation over the Maritime Continent. Geophysical Research Letters, 43(15), 82698276. https://doi.org/10.1002/2016GL069602.

Baranowski, D.B. et al., (2020Social-media and newspaper reports reveal large-scale meteorological drivers of floods on Sumatra. Nature Communications, 112503. https://doi.org/10.1038/s41467-020-16171-2.

Ferrett, S. et al., (2020Linking extreme precipitation in Southeast Asia to equatorial waves. Quarterly Journal of the Royal Meteorological Society, 146(727), 665684. https://doi.org/10.1002/qj.3699.

Latos, B. et al., (2021Equatorial waves triggering extreme rainfall and floods in Southwest Sulawesi, Indonesia. Monthly Weather Review, 149(5), 13811401. https://doi.org/10.1175/MWR-D-20-0262.1.

Senior, N.V. et al., (2023Extreme precipitation at Padang, Sumatra triggered by convectively coupled Kelvin waves. Quarterly Journal of the Royal Meteorological Society, 149(755)22812300.  https://doi.org/10.1002/qj.4506

How to cite: Senior, N., Matthews, A., Webber, B., Sanchez, C., Jones, R., and Nurrahmat, M. H.: Introducing synthetic convectively coupled Kelvin waves into the Met Office Unified Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13846, https://doi.org/10.5194/egusphere-egu25-13846, 2025.

EGU25-14182 | Posters on site | AS1.23

Easterly wave disturbances on tropical south Atlantic and their impact over northeast Brazil 

Helber Gomes, Kevin Hodges, Pallav Ray, Maria Cristina Lemos da Silva, Hakki Baltaci, Matheus José Arruda Lyra, Dirceu Herdies, Fabrício Daniel dos Santos Silva, and Heliofábio Barros Gomes

This study presents a 21-year climatology (1998–2018) of Easterly Wave Disturbances (EWDs) over the Tropical South Atlantic (TSA). The identification of these systems was performed subjectively using infrared satellite images and fields of relative vorticity and streamlines at 1000, 850, 700, 500, and 200 hPa levels from the ERA-Interim (ERAI) reanalysis. Additionally, the TracKH automatic tracking algorithm was applied, successfully capturing approximately 66% of the subjectively identified events. A total of 518 EWDs were recorded during the study period, with 97% reaching the Northeast Brazil (NEB) region, and 64% exhibiting convective characteristics. The highest frequency of events was observed between April and August, with an average of approximately 25 EWDs per year. The primary genesis areas were located between 20°S–5°N and 35°W–15°W. The trajectories and dissipation predominantly occurred along the NEB's eastern coastline, particularly between Alagoas and Rio Grande do Norte. Dissipation generally occurred rapidly after the systems moved inland. Several atmospheric systems were identified as key contributors to EWD genesis, including the Intertropical Convergence Zone (ITCZ), Upper-Tropospheric Cyclonic Vortices (UTCV), cold fronts, and convective clusters originating from the west coast of Africa. These factors played a significant role in the intensification and organization of the disturbances.  During the wet season, the synoptic patterns associated with EWDs revealed anomalous cyclonic and confluent circulations, along with convergence and negative vorticity from low levels up to 200 hPa, where only a trough feature was observed. Negative anomalies of vertical motion and temperature, coupled with increased relative humidity, were also identified, fostering favorable conditions for enhanced convection and precipitation associated with the disturbances. 

How to cite: Gomes, H., Hodges, K., Ray, P., Silva, M. C. L. D., Baltaci, H., Lyra, M. J. A., Herdies, D., Silva, F. D. D. S., and Gomes, H. B.: Easterly wave disturbances on tropical south Atlantic and their impact over northeast Brazil, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14182, https://doi.org/10.5194/egusphere-egu25-14182, 2025.

Mesoscale convective processes and related dynamic/thermodynamic responses may play an important role in the Tropical Cyclone (TC) genesis, in addition to the favorable environmental conditions. The objective of this study is to determine whether and how unique are mesoscale organizations and convective properties of tropical disturbances prior to TC formation in the Northwest Pacific. Previous studies with a similar goal are based on either a small sample size or limited observational source (e.g., only Infrared). This study identifies over 3000 episodes of developing (Dev) and nondeveloping (Nondev) tropical disturbances and utilizes a large amount of multi-source satellite observations (precipitation, infrared, microwave, spaceborne radar, etc.) to comprehensively compare their convective structures. The Dev and Nondev disturbances were borne in similar large-scale environments such as SST, low-level vorticity, vertical wind shear, except that the Dev tropospheric conditions are slightly moister. However, the frequency, organization, intensities, and ensemble microphysics of the convection are significantly different between Dev (48-96h prior to TC formation) and Nondev. Both Dev and Nondev show very asymmetric distributions of convection with maxima in the down-shear quadrants, but Dev systems have greater areas of precipitation and cold clouds. The embedded individual convective systems of Dev are also more organized, i.e., greater areas and higher stratiform rain fraction. Furthermore, Dev convection is stronger and present greater ice-phase content as indicated by both the passive microwave and spaceborne measurements. Interestingly, Dev disturbances also have markedly higher frequency of shallow warm convection, especially in the up-shear regions, which may help moistening the lower-to-middle troposphere and beneficial for further deep convective developing. In most of the Dev storms, convection rapidly become more organized and deeper during 24-48 prior to the TC genesis. This study further compares the organization and convective properties among Dev systems generated under different types of large-scale flow pattern such as monsoon trough and easterly wave.                             

How to cite: Zhang, Z. and Xu, W.: Mesoscale Organizations and Convective Properties of Developing and Nondeveloping Tropical Disturbances over the Northwest Pacific Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14555, https://doi.org/10.5194/egusphere-egu25-14555, 2025.

EGU25-14926 | Orals | AS1.23

Advancing spaceborne observations of tropical cyclones by the WIVERN 94 GHz Doppler radar: the case study of the rapid intensification of hurricane Milton 

Alessandro Battaglia, Massimo Milelli, Martina Lagasio, Riccardo Rabino, Frederic Tridon, Maryam Pourshamsi, Marcel Kleinherenbrink, and Antonio Parodi

Hurricane rapid intensification (HRI) refers to a phenomenon in which a tropical cyclone undergoes a sudden and significant increase in wind speed over a short period, typically defined as an increase of at least 35 mph (30 knots) in maximum sustained winds within 24 hours. Key factors influencing the rapid intensification phenomenon are the presence of warm sea surface temperatures (SSTs) in combination with significant ocean heat content, a low wind shear, a high atmospheric water vapour content, as well a pre-existing well-organized storm structure. The combination of these factors can lead to disruptive HRI as observed for Hurricane Milton (2024), whose winds increased by 78 knots in the 24-hour period from 00:00 UTC October 7 to 00:00 UTC October 8. Monitoring and predicting HRI is crucial for disaster preparedness: a WRF hindcast study at 1.5 km grid spacing for Milton, which well reproduce the trajectory of the hurricane and its maximum wind intensity is presented.

The simulated Hurricane Milton three dimensional cloud and wind structure has been exploited to assess how the WIVERN 94 GHz radar, currently under study in the ESA Earth Explorer program, could sample the systems in correspondence to successive orbits during the hurricane lifetime. The proposed WIVERN radar has ground-breaking Doppler and scanning capabilities that enable to map very strong winds across a large swath of the order of 800 km (Illingworth et al., 2018; Battaglia et al.,2022, Tridon et al., 2023). Different overpasses simulated before and after the HRI demonstrate that the WIVERN system will be able to provide, for the first time from space, information about the mesoscale vertical structure of clouds and dynamics of the cyclone, particularly in the region above the freezing level (94 GHz are strongly attenuated inside the convective regions and the heavily precipitating rain bands). This suggests that WIVERN observations may have great potential to improve the prediction of hurricane intensification.  

 

 

 

Illingworth, A. J., Battaglia, A. et al., 2018: Wivern: A new satellite concept to provide global in-cloud winds, precipitation and cloud properties. Bull.Amer. Met. Soc., DOI: 10.1175/BAMS-D-16-0047.1, 1669-1687.

 

Battaglia, A., Martire, P., Caubet, E., Phalippou, L., Stesina, F., Kollias, P., and Illingworth, A.: Observation error analysis for the WInd VElocity Radar Nephoscope W-band Doppler conically scanning spaceborne radar via end-to-end simulations, Atmos. Meas. Tech., 15, 3011–3030, https://doi.org/10.5194/amt-15-3011-2022, 2022.

 

Tridon, F., Battaglia, A., Rizik, A., Scarsi, F. E., & Illingworth, A., 2023: Filling the gap of wind observations inside tropical cyclones. Earth and Space Science, 10, e2023EA003099. https://doi.org/10.1029/2023EA003099

How to cite: Battaglia, A., Milelli, M., Lagasio, M., Rabino, R., Tridon, F., Pourshamsi, M., Kleinherenbrink, M., and Parodi, A.: Advancing spaceborne observations of tropical cyclones by the WIVERN 94 GHz Doppler radar: the case study of the rapid intensification of hurricane Milton, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14926, https://doi.org/10.5194/egusphere-egu25-14926, 2025.

EGU25-16482 | Posters on site | AS1.23

Trends in Cyclone Intensity and Their Drivers in the Bay of Bengal 

Abhishek Singh, Ashish Saini, and Vinayakam Jothiprakash

From 2000 to 2024, the Bay of Bengal has exhibited significant shifts in tropical cyclone behavior, reflecting the intricate interplay between oceanic and atmospheric processes in a warming climate. Cyclone intensity has surged markedly, with the frequency of super cyclonic storms (wind speeds >221 km/h) increasing by over 30% compared to the early 2000s. Despite a modest decline in overall cyclone frequency post-2015, a consistent rise in median wind speeds highlights the escalating severity of these events, underscoring an increased threat to coastal and marine ecosystems. Comprehensive analysis attributes these changes to a combination of rising sea surface temperatures (SSTs), frequently surpassing critical thresholds of 28°C to 31°C, and a progressive weakening of vertical wind shear in the region. Elevated SSTs have enhanced ocean-atmosphere heat and moisture fluxes, creating conditions conducive to rapid intensification (RI) events. These factors have not only increased the likelihood of more intense cyclones but also shortened the response time for disaster preparedness. Atmospheric shifts, including alterations in the Indian Ocean Dipole (IOD) phases and the Madden-Julian Oscillation (MJO), have further modulated cyclone genesis, track trajectories, and landfall patterns. Notably, a westward shift in cyclone landfall locations has increased the vulnerability of previously less-affected areas, necessitating the reassessment of risk management strategies. These atmospheric oscillations have also contributed to changes in the temporal clustering of cyclonic events, presenting new challenges for seasonal forecasting models. This study integrates satellite observations, reanalysis datasets, and advanced climate models to quantify the physical mechanisms driving these trends. By coupling high-resolution modeling with real-time atmospheric monitoring, the findings emphasize the need for predictive frameworks capable of capturing the complex dynamics of cyclone behavior. Such advancements are critical for enhancing early warning systems, informing regional climate adaptation policies, and mitigating the socio-economic and environmental impacts in one of the world's most cyclone-prone regions.

How to cite: Singh, A., Saini, A., and Jothiprakash, V.: Trends in Cyclone Intensity and Their Drivers in the Bay of Bengal, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16482, https://doi.org/10.5194/egusphere-egu25-16482, 2025.

EGU25-16637 | ECS | Posters on site | AS1.23

LAM-ORCESTRA: a Numerical Campaign over the Atlantic ITCZ  

Romain Fiévet, Luis Kornblueh, Leonidas Linardakis, Cathy Hohenegger, and Bjorn Stevens

Over the summer of 2024, a wealth of experimental data was collected over the tropical Atlantic. First, the ORCESTRA campaign measured the ITCZ from the ground, sea, and air, offering a rich and detailed description of its complex structure. Coincidentally, the EarthCARE mission started releasing highly-resolved vertical profiles of deep convective systems. In parallel to these experimental studies, a numerical campaign was run almost in real time in the form of a limited-area model of the ITCZ. The model ran at 1.25 km resolution using the storm-resolving ICON-Sapphire configuration, in 48-hour-long bursts overlapping halfway through. This staggered approach was born of a compromise between 1) ensuring enough spinup time (first simulated day) and 2) keeping synoptic conditions close to ground observation for analysis (second simulated day). The resulting dataset allows us to compare the model with the aforementioned experimental missions, and assess its strength and weaknesses. Specifically, the model's capability in resolving the ITCZ structure and organisation of convection is scrutinized.

How to cite: Fiévet, R., Kornblueh, L., Linardakis, L., Hohenegger, C., and Stevens, B.: LAM-ORCESTRA: a Numerical Campaign over the Atlantic ITCZ , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16637, https://doi.org/10.5194/egusphere-egu25-16637, 2025.

Numerous studies focus on the impacts of ENSO diversity on tropical cyclone (TC) activities in the western North Pacific (WNP). In recent years, there is a growing threat of landfalling and northward-moving TCs in East Asia, accompanying an increase in central Pacific (CP) El Niño. Here, we aim to discover variations in landfalling TCs during various types of CP El Niño (CP-I and CP-II El Niño). It is found that significant changes in landfalling and going northward TCs over East Asia north 20N are modulated by CP-I El Niño. During CP-I El Niño, TCs tend to landfall more often over the mainland of China with longer duration, moving distance, and stronger power dissipation index (PDI) after land fall and increased TC-induced rainfall, due to favorable conditions (beneficial steering flow, weak vertical wind shear, increased specific humidity, increased soil moisture, and temperature), especially significant over the northeastern part. The situation over the mainland of China is reversed during eastern Pacific (EP) El Niño and CP-II El Niño, with a significant decrease in the characteristics with corresponding unfavorable environments. Over the Korean Peninsula and Japan, the frequency of TC landfalls, as well as the duration and the moving distance after landfall, exhibits greater levels during CP-I and CP-II El Niño than during EP El Niño due to favorable steering flow, and thus, TC-induced rainfall enhances correspondingly. Regarding the PDI over the Korean Peninsula and Japan, it remains relatively consistent across all El Niño types. However, a notable increase in the PDI during EP El Niño could be attributed to the higher intensity of TCs prior to landfall.

How to cite: Pan, L.: Distinct Features of Tropical Cyclone Landfall over East Asia during Various Types of El Nino, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17585, https://doi.org/10.5194/egusphere-egu25-17585, 2025.

EGU25-18104 | ECS | Orals | AS1.23

Tropical Cyclones in Decadal High-Resolution Simulations 

Mikael Karvinen, Nils Brüggemann, and Jochem Marotzke

Earth system models require high resolution to capture the mesoscale dynamics in the eye of a tropical cyclone (TC), which in turn allows more accurate simulation of TC intensity. We approach this so-called TC-resolving regime by using the coupled ICON model with a 10 km grid spacing in the atmosphere and ocean. Our simulations are 30 years long, which allows us to compute climate statistics for TC frequency and intensity. Although relatively high resolutions have been used before, we are among the first to study tropical cyclones with coupled simulations that have global and multi-decadal coverage at 10 km resolution.

We find that ICON is able to reproduce the TC frequency quite well, with about 57 hurricane-scale tropical cyclones per year compared to the observed 48 (as suggested by the "best tracks" dataset). Despite this positive bias in TC frequency, the seasonal cycle of TCs is very close to observations. A TC density map shows good agreement between model and observations, but the model tends to shift cyclone tracks slightly poleward. These differences can be attributed to different large-scale climate conditions, such as vertical wind shear and mid-tropospheric humidity. No category 5 cyclones are simulated, but the model is able to attain higher wind speeds (69 m/s) than any of the coupled climate models in the CMIP6 HighResMIP ensemble. We conclude that ICON, in its high-resolution configuration, is well suited for TC research.

How to cite: Karvinen, M., Brüggemann, N., and Marotzke, J.: Tropical Cyclones in Decadal High-Resolution Simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18104, https://doi.org/10.5194/egusphere-egu25-18104, 2025.

EGU25-18495 | ECS | Orals | AS1.23

Cooperative effects of QBO and ENSO on controlling the favorableness of the MJO realization 

Daisuke Takasuka, Tsubasa Kohyama, Tamaki Suematsu, and Hiroaki Miura

A mechanism for the interannual variability of the Madden–Julian Oscillation (MJO) realization frequency is examined. Based on the number of active days of MJO events detected using the tracking method for the Real-time Multivariate MJO Index, we quantify the year-to-year variability in the initiation and propagation of boreal-winter MJOs. Active years of MJO realization (MJO-A) are characterized by more frequent MJO initiation, leading to complete propagation into the western Pacific (WP), whereas this is less common in inactive years (MJO-IA) due to stronger advective drying and the resultant hindrance of column moistening over the WP. This contrast is linked to differences in boreal-winter mean convection and circulations: MJO-A (MJO-IA) years are characterized by enhanced and suppressed (suppressed and enhanced) convection over the WP/IO and Maritime Continent (MC), respectively. This modulation is driven by the combined effects of the El Niño-Southern Oscillation (ENSO) and the quasi-biennial oscillation (QBO). During moderate-to-strong El Niño events, MJO realization manifests actively regardless of QBO phase or amplitude, unless additional convective suppression occurs in the eastern Indian Ocean and/or MC due to other forcings, such as a positive Indian Ocean Dipole. In contrast, during ENSO-neutral and La Niña conditions, stronger QBO easterly phases tend to favor MJO realization, independent of ENSO. This QBO–MJO connection (except during El Niño conditions) is due to the zonal heterogeneity of QBO impacts; changes in the seasonal mean static stability near the tropopause over the WP modify the mean convective activity in that region. The zonal heterogeneity and ENSO phase-dependency of QBO impacts are interpreted by focusing on the vertical propagation of the Kelvin wave structure over the MC, influenced by both QBO winds and background Walker circulations.

How to cite: Takasuka, D., Kohyama, T., Suematsu, T., and Miura, H.: Cooperative effects of QBO and ENSO on controlling the favorableness of the MJO realization, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18495, https://doi.org/10.5194/egusphere-egu25-18495, 2025.

EGU25-18675 | Orals | AS1.23

The role of entrainment in axisymmetric tropical cyclones 

Tom Dörffel, Rupert Klein, Sabine Doppler, and Boualem Khouider

The intensification of tropical cyclones (TCs) results from the transport of conserved angular momentum, at least in an axisymmetric context. While there is general agreement on the role of moist cloud convection in driving the system, its precise contribution to intensification remains unclear. Additionally, the mechanisms by which convection facilitates angular momentum transport are still not well understood.

Two prominent but seemingly contradictory explanations for this phenomenon exist in the literature: the Conditional Instability of the Second Kind (CISK) and Wind-Induced Surface Heat Exchange (WISHE). Although these models offer different perspectives, we propose that they represent limiting, asymptotic scaling regimes of the same underlying physical process.

To reconcile these differing views, we use matched asymptotics to combine the three distinct regimes suggested by CISK and WISHE, thus providing a unified framework. Our analysis shows that the transport of angular momentum plays a crucial role in ensuring consistency with the asymptotic matching principle.

Interestingly, this work uncovers a new, previously undocumented pathway for angular momentum transport that may serve as a plausible mechanism for TC intensification. A key element of this process is the special role of the top-of-boundary-layer (BL) inflow, which is closely linked to the entrainment of convective cloud towers.

Through this combined approach, we offer a fresh perspective on TC intensification dynamics, confirming the validity of CISK and WISHE within their respective scopes and reconciling them into a more general theory.

How to cite: Dörffel, T., Klein, R., Doppler, S., and Khouider, B.: The role of entrainment in axisymmetric tropical cyclones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18675, https://doi.org/10.5194/egusphere-egu25-18675, 2025.

EGU25-18953 | ECS | Orals | AS1.23 | Highlight

The impact of Sulphate Aerosol Geoengineering on Tropical Cyclones 

Jasper de Jong, Michiel Baatsen, and Claudia Wieners

Sulphate Aerosol Geoengineering (SAG) works by increasing reflection of incoming solar radiation in the stratosphere and is a proposed way to mitigate global warming effects. Careful consideration of this method must include its impact on extreme weather, such as tropical cyclones. However, little to no SAG simulations exist at a resolution that is sufficient to explicitly model tropical cyclones due to the high computational cost of stratospheric chemistry. Recent work has shown a simple yet effective way to dynamically scale the stratospheric aerosol field from pre-existing SAG simulations to control global temperature, reducing the need for active stratospheric chemistry. Applying this method, we force a delayed SAG scenario in global fully-coupled CESM1 simulations with an atmosphere (ocean) grid resolution of 0.25 (0.1) degrees and compare it to a high forcing scenario. We present an examination of the impact of SAG on intensity, precipitation and track density of tropical cyclones.

How to cite: de Jong, J., Baatsen, M., and Wieners, C.: The impact of Sulphate Aerosol Geoengineering on Tropical Cyclones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18953, https://doi.org/10.5194/egusphere-egu25-18953, 2025.

EGU25-20415 | ECS | Orals | AS1.23 | Highlight

Climatic Trends in Tropical Cyclone Rainfall from High-Resolution Satellite Observations 

Shifei Tu, Jianjun Xu, and Johnny Chan

Heavy rainfall is a defining characteristic of tropical cyclones (TCs) and a significant contributor to the disasters they cause. Understanding how TC rainfall responds to climate change is critical, yet studies based on observational data remain limited compared to those relying on climate model simulations. Here, using high-resolution satellite observational rainfall data and numerical model results, we find that between 1999 and 2018, TC rain rates have exhibited contrasting trends in different regions. Globally, the TC rain rate increased by 8 ± 4%, primarily driven by enhanced rainfall in the outer regions due to increased atmospheric water vapor associated with rising surface temperatures. In contrast, the rain rate in the inner-core region of TCs decreased by 24 ± 3%, likely attributable to an increase in atmospheric stability. These findings provide valuable insights into the evolving climate characteristics of TC rainfall and their underlying mechanisms.

How to cite: Tu, S., Xu, J., and Chan, J.: Climatic Trends in Tropical Cyclone Rainfall from High-Resolution Satellite Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20415, https://doi.org/10.5194/egusphere-egu25-20415, 2025.

EGU25-313 | ECS | Orals | AS1.24

Forced Response in the Mean State and Interannual Variability of the Indian Summer Monsoon in Future Projections 

Nithya Kunnath, Aneesh Sundaresan, and Sijikumar Sivarajan

The Indian summer monsoon (ISM) is a complex system that plays a significant role in the climate of South Asia. We used Community Earth System Model 2-Large Ensemble (CESM2-LE) simulations to explore the forced response in the mean state and interannual variability of the ISM in future projections. The model is able to reproduce the mean state and interannual variability of the ISM during historical periods. The strengthening of monsoon circulation during excess rainfall years and weakening during deficient years are also well simulated by the model. It is also noticed that though the low-level jet stream shows a weakening during deficit monsoon years, it has more eastward extension up to the western Pacific Ocean compared to excess monsoon years. In simulations for future years, the mean structure of both the low-level jet stream and the tropical easterly jet stream becomes weaker compared to historical years. However, the precipitation pattern shows an enhancement in the future periods, and also the excess rainfall years in the future can be wetter than the historical excess years. Thus, the outcomes of CESM2-LE simulations are essential for formulating better plans for handling the effects of monsoon variability and policy-making efforts aimed at mitigating the impacts in a warming world. 

How to cite: Kunnath, N., Sundaresan, A., and Sivarajan, S.: Forced Response in the Mean State and Interannual Variability of the Indian Summer Monsoon in Future Projections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-313, https://doi.org/10.5194/egusphere-egu25-313, 2025.

The Madden-Julian Oscillation (MJO) has been a topic of great scientific interest due to its higher predictability and significant impact on global climate and weather, including the South American monsoon system. As a pillar of subseasonal predictability, it is important to investigate the influence of major interdecadal oscillations, such as the Interdecadal Pacific Oscillation (IPO) and the Atlantic Multidecadal Oscillation (AMO), to assess the potential modulation of MJO impacts by these oscillations. How do variations induced by these slower oscillations influence MJO teleconnections to South America (SA)? What is the frequency of MJO phases during the austral summer, and how might the interaction between the MJO and these oscillations affect the monsoon in SA? The combined impact of the MJO and low-frequency oscillations was characterized by composites of daily anomalies filtered in the 20-90 days band during the austral summer (DJF, rainy season), when the MJO is strongest. Composite anomalies of convection and circulation were analysed over the entire period from 1979 to 2020, as well as during two periods characterized by distinct combinations of opposite phases of the IPO and AMO: IPO(+)/AMO(-) (1979-1999, Period 1) and IPO(-)/AMO(+) (2000-2020, Period 2). Results indicate that during DJF, convection anomalies and the frequency of extreme events over SA are more pronounced in the Period 1 compared to Period 2, particularly in the central-east SA (CESA), the core monsoon region. In this region, increased (reduced) precipitation is observed during MJO phases 8 and 1 (4 and 5). Previous findings (Grimm, 2019) using Influence Function analysis, based on an extended vorticity equation model, and simulations, indicated a link between anomalous convection over the central subtropical South Pacific (CSSP) and the SA during phase 8 of the MJO, which may be responsible for the convection pattern in the CESA in phase 1. This anomalous convection in CSSP is stronger in Period 1 than in Period 2. Furthermore, there is a reversal in the sign of convective anomalies from reduced to enhanced precipitation in phase 6 over CESA from Period 1 to Period 2 and this may be associated with the change from reduced to enhanced convection over CSSP during phase 5, through teleconnections. Therefore, convection associated with MJO events during Period 1 is stronger (weaker) than in Period 2 in the CESA region during phases 8 and 1 (4, 5, 6 and 7). In contrast, in southern Brazil, positive convection anomalies persist from phases 3 to 5 in Period 1, whereas in Period 2 these anomalies are observed only in phases 3 and 4. Additionally, during Period 2, a reversal of the anomalies occurs in phases 1 and 2 compared to Period 1.

How to cite: Scheibe, L. A. and Grimm, A. M.: The Relationship of the Madden-Julian Oscillation with Interdecadal Variability Modes During the Monsoon Season in South America, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-315, https://doi.org/10.5194/egusphere-egu25-315, 2025.

EGU25-1017 | ECS | Posters on site | AS1.24

Dynamical Influence of Subtropical Jet Stream (STJ) and Tropical Easterly Jet (TEJ) on Indian Summer Monsoon Rainfall 

Rona Maria Sunil and Manoj Manguttathil Gopalakrishnan

The subtropical jet stream (STJ) and tropical easterly jet (TEJ) are critical upper-tropospheric features shaping the Indian summer monsoon (ISM). BY analysing data for the period 2000–2023, this study investigates the positional dynamics of these jets and their relationship with rainfall variability over the Indian region. Using ERA5 reanalysis data and daily rainfall records from the India Meteorological Department (IMD), we analysed the zonal and meridional wind fields at 200 hPa along with rainfall observations.

Four distinct jet stream cases were examined: both southern and northern hemispheric STJs shifting: (i) equator-ward, (ii) pole-ward, (iii) northward, and (iv) southward. Results reveal that equatorward shifts of the STJ weaken the TEJ and displace it southward, reducing rainfall over central India. Conversely, poleward migration of the STJ strengthens the TEJ, driving its northward extension and intensifying monsoonal rainfall, including extreme rainfall events. Northward shifts of both hemispheric STJs enhance TEJ strength, while southward shifts suppress it, altering the spatial distribution of rainfall. Strengthening of TEJ is expected to enhance the vertical velocity and LLJ through easterly vertical shear mechanism, and result in enhanced rainfall over the central Indian region. A TEJ Index (TEJI) was developed by area-averaging the TEJ core at 200 hPa, demonstrating strong correlations with rainfall intensity.

These findings underscore the complex interplay between STJ and TEJ and their dynamical role in modulating ISM rainfall. Understanding these mechanisms provides essential insights into atmospheric circulation patterns and their influence on monsoonal extremes, aiding improved prediction and climate resilience strategies in the region.

How to cite: Sunil, R. M. and Manguttathil Gopalakrishnan, M.: Dynamical Influence of Subtropical Jet Stream (STJ) and Tropical Easterly Jet (TEJ) on Indian Summer Monsoon Rainfall, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1017, https://doi.org/10.5194/egusphere-egu25-1017, 2025.

This study utilizes the monitoring of the onset dates of the rainy season across India, Southeast Asia, Central America, and West Africa to predict the upcoming season. By employing a straightforward objective method based on daily rainfall data, we pinpoint the onset date of the rainy season at each grid point of the rainfall analysis by identifying the minimum on the corresponding daily cumulative anomaly curve of rainfall. To accurately estimate the onset and retreat dates for each year, we introduce a perturbation technique that generates an ensemble of 100 time series of rainfall at every grid point.

Our research demonstrates that the onset data anomalies of the rainy season are directly linked to the length and seasonal rainfall anomaly of the season in all these regions. Specifically, seasons with an earlier onset tend to be longer and wetter, while those with a later onset are shorter and drier. Furthermore, we explore the relationship between onset, retreat, seasonal length, rainfall, and various large-scale climate drivers, revealing that although these relationships are local and relatively weaker, the intrinsic connections among the variables are robust.

In this study, we leverage the 12-hour latency product of Integrated Multi-Satellite Retrievals for the Global Precipitation Mission version 6 (IMERG) for near real-time monitoring of the season's evolution. The probabilistic skill scores, assessed using the area under the relative operating characteristic curve method, confirm the high predictive skill of anomalous onset dates.

How to cite: Misra, V.: The variations of the regional monsoons and their predictability from monitoring their evolution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1267, https://doi.org/10.5194/egusphere-egu25-1267, 2025.

EGU25-1484 | ECS | Orals | AS1.24

The role of the North American continent in strengthening the Asian monsoon 

Linlin Chen, Paul Valdes, and Alexander Farnsworth

Most studies on the formation of the modern Asian monsoon focus on mechanisms arising on the Afro-Eurasian continent. While few compare the effects of other remote continents. Using a fully coupled general circulation model, this study decomposes the relative contribution of each continent on the formation, distribution and intensity of the Asian monsoon. Here we show that the existence of the North American continent is critical for the formation and intensity of the Asian summer monsoon. The mechanism involves North America acting as an additional heating center, resulting in the strengthening and extension of oceanic advection towards the Asian monsoon region. This is achieved by the Rodwell-Hoskins mechanism that strengthens the North Pacific subtropical high and through a wide-spread Northern Hemispheric heating that shifts poleward the subsidence center of Hadley circulation. This teleconnection is not dependent on the Tibetan Plateau and its impact on East Asian summer precipitation is found to be smaller but comparable to the Tibetan Plateau. The individual role of the other non-Afro-Eurasian continents was found to be less important. Previous work has shown that the Asian monsoon has global impact, including changing the climate of North America. This study firstly shows the "reversed" teleconnection that North America can have a very significant impact on the Asian monsoon. Although these experiments are idealized and based on contemporary land-sea geometry, they also highlight the role of North America in the geologic evolution of the Asian monsoon, and imply the impacts of the anthropogenic climate change of North America to the Asian monsoon in the recent history and future.

How to cite: Chen, L., Valdes, P., and Farnsworth, A.: The role of the North American continent in strengthening the Asian monsoon, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1484, https://doi.org/10.5194/egusphere-egu25-1484, 2025.

EGU25-2173 | ECS | Orals | AS1.24 | Highlight

Atmospheric Influence of Summer Monsoon on Sea Ice Variability 

Jiawei Zhu and Zhiwei Wu

The impacts of tropical systems on polar sea ice have been relatively underestimated, which could potentially offer insights into the mechanisms driving sea ice variability and enhance predictive skills regarding sea ice extent. Our recent study delves into the influence of July-August Indian Summer Monsoon (ISM) precipitation on shaping Arctic sea ice variability from August to October, alongside exploring how the December-February Australian Summer Monsoon (AUSSM) modulates simultaneous Antarctic sea ice. Our findings suggest that ISM could explain up to 20% of Arctic sea ice concentration (SIC) variance across the marginal Arctic Ocean, while AUSSM could account for roughly 10% of SIC variance in the Pacific sector of the Southern Ocean including Amunsen and Ross Seas. Insights from both observation and model experiments demonstrate that the diabatic heating associated with ISM and AUSSM can trigger the poleward propagation of Rossby waves, culminating in barotropic anomalous circulations over the Arctic and Antarctic regions. These anomalous atmospheric patterns, characterized by highs and lows, have the potential to influence surface downwelling longwave radiation and surface winds, thereby shaping sea ice variability through a combination of thermodynamic and dynamic processes.

How to cite: Zhu, J. and Wu, Z.: Atmospheric Influence of Summer Monsoon on Sea Ice Variability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2173, https://doi.org/10.5194/egusphere-egu25-2173, 2025.

EGU25-2285 | Posters on site | AS1.24

Reconciling roles of the South China Sea summer monsoon and ENSO in prediction of the Indian Ocean dipole 

Jianping Li, Yazhou Zhang, Yina Diao, Qiuyun Wang, Renguang Wu, Ting Liu, Yishuai Jin, Zhaolu Hou, and Haili Wang

The Indian Ocean dipole (IOD) is a remarkable interannual variability in the tropical Indian Ocean. The improved prediction of IOD is of a great value because of its large socioeconomic impacts. Previous studies reported that both El Ni˜ no-Southern Oscillation (ENSO) and South China Sea summer monsoon (SM) play a dominant role in the western and eastern pole of the IOD, respectively. They can be used as predictors of the IOD at 3 month lead beyond self-persistence. Here, we develop an empirical model of multi-factors in which the western pole is predicted by ENSO and persistence and the eastern pole is predicted by SM and persistence. This new empirical model outperforms largely the average level of the dynamical models from the North American multi-model ensemble (NMME) project in predicting the peak IOD in boreal autumn, with a correlation coefficient of ∼0.86 and a root mean square error of ∼0.24°C. Furthermore, the hit rate of positive culminated IOD in this new empirical model is equivalent to that in current NMME models (above 65%), much higher than that for negative culminated IOD. This improvement of skill using the empirical model suggests a perspective for better understanding and predicting the IOD.

How to cite: Li, J., Zhang, Y., Diao, Y., Wang, Q., Wu, R., Liu, T., Jin, Y., Hou, Z., and Wang, H.: Reconciling roles of the South China Sea summer monsoon and ENSO in prediction of the Indian Ocean dipole, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2285, https://doi.org/10.5194/egusphere-egu25-2285, 2025.

EGU25-2330 | ECS | Orals | AS1.24

Unravelling large-scale onset and progression of the Indian monsoon from the evolution of clusters of local onsets using network science 

Gaurav Chopra, Yogenraj Patil, Shruti Tandon, Bhupendra Nath Goswami, and Raman I Sujith

Developing an accurate definition of the onset and progression of the Indian monsoon is an outstanding research area in climate science. Determining monsoon onset dates is critical for agricultural planning and ensuring food security for billions of people in India and the world. The onset of the Indian monsoon is associated with the northward shift of the planetary-scale intertropical convergence zone (ITCZ) from the equator. ITCZ is a zone of intense convective activity, cloudiness and high precipitation girdling the Earth. As a result, the onset and progress of the Indian monsoon are interconnected on a planetary scale.

The monsoon onset definition can be classified into local and large-scale definitions. Local-scale definitions utilize daily precipitation over a small region to determine the onset. However, they are prone to bogus onsets because of pre-monsoon rains and transient weather systems. Large-scale definitions are based on precipitation and wind/cloudiness over a bigger area. However, such averaging does not guarantee separation of the ‘large-scale’ component of ITCZ precipitation from the ‘small-scale’ local contributions and is still prone to bogus onsets. Large-scale onset definitions are largely confined to defining the monsoon onset over Kerala (MoK) while representing the progression of monsoon is based entirely on local onsets. We overcome this limitation by developing a large-scale definition from small-scale local onsets interconnected on a planetary scale.

We utilize networks and their phase transitions to develop a large-scale definition. We construct time-varying spatial proximity networks based on daily precipitation, where nodes are the geographical locations in a domain encompassing India. Links are established only between nodes that are in geographical proximity and if they have undergone local onsets. Next, we estimate connected components in the network that represent clusters of local onsets. The spatiotemporal evolution, involving the growth and coalescence of clusters disentangles the true large-scale monsoon onset and progression.

We discover two abrupt phase transitions in the size of the largest cluster of the local onsets. These phase transitions are associated with the formation of large clusters representing the local onsets interconnected at a planetary scale. Thus, we unravel the setting up of the ITCZ and other synoptic-scale convective systems that facilitate consistent monsoon activity over India. We define large-scale onsets when a location becomes part of the largest cluster following the first transition.

Using lead-lag composites of precipitation for the past 84 years centred on large-scale onsets, we find that our definition captures important characteristics of the Indian monsoon usually missed by conventional large-scale definitions. During our onsets, the rainfall is strong at a large scale along the western ghats and northeast India (NEI). Further, they are followed by a rapidly northward propagating rainfall pulse, also known as the monsoon intraseasonal oscillation. Our method captures that the onset over NEI occurs before MoK, which is consistent with several recent studies but missed by conventional definitions. These new findings necessitate a reexamination of the interannual variability in the Indian monsoon, which will be discussed in the talk.

How to cite: Chopra, G., Patil, Y., Tandon, S., Goswami, B. N., and Sujith, R. I.: Unravelling large-scale onset and progression of the Indian monsoon from the evolution of clusters of local onsets using network science, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2330, https://doi.org/10.5194/egusphere-egu25-2330, 2025.

EGU25-2552 | ECS | Orals | AS1.24

The role of dry intrusions in breaks of the Indian summer monsoon 

Akshay Deoras, Andrew Turner, Ambrogio Volonté, Reinhard Schiemann, Laura Wilcox, and Arathy Menon

The Indian summer monsoon (ISM) is of great importance to over a billion people since it supplies over 75% of the country’s annual precipitation. Significant intraseasonal variability in rainfall affects people, with breaks responsible for causing water shortage. It is known that dry intrusions play a role in breaks; however, it is not well understood compared to the role dry intrusions play during progressions of the onset and withdrawal of the ISM. In this study, we use observations and the ERA5 reanalysis to understand the role of dry intrusions in breaks during 1940–2023. We develop an index based on moisture deficit to identify dry intrusions, and find that most breaks are associated with dry intrusions emanating from arid regions to the west and northwest of India. These dry intrusions begin to enter India around a week prior to the middle day of breaks, reaching their peak strength over north India three days prior to the middle day of breaks. Vertical profiles reveal that these are mid-level dry intrusions, which are similar to those driving the direction of the withdrawal of the ISM. As breaks evolve, these dry intrusions deepen throughout their horizontal extent and descend into the country, stabilising the troposphere and creating an unfavourable environment for deep convection. We also find that extended breaks have stronger dry intrusions as precursors. This work provides a new perspective on the causal relationship between mid-level dry intrusions and breaks. The results could help improve forecasts of breaks, ultimately benefiting stakeholders in improving long-term planning.

How to cite: Deoras, A., Turner, A., Volonté, A., Schiemann, R., Wilcox, L., and Menon, A.: The role of dry intrusions in breaks of the Indian summer monsoon, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2552, https://doi.org/10.5194/egusphere-egu25-2552, 2025.

The East Asian monsoon is one of the most important features in the global climate system. Understanding the variation and moisture sources of East Asian monsoon precipitation is crucial for improving land-atmosphere interactions, developing more accurate global climate models, and optimizing the region’s water management strategies. Monsoon precipitation is produced from both local moisture through evapotranspiration and remote moisture transported from oceans via large-scale circulation. This study investigates the relative contribution of local and remote moisture sources to total monsoon precipitation in East China using model outputs from 12 CMIP6 simulations. Simulations from the historical experiments of CMIP6 are selected for the period of 1950-2014. These 12 CMIP6 models are selected based on the availability of data related to convective precipitation and soil moisture. In this study, we focus on the percentage of convective precipitation in total monsoon precipitation and soil moisture-precipitation relationship in East China. East China is divided into five regions based on their climate conditions. Our analysis suggests a significant spatial and temporal variation in the contribution of local convective precipitation to overall monsoon precipitation among different models. On average, the Southeast region shows a higher percentage of convective precipitation and a stronger soil moisture-precipitation correlation than other regions. Additionally, the percentage of convective precipitation varies significantly between models. The findings from this analysis could offer insights for enhancing the development of future climate models.

How to cite: Meng, L.: Relative contribution of local and remote sources of moisture to East Asian monsoon precipitation in CMIP6 simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2584, https://doi.org/10.5194/egusphere-egu25-2584, 2025.

We present novel explainable deep learning techniques for reconstructing South Asian palaeomonsoon rainfall over the last 500 years, leveraging long instrumental precipitation records and palaeoenvironmental datasets from South and East Asia to build two types of models: dense neural networks (“regional models”) and convolutional neural networks (CNNs). The regional models are trained individually on seven regional rainfall datasets, and while they capture decadal-scale variability and significant droughts, they underestimate inter-annual variability. The CNNs, designed to account for spatial relationships in both the predictor and target, demonstrate higher skill in reconstructing rainfall patterns and produce robust spatiotemporal reconstructions. The 19th and 20th centuries were characterised by marked inter-annual variability in the monsoon, but earlier periods were characterised by more decadal- to centennial-scale oscillations. Multidecadal droughts occurred in the mid-17th and 19th centuries, while much of the 18th century (particularly the early part of the century) was characterised by above-average monsoon precipitation. Extreme droughts tend to be concentrated in southern and western India and often coincide with recorded famines. The years following large volcanic eruptions are typically marked by significantly weaker monsoons, but the sign and strength of the relationship with the El Niño–Southern Oscillation (ENSO) vary on centennial timescales. By applying explainability techniques, we show that the models make use of both local hydroclimate and synoptic-scale dynamical relationships. Our findings offer insights into the historical variability of the Indian summer monsoon and highlight the potential of deep learning techniques in palaeoclimate reconstruction.

How to cite: Hunt, K. and Harrison, S.: A novel explainable deep learning framework for reconstructing South Asian palaeomonsoons, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2815, https://doi.org/10.5194/egusphere-egu25-2815, 2025.

EGU25-2958 | ECS | Posters on site | AS1.24

Indian Summer Monsoon rainfall changes beyond the 21st century 

Sahil Sharma, Kyung-Ja Ha, Keith Rodgers, Eui-Seok Chung, Sun-Seon Lee, and Arjun Babu Nellikkattil

Future rainfall changes in India are of paramount importance for crop production and water management, but to date, longer-term changes beyond the year 2100 have not been evaluated. Here, we leverage a 10-member extension of the CESM2 Large Ensemble under relatively strong emissions (SSP3-7.0) to identify projected rainfall changes and the underlying physical mechanism out to 2500. Our main finding is that after 2100, substantial changes occur in large-scale atmospheric circulation patterns, which are more pronounced and distinct from the changes projected over the 21st century. We test the hypothesis that under substantial thermal perturbations to the climate system after 2100, the increased atmospheric stability caused by the enhanced differential heating in the upper troposphere relative to land weakens the large-scale monsoonal circulation, while enhanced warming over the Tibetan Plateau causes a poleward shift in low-level monsoonal circulation and the climatological pressure belt. This projected shift promotes enhanced northward moisture transport, resulting in a strengthened anomalous ascending motion over northern India, ultimately leading to increased Indian summer monsoon rainfall post-2100. These changes reflect local expression of large-scale climate dynamical perturbations and provide a broader mechanistic framework for understanding long-term future climate change over India. 

How to cite: Sharma, S., Ha, K.-J., Rodgers, K., Chung, E.-S., Lee, S.-S., and Nellikkattil, A. B.: Indian Summer Monsoon rainfall changes beyond the 21st century, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2958, https://doi.org/10.5194/egusphere-egu25-2958, 2025.

EGU25-3589 | Posters on site | AS1.24

Future South American monsoon changes are sensitive to Atlantic SST pattern changes 

Robin Chadwick, Peter Good, Jorge Garcia-Franco, Lincoln Alves, Neil Hart, Marcia Zilli, Herve Douville, Marion Saint-Lu, and Brian Medeiros

Future projections of South American Monsoon (SAM) precipitation from CMIP6
(Coupled Model Intercomparison Project phase 6) show a consistent drying during the early part
of the monsoon season (September to November), which is also seen in a convection-permitting
model simulation. Using a set of idealised atmosphere-only GCM experiments, this drying signal
is shown to be mainly driven by sea surface temperature (SST) changes: uniform SST warming
and patterned SST change. Different processes appear to be more important in different months
for the ensemble mean drying signal, with this primarily driven by SST pattern change in October
and by uniform SST warming in November. There is significant inter-model uncertainty in the
SAM precipitation response to each of these drivers, particularly SST pattern change. For uniform
SST warming, an existing hypothesis which suggests that SAM drying is driven by the enhanced
land-sea temperature contrast is tested, but we find that this process is not dominant. For patterned
SST warming, moderate inter-model correlations (across the coupled CMIP6 models) are found
between SAM precipitation change and changes in meridional and zonal Atlantic SST gradients.
In November, a combined zonal and meridional Atlantic SST gradient index can explain more than
half of CMIP6 inter-model uncertainty in SAM core region precipitation change.

How to cite: Chadwick, R., Good, P., Garcia-Franco, J., Alves, L., Hart, N., Zilli, M., Douville, H., Saint-Lu, M., and Medeiros, B.: Future South American monsoon changes are sensitive to Atlantic SST pattern changes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3589, https://doi.org/10.5194/egusphere-egu25-3589, 2025.

EGU25-3823 | ECS | Orals | AS1.24

Monsoonal mixed layer heat budget of the Indian Ocean: Understanding the biases in coupled forecast models. 

Aparna Anitha Reghunathan, Ben Webber, Adrian Matthews, Dan Copsey, and José Rodriguéz

The Indian Ocean plays an important role in modulating the global weather and climate. However, many state-of-the-art climate models can't predict the dynamically complex mechanisms of the Indian Ocean accurately. Studies show that the biases in the earlier versions of the Met Office Climate Model developed during the initial days of model simulation and persisted up to climate time scales. To investigate biases in the revised GC5 model, we analyzed 208 monthly forecasts initialized every five days from June to November (2018–2023). The spatial evolution of the SST biases over the Indian Ocean from these forecasts showed specific regions of warm and cold biases with up to a magnitude of ~ -1°C to 1°C. This regional bias formation is examined using the mixed layer heat budget analysis during the Indian summer and winter monsoons to understand the relative contribution of the various parameters in driving this variability. We have selected three warm SST bias regions, on the east coast of Africa, near the Indian Peninsula and on the west coast of Sumatra. The cold bias regions are in the northern Arabian Sea and on the west coast of Java. The primary analysis from the mixed layer heat budget shows that the warm and cold SST biases in the model are modulated mainly by some common parameters such as the net heat flux and total advection. However, further analysis showed that the total advection is more important in the warm bias regions. The vertical mixing term is also significant in generating cold SST biases and this can be a consequence of the positive wind speed biases in the model. Our study also concludes that even though the biases have comparable spatial and temporal magnitude and evolution, the parameters which modulate the SST variability have regional variations. Additionally, anomalously positive precipitation in the equatorial Indian Ocean and the west coast of India and a negative precipitation bias along the east coast of India were also identified. Hence removing these discrepancies in the SST might be crucial for accurately simulating the Indian monsoon. 

How to cite: Anitha Reghunathan, A., Webber, B., Matthews, A., Copsey, D., and Rodriguéz, J.: Monsoonal mixed layer heat budget of the Indian Ocean: Understanding the biases in coupled forecast models., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3823, https://doi.org/10.5194/egusphere-egu25-3823, 2025.

EGU25-4614 | ECS | Orals | AS1.24

Investigation and Future Projection of Warm Rain During Winter Monsoon in Java Sea, Indonesia 

Wendi Harjupa and Eiichi Nakakita

This study investigates the characteristics and future trends of warm rain during the winter monsoon season (December, January, February; DJF) over Indonesia, with a focus on the Java Sea. The analysis integrates satellite observations from the Tropical Rainfall Measurement Mission (TRMM), reanalysis datasets (ERA5), and model simulations from the Atmospheric General Circulation Model (AGCM). An analysis of ERA5 data (1950–2009) reveals a pronounced upward trend in SST across the broader Indonesian region (slope 0.0070) and the Java Sea (slope 0.0094), with the most significant increases occurring during DJF. Cloud Liquid Water Content (CLWC), positively correlated with SST and rainfall, is used as a proxy for warm rain. TRMM satellite observations confirm that warm rainfall corresponds spatially with CLWC distribution. AGCM simulations effectively replicate observed CLWC patterns, showing strong alignment with TRMM data, particularly over western Indonesia, including the Java Sea. Convergence patterns derived from ERA5 and AGCM data exhibit similar trends, emphasizing the role of atmospheric convergence in CLWC formation over the Java Sea. An analysis of 95th percentile CLWC values at lower atmospheric levels (1000–700 hPa) highlights a significant increase in CLWC during DJF over the northwestern Indonesian region, including the Java Sea, across 30-year intervals spanning 150 years (1950–2099). These findings underscore the critical influence of the winter monsoon on warm rain processes in the Java Sea and its connection to extreme weather events, such as flooding in Jakarta, located on the southern coast of the Java Sea.

How to cite: Harjupa, W. and Nakakita, E.: Investigation and Future Projection of Warm Rain During Winter Monsoon in Java Sea, Indonesia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4614, https://doi.org/10.5194/egusphere-egu25-4614, 2025.

EGU25-5379 | ECS | Orals | AS1.24

Aerosol mitigation matters to future water availability in the global monsoon region 

Jie Jiang, Tianjun Zhou, and Wenxia Zhang

Water availability, as measured by precipitation minus evaporation (P-E), is projected to increase in the 21st century across global monsoon regions. However, while the impacts of increased greenhouse gas (GHG) concentrations are highlighted in existing studies, the contribution of reduced anthropogenic aerosol (AA) emissions is likely to be overlooked. Here, utilizing single-forcing projections under the SSP2-4.5 scenario, we elucidate the fingerprints of GHG and AA forcings on future P-E evolution. We reveal that the future wetting trend is primarily driven by an increase in P-E during the wet season. The escalation of GHG concentrations is projected to increase P-E over Asian-African monsoon domains while decreasing it over American monsoon domains. Conversely, aerosol reductions will drive a transition from current widespread drying to future wetting. While both the GHG increase and AA reduction can elevate atmospheric moistening through radiative warming, the disparate P-E responses come from dynamic processes that favor drying trends in American monsoon domains under GHG forcing. In contrast, strengthened monsoon circulations contribute to a wetting trend in Asian monsoon domains under AA reductions, attributable to greater interhemispheric thermal contrast. Our finding highlights the importance of considering aerosol mitigation in climate risk assessment for densely populated monsoon regions.

How to cite: Jiang, J., Zhou, T., and Zhang, W.: Aerosol mitigation matters to future water availability in the global monsoon region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5379, https://doi.org/10.5194/egusphere-egu25-5379, 2025.

Using 51 models of the AMIP and historical experiments of CMIP6, we investigate the inter-model diversity of atmospheric and coupled models in the strength of the Indian Summer Monsoon Rainfall (ISMR)–El Niño-Southern Oscillation (ENSO) relationship. In atmospheric models, the Walker Circulation (WC) intensity associated with the western Pacific convective activity is most responsible for the inter-model diversity. Models with strong WC have a strong ISMR–ENSO relationship via enhancing ENSO-induced anomalies of the WC and monsoon circulation. The secondary source is the monsoon circulation differences associated with meridional rainfall contrast over the Indian monsoon region. In coupled models, the primary (secondary) source is the ENSO amplitude (WC intensity). In observation, the decadal variation of WC can also explain the changes in the ISMR–ENSO relationship. This study provides a basis for improving the model performance and advances our understanding of the observed ISMR–ENSO relationship changes.

How to cite: Yu, S.-Y.: Sources of Inter-Model Diversity in the Strength of the Relationship Between the Indian Summer Monsoon Rainfall and El Niño-Southern Oscillation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5422, https://doi.org/10.5194/egusphere-egu25-5422, 2025.

EGU25-6038 | ECS | Posters on site | AS1.24

Distinct Characteristics of Active and Break Spells in Flood and Drought Years of the Indian Summer Monsoon  

Ritesh Jha, Ravi Nanjundiah, and Ashwin Seshadri

The Indian summer monsoon displays intraseasonal variability with alternating "active" (intense rainfall) and "break" (deficient rainfall) phases. Analysis of Indian Meteorological Department (IMD) daily rainfall data (1979–2020, June–September) over Central India (CI) shows that active spells are more frequent during flood years (4.6 events/year) than drought years (2.3 events/year), with similar durations (3–4 days). In contrast, break spells are more frequent and prolonged in drought years (3.9 events/year, 6–7 days, occasionally exceeding 10 days) compared to flood years (1.2 events/year, 3–4 days).  

 Composites of mean sea level pressure reveal distinct intraseasonal dynamics between flood and drought years. During flood years, positive pressure anomalies propagate northwestward from the Bay of Bengal, while in drought years, they propagate poleward and stagnate over Central India, reducing active spell frequency. Similarly, break spells exhibit westward-moving anomalies in flood years, whereas drought years are characterized by stationary anomalies and poleward propagation.  

 Intraseasonal oscillations (ISOs) derived from IMD rainfall data strongly influence active and break spells. Flood years are characterized by high-frequency ISOs (HF-ISOs) with westward propagation, enhancing active spells, while drought years are dominated by low-frequency ISOs (LF-ISOs) with poleward movement, leading to prolonged breaks. Over 90% of these spells align with HF-ISO in flood years and LF-ISO in drought years. Total column water composites reveal frequent midlatitude dry air intrusions during drought years, contributing to extended break spells. Moisture budget analysis indicates that differences in mean moisture advection by mean winds drive anomalies, with positive values during flood years and negative values during drought years. 

 K-means clustering reveals the relationship between ISO variability and seasonal rainfall through four clusters based on variance explained by LF-ISO and HF-ISO. The cluster with the strongest LF-ISO and weakest HF-ISO records the lowest rainfall (92% of the long-term mean), while the opposite cluster experiences the highest rainfall (112% of the long-term mean). These findings align with observed HF and LF ISO intensities during flood and drought years. Strong HF-ISO activity is associated with enhanced formation and northwestward propagation of low-pressure systems from the Bay of Bengal to Central India, contributing to above-normal rainfall. Additionally, the strong HF-ISO cluster features strong low-level westerlies supported by upper-level easterlies, alongside tropospheric conditions limiting dry air intrusion from midlatitudes. In contrast, low rainfall in the cluster with large LF-ISO variance coincides with low-level easterly anomaly, and concomitantly weaker moisture transport from the Arabian Sea (AS).  Clusters with maximum LF-ISO intensity feature mid-tropospheric high pressure over CI, reflecting downdrafts of dry, cold upper-level air that suppress convection and cause seasonal rainfall deficits. Midlatitude intrusions are observed in clusters with moderately strong LF-ISO intensity, accompanied by southeasterly winds northwest of CI. These intrusions are weaker, maintaining rainfall near the long-term mean.  

This study underscores the contrasting active and break spells during flood and drought years, highlighting the role of ISOs, atmospheric dynamics, and thermodynamic processes. 

How to cite: Jha, R., Nanjundiah, R., and Seshadri, A.: Distinct Characteristics of Active and Break Spells in Flood and Drought Years of the Indian Summer Monsoon , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6038, https://doi.org/10.5194/egusphere-egu25-6038, 2025.

EGU25-6560 | ECS | Posters on site | AS1.24

Environmental features related to the decadal variation of South China Sea tropical cyclogenesis in the context of summer monsoon 

Yuhao Cai, Song Yang, Huan Wu, Weizhen Chen, and Juying Xu

This study investigates the changes in environmental conditions related to the decadal variation of genesis frequency of tropical cyclones (TCGF) over the South China Sea (SCS) during summer. Corresponding to the decadal increase in the TCGF, the seasonal mean anomalies of the genesis potential and environmental fields over the SCS are not favorable for tropical cyclogenesis, indicating their limited role in the decadal variation of SCS TCGF. It is found instead that the decadal change in tropical cyclogenesis over the SCS is more attributed to the local environmental fields associated with atmospheric intraseasonal oscillation (ISO). The decadal change in SCS TCGF is closely linked to the northward extension of ISO-related convection from the central SCS, which is contributed by the horizontal advection by background monsoon flow and the vertical advection by ISO-related vertical motions. Further analyses indicate that the anomalous upper-level cyclonic circulation over East Asia and the lower-level anticyclonic circulation over the western Pacific produce the unfavorable seasonal mean environmental fields in the SCS, whereas the resultant strong summer mean SCS monsoon flow facilitates the northward extension of ISO-related convection. This study highlights the importance of ISO activity for projections of the long-term change in SCS TC activity.

 

How to cite: Cai, Y., Yang, S., Wu, H., Chen, W., and Xu, J.: Environmental features related to the decadal variation of South China Sea tropical cyclogenesis in the context of summer monsoon, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6560, https://doi.org/10.5194/egusphere-egu25-6560, 2025.

This study examines how the summertime Indian Ocean (IO) SST anomalies (SSTAs) affect the Indian Summer Monsoon (ISM) and its predictability in the El Niño developing years from the perspective of seasonal predictions of 1972 and 1997 when observed drastically different ISM states. The CFSv2-COLA ensemble seasonal reforecasts produce a successful ISM prediction in 1972 but a failed one in 1997. Our sensitivity experiments, in which the ocean and atmosphere are decoupled in the tropical IO with the prescribed SST, reveal that the erroneous prediction of cold IO SSTAs in 1997 exacerbates an El Niño-induced ISM drought and “correcting” these SST errors improves the ISM prediction substantially, whereas a good prediction of the summertime IO SSTAs contributes positively to the skillful ISM reforecast in 1972. It is also demonstrated that the warm IO SSTAs centered in the Arabian Sea in 1997 reduce sea-level pressures locally and steer the low-level anomalous winds to transport water vapor into the India. This regional process counters the El Niño-induced drought tendency and results in a nearly normal ISM that defies the historical El Niño-ISM relation. However, the warm SSTAs centered at the western equatorial IO in 1972 strengthen the anomalous Walker circulations originally set up by the developing El Niño in the Indo-Pacific domain, which further enhance the El Niño evolution and its teleconnection to the ISM. This inter-basin feedback process intensifies the typical El Niño-ISM relation. The spatial structure of the summer IO SSTAs may determine whether the IO regional process or the inter-basin process prevails. 

How to cite: Shin, C.-S.: Influences of the Indian Ocean SST on the Indian Summer Monsoon and its Seasonal Prediction in El Niño Developing Years , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7074, https://doi.org/10.5194/egusphere-egu25-7074, 2025.

Large mountain regions influence local- and global-scale atmospheric flow through mechanical forcing and changes in temperature and pressure fields. The topography of High-Mountain Asia (HMA), for example, is critical for the development of important characteristics of the Indian Monsoon. In this study, global climate model sensitivity experiments are applied to quantify the magnitude and geographical extent of the effects of HMA topography on Northern Hemisphere atmospheric flows. A series of ECHAM5-wiso (climate model) experiments were set up, in which HMA topography is reduced incrementally by 25% of its current height. All other boundary conditions, such as greenhouse gas concentrations and ice cover, are kept constant. The impact of the simulated topographic changes on the Eurasian Wave Train (EWT), which is critical for Northern Hemisphere atmospheric transport, is evaluated by examining the loading patterns from empirical orthogonal functions analyses conducted on the simulated pressure and wind fields. The impact of HMA topography on the intensity and extent of meridional flow in South Asia is assessed by examining wind speeds at different pressure levels. Changes in the EWT are particularly prominent in (Central) Asia. These may be attributed to the significant changes in pressure fields west of the Tibetan Pleateau as the topography in the HMA region is varied. Furthermore, increasing HMA topography from 0% to 100% significantly increases 1) average meridional summer wind speeds (by ≤10 m/s) at the 200hPa and 1000hPa levels, and 2) the extent of northward, monsoonal flow over the Indian subcontinent. The simulations only predict notable northward flow over western and northern India in summer if HMA topography is set to 50% of its modern height. The flow’s northeastern extent is restricted to 25°N-65°E in the absence of HMA topography, but reaches 33°N-75°E when it is fully developed.

How to cite: Mutz, S. G.: The Effect of High-Mountain Asia Topography on Northern Hemisphere Atmospheric Flow, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7283, https://doi.org/10.5194/egusphere-egu25-7283, 2025.

EGU25-9304 | ECS | Orals | AS1.24

Indian Summer Monsoon Onset Delayed by the Weakening of Hadley Circulation  

Vaishnavi Wadhai, Balaji Senapati, and Mihir Kumar Dash

The timing of the Indian Summer Monsoon (ISM) onset significantly impacts agriculture, food production, the economy, and livelihoods in India. Parker et al. (2016) highlighted the role of both mid-level dry northwesterly winds and low-level moist southwesterly winds in influencing the climatological ISM onset. However, the question of what drives the delay in ISM onset remains unclear and uncertain. Is it primarily due to mid-level dry northwesterly winds, low-level moist southwesterly winds, or a combination of both? In this study, we find that the weakening of low-level moist southwesterly winds is the primary factor, while the mid-level dry northwesterly winds remain unaltered during delayed onset years. This weakening of southwesterly winds is associated with the low-level circulation anomaly caused by the anomalous high pressure over the Arabian Sea, which is further linked to the weakening of the Hadley circulation. The relatively low pressure over the Mascarene High reduces the cross-equatorial pressure gradient, weakening the Hadley circulation, which in turn weakens the southwesterly winds, thereby delaying the ISM onset. Understanding the underlying mechanisms of delayed monsoon onset provides critical insights for improving Indian monsoon modelling and prediction. 

How to cite: Wadhai, V., Senapati, B., and Dash, M. K.: Indian Summer Monsoon Onset Delayed by the Weakening of Hadley Circulation , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9304, https://doi.org/10.5194/egusphere-egu25-9304, 2025.

EGU25-10023 | ECS | Posters on site | AS1.24

Understanding the Uncertainty in the West African Monsoon Precipitation Response to Increasing CO2 

Harry Mutton, Robin Chadwick, Matthew Collins, F. Hugo Lambert, Christopher Taylor, Ruth Geen, Hervé Douville, and Marion Saint-lu

The West African Monsoon (WAM) precipitation response to increased CO2 is uncertain, with both large increases and decreases predicted by  CMIP6 models. To address this, the full impact of increased CO2 has been decomposed into several drivers, three of which are shown to contribute most to  the uncertainty in WAM precipitation; the direct radiative effect of increased CO2, the impact of a uniform Sea Surface Temperature (SST) warming, and the impact of a patterned SST change. Much of the uncertainty associated with the response to the direct radiative effect and uniform SST warming is shown to be related to differing changes in 700hPa moisture flux divergence associated with the shallow meridional circulation over West Africa as well as differences in a soil moisture - surface heat flux feedback over the Sahel. For the SST pattern effect, the difference between North Atlantic SSTs as well as inter-hemispheric gradients in surface temperatures are key drivers of intermodel spread.

How to cite: Mutton, H., Chadwick, R., Collins, M., Lambert, F. H., Taylor, C., Geen, R., Douville, H., and Saint-lu, M.: Understanding the Uncertainty in the West African Monsoon Precipitation Response to Increasing CO2, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10023, https://doi.org/10.5194/egusphere-egu25-10023, 2025.

EGU25-10438 | Orals | AS1.24

Attribution of the Extreme Drought Event over the Yangtze River Valley in China 

Lixia Zhang, Tianjun Zhou, Xing Zhang, Wenxia Zhang, Lijuan Li, and Laurent Li

Global warming has led to the intensification and increased frequency of drought events. Determining the extent to which these events are influenced by human activities is critical for developing effective strategies to address climate change. However, detecting human impacts and providing robust attribution results remain key challenges in drought research. In the summer of 2022, the Yangtze River Valley of China experienced an unprecedented extreme drought, marked by record-high surface temperatures and record-low precipitation over the past 60 years. This event caused substantial socio-economic and ecological disruptions. To assess the role of anthropogenic climate change in the intensity and frequency of such events, this study established an attribution framework based on GAMIL3.0. This study evaluated anomalies in surface temperature, precipitation, and large-scale circulation patterns during the summer of 2022. Results indicate that human activities have intensified the Western North Pacific Subtropical High and South Asian High, increasing their strength and frequency and thereby amplifying the intensity and likelihood of extreme drought events in the Yangtze River Valley. Anthropogenic forcing contributed to an additional 0.8°C rise in surface temperature (95% confidence interval: 0.1–1.5°C) and a 7.9% reduction in precipitation (-24.1% to 7.8%) during the 2022 summer. The anthropogenic forcing increased the probability of surface temperature anomalies associated with such an extreme drought event like 2022 by 1300 times (range: 87–3,001) and precipitation anomalies by 65 times (range: 1–90). This study highlights the urgent need to strengthen adaptive capacities to mitigate the impacts of extreme drought in the Yangtze River Valley.

How to cite: Zhang, L., Zhou, T., Zhang, X., Zhang, W., Li, L., and Li, L.: Attribution of the Extreme Drought Event over the Yangtze River Valley in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10438, https://doi.org/10.5194/egusphere-egu25-10438, 2025.

The Hengduan Mountains region (HM), located in the Eastern Tibetan Plateau, is renowned for its rich biodiversity. High-resolution climate data from past periods are essential for gaining deeper insights into the ecological and evolutionary processes that have shaped this unique and diverse region. In this study, we applied the non-hydrostatic limited-area model COSMO, with a resolution of 12 km over East Asia, to simulate two distinct climatic periods: the mid-Pliocene (~3 Ma), representing a warmer period, and the Last Glacial Maximum (LGM; ~21 ka), a colder period, both compared to present-day conditions.

Our results reveal that, despite contrasting changes in moisture supply, both warm and cold periods experienced a weakened Indian summer monsoon, attributed to the exposure of the Indochina continental shelf during these times—caused by sea-level drops during the LGM and dynamic topography during the mid-Pliocene. During the mid-Pliocene, an earlier northward migration of the Western Jet led to an earlier onset of the Indian summer monsoon and a wetter spring in the HM. In contrast, the HM experienced increased precipitation during the LGM in both summer and winter. Increased summer precipitation was driven by enhanced moisture supply from the south, while enhanced winter precipitation, primarily in the form of snowfall at high elevations, was associated with more unstable atmospheric stratification.

The local precipitation characteristics of the HM are thus influenced by the interplay between large-scale atmospheric dynamics and regional topographical features such that, in contrast to most mid-latitude regions, the HM did not experience drying and wetting during glacial-interglacial cycles. The stability of mean precipitation across different climatic periods likely played a pivotal role in supporting the HM's high biodiversity, providing a stable and moist environment conducive to supporting diverse ecosystems.

How to cite: Xiang, R., Steger, C. R., Willett, S. D., and Schär, C.: Influence of Asian Monsoon Dynamics on Precipitation Characteristics of the Eastern Tibetan Plateau in Cold and Warm Climates: Insights from a Regional Climate Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13143, https://doi.org/10.5194/egusphere-egu25-13143, 2025.

Analysis of ground-based and remotely retrieved precipitation data reveals that heavy Meiyu precipitation events (HMPEs) produce a relatively independent rain-belt over eastern China. A rotating calipers algorithm is applied to quantify the spatial scales of HMPEs. We find that HMPEs have regular spatial scales with an average length, width and extent of about 1400 km, 500 km and 40.00 × 104 km2, respectively, through a comprehensive assessment of different types of HMPE, illustrating that HMPEs have a size similar to that of the sub-synoptic-scale Meiyu front (1500–2000 km). Convective activities along the Meiyu front zone and the upper westerly jet stream strongly affect the position and orientation of rain-belts of HMPEs. The Meiyu front zone, strong vertical motions and large transport of warm moisture have a comparable spatial scale to the HMPE rain-belts over eastern China.

How to cite: Du, Y., Xie, Z., and Miao, Q.: Spatial Scales of Heavy Meiyu Precipitation Events in Eastern China and Associated Atmospheric Processes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13901, https://doi.org/10.5194/egusphere-egu25-13901, 2025.

EGU25-13961 | ECS | Orals | AS1.24

Timescale-dependent fingerprint of the Asian Summer Monsoon during the last Glacial and its impact on vegetation 

Nils Weitzel, Martina Stebich, Moritz Adam, Jens Mingram, and Kira Rehfeld

The Asian Summer Monsoon is fundamental for the water supply of billions of people. It has undergone major changes over the Pleistocene in response to greenhouse gas and ice sheet forcing during glacial-interglacial transitions, orbital forcing from varying obliquity and precession, and millennial-scale shifts in the ocean circulation. Yet, the spatial fingerprint of these variations and their impact on local vegetation remain uncertain. Here, we present vegetation and climate reconstructions from a pollen record in Northeastern China covering the last 70kyr with unprecedented sub-centennial resolution. During the last Glacial, its position at the ecotone between cool mixed forest and steppe led to pronounced local vegetation changes, most likely driven by varying moisture availability. The vegetation changes occur synchronously with oxygen isotope variations in Chinese speleothems. However, the timescale-dependent contributions to the total variability differ between our precipitation reconstruction and the isotope record. A regional analysis of high-resolution proxy records covering the last Glacial supports comparatively stronger contributions from orbital-scale variability along the northern monsoon edge and from millennial-scale variability in India and Southern China. This suggests that orbital forcing and Atlantic Meridional Overturning Circulation (AMOC) variations possess distinct spatial fingerprints. Climate simulations indicate that the differences are driven by stronger North Pacific sea surface temperature changes in response to orbital forcing compared to AMOC shifts. The detected spatial heterogeneity of past monsoon variations can provide valuable insights into potential regional impacts of future monsoon changes.

How to cite: Weitzel, N., Stebich, M., Adam, M., Mingram, J., and Rehfeld, K.: Timescale-dependent fingerprint of the Asian Summer Monsoon during the last Glacial and its impact on vegetation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13961, https://doi.org/10.5194/egusphere-egu25-13961, 2025.

EGU25-14693 | ECS | Posters on site | AS1.24

Leading mode and physical dynamics of spring-to-summer rainfall evolution in eastern China 

Ruoyu Ma, Yue Zhang, and Chao He

Eastern China experiences substantial precipitation variability, primarily driven by the East Asian monsoon system, which is characterized by the stepwise northward progression of rainfall belt. The movement of the rainfall belt has significant socio-economic implications, necessitating precise forecasting to mitigate the risks associated with extreme weather events. This study employs Seasonal Empirical Orthogonal Function (S-EOF) analysis to examine precipitation variations, focusing on the transition of rainfall belt from spring (April-May) to summer (June-July). The results reveal that the northward shift of rainfall belt during the spring-to-summer period is strongly linked to variations in the East Asian Summer Monsoon activity. The leading mode exhibits a center of maximum rainfall in South China (SC) during spring, shifting to the middle and lower reaches of the Yangtze River basin (MLYZB) in summer, which emphasizes the spatial progression of rainfall patterns between these regions. In positive phase years, enhanced precipitation in SC during spring is related to increased moisture transported by an anomalous anticyclonic circulation over the western North Pacific (WNP). Subsequently, during summer, the enhanced rainfall moves to MLYZB along with the northward migration of the anomalous anticyclone in WNP. During negative phase years, precipitation markedly reducing in the two regions, mainly due to an anomalous cyclonic circulation over the WNP obstructs the influx of moisture from the Pacific. In summer, a cyclonic circulation over the South China Sea redirects moisture from the Indian Ocean to SC, resulting in reduced precipitation in the MLYZB. These large-scale atmospheric circulation patterns also indicate that the dominant transition of rainfall from spring to summer in eastern China can be associated with the monsoonal dynamics in the Bay of Bengal during spring. In particular, anomalous Bay of Bengal Summer Monsoon (BOBSM) activity triggers atmospheric convective heating and amplifies soil moisture anomalies in the Indochina Peninsula, thereby influencing and modulating rainfall patterns over eastern China. To further elucidate the mechanisms underlying this influence, numerical experiments are conducted to investigate the detailed processes through which BOBSM impacts the seasonal transition of rainfall in eastern China. In conclusion, this study can offer significant theoretical insights that enhance precipitation forecasting and inform extreme weather analysis.

How to cite: Ma, R., Zhang, Y., and He, C.: Leading mode and physical dynamics of spring-to-summer rainfall evolution in eastern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14693, https://doi.org/10.5194/egusphere-egu25-14693, 2025.

EGU25-17038 | ECS | Orals | AS1.24

The role of convection-circulation coupling in expediting South Asian monsoon onset: Insights from SP-CAM 

Yung-Jen Chen, Yen-Ting Hwang, Wei-Ting Chen, Chien‐Ming Wu, and Ding‐Rong Wu

This study emphasizes the role of shallow circulation in transporting lower-level moist static energy northward, thereby intensifying the onset of summer cross-equatorial circulation in the South Asia monsoon region. Previous research has suggested that the monsoon onset can be considered as a transition between an eddy-driven regime and an angular-conserving regime, and momentum budget analyses from these studies support the theory of regime transition (Bordoni and Schneider 2008; Plumb 2005; Geen et al. 2018; Shaw 2014). Additionally, studies have highlighted the significant role of boundary layer entropy during the summer monsoon period (Emanuel 1995; Plumb 2005; Nie et al. 2014), when the circulation operates within the angular-momentum-conserving regime. Adopting this boundary-layer-entropy-centric perspective, many studies emphasizing the role of topography in blocking low entropy inflow from the north and intensifying the South Asian Monsoon (Boos and Kuang 2010; Privé and Plumb 2007; Geen et al. 2014). Meanwhile, the role of synoptic systems and the early onset in the Bay of Bengal (Parker et al. 2016), as highlighted in observational data, in establishing the strong cross-equatorial summer cell remains unclear.

To bridge the gaps between observational studies and theoretical frameworks, this study investigates the mechanisms shaping the evolution of the boundary layer entropy throughout the regime transition. With the goal of understanding the interactions between convective processes and large-scale circulation, we utilize the Superparameterized Community Atmosphere Model (SPCAM), which demonstrates higher convection variability and increased precipitation near the South Asian coastal region compared to traditional global climate models, aligning well with observational data. Compared to simulations without SPCAM coupling, the SPCAM simulations show a more abrupt monsoon onset in South Asia. The sector zonal mean analysis demonstrates that the higher convection variability in SPCAM runs results in more shallow convections before the monsoon onset. Also, the shallow circulation accompanied with these shallow convections can transport higher lower-level entropy northward, causing energy convergence near the coastal region and intensifying the abruptness of the monsoon onset. In contrast, simulations without SPCAM coupling exhibit an unrealistic jump of boundary layer entropy maximum from the equator to the mountainous terrain. Our energy budget analysis highlights that the shallow overturning cell associated with the deep and shallow convections in the coastal regions holds the key for the northward migration of boundary layer entropy maximum. Such a relaxed quasi-equilibrium perspective provides an interpretation for how convection-circulation coupling contributes to the theoretical framework of regime transition.

How to cite: Chen, Y.-J., Hwang, Y.-T., Chen, W.-T., Wu, C., and Wu, D.: The role of convection-circulation coupling in expediting South Asian monsoon onset: Insights from SP-CAM, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17038, https://doi.org/10.5194/egusphere-egu25-17038, 2025.

EGU25-17380 | ECS | Posters on site | AS1.24

Neogene paleoclimatic evolution in Northwestern Luzon, Philippines: Insights from Lower Miocene to Lower Pliocene sedimentary records 

Kenneth Jan Sangalang, Mark Joshua Novero, Jillian Aira Gabo-Ratio, Betchaida Payot, Carla Dimalanta, Mariz Alcancia, Karl Jabagat, and Yuan-Hsi Lee

Geochemical analyses of Neogene clastic sediments overlying the Zambales Ophiolite Complex (ZOC) in northwestern Luzon, Philippines provide insights into paleoweathering and paleoclimatic conditions. This study examines the Early Miocene Cabaluan Formation and Late Miocene to Early Pliocene Santa Cruz Formation using weathering proxies, such as the Chemical Index of Alteration (CIA), Revised Chemical Index of Alteration (CIX), Chemical Index of Weathering (CIW), and dual-elemental ratios (e.g., Al/Ti, Sc/Ti, Na/Al). Elevated CIA, CIX, and CIW values in the Cabaluan Formation indicating intense weathering suggests warm and wet conditions during the Early Miocene. Conversely, lower values and reduced Al/Ti and Sc/Ti ratios in the Santa Cruz Formation reflect a shift to cool and dry conditions at the onset of the Late Miocene period. 

These findings align with regional patterns derived from similar geochemical proxies and δ18-O values in the northern South China Sea and global climatic cooling trends during the Neogene. They also highlight the influence of the East Asian Summer Monsoon (EASM) on the prevailing local weathering regime, supported by mobility indices (αᴬˡE) showing distinct elemental depletions and enrichments linked to climatic variations.

This study contributes to the scarce but growing paleoclimate studies in the Philippines using geochemical signatures in the sedimentary record. It provides a pioneering view into the Neogene paleoclimatic shift from a warm to cool climate in northwestern Luzon, Philippines, underscoring the influence of the EASM in the local and regional climatic evolution since the Early Miocene.

How to cite: Sangalang, K. J., Novero, M. J., Gabo-Ratio, J. A., Payot, B., Dimalanta, C., Alcancia, M., Jabagat, K., and Lee, Y.-H.: Neogene paleoclimatic evolution in Northwestern Luzon, Philippines: Insights from Lower Miocene to Lower Pliocene sedimentary records, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17380, https://doi.org/10.5194/egusphere-egu25-17380, 2025.

EGU25-18478 | ECS | Orals | AS1.24

Precipitation extremes during Madden Julian Oscillation over India 

Akanksha Sharma, Pyarimohan Maharana, and Ashok Priyadarshan Dimri

The Madden-Julian oscillation (MJO) is the predominant ocean-atmospheric phenomenon that influences the intraseasonal variabilities in the tropical atmosphere and is associated with weather extremes across the globe. This study aims to investigate the influence of MJO on extreme precipitation during Indian summer monsoon over India using ERA5 reanalysis data from 1974 to 2022. The MJO phases are calculated following Wheeler & Hendon, (2004) methodology which utilizes variables outgoing longwave radiation (OLR), zonal wind at 200hPa and 850hPa in the near-equatorial region between 15°S and 15°N. 99th percentile is used as a threshold to identify extreme precipitation. The study employs the Theil Sen slope trend test and Pettitt test for change point detection to study extremes. Further the OLR, vertically integrated moisture divergence (VIMD), and zonal wind at 850hPa are examined to study the change in dynamics. The preliminary results suggest that active phases 3 and 4 shows positive trend of extreme precipitation over southern northwest, west central and Peninsular India while active phase 2 and inactive phases 6 and 7 shows overall positive trend except for northeast India. Apart from extreme precipitation, frequency of extremes has also increased in phases 1, 2, 4, and 5. The change point analysis indicates these changes are observed after 1997. The percentage change of VIMD after change point show increased moisture availability in inactive phases which is evidently due to enhanced convective activity in recent times as also suggested by OLR. Overall, the study contributes in understanding the pattern of extremes over Indian landmass which will helps in predicting and mitigating the effect of severe weather.

How to cite: Sharma, A., Maharana, P., and Dimri, A. P.: Precipitation extremes during Madden Julian Oscillation over India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18478, https://doi.org/10.5194/egusphere-egu25-18478, 2025.

EGU25-18490 | Orals | AS1.24

How can we narrow down the uncertainty in Afro-Asian monsoon projection? 

Tianjun Zhou and Ziming chen

The Afro-Asian summer monsoon (AfroASM) sustains billions of people living in many developing countries covering West Africa and Asia, vulnerable to climate change. Future increase in AfroASM precipitation has been projected by current state-of-the-art climate models, but large inter-model spread exists. Here we show that the projection spread is related to present-day interhemispheric thermal contrast (ITC). Based on 30 models from the Coupled Model Intercomparison Project Phase 6 (CMIP6), we find models with a larger ITC trend during 1981-2014 tend to project a greater precipitation increase. Since most models overestimate present-day ITC trends, emergent constraint indicates precipitation increase in constrained projection is reduced to 70% of the raw projection, with the largest reduction in West African (49%). The land area experiencing significant increases of precipitation is 57% of the raw projection. Given that the emergent constraint improves the reliability in AfroASM precipitation projections, we further investigate the impacts of the constrained projection on the potential water availability. The fractions of land area that will experience a significant increase of potential water availability are about 66% of the raw projection. We find that global surface air temperature warming plays a dominant role in the emergent constraint on precipitation changes, while the contribution from hydrological sensitivity should not be neglected. The smaller increase of potential water availability in the constrained projection than the raw projection may pose a challenge to climate change adaptation and mitigation activities related to water management and food security, although a smaller than expected increase in rainfall will also reduce the risk of extreme precipitation and flooding.

How to cite: Zhou, T. and chen, Z.: How can we narrow down the uncertainty in Afro-Asian monsoon projection?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18490, https://doi.org/10.5194/egusphere-egu25-18490, 2025.

EGU25-20535 | Orals | AS1.24

Role of large and local scale drivers in the recent rise in heavy precipitating events over western India 

Ayantika Deychoudhury, Sumit Kumar Mukherjee, Krishnan Raghavan, and Dipanjan Dey

Over the recent decades, the South Asian monsoonal environment has evolved, leading to a rise in heavy precipitation events over the Indian subcontinent. These events have increased in frequency and intensity, particularly over Western India since the 1980s. The present study employs Self-Organizing Map (SOM) clustering to examine atmospheric patterns associated with heavy rainfall over Western India, identifying two key clusters, which have shown a significant rise in occurrence since the 1970s. The first cluster is marked by a large-scale mid-level vortex stretching from the Bay of Bengal to the Arabian Sea, driven by strong easterly anomalies and low-pressure systems (LPS) along central India. In contrast, the other cluster is manifested as a localized system centred over Western India, with low geopotential heights and LPS activity, supported by moisture from the Arabian Sea and regional land evaporation. The development of the first pattern is linked to remote influences such as Indian Ocean Dipole (IOD) events, while local soil moisture conditions influence the second pattern. This study underscores the complex interactions between large-scale dynamics, land-atmosphere coupling, and extreme weather patterns, highlighting the need for enhanced understanding of multis-scale interactions and increased observational networks to improve predictions and management of hydrological extremes in Western India.

How to cite: Deychoudhury, A., Kumar Mukherjee, S., Raghavan, K., and Dey, D.: Role of large and local scale drivers in the recent rise in heavy precipitating events over western India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20535, https://doi.org/10.5194/egusphere-egu25-20535, 2025.

Understanding the dynamics of precipitation in the western Himalayas (WH) during the Indian Summer Monsoon (ISM) is vital for societal well-being and effective disaster management. The region's complex terrain, diverse meteorological conditions, and observational uncertainties pose significant challenges in comprehending precipitation disparities and predicting extreme precipitation events (EPEs) across the WH. The present study provides a comprehensive investigation into the characteristics, drivers, and variability of summer monsoon precipitation, with a focus on EPEs and their underlying mechanisms in the WH. The findings reveal that EPEs, over the WH, defined as precipitation exceeding the 99th percentile, are influenced by both large-scale (61%) and convective precipitation (39%). Monsoon depressions contribute to 25.49% of these events. Atmospheric patterns such as upper-tropospheric gyres, zonal waves, and omega-type blocking emerge as key precursors, facilitating the southward extension of moisture-laden winds and enhancing low-level moisture convergence. The tropical-extratropical interactions, including the shifting of the Intertropical Convergence Zone and baroclinic wave activity characterized by zonal wave numbers 5 and 8, play a crucial role in intensifying EPE. Furthermore, High-resolution simulation using WRF demonstrate improved representation of spatiotemporal precipitation patterns, interannual variability, and EPEs compared to observational datasets. Overall, this study provides valuable scientific insights into the complex interactions governing precipitation extremes in the Himalayas. The findings enhance the understanding of ISM precipitation variability and improve the ability to predict and mitigate the impacts of extreme events in the region.

Keywords: Western Himalayas, Indian Summer Monsoon, Extreme Precipitation Events, Physical Drivers

How to cite: Saini, R. and Attada, R.: Deciphering Characteristics, Variability, and Drivers of Summer Monsoon Precipitation and Extremes over the Western Himalayas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20634, https://doi.org/10.5194/egusphere-egu25-20634, 2025.

EGU25-217 | ECS | Posters on site | AS1.26

The Role of Tropical Synoptic-Scale Disturbances in Modulating the Strength of East Pacific Hadley Circulation 

Pratiksha Priyam Baruah, Neena Joseph Mani, and Suhas Ettammal

The east Pacific, dominated by synoptic scale convective activity, presents a unique environment to explore the question of how synoptic scale disturbances can modulate the strength of mean meridional circulation. The role of mixed Rossby-Gravity (MRG) waves in modulating the east Pacific Hadley circulation (EPHC) strength is explored during boreal summer season using ERA5 reanalysis data. Composite analysis of MRG activity for five strong and five weak EPHC seasons identified based on a mass stream function based metric reveal that strong EPHC seasons are associated with pronounced MRG activity while the MRG activity is weak during weak EPHC seasons. While the SST background state over east Pacific is not favourable for thermally driven deep convection, low-level convergence induced by synoptic scale disturbances like the MRG waves can trigger deep convection over the region, and in turn influence the EPHC strength. The question of whether boundary forced convergence can have an impact on the EPHC strength is further investigated using an atmospheric mixed layer model. Surface convergence driven by meridional SST gradients are not found to be significantly different during strong and weak EPHC seasons, implying the dominant role of MRG in modulating the strength of EPHC. The study also reveals a new possible mechanism via which the El Niño Southern Oscillation (ENSO) modulates the strength of EPHC –ENSO induced changes in the mean background state modulates the spatio-temporal characteristics of MRG waves which in turn affect the low-level convergence over the region and impacts the strength of EPHC.

How to cite: Baruah, P. P., Mani, N. J., and Ettammal, S.: The Role of Tropical Synoptic-Scale Disturbances in Modulating the Strength of East Pacific Hadley Circulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-217, https://doi.org/10.5194/egusphere-egu25-217, 2025.

Recent studies have identified the Asian–Bering–North American (ABNA) teleconnection as a distinct atmospheric pattern influencing winter climates in Eurasia and North America, independent of the well-known Pacific–North America (PNA) pattern. However, the origins of the winter ABNA remain unclear. This study explores the interannual variability of the winter ABNA during 1979–2022 and examines its associated preceding surface boundary forcings. The ABNA pattern accounts for coherent surface air temperature variations across northern Asia, eastern Siberia–Alaska, and eastern North America, even after removing the influences of the PNA, the Arctic Oscillation, the North Atlantic Oscillation, and the North Pacific Oscillation. Surface boundary conditions linked to the ABNA can be traced back to a Eurasian Snow Cover Dipole Pattern (ESCDP) and a Maritime Continent Sea Surface Temperature (MCSST) anomaly in November. The ESCDP leads to a displacement of the Arctic stratospheric polar vortex via troposphere–stratosphere coupling. This anomalous polar vortex subsequently propagates downward during the following winter, generating the tropospheric ABNA pattern. The MCSST induces a diabatic heating anomaly, which is associated with a Tropical Western Pacific Precipitation (TWPP) anomaly in winter. The TWPP excites a poleward-propagating Rossby wave train across the North Pacific, directly amplifying the winter ABNA. These physical processes are well reproduced by a linear baroclinic model (LBM). Leveraging the ESCDP and MCSST as predictors, an empirical model is developed, demonstrating promising prediction skills for winter ABNA during the hindcast period. This approach provides a valuable strategy for improving seasonal prediction of winter climates in the Northern Hemisphere extratropics.

How to cite: Zhong, W. and Wu, Z.: Interannual variability of winter Asian–Bering–North American teleconnection linked to Eurasian snow cover and Maritime Continent SST, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1887, https://doi.org/10.5194/egusphere-egu25-1887, 2025.

EGU25-2418 | ECS | Posters on site | AS1.26

Anthropogenic Climate Change-driven Atmospheric Angular Momentum Increases Length of Day 

Susmit Subhransu Satpathy, Christian L.E. Franzke, Naiming Yuan, Nicola Maher, Wonsun Park, and Sun-Seon Lee

Increasing atmospheric angular momentum can alter the fundamental circulation cells that drive the Earth’s climate system and also slow the Earth’s rotation. Prominent examples include the expansion of the Hadley Cell and increasing Length of Day (LOD). Utilising the hundred ensemble member simulations of CESM2-LE with the SSP3-7.0 scenario, we reveal an equatorial super-rotation state of the earth with increased greenhouse gas emissions. With global warming, the momentum exchange between the solid earth and the atmosphere diminishes with reduced surface torques, suggesting slowing of the earth’s rotation. An accelerating atmosphere decelerates the earth’s rotational speed, bringing about challenges to precise time-keeping through increasing LOD. Our results demonstrate that climate-driven LOD changes due to atmospheric angular momentum variations can start as early as 2050, posing problems to global timekeeping. These findings illustrate that with continued warming along with astronomical tidal forcings and postglacial rebound processes, anthropogenic climate change will influence the earth’s rotational rate. 

How to cite: Satpathy, S. S., Franzke, C. L. E., Yuan, N., Maher, N., Park, W., and Lee, S.-S.: Anthropogenic Climate Change-driven Atmospheric Angular Momentum Increases Length of Day, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2418, https://doi.org/10.5194/egusphere-egu25-2418, 2025.

EGU25-3716 | ECS | Orals | AS1.26

Climate change induced by equatorial superrotation 

Tim Marino, Michael P. Byrne, and Corentin Herbert

Understanding the potential reorganizations of the large-scale atmospheric circulation in the tropics is important in the context of anthropogenic climate change and from a theoretical point of view, but also because they might be connected with warm climates of the past. A particularly spectacular, albeit hypothetical, example of such a reorganization is the case of equatorial superrotation, characterized by strong westerly winds at the equator. While potential dynamical processes underlying a transition to equatorial superrotation have been studied to some extent, the question of how the circulation changes would be coupled to the broader climate features has not yet been addressed. In this work, we adopt this perspective and investigate the consequences of such a circulation change on Earth's surface climate and hydrological cycle.

Using general circulation model (GCM) simulations in an aquaplanet setup with an imposed equatorial torque to force superrotation in the atmosphere, we observe large changes in the surface temperature and precipitation distribution. The results show an important global surface warming, comparable to a doubling of the CO2 concentration, which affects in particular regions outside of the tropics, such as the mid-latitudes. In addition, the meridional structure of the precipitation profile becomes flatter; the tropics become drier and the subtropics wetter. These changes are strongly linked to the effect of the circulation changes on the meridional transport of energy and moisture. We analyze these changes and the associated radiative budget changes using a forcing/feedback framework.

Overall, this study demonstrates that equatorial superrotation can have a significant impact on the surface climate, independently of any external radiative forcing. This provides further evidence that such major changes in the large scale circulation might be relevant for warm climates of the Earth, in the past or in the future.

How to cite: Marino, T., Byrne, M. P., and Herbert, C.: Climate change induced by equatorial superrotation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3716, https://doi.org/10.5194/egusphere-egu25-3716, 2025.

EGU25-4119 | ECS | Posters on site | AS1.26

Multi-method quantification of the contribution of circulation changes to summer temperature trends in the northern hemispheric mid-latitudes 

Peter Pfleiderer, Anna Merrifield, István Dunkl, and Sebastian Sippel

Observed summer temperature trends differ strongly around the northern hemispheric latitudes. Besides changes in aerosol emissions, changes in atmospheric circulation patterns - whether forced or not - are expected to contribute to considerable variation in summer temperature trends. Different statistical and machine learning methods have been developed and applied to quantify this contribution of circulation changes to summer temperatures. Here we test the accuracy of multiple methods by applying them to historical climate simulations and comparing the circulation contribution obtained by different methods to trends found in nudged circulation simulations with wind fields of the historical simulations but pre-industrial control forcing. After validating the methods we apply them to ERA5 and over the entire northern hemispheric mid-latitudes (over land). Our results consistently suggest that especially over Europe circulation changes have contributed to an increase in summer temperatures. In parts of central Asia and eastern North America, circulation changes have contributed to a cooling in summer temperatures.

While providing a systematic overview of circulation contributions to local temperature trends in the northern hemispheric mid-latitudes we also show how nudging experiments can help to validate and consolidate methods. We argue that such method evaluation studies become increasingly important with the ongoing expansion of applications of statistical and machine learning analyses on the observational record.

How to cite: Pfleiderer, P., Merrifield, A., Dunkl, I., and Sippel, S.: Multi-method quantification of the contribution of circulation changes to summer temperature trends in the northern hemispheric mid-latitudes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4119, https://doi.org/10.5194/egusphere-egu25-4119, 2025.

EGU25-4211 | Orals | AS1.26

Diagnosing and analysing Rossby wave resonance along a circumglobal jetstream 

Volkmar Wirth and Nili Harnik

A method is presented which allows one to diagnose and to analyze Rossby wave resonance along a circum-global midlatitude jet in the framework of the inviscid linear barotropic model with beta-plane geometry. Zonally symmetric Gaussian-shaped jets of varying amplitude and width are specified as a basic state. The system is forced by a pseudo-orography which varies sinusoidally in the zonal direction, and which has a very small meridional extent. Solutions are obtained through straightforward numerical methods. The strength of resonance is diagnosed by systematically varying the zonal wavenumber s, plotting the resulting wave amplitude as a function of s and quantifying the sharpness of the peak (if existent). The numerical solutions for jet-like basic states are interpreted by reference to analytical solutions obtained for more idealized model configurations

 

It is shown that a jet with realistic amplitude and width may be subject to a weak form of resonance provided that the jet is truly circum-global and there are no other forms of damping. Given that the zonal scale of a jet is much larger than its meridional scale, one may expect resonance at no more than one zonal wavenumber s_res. This resonant peak is associated with the gravest meridional mode, which is established through partial reflection of wave activity at the periphery of the jet flanks. These results are reproduced well in the classic Charney-Eliassen model with an appropriate choice for the channel width. A spherical version of our diagnostic tool is expected to provide a reliable method to detect the potential for resonant amplification of Rossby waves in observed episodes

How to cite: Wirth, V. and Harnik, N.: Diagnosing and analysing Rossby wave resonance along a circumglobal jetstream, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4211, https://doi.org/10.5194/egusphere-egu25-4211, 2025.

EGU25-5070 | ECS | Posters on site | AS1.26

Inter-model spread of AMO-related tropical precipitation in CMIP6 

Qi Su and Riyu Lu

As a prominent large-scale mode in the Northern Hemisphere, the Atlantic Multidecadal Oscillation (AMO) can have a profound impact on regional and global climate. This study investigates inter-model spread of AMO-related tropical precipitation anomalies by using 52 models in the historical simulation from Coupled Model Intercomparison Project phase 6 (CMIP6). The results indicate that there is a significant spread in AMO-related precipitation anomalies among models in the tropics, particularly in the Maritime Continent–tropical western Pacific. In addition, the inter-model spread is characterized by a seesaw pattern between the Maritime Continent and tropical western Pacific, identified as the primary mode through inter-model EOF analysis. Furthermore, associated with the differences in AMO-related tropical precipitation anomalies, there are substantial differences in sea surface temperature anomalies in the tropics and surface air temperature anomalies in the Eurasian continent.

How to cite: Su, Q. and Lu, R.: Inter-model spread of AMO-related tropical precipitation in CMIP6, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5070, https://doi.org/10.5194/egusphere-egu25-5070, 2025.

Tropical and subtropical precipitation impact millions of people via agriculture and rainfall-driven disasters, driving interest in their potential future change. CMIP6 simulations broadly predict an increase in global monsoon precipitation. However, regional projections from individual models vary in magnitude and sign, and projected changes by the end of the century are often small compared with model biases. This motivates an interest in understanding model biases, and how to interpret the future shifts in rainfall.

The Hadley and Walker circulations transport Moist Static Energy in the direction of their upper branches, so that the change in sign of MSE transport acts as a proxy for mass convergence in the tropical rainband. MSE transport can then be interpreted in terms of top-of-atmosphere and surface energy fluxes using the column energy budget.

Recent work attributes contributions to annual- and zonal-mean divergent MSE transport to radiative fluxes, evaporative fluxes and sensible heat, and suggests that evaporative fluxes are key in setting the spatial structure of MSE transport. Here we extend this approach to regional and seasonal scales, and explore inter-model differences in CMIP6 historical simulations, and projected changes under SSP585.

MSE transport attributed to evaporative and radiative fluxes dominate the regional JJA & DJF transport. Empirical Orthogonal Functions (EOFs) are used to express historical intermodel differences in MSE transport in a 2-dimensional space of leading EOFs linked to land-sea thermal contrast and interhemispheric thermal contrast. Changes in MSE transport components under SSP585 are then projected into this space and decomposed into terms attributed to the top of atmosphere and surface fluxes. This reveals energetic signatures of model bias and future change, that illustrate how different processes contribute to the overall differences in energy transport.

Shared energetic signatures of bias are predominantly seen within model families. In contrast, shared signatures of future change emerge across (and differ within) model families, with a shared bias signature not implying a shared change signature. This suggests a set coherent but differing pathways through which climate change affects the energy budget and associated tropical rainfall in particular groups of models.

How to cite: Geen, R.: Energetic signatures of tropical rainband biases & shifts in CMIP6, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7062, https://doi.org/10.5194/egusphere-egu25-7062, 2025.

EGU25-7090 | Posters on site | AS1.26

Historical trends in windspeed over the Northern Hemisphere in observations and reanalyses  

Paul-Arthur Monerie, Reinhard Schiemann, Jon Robson, and David Brayshaw

We analyse trends in annual mean wind speed from 1980 to 2010. Observational data (HadISD3) indicate a decline in wind speed across North America, Europe, and central and eastern Asia, a phenomenon referred to as global wind speed stilling. However, a suite of reanalyses fails to accurately reproduce this trend, often showing inconsistencies in the direction of the trend. Additionally, the reanalyses significantly underestimate wind speed variability. We further investigate the sources of discrepancies between the observations and reanalyses. Our findings suggest that the erroneous trends in the reanalyses primarily stem from inaccuracies in simulating high-frequency wind speed variability. In contrast, lower-frequency variability remains consistent between observations and reanalyses. These errors in simulating wind speed trends have significant implications for understanding and predicting wind power variability.

How to cite: Monerie, P.-A., Schiemann, R., Robson, J., and Brayshaw, D.: Historical trends in windspeed over the Northern Hemisphere in observations and reanalyses , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7090, https://doi.org/10.5194/egusphere-egu25-7090, 2025.

EGU25-7437 | ECS | Posters on site | AS1.26

Simulated Changes in Large-scale Atmospheric Circulation Energetics from Volcanic Aerosol Forcing 

Anatoly Poroshenko and Matthew Toohey

Understanding the response of large-scale atmospheric circulation to radiative forcing agents is important for climate prediction. The radiative forcing from volcanic stratospheric aerosol is one of the most important natural climate forcings, with impacts on surface temperature and atmospheric dynamics. In this study, we explore changes in the energetic properties of the Hadley and Ferrel systems under the influence of radiative forcing associated with large volcanic eruptions in multi-model simulations performed as part of the Model Intercomparison Project on the Climatic Response to Volcanic Forcing (VolMIP) within the Coupled Model Intercomparison Project Phase 6 (CMIP6). In the Earth’s atmosphere, the Hadley and Ferrel systems are examples of thermally direct (warm air rises and cold air sinks) and indirect (cold air rises and warm air sinks) circulations, respectively. Being the part of Lorenz cycle of energy transformation in the atmosphere, the direct circulation converts zonal-mean available potential energy into zonal-mean kinetic energy. The indirect circulation in the midlatitude, however, converts some of the zonal-mean kinetic energy back into zonal-mean available potential energy. Averaged over the 4 models that provided the required model output from the VolMIP Pinatubo simulations, the mean power associated with the Hadley system in preindustrial simulations is 235.6 TW. The mean decrease of the power in VolMIP simulations of the 1991 Pinatubo eruption is 7.58 TW (3.22%) for the first post-eruption northern-hemisphere (NH) winter and 6.59 TW (2.80%) for the second one. For the Ferrel system, the preindustrial mean DJF power is 326.10 TW, and post-volcanic anomalies are 16.3 TW (5.00%) and 18.3 TW (5.61%) in NH winters 1 and 2, showing a stronger anomaly in the second NH winter than the first one. In additional VolMIP experiments, we also explore the response of the Hadley and Ferrel cells to the relatively strong forcing associated with the 1815 Tambora eruption and find the Hadley system weakening by 15.3 TW (6.48%) and 11.5 TW (4.90%) for the first two NH winters. We explore how post-eruption changes in the meridional atmospheric circulation strength and the cells' location can be explained with simple theoretical models of atmospheric thermodynamics.

How to cite: Poroshenko, A. and Toohey, M.: Simulated Changes in Large-scale Atmospheric Circulation Energetics from Volcanic Aerosol Forcing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7437, https://doi.org/10.5194/egusphere-egu25-7437, 2025.

EGU25-7766 | ECS | Posters on site | AS1.26

Influence of baroclinic eddies on the Hadley cell edge  

Seungpyo Lee, Woosok Moon, Seok-Woo Son, and Kyong-Hwan Seo

The Hadley cell (HC) is a thermally direct circulation in the tropics that transports heat from the tropics to the mid-latitudes. HC is known as the primary cause of subtropical desert formation, and with the recent observation of poleward shift of both the HC and desert regions, extensive studies has been made to understand its formation. The most foundational theory on the HC was proposed by Held and Hou (1980). This theory pinpointed the importance of angular momentum conservation and energy flux balance, while providing approximations for the edge and intensity of the HC. However, it did not consider the influence of baroclinic eddies. By extending this theory, the present study incorporates eddy heat fluxes and changes of adiabatic processes induced by eddy momentum fluxes in the subtropical upper troposphere into the energy flux balance HC dynamics. It is proposed that HC contracts when losing heat and expands when gaining heat due to thermal interactions with baroclinic eddies. This finding is verified through a series of dynamical core model experiments with varying baroclinicity. 

How to cite: Lee, S., Moon, W., Son, S.-W., and Seo, K.-H.: Influence of baroclinic eddies on the Hadley cell edge , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7766, https://doi.org/10.5194/egusphere-egu25-7766, 2025.

EGU25-7843 | Posters on site | AS1.26

An idealized model for the spatial structure of the eddy-driven Ferrel cell in mid-latitudes 

Woosok Moon, Seoungpyo Lee, Elian Vanderborght, Georgy Manucharyan, and Henk Dijkstra

Conceptual models of the midlatitude atmospheric circulation have added greatly to understanding its behavior. Here,  we present a new conceptual model for the spatial structure of the Ferrel cell. The poleward heat flux resulting from the baroclinic growth of eddies leads to a decrease in the meridional temperature gradient, which is parameterized through a down-gradient eddy diffusion coefficient D. Similarly, the eddy momentum flux, influenced by barotropic wave breaking, is assumed to be proportional to a factor M>0 to the horizontal shear of the zonal mean zonal wind, 
thereby enhancing the intensity of the zonal mean zonal wind at upper levels. By incorporating the parameterization of turbulent eddies into the zonal-mean quasi-geostrophic potential vorticity equation, a balance is achieved, resulting in eddy-driven circulations in mid-latitudes akin to the Ferrel cell. 
The meridional structure of the temperature exhibits two primary features. The first feature is a linear decline in anomalous potential temperature, 
inducing westerly winds in mid-latitudes. The second feature corresponds to jet streams generated by eddy momentum fluxes. Along with the jet streams, the eddy driven circulations exhibit the downward (upward) motion at the southern (northern) flank of the jets. The meridional structure of the circulation is influenced by three key factors. The first factor is a structural number denoted as D/SM, where S is the dry static stability affecting the life cycle of synoptic eddies in mid-latitudes. The second factor relates to the planetary size and the third factor is the vertical structure of the atmosphere, associated with eigenvalues of the vertical mode in the heat equation. The combination of these three factors within the characteristic equation also
determines the location and number of eddy-driven jets in mid-latitudes.

How to cite: Moon, W., Lee, S., Vanderborght, E., Manucharyan, G., and Dijkstra, H.: An idealized model for the spatial structure of the eddy-driven Ferrel cell in mid-latitudes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7843, https://doi.org/10.5194/egusphere-egu25-7843, 2025.

EGU25-10184 | ECS | Posters on site | AS1.26

The joint effects of Interhemispheric Oscillation and Arctic Oscillation on climate anomlies in winter 

Nian Qiao, Chuhan Lu, Zhaoyong Guan, Yang Hu, and Lei Zhong

The winter temperature anomalies are influenced by the joint effects of multiple factors. Using NCEP/NCAR reanalysis data from 1979 to 2022,this paper analyzes the circulation patterns and mechanisms influencing temperature anomalies in the mid-to-high latitudes of the Northern Hemisphere under the joint effects of Interhemispheric Oscillation (IHO) and Arctic Oscillation (AO). It was found that the temperature changes under the joint effects of IHO and AO were mainly influenced by AO, with IHO playing a disruptive role. Specifically, when IHO and AO were in the same phase, the disturbance in the polar region would weaken due to the cancellation of different signals, while the disturbance in the mid latitudes would strengthen due to the superposition of the same signals. There is a significant meridional horizontal propagation of Rossby wave energy in the North Pacific and North Atlantic. Stratospheric planetary waves mainly propagate downward over the Eurasian continent, while areas north of 60 °N in North America exhibit oblique downward propagation of stratospheric planetary waves, and areas south of 60 °N exhibit significant southward propagation of planetary waves in the troposphere. When IHO and AO are in opposite phases, disturbances in the Arctic region are enhanced due to the superposition of the same sign, but disturbances in the mid latitude region are weakened due to the cancellation of opposite signs. There is obvious Rossby meridional propagation in the North Pacific and North Atlantic, with wave energy dispersed upwards at high latitudes and propagating towards low latitudes. In addition, the maximum contribution of IHO and AO to surface air temperature is mainly due to the disturbance of horizontal temperature advection caused by the steady wind field and diabatic heating. These conclusions provide reference for studying temperature anomalies and can better understand the mechanisms and impacts of atmospheric circulation anomalies.

How to cite: Qiao, N., Lu, C., Guan, Z., Hu, Y., and Zhong, L.: The joint effects of Interhemispheric Oscillation and Arctic Oscillation on climate anomlies in winter, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10184, https://doi.org/10.5194/egusphere-egu25-10184, 2025.

EGU25-10239 | ECS | Orals | AS1.26

Missing Increase in Summer Greenland Blocking in Climate Models 

Jacob Maddison, Jennifer Catto, Edward Hanna, Linh Luu, and James Screen

Atmospheric blocking events in summer over Greenland promote melting of the Greenland ice sheet, a major contributor to sea level rise. Recent observations indicate that, during the early part of the twenty-first century, summertime atmospheric blocking over Greenland has become markedly more frequent. This increasing trend in blocking activity appears to be missing in climate model simulations. The temporal evolution of Greenland blocking (GB) is assessed here in a larger ensemble of around 500 members from the CMIP6 archive. The observed increase in GB is also not present in the larger ensemble of members considered: the maximum 10-year trend in GB in the reanalysis lies almost outside the distributions of trends in the climate models and a period of such increased GB activity is rarely found in the full historical period of the model simulations.

The climate model simulations do however suggest that variability in GB is partly driven by sea surface temperatures (SSTs) and/or sea ice concentrations (SICs), as well as/or by anthropogenic aerosols, but the response of the models to these forcings may be too weak. To understand if it is forcing from the surface or from aerosols that dominates, a set of climate model experiments is performed with the Met Office climate model. Historical simulations are performed with prescribed SSTs/SICs and both with and without aerosol forcing. Results from the experiments indicate that variability in SSTs/SICs is key for capturing variability in GB. Further work is required to understand why climate models cannot represent a period of increased GB, how SST/SIC variability relates to that in GB, and what implications these have for future projections of Greenland climate change.

How to cite: Maddison, J., Catto, J., Hanna, E., Luu, L., and Screen, J.: Missing Increase in Summer Greenland Blocking in Climate Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10239, https://doi.org/10.5194/egusphere-egu25-10239, 2025.

EGU25-10561 | ECS | Posters on site | AS1.26

Exploring the Dynamics of Climatological Mean Monsoon Using a Machine Learning Based Empirical Leading Order Analysis 

Arijeet Dutta, Ruth Geen, and Maike Sonnewald

The global monsoon circulation, which governs the subtropical rainband, can be interpreted as a manifestation of the seasonal migration of tropical overturning circulation (Hadley cell). However, the dynamics of regional monsoons is additionally controlled by zonal asymmetries occurring from land sea distribution, zonal gradients in sea surface temperature, and other stationary wave forcings. Despite its importance, the dynamics of regional monsoons remain poorly understood. Here, we demonstrate, using a machine learning guided empirical leading order analysis, emergence of distinct dynamical regimes that describe the complex evolution of regional monsoons. Conservation of angular momentum plays an important role in our understanding of the climatological and zonal mean picture of monsoon. It suggests, during the solstitial seasons the dominant balance in the momentum budget comes from the mean meridional circulation and the advection of mean zonal wind by the divergent wind. However, for regional monsoons the resulting angular momentum budget now includes many terms arising from the drivers mentioned above. We deploy an unsupervised machine learning algorithm to find the dominant balances in the momentum budget. This enables us to find spatio-temporal clusters characterized by distinct balances in the momentum budget and to study how they evolve throughout the seasonal cycle. The inherent stochastic nature of the algorithm is leveraged to find the robustness of the identified clusters. Entropy is used to measure uncertainty for the clusters recognized by the algorithm. The algorithm is successfully applied to idealized simulations with varying complexities ranging from aquaplanet to different distributions of land-sea-topography. Consistent with zonal mean theory, resulting clusters capture the dominant tropical overturning. However, zonal asymmetries result in additional clusters with distinct dynamical regimes

How to cite: Dutta, A., Geen, R., and Sonnewald, M.: Exploring the Dynamics of Climatological Mean Monsoon Using a Machine Learning Based Empirical Leading Order Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10561, https://doi.org/10.5194/egusphere-egu25-10561, 2025.

EGU25-10703 | ECS | Posters on site | AS1.26

The effect of model biases on the simulated future changes of the North Atlantic jet stream 

Juho Koskentausta, Alexey Karpechko, Raphael Köhler, Xavier Levine, René Wijngaard, and Victoria Sinclair

Future projections of the European climate suffer from uncertainties in the changes of the North Atlantic jet stream. Previous studies of multi-model ensembles have suggested that the jet will shift poleward, and that the shift is anticorrelated with the simulated present-day latitude of the jet. Model basic state biases are a possible cause for the uncertainty, but their effect is difficult to assess because the spread in simulations may be caused by any inter-model differences. Here, we isolate the effect of model biases on future projections by modifying the basic state of a single atmospheric model with a run-time correction method aiming to adjust the model climatology towards those of three other models and a reanalysis. The effect of model biases was found to be strongly seasonal. In winter, changes in the frequencies of two of the three preferred positions of the jet were found to be sensitive to the model biases, but in summer the impact of biases is small relative to the magnitude of the changes. The results demonstrate that even though the anticorrelation of jet latitude and shift is only partly caused by biases, there is potential to reduce uncertainty in jet stream changes by improving model basic states.

How to cite: Koskentausta, J., Karpechko, A., Köhler, R., Levine, X., Wijngaard, R., and Sinclair, V.: The effect of model biases on the simulated future changes of the North Atlantic jet stream, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10703, https://doi.org/10.5194/egusphere-egu25-10703, 2025.

Understanding how greenhouse gases (GHGs) perturb the tropical Pacific warming pattern is crucial due to its impact on circulation and the hydrological cycle. A global CO2 increase is known to initially induce cooling in the tropical Pacific, particularly in the eastern basin, which gradually evolves into equatorially peaked warming amplified in the eastern basin. To disentangle the mechanisms driving the evolution of the CO2-induced equatorial Pacific warming pattern, we construct large-ensemble climate model experiments with CO2 increases confined to discretized latitudinal bands. On a fast timescale (years 1-3), Northern Hemisphere off-equatorial forcing (NH_OFFEQ) induces the basin-wide equatorial Pacific cooling due to intensified trade easterlies associated with a northward ITCZ shift. Local equatorial forcing (EQ) drives eastern equatorial Pacific cooling through enhanced climatological upwelling. In contrast, Southern Hemisphere off-equatorial forcing (SH_OFFEQ) leads to basin-wide equatorial Pacific warming, with an amplified response in the eastern basin due to the weakening of the southern subtropical ocean cell (STC). The effect of NH_OFFEQ and EQ forcing on equatorial Pacific SST changes diminishes over time due to dynamical ocean adjustments. Consequently, the fast strengthening of the zonal SST gradient induced by NH_OFFEQ and EQ forcing transitions into a weakening driven by SH_OFF forcing, which becomes dominant during the slow response. Our results suggest that the recent cooling in the eastern tropical Pacific could be part of the CO2-driven fast response.

How to cite: Kang, S. and Olonscheck, D.: Contrasting responses to hemispheric forcing govern the evolution of the CO2-induced equatorial Pacific warming pattern, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10898, https://doi.org/10.5194/egusphere-egu25-10898, 2025.

EGU25-15963 | ECS | Posters on site | AS1.26

Competing influences of energy budget variability and gross moist stability on tropical circulation variance under climate change 

Zhenghe Xuan, Clarissa Kroll, and Robert Jnglin Wills

It is generally thought that the climate responses of El Niño-Southern Oscillation (ENSO) variability and precipitation variability are tightly linked. The reasoning is that ENSO variability leads to sea-surface temperatures and surface heat flux variability, affecting the net-energy input (NEI) and thereby precipitation. We show that equally important are changes in the gross moist stability (GMS), which is the sensitivity of the atmospheric circulation to changes in the NEI. We analyze the variance of vertical velocity in monthly outputs of the Community Earth System Model 2 Large Ensemble. Under the SSP3-7.0 scenario, we find that variance of vertical velocity changes result from the competition of spatially varying responses of NEI variance and GMS. While NEI variance changes are complex and influenced by many mechanisms such as ENSO and radiative feedbacks, GMS increases in the sub-tropics can be explained by the rising tropopause and GMS decreases near the equator can be can be explained by the enhanced heating and moistening of the near-surface eastern equatorial Pacific. Together, these changes have important implications for future changes in precipitation variability in the tropics.

How to cite: Xuan, Z., Kroll, C., and Jnglin Wills, R.: Competing influences of energy budget variability and gross moist stability on tropical circulation variance under climate change, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15963, https://doi.org/10.5194/egusphere-egu25-15963, 2025.

EGU25-17675 | ECS | Orals | AS1.26

Altered NAO - North Atlantic SST Feedback in Mesoscale Resolving Simulations 

Joas Müller, Adam Herrington, and Robert C. Jnglin Wills

Recent studies using mesoscale resolving simulations have shown a stronger and spatially different large-scale atmospheric response to North Atlantic (NA) sea-surface temperature (SST) anomalies compared to more coarse-resolution simulations. An idealized setup proved that moving from a horizontal resolution of 110-km of more classic general circulation models to 28-km and further to 14-km leads to distinct large-scale responses to Gulf Stream SST anomalies. 

Here, we investigate a new set of simulations using a variable resolution version of the Community Atmospheric Model (CAM6) and more realistic specified SST anomalies. The horizontal resolution is regionally refined in the NA domain from the global 110-km resolution to 28-km, which is not fully mesoscale resolving, and further to 14-km, capable of resolving weather fronts which are crucial features for ocean-atmosphere coupling. 
The specified SST anomaly forcing the simulations is created by regressing the observational North Atlantic Oscillation (NAO) index onto SSTs over the period 1958–2018, resulting in a cold-warm-cold tripole anomaly and enabling a comparison of the NAO - NA SST feedback between the different resolutions. 

We find that the resulting NA SST tripole anomaly feeds back positively onto the NAO in the 14-km simulations. This positive NAO–SST–NAO feedback is not present in the 28-km and 110-km simulations which show a distinct spatial structure and generally a weaker response.
With the overall push towards more expensive higher-resolution coupled simulations, our results will provide valuable insights into the required atmospheric resolution needed to correctly represent ocean-atmosphere coupling.

How to cite: Müller, J., Herrington, A., and Jnglin Wills, R. C.: Altered NAO - North Atlantic SST Feedback in Mesoscale Resolving Simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17675, https://doi.org/10.5194/egusphere-egu25-17675, 2025.

EGU25-18003 | Posters on site | AS1.26

A Methodological Framework to Isolate Forced Dynamic Responses in Heat Extremes Using Nudged Climate Simulations 

Jitendra Singh, Sebastian Sippel, Lei Gu, Reto Knutti, and Erich Fischer

Regional trends in heat extremes are significantly influenced by large-scale atmospheric circulation changes across the Northern Hemisphere, with circulation-induced changes contributing up to one-third of the observed warming in regions like Western Europe. Understanding whether these trends are driven by external forcing or internal variability is key for improving model evaluation, trend detection, attribution, and reducing uncertainties in future climate projections. Here, we present a novel methodological framework to isolate the forced dynamic components of heat extremes. We nudge tropospheric winds in CESM2 pi-control simulations towards transient climate conditions, which provides an estimate of the forced thermodynamic component. By subtracting these thermodynamic contributions from the large ensemble mean, we effectively isolate the forced dynamic contributions to heat extremes. Our results reveal distinct regional patterns. Previously identified heatwave hotspots such as the Pacific Northwest, Central Europe, South Siberia, and North China/Mongolia exhibit substantial warming of up to 1°C since 1950, which is attributable to forced circulation changes. In contrast, forced circulation chnages induces cooling of up to 1°C in regions such as the northeastern United States, parts of Asia, and central Africa. We have rigorously tested the sensitivity of our approach through various experiments and nudging strategies. This framework provides a valuable tool for disentangling forced thermodynamic and dynamic signals from internal variability, offering critical insights to reduce uncertainties in future climate projections.

How to cite: Singh, J., Sippel, S., Gu, L., Knutti, R., and Fischer, E.: A Methodological Framework to Isolate Forced Dynamic Responses in Heat Extremes Using Nudged Climate Simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18003, https://doi.org/10.5194/egusphere-egu25-18003, 2025.

EGU25-18030 | Orals | AS1.26

Jet streams in a changing climate: evidence for large increases in shear and turbulence since 1979 

Paul Williams, Mark Prosser, and Isabel Smith

The jet streams are a crucial part of the global atmospheric circulation. Jet streams are highly sheared regions of the atmosphere, leading to Kelvin–Helmholtz instability and the generation of clear-air turbulence (CAT), which affects flying aircraft. Wind shear and CAT at flight cruising altitudes are projected to increase in response to future climate change, as the meridional temperature gradient across the jet streams strengthens, largely due to amplified warming at low latitudes associated with the tropical upper-tropospheric warming hotspot. However, our understanding of past trends in jet stream wind shear and CAT is currently limited. Here we analyse past trends in jet stream vertical wind shear in three different reanalysis datasets since 1979. We find that the shear at flight cruising altitudes has strengthened by 15%, and we show that this change is attributable to the thermal wind response to the enhanced upper-level meridional temperature gradient. We then analyse CAT trends globally during 1979–2020 in a reanalysis dataset using 21 diagnostics. We find clear evidence of large increases around the globe at aircraft cruising altitudes. For example, at an average point over the North Atlantic, the total annual duration of light-or-greater CAT increased by 17% from 466.5 hours in 1979 to 546.8 hours in 2020, with even larger relative changes for moderate-or greater CAT (increasing by 37% from 70.0 hours to 96.1 hours) and severe-or-greater CAT (increasing by 55% from 17.7 hours to 27.4 hours). Future projections using climate models indicate a 17-29% increase in vertical wind shear in the upper-level jet streams by 2100, as well as a possible tripling in the amount of severe CAT. We conclude that the jet streams are becoming more sheared because of climate change, generating more turbulence, with important implications for the future of air travel.

How to cite: Williams, P., Prosser, M., and Smith, I.: Jet streams in a changing climate: evidence for large increases in shear and turbulence since 1979, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18030, https://doi.org/10.5194/egusphere-egu25-18030, 2025.

The ascending branch of the Hadley circulation forms the band of heavy precipitation, the Intertropical Convergence Zone (ITCZ). Due to its sharp meridional gradient, even a small change in its structure can lead to drastic changes in local precipitation patterns, affecting large populations dependent on agriculture. Consequently, understanding its response to a warming climate has been a major focus of research over the past decades. Previous studies have identified a robust strengthening of the ascending branch of the Hadley cell, often referred to as a “deep tropics squeeze”, characterized by the narrowing of the ITCZ in response to increased CO2. However, much of the research has concentrated on the quasi-equilibrated response, with little attention given to its response on shorter timescales, which are more relevant for near-term climate projections.

To examine the evolution of the ITCZ response, we construct a 30-member ensemble of abrupt 4xCO2 simulations using the MPI-ESM. Our experiments reveal distinct phases in the Hadley cell response, starting with a weakening ascent and widening of the ITCZ in the initial years, followed by a reversal of these trends in subsequent decades. This reversal is primarily driven by a shift in the spatial pattern of sea surface temperature (SST) warming, transitioning from cooling to warming over the eastern equatorial Pacific due to dynamical ocean adjustments. Our findings underscore the value of large-ensemble 4xCO2 experiments, which allowed us to identify the shifting dynamics of the ITCZ, with the fast response distinct from the well-established slow response. 

How to cite: Zhang, J. and Kang, S.: Shifting dynamics of the ITCZ: from widening to narrowing in response to abrupt 4xCO2, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18271, https://doi.org/10.5194/egusphere-egu25-18271, 2025.

EGU25-18509 | ECS | Orals | AS1.26

Anti-correlated Hadley and Walker circulations through cloud radiative feedback 

Rolf Schimmer and Sarah Kang

The Pacific Ocean plays a pivotal role in driving Earth’s climate, as it is the primary region for strong deep convection that forms the ascending branch of the zonally symmetric Hadley circulation (HC) and the zonally asymmetric Walker circulation (WC). The HC is characterized by ascending motion in the equatorial region and descending motion in the subtropics, governed by energy and angular momentum conservation. In contrast, the WC features strong ascent over the western Pacific and descent over the central to eastern equatorial Pacific, driven by the zonal sea surface temperature (SST) gradient. Although the HC and WC share an ascending branch, their coupling remains poorly understood from a theoretical perspective. To investigate their coupling, we use an idealized aquaplanet slab ocean model. By prescribing zonally asymmetric warm and cold surface fluxes in the tropics, we deliberately alter the strength of the WC. The results show an anticorrelated relationship between the two circulations, with the HC weakening in proportion to the WC strengthening. This behaviour is attributed to the dominant cloud radiative effect in the cold patch region compared to the warm patch. These findings are further supported by cloud-locked experiments that isolate the contributions of cloud radiative feedback. While the shared ascending branch in the western Pacific is often considered the determining factor governing the dynamics, our idealized experiments suggest that the interplay between the two circulations may instead be driven by cloud radiative feedback in the eastern Pacific. The results therefore highlight the critical role of the cold tongue region in shaping the pattern effect in the tropical Pacific.

How to cite: Schimmer, R. and Kang, S.: Anti-correlated Hadley and Walker circulations through cloud radiative feedback, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18509, https://doi.org/10.5194/egusphere-egu25-18509, 2025.

Observations reveal an increasing frequency and intensity of climate extremes during summer under global warming. Pronounced warming in the tropical upper troposphere and Arctic amplification play as key contributors to these changes. Such warming patterns affect the thermal gradients between the tropics and high latitudes, leading to changes in midlatitude baroclinicity, a key factor for synoptic dynamics. Investigating a comprehensive understanding of the links between global warming and atmospheric energy cycle is crucial for identifying the mechanisms responsible for extreme events.

The Lorenz energy cycle provides a robust framework for examining the generation, conversion, and distribution of atmospheric energy. It effectively explains the formation of available potential energy resulting from differential heating in the atmosphere and its subsequent conversion into kinetic energy through large-scale dynamical processes. Analyzing the Lorenz energy cycle offers crucial insights into the ways global warming impacts large-scale circulation.

This study revisits and evaluates the Lorenz energy cycle to provide a more comprehensive understanding of how global warming influences the global energy cycle and general circulation. Furthermore, it explores the potential implications of these changes for the development and intensification of extreme weather phenomena.

How to cite: Noh, E. and Kim, J.: Revisiting the Loreanz Energy Cycle: Impacts of Global Warming on Atmospheric Energy Cycle, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19098, https://doi.org/10.5194/egusphere-egu25-19098, 2025.

EGU25-19200 | ECS | Orals | AS1.26

The dynamics of extreme wave-activity events in a warming climate. 

Pragallva Barpanda and Camille Li

Climate change is projected to have wide ranging impacts on the atmospheric waves and mean-flow. However, it remains uncertain as to how exactly the warming climate will influence the mean-waviness of the jet stream and extreme wave-activity events in the midlatitude storm track. An objective identification of this phenomena is important as wave-activity aloft plays an important role in driving the extreme weather events over the continents. Here we use the local wave activity (LWA) metric to quantify stationary and transient wave activity during winter-time from multi-member ensembles of state-of-the-art climate model simulations including, NorESM, CESM-LENS2 and MPI-LE simulations for Historical and various SSP warming scenarios. Our analysis reveals a statistically significant decrease in the mean-waviness of the jet stream and region-specific changes in the probability of extreme wave-activity events in the midlatitudes. These changes are found to be dynamically consistent with the theoretical predictions from the non-acceleration relation and the recently proposed traffic-jam theory of atmospheric blocking.

How to cite: Barpanda, P. and Li, C.: The dynamics of extreme wave-activity events in a warming climate., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19200, https://doi.org/10.5194/egusphere-egu25-19200, 2025.

EGU25-19675 | ECS | Posters on site | AS1.26

Large-scale tropospheric wave activity involved in the winter NAO-related variability 

Marta Brotons, Javier García-Serrano, and Reindert J. Haarsma

In the last decades, there has been an ongoing discussion whether the winter North Atlantic Oscillation (NAO) is a zonally-symmetric hemispheric mode of variability driven by transient eddies and strongly coupled to the stratosphere [Arctic Oscillation/Northern Annular Mode (AO/NAM)]; or a regional mode of variability forced locally by transient eddies (NAO) but with associated hemispheric anomalies related to stationary eddies in the Circumglobal Waveguide Pattern (CWP). We revisit this question using zonal wavenumber decomposition of NAO-related circulation anomalies in reanalysis (ERA5, NCEP-NCAR). At upper-tropospheric levels, the NAO exhibits a wave-like structure that resembles the CWP, where wavenumber 3 seems to dominate at subpolar latitudes and  wavenumber 5 is more prominent at suptropical latitudes. Wavenumber 4 does not significantly contribute to the NAO pattern in the total field. The wave activity flux of NAO-related variability reveals downstream propagation and splitting of wave energy which appears to be consistent with the meridional component of the wind and with theoretical arguments of stationary wavenumber based on the background flow. These results support the relevance of large-scale stationary waves in the hemispheric signature of the NAO. To further diagnose the tropospheric propagation of NAO-related anomalies, additional analysis using ray tracing and experiments with a linear barotropic model are performed.

How to cite: Brotons, M., García-Serrano, J., and Haarsma, R. J.: Large-scale tropospheric wave activity involved in the winter NAO-related variability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19675, https://doi.org/10.5194/egusphere-egu25-19675, 2025.

The most serious heavy precipitation in the past 43 years (1979-2021) occurred over Fujian-Jiangxi region from late May to early June of 2006, causing significant economic losses. Using the daily precipitation collected at 2479 surface meteorological stations in China and ERA5 reanalysis database, the present study investigates the relationship between the heavy precipitation over Fujian-Jiangxi region in late spring-early summer of 2006 and baroclinic Rossby wave packets in the upper troposphere. Information flow between the two systems has been diagnosed. Results indicate that the disturbance source for this heavy precipitation originated from areas near the Syrian Desert to the north of the Arabian Peninsula and propagated along the northwest-southeast direction, reaching Fujian-Jiangxi region four days later. This kind of baroclinic Rossby wave packets provide the necessary energy for the occurrence and persistence of heavy precipitation. Analysis of wave activity flux vectors indicates that during the heavy precipitation period, disturbance energy was transported from the upstream westerly belt to Fujian-Jiangxi region almost every day. Obviously, there existed information transfer between the two regions, re-confirming that the upstream Rossby wave packets affect the Fujian-Jiangxi precipitation. The above results provide helpful hints for a better understanding of the mechanisms for heavy precipitation in this region and will be helpful for its effective prediction.

How to cite: Ye, D., Guan, Z., Sun, S., and Jin, D.: The connection between baroclinic Rossby wave packets in the upper troposphere and regional-scale heavy precipitation over Fujian-Jiangxi region in the late spring-early summer of 2006, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-226, https://doi.org/10.5194/egusphere-egu25-226, 2025.

EGU25-1363 | ECS | Orals | AS1.27 | Highlight

The role of Rossby wave breaking in coral bleaching on the Great Barrier Reef 

Lara Richards, Steven Siems, Yi Huang, Wenhui Zhao, Daniel Harrison, Michael Manton, and Michael Reeder

The frequencies of thermal coral bleaching events (CBEs) over the Great Barrier Reef (GBR) continue to increase with five mass CBEs reported since 2016. While changes in the local meteorology, such as reduced wind speeds and decreased cloud cover, are known to heat the shallow reef waters, little consideration has been given to the overriding synoptic meteorology. The 2022 CBE, occurring under La Niña conditions, saw ocean temperatures at Davies Reef increase 1.9℃ over 19-days and subsequently cool 2.1℃ back to seasonal norms over eight days. 

This event was found to be triggered by repeated Rossby wave breaking disrupting the local trade winds. As the trades broke down, calm winds and clear skies covered the reef, thus inhibiting the latent heat flux, allowing for the build-up of ocean heat to at least 18m. Following the re-establishment of the trade winds via coastal ridging, latent heat fluxes, the primary driver of the event, tripled allowing the ocean to rapidly cool. 

Concurrent to the mass bleaching event, these are the same Rossby wave breaking events found to cause the historic Lismore flooding located hundreds of kilometres south of the GBR. This case study notes the first reported linkage between mass coral bleaching and a severe flooding event.

How to cite: Richards, L., Siems, S., Huang, Y., Zhao, W., Harrison, D., Manton, M., and Reeder, M.: The role of Rossby wave breaking in coral bleaching on the Great Barrier Reef, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1363, https://doi.org/10.5194/egusphere-egu25-1363, 2025.

EGU25-2523 | ECS | Posters on site | AS1.27

AMO and PDO modulate the multidecadal variability of WACE 

Yongyue Luo, Gerrit Lohmann, Monica Ionita, Xiadong An, Yuchen Sun, and Chun Li

Since global warming, the Warm Arctic-Cold Eurasia (WACE) has experienced significant interdecadal variabilities, and its interdecadal variability has increased significantly after Arctic amplification. Temperature changes over Barents-Kara Seas region play a leading role in the interdecadal variability of WACE. Before Arctic amplification, the circulation influencing WACE was primarily characterized by the meridional circulation of the Arctic-Eurasian Dipole. After Arctic amplification, however, the circulation is mainly represented by the north-south Rossby wave trains over the Eurasian continent. Before Arctic amplification, the Atlantic Multidecadal Oscillation (AMO) and the Pacific Decadal Oscillation (PDO) changed in phase, stimulating the eastward propagation of Rossby wave trains along the mid-latitudes. The PDO-induced Arctic-Eurasian Dipole circulation played a leading role over Eurasian, while the AMO weakened the PDO signal in the key North Atlantic and Arctic regions. While after Arctic amplification, the AMO and PDO change in an out-of-phase relationship, with the eastward propagation of Rossby wave trains still occurring along the mid-latitudes. In this phase, the south-north Rossby wave trains excited by the AMO dominate over Eurasian, with the PDO weakening the AMO signal in the North Atlantic and enhancing the AMO signal in the critical Arctic region. Since the interdecadal variability of WACE is primarily driven by temperature changes in the key regions of Arctic, both the PDO and AMO play crucial roles in modulating the interdecadal changes in WACE before and after Arctic amplification. The two exhibit an antagonistic relationship before Arctic amplification, while their relationship becomes primarily synergistic after amplification.

How to cite: Luo, Y., Lohmann, G., Ionita, M., An, X., Sun, Y., and Li, C.: AMO and PDO modulate the multidecadal variability of WACE, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2523, https://doi.org/10.5194/egusphere-egu25-2523, 2025.

EGU25-2544 | ECS | Posters on site | AS1.27

Linking Northern Hemisphere extreme cold weather events to upper atmospheric circulation 

Morteza Babaei, Rune Grand Graversen, and Johannes Patrick Stoll

Previous studies have indicated that increased probability of extreme events in many regions of mid-latitude is linked to amplified waviness and slow upper-atmosphere circulation. However, this linkage appears to be dependent on region, and details regarding the waviness or slowness required to promote extreme events locally remain unclear. The objective of this study is to examine the upper atmospheric circulation and the linkage between the occurrence of cold extremes in different regions of the Northern Hemisphere in winter. We examine this link using the fifth-generation ECMWF reanalysis data (ERA5).

The upper atmospheric waviness—both in the vertical and the meridional direction—is computed based on geopotential height at 300 hPa. At each latitude, the vertical waviness is estimated as the circumglobal amplitude of the first five zonal wave numbers based on a Fourier decomposition. For the meridional waviness, the amplitude of each specific ridge and trough is defined as the latitudinal deviation of the isoheight taken as the zonal geopotential height mean over the region of the ridges and troughs. The speed of planetary wave zonal propagation is computed through the utilization of a top-ridge and bottom-trough tracking algorithm.

In most of the studied regions, there is a significant slowdown in the upstream ridge and downstream trough during a cold spell, confirming earlier results. For the North American cold spells, this pattern is mainly observed at high latitudes, particularly between 60° and 75° N. During cold spells over the British Isles, Europe, and Nordic countries, the speed of the ridges and troughs decreases at mid-latitude yet continues moving eastward. For cold spells over Central Asia, the ridges and troughs become significantly slower at high latitudes (60°N–80°N) but faster at lower latitudes (35°N–45°N). Contrary to our expectations, the circumglobal vertical amplitude over mid-latitudes for most regions’ cold spells exhibits less waviness. However, each local meridional wave amplitude associated with upstream ridges and downstream troughs in the vicinity of the cold spell’s location becomes significantly larger. Hence, the waviness and slow upper-atmosphere circulation associated with each region's cold extremes occur more locally than globally. Our results also indicate that amplified local meridional wave amplitude always precedes cold spells, but ridges and troughs become slower—depending on the locations of the cold spells—before or during cold spells.

How to cite: Babaei, M., Grand Graversen, R., and Patrick Stoll, J.: Linking Northern Hemisphere extreme cold weather events to upper atmospheric circulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2544, https://doi.org/10.5194/egusphere-egu25-2544, 2025.

EGU25-4152 | ECS | Posters on site | AS1.27

The temporal mean of transient Rossby wave packets 

Wolfgang Wicker and Daniela Domeisen

Extremes of temperature or precipitation on intra-seasonal time scales are commonly structured in a circumglobal wave with a synoptic-scale zonal wavenumber. The mechanism that determines this wavenumber and the relationship with processes on shorter timescales, such as Rossby wave packets, are not fully understood. We employ a simple kinematic model to demonstrate how a transient Rossby wave packet produces significant temporal mean circulation anomalies with a wavelength that is larger than the wavelength of the instantaneous wave packet itself. This demonstration is verified by comparison with a linear, quasi-geostrophic channel model where we can assess sensitivities to the latitude and the meridional extent of the wave packet. These two highly idealized models help us to better understand the role of Rossby wave packets in concurrent and compound weather extremes.

How to cite: Wicker, W. and Domeisen, D.: The temporal mean of transient Rossby wave packets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4152, https://doi.org/10.5194/egusphere-egu25-4152, 2025.

Mesoscale heating can influence the mid-latitude large-scale flow by redistributing potential
vorticity (PV) along the tropopause, impacting Rossby wave evolution. This study explores how
mesoscale heating not only perturbs the mid-latitude circulation but may also catalyze Rossby
wave breaking along the jet stream.

A forecast bust of a Rossby wave breaking event over the North Atlantic in April 2020 is
examined. The case involves a warm conveyor belt (WCB) with embedded convection and
upstream thunderstorms over North America. The case is evaluated using archived forecast data
from various weather centers and reforecasts conducted with the Model for Prediction Across
Scales (MPAS) at horizontal resolutions from 60 to 3.75 km. Potential vorticity tendencies (i.e.,
microphysics, convection, radiation) are output to diagnose multi-scale interactions.

Key findings show mesoscale heating on the jet stream's equatorward side is critical for Rossby
wave predictability. Higher-resolution simulations capture a more persistent WCB and stronger
PV reduction along the tropopause due to microphysics, amplifying the Rossby wave. In
contrast, coarser simulations failed to sustain WCB persistence, favoring cyclonic wave breaking
regardless of initial conditions.

Ensemble members with persistent mesoscale convective systems over North America were
associated with slowed Rossby wave packet progression, leading to anticyclonic wave breaking
over the Atlantic, and the most accurate forecasts. This outcome was sensitive to initial
conditions and to the persistence of the adjacent WCB.

The presented findings highlight the importance of faithfully simulating mesoscale heating
across a RWP to successfully forecast an individual Rossby wave breaking event. Implications of
these results for ongoing global convection-resolving MPAS simulations at the National Center
for Atmospheric Research are also discussed.

How to cite: Lojko, A.: The Importance of Mesoscale Heating Along a Rossby Wave Packet for the Predictability of a Rossby Wave Breaking Event, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4590, https://doi.org/10.5194/egusphere-egu25-4590, 2025.

EGU25-4858 | ECS | Posters on site | AS1.27

The influence of diabatic processes on North Atlantic winter jet streaks and their extremes 

Mona Bukenberger, Sebastian Schemm, Lena Fasnacht, and Stefan Rüdisühli

The jet stream — the hemispheric-wide band of westerly winds that circles the mid-latitudes and shapes day-to-day weather by guiding large-scale flow features — has been a long-standing area of interest in atmospheric dynamics. Within this stream, jet streaks are regions of enhanced wind speed. These important features of atmospheric flow are frequently accompanied by clear-air-turbulence, affecting air travel flight times, comfort, and safety. 

Moreover, upper level divergence in the equatorward entrance and poleward exit regions couples jet streaks to surface weather via vertical motion. This links jet streaks to rapid cyclogenesis, intense precipitation, and extreme wind events. Extreme jet streaks are also often linked to poor performance of numerical weather prediction (NWP).  Understanding the dynamics of (extreme) jet streaks is hence important to further the mechanistic understanding of extreme weather events as well as error busts, and ultimately improving forecast quality.

Traditional tools, like the PV gradient and PV frontogenesis frameworks, have shed light on the dry dynamics of jet streaks. Similarly, the classical four-quadrant model explains their influence on surface weather. However, diabatic processes have been shown to play an important role in jet streak development. They are also key for the (mis)representation of jet streak in NWPs, warranting systematic and quantitative analysis. 

In this study, we explore the impact of diabatic processes on jet streak evolution using composite analysis and a Lagrangian PV-gradient diagnostic. It is based on ERA5 data from North Atlantic winters (DJF) spanning 1979–2023. We begin by characterizing the life cycle of jet streaks and extreme jet streaks and their relationship with Rossby waves and Rossby wave breaking.
Our findings show that stronger jet streaks tend to last longer, with their maximum wind speeds scaling with the PV gradient at their core. Extreme jet streaks frequently coincide with intense low-pressure systems, heavy precipitation, and upstream warm conveyor belts, indicating a heightened role of diabatic processes in their evolution. Using the Lagrangian PV gradient framework, we quantify the influence of diabatic processes, comparing extreme and non-extreme jet streaks. The results reveal a clear upward interaction between surface weather and jet streak development, with diabatic effects more pronounced in extreme cases.

Our findings underscore the need for further research into individual diabatic processes driving jet streak evolution. They also add to the growing evidence that extreme jet streak events may become more frequent in a warming climate.

How to cite: Bukenberger, M., Schemm, S., Fasnacht, L., and Rüdisühli, S.: The influence of diabatic processes on North Atlantic winter jet streaks and their extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4858, https://doi.org/10.5194/egusphere-egu25-4858, 2025.

Stationary Rossby waves can counteract the eastward drift of westerly wind and persist over a region for extended periods. This prolonged influence over a fixed region makes it highly conducive to the occurrence of extreme event. The propagation of stationary Rossby wave is significantly influenced by the configuration of mean flow. The jet stream, characterized by a narrow region in the atmosphere with high zonal wind speed, is particularly favorable for the propagation of stationary Rossby wave. The jet stream affects the propagation of stationary Rossby wave primarily through the strong lateral wind shear, so can be seen as a barotropic waveguide. In a three-dimensional basic state, a waveguide can also form without the presence of strong lateral wind shear. Instead, it can arise due to significant variations in stratification, forming a baroclinic waveguide. The baroclinic waveguide is particularly pronounced during summertime over northern Eurasia, resulting in nearly twice as much stationary Rossby wave activity at high latitudes compared to that at middle latitudes. These stationary Rossby waves are believed to be directly responsible for the occurrence of extreme heatwaves in Europe, such as those experienced in 2010 and 2019, as well as the Northern China heatwave in 2023. In this talk, I will introduce the characteristics and dynamics of these stationary Rossby waves in the baroclinic waveguide. In addition, I will also discuss the predictability of these stationary Rossby waves in current operational numerical models. It will be shown that these stationary Rossby waves exhibit a zonally-oriented spatial structure along the baroclinic waveguide. The evolution of these waves is primarily determined by the nonlinear interactions with transient eddies. This strong nonlinearity poses a significant challenge for current operational numerical models in accurately predicting them.

How to cite: Xu, P.: Stationary Rossby waves in a baroclinic atmospheric waveguide , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5000, https://doi.org/10.5194/egusphere-egu25-5000, 2025.

North American cold spells are frequently associated with the amplification of a large-scale atmospheric circulation pattern known as the Alaskan Ridge. This pattern is characterised by a persistent high over Alaska and two low-pressure centres over the Pacific Ocean and Hudson Bay. While the Alaskan Ridge (particularly the high over Alaska) has been widely discussed in the literature, a comprehensive understanding of the multiple drivers behind its amplification remains elusive. Here, we consider the dynamical drivers of the intensified high over Alaska leading to cold spells in central North America. First, we separate the cold spells based on whether they are associated with stratospheric wave reflection. This separation reveals two distinct atmospheric states resulting in upper-tropospheric high formation. Second, we employ a wave decomposition technique based on normal-mode functions to understand the role of tropospheric dynamics on different scales in favouring the Alaskan Ridge amplification. This methodology's advantage is the ability to separate Rossby and inertia-gravity regimes as opposed to the widely utilised Fourier decomposition. The focus is on planetary (zonal wavenumbers 1-3) and synoptic (zonal wavenumbers 4-8) scales. The results show enhanced synoptic-scale Rossby wave activity prior to the Alaskan Ridge amplification. Based on the shape and location of the synoptic anomalies, we attribute the enhancement to an extratropical-midlatitude interaction, a driver previously proposed in the literature. Our approach enables a holistic picture of the atmospheric evolution leading to the central North American cold spells, supporting a dynamical understanding of their origin.

How to cite: Strigunova, I. and Messori, G.: Scale-Dependent Dynamics of Alaskan Ridge Amplification: A Holistic View of Circulation Driving North American Cold Spells, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7089, https://doi.org/10.5194/egusphere-egu25-7089, 2025.

The boreal summer Circum-global teleconnection (CGT) pattern is identified as a stationary Rossby wave train propagating along the subtropical jet at interannual timescale. The variation of CGT is closely linked to the occurrence of heat extremes over mid-latitude regions. How CGT would change under global warming and the associated climatic effect remains unclear. Here, based on 34 models from Coupled Model Intercomparison Project phase 6 (CMIP6), we show evidence that the amplitude of CGT wave train will reduce robustly by 2100, with multi-model ensemble mean decrease of 31.8%. The reduction of CGT amplitude is reflected in the decrease of Rossby wave source (RWS) anomalies, with upstream signal located at jet entrance over eastern Mediterranean. The weakening of eastern Mediterranean RWS anomalies is further resulted from decreased circulation anomalies. The weakened CGT further alters the pattern of associated heat extreme events. Heat extreme days during each positive CGT event significantly increase from 5.5 days to 7.0 days at four hotspot regions across mid-latitudes: eastern Europe, Tibetan Plateau, northeastern Asia and southern Great Plains. Our findings highlight the aggravation of heat extremes induced by change of atmospheric teleconnection under global warming and additional burden on food security and ecosystems for policymakers to consider.

How to cite: Yu, H.: Weakened Circum-global Teleconnection Pattern under global warming would exacerbate heat extremes across Eurasia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8255, https://doi.org/10.5194/egusphere-egu25-8255, 2025.

EGU25-8345 | ECS | Posters on site | AS1.27

Quantifying the relationship between extratropical cyclones' intensity measures and their background state: systematic exploration of a baroclinic wave simulation ensemble 

Clément Bouvier, Joona Cornér, Andy Bowery, Glenn Carver, Sarah Sparrow, David Wallom, and Victoria Sinclair

Extreme extratropcial cyclones (ETC) are associated with heavy precipitation, and strong winds causing damage to infrastructure, or diverse economic losses. They can be characterised by a set of variables or diagnosis named intensity measures. Based on them, meteorologists are able to study the intricate relationship between dynamical features and impacts of ETCs. However, considerable additional research is required to improve our understanding of the relationship between ETCs' intensity and the the background state they develop in. Our baroclinic wave simulation setup implemented in OpenIFS 43r3 has shown the possibility to create stable and flexible background states able to run with moisture and full physics. Moreover, 7 parameters can be easily varied to produce a vast array of different background states. By varying these parameters, an ensemble of 6,500 baroclinic waves are simulated using OpenIFS@home, a version of OpenIFS that runs within a volunteer computing framework. In these cases, the developing ETCs are physically realistic with poleward motion, upstream and downstream development and sensible minimum mean sea level pressure.

This study proposes a Machine Learning based and systematic approach to link the 6,500 background states with their developing ETCs. Each ETC is isolated and tracked. A total of 75 features are extracted from tracked ETCs for each case. A Random Forest Regressor (RFR) is use to predict each 13 intensity measures with 5 background features. One of the properties of the RFR is its ability to rank its input features during the training. As a result, this embedded feature selection allow to quantify the strength of relationship - called feature importance. For example, the feature importance between the initial average temperature with the resulting accumulated precipitation, or the horizontal temperature gradient at 300hPa with the maximum relative vorticity at 850hPa can be estimated. The proposed methodology is able to (1) predict 13 intensity measure, (2) link them to 5 background features, and (3) reduce the training dataset by filtering the ETCs to the most intense. To stabilise the feature selection, a bootstrapping-based approach has been implemented. Using the distributed nature of the workflow, the whole ensemble of 6,500 baroclinic waves is processed within 1.5 days on 40 cores and the computational time reduces linearly with the number of cores.

With the exception of the storm severity index, the RFR is able to predict the intensity measures with a coefficient of determination between 0.65 and 0.92. Moreover, this study demonstrates an increase feature importance of the upper-troposphere baroclinicity as the training dataset is reduced to the most intense ETCs. Concurrently, the importance of the lower-tropospheric baroclinicity decreases. The feature importance of friction, initial relative humidity, initial laps rate and average surface virtual temperature stays constant. Future work will include the use of Deep Learning Regressor and wrapped feature selection in order to validate and extend the main result of this study.

How to cite: Bouvier, C., Cornér, J., Bowery, A., Carver, G., Sparrow, S., Wallom, D., and Sinclair, V.: Quantifying the relationship between extratropical cyclones' intensity measures and their background state: systematic exploration of a baroclinic wave simulation ensemble, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8345, https://doi.org/10.5194/egusphere-egu25-8345, 2025.

Record-breaking rainfall occurred coherently over subtropical West Asia (WA) and East Asia (EA) in April 2024, causing catastrophic damages around the Persian Gulf and South China. Strong barotropic cyclones are directly responsible for the long-lasting extreme rainfall over WA and EA. Based on observational analyses and numerical simulations by a linear baroclinic model (LBM), here we show evidences that these two rainfall extremes are tele-connected and are tied to the record-breaking latent heat release over tropical Indian Ocean (TIO). The record-breaking latent heat release over TIO triggers a stationary Rossby wave train propagating northward, with a barotropic anticyclone over Northern Indian Ocean and a barotropic cyclone over WA, leading to extreme WA rainfall. The intense latent heat release associated with the extreme rainfall over WA triggers another stationary Rossby wave train along the Asian subtropical jet (ASJ), with a wavelength of about 50~55 degrees in longitude. This wave train anchors a downstream barotropic cyclone anomaly on the eastern periphery of Tibetan Plateau with southerly flow from South China Sea to Eastern China, in favor of excessive rainfall over the EA region.

The above mechanism not only explains why rainfall extremes in WA and EA are located at a same latitude (20°-30°N) along the ASJ, but also clarifies why the intense rainfall over WA and EA occurred in April 2024 rather than other seasons. Spring 2024 was associated with a rapid decay of an El Niño event, and convection over TIO was suppressed by descending branch of Walker circulation before April. Along with the decay of warm SST anomaly over equatorial Pacific, TIO became warmer than Pacific in April, giving rise to intense convection over TIO which triggered the stationary Rossby waves. Although record-strong latent heating anomaly over TIO persisted from April into May in 2024, the substantially northward shifted ASJ in May cannot anchor the stationary Rossby waves in response to TIO heating, since subtropical circulation response to tropical heating is strongly dependent on the basic state flow. This work highlights the importance of both basic state and tropical heating anomaly in shaping tele-connected Asian climate extremes during the decaying phase of El Niño.

 

References: He C, Kucharski F (2025) Tele-connected rainfall extremes over West and East Asia in April 2024 tied to Indian Ocean heating. Accepted by Clim Dynam.

How to cite: He, C. and Kucharski, F.: Tele-connected rainfall extremes over West and East Asia in April 2024 tied to Indian Ocean heating, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8636, https://doi.org/10.5194/egusphere-egu25-8636, 2025.

EGU25-9873 | ECS | Posters on site | AS1.27

Summer Greenland Blocking in observations and in SEAS5.1 seasonal forecasts: robust trend or natural variability? 

Giorgia Di Capua, Johanna Beckmann, and Paolo Davini

Summer Greenland blocking - a persistent anticyclone in the mid-troposphere in proximity of Greenland – has shown to severely impact melting of the Greenland ice sheet. Thus, changes in its frequency and characteristics would likely affect the stability of the Greenland Ice sheet, and potentially sea level rise. Despite in recent decades the occurrence of such atmospheric pattern has seen a marked increase, such observed trend is not captured by any simulation from state-of-the-art global climate models.

Here we aim to assess whether the lack of trend is caused by (i) a misrepresentation of key physical mechanisms in climate models or (ii) whether such trend is mainly attributable to decadal variability, or both. We analyze Greenland blocking characteristics in reanalysis (ERA5) and ECMWF seasonal forecasts (SEAS5.1) over the period 1981-2023, showing that about 10% of the 1000 permutations of SEAS5.1 runs can simulate a 43-year trend equal or larger to the ERA5 one. Such capacity of partially replicating the observed trend shows that the initialization of the seasonal forecast – as well as the higher model resolution - contribute to a more realistic representation of the blocking dynamics than in freely evolving climate runs.

We then apply the Peter and Clark momentary conditional independence (PCMCI) algorithm to assess monthly causal pathways. Results show that while the relationship among Arctic temperature, snow cover, Atlantic multidecadal variability and Greenland blocking is consistent both in ERA5 and SEAS5.1, the effect of early snow melt over North America on Greenland blocking is mostly absent in SEAS5.1. Therefore, while it is possible that the observed trend is due to internal decadal variability, the misrepresentation of the snow cover processes may explain the rare occurrence of a positive trend in SEAS5.1. This deficit in representing the snow impact on the atmospheric circulation might also be the culprit of the missing trend in climate models, raising the question whether long-term projections underestimate a future increase in Greenland blocking and ice melt.

Beckmann, J., Di Capua, G., and Davini, P.: Summer Greenland Blocking in observations and in SEAS5.1 seasonal forecasts: robust trend or natural variability?, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2024-3998, 2025.

 

How to cite: Di Capua, G., Beckmann, J., and Davini, P.: Summer Greenland Blocking in observations and in SEAS5.1 seasonal forecasts: robust trend or natural variability?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9873, https://doi.org/10.5194/egusphere-egu25-9873, 2025.

EGU25-10085 | Orals | AS1.27

Driving of the subtropical jet by tropical convection 

Orli Lachmy, Ian White, and Nili Harnik

A moist, idealized model is used to examine the driving influence of deep tropical convection on the wintertime subtropical jet. The model is run with fixed zonally symmetric sea surface temperatures under perpetual solstice conditions. To focus on the strongest convective activity, the daily data is re-centered around the longitude of maximum tropical convection. The qualitative picture that emerges suggests that deep tropical convection in the summer hemisphere drives an anomalous localized Hadley cell that crosses into the winter hemisphere and drives a locally strengthened subtropical jet downstream via advection of planetary angular momentum. Momentum fluxes associated with both the divergent overturning circulation and rotational eddies drive a local longitudinal minimum of angular momentum where the localized Hadley cell crosses the equator, thus highlighting the complexity in interpreting the angular-momentum budget due to the inherent zonally asymmetric nature of tropical convection. The results are compared with the circulation in a dry model, where a single jet inside the Ferrel cell dominates the zonal mean flow. The role of moisture in driving a subtropical jet is discussed.

How to cite: Lachmy, O., White, I., and Harnik, N.: Driving of the subtropical jet by tropical convection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10085, https://doi.org/10.5194/egusphere-egu25-10085, 2025.

EGU25-11835 | ECS | Posters on site | AS1.27

The circulation response to Arctic Amplification in zonally symmetric and asymmetric aquaplanets 

Michele Filippucci, Stephen Thomson, Neil Lewis, and Simona Bordoni

This study investigates the impact of Arctic Amplification (AA) on midlatitude temperature extremes using aquaplanet simulations within the ISCA intermediate complexity modeling framework. We use a mixed-layer ocean as boundary condition and grey radiation. Simulations are run with two setups: a zonally symmetric control and a zonally asymmetric experiment. In the asymmetric experiment a localized oceanic heating is prescribed in the midlatitudes to mimic a western boundary current and generate a eddy transient kinetic energy maximum (or storm track). For each setup, we run simulations without and with AA, whereby anomalous heating is imposed in the northern polar region.

We investigate the autocorrelation of local wave activity (LWA) in our experiments, as this allows us to focus on persistent LWA regimes, which can be linked with temperature extremes such as heatwaves and cold spells. We find that the autocorrelation maxima in the asymmetric configuration correlate with well known atmospheric patterns such as atmospheric blocking, demonstrating that our model setup, despite its simplicity, can reproduce realistic features of Earth’s atmospheric circulation. Early results show how the LWA autocorrelation slightly increases with AA in the zonally symmetric setup, and decreases with AA in the zonally asymmetric setup, indicating that the sign of the change depends on the zonal symmetry. This suggests that the LWA climatology, highly sensitive to the presence of a storm track region, plays a crucial role in the atmospheric response to AA.

How to cite: Filippucci, M., Thomson, S., Lewis, N., and Bordoni, S.: The circulation response to Arctic Amplification in zonally symmetric and asymmetric aquaplanets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11835, https://doi.org/10.5194/egusphere-egu25-11835, 2025.

EGU25-13583 | Orals | AS1.27

On storm tracks, weather regimes, and a wave breaking recipe 

Talia Tamarin-Brodsky and Nili Harnik

The atmospheric circulation is often decomposed into high- and low- frequency variability. For example, the low-frequency variability in the North-Atlantic includes slowly varying weather regimes such as the North Atlantic Oscillation, with timescales of weeks. The high frequency variability includes the synoptic weather systems, which shape our daily weather fluctuations. The interaction among these timescales is often mediated by Rossby Wave Breaking (RWB) events, which involve the irreversible breaking and dissipation of the baroclinic waves. To investigate this interaction, a simple RWB recipe is derived by exploring which processes contribute to a meridional overturning of high-frequency PV contours. A picture emerges in which the slowly-varying weather regimes influence the tracks of high-frequency systems, which in turn, depending on the position relative to the low-frequency flow, determines whether the frequency of RWB (cyclonic or anticyclonic) is enhanced or suppressed. The recurrence of same-type RWB in a similar position then shapes the overall mean structure of the weather regime.

How to cite: Tamarin-Brodsky, T. and Harnik, N.: On storm tracks, weather regimes, and a wave breaking recipe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13583, https://doi.org/10.5194/egusphere-egu25-13583, 2025.

EGU25-13852 | ECS | Posters on site | AS1.27

Intra-seasonal differences in summer blocking patterns over Greenland 

Linh Nhat Luu, Edward Hanna, and Xavier Fettweis

Summer Greenland blocking, a persistent anticyclonic pattern, has high impacts on local and regional weather and climate, especially on triggering huge melt over the Greenland ice sheet. The phenomenon is observed to increase in intensity (based on Greenland blocking index, GB2) in recent decades. This increase is highly correlated with the negative phase of the dominant climate oscillation in the North Atlantic, namely the NAO. However, summer NAO shows different behavior in June in comparison with high summer months, i.e., July and August. In this study, we analyse the spatial patterns of Greenland blocking events in these individual months to evaluate how different they are. We use different approaches including a clustering analysis with Self-Organising Map (SOM) to evaluate individual blocking days, and an event-based analysis to assess the development of blocking events over the course of 9 days centred at the day when GB2 reach maximum value during that event. The results from both analyses show that Greenland blocking patterns are more alike between July and August, while those of June are different.

How to cite: Luu, L. N., Hanna, E., and Fettweis, X.: Intra-seasonal differences in summer blocking patterns over Greenland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13852, https://doi.org/10.5194/egusphere-egu25-13852, 2025.

With increasing global temperatures, there has been an observed increase in the quantity and intensity of extreme weather events, particularly heat extremes in the midlatitude regions. Some recent studies have attributed this increase at least partially to an amplification of upper tropospheric jet stream waves. Whilst there is significant scientific uncertainty over causes of recent trends in jet stream waviness, the impact atmospheric waves have on extreme events is clear. Therefore it is key to quantify whether the relative importance of jet stream waviness on the formation of extreme temperature events changes in the future.

We achieve this by studying the probability ratio between co-occurring high magnitude geopotential height anomalies at 500 hPa, and coincident surface temperature extremes. We calculate this for the historical period (1980-2015) and the future (2065-2100), and compare how this probability ratio - the association between atmospheric circulation and surface temperature extremes - changes between these two periods. To understand the changes seen, we also look at projected changes in the frequency of high magnitude geopotential height anomalies.

Results from three large ensembles show that cold extremes in boreal winter (December-February) exhibit a clear decrease in association between the historical to the future period, indicating that cold extremes at the end of the 21st century become less associated with strong atmospheric circulation anomalies compared to the current historical period. Conversely, hot extremes in boreal summer (June-August) exhibit small regional changes in association for the future period but hemispherically show no clear trend. We further explore the boreal winter trend in CMIP6 models, and explore mechanisms for this trend by comparing across different models with different changes. 

How to cite: Roocroft, E. and White, R.: Future changes in association between atmospheric circulation anomalies and extreme temperature events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14079, https://doi.org/10.5194/egusphere-egu25-14079, 2025.

EGU25-14224 | ECS | Orals | AS1.27

Does ‘Blocking’ Shape the Future of Antarctic Heat Extremes? 

Prasad Shelke and James Renwick

2024 has been recorded as the hottest year in human history. Antarctica, already an ‘extreme’ environment, has been continuously witnessing unprecedented records in heat extremes in recent years. A record-shattering Antarctic heatwave in March 2022 highlights the importance of large-scale atmospheric circulations in the Southern Hemisphere (SH), such as atmospheric blocking. However, the presence of blocking patterns over the Antarctic continent is rarely discussed, often dismissed as 'too far south' to warrant attention.

This study examines the influence of SH blocking patterns on Antarctic heat extremes. We assess the ability of Community Earth System Model 2 (CESM2) to represent this complex relationship. Our findings suggest that SH blocking patterns exhibit elevated occurrences over the Antarctic Peninsula and East Antarctica. The future projections suggest a decline of SH blocking by 30% under SSP370 scenario by the end of the 21st century. We explored the evolving relationship between blocking and heat extremes under a warming climate and found that the future decline in blocking occurrences is disproportionate to the corresponding changes in this relationship. This underscores that the role of blocking in future heat extremes will remain significant, especially due to the poleward expansion of the subtropics.

How to cite: Shelke, P. and Renwick, J.: Does ‘Blocking’ Shape the Future of Antarctic Heat Extremes?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14224, https://doi.org/10.5194/egusphere-egu25-14224, 2025.

EGU25-15789 | Orals | AS1.27

Double jet streams and their connection to heatwaves in the Northern Hemisphere 

Andrea K. Steiner, Martin Kriegl, and Moritz Pichler

Heat extremes are exacerbated by ongoing climate change and have severe consequences on humans and the environment. Climate change also leads to changes in atmospheric circulation that affect the jet stream. One configuration of the jet stream is the double jet, where the jet splits into two branches, potentially triggering persistent weather patterns and prolonged heat extremes. We conducted a comprehensive assessment of double jet stream states over the Northern Hemisphere and their connection to heatwaves in the extended summer period May to October for 1979 to 2023, using ERA5 data. The results show an increase in double jet frequency over North America, as well as in persistence over Asia and North America. More persistent double jets are associated with higher heatwave cumulative intensity. We identified Europe as a double jet stream hotspot region, with the most pronounced connection to heatwaves. 40–80% of heatwaves co-occur with double jet events in Europe, 30–60% in Asia, and 15–50% in North America, particularly in northern regions. Northern Europe, particularly areas north of 50°N, such as Scandinavia, the British Isles, the Baltic region, and western Russia, exhibit a pronounced and statistically significant connection between double jet stream occurrences and heatwaves. We also found a significant relationship between double jet events and heatwaves in some regions of Asia, particularly between 60°N to 80°N, as well as in central China. The pronounced connection in areas northward of 50°N broadly aligns with the position of the double jet stream wind minimum, where persistent weather conditions tend to prevail. Overall, our results reveal a significant connection between double jet events and land heat extremes in the Northern Hemisphere and the shift towards more persistent double jet events, underpinning their importance for extreme weather.

How to cite: Steiner, A. K., Kriegl, M., and Pichler, M.: Double jet streams and their connection to heatwaves in the Northern Hemisphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15789, https://doi.org/10.5194/egusphere-egu25-15789, 2025.

EGU25-15844 | ECS | Orals | AS1.27

Observed circulation trends in boreal summer linked to two spatially distinct teleconnection patterns 

Tamara Happé, Chiem van Straaten, Raed Hamed, Fabio D'Andrea, and Dim Coumou

Various regions in the Northern Hemispheric midlatitudes have seen pronounced trends in upper-atmosphere summer circulation and surface temperature extremes over recent decades. Several of these regional trends lie outside the range of historic CMIP6 model simulations, and they might constitute a joined dynamic response that is missed by climate models. Here, we examine if the regional trends in circulation are indeed part of a coherent circumglobal wave pattern. Using ERA5 reanalysis data and CMIP6 historical simulations, we find that the observed upper-atmospheric circulation trends consist of at least two separate regional signatures: a US-Atlantic and a Eurasian trend pattern. The circulation trend in these two regions can explain up to 30% of the observed regional temperature trends. The circulation trend in the CMIP6 multi-model-mean does not resemble the observed trend pattern and is much weaker overall. Some individual CMIP6 models do show a resemblance to the observed pattern in ERA5, although still weak. We show that the regional wave patterns in ERA5 resemble known teleconnection patterns, while CMIP6 models appear to lack these teleconnections. Our findings highlight the limitations of CMIP6 models in reproducing teleconnections and their associated regional imprint, creating uncertainty for regional climate projections on decadal to multi-decadal timescales.

How to cite: Happé, T., van Straaten, C., Hamed, R., D'Andrea, F., and Coumou, D.: Observed circulation trends in boreal summer linked to two spatially distinct teleconnection patterns, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15844, https://doi.org/10.5194/egusphere-egu25-15844, 2025.

The PDFs of daily mean 2m temperature (T2m) in observational data have been characterized using the first three moments. For identifying the role of dynamical processes, studies focussed on the midlatitudes have analyzed temperature variability at 850 hPa, which represents the free troposphere. The observed skew could not be reproduced by linear theory of advection ([1]), but was owed to the covariance between anomalous winds and anomalous temperature ([2], [3]). Recently, frameworks have also been developed for studying the roles of different processes in driving temperature tendencies in different percentiles of temperature ([3]). However, most of the studies involving advection consider a purely meridional mixing process. Given the dynamical links between meridional and vertical advection, it is unclear if this is sufficient. 

We turn focus to T2m, and consider 3D advection. We use the ERA5 reanalysis dataset to study the drivers of variability of T2m anomaly over the northwest Indian heatwave hotspot region during March and April, 1980-2022. We characterize the dry static energy (DSE) fluxes into this region, and develop a framework to identify quasilinear (QL) and nonlinear (NL) advective contributions to the temperature anomaly lifecycle. 

Daily change in T2m was highly correlated with daily advection of DSE into a 600-900 hPa box over the region. Leveraging the decision tree framework to identify the dominant weather patterns explaining different terciles of advected DSE, we found that the zonal mean flow and anomalous vertical flow ([1], [2]) acted to reverse the effect of the anomalous meridional flow. Using regression, we established that an additive combination of QL terms involving these flow components served as the dominant mechanism acting throughout the distribution of net advection, with r2 > 0.65. The rest of the variability was almost entirely explained by the sum of NL terms. We saw that the NL sum acts to saturate the growth of the QL sum in its tails, supporting the observations made by [2]. Net advection peaked before the peak of the QL sum due to such a relationship, restricting the growth of net advection. 

Furthermore, we study the patterns of advection in a phase space generated by the NL and QL terms. Regimes of advection were readily identified by identifying the NL terms dominating a particular region of the phase space. 

We show how interpretable machine learning algorithms, like decision tree and regression, can be used to identify dominant circulation patterns and provide a mapping between magnitude of advection and eddy configurations with respect to the region of interest. 

References 

[1] Schneider, T., T. Bischoff, and H. P lotka, 2015: Physics of Changes in Synoptic Midlatitude Temperature Variability J. Climate, 28, 2312–2331. 

[2] Garfinkel, C. I., and N. Harnik, 2017: The Non-Gaussianity and Spatial Asymmetry of Temperature Extremes Relative to the Storm Track: The Role of Horizontal Advection. J. Climate, 30, 445–464. 

[3] Tamarin-Brodsky, T., K. Hodges, B. J. Hoskins, and T. G. Shepherd, 2019: A Dynamical Perspective on Atmospheric Temperature Variability and Its Response to Climate Change. J. Climate, 32, 1707–1724.

 

How to cite: Shah, H. and Monteiro, J.: Composition and Regimes of Advection Driving the Temperature Anomaly Lifecycle in Northwest India: A Machine Learning Based Framework , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16295, https://doi.org/10.5194/egusphere-egu25-16295, 2025.

EGU25-16688 | ECS | Posters on site | AS1.27

Impacts of the Indian summer monsoon on the Antarctic climate and sea ice 

Qianghua Song, Chunzai Wang, Lei Zhang, and Hanjie Fan

In recent decades, Antarctica has experienced significant climate change, with previous studies predominantly focusing on the impact of oceanic multiscale variability on Antarctica, especially West Antarctica. However, our research reveals that Indian summer monsoon (ISM) rainfall significantly affects the austral winter (JuneAugust) Antarctic climate and sea ice through atmospheric teleconnection. The diabatic heating of ISM rainfall causes northward movement of the Hadley cell, triggering a Rossby wave train that propagates from the southern Indian Ocean into Antarctica, which changes sea level pressure and introduces warm advection to East and West Antarctica, causing widespread warming across the Antarctic continent. Under the influence of surface wind stress and temperature advection, the sea ice in the Ross Sea-Amundsen Sea exhibits a dipole distribution, characterized by an increase in the Ross Sea and a decrease in the Amundsen Sea. Our findings have significant implications for climate change research in Antarctica, particularly East Antarctica.

How to cite: Song, Q., Wang, C., Zhang, L., and Fan, H.: Impacts of the Indian summer monsoon on the Antarctic climate and sea ice, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16688, https://doi.org/10.5194/egusphere-egu25-16688, 2025.

EGU25-16723 | Posters on site | AS1.27

Trans-Arctic Influence on Far East Cold Waves: A Case Study of the 2020-2021 Events 

Takeshi Enomoto, Suzune Nomura, and Minori Fukushima

Two intense cold wave events impacted Japan between late December 2020 and early January 2021, motivating us to conduct a case study for the predictability of such high-impact weather. This study utilizes operational forecasts, a hybrid-machine learning weather model and ensemble adjoint sensitivity analysis to investigate the synoptic-scale mechanisms leading to these cold air outbreaks. We find that both events were preceded by distinctive cross-polar flows, which originated from cyclogenesis south of Greenland. These cyclonic systems generated cross-polar flows in addition to Rossby wave trains along the subpolar jet, efficiently transporting Arctic air masses towards the Far East. The second cold wave, occurring on January 8th, demonstrated a shorter predictability window, likely due to the weaker intensity and more compact spatial scale of the precursor storm than those of Storm Bella, highlighting the influence of storm characteristics on cold wave development and predictability. Both operational and machine learning models fail to predict from the state initialized on 28 December, implying an existence of predictability limit. Adjoint sensitivity analysis for the latter case reveals a coherent European (EU)-like pattern and a geopotential height anomaly off the east coast of Greenland two to four days prior to the spell. This study underscores the interconnectedness of storm track activity in the North Atlantic and North Pacific via the Arctic, demonstrating the influence of this trans-basin pathway on high-impact weather in East Asia. Our findings emphasize the crucial role of accurately representing these large-scale interactions for improving the predictability of extreme weather events.

How to cite: Enomoto, T., Nomura, S., and Fukushima, M.: Trans-Arctic Influence on Far East Cold Waves: A Case Study of the 2020-2021 Events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16723, https://doi.org/10.5194/egusphere-egu25-16723, 2025.

EGU25-19170 | ECS | Posters on site | AS1.27

Aspects of North Atlantic jet stream persistence and impacts on the surface weather in Europe 

Hugo Banderier, Alexandre Tuel, Tim Woollings, and Olivia Martius

Recent studies have highlighted the link between upper-level jet dynamics, especially the persistence of certain configurations, and extreme summer weather in Europe. Using our recently published toolbox for jet dynamics characterization, we use the various persistence metrics developed therein to find the most persistent episodes in recent data, as well as in a large ensemble containing future scenarios. We study precursors to these persistent episodes with potential for added predictability, as well as the surface weather extremes that can co-occur with these episodes.

First, we apply a jet axis detection and tracking algorithm in order to extract individual jets and classify them in the canonical categories of polar and subtropical jets. This allows us to measure the jets' instantaneous advection speed, as well as their lifetime, until they have weakened and cannot be extracted from the background wind anymore, or until they are advected out of the domain. These two metrics, advection speed and lifetime, provide measures of object persistence for each of the jets, that are, respectively, local and non-local in time.

Second, we apply the self-organizing map (SOM) clustering algorithm to the same data to create a distance-preserving, discrete, 2D phase space. The dynamics can then be described by the time series of visited SOM nodes, in which a long stay in a given node relates to a persistent state and a rapid transition between nodes that are far apart relates to a sudden dramatic shift in the configuration of upper-level flow. This allows us to quantify state persistence using the average length of a stay on a given SOM node.

Under these different views of persistence in the Euro-Atlantic sector, we establish certain jet properties as precursors for persistent episodes, study the role of Rossby wave breaking before and during these episodes, and explore the impacts of a persistent upper-level flow on surface weather and weather extremes in Europe.

How to cite: Banderier, H., Tuel, A., Woollings, T., and Martius, O.: Aspects of North Atlantic jet stream persistence and impacts on the surface weather in Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19170, https://doi.org/10.5194/egusphere-egu25-19170, 2025.

Few classes of weather events have more acute or dramatic impacts on Europe than extreme rainfall. In a warmer world, both thermodynamical and dynamical factors will interact to alter European rainfall; both its average and extreme characteristics, and at both seasonal-mean and synoptic timescales. Understanding these changes is societally vital and yet complex, as we are faced by the challenge that CMIP6 class models are not able to resolve rainfall directly. Meanwhile, kilometre scale simulations are either limited in geographical extent, simulation length or both, and have not yet been extensively validated from a physical perspective.  Indeed, developing a coherent, continent-wide perspective on the physics of rainfall is complicated by the fact that the dynamics of rainfall vary tremendously between seasons and between regions. As just a few examples of this dynamical richness, Atlantic Rossby wave packets favour downstream cyclogenesis in the lee of the Alps and so bringing storms to Italy and the Aegean, southern deflections of the wintertime jet stream can direct atmospheric rivers to Iberia — and cutoff-lows can bring the same region torrential rain in Summer. 
 
In this presentation we adopt a 'dynamics-first' approach to understanding rainfall in CMIP6-class climate models, focusing on their flow-dependent biases in rainfall in order to understand their errors and assess the physical plausibility of their projections. To practically handle the dynamical richness of Euro-Mediterranean rainfall dynamics we use a flow-precursor approach, developed for weather forecasting applications, in order to systematically identify the circulation patterns that drive extreme precipitation across Europe and reduce them to scalar metrics. By doing so, we are able to distill the multi-faceted synoptic dynamics into a manageable, low-dimensional space. Using this novel approach, we explore the potential of bias correcting climate model rainfall using dynamically-aware AI methods and, additionally, compare the calibrated results to those obtained from convection-permitting regional simulations carried out over the Alps.

How to cite: Dorrington, J.: A systematic exploration of the relationship between synoptic dynamics and Euro-Mediterranean extreme rainfall in a changing climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21020, https://doi.org/10.5194/egusphere-egu25-21020, 2025.

EGU25-1559 | ECS | Posters on site | AS1.28

Changing characteristics of Western Disturbances precipitation over Western Himalayas  

Pooja Pooja and Ashok Priyadarshan Dimri

The Indian subcontinent experiences winter precipitation (December, January, and February) due to Western Disturbances (WDs), which are synoptic scale weather systems embedded in subtropical westerly jets (SWJs) at upper tropospheric levels. For Himalayan rivers, WDs precipitation is crucial for hydrological budget as it causes heavy precipitation, flooding, and snowfall. The precipitation caused by WDs is beneficial for agricultural activities such as sowing of wheat crop, barley etc. WDs and NON-WDs precipitation are classified into active and break phase. Active and break peaks of WDs and NON-WDs are computed based on the maximum precipitation occurring in each WDs and NON-WDs days. This study, highlights the changes in precipitation climatology of active WDs and NON-WDs during 1987-2020 using hourly ERA5 reanalysis dataset. Various statistical techniques such as Theil-Sen slope test is used to calculate the trend and to investigate the decline in frequency of active WDs precipitation. Further, the structure, dynamics, and moisture availability associated with changing WDs and NON-WDs are also examined in this work.  It has been observed that some characteristics of WDs have changed in the recent decade due to climate change. This is associated with decrease in active WDs precipitation but the precipitation amount is increasing in the recent years. Active WDs precipitation pattern has primarily been shifted towards the months of January and February. The dynamics showed that active NON-WDs days derive moisture from Bay of Bengal region which is due to ‘Ω shape’ amalgamated structure and ‘∞ shape’ wind formation leading to precipitation forming mechanism over Western Himalayas. This study helps in insightful understanding of WDs and NON-WDs precipitation during the recent years which is necessary to improve headwater storage policies and meet agricultural demands.

How to cite: Pooja, P. and Dimri, A. P.: Changing characteristics of Western Disturbances precipitation over Western Himalayas , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1559, https://doi.org/10.5194/egusphere-egu25-1559, 2025.

EGU25-2146 | ECS | Posters on site | AS1.28

Is Europe becoming stormier? Extratropical cyclone clustering over the last century 

Zhi-Bo Li, Céline Heuzé, Jianing Song, and Deliang Chen

Extratropical cyclone clustering significantly impacts European weather extremes, such as heavy rainfall, strong winds, and flooding, often causing severe socio-economic consequences. Despite its importance, the long-term trends and variability of cyclone clustering remain poorly understood. In this work, we analyze the temporal and spatial evolution of extratropical cyclone clustering affecting Europe from 1940 to 2024, utilizing the high-resolution hourly ERA5 reanalysis dataset. This study provides unprecedented insights into century-scale changes in storminess and explores the underlying mechanisms driving these patterns. Our findings aim to enhance the understanding of extratropical cyclone behavior and their potential links to climate change, offering critical implications for risk assessment and adaptation strategies in Europe.

How to cite: Li, Z.-B., Heuzé, C., Song, J., and Chen, D.: Is Europe becoming stormier? Extratropical cyclone clustering over the last century, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2146, https://doi.org/10.5194/egusphere-egu25-2146, 2025.

EGU25-2792 | Orals | AS1.28

Asymmetric hysteresis response of mid-latitude storm tracks to CO2 removal 

seok-woo son, Jaeyoung Hwang, Chaim I. Garfinkel, Tim Woollings, Hyunsuk Yoon, Soon-Il An, Sang-Wook Yeh, Seung-Ki Min, Jong-Seong Kug, and Jongsoo Shin

In a warming climate, storm tracks are projected to intensify on their poleward side. Here we use large-ensemble CO2 ramp-up and ramp-down simulations to show that these changes are not reversed when CO2 concentrations are reduced. If CO2 is removed from the atmosphere following CO2 increase, the North Atlantic storm track keeps strengthening until the middle of the CO2 removal, while the recovery of the North Pacific storm track during ramp-down is stronger than its shift during ramp-up. By contrast, the Southern Hemisphere storm track weakens during ramp-down at a rate much faster than its strengthening in the warming period. Compared with the present climate, the Northern Hemisphere storm track becomes stronger and the Southern Hemisphere storm track becomes weaker at the end of CO2 removal. These hemispherically asymmetric storm-track responses are attributable to the weakened Atlantic meridional overturning circulation and the delayed cooling of the Southern Ocean.

How to cite: son, S., Hwang, J., Garfinkel, C. I., Woollings, T., Yoon, H., An, S.-I., Yeh, S.-W., Min, S.-K., Kug, J.-S., and Shin, J.: Asymmetric hysteresis response of mid-latitude storm tracks to CO2 removal, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2792, https://doi.org/10.5194/egusphere-egu25-2792, 2025.

The Tibetan Plateau (TP), known as the "Asian Water Tower," plays a crucial role in regional water resources, with summer storms contributing significantly to annual precipitation. However, the spatial structural changes of these storms remain understudied. This study analyzed satellite-retrieved precipitation data from 2001 to 2020 to investigate the changes in the spatial structure of summer storms over the TP and their underlying mechanisms. Results showed distinct regional differences: in the monsoon-dominated zone, reduced precipitation particularly at the storm center, led to a "dulling" of storm structures. In contrast, in the westerly-dominated and transition zones, a greater increase in precipitation was found at the center compared to other regions of storms, especially for extreme storms, resulted in a "sharpening" of storm structures. Ignoring the changes of spatial structural changes may overestimate the changes of storm-induced precipitation. Further analysis linked these changes to dynamic environmental factors, particularly stronger variations in vertical velocity near the storm center, driven by large-scale circulation changes around the TP.

How to cite: Jin, G. and Zou, L.: Spatial structural changes of summer storms over the Tibetan Plateau during 2001-2020 based on GPM IMERG data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2966, https://doi.org/10.5194/egusphere-egu25-2966, 2025.

EGU25-5700 | ECS | Orals | AS1.28

Cloud-radiative impact on the dynamics of extratropical cyclones during NAWDEX 

Behrooz Keshtgar, Aiko Voigt, and Corinna Hoose

Cloud-radiative heating (CRH) affects the dynamics of extratropical cyclones and near-tropopause circulations. Previous studies on the impact of CRH were mostly limited to simulations of idealized baroclinic life cycles. To bridge the gap between idealized studies and practical applications, we investigate the impact of CRH on the dynamics of North Atlantic cyclones. Using the ICOsahedral Nonhydrostatic (ICON) model, we simulate four cyclones during the North Atlantic Waveguide and Downstream Impact Experiment (NAWDEX) field campaign, and apply the Clouds On-Off Klimate model Intercomparison Experiment (COOKIE) method to compare simulations with and without CRH. We find that CRH systematically affects latent heating, vertical motion, and precipitation rates within the ascending regions of the cyclones, and that the impact of CRH is more prominent at upper levels. Furthermore, we investigate the impact of CRH on near-tropopause dynamics by diagnosing the evolution of differences in potential vorticity (PV). Consistent with idealized studies, CRH affects North Atlantic cyclones and PV near the tropopause mainly through changes in latent heating, and subsequently through changes in the divergent and rotational flows. Finally, we perform simulations with different ice optical parameterizations and radiation solvers. These simulations show that uncertainties in CRH can indeed affect the evolution of cyclones and PV near the tropopause. Our study highlights the importance of correctly simulating CRH for model predictions of extratropical cyclones.

How to cite: Keshtgar, B., Voigt, A., and Hoose, C.: Cloud-radiative impact on the dynamics of extratropical cyclones during NAWDEX, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5700, https://doi.org/10.5194/egusphere-egu25-5700, 2025.

EGU25-6430 | ECS | Posters on site | AS1.28

Is Europe under UNSEEN Risk of Cyclones of Tropical Origin? 

Kelvin S. Ng and Gregor C. Leckebusch

Traditionally, European windstorms – the costliest meteorological hazards in Europe, are associated with extratropical cyclones in winter. However, in recent years, unorthodox cyclones such as Ophelia (2017), Leslie (2018), and Kirk (2024) have had noticeable impacts on Europe during autumn. These cyclones, referred to as Cyclones of Tropical Origin (CTOs), form in tropical or subtropical regions and can migrate toward Europe during their lifecycle. Although CTOs do not always cause significant impacts, they can exhibit exceptional intensity, posing unique hazards distinct from typical extratropical cyclones.

This raises important questions: Are these isolated events? Will these events become more common in future climates? Current efforts to quantify the risk posed by CTOs are hindered by limited observational data and an incomplete theoretical understanding of these phenomena. As a result, Europe may face an unseen hazard from CTOs.

In this presentation, we analyse CTO events using a physically consistent UNSEEN event set constructed from twentieth-century seasonal hindcast outputs (CSF-20C and SEAS5-20C). Our results show that while CTOs are rare, they are not isolated. We examine the interdecadal variability of CTO impact potentials—including wind, rainfall, and compound hazards—and assess their impact probabilities during the twentieth century. Finally, we present preliminary findings that highlight the genuine and previously unseen risk posed by CTOs to Europe.

How to cite: Ng, K. S. and Leckebusch, G. C.: Is Europe under UNSEEN Risk of Cyclones of Tropical Origin?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6430, https://doi.org/10.5194/egusphere-egu25-6430, 2025.

EGU25-6685 | ECS | Orals | AS1.28

Forced trends and internal variability in projections of European windstorms associated with extratropical cyclones 

Matthew Priestley, David Stephenson, Adam Scaife, and Daniel Bannister

Climate change projections of windstorms associated with extratropical cyclones for Europe are highly uncertain. This is due to differences between models and large internal variability present. Furthermore, year-to-year variations are very high, and the different representations of the driving extratropical cyclones are large, resulting in any forced changes from a warming climate being hard to detect. Windstorms and the associated extratropical cyclones are objectively identified in 20 CMIP6 models, and then Generalized Linear Models and a weighted median estimation are used to extract forced trends for a number of storm impact metrics. Trends are assessed over time, but also as a function of global mean surface temperature changes. Trends in aggregate severity are attributed to changes in storm average severity, frequency, and area impacted, with changes in area being the dominant driver of changes to average storm severity. Using a large ensemble we find that trends between individual members can vary significantly, however the uncertainty due to internal variability is generally 2-3 times lower than model variability. With largest uncertainty coming from model differences, a large proportion of uncertainty in future windstorms is therefore potentially reducible with modelling advances.

How to cite: Priestley, M., Stephenson, D., Scaife, A., and Bannister, D.: Forced trends and internal variability in projections of European windstorms associated with extratropical cyclones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6685, https://doi.org/10.5194/egusphere-egu25-6685, 2025.

EGU25-9818 | ECS | Orals | AS1.28

CMIP6 Multi-model Assessment of Northeast Atlantic and German Bight Storm Activity 

Daniel Krieger and Ralf Weisse

We assess the evolution of Northeast Atlantic and German Bight storm activity in the CMIP6 multi-model ensemble, as well as the Max Planck Institute Grand Ensemble with CMIP6 forcing (MPI-GE), using historical forcing and three emission scenarios. We define storm activity as upper percentiles of geostrophic wind speeds, obtained from horizontal gradients of mean sea-level pressure. We detect robust downward trends for Northeast Atlantic storm activity in all scenarios, and weaker but still downward trends for German Bight storm activity. In both the multi-model ensemble and the MPI-GE, we find a projected increase in the frequency of westerly winds over the Northeast Atlantic and northwesterly winds over the German Bight, and a decrease in the frequency of easterly and southerly winds over the respective regions. We also show that despite the projected increase in the frequency of wind directions associated with increased cyclonic activity, the upper percentiles of wind speeds from these directions decrease, leading to lower overall storm activity. Lastly, we detect that the change in wind speeds strongly depends on the region and percentile considered, and that the most extreme storms may become stronger or more likely in the German Bight in a future climate despite reduced overall storm activity.

How to cite: Krieger, D. and Weisse, R.: CMIP6 Multi-model Assessment of Northeast Atlantic and German Bight Storm Activity, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9818, https://doi.org/10.5194/egusphere-egu25-9818, 2025.

EGU25-10092 | ECS | Orals | AS1.28

Intensity-based classification of North Atlantic and European extratropical cyclones 

Joona Cornér, Clément Bouvier, Benjamin Doiteau, Florian Pantillon, and Victoria A. Sinclair

Most of the day-to-day variability in weather in Europe, including damaging events, is caused by extratropical cyclones (ETCs). ETCs are very different from one another and to more easily study their development, intensity, and structure, various ETC classification schemes have been proposed. Here, we propose an intensity-based scheme in which we first identify necessary ETC intensity measures to describe ETC intensity comprehensively from both dynamical and impact-relevant perspective, and then use them to produce an ETC classification.

ERA5 reanalysis data from 1979 to 2022 was used to track ETCs and compute their intensity measures in the extended winter season (October-March). A total of 7361 ETC tracks were identified in the North Atlantic and Europe. Eleven intensity measures were analysed including 850-hPa relative vorticity, mean sea level pressure, wind speeds at various levels, wind gust, wind footprint, precipitation, and storm severity index. Among the 11 intensity measures, relevant ones were identified by analysing their correlation with each other combined with a sparse principal component analysis (sPCA). The selected measures were used to classify the ETCs by performing a cluster analysis with Gaussian mixture modelling.

Based on the sPCA and relationships between the intensity measures, the set was reduced to 5 measures: 850-hPa relative vorticity, 850-hPa wind speed, wind footprint, precipitation, and storm severity index. Therefore, to describe ETC intensity comprehensively, one needs to use more than one or two intensity measures. The cluster analysis with these 5 measures as input produced 4 discernible clusters. Between these clusters ETCs differed in terms of their intensity, life cycle characteristics, and geographical location. Despite only 9 % of all ETCs belonging to the most intense cluster, it contained 17 out of 21 investigated impactful named storms, which demonstrates the relevance of the classification and its ability to identify potentially impactful ETCs.

How to cite: Cornér, J., Bouvier, C., Doiteau, B., Pantillon, F., and Sinclair, V. A.: Intensity-based classification of North Atlantic and European extratropical cyclones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10092, https://doi.org/10.5194/egusphere-egu25-10092, 2025.

EGU25-10733 | Posters on site | AS1.28

Multi-model assessment of hazard uncertainties in a European windstorm NatCat model 

Hugo Rakotoarimanga, Rémi Meynadier, Gabriele Messori, and Joaquim G. Pinto

Extra-tropical winter storms are one of the most impactful natural hazards for the European insurance market causing large socio-economic damages.

AXA has been developing stochastic natural hazard models (also called natural catastrophe models) to quantify the impact of such events on its portfolios, including European extra-tropical cyclones. However, the correct representation of windspeeds and their spatial distribution across Europe during a storm is crucial to determine the risk posed by an event. The characterization of uncertainties in natural catastrophe models stemming from the hazard data used and its resolution is crucial to understand their limitations and guide decision-making.

We rely on a novel publicly available dataset of 50 extreme European windstorms for the period 1995–2015 (Flynn et al., 2024; doi:10.5194/essd-2024-298) with wind gust footprints derived consistently from four different datasets with different horizontal resolutions. Risk being a function of hazard, vulnerability and exposure, we set constant vulnerability and portfolio, and we quantify the range of uncertainties in the reproduction of historical insured losses stemming from the sole hazard component. We compare the losses derived from AXA’s model to the range of losses derived from this novel extreme windstorms dataset.

How to cite: Rakotoarimanga, H., Meynadier, R., Messori, G., and Pinto, J. G.: Multi-model assessment of hazard uncertainties in a European windstorm NatCat model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10733, https://doi.org/10.5194/egusphere-egu25-10733, 2025.

EGU25-14002 | ECS | Orals | AS1.28

Resolution-Dependent Impact of Extratropical Cyclones on Winter U.S. Precipitation Bias in the GFDL SPEAR Model 

Jaeyeon Lee, Xiaosong Yang, and Edmund Chang

Extratropical cyclones (ETCs) are the primary drivers of winter precipitation across the United States, accounting for up to 85% of total precipitation. This study uses the GFDL SPEAR models at atmospheric resolutions of 100 km, 50 km, and 25 km to examine how ETC dynamics impact precipitation patterns and biases across the United States. Higher-resolution models reduce ETC-related precipitation biases in the Southwest and Midwest but increase biases in coastal regions, including the West Coast and the Eastern United States. To understand these biases, we decompose ETC-related precipitation biases into those driven by precipitation frequency and intensity. Coastal precipitation biases are mainly due to overestimations of both the occurrence and intensity of precipitation, which are related to ETC frequency and intensity, respectively. In inland areas, biases are largely driven by occurrence bias associated with ETC frequency. Notably, higher-resolution models simulate amplified ETC frequency and intensity biases in coastal regions, while showing a decrease in ETC frequency bias in inland regions. This increase is especially linked to the overestimation of small-scale ETCs, which considerably inflate frequency-driven precipitation bias. Additionally, improvements in AMIP runs suggest that these biases are partly connected to SST bias. These findings emphasize the sensitivity of precipitation representation to ETC dynamics and underscore the importance of addressing resolution-dependent and SST related biases to improve midlatitude precipitation simulations in climate models.

How to cite: Lee, J., Yang, X., and Chang, E.: Resolution-Dependent Impact of Extratropical Cyclones on Winter U.S. Precipitation Bias in the GFDL SPEAR Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14002, https://doi.org/10.5194/egusphere-egu25-14002, 2025.

EGU25-14515 | Orals | AS1.28

Warm core intensification of a Tasman Sea cyclone linked to Coral Sea sea-surface temperatures. 

Christopher Chambers, Yi Huang, and Dale Roberts

In early June 2016 a large rainband with an embedded subtropical cyclone, associated with a deep upper-level trough, brought extensive heavy rainfall along Australia’s east coast, from southern Queensland to Tasmania. In the lead-up to this event, sea-surface temperatures (SSTs) in the Coral and Tasman Seas were the warmest on record for the time of year. 
To investigate how the anomalously high SST, and its distribution, influenced the development of the cyclone, a high-resolution configuration of the Australian Community Climate and Earth System Simulator (ACCESS) over Australia, known as AUS2200, has been run under different SST scenarios. All simulations were run from 0000 UTC 3 June to 0000 UTC 8 June 2016, and use ERA5 data for the SST calculations.
A more intense subtropical cyclone develops off the New South Wales (NSW) coast in two simulations run with observed SST — one with fixed initial SST (Control) and the other with daily evolving SST (Evolving) — compared with a simulation using 3 June climatological SST (Climatology). The cyclone also stalls longer near the NSW coast in the observed SST runs.
Two additional simulations examine the role of the East Australian Current in the Tasman Sea. One smooths a prominent warm eddy (Smooth), and another replaces the Tasman Sea SST with climatological values (Tasclim). Both simulations retain the cyclone intensification seen in Control. A final simulation that replaces the Coral Sea SST with climatological values (Corclim) produces a weaker cyclone similar to Climatology.
Taken together, the results indicate that the anomalously warm Coral Sea SSTs were more important for the cyclone intensification than those of the Tasman Sea even though the greatest intensification occurred over the Tasman Sea. The greater cyclone intensity and slower southward movement over the Tasman Sea resulted in stronger and more prolonged onshore winds along the southern NSW coast, increasing the potential for coastal damage.
The greater intensity of the subtropical cyclone seen in Control, Evolving, Smooth, and Tasclim is associated with the formation of a warmer deep-tropospheric storm core than seen in Climatology and Corclim. This is linked to a greater reservoir of deep-tropospheric warm air that develops when using observed SST over the Coral Sea. These findings highlight the critical role of the Coral Sea’s warm SST as a driver of the cyclone’s development and intensification.

How to cite: Chambers, C., Huang, Y., and Roberts, D.: Warm core intensification of a Tasman Sea cyclone linked to Coral Sea sea-surface temperatures., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14515, https://doi.org/10.5194/egusphere-egu25-14515, 2025.

EGU25-15033 | Posters on site | AS1.28

Explicit risk modelling of sting-jet extratropical cyclones.  

Emmanouil Flaounas, Remi Meynadier, Hugo Rakotoarimanga, Anyssa Diouf, and Rudy Mustafa

Extratropical cyclones (ETCs) are a major hazard for Europe as they cause most of the windstorms and floods in the mid-latitudes, resulting in high economic and social costs.

Sting jets (SJ) are responsible for windstorm damages well ahead the cyclone center. In this study we employ dedicated diagnostics and modeling approaches that identify -along with cyclone tracks- the spatial extent where actual impacts take place. The fine scales of processes involved in SJ generation demand exceptionally high spatial resolutions and dense vertical levels in model simulations (Rivière et al. 2020).

In this study we use the WRF model to simulate 143 historical ETC from 1980 to 2018 that potentially involve SJs. The model simulations use two domains: one parent domain that encompasses the whole cyclone track at a resolution of about 15 km, and another, square-sized domain with each side measuring 1300 km. The nested domain always follows the ETC centers, aiming to resolve explicitly the development of SJs. SJ detection has been achieved through lagrangian modeling, by identifying airstreams that sharply descend ahead of the cloud head and behind the cold front of the cyclones. Historical ETC footprints from ERA-5 and WRF physical downscaling of ERA-5 in convection-permitting resolutions are then used to assess the impact in term of financial losses of an explicit simulation of sting-jets processes.

How to cite: Flaounas, E., Meynadier, R., Rakotoarimanga, H., Diouf, A., and Mustafa, R.: Explicit risk modelling of sting-jet extratropical cyclones. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15033, https://doi.org/10.5194/egusphere-egu25-15033, 2025.

Atmospheric bomb cyclones that form off the United States east coast are high impact, complex weather systems. Many ingredients must come together to produce a storm of this magnitude. In recent years, high-resolution studies have indicated that one such critical ingredient is fine-scale Gulf Stream sea-surface temperature (SST) variability. However, studies still lack consensus on which particular aspect of the variability is most critical (e.g. absolute SST vs. the SST gradient, pre-conditioning vs. direct influence). Through novel high-resolution simulations in Community Earth System Model 2 (CESM2), this study attempts to isolate the influence of the fine-scale SST gradient specifically, motivated by the impact fine-scale heat flux gradients are expected to have on lower-level frontogenesis and subsequent cyclone development. Through targeted fine-scale SST gradient perturbations, the results illustrate how preexisting SST gradients can impact the frequency and intensity of bomb cyclones and may offer useful information regarding seasonal forecasting of these systems.

How to cite: Hair, J., Parfitt, R., Wills, R., and Müller, J.: Investigating the Impact of Fine-Scale Gulf Stream SST Gradients on the Development of Bomb Cyclones in the Community Earth System Model 2, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15631, https://doi.org/10.5194/egusphere-egu25-15631, 2025.

EGU25-15755 | Posters on site | AS1.28

Assessment of the origin of moisture for the precipitation of North-Atlantic extratropical cyclones 

Raquel Nieto, Patricia Coll-Hidalgo, José Carlos Fernández-Alvarez, and Luis Gimeno

This study uses high-resolution simulations and Lagrangian diagnostics to identify the sources of moisture contributing to precipitation at the deepest stage of extratropical cyclones (ECs) over the North Atlantic (NATL). Precipitation was associated with target regions defined by a radius, warm conveyor belt (WCB) footprint, and square root spiral contours centred on the cyclone. The NATL region was divided into sectors for detailed analysis. In the northern North Atlantic (NNATL), moisture sources extend westward across the ocean. Subtropical moisture supports precipitation in non-central areas of ECs, which intensify over the central and western NNATL. The moisture uptake patterns of ECs in the higher latitudes of the western North Atlantic (WNATL) are similar to those in the NNATL, with southwestward extension and moisture uptake from the eastern American coast. For ECs in the lower latitudes of the WNATL, moisture uptake is more symmetric around the cyclone centre, with major contributions from the Caribbean and limited moisture flow from the Gulf of Mexico due to migrating anticyclones. For ECs in the eastern NATL, moisture comes from the surrounding ocean. Overall, 75% of the moisture gain occurs below 600 hPa, with a significant concentration observed around 800 hPa. Continental mass influence is observed for ECs deepening near the coasts of East America and Western Europe. ECs at higher latitudes in the WNATL and NNATL exhibit extensive synoptic-scale disturbances, with moisture sources for WCB and spiral precipitation extending 3,000 to 4,000 km southwest of their centres. The most intense moisture uptake occurs over the WNATL, particularly for lower latitude ECs.

How to cite: Nieto, R., Coll-Hidalgo, P., Fernández-Alvarez, J. C., and Gimeno, L.: Assessment of the origin of moisture for the precipitation of North-Atlantic extratropical cyclones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15755, https://doi.org/10.5194/egusphere-egu25-15755, 2025.

We propose the first unified objective framework (SyCLoPS) for detecting and classifying all types of low-pressure systems (LPSs) in a given data set. We use the state-of-the-art automated feature tracking software TempestExtremes (TE) to detect and track LPS features globally in ERA5 and compute 16 parameters from commonly found atmospheric variables for classification. A Python classifier is implemented to classify all LPSs at once. The framework assigns 16 different labels (classes) to each LPS data point and designates four different types of high-impact LPS tracks, including tracks of tropical cyclone (TC), monsoonal system, and tropical-like cyclones (subtropical storm and polar low). The framework thus provides the first global tropical-like cyclones (TLC) detection scheme by detecting similar physical features to TCs among non-tropical system candidates and optimizing detection thresholds against subjective data sets. The vertical cross section composite of the four types of high-impact LPS we detect each shows distinct structural characteristics. 

The classification process involves disentangling high-altitude and drier LPSs, differentiating tropical and non-tropical LPSs using novel criteria, and optimizing for the detection of the four types of high-impact LPS. A comparison of our labels with those in the International Best Track Archive for Climate Stewardship (IBTrACS) revealed an overall accuracy of 95% in distinguishing between tropical systems, extratropical cyclones, and disturbances, and a median error of 6 hours in determining extratropical transition completion time. We demonstrate that the SyCLoPS framework is valuable for investigating various aspects of mid-latitude storms and post-TCs in climate data, such as the evolution of a single storm track at every stage, patterns of storm frequencies, and precipitation or wind influence associated with impactful mid-latitude storms.

How to cite: Han, Y. and Ullrich, P.: The System for Classification of Low-Pressure Systems (SyCLoPS): An All-In-One Objective Framework for Large-Scale Data Sets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15800, https://doi.org/10.5194/egusphere-egu25-15800, 2025.

EGU25-16278 | Orals | AS1.28

Enhanced C3S Windstorm Service: A Novel Dataset of European Extratropical Cyclone Windstorms Based on ERA5 Reanalysis 

Lorenzo Sangelantoni, Stefano Tibaldi, Leone Cavicchia, Enrico Scoccimarro, Pier Luigi Vidale, Kevin Hodges, Vivien Mavel, Mattia Almansi, Chiara Cagnazzo, and Samuel Almond

Extratropical cyclones (ETCs) are dominant meteorological structures playing a crucial role in midlatitudes climate. ETCs are also responsible for heavy precipitation events, strong surface winds and wind gusts exposing populations to hazards and causing widespread and significant damages. The response of ETCs to a warming atmosphere is characterized by substantial uncertainty. This arises primarily from two key factors: significant inter-annual variability, which complicates trend detection, and the interplay of non-linear and potentially compensating mechanisms, which render future changes in the ETC climate challenging to evaluate, understand and predict. Additionally, North Atlantic ETC trend evaluation and understanding crucially depend on methodological analysis choices regarding datasets (e.g., observations, reanalysis, proxies, model simulations and analysis period) and approaches to examine storm features (i.e., Eulerian vs. Lagrangian).

Here, we present and preliminarily evaluate a novel dataset of European windstorms associated with ETCs based on the whole ERA5 reanalysis period (1940-present). This dataset is produced within the Copernicus Climate Change Service (C3S) Enhanced Operational Windstorm Service (EWS), to promote a knowledge-based assessment of the nature and temporal evolution of European windstorms associated with ETC. Such a dataset is primarily thought to provide high-quality, standardized data on windstorms which support various industrial sectors, particularly insurance and risk management, by offering insights into the intensity, frequency, vulnerability and impact of windstorms. EWS includes two datasets: windstorm tracks, based on two tracking algorithms (TRACK and TempestExtremes), and windstorm footprints, produced considering both original-resolution ERA5 variables and statistically downscaled ERA5 variables, with a target grid at 1 km resolution.

A preliminary analysis of the datasets shows increasing trends of cold-semester windstorm frequency and of the associated footprint magnitude over a portion of the European territory. The choice of the tracking algorithm is shown to be an important factor in the analysis process, as it results in non-negligible uncertainties in main windstorm statistics.

 

How to cite: Sangelantoni, L., Tibaldi, S., Cavicchia, L., Scoccimarro, E., Vidale, P. L., Hodges, K., Mavel, V., Almansi, M., Cagnazzo, C., and Almond, S.: Enhanced C3S Windstorm Service: A Novel Dataset of European Extratropical Cyclone Windstorms Based on ERA5 Reanalysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16278, https://doi.org/10.5194/egusphere-egu25-16278, 2025.

EGU25-17891 | ECS | Posters on site | AS1.28

Temporal clustering of severe European winter windstorms on intra-seasonal timescales and the explanatory power of large-scale modes 

Sophie Feltz, Kelvin Ng, Christopher Allen, Tim Kruschke, Michael Angus, Andrew Quinn, and Gregor C. Leckebusch

When severe European winter windstorms cluster in time, socioeconomic impacts and losses are magnified. Yet, the behaviour and drivers on shorter, intra-seasonal timescales have not been fully investigated. The impact-relevant footprint of the storm system is identified using the wind-based impact-oriented tracking algorithm WiTRACK (Leckebusch et al., 2008), for the core winter seasons (DJF) 1980/01-2022/23 from ERA5 reanalysis. Derived from a Poisson Process, we quantify the magnitude of clustering through the widely established dispersion statistic (Mailier et al., 2006). On fixed 45- and 30-day timescales, the spatial distribution of the dispersion statistic has been analysed. The time-development of the dispersion statistic on shorter time horizons is investigated through 21-, 15- and 11-day moving windows. Preliminary results reveal an increase in clustering in the latter half of the winter season on the fixed 45- and 30-day timescales. Shorter time horizons reveal clear peaks at the middle and the end of the season.

To analyse mechanisms that drive the defined intra-seasonal behaviour on the shorter time horizons (<30 -days), we examined the roles of several large-scale variability modes, namely the North Atlantic Oscillation (NAO), the East Atlantic pattern (EA), and the Scandinavian pattern (SCA). Results reveal a correlation between intra-seasonal variability of clustering and the occurrence of such large-scale modes, suggesting the EA as a key driver for increasing clustering. In addition, the individual contributions of large-scale modes to clustering at different times of the season can be diagnosed.

How to cite: Feltz, S., Ng, K., Allen, C., Kruschke, T., Angus, M., Quinn, A., and Leckebusch, G. C.: Temporal clustering of severe European winter windstorms on intra-seasonal timescales and the explanatory power of large-scale modes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17891, https://doi.org/10.5194/egusphere-egu25-17891, 2025.

In this study, the interdecadal variation of extreme precipitation in May over southwestern Xinjiang (SWX) and related mechanisms were investigated. The extreme precipitation in May over SWX exhibited a decadal shift in the 1990s (negative phase during 1970–86 and positive phase during 2003–2018). The decadal shift corresponded to strengthened moist airflow from the Indian Ocean and an anomalous cyclone over SWX during 2003–2018. It is found that the interdecadal change of the wave trains in Eurasia might account for the differences in atmospheric circulation between the above two periods. Further analyses reveal that spring snow cover over Eurasia is closely linked to extreme precipitation over SWX during 2003–2018. Increased snow cover in western Europe (WE) from February to March is accompanied by more snowmelt. This resulted in less local snow cover and lower albedo which lead to warm temperature over WE in May. The changes in temperatures increase the local 1000–500-hPa thickness over WE. These factors provide favorable conditions for the enhancement of the Eurasian wave trains which significantly influence extreme precipitation over SWX. On the other hand, corresponding to decreased albedo caused by the reduction of northern Eurasia (NE) snow cover in May, anomalous surface warming occurs over NE. The anomalous warming result in positive geopotential height anomalies which intensifies the meridional geopotential height gradient over Eurasia and causes an acceleration of the westerly jet in May. Anomalous upper-level divergence in SWX induced by the enhanced westerly jet provides a favorable dynamical condition for increased extreme precipitation.

How to cite: Chen, P. and Li, W.: Increased extreme precipitation in May over southwestern Xinjiang in relation to Eurasian snow cover in recent years, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-58, https://doi.org/10.5194/egusphere-egu25-58, 2025.

Droughts in Western Central Europe (WCE) have recently attracted attention due to their detrimental impact on crops, ecosystems, and society, as evidenced by events in 2018 and 2022. In this region, however, their variability and underlying causes remain unclear. This study aims to associate droughts with the atmospheric circulation to gain insight into their drivers. We employed reanalysis datasets (ERA5, 20CRv3, and ModE-RA) to identify meteorological drought events using the Standardized Precipitation Evapotranspiration Index at a 3-month scale and consistently connect them to atmospheric circulation patterns through k-means clustering. The three datasets are evaluated over the WCE regions, showing that they are highly reliable over periods ranging from 70 to 180 years, providing a long perspective on the recent events. Firstly, we demonstrate that droughts in WCE display a strong multidecadal variability with no significant long-term trend. Although precipitation has increased over time, this has been offset by the rising atmospheric evaporative demand due to warming. Secondly, we identify three distinct atmospheric circulation patterns associated with drought events in WCE: a high-anomaly geopotential height centred over Western Central Europe (WCE+); a dipole of high-anomaly geopotential height over the British Isles and low-anomaly geopotential height over the Maghreb (BIM+); and the negative phase of the North Atlantic Oscillation (NAO-), predominantly in winter. Our analysis shows that droughts have become increasingly associated with WCE+ over the last century, while their association with NAO- has decreased over the past 180 years. This research provides a regional historical analysis of meteorological drought and its drivers, offering better insight into long-term regional climate change.

How to cite: Neimry, E., Goosse, H., and Jonard, M.: Connecting Drought Events with Atmospheric Circulation Patterns in Western Central Europe: A Historical Perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-478, https://doi.org/10.5194/egusphere-egu25-478, 2025.

EGU25-592 | ECS | Orals | CL3.1.1

Asymmetric response of Atlantic Nino on heatwaves over Northern India 

Ganaraj Dalal, Vittal Hari, and Shushobhit Chaudhary

Due to global warming, climate extremes like heatwave events will rise further in the 21st century. Earlier, heatwave characteristics like duration, intensity, and frequency have been studied independently, ignoring interdependence among them, leading to biases in the heatwave impact assessment. The heatwave intensity duration frequency(HIDF) model provides a feasible framework incorporating interdependencies among heatwave characteristics, helping quantify heatwave hazards more accurately. HIDF curves are produced for six metropolitan cities, namely, Ahmedabad, Bhopal, and Gwalior over the western part and Patna, Varanasi, and Deoghar over the eastern part of northern India using the Indian Meteorological Department daily maximum temperature from 1961-2023 for March-June months. Heatwave events of durations ranging from one to ten and their respective intensities are modeled using the nonparametric kernel distribution method. HIDF curves reveal that the intensity and frequency of heatwave events for each duration increased(decreased) in the western(eastern) cities. In Ahmedabad city, the likelihood of a six-day heatwave event increased by 59 %, whereas it decreased by 66 % over Patna, reflecting east-west asymmetry. We found that a positive anomaly pattern over the southern Atlantic Ocean, i.e., Atlantic Nino, influences heatwaves occurring over northern India, causing east-west asymmetry. Due to the Atlantic Nino, the cross-equatorial flow reversed its direction as the moisture from the northern Indian Ocean, instead of traveling towards north China, entered the eastern part of India. This resulted in entry of moisture laden winds from the Bay of Bengal and it contributed to more convection activity in northeast India causing temperature drop in the region. The strength of moisture-laden winds is reduced when they reach the western part; the chance of convection decreases, contributing to a rise in temperature. Our results provide significant inputs in understanding heatwave dynamics over northern India, which will be helpful in predicting the heatwaves more accurately in the future.

 

How to cite: Dalal, G., Hari, V., and Chaudhary, S.: Asymmetric response of Atlantic Nino on heatwaves over Northern India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-592, https://doi.org/10.5194/egusphere-egu25-592, 2025.

EGU25-1557 | ECS | Orals | CL3.1.1

Linking European droughts to year-round weather regimes 

Onaïa Savary, Constantin Ardilouze, and Julien Cattiaux

Droughts are extreme events with major economic, social and environmental impacts, and it is crucial to be able to anticipate them.  To improve their prediction on a seasonal timescale, it is essential to better understand the underlying conditions that precede them. In  Europe, intra-seasonal to seasonal climatic variations are linked to atmospheric circulation and are weakly constrained by tropical teleconnections.

This study employs year-round weather regimes to demonstrate that the North Atlantic atmospheric circulation plays a fundamental role in precipitation deficits across Europe. Precipitation deficits are quantified using the reanalysed 3-month standardised precipitation index (SPI3). We use the SPI3 to define drought events and propose a new regionalisation of Europe, divided into regions with the same drought-related characteristics. We demonstrate that each weather regime is associated with a distinct precipitation pattern across regions, that remains relatively stable throughout the year. The representation of the regime-drought relationship in CMIP6 model simulations is then discussed.

How to cite: Savary, O., Ardilouze, C., and Cattiaux, J.: Linking European droughts to year-round weather regimes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1557, https://doi.org/10.5194/egusphere-egu25-1557, 2025.

Under global warming, the occurrence of compound extreme weather and climate events has increased, resulting in profound ecological and societal damages. Understanding the forming mechanisms of these events is imperative for formulating effective mitigation and adaptation strategies. This research focuses on causality of the compound extreme heat and precipitation events (CEHPEs) in northeastern China. From 1961 to 2018, a total of 55 heatwave events occurred in this region, with 18 identified as the CEHPEs.

The formation of CEHPEs in northeastern China is closely related to the southeastward propagating quasi-barotropic anomalous anticyclone. As the center of the anomalous anticyclone approaches northeastern China, the associated descent reduces the cloud cover and increases downward shortwave radiation. The thus-heated ground increases the upward longwave radiation and sensible heat, predominantly warming the surface air and causing the heatwave. During the development of the heatwave, the increased lower-level moisture due to the enhanced surface evaporation and the increased column moist static energy due to the warming air temperature destabilize the atmosphere. When the anomalous anticyclone moves out of northeastern China after the heatwave, intense convection rapidly develops, resulting in extreme precipitation and completing the CEHPEs.

Comparison between the CEHPEs and the mere heatwave events is also conducted. The major difference resides in the zonal scale of the anomalous anticyclone. In the CEHPEs, the anomalous anticyclone has a small zonal scale and decays locally due to the advection by the climatological westerly acting on the zonal gradient of anomalous vorticity. In contrast, the zonal scale of the anomalous anticyclone in the mere heatwave events is much larger, which slowers the decaying due to the weaker zonal advection and thus impedes the convection development and extreme precipitation.

How to cite: Yang, Y.: Causality of Compound Extreme Heat-Precipitation Events in Northeastern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1872, https://doi.org/10.5194/egusphere-egu25-1872, 2025.

EGU25-2403 | Orals | CL3.1.1

Linking extreme precipitation during June in central eastern China to the East Asian jet stream changes 

Renguang Wu, Peijun Zhu, Ping He, and Wen-Jun Zhang

Extreme precipitation occurs under specific atmospheric circulation patterns. In this talk, we show the connection of extreme precipitation in central eastern China to the East Asian jet stream changes during June, the month with frequent occurrence of extreme precipitation. Two types of distinct East Asian jet stream configurations are detected for the occurrence of extreme precipitation. One is a latitudinal shift of the East Asian jet stream and the other is an intensification of the East Asian jet stream. The former corresponds to extreme precipitation to south of the Yangtze River and the latter corresponds to extreme precipitation along the Yangtze River. The changes in the location and intensity of the East Asian jet stream are associated with meridional wave patterns along East Asia and zonal wave patterns over mid-latitude Eurasia. The role of the western North Pacific subtropical high is robust but relatively larger for extreme precipitation south of the Yangtze River. The South Asian high plays an important role for extreme precipitation south of the Yangtze River, but its role is weak for extreme precipitation along the Yangtze River. Wind-induced temperature anomalies modulate the vertical change of the meridional height gradient over eastern China and thus contributes to the latitudinal shift and intensity change of the East Asian jet stream.

How to cite: Wu, R., Zhu, P., He, P., and Zhang, W.-J.: Linking extreme precipitation during June in central eastern China to the East Asian jet stream changes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2403, https://doi.org/10.5194/egusphere-egu25-2403, 2025.

With the significant warming, Central Asia (CA) has suffered from frequent drought events and vegetation degradation. However, whether it is the large-scale circulation dynamics or the surface local thermal mechanism that plays the dominant role in the drought remains unknown. Here we used 3-month Standardized Precipitation Evaporation Index in August to identify the summer drought events for 1980-2022 and conducted a composite analysis. Results indicate that the drought related wave train, originating from mid-high latitude North Atlantic (NA), has a barotropic vertical structure and propagates eastward, featuring a positive geopotential height center in CA. The pronounced warm sea surface temperature (SST) over the middle-latitude NA and cold SST over the high-latitude NA contribute to the Rossby wave formation, which is verified by an analysis of the apparent vorticity anomaly and linear baroclinic model experiments. The anticyclone anomaly over CA, corresponding to strong vertical subsidence, enhances downward shortwave radiation and surface sensible heat flux, while significantly reducing surface latent heat flux. The maintenance of drought is usually associated with persistent precipitation deficits. By using the backward moisture tracking model, we further found that the recycled precipitation, induced by the local evapotranspiration, contributes to the 88.39% reduction of total precipitation during drought periods, whereas the inflow of external advected moisture shows no significant decrease. The above results highlight the dominated role of local land-atmosphere interactions responsible for the drought through reduced local evapotranspiration, with large-scale circulation anomalies providing a conducive background for the drought.

How to cite: Ren, Y. and Yu, H.: Impact of Mid-high Latitude Circulation and Surface Thermal Forcing on Drought Events in Central Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2533, https://doi.org/10.5194/egusphere-egu25-2533, 2025.

EGU25-2668 | Orals | CL3.1.1

The Impact of the Madden-Julian Oscillation on Spring and Autumn Afternoon Diurnal Convection in Sri Lanka 

Wan-Ru Huang, Suranjith Bandara Koralegedara, Tzu-Yang Chiang, Cheng-An Lee, Po-Han Tung, Yu-Tang Chien, and Liping Deng

This study examines how the Madden-Julian Oscillation (MJO) phases affect afternoon diurnal convection (ADC) patterns in Sri Lanka during 2001-2020. Sri Lanka experiences the highest frequency of ADC events in the Indian subcontinent region while located in a pivotal position within the propagation pathway of the MJO. To address the research gap regarding the MJO’s impact on seasonal diurnal rainfall in Sri Lanka, we analyze both the spring and autumn seasons, which are the two seasons with greater diurnal rainfall variability, focusing on strong MJO phases (P1-P8). Our findings show that daily rainfall increases during the P2-to-P3 phases and decreases during the P6-to-P7 phases in both seasons. The diurnal rainfall patterns, however, show seasonal differences. In spring, the diurnal rainfall amplitude peaks during P2-to-P3 phases, while in autumn, it peaks during P8-to-P1 phases. ADC events are more frequent and intense during these respective phases. The MJO's effect on both diurnal rainfall amplitude and ADC events is stronger in autumn compared to spring. During active MJO phases, we observe enhanced westward propagation of diurnal rainfall linked to ADC events, driven by moisture convergence and increased upward motion. The combination of mid-to-upper level easterly winds and deep convection over Sri Lanka leads to more distinct westward propagation during P2-to-P3 phases in spring and P8-to-P1 phases in autumn. These findings enhance our understanding of how the MJO influences local rainfall patterns and can aid in improving regional weather forecasting.

How to cite: Huang, W.-R., Koralegedara, S. B., Chiang, T.-Y., Lee, C.-A., Tung, P.-H., Chien, Y.-T., and Deng, L.: The Impact of the Madden-Julian Oscillation on Spring and Autumn Afternoon Diurnal Convection in Sri Lanka, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2668, https://doi.org/10.5194/egusphere-egu25-2668, 2025.

EGU25-3062 | ECS | Orals | CL3.1.1

Quantifying Relative Contributions of Three Tropical Oceans to the Western North Pacific Anomalous Anticyclone 

Zhiyuan Lu, Lu Dong, Fengfei Song, Bo Wu, Shuyan Wu, and Chunzai Wang

The western North Pacific anomalous anticyclone (WNPAC) often exists during the mature and decaying phases of El Niño, significantly affecting the East Asian summer monsoon. Previous studies have revealed the importance of the Indian, Pacific, and Atlantic Oceans in generating and maintaining the WNPAC. However, a quantitative comparison of the contributions from these three oceans is still lacking. This study uses pacemaker experiments with a state-of-the-art model to quantify the relative contributions of the three tropical oceans to the interannual WNPAC variability. We find that the Pacific accounts for over 50% of the interannual variance in boreal winter and the following spring, while the roles of the Atlantic and Indian Oceans become more pronounced in spring. In summer, all three oceans contribute significantly and equally. The Indian Ocean SST is influenced by remote forcing from the Pacific Ocean, while the Atlantic Ocean operates more independently, with no evident effect from other oceans.

How to cite: Lu, Z., Dong, L., Song, F., Wu, B., Wu, S., and Wang, C.: Quantifying Relative Contributions of Three Tropical Oceans to the Western North Pacific Anomalous Anticyclone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3062, https://doi.org/10.5194/egusphere-egu25-3062, 2025.

EGU25-4406 | Orals | CL3.1.1

Numerical investigations of turbulence in Mediterranean cyclone events: insights from the Turbimecs project 

Christian N. Gencarelli, Leonardo Primavera, Giuseppe Ciardullo, Jacopo Settino, and Francesco Carbone

The tropical cyclones are one of the biggest hazards to life and socio-economic activities even in the formative stages of their development. Some of their main features, especially in the shape evolution and in the dynamics, are common with events that in recent years are increasingly affecting the Mediterranean basin, defined as Mediterranean Tropical-Like Cyclones (MTLCs), or Medicanes.

In this study, we investigate the spatial and temporal properties of two Medicanes through high spatial resolution (1 km) reanalysis-based numerical simulations, generated using the Weather Research and Forecasting (WRF) model. The events examined are Qendresa (occurred in November 2014) and Ianos (occurred in September 2020), both developing over the Mediterranean Sea.

The WRF reanalyses were also used to conduct sensitivity studies on the parameterizations of atmospheric physics, focusing on PBL, radiation and microphysics schemes.

In order to address the problem in the classical fluid turbulence picture, the results were also analyzed using the Proper Orthogonal Decomposition (POD) method. With the aim of providing a first approach to understand how different contributions, operating on distinct spatio-temporal scales, can influence the local dynamics and the evolution of the medicanes. In addition the analysis will uncover the formation of coherent structures in the extreme event maturation.

How to cite: Gencarelli, C. N., Primavera, L., Ciardullo, G., Settino, J., and Carbone, F.: Numerical investigations of turbulence in Mediterranean cyclone events: insights from the Turbimecs project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4406, https://doi.org/10.5194/egusphere-egu25-4406, 2025.

Abstract. Western Ukraine has encountered significant challenges due to three extensive summer rainfall events and major floods in July 2008, July 2010, and June 2020, resulting in numerous fatalities and substantial economic damage. This study investigates the hydrometeorological factors, as well as the atmospheric processes, that led to these three devastating flood events in the basins of the Tisza, Prut, Siret, and Dniester rivers in western Ukraine. The 2008 flood was the most severe, with river levels surpassing historical records. The flood in 2020 was notable for its hydrological complexity and was evolving more rapidly than the 2008 flood. The 2010 flood was more localized. 

A series of intense precipitation events extending over about 5 days were one of the key factors resulting in floods in all three cases. The prolonged heavy precipitation that caused these floods mainly occurred during the transition of the large-scale flow from a Scandinavian blocking pattern to a western Russian blocking regime and typically formed beneath an upper-level trough located over southeastern Europe. An essential synoptic feature for initializing the heavy rain events was a quasi-stationary upper-level cutoff low  that existed for about 5 days.  This persistence of the synoptic flow pattern allowed for the advection of warm, moist air from the Black Sea at low to mid-tropospheric levels toward the eastern slopes of the Carpathians, leading to orographic lifting that strongly contributed to precipitation in the region. While each flood event shared common mechanisms, such as Rossby wave breaking with subsequent formation of cutoff lows, atmospheric blocking and orographic lifting, the arrangement, interaction, and intensity of these processes varied. The 2010 event was marked by a combination of two consecutive Rossby wave breaking events and an intense atmospheric block in western Russia. In contrast, the 2008 and 2020 floods were characterized by a merging of the Scandinavian blocking regime with a blocking system over western Russia, resulting in the formation of a cutoff cyclone over Romania.  Thus, through the characterization of hydrometeorological conditions during western Ukraine floods, we aim to provide knowledge for better preparedness for future floods both in the region and throughout Eastern Europe.

How to cite: Agayar, E., Armon, M., and Wernli, H.: The catastrophic floods in 2008, 2010 and 2020 in western Ukraine: Hydrometeorological processes and the role of upper-level dynamics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5086, https://doi.org/10.5194/egusphere-egu25-5086, 2025.

EGU25-6112 | ECS | Orals | CL3.1.1

Systematic approach for global identification of extreme weather events associated with atmospheric blockings and subtropical ridges 

Miguel M. Lima, Pedro M. Sousa, Tahimy Fuentes-Alvarez, Carlos Ordóñez, Ricardo García-Herrera, David Barriopedro, Pedro M. M. Soares, and Ricardo M. Trigo

It is known that some extreme weather events are associated with the appearance of large-scale blocking patterns (e.g. heatwaves and droughts), while others are linked to cut-off low systems that often occur on the southern flanks of the blocking patterns (e.g. extreme precipitation, intense snow storms). These quasi-stationary high-pressure systems disrupt the atmospheric flow, producing significant extreme weather and influencing surface impacts. However, identifying and tracking atmospheric blocks is challenging due to their diverse dynamics.

BLOCS (Blocking Location and Obstruction Cataloguing System) is an open-source, Python-based framework designed to systematically identify, classify, and track atmospheric blocking events. It is based on the state-of-the-art geopotential height gradient methodology (e.g., Sousa et al., 2021) and provides a robust tool applicable to different regular-grid datasets, such as NCEP-NCAR and ERA5. The method captures blocking subtypes (e.g., ridge, omega, Rex) and their life cycles, enabling detailed analyses of their spatial and temporal variability. By integrating customizable parameters, BLOCS can be adapted for studying atmospheric blocking and subtropical ridges under changing climate conditions across diverse datasets (e.g. Coupled Model Intercomparison Project, CMIP; Paleoclimate Modelling Intercomparison Project, PMIP).

Outputs from BLOCS include daily- and event-based catalogues, facilitating the study of blocking dynamics and their influence on extreme weather conditions, such as temperature anomalies and precipitation extremes. BLOCS has been used to analyze historic events like the 2003 European heatwave and the 2010 Russian mega-heatwave, demonstrating its ability to connect blocking patterns to surface impacts. Its applications extend to regional and global studies, enabling users to systematically explore blocking-driven socio-economic and environmental impacts.

By offering a user-friendly community-driven tool, BLOCS can be used to bridge traditional meteorological approaches with data-driven methods, provide a benchmark for assessing the prediction of extreme weather events, address critical gaps in atmospheric blocking research, and ultimately advance our understanding of these phenomena and their role in shaping extreme events.

Acknowledgements: This work is supported by the Portuguese Fundação para a Ciência e a Tecnologia (FCT) I.P./MCTES through national funds (PIDDAC): UIDB/50019/2025 and LA/P/0068/2020 (https://doi.org/10.54499/LA/P/0068/2020). M. M. Lima was supported through the PhD MIT Portugal MPP2030-FCT programme grant PRT/BD/154680/2023. Additional support comes from the EU-funded H2020 project CLINT (Grant Agreement No. 101003876), and MALONE (PID2021-122252OB-I00), funded by MICIU/AEI/10.13039/501100011033 and ERDF, EU.

How to cite: M. Lima, M., M. Sousa, P., Fuentes-Alvarez, T., Ordóñez, C., García-Herrera, R., Barriopedro, D., M. M. Soares, P., and M. Trigo, R.: Systematic approach for global identification of extreme weather events associated with atmospheric blockings and subtropical ridges, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6112, https://doi.org/10.5194/egusphere-egu25-6112, 2025.

EGU25-6295 | Posters on site | CL3.1.1

Heavy convective and stratiform precipitation and their links to atmospheric circulation 

Romana Beranova and Zuzana Rulfová

Precipitation in Central Europe can be classified as stratiform or convective based on its origin. Heavy convective precipitation is associated with intense storms, develops rapidly in localized areas, and can cause flash floods. In contrast, heavy stratiform precipitation is linked to longer-lasting, less intense rainfall events that may lead to large-scale flooding. These two types of precipitation also differ in their causal conditions, such as atmospheric circulation patterns and thermodynamic properties.

This study analyses heavy precipitation using time series from 19 observation stations across the Czech Republic for the period 1982–2021. An algorithm based on SYNOP reports was applied to classify precipitation totals as either convective or stratiform. Days with heavy precipitation (totals exceeding the 90th percentile) were assigned a circulation type using the Jenkinson & Collins (1977) method. This approach identifies 27 circulation types based on three indices: flow direction, strength, and vorticity.

The circulation types associated with heavy precipitation vary by season, precipitation type, and station location. Across all seasons, heavy precipitation is predominantly linked to cyclonic circulation and directional types with westerly and northerly flow components. In summer, heavy convective precipitation is additionally associated with anticyclonic conditions and unclassified patterns.

As climate change may significantly alter the atmospheric conditions driving heavy precipitation, understanding these phenomena and projecting their future behaviour is essential. To achieve this, the regional climate model ALADIN-CLIMATE/CZ operated by the Czech Hydrometeorological Institute will be used to evaluate the future relationship between heavy convective and stratiform precipitation and atmospheric circulation.

How to cite: Beranova, R. and Rulfová, Z.: Heavy convective and stratiform precipitation and their links to atmospheric circulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6295, https://doi.org/10.5194/egusphere-egu25-6295, 2025.

EGU25-6372 | Orals | CL3.1.1

Widespread multi-year droughts in Italy: identification and causes of development 

Salvatore Pascale and Francesco Ragone

Multi-year droughts pose a significant threat to the security of water resources, putting stress on the resilience of hydrological, ecological, and socioeconomic systems. Motivated by the recent multi-year drought that affected Southwestern Europe and Italy from 2021 to 2023, here we utilize two indices - the Standardized Precipitation Evapotranspiration Index (SPEI) and the Standardized Precipitation Index (SPI) - to quantify the temporal evolution of the percentage of Italian territory experiencing drought conditions in the period 1901-2023 and to identify Widespread Multi-Year Drought (WMYD) events, defined as multi-year droughts affecting at least 30% of Italy. Seven WMYD events are identified using two different different precipitation datasets: 1921-22, 1942-43, 1945-46, 2006-08, 2011-13, 2015-19 and 2021- 23. Correlation analysis between the time series of Italian drought areas and atmospheric circulation indicates that the onset and spread of droughts in Italy are related to specific phases of the winter North Atlantic Oscillation (NAO), the Scandinavian Pattern (SCAND), East Atlantic/Western Russia (EAWR) pattern and of the summer East Atlantic (EA) and East Atlantic/Western Russia (EAWR) patterns. Event-based analysis of these drought episodes reveals a variety of atmospheric patterns and combinations of the four teleconnection modes that contribute to persistently dry conditions in Italy during both winter and summer. This study offers new insights into the identification and understanding of Italian WMYD events and serves as a first step toward a better understanding of the impacts of anthropogenic climate change on them.

How to cite: Pascale, S. and Ragone, F.: Widespread multi-year droughts in Italy: identification and causes of development, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6372, https://doi.org/10.5194/egusphere-egu25-6372, 2025.

EGU25-6883 | ECS | Orals | CL3.1.1

The role of Rossby wave dynamics in spatially compounding heatwaves in mid-summer 2023 

Caihong Liu, Vera Melinda Galfi, Fenying Cai, Walter A. Robinson, and Dim Coumou

In July 2023, a series of heat extremes hit the North Hemisphere, which posed threats to the high-risk population and societal infrastructure in Eastern Canada, the Mediterranean, and Central Asia. Here we identify a dynamical linkage behind the spatiotemporal compounding nature of heatwaves over the three regions. However, it remains unclear whether these record-shattering extremes were amplified by specific recurrent atmospheric teleconnection patterns. By investigating the 2023 case and conducting historical analysis, we show that the Northern Hemispheric concurrent heatwaves in July 2023 were attributed to a recurrent wave-6 pattern. In particular, pre-existing warmth and drought over Eastern Canada in early-July intensified the wave-6 teleconnection; which then led to extreme heatwaves over the Mediterranean and Central Asia in mid-July 2023. Furthermore, we reveal that the wave train was generated by early-July convection over the northern subtropical Pacific together with the lowest May snow cover over North America in the past 40 years helped to warm Eastern Canada. Multiple models from the Coupled Model Intercomparison Project 6 can also simulate those compound extremes connected by the wave-6 pattern with a high inter-model agreement. Our research offers insights into record-breaking compounding heatwaves in disparate parts of world during the mid-summer of 2023, with implications for disaster decision-making and risk management.

How to cite: Liu, C., Galfi, V. M., Cai, F., Robinson, W. A., and Coumou, D.: The role of Rossby wave dynamics in spatially compounding heatwaves in mid-summer 2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6883, https://doi.org/10.5194/egusphere-egu25-6883, 2025.

EGU25-7402 | ECS | Orals | CL3.1.1

Sketching the spatial disparities in heatwave trends by changing atmospheric teleconnections in the Northern Hemisphere 

Fenying Cai, Caihong Liu, Dieter Gerten, Song Yang, Tuantuan Zhang, Kaiwen Li, and Jürgen Kurths

Pronounced spatial disparities in heatwave trends are bound up with a diversity of atmospheric signals with complex variations, including different phases and wavenumbers. However, assessing their relationships quantitatively remains a challenging problem. Here, we use a network-searching approach to identify the strengths of heatwave-related atmospheric teleconnections (AT) with ERA5 reanalysis data. This way, we quantify the close links between heatwave intensity and AT in the Northern Hemisphere. Approximately half of the interannual variability of heatwaves is explained and nearly 80% of the zonally asymmetric trend signs are estimated correctly by the AT changes in the mid-latitudes. We also uncover that the likelihood of extremely hot summers has increased sharply by a factor of 4.5 after 2000 over areas with enhanced AT, but remained almost unchanged over the areas with attenuated AT. Furthermore, reproducing eastern European heatwave trends among various models of the Coupled Model Intercomparison Project Phase 6 largely depends on the simulated Eurasian AT changes, highlighting the potentially significant impact of AT shifts on the simulation and projection of heatwaves.

How to cite: Cai, F., Liu, C., Gerten, D., Yang, S., Zhang, T., Li, K., and Kurths, J.: Sketching the spatial disparities in heatwave trends by changing atmospheric teleconnections in the Northern Hemisphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7402, https://doi.org/10.5194/egusphere-egu25-7402, 2025.

EGU25-7615 | ECS | Posters on site | CL3.1.1

Delayed impacts of NPO on wintertime surface air temperature in East Asia 

Sunyong Kim and Jin Ho Yoo

Observations show that anticyclonic circulation anomalies over the subtropics associated with North Pacific Oscillation (NPO) in December are responsible for surface warming in East Asia of the following January, a 1-month lag. We demonstrate that the lagged impacts of December NPO anomalies on the East Asian surface warming in January are attributable to two possible pathways by way of the tropics-extratropics teleconnections and local air-sea interactions. The northeasterly anomalies along the southern edge of the December NPO-related anticyclonic circulation anomalies efficiently advect dry air towards the western North Pacific (WNP), leading the intensified negative precipitation anomalies from December to January. This results in a Rossby wave propagation forced by upper-tropospheric divergence in the WNP, and thus affects the persistence of anticyclonic anomalies over East Asia into January. Over the Kuroshio region the easterly anomalies along the southern edge of the December NPO anticyclonic circulation anomalies oppose the prevailing westerly winds. The significant weakening of wind speeds, which in turn give rise to sea surface temperature (SST) warming along the Kuroshio region as a result of wind-evaporation-SST feedback, lead to favorable conditions for the East Asian warming in January. Additionally, the Coupled Model Intercomparison Project Phase 6 (CMIP6) models reasonably simulate the delayed impacts of December NPO anomalies on the East Asian climate in January supporting observations.

How to cite: Kim, S. and Yoo, J. H.: Delayed impacts of NPO on wintertime surface air temperature in East Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7615, https://doi.org/10.5194/egusphere-egu25-7615, 2025.

This study presents a revised Tropical Cyclone Genesis Potential Index (χMqGPI) for projecting tropical cyclone genesis in the Western North Pacific (WNP) and evaluates its performance against the traditional χGPI index. Using simulations from 22 CMIP6 models, both indices were calculated and assessed for their accuracy in historical and future warming scenarios. The results indicate that in historical simulations, both χGPI and χMqGPI exhibit strong correlations with observed tropical cyclone data, with correlation coefficients exceeding 0.9. Both indices also effectively capture the primary genesis regions of tropical cyclones in the WNP in terms of spatial distribution.

Under future warming scenarios, however, the two indices project contrasting trends in tropical cyclone genesis frequency (TCGF). χGPI consistently predicts an increase in TCGF, while χMqGPI projects a declining trend that aligns more closely with recent findings from high-resolution models. This declining trend underscores the robustness and reliability of χMqGPI in climate projections.

Decomposition analysis of χMqGPI revealed that large-scale dynamic parameters, particularly absolute vorticity and vertical wind shear, are critical in explaining discrepancies between model simulations. These differences become increasingly pronounced with the severity of warming, highlighting the importance of accurately representing large-scale environmental dynamics in models to improve tropical cyclone projections under climate change.

These findings offer valuable insights into the potential future behavior of tropical cyclones and emphasize the significance of adopting refined indices, such as χMqGPI, for reliable climate predictions. This work underscores the critical role of advanced metrics in understanding the impact of global warming on tropical cyclone activity in the WNP and beyond

How to cite: Hsiao, L.-P. and Hsu, H.-H.: Evaluating the Impact of Global Warming on Tropical Cyclone Genesis in the Western North Pacific: A Comparative Study of Tropical Cyclone Genesis Indices Using CMIP6 Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7700, https://doi.org/10.5194/egusphere-egu25-7700, 2025.

EGU25-7953 | Posters on site | CL3.1.1

The intensification of future extreme-rainfall events over Belgium and their dynamic and thermodynamic contributions 

Bert Van Schaeybroeck, Jozefien Schoofs, Kobe Vandelanotte, Hans Van de Vyver, Line Van Der Sichel, Matthias Vandersteene, Fien Serras, and Nicole P. M. van Lipzig

Climate change is expected to amplify extreme-rainfall intensity and frequency over Europe due to the increase in atmospheric moisture with warming, ensuing severe socio-economic impacts. The influence of future dynamic changes i.e. changes to atmospheric circulation patterns, on extreme-rainfall over Europe, on the other hand, remains unclear. Additionally, recent works point out that inadequate representation of regional circulation patterns by climate models may strongly impact their climate-change results over Europe (Vautard et al., 2023).

This study presents a methodology for assessing the dynamical and thermodynamical contributions to the changes in extreme daily rainfall based on the Lamb weather type classification and with an application over Belgium. Thereby, GCMs from CMIP6 are first sub-selected based on their ability to accurately represent the overall atmospheric circulation (Serras et al., 2024) and the atmospheric circulation during days of extreme rainfall. We find that models with a good circulation probability distribution do not necessarily feature a good circulation-probability representation when restricting to days with extreme rainfall events, and vice versa. This means that, for our purpose, additional to the model selection based on all days, a selection based on the circulation probability distribution during days of extreme rainfall is implemented. Additionally, the increase in extreme-rainfall intensity and likelihood at the end of century under the SSP3-7.0 scenario for Belgium, are driven by thermodynamic factors rather than dynamic changes. While the probability of extreme rainfall rises predominantly in fall and winter, the most significant intensity increases are projected for spring and summer. 

  • Vautard, R., Cattiaux, J., Happé, T., Singh, J., Bonnet, R., Cassou, C., ... & Yiou, P. (2023). Heat extremes in Western Europe increasing faster than simulated due to atmospheric circulation trends. Nature Communications, 14(1), 6803.
  • Serras, F., Vandelanotte, K., Borgers, R., Van Schaeybroeck, B., Termonia, P., Demuzere, M., & van Lipzig, N. P. (2024). Optimizing climate model selection in regional studies using an adaptive weather type based framework: a case study for extreme heat in Belgium. Climate Dynamics, 1-23.

How to cite: Van Schaeybroeck, B., Schoofs, J., Vandelanotte, K., Van de Vyver, H., Van Der Sichel, L., Vandersteene, M., Serras, F., and van Lipzig, N. P. M.: The intensification of future extreme-rainfall events over Belgium and their dynamic and thermodynamic contributions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7953, https://doi.org/10.5194/egusphere-egu25-7953, 2025.

EGU25-8108 | ECS | Orals | CL3.1.1

Drivers of multi-year droughts in large ensemble simulations 

Jonna van Mourik, Denise Ruijsch, Karin van der Wiel, Wilco Hazeleger, and Niko Wanders

Multi-year droughts (MYDs) are severe natural hazards that have become more common due to climate change. Given their significant societal impact compared to normal droughts (ND) of shorter duration, it is crucial to better understand the drivers of MYDs. In this work we used a combination of a large-ensemble of climate models and reanalysis data to study the difference between MYDs and NDs. For six different climatic regions, chosen to be of similar size to the dominating regional atmospheric circulation patterns, we used reanalysis data of precipitation and potential evapotranspiration to show the regional characteristics and drivers of MYDs and contrast these with characteristics of NDs. Our findings reveal that MYD occurrence and duration varies significantly between the regions, where relatively larger differences in duration between MYD and NDs can indicate different drivers resulting in the different drought durations. Regions with distinctive seasonality in their precipitation climatology tend to experience faster drought onsets compared to regions with climatologically steady precipitation. Furthermore, our analysis shows that MYDs and NDs often start with similar conditions but diverge over time, and that longer-term memory is present in some regions, which might provide avenues for the predictability of MYDs. However, since MYDs are rare events (2 to 6 MYDs per region between 1950-2023 in this study), we supplement reanalyis data with that of CMIP6 climate models with a large number of ensembles to assess the drivers of MYDs with more statistical rigour. This creates the opportunity to study the contributions of oceans, soil moisture, snow, and other climate variables on the persistent circulation patterns leading to MYDs, and to find the influence of climate variability on the occurrence of MYDs.

DOI: http://dx.doi.org/10.2139/ssrn.4974995

How to cite: van Mourik, J., Ruijsch, D., van der Wiel, K., Hazeleger, W., and Wanders, N.: Drivers of multi-year droughts in large ensemble simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8108, https://doi.org/10.5194/egusphere-egu25-8108, 2025.

EGU25-8195 | Orals | CL3.1.1

Cluster analysis of HYSPLIT backward trajectories for major heatwaves in Spain and Ukraine (1940–2023) 

Oleg Skrynyk, Enric Aguilar, Olesya Skrynyk, and Caterina Cimolai

Heatwaves (HWs) are extremely harmful weather phenomena that cause significant damage to the environment and society. Numerous studies have shown a substantial increase in the frequency and intensity of HWs in various parts of the world. Therefore, investigating the meteorological factors contributing to HW formation is an important task. In this study, we investigated the main air transport patterns associated with the most severe HWs observed during 1940-2023 in Spain and Ukraine.

Firstly, based on ERA5 (2 m) air temperature data, we identified all HW events for each grid point in both countries with the heatwaveR package. Following the approach used in many studies, a HW was defined as an extreme weather phenomenon when daily maximum air temperature exceeds 90-th percentile at least for three consecutive days. Additionally, each detected HW episode was categorized as moderate, strong, severe, or extreme based on its maximum observed intensity. A final list of HWs for further analysis in each country was compiled by selecting events with a spatial extent covering more than 20% of the country’s territory and with severe or extreme category identified in at least one grid point. Using this methodology, we selected 80 HW episodes in Spain and 18 in Ukraine.

Backward trajectories for the selected HW episodes were calculated using the HYSPLIT model, with ERA5 3D-data serving as input meteorology. For each HW event, only first three days were considered, regardless of the event's total duration. A starting location for backward trajectories for each HW was defined as a midpoint of its spatial extent. Additionally, to assess the influence of vertical wind shear on trajectory calculations, three altitudes (10, 1500, and 5000 m AGL) were defined as the starting heights. Backward trajectories were initiated hourly over the 3-day period and calculated for the seven days preceding each release hour. In total, 216 backward trajectories were calculated for each HW episode (72 trajectories per release height). The calculated trajectories were then grouped into three clusters based on the HYSPLIT clustering approach and a mean trajectory was determined for each cluster. Along with the cluster analysis, we also identified the dominant circulation types and their evolution during the selected HW episodes. This analysis was performed using the synoptReg package based on ERA5 mean sea level pressure data.

The mean cluster trajectories, calculated for all selected HWs, were used to build trajectory frequency maps, showing the most preferential routes of air masses associated with the severe and extreme HWs. Analysis of these maps revealed that a westerly trajectory flow is the most likely route for air masses responsible for the most intense HWs in Spain and Ukraine. In Spain, air masses are typically transported from the Atlantic, whereas in Ukraine, they traverse across Western Europe. Other directions of air mass transport, including from the south, occur relatively rarely. Our findings align with other similar studies for other regions in Europe, which suggest that heat advection is not dominant mechanism for HW formation.

This work has received funding through the MSCA4Ukraine project, funded by the European Union

How to cite: Skrynyk, O., Aguilar, E., Skrynyk, O., and Cimolai, C.: Cluster analysis of HYSPLIT backward trajectories for major heatwaves in Spain and Ukraine (1940–2023), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8195, https://doi.org/10.5194/egusphere-egu25-8195, 2025.

EGU25-8369 | Posters on site | CL3.1.1

Heatwave climatology in Ukraine: current (1946-2020) and projected (2020-2100) 

Olesya Skrynyk, Enric Aguilar, Vladyslav Sidenko, and Oleg Skrynyk

Climatological and meteorological aspects of heatwaves (HWs) have been extensively studied in various parts of the world, as these extreme weather events have significant harmful effects on both humans and the environment. Several studies have examined HW climatology in Ukraine for specific historical periods using observational air temperature data. However, these results were obtained based on a relatively small number of meteorological stations.

In our study, we calculated HW climatology in Ukraine for both the current historical (1946–2020) and the projected (2020–2100) periods. For the historical period, we utilized the observation-based gridded dataset ClimUAd, which was recently developed for Ukraine. These gridded data are based on a comprehensive collection of instrumental meteorological measurements collected at 178 stations during 1946-2020 across the country. The dataset provides gridded daily time series of four essential climate variables: minimum, mean, and maximum surface air temperature, as well as atmospheric precipitation. The spatial resolution of ClimUAd is 0.1° × 0.1° in both longitude and latitude, enabling the analysis of HW climatology with fine spatial detail across Ukraine.

For the projected period, we applied a mini-statistical ensemble of climate simulations obtained with seven global climate models (GCMs) from the Coupled Model Intercomparison Project Phase 6. GCMs were selected for the ensemble based on two criteria: the use of the Gregorian calendar and a computational grid resolution no courser than 1.5o×1.5o. Our analysis incorporated climate projections obtained under two Shared Socioeconomic Pathways (SSP) scenarios: SSP2-4.5 and SSP5-8.5. Prior to calculating HW metrics, all climate projections of surface air temperature were bias-corrected using the quantile delta mapping method. In the bias-correction procedure, ClimUAd data were used along with historical climate simulations for the period 1985-2014.

For both the historical and projected periods, HWs were identified using daily maximum air temperature (TX) data. To detect HWs, we define this extreme weather phenomenon as an event when TX exceeds the 90-th percentile, calculated based on the WMO standard reference period of 1961-1990, for at least three consecutive days, allowing for a one-day gap. This approach is frequently used and widely recommended in studies as the most suitable for HW analysis with pure climatological purposes. The applied definition enables the identification of HWs throughout an entire year. To quantify HW peculiarities, we calculated four HW metrics on a yearly scale: HW number, HW frequency, HW duration, and HW amplitude. All HW calculations were performed using the heatwaveR package.

Our findings revealed a significant increase in all HW metrics during the historical period, with the most pronounced changes observed in the western part of Ukraine. In the projected period, the HW metrics continue to increase at a similar rate for both considered SSPs until approximately the mid-century. However, in the latter part of XXI, changes in HW climatology under SSP5-8.5 differ considerably from those under SSP2-4.5. The SSP5-8.5 scenario indicates that more than half of days in a year at the end of XXI could qualify as HWs.

This work has received funding through the MSCA4Ukraine project, funded by the European Union

How to cite: Skrynyk, O., Aguilar, E., Sidenko, V., and Skrynyk, O.: Heatwave climatology in Ukraine: current (1946-2020) and projected (2020-2100), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8369, https://doi.org/10.5194/egusphere-egu25-8369, 2025.

Cut-off lows (COLs), which are warm season high altitude cold depressions originating from the pole, have lead to the most extreme precipitation events in Belgium in the past decades, notably in July 2021. Their frequency is expected to rise with Global warming due to slowing dynamics during the warm season. On top of this, extreme precipitation events are becoming more frequent, and more extreme due to the increase of atmospheric moisture content resulting from its warming (Brajkovic et al., 2025 in prep.). To understand the cause of this increased frequency, we want to assess the evolution of the frequency of COLs which lead to extreme precipitation events in Belgium.

First, over 1940-2023, using our bias-adjusted high-resolution (5-km) Regional Climate model MAR (Modèle Atmosphérique Régional) precipitation data over Belgium and ERA5 reanalysis 500hPa geopotential data over Europe, we identify COLs which lead to extreme precipitation over the country. We find COLs leading to extreme precipitation all over the period. Their occurence has increased over the last decades reaching a frequency of 1 COL per year. However, we find periods with less COLs like in the 1970s.

Second, MAR is forced 6 CMIP6 Earth System Models over 2015-2100. Four Shared Socioeconomic Pathways baseline scenarios (SSP) are used ranging from low-end (SSP1-2.6) to high-end emissions (SSP5-8.5). Again, using ESM 500hPa geopotential and bias-ajusted MAR precipitation data, we proceed to the same detection over the future. We find that the occurrence of COLs is stochastic and without clearly identified trends. Intense precipitation events occur irrespective of the scenario at timings which are challenging to predict. However, the frequency of COLs reaches 1 COL per year irrespective of the model or of the scenario. This analysis shows that a large amount of the uncertainty over future computed extreme precipitation statistics lies in the occurrence of COLs.

 

How to cite: Brajkovic, J., Fettweis, X., Ghilain, N., and Doutreloup, S.: Past and future evolution of synoptic weather patterns leading to extreme precipitation events in Belgium. Linking synoptic scale events to their local impacts. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9805, https://doi.org/10.5194/egusphere-egu25-9805, 2025.

EGU25-10214 | Orals | CL3.1.1

Using causal networks to constrain regional drought projections 

Marina Friedel, Marlene Kretschmer, and Bruce Hewitson

Severe droughts in the Cape Town region (CTR) are projected to become more frequent in the coming decades, posing significant societal challenges. However, while climate models consistently predict a precipitation decline for the CTR until the end of this century, these projections carry substantial uncertainties, with decreases ranging from almost zero to as much as -50%.

In this study, we employ causal networks to evaluate climate models based on their ability to accurately represent the large-scale dynamical processes that drive precipitation in the CTR. While previous research has identified links between precipitation in the CTR  and various large-scale drivers, such as the eddy-driven jet and sea surface temperatures in the South Atlantic, the interactions between these drivers remain poorly understood and the relative contributions of individual drivers to precipitation in the CTR remain unexplored.

Following causal inference theory, the causal relationships among the large-scale drivers of precipitation in the CTR are quantified in reanalysis data, pinpointing the main precipitation drivers, their interactions and relative contributions to precipitation and drought events. The resulting causal network is then applied to constrain precipitation projection. The study’s insights into the links between planetary-scale circulation patterns and regional processes could enhance our understanding of extreme and compound events, with potential implications for drought management.

How to cite: Friedel, M., Kretschmer, M., and Hewitson, B.: Using causal networks to constrain regional drought projections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10214, https://doi.org/10.5194/egusphere-egu25-10214, 2025.

EGU25-10994 | ECS | Orals | CL3.1.1

Pathways to concurrent North American cold and European wind extremes 

Richard Leeding and Gabriele Messori

We examine near-simultaneous occurrences of cold extremes in North America and wind extremes in Europe, referred to as pan-Atlantic compound extremes. Previous studies have established a robust spatial and temporal relationship between the location of cold extremes and the footprint of wind extremes. Individually, cold and wind extremes are highly impactful, but their coincident occurrence amplifies effects and exposes international actors to correlated losses. This study analyzes the large-scale circulations responsible for pan-Atlantic compound extremes through the lens of weather regimes and Fourier decomposition.

Five distinct dynamical pathways are identified, which non-uniformly govern the occurrence of cold extremes across three regions of North America. Three of these pathways also engender European wind extremes, providing a mechanistic explanation for the observed spatial and temporal relationships of pan-Atlantic extremes. The pathways are as follows:
(i) A persistent Atlantic low producing cold spells in eastern Canada and wind extremes in the British Isles.
(ii) A wave train generating cold spells in the eastern United States, culminating in an Atlantic low and wind extremes in Iberia and the British Isles.
(iii) A wave train producing cold spells in eastern Canada, culminating in Scandinavian blocking.
(iv) A quasi-stationary wave-2 pattern driving cold spells in central Canada and Scandinavian blocking.
(v) An Arctic high generating cold spells in the eastern United States and wind extremes in Iberia.

How to cite: Leeding, R. and Messori, G.: Pathways to concurrent North American cold and European wind extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10994, https://doi.org/10.5194/egusphere-egu25-10994, 2025.

EGU25-11026 | ECS | Orals | CL3.1.1

The Role of Teleconnection Indices in Modulating Rainfall and Drought in Central Brazil 

Lívia Sancho, Louise Aguiar, Vitor Luiz Victalino Galves, Priscila Esposte Coutinho, and Marcio Cataldi

Increasing temperatures due to climate change pose challenges to countries worldwide, including Brazil, where extreme weather may result in biodiversity loss, water resource availability changes, and significant economic and health impacts. This study evaluates the influence of various teleconnection indices on the variability patterns of atmospheric blocking events occurring in central Brazil and episodes of the South Atlantic Convergence Zone (SACZ). Nearly all teleconnection indices made available in the NOAA’s website were analysed, including those related to the Pacific, Atlantic, Indian Oceans and global-scale indices. Additionally, four new indices were explicitly developed for this study, focusing on NOAA’s OISST Sea Surface Temperature anomalies in the North Atlantic Ocean near the Moroccan coast. The characterization of atmospheric blocking events and SACZ episodes was carried out using indices developed at LAMMOC/UFF, which effectively capture the behaviour of these atmospheric systems across different regions of Brazil. The SACZ index was calculated using NCEP Reanalysis data, while the atmospheric blocking index used ERA5 reanalysis data, resulting in a time series spanning from 1981 to 2023. All data were normalized for statistical analyses, and methods including Pearson’s correlation coefficient, Principal Component Analysis, K-means clustering techniques, trend analysis, and the Mann-Kendall test were applied to identify and quantify trends in the data. Atmospheric blocking and SACZ episodes have contrasting yet significant influences on the rainfall in central Brazil. Atmospheric blocking events are typically associated with prolonged droughts, whereas SACZ episodes are linked to intense and spatially well-distributed precipitation. This region is vital for the country’s agriculture, industry, and energy production. The analysis revealed that a significant portion of oceanic indices from the Atlantic and the Pacific Oceans, along with atmospheric blocking events, exhibit strong increasing trends. These trends are accompanied by positive correlations, observed in the trend-inclusive and detrended series. For instance, correlations reach 0.7 values with the Global Mean Land/Ocean Temperature, 0.45 with ENSO indices, 0.55 with North Atlantic indices near the Moroccan coast, and 0.67 with the Pacific Warmpool Area Average. In contrast, the SACZ index showed no clear trend in the Mann-Kendall tests. Correlations between SACZ and the same oceanic indices often exhibited an inverse relationship compared to those with blocking indices and were also generally weaker, ranging between -0.15 and -0.30. One exception was a positive correlation of around 0.34 with the East Pacific/North Pacific Oscillation index. Overall, the study highlights that atmospheric blocking events are becoming increasingly frequent and intense in central Brazil, closely following the warming trend of the oceans. This poses a warning for the region’s hydrometeorological regime. While the absence of an evident decline in SACZ episodes provides some relief, the escalating deforestation in the Amazon, one of the primary sources of moisture driving precipitation during SACZ episodes, may become the decisive factor in altering the region’s precipitation patterns, potentially exacerbating the ongoing water crisis in central Brazil.

How to cite: Sancho, L., Aguiar, L., Victalino Galves, V. L., Esposte Coutinho, P., and Cataldi, M.: The Role of Teleconnection Indices in Modulating Rainfall and Drought in Central Brazil, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11026, https://doi.org/10.5194/egusphere-egu25-11026, 2025.

EGU25-11431 | ECS | Orals | CL3.1.1

Influence of Atmospheric Blocking and SACZ Episodes on Extreme Heatwaves in Brazil: A Long-Term Analysis 

Louise da Fonseca Aguiar, Vitor Luiz Galves, Priscila Esposte Coutinho, Lívia Sancho, and Marcio Cataldi

Rising temperatures driven by climate change pose significant challenges worldwide. In Brazil, these challenges include extreme weather events such as heatwaves, which can have severe health impacts. This study investigates the influence of atmospheric blocking events and episodes of the South Atlantic Convergence Zone (SACZ) on Brazil's occurrence and intensity of extreme heatwaves. Atmospheric blocking and SACZ episodes were characterized using indices developed at LAMMOC/UFF, which effectively capture the behavior of these systems across different regions of the country. Atmospheric blocking events are typically associated with prolonged droughts, while SACZ episodes are linked to intense, spatially well-distributed precipitation. The newly developed Extreme Heatwave (XHW) index was applied in this study due to its global applicability, covering all 26 state capitals and the Federal District of Brazil. The SACZ index was calculated using NCEP Reanalysis data (I and II) while blocking and XHW indices were calculated using ERA5 reanalysis data, generating a time series from 1960 to 2024. To facilitate statistical analyses, all data were normalized. Methods such as Pearson’s correlation coefficient, Principal Component Analysis (PCA), K-means clustering, trend analysis, and the Mann-Kendall test were applied to identify and quantify trends in the series. The results showed an increase in extreme heat events in most cities, except for Florianópolis (in the South) and Fortaleza (in the Northeast), which displayed no significant trend. Atmospheric blockings also showed a clearer upward trend across all evaluated regions compared to SACZ episodes. The correlation between the SACZ and heatwaves is statistically insignificant across most of Brazil, with values close to zero, as the SACZ is not associated with significant temperature gradients, causing little to no impact on the occurrence of heatwaves. In contrast, atmospheric blockings show statistically significant positive correlations with heatwaves, particularly in geographically specific regions. For example, in the North region, Palmas (TO) stands out with a correlation of 0.44, while Manaus (AM) approaches a value of 0.38. These cities are more responsive to northern-located blockings. Rio de Janeiro (RJ), in the Southeast, and Cuiabá (MT), in the Central-West, exhibit a correlation of 0.37 due to southern and northern-located blockings, respectively. In the South, Porto Alegre (RS) is the most responsive to southern-located blockings with a correlation of 0.18. In the Northeast, values are generally low, with Recife (PE) showing the highest correlation (0.16) for northern-located blockings. This study emphasizes the importance of spatial analysis in understanding the influence of atmospheric blockings on extreme heatwaves events, revealing a direct relationship between the position of blockings and their impact, as evidenced by the varying responses of different cities. As atmospheric blockings increase in frequency due to climate change, heatwaves are also expected to become more frequent and intense. This trend poses a growing risk to public health and mortality, as well as significant challenges to the healthcare system.

How to cite: da Fonseca Aguiar, L., Galves, V. L., Esposte Coutinho, P., Sancho, L., and Cataldi, M.: Influence of Atmospheric Blocking and SACZ Episodes on Extreme Heatwaves in Brazil: A Long-Term Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11431, https://doi.org/10.5194/egusphere-egu25-11431, 2025.

EGU25-11580 | ECS | Posters on site | CL3.1.1

Exploring and characterizing the life cycles of tracked anticyclones on the northern hemisphere 

Michael Thomas and Stephan Pfahl

Summer heat waves are among the most severe natural hazards in the mid-latitudes and known to be strongly associated with anticyclonic activity. Despite their frequent occurrence, gaps remain in the understanding of the processes that drive persistent heat outbreaks during the lifetime and in the vicinity of some anticyclones. A closer look at the life cycles of these anticyclones could be beneficial for understanding the circumstances under which there is an increased likelihood of near-surface extremes.
To date, numerous studies have performed some form of feature tracking on anticyclones, but many are limited to a specific region or context, while those that take a broader view focus on climatology rather than individual life cycles.
In this work, mid-tropospheric anticyclones are identified though geopotential height anomalies, tracked over time and analyzed based on their shape, propagation speed and overlap with other atmospheric phenomena, such as heat waves, droughts and blocking. Using 40 years of northern hemisphere reanalysis data, a detailed track dataset for around 5900 individual anticyclones is examined. It is shown that the most extreme temperature anomalies are systematically more likely to be associated with anticyclones with longer life times. Furthermore there is evidence that the probability for a heat wave maximum is higher in the early and late phases of the anticyclonic life cycles, with the former (latter) being particularly true for shorter-lived (longer-lived) high pressure systems.

How to cite: Thomas, M. and Pfahl, S.: Exploring and characterizing the life cycles of tracked anticyclones on the northern hemisphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11580, https://doi.org/10.5194/egusphere-egu25-11580, 2025.

In mid-latitude regions, the development of a heatwave is closely linked to a quasi-stationary anticyclonic flow anomaly. For many cases over Europe, these anomalies are associated with atmospheric blocking events, which in summer usually manifest themselves in form of a so-called Omega blocking. However, not all heatwaves necessitate atmospheric blocking. Indeed, some heatwaves are enabled by poleward extensions of the subtropical high pressure belt, forming an atmospheric ridge pattern. We hypothesize that both the origin of the involved air masses as well as the processes modulating the air mass along its path to Central Europe may differ fundamentally between heatwaves forming under an Omega blocking and those that are initiated by a subtropical ridge.

In this work, we therefore select the respective 20 most textbook-like cases of Omega and ridge-type Central European heatwaves in the period of 1950 to 2023. Based on high-resolution ERA5 data, we conduct a Lagrangian analysis into the properties of air masses and the relative importance of the three processes warming the involved air masses, namely advection, adiabatic warming by subsidence and diabatic warming through sensible heat fluxes. By computing a large number of backward trajectories using Lagranto and the subsequent application of a Lagrangian temperature decomposition algorithm, we quantify the relative importance of each of the three mentioned processes. This analysis is done separately for the onset day and the subsequent three days of the heatwave.

Omega- and ridge-type heatwaves feature some significant differences in both air mass origin and the relative importance of the processes leading to anomalously high near-surface temperatures, which tend to become more apparent in the more mature stage of the respective type of heatwave. Overall, ridge-type heatwaves tend to be characterized by a higher advective contribution to the overall temperature anomaly. This is directly related to the fact, that the involved air masses tend to originate from slightly more southern and climatologically warmer regions. Particularly two or three days after heatwave onset, anomalous subsidence and associated adiabatic heating contributes significantly more to warming in ridge-type than in omega-type heatwaves. In turn, omega-type heatwaves are characterized by a significantly stronger contribution of diabatic heating. This is mostly due to air masses spending more time in the planetary boundary layer and stronger short-wave radiation along the air masses' path.

How to cite: Lemburg, A., Fink, A. H., and Pinto, J. G.: Lagrangian analysis of two flavours of Central European heatwaves: development under Omega blocking vs. initiation by subtropical ridges, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11816, https://doi.org/10.5194/egusphere-egu25-11816, 2025.

EGU25-11855 | ECS | Orals | CL3.1.1

An analog-based weather generator using re-forecast data 

Jonathan Wider, Daniel Klotz, and Jakob Zscheischler

Accurately estimating the risks of weather-related impacts requires comprehensively simulating weather conditions that could occur but have not occurred in the historical record. This is the aim of weather generators. Analog-based weather generators exploit the fact that the large-scale atmospheric circulation constrains regional weather and generate multivariate spatiotemporal meteorological fields by resampling historical data. During the resampling, constraints are employed to ensure that successive samples have consistent circulation patterns. Compared to other types of weather generators, resampling-based methods have the advantage that dependencies between variables and between locations are automatically correctly captured. However, the generated time series are limited to observed ranges, and even “close” analogs in the historical record are relatively far away from each other.

We overcome these limitations by constructing a (daily) analog weather generator using ECMWF extended ensemble forecast hindcast (re-forecast) data, which provides a much larger sample size and the ability to sample values larger than the observed records. We choose this dataset because it has high spatial resolution and provides a large set of states from a relatively constant climate, while model biases remain limited because the forecasts are initialized from reanalysis data. With the ensemble hindcasts, we can also assess how “close” analogs are compared to typical ensemble spreads. We test our methodology by applying it to simulate weather over a European domain. Analogs are defined in terms of geopotential height at 500hPa and computed over an extended region including parts of the North Atlantic. With our approach, we can find better analogs compared to a baseline using only ERA5 data. We evaluate key properties of the simulated time series, such as their annual cycle, extremes, and lengths of wet and dry spells. The weather generator can be widely applied to estimate potential climate impacts, for instance with impact models. It is especially useful in cases where an accurate representation of dependencies between variables or across space is important for the impacts, which is the case for a number of different types of compound events.

How to cite: Wider, J., Klotz, D., and Zscheischler, J.: An analog-based weather generator using re-forecast data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11855, https://doi.org/10.5194/egusphere-egu25-11855, 2025.

EGU25-12052 | ECS | Orals | CL3.1.1

Impacts of Atmospheric Phenomena on River Flow and Hydropower Stability in Brazil 

Priscila Esposte Coutinho, Lívia Sancho, Louise da Fonseca Aguiar, Vitor Luiz Victalino Galves, Franciele Zanandrea, and Marcio Cataldi

Renewable energy sources are inherently influenced by environmental variability. In Brazil, hydropower constitutes approximately 65% of the country’s electricity matrix, relying directly on river flow, which is strongly governed by precipitation on an operational timescale. This study investigates the influence of atmospheric blocking events and episodes of the South Atlantic Convergence Zone (SACZ) on the occurrence and magnitude of natural flow in several hydropower plants in river basins across Brazil. Atmospheric blocking and SACZ episodes were characterized using indices developed at LAMMOC/UFF, which effectively capture the behavior of these systems in different regions of the country. The SACZ index was calculated using NCEP reanalysis data, while the blocking index was derived from ERA5 reanalysis data. Natural flow data for the power plant areas were provided by the National Electric System Operator (ONS). To maximize the availability of records for this study, the time series was defined from 1960 to 2023. All data were normalized for statistical analyses, and methods such as Pearson’s correlation coefficient, Principal Component Analysis (PCA), K-means clustering, trend analysis, and the Mann-Kendall test were employed to identify and quantify trends. Results indicate that blocking events have shown a rising trend across all evaluated regions, whereas SACZ episodes do not display an increasing trend uniformly throughout the country. Regarding river flow trends, increases were observed in Southern Brazil, while decreases predominate in the Southeast, Central-West, Northeast, and North regions. SACZ episodes positively influence flow in hydropower plants in the Central-West, North, and Northeast regions, while inhibiting precipitation in the South as their effects shift northward, away from the basins. For instance, the Paranaíba River basin in the Northeast shows a correlation of 0.55 with SACZ episodes, and the Paraopeba River basin located between the Southeast and Central-West Regions, presents a correlation of 0.57. Notable SACZ-related correlations are also observed in the Grande, Paranaíba, and Baixo Paraná basins, with values exceeding 0.3 and increasing towards the South, reaching over 0.5 for Baixo Paraná and 0.6 for Grande and Paranaíba basins. Conversely, the Araguaia-Tocantins basin in the North exhibits one of the highest correlations, at 0.69. Atmospheric blocking events, in turn, are positively correlated with river flow in the South, particularly in the Uruguai and Jacuí basins, which exhibit the highest correlation values. However, they produce a negative correlation in basins of other regions, as their associated high-pressure systems inhibit atmospheric dynamics, reduce precipitation, and prevent the advance of cold fronts, concentrating precipitation in Southern areas. The results reveal a decline in river flow across most hydropower plant areas, posing risks to Brazil’s electricity production, with potential impacts on the country’s Gross Domestic Product (GPD). SACZ and atmospheric blocking events significantly influence river flow, especially in the power plants of the Central-West, North, and Northeast regions. Developing indices for these atmospheric phenomena offers valuable insights into regional water availability, supporting strategies to mitigate risks from shifting precipitation regimes across Brazil’s diverse climates and biomes.

How to cite: Esposte Coutinho, P., Sancho, L., da Fonseca Aguiar, L., Victalino Galves, V. L., Zanandrea, F., and Cataldi, M.: Impacts of Atmospheric Phenomena on River Flow and Hydropower Stability in Brazil, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12052, https://doi.org/10.5194/egusphere-egu25-12052, 2025.

EGU25-13453 | ECS | Posters on site | CL3.1.1

Seasonality of Heatwaves in Central Europe: Insights from Dynamical Systems Theory and Weather Regimes 

Ines Dillerup, Alexander Lemburg, Sebastian Buschow, and Joaquim Pinto

Heat extremes have severe impacts on human health, economies, and ecosystems. In particular in Europe, heatwaves are expected to become more frequent and intense with climate change, making it essential to understand and quantify the key factors driving these events, such as soil moisture deficits and atmospheric circulation. Further, global warming is likely not only to increase the frequency and intensity of heatwaves in the summer, but also in early autumn, highlighting the need to explore seasonal variations in their drivers.

We analyze heatwaves in Central Europe (45–55°N, 4–16°E) in the historical period (1950-2023) by quantifying atmospheric persistence and exploring the link between surface temperatures and atmospheric circulation patterns using dynamical system theory. This approach is further contextualized by an analysis of weather regimes representing the low-frequency variability of the atmosphere over the North Atlantic and Europe. Using ERA5 reanalysis data, we examine intra-seasonal variations of heatwaves during the extended summer months (May–September). Our results show an anomalously strong link between atmospheric circulation and surface temperatures on heatwave days. In July and August, an anomalously high persistence of the atmospheric circulation is found on heatwave days, associated with an enhanced frequency of Scandinavian and European blocking weather regimes. Moreover, we investigate additional drivers of heatwaves such as soil moisture, and examine the life cycle of heatwaves.

How to cite: Dillerup, I., Lemburg, A., Buschow, S., and Pinto, J.: Seasonality of Heatwaves in Central Europe: Insights from Dynamical Systems Theory and Weather Regimes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13453, https://doi.org/10.5194/egusphere-egu25-13453, 2025.

EGU25-15158 | ECS | Posters on site | CL3.1.1

Role of the Siberian Summer Cold Wave in Intensifying East Asian Summer Precipitation 

Kwang-hee Han, Baek-Min Kim, Ho-Young Ku, Hayeon Noh, Jee-Hoon Jeong, and Sung-Ho Woo

In this study, we clarify the role of a distinguished weather pattern over Siberia that has contributed to intense summer precipitation across East Asia, particularly in recent decades. This weather pattern, termed the Siberian Summer Cold Wave (SSCW), is defined through rigorous criteria and retrospective case selection. SSCW is characterized by the rapid influx of cold air from the Siberian region into East Asia during summer, which is associated with an increase in the potential temperature gradient, leading to the development of precipitation. Since the early 2000s, the frequency of SSCW events has increased, coinciding with a rise in severe precipitation events, underscoring its significance. Although SSCW has played a crucial role in influencing precipitation in East Asia, previous studies have predominantly focused on mechanisms related to heavy rainfall occurring in southern regions of East Asia. Consequently, there has been a relative lack of research investigating systems contributing to heavy precipitation from the north. This study provides a comprehensive analysis of SSCW events and elucidates their precipitation characteristics, positioning SSCW as a pivotal precipitation pattern within the East Asian summer climate. Our findings highlight the need for continued research to better understand SSCW dynamics and effectively mitigate associated risks.

How to cite: Han, K., Kim, B.-M., Ku, H.-Y., Noh, H., Jeong, J.-H., and Woo, S.-H.: Role of the Siberian Summer Cold Wave in Intensifying East Asian Summer Precipitation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15158, https://doi.org/10.5194/egusphere-egu25-15158, 2025.

EGU25-16474 | Orals | CL3.1.1

Contemporary Megadrought on Easter Island (Rapa Nui) since 2010  

Nathan Steiger and Eden Markovitz

Since 2010 Easter Island (Rapa Nui) has experienced an exceptional decadal-scale megadrought. Observations show a significant and unusual decrease in precipitation on Rapa Nui: every year from 2010-2023 has had lower precipitation than the average from 1979-2009, resulting in an average precipitation that is 67% of normal. This reduction in precipitation coincides with decadal-scale climate shifts: an intensification of the South Pacific Anticyclone and its shift closer to the island along with a poleward shift of the Southern Hemisphere storm track. Each of these phenomena are trending near or beyond their most extreme values since 1979 and each of them are directly linked to reduced precipitation on Rapa Nui. These trends are shown to continue into mid-century under an intermediate greenhouse gas emissions scenario. We therefore argue that the current megadrought is best explained by anthropogenic climate change and that Rapa Nui may be entering a fundamentally drier climate state.

How to cite: Steiger, N. and Markovitz, E.: Contemporary Megadrought on Easter Island (Rapa Nui) since 2010 , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16474, https://doi.org/10.5194/egusphere-egu25-16474, 2025.

The El Niño-Southern Oscillation (ENSO) influences the global temperature and precipitation patterns. Generally, the ENSO influence has been related to its amplitude. We use information-theoretic generalization of Granger causality to observe the causal influence of phases of ENSO oscillatory components on scales of precipitation variability in Yangtze and Yellow River basins, with a focus on its quasi-oscillatory dynamics spanning various timeframes. We find that the ENSO quasi-biennial component has a causal effect on precipitation variability on and around the annual scale, while the amplitude of the precipitation quasi-biennial component is controlled by low-frequency ENSO components with periods of around 6 years. This cross-scale causal information flow is particularly noticeable in the Yellow River basin, whereas in the Yangtze River basin, the ENSO amplitude has the greatest causative effect. The provided results indicate that different components of ENSO dynamics should be used to predict precipitation in different regions.

This study is supported by the Czech Academy of Sciences, Praemium Academiae awarded to M. Paluš.

Latif, Y., Fan, K., Wang, G., & Paluš, M. (2024). Cross-scale causal information flow from the El Niño–Southern Oscillation to precipitation in eastern China. Earth System Dynamics, 15(6), 1509-1526

How to cite: Latif, Y., Fan, K., Wang, G., and Paluš, M.: A cross-scale causal information flow from the El Niño–Southern Oscillation to precipitation in the Yangtze and Yellow River basins, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17086, https://doi.org/10.5194/egusphere-egu25-17086, 2025.

Rainfall intensification due to planetary warming is increasingly impacting nearly all regions of the globe. South America is no exception with unprecedented landslides (São Sebastião, February 2023) and river catchment-scale flooding (Rio Grande do Sul, September 2023 and May 2024) being observed more frequently. Over South America, tropical-extratropical cloud bands in the South Atlantic Convergence Zone (SACZ) produce most of the rainy season precipitation. Droughts can occur in years with fewer SACZ events while intensely raining clusters within the cloud bands can trigger flash floods and landslides. Here, we diagnose the impacts of future precipitation intensification on the frequency and intensity of SACZ tropical-extratropical cloud bands using the first-of-its-kind continental-scale convection-permitting climate simulation. While cloud bands will see a future 20-30\% decrease in their frequency, intense events with a likelihood of 1-in-5 in the present day will become more frequent in the future, with 3-in-5 likelihood, increasing the risk of heavily raining clusters. This tripling in intense cloud band frequency results from intensified mesoscale rainfall structures within the continental-scale cloud bands, a risk better captured by convection-permitting models. Geographically, the intensification of mesoscale rainfall structures is most prevalent in the highly populated coastal regions of Southeastern and Southern Brazil, areas already highly exposed to extreme weather events, floods, and landslides. This increased risk significantly exceeds the projections from traditional climate models with convection parametrizations and highlights the growing risk of intense cloud-band rainfall over South America under warming. 

How to cite: Zilli, M., Hart, N., Halladay, K., and Kahana, R.: Increased frequency of intense South Atlantic Convergence Zone-related cloud band events by 2100 in convection-permitting simulation , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17349, https://doi.org/10.5194/egusphere-egu25-17349, 2025.

EGU25-17361 | ECS | Orals | CL3.1.1

Changes in the Timing of the Thermal Spring Season Across Finland and Its Turning Point Over the Past Six Decades. 

Sadegh Kaboli, Ville Kankare, Ali Torabi Haghighi, Cintia Bertacchi Uvo, and Elina Kasvi

Thermal season variations contribute to shaping natural hydrological processes in Nordic regions. Although changes in seasonal hydro-climatological factors due to global warming at both global and regional scales have been widely studied, there remains a limited understanding of the timing characteristics of these seasonal shifts. Given the critical role of the annual temperature transition from the cold to the warm phase in controlling hydrological events in Nordic regions, this research focuses on the temporal variation of the thermal spring season across Finland. We investigate how the timing of the thermal spring has changed over the past six decades across Finland and how the changes vary spatially. We also identify temporal turning points in these transitions.

This research utilizes high-resolution (1x1 km) daily mean temperature data over Finland, spanning past six decades, publicly provided by the Finnish Meteorological Institute. Several indices were calculated based on a fixed thermal threshold to track both spatial and temporal variations in the thermal spring season, and to identify possible trends and correlations using various statistical methods. Temporal changes in the indices were analyzed using Mann-Kendall test, while the Theil-Sen estimator was applied to determine the slope of the observed trends. To mitigate the influences of potential autocorrelation in the dataset, the Trend-Free Pre-Whitening (TFPW) method was employed. For spatial analysis, Empirical Orthogonal Function (EOF) decomposition was used to identify dominant spatial pattens. To separate significant physical signals from noise in the estimated spatial patterns, the North significance test was used. Furthermore, the Pettitt test was applied to assess the turning points in spatial behavior of timing indices. By analyzing an extensive dataset covering Finland, coupled with a long data period, this research provides valuable insights into temporal shifts in the thermal spring season and their potential connections to other hydro-climatological factors.

How to cite: Kaboli, S., Kankare, V., Torabi Haghighi, A., Bertacchi Uvo, C., and Kasvi, E.: Changes in the Timing of the Thermal Spring Season Across Finland and Its Turning Point Over the Past Six Decades., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17361, https://doi.org/10.5194/egusphere-egu25-17361, 2025.

EGU25-17426 | ECS | Posters on site | CL3.1.1

Variability of spring temperature extremes in Europe 

Sophie Häfele, Johanna Baehr, Daniel Krieger, and Leonard Borchert

Spring in particular can carry impact-relevant extreme events over Europe, such as late frost or early summer heat. However, the dominating mechanisms and drivers of such temperature extremes in European springtime are currently not well understood. Across all seasons, one mechanism relevant for temperature extremes in Europe is atmospheric blocking. Unlike winter, where blocking is predominantly related to cold spells, and summer, where blocking is predominantly related to warm spells, spring is a transition period during which both cold and warm spells might be connected to blockings.

While this transition has been statistically analyzed before, available time series were limited, as was, in turn, the spatial analysis. Here, using ERA-5 and E-OBS for the period 1950-2023, with more than doubling the time series, we confirm existing literature on the statistics and the change of blocking patterns throughout the spring season, although our work indicates more early spring warm spells than previously found. The greater data availability also allows the spatial division into blocking regions, allows us to characterize the sensitivity of warm spell frequency to blocking location. We show that blockings over Scandinavia and the UK lead to Northern European warm spells. Comparing springtime occurrences of blocked and unblocked warm spell days shows that in Northern Europe, warm spells often occur simultaneously with blocking, whereas in Southern Europe, warm spells less frequently occur simultaneously with blocking. We identify temporal clusters of preferred occurrences of blocked or unblocked warm spell occurrences in Northern and Southern Europe to trace their seasonal drivers, thus indicating the potential for seasonal predictions of spring warm spells over Europe.

How to cite: Häfele, S., Baehr, J., Krieger, D., and Borchert, L.: Variability of spring temperature extremes in Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17426, https://doi.org/10.5194/egusphere-egu25-17426, 2025.

EGU25-19094 | Posters on site | CL3.1.1

Synoptic and Large-Scale Drivers of Extreme Precipitation Events in the Western Himalaya 

Pranab Deb, Priya Bharati, and Kieran Hunt

This study investigates the synoptic and large-scale atmospheric circulation associated with extreme precipitation events (EPEs) that occurred during the period 1979-2023 in the Western Himalaya (WH). These EPEs are defined as days when the mean precipitation exceeds the 99th percentile threshold of daily precipitation for each month from 1979 to 2023 across all grid points in the Indian Himalayan region (Karakoram, WH, Central and Eastern Himalaya). The weather regimes associated with these events are then classified using K-means clustering of geopotential height at 500hPa and vertical integrated moisture flux components. We have identified six clusters and determined that EPEs linked to four of these clusters predominantly occur during the monsoon months, whereas the other two clusters are characterized by WD (Western Disturbance)-driven EPEs that appear in the winter months. The EPEs in cluster-1 are mainly driven by the low-pressure system (LPS) in the Bay of Bengal and Rossby-wave breaking (atmospheric blocking by Siberian anticyclone) in the upper-atmosphere along with the midlatitude forcing of North Pacific Oscillation (NPO) (positive phase). The EPEs in clusters 2 and 5 resulted from a break in the monsoon caused by the northward displacement of LPS close to the Himalayan foothills, along with an omega type of blocking with a strong anticyclone over the WH, which is located between two cyclones. The midlatitude forcings of the negative phase of NPO and the negative phase of ENSO during EPEs in clusters 2 and 5, respectively, support the occurrence of EPEs in the WH. The EPEs in cluster-6 occurred due to incursion of a WD into the WH, along the northward migration of LPS in the break-monsoon phase over the WH; tropical forcing of positive phase of ENSO promotes the EPEs in this cluster. The WDs-driven clusters (cluster-3 and 4) mainly support higher amount of precipitation over the WH, and account for 80-95% of mean precipitation over the region, primarily driven by subtropical jet stream dynamics and upper-level trough over the WH. The EPEs in cluster-3 are linked with positive phase of North Atlantic Oscillation, while weaker Tibetan anticyclonic circulation is observed in the cluster-4 compared to cluster-3.

How to cite: Deb, P., Bharati, P., and Hunt, K.: Synoptic and Large-Scale Drivers of Extreme Precipitation Events in the Western Himalaya, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19094, https://doi.org/10.5194/egusphere-egu25-19094, 2025.

We show that the wintertime (December-January-February) North Pacific jet in ERA5 has shifted northwards over the satellite-era (1979-2023) at a faster rate than any of the state-of-the-art CMIP6 coupled climate models used in this study. Differences in tropical sea surface temperature (SST) trends can only partially explain the discrepancy in jet trends between models and observations and a small minority of simulations forced with observed SSTs match the magnitude of the observed jet trend. However, analysis of longer-term jet variability in reanalysis suggests that the jet trend has not clearly emerged from multi-decadal internal climate variability. Consequently, it is unclear whether the difference in observed and modelled jet trends arises due to differing responses to anthropogenic forcing or overly weak long-term internal variability in models. These results have important implications for future climate projections for North America and motivate further research into the underlying causes of long-term jet trends.

How to cite: Patterson, M. and O'Reilly, C.: Climate models struggle to simulate observed North Pacific jet trends, even accounting for tropical Pacific sea surface temperature trends, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19419, https://doi.org/10.5194/egusphere-egu25-19419, 2025.

EGU25-733 | ECS | Orals | AS1.30

Wintertime Transarctic Warm and Moist Air Intrusions Tracked in Present and Future Climate 

Eva Lüdke, Jan Landwehrs, Johannes Riebold, Sofie Tiedeck, and Annette Rinke

The Arctic region is strongly impacted by climate change. Poleward transport of warm and moist air is one of the mechanisms contributing to accelerated Arctic wintertime warming. Warm and moist air intrusions (WAIs) into the Arctic are often associated with warm extremes and positive surface energy balance (SEB) anomalies by increased longwave downward radiation (LWD), impacting sea ice extent and recovery. WAIs are expected to increase in frequency in a warming climate until the end of the century, but uncertainties remain regarding their life cycle characteristics, as well as their local impacts and seasonality.

This study focusses on intrusion events that travel from the Greenland and Barents Seas far through the central Arctic. These transarctic WAIs are identified as anomalously high column-integrated water vapor transport (IVT) events and are tracked in space and time with the MOAAP algorithm (Prein et al. 2023).

Focusing on boreal winter (DJF) the occurrence, impacts and life-cycle characteristics of transarctic intrusion events along their path are initially studied using ERA5 data. A first analysis identified 14 transarctic WAIs between 1979-2022, which on average travel 7500 km within a common lifetime of five days. We show that these events are associated with increased integrated water vapor (IWV), LWD, precipitation, and near-surface wind speeds over Arctic sea ice and that these effects become less pronounced towards the end of the WAIs lifecycle. 

Furthermore, we find that during the transarctic WAI’s onset stage in the Greenland and Barents Seas, the associated transport of moist air masses towards the central Arctic is dynamically driven by a strong Icelandic low linked to a positive NAO state or a Scandinavian blocking. As these pressure patterns gradually shift northwards, the WAIs are directed through the Arctic, eventually reaching the Beaufort or East Siberian Seas.

The upcoming analysis will be extended by using data from regional Arctic model simulations with the atmospheric model ICON. Those are forced with ERA5 and two selected global CMIP6 climate models under the SSP370 scenario. The latter represent two distinct Arctic warming scenarios until the end of the century. This allows to assess future changes of transarctic WAIs and their impacts under different future Arctic warming storylines.

How to cite: Lüdke, E., Landwehrs, J., Riebold, J., Tiedeck, S., and Rinke, A.: Wintertime Transarctic Warm and Moist Air Intrusions Tracked in Present and Future Climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-733, https://doi.org/10.5194/egusphere-egu25-733, 2025.

Processes controlling the timing of the Arctic sea ice melt onset still remain unclear, but possible factors include variations in atmospheric circulation patterns and anomalies in clouds, moisture and surface energy budget, all of which are linked to narrow bands of warm and moist-air advection. These filaments, accounting for the majority of the poleward moisture transport, are called Atmospheric Rivers (ARs). Although spring is an important transition period for the sea ice evolution, there are hardly any in-situ observations in the Arctic Ocean for that period. To narrow down the knowledge gaps, the ARTofMELT expedition took place on the Swedish research Icebreaker Oden in the Fram Strait in May-June 2023 with two main objectives: to study processes leading up to the melt onset of Arctic sea ice and to investigate the role of ARs in affecting this timing. This study is motivated by the ARTofMELT expedition, during which the observed surface temperature exceeded the melting point on the 10th of June 2023 – much later than expected. Questions raised were “was this an anomalously late melt onset?” and “if yes, why?”. To address these questions, we put the year 2023 into a climatological (1981-2020) perspective by linking satellite-derived melt-onset (MO) dates with large-scale circulation features. Due to lack of MO-dates along the track in June 2023, the location of Oden during ARTofMELT is represented by a “Fram Strait sector”. Years are categorized into early and late MO-years based on the relative number of significant MO-anomalies within the sector.

The melt onset timing in the sector within the climatological period has a significant negative trend of -5 days in 10 years. In spring 2023, the average melt onset occurs on 8 June, corresponding to a MO-anomaly of almost 2 weeks relative to a transient climatology. As nearly 60 % of all grid-points obtain significant positive MO-anomalies and only a negligible fraction has significant negative MO-anomalies, we conclude that the melt onset in the sector region during ARTofMELT in spring 2023 was anomalously late.

The period before the MO in the sector was characterized by significant negative SLP anomalies over the whole Arctic Ocean and positive anomalies in SLP and atmospheric blocking over Eurasia. These circulation anomalies were associated with a strong cyclonic activity along the sea ice edge, directing warm and moist air, and most of the ARs, east of Svalbard into the BKS region – leading to an early MO there. The central Arctic Ocean was anomalously dry. The circulation patterns weakened and rather normal conditions prevailed during the MO period in the Fram Strait, where the MO was finally triggered by a transient AR on 10 June 2023.

Analysis between six most extreme early and late MO-years reveal that specific circulation patterns favoring moist and warm air transport towards and the occurrence of ARs within the Fram Strait sector are of more importance in determining the timing of MO for extreme early MO-years, whereas extreme late MO-years seem to be due to an absence of such large-scale features.

How to cite: Murto, S. and Tjernström, M.: ARTofMELT spring 2023 expedition: Investigating the Arctic sea ice melt onset in the context of climatology and atmospheric circulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1741, https://doi.org/10.5194/egusphere-egu25-1741, 2025.

EGU25-2319 | ECS | Orals | AS1.30

Regional and Temporal Variability of Atmospheric River Seasonality: Influences of Detection Algorithms and Moisture Transport Dynamics 

Diya Kamnani, Travis A. O'Brien, Samuel Smith, Paul W. Staten, and Christine A. Shields

Understanding the regional and temporal variability of atmospheric river (AR) seasonality is crucial for preparedness and mitigation of extreme events. While ARs were thought to peak in winter, recent research shows they exhibit region-specific seasonality and are heavily influenced by the chosen detection algorithm. This study examines the link between the year-to-year consistency of peak AR activity to the presence of a dominant seasonal pattern, considering both location and algorithm choice. Regions are categorized by their temporal characteristics: consistent patterns (e.g., India, Central Asia), patterns with occasional outliers (e.g., British Columbia coast, Gulf of Alaska), and regions lacking a clear dominant peak season (e.g., South Atlantic, parts of Australia). Hence, not all regions display a consistent seasonal cycle of AR activity. This study quantifies the extent to which a region experiences a dominant peak season of AR activity (or lacks one) and offers insights to enhance decision-making in water management, natural hazard preparedness, and forecasting. Furthermore, given our finding that detection algorithms influence the peak season of AR activity, we also examine two diagnostic variables representative of moisture transport to corroborate our results. Integrated Vapor Transport, which captures meridional and zonal moisture transport, and Moist Wave Activity, representing moisture intrusions from lower to higher latitudes, are examined. Our analysis indicates that inconsistencies in the seasonal cycle of AR activity are not solely due to discrepancies in detection algorithms but also arise from changes in moisture transport.

How to cite: Kamnani, D., O'Brien, T. A., Smith, S., Staten, P. W., and Shields, C. A.: Regional and Temporal Variability of Atmospheric River Seasonality: Influences of Detection Algorithms and Moisture Transport Dynamics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2319, https://doi.org/10.5194/egusphere-egu25-2319, 2025.

EGU25-2964 | ECS | Orals | AS1.30 | Highlight

Global scale impact of atmospheric rivers on the severity of flooding  

Sucheta Pradhan, Conrad Wasko, and Murray Peel

Atmospheric rivers (ARs) are narrow, elongated corridors of concentrated moisture that transport substantial amounts of water vapour from the tropics to the mid-latitudes. These meteorological phenomena are known to significantly influence extreme precipitation events and are often linked to major flood occurrences. Despite their recognized importance in regional hydrology, the overall contribution of ARs to global flood risk—the hazard posed by extreme precipitation events—has not been comprehensively quantified. In this study, we assess the relationship between ARs and extreme hydrological events using data from 2686 largely regulation-free catchments distributed across the globe. Our findings reveal that on a regional scale, ARs are responsible for over 70% of the largest precipitation and streamflow events in the last four decades. Furthermore, AR-related precipitation leads to a significant reduction in the recurrence intervals of these extreme events, increasing the likelihood of large-scale flooding by a factor of 2 to 4. In certain regions, such as parts of North America, Europe, and Australia, rare flood events are up to 12 times more likely when ARs are present. These results underscore the critical role that ARs play in driving the frequency and severity of extreme hydrological events globally. Our findings highlight the need for greater attention to the influence of ARs on flood risk, particularly as climate change may alter their frequency and intensity in the future.

How to cite: Pradhan, S., Wasko, C., and Peel, M.: Global scale impact of atmospheric rivers on the severity of flooding , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2964, https://doi.org/10.5194/egusphere-egu25-2964, 2025.

The Arctic has witnessed significant sea-ice melt and rising temperatures as major indicators of climate system alterations. As a severe weather event conveying heat and moisture from lower latitudes to the higher, atmospheric rivers (ARs) can lead to significant sea-ice loss and Arctic warming. Sea ice thickness is applied in this study to quantitatively explored the thermodynamic and dynamic impacts of ARs in winters from 2000 to 2020. ARs from the North Atlantic (AAR) and North Pacific (PAR) account for 44% of AR events and 40% of AR-driven sea-ice loss. The AR-induced melting process occurs in three successive stages. In Stage I, warm, moist air driven by dipole circulation anomalies ahead of AR causes sea ice melting, with thermal effects accounting for 53% for AAR and 58% for PAR. Stage II starts when the AR enters the Arctic and ends as its moisture transport weakens. Early sea-ice loss is driven by wind dynamics, while poleward progression elevates warm, moist air, forming clouds that intensify melting thermodynamically. This stage sees the most significant sea-ice melt, dominated by dynamic effects for AAR (59%) and thermodynamic effects for PAR (55%).In Stage III, as AR moisture dissipates, sea-ice melt continues for about a week, primarily driven by thermodynamic effects. Accompanied by the above three stages, the anticyclonic circulation anomaly on the right side of where AR is headed can also enhance downdrafts and melt perennial ice. By contrast, Pacific-channel ARs have a higher impact on the central Arctic than their Atlantic counterparts, suggesting extensive responses to climate variability.

How to cite: Gong, Z.: Dynamic and thermodynamic impacts of atmospheric rivers on sea-ice thickness in the Arctic since 2000, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3436, https://doi.org/10.5194/egusphere-egu25-3436, 2025.

Atmospheric rivers (ARs) play an important role in both the global and regional climate systems. While there is extensive research on ARs and their relationship to precipitation in North America and East Asia, the role of ARs in the regional climate of Scandinavia remains understudied.

In this study, we investigated the characteristics of ARs making landfall over Scandinavia, their influence on regional precipitation, and how they are affected by the North Atlantic Oscillation (NAO). To achieve this, we analysed the ARs between 1980 and 2019 detected by four different AR Detection and Tracking algorithms (ARDT), from the Atmospheric River Tracking Method Intercomparison Project (ARTMIP). Combined with ERA5 reanalysis precipitation data, we quantified the AR related precipitation over the region.

We found that ARs are present during up to 35% of the total annual precipitation in Scandinavia, with the average AR-associated rainfall rate exceeding the non-AR rates. Clustering the ARs that intersect Scandinavia revealed four main AR patterns. For the two most frequent patterns, located in southern Scandinavia, ARs account for up to 32% of the total annual precipitation. Furthermore, for all patterns, AR activity reaches a maximum during autumn and whilst the NAO is in a strong positive phase. The results from the four ARDTs show similar spatial patterns, but with a notable difference in the magnitude of AR influence on precipitation. Our findings indicate that ARs are an important factor in Scandinavian precipitation, and highlight the value of using multiple ARDTs to obtain more robust results. 

How to cite: Holmgren, E. and Chen, H.: Spatial and temporal characteristics of atmospheric rivers in Scandinavia and their influence on the regional precipitation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3577, https://doi.org/10.5194/egusphere-egu25-3577, 2025.

EGU25-3695 | ECS | Posters on site | AS1.30

The Global Atmospheric River Network: A Complex Network Approach to Global Moisture Transport Dynamics 

Tobias Braun, Sara M. Vallejo-Bernal, Norbert Marwan, Juergen Kurths, Sebastian Sippel, and Miguel Mahecha

The increasing frequency and severity of hydrological extremes, such as heavy precipitation events, are significant challenges for human-environmental systems. Atmospheric rivers (ARs) are key drivers of these extremes, but the complex transport patterns of ARs at global scale remain underexplored. Our research introduces a novel network-based approach to studying global AR dynamics, applying methods from complexity science to reveal the “global road network” of ARs.

In analogy to terrestrial river networks, the pathways that ARs follow through the Earth’s atmosphere can be effectively represented by a transport network. Generally, the paradigm of complex networks encodes interactions between the units of a system through interlinked nodes. Recent applications illustrate that complex networks have provided novel insights into climate teleconnection patterns, synchronization of extremes and vegetation-atmosphere feedbacks. We draw on the vast array of existing methods from complex network theory to reveal the global atmospheric river network. We define it on a hexagonal grid to avoid distortions due to the Earth’s spherical geometry. Multiple AR catalogs can be integrated seamlessly. To quantitatively assess the significance of a transport property, the framework is equipped with a hierarchy of data-adaptive null models that are based on random walker ensembles.

We dissect the global transport infrastructure of ARs which reveals prominent AR pathways, regions of complex multi-directional transport, the predictability of single AR tracks, and scale-dependent spatial clusters. We demonstrate that there exists complexity above and beyond the previously identified four main branches of AR transport. These main oceanic bands can be decomposed into significant sub-branches. Exploiting all these novel tools to characterise AR transport, we unveil how the AR network is evolving in a changing climate. This talk underscores the potential of complexity science to advance our understanding of ARs as critical components of the integrated human-Earth system.

How to cite: Braun, T., Vallejo-Bernal, S. M., Marwan, N., Kurths, J., Sippel, S., and Mahecha, M.: The Global Atmospheric River Network: A Complex Network Approach to Global Moisture Transport Dynamics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3695, https://doi.org/10.5194/egusphere-egu25-3695, 2025.

EGU25-5904 | ECS | Orals | AS1.30

Investigating the Role of Anomalous Moisture Transport in Indian Subcontinent's Extreme Precipitation Events: A PIKART Perspective 

Sree Anusha Ganpathiraju, Sara M. Vallejo-Bernal, Norbert Marwan, and Maheswaran Rathinasamy

The dynamics of atmospheric moisture transport plays a dominant role in understanding the physical mechanisms that lead to extreme precipitation events (EPEs). In mid-latitudes, 90% of poleward moisture transport occurs along transient channels known as atmospheric rivers. However, due to the complex interactions of regional weather systems, they are challenging to define, detect, and analyze in tropical regions. In this context, the PIK Atmospheric River Trajectories (PIKART) catalog offers a unique capability to detect coherent channels of intense moisture transport, particularly in the tropical region. These are referred to as anomalous moisture transport pathways (AMTPs) to ensure clarity and avoid ambiguity. The existence of AMTPs in the tropics remains an open question and the role of their differentiated atmospheric dynamics in driving EPEs across the Indian subcontinent is yet unclear. To address this, we employ a novel database of EPEs created using the weather extremity index coalesced with the peak over threshold method, together with the PIKART catalog. We systematically identify the co-occurrence of AMTPs and EPEs in the Indian subcontinent. Our results reveal that among the top 100 EPEs, more than 47% displayed AMTPs. To understand the contribution of AMTPs to the severity of EPE, we also present a case study of the 2018 Kerala floods, for which the presence of an AMTP has been documented. Although previous studies identified an AMTP on August 13, 2018, we detected the occurrence of an earlier one on August 9, 2018, preceding the landfall of the event that unfolded between August 13 and 17, 2018. The decomposition of moisture contributions indicates that over 45% of the total moisture is attributed to this earlier AMTP trajectory, suggesting enhancement in the monsoon circulation. Our results shed light on the concept of AMTP in the tropics and contribute to comprehend its influence on climate extremes, a critical task to improve risk management and develop mitigation strategies.

How to cite: Ganpathiraju, S. A., M. Vallejo-Bernal, S., Marwan, N., and Rathinasamy, M.: Investigating the Role of Anomalous Moisture Transport in Indian Subcontinent's Extreme Precipitation Events: A PIKART Perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5904, https://doi.org/10.5194/egusphere-egu25-5904, 2025.

EGU25-6689 | Orals | AS1.30

The NCEI Climate Data Record for Atmospheric Rivers: Initial Results over the Western United States 

Emily Slinskey, Jonathan Rutz, Bin Guan, and F. Martin Ralph

The U.S. National Centers for Environmental Information (NCEI) is sponsoring development of an atmospheric river (AR) climate data record (CDR) to serve as a valuable resource for the scientific, water management, and decision-making communities across the Western US (and soon, globally). The CDR uses a novel combination of two techniques: (1) the AR Scale, which broadly characterizes the AR strength from 1-5 based on the peak integrated water vapor transport (IVT) and duration of AR conditions (i.e., IVT ≥ 250 kg m-1 s-1) at a given location, and (2) the tARget algorithm–a tool that uses climatological, geometric, and directional thresholds to identify ARs. Since the AR scale has no geometric criteria (and thus ranks non-AR events such as tropical cyclones, cutoff lows, and monsoons) and tARget does not provide characterization of AR strength, these two methods complement each other, with AR Scale-identified events “filtered” by tARget. This presentation highlights the resulting data and effects of this “filtering” through selected cases, long-term climatology, and interannual variability across various global regions. In addition, we explore attribution of precipitation to AR events identified in the CDR. All historical atmospheric data is sourced from the ERA5 reanalysis.

How to cite: Slinskey, E., Rutz, J., Guan, B., and Ralph, F. M.: The NCEI Climate Data Record for Atmospheric Rivers: Initial Results over the Western United States, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6689, https://doi.org/10.5194/egusphere-egu25-6689, 2025.

EGU25-7213 | ECS | Orals | AS1.30

Identifying Antarctic Atmospheric River Families 

Michelle Maclennan, Jimmy Butler, Becca Baiman, Grant LaChat, and Christine Shields

Despite their rarity, atmospheric rivers (ARs) bring powerful impacts to Antarctica when they make landfall on the ice sheet. Antarctic ARs contribute 10% of the annual precipitation and are major drivers for heatwaves, foehn events, and surface melting on ice shelves. While snowfall is currently the dominant impact of Antarctic ARs, helping to offset sea level rise due to ice discharge from West Antarctica, the relative contribution of ARs to snowfall, rainfall, and surface melt may change in a warming climate, along with the frequency and intensity of AR events themselves, motivating the study of these rare, impactful events. In this study, we examine the occurrence of Antarctic AR families, in which two or more ARs occur in rapid succession in a region. While individual ARs have been shown to have pronounced and widespread impacts in Antarctica, latent heat release from ARs in a family can reinforce associated downstream high-pressure systems to produce extended, high impact AR conditions on the ice sheet, including multiple days of intense snowfall and temperatures above the melting point. Here we present initial results from an Antarctic-wide study of the occurrence and impacts of AR family events. First, we use a density-based clustering algorithm to classify AR events as objects from an Eulerian, Antarctic-specific detection tool based on MERRA-2 reanalysis. From this, we construct a database of AR events around Antarctica from 1980-2022, with information on the location, duration, and landfall (if it occurred) for each AR. Then, we cluster the AR events by location and time once more, to identify the occurrence of AR family events. We explore the sensitivity of the number of AR family events detected, and the number of ARs per family, to the chosen aggregation period (two to six days) and distance parameter (500 – 1000 km). Finally, we utilize a novel atmospheric Rossby wave breaking detection tool to compare the frequency of cyclonic and anticyclonic wave breaking events over the Southern Ocean to the frequency of AR family and non-family events. Ultimately, our study aims to diagnose the occurrence, synoptic drivers, characteristics, and impacts of AR family events on the Antarctic Ice Sheet in the last four decades, to provide a baseline assessment of how these extreme events can compound to produce lasting, high-impact conditions.

How to cite: Maclennan, M., Butler, J., Baiman, B., LaChat, G., and Shields, C.: Identifying Antarctic Atmospheric River Families, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7213, https://doi.org/10.5194/egusphere-egu25-7213, 2025.

EGU25-8024 | Orals | AS1.30

Atmospheric rivers in the Mediterranean basin and heavy precipitation over northern Italy 

Silvio Davolio, Isacco Sala, Alessandro Comunian, Daniele Mastrangelo, Sante Laviola, Giulio Monte, Barbara Tomassetti, Annalina Lombardi, Marco Verdecchia, Federico Grazzini, and Valentina Colaiuda

Recent studies of extreme precipitation and flood events affecting the Alpine area in northern Italy have revealed that besides the local contribution due to evaporation from the Mediterranean Sea, a relevant amount of moisture may move from remote areas towards the Mediterranean within long and narrow filament-shaped structures, known as atmospheric rivers.

High-resolution numerical simulations have demonstrated that the presence of an intense atmospheric river, whether coming from Africa tropical areas or from the Atlantic, represented a distinguishing aspect of those events, superimposed on the well-known mesoscale dynamic mechanisms of heavy precipitation over the Alps. The orographic uplift of water vapour transported by the atmospheric rivers represented a critical ingredient for the occurrence of extreme rainfall, and the characteristics of the atmospheric rivers determined the distribution and the intensity of the precipitation.

In order to investigate further the possible link between atmospheric rivers across the Mediterranean basin and high-impact weather, a detection algorithm, designed for the open oceans, has been adapted to the peculiar complex morphology of the region. It has been applied to conduct a climatological analysis on the presence of atmospheric rivers in the Mediterranean, exploiting ERA5 reanalysis, and to assess their relationship with extreme rainfall events over northern Italy during the last decades, exploiting a precipitation dataset with raingauge observations aggregated over civil protection warning areas. The study is undertaken in the framework of the national project ARMEX, funded by the Italian Ministry of Universities and Research, which involves also expertise in remote sensing and hydrological modelling to fully investigate characteristics and hydro-meteorological impact of atmospheric river over the national territory.

How to cite: Davolio, S., Sala, I., Comunian, A., Mastrangelo, D., Laviola, S., Monte, G., Tomassetti, B., Lombardi, A., Verdecchia, M., Grazzini, F., and Colaiuda, V.: Atmospheric rivers in the Mediterranean basin and heavy precipitation over northern Italy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8024, https://doi.org/10.5194/egusphere-egu25-8024, 2025.

EGU25-9886 | ECS | Posters on site | AS1.30

Gulf Stream Ocean Conditions Influence on Atmospheric Rivers 

Ferran Lopez-Marti, Arnaud Czaja, Gabriele Messori, Lichuan Wu, and Anna Rutgersson

Extreme precipitation and wind events in Western Europe are driven by Atmospheric Rivers (ARs) developing over the North Atlantic Ocean. While extensive research has been conducted on the atmospheric dynamics of ARs in this region and their connection with the North Atlantic Storm Track, gaps persist in understanding how oceanic variability influences AR activity, particularly in the eddy-rich environment of the Gulf Stream extension. The enhanced ocean heat supply and high mesoscale eddy activity over these western oceanic currents increase the surface latent heat flux in the area, thereby increasing moisture availability in the lower atmosphere and potentially facilitating AR genesis.

This study focuses on evaluating the status of mesoscale eddies and oceanic conditions within the Gulf Stream extension and their downstream impact on AR activity. To achieve this, we employ a high-pass Fourier Filter Transformation to isolate and quantify the mesoscale eddy activity (smaller than ~500 km) of the Gulf Stream extension region in a high-resolution (0.125º) satellite product for the sea surface height. Additionally, we utilise different observational products (OAFlux, ARGO and RAPID) to quantify the surface heat fluxes, the ocean heat content in the Gulf Stream extension region and the oceanic heat supply through the Florida Straight. Finally, we identify and track Atmospheric Rivers in the ECMWF reanalysis ERA5 dataset over the North Atlantic.

Our analysis provides a spatial and temporal cross-correlation analysis between the Gulf Stream state and the AR activity downstream. Furthermore, we investigate temporal lags between various oceanic conditions and their impact on ARs, thereby identifying oceanic precursors for AR genesis. Consequently, our study establishes a novel statistical relationship between Gulf Stream state and AR activity, with a particular emphasis on the role of mesoscale features. This includes a comprehensive characterisation of mesoscale eddy activity within the region, contributing to a deeper understanding of the mechanisms driving AR formation and propagation in Western Europe.

How to cite: Lopez-Marti, F., Czaja, A., Messori, G., Wu, L., and Rutgersson, A.: Gulf Stream Ocean Conditions Influence on Atmospheric Rivers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9886, https://doi.org/10.5194/egusphere-egu25-9886, 2025.

EGU25-12461 | ECS | Orals | AS1.30

Unravelling the sources of moisture for precipitation in atmospheric rivers 

Alfredo Crespo-Otero, Damián Insua-Costa, and Gonzalo Míguez-Macho

Atmospheric rivers (ARs) are filaments of enhanced moisture in the atmosphere, which often produce intense or even extreme precipitation when the enormous amounts of water vapor in them are forced upwards. In this sense, one of their most studied and debated properties is the origin of the moisture they transport. Although some studies have identified sources using different diagnostic tools for specific AR cases, it remains unclear whether tropical or extratropical contributions are generally more prevalent, and even the AR definition in the Glossary of Meteorology reflects this lack of consensus.

To fill this gap, a climatology of moisture sources for precipitation in ARs is needed. There are a variety of moisture source diagnostics that can be employed to address this issue. Here we use the Lagrangian model FLEXPART together with an implementation of the Dirmeyer and Brubaker, (1999) methodology, which we previously validated using the WRF with Water Vapor Tracers (WRF-WVTs) model. This allows us to efficiently simulate air particle trajectories and compute moisture sources for precipitation within a wide range of ARs with a Lagrangian methodology, while maintaining consistency with the WRF-WVTs model, assumed to be one of the most accurate moisture tracking tools. Preliminary results reveal a wide diversity of moisture sources, including both oceanic and continental regions, with substantial variability in their contributions across different AR cases. Importantly, our findings also indicate a less relevant role of tropical moisture than previously known. Ultimately, this highlights the complexity of the moisture uptakes in ARs.

Dirmeyer, P. A. and Brubaker, K. L.: Contrasting evaporative moisture sources during the drought of 1988 and the flood of 1993, J. Geophys. Res. Atmospheres, 104, 19383–19397, https://doi.org/10.1029/1999JD900222, 1999.

How to cite: Crespo-Otero, A., Insua-Costa, D., and Míguez-Macho, G.: Unravelling the sources of moisture for precipitation in atmospheric rivers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12461, https://doi.org/10.5194/egusphere-egu25-12461, 2025.

EGU25-14595 | ECS | Posters on site | AS1.30

Atmospheric Rivers as Interacting Elements of the Earth System: A Complexity Science Perspective 

Sara M. Vallejo-Bernal, Tobias Braun, Norbert Marwan, Ana Bastos, Miguel D. Mahecha, and Jürgen Kurths

The critical role of atmospheric rivers (ARs) in the global water cycle, along with their intensification under global warming, underscores the urgency of understanding and predicting their dynamics and impacts at both regional and global scales. Despite significant advances, this endeavor remains challenging because ARs lie at the interface of weather and climate. These synoptic-scale systems produce short-term, localized impacts while shaping long-term global patterns of moisture, wind, and precipitation. AR genesis and evolution emerge from interactions within the coupled ocean-atmosphere system, while AR-induced precipitation can lead to natural disasters through land-atmosphere interactions. By transporting vast amounts of moisture over great distances, ARs establish teleconnections that influence weather across thousands of kilometers. At the same time, their activity is shaped by large-scale climate phenomena such as the El Niño–Southern Oscillation and the Pacific Decadal Oscillation. Advancing AR science, therefore, requires treating ARs as integral components of the Earth system and unraveling their interactions across a broad range of spatial and temporal scales.

In this talk, we present and discuss the paradigm of complexity science and the exciting opportunities it offers for advancing AR science. Building on a solid foundation of dynamical systems, stochastic climate theory, and network theory, complexity science integrates nonlinearities, feedbacks, and uncertainties into the study of ARs. By employing novel methods such as event synchronization, climate networks, and probabilistic causation, complexity science provides powerful tools to investigate non-local interactions, uncover hidden dynamics, and refine impact attribution in AR research. To ensure the robustness of findings, complexity science integrates null models, hypothesis testing, confidence bounds, and sensitivity analyses. Emerging research avenues, such as AR networks, community detection, low-order modeling, and tipping dynamics, can now be explored through the lens of complexity science. By establishing a rigorous theoretical and methodological foundation, complexity science paves the way for innovative research on AR dynamics, impacts, and prediction.

 

How to cite: Vallejo-Bernal, S. M., Braun, T., Marwan, N., Bastos, A., Mahecha, M. D., and Kurths, J.: Atmospheric Rivers as Interacting Elements of the Earth System: A Complexity Science Perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14595, https://doi.org/10.5194/egusphere-egu25-14595, 2025.

EGU25-14684 | Orals | AS1.30

Atmospheric River Over the Middle East  

Diana Francis, Ricardo Fonseca, and Narendra Nelli

Atmospheric Rivers (ARs) are narrow and long bands of high water vapour content, which largely originate in the tropics or subtropics and propagate into mid- and high-latitudes. They can bring beneficial rain and snow but, in particular the most intense, can lead to catastrophic flooding and loss of life. One of such occurrences in the Middle East in mid-April 2023 is investigated using model and observational data. The high-resolution (2.5 km) simulation put in evidence narrow (5-15 km) and long (100-200 km) convective structures within the AR, known as AR rapids, which produced heavy precipitation (>4 mm hr-1), further enhanced by gravity waves that developed over the high terrain in western Saudi Arabia, and propagated at high speeds (>30 m s-1). ARs are occurring more frequently in the Middle East as they are globally, and with increased atmospheric water vapour in a warming climate, AR rapids may be even more destructive.

How to cite: Francis, D., Fonseca, R., and Nelli, N.: Atmospheric River Over the Middle East , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14684, https://doi.org/10.5194/egusphere-egu25-14684, 2025.

Atmospheric Rivers (ARs) play a critical role in the Arctic climate system, providing the majority of water vapor transport into the Arctic. The potential of such events to impact especially the ice-covered regions of the Arctic have been explored in recent studies: ARs can trigger surface melt of the Greenland ice sheet and slow the seasonal recovery of the Arctic ice sheet. Furthermore, the low Arctic sea-ice extents of the years 2012 and 2020 could be linked to a more frequent occurrence of ARs. These case studies highlight the warming effect of individual cases of ARs.

We statistically investigate the warming effect of ARs on the Arctic sea-ice and ocean surface by examining anomalies in the atmospheric part of the surface energy budget (SEB). This climatological analysis is based on the ERA5 reanalysis from 1979 to 2021. ARs are detected using the algorithm by Guan and Waliser. Overall, a net energy gain of the surface associated with the occurrence of ARs is found, with the highest anomalies in winter over the open ocean. For a deeper understanding of the impact, complementary information on the climatological relevance of these events for the SEB is provided. Furthermore, we analyze the physical processes leading to the AR-related SEB anomalies, explaining the seasonal changes and the dependence of the anomalies on the surface type.

Within the rapidly changing Arctic climate, also changes in AR occurrence and their impact on the SEB can be expected. We investigate these changes by comparing the “old Arctic” (1979-1999) with the “new Arctic” (2000-2021). An overall increase in the occurrence frequency of ARs is found. Changes in the AR-related SEB anomalies are mostly linked to sea-ice decline.

How to cite: Tiedeck, S. and Rinke, A.: Arctic Atmospheric Rivers: An in-depth Investigation of their Impact on the Surface Energy Budget, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18198, https://doi.org/10.5194/egusphere-egu25-18198, 2025.

EGU25-18254 | ECS | Orals | AS1.30

Relationship between atmospheric rivers and aerosol atmospheric rivers in the Iberian Peninsula 

Diogo Luís, Irina Gorodetskaya, and Carla Gama

Recently, the water vapour atmospheric river (AR) concept was extended to aerosols, introducing the term aerosol atmospheric river (AAR) into the literature. Equivalently to ARs, AARs are narrow and transient filaments of intense aerosol transport in the lower troposphere. The Iberian Peninsula (IP) is one of the regions regularly affected by ARs and is also frequently impacted by Saharan dust outbreaks. While the impacts of ARs in the IP were extensively studied, there is a lack of regional studies on the impact of AARs in the IP. Moreover, the relationship between ARs and AARs in the IP has not yet been investigated. Therefore, this work aims to better understand the relationship between ARs and AARs in the IP and to quantify the co-occurrence of these phenomena. In this sense, a modified algorithm originally designed to detect ARs was applied to the Modern-Era Retrospective analysis for Research and Applications, version 2 (MERRA-2) reanalysis in order to identify the AARs that affected the IP over a 20-year period. Five aerosol types were used: dust, sea salt, sulphate, organic carbon and black carbon. In this presentation, we will show and discuss the climatology, the seasonality, and the characteristics of each type of Iberian AAR and how often these events are associated with ARs. This work contributes to a better understanding of the differences between ARs and AARs, as these phenomena share similarities but can also have different origins and trajectories.

 

This work was supported by the Portuguese Foundation for Science and Technology (FCT) through a PhD grant (2023.03574.BD) for Diogo Luís.

How to cite: Luís, D., Gorodetskaya, I., and Gama, C.: Relationship between atmospheric rivers and aerosol atmospheric rivers in the Iberian Peninsula, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18254, https://doi.org/10.5194/egusphere-egu25-18254, 2025.

EGU25-20603 | ECS | Orals | AS1.30

Response of sea surface temperature to atmospheric rivers 

Tien-Yiao Hsu, Matthew Mazloff, Sarah Gille, Mara Freilich, Rui Sun, and Bruce Cornuelle

Atmospheric rivers (ARs), responsible for extreme weather conditions, are mid-latitude systems that can cause significant damage to coastal areas. While forecasting ARs beyond two weeks remains a challenge, past research suggests potential benefits may come from properly accounting for the changes in sea surface temperature (SST) through air–sea interactions. In this paper, we investigate the impact of ARs on SST over the North Pacific by analyzing 25 years of ocean reanalysis data using an SST budget equation. We show that in the region of strong ocean modification, ocean dynamics can offset over 100% of the anomalous SST warming that would otherwise arise from atmospheric forcing. Among all ocean processes, ageostrophic advection and vertical mixing (diffusion and entrainment) are the most important factors in modifying the SST tendency response. The SST tendency response to ARs varies spatially. For example, in coastal California, the driver of enhanced SST warming is the reduction in ageostrophic advection due to anomalous southerly winds. Moreover, there is a large region where the SST shows a warming response to ARs due to the overall reduction in the total clouds and subsequent increase in total incoming shortwave radiation.

How to cite: Hsu, T.-Y., Mazloff, M., Gille, S., Freilich, M., Sun, R., and Cornuelle, B.: Response of sea surface temperature to atmospheric rivers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20603, https://doi.org/10.5194/egusphere-egu25-20603, 2025.

Global chemical transport models often overestimate stratospheric methane concentrations due to inaccuracies in simulating stratospheric circulation. If uncorrected, these biases can distort inverse analyses of satellite methane column observations (e.g., GOSAT), which encompass contributions from both the troposphere and stratosphere, and lead to erroneous estimates of surface emissions and tropospheric sinks. In this study, we assess the impact of stratospheric biases on the global inversion of satellite column observations. We implemented several correction methods, including empirically derived polynomial corrections, age-of-air proxies, and both offline and online replacements of stratospheric methane fields with independent observations. Correcting for stratospheric biases on average resulted in a 22 Tg a-1 increase in inferred global methane emissions from GOSAT data, with notable latitudinal shifts. The correction increased extratropical emissions by 46 Tg a-1 but decreased tropical emissions by 24 Tg a-1. Different correction methods varied in their impact on the inversion estimates of emissions and OH concentrations, underscoring uncertainties in bias correction. Our results also indicate that stratospheric biases can induce tropospheric biases in the simulation through stratosphere-troposphere exchange, potentially affecting the analysis of surface methane observations.

How to cite: Zhang, P., Zhang, Y., and liang, R.: Correction of simulation biases in stratospheric methane concentrations for the inverse analysis of satellite column observations , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1327, https://doi.org/10.5194/egusphere-egu25-1327, 2025.

Using observations, reanalysis data sets, a linear barotropic model, and a state-of-art chemistry-climate model, we investigated the influence of Arctic stratospheric polar vortex (SPV) and ozone variabilities on surface air temperature (SAT) and precipitation in Asia. An out‐of‐phase interannual linkage between the SPV in December‐January and SAT in February during 1979–2022 has been observed, that is, a strong (weak) SPV corresponds to a cooling (warming) over Asia. This relationship is independent of the Arctic Oscillation. The influence of the SPV on SAT over Asia cannot be solely explained by radiative processes, but is instead related to circulation anomalies in the troposphere. Specifically, the influence of the SPV on Asian SAT is mediated through the "downward control" mechanism. A strong SPV signal propagates downward to the Atlantic sector, weakening the Northeast Atlantic-East Europe-Asia tripolar teleconnection wave train. This weakens planetary wave propagation from the North Atlantic to Asia, leading to negative geopotential height anomalies and cyclonic circulation anomalies over the region. These circulation anomalies, accompanied by anomalous northerly winds, are beneficial to the colder air transportation from the higher latitudes to Asia, facilitating a surface cooling over Asia. We also found the robust influences of March Arctic stratospheric ozone (ASO) on the differences in the precipitation and evaporation in April over Eastern China. When ASO decreases in March, it tends to result in a higher and colder tropopause in the polar, a stronger subtropical jet stream, an intensified local Hadley circulation accompanied by anomalous downward motion over Eastern China, and consequently, drying in this region, and vice versa. These findings suggest that Arctic stratospheric variability could serve as potential predictors for temperature and precipitation changes in East Asia.

How to cite: Hu, D.: Impacts of stratospheric polar vortex and ozone on surface air temperature and precipitation over Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1606, https://doi.org/10.5194/egusphere-egu25-1606, 2025.

Anomalies in the stratospheric polar vortex (SPV), such as sudden stratospheric warming (SSW) events, significantly impact surface weather patterns. While the general influence of SSWs on the troposphere is robust, individual events exhibit large variability, partly due to the substantial difference in dynamics and SPV evolution across events. Understanding the physical processes driving SSWs is therefore essential. In this study, we investigate SPV dynamics, focusing on non-linear coupling between planetary wave modes.
We use potential enstrophy and eddy total energy budget analyses to quantify the contributions of different physical processes to SPV evolution. Applying this framework to both an idealized simulation and reanalysis data of the 2003 SSW event, we find that non-linear wave–wave interactions play a crucial role. In the idealized simulation, wave-2 structures emerge in the stratosphere without a prescribed wave-2 source, attributed to non-linear transfer of enstrophy and energy from wave-1 to wave-2. In the 2003 case study, interactions between wave-1 and wave-2 contribute to the transition from a displacement to a split structure. We also find indications of quasi-linear coupling and upscale enstrophy fluxes from wave-2 to wave-1 during this period.
Our findings highlight the significant impact of non-linear wave–wave interactions in transitioning the SPV between configurations. These complex interactions contribute to the uniqueness of each SSW event and may help explain the variability observed across different SSWs.

How to cite: Rupp, P., Hitchcock, P., and Birner, T.: Coupled planetary wave dynamics in the polar stratosphere analyzed with potential enstrophy and eddy energy budgets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2534, https://doi.org/10.5194/egusphere-egu25-2534, 2025.

EGU25-3360 | ECS | Orals | AS1.31

Impact of Sudden Stratospheric Warmings on the Stratosphere-to-Troposphere Transport of Ozone 

Jaewon Lee, Amy Butler, John Albers, Yutian Wu, and Simon Lee

Sudden stratospheric warmings (SSWs) can significantly impact tropospheric weather systems. Previous studies suggest that SSWs may also influence stratosphere-to-troposphere transport (STT), but their spatial and temporal distribution and mechanisms are not fully understood. The complex relationships between SSWs and the El Niño-Southern Oscillation (ENSO) have also made it difficult to isolate the effects of SSWs on STT. From an idealized ENSO simulation with the WACCM4 model using a stratospheric origin ozone tracer, we investigate the effect of SSWs on the STT of ozone under different ENSO phases. We find a significant increase in lower tropospheric ozone from the SSW onset up to 3 months later over the Arctic, North America, and Europe, regardless of the ENSO phase. This study highlights the significant influence of SSWs on STT on a subseasonal scale. Our results also emphasize the need to consider SSWs when addressing the ENSO impact on STT.

How to cite: Lee, J., Butler, A., Albers, J., Wu, Y., and Lee, S.: Impact of Sudden Stratospheric Warmings on the Stratosphere-to-Troposphere Transport of Ozone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3360, https://doi.org/10.5194/egusphere-egu25-3360, 2025.

EGU25-4427 | ECS | Orals | AS1.31

Rare Sudden Stratosphere Warming Events  in the Southern Hemisphere in 2024 

Yucheng Zi, Zhenxia Long, Jinyu Sheng, Gaopeng Lu, William Perrie, and Ziniu Xiao

In July and August 2024, two rare consecutive stratospheric sudden warming (SSW) events, SW07 and SW08 occurred in the Southern Hemisphere. These events were marked by a rapid Antarctic temperature increase of nearly 17°C at 10 hPa within a few days and a significant deceleration of the stratospheric polar vortex (SPV). In particular, SW07 represents the earliest warming event recorded in the satellite era. Both events meet the criteria for minor SSWs and set new historical temperature records. The analysis reveals that planetary wave anomalies, dominated by nonlinear processes driven by strong tropospheric blocking highs and stratospheric preconditions, played a crucial role in SW07. Additionally, the rapid downward propagation of negative SAM into the troposphere, induced by SW07, created a favorable circulation background for planetary wave perturbations before SW08. These perturbations enhanced ozone transport from low-latitudes ozone to the pole, warming the atmosphere through the absorption of solar shortwave radiation and providing a warm background conducive to triggering SW08.

How to cite: Zi, Y., Long, Z., Sheng, J., Lu, G., Perrie, W., and Xiao, Z.: Rare Sudden Stratosphere Warming Events  in the Southern Hemisphere in 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4427, https://doi.org/10.5194/egusphere-egu25-4427, 2025.

EGU25-7908 | ECS | Posters on site | AS1.31

Stratosphere-Troposphere Dynamics and North American Cold Spells: A Quantile Generalized Additive Approach 

Michael Schutte, Gabriele Messori, and Leonardo Olivetti

Stratospheric variability can significantly impact the tropospheric circulation and influence surface weather conditions. While many studies have established links between changes in the stratospheric polar vortex strength or the downward reflection of Rossby waves and modulations of the mid-latitude tropospheric circulation, challenges remain in developing quantitative approaches to explore these interactions systematically. Addressing this gap, we propose applying quantile generalized additive models (QGAMs) to statistically explore the connections between stratospheric variability, tropospheric circulation patterns and 2-m temperatures.

This study focuses on the North Pacific and North America, regions where stratospheric processes are known to modulate tropospheric circulation patterns and surface extremes. While the lower quantiles of 2-m temperatures are predominantly governed by tropospheric weather regimes, incorporating stratospheric information can further improve the representation of cold temperatures in some regions of North America at time lags of about two weeks. Given the potential of the stratosphere as an additional predictor for North American cold spells, we further investigate the statistical link between stratospheric dynamics and North American weather regimes.

By providing new insights into stratosphere-troposphere coupling mechanisms we can improve our understanding of the large-scale circulation features driving cold spells and other surface weather extremes. This approach has important implications for advancing their predictability on sub-seasonal to seasonal timescales, potentially informing more effective early-warning systems.

How to cite: Schutte, M., Messori, G., and Olivetti, L.: Stratosphere-Troposphere Dynamics and North American Cold Spells: A Quantile Generalized Additive Approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7908, https://doi.org/10.5194/egusphere-egu25-7908, 2025.

EGU25-7938 | ECS | Posters on site | AS1.31

Long-term changes in planetary wave and SSW parameters in the Northern Hemisphere 

Ruixian Yu, Oksana Ivaniha, Yu Shi, Oleksandr Evtushevsky, Gennadi Milinevsky, Asen Grytsai, Andrew Klekociuk, and Xiaolong Wang

Sudden stratosphere warming (SSW) is a distinctive phenomenon characteristic of the winter stratospheric circulation. SSW is linked to the activity of planetary waves. Planetary waves are one of the most prominent waves in the stratosphere, and their evolution, propagation, and anomalies are critical scientific issues in atmospheric dynamics. This study primarily investigates the persistent trend changes in planetary waves and SSW-related climate indices within the stratosphere. Analyzing these trends to enhance the prediction of stratospheric atmospheric evolution. We conducted a zonal harmonic analysis using the potential height fields from ERA5, MERRA-2, and MLS satellite data to determine the amplitudes of planetary waves with wave numbers 1 to 3, analyzing a time period covers 40 winter-spring seasons in the Northern Hemisphere. Climatology for the last four decades allows us to reliably determine the average indicators that characterize zonal waves 1 – 3 during 4 months (December – March) in the stratosphere and lower mesosphere. We are looking for signs and possibilities of the SSW prediction by analyzing the trends of anomalous changes in planetary wave activity. We also discuss the trend changes in climate indices associated with stratospheric atmospheric dynamics, mainly focusing on El Nino Southern Oscillation, Arctic Oscillation, Equivalent Effective Stratospheric Chlorine, Quasi-Biennial Oscillation and NH Coupled Mode Index, over the 40 winter and spring season in the Northern Hemisphere from 1980 to 2023. We investigate the possible connections between these indices and SSW events to identify potential precursors associated with SSW. We try to find appropriate parameters that can trigger SSW. Therefore, the analysis of planetary wave parameters and climate indices can provide insights into SSW events' frequency and dynamic characteristics.

How to cite: Yu, R., Ivaniha, O., Shi, Y., Evtushevsky, O., Milinevsky, G., Grytsai, A., Klekociuk, A., and Wang, X.: Long-term changes in planetary wave and SSW parameters in the Northern Hemisphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7938, https://doi.org/10.5194/egusphere-egu25-7938, 2025.

EGU25-9214 | Posters on site | AS1.31

 Quasi-observational climatology of the gravity wave forcing in the stratosphere. 

Petr Šácha, Zuzana Procházková, and Radek Zajíček

Gravity waves contribute to the energy and momentum transport and budget in the atmosphere, in the stratosphere in particular. Observations and simulations of their effects poses significant challenges due to diverse spatial and temporal scales involved. Despite these challenges, incorporating the effects of gravity waves is essential for global climate and weather prediction models. This study presents a first climatological analysis of resolved gravity waves based on the ECMWF's ERA5 reanalysis and their impacts on the mean flow over more than 43 years. The spatiotemporal distribution of the gravity wave drag is investigated, short and long-term variability analysed locally above the hotspots and in a zonal mean. The results match very well the theoretically assumed properties of gravity waves in the atmosphere, which is very encouraging with respect to the question, how realistic are resolved gravity waves in reanalyses. Our research enhances our understanding of gravity wave drag in the stratosphere and can be used for informing and validating the gravity wave parameterization schemes in climate models.

How to cite: Šácha, P., Procházková, Z., and Zajíček, R.:  Quasi-observational climatology of the gravity wave forcing in the stratosphere., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9214, https://doi.org/10.5194/egusphere-egu25-9214, 2025.

EGU25-10722 | ECS | Posters on site | AS1.31

On the predictive value of upper stratosphere dynamics for winter NAO 

Lizzie Collingwood, Adam Scaife, Bablu Sinha, Robert Marsh, Gareth Marshall, and John King

Recent research is highlighting the importance of the stratosphere and stratosphere-troposphere coupling for subseasonal-to-seasonal prediction of the winter North Atlantic Oscillation (NAO), the dominant mode of variability in the Northern Hemisphere.

Collingwood et al 2024 demonstrated the relevance of the October upper stratosphere to polar vortex development and predictability of winter NAO. They found that anomalous meridional wind in the upper stratospheric “surf zone”, resulting primarily from anomalous eddy momentum flux convergence, generates a signal that propagates down and impacts the vortex and surface NAO, with correlation coefficients of r=0.36 and 0.40 respectively.

Further investigation finds that the relevance of this upper stratospheric meridional wind to winter NAO is not limited to October, but extends to the preceding summer too. This study seeks to better understand the curious mechanisms dictating this teleconnection as well as its decadal variability.

How to cite: Collingwood, L., Scaife, A., Sinha, B., Marsh, R., Marshall, G., and King, J.: On the predictive value of upper stratosphere dynamics for winter NAO, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10722, https://doi.org/10.5194/egusphere-egu25-10722, 2025.

EGU25-11644 | ECS | Orals | AS1.31

An idealized two-dimensional modelling framework to simulate QBO-like oscillations 

Vincent Bremaud, Aurelien Podglajen, Albert Hertzog, and Riwal Plougonven
The quasi-biennial oscillation (QBO) is the dominant mode of interannual variability in the tropical stratosphere, and has global impacts on stratospheric dynamics and composition as well as tropospheric weather. Although a general understanding of its principles was established more than 40 years ago, fundamental uncertainties persist regarding the forcing of the QBO and the relative contribution of the different types of waves involved. As a consequence, climate models predict very different responses of the QBO to climate change or geoengineering scenarios.
 
In this study, we investigate wave-mean flow interaction and QBO-like dynamics in idealized 2D atmospheric simulations using the Weather Research and Forecasting (WRF) model. Our aim is to explore the gap between 1D conceptual toy models of the QBO and general circulation models (GCM) of various resolution with or without parameterized gravity waves. We first reproduce in 2D the minimal 1D configuration described by Plumb (1977) with two gravity waves of opposite phase speed. The waves are forced through thermal forcing and a Newtonian cooling induces radiative dissipation. In this configuration, we obtain a QBO-like oscillation similar to the 1D Plumb model. Then, we explore the evolution of the wave field and the sensitivity of the mean flow to wave and dissipation parameters as well as model resolution and compare with theoretical predictions. Particular attention will be spent on dynamical processes which naturally emerge in the 2D set-up but are negelected in the conceptual model. Potential implications for QBO modelling in GCMs will be discussed.
 

How to cite: Bremaud, V., Podglajen, A., Hertzog, A., and Plougonven, R.: An idealized two-dimensional modelling framework to simulate QBO-like oscillations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11644, https://doi.org/10.5194/egusphere-egu25-11644, 2025.

EGU25-12487 | ECS | Orals | AS1.31

Stratospheric subtropical transport barriers in CESM-WACCM and observations: climatology, variability, and trends 

Oksana Ivaniha, Marta Abalos, Natalia Calvo, Gabriele Stiller, Kasturi Shah, and Sean Davis

Accurate representation of the large-scale stratospheric transport in chemistry-climate models is crucial for interpreting observed variability in chemical species, such as ozone, and making reliable projections regarding future changes. Subtropical transport barriers separate the tropical stratosphere, influenced by slow upwelling, from the surf zones, where rapid mixing occurs due to wave breaking. Long-lived tracer contours reflect the combined effects of advection and mixing and can be used to identify the location of the subtropical transport barriers. This study comprehensively compares tracer- and dynamics-based diagnostics of the subtropical transport barriers in the CESM-WACCM4 chemistry-climate model and various observational datasets. The model tracer-based estimates show excellent agreement with observations regarding seasonal climatology and variability linked to the Quasi-Biennial Oscillation (QBO). The chemical boundaries shift due to the secondary meridional circulation induced by the QBO in the winter hemisphere and due to the enhanced isentropic mixing associated with waves crossing the equator in the summer hemisphere. Consistent with previous studies, the observational tracer metrics feature a southward shift of the tropical pipe over 2005–2012. The model, which nudges the QBO to observations, captures qualitatively the shift over this period. Dynamical metrics represent individual transport processes and thus fail to capture the variability and trends in the tracer-based boundaries.

How to cite: Ivaniha, O., Abalos, M., Calvo, N., Stiller, G., Shah, K., and Davis, S.: Stratospheric subtropical transport barriers in CESM-WACCM and observations: climatology, variability, and trends, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12487, https://doi.org/10.5194/egusphere-egu25-12487, 2025.

EGU25-12791 | Posters on site | AS1.31

Stratospheric drivers of precipitation and temperature in southern Africa 

Shingirai Nangombe and Daniela Domeisen

 
The winter stratosphere has been shown to influence surface climate, leading to persistent changes in temperature and precipitation patterns, which can be associated with extreme events such as cold air outbreaks, heavy precipitation and flooding, dry spells, as well as dust storms. These influences on surface weather have dominantly been investigated for the Northern Hemisphere, especially with respect to extreme stratospheric events such as sudden stratospheric warmings and strong vortex events, which have their dominant impact over the North Atlantic area. In the Southern Hemisphere, although such extreme stratospheric events are much less frequent, surface impacts of the stratosphere have also been observed. However, some regions, like southern Africa, have received very little attention. We here explore to what extent stratospheric variability related to the final stratospheric warming, the final breakdown of the stratospheric polar vortex in winter through spring, can have an impact on southern African weather through variability of the Southern Annular Mode (SAM). We find that indeed, the influence of anomalies in the SAM driven by the stratosphere extends to the southern part of Africa, leading to anomalous pressure patterns that influence temperature and precipitation distribution. This contribution is intended to spark research into less explored regions of stratospheric influence in the Southern Hemisphere.

How to cite: Nangombe, S. and Domeisen, D.: Stratospheric drivers of precipitation and temperature in southern Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12791, https://doi.org/10.5194/egusphere-egu25-12791, 2025.

EGU25-13230 | Orals | AS1.31

Using MIPAS Tracer Measurements to Investigate the Quasi-Biennial Oscillation and Mean Meridional Circulation 

Tobias Kerzenmacher, Peter Braesicke, Udo Grabowski, and Gabriele Stiller
This study investigates the Quasi-Biennial Oscillation (QBO) influence on the mean meridional circulation during the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) operational period (2002-2012). We employ ERA-Interim, JRA-55, and ERA5 reanalysis data alongside MIPAS tracer-derived velocities. Following the SPARC Reanalysis Intercomparison Project (S-RIP) methodology, we deseasonalize and composite QBO-W onsets at 20 hPa. This allows for comparisons of zonal-mean vertical and meridional velocities derived from MIPAS tracers with reanalysis data.
 
To derive effective transport velocities within the 2-dimensional atmosphere, we leverage a direct inversion technique based on MIPAS tracer measurements. This method, as detailed in Clarmann et al. (2016), integrates the continuity equation over time to determine mean velocities that replicate observed trace gas distributions. This approach offers observation-based insights into the mean meridional circulation independent of dynamical models. We analyze various atmospheric layers for the tracers CH4, CO, H2O, and N2O, and supplement them with SF6 and CCl4 to mitigate uncertainties.
 
Our analysis reveals distinct QBO patterns in tracer-retrieved velocities, demonstrating good qualitative agreement with ERA5, ERA-Interim, and JRA-55 reanalysis results. However, comparisons also expose differences, potentially highlighting areas for improvement in current models or limitations inherent to tracer-based continuity equation inversions.
 
These findings emphasize the significance of MIPAS tracer measurements for enhancing our understanding and modelling of the mean meridional circulation in Earth's atmosphere.
 
von Clarmann, T. and Grabowski, U.: Direct inversion of circulation and mixing from tracer measurements – Part 1: Method, Atmos. Chem. Phys., 16, 14563–14584, https://doi.org/10.5194/acp-16-14563-2016, 2016.

How to cite: Kerzenmacher, T., Braesicke, P., Grabowski, U., and Stiller, G.: Using MIPAS Tracer Measurements to Investigate the Quasi-Biennial Oscillation and Mean Meridional Circulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13230, https://doi.org/10.5194/egusphere-egu25-13230, 2025.

EGU25-13831 | Posters on site | AS1.31

Tropical Impacts From Polar Vortex Events 

Thomas Reichler and Zheng Wu

Stratospheric sudden warmings and other polar vortex events have well-documented impacts on winter surface weather and climate over middle to high latitudes. However, the scientific understanding of the influence of the polar stratosphere on the tropics remains in its early stages. There are two primary pathways through which these influences can occur. In the first pathway, polar vortex events modulate the strength of the Brewer-Dobson circulation, affecting both the tropical stratosphere and troposphere. In the second pathway, the dynamical downward coupling from the stratosphere into the extratropical troposphere may also influence the tropical troposphere. To investigate the type and magnitude of tropical impacts from polar vortex events, we employ a composite analysis of ERA5 reanalysis data spanning from 1957 to 2024. Our findings reveal that stratosphere-related changes in the Brewer-Dobson circulation not only affect the tropics but also extend into the subtropics and extratropics of the opposite hemisphere. These impacts manifest in various variables, including tropical upwelling, the descent rate of the Quasi-Biennial-Oscillation, tropical stratospheric water vapor, the height and temperature of the tropical tropopause, and tropical column ozone. Furthermore, we find that stratospheric circulation events are associated with shifts in the poleward extent of the tropical Hadley cell. While these tropical changes are generally weaker compared to those observed at higher latitudes, they are nonetheless of comparable duration and statistically significant.

How to cite: Reichler, T. and Wu, Z.: Tropical Impacts From Polar Vortex Events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13831, https://doi.org/10.5194/egusphere-egu25-13831, 2025.

EGU25-18971 | ECS | Orals | AS1.31

Stratospheric Drivers of Extreme Weather: Implications for European Storm Damage and Flood Risk 

Hilla Afargan Gerstman, Rachel Wu, and Daniela Domeisen

The downward coupling between the stratosphere and the troposphere, as occurs during sudden stratospheric warmings (SSWs) or strong polar vortex events, can have a detectable impact on surface weather in winter, especially over Europe and the North Atlantic. These changes include shifts in the pathways of extratropical cyclones and the associated change in the location of the risk of extreme winds, flooding, or heavy snowfall. 

As changes in the stratospheric circulation contribute to predictability at the surface, understanding the stratospheric drivers to surface weather - from precursors to hazards and impacts - is essential for enhancing societal preparedness and building effective early warning systems for these events. However, there has been no systematic effort to quantify the impacts with respect to stratospheric forcing. 

This work establishes the connection between stratospheric extremes and midlatitude storm damage and flooding events in the Euro-Atlantic region using a combination of ERA5 reanalysis and multiple impact datasets for the period 1998-2023. We show that stratospheric extremes contribute up to 34% of the total counts of storm-related disasters and up to 12% of flood-related disasters in Europe during winter. The geographic distribution of storm-related disasters is influenced by stratospheric forcing, with more frequent storm impacts found over Scandinavia, northern and central Europe and the UK following strong vortex events as compared to the period after SSW events.

Furthermore, using multi-model ensemble of climate models (CMIP6) under future socio-economic scenarios, we examine the variability of extreme storms over the Euro-Atlantic region and investigate their connection to stratospheric drivers and biases in present-day climate and under climate change. Quantifying the connections between stratospheric drivers and surface extremes across various timescales can enable earlier warnings and risk mitigation in both present-day climate and under climate change conditions.



How to cite: Afargan Gerstman, H., Wu, R., and Domeisen, D.: Stratospheric Drivers of Extreme Weather: Implications for European Storm Damage and Flood Risk, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18971, https://doi.org/10.5194/egusphere-egu25-18971, 2025.

EGU25-20115 | Orals | AS1.31

Role of Oceanic SST Fronts in the Interhemispheric Asymmetry of Stratospheric Dynamics and Associated Extremes 

Nour-Eddine Omrani, Noel Keenlyside, Hisashi Nakanura, Fumiaki Ogawa, and Sandro Lubis

The stratospheric dynamics and associated extremes, such as sudden stratospheric warmings (SSWs) and the formation of polar stratospheric clouds (PSCs), exhibit a pronounced interhemispheric asymmetry. SSWs are exceedingly rare in the Antarctic, while the extreme cooling conditions required for the formation of water-based PSCs (Type II) are infrequent and short-lived in the Arctic. To investigate the drivers of this asymmetry, we conducted a series of semi-idealized model experiments, progressing from aqua-planet configurations mimicking Southern Hemisphere (SH) conditions to more realistic Northern Hemisphere (NH) setups.

 

Our results reveal that orography and land-sea thermal contrast (LSCO) alone cannot fully explain the observed interhemispheric asymmetry. Crucially, midlatitude oceanic sea surface temperature (SST) fronts, associated with western boundary currents, play a pivotal role in aligning stratospheric dynamics and extremes with NH-like conditions. Similar to LSCO, SST fronts significantly enhance the stratospheric convergence of planetary wave activity, which strengthens the Brewer-Dobson Circulation. This leads to substantial increases in high-latitude adiabatic warming, elevating the frequency of Arctic SSWs while simultaneously suppressing conditions conducive to PSC formation. These findings highlight the critical yet underexplored role of oceanic SST fronts in shaping the interhemispheric differences in stratospheric dynamics and extremes.

How to cite: Omrani, N.-E., Keenlyside, N., Nakanura, H., Ogawa, F., and Lubis, S.: Role of Oceanic SST Fronts in the Interhemispheric Asymmetry of Stratospheric Dynamics and Associated Extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20115, https://doi.org/10.5194/egusphere-egu25-20115, 2025.

EGU25-295 | PICO | AS1.32

Combined mixing in coastal regions from Internal Solitary Waves and Wind   

Jorge Magalhaes, Martin Coubard, Jose da Silva, Maarten Buijsman, Ana Santos, Ana Amorim, and Paulo Oliveira

Well-developed surface mixed layers up to 10 meters (or more) are known to result from strong winds. In addition, Internal Solitary Waves (ISWs) in coastal regions have already been shown to induce strong mixing in both intermediate and bottom depths, and recent evidence suggests they also increase surface wave breaking. Altogether, it can be wondered if mixing from wind and ISWs combined can exceed that of their individual contributions. This possibility could ultimately mean large-scale sections of vertical mixing in the water column with unforeseen implications ranging from mixing parametrizations in ocean models to our current understanding of biogeochemical processes relying on diapycnal mixing. We add to this possibility via a large sample of ISWs collected during 12 days with moored instrumentation off the Portuguese (Iberian) Coast. Richardson numbers show that high winds and ISWs are associated with a higher frequency and larger-scale shear-instabilities and temperature overturns connecting surface to intermediate depths.

How to cite: Magalhaes, J., Coubard, M., da Silva, J., Buijsman, M., Santos, A., Amorim, A., and Oliveira, P.: Combined mixing in coastal regions from Internal Solitary Waves and Wind  , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-295, https://doi.org/10.5194/egusphere-egu25-295, 2025.

EGU25-773 | ECS | PICO | AS1.32

The Internal Tides of the Eastern Arabian Sea: A Seasonal Perspective 

Pragnya Makar, Ambarukhana Devendra Rao, Badarvada Yadidya, and Vimlesh Pant

Internal tides (ITs) are internal waves characterized by tidal or quasi-tidal period, resulting from the interplay between barotropic tidal flow and submarine topography features in a stratified ocean. The dominant tidal constituents in this region are identified as M2 and K1 through in-situ observations from the moored buoys at AD08, AD09, AD10, and RAMA, with S2 and O1 following, respectively. A 3D Massachusetts Institute of Technology General Circulation model simulation is used to identify the key generation sites in the eastern Arabian Sea. The analysis revealed three primary locations: (1) the continental shelf-slope break off Mumbai (SD1), (2) the Lakshadweep region (SD2), and (3) the vicinity of the Maldives Islands (SD3). Among these, the SD1 and SD3 are identified as the major generation sites, collectively contributing approximately 70% of the total baroclinic energy within the study area. The energy budget analysis reveals that the semidiurnal energy conversion reaches its maximum in April at SD1 and in July at SD3, whereas the diurnal energy conversion exhibits peak values in October at SD1 and in July at SD3. SD2 demonstrated minimal seasonal variation in both semidiurnal and diurnal energy conversions. The energy flux patterns reveal south-westward propagation originating from the Mumbai region and westward propagation emanating from the Maldives. The findings highlight that the seasonal variability of ITs in the eastern Arabian Sea is predominantly governed by variations in stratification, offering valuable insights into the region's IT dynamics.

How to cite: Makar, P., Rao, A. D., Yadidya, B., and Pant, V.: The Internal Tides of the Eastern Arabian Sea: A Seasonal Perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-773, https://doi.org/10.5194/egusphere-egu25-773, 2025.

EGU25-3799 | PICO | AS1.32

Internal Solitary Waves within the Cold Tongue of the Equatorial Pacific Generated by Buoyant Gravity Currents 

José Da Silva, Adriana Santos-Ferreira, Bruno St.-Denis, Daniel Bourgault, and Leo Maas

We present a hypothesis for the generation mechanism of trains of Internal Solitary Waves (ISWs) that are observed in the eastern equatorial Pacific Ocean, within a zonal band from 5 S to 5 N and from 210 to 265 E in longitude.  The presence of these ISWs in this region is remarkable given the absence of steep bottom topography and tides that could explain their presence from classical theories, and to date had not been explained. In this study (Santos-Ferreira et al., 2023), we provide estimates and model-based predictions of some ISW characteristics such as their wavelength, crest length, typical amplitude, as well as age. In total, we identified 116 ISW trains during one full year (2020), with an average crest length of 300 km, typical wavelengths of 1500 m, and modelled amplitude of 10 m. The origin of these trains of ISWs is consistent with a generation mechanism that involves buoyant gravity currents with sharp fronts detectable in satellite imagery (visible and thermal infrared from Sentinel-3). The propagation of gravity currents into stably stratified environments is known to generate internal waves but reports of such phenomena in the open ocean are scarce. Here we report indications that such an internal wave generation mechanism is ubiquitous along the equatorial Pacific, and we suggest that ISWs may have been overlooked in many other frontal regions in the deep ocean. Energetic Tropical Instability Waves (TIWs) have been linked to buoyant gravity currents in Warner et al. (2018), which propagate within the equatorial cold tongue that is strongly stratified, hence providing conditions for the propagation of ISWs initiated by the gravity currents. These internal waves provide a physical link between frontal zones of 1000-km scale TIWs with viscous mixing scales.

 

Santos-Ferreira, A. M., da Silva, J.C.B., St-Denis, B., Bourgault, D., & Maas, L. R. M., 2023: Internal solitary waves within the cold tongue of the equatorial pacific generated by buoyant gravity currents. Journal of Physical Oceanography, 53(10), 2419-2434.

Warner, S. J., R. M. Holmes, E. H. M. Hawkins, M. Hoecker-Martinez, A. C. Savage, and J. N. Moum, 2018: Buoyant gravity currents released from tropical instability waves. J. Phys. Oceanogr., 48, 361–382, https://doi.org/10.1175/JPO-D-17-0144.1.

How to cite: Da Silva, J., Santos-Ferreira, A., St.-Denis, B., Bourgault, D., and Maas, L.: Internal Solitary Waves within the Cold Tongue of the Equatorial Pacific Generated by Buoyant Gravity Currents, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3799, https://doi.org/10.5194/egusphere-egu25-3799, 2025.

EGU25-3820 | ECS | PICO | AS1.32

Stratospheric Gravity waves in AIRS observations and high-resolution models 

Phoebe Noble, Haruka Okui, Joan Alexander, Manfred Ern, Neil Hindley, Lars Hoffmann, Laura Holt, Annelize van Niekerk, Riwal Plougonven, Inna Polichtchouk, Claudia Stephan, Martina Bramberger, Milena Corcos, and Corwin Wright

Atmospheric gravity waves vary hugely in scale; with horizontal wavelengths ranging from a few to thousands of km. Typically, gravity waves are smaller than model grid-size and as a result, their effects are parametrised instead of being explicitly resolved. However, recent computational and scientific advancements have allowed for the development of higher resolution global-scale models. These models have horizontal resolutions of order a few km with around 1km vertical resolution in the stratosphere. At such scales, it should in principle be possible to accurately simulate the majority of GWs without relying on parametrisation.

In this work, we use data from three models from the DYAMOND Initiative (DYnamics of the Atmospheric general circulation Modeled On Non-hydrostatic Domains). Specifically, IFS (Integrated Forecast System – produced by ECMWF) at 4km horizontal resolution, ICON (Icosahedral NonHydrostatic) at 5km horizontal resolution and GEOS (Goddard Earth Observing System model) at 3km horizontal resolution. All models are initialised with the same initial conditions and are free running for 40 days. We then compare the properties of resolved gravity waves with observations from the AIRS instrument (Atmospheric InfraRed Sounder) onboard NASA’s Aqua satellite. Importantly, we note that the AIRS observations are limited by the ‘observational filter’, wherein each observing system can only `see' a limited portion of the full GW spectrum. To account for this, an important step in this work is in resampling the model atmospheres as though viewed by the AIRS instrument.

We compare the representation of resolved waves in the three models and AIRS observations across 40-days in Austral winter. We use a recently developed machine learning wave identification method to separate gravity waves in the dataset and determine gravity wave occurrence frequencies. Next, we use spectral analysis to estimate gravity wave amplitudes, wavelengths and calculate momentum fluxes and the intermittency of gravity waves. This work provides an essential evaluation of the accuracy of current gravity wave modelling capabilities.

How to cite: Noble, P., Okui, H., Alexander, J., Ern, M., Hindley, N., Hoffmann, L., Holt, L., van Niekerk, A., Plougonven, R., Polichtchouk, I., Stephan, C., Bramberger, M., Corcos, M., and Wright, C.: Stratospheric Gravity waves in AIRS observations and high-resolution models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3820, https://doi.org/10.5194/egusphere-egu25-3820, 2025.

An idealized reentrant channel model is utilized to investigate whether wind forcing alone can generate a Garrett-Munk (GM) internal wave (IW) spectrum and where the bulk of the IW energy comes from. It is shown that high-frequency winds can easily generate a GM-like IW spectrum in an eddying ocean without sophisticated model settings. During the formation of a GM-like spectrum, energy transferred from mesoscale eddies to IWs is comparable to that from submesoscale motions. In the pycnocline, IW energy is partially absorbed into mesoscale eddies, which may partly explain why only a small portion of wind-induced IWs penetrates into the deep ocean. This study complements previous study that tidal forcing alone can generate a GM-like IW spectrum. These two studies together imply that a GM-like spectrum can be easily generated through a forcing agent alone, suggestive of a reason why it is ubiquitously observed in the ocean.

How to cite: Chen, Z. and Zhang, Q.: Formation of a Garrett-Munk-like internal wave spectrum in an eddying ocean by wind forcing alone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4985, https://doi.org/10.5194/egusphere-egu25-4985, 2025.

EGU25-5174 | PICO | AS1.32

Gravity Wave-Induced Perturbations in Lidar Backscatter Profiles above La Réunion (21°S, 55°E) 

Fabrice Chane Ming, Samuel Tremoulu, Dominique Gantois, Guillaume Payen, Michael Sicard, Sergey Khaykin, Alain Hauchecorne, Philippe Keckhut, and Valentin Duflot

Atmospheric gravity waves (GWs) play a crucial role in vertically coupling the lower and upper atmosphere, significantly impacting middle atmosphere dynamics. Despite their importance, accurately representing GWs remains a persistent challenge for numerical weather prediction and global atmospheric models.

Atmospheric particulate matter or aerosols present in both the troposphere and the stratosphere are deeply involved in radiative processes and atmospheric chemistry. A strong interplay exists between GWs and aerosols, particularly in the formation and evolution of cirrus clouds. Furthermore, aerosol-induced warming processes can also generate GWs within the atmospheric boundary layer, especially over polluted tropical cities. The dynamics of the aerosol vertical distribution can, in certain cases, serve as tracers for GWs, particularly during intense aerosol mixing driven by strong meteorological events in the troposphere and stratosphere.

This study examines GW-induced perturbations in lidar backscatter profiles observed above the Maïdo Observatory at La Réunion (21°S, 55°E) on the night of November 21, 2023 near the southern subtropical barrier.  Complementary data from lidar-based temperature and wind measurements, radiosondes, COSMIC-2 satellite observations, and ERA5 reanalysis confirm key GW characteristics in the mid-troposphere. These include a vertical wavelength of 5-6 km, an observed period of approximately 24 hours, an downward phase propagation, and an upward energy propagation into the stratosphere.

How to cite: Chane Ming, F., Tremoulu, S., Gantois, D., Payen, G., Sicard, M., Khaykin, S., Hauchecorne, A., Keckhut, P., and Duflot, V.: Gravity Wave-Induced Perturbations in Lidar Backscatter Profiles above La Réunion (21°S, 55°E), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5174, https://doi.org/10.5194/egusphere-egu25-5174, 2025.

EGU25-5853 | ECS | PICO | AS1.32

Evaluation of gravity wave parameterization schemes in a climate model using high-resolution ICON and IFS simulations 

Iman Toghraei, François Lott, Laura Köhler, Claudia Stephan, and Joan Alexander

Expanding upon our previous work1, we extend the evaluation of gravity wave parameterization schemes in the Atmospheric Component of the IPSL Climate Model (LMDZ6A) by incorporating comparisons with high-resolution datasets from the ICOsahedral Nonhydrostatic Weather and Climate Model (ICON) and the Integrated Forecasting System (IFS). The ICON dataset corresponds to ~ 5 km horizontal resolution simulations for spring 2020, coarse-grained to a ~ 100 km grid (1°). The IFS dataset corresponds to 1 km horizontal resolution simulations for winter 2018, coarse-grained to a T42 grid (~2.8°). In both models, we assume that at each time and place in the stratosphere, the momentum fluxes due to the disturbances that are filtered out during coarse graining are due to subgrid-scale gravity waves. The parameterizations have been then run offline using ICON and IFS coarse-grained meteorological fields to predict these subgrid-scale gravity wave momentum fluxes. 

The comparison shows that the parameterizations have some skills in predicting the geographical distribution of the simulated fluxes in different regions. More specifically, the gravity wave momentum fluxes due to the orographic and convective gravity waves are reasonably well predicted in the mountainous and tropical regions, respectively. The results are more contrasted concerning the gravity waves generated within fronts. Aloft the storm tracks the parameterized gravity wave momentum fluxes are larger than the ICON gravity wave fluxes and smaller than the IFS gravity wave fluxes. This challenges the dynamics at work in these models during geostrophic adjustment, suggesting that some high-resolution models potentially produce more gravity wave fluxes than are needed in GCMs to simulate the right climate. These results also highlight the importance of considering multiple high-resolution datasets to understand gravity wave characteristics better and tune their parameterizations more effectively.

Using insights from these comparisons, we vary the parameters in the schemes to improve the fit with the high-resolution simulations and test impacts in online runs done with the  LMDZ6A climate model. Our results illustrate how high-resolution model datasets can improve gravity wave parameterizations in climate models.

 

 

1Toghraei, I., Lott, F., Köhler, L., Stephan, C., and Alexander, J.: Comparison between the gravity wave stress parameterized in a climate model and simulated by the high-resolution non-hydrostatic global model ICON, EGU General Assembly 2024, Vienna, Austria, 14–19 Apr 2024, EGU24-5181, https://doi.org/10.5194/egusphere-egu24-5181, 2024.

How to cite: Toghraei, I., Lott, F., Köhler, L., Stephan, C., and Alexander, J.: Evaluation of gravity wave parameterization schemes in a climate model using high-resolution ICON and IFS simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5853, https://doi.org/10.5194/egusphere-egu25-5853, 2025.

The atmosphere's flow becomes unpredictable beyond a certain time due to the inherent growth of small initial-state errors. While much research has focused on tropospheric predictability, predictability of the middle atmosphere remains less studied. This work contrasts the intrinsic predictability of different layers, with a focus on the mesosphere/lower thermosphere (MLT, ~50–120 km altitude). Ensemble simulations with the UA-ICON model for an austral winter/spring season are conducted with a gravity-wave permitting horizontal resolution of 20 km, and are contrasted to coarser resolution simulations. Initially small perturbations grow fastest in the MLT, reaching 10% of saturation after 5–6 days, compared to 10 days in the troposphere and two weeks in the stratosphere. However, perturbation energy in the MLT reaches 50% saturation only after about two weeks, similar to the troposphere. Those saturation times are overestimated  by up to a factor of two when using a coarser resolution (grid size 160km),  highlighting the need for gravity wave-resolving models. Predictability in the MLT depends on horizontal scales. Motions on scales of hundreds of kilometers are predictable for less than five days, while larger scales (thousands of kilometers) remain predictable for up to 20 days. This scale-dependent progression of predictability cannot be explained by simple scaling for upscale error growth. Vertical wave propagation plays a significant role, with gravity waves transmitting perturbations upward at early lead times and planetary waves enhancing long-term predictability. In summary, the study shows that MLT predictability is scale-dependent and highlights the necessity of high-resolution models to capture fast-growing perturbations and assess intrinsic predictability limits accurately.

How to cite: Garny, H.: Role of resolving gravity waves for estimating the intrinsic predictability of the middle atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6057, https://doi.org/10.5194/egusphere-egu25-6057, 2025.

EGU25-6975 | ECS | PICO | AS1.32

Tropospheric gravity waves in the subtropics: Optical detection on low cloud decks  

Mathieu Ratynski, Brian Mapes, and Hanna Chaja

Internal gravity waves with wavelengths of tens to hundreds of kilometers are frequently seen as ripples on high-resolution geostationary satellite animations of subtropical stratocumulus decks. To systematically detect and characterize these waves, several satellite data fields are employed. Daytime visible reflectance images have high contrast, with units of reflected insolation relevant to climate impacts. IR brightness temperature is available day and night, but requires high-pass filtering and contrast enhancements. The divergence of low cloud tracking winds, retrieved via Particle Image Velocimetry (PIVdiv), is a scalar field independent of those radiative quantities. Water vapor channel time differences show wave vertical displacements at midlevels. 

In any given image array, Matlab’s Cauchy continuous wavelet transform detects packets of elongated phase crests and projects them into 10 logarithmic half-wavelength bins between 20-500 km, with angle discrimination of about 15 degrees, all on a 5 degree coarse geographical mesh. Cross-wavelet analysis probes for connections between pairs of images. Time pairs of the same field lead to estimates of wave propagation speed. Cross spectra of PIVdiv and radiative brightnesses help to quantitatively relate wave modulations of cloudiness to the vertical displacement of PBL top where the clouds reside. Connecting low level cloud signals to midlevel water vapor signals allows us to estimate vertical wavelength, allowing an independent check against propagation speed via the dispersion relation.

Preliminary wave rose maps, generated for the southeast Pacific during October–December 2023 reveal multiple source regions: synoptic jet-front disturbances in the South Pacific upper-level westerlies, intertropical convergence zone (ITCZ) convection, and orographic or thermal forcing from South America. We hypothesize that similar processes, plus tropical cyclones absent in this sample, drive similar wave activity in other basins and seasons. 

The results may have several applications. Any novel observed signal stands as a challenge or target for high-resolution models. Wave sources inferred from these observations may usefully constrain estimates of physical and nonlinear processes in the atmosphere. Low cloud dependence on vertical velocity could have climate relevance, for instance case studies of strong waves have shown they can be rectified in closed to open cell transitions. If periodic waves are trackable for much longer than their inverse frequency, they could comprise a subtle source of surprisingly long predictability of convective initiation, coastal fog/clearing, or other local effects. Like all gravity waves, these redistribute zonal momentum via meridional and vertical fluxes, a process whose contribution to larger scale flows can now be estimated quantitatively. 

By offering open-access wave data products, we hope to inspire collaborative efforts on all these application areas. By scaling up computations from 3 months in one region to many years around the globe, downgrading newer data to be comparable to older data as needed, we can build up a nearly global daily picture of tropospheric internal waves over the subtropical oceans through time. With so many degrees of freedom contributing to these high-resolution measurements, very subtle trends and differences should be detectable.

How to cite: Ratynski, M., Mapes, B., and Chaja, H.: Tropospheric gravity waves in the subtropics: Optical detection on low cloud decks , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6975, https://doi.org/10.5194/egusphere-egu25-6975, 2025.

EGU25-7277 | PICO | AS1.32

Deep Learning-Based Reconstruction of Nonorographic Gravity Wave Patterns in the Lower Stratosphere 

Elahe Khanlari, Mozhgan Amiramjadi, Ali R. Mohebalhojeh, and Mohammad Mirzaei

Recently, there has been a significant interest in applying machine learning (ML) to improve the performance of general circulation models (GCMs). Subgrid processes not resolved directly in weather and climate models still require to be parameterized. ML constitutes a set of promising methods to address the problems such as computational cost and uncertainty introduced by parameterization in numerical simulations.

The current study examines the performance of deep learning in reconstructing nonorographic gravity waves (GWs) over midlatitude oceanic regions. A convolutional neural network (CNN) is employed to predict high-resolution variables—standard deviation of momentum flux, horizontal divergence, and vertical velocity—reflecting GW activity in the lowermost stratosphere. Both the targets and the coarse-resolution explanatory variables, spanning the troposphere, are obtained from the ERA5 dataset produced by the European Centre for Medium-Range Weather Forecasts (ECMWF), as outlined by Amiramjadi et al. (2023).

The results demonstrate that the model effectively reconstructs the GW signal and captures the seasonal cycle of GW activity with a reasonable computational cost. The mean coefficient of determination (R²) and Pearson’s correlation coefficient (R) across all grid points in the study area are approximately 0.42 and 0.67, respectively, using all predictors.

 

Reference:

Amiramjadi, M., Plougonven, R., Mohebalhojeh, A. R., & Mirzaei, M. (2023). Using machine learning to estimate nonorographic gravity wave characteristics at source levels. Journal of the Atmospheric Sciences, 80(2), 419–440.

How to cite: Khanlari, E., Amiramjadi, M., Mohebalhojeh, A. R., and Mirzaei, M.: Deep Learning-Based Reconstruction of Nonorographic Gravity Wave Patterns in the Lower Stratosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7277, https://doi.org/10.5194/egusphere-egu25-7277, 2025.

EGU25-8424 | PICO | AS1.32

Does the jet stream generate gravity waves? 

Carsten Eden, Manita Chouksey, and Silvano Rosenau

Numerical simulations of the baroclinic lifecycle of the jet stream show gravity wave-like structures in the upper troposphere. Here, we employ a novel method to decompose any flow into slow (geostrophically) balanced part and fast wave part to these structures. The method originates from the optimal potential vorticity balance method by Viudez and Dritschel (2004) but is modified to be applied to general flow. It was compared earlier to the asymptotic decomposition method by Warn et al (1995) and was shown to perform equally well. Here, we apply the novel method to an idealised  numerical model of the baroclinic lifecycle of the jet stream and show how much of the gravity wave-like structures in the upper troposphere are part of the balanced part of the flow, and how much of it are really gravity waves.

How to cite: Eden, C., Chouksey, M., and Rosenau, S.: Does the jet stream generate gravity waves?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8424, https://doi.org/10.5194/egusphere-egu25-8424, 2025.

EGU25-8479 | ECS | PICO | AS1.32

Modeling and propagation evolution of ocean internal solitary waves 

Di Yu and Jinbao Song

Under investigation in this article is the propagation of internal solitary waves in the deep ocean. Based on the principles of nonlinear theory, perturbation expansion and multi-scale analysis, a time-dependent modified cubic Benjamin-Ono (mCBO) equation is derived to describe internal solitary waves in the deep ocean with stronger nonlinearity. When the dispersive term vanishes, the mCBO equation transforms into the cubic BO equation. Under certain conditions, the mCBO equation can be converted to BO or modified Korteweg-de Vries (mKdV) equation. Compared with the traditional BO model, the mCBO model takes into account stronger nonlinearity. To gain deeper insights into solitary waves' characteristics, conservation of mass and momentum associated with them are discussed. By employing Hirota's bilinear method, we obtain the bilinear form and soliton solutions for mCBO equation, and subsequently investigate interactions between two solitary waves with different directions leading to the occurrence of important events such as rogue waves and Mach reflections. Additionally, we explore how certain parameters influence Mach stem while drawing meaningful conclusions. Our discoveries reveal the complex dynamics of internal solitary waves within the deep ocean and contribute to a broader understanding of nonlinear wave phenomena.

How to cite: Yu, D. and Song, J.: Modeling and propagation evolution of ocean internal solitary waves, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8479, https://doi.org/10.5194/egusphere-egu25-8479, 2025.

EGU25-8712 | PICO | AS1.32

Gravity wave dynamics influencing ice clouds 

Stamen Dolaptchiev and Ulrich Achatz

Gravity waves (GWs) have a significant influence on the formation,
microphysical properties, and life cycle of ice clouds. However,
understanding how to accurately account for the complex interactions
between GWs and ice physics in atmospheric models remains a
challenge. For instance, some ice nucleation parameterizations
consider only the strong vertical updraft velocities generated by GWs,
which lead to high ice crystal number concentrations. However,
temperature and pressure fluctuations associated with GWs can locally
produce high supersaturation levels, triggering ice crystal nucleation
even when the large-scale saturation ratio is below the critical
threshold or in region where GW vertical velocity is zero.

In this study, we present a testbed for coupling transient GW dynamics
with ice physics used for the development of corresponding
parameterizations. We utilize a model capable of operating in two
modes: one that resolves both wave dynamics and nucleation explicitly,
and another that parameterizes those processes. To test our coupling
strategy, we perform idealized experiments involving the superposition
of wave packets passing through an ice-supersaturated region. We
evaluate the resulting microphysical properties of ice clouds and
cloud cover fraction in different simulations. Our findings suggest
that this approach can be successfully implemented in climate models
equipped with transient GW parameterization.

How to cite: Dolaptchiev, S. and Achatz, U.: Gravity wave dynamics influencing ice clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8712, https://doi.org/10.5194/egusphere-egu25-8712, 2025.

EGU25-9483 | ECS | PICO | AS1.32

Sensitivity of an orographic drag parametrisation scheme to empirical parameters revealed by ensemble simulations 

Georgios Thalassinos, Stefano Serafin, and Martin Weissmann

Mountains affect the general circulation of the atmosphere on multiple spatial scales, some of which are too small to be explicitly resolved by weather and climate models. To represent the drag exerted by unresolved mountains and unresolved gravity waves, orographic drag parametrisations use statistics of unresolved orography to calculate the sub-grid-scale (SGS) drag. Processes such as large scale wave breaking and flow-blocking become resolved at today's model resolutions, but small-scale drag and turbulent orographic form drag remain in the SGS regime. This poses the open problem of a correct partitioning between resolved and unresolved orographic drag.

Recent studies have used ensemble data assimilation methods, in particular joint state and parameter estimation, to improve the representation of SGS boundary-layer turbulence in models. Inspired by those studies, we aim to to evaluate the sensitivity of an orographic drag scheme to its empirical parameters to identify candidates for effective parameter estimation experiments. Using the Weather Research and Forecasting (WRF) model, we conducted numerical experiments of mountain waves over complex terrain with a grid spacing of 10 km using the GSL drag scheme. This parametrisation represents large-scale gravity wave drag, flow blocking drag, turbulent orographic form drag, and small-scale gravity wave drag.

Using ensemble experiments with perturbed empirical parameters, we evaluate the correlation between individual parameters and the model state. The parameters that display the highest ensemble correlation with the model state have the greatest impact on the behaviour of the orographic drag parametrisation, making them candidates for parameter estimation. Our preliminary results refer to two parameters in the scheme that affect low-level wave breaking and the separation between blocking and non-blocking states, and illustrate their ensemble correlations with the model state.

How to cite: Thalassinos, G., Serafin, S., and Weissmann, M.: Sensitivity of an orographic drag parametrisation scheme to empirical parameters revealed by ensemble simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9483, https://doi.org/10.5194/egusphere-egu25-9483, 2025.

EGU25-10840 | PICO | AS1.32

Measurements of Quasi-monochromatic Gravity Waves and Estimates of Turbulence in the Polar Night Jet 

Robin Wing, Irina Strelnikova, Facundo Poblet, Boris Strelnikov, Michael Gerding, Mohamed Mossad, and Gerd Baumgarten

Using the Doppler-Rayleigh lidars at Kühlungsborn (54°N, 12°E) and ALOMAR (69° N, 16° E), we have obtained simultaneous vertical profiles of horizontal wind and temperature on the poleward flank of the Polar Night Jet. This study presents a case where a modified hodograph technique was applied to identify quasi-monochromatic gravity waves within the high wind speed regime of the jet's flank. Our analysis reveals a reduction in gravity wave kinetic and potential energy within the core of the Polar Night Jet for both upward- and downward-propagating waves, attributed to a strong wind shear layer.

We will present a statistical overview of intrinsic gravity wave parameters for all resolved waves in the observation.  We will demonstrate our ability to resolve low amplitude waves in the lidar observation down to amplitudes of ~0.5 K in the stratosphere.

As an extension, we will show preliminary attempts to estimate energy fluxes from the lidar data using structure-function and compared these results with hodograph-derived gravity wave energies to investigate turbulent energy transfer rates within the Polar Night Jet.

How to cite: Wing, R., Strelnikova, I., Poblet, F., Strelnikov, B., Gerding, M., Mossad, M., and Baumgarten, G.: Measurements of Quasi-monochromatic Gravity Waves and Estimates of Turbulence in the Polar Night Jet, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10840, https://doi.org/10.5194/egusphere-egu25-10840, 2025.

EGU25-11207 | ECS | PICO | AS1.32

Gravity wave analyses with CAIRT – Temperature measurements, GWMF, and ray-tracing 

Sebastian Rhode, Manfred Ern, Peter Preusse, Hanli Liu, Pramitha Maniyattu, Arun Mathew, Nick Pedatella, Björn-Martin Sinnhuber, and Jörn Ungermann

CAIRT, the Middle-Atmosphere candidate and one of two finalists for ESA’s Earth Explorer
11 mission, offers unprecedented capabilities for observing and understanding atmospheric
dynamics. With an advanced infrared limb imager with high spectral resolution in the range of
720 cm-1 to 2200 cm-1, CAIRT is designed to measure a wide range of trace gas
concentrations and temperature from the upper troposphere and lower stratosphere (UTLS)
up to the lower thermosphere. The instrument enables 3D tomographic retrieval along the
satellite track with an along-track resolution of 50 km and an across-track resolution of 25 km
within a 400 km swath. In particular, temperature observations span altitudes of about 10 to
110 km with a 500 m vertical resolution, making CAIRT well-suited for observing Gravity Wave
(GW) activity throughout the middle atmosphere.
Here, we highlight CAIRT’s capabilities for GW observation and analysis based on model
simulations and synthetic retrieval runs. First, we present the methodology to isolate a
planetary wave (PW) background directly from the temperature observations, which is
essential for deriving the residual, GW-induced temperature perturbations.
Secondly, we demonstrate the analysis of the temperature residuals using the S3D
methodology (based on sinusoidal fits in limited volume data cubes). The analysis enables
robust estimation of individual GW parameters and allows the calculation of GW momentum
fluxes and the associated GW drag, thereby shedding light into the role of GWs in the middle
atmosphere dynamics. In particular, we investigate the GW contribution to the sudden
stratospheric warming (SSW) event during northern hemisphere winter 2018/2019.
Furthermore, the S3D methodology determines the 3D wave vector for individual GWs,
which we use for the initialization of GW ray-tracing to extend our analysis beyond the
observation window, offering insights into GW evolution and potential source regions.
If CAIRT is chosen as the Earth Explorer 11 following the User Consultation Meeting in July
2025, the mission would greatly increase our observational capabilities within the middle
atmosphere and advance our understanding of the middle atmosphere dynamics.

How to cite: Rhode, S., Ern, M., Preusse, P., Liu, H., Maniyattu, P., Mathew, A., Pedatella, N., Sinnhuber, B.-M., and Ungermann, J.: Gravity wave analyses with CAIRT – Temperature measurements, GWMF, and ray-tracing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11207, https://doi.org/10.5194/egusphere-egu25-11207, 2025.

EGU25-12691 | ECS | PICO | AS1.32

Determining Oceanic Internal Solitary Waves Properties from Surface Signatures captured by SWOT Observations 

Tao Xu, Xu Chen, Qun Li, Xiao He, and Jing Meng

Internal solitary waves (ISWs) affect oceanic human activities and play an essential role in ocean mixing. Satellite observations provide a wide-ranging perspective for understanding ISWs. The surface current induced by ISWs can create rough and smooth regions on the sea surface due to the modulated roughness, presenting alternating bright and dark stripes in radar images. Moreover, the pressure distribution characteristic of ISWs creates surface solitons, leading to significant sea surface height anomalies in satellite altimetry. These signatures can be observed synchronously in a swath mode and high spatial resolution by surface water and ocean topography (SWOT) satellite, providing a unique new opportunity to understand both the surface and subsurface characteristics of ISWs. Numerous studies have established the correlation between the surface features and the ISWs parameters in the ocean interior, enabling the inversion of ISWs using remote sensing datasets. However, existing methods still require further improvement, as they are generated from specific assumptions and are highly dependent on the selection of ocean stratifications. By measuring surface divergence and surface height anomalies in laboratory experiments, this study establishes the relationship between surface features and internal characteristics of ISWs. The results reveal that both the strong nonlinearity and the effects of non-hydrostatic contribute significantly to the interpretation of ISWs' surface features, which pose challenges to the accurate retrieval of ISWs parameters. To address these problems, a fully nonlinear, non-hydrostatic method is developed and tested under different laboratory and oceanic conditions, demonstrating a precise connection between surface divergence, surface height anomaly and ISWs parameters. Based on this method, we use sea surface height anomalies and radar backscatter intensities provided by SWOT to perform the inversion. The results indicate that the combination of these two signatures enables accurate retrieval of ISWs parameters and the corresponding pycnocline depth, even if the real-time measurement of stratifications is not available. This study establishes a reliable method to understand ISWs in the global oceans and also provides insights into the challenge of separating ISWs signatures from other oceanic phenomena in SWOT observations.

How to cite: Xu, T., Chen, X., Li, Q., He, X., and Meng, J.: Determining Oceanic Internal Solitary Waves Properties from Surface Signatures captured by SWOT Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12691, https://doi.org/10.5194/egusphere-egu25-12691, 2025.

EGU25-12924 | ECS | PICO | AS1.32

How variable are gravity wave spectral energies? Insights from a seven-year lidar climatology at 69°N 

Mohamed Mossad, Irina Strelnikova, Robin Wing, Gerd Baumgarten, Michael Gerding, Jens Fiedler, and Yanmichel Morfa-Avalos

Despite significant progress in observational and theoretical studies on gravity wave (GW) dynamics, gaps remain in characterizing their variability and accurately representing their impact on the average state of the atmosphere in models. In particular, there is an altitudinal gap in estimating the kinetic and potential energy spectra of GWs between 30 and 70 km.

This study investigates the seasonal and altitudinal variations of GW energy spectra using high-resolution temperature and horizontal wind data recorded over seven years (2017-2023) by a Doppler Rayleigh lidar at the ALOMAR observatory (69°N, 16°E). We analyze spectral potential and kinetic energies across different frequencies and vertical wavenumbers to quantify the variability of dominant wave scales, amplitudes and spectral slopes. We also estimate the temporal and spatial variability of kinetic to potential energy ratio and its implication for the intrinsic values of observed GW frequencies. The findings aim to improve estimates of the atmospheric energy budget, compare theoretical predictions to observed data, and advance our understanding of the GW natural variability.

How to cite: Mossad, M., Strelnikova, I., Wing, R., Baumgarten, G., Gerding, M., Fiedler, J., and Morfa-Avalos, Y.: How variable are gravity wave spectral energies? Insights from a seven-year lidar climatology at 69°N, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12924, https://doi.org/10.5194/egusphere-egu25-12924, 2025.

EGU25-13965 | ECS | PICO | AS1.32

Reduction of the estimated gravity wave momentum flux by concurrent wave packets 

Brian Green, Aditi Sheshadri, and Aurelien Podglajen

Starting with simulations of idealized linear gravity wave packets, we show how interference between multiple gravity wave packets can result in an underestimation of their combined vertical flux of horizontal momentum by up to 50%. The two key ingredients for this result are the packets must have similar enough frequencies that their projections onto the time-frequency domain overlap, and that they propagate in different horizontal directions. This combination results in errors in the estimated phase relationship between wave-induced horizontal and vertical wind anomalies and reduces the estimate of the magnitude of the packets’ combined momentum flux. Because this mechanism doesn’t affect estimates of the power of a single variable, we propose using a scaling relationship derived from the theory of linear gravity waves in a Boussinesq atmosphere to estimate the momentum flux from the wave energy. We then apply this relationship to data from three lower stratosphere super-pressure balloon campaigns: Loon, Concordiasi, and Strateole-2. We find that both ingredients for wave interference are typically present in the data, evidence that our scaling relationship is appropriate for these calculations, and that momentum fluxes may be underestimated by even more than our simulations of idealized waves suggest. Our results show that the upward flux of horizontal momentum from the troposphere into the stratosphere by gravity waves is likely higher than previously thought, and that care must be taken analyzing output from models that resolve part of the gravity wave spectrum.

How to cite: Green, B., Sheshadri, A., and Podglajen, A.: Reduction of the estimated gravity wave momentum flux by concurrent wave packets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13965, https://doi.org/10.5194/egusphere-egu25-13965, 2025.

EGU25-33 | ECS | PICO | AS1.33

Automatic infrasound monitoring at the Central and Eastern European Infrasound Network via Machine Learning 

Marcell Pásztor, Tereza Šindelářová, Daniela Ghica, Ulrike Mitterbauer, Alexander Liashchuk, Giorgio Lacanna, Maurizio Ripepe, and István Bondár

The Central and Eastern European Infrasound Network (CEEIN) consists of nine infrasound arrays managed by research institutes in the Czech Republic, Austria, Hungary, Ukraine, and Romania. A hybrid machine learning model was previously developed to differentiate between natural and anthropogenic sources of infrasound. This model categorizes signals from thunderstorms, activity from Mount Etna, and human-related sources, including quarry blasts, power plants, oil refineries, and the conflict in Ukraine. The dataset includes more than 100,000 labeled detections spanning from 2017 to 2024. The hybrid model combines a Convolutional Neural Network, trained on spectrograms, with a Random Forest classifier, trained on features derived from the Progressive Multi-Channel Correlation (PMCC) method, which is used for processing the raw data. The model performed well on the test data (F1 score > 0.9); however, to assess its capabilities for near-real-time monitoring, the model was retrained with randomly selected, unlabeled detections from outside the aforementioned classes. Here, we present findings from several months of automatic monitoring, assessing both single array and network processing performance.

How to cite: Pásztor, M., Šindelářová, T., Ghica, D., Mitterbauer, U., Liashchuk, A., Lacanna, G., Ripepe, M., and Bondár, I.: Automatic infrasound monitoring at the Central and Eastern European Infrasound Network via Machine Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-33, https://doi.org/10.5194/egusphere-egu25-33, 2025.

EGU25-783 | ECS | PICO | AS1.33

Enhanced Lidar Signal Interpretation of Gravity Waves Using Multiresolution Analysis 

Samuel Trémoulu, Fabrice Chane-Ming, Sergey Khaykin, and Philippe Keckhut

Atmospheric gravity waves (GWs) are a key area of research due to their significant impact on atmospheric dynamics and chemistry, as well as the ongoing challenges in resolving small-scale structures in weather prediction and climate models. Over the past four decades, lidars have proven to be invaluable observational instruments for providing detailed insights into vertically propagating GWs in the middle atmosphere.

To advance the characterization of GWs, various signal processing techniques have been developed to extract GW-induced perturbations and calculate their associated potential and kinetic energy densities. In this study, we introduce a multiresolution analysis (MRA) method that enhances the interpretation of lidar signals by decomposing GWs into successive vertical wavelength bands, enabling a more refined understanding of their structure and dynamics. The MRA method is compared to conventional approaches by extracting perturbations and computing energy density profiles from temperature (from 30 to  80 km) and wind (from 7 to 60 km) lidar profiles observed on the night of November 20, 2023, over La Réunion (21.0°S, 55.5°E). 

The results highlight the MRA method's superior efficiency in analyzing GWs embedded within lidar vertical profiles of temperature and horizontal wind, offering a powerful tool for advancing the study of atmospheric wave processes in the middle atmosphere.

How to cite: Trémoulu, S., Chane-Ming, F., Khaykin, S., and Keckhut, P.: Enhanced Lidar Signal Interpretation of Gravity Waves Using Multiresolution Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-783, https://doi.org/10.5194/egusphere-egu25-783, 2025.

EGU25-3753 | ECS | PICO | AS1.33

Using an oceanic acoustic noise model to evaluate simulated atmospheric states 

Pierre Letournel, Constantino Listowski, Marc Bocquet, Alexis Le Pichon, and Alban Farchi

Infrasound of oceanic origin, known as microbaroms, are globally and continuously detected by the infrasound stations of the International Monitoring System. They propagate over thousands of kilometers thanks to acoustic waveguides in the middle and upper atmosphere (~30-120 km). At these altitudes, Numerical Weather Prediction (NWP) models are biased, partly due to the lack of operationally assimilated observations that constrain model predictions (especially for winds). We present a processing chain that simulates microbarom arrivals at infrasound stations by coupling a microbarom source model and infrasound propagation modelling. These arrivals are modelled using atmospheric specifications from different NWP models and compared to the microbarom observations using a multidirectional metric. The objective of this processing chain is twofold: evaluating the relative performances of NWP models in support of operational infrasound monitoring activities and demonstrating the benefit of assimilating unconventional observations such as microbaroms in NWP models. To this end, we apply the processing chain to several infrasound stations and highlight NWP performance assessments during a sudden stratospheric warming and other dynamical events of the middle and upper atmosphere.

How to cite: Letournel, P., Listowski, C., Bocquet, M., Le Pichon, A., and Farchi, A.: Using an oceanic acoustic noise model to evaluate simulated atmospheric states, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3753, https://doi.org/10.5194/egusphere-egu25-3753, 2025.

A new 4-element infrasound array (AGIR) of 0.2 km aperture was deployed by National Institute for Earth Physics (NIEP) in August 2024 in Eastern Romania, on the Black Sea coast. Between August and October, during the strong thunderstorms that crossed this region, long-duration trains of frequent sharp spikes in the amplitude associated with lightning discharges were observed into AGIR infrasound recordings. Some of these storm episodes could be correlated to cyclones moving over the Black Sea and greatly affecting Romania's regional climate in 2024.

We examined data from NIEP's current infrasound network – BURARI, IPLOR and AGIR stations –, in order to study the possibilities of infrasound-based monitoring of extratropical cyclones over the Black Sea. Association between infrasound detections into 0.5 to 7 Hz frequency band and lightning flashes detected by MTG Lightning Imager within 50 km from the AGIR infrasound station was investigated, assuming direct wave propagation path. Acoustic signatures of lightning activity show short-lived disturbances with dominant frequency of approx. 3 Hz and amplitudes up to about 3.5 Pa.

In addition to the strong lightning discharges during the storms, the cyclones were also accompanied by strong winds that produced waves in the Black Sea. We can consider these waves to be the cause of the significant fluctuations observed into the microbarom detections in the Black Sea region at BURARI and IPLOR stations, into the 0.1 Hz to 1 Hz frequency band. Microbarom power spectral noise amplitudes peak was observed around 0.3 Hz. Microbaroms detections are strongly influenced both by seasonally dependent stratospheric winds and local turbulence-induced pressure fluctuations. Local wind was averaged for the BURARI and IPLOR locations using NRL-G2S wind fields.

Infrasound signatures linked with certain extratropical cyclonic episodes were well identified. To improve storm track estimates, these infrasound-based detections were subsequently combined with conventional meteorological data including surface observations, electric field measurements, and satellite data. This study shows the potential of Romania's current infrasound infrastructure to support extratropical cyclone surveillance and improve forecasting capability in the region, even when more calibration of detection thresholds and source characterisation is required.

How to cite: Ghica, D., Antonescu, B., and Ene, D.: Using Romanian infrasound observations to analyze thunderstorms generated by extratropical cyclones over the Black Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5592, https://doi.org/10.5194/egusphere-egu25-5592, 2025.

EGU25-6678 | ECS | PICO | AS1.33 | Highlight

Observation of mountain waves and secondary gravity waves in the MLT over Patagonia 

Robert Reichert, Dominique Pautet, Bernd Kaifler, Diego Janches, Jörn Ungermann, Sebastian Rhode, and Kaoru Sato

On the night of 21/22 May 2018, clear-sky conditions enabled a 12-hour-long temperature measurement of the Advanced Mesospheric Temperature Mapper (AMTM) in the mesosphere-lower thermosphere (MLT) region over Río Grande, Argentina. Given a westerly forcing over Patagonia, we observe North-South-oriented phase lines in the AMTM temperature maps exclusively during the westerly phase of the semi-diurnal tide, indicating the deep propagation of mountain waves (MWs) with horizontal wavelengths between 20 km and 40 km. After a wind reversal in the MLT, we observe two large-scale gravity waves (GWs) propagating rapidly in a south-eastward direction. We use one- and two-dimensional wavelet analysis to characterize the observed GWs and find that their wavelengths and phase speeds are consistent with secondary GW theory. Ray tracing results suggest a possible source region for these 2GWs located north-westward, near the Chilean Torres del Paine region. In addition, co-located temperature and wind measurements from the Compact Rayleigh Autonomous Lidar (CORAL) and the Southern Argentine Agile Meteor Radar (SAAMER), in combination with a Monte Carlo approach, allow for the accurate determination of both the GW momentum flux and its uncertainty. Although we exclude a direct cause-and-effect relationship within our field of view, we find that, on average, the observed MWs carry momentum fluxes an order of magnitude larger than those of the 2GWs.

How to cite: Reichert, R., Pautet, D., Kaifler, B., Janches, D., Ungermann, J., Rhode, S., and Sato, K.: Observation of mountain waves and secondary gravity waves in the MLT over Patagonia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6678, https://doi.org/10.5194/egusphere-egu25-6678, 2025.

EGU25-7087 | ECS | PICO | AS1.33

Studying infrasound propagation in the middle atmosphere with UA-ICON: parameterisation and characterisation of gravity waves with the Multi-Scale Gravity Wave Model 

Samuel Kristoffersen, Constantino Listowski, Georg-Sebastian Voelker, Ulrich Achatz, Julien Vergoz, and Alexis Le Pichon

Infrasound signals are used to monitor various anthropogenic and natural sources. To determine accurate source locations and energy, an accurate model of wind and temperature from the surface up to the lower thermosphere is necessary, hence operational NWP products are of great importance for routine infrasound monitoring activities. However, many of these models focus on tropospheric conditions, and the middle and upper atmosphere, where the relevant infrasound waveguides for long-range propagation are found, is not well represented. UA-ICON is an upper atmosphere version of the ICOsahedral Non-hydrostatic weather and climate model (ICON) that provides modelled atmospheric parameters up to 150 km. From an infrasound perspective, small-scale perturbations - most notably gravity waves - can have a large impact on propagation due to the effects on both the background winds and temperatures, hence on the acoustic waveguides, but also due to the small perturbations they produce, which cause partial reflections of acoustic waves. Therefore, the transient-3D Multi-Scale Gravity Wave Model (MSGWaM) was used within UA-ICON to produce accurate background conditions, and predict the global gravity wave activity. We will present the methodology used to generate the wind and temperature gravity wave perturbation profiles, as well as analysis of infrasound propagation using these gravity wave realisations. 

How to cite: Kristoffersen, S., Listowski, C., Voelker, G.-S., Achatz, U., Vergoz, J., and Le Pichon, A.: Studying infrasound propagation in the middle atmosphere with UA-ICON: parameterisation and characterisation of gravity waves with the Multi-Scale Gravity Wave Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7087, https://doi.org/10.5194/egusphere-egu25-7087, 2025.

EGU25-7109 | PICO | AS1.33

A revisited Bayesian framework to predict the performance of the IMS infrasound network 

Alexis Le Pichon, Julien Vergoz, Patrick Hupe, Constantino Listowski, and Samuel Kristoffersen

The detection capability of the International Monitoring System (IMS) deployed to monitor compliance with the Comprehensive Nuclear-Test ban Treaty (CTBT) is highly variable in space and time. Previous studies estimated the source energy from remote observations using empirical yield-scaling relations. However, these relations simplified the complexities of infrasound propagation as the wind correction applied does not account for an accurate description of the middle atmosphere along the propagation path. In order to reduce the variance in the calculated transmission loss, massive frequency and range-dependent full-wave propagation simulations are carried out, exploring a wide range of realistic atmospheric scenarios. A cost-effective approach is proposed to estimate the transmission losses at distances up to 4,000 km along with uncertainties derived from multiple gravity wave realizations. Transmission loss statistics are combined with an explosive source model and noise statistics to quantify the 90% probability detection threshold of the IMS network. In the context of the future verification of the CTBT, this approach helps advance the development of network performance simulations in higher resolution and the evaluation of middle atmospheric models at a global scale with limited computational resources.

How to cite: Le Pichon, A., Vergoz, J., Hupe, P., Listowski, C., and Kristoffersen, S.: A revisited Bayesian framework to predict the performance of the IMS infrasound network, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7109, https://doi.org/10.5194/egusphere-egu25-7109, 2025.

EGU25-7111 | PICO | AS1.33

Using seismic data to detect and locate meteors with the Epos-France Permanent Broadband Network 

Aurélien Dupont, Gilles Mazet-Roux, Sami Azzaz, and Alexis Le Pichon

The Epos-France Permanent Broadband Network (RLBP), originally designed for earthquake monitoring, provides real-time seismic data from over 200 stations across mainland France, enabling the detection and localization of atmospheric events such as meteors. This is achieved through seismic-acoustic coupling, where shock waves generated by meteors can be recorded by the network's sensors. We apply the Reverse Time Migration (RTM) method to identify acoustic sources of interest with accuracy. The method uses a "grid search" approach to evaluate potential source points, ordering seismic traces by distance (hodochrone) and calculating the sum of the envelopes of interest according to the velocity model considered. The integration of atmospheric data from the ECMWF model and an attenuation law optimizes this process by selecting the most relevant seismic stations, increasing signal-to-noise ratios, and improving localization precision. We present case studies including the fragmentation of a meteor over Normandy, France (February 13, 2023) and the eruption of Stromboli Volcano, Italy (July 11, 2024) enabling precise dating of the paroxysm and localization to within a few kilometers of the Sciara del Fuoco (i.e. ground truth validation). This approach, which allows for the localization of a meteor without direct visual observation, regardless of weather conditions or time of day, aims to complement the optical observations of the FRIPON network. Ongoing work that we also present aims to further refine the method to detect other anthropic phenomena in the atmosphere, such as satellite debris and jet shock waves, thereby enhancing the seismic network's ability to monitor an increasingly wide range of events.

How to cite: Dupont, A., Mazet-Roux, G., Azzaz, S., and Le Pichon, A.: Using seismic data to detect and locate meteors with the Epos-France Permanent Broadband Network, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7111, https://doi.org/10.5194/egusphere-egu25-7111, 2025.

EGU25-7290 | ECS | PICO | AS1.33

The Volcanic Information System: Long-Range Infrasound Monitoring of Volcanic Eruptions With Open-Access Datasets And Year-Long Back-Azimuth Deviation Bias Predictions 

Rodrigo De Negri, Patrick Hupe, Duccio Gheri, Alexis Le Pichon, Emanuele Marchetti, Peter Näsholm, Pierrick Mialle, and Philippe Labazuy

Energetic volcanic eruptions can inject large amounts of ash into the atmosphere, posing a direct threat to commercial flights and potentially overwhelming populations down the ash plume path. These eruptions also produce infrasound –acoustic waves below 20 Hz– which can propagate over hundreds to thousands of kilometers in the atmosphere due to favorable ducting conditions and its intrinsic low attenuation.

Within the Atmospheric dynamics Research InfraStructure in Europe (ARISE) project (FP7, H2020), in collaboration with the Toulouse Volcanic Ash Advisory Centre (VAAC), the Volcanic Information System (VIS) was created as a prototype monitoring system that uses long-range (>250 km) infrasound recordings to remotely detect and notify of explosive eruptions.

The VIS was designed to primarily use data recorded by the global International Monitoring System (IMS) infrasound network (53 stations of 60 planned stations), but it can also include non-IMS arrays (e.g., AMT, Florence, Italy) to increase the coverage. At its core, the VIS relies on a data processing output denoted the Infrasound Parameter (IP) to establish when an eruption occurs. The IP value accounts for propagation effects, detection persistency, and infrasound signal amplitude.

Currently, we are thoroughly testing the capabilities of the VIS, and considering the future developments that can be implemented to improve its reliability, before it is made publicly available.

Our recent efforts have expanded the VIS capabilities to use open-access (OA) streamlined and standardized IMS-derived infrasound array signal processing data products. We found that the eruption notification results using OA data were comparable to the notifications calculated with regular IMS data (i.e., PMCC detections).

In this work, we look in detail into the eruptive periods of April 2010 Eyjafjallajökull (Iceland), May 2016 Etna (Italy), and April 2021 La Soufrière (Saint Vincent island, Saint Vincent and the Grenadines), and test how year-long back-azimuth deviation predictions (i.e., pre-calculated back-azimuth bias values) for the nearest IMS stations (<2500 km) can help decreasing the eruption notification false positives and improve the VIS overall reliability. We compare the VIS notification results with detections calculated using both OA and PMCC data, and incorporate the available HOTVOLC webGIS satellite notifications (2010-2022), plus other available eruption catalogues (e.g., Global Volcanism Program). We present a preliminary eruption catalogue for these cases, and show to what extent infrasound-only, and infrasound+satellite monitoring (ASH2/ASH5 products from HOTVOLC) can achieve reliable eruption notifications in the studied areas.

As part of the European Geo-INQUIRE project (HORIZON-INFRA-2021-SERV-01), the VIS will be integrated into the Thematic Core Service Volcano Observation (TCS-VO) of the European Plate Observing System (EPOS). Future developments will also include integration into web services such as the HOTVOLC web-GIS interface (OPGC, CNRS-INSU) or the EPOS Data Portal.

How to cite: De Negri, R., Hupe, P., Gheri, D., Le Pichon, A., Marchetti, E., Näsholm, P., Mialle, P., and Labazuy, P.: The Volcanic Information System: Long-Range Infrasound Monitoring of Volcanic Eruptions With Open-Access Datasets And Year-Long Back-Azimuth Deviation Bias Predictions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7290, https://doi.org/10.5194/egusphere-egu25-7290, 2025.

EGU25-9300 | ECS | PICO | AS1.33

Tracking jet stream winds through gravity waves arriving on surface based pressure sensors 

Falco Bentvelsen, Jelle Assink, and Läslo Evers

Jet stream winds play an important role in our daily weather. Accurate wind and temperature estimations in the upper troposphere can lead to better medium to long-term weather forecasts. However, continuous measurement in the upper troposphere poses challenges, resulting in relatively sparse data.

This study revisits research from the 1960s and 1970s, on the use of ground-based pressure measurements as a measure for jet stream winds. It has been established that the jet stream can generate atmospheric gravity waves that radiate to the ground. Since the previous work, a global network of microbarometers has been established for verification of the Comprehensive Nuclear-Test-Ban Treaty (CTBT). This network provides continuous pressure data that holds valuable information about the jet stream.

We present results from a microbarometer array in Southern Germany (IS26). The pressure data has been processed for frequencies within a range of 0.1 - 2 mHz, where gravity waves are detected. Signal characteristics from the array analysis, such as direction-of-arrival and incidence angle, enable a detailed monitoring of the jet stream strength and direction. The characteristics of these gravity waves are compiled, and compared to hourly ECMWF ERA5 model data and other observations, such as radiosonde balloon measurements.

How to cite: Bentvelsen, F., Assink, J., and Evers, L.: Tracking jet stream winds through gravity waves arriving on surface based pressure sensors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9300, https://doi.org/10.5194/egusphere-egu25-9300, 2025.

EGU25-10204 | ECS | PICO | AS1.33

Deep learning-based method for near-real time estimation of infrasound transmission losses in theatmosphere 

Alice Janela Cameijo, Youcef Sklab, Souhila Arib, Alexis Le-Pichon, Samir Aknine, Quentin Brissaud, and Sven Peter Näsholm

Accurately modeling transmission loss is essential for a variety of applications, such as
improving atmospheric data assimilation for numerical weather prediction, assessing attenuation
maps of sources of interest, or estimating detection capabilities of the International Monitoring
System infrasound network. However, the high computational cost of numerical modeling solvers
makes them impractical for a near-real-time analysis. To address this, a previous study trained a
Convolutional Neural Network on regional wind fields, predicting transmission losses in less than 0,05
seconds with a mean-squared error of 5 dB. However, this approach uses interpolated atmospheric
specifications and focused only on winds, limiting its applicability for long-range modeling. In this
work, we develop a convolutional recurrent network to predict transmission losses leveraging
realistic, range-dependent atmospheric specifications combining horizontal winds and temperatures,
including small-scale perturbations. The resulting model reaches an error of 4 dB while extending
propagation range up to 4,000 km and providing epistemic and data uncertainty estimates. First
studies of such an algorithm on regional scaled events (Tonga-Hunga eruption, Hukkakero explosions,
etc.) were performed to further evaluate the model. Predicted attenuation are compared with
results from an alternative regionally fine-tuned neural network. The model also demonstrated its
ability to adapt to new frequencies.

How to cite: Janela Cameijo, A., Sklab, Y., Arib, S., Le-Pichon, A., Aknine, S., Brissaud, Q., and Näsholm, S. P.: Deep learning-based method for near-real time estimation of infrasound transmission losses in theatmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10204, https://doi.org/10.5194/egusphere-egu25-10204, 2025.

EGU25-12989 | ECS | PICO | AS1.33

A mobile universal Doppler-lidar for collocated, high-resolution measurements of winds and temperatures in the middle atmosphere 

Thorben Mense, Josef Höffner, Jan Froh, Ronald Eixmann, Alsu Mauer, Gerd Baumgarten, Alexander Munk, Michael Strotkamp, and Sarah Scheuer

Precise knowledge of winds and temperatures in the middle atmosphere is critical for the localization and characterization of infrasound sources. We present the concept, design, and measurement capabilities of a compact, mobile Doppler lidar system developed at the Leibniz Institute of Atmospheric Physics (IAP). This system, is designed for Doppler-Mie, -Rayleigh, and -resonance measurements in the middle atmosphere.

The daylight-capable instrument features a compact volume of about 1 m³ and is engineered for easy deployment as part of an array of lidar units. We highlight recent results, emphasizing collocated, high-resolution measurements of wind and temperature. By employing three to five individual fields of view, the system can measure both horizontal and vertical wind components. Between altitudes of 3 and 25 km, the instrument utilizes the narrowband properties of Mie backscatter, relying solely on aerosol backscatter to achieve precise three-dimensional wind measurements. In this altitude range, a novel method enables the measurement of vertical winds with an accuracy better than 0.5 m/s and a time resolution of just 60 seconds.

Above 25 km, winds will be measured using Doppler-Rayleigh and -resonance techniques. Concurrent Rayleigh temperature measurements utilize advanced aerosol correction methods, taking advantage of the instrument's high sensitivity to aerosols.

The feasibility of integrating this lidar system into a European lidar array is being investigated within the EULIAA (European Lidar Array for Atmospheric Climate Monitoring) project. The transfer of this technology to industry is currently being developed through the LidarCUBE project.

How to cite: Mense, T., Höffner, J., Froh, J., Eixmann, R., Mauer, A., Baumgarten, G., Munk, A., Strotkamp, M., and Scheuer, S.: A mobile universal Doppler-lidar for collocated, high-resolution measurements of winds and temperatures in the middle atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12989, https://doi.org/10.5194/egusphere-egu25-12989, 2025.

EGU25-14647 | PICO | AS1.33

Using infrasound observations and data assimilation to detect atmospheric variability over short timescales 

Javier Amezcua, Gil Averbuch, Sven Peter Nasholm, and Stephen Arrowsmith

Atmospheric variability at short time-scales (seconds to minutes) is challenging to detect, quantify, and include in numerical models of atmospheric circulation. Infrasound can be generated by natural and anthropogenic sources, and due to the low frequency of the signal, it can travel relatively long distances (hundreds to thousands of kilometers) and be detected by acoustic arrays. When detected, the observed wavefront properties quantities (travel time, backazimuth angle, apparent velocity) contain integrated effects of the atmospheric slab through which the wave traveled. We use data assimilation, in particular an ensemble Kalman filter, to invert these observations to atmospheric quantities. As observations, we use three days of daily infrasonic signals originating from 52 explosions. The signals propagated through the stratospheric waveguide and were recorded at a distance of 256 km. The assimilation background field is provided by the 10-member ERA ensemble reanalysis product, which is valid every 3 hours. The departures with respect to the background shed light to the atmospheric variability in very short time-scales (minutes). 

How to cite: Amezcua, J., Averbuch, G., Nasholm, S. P., and Arrowsmith, S.: Using infrasound observations and data assimilation to detect atmospheric variability over short timescales, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14647, https://doi.org/10.5194/egusphere-egu25-14647, 2025.

EGU25-18062 | ECS | PICO | AS1.33

Source and subsurface inversion using earthquake-generated infrasound recorded at a balloon platform: application to the 2021 Mw 7.3 Flores earthquake 

Marouchka Froment, Quentin Brissaud, Sven Peter Näsholm, Johannes Schweitzer, and Tina Kaschwich

Seismic waves can couple to the atmosphere and propagate as acoustic waves, including infrasound at frequency below 20 Hz. Seismically generated infrasound can be recorded by ground-based microbarometers, but also at higher-altitude by pressure sensors carried by balloons. Balloon-borne acoustic observations could be the key to exploring Venus' interior, as surface conditions do not allow for the deployment of seismometers. However, it remains unclear how much information about the subsurface is contained in seismically generated infrasound.  

In this contribution we use the recent earthquake-induced acoustic observations from a balloon network on Earth belonging to the Strateole2 campaign, following the 2021 Mw 7.3 earthquake in the Flores Sea, to invert for subsurface velocities. Seismic infrasound signals show body wave arrivals and surface wave dispersion similar to pure seismic signals recorded on the ground. Thus, beyond their detection capability, balloon infrasound also enables the use of classical inversion techniques to retrieve source and subsurface properties. We develop an inversion framework to jointly retrieve earthquake source location and seismic velocities of the subsurface based on arrival time measurements for P, S and Rayleigh waves at multiple balloon stations. We apply this approach to the Flores earthquake using data from four Strateole2 balloons.  

The inversion results are the probability density distribution of the seismic source location and of the subsurface velocities in a layered model. Both the resulting location and subsurface model are in good agreement with those obtained from traditional seismic data, confirming balloon seismology as a credible alternative for the seismic exploration of the Earth and other celestial bodies with atmospheres, such as Venus. 

How to cite: Froment, M., Brissaud, Q., Näsholm, S. P., Schweitzer, J., and Kaschwich, T.: Source and subsurface inversion using earthquake-generated infrasound recorded at a balloon platform: application to the 2021 Mw 7.3 Flores earthquake, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18062, https://doi.org/10.5194/egusphere-egu25-18062, 2025.

EGU25-19412 | ECS | PICO | AS1.33

High-resolution analysis of spatiotemporal ambient noise variations across the infrasound network of the International Monitoring System 

Patrick Hupe, Alexis Le Pichon, Julien Vergoz, and Christoph Pilger

Temporal variations of the noise conditions constrain the ability to detect and identify signals of interest at infrasound stations. Station-dependent factors that contribute to the noise include incoherent wind and turbulence. A coherent source of ambient noise at the global infrasound station network of the International Monitoring System are microbaroms from the oceans, which vary seasonally such that most stations observe the maximum noise during local winter.

For a realistic estimate of the station noise statistics, we computed the power spectral density (PSD) at all 53 elements of the operational IMS stations on an hourly basis over a four-year period (2021-2024), resulting in more than 10 million computed PSDs. This systematic processing of the background noise allows an assessment of the sensitivity of each measurement system to geographic and environmental parameters that include both wind-generated noise and coherent signals from geophysical and anthropogenic events. Using this unique high-resolution PSD dataset, we analyse the spatiotemporal noise variation across the IMS network and also examine local effects at the array sites such as vegetation or snow cover that also contribute to the noise level. This work aims at updating earlier statistical ambient noise models and facilitating detection capability simulations with high temporal resolution.

How to cite: Hupe, P., Le Pichon, A., Vergoz, J., and Pilger, C.: High-resolution analysis of spatiotemporal ambient noise variations across the infrasound network of the International Monitoring System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19412, https://doi.org/10.5194/egusphere-egu25-19412, 2025.

EGU25-848 | ECS | Posters on site | CL3.2.4

Heat Stress Threats in Europe: A Comprehensive Analysis of sWBGTVariations and Trends (1979 -2023) 

Qi Zhang, Joakim Kjellsson, Emily Black, and Julian Krüger

Heat stress has lately been acknowledged as a significant threat to public health, with heat waves becoming more frequent and severe due to global warming. The Simplified Wet Bulb Globe Temperature (sWBGT) is a effective indicator for heat stress, combining both temperature and relative humidity. Using observations and reanalysis datasets, we identify annual heatwave days (HWD) and analyze sWBGT variations and trends during HWD. We focus on three European regions: Northern Europe (NEU), Western and Central Europe (WCE), and the Mediterranean (MED). We observed an increasing trend in sWBGT over most of Europe , with the exception of areas around the Black Sea, parts of eastern and western WCE, and the western MED. Importantly, the  contribution of temperature and humidity on heat stress vary by regions. In NEU, positive trends in both temperature and relative humidity contribute to increased heat stress, with temperature showing a more significant rising trend (0.4°C/decade). In WCE, while the overall trend in sWBGT is positive, changes in relative humidity are minimal (0.007% /decade), with temperature trends being the primary driver. In MED, a positive trend in sWBGT of 0.3 /decade is a residual of a  negative trend in relative humidity and a positive temperature trend. Comparing ERA5 dataset with meteorological station data revealed biases in the ERA5 data in Mediterranean cities with pronounced urban heat island effects. Analysis of sWBGT threat levels showed that NEU and WCE regions currently remain at safe levels. In contrast, most MED regions are at alert levels, with some areas escalating to caution levels. Our research provides comprehensive insights into heat stress variations across European regions over recent decades. This work can provide scientific evidence to help policymakers develop effective adaptation to address potential future heat stress threats.

How to cite: Zhang, Q., Kjellsson, J., Black, E., and Krüger, J.: Heat Stress Threats in Europe: A Comprehensive Analysis of sWBGTVariations and Trends (1979 -2023), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-848, https://doi.org/10.5194/egusphere-egu25-848, 2025.

EGU25-916 | ECS | Orals | CL3.2.4

Atmospheric and Oceanic Processes Behind Extreme Precipitation: A Case Study of the Western Ghats 

Leena Khadke, Sachin Budakoti, Akash Verma, Moumita Bhowmik, and Anupam Hazra

India has experienced a notable rise in the intensity, frequency, and spatial extent of extreme weather events in recent decades, with extreme precipitation along the southwest coast being particularly alarming. The drivers behind these events remain uncertain due to the variability in meteorological and oceanic factors and associated large-scale circulations. The present study attempted to identify a combination of dynamic, thermodynamic, and cloud microphysics processes contributing to the anomalous precipitation over the southwest coast of India from 1-10 August 2019 against its climatology using reanalysis and observational datasets. Key findings reveal the critical role of warm sea surface temperature anomalies (>1.4°C), reduced outgoing longwave radiation (<-50 W/m²), and elevated atmospheric temperatures (>1.6°C over the ocean) in enhancing atmospheric moisture capacity by nearly 10%. Strengthened low-level winds (anomalies >4 m/s) transported this moisture from the ocean to the land, while vertical updrafts (> -0.4 m/s anomalies) increased atmospheric instability and moisture convergence. Additionally, significant anomalies in cloud hydrometeors (>2.5×10⁻⁴ Kg/Kg) supported prolonged intense precipitation. These results improve our understanding of the interaction between ocean-atmosphere dynamics and wind patterns, highlighting their vital role in shaping regional weather and climate.

Keywords: Extreme precipitation, Western ghats, Atmospheric processes, Reanalysis.

How to cite: Khadke, L., Budakoti, S., Verma, A., Bhowmik, M., and Hazra, A.: Atmospheric and Oceanic Processes Behind Extreme Precipitation: A Case Study of the Western Ghats, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-916, https://doi.org/10.5194/egusphere-egu25-916, 2025.

EGU25-1049 | ECS | Posters on site | CL3.2.4

Analysis of projected monthly changes of extreme temperature indices to support decision-makers 

Ferenc Divinszki, Anna Kis, and Rita Pongrácz

As global warming intensifies, the building of adaptation and mitigation strategies has become an urgent task. In the centre of these strategies often lie extreme weather events, which are expected to become even more severe and more frequent in the next decades. Therefore, extending our knowledge on the potential changes in these events is crucial to provide assistance for appropriate preparation and planning necessary actions. Using the latest CMIP6 global climate model simulations available in the IPCC’s Interactive Atlas (IA), a study on extreme events focusing on Europe was completed, with special emphasis on Central Europe.

Our goal was to study the potential changes of extreme temperatures over the continent, in order to analyse the spatial patterns and trends of changes for the end of the 21st century. First, monthly multi-model mean data were downloaded from the IA for two different extreme temperature indices. The number of days with maximum temperature above 35 °C (i.e. TX35) and the number of days with a minimum temperature below 0 °C (i.e. frost days or FD) were selected for the analysis. The use of both hot and cold extreme temperature indices enabled us to cover every month in our study with TX35 analysed in the May–September and FD in the October–April period. Our target period was the 2081–2100 period compared to the values of 1995–2014 (i.e. the last two decades of the historical simulation period) as a reference. Every scenario available in the IA was considered, namely, SSP1-2.6, SSP2-4.5, SSP3-7.0 and SSP5-8.5.

Six zonal segments were defined over Europe to analyse the projected changes, ensuring that the segments fairly cover the continent. This approach is able to reveal the major effects creating the spatial patterns in different regions. The most important effects are (i) the differences due to the north-south or east-west locations (i.e. the zonal and continental effects), (ii) elevation above sea level (i.e. the orographical effect), and (iii) the different levels of anthropogenic forcing (i.e. the different scenarios).

Our results show that the anthropogenic effect is a key factor due to the direct connection between the greenhouse effect and air temperature. Moreover, the sea-land surface differences have the greatest effect on the magnitude of changes in the indices, while continentality is also an important factor. Potential differences due to elevation, however, are often supressed by the spatial patterns created by sea-land differences.

How to cite: Divinszki, F., Kis, A., and Pongrácz, R.: Analysis of projected monthly changes of extreme temperature indices to support decision-makers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1049, https://doi.org/10.5194/egusphere-egu25-1049, 2025.

EGU25-1556 | ECS | Orals | CL3.2.4

A global Lagrangian analysis of near-surcface warm and cold temperature extremes 

Amelie Mayer and Volkmar Wirth

Temperature extremes have a substantial impact on society and the environment, however a full physical understanding of their formation mechanisms is still lacking. In particular, the relative importance of the three key processes – horizontal temperature transport, subsidence accompanied by adiabatic warming, and diabatic heating – is still debated. Here, we present a global quantification of the contributions from these processes to near-surface warm and cold extremes using the Lagrangian framework. To this end, we apply two different Lagrangian temperature anomaly decompositions: one based on the full fields of the respective terms, and the other one based on the anomaly fields of the respective terms (i.e., deviations from their corresponding climatologies). We will show that the results from the full-field decomposition mostly align with those of a previous study, while the anomaly-based decomposition offers a completely new assessment of the roles of the different processes, especially with regard to warm extremes.

How to cite: Mayer, A. and Wirth, V.: A global Lagrangian analysis of near-surcface warm and cold temperature extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1556, https://doi.org/10.5194/egusphere-egu25-1556, 2025.

EGU25-1678 | Orals | CL3.2.4

How do transitions from dry to wet states propagate to drought-to-flood transitions? 

Manuela Irene Brunner, Bailey Anderson, and Eduardo Munoz-Castro

Transitions from dry to wet states challenge water management and can lead to severe impacts on infrastructure and water quality. Such transitions occur both in the atmosphere and hydrosphere, that is, from dry-to-wet spells and from droughts to floods, respectively. While transitions from dry-to-wet spells, i.e. from negative to positive precipitation anomalies, are relatively well studied, it is yet unclear how they propagate to hydrological transitions from negative to positive streamflow anomalies. Here, we address the question of how often, where, when, and why meteorological transitions do propagate to drought-to-flood transitions using a large-sample dataset of precipitation and streamflow observations over Europe. Our analysis of the relationship between meteorological and hydrological transition events shows that only 10% and 25% of the dry-to-wet transitions propagate to drought-to-flood transitions at a monthly and annual time scale, respectively. The limiting factors for transition propagation are clear differences in the seasonality of meteorological and hydrological transitions and the limited propagation of wet spells, in particular those with low precipitation intensities and small volumes. Transition propagation is most likely in small and rainy catchments, that is, catchments with a relatively direct link between precipitation and streamflow and limited storage influences. We conclude that hydrological transitions are only weakly related to meteorological transitions, which highlights the important influence of land-surface and storage processes for the development of hydrological transitions. As a consequence, changes in dry-to-wet transitions are a relatively poor proxy for future changes in drought-to-flood transitions.

How to cite: Brunner, M. I., Anderson, B., and Munoz-Castro, E.: How do transitions from dry to wet states propagate to drought-to-flood transitions?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1678, https://doi.org/10.5194/egusphere-egu25-1678, 2025.

Humid heatwaves negatively affect human health due to the integrating effect of temperature and humidity, and thus the early warning and timely mitigating on climate extremes are essential. Yet, systematic assessment on the intra‐annual onset and end of humid heatwaves, which is associated to the occurrence of first and last humid heatwaves, are missing globally. Using a new station‐based data set of daily maximum wet‐bulb temperature, the start and end dates, cumulative anomaly and extremely humid heat of the first and last humid heatwaves in the Northern Hemisphere were explored. It was found that at 91.54% of stations, humid heatwaves started earlier or ended later in the period of 2001–2020 compared to 1981–2000. High cumulative anomalies of the first or last humid heatwaves were found in the mid‐ and high‐latitude regions. Average difference between all humid heatwaves and the first humid heatwaves in cumulative anomalies increased steadily at stations north of 35°N. At regional scales, South East Asia had become the most prominent area with intensification of intra‐annual onset and end of humid heatwaves and will experience more frequent extreme events by 2100.

Furthermore, our focus goes from physical understanding to exposure impacts. Human exposure to humid heatwaves develops with the significant intensification of extreme humid-heat and population agglomeration. Although urban areas are typical spaces of the heat stress, urban heat is expanding outward to rural areas spatially. However, the difference of long-term changes and attributions between urban and rural human exposure to humid heatwaves is still unclear, especially lacking global comparisons supported by continuous series. We also used the new wet-bulb temperature dataset and integrated scenario data to assess historical and future human exposure to humid heatwaves in the Northern Hemisphere. The differences between urban and rural areas in the contribution of enhanced heatwaves and increasing population were quantified. The results showed that about 96.62 % of the stations had pronounced increases in human exposure among those with significant changes. The domination of enhanced heatwaves to human exposure rate was stronger in urban areas in typical developed countries, while domination of increasing population was higher in rural areas in eastern China, with 87.5 % of rural stations dominated by population growth. Under extremely increasing conditions in SSP5 scenario, average rates of human exposure to humid heatwaves in rural areas would be 11.78 % higher than urban areas.

Our findings demonstrated more intensified characteristics of the intra‐annual onset and end of humid heatwaves and provide a scientific cognition for the local risk of humid heatwaves.

How to cite: Dong, J.: Intra‐annual occurrence and risk of humid heatwave in the Northern Hemisphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2790, https://doi.org/10.5194/egusphere-egu25-2790, 2025.

EGU25-2889 | ECS | Orals | CL3.2.4

Storyline climate attribution for compound flooding from tropical cyclone Idai in Mozambique.  

Doris Vertegaal, Bart van den hurk, Anaïs Couasnon, Natalia Aleksandrova, Tycho Bovenschen, Simon Treu, Matthias Mengel, and Sanne Muis

It is widely recognized that climate change is altering the likelihood and intensity of extreme weather events globally, including hydrological extremes such as floods. Compound flooding is driven by fluvial, pluvial and coastal flooding occurring simultaneously, resulting in a potentially larger impact when co-occurring than the sum of the univariate drivers happening separately. Identifying and communicating the effect of climate change on compound flooding remains challenging. A method to quantify the effect of climate change on these events is through climate attribution assessments. 

This research assesses how existing climate attribution methods can be applied to compound events instead of univariate events. An event-based storyline attribution approach for compound flooding from historical tropical cyclones (TCs) in Mozambique is used to examine the effect of climate change on multiple flood drivers propagated to impact. TC Idai hit Mozambique in 2019 and caused over 600 fatalities, affected over 1.8 million people, resulting in $3 billion in damages. Idai is used as a case study, representing a highly destructive compound flood event. 

Compound flooding is modelled using a state-of-the-art hydrodynamic modelling chain that combines the Super-Fast INundation for coastS (SFINCS) model with the hydrodynamic model Delft3D Flexible Mesh and hydrological model wflow, linked to a fast impact assessment tool Delft-FIAT to calculate the flood impact, here the direct economic damages. The drivers of compound flooding from TCs that are known to be affected by climate change, such as precipitation, wind and sea-level rise, are adjusted to create counterfactual scenarios. The compound flooding is modelled for the multiple factual and counterfactual scenarios, adjusting the separate drivers individually and simultaneously.  

This approach enables the attribution of climate change effects on compound flooding from TCs while identifying potential changes in the contributions of individual flood drivers. Next steps include attribution uncertainty partitioning, comparing multiple climate attribution approaches for these events, assessing regional differences with relation to climate change effects on compound flood impact and comparing this methodology for multiple TCs in the same region, which may have different driver contributions.

How to cite: Vertegaal, D., van den hurk, B., Couasnon, A., Aleksandrova, N., Bovenschen, T., Treu, S., Mengel, M., and Muis, S.: Storyline climate attribution for compound flooding from tropical cyclone Idai in Mozambique. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2889, https://doi.org/10.5194/egusphere-egu25-2889, 2025.

EGU25-3474 | ECS | Orals | CL3.2.4

Dynamical evolution of extremely hot summers in Western Europe in response to climate change 

Robin Noyelle, Arnaud Caubel, Yann Meurdesoif, Davide Faranda, and Pascal Yiou

The study of the statistical and dynamical characteristics of extreme and very extreme events in the climate system is impaired by a strong under-sampling issue. Here we use a rare events algorithm to massively increase the number of extremely hot summers simulated in the state-of-the-art IPSL-CM6A-LR climate model under present and future anthropogenic forcings. This allows us to reach precise climatological results on the dynamics leading to centennial hot summers. We demonstrate that the dynamics leading to these hot summers tend to be more local and less large scale-organized with climate change. In the future, high temperatures are still reached via a large anticyclone, but anomalies do not extend as far longitudinally as in the present and arise mainly as a result of an increase in the intensity of surface heat fluxes.

How to cite: Noyelle, R., Caubel, A., Meurdesoif, Y., Faranda, D., and Yiou, P.: Dynamical evolution of extremely hot summers in Western Europe in response to climate change, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3474, https://doi.org/10.5194/egusphere-egu25-3474, 2025.

EGU25-4554 | ECS | Orals | CL3.2.4

Future Changes to Extreme Rainfall over Puerto Rico in an Ensemble of Convection-Permitting Simulations 

Erin Dougherty, Andreas Prein, and Paul O'Gorman

Puerto Rico is a tropical island that frequently receives heavy rainfall from a variety of systems, including tropical cyclones like Hurricane Maria (2017), mesoscale convective systems (MCSs), and isolated convection. Its two distinct rainy seasons are dictated by moisture convergence associated with the North Atlantic Subtropical High, while sea breezes and complex topography influence precipitation on the mesoscale. Previous research has examined how tropical precipitation could change in a future climate, showing a decrease in precipitation by 2100 using global climate models (GCMs). However, relatively little research has been conducted using convection-permitting climate models over the tropical Atlantic to understand how precipitation extremes could change in a warmer climate. Here, we fill this gap by dynamically downscaling a 0.25 degree GCM 10-member ensemble to 3 km using the Model Prediction Across Scales (MPAS) model for extreme precipitation events in a current (2001-2021) and future climate (2041-2061) over Puerto Rico. We show that MPAS is largely able to reproduce extreme precipitation events in the current climate when compared to observations and captures a variety of systems. We explore how future changes in extreme rainfall events in the early rainy season, which are largely driven by MCSs and isolated convection, compare to changes in the late rainy season, which are primarily due to tropical cyclones. 

How to cite: Dougherty, E., Prein, A., and O'Gorman, P.: Future Changes to Extreme Rainfall over Puerto Rico in an Ensemble of Convection-Permitting Simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4554, https://doi.org/10.5194/egusphere-egu25-4554, 2025.

Possibility of the occurrence of extreme weather and climate is often predicted in recent climate impact studies under certain global warming scenarios using climate models. However, it is usually unclear how such weather extremities occur as the resolution of the current generation climate models is not good enough to resolve individual storm system let alone pinning down the physical mechanisms. This ambiguity in physical mechanism impedes the better understanding of the nature of these extreme weather/climate events and can lead to ineffective mitigation and/or adaptation measures. For example, when the term extreme rainfall is mentioned, it is unclear whether it is caused by severe convective storms or by regular storms that have higher liquid water contents (LWC), as both can lead to large amount of rainfall. But the detailed physical mechanisms of these two types of storms are different. Clearly it is desirable to remove such ambiguity and clarify what type of storms would occur in certain climate regime.

 In this study, we utilize the meteorological series derived from the REACHES climate database compiled from Chinese historical documents (Wang et al., 2018; 2024) as well modern weather data to pin down the type of storms and the respective physical mechanisms responsible for the extreme events that preferably occur in cold versus warm climate regime. We use the REACHES reconstructed temperature series in China in 1368-1911 and construct convection index series to show that the severe deep convective storms are the preferable type that causes extreme weather events in cold climate regime and utilize modern observational data to demonstrate that the high LWC (but not necessarily severe) storms are the type most likely to lead to extreme events.

Finally, physics-based storm model simulation results will be used to illustrate the dynamical processes of these two types of storms and explain why they lead to different precipitation patterns.  

How to cite: Wang, P. K.: Extreme weather types and their physical mechanisms in cold versus warm climate regimes: evidence from historical and modern climate data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4671, https://doi.org/10.5194/egusphere-egu25-4671, 2025.

EGU25-5022 | Orals | CL3.2.4

Human and land exposure to future recurrent unprecedented extremes 

Jonathan Spinoni, Marta Mastropietro, Carlos Rodriguez-Pardo, and Massimo Tavoni

In the last decades, highly impacting climate extremes have become increasingly frequent in many different global hotspots. According to climate projections, such events are likely to become even more severe during the 21st century, to the point that under the less conservative scocio-economic scenarios, they could become so recurrent that they possibly constrain the ability to adapt and mitigate, especially in poorly developed countries.


This study investigates the future occurrence of unprecedented heatwaves, droughts, rainfall and snowfall, namely the time of their emergence and when and where they will become the new climate normals, defined here as at least one such event any other year. As input data, we use an ensemble of high-resolution bias-adjusted climate simulations from the ISIMIP3b family and we focus on four SSPs (SSP1 to SSP5, excluding SSP4). Using population, land-use, and GDP projections without climate change, we also analyse their exposure to such unprecedented climate extremes from 2041 to 2100, focusing on continental and macro-regional scales.


We also present preliminary results obtained by using emulated scenarios, with a special focus on the possibility of preventing such unprecedented extremes under low-emission scenarios (SSP1-1.9 and SSP1-2.6) with specific temperature overshoot trajectories. We show that limiting frequent record-breaking heatwaves and droughts could be highly beneficial, especially in regions with lower income and higher vulnerabilities as Africa and Latin America.


The results presented in this study are included in the framework of the EUNICE project, which aims at quantifying the economic and non-economic impacts of future climate extremes, providing robust quantification of uncertainties. 

How to cite: Spinoni, J., Mastropietro, M., Rodriguez-Pardo, C., and Tavoni, M.: Human and land exposure to future recurrent unprecedented extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5022, https://doi.org/10.5194/egusphere-egu25-5022, 2025.

EGU25-5625 | ECS | Orals | CL3.2.4

The importance of internal variability for climate extreme indices 

Leonard Borchert, Benjamin Poschlod, Lukas Brunner, Vidur Mithal, Natalia Castillo, and Jana Sillmann

The occurrence of climate extremes is influenced by climate forcing as well as internal climate variability: internal variability may temporarily obscure or enhance the forced signal in climate extremes. The role of signal versus noise plays an important role, for instance in the analysis of emergence. The climate extreme indices from the Expert Team on Climate Change Detection and Indices (ETCCDI) are routinely used to assess the impacts of forced change on climate extremes, but in such analyses internal variability is often ignored. We present a comprehensive catalogue of the importance of internal variability for the 27 ETCCDI indices to inform climate extreme analysis and guide impact science.

In our assessment, we use a 50-member ensemble of the CMIP6 generation MPI-ESM 1.2 LR Earth System Model for 1961-2014 to highlight combinations of regions and indices that are strongly affected by internal variability. Unlike previous work, we consider all ETCCDI indices in the same model ensemble to provide a clean identification of internal variability. Using the coefficient of variation as initial metric, we find that the total signal is strongly affected by internal variability  

  • over ocean regions for temperature indices based on percentile thresholds (e.g. tx90p), 
  • along quasi-zonal mid-latitude bands for absolute maximum/minimum temperature indices (e.g. txx), and 
  • in characteristic (sub-)tropical “hot-spot” regions such as northern Africa, the eastern central Pacific, and the south-east of all ocean basins for precipitation-based indices (e.g. r95p). 

This grouping illustrates the differing relative importance of internal variability for the extreme signal depending on the index and the region, and sheds light on processes that contribute to the occurrence of climate extremes. Further, the catalogue provides a tangible resource that enables users of ETCCDI indices to better understand the robustness of index information they might derive from single model runs or observations. Based on our catalogue, users, e.g. impact scientists, may select suitable indices specific to their region of interest and application.

How to cite: Borchert, L., Poschlod, B., Brunner, L., Mithal, V., Castillo, N., and Sillmann, J.: The importance of internal variability for climate extreme indices, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5625, https://doi.org/10.5194/egusphere-egu25-5625, 2025.

EGU25-6589 | Orals | CL3.2.4 | Highlight

The perfect storm: loss potential of Eunice-like cyclones in a counterfactual climate 

Nicholas Leach, Shirin Ermis, Aidan Brocklehurst, Dhirendra Kumar, Alexandros Georgiadis, Lukas Braun, and Len Shaffrey
Storm Eunice was a severe windstorm that impacted Central Europe in February 2022, causing over €2.5 Bn in insured loss. It formed on a cold front west of the Azores before undergoing explosive cyclogenesis and tracking across Central Europe, producing recorded wind gusts of up to 55 ms-1. The contribution of climate change to the storm dynamics and severity was examined by Ermis et al., who found that in counterfactual weather forecasts - given an identical initial synoptic setup - climate change had measurably increased the severity of the storm. 
 
Here we move beyond their meteorological attribution and quantify the role of climate change in the losses incurred during Eunice. We combine the same counterfactual weather forecasts with two loss models, including one state-of-the-art catastrophe model, finding that the increases in meteorological severity do translate through to substantial increases in estimated loss. We compare the loss model results with a commonly used “loss index” finding that the index inadequately represents the heavy tail of the loss distribution, demonstrating the importance of using impact models for quantitative assessments of loss in a changing climate.
 
Of particular note is the existence of several “boosted” members within the forecast ensembles whose losses are far greater than what unfolded in reality. This includes one realisation, simulated in a warmer “future” climate, in which the total loss nearly reaches €50 Bn. The plausible existence of such a catastrophic loss is of considerable relevance to a wide variety of stakeholders across adaptation planning, and the financial sector. We suggest that our results demonstrate not only the potential utility of weather forecast models in quantifying impacts attributable to climate change, but also the value of academic - private partnerships in which the two sectors are able to bring different areas of expertise.

How to cite: Leach, N., Ermis, S., Brocklehurst, A., Kumar, D., Georgiadis, A., Braun, L., and Shaffrey, L.: The perfect storm: loss potential of Eunice-like cyclones in a counterfactual climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6589, https://doi.org/10.5194/egusphere-egu25-6589, 2025.

EGU25-6594 | ECS | Posters on site | CL3.2.4

A Counterfactual Emulator for Circulation-Driven Extremes in Southeast Asia 

Xinyue Liu, Xiao Peng, and Xiaogang He

Climate extremes jeopardize human health and the environment. Recent unprecedented extremes suggest a complex interplay between anthropogenic warming and internal variability of the climate system, with large-scale circulations exhibiting considerable uncertainty in response to climate change. Therefore, understanding the influence of large-scale atmospheric and oceanic circulations on extreme events in a changing climate is crucial for climate adaptation and risk assessment. Traditional physical climate models, while powerful, require extensive computational resources to explore the broad spectrum of potential future circulation states and their implications for the infrequent occurrence of extreme events. This study takes Southeast Asia as an example to demonstrate the influence of Madden–Julian Oscillation (MJO) on extreme precipitation and droughts in a changing climate, as MJO strongly modulates local convective systems in Southeast Asia. We develop an AI-empowered emulator framework based on a conditional diffusion model to generate the precipitation field in a counterfactual world, where the enhanced convective phases of MJO are more (less) frequent than the current climate. We then estimate the intensity-frequency curves of extreme precipitation (drought) events and quantify the uncertainty using the generated large ensemble of samples. This counterfactual emulator allows us to isolate the influence of MJO phases and frequencies on extreme event probabilities, making it feasible to simulate a wide array of circulation states and examine their impacts under various climate change scenarios. By overcoming computational barriers, the study offers a clearer understanding of climate extremes in response to changing circulations for policymakers and stakeholders, enabling climate-informed resilience planning and evidence-based governance policy.

How to cite: Liu, X., Peng, X., and He, X.: A Counterfactual Emulator for Circulation-Driven Extremes in Southeast Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6594, https://doi.org/10.5194/egusphere-egu25-6594, 2025.

Between July 19 and 24, 2023, a multi-day outbreak of severe convective storms impacted Europe, affecting several countries. Northern Italy experienced multiple severe storms during this period, with July 24 marking the most intense day, particularly for hailstorms. On this day, three long-lived hailstorms caused significant damage, injured 119 people, and produced the largest hailstone ever observed in Europe—and the second largest globally—with a diameter of 19 cm. Recent studies highlight positive trends in both the frequency and intensity of convective environments favorable to thunderstorm activity in this region, alongside an increase in reports of large hail events.

This case study examines these trends in the context of the July 24, 2023, event, aiming to determine whether significant changes have occurred that may have increased the likelihood or severity of such an event. We employ a storyline approach based on circulation analogs to analyze the atmospheric conditions leading to this hailstorm.

Results show that similar events are fuelled by much larger CAPE today compared to just a few decades ago, likely linked to the strong upward trend in Mediterranean sea surface temperatures, coupled with a modest decrease in bulk wind shear. Additionally, the data suggest a potential intensification of the dynamics underlying similar configurations over the past 70 years, due to steepening of the horizontal geopotential gradient across the region. 

How to cite: Pons, F.: Analogs-based attribution of the July 24th, 2023 extreme hail storms in northeastern Italy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6770, https://doi.org/10.5194/egusphere-egu25-6770, 2025.

Extreme weather events have been increasing as global temperatures rise. Semi-enclosed basins such as the Black Sea and the Mediterranean are particularly susceptible to extreme weather due to their unique topographic features and land-sea distribution. Extreme precipitation events on the north-facing slopes of the mountains in the Black Sea Region occur due to relatively cold air interacting with the warm sea and being orographically lifted over the mountains. On August 10-12 2021, a deadly flash flood occurred on the coast of the Black Sea in Northern Türkiye which resulted in excessive precipitation (200-450 mm) causing loss of lives of 97 people and leaving 228 injured. We investigated extreme weather event which occurred near the Black Sea along with future climate conditions using the Pseudo-Global Warming method. In order to analyze the event, we used a numerical weather prediction model (WRF) in convection-permitting 3 km horizontal resolution with a domain covering the Black Sea and surrounding area. The model simulations are driven by ECMWF Reanalysis 5th Generation (ERA5) data for initial and boundary conditions. To derive climate change signals, we used 25 CMIP6 Earth System Models and eliminating the rest of the models that have no ocean model component over the Black Sea. The signals are computed for three different future periods (2025–2049, 2050–2074, and 2075–2099) relative to the 1990–2014 historical period. Each climate change signal which represents different periods were added to ERA5 6-hourly data as ensemble means. In the first future period (2025-2049), sea surface temperature (SST) in August is projected to increase by 1.7 °C, and by the end of the period (2075-2099), SST is expected to rise by 5 °C over the Black Sea. Additionally, while near-surface air temperatures in August are projected to increase by 1.5 °C to 2.5 °C initially, they are expected to rise by approximately 5.5 °C to 8.5 °C in the final period over the simulation domain. Moreover, near-surface relative humidity over land in August is simulated to decrease by nearly 10% in the last quarter of the century. The findings of this study will contribute to our understanding of how extreme precipitation events develop under future climate conditions and provide insights of the physical and dynamic processes that could drive these events in a warmer world.

How to cite: Şahinoğlu, S. and Önol, B.: Convective Permitting Simulations for Excessive Precipitation Event Under Pseudo-Global Warming in the Black Sea Region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6834, https://doi.org/10.5194/egusphere-egu25-6834, 2025.

EGU25-8204 | Orals | CL3.2.4 | Highlight

Was July 2021 extreme rainfall in western Germany close to the worst possible?  

Vikki Thompson, Rikke Stoffels, Hylke de Vries, and Geert Lenderink

In July 2021 extreme rainfall associated with a cut-off low pressure system led to huge impacts in western Germany, Belgium, and the Netherlands. The event was costly both in terms of loss of life and insurance damages. We use a multi-method approach to examine the event and to assess whether it could have been even worse. Using atmospheric analogues from reanalysis, pseudo global warming simulations, and a boosted ensemble of a dynamically similar event we show that the observed rainfall pattern is highly sensitive to the large-scale dynamics. For example, although good dynamical analogues are found in reanalysis, these do not all show the same hazards – with many showing very little rainfall.  

Our results suggest the magnitude of rainfall experienced was very unusual, perhaps close to the worst possible in the current climate, as small dynamical changes lead to a drastic reduction of the rainfall. 

How to cite: Thompson, V., Stoffels, R., de Vries, H., and Lenderink, G.: Was July 2021 extreme rainfall in western Germany close to the worst possible? , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8204, https://doi.org/10.5194/egusphere-egu25-8204, 2025.

EGU25-8539 | ECS | Posters on site | CL3.2.4

Meteorological Conditions during Compound Wind and Precipitation Extremes in Coastal Southeast Asia 

Diah valentina lestari, Wei jian, and Edmond yatman lo

Compound precipitation and wind (CWP) extreme events can bring a destructive impact to cities located along coastal areas. Total seasonal occurrence of CWP extreme events reaches its highest number of more than sixty events per year in several coastal cities of Southeast Asia (SEA) with a peak occurrence during summer (June-September). This study investigates nine meteorological variables to identify linkages between atmospheric conditions and CWP extreme events using the Coordinated Regional Climate Downscaling Experiment for Southeast Asia (CORDEX-SEA) dataset. These nine variables are chosen due to their importance as trigger factors to convections and wind gusts, e.g. equivalent potential temperature to represent moist enthalpy and atmospheric static stability as affecting wind gusts. Twelve coastal cities across Vietnam (five cities), the Philippines (three cities), Thailand (two cities), Cambodia (one city), and Myanmar (one city) are grouped into four groups with similar climatological patterns of the nine meteorological variables during the historical summer period (1975-2005). All groups imply the importance of their regional underlying zonal and meridional wind anomaly, outgoing longwave radiation (OLR) anomaly, and low-level moisture flux conditions during CWP extreme events days. CWP days for Group 1 (Cebu, Davao, and Metro Manila) are associated with low-level moisture convergence, negative OLR anomaly, and stronger zonal wind anomaly that enhances the precipitation intensity and wind gusts. The presence of a low-pressure system over the northern part of Metro Manila may also influences the CWP extremes for Group 1. Similarly, as a group that is prone to tropical cyclones, Group 2 (Da Nang, Hanoi, and Hai Phong) are also affected by similar dominant factors as Group 1 with an additional factor from the meridional wind anomaly. Located in between the South China Sea and the Indian Ocean, Group 3 (Yangon, Bangkok, and Chon Buri) is dominantly affected by low-level moisture convergence, zonal wind anomaly, and warm-moist transports from the Indian Ocean. Group 4 (Can Tho, Ho Chi Minh City, and Phnom Penh) shows a similar metrological pattern as Group 3 without notable changes in warm-moist transports. The regional means of these nine meteorological variables are further applied to train a Support Vector Machine (SVM) with an additional unbalanced data handling stage prior to the model training process. The best-trained SVM model results in the highest f1 score of 0.78 and 0.76 on the model’s testing set for Group 3 and 4. Further evaluation of the trained SVM model shows that the model’s predictions on a testing dataset fall within the 95% confidence interval. The best model is next used to predict the occurrence of CWP extreme events in the summer of 2006-2023. This model results in a predictive f1 score of 0.61 for Group 3 and 0.54 for Group 4, corresponding to a total of 98% and 97% correctly predicted (true positive), respectively.

How to cite: lestari, D. V., jian, W., and lo, E. Y.: Meteorological Conditions during Compound Wind and Precipitation Extremes in Coastal Southeast Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8539, https://doi.org/10.5194/egusphere-egu25-8539, 2025.

EGU25-8602 | ECS | Orals | CL3.2.4

Climate change caused the catastrophic severity of Cyclone Daniel over Libya in 2023 

Laurenz Roither, Douglas Maraun, and Heimo Truhetz

Cyclone Daniel was the deadliest Mediterranean storm on record and struck Greece and Libya in September 2023. In our study, we aim to disentangle the factors contributing to the severity of the event, with a focus on the influence of anthropogenic climate change. To this end we utilized a process-based, conditional attribution approach and simulated storylines of the event with a convection permitting regional climate model under actual and counterfactual conditions. Specifically, we tested how cyclone Daniel would have unfolded (1) in a 1970s world with 1°C less climate change; (2) without the prevalent Mediterranean sea surface temperature anomaly of +1.3 °C; and (3) with decreased soil moisture in the Balkans assuming no rainfall anomalies had occurred in the months prior to the event. Climate response uncertainties have been approximately accounted for by imposing climate change signals from different GCMs. 

Our simulations show that 1°C of climate change only moderately influenced the cyclone's extreme precipitation during its early phase in Greece. In contrast, during its tropical-like Libyan phase, this level of climate change has amplified the severity of the event by a staggering 30 to 60%. Increased energy availability and convection led to the formation of a rare and destructive Medicane with a warm and rapidly deepening core. Artificially lowering only the sea surface temperatures reduced the meteorological hazards in both phases and underpins the importance of the Mediterranean as an energy and moisture source. Reducing soil moisture over the Balkans alone, although an important source for evapotranspiration during the early phase, did not substantially affect the intensity of the cyclone.

Our results demonstrate that current climate change can already be a game changer for individual extreme events and highlight the power of storylines to analyze the potentially destructive influence of climate change on rare extreme weather events.

How to cite: Roither, L., Maraun, D., and Truhetz, H.: Climate change caused the catastrophic severity of Cyclone Daniel over Libya in 2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8602, https://doi.org/10.5194/egusphere-egu25-8602, 2025.

EGU25-9252 | ECS | Posters on site | CL3.2.4

How can the catastrophic risk potential of unseen climate extremes be understood? 

Tom Wood, Hebe Nicholson, Jenix Justine, and Tom Matthews

The Earth’s climate is heading into unprecedented territory, with the global mean surface temperature reaching record-breaking levels in 2024. Meanwhile, on regional scales, extreme events are becoming both more frequent and more severe, with some events being without precedent in the observational record. These types of ‘unseen’ events could result in very high-impact, potentially catastrophic impacts for society on a variety of temporal and spatial scales. However, due to the inherent uncertainty in the complex climate system, we have a poor understanding of the risk of unprecedented events, including what is physically and statistically plausible, and the role of critical thresholds in both the physical climate and societal responses. We also have limited capacity to imagine and anticipate events with no historical precedent. Given the risk of very high societal impacts, including mortality, morbidity, and other socio-economic vulnerabilities already possible under present climate conditions, and the potential for a substantial increase in the number of people exposed to these threats under climate change, it is critical that we improve our understanding of these unknown-likelihood unseen events.

In late 2024, a workshop was hosted at King’s College London to address the question of how to reduce the catastrophic risk potential from unseen climate extremes. Twenty-seven researchers participated from a range of disciplines to solicit a variety of perspectives on the question. This included, amongst others, contributions from physical climate scientists, researchers in existential threats, and social scientists. Here, we present the outcomes from these interdisciplinary discussions, including perspectives on the framing and definition of the problem, open research questions, and a research agenda to advance toward a more comprehensive understanding of risk and improved societal preparedness to facilitate pragmatic policy decisions. Areas of discussion included developments in large ensemble climate modelling; modelling of connected systems; counterfactual thinking; and risk-based limits to adaptation; as well as wider philosophical questions regarding what constitutes a catastrophic or existential risk and how this should be defined in a climate context.

How to cite: Wood, T., Nicholson, H., Justine, J., and Matthews, T.: How can the catastrophic risk potential of unseen climate extremes be understood?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9252, https://doi.org/10.5194/egusphere-egu25-9252, 2025.

EGU25-9371 | Posters on site | CL3.2.4

Storylines of heatwaves over Po Valley in a warmer World: drivers and impacts  

Antonello A. Squintu, Ronan McAdam, Jorge Pérez-Aracíl, César Peláez Rodríguez, Carmen Álvarez-Castro, and Enrico Scoccimarro

Heatwaves heavily affect European public health, society and economy. A full understanding of the drivers behind the occurrence and intensity of heatwaves (HWs) is one of the priorities of H2020 CLimate INTelligence (CLINT) project. Particular attention is given to the detection and attribution of HW and on the understanding of their future evolution thanks to the Storylines method. For the implementation of this technique, it is important to assess the capability of climate models in thoroughly identifying relationships between the drivers and the occurrence and intensity of HW. The relevant drivers of this extreme event are selected among a set of clustered variables on European and Global domains. This step is performed applying a feature selection algorithm (Probabilistic Coral Reef Optimization with Substrate Layers, PCRO-SL, Pérez-Aracil et al., 2023) to ERA5 summer data between 1981 and 2010, using as a target the Po Valley HW occurrence. The PCRO-SL is then applied to CMIP6 models, considering for each of them the period in which their Global Surface Air Temperature (GSAT) corresponds to the one of ERA5 between 1981 and 2010 (“current-climate”, 14.2°C). If a benchmark driver is selected for a CMIP6 model, its relationship with the target event is well resolved. The models that satisfy this requirement can be considered for an inspection of the non-linear and joint impacts of the drivers on Po Valley HWs in a future-climate scenario with higher GSAT. Thanks to this procedure it is possible to identify relevant pairs of drivers, whose combined influence on the target event is inspected by constructing Storylines. The projected evolutions of HWs over Po Valley corresponding to each scenario are displayed, highlighting the role of teleconnections and unveiling undocumented impacts.

Pérez-Aracil, J., Camacho-Gómez, C., Lorente-Ramos, E., Marina, C. M., Cornejo-Bueno, L. M., & Salcedo-Sanz, S. (2023). New probabilistic, dynamic multi-method ensembles for optimization based on the CRO-SL. Mathematics11(7), 1666.https://doi.org/10.3390/math11071666 

How to cite: Squintu, A. A., McAdam, R., Pérez-Aracíl, J., Peláez Rodríguez, C., Álvarez-Castro, C., and Scoccimarro, E.: Storylines of heatwaves over Po Valley in a warmer World: drivers and impacts , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9371, https://doi.org/10.5194/egusphere-egu25-9371, 2025.

EGU25-10026 | ECS | Posters on site | CL3.2.4

Using seasonal forecast ensembles to estimate of low-probability high-impact events and unprecedented extremes 

Irene Benito Lazaro, Jeroen C. J. H. Aerts, Philip J. Ward, Dirk Eilander, Timo Kelder, and Sanne Muis

Extratropical cyclones (ETCs) can cause severe storm surges, leading to extreme sea levels, coastal flooding and significant economic losses. Accurate estimates of storm surge frequency and intensity are crucial for flood hazard assessments and effective risk mitigation. However, limited observational records pose a challenge for predicting low-probability high-impact events and unprecedented extreme surges, particularly in regions yet to experience such events.

Global synthetic datasets have demonstrated to be crucial in addressing these limitations by providing larger datasets that reduce uncertainties in risk estimates and capture unprecedented events. Despite their potential, a comprehensive large-scale dataset for ETC-induced storm surges is currently lacking.

In this study, we explore the feasibility of pooling ensembles from ECMWF’s SEAS5 seasonal forecasting system and integrating them with the Global Tide and Surge Model (GTSM) to generate realistic synthetic storm surge events. Using the resulting extended storm surge time series, we assess the storm surge risk for Europe, identify unprecedented surge events, and advance our understanding of their underlying large-scale physical drivers.

How to cite: Benito Lazaro, I., Aerts, J. C. J. H., Ward, P. J., Eilander, D., Kelder, T., and Muis, S.: Using seasonal forecast ensembles to estimate of low-probability high-impact events and unprecedented extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10026, https://doi.org/10.5194/egusphere-egu25-10026, 2025.

EGU25-10125 | ECS | Orals | CL3.2.4

Extremely Warm European Summers predicted more accurately by considering Sub-Decadal North Atlantic Ocean Heat Accumulation 

Lara Wallberg, Laura Suarez-Gutierrez, and Wolfgang A. Müller

In the past decades European summers were marked by extreme heat, marking the most severe warm seasons of temperature records. In particular, in 2003, 2018, and 2022, Europe experienced unprecedented extreme temperatures with temperature anomalies exceeding 2.5 standard deviations. The prolonged heat affected human health, agriculture, economy, and our whole ecosystem, highlighting the need for reliable climate predictions. By using the Max-Planck-Institute Earth System Model, we demonstrate that these extreme summers could have been predicted at least three years in advance by taking into account the preceding sub-decadal variations of heat content in the North Atlantic Ocean. By using a subset of ensemble members that can explicitly include the heat accumulation in the North Atlantic, the prediction skill of physical states, i.e. temperature could be improved, but also user-specific quantities in the agricultural sector, such as growing degree days, for both, Europe-wide and smaller scales for certain regions and specific growing degree day thresholds for crop harvests. These findings underscore the value of incorporating sub-decadal oceanic processes into user-relevant climate prediction methodologies. We demonstrate that the agricultural sector particularly benefits from improved predictions for growing degree days which allow for timely adaption and preparation against extreme heat.

How to cite: Wallberg, L., Suarez-Gutierrez, L., and Müller, W. A.: Extremely Warm European Summers predicted more accurately by considering Sub-Decadal North Atlantic Ocean Heat Accumulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10125, https://doi.org/10.5194/egusphere-egu25-10125, 2025.

EGU25-10393 | ECS | Orals | CL3.2.4

Estimating Return Periods for Extreme Climate Model Simulations through Ensemble Boosting 

Luna Bloin-Wibe, Robin Noyelle, Vincent Humphrey, Urs Beyerle, Reto Knutti, and Erich Fischer

With climate change, heavy-impact extremes have become more frequent in different regions of the world. It is therefore crucial to further physical understanding of extremes, but due to their rarity in samples, this remains challenging.

One way to overcome this under-sampling problem is through Ensemble Boosting, which uses perturbed initial conditions of extreme events in an existing reference climate model simulation to efficiently generate physically consistent trajectories of very rare extremes in climate models. However, it has not yet been possible to estimate the return periods of these storylines, since the conditional resampling alters the probabilistic link between the boosted simulations and the underlying original climate simulation they come from.

Here, we introduce a statistical framework to estimate return periods for these simulations, by using probabilities conditional on the shared antecedent conditions between the reference and perturbed simulations. This theoretical framework is evaluated in and applied to simulations of the fully-coupled climate model CESM2. Our results show that return periods estimated from Ensemble Boosting are consistent with those of a 4000-year control simulation, while using approximately 5.8 times less computational resource use.

We thus outline the usage of Ensemble Boosting as a tool for gaining statistical information on rare extremes. This could be valuable as a complement to existing storyline approaches, but also as an additional method of estimating return periods for real-life extreme events.

How to cite: Bloin-Wibe, L., Noyelle, R., Humphrey, V., Beyerle, U., Knutti, R., and Fischer, E.: Estimating Return Periods for Extreme Climate Model Simulations through Ensemble Boosting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10393, https://doi.org/10.5194/egusphere-egu25-10393, 2025.

EGU25-10851 | Orals | CL3.2.4

Projected Evolution of Compound Temperature-Precipitation Extremes in the Arctic: Insights from a multi-model High-Resolution regional climate ensemble  

Chiara De Falco, Priscilla A. Mooney, Alok Kumar Samantaray, Ruth Mottram, Jan Landwehrs, Annette Rinke, Willem Jan van de Berg, Christiaan van Dalum, Oskar A. Landgren, Hilde Haakenstad, Bhuwan C. Bhatt, Clara Lambin, and Xavier Fettweis

 

The polar regions are among the most affected by global warming, making them particularly vulnerable to extreme events with significant impacts on the cryosphere, permafrost, and wildfires. Record-breaking temperature and precipitation extremes are becoming increasingly widespread and intense globally.  Extreme heat events are projected to increase in frequency, intensity, and duration throughout the 21st century. Furthermore, a sea-ice-free Arctic is becoming a probable scenario. This raises critical questions with significant implications for hazard assessment and adaptation policies: how will compound temperature-precipitation extremes evolve in the polar regions, and which areas will be most vulnerable? Addressing these questions is challenging due to the coarse resolution of current state-of-the-art (CMIP6) future projections. We use state-of-the-art simulations from the EU project PolarRES. They offer an unprecedentedly high-resolution (11 km) Pan-Arctic ensemble developed within the Polar-CORDEX framework. The simulations downscale two different CMIP6 models that are representative of the spread for CMIP6 projections under the SSP3-7.0 scenario. They provide a continuous 120-year (1985-2100) time series of hourly temperature and precipitation data.  We assess compound temperature-precipitation extreme events in the Arctic by mid and end of the century, with a focus on the intensity and persistence of these extremes. This extensive dataset allows us to confidently (1) pinpoint areas that may become more vulnerable to increased occurrences of extreme events in the future, (2) compare near-term, mid-century and end-century distributions and patterns, and (3) identify emerging trends. A clustering analysis will be used to identify regions of the Arctic with similar precipitation-temperature characteristics. With this approach, we can determine whether regions with distinct climate profiles exhibit different trends and behaviours. 

How to cite: De Falco, C., Mooney, P. A., Kumar Samantaray, A., Mottram, R., Landwehrs, J., Rinke, A., van de Berg, W. J., van Dalum, C., Landgren, O. A., Haakenstad, H., Bhatt, B. C., Lambin, C., and Fettweis, X.: Projected Evolution of Compound Temperature-Precipitation Extremes in the Arctic: Insights from a multi-model High-Resolution regional climate ensemble , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10851, https://doi.org/10.5194/egusphere-egu25-10851, 2025.

EGU25-11051 | ECS | Posters on site | CL3.2.4

Preferred pathways of traveling extreme events in land precipitation and temperature 

Yu Huang, Kaiwen Li, Mingzhao Wang, and Niklas Boers

Extreme precipitation events and hot-weather events are usually examined at separate grids of a longitude-latitude map. A spatiotemporal perspective can provide additional insights, such as the spatial extent of extreme events and their potential traveling across the spatial domain over time. Here, we present the regular long-distance traveling patterns of these extreme events, highlighting the preferred spatial pathways through which the extreme precipitation events and hot-weather events tend to travel. Our in-depth analysis reveals that such long-distance traveling behaviors are influenced by midlatitude Rossby waves, and these preferred pathways can offer valuable information for early warning of downstream extreme events, potentially enhancing preparedness and response strategies.

How to cite: Huang, Y., Li, K., Wang, M., and Boers, N.: Preferred pathways of traveling extreme events in land precipitation and temperature, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11051, https://doi.org/10.5194/egusphere-egu25-11051, 2025.

EGU25-11794 | ECS | Orals | CL3.2.4

The drivers of summer extreme temperature trends in Europe 

Luca Famooss Paolini, Salvatore Pascale, Paolo Ruggieri, Erika Brattich, and Silvana Di Sabatino

The frequency, duration and intensity of summer extreme temperatures over Europe have increased since the mid-20th century due to dynamic changes, thermodynamic factors, and their interaction via land—atmosphere feedbacks. However, a comprehensive analysis of all the mechanisms underlying their future trends, including an assessment of uncertainties due to inter-model differences and internal variability, is still lacking.

In this study, we investigate historical and future trends in the occurrence of atmospheric circulation patterns that triggered the three most intense heat waves during 1940—2022, identified using the Heat Wave Magnitude Index daily (Russo et al., 2015): the 2010 Russian, the 1972 Scandinavian and the 2003 French heat wave. To do that, we adopt the atmospheric flow analogue technique. We then decompose the trends of summer extreme temperature occurrences associated with these analogues in their thermodynamic, dynamic and interaction components, following Horton et al. (2015). The analyses are performed using large ensemble of climatic projections from six different models (three CMIP5 and three CMIP6), under the “business-as-usual" emission scenario. This approach allows us to investigate the role of the global warming, internal climate variability and model uncertainties on the European extreme temperature trends.

The results show a future increase in the occurrence of atmospheric circulation patterns similar to the 2003 French heat wave across all models. However, models generally underestimate observed historical trends, suggesting that future trends may be even higher. Furthermore, the results show that the extreme temperature occurrences associated with these analogues have increased in the historical period and will keep increasing in the future. In this context, trend partition analysis indicates that, while the historical trends were primarily driven by thermodynamic component, the future trends will be mainly driven by the interaction term. Interestingly, the interaction and dynamic components will explain a larger percentage of the total trend compared to the past, while the thermodynamic contribution will become less significant. Finally, the results suggest that land—atmosphere coupling processes will play a critical role in explaining the physical meaning of future interaction term and, thus, in driving projected increase in extreme temperature occurrences.

Results for the 2010 Russian and 1972 Finland heat waves generally align with those of the 2003 French heat wave. However, their dynamic trends are subjected to a certain degree of uncertainty due to inter-model differences, limiting the reliability of future dynamic projections and trend partition.

Bibliography

Horton, D. E., et al. (2015). Contribution of changes in atmospheric circulation patterns to extreme temperature trends. Nature, 522 (7557), 465-469.

Russo, S., et al., (2015). Top ten European heatwaves since 1950 and their occurrence in the coming decades. Environmental Research Letters, 10 (12), 124003.

How to cite: Famooss Paolini, L., Pascale, S., Ruggieri, P., Brattich, E., and Di Sabatino, S.: The drivers of summer extreme temperature trends in Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11794, https://doi.org/10.5194/egusphere-egu25-11794, 2025.

EGU25-12412 | Posters on site | CL3.2.4

The CANARI HadGEM3 Large Ensemble: Design and evaluation of historical simulations 

Reinhard Schiemann, Grenville Lister, Rosalyn Hatcher, Dan Hodson, Bryan Lawrence, Len Shaffrey, Ben Harvey, Steve Woolnough, Jon Robson, David Schröder, Adam Blaker, Hua Lu, and Tony Phillips

Large Ensembles, or Single Model Initial Condition Large Ensembles (SMILEs) of climate model simulations, have been produced by different modelling centres in recent years. Here, we present the HadGEM3 Large Ensemble recently completed within the UK NERC multi-centre CANARI project. In the context of existing all-forcings Large Ensembles, noteworthy properties of the CANARI Large Ensemble are (i) a relatively high model resolution (60 km in the atmosphere in the mid latitudes, and about 25 km in the ocean), (ii) the availability of sub-daily output on a range of pressure levels to study weather systems, and (iii) boundary conditions allowing for regional modelling driven by the CANARI Large Ensemble for a range of CORDEX-like domains covering most land regions.

In this poster, we document the ensemble design and evaluate key aspects of historical ensemble performance against observational data, such as the global mean surface temperature evolution, the climatology of the Stratospheric Polar Vortex and of Sudden Stratospheric Warmings, the historical evolution of the Atlantic Meridional Overturning Circulation (AMOC), and trends of midlatitude storm tracks, Arctic Sea Ice area, and tropical Pacific sea surface temperature. Furthermore, an application is presented showing that analogues of the extremely hot North Atlantic sea surface temperature anomalies in the summer of 2023 can be found in the CANARI Large Ensemble, whereas there are no close analogues in the historical record.

(This poster has 40 authors, which exceeds the number of authors allowed in the abstract submission form.)

How to cite: Schiemann, R., Lister, G., Hatcher, R., Hodson, D., Lawrence, B., Shaffrey, L., Harvey, B., Woolnough, S., Robson, J., Schröder, D., Blaker, A., Lu, H., and Phillips, T.: The CANARI HadGEM3 Large Ensemble: Design and evaluation of historical simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12412, https://doi.org/10.5194/egusphere-egu25-12412, 2025.

EGU25-12916 | ECS | Orals | CL3.2.4

Evolution of the probability of record-shattering spatially compounding droughts in a changing climate  

Ji Li, Jakob Zscheischler, and Emanuele Bevacqua

Record-shattering events, defined as extreme events that exceed previous records by large margins, pose increasing risks under climate change. Concurrent soil moisture droughts across multiple crop-growing regions can severely impact the agricultural sector and global food security by exposing a large fraction of the global crop area to water stress. Here, using soil moisture data from Single Model Initial-condition Large Ensembles (SMILEs) over 1950-2099, we investigate the evolution of the probability of spatially compound droughts that shatter previous records in terms of total global crop area affected by droughts within the same year. Our results indicate that trends in mean soil moisture related to climate change are the major driver in the evolution of the record-shattering compound drought probability, while changes in variability (standard deviation of the time series)  are less important. We further attribute changes in the probability of such global-scale record-shattering events to trends in soil moisture in individual large crop-growing regions. By separating the distinct roles of long-term trends in mean conditions, variability of the soil moisture time series, as well as contributions from individual regions to global-scale record-shattering droughts across breadbaskets, this study provides novel insights on compound events threatening the global food security system.

How to cite: Li, J., Zscheischler, J., and Bevacqua, E.: Evolution of the probability of record-shattering spatially compounding droughts in a changing climate , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12916, https://doi.org/10.5194/egusphere-egu25-12916, 2025.

EGU25-13073 | ECS | Orals | CL3.2.4

Dynamics-informed attribution of a record-shattering heavy precipitation event over Central Europe during Storm Boris (2024) 

Jacopo Riboldi, Ellina Agayar, Hanin Binder, Marc Federer, Robin Noyelle, Michael Sprenger, and Iris Thurnherr

Statistics-based extreme event attribution is often limited by the scarce availability of data and by the potentially inadequate representation of relevant physical processes in climate models. Storyline approaches, such as the ones involving large-scale flow analogs, can be used to constrain the impact of anthropogenic climate change on extreme events in a physically robust manner, complementing the information gained from statistics-based approaches.

In this work, we employ operational ECMWF analysis data and simulations from the CESM large ensemble (providing up to 1000 years of data) to characterize the dynamical evolution of Storm Boris, that brought a record-shattering precipitation event over central Europe between the 13th and the 16th of September 2024. Leveraging on the available large ensemble, we perform an analog-based attribution of the associated extreme precipitation informed by the peculiar atmospheric dynamics of the event.

The analysis is articulated in two parts. The first concerns a description of the salient dynamical features that made Storm Boris so extreme. Such features are: 1) a deep upper-level cut-off cyclone over the Mediterranean; 2) a slow-moving surface cyclone over eastern Europe; 3) a strong high-latitude blocking anticyclone building up during the event; and 4) moisture contributions from several sources across storm lifetime, rotating from the North Atlantic to the central and the eastern Mediterranean/Black Sea.

The second part is an analog-based attribution of the extreme precipitation that takes into account the pinpointed dynamical features. We show that a correct representation of the upper-level cut-off cyclone (using potential vorticity as a target field to determine analogs) and of the surface cyclone position at the time of the extreme precipitation (using a cyclone detection algorithm) drastically improves the quality of the detected large-scale flow analogs. Those two adjustments, informed by the knowledge of the dynamics of the event, allow to isolate the thermodynamical effect of climate change in a consistent manner and indicate a robust enhancement of extreme precipitation over central Europe for Boris-like storms occurring in a warmer climate.

How to cite: Riboldi, J., Agayar, E., Binder, H., Federer, M., Noyelle, R., Sprenger, M., and Thurnherr, I.: Dynamics-informed attribution of a record-shattering heavy precipitation event over Central Europe during Storm Boris (2024), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13073, https://doi.org/10.5194/egusphere-egu25-13073, 2025.

An increase in the intensity of daily precipitation extremes is among the most robust responses to anthropogenic climate change. However, while many studies have focused on moderate extremes corresponding to the mean of annual maxima, or their median which corresponds to a return period of 2 years, high-impact extreme precipitation events are related to less studied events with much longer return periods (e.g. 100 years, or longer). The physical and statistical study of these events is hampered by the difficulty in building robust statistics in climate records only a few-decades long. In particular, it is still poorly understood whether moderate and high-impact precipitation extremes may intensify at the same rate, or whether differences may arise due to, for instance, changes in the frequency or meteorology of the driving weather events, in their seasonality, or in the balance between convective and stratiform precipitation.

We address this question by exploring the projected changes in tail heaviness of daily  precipitation extremes in 63 single-member simulations from the EURO-CORDEX ensemble, run at 12km resolution, in the RCP8.5 scenario. Tail heaviness (TH) is here defined as the ratio between the quantiles corresponding to the 100-year return period relative to the 2-year return period. Due to the difficulty in evaluating long return periods from single-member simulations, we first use the 50-member initial condition CRCM5 regional large ensemble, for which statistics can be accurately estimated, to test the ability of extreme value theory (GEV distribution) and Simplified Metastatistical Extreme Value theory (SMEV) in estimating changes in TH.

The results show that SMEV has a smaller root mean squared error than GEV in estimating changes in TH from 30-year long climate records extracted from the CRCM5 ensemble, proving it a better methodology for this purpose. When SMEV is applied to the CORDEX ensemble, a likely (66% to 90% of models) increase in TH is found in the Mediterranean region, while small and non robust changes are found in Central and Northern Europe. The robustness of the Mediterranean response is not detectable using GEV. The increase in TH is shown to constitute a sizable contribution to the increase in the 100-year level of Mediterranean precipitation extremes. A reduction in the number of precipitation events partly balances the increase in the 2-year return period, but has little impact on the 100-year return period, contributing to its faster relative intensification. 

We conclude that while in Central and Northern Europe the rate of change in moderate (2-year) and high-impact extremes cannot be distinguished from estimation uncertainties, great care is needed in the Mediterranean region, where the risk of exposure to high-impact precipitation events due to climate change may be increasing faster than what perceived based on the trends of moderate extremes

How to cite: Zappa, G., Marra, F., and Pascale, S.: High-impact Mediterranean precipitation extremes to increase faster than moderate extremes in the CORDEX future projections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13285, https://doi.org/10.5194/egusphere-egu25-13285, 2025.

EGU25-14675 | Posters on site | CL3.2.4

High-impact climate extremes in India 

Vimal Mishra, Dipesh Singh Chuphal, Urmin Vegad, Iqura Malik, Hiren Solanki, and Rajesh Singh
India's large population, high socio-economic vulnerability, intensive agriculture, and rapidly growing infrastructure make it particularly susceptible to extreme climate and weather events. Despite their significant economic implications and the costs of adaptation, high-impact climate extremes over the last 45 years (1980-2024) have not been comprehensively documented. In this study, we identify high-impact heatwaves, extreme precipitation events, floods, droughts, and combined hot and dry extremes that occurred during this period, using observations and model simulations. We also utilize climate model projections from the Coupled Model Intercomparison Project Phase 6 (CMIP6) and the CESM2 Large Ensemble Community Project (LENS2) to explore the analogues of these observed high-impact climate extremes. Furthermore, we investigate the occurrence and driving factors of these extremes in India under various levels of global warming. Our findings indicate that there will be a substantial increase in high-impact climate extremes in India if global mean temperatures exceed 2°C.
 

How to cite: Mishra, V., Chuphal, D. S., Vegad, U., Malik, I., Solanki, H., and Singh, R.: High-impact climate extremes in India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14675, https://doi.org/10.5194/egusphere-egu25-14675, 2025.

EGU25-14842 | Orals | CL3.2.4

Assessing record-breaking North Atlantic warming extremes in summer 2023 using reanalysis and Grand Ensemble simulations 

Katja Lohmann, Hayat Nasirova, Quan Liu, Johann Jungclaus, Daniela Matei, and Ben Marzeion

The marine heatwave in the North Atlantic in summer 2023 set new temperature records and raised concerns about the impact of climate change on oceanic extreme events. This study examines this record-breaking marine heatwave with a focus on the subpolar North Atlantic by analysing ECMWF ERA5 reanalysis data and the Max Planck Institute Grand Ensemble CMIP6 version (MPI-GE CMIP6).

We demonstrate that due to a superposition of the global warming background state and natural variability, individual members of MPI-GE CMIP6 reproduce a North Atlantic summer heat wave within recent decades, which matches the strength of the observed 2023 heatwave. We assess possible atmospheric and oceanic drivers, including those not discussed in the literature so far, such as the atmospheric circulation state and associated surface heat flux in the preceding winter or the oceanic heat transport convergence across the subpolar North Atlantic. Our results indicate that for the subpolar North Atlantic processes related to oceanic and atmospheric variability have significantly contributed to the record observed and simulated heatwaves. Based on the historical and future scenarios of MPI-GE CMIP6, we suggest that both frequency and intensity of marine heatwaves in the North Atlantic will increase significantly, which may have various impacts on marine ecosystems and regional climate.

How to cite: Lohmann, K., Nasirova, H., Liu, Q., Jungclaus, J., Matei, D., and Marzeion, B.: Assessing record-breaking North Atlantic warming extremes in summer 2023 using reanalysis and Grand Ensemble simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14842, https://doi.org/10.5194/egusphere-egu25-14842, 2025.

EGU25-14912 | Posters on site | CL3.2.4

Study on the Establishment of Dispatch Mechanism for Mobile Pumps Under Climate Change: A Case Study of Taiwan 

Jian-Li Lin, Hsun-Chuan Chan, and Chia-Chi Tang

Taiwan faces significant challenges due to climate change, as rainfall patterns are increasingly shifting toward short-duration, high-intensity events. Although the government has implemented various flood control projects, the protective capacity of existing infrastructure remains limited. Extreme rainfall can still lead to severe flooding, as evidenced by the 2018 flood in southern Taiwan. In addition to structural measures, non-structural approaches—such as the mobile deployment of mobile pumps, community-based disaster prevention initiatives, and water monitoring systems—are essential for mitigating risks and reducing losses.

Currently, the deployment of mobile pumps heavily relies on personnel experience and ad hoc government requests, underscoring the need for systematic and scientific dispatch mechanisms. This study integrates data from rainfall forecasts, QPESUMS, flood sensors, and pump distribution to develop a comprehensive dispatch mechanism for proactive deployment and disaster response. The proposed strategy aims to enhance the efficiency of flood prevention and mitigation efforts in vulnerable areas during extreme weather events.

Keywords: Mobile Pumps; Dispatch Mechanism; Climate Change

How to cite: Lin, J.-L., Chan, H.-C., and Tang, C.-C.: Study on the Establishment of Dispatch Mechanism for Mobile Pumps Under Climate Change: A Case Study of Taiwan, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14912, https://doi.org/10.5194/egusphere-egu25-14912, 2025.

EGU25-15386 | ECS | Orals | CL3.2.4

Increased central and northern European summer heatwave intensity due to the forced changes in internal climate variability 

Goratz Beobide-Arsuaga, Laura Suarez-Gutierrez, Armineh Barkhordarian, Dirk Olonscheck, and Johanna Baher

In the past two decades, the intensity of European summer heatwaves has strongly increased due to anthropogenic emissions and associated rising global mean temperatures. On the one hand, the anthropogenic forcing is causing an increase in European summer temperatures, shifting European summer temperature distributions towards warmer values and intensifying European summer heatwaves. On the other hand, the anthropogenic forcing is expected to affect the internal climate variability under global warming, changing the variability of European summer temperatures. While the effects of the forced changes in internal variability have been long debated for mean or maximum summer temperatures, the effects of the forced changes in internal variability on European summer heatwave intensity under increasing global warming levels remain unknown. Using four state-of-the-art global climate model large ensembles, we find that the forced changes in internal variability will intensify central and northern European summer heatwaves. In central and northern Europe, soil moisture is projected to decrease, leading to frequent moisture limitations, enhancing land-atmospheric feedback, and increasing heatwave intensity and variability. On the contrary, the forced changes in internal variability will weaken southern European summer heatwaves. Southern Europe is projected to face significant soil moisture depletion, leading to more stable moisture-depleted conditions that reduce extreme temperature variability and heatwave intensity. Our findings imply that while adaptation to increasing mean temperatures in southern Europe should suffice to reduce the vulnerability to increasing European summer heatwave intensity, adaptation to increased temperature variability will also be needed in central and northern Europe.

How to cite: Beobide-Arsuaga, G., Suarez-Gutierrez, L., Barkhordarian, A., Olonscheck, D., and Baher, J.: Increased central and northern European summer heatwave intensity due to the forced changes in internal climate variability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15386, https://doi.org/10.5194/egusphere-egu25-15386, 2025.

EGU25-15441 | ECS | Posters on site | CL3.2.4

On the role of sea surface temperature variability in southern Arabian Peninsula extreme rainfall on 16th April 2024 

Subrota Halder, Basit Khan, Olivier Pauluis, Zouhair Lachkar, and Francesco Paparella

The United Arab Emirates (UAE) experienced unprecedented rainfall on 16th April 2024, with Al-Ain recording 254 mm and Dubai 142 mm in a single day, driven by a Mesoscale Convective System (MCS). This extreme event resulted from the interaction of cold air from higher latitudes pushed eastward by the subtropical jetstream with warm, moist air from the Arabian Sea. The unusually high sea surface temperature (SST) in the Arabian Sea, reaching 30.5°C (1°C above the 40-year average), was influenced by El Niño and one of the strongest positive Indian Ocean Dipole episodes on record, which enhanced evaporation and atmospheric moisture content. 

 

To investigate the role of anomalous SSTs, we conducted two numerical experiments using the Weather Research and Forecasting (WRF) model: one with the actual 2024 SST conditions from ERA5 and another with 1981-2020 SST climatology. Time series and probability density function analyses revealed that extreme rainfall was more widespread in the 2024-SST simulation compared to the climatology, with higher precipitable water content (40–60 mm) observed in the former, a range rarely seen in the latter. Further analysis of moisture transport and equivalent potential temperature confirmed that the warm SST-induced moisture played a pivotal role in driving the enhanced transport and heavy precipitation. 

 

These findings underscore the critical role of anomalously high SSTs in intensifying extreme rainfall events, highlighting the need for improved predictive models and resilient infrastructure to mitigate the growing risks posed by climate change in the region.

How to cite: Halder, S., Khan, B., Pauluis, O., Lachkar, Z., and Paparella, F.: On the role of sea surface temperature variability in southern Arabian Peninsula extreme rainfall on 16th April 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15441, https://doi.org/10.5194/egusphere-egu25-15441, 2025.

EGU25-15644 | Orals | CL3.2.4

  Recent extreme cold waves are likely not to happen again this century 

Aurélien Ribes, Yoann Robin, Octave Tessiot, and Julien Cattiaux

As the climate warms, cold waves are expected to become less intense and less frequent. Is there still a risk of reliving events comparable to the most intense cold spells we can remember? We analyze four remarkable cold spells that have occurred since 2010 in different regions: Western Europe, Texas, China, Brazil. We show that all these recent events have a moderate to high probability of not happening again by 2100 – typically 50% to 90% in an intermediate emissions scenario, depending on the event. The probabilities are even higher for iconic events of the 20th century or earlier. Our results suggest that the most intense cold snaps, and their associated icy landscapes in mid-latitude regions, are disappearing or have already disappeared due to anthropogenic climate change.

How to cite: Ribes, A., Robin, Y., Tessiot, O., and Cattiaux, J.:   Recent extreme cold waves are likely not to happen again this century, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15644, https://doi.org/10.5194/egusphere-egu25-15644, 2025.

EGU25-15749 | Orals | CL3.2.4

Many reasons to safeguard the polar regions from dangerous geoengineering 

Marie G. P. Cavitte, Martin Siegert, and Heidi Sevestre and the Authors of "Safeguarding the polar regions from dangerous geoengineering"

Continued greenhouse gases emissions are warming our planet, with catastrophic consequences for its habitability and the natural world. Rapid and deep decarbonization to "net zero" carbon dioxide emissions will be needed to halt global warming, and must be achieved by 2050 to stay within the 2015 Paris Agreement thresholds. However, the public debate is increasingly exposed to claims that technological geoengineering "fixes" could reduce projected climate impacts, including in polar regions where current and projected changes have severe and irreversible consequences locally and globally. 

As a community of polar and cryosphere scientists, we have evaluated five highly publicized geoengineering proposals that are either focused on the polar regions or would have major impacts on these systems: stratospheric aerosol injection, sea curtains/sea walls to prevent warm waters reaching glaciers and ice shelves, sea ice management through modifying albedo and thickening sea ice, slowing ice sheet flow through basal water removal and ocean fertilization. Based on our rigorous analysis of technological availability, logistical feasibility, cost, predictable adverse consequences, environmental damage, scalability (in time and space), governance, and ethics, we conclude that none of these geoengineering ideas pass an objective and comprehensive test regarding its use in the coming decades. Instead, many of the proposed ideas are environmentally dangerous. Furthermore, funds spent in researching these ideas further is divesting from much needed research on mitigation and adaptation to climate change and bestow unwarranted public credibility to these geoengineering schemes. We stress that given their feasibility challenges and risks of negative consequences, these ideas should not distract from the foremost priority to reduce greenhouse gas emissions and achieve successful adaptation.

How to cite: Cavitte, M. G. P., Siegert, M., and Sevestre, H. and the Authors of "Safeguarding the polar regions from dangerous geoengineering": Many reasons to safeguard the polar regions from dangerous geoengineering, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15749, https://doi.org/10.5194/egusphere-egu25-15749, 2025.

EGU25-15809 | ECS | Orals | CL3.2.4

From Greenland to the Mediterranean Sea: Unveiling a new cascade mechanism under anthropogenic warming? 

Juan Jesús González-Alemán, Marilena Oltmanns, Sergi González-Herrero, Markus Donat, Francisco Doblas-Reyes, Frederic Vitard, Jacopo Riboldi, Carmen Álvarez-Castro, David Barriopedro, and Bernat Jiménez-Esteve

On 17 August 2022, the western Mediterranean experienced an unusual thermodynamic environment with extremely high unstable atmospheric conditions, combined with strong wind shear. These conditions, occurring ahead of an eastward-moving weather disturbance called a shortwave trough, led to the formation of a bow-shaped system of thunderstorms. This system produced a long path of severe winds, stretching from the Balearic Islands to southern Czech Republic on 18 August. The strongest wind gust reached 62.2 m s⁻¹ at Corsica, where numerous records were beaten. Unfortunately, 12 people lost their lives, and 106 were injured during this event. Such a system was classified as a derecho, a type of long-lasting and severe windstorm generated by a line of thunderstorms.

A record-breaking marine heatwave (MHW) was present in the western Mediterranean simultaneously during the summer of 2022, peaking in July. The sea surface temperature (SST) was more than 3 °C above normal levels in the region where the storm developed. The extremeness of the summer 2022 MHW is evidenced by the high SST anomalies in the first half of August 2022, ranking first among all years since 1940. An attribution exercise with numerical experiments and novel results (González-Alemán et al., 2023) indicated that this derecho event was substantially amplified by the extreme MHW and suggested that current anthropogenic climate change forcing contributed to triggering the severe storm by creating an environment more favourable for convective amplification. The study demonstrated that in case a similar dynamical synoptic situation had happened in a preindustrial climate, the derecho would have not developed, highlighting the role of thermodynamic contributions from global warming. However, no answers can be obtained regarding its dynamical contribution.

Thus, to further investigate this event and the dynamical role of global warming in it, we explore the atmospheric mechanisms that potentially can lead to such a record-breaking event, from the atmospheric dynamics and circulation point of view, and try to answer why climate change has played a crucial role from this perspective.

How to cite: González-Alemán, J. J., Oltmanns, M., González-Herrero, S., Donat, M., Doblas-Reyes, F., Vitard, F., Riboldi, J., Álvarez-Castro, C., Barriopedro, D., and Jiménez-Esteve, B.: From Greenland to the Mediterranean Sea: Unveiling a new cascade mechanism under anthropogenic warming?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15809, https://doi.org/10.5194/egusphere-egu25-15809, 2025.

EGU25-15941 | ECS | Orals | CL3.2.4

Anthropogenic Climate Change Attribution to a Record-breaking Precipitation Event in October 2024 in Valencia, Spain  

Carlos Calvo-Sancho, Javier Díaz-Fernández, Juan Jesús González-Alemán, César Azorín-Molina, Amar Halifa-Marín, Ana Montoro-Mendoza, Pedro Bolgiani, Santiago Beguería, Sergio M. Vicente-Serrano, Ana Morata, and María Luisa Martín

Cut-off lows are, and will be in the future, one of the main threats related to severe weather in the Iberian Peninsula, especially in the Mediterranean arc. Cut-off lows are often accompanied by heavy precipitations in a short time promoting flash-floods, as well as hail, strong convectively wind gusts and/or tornadoes.   

On the week of October 27th – November 4th, 2024, a cut-off low affected the Iberian Peninsula with extreme socio-economical impacts in several Spanish regions and, especially, in the Valencia area. The phenomena on the surface have varied depending on the region: large hail (5-7 cm), several tornadoes, strong wind gusts and, above all, extreme precipitations. The most severe day was October 29th in the Valencia region, with rainfall accumulations higher than 300 mm in a notable area and locally registering 771 mm in 24 hours. In addition, the Turís official weather station registers numerous rainfall intensity national records. Moreover, the convective system promotes 11 tornadoes (two of them with intensity IF2) and large hail (~ 5 cm). The social impact of the floods in Valencia was very high, with more than 16.5 billion euros of damage to infrastructure (roads, railways, etc.), housing and croplands, as well as 231 fatalities and three missing.

In this survey, we focus on Valencia’s floods on October 29th. Here, by performing model simulations with the WRF-ARW model and using a storyline approach, we find an enhancement in intensity and a significant increase in extreme accumulated rainfall area (e.g., 100 mm, 180 mm, 200 mm, and 300 mm) caused by current anthropogenic climate change conditions compared to preindustrial ones.

How to cite: Calvo-Sancho, C., Díaz-Fernández, J., González-Alemán, J. J., Azorín-Molina, C., Halifa-Marín, A., Montoro-Mendoza, A., Bolgiani, P., Beguería, S., Vicente-Serrano, S. M., Morata, A., and Martín, M. L.: Anthropogenic Climate Change Attribution to a Record-breaking Precipitation Event in October 2024 in Valencia, Spain , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15941, https://doi.org/10.5194/egusphere-egu25-15941, 2025.

EGU25-16597 | Orals | CL3.2.4 | CL Division Outstanding ECS Award Lecture

Physical drivers and statistical properties of high impact climate extremes  

Kai Kornhuber

Accurately modeling emerging physical climate risks to natural and societal systems—such as global supply chains, the food system, health, and critical infrastructures—is essential for effective preparedness and honest discussions about the consequences of rising greenhouse gas emissions.

A series of anomalous weather events that shattered previous records by wide margins has —yet again—highlighted the need for an improved understanding of the physical processes behind weather and climate extremes, their statistical characteristics, and our ability to project them under future emission scenarios using climate models.

In this Award lecture, I will present an overview of recent studies and preliminary findings that explore the mechanisms and physical drivers of high-impact climate extremes, as well as their statistical characteristics, such as simultaneous or sequential occurrences, which can lead to high societal impacts under current and future climate conditions and will reflect on our capacity to reproduce such events in climate models.

How to cite: Kornhuber, K.: Physical drivers and statistical properties of high impact climate extremes , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16597, https://doi.org/10.5194/egusphere-egu25-16597, 2025.

EGU25-16878 | Posters on site | CL3.2.4

The impact of carbon neutrality timing on climate extremes in East Asia 

Su-Jeong Kang, Hyun Min Sung, Jisun Kim, Jae-Hee Lee, Sungbo Shim, Hyomee Lee, Pil-Hun Chang, and Young-Hwa Byun

Carbon neutrality is an essential approach for the mitigation of climate change and plays a key role in the implementation of the Paris Agreement. This study analyzes future climate change in East Asia using carbon neutrality scenarios(Shared Socioeconomic Pathways SSP1-1.9, SSP1-2.6, SSP4-3.4, and SSP5-3.4-OS) and evaluates how earlier carbon neutrality could mitigate the impact of extreme climate events. Using carbon neutrality scenarios and indices of temperature and precipitation based on ETCCDI(Expert Team an Climate Detection and Indices), we analyzes frequency and intensity of climate extremes.  Furthermore, we defined the Fraction of Avoidable Impact(FAI) to evaluate the extent of impact that can be avoided when achieving carbon neutrality, similar to the SSP1-1.9 scenario. For the extreme temperature, FAI values of intensity(frequency) were projected to be approximately 33-42%(33-35%) in the SSP1-2.6 scenario and 49-54%(49-53%) in the SSP4-3.4 scenario, indicating a relatively larger increase in intensity.  In the case of extreme precipitation, FAI values of intensity(frequency) were projected to be about 25%(26-31%) in the SSP1-2.6 scenario and 40%(38-47%) in the SSP4-3.4 scenario, showing a similar trend of relatively larger increase in intensity as observed for extreme temperature. These findings emphasize that if the timing of achieving carbon neutrality is advanced to align with the Paris Agreement, the impact of climate extremes will be significantly reduced. 

This research was funded by the Korea Meteorological Administration Research and Development Program “Development and Assessment of Climate Change Scenario” under Grant (KMA2018-00321). 

How to cite: Kang, S.-J., Sung, H. M., Kim, J., Lee, J.-H., Shim, S., Lee, H., Chang, P.-H., and Byun, Y.-H.: The impact of carbon neutrality timing on climate extremes in East Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16878, https://doi.org/10.5194/egusphere-egu25-16878, 2025.

Following the extreme European summer heatwave of 2003, it has been suggested that the event might have been associated with changes in the distribution of summer temperatures. Here we revisit this hypothesis and investigate observed European and Swiss summer temperatures for the period 1864-2024.

The pronounced increase in skewness has a number of important implications: (1) It implies that extreme hot summers have become more frequent than expected from the median warming. In particular, the increase in skewness strongly affects estimates of the probability of extreme summer heatwaves such as 2003 and 2018. (2) It is demonstrated that the increase in skewness can partly be explained by the accelerating warming around 1980. It is thus not clear whether the high values in skewness will persist into the future. (3) There is a statistically significant difference in the trends of median and mean warming, with mean temperatures warming stronger than the median. (4) These different warming rates explain a non-negligible fraction of the so-called mismatch (i.e., summer temperatures in observations have warmed stronger than in CMIP and CORDEX scenarios). (5) It is demonstrated that understanding this mismatch requires an assessment of extreme summer temperatures, beyond the more commonly used mean summer temperature trends.

We will also provide estimates of the frequency of 2003-like summer heatwaves for the current and future climate, making different assuptions about the persistence of the aformentioned changes in skewness.

How to cite: Schär, C. and Chiriatti, F.: Revisiting recent changes in European summer temperature distributions and assessing their role for extreme summer temperatures, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17421, https://doi.org/10.5194/egusphere-egu25-17421, 2025.

EGU25-17450 | Orals | CL3.2.4

Future Heat Stress Projections in Northwestern Türkiye: Urbanization and Population Impacts in Istanbul 

Gökberk Ozan Tiryaki, Cemre Yürük Sonuç, Ayşegül Ceren Moral, and Yurdanur Ünal

The frequency and intensity of heat stress are expected to escalate markedly in the near future under various global climate change scenarios, with densely populated cities becoming hotspots because of the urban heat island effect. Therefore, heat stress analysis for highly populated cities is crucial since changes in this stress exacerbate vulnerability, increase health-related risks and impose constraints on outdoor activity. This study investigates changes in heat stress during 21st century in terms of frequency, intensity and durations while quantifying population exposure to heat stress covering Northwestern Türkiye, with particular attention to Istanbul, the most populous city in Türkiye with nearly sixteen million population.

In this study, we use climate simulations from convection-permitting model COSMO-CLM under SSP3-7.0 emission scenario to investigate future changes in heat stress. The analysis focuses on calculating Wet Bulb Temperature (WBT) values and assessing consecutive hours when Wet Bulb Temperature (WBT) is above specific thresholds, which are critical indicators of heat stress severity. In addition, we conduct comprehensive heat stress evaluation by computing Environmental Stress Index (ESI) values, an effective alternative to WBGT, to assess outdoor activity limitations. These analyses are performed for the reference period of 1985-2015 and extended to future periods of 2030-2039, 2050-2059, 2070-2079 and 2090-2099, providing a detailed temporal perspective on the progression of heat stress and its implications under changing climatic conditions.

WBT uses air temperature and relative humidity as its primary parameters while ESI incorporates radiation alongside air temperature and relative humidity. Thus, this study also comprehensively analyzes the role of radiation in amplifying heat stress. Our results reveal a remarkable seasonal shift in heat stress pattern within the study area with Istanbul standing out as a hotspot where heat stress indices are notably higher than those of other cities in the covered region, highlighting the effect of urbanization in heat stress dynamics.

Notably, ESI values in the southern parts of Istanbul, where urbanization is more concentrated, exceed critical thresholds that makes any physical activity to be hazardous especially by the end of this century. Moreover, projections demonstrate that in the late 21st century, majority of Istanbul’s population will be exposed to heat stress levels exceeding the risky thresholds. Furthermore, this study explores the extent of population exposure to heat stress, the duration of consecutive hours exceeding critical thresholds, and the percentage of areas where indices exceed their limits.

Key words: Climate modelling, heat stress, heat extremes, population exposure, COSMO-CLM

How to cite: Tiryaki, G. O., Sonuç, C. Y., Moral, A. C., and Ünal, Y.: Future Heat Stress Projections in Northwestern Türkiye: Urbanization and Population Impacts in Istanbul, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17450, https://doi.org/10.5194/egusphere-egu25-17450, 2025.

EGU25-17451 | ECS | Posters on site | CL3.2.4

Disentangling drivers of compound heat and drought in Europe 

Victoria Dietz, Laura Suarez-Gutierrez, Leonard Borchert, and Wolfgang Müller

Future projections suggest that compound heat and drought in Europe will occur more frequently under increasing global warming. Year-to-year variability driven by atmospheric circulation patterns and decadal phenomena like the Atlantic Multidecadal Variability (AMV) temporarily dampens or amplifies these changes. As such, the frequency and intensity of these events can be affected by anthropogenic and natural drivers.
Disentangling these contributions is essential for understanding current events and the reliability of future projections, as well as for improving long-term predictions of such events and refining risk assessments. Although recent attribution studies have started to address the impact of natural climate variability, these studies are often limited to heat waves and do not explore other high-impact phenomena. Further, they are often based on observational data exclusively and therefore lack the sampling of internal variability that is required for a robust assessment. To address these gaps, we present a comprehensive analysis that quantifies the dynamical and thermodynamical contributions of not only global warming, but also considers internal climate variability using conditional attribution with atmospheric flow analogues. We use the CMIP6 version of the MPI Grand Ensemble (MPI-GE6) single-forcing (30 member) and historical (50 member) experiments to identify analogues based on real events from ERA5. This approach enables a clear separation and quantification of dynamical and thermodynamic contributions and how these change under different global warming states and under different forcing configurations, helping to better distinguish how both anthropogenic and natural factors influence high-impact heat and drought events in Europe.

How to cite: Dietz, V., Suarez-Gutierrez, L., Borchert, L., and Müller, W.: Disentangling drivers of compound heat and drought in Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17451, https://doi.org/10.5194/egusphere-egu25-17451, 2025.

The severity of the impacts of (convective) rainfall extremes in the past year alone, e.g., storm Boris and the flooding in middle Europe, or the flooding in the Valencia region, is mind blowing. With several hundreds of millimeters of rain falling in often fewer than 48 hours, the flooding was locally very disruptive, or even catastrophic. While often embedded in large-scale and reasonably well predictable (but anomalous) flow conditions, the level of small-scale detail and the role of smaller-scale (convective) processes that ultimately determine whether the situation "gets out of hand" - or not - is challenging both observation networks, and the NWP and climate-modelling centers. 

In this presentation we take the example of storm Boris that caused widespread flooding in Middle Europe in September 2024 to illustrate that only by simulating the event at very high resolution the true changes in the impacts are revealed. Using a pseudo-global warming (PGW) framework in which the event is placed in historic and possible future climate conditions, we show that on a local scale the response strongly exceeds the regional response. By subsequently matching the patterns to underlying population densities an impression is obtained of how this leads to a greatly elevated impact on society.

Different frameworks have been developed to analyse, attribute and project extreme events often immediately after, or even prior to the event. The regional PGW framework we are adopting here is but one of the several existing approaches based on analysing 'counterfactuals', i.e., simulating the event in a different climate. Another framework is that of dynamic analogues which relies on deriving paste-to-present or present-to-future changes, by selecting and comparing similar (observed or modelled) events based on large-scale flow similarity. In this approach therefore, the event is also captured. Structural similarity in terms of flow conditions is not required by the approach of world-weather attribution (WWA). The WWA-approach examines changing frequency and intensity of local or regional extremes using non-stationary extreme-value analysis of observational and model data, and blends these two lines of information. All methods have their advantages and disadvantages. At best, these methods give overlapping results, but in practice they highlight different aspects of the (past or future) changes. This forces one to think how to combine or merge the output from the different methodologies to provide society with the most relevant information and to better anticipate on the future changes. 

How to cite: de Vries, H. and Lenderink, G.: Local versus regional impact changes for storms like Boris (2024): insights from high-resolution pseudo global warming simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19142, https://doi.org/10.5194/egusphere-egu25-19142, 2025.

EGU25-19550 | Orals | CL3.2.4

Interlinks between marine heatwaves, multi-hazard extratropical cyclones, meteotsunamis and phytoplankton blooms over Northwest Europe: insight from a km-scale regional coupled model 

Segolene Berthou, Nefeli Makrygianni, Sana Mahmood, Dale Partridge, Juan Castillo, Alex Arnold, and Piyali Goswami

Climate change is bringing more marine heatwaves and more rainy extratropical cyclones, both trends already detectable. In parallel, storms are usually responsible for the ending of surface-based marine heatwaves. We employ a newly-developed regional coupled system at km-scale over Northwest Europe to show the relationships between marine heatwaves, storms and phytoplankton activity. We show that a marine heatwave amplified the rainfall, river flows, waves and surge of the most impactful storm of 2023 over the United Kingdom (storm Babet). We also show that storms terminating marine heatwaves can either increase or decrease phytoplankton activity, depending on seasonality. Finally, we show the high resolution, high frequency coupling system is also able to represent meteotsunamis (sub-tidal sea surface disturbances linked with slow-moving pressure disturbances), and opens a whole new area of research on compound convective systems and meteotsunami research. In addition to case-studies, we will present plans to use this coupled system across weather and climate time-scales, to increase our understanding and resilience to extreme compound events.

How to cite: Berthou, S., Makrygianni, N., Mahmood, S., Partridge, D., Castillo, J., Arnold, A., and Goswami, P.: Interlinks between marine heatwaves, multi-hazard extratropical cyclones, meteotsunamis and phytoplankton blooms over Northwest Europe: insight from a km-scale regional coupled model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19550, https://doi.org/10.5194/egusphere-egu25-19550, 2025.

EGU25-19798 | Orals | CL3.2.4

Moisture origin for the heavy precipitation event in Central and Eastern Europe in September 2024 

Marina Duetsch, Sarah Furian, Lucie Bakels, and Andreas Stohl

In September 2024, cyclone Boris brought intense precipitation to Central and Eastern Europe, causing severe flooding in Austria, Czech Republic, Poland, and neighboring countries. Understanding the processes that led to this event is important for improving the prediction and mitigation of similar events in the future. Here we trace the origin and transport pathways of the moisture contributing to the precipitation during the event using a Lagrangian moisture source diagnostic. The results show that evapotranspiration from land played a more important role than previously thought: most of the moisture came from the European continent, with additional contributions from the Mediterranean, Black, and Baltic Seas. To place the results in a broader context we compare them with a climatology of moisture sources based on a Lagrangian reanalysis dataset for the years 1940 - 2023. This provides additional insight into atmospheric processes driving heavy precipitation events in this region and highlights anomalous patterns associated with cyclone Boris.

Contributions of different source regions to precipitation in Central and Eastern Europe in September 2024. The figure shows the total precipitation from ECMWF (orange line) compared with the precipitation estimated by the Lagrangian moisture source diagnostic (blue line) and the contributions of different regions (defined in the upper left panel) in colors.

How to cite: Duetsch, M., Furian, S., Bakels, L., and Stohl, A.: Moisture origin for the heavy precipitation event in Central and Eastern Europe in September 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19798, https://doi.org/10.5194/egusphere-egu25-19798, 2025.

EGU25-21505 | Posters on site | CL3.2.4

Assessment of Surface Urban Heat Island over Bengaluru City in India 

Swadesh Mohapatra and Krushna Chandra Gouda

The population approaching 14 million in the Bengaluru's metropolitan area in South India and is grappling with various environmental challenges like poor urban planning, including unchecked urbanization, air pollution, water scarcity, and waste management issues etc. The impact of climate change (CC) is also well observed in the urban Bengaluru resulting in the local Urban Heat Island (UHI). The interaction between local UHI and global CC creates challenges to human health, wellbeing and development. This study uses MODIS-Aqua Land Surface Temperature (LST) data for a decade (i.e., 2015-2024) to examine the UHI effect over the city. Climatological analysis of night time LST shows an average annual temperature-increasing trend between the urban Bengaluru and its neighboring suburbs and villages. This difference is computed at monthly scale and the fluctuations are being estimated using the satellite and validated against the ground observations. The Land use Land cover estimation are also linked to the UHI effect and the role of vegetation cover in the LST distribution is also quantified and it indicates the direct impact. This study will help in understanding the LST dynamics in the UHI effect over a rapidly urbanization city and can be used in the climate projection studies offering a ways to guide the urban planners, disaster managers and policy makers.

How to cite: Mohapatra, S. and Gouda, K. C.: Assessment of Surface Urban Heat Island over Bengaluru City in India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21505, https://doi.org/10.5194/egusphere-egu25-21505, 2025.

EGU25-796 | ECS | Orals | CL4.10

Evaluating the influence of Land Cover transformation on Coastal Land and Sea Surface Temperature Dynamics in Indian Peninsula 

Dyutisree Halder, Pritipadmaja Pritipadmaja, and Rahul Dev Garg

Understanding the dynamics of land surface temperature (LST) and sea surface temperature (SST) in coastal regions is crucial for addressing climate change impacts. This study investigates 20 years of MODIS-derived LST and SST data to assess the influence of land cover transformations on temperature patterns in the Indian Peninsula. Contrary to the prevailing emphasis on urbanization, our analysis reveals that shifts from forested areas to agricultural or barren lands have a more significant impact on temperature dynamics. Using geospatial techniques, we identify long-term trends and quantify the relative contributions of various land cover types to LST and SST variations. The findings highlight the critical role of non-urban land use changes in coastal temperature dynamics, challenging traditional perspectives. This study provides actionable insights for sustainable land management and climate adaptation strategies in coastal regions, emphasizing the need for integrated land use planning to mitigate thermal vulnerabilities in the face of global climate change.

How to cite: Halder, D., Pritipadmaja, P., and Garg, R. D.: Evaluating the influence of Land Cover transformation on Coastal Land and Sea Surface Temperature Dynamics in Indian Peninsula, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-796, https://doi.org/10.5194/egusphere-egu25-796, 2025.

EGU25-979 | Orals | CL4.10

Explaining climate change in South America 

Alice M Grimm and Dayane Padoan

Projections from a CMIP6 multimodel ensemble show weak signal of climate change in annual and seasonal precipitation over most of South America (SA), with low agreement among models as to the sign of the change over most of the continent. Besides, climate change information from different analyses frequently seems confusing for the public and decision makers. Since climate has a crucial influence on important economic sectors in SA, such as hydroelectric power generation and agriculture, and natural disasters associated with extreme events of drought and excessive rainfall have become more frequent and intense, the future climate behavior should be more clearly described, and supported by a dynamical framework able to explain it, so as to better serve decision-makers in planning actions and adopt effective policies for climate adaptation.

Although weak and with low agreement between models, the climate change projected by the CMIP6 multimodel ensemble for SA shows similarity with the seasonal impacts of El Niño (EN) events on precipitation. Since model projections of future SST indicate an El Niño-like warming pattern in the central-east equatorial Pacific, it is reasonable to hypothesize that changes in precipitation over South America would have the patterns of EN impact and would be mainly due to the strengthening of an EN-type SST anomaly pattern in the Pacific Ocean.

Therefore, to clearly determine the future climate changes, it is necessary to select models that not only simulate well the SA climatology, but also the El Niño-Southern Oscillation (ENSO) and its teleconnections with SA, since ENSO is responsible for most of the climate variability in SA. The assessment covered 31 models that provided at least three runs from the present  (1979-2014) to the future climate (2065-2100). Based on relevant and comprehensive criteria, the models were classified according to both assessments (climatology and ENSO), and four best-performing models were selected.

The changes projected by the ensemble of best models indicate a more EN-like future climate, in which the main climate changes projected for SA resemble the observed EN impacts, remarkably including the tendency to spring-summer reversal of precipitation anomalies in Central-East SA, from dryer spring to wetter summer. While the total monsoon precipitation shows little or no change in this region, there is reduction (enhancing) of early (peak) monsoon rainfall, resulting in a delay and shortening of the monsoon season. The spring response in this region is due to the dynamical effect of the EN-like SST changes via teleconnection, and the reversal in summer is triggered by surface-atmosphere interactions. Also coherently with EN impacts, drier conditions prevail in central-northern-eastern Amazon throughout the monsoon season thanks to changes in the Walker circulation, while in southeast SA, precipitation increases due to tropics-extratropics teleconnection.

The changes projected by the all-model ensemble are much weaker and confusing. This clear description of climate change and its dynamical connection with intensified EN effects give coherence to the different changes throughout different seasons, which otherwise seem incomprehensible and can lead to discrepant interpretations if not understood within a correct dynamic context.

How to cite: Grimm, A. M. and Padoan, D.: Explaining climate change in South America, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-979, https://doi.org/10.5194/egusphere-egu25-979, 2025.

Accurate and reliable future climate information is key for successful implementation of climate change adaptation plans especially on regional scales. Predicting the winter climate over Eurasia is challenging as both the initialized predictions and uninitialized climate projections show limited skill in reproducing observed variability on multi-annual to decadal timescales. It has been long recognized that the climate over Eurasia is strongly influenced by the North Atlantic Oscillation (NAO), especially in winter. The observed NAO indices show strong year to year variations that can be associated with climate conditions in Europe and Asia.  Numerous efforts have been made to use NAO as one of the major predictors for European climate. However,  the strength and spatial patterns of the NAO-related teleconnections vary with time, for example on multi-annual to decadal timescales, resulting in limited success in predictions on these time scales.

This study presents a novel approach to constrain variability in projection simulations over Eurasia by exploiting the teleconnection between the North Atlantic Oscillation (NAO) and the surface air temperature in the northern hemisphere. The constrained ensemble shows significantly higher skill and added value in predicting the multi-annual winter surface air temperature over Eurasia as compared to both the unconstrained ensemble of historical simulations and the initialized decadal predictions. The sensitivity analysis suggests that the constraining based on teleconnection during the previous 15 to 20 winter seasons is optimum for skillful predictions of multi-annual to decadal mean winter climate over Eurasia.

How to cite: Mahmood, R., Yang, S., and G. Donat, M.: Skillful predictions of Eurasian winter climate by constraining variability in CMIP6 simulations using NAO-temperature teleconnections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1485, https://doi.org/10.5194/egusphere-egu25-1485, 2025.

EGU25-3808 | ECS | Posters on site | CL4.10

Bayesian uncertainty quantification of internal climate variability 

Vincent Verjans and Markus Donat

Dimensionality reduction techniques are powerful for extracting modes of climate variability from observational data sets and climate model output. Over the past decades, multiple studies have shown that dominant climate patterns can be identified, and that climate evolution can be approximately linearized in such subspaces. In this work, we apply novel dimensionality reduction techniques to global climate data sets. In particular, we optimize such methods for finding patterns that maximize their inherent predictability on multi-annual time scales. We develop a fully Bayesian framework. The record of high-quality climate data sets (20-100 years) is relatively short compared to our predictability time scales of interest (1-10 years). This necessarily causes large uncertainty in data-driven analyses of internal climate variability due to sampling variability and biases. In a Bayesian analysis, we are able to rigorously quantify the uncertainty in observed internal climate variability: both in the spatial patterns, and in their dynamic time evolution.

 

We use linear inverse modeling to represent the climate dynamics in a subspace that optimizes predictability measures. We then use advanced Bayesian methods to calibrate the parameters of the linear model. The resulting uncertainty analysis allows to identify which climate modes – and interactions between modes – are well- or poorly-constrained within the observational record. This novel method further allows to explore if climate models can reproduce the linearized dynamics within observational uncertainties, or if they fail in representing some specific modes of climate variability.

While still in its early stages, this research is aimed at addressing key climate predictability challenges, in particular identifying the factors that contribute to accurate and reliable multi-annual climate predictions.

How to cite: Verjans, V. and Donat, M.: Bayesian uncertainty quantification of internal climate variability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3808, https://doi.org/10.5194/egusphere-egu25-3808, 2025.

The summer climate in the Northern Hemisphere during recent decades has shown distinct trend patterns, with warming hotspots that spatially match with the ridges of a circumpolar atmospheric wave pattern. The drivers behind this wave-like trend and warming pattern are not yet well understood. On the one hand, the CMIP6 multi-model ensemble mean presents a high degree of spatial pattern correlation over some regions but at a very small magnitude relative to observations. When considering individual single-model ensembles, however, we find: (i) a substantial spread in the forced response across models and (ii) a large spread in pattern similarity across the different ensemble members of the same models. This suggests that a combination of both forcing and internal climate variability may have contributed to the observed changes in atmospheric circulation. In ongoing work we are aiming to better understand the specific roles of forcing and climate variability, e.g., by investigating specific composites of those simulations most closely resembling the observed trends or by constraining ocean temperature variability patterns.

How to cite: Marcet-Carbonell, G., Donat, M. G., and Delgado-Torres, C.: Understanding the recent changes in summer atmospheric circulation on the Northern Hemisphere: the roles of external forcing and sea surface temperature variability., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3999, https://doi.org/10.5194/egusphere-egu25-3999, 2025.

EGU25-5784 | ECS | Posters on site | CL4.10

Attribution of flood event: a case study of the April/May 2024 floods in Southern Brazil 

Luiza Vargas-Heinz, Chen Lu, and Erika Coppola

The flood event of April/May 2024 that hit the Southernmost State of Brazil, Rio Grande do Sul, broke local records, with rivers reaching their highest level in recorded history. Around 2.4 million people are estimated to have been affected by the flood, with hundreds of thousands displaced and/or without access to potable water and electricity in their homes. Extreme precipitation, linked to a negative surface pressure anomaly, as suggested in the ERA5 dataset, was the primary driver. 

While attributing extreme precipitation events is an established practice, less work has been done to directly attribute river flood events to climate change, often due to a lack of long-term data in the region of interest. This study explores the feasibility of employing the existing attribution framework for attributing extreme discharge events.

We analyzed daily precipitation and river discharge data from over 40 stations (1960–2023, <10% missing) using two approaches. First, a "factual" distribution was developed using all the data available. A “counterfactual” distribution was obtained by fitting a distribution with the global mean surface temperature as covariate and a constant dispersion parameter, and then deriving the distribution assuming a 1.2°C cooler world.  Second, the data was divided into two separate periods: 1960-1991 (“past”) and 1992-2023 (“present”).  In both cases, differences in extreme values between these distributions were statistically assessed. Additionally, the surface pressure anomaly in ERA5 was used for analog attribution study, to assess the significance of the changes in surface pressure, precipitation, temperature, and discharge fields, between the “past” and “present” time periods.

Hydrological simulations performed with the CETEMPS Hydrological Model (CHyM) coupled with the CORDEX (Coordinated Downscaling Experiment)-CORE models output, both for a historical period and under the rcp85 scenario, were also used.  The model validation done for the historical period, comparing CHyM outputs against discharge station data, showed quite good agreement between the two for several statistics. Both the hydrological simulations and the regional climate CORDEX-CORE simulations were used in the analog attribution study to confirm the attribution of the event to global warming. This analysis investigates the potential of integrating hydrological modeling and observational discharge data to advance the attribution of extreme flood events to climate change.

How to cite: Vargas-Heinz, L., Lu, C., and Coppola, E.: Attribution of flood event: a case study of the April/May 2024 floods in Southern Brazil, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5784, https://doi.org/10.5194/egusphere-egu25-5784, 2025.

EGU25-6337 | Orals | CL4.10

Research opportunities for combining climate models with moisture tracking 

Ruud van der Ent, Imme Benedict, Victoria Deman, Damián Insua-Costa, Peter Kalverla, Hilde Koning, Gerbrand Koren, Chiel Lokkart, Bart Schilperoort, Arie Staal, Lan Wang-Erlandsson, Chris Weijenborg, and Ke Yang

Global warming as well as human modification of the Earth’s surface profoundly affects the water cycle in regional climates. A key question for ecosystem health and humanity in general is how exactly water resources and water-induced hazards will be affected. Atmospheric moisture tracking methods have the potential to help unravel the mechanisms of changes in precipitation patterns.

In the climate we had around the year 2000, moisture tracking tools have shown that about 40% of the rainfall on land originated from the land itself and 60% was supplied by the oceans. Several studies have also indicated that due to the land being water-limited for evaporation, the relative importance of the oceans will increase in a warming climate. For more detailed moisture tracking studies into past and future climates, however, the provided data from climate model intercomparison projects is often a limiting factor.

In this presentation, we present a position paper that aims to unlock the potential of addressing novel research questions by combining climate modelling and moisture tracking. First, we review the state-of-the-art regarding moisture tracking with climate models. Second, we present the data requirements for moisture tracking models, which typically consist of a limited set of surface and atmospheric variables, but have specific requirements regarding temporal, horizontal and vertical resolution. Third, we evaluate typical uncertainties in moisture tracking that may arise from working with suboptimal resolutions. Fourth, we analyze to what extent some climate models are already providing sufficient data to perform moisture tracking studies. data request. Fifth, we map potentially interesting research avenues linked to specific Model Intercomparison Projects (MIPs) within the ongoing CMIP6 to illustrate how more synergies could be created.

In conclusion, we systematically evaluated the current research interest, limitations and potential for moisture tracking studies with climate model output. With this presentation we hope to stimulate CMIP7 and other climate data providers to work together with the moisture tracking community to align the supply and demand side of climate variables. Doing so, would allow us to tap the now largely untapped potential of using moisture tracking to gain more insight into past and future water cycle changes.

How to cite: van der Ent, R., Benedict, I., Deman, V., Insua-Costa, D., Kalverla, P., Koning, H., Koren, G., Lokkart, C., Schilperoort, B., Staal, A., Wang-Erlandsson, L., Weijenborg, C., and Yang, K.: Research opportunities for combining climate models with moisture tracking, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6337, https://doi.org/10.5194/egusphere-egu25-6337, 2025.

EGU25-6554 | Orals | CL4.10

New look at humidity trends 

Cathy Hohenegger, Sarah Warnau, Tiffany Shaw, and Sarah Kang
Past studies have revealed a discrepancy between observed and simulated humidity trends in the satellite era. Especially over arid and semi-arid land regions, no trend in specific humidity is discernible in observations, whereas both uncoupled and coupled climate model simulations from the last CMIP exercise show a moistening trend. We revisit trends in specific humidity using global simulations that were conducted at a grid spacing of 10 km over multi decades. We consider two different models (IFS and ICON) as well as coupled and AMIP-type simulations. The coupled historical IFS simulation shows a moistening trend over the semi-arid and arid regions, similar to the result of the past coarse-resolution climate models. In contrast, the AMIP ICON simulation shows no discernable trend, in agreement with observations. One key difference between the two models is that IFS still uses parameterizations for shallow and partly deep convection, whereas ICON does not. Using the output of the two models, we further explore reasons for this distinct trend behavior between the two models.

How to cite: Hohenegger, C., Warnau, S., Shaw, T., and Kang, S.: New look at humidity trends, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6554, https://doi.org/10.5194/egusphere-egu25-6554, 2025.

EGU25-6885 | ECS | Posters on site | CL4.10

Using an explainable neural network to identify tropical drivers of the Northern Hemisphere wave-5 trend pattern 

Rikke Stoffels, Dim Coumou, and Vera Melinda Galfi

The recent trend in the Northern Hemisphere summer atmospheric circulation resembles a Rossby wave with wave number 5. These quasi-stationary circumglobal Rossby waves are associated with extreme events, such as heatwaves, droughts, and floods, that can have catastrophic societal impacts. Therefore, understanding the drivers of these Rossby waves and evaluating their representation in climate models is a key scientific challenge. However, identifying the drivers of such patterns can be difficult because traditional approaches such as simple correlation analysis may not capture the complex, nonlinear interactions inherent in atmospheric teleconnections. To address this, explainable artificial intelligence (XAI) offers a promising alternative. 

In this study, we test the hypothesis that the observed trend is partially driven by changes in the tropical oceans, which can influence midlatitude weather patterns through tropical-extratropical teleconnections. Using an explainable neural network approach, we aim to identify key tropical regions that drive the midlatitude wave-5 pattern on subseasonal timescales. The methodology is composed of two steps. First, the neural network is trained to predict the wave-5 pattern using tropical outgoing longwave radiation (OLR) fields as input. Next, we apply layer-wise relevance propagation, an explainability technique, to identify which input features are most important for accurate predictions. This process generates heat maps highlighting tropical regions that are important for the generation of a wave-5 pattern. Subsequently, changes in sea surface temperatures (SSTs) and OLR in the identified regions can be assessed as well as their correlation to the trend in the Northern Hemisphere circulation. We will present some preliminary outputs of this analysis.

How to cite: Stoffels, R., Coumou, D., and Galfi, V. M.: Using an explainable neural network to identify tropical drivers of the Northern Hemisphere wave-5 trend pattern, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6885, https://doi.org/10.5194/egusphere-egu25-6885, 2025.

EGU25-7065 | Orals | CL4.10

Lessons from the ‘hiatus‘ controversy for the 2023/2024 warming spike 

Karsten Haustein, Nadine Theisen, and Sebastian Sippel

Global mean annual temperature in 2023 did end up much warmer than anticipated, stirring up a lively debate as to what the potential reasons might be. 2024 continued that trend with another record warm year on top, exceeding 1.5°C globally for the first time in all temperature data sets on an annual basis.

Here we argue (1) that 2023 is entirely compatible with our understanding of the climate system and (2) that the so-called ‘hiatus‘ controversy from the early 2010s should be used as a reminder to be rather cautious with claims that suggest something puzzling might be going on.

We present results from statistical and model based analysis, demonstrating that the magnitude of the new September and annual temperature record in 2023 lies within the range of possible record margins under current warming / forcing conditions. We also show that random shifts in large scale circulation patterns led to record warm conditions in the North Atlantic and Antarctica, contributing to the 2023 and 2024 outcome (in addition to anthropogenic factors as well as El Niño).

We also discuss whether or not these shifts are partially attributable (directly or indirectly) to the 2022 Hunga Tonga eruption or the regulation-induced sulphur emissions reduction in the global shipping sector.

How to cite: Haustein, K., Theisen, N., and Sippel, S.: Lessons from the ‘hiatus‘ controversy for the 2023/2024 warming spike, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7065, https://doi.org/10.5194/egusphere-egu25-7065, 2025.

Uneven economic impacts of climate change have been caused by differentiated warming rates across different geographical regions, threatening the well-being of millions to billions of people. Region-dependent historical and future warming rates are often obtained from global climate models, which, however, exhibit wide spreads in both global mean temperature change and regional deviates. While the multi-model spread in global mean warming rate has been widely reported in past literature, the multi-model spread in terms of global warming pattern and its temporal evolution remain unclear. Here we show that the multi-model spread in the simulated global warming pattern is dependent on the level of warming. We find that the simulated global warming pattern deviates substantially among CMIP6 models before 1985. The multi-model consistency rises afterwards, as the greenhouse gases level and global mean warming rate increase. Furthermore, the consistency of model-predicted future warming pattern varies by emission scenario. Models predict highly consistent warming patterns under the high emission scenario during the entire 21st century; whereas under low and intermediate emission scenarios, future warming patterns diverge among these models around middle of the 21st century. While our study detects the anthropogenic signal in the temporal evolution of multi-model consistency in the global warming pattern, the physical mechanisms underlying such varying multi-model consistency in the warming pattern merits further investigation.

How to cite: Meng, Y., Yu, Y., and Nie, J.: Reduced spread of simulated global warming patterns among CMIP6 models with accelerated pace of warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8252, https://doi.org/10.5194/egusphere-egu25-8252, 2025.

EGU25-8966 | ECS | Orals | CL4.10

Influence of Global Warming on Extreme Sea Level Events Along European Coasts 

Maria Mulet, Marta Marcos, Angel Amores, and Miguel Agulles

Coastal sea level extremes are among the potentially most hazardous events for the densely populated coastal regions. Changes in extreme sea levels, combined with rising mean sea level, increase coastal vulnerability, and will continue to do so in the future. It is thus necessary to understand and quantify the role of global warming in the likelihood and intensity of extreme sea levels. In this study, we aim at testing whether the probability of extreme sea levels has changed in any way due to global warming. To do so, we analyse annual sea level maxima of a large ensemble of hydrodynamic simulations along the European coasts forced with the outputs of state-of-the-art climate models, simulating a total of nearly 1800 years of data that are representative of the climate of the past 6 decades, as well as 2500 years of data that are representative of the pre-industrial climate. The data have been bias-corrected to improve their reliability and accuracy in representing local sea level variations. We rely on the largely extended dataset to compute the Fraction of Attributable Risk (FAR) for different sets of sea level extremes along the entire European coastline. The results reveal that present-day regional climate conditions are altering the probability of likelihood of extreme sea levels along a large fraction of the European coastlines.

How to cite: Mulet, M., Marcos, M., Amores, A., and Agulles, M.: Influence of Global Warming on Extreme Sea Level Events Along European Coasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8966, https://doi.org/10.5194/egusphere-egu25-8966, 2025.

Historical changes in the North Atlantic atmospheric and oceanic circulation are re-evaluated using output from the Large Ensemble Single Forcing Model Intercomparison Project (LESFMIP). We focus on five of the single forcing experiments included in Phase 1 of the LESFMIP protocol: hist-GHG, hist-aer, hist-volc, hist-solar, and hist-totalO3. For each of these five, at least 10 ensemble members have been simulated over the period 1850 to 2020 by ~10 models. This dataset offers an unprecedented view of how these forcings have affected surface climate and the tropospheric and oceanic circulation, and their associated extremes. Specifically, the large-ensemble allows for isolating weak signals that otherwise would be buried under internal variability, while also offering a testbed for methods to extract predictable signals with correct amplitude.
Preliminary work shows a clear effect of greenhouse gases and aerosols on jets. In June-August, the influence of aerosols is as strong as that of greenhouse gases. Furthermore, the inter-model spread in the NH vortex responses dominates the intermodel spread in the NAO response. Ongoing work is aimed at formulating emergent constraints to sort out intermodel differences in the forced response of the polar vortex to historical forcings. Ongoing work is also aimed at understanding the impacts on surface temperature and precipitation. This is a community effort from the WCRP's APARC LEADER and EPESC projects.

How to cite: Avisar, D., Kuchař, A., Garfinkel, C., and Simpson, I.: Understanding historical changes in the North Atlantic atmospheric and oceanic circulation: insights from the Large Ensemble Single Forcing Model Intercomparison Project , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9609, https://doi.org/10.5194/egusphere-egu25-9609, 2025.

EGU25-10729 * | ECS | Orals | CL4.10 | Highlight

Combination of Internal Variability and Forced Response Reconciles Observed 2023 Warming 

Gergana Gyuleva, Reto Knutti, and Sebastian Sippel

The record-breaking global mean surface temperature (GMST) in 2023 came as a surprise to the scientific community, raising the question whether 2023 provides evidence for a recent and abrupt increase in the global warming rate. Here, we quantify the variability and forced contribution to annual GMST by training a statistical learning model on surface temperature anomalies from historical and future climate model simulations. Our method presents a novel approach to separting variability from forced changes in GMST, providing a computationally simple and powerful alternative to existing atmospheric Green’s function approaches. We find that more than half of the 2023 jump in GMST is explained by internal variability, largely owing to anomalously cool conditions in 2022. An unlikely combination of strong but not unprecedented forced and internal contributions occurring simultaneously appears to have led to the extreme jump in 2023 GMST, with North Atlantic warming being a key contributor. When adjusting for variability, we find a steady increase in forced warming rate over the past decades, consistent with previous studies. There is insufficient evidence for an acceleration of forced warming in 2023 and 2024 beyond the expected increase from continued carbon dioxide emissions and decreasing aerosol forcing in the past decades. Our results highlight the role of internal variability for short-term GMST fluctuations and call for an improved understanding of the Atlantic warming observed in 2023. 

How to cite: Gyuleva, G., Knutti, R., and Sippel, S.: Combination of Internal Variability and Forced Response Reconciles Observed 2023 Warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10729, https://doi.org/10.5194/egusphere-egu25-10729, 2025.

EGU25-10906 | ECS | Orals | CL4.10

Attributing changes in extreme precipitation across the Northeast U.S. under different climate scenarios  

Bor-Ting Jong, Thomas Delworth, Zachary Labe, William Cooke, and Hiroyuki Murakami

The Northeast United States has experienced the most rapidly increasing occurrences of extreme precipitation within the U.S. over recent decades, particularly during the warm season. This trend is primarily linked to events associated with tropical cyclones. Understanding the drivers leading to long-term trends in regional extreme precipitation under different future climate scenarios is critical to adaptation and mitigation planning.

New simulations with the fully-coupled 25-km GFDL (Geophysical Fluid Dynamics Laboratory) SPEAR (Seamless System for Prediction and EArth System Research) model and its 10 ensemble members, present a unique opportunity to study changes in regional extreme precipitation and relevant physical processes. Under the SSP5-8.5 scenario, SPEAR projects top 1% extreme precipitation events over the Northeast U.S. to increase by up to 2.4% by the end of the 21st century. The projected increase is driven by higher anthropogenic radiative forcing and is distinguishable from natural variability by the mid-century. From the meteorological perspective, the occurrences of warm season extreme precipitation related to both atmospheric rivers and tropical cyclones are projected to increase, even though the frequency of tropical cyclones in the North Atlantic is projected to decrease in the model.

The SSP5-8.5 scenario, however, represents a highly unlikely trajectory, prompting the scientific community to explore scenarios with rapid reductions in greenhouse gas (GHG) concentrations through various climate mitigation efforts. Using the SSP5-3.4OS overshoot scenario from the SPEAR model—where GHG emissions decline sharply after 2040 and reach net-negative levels by 2070—we assess the impact of mitigation on extreme precipitation over the Northeast U.S. Our results show that extreme precipitation frequency over the Northeast U.S. is projected to decrease as GHG concentrations decline. However, the timing of this reversal is seasonally dependent: warm-season trends reverse shortly after global mean surface temperature starts to decline, while cold-season trends lag by approximately 15 years. These results suggest that the response of extreme precipitation to GHG reductions may depend on the underlying mechanisms driving these events. For example, cold-season extremes are more often associated with large-scale extratropical cyclones, where dynamical processes play a significant role. Our study underscores the urgent need for a deeper understanding of the physical processes governing regional climate extremes in response to GHG mitigation. Such insights are essential for informing adaptation strategies and policymaking for effective climate risk management.

How to cite: Jong, B.-T., Delworth, T., Labe, Z., Cooke, W., and Murakami, H.: Attributing changes in extreme precipitation across the Northeast U.S. under different climate scenarios , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10906, https://doi.org/10.5194/egusphere-egu25-10906, 2025.

While the influence of well-mixed greenhouse gas emissions on global warming is well-documented and robustly attributed through multiple lines of evidence, regional attribution remains more challenging and dependent on the performance and resolution of climate models. This study proposed an observational-based statistical analysis utilizing the real-time Global Warming Index (GWI) to investigates the extent to which observed regional temperature trends are attributable to global-scale anthropogenic factors, mainly the direct effects of CO2, aiming to differentiate the portion of the change attributable to regional-scale drivers (such as regional industrial aerosols, black carbon aerosols, and land-use/land-cover change, etc).

To quantify the contribution of global– and regional–scale climate drivers to observed temperature change, I performed regression analyses using the HadCRUT4 temperature data and the Global Warming Index (GWI). The GWI, calculated through a least squares method, correlates observed global average temperatures with expected responses to global radiative forcing series. 

Results indicate that in certain regions — specifically West Asia, East N. America, West Africa, and the Amazon basin — 62±7%, 61±13%, 58±7%, and 61±10% of the warming observed over 1991-2020 can be attributed to global anthropogenic warming, primarily the direct effects of CO2. The remaining portion, which represents 22±8%, 21±16%, 27±9%, 23±14% of the observed warming, is attributable to regional climate drivers. The Mediterranean showcases high sensitivity, with regional drivers contributing 31±13% of the observed 1.2°C warming, amplifying the warming attributed to global anthropogenic drivers. The Arctic Ocean along with the Russian-Arctic region exhibits a substantial contribution from regional drivers and local feedback mechanisms to the observed warming amplification, quantified at 43±15% of the 3°C warming over 1991-2020. Regional cooling drivers, however, are significant in East Asia and the Tibetan Plateau, with the latter experiencing a cooling contribution of -42±17% (with a ±95% uncertainty due to internal variability derived from control simulations).

The novel approach presented in this study helps in understanding how different scales of climate change drivers contribute to local temperature change. This understanding can foster more effective, localized mitigation strategies that complement global efforts to address climate change.

How to cite: Barkhordarian, A.: Disentangling Regional Climate Change: Assessing the contribution of global– and regional–scale anthropogenic drivers to observed regional warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11006, https://doi.org/10.5194/egusphere-egu25-11006, 2025.

EGU25-12604 | Orals | CL4.10

Minimal impact of methane on satellite-era climate change 

Tiffany Shaw, Masaki Toda, and Sarah Kang

The attribution of global and regional climate change to anthropogenic greenhouse gases (GHGs) is well appreciated. Existing estimates based on radiative forcing studies suggest CO2 dominates global warming since 1850 with CH4 the second largest contribution (33-66% of CO2). However, radiative forcing studies involve several assumptions and GHG attribution beyond global-mean warming is unknown. Here we quantify the impact of individual GHGs on global warming indicators and regional climate change using single-forcing historical experiments of CO2, CH4, and other GHGs. CO2 is shown to dominate global warming in the satellite era with CH4 only 20% of the CO2 contribution, smaller than the amplitude of internal variability. Methane is also a small contribution for other global warming indicators, including Arctic Sea ice loss, extreme temperatures and continental scale warming. The results demonstrate that, on multi-decadal or longer time scales, CO2 is the dominant control knob and the contribution of CH4 to regional climate change is very small, undistinguishable from noise. Thus, CH4 mitigation may not be as effective as previously thought, particularly for regional scale impacts.  

How to cite: Shaw, T., Toda, M., and Kang, S.: Minimal impact of methane on satellite-era climate change, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12604, https://doi.org/10.5194/egusphere-egu25-12604, 2025.

EGU25-15359 | Orals | CL4.10

Anticipating Hot Summer Nights 

Johanna Baehr, Leonard Borchert, Sebastian Brune, Mrunali Damania, Moritz Drupp, Andreas Lange, Enrico Longo, Shivanshi Asthana, and Grischa Perino

Summer heat waves pose health threats to the general population, in particular, vulnerable groups. The skill for seasonal prediction of such heat waves has recently advanced. Yet, whether forecast information on this time scale, a time scale at which individual preparedness could still be improved, might be taken up by the general population, has—so far—not been investigated. Here, we present results from a large-scale online experiment with a general population sample in Germany (N = 4,251) to test how households respond to risk assessments for the number of heat events in their regions for the summer of 2024. Heat events are the number of tropical nights, i.e., with a temperature minimum of at least 20°C, during summer 2024 (June 1st – August 31st). As a risk assessment we use the 75percentile of an ensemble with 30 members originating from the operational seasonal forecasts with the German Climate Forecast System (GCFS2.1, Deutscher Wetterdienst, DWD). Participants were exposed in May 2024 to forecast information for the number of heat events in their region of residence, and in addition were provided with the typical summer in the absence of anthropogenic climate change. We present the consequential choices for self-interested and altruistic preventive adaptation measures, as well as for support for mitigation efforts participants demonstrated. Our results identify the impact of ’forward attribution’ to climate change, i.e., information on how the risk assessments would have differed for a world without anthropogenic climate change. We also check whether the perceived reliability of the seasonal prediction spills over to the perceived reliability of long-term climate predictions.

How to cite: Baehr, J., Borchert, L., Brune, S., Damania, M., Drupp, M., Lange, A., Longo, E., Asthana, S., and Perino, G.: Anticipating Hot Summer Nights, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15359, https://doi.org/10.5194/egusphere-egu25-15359, 2025.

EGU25-17291 | Orals | CL4.10

Representation of tropical and extratropical trends in ECMWF seasonal hindcasts 

Michael Mayer, Daniel Befort, and Antje Weisheimer

Climate trends represent one source of predictability for climate forecasts. Hence, it is important for seasonal prediction systems to reproduce observed trends in the climate system. This contribution presents an assessment of trends in seasonal hindcasts from the European Centre for Medium-Range Weather Forecasts (ECMWF). We investigate trends in the tropics and extratropics, as well as potential links between those.

In the tropics, the focus is on processes related to El Nino – Southern Oscillation (ENSO). The hindcasts exhibit a spurious sea surface warming trend in the equatorial Pacific (i.e., a tendency towards El Nino in more recent years), which is mainly related to an underestimation of the atmospheric circulation response to the observed strengthening of the equatorial Pacific zonal sea surface temperature gradient. The trend errors are most pronounced for boreal summer and autumn (independent of start date). Furthermore, the trend errors are similar to those found in free coupled climate model simulations and suggest a biased response of the atmospheric model to changes in the anthropogenic forcing.

In the extratropics, we focus on summer-time upper tropospheric circulation and surface temperature. The ensemble mean completely misses the clear observed circulation trends (resembling a wave-5 pattern) and the associated centers of enhanced surface warming. Possible implications and causes of the missed trends will be discussed.

How to cite: Mayer, M., Befort, D., and Weisheimer, A.: Representation of tropical and extratropical trends in ECMWF seasonal hindcasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17291, https://doi.org/10.5194/egusphere-egu25-17291, 2025.

EGU25-17493 | Posters on site | CL4.10

Quantifying changes in seasonal temperature variations using a functional data analysis approach 

Eva Holtanová, Lukas Brunner, and Jan Koláček

Ever-worsening climate change increases near-surface air temperatures for almost the entire Earth and threatens living organisms and human society. While annual mean changes are frequently used to quantify past and expected future changes, the increase is actually rarely uniform throughout the year. 

The shape of the annual cycle and its changes differ significantly between regions around the globe. Therefore, performing a global analysis implies the necessity to focus on diagnostics that can be evaluated for all these different shapes (e.g., single and double waves, different timing of seasons, etc.). Many previous studies relied on Fourier-transform-based methods, which assume a sinusoidal shape of the mean annual cycle. Here, we introduce an innovative approach based on functional data analysis. The evolution of the mean annual cycle is estimated from daily long-term mean temperature values, which are converted to functional form. This way, we can assess arbitrary shapes of the annual cycle. We concentrate on diagnostics that evaluate the change in absolute temperature, its seasonal slope, and the position of the maximum. We analyze two reanalysis datasets (coupled CERA20C and atmospheric ERA5) and a subset of CMIP6 Earth system models (ESMs). Recent changes in the second half of the 20th century are assessed, and the ability of ESMs to represent them is evaluated. Then, the changes projected for the end of the 21st century under the SSP3-7.0 pathway are analyzed.

Among other results, we highlight distinct differences between the two reanalyses, especially over equatorial and polar regions. Further, the projections show, for example, different rates of warming between seasons, resulting in changes in the amplitude. The largest amplitude increase is projected over the Mediterranean region and the largest decrease over the Arctic Ocean.  

How to cite: Holtanová, E., Brunner, L., and Koláček, J.: Quantifying changes in seasonal temperature variations using a functional data analysis approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17493, https://doi.org/10.5194/egusphere-egu25-17493, 2025.

EGU25-17706 | Orals | CL4.10

Forced Component Estimation Statistical Methods Intercomparison Project (ForceSMIP) 

Robert Jnglin Wills, Clara Deser, Karen McKinnon, Adam Phillips, Stephen Po-Chedley, Sebastian Sippel, and Anna Merrifield and the ForceSMIP Tier1 Contributors

Anthropogenic climate change is unfolding rapidly, yet its regional manifestation is often obscured by atmosphere-ocean internal variability. A primary goal of climate science is to identify the forced response, i.e., spatiotemporal changes in climate in response to greenhouse gases, anthropogenic aerosols, and other external forcing, amongst the noise of internal climate variability. Separating the forced response from internal variability can be addressed in climate models by using a large ensemble to average over different possible realizations of internal variability. However, with only one realization of the real world, it is a major challenge to isolate the forced response in observations, as is needed for attribution of historical climate changes, for characterizing and understanding observed internal variability, and for climate model evaluation.

In the Forced Component Estimation Intercomparison Project (ForceSMIP), contributors used existing and newly developed statistical and machine learning methods to estimate the forced response during the historical period within individual ensemble members and observations, across eight key climate variables (SST, surface air temperature, precipitation, SLP, zonal-mean atmospheric temperature, monthly max. and min. temperature, and monthly max. precipitation). Participants could use five CMIP6 large ensembles to train their methods, but they then had to apply their methods to individual evaluation members, the identity of which was hidden. Participants used methods including regression methods, convolutional neural networks, linear inverse models, fingerprinting methods, and low-frequency component analysis. Here we show how the different methods performed on climate models and what they determined to the be the forced response in observations. Our results show that many different types of methods are skillful for estimating the forced response and that the most skillful method depends highly on which variable and metric is evaluated. Furthermore, methods that show comparable skill can give very different estimates of the forced response in observations, illustrating the epistemic uncertainty in estimating the forced climate response from observations. ForceSMIP gives new insights into the forced response in observations across multiple key variables, but also the remaining uncertainty in its estimation.

How to cite: Jnglin Wills, R., Deser, C., McKinnon, K., Phillips, A., Po-Chedley, S., Sippel, S., and Merrifield, A. and the ForceSMIP Tier1 Contributors: Forced Component Estimation Statistical Methods Intercomparison Project (ForceSMIP), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17706, https://doi.org/10.5194/egusphere-egu25-17706, 2025.

In 2022, Europe experienced a severe and extensive drought with substantial ecological and economic impacts. The climatic hazard that led to these impacts can be attributed to two primary causes. First, thermodynamic warming due to climate change reduces water availability through increased evaporative demand. Second, an unusual atmospheric circulation pattern during the event compounded the situation. This was further exacerbated by strong decadal trends in atmospheric circulation. While thermodynamic changes are physically well understood, our understanding of the impact of circulation-driven trends on climate is largely limited to its impact on trends in surface temperature. To attribute the role of these different climatic drivers on the drought impacts, we use a storyline approach by nudging the Community Earth System Model Version 2 (CESM2) to atmospheric circulation patterns from the ERA5 reanalysis data at different forcing levels. Our findings indicate that the dynamical conditions leading to the 2022 drought were the most extreme in the observed period, following a long-term atmospheric circulation trend that explains around 50% of European drying. Moreover, the 2022 circulation patterns not only intensified the drought but also interacted with thermodynamic effects, exacerbating the hydroclimatic impacts. By distinguishing between circulation-induced trends and thermodynamic changes, we provide a nuanced understanding of the drivers of European hydroclimatic variability and their contribution to extreme events. We highlight the critical need to consider both atmospheric circulation changes and thermodynamic influences to evaluate accurately and project future hydroclimatic trends in Europe.

How to cite: Dunkl, I., Sippel, S., and Bastos, A.: Disentangling the role of trends in Atmospheric Circulation Patterns from Thermodynamic Effects for European Hydroclimate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18544, https://doi.org/10.5194/egusphere-egu25-18544, 2025.

EGU25-18816 | Orals | CL4.10

Reconstructing Historical Climate Data using Deep Learning 

Étienne Plésiat, Robert J. H. Dunn, Markus Donat, and Christopher Kadow

Understanding past climate conditions is essential for addressing future climate challenges. However, observational climate datasets often contain missing values, especially in older records, leading to incomplete and inaccurate analyses. Interpolation methods like kriging are commonly employed to address this issue by filling data gaps. Nevertheless, these approaches often fail to effectively reconstruct complex climatic patterns [1, 2].

This study leverages the transformative power of deep learning to accurately reconstruct two observational datasets. The first dataset is an intermediate product of HadEX3 [3], which contains gridded extreme indices over land regions, such as the TX90p index, corresponding to the percentage of days where daily maximum temperature is above the 90th percentile. The second dataset is the Full data GPCC product [4], containing global precipitation fields at monthly frequency. To reconstruct these two datasets with high accuracy, we employ and compare three deep learning approaches: a U-Net with partial convolutional layers, a diffusion model and a graph neural network. In all cases, models are trained on CMIP6 climate model data, evaluated on unseen CMIP6 and ERA5 data and compared to Kriging. The best-performing models are then applied to the observational datasets, providing new insights into historical climate conditions to inform more effective climate adaptation strategies. The reconstructed datasets are being prepared for the community in the framework of the H2020 CLINT project [5] and the Horizon Europe EXPECT project [6].

[1] Kadow C. et al., Nat. Geosci., 13, 408-413 (2020)
[2] Plésiat É. et al., Nat. Commun., 15, 9191 (2024)
[3] Dunn R.J.H. et al., J. Geophys. Res. Atmos., 125, 1 (2020)
[4] Schneider, U. et al., DOI: 10.5676/DWD_GPCC/FD_M_V2022_100 (2022)
[5] https://climateintelligence.eu/
[6] https://expect-project.eu/

How to cite: Plésiat, É., Dunn, R. J. H., Donat, M., and Kadow, C.: Reconstructing Historical Climate Data using Deep Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18816, https://doi.org/10.5194/egusphere-egu25-18816, 2025.

EGU25-20122 | ECS | Posters on site | CL4.10

Advancing climate research through the WCRP core project on Earth System Modelling and Observations (ESMO) 

Bimochan Niraula, Sara Pasqualetto, and Fanny Adloff

Earth System Modelling and Observations (ESMO) is a new core project of the World Climate Research Project (WCRP) that coordinates, advances, and facilitates all modelling, data assimilation and observational activities within WCRP, working jointly with all other WCRP projects. Our mission is to facilitate the coordination and advancement of climate modeling and observational efforts. Through collaborative approaches, interdisciplinary partnerships, and identification of critical research gaps ESMO aims to enhance the accuracy, reliability, and accessibility of climate data and projections. Alongside three pre-existing Working Groups - on Coupling Modelling (WGCM), Numerical Experimentation (WGNE), and Sub-seasonal to Interdecadal Prediction (WGSIP), an additional working group on Observations for Researching Climate (WGORC) has now been established. WGORC in particular will focus on observations and needs for observation across WCRP, including observations for reanalyses and emerging technologies. This, alongside the other WGs focused on modelling, will be instrumental in identifying gaps and bridging research communities in climate science. Here, we present the exciting new structure of ESMO, and how we hope to bring together experts across modelling and observational disciplines, to further scientific advances.

How to cite: Niraula, B., Pasqualetto, S., and Adloff, F.: Advancing climate research through the WCRP core project on Earth System Modelling and Observations (ESMO), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20122, https://doi.org/10.5194/egusphere-egu25-20122, 2025.

Land surface and the planetary boundary layer are linked by the water and energy cycles, and the effects of soil water-air coupling modulate near-surface temperatures. In particular, late spring soil moisture anomalies may uncover predictability to the system, and then contribute to predictions of extreme events such as heatwaves at the subseasonal to seasonal scale. In this study, we use a data-driven seasonal forecast for summer heat waves in the Western Mediterranean, and a downstream explainable artificial intelligence helps us separate the individual contribution of the predictors and quantify and rank them in terms of their relative importance. Soil moisture emerges as one of the heat wave predictors, along with SST in the North Atlantic and the background global warming. Results show that soil largely contributes to heatwaves predictability when it is dry at the beginning of the season, otherwise its importance is limited. In addition, soil moisture contribution substantially increases from the beginning of the 1990s, when the local warming quickly arises and summer precipitation declines sharply. When atmospheric patterns are favorable for the advection of hot and dry air, conditions for persisting and more intense heatwaves are supported by an interacting land surface. With little water available for evaporation, the increased atmospheric evaporative demand may not be met, therefore the lack of latent cooling in the atmosphere enables more intense and persistent heatwaves.

How to cite: Materia, S. and Donat, M.: Growing importance of soil moisture anomalies for prediction of summer heatwaves in the Western Mediterranean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20837, https://doi.org/10.5194/egusphere-egu25-20837, 2025.

EGU25-789 | ECS | Orals | CL4.12

Evaluating Surface Heat Feedbacks: Insights from CMIP Models 

Kwatra Sadhvi, Lengaigne Matthieu, Danielli Vincent, Iyyappan Suresh, and Vialard Jérôme

Surface feedbacks are critical to understanding global temperature patterns, as they directly regulate the exchange of energy at the ocean-atmosphere boundary. While surface feedbacks have been studied using methods like the Gregory regression, Climate Feedback-Response Analysis Method (CFRAM) and Partial Radiative Perturbation (PRP) approaches, their role in shaping climate responses remains less explored through analytical frameworks. Here, we assess surface feedbacks across 48 models from the Coupled Model Intercomparison Project Phases 5 and 6 (CMIP5/6) using a novel analytical formulation. This approach focuses on net surface heat flux feedbacks (latent and longwave), with observational constraints to improve robustness.
Our results indicate that the globally averaged surface feedback is dominated by the latent heat component for both the multi-model mean and the diversity. This is because of strong compensation between upward and downward longwave feedbacks. Observational constraints further reveal that CMIP models tend to overestimate the negative latent heat feedback in the tropics, attributed to an exaggerated air-sea temperature gradient . This bias may contribute to a ~10% underestimation of the global warming signal in these models.
By leveraging this novel analytical approach, we provide insights into surface feedback processes that are obscured in traditional TOA-based analyses. While our findings for net longwave feedbacks align closely with the standard regression approach, the analytical method reveals systematically higher negative latent feedback values. This divergence points to the need of further investigating the roles of short-term feedback processes and dynamical contributions, paving the way for reconciling analytical and regression-based methodologies.

How to cite: Sadhvi, K., Matthieu, L., Vincent, D., Suresh, I., and Jérôme, V.: Evaluating Surface Heat Feedbacks: Insights from CMIP Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-789, https://doi.org/10.5194/egusphere-egu25-789, 2025.

EGU25-1486 | ECS | Orals | CL4.12

How to think about the shortwave water vapor feedback 

Florian E. Roemer, Stefan A. Buehler, and Kaah P. Menang

Recent studies have provided analytical descriptions of Earth’s longwave feedback λLW; to expand on this, we propose an analytical model for the shortwave water vapor feedback λSW. In this model, λSW is proportional to the change in the square of atmopsheric transmissivity tatm with temperature T and thus mainly originates from spectral regions that ”transition” from optically thin to optically thick. Following Jeevanjee (2023, DOI: 10.1119/5.0135727), we approximate tatm based on the column water vapor MH2O and the water vapor mass absorption cross-section κH2O. We show that in order to capture the weak T dependence of λSW, it is crucial to account for spectral variations in κH2O, which can already be achieved by a simple exponential fit.

We further demonstrate that the T dependence of λSW can be explained by the opposing effects of two main processes: At low T, more optically thin parts of the spectrum ”start” their transition than optically thick parts ”complete” their transition, leading to an increase in λSW with T. At high T, the inverse T dependence of the Clausius-Clapeyron relation leads to a decrease in λSW.

We can also extend our model to incorporate second-order effects such as spectral variations in solar irradiance and deviations of κH2O from the idealized exponential fit. This version of the model is in good agreement with full radiative transfer simulations. The remaining discrepancies can be attributed to non-linear absorption by the water vapor continuum, deviations in MH2O from the approximated Clausius-Clapeyron scaling, and the effects of molecular Rayleigh scattering.

In conclusion, we demonstrate that the shortwave water vapor feedback λSW can be understood using a simple analytical model. This model also demonstrates the merits of a spectral approach to understand λSW and illuminates the two key processes that drive its T dependence.

How to cite: Roemer, F. E., Buehler, S. A., and Menang, K. P.: How to think about the shortwave water vapor feedback, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1486, https://doi.org/10.5194/egusphere-egu25-1486, 2025.

EGU25-1658 | Orals | CL4.12

Circulation and cloud responses to patterned SST warming 

Michael Byrne, Anna Mackie, Emily Van de Koot, and Andrew Williams

The climatological atmospheric circulation is key to establishing the tropical 'pattern effect', whereby cloud feedbacks induced by sea surface temperature (SST) warming depend on the spatial structure of that warming. But how patterned warming-induced circulation changes affect cloud responses is less clear. Here we use idealized simulations with prescribed SST perturbations to understand the contributions to changes in tropical-mean cloud radiative effects (CRE) from different circulation regimes. We develop a novel framework based on moist static energy to understand the circulation response, targeting in particular the bulk circulation metric of ascent fraction. Warming concentrated in regions of ascent leads to a strong 'upped-ante' effect and spatial contraction of the ascending region. Our framework reveals substantial contributions to tropical-mean CRE changes not only from traditional 'pattern effect' regimes, but also from the intensification of convection in ascent regions as well as a smaller contribution from cloud changes in convective margins.

How to cite: Byrne, M., Mackie, A., Van de Koot, E., and Williams, A.: Circulation and cloud responses to patterned SST warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1658, https://doi.org/10.5194/egusphere-egu25-1658, 2025.

Cloud feedback remains a leading source of uncertainty in climate model projections under increasing atmospheric carbon dioxide. Cloud-controlling factor (CCF) analysis is a method used to observationally constrain cloud feedback and, subsequently, the climate sensitivity. Although high clouds contribute significantly to this uncertainty, they have historically received comparatively little attention in CCF studies. Here, we apply CCF analysis to observationally constrain high-cloud feedback, focusing on feedback associated with changes in cloud amount due to its dominant contribution to uncertainty. Our observational constraints reveal larger decreases in high cloud amount with warming than climate models predict, yet the net high-cloud radiative feedback remains near-neutral due to compensating shortwave and longwave effects. We also show that including upper-tropospheric static stability as a predictor effectively captures the stability iris mechanism and associated changes in cloud amount. This work highlights the importance of using physically relevant CCFs for robust observational constraints on high-cloud feedback and improving mechanistic understanding of its underlying drivers.

How to cite: Wilson Kemsley, S. J., Nowack, P., and Ceppi, P.: Observational high-cloud feedback constraints indicate climate models underestimate global reductions in high-cloud amount with warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2499, https://doi.org/10.5194/egusphere-egu25-2499, 2025.

EGU25-2583 | ECS | Orals | CL4.12

Estimates of the Global Clear-Sky Longwave Radiative Feedback Strength from Reanalysis Data 

Helene Gloeckner, Lukas Kluft, Hauke Schmidt, and Bjorn Stevens

We use atmospheric profiles from ERA5, JRA55 and MERRA2 between 1993 and 2023 to estimate Earth’s global clear-sky longwave feedback strength on the seasonal and interannual timescale. Differences in the relationship of relative humidity with skin temperature prior to 2008 lead to interannual feedback strengths between 1.34 W m2 K1 (JRA55) and 1.89 W m2 K1 (MERRA2). Restricting the analysis to the last 16 years
yields more consistent interannual estimates of 2.05 W m2 K1 on average, which is larger than the overall seasonal estimate of 1.91 W m2 K1. The mid-tropospheric drying causing this difference suggest a substantial influence of ENSO variability on the interannual timescale. This indicates a long-term feedback strength smaller than 2.0 W m2 K1, which is already at the lower end of previous estimates; emphasizing the importance of accurate long-term RH measurements to reliably project Earth’s clear-sky feedback strength.

How to cite: Gloeckner, H., Kluft, L., Schmidt, H., and Stevens, B.: Estimates of the Global Clear-Sky Longwave Radiative Feedback Strength from Reanalysis Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2583, https://doi.org/10.5194/egusphere-egu25-2583, 2025.

EGU25-3714 | ECS | Posters on site | CL4.12

Positive forcing over land cools the Eastern Pacific Ocean 

Moritz Günther, Sarah Kang, and Yohai Kaspi

We set out to disentangle the impacts of forcing over land vs. forcing over ocean on the sea surface temperature (SST) pattern. Based on previous research showing that forcings over land and ocean have distinct impacts on the circulation, we hypothesize that they would also affect the pattern of sea surface temperatures in different ways. We investigate the research question by quadrupling the CO2 concentration either only over ocean or only over land in the coupled global climate model MPI-ESM-1.2.

Our main results are:

  • the climate response to 4 x CO2 forcing only over land surface and forcing only over ocean adds up surprisingly linearly to the climate response to forcing everywhere.

  • 4 x CO2 forcing over land causes a cooling of up to 1.4 K in the equatorial, Eastern, and Southeastern Pacific Ocean within two years. In contrast, positive forcing over the ocean does not produce such a cooling on any time scale

  • Two main mechanisms contribute to the Pacific cooling in response to positive forcing over land:

    • (a) a northward ITCZ shift originating from the fact that there is more land in the Northern than the Southern hemisphere, enhancing equatorial upwelling and cooling from strengthened trade winds

    • (b) the monsoon-desert mechanism (Rodwell & Hoskins 1996), which strengthens the subtropical highs in response to atmospheric heating over the Americas, increasing the equatorward advection of cold air and initiating a wind-evaporation-SST feedback.

 

We find an equatorial and Eastern Pacific cooling not only in the abrupt land-forced simulation, but also in a transient simulation forced with a 1% / year CO2 increase over land, on a time scale of 20 years. The surprising finding that a positive forcing can cause a cooling in the Eastern Pacific, along with the mechanisms we describe, may contribute to better understanding the recent cooling of the Eastern Pacific Ocean as well as the long-standing model bias in simulating Eastern Pacific sea surface temperature patterns.

How to cite: Günther, M., Kang, S., and Kaspi, Y.: Positive forcing over land cools the Eastern Pacific Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3714, https://doi.org/10.5194/egusphere-egu25-3714, 2025.

EGU25-4227 | ECS | Orals | CL4.12

Observational quantification of high cloud radiative effect and feedback: An Analysis of differences across the tropical Pacific 

Paula Veronica Romero Jure, Declan Finney, Amanda Maycock, Alan Blyth, Anna Mackie, and Hugo Lambert

Tropical high cloud feedback remains a key uncertainty in estimating Equilibrium Climate Sensitivity, particularly the optical depth feedback. The Pacific Intertropical Convergence Zone is a major contributor to tropical cloud radiative effect (CRE). The Tropical Pacific is also projected to see shifts in convection from West to East. In this study, we analyse the key differences in the observed high cloud radiative effect, optical depth and feedback between the East and West Pacific. Notably, we find that the strongest climatological high cloud optical depths and net radiative effects in the tropical region are found in the East Pacific, despite greater high cloud amounts in the West Pacific.   

We further estimate the high cloud feedback from the observed variability, using 20 years of CERES Flux By Cloud Type data from MODIS satellite (Sun et al. 2022), following Raghuraman et al [2024] for the regions. We find significant, opposite total high cloud feedbacks between the East and West Pacific, driven primarily by the high cloud amount feedback, with smaller contributions from the optical depth and altitude feedbacks. The shortwave and longwave cloud amount feedbacks are significant in both regions, greater in the West and opposite in sign to the East Pacific. However, the net amount feedback is negative in both regions and twice as strong in the East Pacific than in the West. As expected, the cloud altitude feedback is positive in every region analysed, primarily driven by the longwave component. Only the West Pacific shows a significant optical depth feedback, driven by a positive shortwave feedback.  The distinct high cloud amount and optical depth feedbacks estimated in the regions are not apparent when analysing the entire tropics. 

We find that the estimated cloud feedbacks in the tropical Pacific strongly depend on the inclusion of ENSO events in the record. Since climate projections suggest an El Nino-like warming in response to CO2 forcing, understanding the potential for changes in high cloud properties in the Pacific, as suggested by our observational evidence, is vital. 

 

References: 

Raghuraman, S.P. et al. (2024) ‘Observational Quantification of Tropical High Cloud Changes and Feedbacks’, Journal of Geophysical Research: Atmospheres, 129(7), p. e2023JD039364. Available at: https://doi.org/10.1029/2023JD039364. 

Sun, M. et al. (2022) ‘Clouds and the Earth’s Radiant Energy System(CERES) FluxByCldTyp Edition 4 Data Product’, Journal of Atmospheric and Oceanic Technology, 39(3), pp. 303–318. Available at: https://doi.org/10.1175/JTECH-D-21-0029.1. 

How to cite: Romero Jure, P. V., Finney, D., Maycock, A., Blyth, A., Mackie, A., and Lambert, H.: Observational quantification of high cloud radiative effect and feedback: An Analysis of differences across the tropical Pacific, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4227, https://doi.org/10.5194/egusphere-egu25-4227, 2025.

EGU25-4417 | ECS | Orals | CL4.12

Addressing non-linearities when estimating radiative feedbacks associated with different historical forcing agents 

Maisie Wright, Harry Mutton, Mark Ringer, and Timothy Andrews

Understanding how radiative feedbacks respond to different historical forcing agents (e.g. aerosols or greenhouse gases) improves our ability to relate historical changes (1850-2014) to future projections. This is often investigated using historical single forcing experiments, where only one forcing agent is allowed to vary, to decompose the total (all-forcing) response. However, using a 45-member ensemble, we demonstrate that there are non-linearities in this decomposition which challenge its utility in HadGEM3-GC31-LL. Specifically, strong warming in the Southern Ocean and sea ice loss are seen in the aerosol single forcing experiment despite global cooling, which is found to be a feature that does not combine linearly with other climate drivers. Instead, we calculate the aerosol response as the difference between the all-forcing experiment and an “all-but-aerosol” experiment, where all forcing agents apart from aerosols are included. This method does not show strong Southern Ocean warming and sea ice loss in response to anthropogenic aerosols. We instead see a positive surface albedo feedback in this region, which is more consistent with the feedbacks seen in the all-forcing response. This allows for a more accurate comparison between feedbacks caused by different forcing agents.

How to cite: Wright, M., Mutton, H., Ringer, M., and Andrews, T.: Addressing non-linearities when estimating radiative feedbacks associated with different historical forcing agents, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4417, https://doi.org/10.5194/egusphere-egu25-4417, 2025.

EGU25-4990 | ECS | Orals | CL4.12

Reversal of Precipitation Trend and Large-Scale Atmospheric Temperature Inversion in Hothouse Climates 

Jiachen Liu, Jun Yang, Feng Ding, Gang Chen, and Yongyun Hu

Throughout Earth's history and its potential future, surface temperatures (Ts​) have fluctuated across a far broader range than those of the present-day climate. However, the characteristics of extremely cold or warm climates remain less explored compared to modern climates. This study investigates the hydrological trends and atmospheric stratification in hothouse climates (Ts>330 K). Our results show that in climate models, precipitation decreases as surface temperature rises in hothouse climates, in contrast to the behavior observed in modern climates. This reversal trend results from the upper limit of outgoing longwave radiation and the continuously increasing shortwave absorption by H2O and aligns with a pronounced increase in atmospheric stratification. One remarkable feature of such a highly stable atmosphere is the occurrence of a large-scale “atmospheric temperature inversion”, where the upper atmosphere is warmer than the lower’s. Although this inversion has been noted in previous studies, its formation mechanisms have remained unclear. Our work demonstrates that while radiative heating in the lower troposphere is necessary, it is not independently sufficient to form this atmospheric inversion. Instead, large-scale subsidence-induced dynamic heating plays an essential role in forming this inversion. Hothouse climates, as characterized by these findings, are feeble worlds rather than vibrant worlds.

How to cite: Liu, J., Yang, J., Ding, F., Chen, G., and Hu, Y.: Reversal of Precipitation Trend and Large-Scale Atmospheric Temperature Inversion in Hothouse Climates, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4990, https://doi.org/10.5194/egusphere-egu25-4990, 2025.

EGU25-5900 | ECS | Orals | CL4.12

Influence of Mean State Biases on Projections of the Tropical Warming Pattern 

Alessandra Stoppelli, Christian Éthé, Juliette Mignot, and Jérôme Vialard

The rise in anthropogenic greenhouse gases since the 20th century has led to regionally varying warming rates. Observations over recent decades reveal subdued warming—or even cooling—in the eastern and southeastern tropical Pacific, linked to intensified equatorial trade winds. Understanding this warming pattern is crucial due to its wide-reaching impacts: it alters atmospheric stability, driving rainfall changes through the warmer-get-wetter mechanism; affects El Niño variability and tropical cyclone intensity; and influences cloud cover, planetary albedo, and transient climate sensitivity.

While  models from the Coupled Model Intercomparison Project (CMIP), including IPSL-CM6A-LR, generally capture the subdued warming in the Southeast Pacific, they project enhanced warming in the eastern equatorial Pacific (El Niño-like response) that contradicts observations. A major factor behind this discrepancy could be the persistent cold and dry equatorial Pacific bias in these models, particularly pronounced in IPSL-CM6A-LR

To test this hypothesis, we analyze coupled flux-corrected simulations designed to reduce mean state biases. Corrections to momentum and heat fluxes mitigate cold tongue and western Pacific dry biases, as well as easterly wind errors. However, the double Intertropical Convergence Zone (ITCZ) bias remains substantial. We examine how these biases influence the tropical Pacific warming pattern during the historical period and under 21st-century climate projections, while addressing the limitations of stationary flux correction. Finally, we outline planned sensitivity experiments to explore the key physical processes driving the tropical warming pattern in response to climate change.

How to cite: Stoppelli, A., Éthé, C., Mignot, J., and Vialard, J.: Influence of Mean State Biases on Projections of the Tropical Warming Pattern, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5900, https://doi.org/10.5194/egusphere-egu25-5900, 2025.

EGU25-5950 | ECS | Posters on site | CL4.12

An Estimation of the Efficacy of Methane Radiative Forcing Using Radiative Kernels 

Sumit Kumar, Ashwin K. Seshadri, and Govindasamy Bala

Methane (CH4) and carbon dioxide (CO2) are two major greenhouse gases with distinct radiative properties and climate responses. Using the National Centre for Atmospheric Research (NCAR) Community Atmosphere Model (CAM5) in two configurations (prescribed sea surface temperature and slab ocean) to estimate radiative forcing and climate response and radiative kernel analyses, we compare their slow feedback mechanisms and implications for climate sensitivity. We perform simulations with a 10X increase in CH4 and 1.35X CO2 concentration to simulate global mean warming of about 1.5 K in both cases. We find that CH4 requires a larger effective radiative forcing, indicating a lower efficacy relative to CO2.

We attribute CH4's lower efficacy to differences in slow feedback processes. CH4 exhibits more negative lapse rate feedback (difference of -0.10 Wm-2K-1) and more positive water vapor feedback (difference of 0.06 Wm-2K-1) due to equatorially concentrated radiative forcing and stronger upper-tropospheric warming. Feedback differences also include weaker positive shortwave cloud (difference of -0.05 Wm-2K-1) and smaller albedo (difference of -0.04 Wm-2K-1) feedback responses for CH4, resulting in a net feedback difference of -0.12 Wm-2K-1. These findings underscore the role of spatial forcing patterns, including CH4’s near-infrared shortwave absorption bands and low-latitude warming, in shaping feedback processes.

We find that CO2 forcing results in relatively stronger polar warming, enhancing albedo feedback, and induces larger mid-latitude cloud reductions, amplifying shortwave cloud feedback. Both gases have comparable positive longwave cloud feedback, broadly consistent with fixed anvil temperatures. All individual feedback differences are statistically significant. Our results highlight that distinct feedback responses arise from basic physical mechanisms, such as differing meridional warming patterns and small but distinct relative humidity changes.

Our study advances the understanding of radiative forcing structure and feedbacks in determining greenhouse gas impacts on climate sensitivity. It also highlights the need for multi-model assessments and Earth system modeling to evaluate feedback uncertainties and refine projections of long-term climate responses as relative contributions to radiative forcing evolve.

How to cite: Kumar, S., Seshadri, A. K., and Bala, G.: An Estimation of the Efficacy of Methane Radiative Forcing Using Radiative Kernels, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5950, https://doi.org/10.5194/egusphere-egu25-5950, 2025.

EGU25-7361 | Orals | CL4.12

Perspectives on Climate Sensitivity and Ocean Heat Uptake 

Nadir Jeevanjee, David Paynter, John Dunne, John Krasting, and Lori Sentman

The notion of climate sensitivity has become synonymous with Equilibrium Climate Sensitivity (ECS). But, 21st century warming is affected at zeroth order by ocean heat uptake, which isn't accounted for by ECS but is accounted for by the Transient Climate Response (TCR). In this talk, we highlight some potentially underappreciated aspects of TCR and ocean heat uptake, using the two-box ocean model as a common theoretical framework. We emphasize that i) TCR can be scaled by the forcing to estimate transient temperature change across a variety of scenarios, ii) this scaling can be used to estimate the time to cross a given temperature target in a given forcing scenario, using only a model's TCR, and iii) the two-box model predicts a linear relationship between ocean heat content and surface temperature which is inconsistent with most models. This talk is based on an forthcoming article in Annual Reviews of Earth and Planetary Sciences.

How to cite: Jeevanjee, N., Paynter, D., Dunne, J., Krasting, J., and Sentman, L.: Perspectives on Climate Sensitivity and Ocean Heat Uptake, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7361, https://doi.org/10.5194/egusphere-egu25-7361, 2025.

EGU25-7524 | Orals | CL4.12

An Observational Estimate of the Pattern Effect on Climate Sensitivity 

David WJ Thompson, Maria Rugenstein, Piers M Forster, and Leif Fredericks

We estimate the contributions of the spatially varying temperature field to internal climate feedbacks through the statistical relationships between the observed global-mean radiative response R and the spatially-varying temperature field Ti. The results indicate regions where surface temperature covaries with R and thus provide a statistical analogue to the causal response functions derived from simulations forced with surface temperature “patches”. Notably, the results of the statistical analyses yield patterns in temperature that explain roughly the same fraction of the variability in R as that explained by patch experiments. Consistent with the results of those experiments, the observational analyses indicate large negative internal feedbacks due to temperature variability over the western Pacific. Unlike the results inferred from such experiments, the analyses indicate equally large positive internal feedbacks over the southeastern tropical Pacific and negative internal feedbacks over land areas. When estimated from observations, temperature variability over the land areas accounts for roughly 80% of the global-mean, negative internal feedback; and temperature variability over the southeastern tropical Pacific acts to attenuate the global-mean negative internal feedback by nearly 10%.

How to cite: Thompson, D. W., Rugenstein, M., Forster, P. M., and Fredericks, L.: An Observational Estimate of the Pattern Effect on Climate Sensitivity, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7524, https://doi.org/10.5194/egusphere-egu25-7524, 2025.

EGU25-8415 | ECS | Orals | CL4.12

Decomposing Cloud Radiative Feedbacks by Cloud-Top Phase 

Casey Wall, David Paynter, Yi Qin, Matvey Debolskiy, Margaret Duffy, Takuro Michibata, Brandon Duran, Nicholas Lutsko, Po-Lun Ma, Brian Medeiros, Trude Storelvmo, and Ming Zhao

Changes in cloud scattering properties and emissivity that arise from atmospheric warming cause substantial radiative feedbacks in model projections of anthropogenic climate change, and the relative importance of the underlying mechanisms is poorly understood. One leading hypothesis is that ice-to-liquid conversions cause clouds to optically thicken, producing a major negative feedback. We test this hypothesis by developing a method to decompose cloud radiative feedbacks by cloud-top phase. The method is applied to an ensemble of six state-of-the-art global climate models run with prescribed sea-surface temperature. In these simulations, the global mean of the net cloud scattering and emissivity feedback from cloud-phase conversions ranges from -0.17 to -0.01 W m-2 K-1, while the overall net cloud feedback ranges from 0.02 to 0.91 W m-2 K-1. The multi-model mean of the cloud scattering and emissivity feedback from cloud-phase conversions is approximately 18% of the magnitude of the multi-model mean of the overall cloud feedback (-0.10 W m-2 K-1 vs. 0.52 W m-2 K-1). These results indicate that cloud-phase conversions cause a robust negative feedback by changing cloud scattering and emissivity, but this mechanism makes a modest contribution to the overall cloud feedback at the global scale.

How to cite: Wall, C., Paynter, D., Qin, Y., Debolskiy, M., Duffy, M., Michibata, T., Duran, B., Lutsko, N., Ma, P.-L., Medeiros, B., Storelvmo, T., and Zhao, M.: Decomposing Cloud Radiative Feedbacks by Cloud-Top Phase, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8415, https://doi.org/10.5194/egusphere-egu25-8415, 2025.

EGU25-8545 | Posters on site | CL4.12

Basic physic predicts stronger high cloud radiative heating with warming 

Blaž Gasparini, Giulio Mandorli, Claudia Stubenrauch, and Aiko Voigt

The interaction of cloud droplets and ice crystals with radiation, known as cloud radiative heating, alters temperature gradients in the atmosphere, affecting both cloud evolution as well as circulation and precipitation. Despite its climatic relevance, the response of cloud radiative heating to global warming remains largely unknown.

We study changes to cloud radiative heating profiles in a warmer climate, identify physical mechanisms responsible for these changes, and develop a theory based on well-understood physics to predict them. Our approach involves a stepwise procedure that starts with a simple hypothesis of an upward shift in cloud radiative heating at constant temperature, and gradually incorporates additional physical effects.

We find that cloud radiative heating intensifies as high clouds move upward, despite minimal changes in cloud properties and temperatures. We attribute this intensification to a decrease in air density, which often overcompensates for the decrease in high cloud fraction with warming in idealized multi-model simulations of radiative-convective equilibrium. Furthermore, the density-mediated changes in cloud radiative heating are also observed in satellite-derived retrievals of cloud radiative heating in the tropics.

The density-mediated increment in cloud radiative heating may increase the role of high clouds in controlling atmospheric flows in a warmer climate. Moreover, our results suggest that the uncertainty in model‐predicted changes in atmospheric circulations and hence regional climate could be reduced by narrowing the spread in model‐simulated cloud radiative heating in the present‐day climate.

 

How to cite: Gasparini, B., Mandorli, G., Stubenrauch, C., and Voigt, A.: Basic physic predicts stronger high cloud radiative heating with warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8545, https://doi.org/10.5194/egusphere-egu25-8545, 2025.

EGU25-10273 | ECS | Orals | CL4.12

Why weakening the overturning Walker circulation in the tropical ascent region leads to a reduction in subtropical low clouds 

Danny McCulloch, Hugo Lambert, Mark Webb, and Geoffrey Vallis
Global Climate Models (GCMs) are essential for predicting the impacts of global and regional climate change in the coming decades. However, the primary source of uncertainty in these predictions is our limited understanding of cloud feedback and its representation in models.  The remote effects of deep convection on subtropical low clouds in the warming climate are poorly understood. Improving our knowledge of how deep convection affects low clouds via the tropical overturning circulation is crucial to refining climate projections.
 
In this study, we use an AMIP climate assessment configuration (with CMIP6 forcing) of the Met Office Unified Model to quantify the impact of local and remote changes in the tropical atmospheric circulation on subtropical low clouds.  We conduct a causal intervention analysis by applying a cooling perturbation in the free troposphere above the deep convective western equatorial Pacific Ocean. This method allows us to weaken the large-scale circulation in the ascent region and track the resulting effects on subtropical clouds. We find that when we cool the free troposphere in the tropical west Pacific region, we get a deepening of the subtropical East Pacific boundary layer and a reduction in overall low cloud fraction. This study allows us to determine and present the physical mechanism behind this "tropical ascent → subtropical clouds" interaction and emphasises the benefits of using targeted perturbation methods to conduct causal analyses and disentangle regional and process linkages within models. 

How to cite: McCulloch, D., Lambert, H., Webb, M., and Vallis, G.: Why weakening the overturning Walker circulation in the tropical ascent region leads to a reduction in subtropical low clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10273, https://doi.org/10.5194/egusphere-egu25-10273, 2025.

EGU25-11046 | ECS | Orals | CL4.12

Quantifying all-sky climate sensitivity with idealized clouds 

Lukas Kluft, Bjorn Stevens, Manfred Brath, and Stefan A. Buehler

We include idealised clouds in a single column model to estimate the all-sky climate sensitivity. Our results show that the cloud radiative effects observed from satellites can be accurately reproduced by combining high and low/mid-level clouds. We introduce a "fixed cloud albedo" null hypothesis, which assumes a fixed cloud albedo but allows for changes in cloud temperature as the surface warms. By analysing cloud distributions consistent with present-day observations, we estimate a mean fixed-albedo climate sensitivity of 2.2 K, slightly less than the clear-sky value. Our results highlight the importance of cloud masking effects, especially by mid-level clouds, and the reduction of radiative forcing by high clouds. Giving more weight to low-level clouds, which are assumed to change temperature with warming, results in a reduced estimate of 2.0 K. This provides a baseline to which changes in surface albedo, and a believed reduction in cloud albedo, would add to.

How to cite: Kluft, L., Stevens, B., Brath, M., and Buehler, S. A.: Quantifying all-sky climate sensitivity with idealized clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11046, https://doi.org/10.5194/egusphere-egu25-11046, 2025.

Uncertainty in climate sensitivity remains a critical challenge for effective mitigation and adaptation strategies. While cloud radiative feedbacks are often highlighted as a major source of this uncertainty, here we explore the impact of clear-sky shortwave radiation absorption by water vapor (SWA). Using abrupt 4xCO2 simulations with altered SWA, we show that higher SWA conditions lead to a larger increase in climate sensitivity over time due to the faster and stronger recovery of the initially weakened Atlantic Meridional Overturning Circulation (AMOC). Enhanced SWA reduces surface shortwave radiation, leading to global cooling, particularly in the Arctic, where increased salinity creates conditions favorable for AMOC recovery. This accelerated recovery amplifies warming in the subpolar North Atlantic, intensifying positive lapse rate and cloud feedbacks, ultimately leading to a larger increase in net climate feedback and climate sensitivity. This underscores the need to constrain clear-sky SWA uncertainties to improve projections of climate sensitivity and associated feedback mechanisms.

How to cite: Kang, S. and Lee, D.: Effective climate sensitivity increases with enhanced shortwave absorption by water vapor due to its impact on AMOC recovery, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11416, https://doi.org/10.5194/egusphere-egu25-11416, 2025.

EGU25-12505 | Posters on site | CL4.12

Cloud Feedbacks Affect Hydrological Sensitivity 

Zachary McGraw, Lorenzo Polvani, Blaž Gasparini, Emily Van de Koot, and Aiko Voigt

Cloud responses to warming are a known uncertainty for temperature projections, yet how these same responses affect precipitation has been little evaluated. Here we explore how cloud radiative feedbacks influence the global mean precipitation change per degree of warming (hydrological sensitivity). With radiative kernels, we examine how warming-induced changes in cloud amount, altitude, and optical depth alter the atmosphere’s ability to radiatively cool and form precipitation. Our results suggest that high cloud responses are the single largest cause of spread in hydrological sensitivity across climate models. Applying the cloud locking methodology to one model, we find that cloud radiative responses reduce hydrological sensitivity by 14% and investigate the controls on this value.

How to cite: McGraw, Z., Polvani, L., Gasparini, B., Van de Koot, E., and Voigt, A.: Cloud Feedbacks Affect Hydrological Sensitivity, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12505, https://doi.org/10.5194/egusphere-egu25-12505, 2025.

EGU25-13127 | Orals | CL4.12

Decoding the Anthropogenic Influences on Pacific Warming Patterns 

Yen-Ting Hwang, Shang-Ping Xie, Po-Ju Chen, Hung-Yi Tseng, Clara Deser, Hsiang-Chi Yeh, Yong-Jhih Chen, Yue Dong, Masahiro Watanabe, Sarah M. Kang, and Malte F. Stuecker
The observed lack of surface warming in the Southeast and central equatorial Pacific sharply contrasts with climate model projections, which consistently simulate an enhanced equatorial warming pattern. A recent assessment suggests that the zonal sea surface temperature gradient has historically been controlled by strengthening mechanisms but is projected to shift toward dominance by weakening mechanisms in the future (Watanabe et al., 2024). A pressing question remains: When will the weakening of the equatorial zonal sea surface temperature gradient emerge?
 
To address this question, I will review recent work from my group and collaborators, focusing on identifying the fast and slow components of sea surface temperature pattern responses to anthropogenic aerosols, stratospheric ozone, and greenhouse gases via idealized step-function experiments. Our findings suggest that the superposition of fast and slow responses to these forcings can sustain the equatorial cooling trend for longer than anticipated. Contrary to the interannual and decadal variability literature, which primarily emphasizes wave dynamics, we highlight the critical roles of spatial patterns in the atmospheric energy budget (moist static energy budget) in driving the initial adjustments of Hadley and Walker circulations. The fast components, along with the associated cloud radiative effects, initiate a series of air-sea interactions that set the stage for the slower components. Possible explanations for the discrepancies between model projections and observations will also be discussed.
 

How to cite: Hwang, Y.-T., Xie, S.-P., Chen, P.-J., Tseng, H.-Y., Deser, C., Yeh, H.-C., Chen, Y.-J., Dong, Y., Watanabe, M., Kang, S. M., and Stuecker, M. F.: Decoding the Anthropogenic Influences on Pacific Warming Patterns, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13127, https://doi.org/10.5194/egusphere-egu25-13127, 2025.

EGU25-13431 | ECS | Posters on site | CL4.12

A Simple Spectral Model for Earth’s Albedo 

Zhiping Zhang, Daniel Koll, and Timothy Cronin

It is well-known that Earth's planetary albedo is about 0.3. Less clear is how this value might change in different climates. Here we propose a simple conceptual model for Earth's albedo. Our main insight is that, for a clear-sky N2-H2O atmosphere, the atmosphere can be approximated in the shortwave spectrum as either perfectly absorbing (due to water vapor absorption) or perfectly scattering (due to Rayleigh scattering); in contrast, clouds are approximately perfect scatterers throughout the shortwave spectrum. We use these approximations to derive analytic albedo expressions from the two-stream equations, which we validate against line-by-line model calculations.

Our results indicate that, for a clear-sky atmosphere, as surface temperature rises from 200 K to 500 K, Earth’s planetary albedo initially decreases with warming until around 350 K due to enhanced water vapor absorption, and then increases due to intensified Rayleigh scattering. Turning to idealized high and low cloud scenarios, cloudy atmospheres have significantly higher albedos than a clear-sky atmosphere at low temperatures. However, for an atmosphere with low clouds, albedo generally decreases with warming due to increased water vapor absorption above the clouds. In contrast, an atmosphere with high clouds exhibits nearly constant albedo with temperature, as high clouds mask the influence of the underlying atmosphere. These findings suggest that Earth’s clear-sky shortwave feedback is positive below 350 K and negative above 350 K. As for cloudy scenarios, low clouds induce a strong positive shortwave feedback at low temperatures, while high clouds don’t. Our simple model improves understanding of Earth’s planetary albedo and the role of shortwave feedback for the runaway greenhouse. Furthermore, our work suggests low clouds generally tend to destabilize Earth’s climate, which has potential implications for future climate change adaptation.

How to cite: Zhang, Z., Koll, D., and Cronin, T.: A Simple Spectral Model for Earth’s Albedo, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13431, https://doi.org/10.5194/egusphere-egu25-13431, 2025.

The majority of climate models predict the development of an enhanced eastern equatorial Pacific (EEP) warming pattern (“El Niño-like”) by century-end, characterized by greater mean warming over the Pacific cold tongue compared to the western Pacific warm pool and the corresponding weakening of the Walker circulation. A number of plausible mechanisms have been proposed to explain this pattern; however, it remains unclear which proposed mechanism is dominant in this response. Moreover, the magnitude of the EEP pattern varies greatly across climate models. To understand these differences, we conduct partially coupled experiments with an abrupt 4xCO2 increase, wherein surface wind stress and shortwave fluxes are overridden to values prescribed from the preindustrial control simulations, using two climate models – CESM1 and CESM2. Although both models were developed at NCAR, their behaviors are very different. In the former model, changes in the east-west SST gradient along the equator are relatively small. In contrast, the latter model, known to have a high climate sensitivity, develops a very strong EEP pattern. We find that the key factors that explains these differences are the different strengths of the  Bjerknes (wind stress-SST) and shortwave (low clouds-SST) feedbacks critical in reducing the Pacific zonal SST gradient, whereas differential evaporative cooling in the equatorial region appears to be similar between the two models. We discuss the implications of these results to the ongoing and future changes in the tropical Pacific.

How to cite: Fedorov, A. and Fu, M.: The role of the Bjerknes and low-cloud feedbacks in the formation of the eastern equatorial Pacific warming pattern: contrasting two climate models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14461, https://doi.org/10.5194/egusphere-egu25-14461, 2025.

EGU25-14568 | ECS | Posters on site | CL4.12

Hydrological sensitivity affected by tropical tropospheric stability 

Donghyun Lee and Paulo Ceppi

Climate forcers perturb the energy amount inside the Earth, and atmospheric interactions in the troposphere sequentially vary to pursue the new stable state in the given energy budget. The varied energy amount of longwave, shortwave, and sensible heat flux in the atmosphere is balanced with latent heat flux, equivalent to the changes in precipitation in the global mean sense. For example, rising temperature emits more longwave radiation from the atmosphere (longwave cooling, LWC), and it allows more energy budget room for latent heat flux (LHF) heating, which explains enhanced precipitation.

Although previous studies argued hydrological sensitivity as the linearized scale of precipitation change per the global mean temperature change, this study confirms that tropical tropospheric stability has additionally affected hydrological sensitivity over the decades. Our results reveal that tropical ocean temperature patterns correlate statistically with the stability index. The numerically simplified term of this stability effect improves the prediction skills of the theoretical equation for the global mean precipitation change under scenarios with various forcing conditions.  Lastly, we discuss the possible impacts of recent ocean patterns and the tropical tropospheric stability phase on precipitation by comparing the observed data and climate models’ simulations, which are forced by the observed sea surface temperature.

How to cite: Lee, D. and Ceppi, P.: Hydrological sensitivity affected by tropical tropospheric stability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14568, https://doi.org/10.5194/egusphere-egu25-14568, 2025.

Tropical high cloud feedbacks exhibit considerable spread across climate models. This study applies the cloud radiative kernel technique of Zelinka et al. (2012a; 2013) to 22 models across the Coupled Model Intercomparison Project CMIP5 and CMIP6 ensembles to survey tropical high cloud feedbacks and analyze their relationships to climate sensitivity, changes to the tropical overturning circulation, and changes to deep convective organization across scales. First, the inter-model spread in tropical high cloud net, altitude, and optical depth feedbacks exhibit significant correlations to climate sensitivity in the tropical mean and on convective margins. Additionally, we find that inter-model variability in deep convective organization – at both the mesoscale and planetary scales – relates to the inter-model spread in high cloud feedbacks along convective margins. More specifically, decreases in tropical ascent area and increases in mesoscale organization of deep convection relate to more positive high cloud feedbacks, particularly within weak ascent and weak descent regimes. Increases in mesoscale organization also coincide with a greater weakening of the Pacific Walker circulation. Finally, relationships between the inter-model spread in tropical high cloud feedbacks, convective organization across scales, and sea surface temperature patterns will be discussed. 

How to cite: Schiro, K. and Dawson, E.: Spread in high cloud feedback along tropical convective margins linked to changes in convective organization across scales, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14904, https://doi.org/10.5194/egusphere-egu25-14904, 2025.

We construct a radiative-advective model to investigate the drivers of Arctic amplification. The Rapid Radiative Transfer Model for GCMs (RRTMG) is utilized to calculate radiative heating rates, while the atmospheric horizontal energy transport (AHT) from JRA-55 reanalysis data is used as boundary conditions. We perturb individual factors in the model to assess the warming contributions from radiative forcing by different greenhouse gases, poleward energy transport at different vertical levels, and clouds.

We first examine the Arctic climate sensitivity to CO2, CH4, and O3. The climate sensitivity is defined as the surface temperature change per unit of TOA flux perturbation. The Arctic climate sensitivity to CO2 is 3.46 K/W/m². When CO2 is doubled, the instantaneous radiative forcing at TOA is 1.68 W/m², resulting in 5.7 K surface warming. For CH4, the Arctic climate sensitivity is 1.65 K/W/m², and doubling CH4 leads to a TOA perturbation of 0.46 W/m², leading to merely 0.76 K surface warming. The sensitivity to O3 is 0.21 K/W/m², with a doubling of O3 causing a 3.51 W/m² perturbation and 0.75 K surface warming.

The sensitivity to AHT is strongly dependent on its vertical structure, with greater sensitivity at lower levels. At 975 hPa level, the climate sensitivity reaches its peak value of 3.15 K/W/m², comparable to that of CO2. At the 900 hPa level where climatological AHT peaks, the climate sensitivity dramatically drops to 0.73 K/W/m². At higher altitude, the sensitivity continues to decrease: 0.64 K/W/m² at 850 hPa, 0.62 K/W/m² at 700 hPa, and 0.30 K/W/m² at 500 hPa. The climate sensitivity to clouds is 1.62 K/W/m². The climatological cloud fraction in the Arctic is 15%, with radiative effect of 2.09 W/m² at the TOA, resulting 3.41 K surface warming.

In summary, the Arctic region shows highest climate sensitive to CO2, followed by sensitivity to AHT at 975 hPa and CH4, although CH4 increase does not induce significant flux perturbations at the TOA. Clouds also play an important role. The sensitivities to AHT above 900 hPa and O3 are relatively smaller.

How to cite: Zhang, H. and Wang, Y.: Understanding the drivers of Arctic amplification through an idealized radiative-advective equilibrium model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15286, https://doi.org/10.5194/egusphere-egu25-15286, 2025.

EGU25-15351 | Orals | CL4.12

Strong pattern effect evident in Southern Ocean cloud feedback based on multiple lines of evidence 

Trude Storelvmo, Haochi Che, Jenny Bjordal, Tim Carlsen, Robert David, Ada Gjermundsen, Luke Whitehead, and Greg McFarquhar

The Southern Ocean is known to be one of the cloudiest places on Earth, and the important contribution of Southern Ocean clouds to Earth’s energy budget is undisputed. By changing their composition in response to warming, clouds in this region currently limit the rate of warming, as they become brighter with increasing temperature and thus exert a stabilising feedback on the climate system. Here, based on multiple lines of evidence, we show that in the current state of the Southern Ocean climate, this negative feedback happens to be maximised. Moving away from the present climate state in either direction (cooling or warming) will thus reduce the feedback, such that the climate sensitivity to any perturbation can be expected to grow rapidly with each degree of temperature change. This finding adds urgency to the implementation of effective climate mitigation to limit warming and thus preserve the stabilising climate effect of Southern Ocean clouds.

How to cite: Storelvmo, T., Che, H., Bjordal, J., Carlsen, T., David, R., Gjermundsen, A., Whitehead, L., and McFarquhar, G.: Strong pattern effect evident in Southern Ocean cloud feedback based on multiple lines of evidence, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15351, https://doi.org/10.5194/egusphere-egu25-15351, 2025.

EGU25-17356 | ECS | Orals | CL4.12

Water Vapor Spectroscopy and Thermodynamics Constrain Earth’s Tropopause Temperature 

Brett McKim, Nadir Jeevanjee, Geoff Vallis, and Neil Lewis

As Earth warms, the tropopause is expected to rise, but predictions of its temperature change are less certain. Longstanding theories tie the tropopause temperature to outgoing longwave radiation (OLR), but this contradicts recent work in which simulations exhibit a Fixed Tropopause Temperature (FiTT) even as OLR increases. The FiTT is thought to result from the interaction between upper tropospheric moisture and radiation, but a predictive theory for FiTT has not yet been formulated. Here, we build on a recent explanation for the temperature of anvil clouds and argue that tropopause temperature, defined by where radiative cooling becomes negligible, is set by water vapor's maximum spectroscopic absorption and Clausius-Clapeyron scaling. This "thermospectric constraint'' makes quantitative predictions for tropopause temperature that are borne out in single column and general circulation model experiments where the spectroscopy is modified and both the radiative and lapse-rate tropopause change in response. This constraint provides a theoretical foundation for the FiTT hypothesis, shows how tropopause temperature can decouple from OLR, and suggests a way to relate the temperatures of anvil clouds and the tropopause.

How to cite: McKim, B., Jeevanjee, N., Vallis, G., and Lewis, N.: Water Vapor Spectroscopy and Thermodynamics Constrain Earth’s Tropopause Temperature, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17356, https://doi.org/10.5194/egusphere-egu25-17356, 2025.

EGU25-17908 | ECS | Orals | CL4.12

Quantifying the tuning uncertainty on the climate sensitivity of the EC-Earth climate model 

Federico Fabiano, Chiara Ventrucci, Paolo Davini, Jost von Hardenberg, and Susanna Corti

Despite decades of developments, the inter-model spread in climate sensitivity in the latest CMIP ensemble remains substantial, with relevant implications for mid- to long-term climate projections. The inter-model differences are driven by model biases and structural deficiencies, mostly linked to cloud feedbacks, but the specific processes that dominate this issue remain unclear. Physical parametrizations are of primary importance for the performance of climate models, in particular those regarding microphysics and convection - especially at current model resolutions. Indeed, a fundamental yet often overlooked aspect of coupled model development is the tuning of parameters involved in these parametrizations to align with some specific constraints (e.g. radiative balance and global mean temperature in the pre-industrial state).
Here, we propose a methodology to evaluate the uncertainty in equilibrium climate sensitivity (ECS) arising from parameter tuning and apply it to the EC-Earth3 climate model. Our approach consists in systematically perturbing a set of tuning parameters - primarily those affecting tropical convection and precipitation - aiming to maximize their impact on climate sensitivity while ensuring the parameters remain within a plausible range. We obtain a low and a high sensitivity configuration of the model, resulting in a moderate change in climate sensitivity of approximately ±0.3 K. Finally, the results are discussed in the context of the CMIP6 ensemble, suggesting that the inter-model spread is likely driven by deeper structural differences within the models rather than uncertainties arising from the tuning process.

How to cite: Fabiano, F., Ventrucci, C., Davini, P., von Hardenberg, J., and Corti, S.: Quantifying the tuning uncertainty on the climate sensitivity of the EC-Earth climate model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17908, https://doi.org/10.5194/egusphere-egu25-17908, 2025.

EGU25-20708 | ECS | Orals | CL4.12

CO2-dependence of Longwave Clear-sky Feedback is sensitive to Temperature 

Yue Xu and Daniel Koll

CO2 is widely appreciated as a radiative forcing agent, but recent work showed that CO2 also acts as a climate feedback (Seeley & Jeevanjee 2020). CO2’s ability to emit longwave radiation allows the atmosphere to shed more energy in response to surface warming, and gives rise to a “radiator fin” effect which dominates Earth’s climate sensitivity in hot-and-high-CO2 climates. However, the general CO2-dependence of the longwave feedback is still poorly understood.

Here we explore the CO2-dependence of Earth’s longwave clear-sky feedback using a line-by-line model. We report a dividing surface temperature (Ts) of ~290 K for typical relative humidities. Above 290K, CO2 increases the feedback; below 290K, CO2 decreases the feedback; around 290K, the feedback is CO2-independent. We explain our results via a spectral competition between CO2 radiator fins, which enhance the feedback, and CO2 blocking the surface’s emission, which decreases the feedback. Only at high Ts, once H2O shuts down all window regions, does CO2 enhance the feedback.

Given that Earth’s global-mean temperature is close to ~290K, our results explain why feedback CO2-dependence is weak in our current climate but could have been important for paleoclimates. Finally, because feedback CO2-dependence is identical to forcing Ts-dependence, our results also explain the temperature-dependence of the CO2 forcing. Analogous to the clear-sky feedback, CO2 forcing also changes its behavior above versus below ~290K.

How to cite: Xu, Y. and Koll, D.: CO2-dependence of Longwave Clear-sky Feedback is sensitive to Temperature, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20708, https://doi.org/10.5194/egusphere-egu25-20708, 2025.

EGU25-20772 | ECS | Orals | CL4.12

Changes in the large-scale circulation and the clear-sky response to warming at very slow rotation rates 

Abisha Mary Gnanaraj, Hauke Schmidt, and Jiawei Bao

The clear-sky response to surface warming is generally the result of increases in tropospheric temperature and water vapour, assuming constant relative humidity (RH). While this purely thermodynamic response is fairly well understood, there has been less focus on whether the response of the large-scale circulation to surface warming can alter the clear-sky response. Therefore, in this study, we investigate how the large-scale circulation on Earth-like planets would respond to warming, whether the constant RH assumption holds for different circulation responses, and how deviations from this assumption can affect the clear-sky response. We use the ECHAM6 general circulation model in an aquaplanet configuration and modify the large-scale circulation by changing the planet's rotation rate from 1/32 to 8 times the current Earth's rotation rate. We run two sets of experiments, one with a fixed SST as a control scenario and the other with a +4K warming scenario. We analyse the radiative flux-circulation response as the difference between the warming and control scenarios.

From faster to slower rotation, the Hadley cell expands and strengthens, increasing the dryness of the atmosphere and decreasing the water vapour masking effect. Therefore, at first order, when RH is assumed to be constant, the clear-sky response increases from faster to slower rotation. However, there are second order effects at rates slower than 1/4 of the Earth's current rotation rate, which we associate with the large changes ( > 10%) in RH. At such slow rotation rates, the Hadley cell becomes global. Meanwhile, a secondary circulation develops, characterised by convergence at the equator in the lower troposphere and divergence in the mid-troposphere. We refer to this as the congestus circulation. Changes in RH correlate well with changes in the response of the congestus circulation to warming. The deep Hadley circulation weakens with surface warming like on Earth. But the congestus circulation strengthens, increasing mid-tropospheric RH, which in turn reduces the clear-sky response. We discuss to what extent this effect is due to increased upper-tropospheric radiative cooling that is not compensated by the deep circulation. Alternatively, we discuss whether this effect is due to increased convective self-aggregation with surface warming that increases the congestus outflow.

How to cite: Gnanaraj, A. M., Schmidt, H., and Bao, J.: Changes in the large-scale circulation and the clear-sky response to warming at very slow rotation rates, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20772, https://doi.org/10.5194/egusphere-egu25-20772, 2025.

EGU25-20967 | Orals | CL4.12

Links between internal variability and forced climate feedbacks: The importance of patterns of temperature variability and change 

Luke Davis, David W. J. Thompson, Maria Rugenstein, and Thomas Birner

Understanding the relationships between internal variability and forced climate feedbacks is key for using observations to constrain future climate change. Here we probe and interpret the differences in these relationships between the idealised climate change projections provided by the CMIP5 and CMIP6 experiment ensembles. We find that internal variability feedbacks better predict forced feedbacks in CMIP6 relative to CMIP5 by over 50%, and that the increased predictability derives primarily from the slow (>20 year) response to greenhouse gas forcing. A key novel result is that the increased predictability is consistent with the greater resemblance between patterns of internal and forced temperature change in CMIP6, which suggests temperature pattern effects play a key role in predicting forced climate feedbacks. In general, we find that forced feedbacks are more predictable when the response more closely resembles El Niño, with amplified East Pacific warming and cloud changes reflecting a weakened Walker circulation. Despite the increased predictability, emergent constraints provided by observed internal variability are weak and largely unchanged from CMIP5 to CMIP6 due to the relative shortness of the observational record.

How to cite: Davis, L., Thompson, D. W. J., Rugenstein, M., and Birner, T.: Links between internal variability and forced climate feedbacks: The importance of patterns of temperature variability and change, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20967, https://doi.org/10.5194/egusphere-egu25-20967, 2025.

EGU25-1470 | Orals | CL4.15

Novel and skilful ocean-based predictors for European hydro-meteorological extremes 

Amulya Chevuturi, Marilena Oltmanns, Isaac Abbott, Wilson Chan, Eugene Magee, Maliko Tanguy, Sergio Vicente Serrano, Dhais Peña Angulo, Cecilia Svensson, Ben Harvey, Bentje Brauns, John Bloomfield, and Jamie Hannaford

With anticipated changes in future hydrological extremes over Europe, it is important to better understand their underlying drivers for ultimately improving their forecasting. Previous studies have demonstrated a significant influence of the North Atlantic Ocean on European climate. Building on this, we identify novel North Atlantic Sea surface temperature (SST) indicators that are linked to meteorological and hydrological extremes across various European catchments at long lead times. We evaluate predictor-predictand relationships by assessing the concurrent and lagged statistical links between European hydro-climate variables (e.g., precipitation, evaporation, temperature, streamflow and groundwater levels) with North Atlantic SST indicators. These SST indicators are associated with events that increase freshwater input into the ocean, leading to subsequent shifts in key ocean currents. Combining observations and theory, we trace the associated teleconnection pathways from North Atlantic Ocean changes to atmospheric dynamics influencing the North Atlantic Jet Stream, ultimately impacting the European hydroclimate that can account for the statistical links. Our findings reveal that these North Atlantic SST patterns exert varying influences on the Scandinavian regions, central western Europe and Iberian Peninsula at one-to-two years lead time. Our research therefore has significant potential in practical applications for advancing forecasting of extremes and early warning systems through the identification of novel and skilful predictors, which can contribute to the mitigation of risks associated with hydro-meteorological extremes.

How to cite: Chevuturi, A., Oltmanns, M., Abbott, I., Chan, W., Magee, E., Tanguy, M., Vicente Serrano, S., Peña Angulo, D., Svensson, C., Harvey, B., Brauns, B., Bloomfield, J., and Hannaford, J.: Novel and skilful ocean-based predictors for European hydro-meteorological extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1470, https://doi.org/10.5194/egusphere-egu25-1470, 2025.

EGU25-1901 | ECS | Posters on site | CL4.15

A Climatology of Northern Hemisphere Cold Surge 

Wenling Cui, Lin Wang, and Meng Gao

Cold surges, or cold waves, are extreme weather events marked by abrupt drops in surface temperature and strong winds, making them some of the most impactful and concerning phenomena. Unlike cold air outbreaks, which are defined solely by sustained low temperatures, cold surges are characterized by both significant temperature drops and low temperatures. These events can severely disrupt societal activities, posing serious threats to human health, agricultural production, and economic stability. Despite their importance, there is no universally accepted definition of cold surges, and their tracks are often inferred indirectly, using proxies such as the movement of the Siberian High or air particle trajectories. In this study, we propose a unified definition of cold surges and introduce a novel method for their automatic identification and tracking. This algorithm detects cold surges and provides characteristics such as affected areas, duration, temperature drop, and temperature anomalies. Using this method, a Northern Hemisphere cold surge climatology is obtained.Based on the distribution of the frequency of affected areas, the entire Northern Hemisphere is divided into four regions: (1) Africa-Eurasia (AF-EA) ;(2) Pacific Ocean (PO);(3) North America (NA);(4) Atlantic Ocean (AtlO).The characteristics of cold surges in the Northern Hemisphere and these four regions are described. The frequency of cold surges in the Northern Hemisphere shows an increasing trend before 1970 and a decreasing trend after 1970, which is also observed in AF-EA, PO, NA, and AtlO. The duration shows a decreasing trend in the Northern Hemisphere and all four regions. The mean 24-hour temperature drop and the maximum 24-hour temperature show a slight negative (positive) trend in the Northern Hemisphere, AF-EA, and NA (AtlO). The mean and maximum temperature anomalies show a positive trend in the Northern Hemisphere, AF-EA, AtlO, and PO.

How to cite: Cui, W., Wang, L., and Gao, M.: A Climatology of Northern Hemisphere Cold Surge, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1901, https://doi.org/10.5194/egusphere-egu25-1901, 2025.

EGU25-1955 | Posters on site | CL4.15

Characterizing the local and global climatic factors associated with vegetation dynamics in the karst region of southwest China 

Azfar Hussain, Jianhua Cao, Haider Abbas, Ishtiaq Hussain, Jinxing Zhou, Hui Yang, Abolfazl Rezaei, Qukan Luo, Waheed Ullah, and Zhong Liang

Understanding the relationship between vegetation and climatic drivers is essential for assessing terrestrial ecosystem patterns and managing future vegetation dynamics. This study examines the effects of local climatic factors and remote large-scale ocean–atmosphere circulations from the Pacific, Atlantic, and Arctic Oceans, as well as the East Asian and Indian summer monsoons, on the spatiotemporal variability of the Normalized Difference Vegetation Index (NDVI) in the karst region of southwest China (KRSC) using Mann-Kendall test, Sen’s slope, cross-correlation, and wavelet analysis. We observed a significant increase in NDVI over karst and non-karst regions from 1981 to 2019, with a notable abrupt shift from 2001 onwards, underscoring the importance of understanding the underlying drivers. The significant correlation and coherence of surface air (TMP) and soil temperatures (ST) with NDVI, especially when analyzed using wavelet methods, indicate their crucial role in vegetation dynamics. Additionally, the broad coherence patterns of AMO and WHWP with NDVI at annual and decadal cycles suggest that ocean–atmosphere interactions also play a significant part. At interannual periodicities, most large-scale indices displayed significant coherence with NDVI. These findings highlight the complexity of NDVI variability, which is better explained by the integration of multiple local and global factors rather than by single variables. The integrated local–global drivers, particularly TMP-ST-AMO-NP-WHWP and PCP-SM-AMO-NP-WHWP, with mean coherence of 0.90 and 0.89, respectively, showed the highest mean coherence, emphasizing the need for a multifaceted approach in understanding vegetation changes rather than a single local variable or atmospheric circulation index. These findings have significant implications for policy-makers, aiding in better planning and policy formulations considering climate change and atmospheric variability.

How to cite: Hussain, A., Cao, J., Abbas, H., Hussain, I., Zhou, J., Yang, H., Rezaei, A., Luo, Q., Ullah, W., and Liang, Z.: Characterizing the local and global climatic factors associated with vegetation dynamics in the karst region of southwest China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1955, https://doi.org/10.5194/egusphere-egu25-1955, 2025.

Eurasia is a sensitive and high-risk region for global climate changes, where climate anomalies significantly influence natural ecosystems, human health, and economic development. The North Atlantic tripole (NAT) sea surface temperature anomaly is crucial to interannual precipitation variations in Eurasia. Several studies have focused on the link between the NAT and climate anomalies in winter and spring. However, the mechanism by which the summer NAT impacts climate anomalies in Eurasia remains unclear. This study examines how the NAT impacts interannual variations of summer precipitation in mid–high-latitude Eurasia. Precipitation variations are associated with the atmospheric teleconnection triggered by the NAT. When the NAT is in its positive phase, the anomalous atmospheric diabatic heating over the North Atlantic excites an equivalent-barotropic Rossby wave train response that propagates eastward toward Eurasia, resulting in atmospheric circulation anomalies over the region. The combined effects of atmospheric circulation, radiative forcing, and water vapor transport anomalies lead to decreased precipitation across northern Europe and central Eurasia, with higher precipitation anomalies over northeast Asia. Finally, numerical experiments verify that the summer NAT excites atmospheric teleconnections propagating downstream, affecting precipitation anomalies in mid–high-latitude Eurasia. This study provides a scientific basis for predicting Eurasian summer precipitation and strengthening disaster management strategies.

How to cite: shangling, C. and haipeng, Y.: Impact of Summer North Atlantic Sea Surface Temperature Tripole on Precipitation over Mid–High-Latitude Eurasia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2349, https://doi.org/10.5194/egusphere-egu25-2349, 2025.

Under the backdrop of global warming, heat events have become increasingly frequent and have garnered significant attention.  Northwest China, situated in the drylands of central Eurasia, exhibits a climate and ecological environment that is particularly vulnerable to global warming compared to other regions.  Over the past few decades, the frequency of heat waves in Northwest China has markedly increased, yet their underlying causes remain unclear.  Our research indicates that heat events in Northwest China are closely associated with the Silk Road teleconnection Pattern (SRP), where the occurrence of heat waves frequently corresponds to the strongly positive phase of SRP.  Furthermore, using the Linear baroclinic model, we determined that the wave source of SRP originates from the North Atlantic Ocean.  To explore the possible mechanism, we selected an extreme heat event in Northwest China in 2021 as a typical case study.  The regressed circulation fields to daily SRP were highly consistent with the anomalies observed during July 9–22, 2021, suggesting that the diurnal propagation of SRP modulates the circulation anomaly associated with the heat wave event.  Diabatic heating influenced by SRP was identified as the primary factor contributing to the thermal low over Northwest China.  Specifically, diabatic heating in the lower troposphere was intensified due to enhanced downward shortwave radiation and surface sensible heat flux, accompanied by strong descending motions and reduced cloud cover induced by an anticyclone guided by SRP over Northwest China.  This study enhances our understanding and confidence regarding the effects of large-scale circulation on local temperature anomalies in mid-latitudes.

How to cite: Zhou, J. and Yu, H.: Extreme heat event over Northwest China driven by Silk Road Pattern and its possible mechanism , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2359, https://doi.org/10.5194/egusphere-egu25-2359, 2025.

EGU25-2653 | Orals | CL4.15

QBO modulation of MJO teleconnections in the North Pacific 

seok-woo son, Min-Jee Kang, and Hera Kim

This study examines the influence of the Quasi-Biennial Oscillation (QBO) on the Madden-Julian Oscillation (MJO) teleconnections in the North Pacific using ERA5 data. It is found that the Rossby wave trains induced by MJO phase 6–7 exhibit greater strength and robustness during the westerly QBO winter (WQBO) than during the easterly QBO winter (EQBO), although the MJO itself is weaker during the former. This counter-intuitive dependency of MJO teleconnections on the QBO is attributed to the preexisting MJO teleconnections prior to the MJO phase 6–7. The MJO phase 6–7 is more frequently preceded by stronger MJO phase 3–4 during the EQBO than during the WQBO. The preceding MJO phase 3–4 teleconnections, which have opposed signs to the MJO phase 6–7 teleconnections, result in a considerable attenuation of the MJO phase 6–7 teleconnections by destructive interference. This result is supported by linear model experiments. The subseasonal-to-seasonal prediction models also indicate improved prediction skills of MJO phase 6–7 teleconnections during the WQBO compared to the EQBO. These results suggest that enhanced MJO activities during the EQBO do not necessarily result in stronger and more robust MJO teleconnections in the North Pacific.

How to cite: son, S., Kang, M.-J., and Kim, H.: QBO modulation of MJO teleconnections in the North Pacific, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2653, https://doi.org/10.5194/egusphere-egu25-2653, 2025.

The weakening of the Atlantic Meridional Overturning Circulation (AMOC) leads to a distinct horseshoe pattern of colder sea surface temperatures (SST) anomalies in the North Atlantic as found in many modeling studies. This SST horseshoe pattern is a characteristic feature of the Atlantic extratropical-tropical teleconnection leading to the tropical atmospheric response associated with the AMOC weakening, such as the southward shift of the Atlantic Intertropical Convergence Zone (ITCZ). A similar SST horseshoe pattern associated with the Atlantic Multidecadal variability (AMV) has also been observed in modern climate, with the SST anomalies propagating from the extratropical North Atlantic into the tropical North Atlantic along the horseshoe pathway. Despite its importance, the mechanisms of the Atlantic extratropical-tropical teleconnection associated with the AMOC weakening remain poorly understood. Previous studies suggest the Wind-Evaporation-SST (WES) feedback as a plausible mechanism. Here, we conduct water hosing experiments using a high-resolution fully coupled climate model to elucidate the mechanisms responsible for the Atlantic extratropical-tropical teleconnection associated with the AMOC weakening. Our analysis, focusing on boreal summer, suggests that the WES feedback is not the primary mechanism for the Atlantic extratropical-tropical teleconnection. By examining the transient response as the AMOC weakens, we identify the key mechanisms responsible and reveal the important role of the oceanic and atmospheric circulations involved in the SST horseshoe pattern formation. We also illustrate how the relative importance of the oceanic and atmospheric processes in the Atlantic extratropical-tropical teleconnection changes under different amplitudes of the freshwater forcing applied in the water hosing experiments. The mechanisms of the Atlantic extratropical-tropical teleconnection are crucial for the development of the tropical atmospheric response associated with the AMOC weakening (e.g. the southward shift of the Atlantic ITCZ).

How to cite: Joshi, R. and Zhang, R.: On the Atlantic extratropical-tropical teleconnection in response to external freshwater forcing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3376, https://doi.org/10.5194/egusphere-egu25-3376, 2025.

EGU25-4983 | ECS | Posters on site | CL4.15

Silk Road Pattern on the Intraseasonal Time Scale 

Qianting Yuan and Riyu Lu

Based on reanalysis data from 1968 to 2021, this study investigates the characteristics of Silk Road Pattern (SRP), a teleconnection pattern embedded in the Asian jet during summer, on the intraseasonal timescale. Results showed that the 10–30-day oscillations are the main component of SRP intraseasonal variability. The results of correlation for the base points along the jet axis indicate that the SRP on the 10–30-day timescale, hereafter referred to as the Bi-weekly Silk Road Pattern Oscillation (BSRP), is characterized by 3 alternatively-signed cells of 200-hPa meridional wind anomalies. The teleconnection patterns are highly consistent, no matter with the location of base points, suggesting that the BSRP is not geographically phase-locked, i.e., the BSRP has no preferred locations in the zonal direction, which is quite different with the SRP on the interannual timescale. Therefore, we “merge” the teleconnection patterns for the various base points into a composite pattern, and analyze the composite pattern to highlight the common features. The analyzed results demonstrate that the BSRP propagates eastwards of, and the speed of energy dispersion is estimated to be approximately 25° per day. In addition, the SRP obtains energy from the basic flows through the baroclinic energy conversion. On the other hand, barotropic energy conversion is weak and shows little variation with the change of longitude, failing to contribute to phase locking. Finally, we also explored the climatic impact of BSRP and found that the BSRP can induce remarkable precipitation and temperature anomalies.

How to cite: Yuan, Q. and Lu, R.: Silk Road Pattern on the Intraseasonal Time Scale, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4983, https://doi.org/10.5194/egusphere-egu25-4983, 2025.

The summer North Atlantic Oscillation (SNAO) has been shown to exert a significant influence on downstream climate anomalies, primarily via the Silk Road teleconnection pattern (SRP). However, the linkage between the SNAO and the SRP is not consistently robust, and the SNAO does not invariably excite the SRP. The SRP itself is an upper-tropospheric teleconnection pattern traveling along the midlatitude Asian westerly jet, characterized by alternating southerly and northerly wind anomalies. In this study, we focus on the considerable variability of the SNAO’s southern branch and categorize the interannual SNAO–SRP relationship into two categories: a strongly linked category and a weakly linked category. Our results indicate that, under the strongly linked category, the SNAO’s southern branch retracts westward toward the Baltic Sea, whereas under the weakly linked category, it extends eastward beyond the Ural Mountains. When the southern branch retracts westward, a pronounced negative precipitation anomaly over Europe induces upper-level convergence, producing a strong positive Rossby wave source (RWS) anomaly, which effectively excites the downstream SRP wave train. In contrast, when the southern branch extends eastward, this process does not hold. These findings link the morphology of the SNAO to its capability to initiate the SRP, offering new insights into how the SNAO exerts remote impacts.

How to cite: Yuanxin, G., Riyu, L., and Xiaowei, H.: What type of summer North Atlantic Oscillation will trigger the downstream Silk Road teleconnection pattern, and how?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5054, https://doi.org/10.5194/egusphere-egu25-5054, 2025.

The Pacific Northwest experienced a record-breaking heatwave during the summer of 2021, resulting in significant adverse effects on both human society and ecosystems. This event was so extreme and shattered previous temperature records by an astounding 5 ℃, highlighting the need for a comprehensive understanding of the underlying physical mechanisms. In this study, we employ a hierarchical approach with increasing complexity to demonstrate that the Asian summer monsoon, when accounting for all relevant convective activities, contributed to suppressing the intensity of this event. Without the variability of the Asian summer monsoon, the heatwave's amplitude is estimated to be approximately 0.4°C (3%-4%) greater than the already extraordinary observed amplitude. Since this extreme event occurred against a context of imperfect synchronization among climate systems, it serves as a warning that even more intense heatwave is likely to occur in the future even if global warming remains at current levels.

How to cite: Xu, P.: The 2021 Pacific Northwest heatwave would have been more severe without the influence of Asian summer monsoon, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5081, https://doi.org/10.5194/egusphere-egu25-5081, 2025.

EGU25-5192 | Posters on site | CL4.15

Epoch-based Sea Surface Temperature for Climate System Analysis 

Robert Grumbine

Taking the principle that climate is what one expects, I suggest and illustrate with Sea Surface Temperature (SST) that it is desirable to represent the climatology as linear in time with the first few (3, it turns out) harmonics of the annual cycle. In many regions of the globe the trend is physically and statistically significant. We also expect the seasonal cycle to continue, though amplitude and phase of the harmonics do change — themselves matters of direct interest in climatology. In representing the SST climatology this way, rather than the common average over each month or for each day independently, the approach is similar to how slowly varying terms in astronomy, such as the earth’s eccentricity, are represented by an Epoch (date for time 0) and adjustments for secular changes while moving away in time.  

The Epoch-based climatology approach is shown in comparison to the traditional by developing a 30 year climatology for each and examining the departure from each climatology of the next 10 years observations. The Epoch climatology has markedly reduced anomalies compared to the traditional. A further comparison is to examine the autocorrelation of the anomalies in time. The traditional climatology has inflated times, including excess autocorrelation at annual time scale, meaning that there were things we could and should expect but which are not captured by that approach.

How to cite: Grumbine, R.: Epoch-based Sea Surface Temperature for Climate System Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5192, https://doi.org/10.5194/egusphere-egu25-5192, 2025.

EGU25-5659 | ECS | Posters on site | CL4.15

StoryPy: A Python-based package to compute climate storylines 

Richard Alawode, Julia Mindlin, and Marlene Kretschmer

Dynamical storylines explore qualitatively different changes in climate driven by forced responses
in large-scale remote drivers, such as Arctic Amplification, tropical amplification, and the stratospheric
polar vortex. This approach helps address uncertainties in regional climate responses by using physical
understanding to link large-scale thermodynamic and dynamic climate responses to regional impacts and
present a small set of projections in a conditional way. By contextualizing events within broader climate
patterns, dynamical storylines aim to deepen understanding of the uncertainties associated with climate
change, particularly in relation to polar, tropical, and global warming.


Our project aims to make this advanced methodology accessible to a broader audience through a
user-friendly Python package and an intuitive interface. Our package, termed StoryPy, provides
a set of functions to analyze multi-model ensembles by focusing on the identification of dynamical
storylines. With customizable options for selecting remote drivers, target seasons, and climate variables
or climatic-impact drivers, the StoryPy provides flexibility and adaptability for various research
and policy applications. In this work we show the usability of the tool by applying it to the case of the
Mediterranean region and analyze regional climate uncertainty associated with drivers including Arctic
Amplification and the Stratospheric polar vortex.


By facilitating the technical complexity of identifying coherent narratives that bridge the gap between
complex climate dynamics and specific, actionable impacts, our hope is that in the long-run this tools
helps to facilitate dialogue among scientists, policymakers, and diverse stakeholder communities.

How to cite: Alawode, R., Mindlin, J., and Kretschmer, M.: StoryPy: A Python-based package to compute climate storylines, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5659, https://doi.org/10.5194/egusphere-egu25-5659, 2025.

EGU25-5732 | ECS | Posters on site | CL4.15

Diverse Response of Western North Pacific Anticyclone to Fast-Decay El Niño During Decaying Summer 

Leishan Jiang, Han-Ching Chen, Tim Li, and Lin Chen

Previous studies suggested that fast-decay El Niño events are more favorable in generating the western North Pacific anticyclone (WNPAC) in the decaying summer. However, we found that this is not the case for all fast-decay El Niño events. By comparing two groups of fast-decay El Niño events with significant and insignificant WNPAC in the following summer, we found that the westward extension of the equatorial Pacific cold sea surface temperature anomalies (SSTA) and the subtropical central-north Pacific cold SSTA play important roles in the generation and intensification of the WNPAC during decaying summer. Further analyses indicated that the internal atmospheric mode—North Pacific Oscillation during boreal spring can affect the formation of the cold SSTA over the subtropical central-north Pacific and the westward extension of the equatorial Pacific cold SSTA during summer. Additional effects of tropical Indian and Atlantic forcing on the maintenance of the WNPAC are also shown.

How to cite: Jiang, L., Chen, H.-C., Li, T., and Chen, L.: Diverse Response of Western North Pacific Anticyclone to Fast-Decay El Niño During Decaying Summer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5732, https://doi.org/10.5194/egusphere-egu25-5732, 2025.

The equatorial Atlantic (EA) sea surface temperature anomalies (SSTA) exhibit significant interannual variability, typically peaking during the boreal summer months of May to August. In this study, we utilize an extended recharge-discharge oscillator (RO) model, considering both coupled Atlantic ocean-atmosphere interactions and the remote influence of Pacific ENSO forcing, to explore the dynamics of EA SSTA seasonality. Our results demonstrate that this extended RO model captures the temporal characteristics of EA SSTA well, especially its seasonal variation. Further analysis suggests that the seasonality of EA SSTA is primarily governed by the seasonal modulation of the EA SSTA growth rate, characterized by a robust seasonal cycle transitioning from positive to negative during boreal summer. In contrast, the EA SSTA phase transition rate and the ENSO forcing coefficient contribute relatively little to the seasonal preference of EA SSTA. In most climate models, EA SSTA also shows a tendency to peak during the boreal summer; however, the seasonal preference is significantly weaker compared to observations. This weaker preference in climate models primarily results from the smaller contribution of the EA SSTA growth rate, which is mainly due to the lower (more negative) annual mean of the growth rate and secondarily due to the weaker seasonal cycle amplitude of the growth rate.

How to cite: Chen, H.-C., Cai, Z., Ge, W., and Jiang, L.: Exploring the Seasonal Characteristics of the Equatorial Atlantic SSTA: Insights from an Extended Recharge-Discharge Oscillator Framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7889, https://doi.org/10.5194/egusphere-egu25-7889, 2025.

Teleconnections are crucial in shaping climate variability and regional climate change. The fidelity of teleconnections in climate models is important for reliable climate projections. As the observed sample size is limited, scientific judgment is required when models disagree with observed teleconnections. We illustrate this using the example of the relationship between El Ni.o‐Southern Oscillation (ENSO) and the northern stratospheric polar vortex (SPV), where the MIROC6 large ensemble exhibits an ENSO‐SPV correlation opposite in sign to observations. Yet the model well captures the upward planetary‐wave propagation pathway through which ENSO is known to affect the SPV. We show that the discrepancy arises from the model showing an additional linkage related to horizontal stratospheric wave propagation. Observations do not provide strong statistical evidence for or against the existence of this linkage. Thus, depending on the research purpose, a choice has to be made in how to use the model simulations. Under the assumption that the additional linkage is spurious, a physically‐based bias adjustment is applied to the SPV, which effectively aligns the modeled ENSO-SPV relationship with the observations, and thereby removes the model‐observations discrepancy in the surface air temperature response. However, if one believed that the additional linkage was genuine and was undersampled in the observations, a different approach could be taken. Our study emphasizes that caution is needed when concluding that a model is not suitable for studying teleconnections. We propose a forensic approach and argue that it helps to better understand model performance and utilize climate model data more effectively.

How to cite: Shen, X., Kretschmer, M., and Shepherd, T. G.: A Forensic Investigation of Climate Model Biases inTeleconnections: The Case of the Relationship BetweenENSO and the Northern Stratospheric Polar Vortex, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9462, https://doi.org/10.5194/egusphere-egu25-9462, 2025.

Probabilistic lagged dependence (ranging from months to seasons) between atmospheric-oceanic variables, comes essentially from their linear and nonlinear statistical multivariate correlations. A new technique is presented to estimate the posterior conditional pdf of a scalar predictand y(t+lag) at lag tau, knowing a vector of predictor climatic indices X(t), taken at time t. For that, we apply a variant of the Kernel Canonical Correlation Analysis (KCCA) linking extended feature vectors f(Y) and g(X), filled with nonlinear and mixing functions (e.g. monomials, component products). The issued, leading canonical component pair (u,v) is then used to estimate the copula between X and Y, estimated as the Gaussian copula between Gaussian-anamorphed components ug, vg of u,v respectively. This copula works as a maximum-entropy copula, maximizing the Gaussian correlation Cor-g (Pearson correlation between ug, vg), captured by the feature vectors, and also maximizing the part  -0.5*log(1-cor-g^2) of the mutual information (MI) between X and Y. Moreover, Cor-g is much more outlier-resistant than the Pearson correlation. The above method is applied in two cases: 1) Y being a climatic index, (e.g. El-Niño index with lags tau in the range 0-48 months) and 2) Y being the local monthly temperature or precipitation for lags of 1-2 months. In both cases, X is taken as a set of climatic indices from the pool: El-Niño, NAO, AMO, PDO, IOD; QBO, TNA, TSA, SCAND, WE, EA-WR. The Gaussian-copula model improves the forecast of extreme situations, even beyond 1-2 standard deviations, providing a way of exploring probabilistic nonlinear forecasts and nonlinear lagged teleconnections. This work is supported by the Portuguese Fundação para a Ciência e Tecnologia, FCT, I.P./MCTES through national funds (PIDDAC): UID/50019/2025 and LA/P/0068/2020 https://doi.org/10.54499/LA/P/0068/2020).

How to cite: Pires, C., Hannachi, A., and Vannitsem, S.: Estimation of probabilistic copulas from nonlinear correlations: Application to lagged teleconnections and monthly atmospheric forecasting., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11798, https://doi.org/10.5194/egusphere-egu25-11798, 2025.

EGU25-13940 | ECS | Posters on site | CL4.15

Creating a Database of Climate Extremes and Variability in Polar Ice Cores 

Brooke M. Chase, Tyler R. Jones, Bradley R. Markle, Valerie Morris, Rhys-Jasper León, Kevin S. Rozmiarek, Ella H. Johnson, Adira Lunken, Tirso Jesús Lara Rivas, and Bruce H. Vaughn

Prior results from EGRIP (East Greenland Icesheet Project ice core) indicate that interannual-to-decadal variability in water isotopes lead abrupt Dansgaard-Oeschger event (D-O Events) warming by hundreds of years. As part of the U.S. National Science Foundation funded “Beyond Mean Climate” project, GISP2 (Greenland Ice Sheet Project 2 ice core) is being resampled at the NSF-Ice Core Facility and reanalyzed for high resolution water isotope measurements at INSTAAR, University of Colorado. GISP2 gives us the chance to verify those results from EGRIP and test whether the lead-lag may result from firn processes and diffusion, or from regional climate dynamics. Additionally, for part of this project we are creating a statistical database of climate variability and extremes in multiple Greenland and Antarctic ice cores. This database will include GISP2 and existing records of high-resolution water isotopes and impurities. The initial statistical database of climate indicators will include the mean, standard deviation, extreme values using the tail ends of probability distributions, and spectral analysis to determine the average amplitude in a given frequency band. We will present initial results on the first section of processed data from GISP2, as well as results from WDC (West Antarctic Ice Sheet Divide ice core), SPC (South Pole ice core), and EGRIP (East Greenland Icesheet Project ice core). In particular, we will focus on how the strength of interannual-to-decadal variability is different across geographies (Greenland, Antarctica, interhemispheric), analyze lead-lag between mean temperature and variability (e.g. for D-O Events in Greenland and their Antarctic counterparts, Antarctic Isotope Maxima (AIM) Events), and compare results across the deglaciation.

How to cite: Chase, B. M., Jones, T. R., Markle, B. R., Morris, V., León, R.-J., Rozmiarek, K. S., Johnson, E. H., Lunken, A., Rivas, T. J. L., and Vaughn, B. H.: Creating a Database of Climate Extremes and Variability in Polar Ice Cores, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13940, https://doi.org/10.5194/egusphere-egu25-13940, 2025.

EGU25-16218 | Orals | CL4.15

Observed global response of ocean stratification to climatic forcing 

Raquel Somavilla, Alberto Naveira-Garabato, Cesar González-Pola, Julio M. Fernández-Diaz, and Ignasi Vallès

The global ocean plays a pivotal role in climate by taking up, storing and redistributing vast amounts of heat, carbon and other tracers. A fundamental factor shaping this role is the ocean’s stratification, which accounts for the resistance of a water column to be mixed vertically. As such, stratification modulates the transfer of climatically important properties (e.g., heat, carbon, oxygen and nutrients) between deeper oceanic layers and near-surface waters, which are in frequent contact with the atmosphere and may thus interact with the rest of the climate system.

It has traditionally been assumed that beyond the deepest extent of surface mixing in winter, ocean stratification remains approximately constant or evolves very slowly on the interannual and longer time scales of pertinence to contemporary climate variability – comprising both internal and anthropogenic changes imprinted on the historical record. As a result, most research efforts to document or understand ocean stratification and its climatic function have, to date, primarily focused on near-surface waters. Deeper in the water column, little is known about the extent to (or time scales over) which the stratification of the main pycnocline, extending to depths in excess of 1000 m, is influenced by climate variability.

Here, we test this view by performing the first global-scale, systematic investigation of the spatio-temporal variability of ocean stratification from the surface to the main pycnocline, using 20 years (2003-2022) of data from the Argo float array. We demonstrate that deep-ocean stratification varies significantly with well-defined spatio-temporal patterns. Both near-surface and main pycnocline stratifications are found to exhibit spatially-structured, vertically-coherent, global-scale variations on seasonal-to-decadal time scales, unveiling a new view of ocean stratification from surface to depth as a rapidly-evolving, readily-interactive element of the climate system. Variability in stratification is organized into well-defined patterns that replicate the spatial footprints and time scales of major climate modes such as the El Niño – Southern Oscillation, pointing to these modes of internal variability as important drivers of stratification changes. Our diagnosed patterns and forcings of stratification variability provide an important benchmark for advancing the climate models used to understand and predict the ongoing climate change.

How to cite: Somavilla, R., Naveira-Garabato, A., González-Pola, C., Fernández-Diaz, J. M., and Vallès, I.: Observed global response of ocean stratification to climatic forcing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16218, https://doi.org/10.5194/egusphere-egu25-16218, 2025.

EGU25-18859 | ECS | Orals | CL4.15

Tropical Teleconnections with Summer Temperature Anomalies in the Eastern Mediterranean 

Elizur Berkovitch, Chaim Garfinkel, and Assaf Hochman

The warming trend in the Eastern Mediterranean summer is faster than the global average. Climate projections indicate that this accelerated summer warming will persist in the coming decades. As the region continues to warm, the likelihood of summer months with extreme temperatures will increase, posing significant societal challenges. Understanding the mechanisms driving summer temperatures in the region is crucial for improving regional climate projections and medium-range weather predictability. This study explores the potential link between the African Monsoon and Eastern Mediterranean summer temperatures. ERA5 reanalysis data, at 0.25° horizontal resolution, were analyzed to examine correlations between the two regions and identify possible connecting mechanisms. Additionally, simulations from the Large Ensemble Single Forcing Model Intercomparison Project (LESFMIP) were utilized to isolate potential explanations for the teleconnection. These simulations also demonstrate that this link exists on both decadal and monthly scales. A significant correlation was identified between Sahel Monsoon activity and Eastern Mediterranean summer temperatures. Wetter summer months in the Sahel were associated with warmer conditions in the Eastern Mediterranean. The dynamic patterns observed during warm summers in the Eastern Mediterranean resemble those during anomalously wet Sahel summers. A poleward shift of the Saharan Heat Low, linked to increased Sahel precipitation, appears to drive circulation changes associated with warmer Eastern Mediterranean summers. Several proposed mechanisms could explain this link, although their validity requires further investigation. Understanding this correlation could enhance regional climate change projections and improve medium-range predictions of extreme weather events in both the Sahel and the Eastern Mediterranean.

How to cite: Berkovitch, E., Garfinkel, C., and Hochman, A.: Tropical Teleconnections with Summer Temperature Anomalies in the Eastern Mediterranean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18859, https://doi.org/10.5194/egusphere-egu25-18859, 2025.

EGU25-18886 | ECS | Orals | CL4.15

Disentangling reduced representations of teleconnections using variational autoencoders 

Fiona Spuler, Marlene Kretschmer, Magdalena Alonso Balmaseda, Yevgeniya Kovalchuk, and Theodore G. Shepherd

Studying teleconnections using data-driven methods relies on identifying suitable representations of the relevant dynamical processes involved. Often, these representations are identified through a dimensionality reduction of the dynamical process itself, such as the Niño3.4 index to represent the El-Niño Southern Oscillation or the clustering of circulation regimes to represent states of the North Atlantic eddy-driven jet. The relationship between these representations can subsequently be assessed in a causal model. However, since these representations are identified independently of the teleconnection studied, they do not necessarily capture the dynamical processes relevant for explaining the relationship between the two phenomena. Here, we present a regularised dimensionality reduction approach using variational autoencoders, a deep generative machine learning method, to identify reduced representations of large-scale processes and their teleconnections jointly in a causal framework. Applying the approach to study regional dynamical drivers of precipitation extremes over Morocco at subseasonal lead times, we show that the method is able to identify a representation of the circulation over the North Atlantic, which disentangles the drivers of precipitation over Morocco while maintaining its subseasonal predictability and physical interpretability. Furthermore, we demonstrate the ability of the approach to disentangle large-scale teleconnections at longer lead times.

How to cite: Spuler, F., Kretschmer, M., Balmaseda, M. A., Kovalchuk, Y., and Shepherd, T. G.: Disentangling reduced representations of teleconnections using variational autoencoders, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18886, https://doi.org/10.5194/egusphere-egu25-18886, 2025.

EGU25-846 | ECS | Orals | AS1.38

Elevational dependency of precipitation climatology and trends in global mountains: a model view 

Olivia Ferguglia, Elisa Palazzi, and Enrico Arnone

High-altitude regions have been identified as hotspots of climate change. In particular, the dependence of warming rates on elevation, known as Elevation-Dependent Warming (EDW), has been extensively discussed in the literature. Recently, the focus has expanded to the broader concept of Elevation-Dependent Climate Change (EDCC), with attention to precipitation and its extremes, given their importance for mountain hydrological resources and their role in triggering geo-hydrological hazards. Recent studies have investigated the elevational stratification of precipitation in  in-situ observations and reanalysis datasets, showing a lack of uniform patterns of EDCC across the world, which point to the need for common methodologies and insight in the driving mechanisms. In this study, we extend results we obtained with the ERA5 reanalysis to CMIP6 global climate models, and study EDCC in key mountain regions of the world: Tibetan Plateau, the US Rocky Mountains, the Greater Alpine Region, and the Andes. We focus on precipitation and its extremes, assessing the ability of the models  to reproduce historical patterns of stratification by comparison with ERA5 reanalysis data and other observation-based gridded datasets. We also explore how the stratification in other key climate variables, such as cloud cover, humidity, besides temperature, influence the elevational patterns of precipitation and precipitation extremes and their trends. Our analysis aims to determine whether the observed elevation-dependent precipitation patterns are primarily driven by dynamical, thermodynamical, or microphysical processes, identifying seasonal variations and the specific precipitation type (i.e., stratiform vs convective)  mostly affected. Particular attention is given to the role of the model spatial resolution, including regional climate models in a case study analysis over the Greater Alpine Region.

How to cite: Ferguglia, O., Palazzi, E., and Arnone, E.: Elevational dependency of precipitation climatology and trends in global mountains: a model view, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-846, https://doi.org/10.5194/egusphere-egu25-846, 2025.

Orographic interactions of intense western disturbances (WDs) with western Himalayan (WH) topography often drive persistent extreme precipitation events (EPEs) in the region during the winter season, contributing to significant socio-economic losses. Accurate predictions of such events remain challenging due to the sparse gauge network and complex multi-scale interactions of dynamical and microphysical processes with the region’s heterogenous orography. Numerical weather prediction models, such as the Weather Research and Forecasting (WRF) model, are widely utilized tools for simulating extreme precipitation with high-resolution and physically informed configurations. Kilometer-scale convection-permitting hold potential for improved representation of sub-grid processes, such as orographic effects and land-surface interactions, thus offering more scope for enhancing predictability. The present study investigates the predictability of intense WD-associated EPEs using convection-permitting (3 km) dynamically downscaled WRF simulations and a multi-physics ensemble (ENSM) approach, initialized using ERA5 reanalysis and validated with high resolution IMDAA (12 km) regional reanalysis. Ten persistent EPEs (lasting 3 or more consecutive days) were analyzed to assess sensitivity to sea surface temperature (SST) forcings and eight microphysical parameterization (MP) schemes (Single-moment: WSM7, Thompson8; Double-moment: WDM7, Thompson28, Morrison, P3). The findings reveal minimal variations from SST forcings at 3–4-day time scales, highlighting the dominant role of atmospheric processes at shorter time scales during winter EPEs. Both single- and double-moment MPs exhibited comparable performance, with minor spatial variations. The ENSM demonstrated enhanced prediction skill (>0.6) and accurately captured precipitation characteristics, including diurnal variations and dynamics like atmospheric baroclinicity, vertical wind shear, and stability driven by meridional temperature gradients. Overall, the findings underscore the potential of a convection-permitting multi-physics ensemble frameworks in enhancing the predictability of extreme winter precipitation over the orographic WH region.

Keywords: Convection-Permitting Simulations, WRF Model, Mountain Precipitation Extremes, Prediction, Microphysical Parameterization

How to cite: Sharma, N. and Attada, R.: Enhanced Predictability of Himalayan Orographic Precipitation Extremes Using a Kilometer-Scale Convection-Permitting Multi-Physics Ensemble, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1058, https://doi.org/10.5194/egusphere-egu25-1058, 2025.

EGU25-1443 | ECS | Orals | AS1.38

Quantifying processes of winter daytime and nighttime warming over the Tibetan Plateau 

Fangying Wu, Qinglong You, and Nick Pepin

The Tibetan Plateau (TP) has experienced accelerated warming in recent decades, especially in winter. However, a comprehensive quantitative study of its long-term warming processes during daytime and nighttime is lacking. This study quantifies the different processes driving the acceleration of winter daytime and nighttime warming over the TP during 1961-2022 using surface energy budget analysis. The results show that the surface warming over the TP is mainly controlled by two processes: a) a decrease in snow cover leading to a decrease in albedo and an increase in net downward shortwave radiation (snow-albedo feedback), and b) a warming in tropospheric temperature (850-200 hPa) leading to an increase in downward longwave radiation (air warming-longwave radiation effect). The latter has a greater impact on the spatial distribution of warming than the former, and both factors jointly influence the elevation dependent warming pattern. Snow-albedo feedback is the primary factor in daytime warming over the monsoon region, contributing to about 59% of the simulated warming trend. In contrast, nighttime warming over the monsoon region and daytime/nighttime warming in the westerly region are primarily caused by the air warming-longwave radiation effect, contributing up to 67% of the simulated warming trend. The trend in the near-surface temperature mirrors that of the surface temperature, and the same process can explain changes in both. However, there are some differences: an increase in sensible heat flux is driven by a rise in the ground-atmosphere temperature difference. The increase in latent heat flux is associated with enhanced evaporation due to increased soil temperature and is also controlled by soil moisture. Both of these processes regulate the temperature difference between ground and near-surface atmosphere.

How to cite: Wu, F., You, Q., and Pepin, N.: Quantifying processes of winter daytime and nighttime warming over the Tibetan Plateau, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1443, https://doi.org/10.5194/egusphere-egu25-1443, 2025.

EGU25-2606 | ECS | Orals | AS1.38

Sources of temperature biases in Regional Climate Models over complex orography: a general approach 

Francesca Zarabara and Dario Giaiotti

Amid the alarming pace and effects of human-induced climate change, mountainous regions are warming at about twice the global average rate. Modeling climate and climate change scenarios over regions with highly complex topography, such as the Alps, remains a significant challenge for regional climate modeling. Better characterizing the sources of model biases is a major issue, particularly in areas with complex terrain.

We analyze the sources of bias affecting near-surface temperature (TAS) in an ensemble of EURO-CORDEX models, focusing on the Friulian Alps. By examining the vertical structure of atmospheric thermal profiles, we identify and quantify four main sources that contribute to surface temperature biases at specific locations or grid points.

  • The first source is related to the ensemble's ability to reproduce free-atmosphere temperatures, such as those at the 500 hPa level.

  • The second component accounts for the biased representation of the thermal gradient between the free-atmosphere and the boundary layer top.

  • The third component is associated with model errors in the height of the boundary layer top. Under the environmental lapse rate approximation, this component corresponds to the orographic bias at a station or grid point. In the mountainous region we examined, the orographic bias represents a significant source of error.

  • The final contribution to the TAS bias stems from the inadequate representation of processes within the boundary layer, which exhibit temporal and spatial variability depending on the type of mountain boundary layer.

We provide seasonal and annual estimates for each TAS bias component and suggest that advanced statistical bias correction techniques, including machine learning approaches, may be particularly effective in addressing the specific challenges posed by the boundary-layer-dependent component of the overall TAS bias.

 

 

How to cite: Zarabara, F. and Giaiotti, D.: Sources of temperature biases in Regional Climate Models over complex orography: a general approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2606, https://doi.org/10.5194/egusphere-egu25-2606, 2025.

EGU25-2940 | ECS | Orals | AS1.38

Simulating the submesoscale rotating structures in the bora wind 

Petar Golem, Hrvoje Kozmar, Željko Večenaj, and Branko Grisogono

Wind speed within bora (downslope windstorm) events at the northern Adriatic coast is often found to be “pulsating” in a quasi-periodic manner with a period of a few minutes. In an earlier work, the characteristic horizontal rotational motion of these pulsations at the town of Senj, Croatia was studied using tower measurements. In the present work this analysis is extended to a larger domain using a hectometer-scale numerical simulation (WRF-ARW) of a summer bora event. The model successfully reproduced the rotational motion at the position of the tower: the near-ground wind velocity vector within the band of periods between 3 and 11 min traces out a highly elongated ellipse in the counterclockwise direction, its major axis aligned with the shear vector at the top of the leeside low-level jet. The pulsations are associated with Kelvin-Helmholtz instability between the low-level jet and the stagnation zone. The most interesting finding is that the predominant rotation direction over the rest of the domain, especially over the sea, depends strongly on directional shear within the low-level jet, i.e., which direction the wind turns with height. It is argued that the cause of the predominant rotation direction is deformation of the laterally unstable Kelvin-Helmholtz billows by the directional shear.

How to cite: Golem, P., Kozmar, H., Večenaj, Ž., and Grisogono, B.: Simulating the submesoscale rotating structures in the bora wind, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2940, https://doi.org/10.5194/egusphere-egu25-2940, 2025.

EGU25-3039 | ECS | Orals | AS1.38

Strongly Heterogeneous Surface-Water Warming Trends in High Mountain Asia 

Taylor Smith and Bodo Bookhagen

High Mountain Asia has experienced significant warming in recent decades. Changes in both temperature and precipitation patterns have strongly impacted regional hydrology, including changes to glaciers, snowmelt, and river systems. Here we examine long-term (1983-2023) and high-resolution (30 m) changes in water-surface temperature over a large and topographically diverse region encompassing the world’s highest mountains. We find that water-surface temperatures have significantly increased in the vast majority of the study area -- especially in snow-covered and high-elevation regions -- with a noted acceleration over the past decade. While some of this warming can be explained by increasing regional air temperatures, we find that surface water is warming faster than nearby dry areas. We posit that modifications to snowmelt timing and volume have created strong spatial heterogeneities in surface-water warming. These impacts will be felt both directly by cold-water flora and fauna, and downstream through decreases in surface-water quality.

How to cite: Smith, T. and Bookhagen, B.: Strongly Heterogeneous Surface-Water Warming Trends in High Mountain Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3039, https://doi.org/10.5194/egusphere-egu25-3039, 2025.

Some of the rainiest regions on Earth lie upstream of tropical mountains, where the interaction of prevailing winds with orography produces frequent precipitating convection. Yet, the response of tropical orographic precipitation to the large-scale wind and temperature variations induced by anthropogenic climate change remains largely unconstrained.
Here, we quantify the sensitivity of tropical orographic precipitation to background cross-slope wind using theory, idealized simulations, and observations. We build on a recently developed theoretical framework that characterises the orographic enhancement of seasonal-mean precipitation, relative to upstream regions, as a response of convection to cooling and moistening of the lower free-troposphere by stationary orographic gravity waves. Using this framework and convection-permitting simulations, we show that higher cross-slope wind speeds deepen the penetration of the cool and moist gravity wave perturbation upstream of orography, resulting in a mean rainfall increase of 20--30% per m s-1 increase in cross-slope wind speed.
Additionally, we show that orographic precipitation in five tropical regions exhibits a similar dependence on changes in cross-slope wind at both seasonal and daily timescales. Given next-century changes in large-scale winds around tropical orography projected by global climate models, this strong scaling rate implies wind-induced changes in some of Earth's rainiest regions that are comparable with any produced directly by increases in global mean temperature and humidity. 

How to cite: Nicolas, Q. and Boos, W.: Sensitivity of tropical orographic precipitation to wind speed with implications for future projections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3810, https://doi.org/10.5194/egusphere-egu25-3810, 2025.

Parameterizations of subgrid scale mountains are commonly used in large scale numerical weather prediction and climate models. They try to represent quite separate processes: the enhancement of the turbulent drag by orography, gravity waves and low level flow blocking. Among the gravity waves some schemes eventually separate between the upward propagating waves and the trapped lee waves.  Using a recent theoretical methodology that addresses the interaction of stratified boundary layers with mountains, a theory that handles the transition from neutral to stratified dynamics and trapped waves, we propose a formalism that can include all these effects.  As in most parameterizations it separates the flow between a linear part and a blocked part.  Here  the linear part handles enhanced turbulent drag in the neutral case and gravity waves in the stratified case, trapped lee waves in the transition. In this presentation we evaluate the mountain drag associated to all these processes as well as the fraction of the drag that stays within the boundary layer instead of being radiated in the far field.  We also try to  evaluate the blocked part by combining the sheltering effects that dominate when stratification is small and the blocking effects that dominate when stratification is large.

How to cite: Lott, F., Beljaars, A., and Deremble, B.: Rationale for a subgrid scale orography parameterization that includes turbulent form drag, gravity wave drag and low level flow blocking, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4362, https://doi.org/10.5194/egusphere-egu25-4362, 2025.

EGU25-5859 | Orals | AS1.38 | Highlight

The TEAMx Observational Campaign – First findings from the winter campaign 

Manuela Lehner, Mathias W. Rotach, Ivana Stiperski, Lena Pfister, Alexander Gohm, Christophe Brun, Jutta Vüllers, Jan Cermak, Andrew Orr, Ian Renfrew, Helen F. Dacre, and Charles Chemel

TEAMx (multi-scale transport and exchange processes in the atmosphere over mountains – programme and experiment) is an international research program that aims at improving our understanding of exchange processes over complex terrain and at evaluating and improving the representation of these processes in numerical weather and climate prediction models. As part of TEAMx, a one-year long field campaign, the TEAMx Observational Campaign (TOC), started in September 2024, with dedicated observations being conducted in four target areas aligned in an approximate north-south cross section through the European Alps. In addition to long-term monitoring during the TOC, shorter experiments with a high density of instrumentation target processes under different atmospheric conditions and at a range of spatial scales from turbulence to cross-Alpine transport during two extended observational periods.

The first of these two extended observational periods took place between January and February 2025, with experiments focusing on the Inn Valley, Austria, and the Wipp Valley, Italy. The measurements were designed to observe (i) the three-dimensional structure of the mountain boundary layer, including its turbulence characteristics; (ii) the mean and turbulent structure of katabatic winds over a steep snow-covered slope and its response to larger-scale flows; (iii) the three-dimensional structure of mountain waves; and (iv) the life cycle of low-level stratiform clouds forming in the valley atmosphere. To this purpose, measurements were conducted with a suite of instruments, including research aircraft, radiosoundings, remote-sensing wind and temperature profilers, tethered balloons, and a network of turbulence towers.

This presentation will give a brief overview of TEAMx and highlight some of the very first findings from the experiments conducted during the winter campaign.

How to cite: Lehner, M., Rotach, M. W., Stiperski, I., Pfister, L., Gohm, A., Brun, C., Vüllers, J., Cermak, J., Orr, A., Renfrew, I., Dacre, H. F., and Chemel, C.: The TEAMx Observational Campaign – First findings from the winter campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5859, https://doi.org/10.5194/egusphere-egu25-5859, 2025.

EGU25-6679 | Posters on site | AS1.38

Precipitation Uncertainty Hampers the Understanding of Glacier Response in High Mountain Asia 

Thomas Shaw, Achille Jouberton, Masashi Niwano, Marin Kneib, Koji Fujita, and Francesca Pellicciotti

High Mountain Asia (HMA) provides crucial water resources to more than 1.5 billion people and accurate quantification of high elevation precipitation in this region is essential for understanding the hydrological cycle, patterns of ongoing climatic change, and water resource management. This is particularly the case in high elevation, glacierised catchments where the interplay of complex cryospheric and atmospheric processes limits our understanding of current and future water resource availability. Moreover, the role of precipitation and snow accumulation is critical for the health of glaciers which represent both an important freshwater storage and hydrological buffer to drought conditions, but also pose an increasing hazard to downstream populations through potential lake-damming and outburst floods. In both present-day and future modelling scenarios, precipitation at both macro and local scales generate some of the greatest uncertainties in glacier response to climate, and in few places are these hydroclimatic complexities better demonstrated than in HMA.

 

We explore the variability of precipitation estimates across several of the latest regional gridded products with high spatial (>= 10 km) and temporal (hourly) resolution and provide a specific focus over glacierized areas of HMA. Given the common temporal window of 2001-2019, we find substantial disagreement between precipitation products in terms of i) their annual and seasonal magnitudes, ii) the fraction of precipitation occurring during the summer/monsoon period, iii) the decadal difference of precipitation sums, iv) the inter-annual correlation to station observations, v) diurnal precipitation frequency and, vi) dependence on elevation and topographic complexity. Biases of precipitation amounts against in-situ station data can exceed +400% in steep mountainous areas of the Himalaya and errors between products are 23-120% greater over glacierized areas relative to the HMA-wide mean. 

 

When forcing an energy balance model over select glaciers, annual mass balances can disagree by up to 8 m w.e. (1.5 m w.e.) over a single year without (with) bias correction to local observations, propagating into highly distinct long-term trends of estimated glacier health. The high variability of glacier response at the catchment scale relates to spatial patterns of precipitation occurrence due to orographic effects and the resolution and physical process representation of different products. Differences in the surface energy balance of glaciers is, however, most strongly linked to the sub-daily timing of precipitation events and resultant temperature-driven phase of precipitation in different seasons. 

 

We discuss the implications of process representation by different precipitation products and the uncertainty attached to their application in models of glacier energy and mass balance. We also highlight the role of elevation-dependent temperature changes over HMA during the last decades and the implications for changing precipitation phase as a key driver of regionally distinct patterns of glacier mass balance.

How to cite: Shaw, T., Jouberton, A., Niwano, M., Kneib, M., Fujita, K., and Pellicciotti, F.: Precipitation Uncertainty Hampers the Understanding of Glacier Response in High Mountain Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6679, https://doi.org/10.5194/egusphere-egu25-6679, 2025.

EGU25-6939 | ECS | Orals | AS1.38

Investigating lee wave trapping mechanisms over the UK and Ireland 

Hette G. Houtman, Miguel A.C. Teixeira, Suzanne L. Gray, Simon Vosper, Peter Sheridan, and Annelize van Niekerk

Although various lee wave trapping mechanisms have been studied theoretically since Lyra (1940), not much is known about the relative occurrence of these trapping mechanisms in the real world. For this purpose, vertical atmospheric profiles associated with trapped lee waves are clustered here using self-organising maps.

Because in-situ observations of trapped lee waves are scarce, these vertical profiles are extracted from the Met Office’s convective-scale UKV model (which encompasses the UK and Ireland). To demonstrate that this model accurately represents the conditions relevant to trapped lee wave generation, the wavelength and orientation of trapped lee waves visible in satellite imagery are compared to those in the model. The model is found to reproduce these observed characteristics well.

Subsequently, we use the trapped lee wave identification model developed by Coney et al. (2023) and a linear Taylor-Goldstein equation solver to determine which vertical profiles are associated with trapped lee wave activity. We confirm that high low-level wind speeds are a necessary condition for the generation of trapped lee waves of substantial amplitude. We find that wind speeds increasing with height contribute to wave trapping in most cases. Temperature inversions are present in roughly one-third of trapped lee wave cases. The implications of these results for the development of a trapped lee wave drag parametrisation scheme are discussed.

 

References:

Lyra, G. (1943) Theorie der stationären Leewellenströmung in freier Atmosphäre. Z. Angew. Math. Mech., 23, 1-28.

Coney, J. et al. (2023) Identifying and characterising trapped lee waves using deep learning techniques. Quarterly Journal of the Royal Meteorological Society, 150, 213–231.

How to cite: Houtman, H. G., Teixeira, M. A. C., Gray, S. L., Vosper, S., Sheridan, P., and van Niekerk, A.: Investigating lee wave trapping mechanisms over the UK and Ireland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6939, https://doi.org/10.5194/egusphere-egu25-6939, 2025.

EGU25-7058 | ECS | Posters on site | AS1.38

A KGE-based weighted mean of stations’ ensemble to estimate the air temperature at Jungfraujoch since 1900 

Marco Bongio, Carlo De Michele, and Riccardo Scotti

Air temperature is a key variable in the meteo-climatological fields because impacts the atmospheric stability and clouds formation, drives wind patterns and defines the kind of precipitation. However, there is a scarcity of long-term data, especially at high elevations (more than 2000 m). This study proposes a statistical-based methodology to reconstruct a long-term daily temperature record (maximum, mean, and minimum) for high-altitude sites. We have tested it at Jungfraujoch (3571 m a.s.l.), Switzerland, with a backward simulation extending to 1900. The methodology involves daily data from surrounding meteorological stations (thirty), within the MeteoSwiss database, located at elevations ranging 485-2691m a.s.l., providing uninterrupted observations spanning at least the period from 1971 to 2023. The methodology includes the following steps: 1) long-term temporal consistency was evaluated by removing observations with data gaps exceeding 30 days; 2) the mean monthly trend was removed using a non-linear trend estimation function; 3) for each meteorological station, during the calibration period (1988–2005), the daily temperature at Jungfraujoch was estimated as the sum of the temperature at the selected station plus a deterministic and stochastic component; 4) pairwise model performance was evaluated within two validation periods (1971–1985 and 2005–2023) by calculating biases, RMSE, correlation coefficients, rank-based metrics, and the Kling-Gupta Efficiency (KGE); 5) stations with a KGE greater than 0.9 were selected to calculate ensemble simulations, which were obtained as the weighted mean of these stations, extending back to the year 1900 ; 6) A validation was conducted by comparing the reconstructed time series with the closest grid point from two datasets: HISTALP and that provided by Imfeld et al. (2023).

The results suggest: i) comparable performance with existing datasets (HISTALP, Imfeld et al. 2023), despite using a highly parsimonious model that does not rely on additional variables such as relative humidity, cloud cover, wind velocity, or weather patterns; ii) the selection of stations with temporally consistent long-term observations is critical; iii) model performance, efficiency, and errors are primarily influenced by elevation, rather than latitude, longitude, exposure, or distance; iv) the Kling-Gupta Efficiency (KGE) is the most appropriate metric for selecting stations to be used in the ensemble; v) Temporally consistent time series generated by this methodology can provide a benchmark for evaluating observations anomalies and for deeper analysis of Elevation-Dependent Warming issue.

How to cite: Bongio, M., De Michele, C., and Scotti, R.: A KGE-based weighted mean of stations’ ensemble to estimate the air temperature at Jungfraujoch since 1900, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7058, https://doi.org/10.5194/egusphere-egu25-7058, 2025.

The urban areas of many developing cities are suffering from environmental problems due to overpopulation and inadequate public services, in that sense, air pollution is one of the biggest problems. In general, Latin American cities have a higher density of vehicles and are therefore prone to experience high contributions of vehicular pollution. Considering also that the vehicle fleet is old and, in many cases, poorly maintained compared to more developed cities.

The dispersion of pollutants is mainly influenced by wind characteristics, which in turn are influenced by surface roughness (urban coverage) and mountain topography. The objective of the study is to evaluate the influence of surface roughness and topography on wind profiles and the dispersion of atmospheric pollutants in two populated hills located in the city of Cusco, the first called UNSAAC and the second Independencia Hill.

The analysis will be carried out using the numerical model RANS ENVI-met, which determines the dispersion of air pollutant taking into account the interaction between the cover and the atmosphere. The input of the model will be the topographic information, hourly meteorological data and the concentration of pollutants (NO2, SO2, O3, PM10) measured in the field for two months.

In the UNSAAC area, the urban coverage extends along one of the faces of a mountain with a 21 % slope and in the Indepencia area, the urban coverage is located between two mountains with a slope of 15 % (see Figure 1). Regarding roughness, 3 cases were evaluated: zero roughness (topography without buildings), normal roughness (topography with buildings) and increased roughness (topography with doubled-height buildings). Two wind directions were evaluated: 180° and 360°.

Figure 1: Northern axis of evaluation in the Independencia and UNSAAC area

According to the results, the velocity in the boundary layer is lower when the roughness is increased for both study areas; this difference is greater when the wind direction is 360° (see Figure 2). It can also be observed that the height of the boundary layer is higher in the urban area of Independencia. Here, the velocity exceeds 2 m/s at a height of 20 m, while, in the other profiles it exceeds this value at a height less than 5 m. On the other hand, a peak in the NO2 concentration values ​​with 180 µg/m3 can be observed in the urban area of ​​Independencia (see Figure 3).

The results of the study may be useful to buid a risk map of both areas, in order to identify areas with high concentrations of pollutants, and propose measures to reduce pollution, such as limiting the number of vehicles on certain roads.

Figure 2: Wind profiles for a) UNSAAC zone WD= 180° b) UNSAAC zone WD= 360° c) Independencia zone WD= 180° d) Independencia zone WD= 360°

Figure 3: NO2 concentration for a) UNSAAC zone  and b) Independencia zone

How to cite: Mallqui, R., Horna, D., and Cabrera, J.: Study of the influence of surface roughness and topography on wind profiles and the dispersion of atmospheric pollutant in two populated hills in Cusco, Peru, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7252, https://doi.org/10.5194/egusphere-egu25-7252, 2025.

EGU25-8083 | Posters on site | AS1.38

Mountain waves occurrence in Polish Carpathians and their influence on aviation operations 

Alina Jasek-Kaminska, Łukasz Kiełt, Adrian Góra, and Mirosław Zimnoch

Mountain regions, as defined by the International Civil Aviation Organization (ICAO), cover less than 5% of Poland, but highly variable orography dominates almost whole southern border of the country. Under favorable conditions, orographic gravity waves are observed in the wind field over significant part of southern Poland, influencing airspace users. 

Private aircrafts, weighing around five tons and often less, experience orographically induced turbulence directly but not exclusively over the mountainous areas: rotors occurring downstream generate moderate or severe turbulence as well. Moreover, their presence may not be evident in cloudiness so that the pilot encounters so-called clear air turbulence (CAT). Airports located downstream can experience low level wind shear which creates additional difficulties for take-off and landing operations, and if encountered unprepared, can result in a dangerous loss of lift. It is recommended by the ICAO that mountain waves (MTW) of moderate or severe intensity are included in aviation weather forecasts products. 

This study presents the MTW climatology in Polish Carpathians, focusing mainly on the Tatra mountains, using observational data and ERA5 reanalysis. Typical synoptic situations favorable for MTW occurrence in southern Poland are summarized. Based on an extreme case of a devastating downslope windstorm in the Tatra mountains in 2013, the impact of numerical model resolution on resolving the mountain wave effects is investigated using high resolution WRF (Weather Research and Forecasting model) simulations. 

This project has been supported by the subsidy of the Meteorological Service for Civil Aviation of Institute of Meteorology and Water Management – National Research Institute of Poland, "Excellence Initiative - Research University" program at AGH University of Krakow (grant agreement no. 598707), and the subsidy of the Ministry of Science and Higher Education.

How to cite: Jasek-Kaminska, A., Kiełt, Ł., Góra, A., and Zimnoch, M.: Mountain waves occurrence in Polish Carpathians and their influence on aviation operations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8083, https://doi.org/10.5194/egusphere-egu25-8083, 2025.

EGU25-12489 | ECS | Orals | AS1.38

Forest Transition and its Hydro-Climatic Impacts in the Indian Himalayas: Inferences from Field Observations  

Jyoti Ranjan Mohanty, Jaya Khanna, Sumit Sen, and Jagdish Krishnaswamy

The Himalayas, known as the Earth's third pole, are vital to regional and global climate systems, supporting globally significant biodiversity and livelihoods through ecosystem services such as carbon sequestration and water. However, in the west-central Indian Himalayas, moist, broad-leaved mixed-Oak forests are increasingly being replaced by dry, fire tolerant and fire prone Chir Pine forests, posing ecological concerns. This transition threatens biodiversity, reduces ecosystem functionality, and disrupts water availability, raising significant ecological and societal concerns. While the socio-ecological impacts have been explored, the hydro-climatic consequences remain less understood. To address this knowledge and data gap, we established two research observatories in Uttarakhand’s Chir pine and mixed-oak forests (~1600m elevation, 23° slope) to investigate how these forest transitions affect land -atmosphere energy fluxes, soil moisture, streamflow, and transpiration. Our study integrates field measurements with numerical simulations to provide insights into these changes. Bowen ratio (BR) assemblies were installed at 30m (pine) and 18m (oak) heights, equipped with EE181 and HC2S3 temperature and humidity sensors. Seasonal on-site calibration ensured reliable data collection, resulting in a nearly complete year of high-quality data from these remote locations. During the monsoon season, Pines exhibit higher BR evapotranspiration (ET) compared to Oaks, while during the dry period, their ET is only marginally higher. At the tree level, Pines transpire over a larger sapwood area and exhibit less stringent regulation of sap flow and associated transpiration under varying environmental conditions compared to Oaks. Hydrological analyses indicate that the catchments dominated by Pine have lower baseflow to precipitation percentage compared to Oak, rendering streams in these Pine dominated catchments ephemeral, unlike the more sustained baseflow in Oak-dominated forests. All the measurements corroborate the higher evapotranspiration observed in the Chir pine forest compared to Oak. These observations have been used to parameterize vegetation in the Ocean-Land-Atmosphere Model, enabling high-resolution simulations of regional hydro-climatic conditions under different forest covers  This first ever study of these Himalayan vegetation transitions is likely to provide insights into the future changes in ecohydrology in this biodiversity and water security hotspot. 

How to cite: Mohanty, J. R., Khanna, J., Sen, S., and Krishnaswamy, J.: Forest Transition and its Hydro-Climatic Impacts in the Indian Himalayas: Inferences from Field Observations , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12489, https://doi.org/10.5194/egusphere-egu25-12489, 2025.

EGU25-13871 | Orals | AS1.38

First Results From The TEAMx-FLOW Project: Wintertime Radiosonde Observations And Numerical Modelling Of Mountain Waves Over The Tyrolean Alps 

Neil Hindley, Andrew Orr, Corwin Wright, Andrew Ross, and Philip Rosenberg

The TEAMx programme is a coordinated international research programme focusing on improving our understanding of exchange processes in the atmosphere over mountains and evaluating their representation in numerical weather prediction (NWP) and climate models. TEAMx features several observational and modelling strategies conducted by nationally funded projects centred on the European Alps, including 6-week extended observational periods (EOPs) in both summer and winter 2025. In this presentation, we present the first results from the UK-funded TEAMx-FLOW project, which focuses on the representation of wintertime orographic drag from mountain waves across spatial scales (including sub-km) in the UK Met Office Unified Model (UM) and its evaluation against TEAMx observations. Here we present analysis of the first of these observations, an intensive radiosonde balloon campaign launched throughout January-March 2025 conducted by the UK National Centre for Atmospheric Science (NCAS). The NCAS campaign featured 6-hourly operational launches, complemented with 3-hourly intensive launch periods during mountain wave events and also simultaneous launches of offset pairs of radiosondes. We analyse and quantify mountain waves and their momentum transport in these measurements, including using cross-spectral analysis of the offset pairs to obtain scale separation of observed mountain waves, a process not routinely applied to balloon soundings before. We also explore observations of partial wave breakdown in horizontally sheared flow, a process highly challenging to represent in models. With these new observations, we outline how the representation of mountain waves across multiple spatial scales in the UM and other NWP models can be evaluated and improved to achieve ever more accurate sub-km modelling, leading to improved predictions of mountain weather and climate in next-generation models.

How to cite: Hindley, N., Orr, A., Wright, C., Ross, A., and Rosenberg, P.: First Results From The TEAMx-FLOW Project: Wintertime Radiosonde Observations And Numerical Modelling Of Mountain Waves Over The Tyrolean Alps, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13871, https://doi.org/10.5194/egusphere-egu25-13871, 2025.

EGU25-13987 | Posters on site | AS1.38

Investigating the spatial structure of winds in complex terrain using a mobile wind lidar 

Stephan De Wekker, Jagdish Desai, Gert-Jan Duine, and Leila Carvalho

In the lee of the Santa Ynez Mountains north of Santa Barbara, CA, late afternoon-to-early morning episodes of offshore, northerly gusty downslope surface winds are frequently observed. These downslope winds are locally known as Sundowners. Sundowners are spatially non-uniform and can be accompanied by rapid increases in temperature and decreases in relative humidity with significant impact on fire behavior. Our understanding of the spatial and temporal variability of Sundowners and the underlying mesoscale mechanisms is limited. To address this knowledge gap, the NSF-funded Sundowner Wind Experiment (SWEX) was conducted in Spring 2022.  

In this presentation, we focus on observations made by the surface-based mobile observing platform UWOW (University of Virginia Wind Observatory on Wheels), a trailer-mounted lidar system to measure spatial and temporal variations of lower tropospheric winds.  UWOW uses a HALO photonics StreamLine XR Doppler lidar, a GPS, and an inertial navigation system placed in a custom trailer to measure boundary layer winds while traveling on the road. UWOW can measure wind profiles from approximately 100 to 3000 m above ground with 30 m vertical spacing. During SWEX, UWOW travelled about 7000 km on roads around the Santa Ynez Mountains to document the spatial wind and aerosol variability during Sundowner Wind days and during undisturbed days. Data examples and comparisons with 1-km numerical simulations using the Weather Research and Forecasting (WRF) model will be discussed. 

How to cite: De Wekker, S., Desai, J., Duine, G.-J., and Carvalho, L.: Investigating the spatial structure of winds in complex terrain using a mobile wind lidar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13987, https://doi.org/10.5194/egusphere-egu25-13987, 2025.

EGU25-14115 | ECS | Posters on site | AS1.38

Assessing The Impact of Global Warming on Glacial Elevation of The Bolam Glacier  

Lily Welsh, Sarah Neuhaus, and Slawek Tulaczyk

Mount Shasta, a large stratovolcano in northern California, contains the southernmost glacial system in North America (41.3 degrees N, about the latitude of Rome). Due to its southern position, this glacial system is very vulnerable to climate warming. However, previous research indicated that this glacial system experienced significant growth during the second half of the twentieth century, mainly as a result of the so-called "snowgun effect" at high elevations, operating in the warmer, wetter winters of this ocean-influenced climate (Howat & Tulaczyk, 2005 & Howat et al., 2006). New results indicate recent, significant glacier collapse as a result of continued climate warming leading to increased ablation, which eventually overwhelms the effect of increased snow deposition at high elevations. The Hotlum, Bolam and Whitney glaciers reside on the North face of Mount Shasta while Konwakiton and Wintun reside on the South face. It is evident that glacial bodies have receded in this time period, but a more indepth inspection of the effects of climate change on the Bolam Glacier was deemed necessary. The glaciers within Mount Shasta provide a small percentage of water to the Shasta Reservoir. More notably, the glacial bodies provide water supply to support habitats for immense biodiversity in flora and fauna within the region, including endemic species. Changes in glacial terminus elevation of the Bolam Glacier were observed in the field and through aerial photography. Through topographic and photographic inspection, in field geolocated waypoint collection and analysis of field data, a retreat of nearly 1500 meters at the Bolam Glacier was observed between the years photographs of 1998 and of 2024, suggesting a significant impact on glacial bodies in the region due to changes in climate.

References

Ewert, J. W., Diefenbach, A. K., & Ramsey, D. W. (n.d.). Eruption History of Mount Shasta U.S. Geological Survey. USGS.gov. Retrieved January 6, 2025, from https://www.usgs.gov/volcanoes/mount-shasta

Geology and History of Mount Shasta U.S. Geological Survey. (2023, November 6). USGS.gov. Retrieved January 6, 2025, from https://www.usgs.gov/volcanoes/mount-shasta/science/geology-and-history-mount-shasta 

Howat, I. M., & Tulaczyk, S. (2005, December 8). Climate sensitivity of spring snowpack in the Sierra Nevada. Journal of Geophysical Research, 110.

Howat, I. M., Tulaczyk, S., Rhodes, P., Israel, K., & Snyder, M. (2006, August 18). A precipitation-dominated, mid-latitude glacier system: Mount Shasta, California. Climate Dynamics, 28, 85-98.

Howat, I. M., & Tulaczyk, S. (2005). Trends in spring snowpack over a half-century of climate warming in California, USA. Annals of Glaciology, 40, 151.

Lindsey, R., & Dahlman, L. (2024, January 18). Climate Change: Global Temperature NOAA Climate.gov. Climate.gov. Retrieved January 6, 2025, from

How to cite: Welsh, L., Neuhaus, S., and Tulaczyk, S.: Assessing The Impact of Global Warming on Glacial Elevation of The Bolam Glacier , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14115, https://doi.org/10.5194/egusphere-egu25-14115, 2025.

EGU25-14227 | Orals | AS1.38

Karakoram Anomaly and its connection with the Western Disturbances 

Pankaj Kumar and Aaquib Javed

The global retreat of glaciers is a widely recognized indicator of climate change. However, the Karakoram region of the Himalayas defies this trend, exhibiting a unique phenomenon termed the “Karakoram Anomaly,” characterized by glacier stability or surges. This anomaly has been increasingly linked to the dynamics of western disturbances (WDs), upper-tropospheric synoptic systems propagating eastward along the subtropical westerly jet stream, critical drivers of winter precipitation in the region. This study synthesizes recent analyses of WDs using tracking algorithms applied to reanalysis datasets (ERA5, MERRA2, and NCEP-CFSR/CFSv2) to evaluate their role in sustaining the Karakoram Anomaly. While the frequency of WDs has remained relatively steady, a ∼10% increase in precipitation intensity associated with WDs over the anomaly core region has been observed in recent decades. The Karakoram receives approximately 65% of its total winter snowfall from WDs, emphasizing its pivotal role in modulating regional glacier mass balance. Concurrently, snowfall from non-WD sources has declined by ∼17%, further underscoring the significance of WDs. Changes in atmospheric dynamics, including enhanced baroclinic instability and a latitudinal shift in the subtropical westerly jet, have been identified as contributors to the increased intensity of WDs. Moreover, a statistically significant eastward shift (~9.7°E) in the genesis zone of WDs has been noted, resulting in enhanced cyclogenesis potential, higher moisture availability, and reduced propagation speeds. These factors collectively intensify WD-induced precipitation events over the Karakoram, supporting anomalous glacier behavior. This study highlights the critical influence of strengthening WDs on the Karakoram Anomaly, providing new insights into the interplay between atmospheric dynamics and regional glacier dynamics under climate change.

 

Keywords: Glaciers, Karakoram anomaly, Western Disturbances, TRACK

Acknowledgement: Funding from Science and Engineering Research Board (SERB), Govt. of India, grant number CRG/2021/00l227-G

How to cite: Kumar, P. and Javed, A.: Karakoram Anomaly and its connection with the Western Disturbances, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14227, https://doi.org/10.5194/egusphere-egu25-14227, 2025.

EGU25-15922 | Posters on site | AS1.38

Observed hotspots of changing snow depth and snowfall in European mountain regions 

Dana-Magdalena Micu, Vlad-Alexandru Amihaesei, Gabriele Quinti, Kirsten Halsnæs, Shreya Some, Monica-Gabriela Paraschiv, Alexandru Dumitrescu, and Sorin Cheval

Mountain regions are particularly vulnerable to natural hazards, such as snow avalanches, landslides, or flash-flooding, which are increasingly exacerbated by climate warming and changing climate patterns. This paper leverages the Copernicus Regional ReAnalysis for Europe (CERRA) dataset, with 5 km x 5 km spatial resolution, from the Copernicus Climate Change Service (C3S), covering the period 1985–2020, to analyse the changing of the seasonal patterns of snow depth and snowfall in two major European mountain ranges: the Alps and the Carpathians. More specifically, the study aims to identify the mountain areas with persistent and statistically significant increases or declines in snowfall and snow depth, referred to as "hotspots". The focus of the study is on four key snow depth and snowfall-related indicators including (i) total snow depth, (ii) number of snow cover days, (iii) days with snow depth exceeding 30 cm, and (iv) snowfall water equivalent. The hotspots are identified based on local spatial auto-corelation methods (the Getis and Ord G statistic), using the estimated Mann-Kendall trends of the four snow indicators as inputs. A positive Gi value signifies that a feature and its surrounding neighbours exhibit high values, whereas a negative Gi value indicates low values in the feature and its neighbours. The magnitude of the Gi value reflects the intensity of the clustering. 
The results indicate widespread hotspots characterised by significant declines in both snow depth and snowfall indicators, in all seasons, especially at low and mid-elevations in both mountain regions. The observed shifts are particularly pronounced during winter (December-January-February) and spring (March-April-May). The location of identified hotspots carries multiple implications for the distribution and availability of water resources, ecosystem services, infrastructure and tourism activities, and so for the livelihood of mountain communities. These findings provide critical insights into the shifting snow avalanche hazard and their socio-economic impacts at NUTS3 level and in specific areas where historical snow avalanche events have significantly impacted three key socio-economic sectors—tourism, infrastructures, and forestry. They also could underscore the ongoing challenges in the mountain risk management under a changing climate.
This research received funds from the project “Cross-sectoral Framework for Socio-Economic Resilience to Climate Change and Extreme Events in Europe (CROSSEU)” funded by the European Union Horizon Europe Programme, under Grant agreement n° 101081377.

How to cite: Micu, D.-M., Amihaesei, V.-A., Quinti, G., Halsnæs, K., Some, S., Paraschiv, M.-G., Dumitrescu, A., and Cheval, S.: Observed hotspots of changing snow depth and snowfall in European mountain regions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15922, https://doi.org/10.5194/egusphere-egu25-15922, 2025.

EGU25-16079 | Posters on site | AS1.38

Campaign TEAMx: First results of wind observations compared to model simulations at three sites in the Inn Valley (Austria) 

Rebecca Gugerli, Maxime Hervo, Alexander Gohm, Daniel Leuenberger, and Alexander Haefele

In the framework of the campaign TEAMx, MeteoSwiss deployed a Doppler Wind Lidar (WL, Windcube-100S) in Radfeld, Austria. The WL provides high resolution wind speed and – direction measurements within the Inn Valley at several altitudes. These observations provide a reliable reference to investigate the performance of model wind estimates in alpine valleys. In this study, we use analyses data from the ICON NWP model computed with KENDA, a Km-scale ENsemble-based Data Assimilation system. These data from the KENDA-CH1 NWP system have a spatial resolution of 1.1x1.1 km and a temporal resolution of 1 hour. First results show a good model performance at Radfeld with an average root mean square vector difference (RMSVD) of 3.78 m/s during the period from 23 October 2024 to 16 December 2024.

Furthermore, the comparison between observations and model analyses is extended to the sites of Kolsass and Innsbruck, which are both located in the same valley (Inn Valley) and at both sites wind observations are obtained by a WL (Halo Photonics Systems). In addition, we analyse the observations from a WL permanently deployed in Payerne (Switzerland).

Our results show that the model has an average RMSVD lower than 3.8 m/s for all sites during the given time period. The only exception with a higher RMSVD occurs during the storm Caetano (19-23 November 2024). For Payerne, we find a RMSVD of 2.7 m/s, which is significantly better than for the other sites. This is explained by the assimilation of several observed atmospheric profiles (wind and temperature) in the model, which positively impacts the model analyses. Moreover, Payerne has a flatter topography. Overall, our results confirm a good performance of the simulated wind dynamics by the high resolution KENDA-CH1 NWP system.

How to cite: Gugerli, R., Hervo, M., Gohm, A., Leuenberger, D., and Haefele, A.: Campaign TEAMx: First results of wind observations compared to model simulations at three sites in the Inn Valley (Austria), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16079, https://doi.org/10.5194/egusphere-egu25-16079, 2025.

EGU25-16132 | ECS | Orals | AS1.38

Understanding elevation-dependent warming in the Alps through high-resolution surface energy balance analysis 

Simon Zitzmann, Benjamin Fersch, and Harald Kunstmann

This study investigates elevation-dependent warming (EDW) in the Alps, focusing on Berchtesgaden National Park, Germany, to provide insights into the drivers of warming patterns and their spatial variability.
EDW refers to the variation in warming rates across altitude, often characterized by intensified warming trends at higher elevations. This phenomenon has significant implications for mountainous and downstream ecosystems and water resources. While multiple factors contributing to EDW have been discussed in the literature – such as snow-albedo feedbacks and the increased sensitivity of cold, dry regions to climate change – the roles of soil interactions and topography remain underexplored.

Our research uses high-resolution spatial data and long-term temperature records to uncover how topography, soil properties and surface energy dynamics contribute to EDW. We utilize data from HISTALP, a homogenized observational dataset for the Greater Alpine Region, to examine the relationship between warming trends and topographic factors. Within the national park, 23 long-term stations monitor meteorological variables. Additionally, three temporary stations spanning altitudes from 617 to 1930 m measure surface energy balance components to capture elevation-dependent and small-scale effects.

Preliminary findings indicate that EDW is influenced by factors beyond altitude. Historical data (1910–2010) reveal significant warming across altitudes in the Greater Alpine Region, with rates of 0.4–2.4 K per century. Higher elevations generally experience stronger warming, except in winter, when mid-elevation bands (500–1000 m) warm the most. Slope orientation significantly affects warming rates, with north-facing slopes showing amplified trends. Ongoing research aims to develop a statistical model incorporating topography, vegetation and soil properties to map warming trends across the Alps.
Ground heat flux analysis reveals spatial variations potentially influenced by soil depth and moisture retention at different altitudes. Integrating these observations with simulations from the GEOtop hydrological model will provide spatially detailed and novel insights into relevant land surface processes.

How to cite: Zitzmann, S., Fersch, B., and Kunstmann, H.: Understanding elevation-dependent warming in the Alps through high-resolution surface energy balance analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16132, https://doi.org/10.5194/egusphere-egu25-16132, 2025.

EGU25-16472 | ECS | Orals | AS1.38

Assessing the representation of flow separation in Foehn descent with high-resolution numerical simulations 

Julian Quimbayo-Duarte, Yue Tian, and Juerg Schmidli

Foehn winds are warm, dry, downslope winds that occur on the lee side of mountain ranges. They result when moist air is forced to ascend on the windward side, cooling and losing moisture as precipitation. As the now-drier air descends on the leeward side, it warms adiabatically, leading to distinct temperature and humidity profiles. In the Alps, the descent of foehn winds is often confined to distinct hotspots where the interplay between complex topography, mountain-induced gravity waves, and flow separation processes focuses the descending air. These hotspots are associated with localized warming and drying, which can significantly influence weather conditions, predictability, and their impact on ecosystems and human activities in the affected regions. Previous studies, utilizing the COSMO model, a numerical weather prediction (NWP) model at 1 km resolution, visualized these hotspots and established their connection to mountain-induced gravity wave. However, the adequacy of a 1 km resolution in accurately capturing flow separation at the mountain surface—a key feature influencing foehn dynamics and predictability—remains an open question.

To address this question, we conducted high-resolution simulations for two case studies: one in the Rhine Valley from February 2017 and another in Meiringen, Switzerland, from March 2022. Simulations were performed using the ICON model in NWP mode at a horizontal resolution of 1.1 km and ICON-LES at resolutions of 520 m, 260 m, and 130 m. For the Meiringen case, we validated our model setup using wind and temperature profiles obtained from the Meiringen Campaign (2021–2022). Meanwhile, the Rhine Valley case, previously analyzed at a resolution of 1 km, was revisited to assess whether higher resolutions provide an improved representation of flow separation dynamics. Additionally, we employ offline trajectories to precisely track the descent locations of the foehn air parcels, providing a detailed assessment of how model resolution influences the spatial distribution of descent hotspots in the Swiss Alps.

Our study is the first to combine trajectory analysis with LES simulations in foehn research, enabling a detailed visualization of foehn trajectories. The ultimate goal of this study is to provide guidance on selecting appropriate model resolutions to enhance the accuracy of research on foehn winds and their associated effects.

How to cite: Quimbayo-Duarte, J., Tian, Y., and Schmidli, J.: Assessing the representation of flow separation in Foehn descent with high-resolution numerical simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16472, https://doi.org/10.5194/egusphere-egu25-16472, 2025.

EGU25-16725 | Posters on site | AS1.38

Steps for the identification of Elevation Dependent Warming in the Pyrenees 

Pere Esteban Vea, Marc Prohom Duran, and Jordi Cunillera Grañó

In recent decades, several research efforts have been made to quantify climate change in the Pyrenees, mainly focusing on temperature and precipitation trends since the 1950s. However, as in many mountain regions around the world, the lack of data at the highest elevations makes it difficult to draw solid conclusions about the varying warming rates at different altitudes.

As part of the LIFE-SIP project "Pyrenees4Clima" (2024-2032) various tasks for the detection and analysis of Elevation-Dependent Warming (EDW) have been planned. First, as much climate series as possible above 1,500 meters is being compiled, with trend analysis, quality control, and homogenization (if needed) being carried out. Additionally, temperature and relative humidity sensors will be installed during the summer of 2025 to create or enhance four pilot areas in Spain (Catalonia and Aragón), France, and Andorra for a detailed analysis of EDW and circulation patterns. To support this readings, a complete automatic weather station has been installed in one of the pilote areas (in the Catalan Pyrenees and 1,700 m). By incorporating snow measurements from existing automatic weather stations, the influence of the presence or absence of snow on warming will also be explored.

This presentation aims to show EGU 2025 participants our objectives, intentions, and results to date, learn about other EDW case studies, and share experiences and recommendations during this initial phase of our project.

How to cite: Esteban Vea, P., Prohom Duran, M., and Cunillera Grañó, J.: Steps for the identification of Elevation Dependent Warming in the Pyrenees, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16725, https://doi.org/10.5194/egusphere-egu25-16725, 2025.

EGU25-16963 | ECS | Posters on site | AS1.38

Insight into subsurface - quantification of alpine heat waves and their impact on high mountain permafrost 

Tomasz Gluzinski, Christian Hauck, Christin Hilbich, Coline Mollaret, and Cécile Pellet

In recent years the changing state of the cryosphere has been one of the most visually striking effects of climate change in mountainous terrains, gathering increased attention of not only the scientific community but the general public. Ice loss in the subsurface, caused by a warming ground thermal regime, is not directly visible such as retreating glaciers or annual snow cover changes, but it can have major impacts on ground stability.
Heat waves may contribute twofold to cryospheric changes: (1) as contributors to the general warming trend and (2) by (potentially) irreversibly changing the ground ice content through excessive amounts of heat penetrating the ground during such an event. Here, we focus on the second aspect and its impact on mountain permafrost. Although climatological research provides several tools for heat wave analysis, the application of (often regional) studies to the sparsely available borehole data and discrete meteorological monitoring networks are rare.
We employ the Heat Wave Magnitude Index daily (HWMId) metric to analyse temperature data from several Swiss Permafrost Monitoring Network (PERMOS) and MeteoSwiss stations near well-studied permafrost monitoring sites in the Alps. Historical and reconstructed data are used to determine specific temperature thresholds per site, accounting for local conditions (such as geomorphology, geology or ice content) therefore a systematic heat wave definition can be applied uniformly across all locations.
HWMId is compared to the changes in ground moisture content and observed changes in the permafrost body derived from borehole data. In addition, ice content is independently estimated from time series of 2-dimensional geophysical data, namely seismic refraction tomography and electrical resistivity tomography jointly inverted by petrophysical joint inversion. Initial results from the analysis of decade-long time series show correspondence between ground resistivity decrease with a general increasing trend in heat wave occurrences and intensity. Moreover heat waves precondition the permafrost for further thawing in subsequent years. Resilience of permafrost to the heat wave events in different landforms brings important implications for slope stability and safety of communities and infrastructure in mountainous regions.

How to cite: Gluzinski, T., Hauck, C., Hilbich, C., Mollaret, C., and Pellet, C.: Insight into subsurface - quantification of alpine heat waves and their impact on high mountain permafrost, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16963, https://doi.org/10.5194/egusphere-egu25-16963, 2025.

EGU25-17153 | Posters on site | AS1.38

Refining valley wind days detection from in situ observations and ERA5 reanalysis 

Sebastiano Carpentari, Mira Shivani Sankar, Nadia Vendrame, Dino Zardi, and Lorenzo Giovannini

Numerous studies proposed algorithms to identify days with well-developed valley wind circulations, commonly applying thresholds based on measurements from surface weather stations and/or reanalysis datasets. In the present study, the method suggested by Lehner et al. (2019) was selected as a starting point to detect valley wind days in the Alpine Adige Valley (Italy),  based on a year-long dataset collected at an eddy covariance flux station. The method employs three fixed thresholds: two on geopotential height gradients at 700 hPa in the North-South and West-East directions (synoptic forcing), and one on longwave radiation (Clear Sky Index, local forcing), following Marty and Philipona (2000). 

To refine the procedure, in this study four geopotential pressure levels were considered, using the ERA5 reanalysis dataset covering the period 1991-2020. Additionally, the daily threshold was assessed using a n-day moving window centered on the target day. The Clear Sky Index was calculated, choosing the most suitable emissivity parameterization for the Adige Valley. Furthermore, objective adjustments to the Clear Sky Index reference limit were made. Finally, the method was tested with data from other eddy-covariance stations to verify its performance in different contexts and generalize the results.

How to cite: Carpentari, S., Shivani Sankar, M., Vendrame, N., Zardi, D., and Giovannini, L.: Refining valley wind days detection from in situ observations and ERA5 reanalysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17153, https://doi.org/10.5194/egusphere-egu25-17153, 2025.

EGU25-20147 | Orals | AS1.38

On the structure of the atmospheric boundary layer over highly complex terrain 

Juerg Schmidli and Bruno Neininger

The atmospheric boundary layer (ABL) over mountainous regions plays a crucial role in exchange processes between the surface and the free atmosphere, influencing weather, climate, and air quality. Unlike the relatively uniform ABL over flat terrain, the structure of the mountain boundary layer (MoBL) is highly complex due to the wide spectrum of scales of motion induced by the multi-scale orography. These scales range from small-scale turbulence and coherent structures to slope and valley winds, encompassing both thermally and dynamically forced flows. This intricate interplay of processes creates a highly heterogeneous and variable boundary layer that challenges traditional modeling approaches and necessitates detailed investigation. This study aims to enhance understanding of the convective boundary layer (CBL) over highly complex terrain by addressing the following questions: What are the characteristics of the coherent structures (e.g., thermals) in the CBL and how stationary are they? What is their diurnal cycle, and how do their statistics, such as preferred locations, vary from day to day?

To answer these questions, we utilize the ICON model to perform large-domain, real-world large-eddy simulations (LES) at a resolution of 65 m, incorporating 1.5 million grid points. The simulations employ a nesting strategy with four domains at resolutions of 520 m, 260 m, 130 m, and 65 m, progressively refining the model to capture fine-scale dynamics. Conducted over the Swiss Alps for seven days in August 2022, the simulations reveal a highly heterogeneous boundary layer with preferred locations for thermal formation. These locations exhibit a rather consistent diurnal cycle and remarkably small day-to-day variability, despite changing large-scale forcings. Comparisons with Alptherm, a Lagrangian model designed for forecasting gliding conditions, provide additional context. Insights from this study advance our understanding of the mountain ABL and support improvements in mesoscale and forecasting models for complex terrain.

How to cite: Schmidli, J. and Neininger, B.: On the structure of the atmospheric boundary layer over highly complex terrain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20147, https://doi.org/10.5194/egusphere-egu25-20147, 2025.

EGU25-26 | ECS | Posters on site | ERE2.1

A Novel Metric for Quantifying Solar Irradiance Stability: Mapping Solar Irradiance Variability to Photovoltaic Power Generation 

Qun Tian, Jinxiao Li, Zhiang Xie, Puxi Li, Ya Wang, Dongwei Chen, and Yue Zheng

The daily stability of solar irradiance significantly influences photovoltaic (PV) power generation; however, existing metrics for assessing it normally fail to robustly correlate with daily PV output. To address this gap, we introduce a new metric, the solar instability index (SII), formulated by applying the Wasserstein distance to assess the deviation of intra-day solar irradiance pattern from the anticipated diurnal cycle. In our case station, SII closely correlates with atmospheric moisture and available solar energy, suggesting its strong association with synoptic weather events that lead to solar resource loss. We further scrutinize the efficacy of SII alongside two existing metrics through two case studies. The results demonstrate that SII excels in capturing low-frequency variations in solar irradiance without relying on arbitrarily assigned parameters, thereby outperforming the other two metrics in establishing a robust correlation with PV power output. As such, in scenarios involving site selection for PV power plant, SII stands as a valuable metric for assessing the potential stability of daily PV power generation.

How to cite: Tian, Q., Li, J., Xie, Z., Li, P., Wang, Y., Chen, D., and Zheng, Y.: A Novel Metric for Quantifying Solar Irradiance Stability: Mapping Solar Irradiance Variability to Photovoltaic Power Generation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-26, https://doi.org/10.5194/egusphere-egu25-26, 2025.

Renewable energy sources are gaining increasing importance due to the rising prices, depletion of fossil fuels, and the need to achieve climate protection goals. Solar energy has the advantage of being exploitable to some extent worldwide. In East-Central Europe, particularly in Hungary, the use of solar energy is growing rapidly, with the installed capacity of photovoltaic power plants increasing from 14 MW to ~4 GW between 2012 and 2022.

The estimation of photovoltaic power potential (PVpot) and its changes based on the outputs of general circulation models (GCMs) has become a popular research topic over the past decade, since GCM biases can lead to biases in regional climate models through the downscaling process. In general, previous studies have estimated an increase in PVpot for Central Europe during the 21st century. However, the effects of inter-model variability and internal variability of GCMs on PVpot in Europe, particularly in East-Central Europe, are less thoroughly examined.

This analysis seeks to assess the sensitivity of PVpot to inter-model variability and internal variability of GCMs in Europe, with a focus on East-Central Europe. For this purpose, the number of days with small (or large) PVpot will be calculated which – as it was pointed out by Feron et al. (2021) – may exhibit greater differences in the future compared to historical periods, unlike the PVpot itself. Different realizations of future outputs from CMIP6 GCMs for 2071-2100 (based on the SSP2-4.5 and SSP5-8.5 scenarios) will be compared to historical outputs for 1981-2010, focusing on seasonal changes. For comparison reasons, reanalyses (e.g., ERA5, CERRA) will also be applied for the historical period.

Our findings provide essential insights for energy planners to mitigate the impacts of future weather variability.

Feron et al. (2021). Nature Sustainability, 4(3), 270-276

The research was funded by the National Multidisciplinary Laboratory for Climate Change (RRF-2.3.1-21-2022-00014).

How to cite: Kalmár, T. and Kristóf, E.: Understanding future solar energy trends in Europe: The impact of the variability in CMIP6 GCMs on photovoltaic power potential, with a special focus on East-Central Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-976, https://doi.org/10.5194/egusphere-egu25-976, 2025.

EGU25-1827 | ECS | Posters on site | ERE2.1

Enhanced Offshore Wind Potential in a Warming Climate 

Cheng Shen and Hui-Shuang Yuan

Offshore wind farms, as a rapidly expanding component of the wind energy sector, play a critical role in advancing global carbon neutrality, a trend expected to persist. In this study, we leverage ERA5 reanalysis data to refine offshore wind speed trends projected by CMIP6 models. This methodology provides improved estimates for changes in offshore Wind Power Density (WPD) under four Shared Socioeconomic Pathways (SSP) scenarios. Our results indicate a consistent upward trend in global offshore WPD throughout the 21st century across all SSP scenarios. Among regions with significant existing offshore wind installations, Europe is projected to experience the most pronounced increase, with offshore WPD potentially rising by up to 26% under 4°C of global warming. These findings reveal a significant enhancement of global offshore WPD in a warming climate, offering critical insights for optimizing the strategic development of future wind energy systems worldwide.

How to cite: Shen, C. and Yuan, H.-S.: Enhanced Offshore Wind Potential in a Warming Climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1827, https://doi.org/10.5194/egusphere-egu25-1827, 2025.

EGU25-1947 | ECS | Posters on site | ERE2.1

Ocean-atmospheric drivers of wind and solar energy seasonal variability in tropical South America 

Nicolas Duque-Gardeazabal, Stefan Brönnimann, Andrew R. Friedman, Edgar Dolores-Tesillos, and Olivia Martius

South America is one of the regions with the highest renewable power share in its energy matrix. However, it is heavily affected during drought driven by El Niño/Southern Oscillation (ENSO) and the positive phase of the Atlantic Meridional Mode (AMM), since hydropower is the main source. Wind and solar energy are soaring due to economic development and as an alternative/complement to hydropower and fossil fuels. Nonetheless, they can be affected by climate variability modes and it is thus essential to determine the impacts of ocean-atmospheric modes on these two renewable energies. Our research focuses on understanding the links between climate modes and the seasonal variability of potential wind and solar generation. The understanding of the physical mechanisms driving renewable energy variability might be useful for improving sub-seasonal to seasonal forecasts and, hence, properly managing energy production and storage for the following months.

The analysis is also centred around three energy hubs (regions with multi-annual high production capacity of renewable energy). They are located near or on the north Caribbean coast, the east and east coast of Brazil, and the west coast of Peru and the Bolivian Altiplano. The research mainly uses composites of physically consistent interpolations (i.e. reanalysis ERA5) and some satellite-based observations from CLARA cloud cover (1980 - 2020). The ocean-atmospheric modes are defined using Sea Surface Temperature indices. It analyses the anomalies of wind speed, its direction and wind power density (WPD), but also Sea Level Pressure anomalies when climate modes are active. For solar energy, a capacity factor (CF) is calculated using an empirical method that considers the irradiance and the temperature of the panel (based on 2 m air temperature and incident radiation). To study the mechanisms producing its variability, we also analyse the atmospheric moisture transport (VIMF) and cloud cover. The ocean-atmospheric modes’ activation times are defined with Sea Surface Temperature indices.

We analysed the mechanisms of ENSO and of two climate modes in the Atlantic Ocean (the AMM and the Atlantic El Niño equatorial mode), as we discovered these modes can alter regional atmospheric circulation. Cross-equatorial wind anomalies – driven by the AMM – increase or reduce WPD depending on the region while also creating anomalous VIMF, convergence, and clouds, hence affecting the solar CF, in the north Caribbean and east Brazilian hubs. Not only does ENSO affect solar energy through atmospheric subsidence and reduction of cloud cover, but it also affects WPD attracting and accelerating winds to the equatorial east Pacific. The Atlantic equatorial mode (Atl3) is an important source of climate variability, but we discovered that its effects over the continent and the energy hubs are not so strong and widespread compared to those from the other two modes. We also found that solar and wind are not very often complementary, but they can potentially complement hydropower because stronger winds and less cloud cover are present during droughts.

Future research could focus on evaluating the impacts of sub-seasonal phenomena on renewable energy and their influence on predictability.

How to cite: Duque-Gardeazabal, N., Brönnimann, S., Friedman, A. R., Dolores-Tesillos, E., and Martius, O.: Ocean-atmospheric drivers of wind and solar energy seasonal variability in tropical South America, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1947, https://doi.org/10.5194/egusphere-egu25-1947, 2025.

On 7-9 January 2005 Storm Erwin passed across northern Europe causing damage and interrupting power and transportation networks from Ireland to the eastern Baltic region. In northern England the storm was associated with severe river flooding in Carlisle region that cut transportation links into the city and necessitated evacuations.  Across the Baltic region strong winds were reported, resulting in large scale forest damage and power outages.  In Denmark, wind energy was impacted as wind speeds crossed the 25 m/s cutoff threshold for turbine operations, leading to a mass shut down of wind turbines and requiring electricity to be imported to make up the shortfall.  In Sweden, there were widespread power outages as transmissions lines were blown down in the winds, and coastal nuclear power plants were shut down when sea spray caused short-circuiting problems in power transmission.  The storm was associated with a notable coastal surge and flooding, particularly in Denmark and the eastern Baltic.  The present contribution presents an overview of the societal impacts of the storm.  A detailed analysis is carried out of offshore impacts around the North Sea using tide gauge and wave data recorded during the event, and shipping accidents from media reports.

How to cite: Kettle, A.: Storm Erwin: Societal and energy impacts in northern Europe on 7-9 January 2005, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2140, https://doi.org/10.5194/egusphere-egu25-2140, 2025.

Climate change triggered the necessity of moving to a greener energy generation which includes renewable energy sources, such as wind and solar. However, integrating renewable energy sources into the current energy network is a challenging task, as these are highly weather dependent. The main challenge is to balance energy demand and supply, as both are now weather dependent.

 

In previous work energy shortfall (difference between energy demand and renewable generation) across 28 European countries over the boreal winter was investigated from the perspective of weather regimes. In this work, it was shown that some weather regimes greatly favour the occurrence of periods of high energy demand and low renewable generation i.e. periods of high shortfall.  Previous research has shown that subseasonal drivers can have a significant impact on weather regimes. Therefore, in this study, we aim to quantify the impact of subseasonal drivers on the occurrence of weather regimes and in turn, on energy. The focus is on the Madden-Julian Oscillation and the stratospheric polar vortex.

 

Results show that the Madden-Julian Oscillation, substantially impacts the occurrence of the negative phase of North Atlantic Oscillation and the Scandinavian Trough, but has limited influence on other weather regimes. Comparatively, the stratospheric polar vortex affects the occurrence of all weather regimes. Further on, we observe that both drivers impact the occurrence of energy days (days with extreme energy demand, shortfall or wind generation). This impact varies greatly between countries and depending on the phase of the S2S drivers. The lagged response suggests that there is great potential for these drivers to be predictors.

How to cite: Rouges, E., Kretschmer, M., and Shepherd, T.: High energy shortfall across 28 European countries during the winter: Investigation of the role of the Madden-Julian Oscillation and stratospheric polar vortex, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2479, https://doi.org/10.5194/egusphere-egu25-2479, 2025.

Due to its limited natural resources, Taiwan has historically relied heavily on imported natural gas and coal for power generation. The government has recently emphasized shifting toward renewable energy sources to achieve energy independence. With global initiatives targeting net-zero carbon emissions by 2050 and the European Union planning to implement a carbon tax on heavy industries by 2026, the demand for renewable energy solutions has significantly increased. This research investigates optimal locations for deploying wind turbines and photovoltaic panels to maximize renewable energy output across inland and offshore regions of Taiwan (118°–123°E, 21°–26°N). The wind energy potential is assessed using Wind Power Density (WPD), calculated by the formula E = 0.5ρV³, where ρ represents air density and V denotes wind speed at 10 meters above sea level. Data from satellite-based sensors (GMI, SMAP, ASCAT, AMSR-2, SSMI) were validated against Copernicus reanalysis datasets and in-situ measurements from buoys operated by Taiwan’s Central Weather Administration (CWA). Results indicate that the Taiwan Strait, particularly offshore central Taiwan, is the most suitable area for offshore wind turbine installations, with monthly average wind speeds ranging from 13 to 16 m/s in December between 2015 and 2023. For solar energy assessment, Short Wave Radiation (SWR) data from JAXA’s Himawari geostationary satellites provided insights into the spatial distribution of solar radiation around Taiwan from 2015 to 2024. The analysis identified southwestern Taiwan as the most promising region for photovoltaic installations, with monthly average SWR values ranging from 230 to 280 W/m² in July. Topographic analysis using Earth Topography (ETOPO) data revealed that lower elevations (0–200 meters) are more suitable for photovoltaic systems than mountainous regions, further reinforcing the viability of the southwestern plains for large-scale solar energy projects. Validation of satellite-derived SWR values against ground-based Global Solar Radiation (GSR) measurements from the CWA indicated a consistent overestimation in the Himawari data, with an average difference of 37.2 MJ/m². Overall, this study provides valuable insights into the strategic siting of Taiwan's wind and solar energy infrastructure, supporting global decarbonization efforts and fostering the development of green energy.

How to cite: Wang, C.-Y. and Hsu, P.-C.:  Utilizing Satellite and Meteorological Data to Evaluate Potential Wind Farm and Photovoltaic Panel Sites Inland and Offshore Taiwan , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2999, https://doi.org/10.5194/egusphere-egu25-2999, 2025.

EGU25-3567 | ECS | Orals | ERE2.1

Investigation of low-level jets and their impacts on wind turbine performance in the southern North Sea using Doppler lidars 

Pauline Haezebrouck, Elsa Dieudonné, Anton Sokolov, Hervé Delbarre, Patrick Augustin, and Marc Fourmentin

Low-level jets (LLJs) are fast-moving air streams in the lower part of the troposphere, characterized by wind maxima and wind shear typically occurring at the same level as wind turbine rotors. Technological advances have enabled the design of taller and more efficient wind turbines, making LLJs at higher altitudes potentially significant for their performance. Evaluating LLJ characteristics and understanding their formation mechanisms is essential for accurately assessing turbine loads and power production.

In this context, three years of wind profiles obtained every 15 minutes from two Doppler lidars installed in Dunkirk, a coastal city in northern France, were used to detect LLJs up to 1,500 m. The study focused on assessing the frequency and main characteristics of LLJs in the region and identifying their formation mechanisms. Additionally, the study aimed to evaluate the impact of these jets on wind turbines, especially given the rapid development of offshore installations.

Results indicate that LLJs are a common atmospheric phenomenon, occurring 15 % of the time, predominantly on the nights of the spring and summer seasons. This suggests that frictional decoupling due to radiative cooling is a key factor in LLJ formation. However, the city's coastal location induces additional formation mechanisms driven by the land-sea thermal gradient and the proximity of the English Channel.

The results demonstrated that these jets impact wind turbines since 38 % of the LLJ cores are located in the rotor layer of the most commonly installed offshore wind turbines. However, LLJs are not necessarily beneficial for their power production as the high wind speeds they imply are confined to a relatively thin layer, while the wind outside of this layer exhibits relatively lower velocities. Jet shear has a minimal impact on these turbines since it is similar to the shear observed in non-jet conditions. Indeed, these turbines are mainly located within the surface layer, where ground-induced shear is predominant. On the contrary, future wind turbines will be more impacted by LLJs due to larger rotor sizes and will experience greater negative shear, leading to significant loads on their blades.

How to cite: Haezebrouck, P., Dieudonné, E., Sokolov, A., Delbarre, H., Augustin, P., and Fourmentin, M.: Investigation of low-level jets and their impacts on wind turbine performance in the southern North Sea using Doppler lidars, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3567, https://doi.org/10.5194/egusphere-egu25-3567, 2025.

EGU25-5236 * | Orals | ERE2.1 | Highlight

Probabilistic solar radiation forecasting across Europe using deep learning 

Angela Meyer, Kevin Schuurman, and Alberto Carpentieri

Solar energy plays a major role in climate change mitigation. With rising shares of solar power in the grid, short-term forecasts of surface solar irradiance (SSI) are becoming increasingly important for grid operators to enable cost-efficient supply and demand balancing. Solar nowcast models provide estimates of SSI from minutes to hours ahead. Accurate solar nowcasts are required across spatially extensive areas as most solar power is generated by decentralised photovoltaic systems. Such regional-scale SSI estimates can be derived from geostationary satellites, like Meteosat, that monitor Earth in visible and infrared bands. Existing regional-scale solar nowcast models are usually deterministic, lacking forecast uncertainty awareness, and require satellite Level-2 products of SSI as input obtained from radiation retrievals such as Heliosat. We present the first probabilistic regional-scale solar nowcast models, SolarSTEPS and SHADECast (Carpentieri et al., 2023, 2024), an autoregressive model and a generative diffusion model, that can be applied to regions ranging from tens to several thousand kilometers in extent. Our solar nowcast models improve forecast accuracy and reliability in all cloudiness conditions compared to existing models. SHADECast extends the forecast horizon of our state-of-the-art SolarSTEPS model by 26 minutes at lead times of 15 minutes to 2 hours. We also present a deep-learning-based emulator of Heliosat SARAH-3 (Pfeifroth et al., 2021) that estimates instantaneous SSI across Europe with similar accuracy as SARAH-3. We demonstrate that the emulator, a convolutional residual network, can even outperform SARAH-3 in SSI accuracy when a subsequent fine-tuning step is added in which the emulator is retrained on pyranometer stations, resulting in more accurate SSI initialisations for solar nowcast models. The emulator estimates SSI at kilometer-scale and 15-minute intervals based on visible and infrared images of Meteosat's Spinning Enhanced Visible and Infrared Imager. Pyranometers from BSRN, IEA-PVPS and European national weather services were employed for emulator fine-tuning and testing.

How to cite: Meyer, A., Schuurman, K., and Carpentieri, A.: Probabilistic solar radiation forecasting across Europe using deep learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5236, https://doi.org/10.5194/egusphere-egu25-5236, 2025.

EGU25-6695 | Orals | ERE2.1

Kilometer-scale regional atmospheric modelling reveals underestimation of onshore wind energy potentials over southern Africa 

Shuying Chen, Klaus Goergen, Harrie-Jan Hendricks Franssen, Christoph Winkler, Yoda Wahabou, Stefan Poll, Jochen Linssen, Harry Vereecken, Detlef Stolten, and Heidi Heinrichs

Wind energy is one pillar towards a decarbonized future energy system. A precondition for an efficient expansion and deployment of wind turbines is reliable and highly resolved information on wind energy potentials. Such detailed information is for example rare in many parts of Africa where it is crucially needed to explore large untapped renewable energy potentials. This study used a new high-resolution, kilometer-scale meteorological data set from dedicated ICON model atmospheric simulations in limited area mode over southern Africa (ICON-LAM). The wind speeds at hub height and wind energy potentials from ICON-LAM, the commonly used ERA5, and a statistical downscaling variant of ERA5 using the Global Wind Atlas (ERA5_GWA) were compared. The wind speed evaluation against weather mast measurements shows that ERA5 and ERA5_GWA underestimate hub-height wind speeds with a mean error (ME) of −1.8 m s−1 (−27%) and −0.3 m s−1 (−4.7%), respectively, while ICON-LAM has a ME of −0.1 m s−1 (−1.8%). Noteworthily, ICON-LAM especially outperforms ERA5 and ERA5_GWA by a large margin in simulating the most relevant range of wind speeds (from 11 m s−1 to 25 m s−1) for wind turbines. This leads to a 48% higher average wind energy potential derived from ICON-LAM compared to ERA5. Estimates based on the ERA5_GWA show a similar average wind energy potential to ERA5, resulting from the spatial heterogeneity of wind energy potential. Such an underestimation of wind energy potential may hinder local development and deployment of wind energy by undervaluing the economic payback, which again underlines the importance of using highly resolved atmospheric model simulations.

How to cite: Chen, S., Goergen, K., Hendricks Franssen, H.-J., Winkler, C., Wahabou, Y., Poll, S., Linssen, J., Vereecken, H., Stolten, D., and Heinrichs, H.: Kilometer-scale regional atmospheric modelling reveals underestimation of onshore wind energy potentials over southern Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6695, https://doi.org/10.5194/egusphere-egu25-6695, 2025.

The global target of net-zero emissions and carbon neutrality by the mid-21st century is accelerating the transition to clean energy. Accurately assessing solar energy potential requires high-quality hourly surface solar radiation (SSR) and direct radiation (Rd) datasets. This study evaluates hourly SSR and Rd data from two reanalysis products (ERA5 and MERRA-2) and three satellite-derived products (CERES, SARAH-E, and Solcast) against 22 years of homogeneous surface observations in China. This validation utilizes data from 96 stations for SSR and 17 stations for Rd, and includes both accuracy and stability tests: 

  • According to the accuracy test, SSR and Rdare often overestimated, with lower accuracy observed during sunrise and sunset. SSR exhibits larger seasonal variations in accuracy than Rd, with accuracy declining in the cold season. SARAH-E and ERA5 demonstrate the least overestimation of the diurnal cycle of SSR, indicating the highest accuracy. CERES and SARAH-E demonstrate the highest accuracy for Rd, with CERES underestimating and SARAH-E overestimating throughout the day.  
  • Decadal trends of SSR and Rdare also overestimated by most products. SSR stability is lower in the cold season compared to the warm season. Rd stability decreases notably in cloudy and polluted MERRA-2 and CERES exhibit the highest stability for SSR, while ERA5 demonstrates the highest stability for Rd.

In summary, as highlighted by the bold lines in Figure 1, ERA5 excels in capturing the diurnal cycle of SSR, and CERES demonstrates superior performance for Rd across China.  

                                                                                                                                         

Figure 1. Overall comparison of products over China for hourly surface solar radiation (a) and direct radiation (b), regarding accuracy index (nMABD, the normalized mean absolute bias deviation, %) and stability index (absolute decadal trend bias, % decadal–1). The performance of each product correlates positively with the size of its hexagon.

How to cite: Wang, H. and Wang, Y.: Evaluation of Hourly Solar Radiation Products for Solar Energy Applications over China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8062, https://doi.org/10.5194/egusphere-egu25-8062, 2025.

EGU25-8831 | ECS | Orals | ERE2.1

Near-ground meteorological variations induce by a single wind turbine in a realistic highly stratified stable atmosphere. 

Paul Boumendil, Pierre-Antoine Joulin, Quentin Rodier, and Valéry Masson

Numerical simulations, satellite observations, and field campaigns have demonstrated that wind turbine wakes can alter near-ground air temperature and humidity [Baidya Roy, 2004; Xie, 2017; Wu, 2023; Zhou, 2012; Smith, 2013; Rajewski, 2013; Takle, 2014; Armstrong, 2016; Archer, 2019]. In the wind turbine community, high-resolution large eddy simulations of wind turbine wakes often rely on idealized incident flows and surface conditions, which differ from real-world conditions. Since wind turbine wakes and near-ground air properties are highly sensitive to atmospheric and surface conditions, we employ an online coupling between a realistic atmospheric model, a soil–vegetation–atmosphere transfer model, and an aerodynamic technique based on body forces for the wake of wind turbine following the recommendations of Porté-Agel (2019). The ability of the multi-scale setup to reproduce realistic atmospheric conditions, as well as its capability to reproduce meteorological variations induced by wind turbines, has been validated (under review [Boumendil, 2025] and [Boumendil, 2024]) using measurements from the VERTEX campaign on a 2MW wind turbine turbine located on the East Coast of Delaware, USA [Archer, 2019; Wu, 2021]. Here, we extend this validated setup to investigate a highly stratified stable atmosphere, where wind turbine impacts are expected to be most pronounced.

We employed the atmospheric model Meso-NH [Lac, 2018], initialized and forced with analysis files. Using a grid-nesting configuration, we simulate scales ranging from the mesoscale, capturing diurnal cycles, to the microscale, resolving the flow behavior around wind turbines while accounting for realistic features such as orography, surface cover, clouds, and radiation.

An online coupling with the SURFEX [Masson, 2013] soil–vegetation transfer model is employed to finely model surface properties such as albedo, surface fluxes, ground roughness, or leaf area index depending on land cover. A high-resolution surface database, combining data from OpenStreetMap with the ECOCLIMAP nomenclature [Champeaux, 2005] is uses as inputs for the surface modelling platform SURFEX. Additionally, the effects of wakes from trees [Aumond, 2013] and urban buildings [Schoetter, 2020] were incorporated through added drag forces. The wake of the wind turbine is modeled using an Actuator Disk with Rotation, where rotation speed, blade pitch angle, and rotor direction are updated during the simulation by a controller.

In the highly stratified stable atmosphere, Meso-NH captures the strong near-ground temperature inversion and the wind veer within the rotor area. The interaction between the wake of the wind turbine and the stable atmosphere results in pronounced temperature variations, with warming in the lower rotor area and cooling above. This case study highlights the ability of the model to investigate wind turbine interactions with realistic atmospheric conditions, paving the way for further case studies.

How to cite: Boumendil, P., Joulin, P.-A., Rodier, Q., and Masson, V.: Near-ground meteorological variations induce by a single wind turbine in a realistic highly stratified stable atmosphere., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8831, https://doi.org/10.5194/egusphere-egu25-8831, 2025.

EGU25-9336 | ECS | Orals | ERE2.1

The role of North Atlantic Oscillation teleconnections in solar irradiance nowcasting error variability 

Swati Singh, Sylvain Cros, and Jordi Badosa

The movement and dynamics of clouds significantly impact solar radiation and energy production from photovoltaic (PV) systems. Short-term solar irradiance forecasts, ranging from hours to days, are essential for reliable energy supply through PV plants. Forecasts using geostationary satellites outperform numerical weather prediction models for intraday forecasts. However, forecast accuracy depends heavily on prevailing weather conditions.

The North Atlantic Oscillation (NAO), a key teleconnection over the Euro-Atlantic region, significantly shapes weather patterns in western Europe and impacts the accuracy of satellite-based solar irradiance forecasts. The present study analyzes eight years (2016-2024) of Global Horizontal Irradiance (GHI) forecasts at the SIRTA Observatory in Palaiseau, near Paris (France). The forecasts are generated four hours ahead with 15-minute time step using a cloud motion vector (CMV) computation to extrapolate the cloud over. These forecasts are validated against pyranometer observations. GHI forecast errors are analyzed for two periods (2016-2020 and 2020-2024), focusing on seasonal variations and the impact of NAO teleconnection indices provided by the Climate Prediction Center of the National Centers for Environmental Prediction (NCEP CPC).

The GHI forecast error values were averaged across all forecast horizons (0 to 240 minutes). The results indicated that the relative root mean square mean error (RRMSE) is 32.7% for spring and autumn seasons from 2016 to 2024. NAO+ and NAO- teleconnection indices are respectively associated with lower (29.5%) and higher (36.2%) RRMSE values across spring and autumn seasons and both time periods (2016-2020 and 2020-2024). NAO+ events are characterized by anticyclonic circulations over the Atlantic Ocean, bring reduced precipitation and stable weather across Europe, resulting in clearer skies and lower forecast errors. Conversely, NAO- events lead to higher errors due to less stable conditions. These findings are particularly significant as North Atlantic weather regimes, typically reliable predictors of forecast errors, appear less effective during transitional seasons like spring and autumn.

In winter and summer seasons, distinct patterns in GHI forecast errors were observed. During the winter of 2016-2020, NAO+ and NAO- events yielded higher (44.5%) and lower RRMSE in GHI forecast (31%), respectively. This trend reversed during the winter of 2020-2024, with NAO+ and NAO- events respectively, showed lower (43%) and higher (49%) RRMSE values. These seasonal variations during winter align with changes in the frequency of NAO events from 2020-2024, when NAO- occurrences increased while NAO+ occurrences decreased. During summer, similar seasonal trends were observed, though with reversed magnitudes during both NAO+ and NAO- regimes for 2016-2020 and 2020-2024.

Changes in GHI forecast errors emphasize the importance of understanding large-scale atmospheric patterns for a better interpretation of GHI forecasts. Errors linked to NAO indices in winter and summer should be further studied, as they may also be influenced by other teleconnections and weather regimes. As a dominant teleconnection over Europe and the Atlantic, advanced knowledge of NAO indices and their interaction with other weather systems helps in anticipating forecast errors, offering critical insights for energy traders and grid operators to enhance smart grid management.

 

How to cite: Singh, S., Cros, S., and Badosa, J.: The role of North Atlantic Oscillation teleconnections in solar irradiance nowcasting error variability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9336, https://doi.org/10.5194/egusphere-egu25-9336, 2025.

EGU25-9925 | ECS | Posters on site | ERE2.1

The impact of sudden stratospheric warmings on electricity consumption and wind power generation in Finland 

Veera Juntunen, Timo Asikainen, Antti Salminen, and Mikhail Vokhmianin

In Arctic countries, a large fraction of wintertime electricity consumption is used for heating spaces and, thus, the electricity consumption is highly sensitive to outside temperature variations. Also, the production of electricity by wind turbines depends directly on surface wind speed. Wintertime weather in Northern Europe is significantly influenced by the state of the stratospheric polar vortex, the westerly wind pattern circulating the polar region during winter. When the polar vortex is strong (weak), winter temperatures are more likely mild (cold) and surface wind speeds are higher (lower) in Northern Europe.

Sudden stratospheric warmings (SSWs) are, as the name implies, events where stratospheric temperature abruptly increases due to significant weakening or breaking of the polar vortex. This usually causes a sudden outbreak of cold and less windy weather in Northern Europe which can last for weeks. The occurrence probability of SSW events during the winter season is affected by several factors, e.g., the phase of the so called Quasi-Biennial Oscillation (QBO). During easterly QBO phase, characterized by equatorial stratospheric zonal winds flowing from east towards west, more planetary waves are guided to the polar stratosphere where they weaken the stratospheric polar vortex. As a result, the probability for SSW events is higher in easterly QBO phase compared to the westerly phase.

Here we study Finland’s electricity consumption and wind power generation separately in winters with and without an SSW in different QBO phases. We find that the electricity consumption is significantly higher in winters with SSWs compared to winters where an SSW does not happen, while the opposite is true for the wind power generation. We also evaluate the uncertainties of seasonal predictions of electricity consumption and wind power generation based on seasonal predictions of SSW probability.

How to cite: Juntunen, V., Asikainen, T., Salminen, A., and Vokhmianin, M.: The impact of sudden stratospheric warmings on electricity consumption and wind power generation in Finland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9925, https://doi.org/10.5194/egusphere-egu25-9925, 2025.

EGU25-10807 | ECS | Orals | ERE2.1

Assessment of CAMS Radiation Service over France in different sky conditions 

Diego Rodrigues de Miranda, Faiza Azam, Jorge Lezaca, Yves-Marie Saint-Drenan, and Marion Schroedter-Homscheidt

The assessment of solar irradiance variability is relevant for evaluating irradiance-based models, resource assessment and forecasting applications in the solar energy field. One well-established irradiance-based model database for solar project development is the Copernicus Atmosphere Monitoring Service (CAMS) through its CAMS Radiation Service (CRS) that offers historical all-sky solar irradiance estimates. In this work, the accuracy of the CRS GHI product over France is evaluated under different irradiance variability conditions by applying a sky condition classification method based on 1-minute Global Horizontal Irradiance (GHI) observations. A dense network of GHI measurements over France with more than 230 ground stations in the year 2015 is used as a case study.

The classification method is based on a visual interpretation of GHI measurement patterns for the Baseline Surface Radiation Network (BSRN) station of Carpentras during the years 2012 and 2013, which forms a reference database. This reference database is composed of 280 manually classified hours in minute resolution for GHI into eight different classes (from clear sky to variable and overcast sky conditions). Ten variability indices (VIs) are applied in the classification scheme including the clear sky index (kc); the average, maximum and standard deviation of the absolute values for the first derivative of kc; the VIs proposed by Stein et al. (2012) and Coimbra et al. (2013); VIs based on envelopes curves obtained according to the local maxima and minima time-series; and three VIs that counts GHI values overpassing the clear sky irradiance in 3%, 5% and 10%. The classification model consists of three main steps: a discrimination filter, a probability classification approach and a median distance-based approach. The discrimination filter is a counting step that checks if the VIs are inside the Carpentras reference database domain for a particular class. The class with the most VIs will be the selected class. If the maximum number of VIs counted is the same for two or more classes, then a probability classification approach makes the class decision. This probability approach uses Kernel density estimation to calculate the neighborhood probability of a specific VI to be part of one of the eight classes. The class with the higher mean probability over all classes will be selected. Finally, for all the cases outside the domain of the reference database, the median distance-based approach with normalized VIs is applied as presented by Schroedter-Homscheidt et al. (2018). 

The evaluation of the CRS GHI over France is shown in Figure 1. The highest values of the Root Mean Square Deviation (RMSD) are found in class 6, which is mostly dominated by broken clouds. Also classes 4, 7 and 8 present large RMSD. The identification of this broken cloud conditions cluster is useful for further developments of the CRS algorithm in these challenging situations. 

 

 

 

Figure 1 – CRS RMSD in different sky conditions over France (hourly resolution).

How to cite: Rodrigues de Miranda, D., Azam, F., Lezaca, J., Saint-Drenan, Y.-M., and Schroedter-Homscheidt, M.: Assessment of CAMS Radiation Service over France in different sky conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10807, https://doi.org/10.5194/egusphere-egu25-10807, 2025.

EGU25-11305 | Orals | ERE2.1

A Large Eddy Simulation using the WRF model over the sea: a real case study of a storm 

Sima Hamzeloo, Xiaoli Guo Larsén, Alfredo Peña, and Jana Fischereit

There are very few studies in which the WRF model is used under Large Eddy Simulation (WRF-LES) mode for real time, offshore conditions. This study utilizes WRF-LES to investigate the wind characteristics during a real storm over the North Sea, west of the Danish Jutland coast. A WRF-based multiscale simulation was conducted to examine the storm, which is characterized by strong south-westerly winds, representing open ocean conditions. The simulation setup comprised four nested domains: three outer domains at mesoscale resolution (9.9 km to 1.1 km, domain 1 to 3) and an innermost domain running in LES mode (spatial resolution 100 m, domain 4). ERA5 reanalysis was used to drive the outermost mesoscale domain, while the other were one-way nested domains.

Results from the LES domain, domain 4, were compared to those from the finest mesoscale domain, domain 3. Lidar measurements of wind speed and direction from 40~m to about 250 m inside the studied domain are used to evaluate the simulations. Compared to the results from domain 3, the simulated vertical profiles of wind speed from the LES domain aligned more closely with the measurements up to a height of 150 m. At higher elevations, the profiles from the mesoscale and WRF-LES output converged, with both outputs overestimating the wind speeds. The wind directions were well simulated in both mesoscale and Les domains. The performance of the mesoscale and WRF-LES output in comparison with measurements is further explored using time series analysis at multiple heights. 

How to cite: Hamzeloo, S., Guo Larsén, X., Peña, A., and Fischereit, J.: A Large Eddy Simulation using the WRF model over the sea: a real case study of a storm, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11305, https://doi.org/10.5194/egusphere-egu25-11305, 2025.

EGU25-11490 | ECS | Orals | ERE2.1

Leveraging Spatially Explicit Data for Accurate Renewable Energy Forecasting in France 

Eloi Lindas, Yannig Goude, and Philippe Ciais

To meet France’s CO2 emission reduction of 33 % by 2030 compared to 1990 and reach greenhouse gas neutrality in 2050, sustainable energy sources are key to clean power production and reduced emissions from the energy sector. However, non-dispatchable renewables such as wind and solar photovoltaic (PV) power require accurate forecasts to improve their grid stability, reliability, and penetration level not to mention supply-demand matching. Indeed, those sources are dependent on weather conditions such as solar radiation or wind speeds, making their load highly variable and challenging to balance for grid operators.
Despite the increase of data availability from both weather and energy fields, regional wind and PV supply forecasts are usually indirect. Either a bottom-up approach of plant-level forecasts or a time series prediction incorporating lagged values is used. The potential of spatially explicit data for direct prediction is still underestimated. In this work, we present a methodology for predicting solar and wind power production at the country scale in France using machine learning models trained with spatially resolved weather data combined with geospatial information about production sites’ capacity.

A dataset spanning from 2012 to 2023 is built, using daily power production data from the national grid operator as the target variable, with daily weather data from ERA5, the capacity and location of the production sites, and electricity prices as input features. Three modeling approaches are explored to handle spatially resolved weather data: spatial averaging over the country, dimension reduction through principal component analysis, and a convolutional neural network (CNN) architecture to exploit complex spatial patterns. We benchmarked state-of-the-art machine learning models such as tree-based architectures, additive models, and neural networks on daily power supply for the midterm horizon. Hyperparameter tuning procedures based on different cross-validation methods were also investigated to reach the lowest generalization error possible.

Despite the variance introduced by the model and the data, our cross-validation experiments showed that while using one-to-one models on the spatial average of weather data, the time-series dedicated procedures tend to estimate the generalization error better than standard methods like K-Fold. This allowed us to push the model calibration to reach the best performance on unseen test data. However, they fall short of the CNN ingesting entire weather maps which predicts twice as good. Indeed, CNN is the best model for both PV and wind, achieving errors of around 5 %. This is mainly due to its ability to exploit spatial weather patterns on production site locations to extrapolate the trend in renewable power supply as underlined by an interpretability method. In fact, one-to-one models utilized on both spatial average and principal components extracted from weather maps are struggling to grasp the increase in power supply due to the growth in installed capacity.

Our study highlighted the potential of spatially explicit data and dedicated models to improve the accuracy of direct regional renewable power supply. Such enhancements will lead to a better supply-demand balance while incorporating a growing part of sustainable energy into our electricity mix.

How to cite: Lindas, E., Goude, Y., and Ciais, P.: Leveraging Spatially Explicit Data for Accurate Renewable Energy Forecasting in France, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11490, https://doi.org/10.5194/egusphere-egu25-11490, 2025.

EGU25-12210 | Posters on site | ERE2.1

Saharan Dust and Solar Energy: Quantifying Forecasting Challenges in Hungary’s Rapidly Growing PV Sector 

Ágnes Rostási, Fruzsina Gresina, András Gelencsér, Adrienn Csávics, and György Varga

Accurate forecasting of weather-dependent renewable energy production is vital for energy security and economic stability, especially in regions undergoing rapid photovoltaic (PV) energy expansion. This study investigates the impact of Saharan dust events (SDEs) on PV power generation forecasts in Hungary, a leading European country in terms of PV penetration. Utilising a comprehensive dataset comprising 46 identified SDEs from 2020 to 2023, the research quantifies forecast errors and production deviations under dusty and non-dusty conditions. The analysis reveals that current forecasting models fail to account for dust-related impacts, resulting in significant errors in day-ahead scheduling. During SDEs, PV generation deficits and surpluses were found to be 30.9% and 17.6% higher than during non-dusty periods, respectively. On deficit days, the primary factor reducing irradiance was found to be unforeseen cloud cover, particularly extensive cirrus clouds. Conversely, on days with surplus PV generation, reduced radiative forcing from cirrus clouds, along with the replacement of anticipated stratus and scattered radiation from dusty atmospheres, contributed to prolonged irradiance. These findings underscore the dual impact of atmospheric dust, directly decreasing irradiance and indirectly altering cloud formation mechanisms, which are not adequately captured in current PV production models.

The study emphasises the necessity to incorporate dust-specific atmospheric models and refine dust-cloud interaction parameterisations in energy forecasts. This is of particular relevance as Hungary and other regions increase their reliance on PV energy within their renewable energy portfolios. The research also has broader implications for grid stability, energy policy, and climate change mitigation, highlighting the necessity for accurate and adaptable forecasting systems to address the growing challenges posed by atmospheric variability.

The research was supported by the FFT NP FTA and NRDI projects FK138692, TKP2021-NKTA-21 and RRF-2.3.1-21-2021.

How to cite: Rostási, Á., Gresina, F., Gelencsér, A., Csávics, A., and Varga, G.: Saharan Dust and Solar Energy: Quantifying Forecasting Challenges in Hungary’s Rapidly Growing PV Sector, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12210, https://doi.org/10.5194/egusphere-egu25-12210, 2025.

EGU25-12864 | Orals | ERE2.1

Doppler Lidar Provide New Insights into the Wind Resource over Forests  

Sonia Wharton, Matteo Puccioni, Stephan De Wekker, Robert Arthur, and Jerome Fast

The atmospheric boundary layer above forest canopies is difficult to measure in practice, and our understanding of its flow physics, including the potential wind resource, is limited in part by observational constraints. Most available datasets come from tower point measurements, which do not generally reach into heights encountered by a turbine rotor, or from remote sensing measurements, which are usually located outside of the forest in a clearing and thus do not accurately represent flow conditions above the canopy. Here, we present a field campaign that deployed four Doppler lidars in a U.S. Appalachian Forest including installment on top of a 30 m tall tower. These lidars allow for wind measurements across tall turbine rotor heights to be made directly above forested regions. Nearby wind turbines in the wooded Appalachians have hub-heights approaching 90 m and rotor diameters of 127 m, with maximum and minimum blade heights of 152 m and 25 m, respectively. We describe the experimental set-up, lidar strategies, adjoining radiosonde and UAS IOPs, and novel use of AI to drive optimal lidar scans. These data are being collected as part of the DOE “Addressing Challenges in Wind Forecasting for Tall Turbines Across Regions with Terrain and Land Surface Heterogeneity” project and will be used for analysis of forest-atmosphere interactions and numerical model validation.

How to cite: Wharton, S., Puccioni, M., De Wekker, S., Arthur, R., and Fast, J.: Doppler Lidar Provide New Insights into the Wind Resource over Forests , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12864, https://doi.org/10.5194/egusphere-egu25-12864, 2025.

EGU25-13201 | Posters on site | ERE2.1

The Digital Twins for Winds-Offshore (DTWO) Project 

Xiaoli Larsén and the DTWO consortium

What kind of tools are needed for accurate and precise forecasting of offshore wind power, in an unprecedented fast development of offshore wind and market, now and near future, for the key stakeholders?

The DTWO project aims to be pioneering initiative in the digitalization of offshore wind energy by combining

  • Federated digital twin architecture, allowing users to customize without sharing sensitive data;
  • Seamless model integration of a wide array of existing models and data sources from regional weather model, to wind farm and turbine wakes, to marine environment conditions, to wind resource, energy yield and design parameters, to turbine performance and life time, and to grid balancing and energy market;
  • Granular prediction capabilities by implementing latest scientific outcomes and technology;
  • High-level cybersecurity, addressing concerns around data vulnerability in digital transformation efforts.

DTWO’s federated digital twin platform includes five modules for Earth, Wakes, Siting, Turbines and Grids. DTWO provides a data hub with FAIR and conditionally open data, and a tool hub featuring open and conditionally open tools. The digital twin modules are implemented using industrial use cases, tested through representative test scenarios.

DTWO brings together the expertise of the world’s leading offshore wind industries, alongside research centres, IT consulting and digital service providers, academic institutions, a science communication organisation, energy forecasting experts, and meteorological centres. The project website provides more information about the development of the European Horizon supported project https://dtwo-project.eu/.

Codes for organizations: 1. DTU; 2. VKI; 3. DHI; 4. ECMWF; 5. SSP; 6. ICONS; 7. PG; 8. Fraunhofer-IWES; 9. ENFOR; 10. KNMI; 11. SGRE 

How to cite: Larsén, X. and the DTWO consortium: The Digital Twins for Winds-Offshore (DTWO) Project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13201, https://doi.org/10.5194/egusphere-egu25-13201, 2025.

EGU25-13278 | Orals | ERE2.1

Improving Wind Power Forecasting with Meteomatics High-Resolution Model Resolving Wind Turbine Wake Effects 

Julie Thérèse Villinger, Johannes Rausch, Lukas Umek, Christian Schluchter, Marco Thaler, Julia Schmoeckel, Robert Hutchinson, and Martin Fengler

Wind energy production depends heavily on weather conditions, and the growing deployment of wind turbines in complex terrain and offshore locations presents considerable forecasting challenges. Current numerical weather prediction (NWP) models often struggle to provide accurate forecasts in these environments due to limited spatial and temporal resolutions, infrequent model updates, and the lack of representation of wind turbine induced wake effects on atmospheric flows. These limitations lead to inaccuracies in power production forecasts, impacting the efficiency and reliability of renewable energy systems.

To address these limitations, Meteomatics has developed an operational high-resolution NWP model featuring a horizontal grid spacing of 1 km and an hourly update frequency. This model integrates data from Meteomatics' proprietary network of Meteodrones, along with traditional data sources such as ground-based weather stations, radar, satellite observations, and radiosondes. Meteodrones are small unmanned aircraft systems capable of collecting vertical atmospheric profiles up to altitudes of 6000 m.

Here, the impact of recent enhancements implemented in to Meteomatics' high-resolution NWP model on wind power forecasting is evaluated. Key updates include an extension of the forecast lead time to 72 hours and an increase in temporal resolution to 15-minute intervals, aligning with the interval used in energy trading. Additionally, the model's domain, covering the pan-European region (EURO1k), has been expanded with the introduction of a new domain covering the North American continent (US1k). Importantly, the model now incorporates a parameterization of wind turbine effects, enabling accurate representation of wind wake phenomena. The findings highlight the critical role of state-of-the-art high-resolution numerical weather forecasting in improving the cost efficiency of wind energy production. These advancements facilitate greater integration of wind energy into the broader energy mix, thereby contributing to a reduction in CO2​ emissions and supporting the transition to sustainable energy systems.

How to cite: Villinger, J. T., Rausch, J., Umek, L., Schluchter, C., Thaler, M., Schmoeckel, J., Hutchinson, R., and Fengler, M.: Improving Wind Power Forecasting with Meteomatics High-Resolution Model Resolving Wind Turbine Wake Effects, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13278, https://doi.org/10.5194/egusphere-egu25-13278, 2025.

EGU25-13836 | ECS | Posters on site | ERE2.1

Using the CAMS solar radiation time-series product to model solar PV power potential. Uncertainty evaluation under diverse atmospheric conditions using ground-based measurements. 

Nikolaos Papadimitriou, Ilias Fountoulakis, Antonis Gkikas, Kyriakoula Papachristopoulou, John Kapsomenakis, Stelios Kazadzis, Andreas Kazantzidis, and Christos S. Zerefos

The decarbonization of the power sector is among the most challenging tasks in the effort to mitigate climate change and achieve the 7th United Nations Sustainable Development Goal (SDG-7) for Affordable and Clean Energy by 2030. The rapid growth in the installed capacity of solar photovoltaics (PV) in recent years, driven by their cost-effectiveness, highlights their potential as a promising technology for large-scale transitions. However, solar energy is a variable source, the availability of which depends strongly on atmospheric conditions, particularly clouds and aerosols. Therefore, assessing the expected power output is essential for planning sustainable investments, such as the installation and maintenance of solar farms, while reliable solar power forecasting is crucial for their integration into energy supply grids. The Copernicus Atmospheric Monitoring Service (CAMS) solar radiation time-series product provides historical data for the global horizontal irradiance, along with its components, including direct and diffuse, which renders it suitable for performing estimations of the produced energy from photovoltaics. We use the Global Solar Energy Estimator (GSEE), a widely used open-access model for simulating solar plants, aiming to evaluate the use of CAMS solar radiation time-series product for estimating the solar PV power potential. More precisely, we compare the CAMS-based solar power generation with the output from simulations derived using ground-based actinometric measurements of the direct and diffuse surface solar radiation components that were available at five BSRN sites in Europe and North Africa, obtained from stations with quite different prevailing aerosol and cloudiness conditions. The analysis has been performed for photovoltaics that are positioned at fixed tilt angles and on solar tracking systems. CAMS solar radiation product is widely used to simulate the PV power potential and thus the findings of this study provide valuable insights from the reliability of using it for such assessments.

How to cite: Papadimitriou, N., Fountoulakis, I., Gkikas, A., Papachristopoulou, K., Kapsomenakis, J., Kazadzis, S., Kazantzidis, A., and Zerefos, C. S.: Using the CAMS solar radiation time-series product to model solar PV power potential. Uncertainty evaluation under diverse atmospheric conditions using ground-based measurements., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13836, https://doi.org/10.5194/egusphere-egu25-13836, 2025.

EGU25-14067 | ECS | Posters on site | ERE2.1

AI-Driven Power Forecasting for Renewable Energy: A Multi-Terrain Analysis from Shandong Province Wind Farms 

Guiting Song, Veeranjaneyulu Chinta, and Kailong Wu

Shandong Province, a critical hub for renewable energy in China, presents a diverse set of challenges and opportunities in wind power development. The region's wind farms span inland plains, coastal plains, and hilly terrains, with installed capacities ranging from 28,400 kW to 800,000 kW. While these diverse landscapes offer significant potential for wind power, several challenges persist, including grid integration issues, regulatory inconsistencies, and the need for advanced technologies to enhance energy efficiency. Additionally, social acceptance concerns related to environmental impacts further complicate the development of renewable energy projects. This study leverages wind and power data from multiple wind farms in Shandong Province to develop machine learning-based power forecasting models. Specifically, Random Forest (RF), eXtreme Gradient Boosting (XGBoost), and Long Short-Term Memory (LSTM) networks are employed to address spatiotemporal variability in wind power generation across diverse terrains. Results highlight the influence of geographic and meteorological factors on forecasting accuracy and underscore the potential of AI-driven approaches to mitigate uncertainties associated with wind power integration into the grid. Our findings demonstrate that terrain-specific modeling, coupled with advanced forecasting techniques, can significantly improve the reliability of wind power generation in complex environments. By addressing key challenges unique to Shandong Province, this research contributes valuable insights into sustainable energy planning and the broader integration of renewable energy into China's power grid.

How to cite: Song, G., Chinta, V., and Wu, K.: AI-Driven Power Forecasting for Renewable Energy: A Multi-Terrain Analysis from Shandong Province Wind Farms, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14067, https://doi.org/10.5194/egusphere-egu25-14067, 2025.

In the process of tower photothermal power generation, solar radiation undergoes the attenuation of the whole atmosphere, reaches the heliostat and then is reflected to the heat collector. The transfer of solar radiation from the heliostat to the heat collector occurs at an altitude of 0 to 300m from the ground, which is defined to be the near-surface layer in this study and is concentrated with high aerosol loadings. Thus, the extinction effects of near-surface aerosols are crucial in the site selection of photothermal power generation and in the evaluation of photothermal power generation efficiency.

In this work, we first analyzed the vertical distribution of near-surface aerosol extinction over North China (NC) and its correlation with meteorological factors. CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) is a satellite-borne lidar instrument aboard CALIPSO satellite, which provide globally aerosol vertical profiles with unprecedented coverage and spatial resolution. To circumvent data scarcity of longer-term in situ surface measurement of aerosol vertical profiles over the NC region, here CALIOP Level 2 version 4.1 aerosol profile product at 532 nm from January 2019 to December 2019 were adopted. The screened daytime CALIOP L2 data over the NC region were assigned and aggregated into horizontal grids with a resolution of 0.5°×0.5°. The vertical distribution of aerosol extinction coefficient reveals that in winter, Spring and autumn, the aerosol extinction values from near surface to about 1.5km are significantly higher than that above 1.5km. Especially in winter, high aerosol extinction values are found below 1km, indicating weak vertical mixing in winter. The relatively constant aerosol extinction values from near surface to above 2km indicates a higher well-mixed planetary boundary layer (pbl) height in summer. Aerosol extinction between 0-300m accounts for 32%, 17%, 9% and 20% of the aerosol extinction of the whole atmosphere in winter, spring, summer and autumn separately. PM2.5 concentration and surface relative humidity are positively correlated with near-surface aerosol extinction (r=0.4 and 0.31 respectively). Meanwhile, surface visibility is negatively related to the near-surface aerosol extinction (r=-0.45).

Then the aerosol extinction coefficient in the near-surface layer was adopted in the SMARTS model and we simulated the radiation transfer between 0 to 300m under different weather conditions. Simulation results of SMARTS model considered near-surface aerosol extinction are closer to radiation observations of a 325m meteorological tower in Beijing than the results of the original SMARTS model under all typical weather conditions.

Knowledge of the attenuation of aerosol to solar radiation from the heliostat to the heat collector in the process of tower photothermal power generation is of critical economic importance for the site selection of power station and the evaluation of power generation efficiency.

How to cite: Jia, B., Shen, Y., and Wang, C.: Vertical distribution of near-surface aerosol extinction over North China and its impacts on tower photothermal power generation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14324, https://doi.org/10.5194/egusphere-egu25-14324, 2025.

EGU25-15415 | ECS | Posters on site | ERE2.1

The IEA Wind TCP Task 51 Austria - Stakeholder interaction and priorities for forecasts 

Anna-Maria Tilg, Irene Schicker, Lukas Strauss, Florian Mader, Alexander Niederl, Jakob Messner, and Corinna Möhrlen

This work presents key findings from the first Austrian workshop of IEA Wind TCP Task 51 on "Forecasting for the Weather-Driven Energy System", which brought together 120 participants from over 50 organizations. Through structured stakeholder engagement, the workshop revealed critical priorities for advancing renewable energy forecasting in complex terrain.

Results highlight the continued dominance of day-ahead forecasting (56% of respondents), while identifying growing needs in extreme weather prediction (85% concerned) and artificial intelligence integration (rated 4.35/5 in importance). On the other hand, a number of gaps were identified related to the awareness of extremes and uncertainty and the knowledge and implementation status of such forecast tools. The Alpine context presents unique challenges, where complex terrain and cross-border power flows create specific forecasting requirements. Based on stakeholder feedback, two follow-up workshops will be organised focusing on extreme events and integrated forecasting solutions.

This study provides concrete guidance for developing next-generation forecasting systems and demonstrates the value of structured stakeholder engagement in shaping forecasting solutions for the energy transition.

How to cite: Tilg, A.-M., Schicker, I., Strauss, L., Mader, F., Niederl, A., Messner, J., and Möhrlen, C.: The IEA Wind TCP Task 51 Austria - Stakeholder interaction and priorities for forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15415, https://doi.org/10.5194/egusphere-egu25-15415, 2025.

EGU25-16488 | ECS | Orals | ERE2.1

Interfacial Gravity Waves from a Single Wind Turbine in a Conventionally Neutral Boundary Layer 

Pierre-Antoine Joulin and Valéry Masson

Over the sea, the atmospheric boundary layer is often capped by a shallow, thin, and stable layer, known as the capping inversion, beneath the stable free atmosphere. As offshore wind turbines grow taller, interactions with these stratified layers may become more frequent. Under specific atmospheric conditions, such interactions can generate gravity waves, potentially affecting wind farm performance and environmental impacts.

In his 2010 work, Smith notably highlighted the potential for wind farms to induce gravity waves. Since then, the need to better understand interactions between the atmospheric boundary layer and wind turbines has grown, driven by efforts to optimize the efficiency and design of wind farms. Numerical methods, particularly those employing mesoscale models, have become essential tools for addressing these challenges. Several studies have confirmed the ability of wind farms to excite gravity waves. However, most research has focused on entire wind farms, with limited attention to the specific dynamics of gravity waves generated by individual turbines. A finer-scale understanding of the generation, propagation, and interaction of waves emitted by single turbines within a farm would provide a more comprehensive basis for modeling and analysis at larger scales.

This study aims to improve the understanding and characterization of interfacial gravity waves induced by a single wind turbine operating within conventionally neutral boundary layers. Using the Meso-NH model—capable of decameter-scale atmospheric simulations within a Large Eddy Simulation framework—and its coupling with EOL, an actuator-based aerodynamic model, this work quantifies the properties of gravity waves under various atmospheric conditions and wind turbine configurations. These results will not only help to improve engineering models for estimating production, by better representing wind flow and wind turbine wakes on farms, but also to assess their potential impact on meteorology.

How to cite: Joulin, P.-A. and Masson, V.: Interfacial Gravity Waves from a Single Wind Turbine in a Conventionally Neutral Boundary Layer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16488, https://doi.org/10.5194/egusphere-egu25-16488, 2025.

EGU25-16750 | Posters on site | ERE2.1

Evaluating Global and Regional Weather Models for Solar Energy Forecasting in West Africa: A Case Study in Burkina Faso 

Amélie Solbès, Emmanuel Cosme, Damien Raynaud, and Sandrine Anquetin

The potential for photovoltaic energy in West Africa is high, and the use of this resource is expected to grow in the future. Due to the variability of solar energy, accurate weather forecasts are essential to ensure the smooth operation of the electricity network. In this region, the primary weather prediction challenges include the West African monsoon and the advection of dust from the nearby Sahara Desert.

Currently, SteadySun – a company specializing in power and weather forecasts for renewable energies – relies on low to medium-resolution global models to predict GHI (Global Horizontal Irradiance) for West Africa. It has been previously shown that weather models with higher horizontal resolution provide a more realistic representation of small-scale weather phenomena such as convective clouds. Most global models only take into account aerosols concentration through a monthly climatology which does not give information on AOD (Aerosol Optical Depth) variations on small temporal scales. Given the specific characteristics of the West African climate, employing high-resolution models that account for hourly dust concentration is likely to enhance the forecasting system.

This study aims to assess the benefits, limitations, and differences in GHI predictions from five global models and one high-resolution regional model over Burkina Faso. The five global weather models include IFS (ECMWF), GFS (NOAA), and ICON (DWD), which provide simulations with hourly outputs, as well as ARPEGE (Météo-France) and GDPS (CMC), which provide simulations with 3-hourly outputs. The regional weather model used is an augmentation of the weather model WRF for solar energy forecasting: WRF-Solar (NCAR). It features a spatial resolution of 3 km, outputs data every 15 minutes and integrates hourly aerosol optical depth forecasting data from the global atmospheric composition forecast production system CAMS (ECMWF).

The WRF-Solar forecast is expected to deliver improved accuracy during dust advection events and more realistic variability during cloud passages, potentially benefiting the planned forecasting system. However, the absence of data assimilation in WRF-Solar could result in misplaced convection cells, among other inaccuracies. On the other hand, the global models, with their varied physics and resolutions, may offer some advantages under specific weather conditions. This initial evaluation could also identify models that are less suitable for integration into the planned forecasting system.  To perform this assessment, GHI data with a spatial resolution of 3 km and temporal resolution of 15 minutes, derived from MSG (EUMETSAT) satellite imagery, will be used. Two assessment periods have been defined: the first during the monsoon season (July to September 2023) and the second during the dry season (January to March 2024), when dust advections from the Sahara Desert are common.

How to cite: Solbès, A., Cosme, E., Raynaud, D., and Anquetin, S.: Evaluating Global and Regional Weather Models for Solar Energy Forecasting in West Africa: A Case Study in Burkina Faso, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16750, https://doi.org/10.5194/egusphere-egu25-16750, 2025.

EGU25-17120 | ECS | Posters on site | ERE2.1

Assessment of Medium-Range and Sub-Seasonal Ensemble Forecasts of Solar Irradiance and Wind Speed Over China: Applications for Renewable Energy 

Chen Qian, Tony Song, Veeranjaneyulu Chinta, and Kailong Wu

Renewable energy development in China relies heavily on accurate forecasts of surface solar irradiance and 10-meter wind speed. This study evaluates the medium-range and sub-seasonal forecast performance of the European Centre for Medium-Range Weather Forecasts operational ensemble (ECMWF-ENS) over China. Forecast data, provided at a 6-hour time step, are assessed against gridded observational datasets from the China Meteorological Administration (CMA). Using metrics such as mean absolute error, root mean square error, and mean bias error, the study examines the forecast accuracy across different seasons and regions in China. Results reveal that the ensemble forecasts effectively capture diurnal cycles and regional variability in solar irradiation and wind speed. However, forecast errors vary significantly based on the climate variable and time of year, with solar irradiation forecasts generally demonstrating higher accuracy during summer months. The study highlights the role of the atmosphere in modulating solar and wind energy potential, emphasizing the critical need for accurate, high-resolution forecasts to support renewable energy applications. The findings demonstrate that spatially continuous hourly predictions can reconstruct regional-scale variations, providing valuable insights for optimizing site selection for solar and wind power plants. This research underscores the importance of reliable medium-range and sub-seasonal forecasting systems for advancing renewable energy planning and addressing China's growing energy demands while supporting climate adaptation strategies.

How to cite: Qian, C., Song, T., Chinta, V., and Wu, K.: Assessment of Medium-Range and Sub-Seasonal Ensemble Forecasts of Solar Irradiance and Wind Speed Over China: Applications for Renewable Energy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17120, https://doi.org/10.5194/egusphere-egu25-17120, 2025.

EGU25-18719 | ECS | Orals | ERE2.1

Using AI forecast of satellite imagery to improve solar generation forecasts 

James Fulton, Natalia Efremova, Nathan Simpson, Isabel Fenton, Evie Corcoran, James Robinson, Meghna Asthana, Peter Yatsyshin, and Nilo Pedrazzini

The global transition to low or no carbon electricity grids requires the use of a large amount of renewable energy sources such as photovoltaic solar power. However, to integrate these intermittent energy sources within stable electricity grids requires accurate solar power generation forecasts.

Satellite imagery is highly valuable for making short-term forecasts of solar generation. The stream of satellite data is low latency, usually only minutes behind real-time, is measured frequently, and is a direct measurement of the atmosphere. This complements numerical weather predictions (NWPs) which take several hours to compute from initial conditions, generally produce forecasts at only hourly steps, and are simulated and so have an imperfect and limited expression of the atmosphere.

Including satellite data often makes for better solar forecasts than using NWPs alone. However, for solar forecasts at time horizons beyond a couple of hours, satellite imagery becomes less and less useful as the atmospheric conditions will continue to evolve beyond those captured in the most recently available satellite image.

In this work, we introduce a machine learning model to forecast upcoming satellite images from recent satellite images. This can be done using relatively simple neural network architectures designed for video prediction. We show that we can increase the accuracy of solar generation forecasts in Great Britain by using these forecasted satellite images instead of just using recent satellite images.

We find that using predicted future satellite images complements using NWPs alone in making accurate solar energy predictions. Additionally, we propose that the task of forecasting future satellite images is pertinent to renewable energy generation forecasts and is a task which could be uniquely suited to be tackled with machine learning architectures used for AI weather forecasting.

How to cite: Fulton, J., Efremova, N., Simpson, N., Fenton, I., Corcoran, E., Robinson, J., Asthana, M., Yatsyshin, P., and Pedrazzini, N.: Using AI forecast of satellite imagery to improve solar generation forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18719, https://doi.org/10.5194/egusphere-egu25-18719, 2025.

EGU25-20085 | Posters on site | ERE2.1

A seven year study on the assessment of shortwave surface solar radiation in Cyprus 

Georgia Charalampous, Konstantinos Fragkos, Ilias Fountoulakis, Franco Marenco, Yevgeny Derimian, Andreas Karpasitis, Argyro Nisantzi, Rodanthi-Elisavet Mamouri, Kyriakoula Papachristopoulou, Diofantos Hadjimitsis, and Stelios Kazadzis

Aerosols influence surface solar irradiance directly through scattering and absorption and indirectly by acting as cloud condensation nuclei. Dust aerosols, a significant tropospheric component, play a critical role in climate processes by altering atmospheric energy fluxes at the surface and Top of the Atmosphere (TOA) and hence atmospheric temperature. This study examines the optical properties and direct shortwave radiative effects of dust aerosols at Agia Marina Xyliatou, Cyprus (35.04°N, 33.06°E, 535 m), a region impacted by Sahara and Arabian dust intrusions. Ground-based measurements, including AERONET sun photometer data, pyranometer and pyrheliometer records, combined with radiative transfer (RT) modeling (LibRadtran RT package), provide detailed insights into dust dynamics typing  and radiative effects.

Analysis of the 2015–2022 dataset reveals a seasonal peak in dust events during spring and autumn, with the Sahara contributing 80% of occurrences. Polly-XT lidar profiles from Limassol station expose the vertical aerosol structure and variability in  their extinction, while size distributions show a dominance of coarse-mode particles during intense dust periods. The mean direct Aerosol Radiative Effect (ARE) was −53.01±27.02 W/m² at the surface, indicating substantial cooling, and −16.29 W/m² at the TOA, ranging from −26.33 W/m² in February to −13.96 W/m² in April. March exhibited the strongest radiative effect, associated with the peak in Aerosol Optical Depth (AOD) and the lowest single scattering albedo (SSA) values indicative of more absorbing aerosols. Saharan dust exhibited stronger cooling compared to Middle Eastern dust due to its lower SSA (higher absorption).

This research highlights the significant role of dust aerosols in reducing surface solar radiation, emphasizing the need for detailed aerosol characterization to understand their climatic impacts and optimize solar energy resources in dust-prone regions.

 

 

Acknowledgments:

This research is performed under the auspices of the Memorandum of Understanding between the Eratosthenes CoE and The Cyprus Institute. The authors acknowledge the ‘EXCELSIOR’: ERATOSTHENES: Excellence Research Centre for Earth Surveillance and Space-Based Monitoring of the Environment H2020 Widespread Teaming project (www.excelsior2020.eu). The ‘EXCELSIOR’ project has received funding from the European Union’s Horizon 2020 research and innovation programme under Grant Agreement No. 857510, the Government of the Republic of Cyprus through the Directorate General for the European Programmes, Coordination and Development, and the Cyprus University of Technology. This project has also received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement No. 856612 and the Cyprus Government (EMME-CARE).

Authors would like to acknowledge the Action Harmonia CA21119 supported by COST (European Cooperation in Science and Technology).

 

How to cite: Charalampous, G., Fragkos, K., Fountoulakis, I., Marenco, F., Derimian, Y., Karpasitis, A., Nisantzi, A., Mamouri, R.-E., Papachristopoulou, K., Hadjimitsis, D., and Kazadzis, S.: A seven year study on the assessment of shortwave surface solar radiation in Cyprus, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20085, https://doi.org/10.5194/egusphere-egu25-20085, 2025.

EGU25-20121 | ECS | Orals | ERE2.1

Intense dust events over the Mediterranean Basin and their impact on PV power potential 

S. Yeşer Aslanoğlu, Rizos-Theodoros Chadoulis, Georgia Charalampous, Sara Herrero-Anta, Celia Herrero del Barrio, Dimitra Kouklaki, Anna Moustaka, Michail Mytilinaios, Alkistis Papetta, Nikolaos Papadimitriou, Stavros Solomos, Antonis Gkikas, Christos Spyrou, Sophie Vandenbussche, Emmanouil Proestakis, and Ilias Fountoulakis

The Mediterranean Basin is one of the sunniest regions globally, offering high potential for solar energy production. This makes energy production from photovoltaics a cornerstone to the efforts of the Mediterranean countries for decarbonization. Under cloudless skies, dust aerosols are among the main attenuators of surface solar radiation in the Mediterranean. Over the sunniest regions the role of dust can be even more significant than that of clouds.

In this study we used various earth observation products (from IASI, MODIS, CALIPSO), lidar aerosol extinction profiles, and HYSPLIT trajectories to identify strong dust events in 2021 – 2022. Four events where dust originated from different areas in Africa and the Middle East, and travelled over many AERONET stations (in an area covering latitudes from 30° N to 45° N and longitudes from -10° E to 40° E) were identified. AERONET measurements have been used to study the optical (Optical Depth, Angstrom Exponent, Single Scattering Albedo) and microphysical (size distribution) properties of the aerosol mixture at the affected sites and to discuss the role of the mixing of dust with local pollutants.

Furthermore, AERONET products were used as inputs to the UVSPEC model of the libRadtran package to perform radiative transfer (RT) simulations, assuming cloud-free conditions during the days of the events. The Global Horizontal Irradiance (GHI) and the Direct Normal Irradiance (DNI) were simulated and were subsequently used as inputs to the Global Solar Energy Estimator (GSEE). Finally, the energy production from photovoltaics positioned at fixed tilt angles and on solar tracking systems was simulated. Energy production losses due to the presence of dust have been quantified by comparing the simulated energy production with the corresponding simulations for the same days, assuming aerosol-free conditions. Losses that exceed 80% have been observed over specific locations.

Acknowledgements: Authors would like to acknowledge the Action Harmonia CA21119 supported by COST (European Cooperation in Science and Technology).

How to cite: Aslanoğlu, S. Y., Chadoulis, R.-T., Charalampous, G., Herrero-Anta, S., Herrero del Barrio, C., Kouklaki, D., Moustaka, A., Mytilinaios, M., Papetta, A., Papadimitriou, N., Solomos, S., Gkikas, A., Spyrou, C., Vandenbussche, S., Proestakis, E., and Fountoulakis, I.: Intense dust events over the Mediterranean Basin and their impact on PV power potential, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20121, https://doi.org/10.5194/egusphere-egu25-20121, 2025.

EGU25-21843 | Posters on site | ERE2.1

Sensitivity Analysis of Radiation Schemes in WRF-Solar for SolarEnergy Applications in Senegal 

Aissatou Ndiaye, Windmanagda Sawadogo, Jan Bliefernicht, Cheikh Dione, Mounkaila Moussa, Laouali Dungall, Amadou Gaye, and Harald Kunstmann

Solar irradiance forecasting plays a pivotal role in maximizing the use of solar energy resources and promoting the transition towards a cleaner and more sustainable energy future. This study evaluates the performance of the Weather Research and Forecasting (WRF-Solar) model using two shortwave radiation schemes in estimating Global Horizontal Irradiance (GHI) at two solar power plants in Senegal, i.e. Diass and Ten Merina. The different simulation experiments of WRF-Solar are specifically assessed under different sky conditions using hourly GHI measurements for 2020 from the solar plants operated by energy companies in Senegal. A total of six simulations are performed using different shortwave radiation schemes (Dudhia and RRTMG). There are two simulations run for the RRTMG scheme: one without aerosol optical depth (AOD) and one with AOD (RRTMG_AOD). In addition, the impact of shallow convection on the model performance is investigated. Results indicate that the RRTMG_AERO scheme outperforms other schemes with the highest correlation of 0.85 and the lowest values of RMSE (160 W/m2) and MAE (110 W/m2). It shows superior performance across clear, cloudy, and all-sky conditions. While the inclusion of shallow convection has minimal impact on GHI estimation accuracy under clear skies, some differences are noted under cloudy conditions at Ten Merina. Notably, the model shows biases, particularly under cloudy skies. These findings offer valuable insights that can enhance solar energy forecasting accuracy, support reliable solar power generation and renewable energy optimization, benefiting energy providers, policymakers and communities in Senegal.

How to cite: Ndiaye, A., Sawadogo, W., Bliefernicht, J., Dione, C., Moussa, M., Dungall, L., Gaye, A., and Kunstmann, H.: Sensitivity Analysis of Radiation Schemes in WRF-Solar for SolarEnergy Applications in Senegal, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21843, https://doi.org/10.5194/egusphere-egu25-21843, 2025.

EGU25-21854 | ECS | Orals | ERE2.1

Surface-driven categorisation of extreme wind events in convection-permitting models: Implications for wind energy planning in Central Europe 

Nathalia Correa-Sánchez, Xiaoli Larsén, Eleonora Dallan, Marco Borga, and Francesco Marra

Localised surface properties are essential in assessing wind resources for renewable energy development. Here, we estimate extreme winds using three convection-permitting models (CPMs) through a systematic surface-based categorisation for Central Europe. We developed a comprehensive classification framework integrating three fundamental surface parameters: climate regimes (Koppen-Geiger), aerodynamic roughness length (Z0), and slope variability. The methodology combines these parameters into distinctive surface categories, enabling a detailed analysis of wind extremes at 100m height across different surface configurations.

We analysed wind speed time series from the CPM ensemble for each resulting surface category, focusing on extreme events and their relationship with surface characteristics. The resulting classification has provided a sound basis for 67 unique surface combinations, allowing us to compare models over varying terrain and climate types and establish substantial differences in extreme wind behaviours.

This research contributes to improving wind energy planning by (1) identifying surface configurations that may influence extreme wind predictions, (2) providing a systematic approach to evaluate model performance across different surface conditions, and (3) giving an understanding of the relationship between surface characteristics and wind extremes at turbine height. The findings directly apply to wind farm siting and risk assessment in complex terrain regions.

Our methodology and results are particularly relevant for renewable energy applications. This work addresses critical needs in wind energy planning by improving our understanding of extreme wind behaviour across diverse surface conditions.

How to cite: Correa-Sánchez, N., Larsén, X., Dallan, E., Borga, M., and Marra, F.: Surface-driven categorisation of extreme wind events in convection-permitting models: Implications for wind energy planning in Central Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21854, https://doi.org/10.5194/egusphere-egu25-21854, 2025.

AS2 – Boundary Layer Processes

EGU25-493 | ECS | Orals | AS2.1

Investigating atmospheric mechanisms behind the long-range transport of fire aerosols: from the regional free atmosphere to the local boundary layer in a narrow valley 

K. Santiago Hernández, Daniel Espinosa, G. Alexis Ayala-Parra, Paola A. Montoya, Lina I. Ceballos, Manuel D. Zuluaga, Ana Z. Orrego, and Mauricio Ramírez

Regional fires result in large emissions of pollutants that can be transported through the atmosphere and impact air quality in remote regions. Studying regional fire aerosol transport is essential to understanding and forecasting air pollution events in different urban centers worldwide. However, there is a lack of research analyzing atmospheric patterns and mechanisms during regional fire aerosol transport events in tropical regions with complex topography. We investigate atmospheric conditions during regional fire aerosol transport events in the Aburrá Valley, a mountainous and highly urbanized region in the Colombian Andes. We combine observational and modeling approaches, including reanalysis data, high-resolution meteorological simulations, remote sensing information, and ground-based stations. Initially, regional transport events were selected from information from a Black Carbon monitor and verified using back-trajectories and hotspots data from MODIS. Besides, we performed two-month (February and March) 1-km resolution meteorological simulations with WRF model simulations for five years (2020-2024) to identify characteristic mesoscale patterns during aerosol transport events. Subsequently, we used information from a wind profiler radar, a microwave radiometer, and a series of sonic anemometers to study the incidence of polluted air masses in the local boundary layer. Our results show a notable reduction in precipitation both at a regional scale and in the path of air mass trajectories during regional transport events. Anomalous northwesterly regional winds are characteristic at low levels, and east-southeasterly winds dominate at mid-levels. At a local scale, these regional winds are channeled from the north and katabatic winds are intensified during night and early morning, leading to vertical wind shear within the boundary layer. These conditions favor the generation of mechanical turbulence during the night, enhancing the mixing of external pollutants towards the valley surface. Our study advances the understanding of mechanisms related to the impact of regional fire events on Aburrá Valley’s air quality, which can become more frequent under climate change conditions. Besides, these results contribute to the improvement of forecasting systems in the region, which is essential for comprehensive air quality management.

How to cite: Hernández, K. S., Espinosa, D., Ayala-Parra, G. A., Montoya, P. A., Ceballos, L. I., Zuluaga, M. D., Orrego, A. Z., and Ramírez, M.: Investigating atmospheric mechanisms behind the long-range transport of fire aerosols: from the regional free atmosphere to the local boundary layer in a narrow valley, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-493, https://doi.org/10.5194/egusphere-egu25-493, 2025.

Turbulent fluxes are critical in atmospheric science and are typically calculated using the eddy covariance system. However, the presence of motions of larger scale and biases from observational instruments often affect the accurate procurement of turbulent fluxes. To mitigate the influence of non-turbulent motions, data from multiple observational stations under various stratification conditions are analyzed. From these data, several new aspects of characteristics of atmospheric turbulence can be defined and investigated from statistical points of view, such as the properties of transport, the fractal dimension, and the anisotropy. Based on Hilbert–Huang transform, these novel characteristics can be analyzed across different scales and tested to be scale-dependent with stable patterns. However, for individual cases, it happens that these stable pattern are violated at comparatively large scales, indicating the existence of non-turbulent motions. Identifying these outliers enabled their elimination and the reconstruction of turbulence data, which reveals that the presence of non-turbulent motion leads to an overestimation of turbulent fluxes. The degree of overestimation depends on several predefined properties of non-turbulent motions, such as monotonicity, complexity, and intensity. Therefore, these novel characteristics enable the quantification of turbulent transport with higher precision and a broader application scope, and further reveal the promise in the simulation of atmospheric turbulence and the parameterization in meteorological and climate models.

How to cite: Liu, Z. and Zhang, H.: Reconstructing atmospheric turbulence from its novel characteristics for high-precision turbulent flux estimates, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1163, https://doi.org/10.5194/egusphere-egu25-1163, 2025.

In a stable boundary layer (SBL), turbulence is generally weak and exhibits significant intermittent characteristics. Interactions among motions of different scales complicate its structural evolution, making it difficult to predict. This study focuses on two typical processes in the SBL: Low-Level Jet (LLJ) and Internal Gravity Waves (IGWs), investigating how their interactions influence the evolution of turbulence structures. Utilizing a full boundary layer turbulence observation and data processing system at Zhongchuan International Airport, this study includes eddy covariance system, Doppler Lidar, and wind profiling radar. In a strongly SBL, turbulence energy accumulates in higher layers and, during downward transfer, generates local LLJ and IGWs, triggering intermittent turbulence events. The internal factors of turbulence intermittency dominated the process. The interaction between LLJ and IGWs maintains intermittent turbulence burst, accompanied by the conversion of sub-mesoscale energy to turbulent energy. In a weakly SBL, the conversion of sub-mesoscale motion energy drives intermittent turbulence events, along with energy transfers between different scales of IGWs, resulting in weaker turbulence intermittency. The external factors of turbulence intermittency dominated the process. In both cases, the interaction between LLJ and IGWs alters turbulence structure and atmospheric stability. Turbulent mixing changes the mean gradient field, further influencing the LLJ height. This study elucidates the mechanisms of interaction between internal and external factors in turbulence intermittency. It outlines energy transfer among different scales of motion and clarifies the mechanisms behind state transitions and structural evolution of strongly and weakly SBL. These findings are significant for advancing theoretical research and simulation developments of the SBL.

How to cite: Ren, Y., Ding, J., and Zhang, H.: Mechanism of Turbulence Structure Evolution in the Nocturnal Boundary Layer during the Interaction of Low-Level Jet and Internal Gravity Waves: Based on Full Boundary Layer Turbulence Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1995, https://doi.org/10.5194/egusphere-egu25-1995, 2025.

Detailed convective boundary layer (CBL) structure and the impact factors over the Tibetan Plateau has not been clearly understood, particularly for the level of neutral stability (zn), at which statically unstable lower CBL begins to transit into slightly stable upper CBL. Substantial uncertainties still exist in numerical models with different planetary boundary layer (PBL) schemes to reproduce such detailed structure. In this study, detailed CBL structure and processes over the Tibetan Plateau are examined using multi-year radiosonde data and large-eddy simulation (LES), particularly focusing on the impact of surface heating and entrainment on zn. The results indicated that the values of zn spatially ranged within 0.16–0.38zi on the plateau, with zi representing the CBL depth, and zn was higher in the southwestern region and lower in the southeastern region. Surface-/entrainment-induced large-scale thermals (corresponding to nonlocal fluxes) tended to suppress/elevate zn, due to warm turbulence penetrating into the upper/lower CBL, whereas small-scale eddies (corresponding to local fluxes) played an opposite role on modifying zn. The LES results suggested that zn increased before 08:00 Local Time (about 80 minutes after sunrise) because surface-induced small eddies dominated during the early stage of CBL growth and zn decreased afterwards as large-scale surface-induced thermals became more active. These improved understanding provides guidance for further improvement of PBL schemes.

 

How to cite: Li, X., Hu, X.-M., Wei, W., Zhang, L., Ren, Y., and Zhang, H.: Impact of surface and entrainment heat fluxes on the thermodynamic structure of the convective boundary layer over the Tibetan Plateau: observations and modelling analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2021, https://doi.org/10.5194/egusphere-egu25-2021, 2025.

EGU25-2036 | ECS | Orals | AS2.1

Decay of Turbulence during Evening Transition at the Kempegowda International Airport, Bengaluru, India 

Subham Banerjee, Suryadev Pratap Singh, and Sreenivas Kr

Evening Transition (ET) over Kempegowda International Airport (77.70◦ E, 13.20◦ N) is investigated over 2
seasons to calculate robust statistics of decay of Turbulent Kinetic Energy (TKE) in the Atmospheric Boundary
Layer (ABL). Although previous research on TKE decay during ET has largely relied on Large Eddy Simulations
(LES) and analytical models to determine decay rates of volume-averaged TKE, our study takes a more granular
approach.
We use two remote sensing instruments (Radiometer Physics HATPRO Radiometer and Vaisala Windcube
100S) to measure temperature, humidity, and wind components at multiple levels within the ABL. In addition,
ground instruments like temperature, relative humidity sensors, ground heat flux sensors and radiation sensors
provide near-surface data about temperature, moisture and heat fluxes. Together, these instruments allow us
to track local decay of TKE at various heights within the ABL.
We then apply functional fits for various time intervals during the decay period, generating vertical profiles
of the TKE decay exponents across the ABL. These profiles provide valuable insights into the relative importance
of surface-driven vs. ABL top-driven decay of TKE. Moreover, we observe that separate intervals of time in the
ET might have separate functional forms for the decay of TKE, instead of a commonly used single power-law
fit. The entire investigation enhances our understanding of TKE decay during the ET and could be
helpful for real-life applications such as understanding nighttime pollution dispersal or forecasting condensation
phenomenon like fog or mist. around Bengaluru city.

How to cite: Banerjee, S., Pratap Singh, S., and Kr, S.: Decay of Turbulence during Evening Transition at the Kempegowda International Airport, Bengaluru, India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2036, https://doi.org/10.5194/egusphere-egu25-2036, 2025.

Turbulence intermittency is a challenge facing in the ffeld of atmospheric boundary layer (ABL) and micrometeorology. We employed an automated algorithm for the separation and reconstruction of Sub-Mesoscale and Turbulent motions (SMT) to examine the basic characteristics of turbulence intermittency driven by submesoscale motion over the complex underlying surface of the Loess Plateau. The ffndings revealed that submesoscale motion has a signiffcant inffuence on turbulence statistical parameters. We analyzed ffve cases and found that the turbulent intermittency events were characterized by quiescent and burst periods. During the quiescent (burst) period, the turbulent transport weakened (strengthened), turbulence ffuctuations weakened (strengthened), atmospheric stability increased (decreased), and turbulent energy decreased (increased). These bursts can be triggered by energy conversion from sub-mesoscale to turbulent motion. Actual observations revealed atmospheric conditions where turbulent intermittency events are more likely to occur: wind speed U < 3.5 ms − 1 , wind speed gradient ΔU/ΔZ < 0.2 s − 1 , temperature gradient ΔT/ΔZ > -5.1 K/100 m, or bulk Richardson number Rib > -0.1. The inffuence of turbulence intermittency on the classical energy non-closure issue over the Loess Plateau was explored further. The results show that the presence of sub-mesoscale motions contributed to energy closure, with an energy closure of 78 % during daytime and 36 % during nighttime. And different periods of turbulent intermittency events affected energy non-closure differently, the energy closure during the burst (quiescent) period was approximately 98 % (70 %) during daytime and 68 % (17 %) during nighttime, approaching closure and far exceeding the overall closure rate during the burst period, whereas signiffcantly low during the quiescent period. This suggests that turbulence intermittency is a very important factor causing energy non-closure over complex underlying surfaces, especially in stable boundary layer (SBL) during nighttime. The results are highly signiffcant for a better comprehension of turbulence intermittency and surface-atmosphere interactions over complex underlying surface.

How to cite: Chang, H., Ren, Y., and Zhang, H.: The characteristics of turbulence intermittency and its impact on surface energy imbalance over Loess Plateau, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2131, https://doi.org/10.5194/egusphere-egu25-2131, 2025.

EGU25-2133 | ECS | Posters on site | AS2.1

Improving the Urban Boundary Layer Wind Speed by Coupling the TKE-ACM2 PBL Scheme with the Building Effect Parameterization Model 

Wanliang Zhang, Michael Mau Fung Wong, and Jimmy Chi Hung Fung

Realistically representing the vertical turbulent transport of surface layer fluxes dealt with by the planetary boundary layer (PBL) scheme is of paramount importance in a numerical weather forecasting model. Further complexity arises due to the presence of heterogeneous surface obstacles whose height can be comparable to the model's vertical resolution, which poses a challenge in improving and revisiting the PBL scheme. In this presentation, we derive the numerical method to couple one of the recently validated turbulent kinetic energy (TKE)-based non-local PBL schemes, namely the TKE-ACM2 scheme, with the commonly used multi-layer Building Effect Parameterization (BEP) model in WRF. The behavior of TKE-ACM2+BEP is first examined under idealized convective atmospheric conditions where a simplified staggered urban morphology is prescribed. Its performance is benchmarked against the state-of-the-art large-eddy simulation by PALM and also compared with the operational PBL scheme Boulac+BEP. The idealized simulation results reveal that TKE-ACM2+BEP exhibits superiority in simulating the potential temperature and wind speed profiles compared to Boulac+BEP, corroborating its better non-local treatment of the momentum fluxes near the roughness sublayer. Furthermore, we apply the coupled model to the Pearl River Delta region in South China, where a few extensively urbanized mega-cities exist. The one-month high-resolution wind speed LiDAR observations indicate that TKE-ACM2+BEP provides a more reasonable reproduction of wind speed profiles in the upper surface layer compared to the Bulk methods (i.e., without urban canopy model) by reducing the overestimation at the urban LiDAR site. In addition, the 10-m wind speeds (U10) are compared with surface stations aggregated based on the Local Climate Zone classification. The results suggest that the BEP model can improve the performance of the TKE-ACM2 PBL scheme at low- to moderate-building grids, but may not be consistently better at high-building density grids as it overly reduces U10.

How to cite: Zhang, W., Wong, M. M. F., and Fung, J. C. H.: Improving the Urban Boundary Layer Wind Speed by Coupling the TKE-ACM2 PBL Scheme with the Building Effect Parameterization Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2133, https://doi.org/10.5194/egusphere-egu25-2133, 2025.

Fog is a highly complex weather phenomenon influenced by numerous factors. This study aims to investigate the impact of Changbai Mountain topography on the formation and development of the spring fog in the Bohai Sea. From May 12 to 14, 2021, the Bohai region experienced a sea fog event. Utilizing the Himawari-8 satellite retrieval data, the European Centre for Medium-Range Weather Forecasts (ECMWF) 5th Generation ERA5 reanalysis dataset, land and sea station observations, the WRF model, the topography sensitivity experiment, and the backward trajectory tracking, a study was conducted to assess the influence of Changbai Mountain topography on the evolution of the Bohai sea fog. The results indicated that the Changbai Mountain topography significantly impacted the propagation and concentration of the Bohai sea fog through the dual effects of Venturi Effect and Foehn Clearance Effect. Comparative simulations incorporating and excluding the Changbai Mountain revealed that its topography favored weak convergence (Venturi Effect) of low-level airflow in the Bohai Sea induced by a high-pressure system, promoting westward fog expansion. Additionally, the backward trajectory further indicated that the Foehn Clearance Effect of Changbai Mountain extended its influence far beyond the immediate lee side, contributing to significant changes in atmospheric conditions such as reductions in relative humidity and increases in potential temperature. The dry, warm foehn contributed to a reduction in the liquid water content, ultimately leading to the weakening or even dissipation of the sea fog in the region close to Changbai Mountain. This study emphasizes the crucial role of Changbai Mountain topography in the development and evolution of fog, providing valuable insights for forecasting fog in complex terrain.

How to cite: Tian, M.: Impact of Changbai Mountain Topography on the Spring Fog over the Bohai Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2863, https://doi.org/10.5194/egusphere-egu25-2863, 2025.

EGU25-3520 | Orals | AS2.1 | Highlight

Experimental determination of offshore turbulence spectra and lateral coherences with multiple lidars 

Jakob Mann, Ansh Patel, and Mikael Sjöholm

We demonstrate that we can measure spectral coherence of offshore atmospheric turbulence at heights and with lateral displacements relevant for dynamic loads on modern, large wind turbines. This is done by five coordinated, pulsed Doppler lidars standing on the coast of the North Sea with beams intersecting almost perpendicularly. The six crossing points are 150 to 250 m above the ocean and have lateral separations of up to 200 m, reflecting the scale of modern offshore wind turbines. We compare the measurements with spectral and cross-spectral models. The model of Syed and Mann (Boundary-Layer Meteorology, 2024, vol 190), in general fits the spectra well and predicts the lateral coherences well. However, there are cases where the measured lateral coherence of the v-component is much larger than predicted. This seems not to be due to malfunction of the instruments, but rather due to non-turbulence processes in the atmosphere, e.g . interval gravity waves. We will also touch upon the potential consequences for loads on wind turbines. 

How to cite: Mann, J., Patel, A., and Sjöholm, M.: Experimental determination of offshore turbulence spectra and lateral coherences with multiple lidars, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3520, https://doi.org/10.5194/egusphere-egu25-3520, 2025.

EGU25-4133 | ECS | Posters on site | AS2.1

Mesoscale modeling of the urban boundary layer in a coastal city. The case of Valencia. 

Ángel Sánchez-Lorente, Alberto Martilli, Beatriz Sánchez, and Carlos Yagüe

Extreme weather events, such as heat waves, are increasingly common during summers in the
Mediterranean area. The effect of urban overheating -known as the increase of the average
temperature within the urban canopy caused by the heat storage on their surfaces thanks to their
optical and thermal characteristics, in addition to the heat emissions due to anthropogenic activities-
can cause the thermal stress of the population in the city to increase significantly during these
episodes, leading to serious health consequences. The study of this type of impact must be
quantified by means of thermal comfort indices that establish a relationship between the
meteorological conditions observed or predicted by a model and the physiological response of
human beings, such as the Universal Thermal Climate Index (UTCI). In this work, we study the
spatial-temporal behaviour of the UTCI in the city of Valencia (east coast of Spain) during a heat
wave (HW) and non-heat wave (NHW) period in August 2023 using the mesoscale meteorological
model (WRF, Weather Research and Forecasting) and in situ observations. For this purpose, a
comparison of atmospheric conditions in the planetary boundary layer (PBL) is performed, as well as
a study of the influence of temperature, shortwave and longwave radiation (from the mean radiant
temperature, TMR), wind speed and relative humidity on the behaviour of the UTCI. The main
results show a similar spatial distribution and temporal evolution of the UTCI for both periods,
differing in the magnitude of the UTCI. The positive (negative) temperature anomaly with regards to
the rest of the month is mainly the factor that causes a greater increase (decrease) in UTCI during
the HW (NHW). There is also a less developed PBL during the HW, as a consequence of the lower
intensity of the coastal breeze in the city during this period, which also has a significant effect on the
increase in UTCI during the HW.

How to cite: Sánchez-Lorente, Á., Martilli, A., Sánchez, B., and Yagüe, C.: Mesoscale modeling of the urban boundary layer in a coastal city. The case of Valencia., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4133, https://doi.org/10.5194/egusphere-egu25-4133, 2025.

EGU25-6010 | ECS | Posters on site | AS2.1

Concentration fluctuations and mean time of exceeding of hazard thresholds on industrial sites 

Claudia Schiavini, Massimo Marro, Pietro Salizzoni, Lionel Soulhac, Marco Ravina, Deborah Panepinto, and Mariachiara Zanetti

Knowledge on both the mean field and fluctuations of concentration is necessary to estimate risks linked to pollutant exposure on industrial sites. While time-averaged concentrations provide meaningful information for chronic risk exposure, local exceedance of high concentration values potentially trigger chemical reactions or exceed harmful limits for living organisms. Information on threshold exceeding is thus a key parameter for toxicity assessment and accident management, hence the focus of this work on concentration fluctuations.

Several models for the probability distribution functions (PDF) of pollutant concentrations have been proposed in the literature. Several authors agree on the fact that the gamma distribution provides a reliable model for the one-point concentration PDF in case of localised releases of pollutants in atmospheric boundary layers (Cassiani et al., 2020). However, the accuracy of the gamma distribution was still not properly investigated within domain characterised by a complex geometry.

 

This is indeed the aim of this experimental study, focusing on the one-point concentration PDF due to a localised release of pollutant within a group of buildings. Furthermore, we aim at verifying models predicting average times of exceeding concentration thresholds (e.g. Bertagni et al., 2020).

Wind and concentration fields were characterised on the small-scale model of an idealised industrial site in a wind tunnel reproducing the atmospheric boundary layer. Higher order statistics were computed from concentration time series collected with a fast flame ionisation detector of frequency 400 Hz. In addition to the work presented hereby, this experimental dataset could be used to validate numerical dispersion models in future studies.

 

Best agreement between the experimental one-point concentration PDF and the gamma distribution are observed in the mid- and far-field. In contrast, the gamma distribution induces a systematic underestimation of concentration fluctuations in the near-field. Notably the Gamma distribution does not capture the occurrence of high intensity peaks measured sporadically, especially in recirculating regions in building wakes.

Mean threshold exceeding times are computed assuming a gamma distribution and hence show best correlation with experimental data in the mid- and far-field. Frequency of threshold exceeding show less accurate results for higher limits.

 

Summarising, the gamma distribution is shown to be a reliable model for the one-point concentration PDF in the mid- and far-field, but exhibits poor correlation in the near-field due to the presence of recirculation zones and intense meandering motion of the pollutant plume. The model for mean times of threshold exceeding, relying on the assumption of a gamma distribution, show a similar behaviour.

 

References

Bertagni, M. B., Marro, M., Salizzoni, P., & Camporeale, C. (2020). Level-crossing statistics of a passive scalar dispersed in a neutral boundary layer. Atmospheric Environment, 230, 117518. https://doi.org/10.1016/j.atmosenv.2020.117518

Cassiani, M., Bertagni, M. B., Marro, M., & Salizzoni, P. (2020). Concentration Fluctuations from Localized Atmospheric Releases. Boundary-Layer Meteorology, 177(2), Article 2. https://doi.org/10.1007/s10546-020-00547-4

How to cite: Schiavini, C., Marro, M., Salizzoni, P., Soulhac, L., Ravina, M., Panepinto, D., and Zanetti, M.: Concentration fluctuations and mean time of exceeding of hazard thresholds on industrial sites, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6010, https://doi.org/10.5194/egusphere-egu25-6010, 2025.

EGU25-6841 | Posters on site | AS2.1

Impacts of Terrain Slope and Surface Roughness Variations on Turbulence Generation in the Nighttime Stable Boundary Layer 

Jielun Sun, Sudheer Bhimireddy, David Kristovich, Junming Wang, April Hiscox, Larry Mahrt, and Grant Petty

Terrain-slope increases with and without upslope large surface roughness are found impacting downstream shear-generated turbulence differently in the nighttime stable boundary layer (SBL). Their different influences can be clearly identified in their different derivations in the relationship between turbulence and wind speed at a given height, known as the HOckey STick (HOST) transition, from the HOST relationship over a flat terrain. Due to transport of the cold surface air down from elevated uniform terrain in reducing the downstream air temperature not much stratification, the downstream hydrostatic imbalance increases with terrain slope resulting in enhanced turbulence for a given wind speed. The rate of turbulence increase with wind speed from this downslope flow, on the other hand, is independent of terrain slope. With turbulent mixing enhanced by upslope large surface roughness elements, the upslope cold surface air is elevated from the upslope terrain surface. Horizontal transport of this elevated cold turbulent air layer reduces the downstream upper warm air temperature, resulting in the increasing reduction of the downstream stable stratification with height. As the consequence of the effective wind-shear generation of turbulence with the reduced stratification, the downstream near-neutral turbulence increase with wind speed is enhanced with height in addition to the turbulence intensity enhancement from the cold downslope flow. The study demonstrates important physical mechanisms for turbulence generation captured by HOST and detection of terrain features for their impacts on those mechanisms through their deviations from the HOST relationship over a flat terrain.

This study demonstrates key physical mechanisms for turbulence generation captured by the HOST relationship. It also highlights the influence of terrain features on these mechanisms through deviations from the HOST relationship observed over flat terrain.

The study is supported by US National Science Foundation (NSF), AGS-2203248, AGS-2220664, and AGS-2231229 for JS;  AGS-1733877 and AGS-2220663 for JW, SB, and DK;  AGS-1733746, AGS-1843258, and AGS-2220662 as well as the University of South Carolina Department of Geography for AH; and AGS-1844426 for GP. SB was also partly supported by the NOAA cooperative agreement NA220AR4320151 for the Cooperative Institute for Earth System Research and Data Science (CIESRDS).

How to cite: Sun, J., Bhimireddy, S., Kristovich, D., Wang, J., Hiscox, A., Mahrt, L., and Petty, G.: Impacts of Terrain Slope and Surface Roughness Variations on Turbulence Generation in the Nighttime Stable Boundary Layer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6841, https://doi.org/10.5194/egusphere-egu25-6841, 2025.

EGU25-8050 | ECS | Posters on site | AS2.1

Marine Atmospheric Boundary Layer Characteristics Observed during the FATIMA-YS Campaign at the S-ORS 

Hojin Kim, Ki-Young Heo, Jin-Yong Jeong, and Harindra Joseph Fernando

This study presents findings from the FATIMA-YS campaign, an international collaborative effort to investigate marine atmospheric processes over the Yellow Sea, conducted at the Socheongcho Ocean Research Station (S-ORS) from June 20 to July 9, 2023. The Yellow Sea is a critical region for studying marine atmospheric boundary layer (MABL) dynamics due to its unique air-sea interaction processes driven by seasonal variability and complex coastal influences.

During the campaign, radiosonde observations at S-ORS captured the formation and evolution of a stable boundary layer (SBL) on June 30 and July 1, under conditions of warm air masses overlying cooler sea surfaces, accompanied by weak horizontal winds. These observations revealed a sharp temperature inversion near the surface, indicative of strong atmospheric stability and limited vertical mixing.

Turbulent fluxes were measured using eddy covariance instruments, capturing unique characteristics of air-sea interactions under stable conditions. These observational findings will be presented alongside numerical model simulations to explore the dynamics of the MABL under stable conditions.

How to cite: Kim, H., Heo, K.-Y., Jeong, J.-Y., and Fernando, H. J.: Marine Atmospheric Boundary Layer Characteristics Observed during the FATIMA-YS Campaign at the S-ORS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8050, https://doi.org/10.5194/egusphere-egu25-8050, 2025.

EGU25-8194 | ECS | Orals | AS2.1

Droplet Sedimentation Effects in Stratocumulus Clouds 

Raphael Pistor and Juan Pedro Mellado

Quantifying the effects of stratocumulus cloud feedbacks remains a key challenge, particularly due to the complex interactions between the boundary layer and the cloud top that occur at meter and submeter scales. Droplet sedimentation counteracts cloud-top entrainment by moving droplets away from the warm, dry free troposphere, thereby decreasing cloud-top evaporation and turbulence generation. Assessing how sedimentation influences entrainment and turbulence is essential for determining cloud lifetimes.

Previous works using large-eddy simulations (LES) with 5-10 m resolution demonstrated that sedimentation reduces the mean entrainment velocity (Ackerman 2004, Bretherton 2007, Hill 2009). However, the strength of this reduction remains uncertain because insufficient resolution introduces spurious upward fluxes that oppose the sedimentation flux. Local direct numerical simulations (DNS) studies, focused exclusively on the cloud layer at submeter-scale resolution, reported a reduction of the mean entrainment velocity due to sedimentation of up to 40%, or 3 times higher than LES results (de Lozar 2017, Schulz 2019). The question then remains: do these results also hold when considering the full vertical domain of the stratocumulus-topped boundary layer, spanning from the surface level to the free troposphere?

The novelty of this work lies in using DNS to simulate meter-scale processes at the cloud top, while encompassing the full vertical extent of the stratocumulus-topped boundary layer. We perform sensitivity experiments that involve changing the sedimentation strength and the Reynolds number. Consistent with previous studies, we find that sedimentation reduces the mean entrainment velocity by at least 20%, with the magnitude increasing for higher Reynolds numbers. Interestingly, the turbulence kinetic energy and the turbulent entrainment flux also increase with sedimentation.

To resolve this apparent contradiction, we quantify the mean fluxes of the liquid water static energy at the cloud-top region. Our results show that the magnitude of the sedimentation flux undergoes a more rapid growth than the turbulent flux with sedimentation, effectively compensating for the increase in the turbulent flux. Additionally, the contrast in the vertical velocity between updrafts and downdrafts in the subcloud layer becomes less extreme with sedimentation. The skewness in this region shifts from a predominantly positive profile to a more neutral one. This more balanced distribution of vertical motions results from increased liquid water availability for evaporation in the downdrafts, which in turn accelerates them. In summary, we show that sedimentation effects are as important as turbulent effects at meter-scale resolution. Moreover, sedimentation reshapes the vertical moisture distribution in both cloud and subcloud layers.

How to cite: Pistor, R. and Mellado, J. P.: Droplet Sedimentation Effects in Stratocumulus Clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8194, https://doi.org/10.5194/egusphere-egu25-8194, 2025.

Street canyons are a common feature in many urban environments. They are also arguably the most polluted region of the urban boundary layer due to the presence of heavy traffic and limited penetration of fresh wind for ventilation. Hence a detailed understanding of the processes taking place within the canyon is crucial to ensuring good air quality in urban areas. In this study, we investigate the turbulent flow and pollutant dispersion in four model street canyons having different morphologies, by conducting time-resolved particle image velocimetry (PIV) measurements in a wind tunnel. The street canyons analysed have different aspect ratios (the ratio of the height of the street canyon to its width) and were surrounded by higher or lower buildings, i.e. by street canyons with a higher or lower aspect ratio. First, we introduce an approach for determining pollutant concentrations from PIV data and show that the method can be reliably used to measure the planar pollutant fluxes. Differences in the concentration and flow fields at different planes were observed, thus indicating the importance of considering the three dimensionality of the canyons. The turbulent scalar flux was found to play a dominant role in pollutant transport at the roof level for canyons surrounded by buildings having the same aspect ratio as the canyon. Conversely, advection dominates at roof level when a canyon is surrounded by buildings having different aspect ratios.  Quadrant analysis of the momentum and scalar flux reveals high correlations between ejections and sweeps and ventilation processes at the roof level. We apply the dynamic mode decomposition (DMD) technique, a data-driven algorithm, to extract dynamically relevant coherent structures of the flow and pollutant concentrations from the data. The results of DMD show that roof and ground level coherent structures play a crucial role in the ventilation of the street canyons.

How to cite: Owolabi, B. and Nosek, S.: Flow and Pollutant dispersion from a line source in 3D urban street canyons having different spatial morphologies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9201, https://doi.org/10.5194/egusphere-egu25-9201, 2025.

EGU25-9491 | ECS | Posters on site | AS2.1

Simulation of radiatively driven mixing in a smoke cloud using "one-dimensional turbulence" 

Hanchen Li, Marten Klein, and Heiko Schmidt

Large-eddy simulations (LESs) are known to significantly overestimate entrainment in cloud-topped boundary layers, negatively impacting predictions on cloud mass and cover. This overestimation stems from coarse model resolutions that lead to numerical broadening of the entrainment layer. While it has been shown in direct numerical simulations (DNSs) that down-to-centimetre-scale resolutions can mitigate this issue, such high resolutions are not viable for most applications in the atmospheric sciences. The one-dimensional turbulence model (ODT), introduced by Kerstein [1], offers a computationally efficient alternative that provides full-scale resolution along a 1-D vertical domain. Molecular diffusion is explicitly resolved, while turbulent advection is modelled through a stochastically sampled sequence of spatial mappings, known as eddy events. Physically plausible eddy events are selected based on their current kinetic and potential energy. This allows an accurate representation of local turbulence properties and their dynamical complexity by evolving instantaneous property profiles. This study applies ODT to investigate cloud-top turbulent mixing processes driven by radiative cooling in a smoke cloud, benchmarking the results against DNS. Building on the preliminary findings by Meiselbach [2], we demonstrate improvements in mean profiles and turbulent fluxes of buoyancy and smoke concentration, showing ODT's ability to reproduce salient features observed in DNSs. In addition, we explore convective boundary layer scalings at extended Reynolds and Richardson numbers beyond those accessible in DNS studies.
 

References:
[1] A. R. Kerstein, Journal of Fluid Mechanics 392, 277334 (1999).
[2] F. T. Meiselbach, Application of ODT to Turbulent Flow Problems, doctoral thesis, BTU Cottbus-Senftenberg (2015).

How to cite: Li, H., Klein, M., and Schmidt, H.: Simulation of radiatively driven mixing in a smoke cloud using "one-dimensional turbulence", EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9491, https://doi.org/10.5194/egusphere-egu25-9491, 2025.

EGU25-9850 | ECS | Orals | AS2.1

Marine boundary layer evolution in the transition from low stratocumulus clouds to land fog in the coastal mountains of Atacama 

Felipe Lobos-Roco, Vicente Espinoza, Klaus Keim-Vera, Francisca Munoz, Francisco Suarez, and Oscar Hartogensis

Advection of marine stratocumulus clouds (SCu) from the South East Pacific into the Atacama Desert forms large and semi-permanent fog banks at the top of the coastal mountain range. These fog banks are the sole water input for xeric ecosystems and represent a freshwater resource to be harvested by local communities in the driest place on Earth. The fog maintenance depends on the marine boundary layer (MBL) thermal inversion, which results from the equilibrium between subsidence and ocean heat fluxes. To study these interactions, we performed a field experiment in July 2024 in North West Chile called StraToFog, to measure surface and airborne boundary layer state during the SCu-fog transition. Surface measurements of energy balance fluxes and vertical observations of MBL thermodynamics were performed over a transect following the SCu-fog transition: at the ocean, the top of the mountain range, and inland in the desert. To complement these measurements, a high-precision balance and a standard fog collector transect were installed to measure fog and dew collection. Overall, our experiment reveals two distinctive fog regimes, which depend on the interplay between MBL growth, the strength of subsidence and the development of a sea breeze that pushes the MBL with clouds onto the coastal mountain range. First regime occurs at night when inversion layer is controlled by low surface temperature, resulting in air saturation under lower humidity content (↓es), leading to fog collection ~0.5 L m-2 h-1. The second regime occurs after a dissipation break at noon, where MBL advection increases humidity leading to air saturation under higher air temperatures (↑e), resulting in fog collection ~3 L m-2 h-1. Our results show a SCu top uplift between 150 to 400 m from ocean to inland. This uplifting is explained by the abrupt topography (800 m height; 5 km long) and by the sensible heat flux increases from 32 W m-2 over the ocean to 250 W m-2 over land. Airborne measurements show a diurnal cycle of fog cloud formation, which show a thickness of 20 m in the morning, grow to 200 m at noon, dissipate in the afternoon, and form again up to a thickness of 100 m during the evening. In addition, a very strong inversion layer (~18 K) was observed at the top of the cloud layer at 08:00 LT. The surface soil balance experiment shows a weight increase at night (00:00-06:00 LT) under clear sky conditions, associated with dew deposition. In contrast, during foggy days, the soil weight increases in the morning (06:00-12:00 LT) under windless (<1 m s-1) conditions, followed by a decrease in the afternoon under windy conditions (>4 m s-1), associated with fog deposition/evaporation. Further analysis of this data, accompanied by high resolution numerical simulations, will allow us to better understand fog dynamics in drylands and its potential prediction. 

How to cite: Lobos-Roco, F., Espinoza, V., Keim-Vera, K., Munoz, F., Suarez, F., and Hartogensis, O.: Marine boundary layer evolution in the transition from low stratocumulus clouds to land fog in the coastal mountains of Atacama, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9850, https://doi.org/10.5194/egusphere-egu25-9850, 2025.

Nocturnal Low-Level Jets (NLLJ) are known to be a crucial process in the long-range transport of atmospheric pollutants with a positive or negative impact on air quality. In recent years, the study of NLLJ that occur usually at the top of the atmospheric boundary layer (ABL) has been greatly enhanced by recent technological and methodological advances in ground-based remote sensing instruments. They are now able to provide continuously high-quality profiles of ABL parameters that can be obtained from automatic LIDAR-ceilometers (ALC) providing information about clouds, precipitations, aerosols (including aerosol characteristics and types with depolarization measurements) and from wind Doppler LIDAR (WDL) providing information about wind profile characteristics.

At the Royal Meteorological Institute of Belgium (RMI), we have been developing a new pioneering algorithm (CONIOPOL: CONIOlogy + POLarization) based only on ALC measurements with a depolarization function (VAISALA CL61) to provide in real-time automatic identification of cloud phase, precipitation type and aerosol type. By combining the output of CONIOPOL based on measurements from a CL61 installed in Uccle (Brussels) with measurements from a WDL located at Brussels Airport (15km away from the CL61), it is possible to monitor continuously the transport of aerosols by NLLJ.

The synergy between both instruments will be illustrated by an interesting case study, showing the transport of marine aerosols by NLLJ into the ABL characterized in the presence of dust. The characteristic and the evolution of the synoptic situation will be used to highlight the geographical origin of aerosols. In order to better characterize the type identification of aerosols by CONIOPOL, ground measurements concerning the physical properties of aerosols carried out close to the CL61 will also be presented.

How to cite: Mangold, A., Laffineur, Q., Koistinen, E., and Delcloo, A.: Synergy between ground-based remote sensing instruments: a new approach to better understand the transport and dispersion process of aerosols in the atmospheric boundary layer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10335, https://doi.org/10.5194/egusphere-egu25-10335, 2025.

EGU25-11181 | Orals | AS2.1

Seamless wind profiling of the atmospheric boundary layer 

Finn Burgemeister, Piet Markmann, and Gerhard Peters

Structures and processes in the atmospheric boundary layer (ABL) span a wide range of scales which cannot be fully captured by a single measuring technique. Doppler lidars are a preferred remote sensing tool for the observation of wind profiles in the entire ABL. Typically the relevant scales of ABL flow structures increase with increasing distance from the surface.

While pulsed Doppler lidars (PDLs) are typically sufficiently sensitive to reach the top of the ABL, they leave an unobserved gap in the lowest 50 m. This is because the PDL receiver doesn’t work before the transmit pulse has left the lidar. In addition to the gap, the spatial resolution δr, which is proportional to the pulse length l, is not always satisfying in the lowest range gates, since wind gradients occuring over canopies, urban surface structures or in case of stable stratification cannot be resolved reliably. l cannot be deliberately shortened for the sake of velocity resolution δv and sensitivity s (δvl-1, sl).

Continuous wave lidars (CDLs) are typically restricted to a maximum height of 200 m. The ranging is here achieved by focusing the beam. With this technique the range resolution δr is not constant but becomes finer the shorter the range r. At r = 10 m, a range resolution δr = few centimeters is possible. Since δrr2 the resolution at 200 m is no longer superior to that of PDLs. Thus, a CDL is a perfect complement to a PDL in order to observe near-surface structures of the ABL.

We will present observations obtained with a PDL-, CDL-combination. Both systems are using an identical scanning cone with a zenith angle of 10°. This scan geometry is particularly suitable for operation close to obstacles as trees or buildings, in urban environments or in complex terrain.

How to cite: Burgemeister, F., Markmann, P., and Peters, G.: Seamless wind profiling of the atmospheric boundary layer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11181, https://doi.org/10.5194/egusphere-egu25-11181, 2025.

EGU25-11186 | ECS | Posters on site | AS2.1

Implicit Large Eddy Simulations of Boundary Layer Flows: Modeling Surface Roughness by Stochastic Microtopography 

Elias Wahl, Theresia Yazbeck, and Mark Schlutow

Large Eddy Simulations are widely used to study the Atmospheric Boundary Layer, since they resolve sufficient turbulence features to capture realistic boundary layer dynamics. For this purpose, the surface roughness of the terrain is often implemented by a roughness parameter that increases turbulence production near the surface through the stress tensor of the subgrid-scale model, in accordance with Monin-Obukhov theory. In Implicit Large Eddy Simulations, the absence of a subgrid-scale model simplifies implementation and reduces potential error sources at faster computational speeds, but does not permit the aforementioned implementation of the surface roughness. A drag coefficient can be used to integrate the effects of the surface roughness in Implicit Large Eddy Simulations. However, we propose a novel approach that models the surface roughness through a stochastic height variation of the lowest simulation layer. The method captures the impact of small-scale surface heterogeneity more effectively than a traditional uniform roughness parameter or drag coefficient model, while still just being controlled by a single parameter that prescribes the amplitude of the height variation. We find that this parameter has a linear correlation to the measured surface roughness in the corresponding simulation, with high numeric stability even for high wind speeds.

How to cite: Wahl, E., Yazbeck, T., and Schlutow, M.: Implicit Large Eddy Simulations of Boundary Layer Flows: Modeling Surface Roughness by Stochastic Microtopography, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11186, https://doi.org/10.5194/egusphere-egu25-11186, 2025.

Modeling turbulent air flow accurately is quite difficult, particularly when topographic factors and changing boundary conditions are present. The objective of this research is to combine data from high-resolution Computational Fluid Dynamics (CFD) simulations with a low-resolution meteorological model in order to describe air flow with high accuracy and resolution. To accomplish this, the FLUENT CFD solver was integrated with the widely used Weather Research and Forecasting (WRF) model.

Time-dependent boundary conditions for mesoscale atmospheric conditions are provided by the WRF model, and high-resolution Navier-Stokes simulations are carried out using FLUENT. To ensure ground surface compatibility and resolve inconsistencies caused by variations in mesh-grid structures and resolutions between the models, modified boundary conditions and an unstructured grid framework were applied. Data from the WRF were integrated into FLUENT via User-Defined Functions (UDFs). This approach enhanced the accuracy of turbulent atmospheric flow solutions and improved adaptability to time-dependent variables.

As it known, one of the challenges in the meteorological modeling is representing maximum values, which are expected to observe frequently during climate change. In here, the analyses were conducted for Istanbul Airport, one of the busiest airports in the world, focusing on the dates with the maximum wind speed values. The combined model outputs were compared with observations from the meteorological station in the region, followed by a comprehensive analysis of the wind flow fields across the area. The results demonstrated that low-resolution meteorological models can be successfully integrated into high-resolution CFD simulations, leading to significant improvements in the spatial and temporal resolution of turbulent flow analyses. Moreover, this approach offers broad applicability in areas such as renewable energy and weather forecasting. The study presents a new methodology for atmospheric flow simulations by improving data compatibility and solution accuracy between models.

How to cite: Mut, A. O. and Şahin, A. D.: Coupled Mesoscale Weather Prediction and Computational Fluid Dynamics Modeling for Maximum Wind Flow Analysis: A Case Study for Istanbul Airport, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11687, https://doi.org/10.5194/egusphere-egu25-11687, 2025.

The Ozmidov scale marks the cutoff scale above which overturning fluid motions in stably stratified shear flows are energetically prohibited. A recent study of a turbulent shear layer demonstrates that the Corrsin scale provides an intrinsic cutoff scale when stratification is absent [1]. For the neutral boundary layer, it is proposed by analogy to the mixing layer that the cutoff scale is linked to the Corrsin scale rather than the unbounded Ozmidov scale. The claim is numerically investigated for turbulent Ekman flow with the aid of Kerstein’s one-dimensional turbulence (ODT) model [2], utilizing the case setup described in [3]. ODT offers full-scale resolution along a vertical coordinate by autonomously evolving the instantaneous property profiles. Molecular diffusion is directly resolved, whereas turbulent advection is modeled by a stochastic process that is formulated with the aid of spatial mapping events, which are sampled based on the local available energy. In this model formulation, a cutoff scale is economically prescribed by limiting the sampling range of turbulent scales. Model results in terms of low-order and detailed turbulence statistics will be presented and compared to available reference data and theoretical analysis.

References
[1] F. G. Jacobitz and K. Schneider. Phys. Rev. Fluids 9:044602, 2024.
[2] A. R. Kerstein and S. Wunsch. Bound.-Lay. Meteorol. 118:325–356, 2006.
[3] M. Klein and H. Schmidt. Adv. Sci. Res. 19:117–136, 2022.

How to cite: Klein, M. and Schmidt, H.: Investigating cutoff scales in turbulent Ekman flow with a map-based stochastic modeling approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13495, https://doi.org/10.5194/egusphere-egu25-13495, 2025.

EGU25-14672 | ECS | Orals | AS2.1

Ultra-wideband RF photonics spectrometer for atmospheric boundary layer sensing 

Mehmet Ogut, Shannon Brown, Sidharth Misra, Eric Kittlaus, Pekka Kangaslahti, Janusz Murakowski, and Michael Gehl

Most of the energy exchange in the atmosphere occurs in the atmospheric boundary layer (ABL) with respect to solar heating and evaporation. Remote sensing in the ABL from space is challenging because of its proximity to the surface and potential sharp gradients in air properties. Passive microwave instruments can be a critical component to a ABL observing system since they provide thermodynamic information in both cloudy and clear air, including cloud and precipitation properties, and surface flux information such as temperature and wind speed. However, conventional passive microwave systems fall well short of being optimized for near surface sensing due to limited number of spectral channels and coarse spectral resolution covering only a small portion of the spectrum of interest for ABL sensing.

The near surface thermodynamic structure information is encoded on the microwave spectrum between and on the shoulders of the water vapor absorption and oxygen lines near 183 GHz and 118 GHz respectively. The ultra-wideband photonic spectro-radiometer instrument is funded by NASA ESTO under ACT-20 program to combine low-noise wideband InP RF technology with a novel photonic integrated circuit (PIC) design for obtaining large bandwidth (>50 GHz) with enhanced channel resolution (<1 GHz). A high-speed, low-loss electro-optic modulator is used to convert radio frequency energy into sidebands on an optical carrier. The designed PIC includes an input star-coupler that divides the optical power transmitted from the optical modulator among N waveguides monotonically increasing in length within an arrayed waveguide grating (AWG) that provides chromatic dispersion, an output star-coupler that forms an image of the optical spectrum, and an array of photodiodes that convert the optical power to electrical signals. The combination of a low-noise wide-band RF radiometer with an RF Photonics backend system is a key technology development allowing unprecedented ability to spectrally resolve the complete microwave spectrum which is critically needed for the planetary boundary layer sensing. In this paper, we will describe the capabilities of this system for measuring the thermodynamic structure in the lower ~2km of the atmosphere which is not available with the current state of the art technology launched in the space.

How to cite: Ogut, M., Brown, S., Misra, S., Kittlaus, E., Kangaslahti, P., Murakowski, J., and Gehl, M.: Ultra-wideband RF photonics spectrometer for atmospheric boundary layer sensing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14672, https://doi.org/10.5194/egusphere-egu25-14672, 2025.

EGU25-15291 | ECS | Posters on site | AS2.1

Extending turbulence generation methods for efficient mesoscale-to-LES coupling 

Nicolai Krieger and Christian Kühnlein

Advances in computational power have enabled atmospheric simulations across a broad range of scales, including the coupling of mesoscale simulations to nested large-eddy simulations (LES), where the largest turbulent eddies in the atmospheric boundary layer are resolved. However, resolved turbulence does not instantaneously develop at the mesoscale-LES interface, necessitating turbulence generation methods to accelerate the transition from the smoother mesoscale inflow to resolved turbulence in the domain interior.
We evaluate two turbulence generation methods that both apply pseudo-random perturbations at the lateral inflow boundaries. These methods are the cell perturbation method (CPM), which introduces potential temperature perturbations, and the force CPM (FCPM), which applies vertical force perturbations at the lateral boundaries. Building on the previous suggestion for the FCPM, we derive an optimized scaling law for the perturbation amplitude in this turbulence generation method. The scaling law accounts for simulation setup and inflow characteristics, including wind speed, wind direction, and static stability, and is validated using LES of idealized boundary layers.
Additionally, we perform real-case atmospheric LES that reveal significant limitations of the CPM, such as spurious precipitation under specific atmospheric conditions. In contrast, the FCPM, particularly with our proposed extensions, demonstrates robust performance, producing minimal artefacts while effectively accelerating turbulence generation, making it the preferred method for turbulence generation.
We further discuss pathways to generalize the FCPM for larger domains and longer simulations, addressing challenges such as spatially and temporally varying boundary layer characteristics. These advancements represent a step towards a flow- and scale-aware turbulence generation method, facilitating efficient coupling between mesoscale simulations and LES.

How to cite: Krieger, N. and Kühnlein, C.: Extending turbulence generation methods for efficient mesoscale-to-LES coupling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15291, https://doi.org/10.5194/egusphere-egu25-15291, 2025.

EGU25-15494 | ECS | Orals | AS2.1

Enhancing Microscale Urban Weather Simulations: The Role of High-Resolution Land Cover and Surface Characteristics in Turbulence-Resolving LESs for Murcia, Spain 

Eloisa Raluy-López, Domingo Muñoz-Esparza, Juan Pedro Montávez, and Jeremy Sauer

The influence of surface forcings driven by realistic land cover and surface properties remains underexplored in microscale turbulence-resolving weather simulations, especially within urban settings. Atmospheric models often rely on coarse surface property datasets (typically ranging from 500 m to 10 km), but their low resolution frequently fails to adequately capture critical local surface heterogeneities. Building-resolving large-eddy simulations (LESs) that incorporate detailed land cover and surface characteristics offer a powerful framework for investigating how urban wind speed and turbulence patterns respond to variations in land cover and surface characteristics.

This research examines the significant effects of varying land cover classifications on microscale weather simulations, considering both granularity and resolution, along with other surface characteristics. A series of detailed and comprehensive experiments were carried out for the urban-rural interface of Murcia (Spain) using NCAR-RAL’s GPU-accelerated FastEddy® LES model coupled to WRF. Three case studies over 4-hour periods with distinctive meteorological conditions were used to test different combinations of land use data, roughness length values, urban parametrizations, and driving mesoscale skin forcings. These resulted in a total of 60 LESs with a grid spacing of 10 m spanning a wide range of surface conditions. These simulations incorporated high-quality land cover and soil data, more realistic roughness length estimates, and the implementation of a local terrain smoothing method and a dynamic thermal roughness length parameterization in FastEddy®. These non-standard practices were designed to enhance the skill of the simulations.

The results reveal that configuration details, such as land cover, play a critical role in both mesoscale and microscale simulations, significantly influencing surface fluxes and turbulence generation. While simply increasing the resolution of land cover data produces minimal changes, particularly in rural settings, incorporating more realistic surface property values leads to substantial differences even when resolution remains unchanged. These findings highlight the huge importance of detailed surface characteristics in improving microscale weather predictions.

Acknowledgements: The authors acknowledge the ECCE project (PID2020-115693RB-I00) of the Ministerio de Ciencia e Innovación/Agencia Estatal de Investigación (MCIN/AEI/10.13039/501100011033). ERL thanks her predoctoral contract FPU (FPU21/02464) to the Ministerio de Universidades of Spain.

How to cite: Raluy-López, E., Muñoz-Esparza, D., Montávez, J. P., and Sauer, J.: Enhancing Microscale Urban Weather Simulations: The Role of High-Resolution Land Cover and Surface Characteristics in Turbulence-Resolving LESs for Murcia, Spain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15494, https://doi.org/10.5194/egusphere-egu25-15494, 2025.

EGU25-15917 | Posters on site | AS2.1

Horizontal and vertical analysis of sea breezes in the Gulf of Cádiz (SW Spain) from surface stations and radiosounding data 

Carlos Román-Cascón, Pablo Ortiz-Corral, Esther Luján-Amoraga, Alberto Jiménez-Rincón, Marina Bolado-Penagos, Miguel Bruno, Alfredo Izquierdo, Jielun Sun, and Carlos Yagüe

Sea breezes are mesoscale phenomena formed in coastal regions when winds at the synoptic scale are weak. During the daytime, their general (and well-known) picture includes sea-to-land winds at the surface and land-to-sea ones at a certain height, closing the breeze circulation. However, this canonical picture is rarely observed from observations due to the interactions of the sea breezes with other flows, such as those related to the background (weak to moderate) synoptic conditions, the development of other local flows and/or the interactions with other processes within the atmospheric boundary layer, among others. This study shows an in-depth analysis of these interactions based on data gathered from surface stations and radiosoundings launched during different sea-breeze events detected in the northern zone of the Gulf of Cádiz (SW Spain). These winds have important impacts in this area during summer, especially due to their capacity to refresh warm temperatures and transport humidity.

This study has been developed within the LATMOS-i1, WINDABL2, and WIND4US3 projects, all of which include, among their objectives, the study of the interaction between coastal breezes and upper winds through different observational and modelling strategies. In this work, we present part of the observational strategy developed at the Gulf of Cádiz, which consisted of 1) the installation of meteorological and atmospheric turbulence stations at strategic locations for the long-term monitoring of breezes, as well as; 2) the launching of atmospheric radiosoundings during intensive observation periods characterised by sea-breeze conditions. We also present some results from the analysis of events with different characteristics, allowing us to highlight how they differ during contrasting background winds and under conditions with different thermodynamic vertical structures of the atmospheric boundary layer.

1 The LATMOS-i project (PID2020-115321RB-I00) (Land-ATMOSphere interactions in a changing environment: How do they impact on atmospheric-boundary-layer processes at the meso, sub-meso and local scales in mountainous and coastal areas?), funded by MCIN/AEI/ 10.13039/501100011033.

2 The WINDABL project (PR2022-055) (How are the Surface Thermally Driven Winds influenced by the vertical structure and horizontal inhomogeneities of the Atmospheric Boundary Layer?), funded by Plan Propio de la Universidad de Cádiz, Convocatoria 2022 de Proyectos para investigadores nóveles.

3The WIND4US project (CNS2023-144885) (Disentangling the complexity of the WIND systems in coastal areas FOR a better Understanding of their impacts on Society), funded by Convocatoria 2023 de Proyectos de Consolidación Investigadora.

How to cite: Román-Cascón, C., Ortiz-Corral, P., Luján-Amoraga, E., Jiménez-Rincón, A., Bolado-Penagos, M., Bruno, M., Izquierdo, A., Sun, J., and Yagüe, C.: Horizontal and vertical analysis of sea breezes in the Gulf of Cádiz (SW Spain) from surface stations and radiosounding data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15917, https://doi.org/10.5194/egusphere-egu25-15917, 2025.

Reynolds stress anisotropy is one of the fundamental characteristics of all wall bounded turbulent flows, especially those in the atmosphere. In canonical (flat and horizontally homogeneous) boundary layers, the anisotropy presents a balance between the processes that generate it (shear, buoyancy and wall blocking) and the pressure-redistribution terms that act to redistribute turbulent kinetic energy towards the non-energetic velocity components. This pressure redistribution remains an area of active research, especially in stratified conditions, dominating the atmospheric surface layer.

Here we use observations from four turbulence towers in flat and horizontally homogeneous terrain to explore the evolution of anisotropy as the stratification becomes increasingly unstable. We identify three regions that can be roughly related to dynamic, convective-dynamic, and convection regimes, and show which processes, including turbulence organization into coherent structures, dominate anisotropy in each region, and particularly what is the role of rapid pressure-redistribution terms in driving the decrease of wall-normal and increasing spanwise variance in the dynamic-convective region.

How to cite: Stiperski, I. and Katul, G. G.: Energy anisotropy, turbulence organization and the role of pressure-redistribution in near-surface unstably-stratified turbulence, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16649, https://doi.org/10.5194/egusphere-egu25-16649, 2025.

EGU25-16689 | ECS | Posters on site | AS2.1

Statistical Analysis of Nocturnal Downvalley Flows Over the Annual Cycle: Insights from a Pyrenean Valley (France) 

Pablo Ortiz-Corral, Carlos Román-Cascón, Juan Alberto Jiménez-Rincon, Fabienne Lohou, Marie Lothon, Mariano Sastre, Jielun Sun, and Carlos Yagüe

Nocturnal downvalley flows were examined in a valley located in southern France, near the Pyrenees. Three meteorological stations were strategically placed at different locations within the valley, collecting a year-long dataset of near-surface observations. This dataset enables an investigation of how these flows are organized and evolve throughout the annual cycle.

To identify the downvalley flow events, we applied a breeze detection algorithm (Arrillaga et al., 2018; Román-Cascón et al., 2019). Once detected, the events were characterized in terms of onset, peak intensity, and duration, with particular attention paid to the synoptic conditions conducive to their development. A clustering approach was also employed to classify and compare subtypes of breeze days, providing insights into their controlling factors and distinctive features.

Furthermore, a statistical analysis differentiating various turbulence regimes (incorporating HOckey STick (HOST)  analysis) offers a deeper understanding of how turbulence interacts with flow dynamics. Overall, this work seeks to advance our knowledge of the mechanisms driving thermally-driven flows in complex terrain over a full annual cycle.

How to cite: Ortiz-Corral, P., Román-Cascón, C., Jiménez-Rincon, J. A., Lohou, F., Lothon, M., Sastre, M., Sun, J., and Yagüe, C.: Statistical Analysis of Nocturnal Downvalley Flows Over the Annual Cycle: Insights from a Pyrenean Valley (France), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16689, https://doi.org/10.5194/egusphere-egu25-16689, 2025.

EGU25-16873 | Posters on site | AS2.1

Retrieving Parameters of the Planetary Boundary Layer from Near- and Thermal-infrared Satellite Observations 

Jan El Kassar, Cintia Carbajal Henken, Rene Preusker, and Jürgen Fischer

We present our progress towards satellite-based monitoring of one or more key parameters of the well-mixed, planetary boundary layer (PBL). These may include the boundary layer height and the boundary layer moisture for clear-sky pixels. These influence the initiation and life cycle of convective clouds and storms. Remote sensing of these parameters could be beneficial to short-range forecasting, nowcasting and process studies.

In our work, we utilize observations in the near-infrared (NIR) at 0.9 µm and in the thermal-infrared (TIR) at 11 µm. In the NIR-region we exploit bands placed inside and shortly outside a water vapour (WV) absorption feature which allows us to sense the total column of WV (TCWV). In the TIR-region, we use the so-called split-window bands. Typically, these bands are positioned at 11 µm and 12.2 µm, respectively. The difference of the two channels is the split-window difference (SWD). The SWD is affected by the surface emissivity, the air temperature and the WV content in the layers above. For example, the new Flexible Combined Imager (FCI) on the geostationary satellite Meteosat Third Generation (MTG) carries these measurements, allowing the monitoring at 10 min temporal resolution and at 1 km spatial resolution.

In initial sensitivity studies, we explore the potential of the SWD for PBL remote sensing. The SWD can be linked to the thickness of the mixed layer, as well as the moisture contained in the mixed-layer. However, ambiguity exists in distinguishing between thickening and moistening processes within the PBL. Combining these observations, with their different sensitivities to WV distribution, may help resolve the ambiguity to some extent and provide more robust information on the moisture distribution in the PBL.

Our current efforts focus on investigating how to optimize the integration of these complementary measurements to enhance the retrieval of not only the TCWV but also additional information on the moisture structure in the lower levels of the atmosphere. 

How to cite: El Kassar, J., Carbajal Henken, C., Preusker, R., and Fischer, J.: Retrieving Parameters of the Planetary Boundary Layer from Near- and Thermal-infrared Satellite Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16873, https://doi.org/10.5194/egusphere-egu25-16873, 2025.

The interaction between sea ice and atmosphere depends strongly on the exchange of momentum and heat in the Arctic boundary layer (BL). The representation of the Arctic BL is still a major source of uncertainty in recent climate models since they struggle to accurately model turbulent exchange in the predominantly stable-stratified BL of the Arctic. An additional source of uncertainty is the representation of sea-ice roughness in climate models. Sea-ice roughness is an important factor determining the mechanical production of turbulence. Here, we study the performance of the BL scheme of the numerical weather prediction model ICON-NWP and investigate the sensitivity to different values of sea-ice roughness. Therefore, we set-up ICON limited area simulations forced by ERA5 that include the track of the MOSAiC campaign in 2019-2020 and apply different values for the sea-ice roughness. ICON takes a constant roughness value for sea ice (default: 0.001 m) within a sea-ice tile whenever the ice thickness reaches a critical value. The results are compared to turbulence measurements during MOSAiC and we further investigate regional effects that occur in relation to the changed roughness values.

How to cite: Gebhardt, F. and Handorf, D.: Simulations of Arctic winter stable-boundary layers during MOSAiC campaign using ICON-NWP and the influence of sea-ice roughness, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17533, https://doi.org/10.5194/egusphere-egu25-17533, 2025.

This study evaluates two models for simulating near-field (<200 m) atmospheric dispersion: an operational Lagrangian model, and Computational Fluid Dynamics (CFD) simulations, including Reynolds-Averaged Navier-Stokes (RANS) and Large Eddy Simulation (LES) approaches. The evaluation is conducted against data from a full-scale atmospheric tracer experiment.

The first  model is the Safety Lagrangian Atmospheric Model (SLAM)[1], which implements a Lagrangian stochastic particle dispersion framework coupled with pre-calculated wind and turbulence fields derived from a series of RANS simulations performed with ANSYS Fluent CFD code. On the other hand, the CFD dispersion simulations employ the open-source CALIF3S solver including both RANS and LES methodologies[2] The turbulence closure models correspond respectively to a  standard two-equation RANS model and a hybrid RANS/LES approach based on a Detached-Eddy-Simulation (DES) methodology. The full-scale atmospheric dispersion experiment DIFLU (Dispersion du Fluor 18 en Milieu Urbain)[3], provides the validation dataset. The experiment includes tracer concentration measurements under various meteorological conditions within 500 meters of a cyclotron facility.

The results demonstrate that SLAM predicts concentration values comparable to those obtained by CALIF3S-RANS despite the distinct inlet boundary conditions. SLAM uses similarity theory to calculate the inlet velocity, temperature and turbulent profiles, whereas inlet profiles used in CALIF3S are extracted from precursor simulations that best match the measurements. In the near-source region (<50 m), where turbulence plays a significant role, both CALIF3S-RANS and SLAM overestimate the concentration distributions compared to those given by CALIF3S- LES approach. LES results are closer to the measurement because of its advantage in predicting eddy detachments. The disparity of concentration values between RANS and LES diminishes rapidly beyond 100 m from the source, where the region is free of buildings. Overall, SLAM and CALIF3S-LES achieve similar performance in terms of the fraction of simulated values within a factor of two of the measurements under neutral atmospheric conditions. Hence, using RANS simulation is sufficient to achieve acceptable results in the near-field dispersion simulation (<200m) under neutral atmospheric conditions. Nevertheless, more precise results can be achieved with LES method in the near source region (<50m). Future work will focus on other experimental cases, including unstable atmospheric conditions.

 

[1]        S. Yang, I. Korsakissok, P. Laguionie, and P. Volta, “Dispersion du FLuor 18 en milieu Urbain near-field (>200m) atmospheric dispersion simulation and sensitivity analysis following a full scale atmospheric tracer experiment,” in 22nd Harmonisation within Atmospheric Dispersion Modelling for Regulatory Purposes

[2]        J. Janin, F. Duval, C. Friess, and P. Sagaut, “A new linear forcing method for isotropic turbulence with controlled integral length scale,” Phys. Fluids, vol. 33, no. 4, Apr. 2021, doi: 10.1063/5.0045818/1065646.

[3]        P. Laguionie et al., “Investigation of a Gaussian Plume in the Vicinity of an Urban Cyclotron Using Helium as a Tracer Gas,” Atmosphere (Basel)., vol. 13, no. 8, pp. 1–16, 2022, doi: 10.3390/atmos13081223.

 

How to cite: Yang, S., Duval, F., and Korsakissok, I.: Comparison of atmospheric dispersion simulations in the near field (<200) with operational Lagrange model and CFD methods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17827, https://doi.org/10.5194/egusphere-egu25-17827, 2025.

EGU25-18484 | ECS | Orals | AS2.1

Parameterization of the Turbulence Averaging Error by Doppler Wind Lidars: a Simulator Approach 

Andreu Salcedo-Bosch, Francesc Rocadenbosch, Simone Lolli, Jakob Mann, and Alfredo Peña

Wind energy is a crucial component of the global energy market due to its minimal environmental impact and continuous technological advancements. Offshore wind energy, characterized by stronger and more homogeneous winds compared to onshore locations, has attracted significant interest from the industry [1]. However, the remote and inaccessible nature of offshore wind farms presents challenges for wind resource assessment. Traditional methods, such as anemometers mounted on masts, are not feasible in these environments. Doppler wind lidars (DWLs) have emerged as a viable alternative, providing cost-effective and flexible measurements of wind vectors at hub-height altitudes. DWL are highly accurate in deteriming the line-of-sight velocity. Despite this, DWLs inherently underestimate or overestimate wind turbulence, a key parameter for wind energy applications, due to the spatial and temporal averaging effect that result from the probe volume and the scanning configuration [2]. This turbulence biase can lead to over-design or increasing loads on wind turbines, significantly increasing costs.

To address this challenge, a DWL and anemometer simulator based on the Mann turbulence spectral model was developed, capable of generating high-resolution synthetic turbulent wind fields using the three Mann model parameters: turbulence length scale (​L), eddy life-time parameter (Γ), and turbulent energy dissipation rate [3]. The simulator replicates the IJmuiden offshore meteorological mast (metmast) measuring setup, allowing direct comparisons between DWL and anemometer measurements at a height of 90 m. Turbulence fields were simulated across a wide range of Mann parameter values to cover a wide range of atmospheric turbulence conditions.

The simulation results revealed that DWLs underestimate turbulence up to 50% with respect to anemometers when L approximated 0 m. Conversely, Γ had negligible influence on DWL turbulence measurements. The error in turbulence estimation by DWLs was successfully parameterized by the lturbulence length scale L, drastically reducing computational complexity while maintaining accuracy.

These findings provide a practical framework for correcting DWL turbulence measurement errors, facilitating their application in diverse atmospheric scenarios. Future work will focus on validating the parameterization with experimental data under varied atmospheric conditions and implementing the correction method to improve DWL performance in operational settings. By addressing this limitation, the results advance the reliability of offshore wind resource assessments, contributing to the broader adoption of wind energy solutions.

REFERENCES

[1] Joyce Lee and Feng Zhao, “Global wind report 2018,” Tech. Rep., Global Wind Energy Council, Apr. 2019.

[2] A. Peña, G. G. Yankova, and V. Mallini, “On the lidar-turbulence paradox and possible countermeasures,” Wind Energy Science, vol. 10, no. 1, pp. 83–102, 2025.

[3] Jakob Mann, “Wind field simulation,” Probabilistic Engineering Mechanics, vol. 13, no. 4, pp. 269–282, 1998.

 

ACKNOWLEDGEMENTS

This research is part of the project PID2021-126436OB-C21 funded by Ministerio de Ciencia e Investigación (MCIN)/Agencia Estatal de Investigación (AEI)/ 10.13039/501100011033 y FEDER “Una manera de hacer Europa” and part of the PRIN 2022 PNRR, Project P20224AT3W funded by Ministero dell’Universit`a e della Ricerca. The European Commission collaborated under projects H2020 ATMO-ACCESS (GA-101008004) and H2020 ACTRIS-IMP (GA-871115).

How to cite: Salcedo-Bosch, A., Rocadenbosch, F., Lolli, S., Mann, J., and Peña, A.: Parameterization of the Turbulence Averaging Error by Doppler Wind Lidars: a Simulator Approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18484, https://doi.org/10.5194/egusphere-egu25-18484, 2025.

EGU25-18608 | Orals | AS2.1

Wind and turbulence measurements with different sonic sensor head geometries 

Hans-Juergen Kirtzel, Finn Burgemeister, and Gerhard Peters

Measurements of wind and turbulence variables have been performed for decades by means of ultrasonic anemometers (sonics), which have proven to be a reliable, cost-effective and accurate measurement technique for both operational and scientific applications. Sonics are using short ultrasonic pulses transmitted between transducers along different measuring paths to retrieve the 3D wind information. While the measurement principle of commercially available sonics follows comparable technical approaches a variety of sensor head geometries and path arrangements are used in order to minimize potential constraints in accuracy. Two main aspects have to be regarded here, a shadow effect appearing lee wards of each transducer element and a flow distortion caused by individual structures of sensor heads. Furthermore, the arrangement of the measuring paths determines the responsiveness of the sensor to specific wind components. For studies in the atmospheric boundary layer typically the vertical wind component is of highest interest. In order to address these various requirements with one system, trade-offs are unavoidable. The Multi-Path approach for sonics allows to establish redundant 3 x 3 measuring paths involving only six transducers. Depending on the inflow angle such overdetermined system of simultaneously measured radial winds allows to select measuring paths with minimized impact from shadowing and flow distortion for data retrieval. Three of these measuring paths are aligned vertically, providing three independent measurements of the vertical wind.

A six-month comparison of five sonic types was performed in northern Germany at an abandoned airfield with a homogenous surface. We will present derived time series of wind and comprehensive turbulences variables including vertical turbulent fluxes of heat and momentum also covering periods of different weather types, e.g. precipitation events. We focus on the sonic similarities and differences, which are also relevant if standardisation of techniques and data retrievals are considered, without discarding technical improvements such as the Multi-Path technology.

How to cite: Kirtzel, H.-J., Burgemeister, F., and Peters, G.: Wind and turbulence measurements with different sonic sensor head geometries, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18608, https://doi.org/10.5194/egusphere-egu25-18608, 2025.

EGU25-438 | ECS | Orals | AS2.2

The Role of Data Assimilation in Enhancing Warm Fog Predictions Over Delhi and NCR 

Avinash Parde and Sachin Ghude

Fog forecasting over highly urbanized and fog-prone regions like Delhi and the National Capital Region (NCR) in the Indo-Gangetic Plain (IGP) is challenging due to the complex interplay between land surface processes and atmospheric conditions. This research investigates the role of advanced data assimilation techniques in enhancing fog forecasting accuracy using high-resolution numerical weather prediction (NWP) models. The focus is on improving the prediction of fog lifecycle events, including onset, duration, and dissipation, by integrating land surface data and non-conventional atmospheric observations into NWP systems.

The study begins with the implementation of the High-Resolution Land Data Assimilation System (HRLDAS) to improve the initialization of critical land surface variables, such as soil moisture and soil temperature. These variables play a key role in surface energy exchanges and boundary layer dynamics. Sensitivity experiments show that incorporating fine-gridded land surface data into the Weather Research and Forecasting (WRF) model significantly improves near-surface temperature, humidity, and wind forecasts. This results in a substantial reduction in soil moisture bias and a more accurate representation of land-atmosphere interactions, leading to enhanced predictions of fog onset and dissipation in the NCR region. Building on this, the research employs cyclic assimilation of microwave radiometer (MWR) observations to improve the vertical profiles of atmospheric temperature and humidity. The combined assimilation of MWR profiles and HRLDAS-generated land surface fields enhances the boundary layer structure, which is critical for fog formation and dissipation. Results demonstrate that the assimilation of non-conventional data sources improves the spatial and temporal accuracy of fog forecasts, reducing errors in predicting fog intensity and duration. These findings emphasize the importance of high-resolution observational data and advanced assimilation techniques for capturing the microphysical and thermodynamic processes governing fog development.

This study demonstrates the importance of integrating land data assimilation and high-resolution atmospheric observations into NWP systems to enhance fog forecasting. The techniques developed address challenges posed by complex land-atmosphere interactions and can be applied to other fog-prone regions. By improving the understanding of fog dynamics, this work enables more accurate and timely forecasts, benefiting critical sectors like aviation, transportation, and public safety in regions such as the IGP.

 

How to cite: Parde, A. and Ghude, S.: The Role of Data Assimilation in Enhancing Warm Fog Predictions Over Delhi and NCR, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-438, https://doi.org/10.5194/egusphere-egu25-438, 2025.

Rain, fog drip, shallow soil water and groundwater were collected for stable isotopic analysis, at a tropical seasonal rain forest site in Xshuangbanna, Southwest China. The fog drip water ranged from -30 to +27% in δD and -6.2 to +1.9% in δ18O, conforms to the equation δD=7.64δ18O+14.32, and was thought to contain water that has been evaporated and recycled terrestrial meteoric water. The rain was isotopically more depleted, and ranged from -94 to -45% in δD, and -13.2 to -6.8% in δ18O. The shallow soil water had a composition usually between those of the rain and fog drip, and was assumed to be a mixture of the two waters. However, the soil water collected in dry season appeared to contain more fog drip water than that collected in rainy season. The groundwater in both seasons had an isotopic composition similar to rainwater, suggesting that fog drip water does not play a significant role as a source of recharge for the groundwater. This groundwater was thought to be recharged solely by rainwater.

How to cite: Zhang, Y. and Liu, W. J.: Fog drip and its relation to groundwater in the tropical seasonal rain forest of Xishuangbanna, Southwest China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-445, https://doi.org/10.5194/egusphere-egu25-445, 2025.

EGU25-1573 | Posters on site | AS2.2

Microphysical Characteristics of Arctic Summer Sea Fog 

Li Yi

The opening of the Arctic Ocean shipping route has significantly benefited the shipping industry. However, low visibility (Vis) in the Arctic Ocean due to fog can lead to a serious challenge during ship navigation. This study proposes a new method for analyzing the ship-based sea fog microphysical observations collected during the ice-breaker Xuelong I expedition to Arctic Ocean in 2016 and 2018, as well as the Xuelong II in 2020. The Vis calculated by droplet size distribution (DSD) using the new method aligns more closely with observed Vis. In the data analysis, both old and new methods are applied to check the droplet size distribution types: (1) double peak DSD model, which influences bulk values of microphysical parameters such as liquid water content (LWC), droplet number concentration (Nd), and effective diameters (Deff) and (2) a single peak gamma distribution model. Both DSDs obtained by two methods suggested that microphysical characteristics of sea fog adhere more closely to a Gamma-exponential size distribution rather than a Gamma distribution, with double peak values at about 6 and 22 µm. It is concluded that DSD of Arctic fog during summer months have two peak values and can affect fog microphysical properties heavily compared to a single Gamma DSD.

How to cite: Yi, L.: Microphysical Characteristics of Arctic Summer Sea Fog, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1573, https://doi.org/10.5194/egusphere-egu25-1573, 2025.

EGU25-1966 | Posters on site | AS2.2

Seasonal fog enhances crop water productivity in a tropical China rubber plantation 

Palingamoorthy Gnanamoorthy, Yiping Zhang, and Qinghai Song

The rapid conversion of tropical rainforests into monoculture plantations of rubber (Hevea brasiliensis) in Southeast Asia (SEA) necessitates understanding of rubber tree physiology under local climatic conditions. Frequent fog immersion in the montane regions of SEA may affect the water and carbon budgets of the rubber trees and the plantation ecosystems. We studied the effect of fog on various plant physiological parameters in a mature rubber plantation in southwest China over 3 years. During the study period, an average of 141 fog events occurred every year, and the majority occurred during the dry season, when the temperature was relatively low. In addition to the low temperature, fog events were also associated with low vapor pressure deficit, atmospheric water potential, relative humidity and frequent wet-canopy conditions. We divided the dry season into cool dry (November-February) and hot dry (March-April) seasons and classified days into foggy (FG) and non-foggy (non-FG) days. During the FG days of the cool dry season, the physiological activities of the rubber trees were suppressed where carbon assimilation and evapotranspiration showed reductions of 4% and 15%, respectively, compared to the cool dry non-FG days. Importantly, the unequal declines in carbon assimilation and evapotranspiration led to enhanced crop water productivity (WPc) on cool dry FG days but insignificant WPc values were found between FG and non-FG days of the hot dry season. Our results suggest that, by regulating plant physiology, fog events during the cool dry season significantly reduce water demand and alleviate water stress for the trees through improved WPc.

How to cite: Gnanamoorthy, P., Zhang, Y., and Song, Q.: Seasonal fog enhances crop water productivity in a tropical China rubber plantation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1966, https://doi.org/10.5194/egusphere-egu25-1966, 2025.

EGU25-2221 | Posters on site | AS2.2

Sea Fog under the North Wind with the Influence of Foehn Wind in the Okhotsk Sea 

Yue-Chao Jiang, Li Yi, and Su-Ping Zhang

The Okhotsk Sea is renowned as one of the world's most foggy regions. Previous studies have identified that sea fog occurring under south winds is mainly advection fog. However, the formation mechanism of sea fog under north winds remains unclear. On August 21, 2019, the research vessel "Xiangyanghong 01" observed a phenomenon where low clouds transformed into sea fog in the waters north of the Kuril Islands under north wind . Analysis of shipborne observations, reanalysis data, and simulation results show that during this sea fog event, the upper-level atmospheric circulation over the Pacific was characterized by a cut-off low and blocking high. The stable circulation provided favorable conditions for the sea fog within the Okhotsk Sea. From August 19 to 21, influenced by east winds between tropospheric systems, the east-west mountain flow over the Kamchatka Peninsula intensified continuously. The Foehn effect on the western coast of the peninsula led to a significant increase in air temperature, enhancing the advection of warm air from land to sea, particularly between 925 hPa and 950 hPa. As this warm dry air ascended above the moist air mass over the sea, it strengthened the temperature inversion and lowered the inversion layer base, thereby promoting cloud descent and the formation of sea fog. Furthermore, under north winds, the subcloud air mass experienced evaporation of warm sea surface and cooling of cold sea surface of the eastern Okhotsk Sea. The subcloud air mass became saturated with moisture, leading the downward development of the cloud layer into sea fog.

How to cite: Jiang, Y.-C., Yi, L., and Zhang, S.-P.: Sea Fog under the North Wind with the Influence of Foehn Wind in the Okhotsk Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2221, https://doi.org/10.5194/egusphere-egu25-2221, 2025.

EGU25-2705 | Posters on site | AS2.2

Sea Fog Top Height Retrieval over the Yellow Sea andBohai Sea Using Island Elevation 

Pinglv Yang, Yuzhu Tang, Xiaofeng Zhao, Yuxing Wang, and Zeming Zhou

Sea fog has significant impacts on both human activities and the natural environment. Sea fog top height (SFTH) reflects the impact of sea fog on vertical space and is a crucial parameter for both Numerical Weather Prediction models and the estimation of sea fog dissipation. The existing SFTH retrieval methods based on spaceborne passive radiometers are prone to significant errors. We focus on the Yellow and Bohai Seas region and introduce a high-precision SFTH retrieval algorithm based on the peak elevation (PE) of islands in the area. In remote sensing images, islands of different PE within the sea fog regions exhibit two distinct appearances either visible or obscured by the fog. Thus, islands are automatically classified into two categories by support vector machine. The relationship between SFTH and the corresponding sea fog reflectance (SFR) in remote sensing images is established by defining a linear decision boundary in the SFR-PE space through logistic regression or support vector machine to effectively separate the two island categories. Validation experiments on twelve sea fog cases show that the proposed method exhibits higher accuracy compared to the MODIS cloud top height product and demonstrates good agreement with CALIPSO data.

How to cite: Yang, P., Tang, Y., Zhao, X., Wang, Y., and Zhou, Z.: Sea Fog Top Height Retrieval over the Yellow Sea andBohai Sea Using Island Elevation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2705, https://doi.org/10.5194/egusphere-egu25-2705, 2025.

EGU25-3435 | Orals | AS2.2

New light on “fog”? 

Otto Klemm and Neng-Huei (George) Lin

„The term ‘fog’ is used when microscopic droplets reduce horizontal visibility at the Earth’s surface to less than 1 km” (https://cloudatlas.wmo.int/en/fog-compared-with-mist.html). This simple, traditional definition has proven very useful, it has been applied for decades in meteorological observations by the naked eye and – more recently – by instrument recordings. The term ‘mist’ is used “when the droplets do not reduce horizontal visibility to less than 1 km” (cloudatlas.wmo.int, see above). Both fog and mist are often associated with air pollution, specifically high aerosol load within the boundary layer, which leads to large number concentrations of small droplets. Such small hydrometeors are often non-activated. The increase of air quality (decrease of aerosol particle concentrations) worldwide leads to a decrease of fog. Yet, what are the microphysical conditions of fog in a clean atmospheric environment? Will fog form only when droplets are activated? Recently employed fog droplet size spectrometers of various manufacturers allow a deeper insight into the microphysical conditions of fog and will shed light on the role of activation of fog condensation nuclei (FCN) on the formation of fog, its interaction with air pollution, and its trends before the backdrop of climate change.

How to cite: Klemm, O. and Lin, N.-H. (.: New light on “fog”?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3435, https://doi.org/10.5194/egusphere-egu25-3435, 2025.

EGU25-3488 | Posters on site | AS2.2

Environmental factors affecting fog formation 

Iva Hunova, Marek Brabec, Marek Malý, Jan Geletič, Alexandru Dumitrescu, and Anna Valeriánová

Fog is an important phenomenon related to both atmospheric physics and chemistry, and has a significant impact on our environment. Although the meteorological factors relevant to fog formation have been extensively studied, other factors remain unexplored. Here we summarise our recent results from several studies (Hůnová et al., 2018, 2021 a, 2021 b, 2022), where we examined observed and measured long-term data from the Czech Republic (1989–2015) and Romania (1981–2017). Our focus was on the environmental factors that drive fog formation. Specifically, we examined the effects of terrain, water and forests (for Romania), and ambient air pollution (for the Czech Republic). The long-term empirical data   were analysed using advanced statistical modelling GAM (generalised additive model). In terms of terrain, apart from altitude, slope and landform appeared to have a strong influence on fog formation. Forests have a significant effect on fog formation, the most significant being the forest area within 3 km of the the fog observation point, with coniferous and broad leave trees having different effects. Not surprisingly, the presence of water body in the vicinity of a fog site affects fog formation, but less so than altitude or seasonality. Freshwater and seawater show clear differences in both the seasonal profile and frequency of fog. Ambient air pollution, indicated by the daily mean concentrations of  sulphur dioxide and nitrogen oxides, was the most important explanatory variable (apart from relative humidity) in modelling the probability of fog at three Centre European sites reflecting different environments (urban, rural and mountain).

References:

Hůnová I., Brabec M., Geletič J., Malý M., Dumitrescu A., 2021 a. Statistical analysis of the effects of forests on fog. STOTEN, https://doi.org/10.1016/j.scitotenv.2021.146675.

Hůnová I., Brabec M., Geletič J., Malý M., Dumitrescu A., 2022. Local fresh- and sea-water effects on fog occurrence. STOTEN, https://doi.org/10.1016/j.scitotenv.2021.150799.

Hůnová I., Brabec M., Malý M., Dumitrescu A., Geletič J., 2021 b. Terrain and its effects on fog occurrence. STOTEN, https://doi.org/10.1016/j.scitotenv.2020.144359.

Hůnová I., Brabec M., Malý M., Valeriánová A., 2018. Revisiting fog as an important constituent of the atmosphere.  STOTEN, https://doi.org/10.1016/j.scitotenv.2018.04.322.

 

Acknowledgements:

We are grateful to the Czech Hydrometeorological Institute and Meteo Romania for providing the input data. Our study was supported by the Technological Agency of the Czech Republic (TAČR) through the project SS02030031 ARAMIS, by the Czech Hydrometeorological Institute research project ʽDlouhodobá koncepce rozvoje výzkumné organizace (DKRVO) Český hydrometeorologický ústav’ financed by the Czech Ministry of the Environment, and by the long-term strategic development financing of the Institute of Computer Science (Czech Republic RVO 67985807).

How to cite: Hunova, I., Brabec, M., Malý, M., Geletič, J., Dumitrescu, A., and Valeriánová, A.: Environmental factors affecting fog formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3488, https://doi.org/10.5194/egusphere-egu25-3488, 2025.

EGU25-3506 | Posters on site | AS2.2

Characteristics of Jet Stream in Low-altitude Airspace and Impact to Fog in Tianjin Urban Areas 

Bingui Wu, Tingting Ju, and Meng Tian

This study analyzed the temporal and spatial distribution characteristics of jet stream in low airspace (1500 meters) and the impact to fog in Tianjin urban areas, based on the data of the boundary layer wind profiler and the 255 m Meteorological Tower during 2016-2018.

The statistical results show that: (1) As for the distribution height of wind jet stream, there are two peak heights within 1500 m, one peak is within 500-600 m, about 23% of the wind stream jet is located at the height; The other peak is located in the 200-300 m range, and about 19% of the jet stream is located at the height; and wind jet streams are more evenly distributed in other low-altitudes airspace. (2) As for the height and frequency seasonal distribution characteristics of the jet stream, the average height of the jet stream is generally located at 700-1000 m, and the seasonal variation of the jet height is not obvious, but the height of the cold season is higher than that of the warm season. The frequency of stream jet in 300-1500 m layer is the lowest in December and the highest in May. In contrast, the low-level jet within the 300 m layer occurs more frequently during the transition from warm to cold season, accounting for about 70% in autumn and winter, with the lowest frequency in June and the highest in October. (3) As for the diurnal distribution characteristics and wind direction of the jet stream, the frequency of wind stream jet at 300-1500 m layer increased at sunset, and the high frequency lasted until dawn of the next day, the character is the same for the low-altitude jet below 300 m, and the frequency during nighttime is more than 70%, far more than the frequency of wind jet at the upper layer. The prevailing jet direction is southwest, accounting for 47%; Followed by northerly wind, accounting for 17%; The southeast (90-180°) jet direction is less than 20%, while the northwest low-level jet stream least frequent. (4) The southerly jet before the fog, which was conducive to the formation of fog, transported water vapor to the fog area; while the northerly jet have bidirectional effect of leading to fog burst or dissipation, which afford to the fog area with cold air and kinetic energy.

In conclusion, Due to sparse vertical layer data, such as the FNL reanalysis data, the features of low-altitude airspace jet are rough, especially those below 300 meters. This study supplemented the understanding of the distribution characteristics of the low-altitude jet under 300 m and the effect to fog in Tianjin urban area, which is important for fog forecasting and low-altitude flight meteorological service .

 

How to cite: Wu, B., Ju, T., and Tian, M.: Characteristics of Jet Stream in Low-altitude Airspace and Impact to Fog in Tianjin Urban Areas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3506, https://doi.org/10.5194/egusphere-egu25-3506, 2025.

EGU25-4376 | Posters on site | AS2.2

Evaluation and improvement study on the planetary boundary-layer scheme for fog-forecasting in North China 

Jianbo Yang, Bingui Wu, Meng Tian, Hailing Liu, and Yunchen Liao

The numerical forecast of fog is still challenging at the current stage, as many models typically show poor fog-forecasting capabilities. Model predictions of fog exhibit strong sensitivity to the selection of planetary boundary layer (PBL) parameterizations, as well as horizontal grid spacing (HGS). To address this issue, this study intercompares the fog-forecasting performance of WRF model using five PBL schemes (YSU, MYJ, MYNN, ACM2 and SH) and different HGS ranging from ten-kilometric- to hectometric-scale (15-km to 500-m). Validation against available in-situ measurements indicates that the YSU scheme produces an overall superior performance in fog forecasting, followed by MYNN and MYJ. For a certain PBL scheme, the model shows distinct forecasting capabilities in terms of different types of fog. That is, the model generally shows better performance in the forecasting of advection fog episodes, compared to radiation fog episodes. Regarding different HGS, intercomparisons of mesoscale modeling (i.e., WRF) with HGS ranging from ten-kilometric- to hectometric-scale (15-, 5-, 2.5-km and 500-m) reveal that, although simulations using finer HGS could generally better represent the spatial distribution of meteorological elements and the influence of small-scale underlying surface, the fog forecasting skills (i.e., the TS scores) does not consistently improve with the refinement of HGS. Fog forecasting at different HGS behaves differently for two types of fog days which are primarily differentiated by whether or not the dissipation of fog is substantially influenced by the background synoptic wind flow. For type-Ⅰ fog days (with no obvious impact of the background synoptic wind), differences in fog forecasting skills (TS values) among different HGS simulations are relatively smaller. Whereas for type-Ⅱ fog days (with the dissipation of fog strongly affected by the invasion of cold airflow), deviations in TS values among simulations using different HGS become more evident, with 2.5-km HGS providing better performance and the coarsest-HGS (15-km) simulation shows a noticeable degradation in the fog forecasting skills. Also note that simulation using the finest HGS (500-m) shows no superiority (or somewhat degradation) in fog forecasting skills for both of the two types of fog days. Additionally, the influence of model HGS on simulating the spatial distribution of fog is more pronounced during the formation and dissipation stage, whereas rather limited during the developing stage. On the basis of comprehensive model evaluation, we further attempt to improve the model performance under stable stratification by incorporating a wind-shear term into the mixing-length formulation for a turbulence scheme. After validation against available observations, results of the sensitivity experiments show that this modification could generally improve the representation of turbulent mixing, near-surface meteorological elements, as well as vertical boundary layer structures during stable conditions.

How to cite: Yang, J., Wu, B., Tian, M., Liu, H., and Liao, Y.: Evaluation and improvement study on the planetary boundary-layer scheme for fog-forecasting in North China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4376, https://doi.org/10.5194/egusphere-egu25-4376, 2025.

EGU25-4880 | Posters on site | AS2.2

Atmospheric water collection across diverse climates along the Chilean coast: unraveling synoptic to local drivers of fog harvesting 

Camilo del Río, Felipe Lobos-Roco, Vicente Espinoza, Klaus Keim-Vera, Nicolás Valdivia, Constanza Vargas, and Diego Rivera

The 3000 km long coast of Chile, characterized by a steep mountain range, interacts almost everywhere with the Southeast Pacific stratocumulus (Sc) low clouds deck, producing narrow but extensive fog banks. This long but narrow fog belt crosses diverse climates such as hyperarid (18°- 23°S), arid (23°- 28°S), semi-arid (28°- 31°S), mediterranean (31°- 34°S), and temperate (34° - 37°S), being essential for unaccountable ecosystem types and a virtual water resource to be tapped. In this work, using an extensive network of meteorological stations and standard fog collectors, combined with remote sensing observations and a numerical fog collection model, we characterize the fog water collection at multiple temporal scales, focusing on the physical conditions that allow this collection at local and larger spatial scales. Preliminary results show that the annual cycle of fog water collection along Chilean coast is closely related to the spatial variability of the thermal inversion strength across the seasons, which is the main controller of the formation of the Sc-fog cloud. Our observations taken in hyperarid climatic zones (18° - 23°S) show the highest seasonal oscillation, with peaks in winter-spring. Over arid and semi-arid climatic zones (23° - 28°S), the fog collection cycle is more constant throughout the year, showing a low seasonal oscillation. Contrary to hyperarid climatic zones, the mediterranean and temperate zones (28° - 37°) show water harvesting peaks over the summer with larger seasonal oscillation than (semi-)arid climates. The fog harvesting diurnal cycles in all climates show a decrease at midday associated with the decrease of the Sc-fog cloud presence. The maximum peaks of water collections are related to fog type being at night during advective fog events (higher liquid water content) and in the afternoon during orographic fog events (higher wind speed). In terms of water yields, these are influenced by the local conditions of the site, especially by wind speed, altitude and distance from the coast. However, the highest water collection volumes (yearly, monthly and diurnal) are found in the hyperarid and arid climatic zones (7 to 3 L m-2 d-1 in average respectively), which is consistent with the frequency of Sc-fog presence (50% in the hyper-arid and 30% in the arid). These zones are characterized by having the most fragile ecosystems and population living under a constant water scarcity. Our fog harvesting observations gathered through the largest fog monitoring network on Earth allow us for the first time to assess fog harvesting as a valuable resource in diverse climates. This network constitutes a key tool for understanding the regional and local dynamics of fog collection under a climate change context, as well as to understand its role in ecosystem conservation.

How to cite: del Río, C., Lobos-Roco, F., Espinoza, V., Keim-Vera, K., Valdivia, N., Vargas, C., and Rivera, D.: Atmospheric water collection across diverse climates along the Chilean coast: unraveling synoptic to local drivers of fog harvesting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4880, https://doi.org/10.5194/egusphere-egu25-4880, 2025.

EGU25-4971 | Posters on site | AS2.2

Research on Sea Fog Prediction in the Northwest Pacific Using Machine Learning 

Suping Zhang and Kejuan Wu

The Northwest Pacific (NWP) is a region with the highest frequency of sea fog occurrence and most widely distributed fog area in the world oceans. The sea fog prone area is located in the mid-latitudes where ocean navigations are getting more and more active. Sea fog is heavy obstacles for navigation due to low visibility in fog. The techniques of sea fog forecasting in the NWP still remains unsatisfactory compared with marginal seas so far. Using observations from ICOADS and ERA5 data from 2013 to 2021, this study tried to make sea fog prediction model in the NWP based on machine learnings. The distribution characteristics of sea fog in the NWP were analyzed and compared with China offshore fog areas. Based on analysis of sea fog occurrence, 12 key factors were identified by mutual information (MI) method, including sea surface temperature (SST), surface air temperature (SAT), SST-SAT, humidity, wind speed and direction, etc. In addition, geographical coordinates (latitude and longitude information) were also taken into consideration as factors. Four machine learning models were constructed for sea fog prediction, employing resampling techniques to address the extreme imbalance between foggy and non-foggy samples. The results demonstrated a significant enhancement in model performance by resampling, especially with oversampling, and a decline in performance was noted upon the removal of the geographical coordinates. Among the four evaluated models, the eXtreme Gradient Boosting (XGBoost), Support Vector Machine (SVM), and Convolutional Neural Network (CNN) exhibited similar performance metrics, with threat score (TS) scores about 0.3 and the Decision Tree (DT) showed more stable results. Regarding individual case performance, the XGBoost model outperformed the others, showing the highest agreement with the fog area range observed in satellite images. This study reveals the complexities of sea fog formation in the NWP and provides a scientific basis for sea fog prediction in vast expanded ocean areas.

How to cite: Zhang, S. and Wu, K.: Research on Sea Fog Prediction in the Northwest Pacific Using Machine Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4971, https://doi.org/10.5194/egusphere-egu25-4971, 2025.

Sea fog often penetrates adjacent coastal areas, a process called sea fog penetration (SFP). SFP can cause traffic accidents and other economic losses. Qingdao, an international port city with a dense population, suffers from SFP originated over the Yellow Sea in the boreal spring (March-May); the process, however, is not well studied. Based on hourly observations from buoys and automatic weather stations distributed in Qingdao and its adjacent islands, we composite SFP events to reveal their spatiotemporal features and to investigate mechanisms involved. Results show that these SFP events often penetrate inland areas from southeast to northwest and last 5-8 hours at night. We further use reanalysis data to reveal that during the daytime before SFP, strong moisture advection at 925-975 hPa brings sufficient water vapor from Yellow Sea to Qingdao; the water vapor then transfers downward to the surface via background descending motion and turbulent mixing. The daytime anomalous moistening, together with the following diurnal cooling at night, saturates the surface atmosphere and hence facilitates SFP. The strength of the SFP depends on the strength of daytime anomalous moistening. Considering the moistening leads SFP by about a day, we use this relationship to predict the intensity of SFP. The accuracy of predicting SFP events could reach 50%~80%, which highlights the predictability of intensity of SFP in Qingdao.

How to cite: Shi, X.: Distribution characteristics and Mechanism of Springtime Sea Fog Penetration, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5025, https://doi.org/10.5194/egusphere-egu25-5025, 2025.

EGU25-7865 | ECS | Posters on site | AS2.2

Aerosol Based Fog Forecasting System and Visibility Parameterization For Delhi and NCR   

Sumit Kumar, Avinash N. Parde, András Peterka, István Geresdi, Anoop Pakkattil, Gaurav Govardhan, and Sachin D. Ghude

Understanding fog microphysics involves examining the size distribution, chemical composition, and hygroscopic properties of aerosols, which influence their activation as cloud condensation nuclei (CCN) and contribute to fog droplet formation. Incorporating these aerosol-driven processes into Numerical Weather Prediction (NWP) models, such as the Weather Research and Forecasting (WRF) model, has proven essential for accurately simulating fog development, sustainment, and dissipation.

India's current operational fog forecasting systems, particularly for urban regions, often lack detailed aerosol representation. The present study integrates water-friendly and carbonaceous aerosols using climatological data (2001–2007) within the Thompson-Eidhammer Aerosol-Aware Microphysics scheme in the WRF model to enhance fog forecasting for Delhi. The system incorporates improved CCN activation to capture the vertical development of fog.

To evaluate model performance, a 10-day winter spell during the 2024–25 season was selected, including hazy conditions and dense fog events. The selected period featured two hazy days with surface visibility oscillating around 1000 meters and seven fog episodes, including four dense radiation fog events and three cloud base-lowering fog occurrences. Model validation of key meteorological variables such as 2 m temperature (T2), relative humidity (RH2), and radiative fluxes (shortwave and longwave) shows strong agreement with ground-based measurements from the Winter Fog Experiment (WiFEX) at Indira Gandhi International Airport (IGI), Delhi.

Additionally, the study introduces the development of the visibility parameterization based on aerosol extinction coefficients and cloud water mixing ratios. This diagnostic approach in the WRF model effectively captures visibility degradation due to hygroscopic aerosols under hazy conditions and during the initial phases of fog formation. The findings underscore the importance of aerosol-aware modeling in urban fog forecasting and contribute to improving visibility diagnostics.

Preliminary results from this research will be presented at the EGU 2025 conference.

How to cite: Kumar, S., Parde, A. N., Peterka, A., Geresdi, I., Pakkattil, A., Govardhan, G., and Ghude, S. D.: Aerosol Based Fog Forecasting System and Visibility Parameterization For Delhi and NCR  , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7865, https://doi.org/10.5194/egusphere-egu25-7865, 2025.

EGU25-9259 | Posters on site | AS2.2

Advancements in fog prediction in weather and climate model guided by DNS 

Anupam Hazra, Moumita Bhowmik, Avishek Ray, Sandeep Wagh, and Sachin D. Ghude

With the changing climate, the study of fog formation is essential and needs of the hour as the nature of fog has changed due to impact of complexity of natural and anthropogenic aerosols. The chemical and physical properties of cloud condensation nuclei (CCN) significantly influence fog formation and visibility, especially in regions like India. Ample water vapor, coupled with the microphysical and thermodynamic properties of CCN, plays a vital role in the occurrence and and sustenance of fog. Weather and Climate models often struggle to simulate fog droplets accurately due to the absence of aerosol indirect effects (AIE), a key factor contributing to uncertainties in aerosol-cloud interaction (ACI). The visibility calculation, which depends on the number of cloud droplets and liquid water content (LWC) in the atmosphere, is closely tied to aerosol dynamics. The conversion of aerosols into fog droplets (Nd) requires external nuclei for water vapor condensation, a process governed by condensation or diffusional growth. The condensation process is influenced by the solute effect (Raoult's effect) and the curvature effect (Kelvin effect) and may happen over a pre-existing Aitken aerosol particle. Droplet growth is determined by the size of CCN and a droplet will always try to maintain an equilibrium state and it happens if the equilibrium supersaturation is less than the amount of water vapor available in the atmosphere. The Köhler curve illustrates the interplay between the 'curvature effect' and the 'solute effect' in droplet behaviour, showing that droplets with higher solute concentrations exhibit lower critical supersaturation values, making them easier to activate into cloud droplets. Thus, hygroscopicity (κ), a key factor in CCN activation, relates to aerosol particle contributions to fog droplet formation. This is encapsulated in the κ-Köhler theory, which combines Kelvin's and Raoult's effects to describe the activation of deliquesced aerosols into cloud droplets. Hygroscopicity is linked with the water activity and thus the thermodynamics of solution governs the aerosols liquid water and hence, better understanding of hygroscopicity is essential in numerical model for the fog and visibility prediction. The evolution of the droplet size distribution (DSD) under varying aerosol-chemical conditions remains poorly understood. To reduce uncertainties in fog forecasting, the Eulerian-Lagrangian particle-based schemes in direct numerical simulation (DNS) are utilized to study the diffusional growth of droplets. Using observational data from the Winter Fog EXperiment (WiFEX) conducted at IGI airport, New Delhi, small-scale model simulations provide valuable insights into droplet activation processes. Additionally, a novel visibility parameterization has been proposed based on the small-scale model using WiFEX observed data, which incorporates both LWC and Nd. This advancement offers a pathway to more accurate fog and visibility forecasts in numerical weather prediction models.

How to cite: Hazra, A., Bhowmik, M., Ray, A., Wagh, S., and Ghude, S. D.: Advancements in fog prediction in weather and climate model guided by DNS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9259, https://doi.org/10.5194/egusphere-egu25-9259, 2025.

EGU25-9989 | ECS | Orals | AS2.2

Leveraging Integrated Water Vapor derived from GPS for fog detection and fog characteristics analysis 

Ismail Sayrou, Anouar El messari, and Driss Bari

This study characterizes the physical processes involved in fog formation through an analysis of Integrated Water Vapor (IWV) measured via GPS, combined with in situ meteorological data, with a particular focus on atmospheric humidity. The research was conducted in the Casablanca-Nouaceur airport, Morocco, where fog events present significant challenges to air transportation by severely reducing visibility. In this study, fog is modeled as a simple function of water vapor and cloud water within the framework of a non-precipitating warm cloud based on the bulk water-continuity model, with the assumption that the atmosphere above the fog layer remains horizontally homogeneous during fog events.

The objectives were to investigate the relationship between IWV and meteorological conditions during the whole lifecycle of fog events and to evaluate the potential of IWV for detecting and classifying these events. Over a six-year period (2017–2022), 207 fog episodes were analyzed in terms of occurrence, duration, intensity, and seasonal variability. The effectiveness of IWV as an indicator for fog detection and classification was also assessed. Using a fog type classification algorithm, the results revealed that that the most prevalent fog types were advection-radiation fog and stratus-lowering fog, followed by radiation fog and, less frequently, advection fog. These episodes exhibited strong seasonal variability, with higher occurrence rates during winter and autumn, corresponding to favorable meteorological conditions such as low temperatures and high relative humidity. Fog formation typically occurred during nighttime or early morning hours, dissipating gradually after sunrise.

Analysis of IWV variations before and during fog episodes revealed a consistent increase in IWV prior to fog formation, signaling an influx of moisture conducive to condensation. During the mature fog phase, IWV remained relatively stable, while the mixing ratio in the lower atmospheric layers decreased, indicating active condensation processes. These trends varied across different fog types, highlighting the complexity of the thermodynamic interactions involved. However, attempts to classify fog types based solely on IWV—using parameters such as IWV magnitude at fog onset, its amplitude during the three hours preceding formation, and its trend—proved challenging. The results demonstrate that GPS-derived IWV is a valuable tool for detecting changes in atmospheric moisture dynamics associated with fog events. However, its capacity for classifying specific fog types is limited due to the influence of additional factors, including temperature, wind patterns, and surface atmospheric conditions, which IWV measurements alone cannot capture.

Keywords : fog; GPS IWV; visibility; fog classification; water vapour; cloud water

How to cite: Sayrou, I., El messari, A., and Bari, D.: Leveraging Integrated Water Vapor derived from GPS for fog detection and fog characteristics analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9989, https://doi.org/10.5194/egusphere-egu25-9989, 2025.

EGU25-11460 | ECS | Posters on site | AS2.2

The influence of aerosol particles on fog microphysics during the Fog and Aerosol InteRAction Research Italy (FAIRARI) campaign 2021/22  

Almuth Neuberger, Rahul Ranjan, Hao Ding, Stefano Decesari, Sabine Eckhardt, Annica M. L. Ekman, Nikolaos Evangeliou, Lea Haberstock, Fredrik Mattsson, Claudia Mohr, Marco Paglione, Ilona Riipinen, Matteo Rinaldi, and Paul Zieger

The Po Valley in northern Italy is an ideal laboratory to study fog-pollution interactions. The peculiar orography of the region (enclosed between the Alps and the Apennines) promotes stable meteorological conditions and radiation fog formation in wintertime. At the same time, high population density and the several agricultural and industrial activities are responsible for high levels of pollutants, among the highest in Europe. The interaction between those factors has been studied since the 1980s, however, the detailed microphysical processes behind the aerosol-fog interactions are still to be elucidated. Therefore, in winter 2021/22, the Fog and Aerosol InteRAction Research Italy (FAIRARI) campaign took place at the research station San Pietro Capofiume, in a rural area close to Bologna. Microphysical as well as chemical aerosol and fog processes from the molecular to the droplet scale were captured.

Stockholm University’s mobile atmospheric laboratory simultaneously measured the total dried aerosol and the dried fog droplets (fog residuals), which then both were analyzed with respect to their size and (re-)activation behavior. Moreover, the chemical composition of the dried aerosol particles was determined. Meteorological parameters such as horizontal wind, updraft, and visibility were measured as well as the size distribution of the fog droplets.

We will present and discuss the influence of aerosol particles on fog microphysics during FAIRARI. For example, hydrated but not activated aerosol particles contributed to more than 50% of the visibility reduction, having implications for the definition of the beginning of fog. This in turn impacted the fog describing parameters such as the effective diameter or liquid water content (LWC), which are crucial when comparing in-situ measurements to data retrieved from satellite observations and modelling predictions. During FAIRARI, if fog is defined as LWC > 0.01 g m-3, the in-fog median LWC increases by 28% (from 0.18 g m-3 to 0.23 g m-3), compared to if fog is defined by visibility < 1km. The hygroscopicity parameter κ was calculated to be around 0.36 in the ambient aerosol out of fog and about 0.47 in the fog residuals. Moreover, sensitivity tests with the large-eddy simulation model MIMICA showed that with the same amount of aerosol particles in the air, changes in the size distributions lead to significant modifications of fog microphysical properties. This work will contribute to constrain the role of aerosol parameters on fog properties and facilitate model improvements.

Financial support from the European Union’s Horizon 2020 research and innovation program (project FORCeS No 821205 and H2020-INFRAIA-2020-1 under grant agreement No 101008004) and the European Research Council (Consolidator grant INTEGRATE No 865799) is gratefully acknowledged.

How to cite: Neuberger, A., Ranjan, R., Ding, H., Decesari, S., Eckhardt, S., Ekman, A. M. L., Evangeliou, N., Haberstock, L., Mattsson, F., Mohr, C., Paglione, M., Riipinen, I., Rinaldi, M., and Zieger, P.: The influence of aerosol particles on fog microphysics during the Fog and Aerosol InteRAction Research Italy (FAIRARI) campaign 2021/22 , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11460, https://doi.org/10.5194/egusphere-egu25-11460, 2025.

EGU25-12141 | ECS | Orals | AS2.2

A new instrument to study fog and clouds: Insights from laboratory characterization and field deployment of the Ground-Based Fog and Aerosol Spectrometer (GFAS 

Lea Haberstock, Almuth Neuberger, Darrel Baumgardner, Dagen Hughes, Ilona Riipinen, and Paul Zieger

Clouds and their interaction with aerosol particles remain one of the largest sources of uncertainty for quantitatively describing the climate system, primarily due to the challenges in accurately representing their microphysical properties. These properties determine, for example, how a cloud interacts with short and longwave radiation or determine its lifetime, and thus, influence the local energy budget. However, microphysical properties of clouds are highly variable in space and time and are difficult to measure with high precision.

The Ground-Based Fog and Aerosol Spectrometer (GFAS, Droplet Measurement Technologies, USA) is a newly developed instrument, designed to characterize microphysical properties of clouds and aerosol particles via forward and backward light scattering. Operating in the diameter size range of 0.4 – 40 µm, the GFAS builds on the capabilities of the Fog Monitor (Droplet Measurement Technologies, USA) but is extended by  backscattered light intensity and changes in the polarization of the backscattered light as measured variables. These new parameters provide information on the particle’s shape and refractive index, enabling differentiation between solid and liquid particles, such as snow crystals, dust, and droplets, while minimizing biases in particle sizing caused by a change in refractive index. Furthermore, the GFAS automatically aligns with the main wind direction to minimize sampling losses.

Laboratory tests have validated the GFAS’ ability to characterize various particle types. Nebulized droplets and solid materials, like dust and ash, were analysed, revealing distinct polarization signatures between solids and liquids at an optical diameter > 10 µm. The backscattering ratio was used to further refine size distributions by investigating particle phase functions.

Field deployment of the GFAS during the ARTofMELT 2023 expedition in the Arctic under extreme environmental conditions provided first valuable insights into the role of low-level clouds and fog during the onset of sea ice melt. Over six weeks, the GFAS captured 46 hours of in-cloud data, showing strong agreement with the Fog Monitor data. These results confirm the GFAS as a new and powerful tool for advancing cloud microphysical measurements, reducing uncertainties in particle characterization, and improving our understanding of cloud-climate interactions.

How to cite: Haberstock, L., Neuberger, A., Baumgardner, D., Hughes, D., Riipinen, I., and Zieger, P.: A new instrument to study fog and clouds: Insights from laboratory characterization and field deployment of the Ground-Based Fog and Aerosol Spectrometer (GFAS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12141, https://doi.org/10.5194/egusphere-egu25-12141, 2025.

EGU25-12492 | ECS | Posters on site | AS2.2

Integrating Ground-Based and Satellite Observations to Map Fog in the Namib Desert 

Deepanshu Malik, Hendrik Andersen, and Jan Cermak

In this study, ground-based remote sensing and in-situ measurements are combined to characterize and estimate cloud base height (CBH) development patterns of fog and low clouds (FLC). The estimated CBH is further integrated with satellite data to map fog in the Namib Desert for the first time.

The Namib Desert, characterized by its hyper-arid conditions and frequent coverage with fog or low level stratus clouds, presents an intriguing environment for the study of low-level clouds and their vertical geometry. Understanding cloud base height (CBH) dynamics in this region is crucial for improving fog detection, particularly in distinguishing fog from low clouds in satellite data. This research aims to close existing knowledge gaps by providing, for the first time, a way to spatially map fog and separating it from other low stratiform clouds by merging ground and space-based observations.

Using ground-based remote sensing, this study reveals distinct and contrasting cloud base height (CBH) seasonality between inland and coastal locations. During the diurnal fog life cycle, stratus lowering and lifting is commonly observed during the formation and dissipation phases of the fog. A robust methodology for estimating CBH through in-situ meteorological observations. Moreover, the integration of CBH estimates with satellite products facilitates spatial mapping of fog, separating it from other low clouds. In the future, this can improve the ability to estimate fog-related water and nutrient input for this unique ecosystem.

How to cite: Malik, D., Andersen, H., and Cermak, J.: Integrating Ground-Based and Satellite Observations to Map Fog in the Namib Desert, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12492, https://doi.org/10.5194/egusphere-egu25-12492, 2025.

EGU25-12588 | ECS | Orals | AS2.2

The importance of aerosol and cloud microphysics on the properties and lifecycle of wintertime radiation fog in Po Valley 

Hao Ding, Almuth Neuberger, Rahul Ranjan, Liine Heikkinen, Karam Mansour, Stefano Decesari, Ilona Riipinen, Paul Zieger, and Annica M. L. Ekman

Similar to other types of clouds, the properties and evolution of fog are potentially sensitive to the interaction withaerosols. Assuming constant liquid water content, an increase in the aerosol concentration leads to water vapor competition, resulting in smaller droplet sizes and higher cloud droplet number concentrations. These changes can further influence the microphysical processes of fog, such as droplet sedimentation and aerosol regeneration (aerosol release upon droplet evaporation). However, substantial uncertainties in the representation of these processes pose challenges for accurately simulating fog evolution and for investigating the impact of aerosols on fog characteristics in climate models.

This study employs the large-eddy model MISU-MIT Cloud and Aerosol (MIMICA) to conduct case studies on wintertime radiation fog in the Po Valley, Italy. Observational data from the Fog and Aerosol InteRAction Research Italy (FAIRARI) campaign during the winter of 2021/22 were used as model input and simulation evaluation. Improvements of the parameterisation schemes in MIMICA were implemented, including surface forcing, warm air advection, droplet sedimentation, and aerosol hygroscopic growth. A series of one-at-a-time sensitivity experiments were performed based on the reference case.

Preliminary results indicate that the lifecycle and microphysical properties of wintertime radiation fog (e.g., droplet concentration, droplet size, and liquid water content) are sensitive to the representation of aerosol size distribution. Furthermore, an accurate description of microphysical processes is critical for capturing fog characteristics. For instance, neglecting droplet sedimentation can lead to a significant overestimation (by approximately an order of magnitude) of fog liquid water; the fog layer structure shows a significant response to different predefined parameters of droplet size distribution; aerosol hygroscopic growth plays a pivotal role in reproducing the water vapor budget and fog liquid water. We also find that an accurate representation of the meteorological conditions, such as surface temperature and humidity variations, is key for capturing the timing of fog onset and dissipation.

Financial support from the European Union’s Horizon 2020 research and innovation program (project FORCeS No 821205) and the Swedish Research council (No 2020-04158) is gratefully acknowledged.

How to cite: Ding, H., Neuberger, A., Ranjan, R., Heikkinen, L., Mansour, K., Decesari, S., Riipinen, I., Zieger, P., and M. L. Ekman, A.: The importance of aerosol and cloud microphysics on the properties and lifecycle of wintertime radiation fog in Po Valley, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12588, https://doi.org/10.5194/egusphere-egu25-12588, 2025.

EGU25-12868 | ECS | Orals | AS2.2

A twelve-year living lab for the experimentation and implementation of fog collection in the Valles Crucenos Region, Bolivia 

Giulio Castelli, Gorka Cubero, Teresa López de Armentia, Pablo Eugenio Osses Mc Intyre, Eleonora Forzini, Limber Cruz Montano, Fabio Salbitano, and Elena Bresci

The region of “Valles Cruceños”, Bolivia, is characterized by intrinsic water scarcity and increasing pressure for food production. In the area, located between the Andean altiplano and the Bolivian lowlands, orographic fog is a phenomenon occurring all year round and represents a sustainable water source to improve farmers’ resilience to dry spells and to promote food security and sovereignty. Here, the NGOs ICO and Zabalketa, and the University of Florence realized the first-ever experience of fog collection in Bolivia, in a structured set of activities, started in 2012 with a pilot project. After that, in 2018, the first scientific study on the potential of fog collection in the area was carried out in 10 locations, with a 1-year experimental analysis made through 1-m2 fog collectors, resulting in a yearly average of 6.01 l/m2/d observed in the best location. Based on these results, a large-scale fog collection system was implemented through international funding with innovative CloudFisher collection meshes starting in 2022, with a total of over 330 m2 of mesh over 4 locations, for multiple water uses (domestic, irrigation, reforestation). In the present contribution, we documented the whole implementation process from 2012, presenting the results of fog collection rates of the new system from 2022 up to the present, including also lessons learned and the main potential development for the area's future.

 

References: 

Castelli, G., et al. (2023). Fog as unconventional water resource: Mapping fog occurrence and fog collection potential for food security in Southern Bolivia. Journal of Arid Environments, 208, 104884. https://doi.org/10.1016/j.jaridenv.2022.104884

Zabalketa (2023). FOG WATER COLLECTION IN BOLIVIA. Experiences with Different Designs, Results and Practical Findings: https://zabalketa.org/archivos/publicaciones/FOG-WATER-BOLIVIA_eng.pdf 

How to cite: Castelli, G., Cubero, G., López de Armentia, T., Osses Mc Intyre, P. E., Forzini, E., Montano, L. C., Salbitano, F., and Bresci, E.: A twelve-year living lab for the experimentation and implementation of fog collection in the Valles Crucenos Region, Bolivia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12868, https://doi.org/10.5194/egusphere-egu25-12868, 2025.

EGU25-13561 | Posters on site | AS2.2

Characterization and forecast of a unique fog and low-level clouds event: microphysics measurements, mesoscale modeling and machine learning 

Dorita Rostkier-Edelstein, Anton Gelman, Pavel Kunin, Elizur Berkovitch, Rong-Shyang Sheu, Tamir Tzadok, Ayala Ronen, and Eyal Agassi

We present a study of the microphysics, mesoscale and synoptic conditions of a rare radiation-fog and low-level clouds event (hereafter, FC event), and build numerical tools to forecast it. The FC event developed in the south-eastern Mediterranean region during January 3-6, 2021. The FC formed during nighttime from south to coastal areas and dissipated at morning hours leaving low-clouds only. The synoptic conditions were dominated by Red Sea Troughs at the surface without cyclonic upper air circulation, suitable for radiation fog development. The following methods were combined to analyze the event and to evaluate the feasibility of accurately numerical forecasting it: 1. in-situ measurements consisting of Forward Scattering Spectrometer Probe FSSP-100, surface meteorological stations and radiosoundings, 2. satellite-retrieved IR and visible imagery [by the Spinning Enhanced Visible and InfraRed Imager (SEVIRI) instrument (https://www.eumetsat.int/seviri) on-board of Meteosat Second Generation (MSG) satellites], 3. high resolution (1-km grid size) Weather Research and Forecast model (WRF) with Real-Time Four-Dimensional Data Assimilation (RTFDDA) model forecasts, 4. post-processing of the model forecasts with simple and machine learning (ML) algorithms. The micro-physical analysis involved measurements of droplet size distribution and visibility range, allowing the calculation of liquid-water content and effective diameter of droplets. The measured visibility range was 90 m. The droplet diameter main mode was 1-2 micrometers, followed by another one around 6 micrometers. Typical liquid-water content values were 0.01-0.025 g/m3. These measurements were in agreement with the classification of the satellite imagery as “small drops fog/low-clouds”. FC forecasting by numerical-weather-prediction models is still challenging, as microphysics parameterizations are too crude. Therefore, we developed two post-processing algorithms based on basic model-forecast variables: wind speed, dew-point temperature and relative humidity at 1000 and 975 hPa vertical levels. The first post-processing algorithm identified FC based on a combination of thresholds of the aforementioned model variables (“Thresholds Algorithm”, TA). It was verified against satellite imagery and independent in-situ observations. The second is a Gradient Boosted Tree (GBT) ML post-processing algorithm in which the aforementioned model variables served as features and satellite imagery as label in the training process. Verification of the GBT algorithm was performed by cross-validation against satellite imagery and against independent in-situ observations, too. Both, the TA and GBT algorithms proved useful to identify FC areas. The GBT algorithm over-performed the TA algorithm during early morning hours, though it overestimates FC areas during the late morning. The combination of the GBT algorithm and TA is able to remove this inaccuracy providing an optimal strategy to post-process model forecasts. While the satellite imagery cannot distinguish between surface fog and low-level clouds, the post-processed model, does show differences between the two analyzed vertical levels, providing the possibility of determining the vertical extent and level of the phenomenon whether fog or low-level clouds.

How to cite: Rostkier-Edelstein, D., Gelman, A., Kunin, P., Berkovitch, E., Sheu, R.-S., Tzadok, T., Ronen, A., and Agassi, E.: Characterization and forecast of a unique fog and low-level clouds event: microphysics measurements, mesoscale modeling and machine learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13561, https://doi.org/10.5194/egusphere-egu25-13561, 2025.

EGU25-14315 | ECS | Posters on site | AS2.2

Contributions of Non-rainfall water inputs to soil surface moisture in arid coastal ecosystems: A case study in Pan de Azúcar National Park (25°59' S and 70°36' O), Atacama Desert, Chile. 

Diego Rivera, Constanza Vargas, Liesbeth Van Den Brink, Fernando D. Alfaro, and Camilo del Río

In the coastal areas of the Atacama Desert, non-rainfall water inputs (NRWI), including fog, dew, and direct vapor adsorption, sustain life in an environment where rainfall is virtually absent. These water sources provide critical moisture to the soil surface, fostering conditions for ecosystems to survive and adapt to extreme water scarcity. However, while the physical processes behind NRWI are better understood, the dynamics of each vector's events and their contributions to soil moisture remain poorly quantified.

Specifically, this research aims to characterize the dynamics of fog, dew, and direct vapor adsorption events and their contributions to soil surface moisture. A high-resolution experimental setup monitored the conditions facilitating NRWI formation—air temperature, relative humidity, surface temperature, and water vapor gradients between the air and soil pores—alongside soil surface moisture fluctuations. Our experimental design integrated a meteorological station, an infrared surface thermometer, a standard fog collector, a flat dew condenser, sensors for soil temperature, relative humidity (RH), volumetric water content (VWC), and a ground-based fog observation camera. These instruments enabled the analysis of individual NRWI vectors to investigate the timing, magnitude, and duration of events in relation to soil moisture changes.

A case study was conducted in the Las Lomitas oasis of Pan de Azúcar National Park (25°59' S, 70°36' W), situated at 731 m a.s.l. and 1.7 km from the coastline. Directly influenced by the marine boundary layer, this site provided an ideal setting to observe NRWI dynamics. Preliminary data collected between October 21 and December 5, 2024, revealed that direct vapor adsorption was the most frequently observed NRWI contributor, driving daily variations of 1–3% in VWC. Dew formation conditions were observed during 28% of the study period, primarily driven by high relative humidity (averaging 96.4%). However, dew events were short and intermittent, averaging 15 minutes, limiting their contribution to soil moisture when analyzed at the scale of individual events.

In contrast, 217 fog events were recorded, with an average duration of 3 hours and a water yield of 1.88 L/m² per event. Interestingly, only 5% of these fog events were associated with significant increases in soil moisture, with VWC rising by more than 1%. The largest fog event lasted 66.83 hours, yielding 83.58 L/m² and resulting in a 14.5% increase in VWC, the highest recorded moisture increase during the study.

The analysis shows the need to characterize and classify fog and dew events to identify strong correlations and demonstrate their impact on soil moisture. In the case of direct water vapor adsorption, it provided the most frequent moisture inputs, although in small magnitudes, that rarely contributed significantly on a daily basis. This research improves our understanding of the dynamics of NRWI events and their influence on soil surface moisture in arid environments. The findings reveal subtle mechanisms supporting coastal ecosystems and highlight their relevance for conservation and adaptation strategies in the face of climate change.

How to cite: Rivera, D., Vargas, C., Van Den Brink, L., Alfaro, F. D., and del Río, C.: Contributions of Non-rainfall water inputs to soil surface moisture in arid coastal ecosystems: A case study in Pan de Azúcar National Park (25°59' S and 70°36' O), Atacama Desert, Chile., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14315, https://doi.org/10.5194/egusphere-egu25-14315, 2025.

EGU25-15078 | ECS | Posters on site | AS2.2

From Haze to Fog: Investigating Aerosol-Fog Interactions and Source Shifts in Wintertime Delhi 

Akash S. Vispute, Narendra Gokul Dhangar, Suresh W. Gosavi, Prasanna Lonkar, Sandeep Wagh, Gaurav R. Govardhan, and Sachin D. Ghude

Severe wintertime air pollution episodes in Delhi, India, often coincide with fog events, amplifying their environmental and health impacts. This study investigates the complicated interactions between aerosols and fog during the winter season of 2023-2024, leveraging high-resolution, time-resolved measurements of non-refractory PM1 (NR-PM1) using High-Resolution Time-of-Flight Aerosol Mass Spectrometry (HR-TOF-AMS). The study highlights the temporal variability of NR-PM1 chemical composition and its transformation during fog events, focusing on processes influencing aerosol acidity, hygroscopicity, and secondary formation.

NR-PM1 mass concentrations varied widely, with organics (OA) constituting the dominant fraction (~65%), followed by nitrate, sulfate, ammonium, and chloride. Ammonium acted as the primary neutralizing agent, with an average aerosol neutralization ratio (ANR) of 0.95 ± 0.12, indicating near-neutral aerosol conditions. Significant shifts in OA composition were observed between fog and non-fog periods, with fog events promoting enhanced oxidation of organic aerosols. Elemental analysis revealed changes in the OA oxidation state. The oxygen-to-carbon (O/C) ratio increased for LV-OOA (from 0.914 to 1.016) and SV-OOA (from 0.920 to 0.838) during fog, indicating enhanced oxidation within fog droplets. The carbon oxidation state (OSc) also increased for these factors during fog, further confirming this observation.

The Positive Matrix Factorization (PMF) method identified six primary OA factors: Hydrocarbon-like OA (HOA), Nitrogen-rich Hydrocarbon OA (NHOA), Biomass Burning OA (BBOA), Solid Fuel OA (SFOA), Low-Volatile Oxygenated OA (LV-OOA), and Semi-volatile Oxygenated OA (SV-OOA). Fog events led to a ~34% increase in LV-OOA, while SV-OOA decreased correspondingly, suggesting a shift towards more oxidized, low-volatility species,  reflects the significant role of fog in promoting secondary organic aerosol (SOA) formation through heterogeneous and aqueous-phase reactions.

The findings emphasize the dual role of fog as both a sink and a facilitator of aerosol transformation, with implications for regional air quality and visibility. This study provides crucial insights into aerosol evolution mechanisms during fog events, emphasizing the need for integrated observational and modeling approaches to mitigate wintertime pollution episodes in megacities like Delhi.

How to cite: Vispute, A. S., Dhangar, N. G., Gosavi, S. W., Lonkar, P., Wagh, S., Govardhan, G. R., and Ghude, S. D.: From Haze to Fog: Investigating Aerosol-Fog Interactions and Source Shifts in Wintertime Delhi, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15078, https://doi.org/10.5194/egusphere-egu25-15078, 2025.

EGU25-15225 | ECS | Posters on site | AS2.2

Contrasting Fog Dynamics between Urban and Rural Environments: Insights from Winter Observations over Delhi and Jewar 

Anoop Pakkattil, Avinash N. Parde, Narendra G Dhangar, Sandeep Wagh, Prasanna Lonkar, Sumit Kumar, and Sachin D. Ghude

Widespread fog is a critical weather phenomenon over the Indo-Gangetic Plain (IGP) during winter, significantly impacting transportation safety and air quality. This study investigates the contrasting mechanisms of fog formation and dissipation over an urban site (Delhi) and a rural site (Jewar, ~80 km aerial distance) using extensive ground-based observations collected during the Winter Fog Experiment (WiFEX) field campaign from December 2023 to February 2024.

Analysis of WiFEX observations at Indira Gandhi International (IGI) Airport, Delhi, and Jewar Airport identified 15 dense fog events in Delhi and 25 in Jewar. The study highlights the influence of urbanization on fog dynamics, driven by a pronounced Urban Heat Island (UHI) effect in Delhi. This urban influence results in delayed fog formation and earlier dissipation compared to Jewar. The earlier onset and prolonged persistence of fog in Jewar are linked to stronger nocturnal cooling, greater moisture availability, and minimal urban heat retention. Jewar experienced a higher frequency of radiation fog events compared to Delhi, with visibility below a few meters persisting for several hours longer. Statistical analysis revealed distinct meteorological differences between the sites: nighttime surface temperatures were consistently lower in Jewar, while relative humidity peaked higher compared to Delhi. The extended fog duration in Jewar is attributed to sustained near-surface temperature inversion and weaker boundary layer mixing, in contrast to the urban environment.

These findings underscore the critical role of urbanization in modulating fog characteristics and highlight the importance of site-specific mitigation strategies for fog forecasting and management. This research advances ongoing WiFEX efforts to enhance fog prediction capabilities across the IGP, providing valuable insights for improving regional weather forecasting and mitigating societal impacts.

How to cite: Pakkattil, A., Parde, A. N., Dhangar, N. G., Wagh, S., Lonkar, P., Kumar, S., and Ghude, S. D.: Contrasting Fog Dynamics between Urban and Rural Environments: Insights from Winter Observations over Delhi and Jewar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15225, https://doi.org/10.5194/egusphere-egu25-15225, 2025.

EGU25-15592 | Orals | AS2.2 | Highlight

Air pollution reduction and climate change drive long-term trends of fog liquid water content in the Po Valley 

Stefano Decesari, Karam Mansour, Matteo Rinaldi, Marco Paglione, Almuth Neuberger, Paul Zieger, Jorma Joutsensaari, Sami Romakkaniemi, and Sandro Fuzzi

Radiation fogs characterize the wintertime climate of many mid-latitude environments, especially in orographic depressions, and exert a profound impact on visibility, surface temperatures and soil-air water vapor fluxes. Trend analysis of fog occurrence based on visibility data supports the potential impact of air pollution decline on reduced fog frequency in several areas of the world, net of the effects of climate warming (van Oldenborgh et al., 2010; Gray et al., 2019). Microphysical models indicate that aerosol-fog interactions manifest on a range of fog physical properties for which, however, we miss relevant observations over decadal time scales. Here, we present a 30-year long timeline of radiation fog liquid water content (LWC) from the Po Valley, Italy, and analyse long-term trends, concomitantly with the trends in potential meteorological and atmospheric composition drivers. In particular, we reconstructed the entire time series of cloud condensation nuclei (CCN) concentrations using a machine learning approach trained on an extended (ca. 15-year long) observation record of differential mobility particle sizer (DMPS) measurements available from the same site (Leinonen et al., 2022). Our results show a consistent decrease of fog LWC in the 90s’ and early 2000’s at a time when aerosols and CCN concentrations underwent a steep decline. By contrast, in the last ten years, aerosol concentrations stabilized while fog LWC has recovered, probably because of an increased daily temperature excursion as a feature of current climate change in the Po Valley. Although the time evolution of Po Valley fog microphysics could not be followed over the three decades, the comparison of the detailed observations performed during recent intensive field campaigns in 2021 and 2022 (Neuberger et al., 2025) with those carried out in the early studies of 1989 and 1994 with state-of-the-art instrumentation (Fuzzi et al, 1992; Wendisch et al., 1998) support the hypothesized effects of CCN on fog LWC be mediated by changes in fog droplet concentration, size distribution and deposition rates. This research provides new insights on the effects of anthropogenic activities on fog occurrence and characteristics, as well as on the mechanisms of aerosol-cloud interactions in regime of high CCN and low supersaturations.

This work was funded by the EU Horizon 2020 project FORCeS (grant no. 821205) and the Horizon Europe project CleanCloud (Grant No. 101137639).

References

Fuzzi et al., The Po Valley fog experiment 1989, Tellus, 44B, 448–468, 1992.

Gray et al., J. Geophys. Res., 124, 10.1029/2018JD029419, 2019.

Leinonen et al., Comparison of particle number size distribution trends in ground measurements and climate models, Atmos. Chem. Phys., 22., 10.5194/acp-22-12873-2022, 2022.

Neuberger et al. From Molecules to Droplets: The Fog and Aerosol Interaction Research Italy (FAIRARI) 2021/22 Campaign. Bull. Amer. Meteor. Soc., 106, E23–E50, https://doi.org/10.1175/BAMS-D-23-0166.1, 2025.

van Oldenborgh et al., On the roles of circulation and aerosols in the decline of mist and dense fog in Europe over the last 30 years, Atmos. Chem. Phys., 10, 10.5194/acp-10-4597-2010, 2010.

Wendisch et al., Drop size distribution and LWC in Po Valley fog, Contrib. Atmos. Phys., 71, 87–100, 1998.

How to cite: Decesari, S., Mansour, K., Rinaldi, M., Paglione, M., Neuberger, A., Zieger, P., Joutsensaari, J., Romakkaniemi, S., and Fuzzi, S.: Air pollution reduction and climate change drive long-term trends of fog liquid water content in the Po Valley, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15592, https://doi.org/10.5194/egusphere-egu25-15592, 2025.

EGU25-16701 | ECS | Posters on site | AS2.2

Spatiotemporal variability of fog and dew occurrence in the Atacama Desert - a view from a network of weather stations  

Christoph Böhm, Jan Schween, Simon Matthias May, and Susanne Crewell

In hyperarid regions, such as the Atacama Desert, fog and dew provide essential water supply to sustain unique ecosystems and drive geomorphological processes. While some studies have quantified the spatiotemporal variability of fog, it remains mostly unclear which phenomenon, i.e. fog or dew, constitutes the more important water source. However, such knowledge is crucial for a better understanding of the interplay between atmospheric, biological and geological processes. In this study, we determine fog and dew occurrence from observations provided by a network of weather stations deployed in the Atacama Desert by the Collaborative Research Center "Earth – Evolution at the Dry Limit" (https://sfb1211.uni-koeln.de/) of the German Science Foundation (DFG SFB1211). The stations are aligned in three west-to-east transects covering the coastal region, the central depression and the Andean foothills, thus, including multiple altitudinal regimes which are affected differently by the marine moisture from the nearby Southeast Pacific. Fog, dew and dry situations are distinguished according to data from a leaf wetness sensor and incoming terrestrial irradiation together with some additional constraints. Terrestrial irradiation is only available for three master stations. To obtain it for all other stations, we trained a multilayer perceptron with relative humidity, incoming solar radiation, 2m and surface temperature together with some auxiliary data as input data. For validation, the final classifications are compared to camera images available for morning and evening hours which constitute the most challenging times when fog and dew dissipate or form. Spatiotemporal variability, including diurnal and seasonal cycles of fog and dew are investigated. Furthermore, the relationship between the derived fog and dew frequencies and soil moisture variability is assessed to provide a more quantitative assessment of the moisture supply. The derived classification can be used as ground truth to build and evaluate satellite-based fog and dew retrievals in future studies.

How to cite: Böhm, C., Schween, J., May, S. M., and Crewell, S.: Spatiotemporal variability of fog and dew occurrence in the Atacama Desert - a view from a network of weather stations , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16701, https://doi.org/10.5194/egusphere-egu25-16701, 2025.

EGU25-17107 | ECS | Posters on site | AS2.2

Satellite observations reveal higher persistence of fog in polluted conditions in the Po valley, Italy 

Eva Pauli, Jan Cermak, Jörg Bendix, and Philip Stier

Fog and low stratus clouds (FLS) form as a result of complex interactions of atmospheric and land surface drivers and their analysis helps to improve traffic safety, solar power planning and to better understand inversion-topped boundary layer clouds in its interaction with the air quality of larger basin areas. A major factor impacting FLS occurrence and life cycle is aerosol loading, but its impact is challenging to disentangle from confounding meteorological factors and measuring both FLS occurrence and aerosol loading simultaneously is challenging.

Here we use satellite observations of FLS persistence, ERA5 reanalysis data and aerosol robotic network (AERONET) observations to disentangle the effect of meteorology and aerosol loading on FLS persistence in the Po valley in northern Italy, one of the most polluted regions in central Europe. After selecting 430 FLS events in the winter (DJF) months from 2006-2015 using a regional FLS occurrence threshold, we apply k‐means clustering to latitudinal transects of relative humidity from 550-1000hPa to identify FLS events with similar FLS formation pathways. Analyzing the average synoptic conditions for the two clusters identified shows that FLS formation in the Po valley is either based on radiative processes or moisture advection from the Mediterranean sea. Radiatively formed FLS events are more persistent, likely due to a stable boundary layer combined with a temperature inversion, whereas advective FLS events form under more dynamic conditions and are on average 2-3 hours shorter. Analysis of AERONET observations at three locations reveals that FLS persistence is significantly higher under high aerosol loading, particularly for radiatively formed FLS events. Aerosol loading further shows a clear increasing trend ahead of persistent FLS events, suggesting an accumulation of pollutants and a subsequent increase in cloud condensation nuclei prolonging FLS events through aerosol-cloud interactions. 

Our results show the combined effect of meteorology, aerosol loading and geographic conditions on FLS persistence in the Po valley and underline the need for further observational studies on the effect of aerosols on the FLS life cycle over different geographic and synoptic backgrounds.

How to cite: Pauli, E., Cermak, J., Bendix, J., and Stier, P.: Satellite observations reveal higher persistence of fog in polluted conditions in the Po valley, Italy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17107, https://doi.org/10.5194/egusphere-egu25-17107, 2025.

EGU25-17344 | ECS | Orals | AS2.2

Implementation of the parameterized and spectral fog models(PAFOG, MIFOG) for simulating fog at the Ioannina mountainouscity (Greece) 

Stefanos Nasikas, Nikolaos Hatzianastassiou, Marios-Bruno Korras-Carraca, and Andreas Bott

Fog and low-level clouds, namely stratus, are of major concern mainly due to their
adverse effects on transportation. Visibility is drastically reduced under the
occurrence of fog conditions, thus affecting aviation and road traffic. For example,
fog causes many troubles to scheduled flights, like cancelations or delays, while
creating dangerous driving conditions, thus having significant socioeconomic impacts.
Moreover, apart from affecting transportation, fog and low-level clouds also affect the
radiation budget, specifically at the Earth’s surface. For all these reasons, the
simulation and forecasting of fog is important, especially when no observational tools,
e.g. radars, are available.
Ioannina is a middle-sized city (~120,000 inhabitants) situated in the Epirus
mountainous region in Northwestern Greece. The city is located on a plateau (basin)
with an average altitude of 500 m, surrounded by high mountains with altitudes higher
than 1500m. The airport of Ioannina lies in an area of the plateau which experiences a
high yearly number of fog events. This is mainly due to: (1) the presence of the
nearby Pamvotis lake (area 23 km 2 , average depth 4 m, maximum depth 10 m), which
locally enriches the overlying air masses with water vapour and (2) the specific
geographical and topographical characteristics of the area, which generally favour
calm (low wind speed) conditions speed and high relative humidity levels, as well as
the creation of temperature inversions. Moreover, due to the local topography and
meteorological conditions, the city frequently suffers from wintertime air pollution
episodes (smog) due to extensive biomass burning for domestic heating activities.
Despite the frequent occurrence of fog and the induced air traffic problems, there are
not available tools for forecasting fog locally. The present work aims to fill this gap
by implementing a numerical model, specifically the parameterized fog model
PAFOG along with the spectral cloud microphysics model MIFOG. The two models
will be operated and evaluated as to their ability to simulate fog under different
conditions.
The fog models will be initialized with available data from local meteorological
stations supplemented by vertically resolved reanalysis and satellite data, due to the
lack of radiosondes in the study area. Local information on aerosol particles, acting as
CCN, will be implemented as well, enabling to investigate their role for the formation
of fog. The performance of the two models will be assessed through comparisons to
available METARs from the Ioannina airport. This study is a first step towards
implementing fog models for a routine fog forecasting at the city/airport.

How to cite: Nasikas, S., Hatzianastassiou, N., Korras-Carraca, M.-B., and Bott, A.: Implementation of the parameterized and spectral fog models(PAFOG, MIFOG) for simulating fog at the Ioannina mountainouscity (Greece), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17344, https://doi.org/10.5194/egusphere-egu25-17344, 2025.

EGU25-19827 | ECS | Posters on site | AS2.2

Classification of Fog Life Cycle Phases Using Ground-based and Satellite-based Observations 

Maria Laura Pinilla, Eva Pauli, Jan Cermak, and Johannes Antenor Senn

A complete understanding of the fog life cycle — defined as formation, maturity, and dissipation phases — provides a basis for better predictions of fog formation and dissipation. While satellites can observe fog and low stratus (FLS) over a large spatial extent, ground-based instruments provide more detailed vertical and temporal information about fog at specific locations. 
In this study, we classify the life cycle phases of radiation fog events in autumn 2009-2015 at a ground station in Southwest Germany by combining geostationary satellite observations with ceilometer and in-situ measurements. For this, we develop a life cycle phase classification algorithm that automatically detects the start and end times of each phase based on visibility trends and thresholds. Unlike other methodologies, we define fog events not only through a visibility threshold of 1000 m but also by the processes involved during fog formation and dissipation. These processes are identified through changes in visibility trends and values and validated against backscatter patterns. Furthermore, we demonstrate that ground-based visibility effectively detects radiation fog phases, while its combination with ceilometer data has the potential to detect the life cycle phases of cloud base lowering fog events. Thus, combining these data sources is essential for effectively detecting the life cycle phases of different fog types. Additionally, we find that ground-based data performs better in phase detection at individual locations compared to a satellite-based FLS life cycle dataset. Consequently, we propose that future satellite-based FLS detection methods incorporate an assessment of the changes in the spectral signals of FLS throughout its life cycle for a more detailed phase characterization over large regions.

How to cite: Pinilla, M. L., Pauli, E., Cermak, J., and Senn, J. A.: Classification of Fog Life Cycle Phases Using Ground-based and Satellite-based Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19827, https://doi.org/10.5194/egusphere-egu25-19827, 2025.

EGU25-19911 | Orals | AS2.2

Statistical analysis of the influence of local and synoptic processes on radiation and stratus lowering fogs at SIRTA Observatory, Paris 

Cheikh Dione, Jean-Charles Dupont, Martial Haeffelin, and Jean-François Ribaud

Based on an instrumental synergy of in-situ and remote sensing measurements collected at SIRTA observatory, a peri-urban site located near Paris, and a fog conceptual model (CM), this study presents a statistical analyses of the local and synoptic processes driving the different phases (formation, evolution and dissipation) of radiation fogs (RADs) and stratus lowering fogs (STLs). The very high resolution of the co-localised BASTA cloud Radar, Ceilometer and visibilimeter, allows to estimate the occurrence of fog during the 2013-2023 period. A microwave radiometer (MWR Hatpro) and the equivalent adiabaticity by closure from the CM are used to estimate the lowest layer atmospheric stability. 191 fogs (82 RADs and 99 STLs) are well documented and divided into several categories depending on their geometry (radiation fogs), their type of dissipation (lifting or lowering cloud base height), and their time of dissipation (nocturnal or diurnal).

By associating fog types with large-scale atmospheric circulations, the result show the role of synoptic regimes on the fog evolution at SIRTA. Longer RADs and STLs are associated with strong temperature inversions driven by the Atlantic Ridge and positive North Atlantic Oscillation (NAO+) regimes. These two regimes promote the advection of warm air to the West of Europe and contribute to the diurnal variability of temperatures in the region.

The analysis of the local processes driving the different phases of fogs is conducted using the turbulent kinetic energy (TKE), the sensible heat flux (SHF) and the fog reservoir of liquid water path (RLWP) estimated by a sonic anemometer and at 30 m a.g.l, the Licor analyzers at 2 m a.g.l, and the CM, respectively. For RAD fogs, mechanical turbulence is the factor favoring the vertical development of fog making it adiabatic. Therefore, fine and very fine RADs remain in their stable phase when the TKE is less than 0.2 m2 s-2. RADs begin their transition as soon as the TKE exceeds this threshold and remains less than 0.4 m2 s-2 and the RLWP > 0 g m-2. The dissipation of thick RADs is observed when the TKE exceeds 0.4 m2 s-2 and the RLWP < 0 g m-2. This strong turbulence can be of mechanical origin associated with an advection across the site or thermal with a diurnal increase in the SHF (50 W m-2). Less SHF (25 W m-2) is needed to dissipate very thin RADs. The amount of heat required for the diurnal dissipation of RADs is proportional to their geometric and microphysical characteristics. STLs persist for a stable TKE around 0.4 m2 s-2 and dissipate by elevation of the CBH when the SHF is low (25 W m-2). Their dissipation by evaporation needs more SHF (75 w m-2). The results indicates that the instrumental synergy and the metrics used in this study allows to produce an early warning tools for the nowcasting of RAD and STL formation, evolution and dissipation.

How to cite: Dione, C., Dupont, J.-C., Haeffelin, M., and Ribaud, J.-F.: Statistical analysis of the influence of local and synoptic processes on radiation and stratus lowering fogs at SIRTA Observatory, Paris, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19911, https://doi.org/10.5194/egusphere-egu25-19911, 2025.

EGU25-21131 | ECS | Orals | AS2.2

Cloud and Fog Monitoring Simplified: Preliminary Validation of the Dark Channel Model with Ceilometer Observations 

Yen-Jen Lai, Po-Hsiung Lin, Chih-Fan Hsu, and Yu-Lun Chang

The impacts of global warming and urban heat island effects have significantly altered atmospheric conditions, leading to a noticeable decline in fog events which uplift to be low clouds. Understanding and monitoring these changes over the long term are crucial for climate studies and environmental management. However, identifying a practical and reliable method for monitoring cloud base height and fog patterns remains a challenge.

This study explores the use of the dark channel model, a computational approach originally developed for haze removal in images, to analyze cloud and fog dynamics. By leveraging the model's ability to estimate cloud base height and distinguish upslope     fog from other atmospheric conditions, we provide a novel method for atmospheric monitoring. The model's performance was validated using observational data from a ceilometer, an instrument known for its precision in measuring cloud base heights. The comparison revealed a strong correlation between the model's predictions and ceilometer measurements, with a coefficient of determination (R²) of 0.85.

The results demonstrate that the dark channel model is an effective tool for long-term monitoring of cloud and fog dynamics, offering both accuracy and convenience. This approach could play a pivotal role in understanding atmospheric changes in the context of climate variability and urbanization, aiding in better management and forecasting of weather and environmental conditions.

How to cite: Lai, Y.-J., Lin, P.-H., Hsu, C.-F., and Chang, Y.-L.: Cloud and Fog Monitoring Simplified: Preliminary Validation of the Dark Channel Model with Ceilometer Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21131, https://doi.org/10.5194/egusphere-egu25-21131, 2025.

EGU25-1437 | Posters on site | AS2.3

Estimating Ground Heat Flux from Net Radiation 

Cheng-I Hsieh and Supattra Visessri

Ground heat flux may play an important role in surface energy balance. In this study we evaluate the performance of the objective hysteresis model (OHM) for estimating ground heat flux from net radiation and compare it with the linear regression model. The experimental sites include residential roofs (concrete), campus grassland, agricultural grassland, and peat bog. Our field measurements show that the mean partition coefficient from net radiation to ground heat flux varied from 0.47 (concrete roof) to 0.079 (agricultural grassland). The mean hysteresis (lag) factors for residential roof, campus grassland, and peat bog were 0.55, 0.26, and 0.11 h, respectively; and the hysteresis factor at the agricultural site was only 0.032 h. However, the partition and hysteresis coefficients in the OHM were found to vary with time for the same surface. Our measurements and analysis show that when the hysteresis factor is larger than 0.11 h, ground heat flux estimates from net radiation can be improved (17–37% reduction in the root mean square error) by using OHM instead of a simple linear regression model.

How to cite: Hsieh, C.-I. and Visessri, S.: Estimating Ground Heat Flux from Net Radiation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1437, https://doi.org/10.5194/egusphere-egu25-1437, 2025.

The Tibetan Plateau (TP) greatly affects climate and environment systems over Asian through the lower atmospheric mass/energy transfer processes. However, the lower atmospheric processes were not clearly understood due to the limitation of observational data, especially over the TP mountain regions. Observations and model simulations suggested a distinguished land-air transfer and vertical structure over the TP mountain regions, which largely differ from those over plateau flat regions. An inhomogeneous distributions are also found in the land-air exchange processes over the whole TP regions, and a new high-resolution dataset are consequently constructed and developed, under the consideration of different TP climate classification.

How to cite: Zhou, L.: Observational Studies on the Land-air Exchange Processes over the Tibetan Mountain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1539, https://doi.org/10.5194/egusphere-egu25-1539, 2025.

EGU25-1695 | Orals | AS2.3

Continuous measurements of O2:CO2 flux exchange ratios above a cropland in central Germany 

Christian Markwitz, Edgar Tunsch, Andrew Manning, Penelope Pickers, and Alexander Knohl

The O2:CO2 exchange ratio of land-atmosphere fluxes (ER) can be used to identify sources and sinks of CO2 in land ecosystems. During photosynthesis, the O2:CO2 ER at the leaf level is approximately -1 mol mol-1, reflecting the uptake of one mole of CO2 associated with the release of one mole of O2. However, the ER at the level of entire ecosystems is largely unknown.

Here we present a unique dataset of two years of continuous O2 and CO2 flux measurements at the agricultural FLUXNET site Reinshof (51°29'24.0"N, 9°55'55.2"E, DE-Rns) near Göttingen, Germany, in 2023 and 2024. Fluxes were calculated using flux-gradient approaches with air sampled from three inlets situated at 0.5, 1.0 and 3.0 m above ground. Dry mole fractions of O2 and CO2 were measured using a modified Oxzilla II differential oxygen analyzer (Sable Systems, USA) and a Li-820 CO2 infrared gas analyser (LiCor Biosciences, USA), respectively.

The results show that O2 and CO2 mole fractions and net O2 and CO2 fluxes were strongly anticorrelated. The O2:CO2 flux ER showed a distinct annual cycle, with values around -1.5 mol mol-1 under bare soil conditions and -1.1 mol mol-1 during the main growing season when sugar beet (2023) and winter wheat (2024) was grown, respectively. An influence from anthropogenic emissions was observed during the winter with stable atmospheric stratification, when winds originated from the city centre of Göttingen or the nearby road. The longer vegetation period of sugar beet in 2023 was well reflected by extended O2 release and CO2 uptake, as well as ERs at around -1.1 mol mol-1.

In conclusion, the O2:CO2 ER of a cropland showed considerable seasonal variability, which offers the opportunity to use O2 flux measurements as a tracer of the carbon cycle.

How to cite: Markwitz, C., Tunsch, E., Manning, A., Pickers, P., and Knohl, A.: Continuous measurements of O2:CO2 flux exchange ratios above a cropland in central Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1695, https://doi.org/10.5194/egusphere-egu25-1695, 2025.

EGU25-2935 | Posters on site | AS2.3

Ensemble machine learning for interpretable soil heat flux estimation 

Darren Drewry and James Cross

Soil heat flux (SHF) is a key component of the surface energy balance and a driver of soil physiochemical and biological processes. Despite its importance accurate estimation of soil heat flux is hindered due to variations in soil composition, overlying vegetation density and phenology, and highly variable environmental forcings. These factors have challenged the development of robust models of SHF, with modeling studies focused on mid-day conditions corresponding to satellite overpass times, missing the significant variability that occurs throughout diurnal periods across a growing season. Here we assess the performance of ensemble machine learning modeling for predicting soil heat flux at half-hourly resolution for multiple agro-ecosystems. Observations span a wide range of phenological and climatological variability over a complete growing season. We utilized the random forest machine learning (ML) approach to develop a wide range of models utilizing combinations of predictor variables that include widely-available meteorological conditions and proximal remote sensing observations of reflectance indices and land surface temperature (LST). The performance of the ML models developed here was compared to a set of six semi-empirical soil heat flux models developed around the use of remote sensing information. The random forest ML ensembles demonstrated a general ability to significantly outperform the six semi-empirical models in capturing diurnal variations across the growing season for each of the four crops examined here (soybean, corn, sorghum and miscanthus). We found ML models using the complete set of meteorological and remote sensing predictors captured over 90% of the variability in SHF across all crops. ML models using only LST and NDVI as predictors were able to capture over 82% of SHF variability across all crops. Shapley additive explanations (SHAP) methods were examined to allow for model interpretability, providing insights into the typically opaque ML modeling process. From a set of seven observation variables an exhaustive search was performed to identify predictor attributions for each of the four crops examined here. Models trained with fewer input variables tended to display more linear and interpretable feature attribution, suggestive of physical consistency. LST and air temperature were often the most crucial predictors when present due to high correlation with soil heat flux, with NDVI the next most crucial predictor due to its ability to quantify canopy density and phenological status. These results suggest that robust and accurate soil heat flux estimations can be made at high-temporal resolution purely through simple proximal remote sensing observations and widely available meteorological observations.

How to cite: Drewry, D. and Cross, J.: Ensemble machine learning for interpretable soil heat flux estimation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2935, https://doi.org/10.5194/egusphere-egu25-2935, 2025.

EGU25-3154 | ECS | Posters on site | AS2.3

Exploring Forest-Atmosphere Interactions Under Heat Extremes in a Semi-Arid Region  

Yotam Menachem, Leehi Magaritz-Ronen, Eyal Rotenberg, Lior Hochman, Shira Raveh-Rubin, and Dan Yakir

The potential effects of desert plantations, such as those used for climate change mitigation, during extreme heat waves remain an important and unresolved question. While the influence of large-scale surface heterogeneity, such as land-sea distribution and mountain ranges on weather, is well established and incorporated in operational numerical weather prediction models, the impact of smaller-scale heterogeneities remains uncertain. Specifically, the interplay between the synoptic forcing and the arising effects of mesoscale interactions is not yet fully understood.  

The Eastern Mediterranean and the Middle East face intensified heat and drought due to climate change, impacting regional weather and local ecosystems. Semi-arid forests, such as the Yatir pine forest on the edge of the Negev Desert, provide a unique lens through which to study land surface-atmosphere feedback, particularly under extreme heat events. 

Ongoing studies show that due to high incoming solar radiation and its low albedo, the Yatir Forest net radiation is higher than in any other eco-regions, balanced by a large sensible heat flux. Thus, the resulting cooler surface suppresses the emission of longwave radiation compared with the surrounding warmer shrubland. The thermal contrast between the forest and the surrounding shrubland can also result in the development of secondary circulations within the PBL. The combined effects of these processes significantly modify the surface-atmosphere energy exchange, can affect the forest microclimate, and, if extended to a larger scale, could potentially impact regional weather and climate.

This research investigates the interactions between the Yatir Forest and the atmosphere under dry heat extremes, focusing on mechanisms driving radiation dynamics, energy fluxes, and local circulations. Our approach combines in-situ measurements from the Yatir Forest, atmospheric reanalysis data, Lagrangian analysis, and high-resolution simulations using the ICON numerical weather prediction model. Through a series of numerical forest configuration experiments incorporating forest-atmosphere feedback, we examine the potential of semi-arid afforestation to influence boundary layer dynamics, exploring the implications for local and potentially regional moderation of extreme climatic events and sustainable land use. We incorporate the concept of the canopy convector effect for semi-arid regions to demonstrate the sensitivity of the numerical results to surface parameters and synoptic conditions causing heat waves.  

  • Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot, Israel (yotam.menachem@weizmann.ac.il)

How to cite: Menachem, Y., Magaritz-Ronen, L., Rotenberg, E., Hochman, L., Raveh-Rubin, S., and Yakir, D.: Exploring Forest-Atmosphere Interactions Under Heat Extremes in a Semi-Arid Region , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3154, https://doi.org/10.5194/egusphere-egu25-3154, 2025.

Open-path (OP) infrared gas analyzers (IRGA) are widely used for CO2 eddy covariance flux measurements in diverse ecosystems, including in arid desert environments. These high sensible heat and low CO2 flux conditions can lead to a systematic bias in the estimation of the carbon exchange. Numerous studies using both open- and closed-path IRGAs report large overestimates of CO2 uptake in the OP measurements, which persists for all seasons and is not driven by biological activity, but rather by instrumentation artefacts. Despite the attempts to address these biases, their origin and the appropriate correction approaches remain unresolved. Sensor-path heat exchange has been considered as a potential source of the bias. Consequently, later models OP gas analyzers have eliminated the self-heating effects, yet they still exhibit apparent CO2 uptake. In this study we consider the influence of ambient air temperature on the absorption in the CO2 spectral band typically used in non-dispersive broadband IRGAs as the source of the bias. We show the results from simulations of infrared transmission in the CO2 spectral band using high resolution molecular transmission (HITRAN) database.  We evaluated the temperature sensitivity of an IRGA by simulating integrated absorption spectra for a typical interference optical filter with a 100 nm passband where the CO2 density was kept constant, and the gas mixture temperature was varied between 244 and 385 K. The data show that if the absorption is not corrected for temperature of the air in the optical sensing path a bias is introduced. The bias causes underestimation of CO2 density at warmer temperatures and overestimation of CO2 density at low temperatures. We conclude that OP gas analyzer measurements need to be corrected for the effects of changes in air temperature in the sensing path. We demonstrate that the correction is not universal, but rather instrument specific and depends on the actual pass band of the specific interference filter used.

How to cite: Bogoev, I.: Addressing a sensible heat bias in open-path eddy covariance carbon dioxide flux measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4594, https://doi.org/10.5194/egusphere-egu25-4594, 2025.

EGU25-5075 | ECS | Posters on site | AS2.3

High-resolution monitoring of CO2/O2 transport in recharge wells 

Ehud Lavner, Avner Gross, and Elad Levintal

The Earth's surface forms a dynamic boundary characterized by continuous gas exchanges between the critical zone and the overlying atmosphere. As global concern grows over climate change driven by increasing levels of greenhouse gases – such as carbon dioxide (CO2) and methane (CH4) – abandoned oil, gas, and even groundwater wells can be significant sources of these emissions. Here, we monitor CO2 and oxygen (O2) and quantify the CO2 flux in two different recharge wells – one that extends below the groundwater level (wet well) and one that reaches into the unsaturated zone above the groundwater level (dry well). Novel monitoring systems that measure CO2, O2, temperature, and relative humidity were installed at the top and bottom of each well, enabling high-resolution, continuous data collection at 1-min time intervals. Using atmospheric measurements taken from a nearby meteorological station, we investigate the mechanisms that influence the air transport between the wells and the atmosphere. The high-resolution measurements indicate different air transport mechanisms between the two wells. In the wet well, there was stratification during the summer, with consistently high CO2 values ​​measured at the bottom of the well while low values ​​were measured at the top of the well. In the dry well, two daily outflow cycles were observed, with high CO2 concentrations and fluxes from the well to the atmosphere. These findings highlight the potential contribution of recharge wells to CO₂ emissions and the importance of understanding their transport mechanisms.

How to cite: Lavner, E., Gross, A., and Levintal, E.: High-resolution monitoring of CO2/O2 transport in recharge wells, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5075, https://doi.org/10.5194/egusphere-egu25-5075, 2025.

EGU25-6444 | Orals | AS2.3

Towards improved understanding on flow decoupling at eddy covariance sites with the aid of a universal coupling metric 

Olli Peltola, Toprak Aslan, Mika Aurela, Annalea Lohila, Ivan Mammarella, Dario Papale, Christoph K. Thomas, and Timo Vesala

Eddy covariance (EC) flux observations deviate from the fluxes at the ecosystem-atmosphere interface when the turbulent flow is decoupled from the surface. This problem severely limits the applicability of the EC technique to monitor ecosystem-atmosphere interactions including trace gas exchange. Despite some progress on understanding vertical coupling processes over the past years, the role and interplay of dynamic stability, canopy drag, and the strength of vertical turbulent mixing remains insufficiently understood. Furthermore, the commonly used metric to identify decoupling, friction velocity, does not represent these processes.

In this work we use the recently developed decoupling metric Omega to detect decoupling at 45 contrasting EC sites across a broad range of canopy architectures and biomes (Peltola et al. 2025, https://doi.org/10.1016/j.agrformet.2024.110326). Omega encapsulates the main processes controlling decoupling in a single dimensionless metric, thus providing a unified framework for studying coupling at all sites. We focus on evaluating the applicability of Omega to detect decoupling at these sites and use it to evaluate the processes controlling decoupling across sites.

The results show that Omega was able to identify coupling at all tested sites satisfactorily. The vertical turbulent carbon dioxide flux showed a similar Omega dependence at all sites, although there was some site-to-site variability. In contrast, when the change in storage flux term was added to the analysis, the similarity between sites disappeared. This suggests that the storage flux term depends on parameters other than those controlling vertical turbulent mixing. Canopy drag played an important role in the formation of decoupling at dense forest sites, and at such sites decoupling was observed even during the day.

Based on these findings, we delineate different Omega regimes in which different mass balance terms (vertical turbulent flux, storage flux and advective components) are important, and discuss improved approaches for detecting the regime where the sum of vertical turbulent flux and storage flux equals the surface gas exchange.

How to cite: Peltola, O., Aslan, T., Aurela, M., Lohila, A., Mammarella, I., Papale, D., Thomas, C. K., and Vesala, T.: Towards improved understanding on flow decoupling at eddy covariance sites with the aid of a universal coupling metric, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6444, https://doi.org/10.5194/egusphere-egu25-6444, 2025.

EGU25-6639 | ECS | Posters on site | AS2.3

Methodological challenges for understory eddy-covariance measurements 

Alexander Platter, Albin Hammerle, and Georg Wohlfahrt

Understory eddy-covariance measurements provide valuable insights into ecosystem CO2 exchange processes, particularly in understanding the interplay between understory and overstory exchange processes. However, their placement deep within the canopy presents some methodological challenges not typically encountered in standard eddy-covariance measurements above the canopy, where surface layer assumptions are generally applicable.

Key challenges arise from the violation of these surface layer assumptions in common flux correction and quality control procedures. Traditional frequency response corrections for flux calculations often rely on idealized cospectra derived from surface layer theory. These assumptions do not hold within the canopy, where spectra and cospectra exhibit distinct characteristics. Furthermore, commonly used turbulence-based quality control metrics, like the integral turbulence test, rely on surface layer scaling relationships to compare measured and modeled fluxes. The application of these relationships within the canopy is questionable due to the altered turbulence structure. For net ecosystem exchange (NEE) measurements, conventional filtering methods, such as friction velocity (u*) filtering, aim to identify periods when measured fluxes are expected to closely represent the true NEE. However, the low fluxes and turbulence characteristic of the understory environment complicate the reliable application of these filtering approaches.

This study critically examines and revises established correction and quality control procedures specifically for understory eddy-covariance measurements. We investigate the impact of these revised methods on understory CO2 exchange estimates using data from an understory site in Tyrol, Austria (At-Mmg). Our results are further compared with the total net ecosystem exchange estimated by an above-canopy eddy-covariance system over the past three years.

 

How to cite: Platter, A., Hammerle, A., and Wohlfahrt, G.: Methodological challenges for understory eddy-covariance measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6639, https://doi.org/10.5194/egusphere-egu25-6639, 2025.

EGU25-6957 | Posters on site | AS2.3

Carbon fluxes controlled by land management and disturbances at a cluster of long-term ecosystem monitoring sites in Central Europe 

Thomas Grünwald, Matthias Mauder, Luise Wanner, Markus Hehn, Uta Moderow, Ronald Queck, Heiko Prasse, and Christian Bernhofer

Terrestrial ecosystems play a crucial role in carbon sequestration and provide vital ecosystem services such as food, energy, and raw materials. Climate change, through rising temperatures, altered precipitation patterns, and extreme events, threatens the carbon sink potential of these ecosystems, with forests and grasslands particularly at risk. Long-term data from flux tower networks offer valuable insights into how different ecosystems respond to climate change and management interventions, helping to develop strategies to mitigate greenhouse gas emissions and maintain ecosystem resilience. In this study, we present such data from a <10 km cluster of long-term FLUXNET/ICOS sites in Central Europe, comprising an old spruce forest (DE-Tha), a young oak plantation after a cleared windthrow (DE-Hzd), a permanent grassland site (DE-Gri), and an agricultural site with a crop rotation typical for this region (DE-Kli). By analysing decades of data from these four eddy covariance measurement sites, the research highlights the influence of drought, management, and land cover changes on CO2 and H2O fluxes. The interannual variability of evapotranspiration depends less on land use than the CO2 exchange. Our findings show that  forests without terminal disturbances can act as larger carbon sinks than previously estimated. DE-Tha is a consistent carbon sink, with thinning helping to maintain the CO2 sequestration at a stable level of 350 gC m−2 a−1. In contrast, disturbances like clear cutting or windthrow can cause ecosystems to become carbon sources for several years, with recovery delayed due to soil carbon losses from increased respiration (DE-Hzd). While DE-Hzd was resilient to drought, the carbon uptake of DE-Tha was significantly reduced by around 50% during dry years compared to wet years. Furthermore, sustainable management maintains carbon sequestration and land-use practices, such as crop selection, significantly impact net ecosystem productivity. These insights are valuable for optimizing land management strategies to enhance carbon sinks in similar regions.

How to cite: Grünwald, T., Mauder, M., Wanner, L., Hehn, M., Moderow, U., Queck, R., Prasse, H., and Bernhofer, C.: Carbon fluxes controlled by land management and disturbances at a cluster of long-term ecosystem monitoring sites in Central Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6957, https://doi.org/10.5194/egusphere-egu25-6957, 2025.

We present first results of a new BROOK90 hydrological model version. This new version includes a closed energy and water balance for subdaily time steps based on an adapted Shuttleworth-Wallace model for the description of energy and water fluxes for different evaporation components, like interception, soil evaporation and transpiration. The simulation results have been compared to ICOS eddy-covariance measurements from the Anchor Station Tharandt for the year 2022.

The comparison shows considerable good result for 30-minute estimates of latent and sensible heat fluxes from dry surfaces, whiles simulated fluxes from wet surfaces perform worse. Snow conditions seem to be almost random, but rainy conditions might possess a certain correlation between measured and simulated fluxes. Reason for these results can be found on the one hand in the choice of model parameters for vegetation like maximal canopy resistances, leaf area index or canopy height in the model and on the other hand, limitations of the eddy-covariance measurements under wet conditions.

How to cite: Kronenberg, R., Vorobevskii, I., and Luong, T. T.: First results of an extended BROOK90 hydrological model to estimate subdaily water and energy fluxes. A case study of ICOS Anchor station in Tharandt, Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9419, https://doi.org/10.5194/egusphere-egu25-9419, 2025.

EGU25-9629 | ECS | Posters on site | AS2.3

Metrological Traceability in Eddy Covariance Measurements of CO2 Flux 

Alberto Bottacin, Michela Sega, Francesca Durbiano, Francesca Rolle, and Nicola Arriga

The Eddy Covariance (EC) technique is widely used to quantify carbon dioxide (CO2) fluxes between the atmosphere and terrestrial ecosystems, playing a crucial role in climate research and carbon cycle studies. To maximize the impact and the meaningfulness of these measurements, they have to be comparable in time and space. The reliability and comparability of EC data critically depend on ensuring metrological traceability to SI units through national standards or internationally agreed references by means of rigorous calibration practices.

This study examines the traceability chain for key EC components (air temperature and pressure, wind components and CO2 concentration in air), emphasizing calibration processes for gas analyzers. Gas analyzers, which measure CO2 amount fractions, are calibrated using traceable gas mixtures, such as Certified Reference Materials, linked to primary national standards, ensuring accuracy and minimizing biases. We assess the impact of the calibration uncertainty on overall flux estimates and propose a methodology for periodic recalibration of the analysers to account for their drift and response to environmental influences.

By establishing robust links to national metrology standards, this work enhances the traceability and reliability of EC data across diverse ecosystems and temporal scales. The outcomes provide a foundation for harmonizing EC networks globally, improving confidence in CO2 flux measurements and their role in shaping evidence-based climate policies. This focus on calibration underscores the importance of metrology in advancing the precision and usefulness of environmental measurements.

 

How to cite: Bottacin, A., Sega, M., Durbiano, F., Rolle, F., and Arriga, N.: Metrological Traceability in Eddy Covariance Measurements of CO2 Flux, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9629, https://doi.org/10.5194/egusphere-egu25-9629, 2025.

EGU25-9912 | ECS | Posters on site | AS2.3

Parametrization of extremely heterogeneous land-surface processes 

Christian Wedemeyer and Yaping Shao

The land surface plays a crucial role in the climate system, significantly influencing the exchanges of energy, mass, and momentum among the atmosphere, biosphere, and lithosphere. While land-surface processes in homogeneous terrains are well understood and effectively integrated into the parameterization schemes of existing weather models, our understanding of these processes in extremely heterogeneous regions remains insufficient. This gap in knowledge limits our capacity to accurately parameterize land-surface interactions in such areas. Extremely heterogeneous surfaces are characterized by a variety of soil types and pronounced orographic features, such as mountains or steep slopes.

State-of-the-art weather models commonly utilize the Monin-Obukhov similarity theory (MOST) for parameterizing surface momentum, heat, and moisture fluxes. However, these similarity functions are based on empirical data obtained from field campaigns conducted in homogeneous environments. When these functions are applied to extremely heterogeneous regions, they can produce large biases between modeled and observed surface sensible or latent heat fluxes. Furthermore, in large-eddy simulations (LES), the underlying assumptions of MOST - such as horizontal homogeneity and stationarity - are often violated. Additionally, inconsistencies arise between the fluxes calculated using subgrid closure schemes and those derived from MOST in the surface layer.

To tackle these challenges, we propose an alternative approach that circumvents the use of MOST for parameterizing surface fluxes. In land-surface-parameterization schemes, surface fluxes are often determined using resistance networks. Instead of estimating these resistances using MOST, our aerodynamic resistance approach (ARA) uses the eddy viscosity/diffusivity calculated by the subgrid closure schemes.

First tests in idealized large-eddy simulations (LES) using the Weather Research and Forecasting model (WRF) show that the ARA-calculated surface fluxes are more consistent with the subgrid closure calculations than the MOST-derived fluxes. Next, the ARA will be tested in real-case simulations of the Tengchong site (China) on the Tibetan plateau which is known for its heterogeneous landscape. Moreover, the simulation results will be compared to observational data which has been available at the site for more than 12 years.

How to cite: Wedemeyer, C. and Shao, Y.: Parametrization of extremely heterogeneous land-surface processes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9912, https://doi.org/10.5194/egusphere-egu25-9912, 2025.

EGU25-10813 | ECS | Orals | AS2.3

Analysing the time scales of variability in carbon dioxide and energy balance components of a tropical Amazon rainforest in central Peru 

Lea Heidemann, Eric Cosio, Rudi Cruz, Juliane Diller, Armin Niessner, Johannes Olesch, Norma Salinas, Rafael Stern, and Christoph Thomas

The Amazon Rainforest plays a vital role in the global carbon and water cycle, yet responses of old growth tropical rainforests to climate change and rising CO2 concentrations remain poorly understood. Especially the western part of the Amazon is underrepresented in ecohydrological studies. At the Panguana research station, as part of the AndesFlux Network, fluxes of CO2, water vapor and the dynamics of the CO2, CH4 and water vapor profile inside the forest and above the 35 m tall canopy have been continuously monitored since December 2023 to fill this gap and determine whether this site acts as a net source or sink for carbon. Building on this objective, our focus extends to understanding the timescales and ecosystem drivers responsible for flux variability, a crucial step toward predicting ecosystem responses to future changes.

As the main objective, we aim at understanding what are the main drivers for ecosystem flux variability, e.g. incoming solar radiation, water availability, or water vapor deficit and on which timescale we can detect the highest variability of ecosystem fluxes. In a tropical region the highest variability in an annual dataset would be expected to occur on a seasonal timescale. However, we did not observe the expected difference in latent heat flux when comparing the mean dial course on a seasonal basis. Surprisingly, we found the highest variability of latent heat flux to occur on much shorter timescales of up to ten days, coinciding with variability of incoming shortwave radiation for which a timescale of highest variability of eight days was detected. Understanding the processes causing this periodicity in latent heat flux in a tropical region and resulting effects on CO2 flux is the primary objective of this analysis.

A further objective of this study presented here is to calculate a CO2-based carbon budget, with the inclusion of the storage term change to understand the effect of ecosystem respiration at night. While the methane exchange to the carbon budget may be significant at this site, it is outside the scope of the current study. Additional objectives of this project include calculating the energy balance of this site and analysing at the surface water balance to better understand seasonal differences and their impact on the carbon cycle.

After calculating the 4h-daytime energy balance closure with different perturbation time scales, we selected a perturbation timescale of 20 min as the best compromise between reducing the systematic and random flux errors. This choice leads to a high energy balance closure of 75% over the course of one year maximizing to 80% when calculated for the rainy season.

These analyses contribute to a deeper understanding of the driving processes of ecosystem exchange in the tropical rainforest near the Andes and help to assess how this part of the Amazon basin may respond to future changes in water availability and atmospheric circulation.

How to cite: Heidemann, L., Cosio, E., Cruz, R., Diller, J., Niessner, A., Olesch, J., Salinas, N., Stern, R., and Thomas, C.: Analysing the time scales of variability in carbon dioxide and energy balance components of a tropical Amazon rainforest in central Peru, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10813, https://doi.org/10.5194/egusphere-egu25-10813, 2025.

EGU25-10940 | ECS | Posters on site | AS2.3

Measuring urban surface fluxes using a mobile eddy-covariance system at a fine resolution to develop a heat mitigation strategy in a mid-sized European city   

Lars Spakowski, Sophie Resch, Johannes Olesch, and Christoph Thomas

As demographic trends continue to point towards urbanisation and urban climate change-related health risks are increasing, a fundamental understanding of the processes that shape the urban boundary layer climate is becoming increasingly important. While previous studies have used mobile measurement devices to measure instantaneous physical weather elements in high spatial resolution in an urban environment, high-resolution measurement data on atmospheric flux densities in cities is scarce.

We present an innovative approach to measure latent and sensible heat fluxes, as well as CO2 fluxes and further flow statistics as TKE in a mid-sized city (75,000 citizens) in Central Europe using a mobile eddy-covariance (EC) system on a cargo bike with first measurements executed during a radiation night and three consecutive heat days in August 2024. Our goal was to gain flux density data for several street transects in a heterogeneous urban environment during the hottest and coldest time periods of the day. To compare the measured temperature and humidity used for the eddy-covariance calculations, we set up eight weather stations mounted on streetlights along our measurement route, at which we stopped for two minutes each. Motion data was observed with an integrated high precision inertial navigation system (INS) to adjust the EC observation for bicycle movements. To ensure nearly steady-state conditions were fulfilled, the perturbation and averaging periods were fitted to calculate flux densities along approximately homogeneous street transects. As the bike velocity of 4 to 6 m s-1 only allows for relatively short averaging periods of up to a minute in the heterogenous environment, only the high-frequency fraction of the turbulence spectrum can be quantified. Assuming a similar distribution of the inertial subrange turbulence across the research area, this choice still allowed for comparison of the fluxes along the route.

With our route traversing a range of land surface conditions from a densely built-up district centre to a floodplain valley adjacent to the city, we were able to determine a strong heterogeneity in the expression of the urban heat and park cool islands within our study area. First results of the EC calculations indicate the capability of our mobile flux system to detect fine differences in flux densities within the heterogeneous urban environment.

Our flux measurements together with the additionally measured weather elements of solar radiation, temperature, humidity, wind direction and wind speed from the eight stationary micro weather stations within the study area provide the foundation for the development of a heat adaption strategy in the city district aiming at creating an environment with diminished health risks and urban heat island effects. 

How to cite: Spakowski, L., Resch, S., Olesch, J., and Thomas, C.: Measuring urban surface fluxes using a mobile eddy-covariance system at a fine resolution to develop a heat mitigation strategy in a mid-sized European city  , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10940, https://doi.org/10.5194/egusphere-egu25-10940, 2025.

EGU25-11746 | ECS | Posters on site | AS2.3

Evaluating a Flux Footprint Model Using Tracer Release Experiments and Tall Tower Eddy Covariance Measurements 

Ziqiong Wang, Konstantinos Kissas, Charlotte Scheutz, and Andreas Ibrom

In complex and heterogeneous landscapes, determining the spatial origin of measured fluxes is critical for interpreting eddy covariance (EC) data accurately. To address this, footprint models are used to simulate the transport of turbulence and quantify the contribution of different areas within the source region. These models rely on theoretical assumptions, such as homogeneous and stationary atmospheric conditions, which often deviate significantly from real-world conditions particularly in terrains with uneven topography or land cover. This discrepancy may lead to substantial uncertainties, as the models may fail to accurately represent the true flux contributions under these non-ideal conditions.

To evaluate the reliability of the Flux Footprint Prediction (FFP) model (Kljun et al., 2015) and its performance under real-world conditions, we conducted three tracer release campaigns in the upwind region of a tall tower EC greenhouse gas observation system located at Hove (55.7169°N, 12.2375°E), a rural area west of Copenhagen, Denmark. The experiments utilized acetylene (C₂H₂) as the tracer gas, released at a controlled and precisely known emission rate.  The FFP model were assessed using data from different averaging intervals, enabling a detailed comparison of temporal resolutions and their impact on flux estimates.

The observed fluxes were systematically compared with the model predictions, allowing us to identify discrepancies and provide critical insights into the strengths and limitations of the FFP model, particularly in rural and heterogeneous landscapes. Moreover, the analysis highlights the influence of averaging intervals on the agreement between measured and modelled fluxes. This work also provides a reference for applying tracer release experiments in heterogeneous terrain using the tall tower EC system, contributing to the understanding of experimental design and model validation in such environments.

How to cite: Wang, Z., Kissas, K., Scheutz, C., and Ibrom, A.: Evaluating a Flux Footprint Model Using Tracer Release Experiments and Tall Tower Eddy Covariance Measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11746, https://doi.org/10.5194/egusphere-egu25-11746, 2025.

For the past five decades, modelers have relied on Monin-Obukhov Similarity Theory (MOST) to model surface exchanges for application in atmospheric models for boundary layer meteorology and weather and climate prediction. During this time, studies have also illuminated some of the limitations of MOST based surface layer parameterizations, particularly when MOST’s foundational assumptions of flat and horizontally homogeneous terrain are violated. Recent work over groups of meteorological towers from Stiperski and Calaf 2023 have provided a promising method to account for these deviations from the ideal, traditional MOST using the anisotropy of turbulence to create new surface exchange relations. These modified relations may be able to capture the deviations from MOST specifically around non-homogeneous surfaces, and non-stationarity. To further assess the validity of the Stiperski relations, we examine them over 7 years of turbulence data from the 47, ecologically diverse eddy-covariance tower sites in the National Ecological Observation Network (NEON) and develop new anisotropy generalized MOST scalings for the scalar variances of moisture and carbon.

 

The relations from Stiperski and Calaf 2023 show significant improvement over traditional MOST based schemes for predicting the velocity variances as well as the variances of heat, moisture and carbon in the NEON network under both stable and unstable stratification. This extends the work of Stiperski and Calaf to vegetated canopies, where the scaling has not been previously examined. The improvement is consistent across the varied ecosystems present in NEON, including tropical, arctic, and mountainous sites. For the streamwise velocity variance, for example, we see a median improvement (measured with a skill score) of 40% at the NEON sites. Characteristics of anisotropy are also examined across the sites, with an eye towards developing model relations for turbulence anisotropy applicable in large scale schemes (i.e. numerical weather prediction and earth system models. Initial results for the scaling of the gradients of heat and momentum, which can be used to parameterize surface fluxes in the modeling context, are also shown, with promising improvement over traditional MOST despite significant scatter. The route for application of these schemes in surface layer parameterizations in ESMs is also briefly explored, with an eye towards the potential for significant improvements in modeling of surface exchange.

 

 

How to cite: Waterman, T., Stiperski, I., and Calaf, M.: Extending Generalized Surface Layer Scaling to Diverse, Complex Terrain and Canopies for Improved Land-Atmosphere Exchange, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11806, https://doi.org/10.5194/egusphere-egu25-11806, 2025.

EGU25-12023 | ECS | Posters on site | AS2.3

Irrigation impacts on the severe summer 2003 drought and heat wave event in Central Europe 

Dragan Petrovic, Benjamin Fersch, and Harald Kunstmann

Irrigation is triggered through climatic conditions, but reversely affects the climate itself. A model sensitivity analysis of the irrigation impacts on the severe summer 2003 drought and heat wave event in Central Europe is carried out here. For this purpose, the Weather Research and Forecasting (WRF) model is employed with a newly developed and modified irrigation scheme. A two-domain nested setup with 12 km horizontal grid resolution in the outer domain and convection-resolving 3 km in the inner domain is selected. Two ensembles, one with and one without irrigation, are initialized to assess the irrigation impacts with greater security. Four subregions are defined: a region containing all of Germany, two small regions with locally higher irrigation amounts within Germany and an area in the Po Valley, the region with highest irrigation quantities in Central Europe. This way, the influence of different irrigation amounts is investigated. Impacts on the following variables are examined in different temporal scales: air temperature, soil moisture, planetary boundary layer height (PBLH), sensible and latent heat flux, moisture flux divergence, convective available potential energy (CAPE), and convective inhibition (CIN). The results indicate that the overall influence of irrigation during the extreme event is rather small. This is related to the comparatively low irrigation amounts and the extreme conditions. A partially significant increase in soil moisture in the topsoil layer occurs in the Po Valley. Generally, irrigation is found to reduce PBLH and sensible heat flux as well as increasing the latent heat flux. In addition, a cooling effect is partly found in the daily mean cycle of temperature. Furthermore, there are visible effects on moisture flux divergence (tendency to decrease or convergence), on CAPE (increase) and on CIN (less increase). These effects are most pronounced in the Po Valley due to the higher irrigation amounts.

How to cite: Petrovic, D., Fersch, B., and Kunstmann, H.: Irrigation impacts on the severe summer 2003 drought and heat wave event in Central Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12023, https://doi.org/10.5194/egusphere-egu25-12023, 2025.

EGU25-12704 | Orals | AS2.3

Spatial source attribution of eddy covariance flux data by inversion optimization 

Mark Schlutow, Ray Chew, Theresia Yazbeck, and Mathias Göckede

Since eddy covariance (EC) flux towers are typically mounted within structured landscapes, interpreting EC flux data is complicated due to spatial heterogeneity, which may exhibit sources and sinks simultaneously. This complexity makes it challenging to understand mechanisms and controls determining flux budgets for the individual land cover types that make up the entire ecosystem. Therefore, it complicates the scaling of flux results in space and/or time, or comparing EC fluxes under different environmental conditions.

We present a novel tool to decompose blended flux data from EC towers into individual components emitted by different land cover types within the tower’s footprint. The tool has two key components: 1) an exceptionally efficient algorithm that solves the steady-state transport equation, and 2) a linear optimizer to solve the inversion problem. This design allows for the analysis of years of continuous EC data on a typical desktop computer in a short time, with output consisting of half-hourly flux data for each land cover type individually.

The approach is entirely data-driven and can be applied to the fluxes of energy and scalars such as methane, N2O, or CO2. The model takes as input a land cover map containing the footprint and the standard output from the raw eddy data processing software, EddyPro. The accuracy of the flux attribution tool was validated using two EC towers in close proximity, sharing the same ecosystem and meteorological conditions, but with different land cover structures in the footprint. The agreement between the inversion results for each of the towers proves its applicability for a wide range of research questions.

How to cite: Schlutow, M., Chew, R., Yazbeck, T., and Göckede, M.: Spatial source attribution of eddy covariance flux data by inversion optimization, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12704, https://doi.org/10.5194/egusphere-egu25-12704, 2025.

While covering only about 3% of the global land surface, peatlands store approximately one-third of all terrestrial carbon (C) and 12–21% of global soil organic nitrogen (N). Pristine peatland soils typically function as minor sinks for carbon dioxide (CO2), moderate sources of methane (CH4), and minor to moderate sources of nitrous oxide (N2O). However, over the past century, extensive drainage of peatlands for forestry, particularly in temperate and boreal regions, has substantially altered the dynamics of greenhouse gases (GHG).

The lowering of the groundwater table has a crucial impact on soil GHG exchange with aerobic conditions inhibiting methanogenesis, thereby reducing CH4 flux, while simultaneously increasing N2O flux and accelerating peat decomposition. These changes transform peatlands from carbon sinks to net carbon sources and intensify their N2O emissions. However, actively growing tree stands may partially offset soil carbon losses through sequestration and indirectly modulate CH4 and N2O fluxes by altering soil moisture and microbial activity.

While the net ecosystem exchange of drained peatland forest soils is relatively well studied, there's limited knowledge regarding ecosystem-scale GHG fluxes, especially in the transitional hemiboreal forest zone. In this study, we present the first years of eddy-covariance measurements of CO2, CH4, and N2O fluxes from a drained peatland forest in Eastern Estonia. The site, drained in the early 1970s via an open-ditch network, is dominated by Downy Birch (Betula pubescens, 64%) and Norway Spruce (Picea abies, 36%). The current soil profile, classified as Drainic Eutric Histosol, features a peat layer approximately one meter thick and a moderate C:N ratio (15.1) in the upper soil horizon. Our findings contribute to the growing body of knowledge on peatland forest GHG fluxes, offering valuable data for managing forested peatlands in a changing climate.

How to cite: Krasnova, A., Soosaar, K., and Mander, Ü.: The greenhouse gas exchange of a drained peatland forest: first insights from eddy-covariance measurements of CO2, CH4 and N2O fluxes in Estonia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13303, https://doi.org/10.5194/egusphere-egu25-13303, 2025.

EGU25-14269 | Orals | AS2.3

Investigating the Role of Kilometer-scale Surface Thermal Heterogeneity in Secondary Circulations Using Satellite Remote Sensing and Doppler Lidars 

Nathaniel Chaney, Peter Germ, Marc Calaf, Eric Pardyjak, and Tyler Waterman

Spatially organized km-scale surface thermal heterogeneity can lead to the formation of secondary circulations, which, in turn, can influence the boundary layer and the initiation, development, and enhancement of cumulus clouds. While the importance of this process is becoming well recognized, quantitative understanding of the relationship between thermal heterogeneity and the corresponding circulations remains largely confined to modeling studies. In this study, we use observational data from the ARM Southern Great Plains (SGP) site to explore how combining satellite remote sensing of land surface temperature (LST) with a mesoscale network of Doppler lidars can help understand the role of surface thermal heterogeneity in driving secondary circulations.
We analyze data from five Doppler lidars at SGP, which have been continuously measuring vertical profiles of wind components (u, v, w) at high temporal frequency since 2016. The combination of the five time-varying profiles are used to compute vertically integrated dispersive kinetic energy (DKE) at each time step as an indirect measure of circulation strength. LST data from GOES-16/17 is then used to quantify surface thermal heterogeneity, particularly in the morning hours. Our analysis focuses on days with minimal synoptic forcing to isolate local effects. Preliminary results show a statistically significant positive correlation between surface thermal heterogeneity and DKE, suggesting a link to the strength of secondary circulations. This study highlights the potential to improve our understanding of this process and provides a valuable tool for evaluating Earth system models that aim to represent the role of km-scale thermal heterogeneity in the atmosphere.

How to cite: Chaney, N., Germ, P., Calaf, M., Pardyjak, E., and Waterman, T.: Investigating the Role of Kilometer-scale Surface Thermal Heterogeneity in Secondary Circulations Using Satellite Remote Sensing and Doppler Lidars, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14269, https://doi.org/10.5194/egusphere-egu25-14269, 2025.

EGU25-15199 | ECS | Orals | AS2.3

Discovering new Influences on Dispersive Heat Fluxes over Heterogeneous Surfaces with Machine Learning 

Benita Wagner, Matthias Karlbauer, Martin Butz, Matthias Mauder, and Luise Wanner

To better understand and quantify the dynamics of surface thermal heterogeneities and their effect on energy transport in form of dispersive fluxes within the atmospheric boundary layer, we investigate the significance and applicability of the heterogeneity parameter after Margairaz et al. (2020). We aim to overcome this non-dimensional scaling quantity, since it depends on parameters such as the heterogeneity length, scale, and temperature amplitude, which are originally determined for checker-board-type surfaces but may be less suited to describe the complexity of real-world surface structures. To address this goal, we train separate artificial neural networks (ANNs) to predict dispersive sensible and latent heat fluxes for a randomized quadratically shaped heterogeneity distribution, as well as for datasets from the CHEESEHEAD19 campaign representing a real-world complex surface heterogeneity with a broad spectrum of patch sizes and gradual changes in surface characteristics. To investigate the role of the different input variables, we train various ANNs receiving different combinations of variables and compute feature importance weightings afterwards. We scrutinize the role of traditional input variables such as the heterogeneity parameter, temperature or humidity gradients, boundary layer height, and atmospheric stability measures. Further, we consider the incorporation of raw input features, such as horizontal and vertical wind speed, temperatures, and humidities. Finally, we incorporate spatial temperature maps, which we pre-process with a convolutional ANN. We make three core observations. First, the incorporation of raw input features beyond traditional variables improves both the dispersive sensible and latent heat flux diagnosis, suggesting room for improvement in the input variable selection and combination. Second, the inclusion of the spatial temperature map is more meaningful for dispersive latent than for sensible heat flux diagnosis. Third, the heterogeneity parameter after Margairaz et al. (2020) is informative for synthetic randomized quadratically shaped surfaces, but not for real-world complex surface heterogeneity environments, in which case the spatial temperature map processed by a convolutional ANN is most valuable. The results imply that the role of the compressed spatial temperature map should be explored further. We ultimately aim to extract an equation from the neural network characterizing heterogeneous surfaces. Furthermore, the incorporation of the other identified useful raw input features – ideally in form of an equation – needs to be assessed in further depth. 

How to cite: Wagner, B., Karlbauer, M., Butz, M., Mauder, M., and Wanner, L.: Discovering new Influences on Dispersive Heat Fluxes over Heterogeneous Surfaces with Machine Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15199, https://doi.org/10.5194/egusphere-egu25-15199, 2025.

EGU25-15275 | ECS | Orals | AS2.3

Urban effects on atmospheric boundary-layer clouds, mixed-layer height and fog detected by a dense network of ceilometers in Berlin, Germany 

Daniel Fenner, Andreas Christen, Sue Grimmond, Simone Kotthaus, Fred Meier, and Matthias Zeeman

Gaining a deeper understanding of dynamic interactions between cities and the atmospheric boundary layer (ABL) and ABL processes in general is crucial for, e.g., the development and application of next-generation numerical weather prediction and climate modelling. In this context, detailed ABL observations provide essential information to identify potential spatial heterogeneity in urban and rural environments with respect to surface-atmosphere exchanges and resulting ABL characteristics such as ABL clouds.

As part of the year-long urbisphere-Berlin measurement campaign in Berlin, Germany (October 2021-September 2022), a wide range of ABL observations were carried out to study impacts of the city on the ABL. Central to the deployed systematic network were 25 sites with ground-based Automatic Lidar and Ceilometers (ALC) to measure aerosol backscatter for investigation of intra-urban, urban-rural, and upwind-city-downwind effects of ABL clouds and detection of the mixed layer.

Here, we present a systematic investigation of year-round effects of the city on ABL cloud-base height and cloud-cover fraction, mixed-layer height, and near-surface fog conditions, exploiting the dense ALC network. The comprehensive data set allows studies along diurnal and annual cycles in high temporal resolution, as well as obtaining robust statistical results for groups of sites, considering spatial heterogeneity due to local effects around the sites. Our analyses show city effects on ABL clouds along the diurnal cycle including upwind-city-downwind effects, yet also depending on cloud type and season. Mixed-layer height undergoes a distinctive annual cycle, being systematically higher above the city and with intra-urban differentiation. Over the year, the occurrence of ground-based fog is on average 1,5 times more frequently found at rural sites compared to city sites, most prominent differences are found during autumn and winter. These results are the first that are based on the complete year-long urbisphere-Berlin ALC data and highlight potentials and benefits of such high-resolution observational data sets from ground-based remote sensing for future investigations.

How to cite: Fenner, D., Christen, A., Grimmond, S., Kotthaus, S., Meier, F., and Zeeman, M.: Urban effects on atmospheric boundary-layer clouds, mixed-layer height and fog detected by a dense network of ceilometers in Berlin, Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15275, https://doi.org/10.5194/egusphere-egu25-15275, 2025.

EGU25-17589 | Orals | AS2.3

Metrology for fluxes: eddy covariance measurement uncertainty 

Nicola Arriga and Alberto Bottacin

The uncertainty evaluation of eddy covariance flux measurements has been thoroughly developed in the last two decades. However, the various methods proposed are not yet fully compliant with the internationally accepted metrological guidelines, e.g. those indicated in the Guide to expression of uncertainty in measurement and related supplements issued by the Joint Committee for Guides in Metrology and internationally adopted as reference in metrology. Scope of this presentation is to implement the formal methodology for the determination of a combined standard uncertainty for the estimated fluxes through the law of propagation of uncertainty, assuming independent variables. Compared to previous methods, this approach considers the complete flux equation, including the coordinate rotations and the physical conversions and, most importantly, provides an easy to implement analytical tool to quantify the individual contributions to the full measurement uncertainty arising from all the variables actually included in the calculation (turbulent wind components, scalar of interest, air temperature and pressure). The linear method adopted for uncertainty propagation has been also validated through a Monte Carlo simulation, which is the gold standard for propagating probability distributions. The methodology has been applied to a full year of carbon dioxide fluxes measured in the San Rossore 2 ICOS Ecosystem Station, a Mediterranean forest, but it is valid for most of the common eddy covariance systems, being based on theoretical principles. The median of the estimated relative uncertainty of the flux over the considered year is 13.5%, assuming an instrumental uncertainty of 30 Pa for the barometer, 0.5 °C for the thermometer, 4 ppm for the CO2 analyzer and 0.4 m/s for the three components of the sonic anemometer. The main uncertainty contributions come from the analyzer and the vertical component of the anemometer, with medians of the evaluated relative uncertainties equal to 11.9% and 3.25%, respectively. Preliminary results suggest that the method is robust and confirm expectations about the relative contribution of the different instruments used for flux determination, but at the same time constitute a tool for a sounder metrological assessment of all eddy covariance measurements and applications.

How to cite: Arriga, N. and Bottacin, A.: Metrology for fluxes: eddy covariance measurement uncertainty, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17589, https://doi.org/10.5194/egusphere-egu25-17589, 2025.

Land-atmosphere (L-A) feedback plays a key role in the evolution of Earth’s weather and climate system. However, the understanding and simulation of land-atmosphere interaction still suffers from severe limitations and errors. For instance, Abramowitz et al. (2024) demonstrated that the simulation of surface fluxes by land-atmosphere models, irrespective of their complexity, strongly deviates from observations. Similarly, Monin-Obukhov Similarity Theory (MOST) seems to be inadequate (Wulfmeyer et al. 2023) for the parameterization of evapotranspiration, but is nevertheless used in almost all coupled land-atmosphere system models.  

The overarching goal of LAFI is to understand and quantify L-A feedbacks via unique synergistic observations and model simulations from the micro-gamma (» 2 m) to the meso-gamma (» 2 km) scales across diurnal to seasonal time scales. In this presentation, we give an overview of the objectives and the current results of LAFI with respect to the understanding of surface-layer flow and fluxes, the energy balance closure (EBC), and entrainment over heterogenous agricultural terrain. More insight will be gained by the LAFI field campaign, which will be performed from Spring to Autumn 2025 at the Land-Atmosphere Feedback Observatory (LAFO) of the University of Hohenheim. The LAFI field campaign will enhance the current sensor synergy at LAFO, in order to capture key variables more fully within the soil, vegetation, and atmosphere compartments (Späth et al. 2023). Highlights of the new LAFI instrumentation include water-vapour isotope sensors, sap-flow sensors, fiber-optical distributed sensors (FODS, Thomas and Selker, 2021),unmanned aerial vehicles (UAVs), and scanning water-vapor, temperature, and wind lidar systems. We demonstrate how these measurements complement each other to gain new insights into flux-driver relationships, soil evaporation, crop transpiration, and entrainment, as well as the impact of land-surface heterogeneities and dispersive fluxes on the EBC. The very first results of this campaign will also be presented. 

 

References: 

Abramowitz et al. 2024: https://bg.copernicus.org/articles/21/5517/2024 

Späth et al. 2023: https://doi.org/10.5194/gi-12-25-2023 

Thomas, C.K., Selker, J.S., 2021. https://doi.org/10.1007/978-3-030-52171-4_20 

Wulfmeyer et al. 2023: https://link.springer.com/article/10.1007/s10546-022-00761-2  

 

How to cite: Wulfmeyer, V.: The Land-Atmosphere Feedback Initiative (LAFI): Field observations, modeling approaches, and first results, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19157, https://doi.org/10.5194/egusphere-egu25-19157, 2025.

EGU25-19174 | ECS | Posters on site | AS2.3

Evaluation of CO2 and energy balance fluxes from a maize canopy in east Tennessee using the SURFATM model 

Taqi Raza, Erwan Personne, Nebila Lichiheb, Neal Eash, and Joel Oetting

Field crops can emit or store carbon depending on the season and cropping practices. A process-based modeling approach allowed us to predict the transfer pattern of the CO2 fluxes and energy balance between soil, vegetation, and atmosphere. In this study, the SURFATM-CO2 model was developed to simulate distinctly the CO2 exchanges between soil, plants, and the atmosphere. The model couples soil respiration, taking into account its temperature sensitivity, with photosynthesis and plant respiration process-based, taking into account the plant's CO2 compensation point. The SURFATM-CO2 process model was evaluated using field measurements obtained from a novel multiport profile system consisting of 4 vertical measurement heights to monitor the spatial and temporal variation of CO2, water, and temperature within and above the maize canopy in east Tennessee. The 5Hz frequency raw data were averaged into 15-minute runs and used as input for the SURFATM model. The model satisfactorily simulates the energy balance, and we are currently testing the model for the CO2 fluxes.  The main objective of this study is to understand the exchanges of CO2 between the soil, vegetation and atmosphere compartments. The finding of the SURFATM-CO2 model will highlight the ability of the SURFATM-model to capture the canopy-atmosphere interaction as well as provide a base for model application in the studies of carbon dynamics, and cropland ecosystem management.

How to cite: Raza, T., Personne, E., Lichiheb, N., Eash, N., and Oetting, J.: Evaluation of CO2 and energy balance fluxes from a maize canopy in east Tennessee using the SURFATM model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19174, https://doi.org/10.5194/egusphere-egu25-19174, 2025.

EGU25-20222 | ECS | Posters on site | AS2.3

 Assessing the discrepancy of energy fluxes over spring wheat under sloping topography conditionsbased on eddy covariance measurements 

Jingyu Yao, Zhongming Gao, Lei Li, Eric Russell, Shelley Pressley, and Yongjiu Dai

Accurately quantifying surface energy budgets in croplands is essential for efficient water resource allocation and sustainable agricultural practices. However, the representativeness of eddy covariance (EC) measurements in hilly agricultural fields remains less examined. In this study, we conducted an experiment employing three EC flux towers to assess the consistency of surface energy budget components across a hilly agricultural field (~90 acres). The experimental field was divided into three zones, each equipped with an EC tower positioned at its central location to ensure that 90% of the flux footprint fell within the corresponding zone (i.e., US-SZ1, US-SZ2 and US-SZ3). The meteorological conditions and energy fluxes were found to be significantly influenced by various agricultural activities, including both growing and non-growing periods, as well as cropland management practices. Despite relatively similar meteorological conditions observed across the three sites during the wheat growing period (WGP), substantial discrepancies were evident in the primary energy budget components, with the exception of net radiation, at both diurnal and seasonal scales. During WGP, the sensible, latent, and ground heat fluxes exhibited differences within 10%, 27%, and 29%, respectively, leading toconsiderable disparities in the energy balance closure. The closure ratios (CRs) for US-SZ1, US-SZ2, and US-SZ3 were approximately 93%, 84%, and 85% respectively. The influence of environmental variables on the discrepancies in their CRs were also investigated. The relationships between CRs and friction velocity, atmospheric stability, turbulent kinetic energy, as well as heat transport efficiency exhibited certain distinctions among the three sites. Our findings indicate that factors like site elevation, topography, and measurement uncertainty differentially affect energy flux components in sloping landscapes. Employing multiple tower/point measurements is crucial for reducing uncertainties in energy flux estimates under sloping terrain conditions.

How to cite: Yao, J., Gao, Z., Li, L., Russell, E., Pressley, S., and Dai, Y.:  Assessing the discrepancy of energy fluxes over spring wheat under sloping topography conditionsbased on eddy covariance measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20222, https://doi.org/10.5194/egusphere-egu25-20222, 2025.

EGU25-1242 | ECS | Orals | AS2.5

The influence of wave-induced variability on ocean carbon uptake 

Paridhi Rustogi, Laure Resplandy, Enhui Liao, Brandon Reichl, and Luc Deike

Traditional gas transfer velocity formulations for air-sea CO2 fluxes scale solely with wind speed, ignoring wave activity, including wave breaking and bubble-mediated transfers that enhance the rate of gas exchange. Here, we incorporate a wind-wave dependent gas transfer velocity formulation into an ocean general circulation model to quantify the effects of wave-induced spatiotemporal variability on CO2 fluxes and ocean carbon storage. Our results reveal that wave activity introduces a hemispheric asymmetry in ocean carbon storage, with gains in the southern hemisphere, where wave activity is robust year-round, and losses in the northern hemisphere, where continental sheltering reduces carbon uptake. Compared to a traditional wind-dependent formulation, incorporating wave activity yields a modest global increase in ocean carbon storage of 4.3 PgC over 1959-2018 (~4%), but on average, enhances the CO2 gas transfer velocity and flux variability by 5-30% on high-frequency and seasonal timescales in the extratropics and up to 200-300% during storms (>15 m s-1 wind speed). The magnitude of fluxes from wave activity is comparable to expected marine carbon dioxide removal (mCDR) efforts. This underscores the need to incorporate wind-wave variability into modeled fluxes to distinguish natural variability from anthropogenic impacts and ensure accurate mCDR verification and monitoring.

How to cite: Rustogi, P., Resplandy, L., Liao, E., Reichl, B., and Deike, L.: The influence of wave-induced variability on ocean carbon uptake, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1242, https://doi.org/10.5194/egusphere-egu25-1242, 2025.

EGU25-1323 | Posters on site | AS2.5

Organic Compounds in the Tropical Oligotrophic Atlantic Ocean: Insights into Sea-to-Air Transfer and Atmospheric Transformations  

Manuela van Pinxteren, Sebastian Zeppenfeld, Khanneh Wadinga Fomba, Nadja Triesch, Sanja Frka, and Hartmut Herrmann

Carbohydrates, amino acids, and lipids are significant contributors to organic carbon in the marine environment, playing key roles in ocean-atmosphere interactions. To investigate their sea-to-air transfer, enrichment in the sea surface microlayer (SML), and potential transformations during atmospheric transport, we conducted field studies in the tropical Atlantic Ocean at the Cape Verde Atmospheric Observatory. This study links measurements of these compounds in surface seawater, including the SML, with their presence and composition in submicron aerosol particles.

The study found moderate enrichment of lipids and carbohydrates in the SML, while amino acids exhibited higher enrichment, despite their relatively lower surface activity. In aerosol particles, lipids were markedly more enriched compared to amino acids and carbohydrates, likely due to their surface-active and lipophilic nature.

Detailed molecular analyses revealed shifts in the relative abundance of organic compounds during atmospheric transport, particularly for amino acids, suggesting in situ atmospheric transformations via biotic or abiotic processes. On average, 49% of aerosol OC was attributable to specific compound groups, with lipids accounting for the largest fraction. Amines, oxalic acid, and carbonyls contributed around 6%, while carbohydrates and amino acids each represented less than 1% of the total aerosol OC. Notably, carbohydrate-like compounds likely reside in glycolipids within the lipid fraction, underscoring the complexity of organic matter in marine aerosols.

These findings advance our understanding of the processes governing organic carbon transfer from the ocean to the atmosphere, including the roles of the SML and atmospheric processing. This knowledge is crucial for refining models of marine aerosols and their impact on atmospheric chemistry and climate.

The study contributes to the international SOLAS program.

Ref: van Pinxteren, M., Zeppenfeld, S., Fomba, K. W., Triesch, N., Frka, S., and Herrmann, H.: Amino acids, carbohydrates, and lipids in the tropical oligotrophic Atlantic Ocean: sea-to-air transfer and atmospheric in situ formation, Atmos. Chem. Phys., 23, 6571–6590, https://doi.org/10.5194/acp-23-6571-2023, 2023.

How to cite: van Pinxteren, M., Zeppenfeld, S., Fomba, K. W., Triesch, N., Frka, S., and Herrmann, H.: Organic Compounds in the Tropical Oligotrophic Atlantic Ocean: Insights into Sea-to-Air Transfer and Atmospheric Transformations , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1323, https://doi.org/10.5194/egusphere-egu25-1323, 2025.

EGU25-1376 | Posters on site | AS2.5

Impact of wildfires ash deposition on iron binding humic substances concentrations in surface waters: Results from a dissolution experiment 

gabriel Dulaquais, Matthieu Bressac, Eva Ortega-Retuerta, Emmanuelle Uher, Barbara Marie, and Nathan Nault

Wildfires contribute significantly to biomass burning. The deposition of ash from wildfires into surface ocean waters is a source of iron (Fe), namely pyrogenic Fe, and may enhance primary production in Fe-limited domains. However, due to the low solubility of Fe and the operational definition of its dissolved fraction, a portion of the dissolved Fe (DFe) released during ash dissolution may reprecipitate as authigenic inorganic colloids. This process can lead to an overestimation of the bioavailable pyrogenic DFe. To remain in a soluble form, Fe must be complexed with organic ligands capable of undergoing biochemical processes such as bacterial degradation, direct uptake, or photoreduction, leading to potentially bioavailable forms of DFe. Among the diverse range of iron-binding ligands, humic-type ligands (LFeHS) are important. LFeHS are ubiquitous in seawater, soluble, and may lead Fe to a bioavailable form. LFeHS are ubiquitous in seawater, soluble, and keep Fe in a bioavailable form. Here we present results from dissolution experiments. Ash samples collected in 2009 after wildfire events in the Spanish Mediterranean region were put in contact with non-euxinic, filtered Mediterranean surface seawater in a 7-day batch experiment. Four deposition fluxes were tested. The concentrations of DFe, fluorescent dissolved organic matter (FDOM), LFeHS, and the amount of Fe complexed by humic-type ligands were measured. Our results indicate that ash dissolution induces an increase in LFeHS, proportional to the ash concentration in the experimental medium. FDOM measurements confirm a time-dependent increase in humic-type material of terrestrial origin. Additionally, the observed increase in protein-like FDOM (C4) suggests that ash deposition enhances the modification of dissolved organic matter by bacteria. Using a simple kinetic model, we determined the dissolution rate constant for the tested ash. This constant can be incorporated into global oceanic models such as PISCES or REcoM to improve predictions of pyrogenic Fe bioavailability and its impacts on marine ecosystems.

How to cite: Dulaquais, G., Bressac, M., Ortega-Retuerta, E., Uher, E., Marie, B., and Nault, N.: Impact of wildfires ash deposition on iron binding humic substances concentrations in surface waters: Results from a dissolution experiment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1376, https://doi.org/10.5194/egusphere-egu25-1376, 2025.

EGU25-1665 | ECS | Orals | AS2.5 | Highlight

Surface microlayer ecosystems as platforms for viral adaptation and dispersal in the Central Arctic 

Janina Rahlff, George Westmeijer, Julia Weissenbach, Alfred Antson, and Karin Holmfeldt

In polar regions, aquatic viruses play a pivotal role in shaping microbial communities yet face significant challenges such as low host availability and harsh environmental conditions. During the Synoptic Arctic Survey 2021 aboard the icebreaker Oden (Snoeijs-Leijonmalm, 2022), we investigated viral diversity, survival mechanisms, and host interactions in the Central Arctic's surface microlayer (SML), the uppermost millimeter of the ocean, and compared them with ~60 cm depth from the ocean and a melt pond. This study addresses the knowledge gap surrounding near-atmosphere aquatic ecosystems, highlighting the SML as a critical platform for viral adaptation and dispersal in one of Earth's most extreme environments. Our study uncovered 1154 viral operational taxonomic units (vOTUs) >10 kb in size, two-thirds of which were predicted bacteriophages (viruses that infect bacteria). Flavobacteriales were identified as key hosts, with one dominant melt pond vOTU linked to a Flavobacterium sp. isolate. Melt pond viral communities displayed lower diversity compared to open water, indicating selective pressures in these transient systems. We found that 17.2% of vOTUs carried 87 unique auxiliary metabolic genes (AMGs) involved in pathways such as amino acid, glycan polymer, and porphyrin metabolism, supporting host survival under extreme conditions. Notably, 16 vOTUs encoded glycerol-3-phosphate cytidylyltransferase (tagD), which may function in cryoprotection. While lytic phages could not be found via plaque assays, prophage induction experiments using the bacterial isolate Leeuwenhoekiella aequorea Arc30 and mitomycin C revealed active phages with siphovirus morphology and minimal protein similarity to known phages. Our findings also highlight the SML’s role in viral dispersal, as vOTU abundance correlated with spread across the Arctic via the boundary layer. These sophisticated viral strategies emphasize their ability to thrive in remote, inhospitable, and host-limited environments (Rahlff et al., 2024). These discoveries underscore the importance of viruses in Arctic ecosystem dynamics, influencing microbial communities, and in the broader context, nutrient cycling, gas exchange and resilience to climate change.

References:

Rahlff, J., Westmeijer, G., Weissenbach, J., Antson, A., & Holmfeldt, K. (2024). Surface microlayer-mediated virome dissemination in the Central Arctic. Microbiome, 12(1), 218. https://doi.org/10.1186/s40168-024-01902-0

Snoeijs-Leijonmalm, P. (2022). Expedition Report SWEDARCTIC Synoptic Arctic Survey 2021 with icebreaker Oden. In: Swedish Polar Research Secretariat.

How to cite: Rahlff, J., Westmeijer, G., Weissenbach, J., Antson, A., and Holmfeldt, K.: Surface microlayer ecosystems as platforms for viral adaptation and dispersal in the Central Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1665, https://doi.org/10.5194/egusphere-egu25-1665, 2025.

EGU25-1770 | Posters on site | AS2.5

Methane distribution, production, and emission in the Western North Pacific 

Guiling Zhang, Haonan Wang, and Ziqiang Zhang

Ocean is a net source of atmospheric methane (CH4), but there are still large uncertainties in the estimations of global oceanic CH4 emission due to sparse data coverage. In this study, we investigated the spatial distribution and influencing factors of CH4 in the Western North Pacific (WNP) during two cruises in 2021 and 2022. High-resolution continuous underway measurements showed that surface CH4 concentrations ranged from 1.95 to 3.92 nM, indicating an obvious spatial gradient with a gradual increase from the south to the north due to the influence of water mixing and primary productivity. Vertically, subsurface CH4 maxima were ubiquitously observed due to in situ production through multiple pathways including MPn degradation and phytoplankton production. Surface water was oversaturated with respect to the atmospheric CH4 with the air-sea CH4fluxes in the tropical Western Pacific (1.28 ± 1.12 μmol/m2/d) higher than those in the Kuroshio Extension region (2021: 0.49 ± 0.89 μmol/m2/d; 2022: 0.37 ± 0.53 μmol/m2/d). Overall CH4 emission from the Western North Pacific is 0.08 Tg/yr, accounting for 13% of the total emission from the open ocean.

How to cite: Zhang, G., Wang, H., and Zhang, Z.: Methane distribution, production, and emission in the Western North Pacific, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1770, https://doi.org/10.5194/egusphere-egu25-1770, 2025.

EGU25-4242 | ECS | Orals | AS2.5

Air-sea ammonia fluxes in the Southern Ocean: Quantifying sources and sinks from surface waters to penguins.  

Simone Louw, Thomas Bell, Jo Browse, Malcolm Woodward, and Mingxi Yang

NH₃ drives nutrient cycling in the surface ocean and contributes to new particle formation in the marine atmospheric boundary layer. Surface ocean NH₃/Ammonium(NH₄⁺) is a vital component of the recycled nutrient pool, and NH₃ air-sea fluxes influence its redistribution. There are significant uncertainties in global NH₃ flux estimates due to a lack of concurrent air-sea measurements and ambiguity surrounding NH₃ sources.  Southern Ocean, a major driver of global climate, is experiencing rapid warming, altering the exchange of climate-relevant aerosols and precursor gases such as NH₃. Models systematically underpredict cloud droplet number concentrations and aerosol production in this region, a bias that arises from poorly captured aerosol precursor sources and lack of detailed microphysical cloud processes. We present atmospheric and seawater NH₃ measurements, along with NH₃ air-sea flux estimates, across the Southern Ocean during November and December 2024. Our study focuses on 1) identifying key NH₃ sources and sinks in the marine polar environment, and 2) quantifying how NH₃ fluxes vary across distinct emission hotspots. Preliminary observations show penguin colonies and volcanic activity drive distinct, localised NH₃ emission hotspots. The open ocean is generally thought to be a source of NH₃, but our data show that the open waters of the Southern Ocean is a sink of NH₃. By quantifying these fluxes, we reveal the variability across NH₃  source/sink regions and their potential to influence regional ocean-atmosphere biogeochemical processes.  

Our findings are crucial for improving the representation of clouds and aerosols in climate models, offering deeper insight into poorly understood aerosol-cloud interactions in this region. Improving these mechanisms will help reduce persistent Southern Ocean biases in model simulations of surface radiation and sea surface temperature and enhance our capacity to model regional and global climate.

How to cite: Louw, S., Bell, T., Browse, J., Woodward, M., and Yang, M.: Air-sea ammonia fluxes in the Southern Ocean: Quantifying sources and sinks from surface waters to penguins. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4242, https://doi.org/10.5194/egusphere-egu25-4242, 2025.

Increasing atmospheric CO₂ concentrations drives ocean acidification, potentially leading to substantial impacts on marine ecosystems and altering marine nutrient dynamics. Phosphorus (P) availability is a key limiting factor for primary productivity in the oceans. Atmospheric particles, such as wildfire ash, supply the oceans with substantial amounts of nutrients such as P. The solubility of P from aerosol particles, especially from wildfire ash, plays a critical role in oceanic nutrient cycles and may significantly impact the biological carbon pump, a key mechanism for atmospheric CO₂ regulation.

As ocean acidification continues and wildfires are projected to increase in intensity and severity with climate change, understanding how changes in seawater pH influence P release from wildfire ash is essential. This study aims to investigate the effect of past, present, and future seawater pH levels on P solubility from different wildfire ash under controlled laboratory conditions. Specifically, the study aims to examine how elevated CO₂ levels, leading to lower pH (ocean acidification), impact the availability of P in wildfire ash compared to lower CO₂ levels.

Using artificial seawater and ash samples derived from Mediterranean and agricultural vegetation, this research will analyze P release patterns under a range of CO₂ concentrations, encompassing current levels, future projections, and historical baselines.

Preliminary results demonstrated a significant dependence of P release from wildfire ash on pCO₂ concentrations and its influence on the pH. Elevated CO₂ levels of the projected future and of ancient atmosphere enhanced P solubility in both Mediterranean vegetation and agricultural vegetation treatments while reduced levels of the preindustrial and pre-Holocene periods decreased P solubility. These findings are anticipated to shed light on the role of wildfire ash in marine nutrient dynamics and its broader impact on ocean productivity and the global carbon cycle, especially in regions experiencing increasing wildfire activity.

These initial findings lay the groundwork for continued research, where I will investigate the cultivation of microalgae under controlled laboratory conditions at varying atmospheric CO2 concentrations. The research will focus on understanding how P release from wildfire ash, influenced by different CO2 levels, impacts the growth rate of phytoplankton. The experiments will assess the role of wildfire ash as a potential P source for phytoplankton grown in P-depleted water.

How to cite: Naiman, N., Gross, A., and Antler, G.: The Effect of Ocean Acidification on Phosphorus Solubility from Wildfire Ash and its Role in Enhancing the Biological Carbon Pump, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5059, https://doi.org/10.5194/egusphere-egu25-5059, 2025.

EGU25-5221 | ECS | Posters on site | AS2.5

Evaluation of Arctic Ocean surface carbon fluxes from Atmospheric Inverse Analysis   

Jayashree Ghosh, Parvadha Suntharalingam, and Zhaohui Chen

Atmospheric inverse analyses use optimization methods to calculate surface CO2 fluxes using atmospheric transport models in combination with observed gradients in atmospheric CO2 concentration. In our present study we present an inverse estimate of Arctic Ocean air-sea CO2 fluxes using the GEOSChem–LETKF  system; this system has previously been used to derive estimates of regional North Atlantic CO2 fluxes (Chen et al. 2021). Our analysis reports on estimates of Arctic Ocean fluxes  and assesses patterns of spatial and inter-annual variability.  Our results indicate significant spatial variability of air-sea CO2 fluxes in the different regional seas of the Arctic Ocean. The western Arctic Ocean predominantly act as a sink region for atmospheric CO2.  However,  the eastern Arctic Ocean act more as a source of CO2 . We also present results of sensitivity analyses conducted to assess the impact of alternate ocean prior flux specifications.

How to cite: Ghosh, J., Suntharalingam, P., and Chen, Z.: Evaluation of Arctic Ocean surface carbon fluxes from Atmospheric Inverse Analysis  , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5221, https://doi.org/10.5194/egusphere-egu25-5221, 2025.

The equatorial Pacific serves as the largest oceanic source of CO2. The contrasting ocean environment in the eastern (i.e., upwelling) and western (i.e., warm pool) regions makes it difficult to fully characterize the CO2 dynamics with limited in situ observations.  In this study, we addressed this challenge using monthly surface partial pressure of CO2 (pCO2sw) and air–sea CO2 fluxes (FCO2) data products reconstructed from satellite and reanalysis data at spatial resolution of 1°×1° in the period of 1982–2021. We found that, during the very strong El Niño events (1997/1998, 2015/2016), both pCO2sw and FCO2 showed significant decrease of 41–58 μatm and 0.5–0.8 mol m-2 yr-1 in the eastern equatorial Pacific, yet remained at normal levels in the western equatorial Pacific. In contrast, during the very strong La Niña events (1999/2000, 2007/2008, and 2010/2011), both pCO2sw and FCO2 showed strong increase of 40–48 μatm and 1.0–1.4 mol m-2 yr-1 in the western equatorial Pacific, yet with little change in the eastern equatorial Pacific. In the past 40 years, pCO2sw in the eastern equatorial Pacific was increasing at a higher rate (2.32–2.51 μatm yr-1) than that in the western equatorial Pacific (1.75 μatm yr-1), resulting in an accelerating CO2 outgassing (at rate of 0.03 mol m-2 yr-2) in the eastern equatorial Pacific. We comprehensively analyzed the potential effects of different factors such as sea surface temperature, sea surface wind speed, and ΔpCO2 in driving CO2 fluxes in the equatorial Pacific, and found that ΔpCO2 had the highest correlation (R ≥ 0.80, at p ≤ 0.05), highlighting the importance of accurate estimates of pCO2sw from satellites. 

How to cite: Chen, S.: Accelerating CO2 outgassing in the equatorial Pacific from sat-ellite remote sensing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5360, https://doi.org/10.5194/egusphere-egu25-5360, 2025.

EGU25-7196 | Posters on site | AS2.5

Laboratory simulation of ocean-atmosphere CO2 exchange 

Brian Durham and Christian Pfrang

At EGU2024 we presented initial laboratory results from bubbling a simulated pre-industrial atmosphere through samples of freshwater and seawater across a range of temperatures, making comparison with literature values for the CO2/water partition equilibrium as determined at a higher partial pressures of the gas as reviewed by Carroll et al 1991.

Two changes have been made. Our 2024 results were based on a temperature range of 0.1’C to 16.5’C, and following valued discussion with Raphael Hebert we have brought that range closer to the global average ocean temperature range since the 1940s hockey-stick, i.e. 15’C to 16.5’C. At the same time, in addressing whether last year’s `paradox’ and `slow-release’ were artefacts of laboratory simulation, we test whether changes in CO2 fraction as measured in the headspace have a reciprocal effect in the liquid phase, measured by a continuous-reading conductivity probe in each flask.

Two recent papers are of relevance within this temperature range. Firstly the Universities of Exeter and Plymouth, UK, report transects in the Atlantic Ocean and note that temperature gradients near the ocean surface will affect the proportion of atmospheric CO2 taken into solution (D Ford et al `Enhanced ocean CO2 uptake due to near-surface temperature gradients’, Nature Geoscience (Sept 2024).  They conclude that `accounting for near-surface temperature gradients would increase estimates of global ocean CO2 uptake.’  In parallel the University of East Anglia, UK, finds ‘that process-based models underestimate the amplitude of the decadal variability in the ocean CO2 sink, but that observation-based products on average overestimate the decadal trend in the 2010s. (N Mayot et al `Constraining the trend in the ocean CO2 sink during 2000–2022’ Nature Communications, September 2024)

We understand from Raphael Hebert (pers. comm.) that the Alfred Wegener Institute, Germany, is also investigating this issue using a different approach, hence our interest in confirming the partition constant at relevant partial pressures, as a fourth contribution.

How to cite: Durham, B. and Pfrang, C.: Laboratory simulation of ocean-atmosphere CO2 exchange, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7196, https://doi.org/10.5194/egusphere-egu25-7196, 2025.

EGU25-7519 | Posters on site | AS2.5

Estimation of Arctic Air-Sea CO2 Fluxes by Inverse Methods: Use of OSSEs to Assess Atmospheric Sampling Strategies  

Parvadha Suntharalingam, Jayashree Ghosh, and Zhaohui Chen

Estimates of atmospheric CO2 uptake by the Arctic Ocean over recent decades from multiple methods indicate accelerating regional carbon uptake (Yasunaka et  al. 2024). This trend is  attributed to such factors as regional climate-change impacts and associated sea-ice loss. Yasunaka et al. (2024) also note a significant range of uncertainty among the various model and data analysis methods that were employed to derive regional Arctic Ocean air-sea fluxes (e.g., from surface ocean pCO2 products, ocean biogeochemical models, and atmospheric inversions). This highlights a need for more robust  flux estimation methods  involving expanded observational networks and improved modelling tools to enable more accurate quantification of regional fluxes and an improved prediction capability to estimate future changes in oceanic CO2 uptake in the rapidly evolving Arctic.

In this analysis we employ the GEOSChem-Local Ensemble Transform Kalman Filter  inverse analysis system (Chen et al. 2021) to develop sets of Observing System Sampling Experiments (OSSEs) that assess alternative atmospheric CO2 sampling strategies and observational network extensions towards improved estimates of Arctic Ocean air-sea CO2 fluxes. We assess the performance of individual sampling strategies using a range of metrics applied to the atmospheric inversions; these include regional CO2 flux error reductions  and model concentration biases at sampling sites.

How to cite: Suntharalingam, P., Ghosh, J., and Chen, Z.: Estimation of Arctic Air-Sea CO2 Fluxes by Inverse Methods: Use of OSSEs to Assess Atmospheric Sampling Strategies , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7519, https://doi.org/10.5194/egusphere-egu25-7519, 2025.

EGU25-8419 | ECS | Posters on site | AS2.5

Investigating Volatile Organic Compound Emissions from Ozonolysis of Phytoplankton Cultures 

Charlotte Stapleton, Rebecca Fenselau, Vaishnavi Padaki, Audrey Lyp, Kimberly Halsey, Lucy Carpenter, and Timothy Bertram

The ocean’s surface is covered by the sea-surface microlayer (SML), a distinct boundary layer that plays a critical role in mediating the air-sea exchange of atmospheric trace gases. The oxidation of unsaturated organic material enriched in the SML by ozone is a significant but poorly quantified abiotic mechanism leading to the emission of volatile organic compounds (VOCs) into the marine boundary layer. The properties of these VOCs make them efficient precursors for secondary organic aerosol formation which can alter the oxidative capacity of the atmosphere. 

In this laboratory study, axenic cultures of the model marine diatom Phaeodactylum tricornutum and its coculture with Yoonia bacteria were selected as biologically and chemically relevant proxies for the SML. Ozone-enriched air was passed over the culture medium in a heterogenous flow reactor, and the emitted gas-phase VOCs were monitored using high resolution proton-transfer-reaction time-of-flight mass spectrometry (PTR-ToF-MS). Experiments were conducted on the cultures in both their exponential and stationary growth phases with nonanal, the C5H8H+ peak, and the C6H10H+ peak being identified as major product ions. Ozonolysis-mediated abiotic VOC emissions were greater from cultures in exponential phase compared to stationary phase. Additionally, emissions from the P. tricornutum axenic monoculture were higher than from the P. tricornutum-Yoonia coculture indicating consumption of precursor compounds by the bacteria. The addition of iodide, a well-known reactant with ozone, to axenic P. tricornutum cultures in the exponential phase was associated with a reduction in the VOC emissions. This research provides a deeper insight into the interactions between iodide and organics during ozone uptake to the SML, and the impact of these competing processes on marine atmospheric chemistry. 

How to cite: Stapleton, C., Fenselau, R., Padaki, V., Lyp, A., Halsey, K., Carpenter, L., and Bertram, T.: Investigating Volatile Organic Compound Emissions from Ozonolysis of Phytoplankton Cultures, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8419, https://doi.org/10.5194/egusphere-egu25-8419, 2025.

EGU25-10303 | ECS | Posters on site | AS2.5

Chemical Drivers of Oceanic Ozone Uptake – Iodide vs Surfactants 

Lucy Brown, David Loades, Charlotte Stapleton, Will Drysdale, Matthew Jones, Rosie Chance, Pascale Lakey, Manabu Shiraiwa, Ming-Xi Yang, Tom Bell, Ian Brooks, Andrew Peters, Rod Johnson, Paul Lethaby, Birgit Quack, and Lucy Carpenter

Due to its position at the air-sea interface, the sea-surface microlayer (SML) modulates the exchange of gases, including the deposition of ozone to the ocean. While ozone deposition to the ocean is a large sink of ozone from the troposphere, the processes involved are not well understood. Previous work has focussed on seawater iodide as a driver of ozone uptake to the ocean, however the SML contains a complex mixture of organic material, which could also impact ozone uptake. The contribution of this organic material to ozone uptake remains particularly unclear.

During this project, ozone uptake to seawater was measured by eddy covariance from coastal towers near Penlee Point (Plymouth, UK) and Tudor Hill (Bermuda), and at sea aboard the RV Atlantic Explorer, operating at and around the Bermuda Atlantic Time-series Study site in the Sargasso Sea. Additionally, the chemical component of ozone uptake to seawater was measured using a flow reactor during a trans-Atlantic cruise. This suite of observations has been combined to investigate the driving forces of oceanic ozone uptake. We present data that demonstrate that iodide was not a strong predictor of ozone uptake, despite its fast chemical reaction with ozone and the ubiquitous presence of iodide in the surface ocean.

Organic compounds in the SML are of interest to this work because some organic compounds have ozone-reactive functional groups. An example of this is carbon-carbon double bonds, present in some oceanic fatty acids. By increasing chemical reactivity, organic material can therefore augment ozone uptake to the ocean. The contribution of chemical reactions between ozone and organic material to ozone uptake was investigated using the kinetic multilayer model of surface and bulk chemistry (KM-SUB). A simplified system of a monolayer of an unsaturated fatty acid (oleic acid) over seawater was modelled and demonstrated that a monolayer of ozone-reactive surfactants on the ocean surface could contribute substantially more to ozone uptake, compared to environmental levels of aqueous iodide.

This work indicates that the commonly applied iodide-based parameterisation for ozone uptake to seawater may not accurately represent the chemical processes involved in ozone deposition to the sea surface. This has implications not only for predicted spatial and temporal variations in the magnitude of ozone deposition, but also for the chemical profile of oxidised gases emitted from the sea surface to the remote marine troposphere.

How to cite: Brown, L., Loades, D., Stapleton, C., Drysdale, W., Jones, M., Chance, R., Lakey, P., Shiraiwa, M., Yang, M.-X., Bell, T., Brooks, I., Peters, A., Johnson, R., Lethaby, P., Quack, B., and Carpenter, L.: Chemical Drivers of Oceanic Ozone Uptake – Iodide vs Surfactants, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10303, https://doi.org/10.5194/egusphere-egu25-10303, 2025.

EGU25-10513 | ECS | Posters on site | AS2.5

Evaluating Methane Emissions and Sea-Air Fluxes in the Southern Ocean 

Evelyn Workman, Anna Jones, Rebecca Fisher, James France, Katrin Linse, Ming-Xi Yang, Thomas Bell, Bruno Delille, Freya Squires, and Yuanxu Dong

The ocean is generally thought to be a small source of atmospheric methane. However, the contribution of the Southern Ocean remains poorly quantified due to its remoteness and lack of measurements. In this study we investigate sea-air methane fluxes in the Southern Ocean measured by two different methods, bulk flux and eddy-covariance, to better understand the region's role in global methane emissions. We focus on both on-shelf and off-shelf areas, including regions where methane seeps from the seabed into the water column, using several years of ship-based measurements.

Our results show that coastal and on-shelf regions of the Southern Ocean, including areas with known seabed seeps, act as small sources of methane to the atmosphere. This is possibly driven by methane produced at the seabed reaching the surface or inputs from terrestrial sources, such as subglacial discharge. We also find possible indications of increased methane release from coastal areas compared to previous studies. Given the potential for increased methane release from these regions in the future under a warming climate, our findings emphasise the importance of ongoing monitoring in the Southern Ocean to quantify its contribution to the global methane cycle and track any changes over time.

Open ocean sea-air methane flux measurements in the Scotia and Weddell Seas during consecutive Antarctic summers revealed a source and a sink of methane depending on the method used (bulk flux or eddy-covariance). As these measurements techniques were not deployed simultaneously, a dedicated measurement campaign is necessary to collect parallel data and better understand whether the observed differences reflect measurement technique variability or potential changes in the Southern Ocean system.

How to cite: Workman, E., Jones, A., Fisher, R., France, J., Linse, K., Yang, M.-X., Bell, T., Delille, B., Squires, F., and Dong, Y.: Evaluating Methane Emissions and Sea-Air Fluxes in the Southern Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10513, https://doi.org/10.5194/egusphere-egu25-10513, 2025.

EGU25-11404 | ECS | Posters on site | AS2.5

North Atlantic fjords are minor sources of nitrous oxide to the atmosphere 

Tobia Politi, Yvonne Y. Y. Yau, Isaac Santos, Alex Cabral, Henry L. S. Cheung, Claudia Majtényi-Hill, Adam Ulfsbo, Anna Wåhlin, and Stefano Bonaglia

Nitrous oxide (N2O) distribution and dynamics in high latitude fjords are relatively unknown. Surface water N2O concentrations were measured in six fjords located in Sweden, Iceland, and Greenland, which represent highly diverse environmental conditions in terms of oxygen, eutrophication and climate. This study provides one of the few high spatial resolution observations of N2O sea-air fluxes currently available in fjords. The two Icelandic fjords showed highest emissions (97.6±10.5 μg N2O m⁻² day⁻¹), likely driven by aquaculture-induced nutrient enrichment and not fully oxygenated subsurface waters. The three Swedish fjords, characterized by inputs from nutrient-rich rivers and by poor water circulation, exhibited relatively high N2O emissions averaging 19.9±19.3 μg N2O m⁻² day⁻¹, with subsurface water anoxia enhancing emissions in By Fjord (64.4±24.0 µg N2O m⁻² day⁻¹). In contrast, the Greenland fjord displayed net N2O uptake (–8.3±7.8 μg N2O m⁻² day⁻¹), likely due to glacier meltwater dilution. Each fjord appeared to be influenced by distinct N2O drivers, including temperature, salinity, chlorophyll, and pH, but no single, unifying driver was found across all fjords. As a preliminary global upscaling effort, we integrated our measured fluxes from six fjords with literature data from thirteen additional fjords. We estimate that global fjords emit 7.9±1.7 Gg N2O yr⁻¹, accounting for 2–13% of global coastal ecosystem emissions and do not significantly offset (3.5%) CO₂ sequestration in fjords. These findings underscore the role of fjords in greenhouse gas dynamics and highlight the need for further spatial and seasonal studies to refine global N2O emissions from coastal ecosystems.

How to cite: Politi, T., Yau, Y. Y. Y., Santos, I., Cabral, A., Cheung, H. L. S., Majtényi-Hill, C., Ulfsbo, A., Wåhlin, A., and Bonaglia, S.: North Atlantic fjords are minor sources of nitrous oxide to the atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11404, https://doi.org/10.5194/egusphere-egu25-11404, 2025.

EGU25-12341 | ECS | Posters on site | AS2.5

Greenhouse Gas Dynamics in Coastal Ecosystems: Insights from the Baltic Sea and Auckland, New Zealand 

Julika Zinke, Matthew Salter, Martijn Hermans, Alexis Armando Fonseca Poza, Joakim Hansen, Linda Kumblad, Emil Rydin, Sofia A. Wikström, Alf Norkko, Nicolas-Xavier Geilfus, Anna Villnäs, Simon Thrush, Marc Geibel, and Christoph Humborg

Coastal ecosystems play a significant role in the cycling of greenhouse gases (GHGs), yet they remain understudied compared to open oceans and terrestrial systems. Here, we present measurements of carbon dioxide (CO₂), methane (CH₄), and nitrous oxide (N₂O) concentrations from shallow coastal environments along the Swedish Baltic Sea coast and Auckland, New Zealand, highlighting the variability and drivers of GHG dynamics across diverse habitats.

In the Baltic Sea, we conducted measurements in April and September 2024, utilizing cavity ring-down spectroscopy coupled with a water equilibration system. Our focus was on shallow coastal bays in the wider Stockholm archipelago, including eutrophic and habitat-altered bays. These environments exhibited exceptionally high CH₄ concentrations in the surface water reaching up to 580 nmol L-1, suggesting the potential for significant CH₄ emissions. Notably, CH₄ concentrations below 200 nmol L-1 showed a negative correlation with N₂O, while CH₄ levels above 200 nmol L-1 revealed a distinct shift to a positive correlation with N₂O. We hypothesize that this transition reflects a change in oxygen availability, where hypoxic conditions (0.2< O2 < 2 mL L-1) favor CH₄ production and reoxygenation of euxinic sediments contributes to an additional late-summer N₂O peak. Furthermore, GHG concentrations in the surface seawater were associated with environmental parameters such as water retention time, vegetation coverage, total organic carbon content, turbidity, chlorophyll-a concentration, pH, and total phosphorus levels.

Expanding our investigation to coastal systems in the suburban regions of Auckland, New Zealand, in January 2025 we conducted a spatial survey across a range of coastal habitats, including tidal flats, mangroves and river estuaries. By linking the findings from the Baltic Sea with emerging insights from New Zealand’s coastal systems, we aim to better understand the influence of habitat type, redox conditions, and nutrient dynamics on GHG emissions in coastal zones globally.

Our comparative study underscores the need for integrated approaches to better understand GHG emissions in coastal zones, which are often subject to compounded anthropogenic pressures, such as excessive nutrient inputs and habitat alteration. These findings contribute to the broader understanding of coastal zones as dynamic interfaces in the global carbon and nitrogen cycles and the development of evidence-based policies.

How to cite: Zinke, J., Salter, M., Hermans, M., Fonseca Poza, A. A., Hansen, J., Kumblad, L., Rydin, E., Wikström, S. A., Norkko, A., Geilfus, N.-X., Villnäs, A., Thrush, S., Geibel, M., and Humborg, C.: Greenhouse Gas Dynamics in Coastal Ecosystems: Insights from the Baltic Sea and Auckland, New Zealand, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12341, https://doi.org/10.5194/egusphere-egu25-12341, 2025.

EGU25-12512 | Posters on site | AS2.5

Nitrous oxide from three temperate estuaries discharging in the North Sea: No estuary is like another  

Kirstin Dähnke, Gesa Schulz, Louise Rewrie, Vlad Macovei, Yoana Voynova, Andreas Neumann, and Tina Sanders

Estuaries are potential sources for the important greenhouse gas nitrous oxide (N2O). Estuaries are among the most complex ecosystems in the world with biogeochemical processes occurring on a range of spatial and temporal scales, depending on geomorphology, tides, and discharge patterns. Due to the high spatiotemporal variability and limited data availability, N2O emissions from estuaries are associated with significant uncertainty, presenting a big challenge for the global N2O emission estimates and budgeting of coastal regions.

This study presents N2O measurements from three temperate German estuaries discharging into the North Sea: Ems, Weser and Elbe, which are all heavily affected by anthropogenic impacts. During a cruise in September 2024, N2O dry mole fractions were measured continuously using an analyzer based on off-axis integrated cavity output (Picarro G2508) absorption spectroscopy coupled with an equilibrator system. For calibration and quality control, distinct water samples were taken in 30-min intervals and preserved for later GC analysis. Based on these measurements, we calculated N2O concentrations and fluxes.

Preliminary results showed N2O oversaturation with distinct peaks observed along the salinity gradient of all three estuaries. The N2O concentration in the Weser estuary was nearly double the concentration recorded in the Ems and Elbe estuaries. The high variability in N2O concentration between the three estuaries indicated potential differences in dominating biological and biogeochemical processes that modulate N2O production in each estuary. We suspect that turbidity, organic matter quality and degradation, as well as nutrient availability are responsible for the observed differences between the estuaries, which all are heavily impacted by anthropogenic river alterations. Therefore, we aim to elucidate the impact of human alterations on N2O production and emissions in these temperate estuaries. Overall, our findings highlight the variability of N2O emissions depending on stream morphology and chemistry, emphasizing the urgent need for comprehensive measurement programs to ensure accurate emission estimates.

How to cite: Dähnke, K., Schulz, G., Rewrie, L., Macovei, V., Voynova, Y., Neumann, A., and Sanders, T.: Nitrous oxide from three temperate estuaries discharging in the North Sea: No estuary is like another , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12512, https://doi.org/10.5194/egusphere-egu25-12512, 2025.

EGU25-12549 | ECS | Orals | AS2.5

Physicochemical properties of nascent versus aged sea spray aerosol – A study from the eastern North Atlantic Ocean  

Sneha Aggarwal, Olga Garmash, Julika Zinke, Delaney Kilgour, Jian Wang, Timothy Bertram, Joel Thornton, Matt Salter, Paul Zieger, and Claudia Mohr

Sea spray aerosol (SSA), produced by bubble bursting at the ocean's surface, plays a critical role in climate regulation and atmospheric chemistry. It also provides a unique microenvironment for gas-to-particle partitioning and aqueous-phase reactions. Understanding these processes requires a detailed examination of the physicochemical properties and the transformations of SSA during atmospheric aging. 
Hence, we designed a comprehensive experimental setup comprising a sea spray simulation tank for generating SSA, a chemical ionization mass spectrometer (CIMS) for analyzing molecular-level composition, an oxidation flow reactor (PAM) for simulating atmospheric oxidation, and a differential mobility particle counter (DMPS) for determining particle size distribution. We deployed this setup in May 2022 during the AGENA campaign on Graciosa Island in the Azores, Portugal, a remote marine site. We collected surface ocean water samples from the Atlantic, and generated SSA using a plunging jet. We used DMPS and CIMS to analyze physicochemical properties of SSA present in the tank headspace, and also collected filter samples for offline CIMS analysis. 
Our results revealed significant particle formation in the PAM chamber at an aging period equivalent to 3–3.5 days in the atmosphere. Notably, the increase was primarily restricted to particles below 100 nm, suggesting that new particle formation dominated over condensation in the PAM environment, likely due to high oxidant concentrations. This observation also indicates the presence of numerous volatile organic compounds (VOCs) in the nascent SSA, which may have condensed onto pre-existing particles in natural settings. Further analysis of the VOCs using CIMS showed that nascent SSA contained compounds with longer carbon chains (1–16 carbons) and higher oxidation states, indicating low volatility. In contrast, gases exiting the PAM chamber exhibited shorter carbon chains (1–10 carbons) and lower oxidation levels, suggesting condensation of oxidation products onto newly formed particles within the reactor. Additionally, we identified oxidation products of dimethyl sulfide (DMS), such as dimethyl sulfoxide (DMSO) and methanesulfonic acid (MSA), in both nascent and aged samples. Intriguingly, nascent SSA also exhibited strong signals for fluorinated compounds, including hydrofluoric acid, likely formed from protonation of fluoride ions (F⁻) and other fluoride-containing salts like MgF⁺, CaF⁺, and NaF⁺ found in sea salt. These findings provide valuable insights into the molecular composition and dynamic behaviour of SSA, with implications for understanding its role in atmospheric processes and climate.

How to cite: Aggarwal, S., Garmash, O., Zinke, J., Kilgour, D., Wang, J., Bertram, T., Thornton, J., Salter, M., Zieger, P., and Mohr, C.: Physicochemical properties of nascent versus aged sea spray aerosol – A study from the eastern North Atlantic Ocean , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12549, https://doi.org/10.5194/egusphere-egu25-12549, 2025.

EGU25-12999 | Posters on site | AS2.5

A 25-year record of atmospheric deposition of iron speciation in the East Mediterranean: The impact of pH 

Maria Kanakidou, Maria Tsagkaraki, and Nikolaos Mihalopoulos

A 25-year record of wet deposition has been collected and analysed for Fe(II), soluble iron (DSRFe) and total Iron (Fe) at Finokalia station on Crete island in the East Mediterranean from 1997 to 2022. A significant temporal increase in rain pH values is observed, mainly due to the reduction in sulfur concentrations. Regardless of the pH value of the rain, the Fe(II)/DSRFe ratio appeared to remain always above 50%, indicating that a significant amount of Fe(II), hence bioavailable iron, enters the sea surface via rain. However, Fe(II)/DSRFe ratio gradually decreases from 0.70 to 0.52 with increasing pH until pH 7.0, while from pH 7.0 and above it increases again, reaching an average value of about 0.67 at very basic pH levels. This is related to the general decrease in Fe solubility with increasing pH and the respective association of the forms in which Fe(II) and Fe(III) exist. It is therefore evident that the observed increase in pH in wet deposition affects the amount of dissolved iron deposited in the oceans, particularly Fe(II), that is directly bioavailable to the marine ecosystem, with consequent impacts on marine productivity.

How to cite: Kanakidou, M., Tsagkaraki, M., and Mihalopoulos, N.: A 25-year record of atmospheric deposition of iron speciation in the East Mediterranean: The impact of pH, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12999, https://doi.org/10.5194/egusphere-egu25-12999, 2025.

EGU25-13484 | Orals | AS2.5

Evidence of seasonal carbon dioxide uptake by the Southern Ocean from a 10-year record of atmospheric carbon dioxide, observed from coastal Antarctica.  

Freya Squires, Anna Jones, Tony Phillips, Zsofia Juranyi, Rolf Weller, and James France

The Southern Ocean plays a critical role in modulating excess atmospheric carbon dioxide, accounting for roughly 40% of global ocean anthropogenic CO2 uptake since industrialisation. Given its significance in the global carbon cycle, understanding the Southern Ocean carbon sink is important but studies show high uncertainties in the magnitude and evolution of this carbon sink. The Southern Ocean is a remote and challenging region to measure, and the resulting sparsity of observational data is the main cause of uncertainty in air-sea carbon flux in the region. Long term, high-temporal-frequency data sets especially are rare for the Southern Ocean, but these can give valuable insights into the carbon cycle processes occurring in the region.

This work presents ten years of high-temporal-frequency in situ atmospheric carbon dioxide mixing ratios measured from two coastal Antarctic research stations; Halley, operated by the British Antarctic Survey, and the German research station, Neumayer. The coastal location of these stations means they are ideally placed to explore air-sea CO2 exchange over the Southern Ocean. 

Both the Halley and Neumayer records show short-term fluctuations in CO2 mixing ratios during austral summer, with over ~0.5 ppm decreases in CO2 sometimes observed over the course of a day - about one fifth of the average annual growth rate (~2.4 ppm per year-1 for this 10-year record). Analysis of air mass trajectories reveal that these fluctuations in CO2 occur when the sampled air has spent considerable time in contact with the Southern Ocean, suggesting CO2 uptake has occurred, leading to the reduced CO2 mixing ratios observed.

We present an in-depth analysis of the drivers of the short-term variability observed during austral summer, including the role of mixing height, sea-ice coverage, wind speed and biology. Observational data represent an important tool with which to tease out key factors determining Southern Ocean CO2 uptake, and thus in assessing how uptake may evolve in the future.

How to cite: Squires, F., Jones, A., Phillips, T., Juranyi, Z., Weller, R., and France, J.: Evidence of seasonal carbon dioxide uptake by the Southern Ocean from a 10-year record of atmospheric carbon dioxide, observed from coastal Antarctica. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13484, https://doi.org/10.5194/egusphere-egu25-13484, 2025.

EGU25-13680 | ECS | Posters on site | AS2.5

Understanding the drivers of the air-sea CO2 flux seasonal variability in the upwelling systems off Peru and Baja California 

Angela Bahamondes Dominguez, Boris Dewitte, Ivonne Montes, Veronique Garçon, Victor Aguilera, Linda Barranco, and Matthew Hammond

The open ocean plays a critical role in mitigating climate change by absorbing approximately 25% of annual anthropogenic carbon dioxide (CO₂). In contrast, Eastern Boundary Upwelling Systems (EBUSs) are net sources of CO2, primarily due to the high concentrations of dissolved inorganic carbon (DIC) from upwelled waters. However, the carbon dynamics in EBUSs exhibit significant variability, both temporally and spatially, with differences between systems. This study focuses on two Pacific Ocean EBUSs with distinct physical characteristics: the upwelling systems off Peru and off Baja California, where the relative contribution of  Ekman transport and pumping, and geostrophic compensation to upwelling differ. Based on seasonal simulations of a regional biogeochemical model configured for the two regions, we characterise the seasonal variability of CO₂ fugacity (FCO₂) in these systems, and identify the processes driving this variability through a Taylor expansion of the flux formulation. Our results show that FCO₂ is highly dynamic and exhibits notable spatial variability. The processes influencing FCO₂ seasonality differ between subregions. Off Peru, the primary drivers of FCO₂ seasonal variability are: the oceanic partial pressure of CO₂ (pCO₂), primarily influenced by changes in DIC, and alongshore winds (Ekman transport). Similarly, off Baja California, changes in pCO₂ are the dominant contributor to the FCO₂ seasonality, with DIC and sea surface temperature (SST) also playing significant roles. This comparative analysis deepens our understanding of how large-scale climate processes shape FCO₂ dynamics, offering valuable insights for interpreting future changes in CO2 fluxes within EBUSs.

How to cite: Bahamondes Dominguez, A., Dewitte, B., Montes, I., Garçon, V., Aguilera, V., Barranco, L., and Hammond, M.: Understanding the drivers of the air-sea CO2 flux seasonal variability in the upwelling systems off Peru and Baja California, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13680, https://doi.org/10.5194/egusphere-egu25-13680, 2025.

EGU25-15135 | ECS | Orals | AS2.5

Global Oceanic Nitrogen Deposition under Future Emission Pathways and Responses to Nitrogen Emission Reductions 

Jialin Deng, Yixin Guo, lin Zhang, Ni Lu, Xingpei Ye, Yuanhong Zhao, Jiayu Xu, and Xiaolin Wang

Oceanic nitrogen deposition influences marine ecosystem eutrophication and the global carbon cycle. Its future global spatiotemporal features still remain unclear driven by changing anthropogenic emissions. Furthermore, existing studies reported air quality and climate benefits of ambitious nitrogen emission reductions, while consequent impacts for global marine ecosystems through atmospheric nitrogen deposition are unexplored. Here we utilize the global atmospheric chemistry transport model GEOS-Chem to evaluate changes in global oceanic nitrogen deposition between 2015 and 2050 under three CMIP6 SSP-RCP emission scenarios and its responses to multiple levels of NH3 and NOx emission reductions. We find that global oceanic nitrogen deposition is projected to change by −24%-+6% between 2015-2050, with a substantially increasing share contributed by NHx-N across all scenarios. Coastal regions respond much more drastically to nitrogen emission reductions than open ocean areas. Ocean carbon sink related to nitrogen-contributed marine primary productivity is projected to decrease from 290 Tg C in 2015 to 222 Tg C (-23%) in SSP1-RCP2.6 scenario in 2050, posing challenges to climate mitigation and affecting global carbon budget. Our findings highlight nitrogen management and the overlooked climate mitigation impacts on marine ecosystems through atmospheric nitrogen deposition and call for increasing attention for holistic assessments of nitrogen management impacts on air, terrestrial and ocean systems.

How to cite: Deng, J., Guo, Y., Zhang, L., Lu, N., Ye, X., Zhao, Y., Xu, J., and Wang, X.: Global Oceanic Nitrogen Deposition under Future Emission Pathways and Responses to Nitrogen Emission Reductions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15135, https://doi.org/10.5194/egusphere-egu25-15135, 2025.

EGU25-15375 | ECS | Orals | AS2.5

Characterizing marine atmospheric VOC diversity and fluxes using PTR-TOF-MS measurements in the Baltic Sea 

Mehrshad Foroughan, Thomas Holst, Lauri Laakso, Heidi Hellén, Jukka Seppälä, Kaisa Kraft, Ken Stenbäck, Mika Aurela, and Riikka Rinnan

We present continuous measurements of volatile organic compounds (VOCs) and their fluxes in the marine atmospheric boundary layer using proton‐transfer‐reaction time‐of‐flight mass spectrometry (PTR-TOF-MS) coupled with a sonic anemometer for direct eddy covariance measurements at the Utö Atmospheric and Marine Research Station in the Baltic Sea. The measurements, conducted from July to September 2024, identified over 200 distinct masses corresponding to a diverse array of volatile compounds, representing a comprehensive characterization of marine VOC composition. Our experimental setup combines VOC mixing ratio and flux measurements with concurrent monitoring of physical and biogeochemical parameters, providing a unique dataset for understanding air-sea gas exchange processes. Preliminary principal component analysis reveals strong correlations between VOC mixing ratio variability and key parameters including water-side pCO2, dissolved oxygen concentration, and air temperature, suggesting complex biogeochemical controls on VOC emissions. The high temporal resolution and sensitivity of the PTR-TOF-MS, combined with direct flux measurements, enables detailed investigation of both abundant and trace VOC species, their diurnal patterns, and their response to varying environmental conditions. This comprehensive dataset will provide valuable insights into the complexity of VOC emissions in marine environments and their coupling with biological and physical processes in the Baltic Sea region.

How to cite: Foroughan, M., Holst, T., Laakso, L., Hellén, H., Seppälä, J., Kraft, K., Stenbäck, K., Aurela, M., and Rinnan, R.: Characterizing marine atmospheric VOC diversity and fluxes using PTR-TOF-MS measurements in the Baltic Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15375, https://doi.org/10.5194/egusphere-egu25-15375, 2025.

EGU25-15858 | ECS | Orals | AS2.5

Compensatory Mechanisms Reduce ENSO-driven Nitrous Oxide Emission Variability in the Eastern Tropical Pacific 

Jana Härri, Daniel McCoy, Meike Vogt, Daniele Bianchi, and Nicolas Gruber

Nitrous oxide (N2O) is a potent greenhouse gas, with the Eastern Tropical Pacific (ETP) being a hotspot of N2O emissions due to high N2O production in the oxygen minimum zones (OMZs). However, N2O emissions in this region remain poorly constrained due to (i) temporal variability, which is hypothesized to be largely driven by the El Niño-Southern Oscillation (ENSO), and (ii) limited process understanding. To address these shortcomings and improve the quantification of N2O emissions and ENSO-driven variability in the ETP, we run a regional ocean model on a telescopic grid (~4km), spanning the entire Pacific Ocean, from 1979 to 2019. The model includes a biogeochemical model and a novel nitrogen module (NitrOMZ), which explicitly resolves the N2O production via incomplete denitrification and ammonium oxidation and accounts for the different oxygen inhibition thresholds of these biological N2O production pathways. We find that 1 Tg N of N2O is emitted annually in the ETP, and that N2O emissions deviate up to ±0.18 Tg N y-1 from the mean during ENSO events across the entire ETP, with La Niña increasing N2O emissions and El Niño decreasing them. Most of the ENSO-driven N2O emission anomalies can be attributed to variability in incomplete denitrification in the oxyclines of the oxygen minimum zones. Compensatory effects among gross N2O production, consumption, and transport reduce both the total N2O emissions and their interannual variability by an order of magnitude. Our results alleviate previously raised concerns that La Niña events may substantially amplify N2O emissions. Such compensatory mechanisms might also reduce N2O emissions in other OMZs and mitigate the impact of climate change on N2O emissions, provided that compensatory mechanisms remain effective in the future.

How to cite: Härri, J., McCoy, D., Vogt, M., Bianchi, D., and Gruber, N.: Compensatory Mechanisms Reduce ENSO-driven Nitrous Oxide Emission Variability in the Eastern Tropical Pacific, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15858, https://doi.org/10.5194/egusphere-egu25-15858, 2025.

EGU25-17040 | Posters on site | AS2.5

Advancing predictions of Dimethylsulfide emissions and biogenic sulfur aerosol in the Mediterranean region via machine learning 

Matteo Rinaldi, Stefano Decesari, Marco Paglione, Silvia Becagli, and Karam Mansour

Dimethylsulfide (DMS) is the main natural source of atmospheric sulfur and plays a critical role in marine aerosol formation (Mansour et al., 2020b; Mansour et al., 2020a; O'Dowd et al., 2004). It influences cloud radiative forcing, with feedback on regional and global climate (Charlson et al., 1987; Mansour et al., 2022). Despite its importance, the accurate representation of biogenic sulfur emissions in climate models remains a challenge (Mansour et al., 2023; Mansour et al., 2024a). We employed machine learning (ML) based approaches to characterize seawater DMS concentrations, sea-to-air DMS emission flux (FDMS), as well as the atmospheric concentrations of marine biogenic methanesulfonic acid (MSA) and non-sea-salt sulfate (nss-SO42–). This study focuses on the Mediterranean Sea, a warm, oligotrophic marine basin and a climate change hotspot with rapidly increasing temperatures.

In our methodology, a set of ML models (Mansour et al., 2024b) is trained and evaluated using nested cross-validation, forced by high-resolution satellite data (chlorophyll-a, sea surface temperature, photosynthetically available radiation) and Mediterranean physical reanalysis (mixed layer depth and seawater salinity) datasets, combined with in situ DMS measurements. The optimized model generates daily gridded fields of DMS and FDMS at mesoscale resolution (0.083° × 0.083°, ~9 km) spanning 23 years (1998–2020). These high-resolution FDMS estimates align with observational data of MSA and nss-SO42–, secondary aerosol products from DMS oxidation, collected at the Lampedusa monitoring site in the central Mediterranean (Becagli et al., 2013). Compared to existing coarse-resolution global DMS datasets, the reconstructed FDMS fields capture seasonal patterns of biogenic sulfur with much greater accuracy across the Mediterranean Sea.

Furthermore, the FDMS outputs are integrated with high-resolution atmospheric datasets from the Copernicus European Regional Reanalysis (CERRA) to predict atmospheric concentrations of MSA and nss-SO42–. The ML models produce daily time-series predictions over the same 23-year period, achieving finer temporal and spatial coverage than observational datasets alone.

This analysis demonstrates the potential of ML techniques to enhance the estimation of seawater DMS fluxes and associated sulfur aerosol concentrations, achieving outstanding predictive performance. The spatiotemporal dynamics of these variables over the 23 years are analysed to elucidate mesoscale oceanographic variability and its influence on sulfur cycling. Ongoing analyses of long-term trends and interannual variability aim to identify the main drivers of these patterns, with results to be presented and discussed in detail.

Funding:

This work was funded by the European Commission’s EU Horizon 2020 Framework program, project FORCeS (grant no. 821205), and the European Union’s Horizon, project CleanCloud (Grant No. 101137639).

References:

Becagli, et al. (2013), Atmospheric Environment, 79, 681-688, 10.1016/j.atmosenv.2013.07.032.

Charlson, et al. (1987), Nature, 326, 655-661, 10.1038/326655a0.

Mansour, et al. (2023), Science of The Total Environment, 871, 10.1016/j.scitotenv.2023.162123.

Mansour, et al. (2024a), npj Climate and Atmospheric Science, 7, 10.1038/s41612-024-00830-y.

Mansour, et al. (2022), Journal of Geophysical Research-Atmospheres, 127, 10.1029/2021jd036355.

Mansour, et al. (2024b), Earth System Science Data, 16, 2717–2740, 10.5194/essd-16-2717-2024.

Mansour, et al. (2020a), Atmospheric Research, 237, 10.1016/j.atmosres.2019.104837.

Mansour, et al. (2020b), Journal of Geophysical Research-Atmospheres, 125, 10.1029/2019jd032246.

O'Dowd, et al. (2004), Nature, 431, 676-680, 10.1038/nature02959.

How to cite: Rinaldi, M., Decesari, S., Paglione, M., Becagli, S., and Mansour, K.: Advancing predictions of Dimethylsulfide emissions and biogenic sulfur aerosol in the Mediterranean region via machine learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17040, https://doi.org/10.5194/egusphere-egu25-17040, 2025.

EGU25-17784 | Orals | AS2.5

Marine emissions of methanethiol increase aerosol cooling in the Southern Ocean 

Julián Villamayor, Charel Wohl, Martí Galí, Anoop S. Mahajan, Rafael P. Fernández, Carlos A. Cuevas, Adriana Bossolasco, Qinyi Li, Anthony J. Kettle, Tara Williams, Roland Sarda-Esteve, Valérie Gros, Rafel Simó, and Alfonso Saiz-Lopez

Ocean-emitted dimethyl sulfide (DMS) is a major source of climate-cooling aerosols. However, most of the marine biogenic sulfur cycling is not routed to DMS but to methanethiol (MeSH), another volatile whose reactivity has hitherto hampered measurements. Therefore, the global emissions and climate impact of MeSH remain unexplored. We compiled a database of seawater MeSH concentrations, identified their statistical predictors, and produced monthly fields of global marine MeSH emissions adding to DMS emissions. Implemented into a global chemistry-climate model, MeSH emissions increase the sulfate aerosol burden by 30 to 70% over the Southern Ocean and enhance the aerosol cooling effect while depleting atmospheric oxidants and increasing DMS lifetime and transport. Accounting for MeSH emissions reduces the radiative bias of current climate models in this climatically relevant region.

How to cite: Villamayor, J., Wohl, C., Galí, M., Mahajan, A. S., Fernández, R. P., Cuevas, C. A., Bossolasco, A., Li, Q., Kettle, A. J., Williams, T., Sarda-Esteve, R., Gros, V., Simó, R., and Saiz-Lopez, A.: Marine emissions of methanethiol increase aerosol cooling in the Southern Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17784, https://doi.org/10.5194/egusphere-egu25-17784, 2025.

EGU25-17950 | Posters on site | AS2.5

Some Recent Contributions from the Heidelberg Aeolotron to Understanding Air-Sea Gas Exchange 

Bernd Jähne, Kerstin Krall, Dennis Hofmann, and Yuanxu Dong

The lack of knowledge about the parameters controlling the transfer velocity of the exchange of gases and volatile species across the air-sea interface besides the wind speed – such as the sea state (wave age), bubbles, and surfactants - hinders progress of a better estimate of fluxes for all relevant chemical species.

In 2021, a laboratory program was started at the large air-sea interaction facility, the Heidelberg Aeolotron. With four innovative key elements, most disadvantages of previous wind-wave tunnel experiments could be overcome:

  • Because of the infinite fetch of the annular facility, wind waves come into equilibrium with the wind that is more similar to the ocean compared to the linear facility.

  • The clean environment (walls coated with Teflon foil) facilitates experiments with surface films.

  • Two imaging techniques are used to measure transfer velocities locally and instantaneously. In this way, it is also possible to get direct insight into the mechanisms.

  • The whole fetch range and non-stationary conditions could be investigated.

An extensive measuring program finished in September 2024. In this talk, the focus is on some of the first results which are regarded to be the most important contributions concerning the conditions in the field:

  • The dependence of the transfer velocity on the fetch (wave age) seems to be only significant at lower wind speeds with an overshoot at young wind fields by more than a factor of two. This is an important contribution to the large variability of the gas transfer velocity at low wind speeds.

  • Once surface active materials, either soluble or insoluble suppress waves, gas transfer velocities are reduced to the same velocities and are governed by the same mechanisms. The measurements included insoluble films of hexadecanol and olive oil and the soluble surfactants TritonX-100 and Tergitol 15-S-12. At wind speeds larger than 8 m/s, wind waves cannot be suppressed by any films.

  • From a statistical analysis of the spatial-temporal patterns gained by both imaging techniques, it is possible to infer the Schmidt number exponent. This means that no longer multi-tracer experiments are required using tracers with a large difference in the diffusion coefficients.

  • At high wind speeds, breaking of the dominant waves does not play a dominant role. It is a rather fast surface renewal taking place all over the surface at scales of a few centimeters, which is associated with the smaller-scale wind wave field riding on the dominant wave.

  • Simplified forms of the two imaging techniques used in the Aeolotron seem to be suitable also for field measurements. A first experiment is planned for the BASS Baltic Sea cruise in June 2025.

  • It was possible to compare gas transfer measured with flux chambers in the Aeolotron with those gained at the free water surface using imaging thermography. The results clearly show that no useful measurements can be performed by flux chambers as soon as wind-induced effects are dominant, which is already the case at wind speeds as low as 2 m/s.

How to cite: Jähne, B., Krall, K., Hofmann, D., and Dong, Y.: Some Recent Contributions from the Heidelberg Aeolotron to Understanding Air-Sea Gas Exchange, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17950, https://doi.org/10.5194/egusphere-egu25-17950, 2025.

EGU25-346 | ECS | Posters on site | OS3.1

BASS Mesocosm Study: trace gas processes during a phytoplankton bloom with extreme slick formation 

Lea Lange, Dennis Booge, Ina Stoltenberg, Hendrik Feil, Hermann W. Bange, and Christa A. Marandino

Short- and long-lived trace gases impact atmospheric chemistry and climate, via processes like hydroxyl radical chemistry, aerosol formation, cloud condensation nuclei formation, or the greenhouse effect. As the oceans serve as sources and sinks for atmospheric trace gases, understanding the drivers of trace gas cycling in surface waters and their release to the atmosphere is crucial for climate predictions. Furthermore, there is a serious lack of information related to trace gas cycling in the uppermost ocean, the Sea surface microlayer (SML). Production and consumption of trace gases was investigated in a five-week mesocosm study with North Sea water at the SURF facility (Wilhelmshaven, Germany), during which an extreme slick formed under a combined diatom and coccolith bloom. In addition to bulk sampling, the glass plate method was used successfully to sample trace gases in the SML. Findings are supported by an extensive set of parameters from other BASS subprojects.

How to cite: Lange, L., Booge, D., Stoltenberg, I., Feil, H., Bange, H. W., and Marandino, C. A.: BASS Mesocosm Study: trace gas processes during a phytoplankton bloom with extreme slick formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-346, https://doi.org/10.5194/egusphere-egu25-346, 2025.

EGU25-6365 | ECS | Orals | OS3.1

The Effects of Algal Blooms on Oxygen Concentration and Temperature in the Sea Surface Microlayer – a Mesocosm Study 

Carsten Rauch, Edgar Cortés, Leonie Jaeger, and Oliver Wurl

The sea surface microlayer (SML) is of global importance as all exchange processes of heat and gases between the ocean and the atmosphere have to pass through it and are regulated by the features of the SML. These exchanges occur not only permanently between the SML and the atmosphere, but also between the SML and the underlying water (ULW). The properties of the SML are strongly influenced by surface-active substances known as surfactants, which are mostly of biological origin. Events such as algal blooms can produce large amounts of surfactants, thus changing the properties of the SML and the ULW. Obtaining in situ data of the SML proved very difficult in the past, due to its small thickness. Using microsensors gives the opportunity to close this gap by obtaining in situ data of the SML and to directly show the influence an algal bloom has on the SML.

A mesocosm experiment was conducted to obtain a more mechanistic understanding of the effect of an algal bloom on the physicochemical properties of the SML. An algal bloom was artificially induced in a seawater basin and physiochemical changes in the SML and ULW were investigated over time by applying multiple techniques. To directly study changes in temperature and oxygen, very precise microsensors (UNISENSE) were used for continuous in situ profiling, measuring from the air, through the SML, and into the ULW on a scale of tens of micrometers. We conducted the experiment over a continuous 30-day period during the algal bloom, allowing us to gain insights into the boundary layer, including the formation of oxygen and temperature gradients and the thickness of the SML.

The microsensor data showed, that the oxygen gradient in the SML is strongly correlated to the chlorophyll a concentration (r = 0.76, p < 0.01) and thus the algal bloom, while the thickness of the oxygen diffusion boundary layer, however, only shows a weak correlation to the surfactant concentration (r = 0.47, p = 0.01). The oxygen measurements deliver the in situ data to verify previous assumptions on oxygen gradients (-10 – 50 µmol L-1) and the thickness of the oxygen diffusion boundary layer (500 – 1500 µm) at the sea surface. The temperature gradient in the SML and the thickness of the thermal boundary layer were not influenced by the algal bloom, but the in situ measurements also confirm previous assumptions on temperature gradients (0.05 – 0.2 °C) and the thermal boundary layer thickness (750 – 2000 µm).

Obtaining gradients of gases or temperature in the SML and calculating the SML thickness was in the past only possible via indirect methods like measuring gas concentration differences between air and ULW or with computing surface temperatures from the emitted longwave irradiance. The in situ microsensor measurements now enable us to directly investigate processes inside the SML without relying on indirect measurements. Overall, we investigated the effect of an algal bloom on the SML and demonstrated a new in situ approach using microsensors to investigate physicochemical changes in and across the SML.

How to cite: Rauch, C., Cortés, E., Jaeger, L., and Wurl, O.: The Effects of Algal Blooms on Oxygen Concentration and Temperature in the Sea Surface Microlayer – a Mesocosm Study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6365, https://doi.org/10.5194/egusphere-egu25-6365, 2025.

The sea surface microlayer (SML) refers to the uppermost millimeter of the ocean surface that is in direct contact with the atmosphere. It has physicochemical and biological properties that are distinct from the underlying water and its properties determine air-sea exchange of momentum, mass and energy. Gas transfer velocity is mostly determined by wind forcing, where gas transfer is enhanced at low to moderate wind speeds. However, biological and pollutant enrichment of the SML with surfactants reduces gas transfer by suppressing turbulence and damping waves. Local impacts from surfactants can be significant, reducing air-sea gas transfer by single to double-digit percentages at moderate wind speeds.

I calculate a timeseries of contemporary global air-sea CO2 fluxes using FluxEngine, adjusting the calculation for the presence of biological surfactants. Surfactant suppression of air-sea gas transfer is estimated as a function of total organic carbon concentration, which is in turn estimated using global satellite products of particulate and dissolved organic carbon. Results will be compared to previous regional estimates of surfactant regulation of CO2 fluxes. This approach will produce a novel global estimate of biological surfactants’ regulation of CO2 fluxes across the air-sea interface, supporting further work isolating pollutants’ role in regulation of gas transfer.

How to cite: Kvale, K.: Surfactants’ global regulation of CO2 fluxes across the air-sea interface, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7269, https://doi.org/10.5194/egusphere-egu25-7269, 2025.

EGU25-8521 | Posters on site | OS3.1

Surfactant distribution can impact air-sea exchange in a Tropical Estuarine System in the Caribbean. 

Mariana Ribas-Ribas, Karen Moreno-Polo, Diomer Tobón-Monsalve, Carola Lehners, Oliver Wurl, Wilberto Pacheco, and Lennin Florez-Leiva

The sea surface microlayer (SML), the critical interface between the ocean and atmosphere (≤ 1000 μm thick), plays a vital role in regulating the exchange of climate-relevant gases, such as CO2. This study provides the first evaluation of the SML in a tropical estuarine system, covering over 80 km of the Gulf of Urabá in Caribbean Colombia. It investigates the distribution and influence of surfactants, focusing on the effect of fluvial inputs during the rainy and dry seasons. Samples were collected from fluvial and marine zones, revealing no significant differences in surfactant concentrations or enrichment factors. However, surfactant concentrations were significantly higher during the rainy season (1011.63 ± 745.21 μg Teq L⁻¹, August 2021) than the dry season (428.34 ± 189.44 μg Teq L⁻¹, April 2022). Notably, all sampling stations exhibited surfactant concentrations exceeding 200 μg Teq L⁻¹, a threshold associated with reductions of up to 23% in the rate of ocean-atmosphere CO2 transfer. Approximately 55% of the recorded concentrations represented a high surfactant regime, while 28% corresponded to slick zones. These values and enrichment factors were higher than those reported in other coastal and oceanic studies. Our findings underscore the significant role of surfactants in tropical biogeochemical cycles and provide valuable new insights into the SML in tropical regions where data is scarce. This research highlights the potential impact of surfactants on CO2 exchange in coastal tropical environments, enhancing our understanding of the ocean-atmosphere interface in such regions.

How to cite: Ribas-Ribas, M., Moreno-Polo, K., Tobón-Monsalve, D., Lehners, C., Wurl, O., Pacheco, W., and Florez-Leiva, L.: Surfactant distribution can impact air-sea exchange in a Tropical Estuarine System in the Caribbean., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8521, https://doi.org/10.5194/egusphere-egu25-8521, 2025.

EGU25-8823 | ECS | Orals | OS3.1

Biogeochemical Links in the Sea-Surface Microlayer: A Multidisciplinary Mesocosm Study 

Riaz Bibi, Mariana Ribas-Ribas, Carola Lehners, Leonie Jaeger, Lisa Gassen, Samuel Mintah Ayim, Thomas H. Badewien, Jochen Wollschläger, Claudia Thölen, Thorsten H. Brinkhoff, Isha Athale, Hannelore Waska, Jasper Zöbelein, Rüdiger Röttgers, Michael Novak, Anja Engel, Josefine Karnatz, and Oliver Wurl

The sea-surface microlayer (SML) represents the thin (< 1000 µm) uppermost layer of the ocean. Due to its unique position between ocean and atmosphere, the SML plays a central role in marine biogeochemical cycles. Changes in the phytoplankton biomass and community composition are linked to profound changes in the physical, chemical, and biological properties of the SML. And this influences air-sea interaction such as heat and gas exchange, organic matter composition, and surface-active substances in the SML and underlying water (ULW). Dynamic interactions between the SML and the ULW and the connectivity of the biogeochemical processes in the SML remain unclear. To fill this knowledge gap, we conducted a multidisciplinary mesocosm study. Here we report the general setup in a 17 m3 mesocosm facility, the progression of an induced phytoplankton bloom, and the general description and coupling of the changes in biogeochemical properties of the SML and the ULW.

SML and ULW samples were collected daily to analyze inorganic nutrients (NO3-, NO2-, PO43-, SiO32-), turbidity, solar radiation, phytopigments, surfactants, dissolved and particulate organic carbon (DOC, POC), total dissolved and particulate nitrogen (TDN, PN), phytoplankton and bacterial abundance, and their utilized substrates.

A self-organizing map (SOM) configuration revealed a clear temporal segregation of nutrient samples in SML and ULW. Based on nutrient levels, phytoplankton bloom progression over the time of the mesocosm experiment could be clearly classified into pre-bloom, bloom, and post-bloom phases. During this time, Chla concentrations varied from 1.0 to 11.4 μg L-1 with an average of 7.3 µg L-1. POC and PN exhibited a strongly positive relationship (r = 0.95) and followed the trend of Chla. Turbidity demonstrated a peak during bloom phase, which was associated with a high biological activity. Phytopigment composition data showed that haptophytes were the dominant phytoplankton group, followed by diatoms which could be confirmed by optical methods.

The daily average solar irradiance aligned with the local weather variability. Surfactants were enriched in the SML compared to the ULW. A discrepancy between the onset of increases in phytoplankton biomass and surfactant concentrations was observed with a lag of five days. This mismatch suggests a physiological acclimation of phytoplankton towards less favorable growth conditions, for example, nutrient limitations after the bloom phase. The high surfactant concentrations were also mirrored as DOC and TDN enrichment in the SML compared to ULW. A distinct slick formation with high turbidity was observed, indicating a biofilm-like SML habitat during the bloom and post-bloom phases. This biofilm was characterized by higher bacterial cell counts in SML. Bacterial metabolic profiles assessed by Biolog EcoPlates showed that the bacterial community utilized amino acids as key substrates in both water layers.

The main findings of our study emphasize that changes in biological parameters were linked to changes in chemical and physical parameters in SML. Our study provides deeper insights into the biogeochemical controls of the SML at a mechanistic level. Further spatio-temporal studies are needed to investigate the coupling of biogeochemical processes between the SML and ULW at both regional and global scales.

How to cite: Bibi, R., Ribas-Ribas, M., Lehners, C., Jaeger, L., Gassen, L., Mintah Ayim, S., H. Badewien, T., Wollschläger, J., Thölen, C., H. Brinkhoff, T., Athale, I., Waska, H., Zöbelein, J., Röttgers, R., Novak, M., Engel, A., Karnatz, J., and Wurl, O.: Biogeochemical Links in the Sea-Surface Microlayer: A Multidisciplinary Mesocosm Study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8823, https://doi.org/10.5194/egusphere-egu25-8823, 2025.

EGU25-8931 | ECS | Orals | OS3.1

Photochemical dynamics of carbonyl compounds in the sea-surface microlayer (SML) based on a mesocosm study 

Olenka Jibaja Valderrama, Thomas Schaefer, Manuela van Pinxteren, and Hartmut Herrmann

The sea-surface microlayer (SML), the thin boundary interface between the ocean and the atmosphere, is of global relevance as oceans are largely assumed to carry an SML. Characterized by its enrichment in organic material and exposure to strong solar radiation, the SML is expected to be a photochemically active zone that plays a critical role in the cycling of organic compounds and that influences air-sea exchange processes. Carbonyl compounds are particularly important as known products of photochemical reactions at the ocean's surface, making their behavior potentially relevant for understanding abiotic reactions and exchanges with the atmosphere. This study investigates the photochemical production and degradation of aldehydes and ketones in both ambient SML and bulk seawater samples. Samples were collected during a mesocosm field campaign at the Sea-surface Facility (SURF), located at the Institute for Chemistry and Biology of the Marine Environment (ICBM) in Wilhelmshaven. To simulate natural conditions, the samples were irradiated for 5 hours using a temperature-controlled aqueous-phase photoreactor equipped with a light source that mimics actinic radiation. The formation and degradation of target carbonyl compounds were analyzed using a derivatization technique with o-(2,3,4,5,6-Pentafluorobenzyl)hydroxylamine (PFBHA), followed by solvent extraction and GC-MS analysis. The findings provide a quantitative evaluation of the formation and degradation dynamics of carbonyl compounds to understand differences between the SML and the underlying bulk seawater. First results suggest the photochemical formation of acetaldehyde and methyl vinyl ketone, and the photochemical degradation of trans-2-hexenal. For other target compounds, including acetophenone, acrolein, butyraldehyde, crotonaldehyde, glyoxal, hexanal, heptanal, hydroxyacetone, methacrolein and propionaldehyde, no consistent trend of formation or degradation was observed. The concentrations of these carbonyl compounds varied significantly depending on the sample, ranging from a few ng L-1 to a few mg L-1. This study contributes to a deeper understanding of the role of the SML as a reactive environment and its implications for biogeochemical cycles and air-sea interactions.

How to cite: Jibaja Valderrama, O., Schaefer, T., van Pinxteren, M., and Herrmann, H.: Photochemical dynamics of carbonyl compounds in the sea-surface microlayer (SML) based on a mesocosm study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8931, https://doi.org/10.5194/egusphere-egu25-8931, 2025.

EGU25-11560 | ECS | Posters on site | OS3.1

Organic Alkalinity in the Sea-Surface Microlayer: Implications for Ocean Acid-Base Chemistry 

Edgar Cortés, Alisa Rosemarie Ingrid Wüst, Ander Lopez Puertas, Oliver Wurl, José Martín Hernández Ayón, Hannelore Waska, and Mariana Ribas Ribas

The air-sea CO₂ exchange is a critical process in regulating Earth's carbon cycle. At the ocean's surface, the sea-surface microlayer (SML) - a thin, organic-rich layer - serves as the critical interface between the air and sea and acts as a microreactor where unique chemical transformations occur, driven by sunlight, biological activity and surface-active materials. However, its role in air-sea CO₂ exchange is not well explored. In this study, we present the first direct measurements of organic alkalinity (OA) in the SML during a mesocosm experiment simulating a coccolithophore bloom of Emiliania huxleyi, aiming to better understand the contribution of organic matter to the air-sea CO₂ exchange.

Our every third day-resolution data on dissolved inorganic carbon (DIC), total alkalinity (TA), pH, and OA, quantified using back-titration, reveal significant differences between the SML and the underlying water (ULW). OA concentrations in the SML were consistently higher, contributing 8.07% ± 2.60 of TA, 2.58 times higher than the 3.12% ± 1.24 contribution observed in the ULW. This enrichment suggests that the SML serve as a significant reservoir for OA, influencing the overall acid-base balance.

During the coccolithophore bloom phase, we observed that photosynthesis and calcification—the dominant biogeochemical processes—resulted in decreases in both TA and DIC in the SML. Normally, changes in DIC would lead to a decrease in pH (increased acidity), while changes in TA might buffer this effect. However, the observed pH variability could not be explained by DIC and TA alone. Only by considering OA concentrations we can explain the observed pH variability. A strong negative correlation between the OA contribution to TA and pH (r = -0.82, p < 0.05) highlighted OA's role in modulating pH only in the SML. While calcification produces CO₂ and lowers pH through the dissociation of carbonic acid, coccolithophores also release organic acids, including humic-like fluorescent dissolved organic matter (fDOM). These acids may contribute to TA, but their primary effect is to release H⁺ ions, further acidifying the surface layer.

The increased OA in the SML contributes to its buffering capacity, but it does not fully counteract the acidification induced by calcification. These findings underscore the importance of incorporating OA dynamics in studies of the SML, particularly in the context of intense biological activity, such as coccolithophore blooms. Our results suggest that pH changes in the SML cannot be fully explained by TA alone, highlighting the need to consider OA in the analysis of the marine carbon system and the air-sea CO₂ exchange. While the specific organic acids contributing to OA remain unidentified for this work, future research into these compounds will be essential for improving our understanding of OA’s role in modulating the Earth's carbon cycle.

How to cite: Cortés, E., Wüst, A. R. I., Lopez Puertas, A., Wurl, O., Hernández Ayón, J. M., Waska, H., and Ribas Ribas, M.: Organic Alkalinity in the Sea-Surface Microlayer: Implications for Ocean Acid-Base Chemistry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11560, https://doi.org/10.5194/egusphere-egu25-11560, 2025.

EGU25-11844 | ECS | Posters on site | OS3.1

Effects of a Phytoplankton Bloom and Photobleaching on Colored and Fluorescent Dissolved Organic Matter in the Sea-Surface Microlayer 

Claudia Thölen, Jochen Wollschläger, Michael Novak, Rüdiger Röttgers, and Oliver Zielinski

The effects of a phytoplankton bloom and photobleaching on the colored and fluorescent dissolved organic matter (CDOM and FDOM, respectively) in the sea-surface microlayer (SML) and the underlying water (ULW) were studied in a 33-day mesocosm experiment at the Institute for Chemistry and Biology of the Marine Environment in Wilhelmshaven, Germany. The SML is the thin (< 100 µm) boundary layer between the ocean and the atmosphere and highly relevant to ocean biogeochemistry and climate-related exchange processes. Previous work has shown that when the SML is enriched in organic matter it can hinder gas, light, momentum, and heat exchanges between ocean and atmosphere. However, the underlying processes of organic matter enrichment in the SML are insufficiently understood. Heterogeneity and dynamics in the open sea make it difficult to differentiate between transport processes, environmental drivers, and biogeochemical processes. Hence, the mesocosm study was conducted to gain a deeper understanding of organic matter formation and degradation processes in the SML and ULW. To gain an understanding of different sources and sinks, the hypotheses tested were (1.) phytoplankton blooms result in different FDOM component compositions in the SML and ULW and (2.) photodegradation affects the component composition of the SML and the ULW differently.
Daily SML and ULW samples were collected for spectral fluorometric and photometric analysis, alternately in the morning and afternoon. Supplementary parameters like irradiance, temperature, and chlorophyll-a were also recorded within the mesocosm basin with high temporal resolution (approx. 1 min). Spectral photometric and fluorometric methods, which exhibit high sensitivity and structural specificity with respect to organic matter are used for CDOM and FDOM analysis.
The mesocosm experiment was divided into three phases (bloom onset, peak, and decay). Degradation of larger, complex molecules or production of new organic matter was assessed via the “humification index” and is dependent on the water layer (SML or ULW), the phase of the bloom, and the sampling time. As samples were taken alternatively in the morning and in the afternoon, the exposure time to UV-light and therefore photodegradation as a sink varies differently for SML and ULW. CDOM slope results showed a high variability and generally higher molecular weights and higher molecule aromaticity in the SML compared to the ULW. Protein-like component concentrations increased in both SML and ULW which indicates higher microbial activity towards the peak and decay phase of the experiment. These results suggest that photodegradation and possibly microbial activity have different effects on SML and ULW, verifying hypothesis 2. The affect of higher biological activity during the phytoplankton bloom led to the most pronounced differences between the concentration and composition of organic matter in the SML and ULW, especially in the protein-like components. This finding supports the premises of hypothesis 1.

How to cite: Thölen, C., Wollschläger, J., Novak, M., Röttgers, R., and Zielinski, O.: Effects of a Phytoplankton Bloom and Photobleaching on Colored and Fluorescent Dissolved Organic Matter in the Sea-Surface Microlayer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11844, https://doi.org/10.5194/egusphere-egu25-11844, 2025.

EGU25-13644 | ECS | Orals | OS3.1

Influence of a Surfactant on Physical Processes Above and Below Wind-Generated Waves in a Wind-Wave Tank  

Camille Tondu, Marc Buckley, and Martin Gade

The air and water flow boundary layers are strongly coupled with the wave field and the physical phenomena involved are essentially based on small submillimeter/millimeter scale features and dynamic processes within the first millimeters above and below the SML (Sea surface Micro Layer). The scale at which these complex feed-back mechanisms operate make their study particularly challenging.

Surfactants at the air-sea interface strongly dampen both the dominant gravity-capillary waves and micro-breaking waves and hence dramatically influence the dynamics and associated air-sea fluxes. Even though the general effect of these monolayers on the waves is well known by the scientific community, their influence on the surface dynamics and air-sea fluxes associated still need to be carefully studied.

A series of experiments were conducted at the 26-m long, 1.5-m high, 1-m wide wind-wave tank of the University of Hamburg (Germany), where a measurement system was developed and installed at a fetch of 15.5m. The system offers the possibility to perform high resolution (33 µm/pixel) PIV (Particle Image Velocimetry) to capture the motion in the air-water flows in the SML’s vicinity, and LIF (Laser Induced Fluorescence) to accurately detect the wavy interface, with a resolution of 55 µm/pixel. Experiments were carried out at a reference wind speed of 4.5 m/s, without and with an insoluble surfactant (oleyl alcohol).

In slick free conditions, high vorticity regions are observed under the wave crests. On the air-side, the viscous sublayer detaches from the crest of most of the observed waves, and is being regenerated on the windward side of the directly following wave. However, thanks to the wide 50-cm field of view, some evidence was found that, under specific conditions, the sheltered region past the airflow separation can overcome a wave, hence strongly affecting its growth. After deployment of oleyl alcohol at the water surface, the dominant gravity-capillary waves are strongly dampened, and the capillaries mostly disappeared. Waves are still sheltering the airflow on their leeward side, but no clear airflow separation is being seen, and the enhanced turbulent regions, which were observed below the crest in slick-free conditions, are thinner, more elongated, and less intense. In the waterside, it has also been noticed that with surfactants, some streaks are being ejected away from the wavy interface.

How to cite: Tondu, C., Buckley, M., and Gade, M.: Influence of a Surfactant on Physical Processes Above and Below Wind-Generated Waves in a Wind-Wave Tank , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13644, https://doi.org/10.5194/egusphere-egu25-13644, 2025.

EGU25-15118 | ECS | Orals | OS3.1

Hydrodynamic Processes and Temperature-Salinity Gradients in Slicks: Insights from Lagrangian Observations in the Near-Surface Layer 

Lisa Deyle, Michelle Albinus, Jens Meyerjürgens, and Thomas H. Badewien

The near-surface ocean is central to exchanging energy, gases, and particles between the atmosphere and the upper ocean. In particular, the interaction processes between the sea surface microlayer and the underlying water are crucial for biogeochemical processes and climate science. An innovative approach using free-floating, minimal-invasive Lagrangian sensor drifters is employed to investigate hydrographic and dynamical processes in the near-surface layer. Each drifter is equipped with a sensor chain containing temperature and salinity sensors, enabling high-resolution vertical measurements down to a depth of 1.8 m.

The Lagrangian measurement method enables the dynamics of a water mass to be recorded in its natural inertial system without external influences such as ship-induced disturbances. During a field campaign in the North Sea near Helgoland in July 2024, temperature and salinity data were collected during slick events associated with algal blooms. Processes inside and outside the slicks, as well as their formation, dispersion and decay processes, were studied to understand the underlying mechanisms. This allows the analysis of horizontal and vertical gradients, as well as the investigation of the spatial and temporal dynamics of slicks, understanding their impact on the exchange processes and quantifying the importance of the sea surface microlayer and the underlying water.

Initial results reveal significant differences in temperature and salinity gradients between slick and non-slick areas. Slicks act as hydrodynamic microhabitats and critical boundaries, influencing vertical convection patterns and current shear in the near-surface layer. These results are confirmed by ADCP backscatter data collected from an autonomous catamaran, providing additional insights into current structures and particle distributions. Horizontal comparisons between multiple sensor-equipped drifters illustrate the variability of processes at small spatial scales.

The presented results demonstrate the potential of Lagrangian drifters as a minimally invasive, innovative and highly accurate method for studying slicks and climate-relevant processes in the near-surface layer. These approaches can significantly improve our understanding of air-sea interaction mechanisms and their role in global biogeochemical cycles.

How to cite: Deyle, L., Albinus, M., Meyerjürgens, J., and Badewien, T. H.: Hydrodynamic Processes and Temperature-Salinity Gradients in Slicks: Insights from Lagrangian Observations in the Near-Surface Layer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15118, https://doi.org/10.5194/egusphere-egu25-15118, 2025.

EGU25-16057 | Posters on site | OS3.1

Detection and Characterization of Mycosporine-like Amino Acids in the Sea Surface Microlayer of the Baltic Sea during Summer 

Michael Novak, Ruediger Roettgers, Claudia Thoelen, and Jochen Wollschlaeger

The Sea Surface Microlayer (SML) in aquatic environments is a thin layer (1–100 μm) at the air-water boundary, characterized by unique biogeochemical properties distinct from the underlying water. The production of organic biofilms and surfactants within the SML stabilizes the layer, often leading to a "slick-like" environment. The organic matrix within the SML can trap phytoplankton, subjecting them to intense light and ultraviolet (UV) radiation. Mycosporine-like amino acids (MAAs) are pigments produced by certain types of phytoplankton, exhibiting photoprotective absorption bands in UV and visible wavelengths. While numerous studies have documented MAAs in surface waters, particularly in equatorial regions, there is limited documentation of MAAs produced specifically within the SML. Here, we present data collected from the Baltic Sea near the summer solstice under both slick and non-slick conditions. Using High-Performance Liquid Chromatography (HPLC), we detected MAAs in SML samples. Absorption spectra measured from these samples revealed distinct UV absorption peaks characteristic of MAAs. Interestingly, many corresponding subsurface water samples contained either no detectable MAAs or only trace amounts. These findings highlight the unique environment of the SML and the biological acclimations that the neuston undergo to survive under these conditions.

How to cite: Novak, M., Roettgers, R., Thoelen, C., and Wollschlaeger, J.: Detection and Characterization of Mycosporine-like Amino Acids in the Sea Surface Microlayer of the Baltic Sea during Summer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16057, https://doi.org/10.5194/egusphere-egu25-16057, 2025.

EGU25-18260 | Orals | OS3.1

Effect of Solar Radiation on Presence and Abundance of Surfactant Associated Bacteria in the Sea Surface Microlayer  

Alexander Soloviev, Georgia Parks, and Aurelien Tartar

The sea surface microlayer (SML) is the boundary layer at the surface of the ocean, distinct from the water below and highly variable in space and time. SML is influenced by organisms that aslicks. Slicks are the result of surfactants dampening capillary waves, which can be seen in synthetic aperture radar (SAR) imagery because the smooth surface reflecting backscatter away from the receiver. This experiment investigated the presence and abundance of surfactant-associated bacteria in the SML above a coral reef and in slicks in a coastal seagrass ecosystem. During the experiment in the Florida Keys, 220 SML and subsurface water (SSW) samples were collected above a coral reef area and in slicks above a coastal seagrass ecosystem. During our previous experiments in the Gulf of Mexico samples were collected in the daylight only; while, in the Straits of Florida, in both daylight and nighttime (due to the study of the coral sponging, which however did not happen at the time of the experiment). All SML and SSW samples were sequenced on the Illumina MiSeq, 12 surfactant associated bacteria genera were found. Increasing wind speed had a negative effect on the abundance of these genera, with lower wind speeds showing a more habitable environment. The ratio of abundance of surfactant-associated bacteria between the SML and SSW was found different and affected by the ultraviolet component of solar radiation. Thus, the concentration of bio-surfactants in the SML may be different during the daylight and nighttime with corresponding consequences for the SAR imagery and air-sea interactions.

How to cite: Soloviev, A., Parks, G., and Tartar, A.: Effect of Solar Radiation on Presence and Abundance of Surfactant Associated Bacteria in the Sea Surface Microlayer , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18260, https://doi.org/10.5194/egusphere-egu25-18260, 2025.

EGU25-19728 | ECS | Orals | OS3.1

Spatial and temporal dynamics of dissolved organic matter in the sea surface microlayer during a bloom of coccolithophores 

Jasper Zöbelein, Thorsten Dittmar, and Hannelore Waska

The sea surface microlayer (SML) is a microscopic boundary that covers the ocean’s surface, influences CO2 exchange with the atmosphere, and is often exposed to high levels of UV irradiation. The SML is a unique biome and shelters diverse microbial communities. Bioaggregates, containing carbohydrates, lipids and proteinaceous material accumulate in the SML, affecting gas exchange. Despite its role in the global carbon cycle, the biogeochemical processes controlling the production and turnover of organic matter in the SML are poorly understood. This study is part of the collaborative research unit ’Biogeochemical processes and Air-sea exchange in the Sea-Surface microlayer’ (BASS). Our goal is to decipher the underlaying forces behind the accumulation of dissolved organic matter (DOM) in the SML and its spatial and temporal dynamics. Furthermore, we aim to link the molecular properties of DOM in the SML to the microbial communities living in the SML, to air-sea gas exchange, and to carbonate chemistry. To address these objectives, we conducted a large-scale mesocosm study with coastal seawater from Jade Bay (North Sea, Germany). Following nutrient addition, a bloom of the coccolithophore Emiliania huxleyi occurred. The SML was sampled with a glass plate, and the underlying water (ULW) was sampled with a tube at a depth of 60 cm. Dissolved organic carbon (DOC) was quantified in filtered samples, which were then desalinated and concentrated for molecular analysis of DOM with ultra-high resolution mass spectrometry. In both the SML and ULW, DOC concentrations almost doubled from pre-bloom to post-bloom conditions. Overall, DOC was higher in the SML than in the ULW, and this discrepancy increased after the algal bloom. Furthermore, the ratio of DOC to DON was significantly higher in the SML than in the ULW after the bloom. Molecular indicators of DOM lability increased concurrently with DOC concentrations, reflecting freshly produced DOM in both SML and ULW during the late algal bloom stages. At the same time, the contributions of aromatic fractions in DOM and a photodegradation index decreased, possibly related to UV exposure of the mesocosm. Overall, our results suggest that primary production is likely to drive organic matter accumulation in the SML.

How to cite: Zöbelein, J., Dittmar, T., and Waska, H.: Spatial and temporal dynamics of dissolved organic matter in the sea surface microlayer during a bloom of coccolithophores, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19728, https://doi.org/10.5194/egusphere-egu25-19728, 2025.

EGU25-20162 | ECS | Orals | OS3.1

Enrichment of Dissolved Organic Matter in the Sea Surface Microlayer During a Phytoplankton Bloom – Preliminary Results from a Mesocosm Study 

Josefine Karnatz, Theresa Barthelmess, Mariana Ribas-Ribas, Carola Lehners, Oliver Wurl, and Anja Engel

The ocean's uppermost layer, the sea surface microlayer (SML), significantly influences physical and chemical properties due to the enrichment with dissolved organic matter (DOM). Biomolecules exhibiting amphiphilic properties are referred to as surfactants and preferentially accumulate in the SML. Surfactants were previously shown to significantly damp capillary waves and reduce air-sea gas fluxes. However, their source dynamics and chemical identity remain unknown. Phytoplankton communities are the primary producers of major biomolecule classes such as carbohydrates and amino acids. We explored how phytoplankton bloom development shapes enrichment and composition processes in SML and in relation to surface activity. As part of the “BASS” (Biogeochemical processes and air-sea exchange in the sea surface microlayer) project, an experiment was conducted in the mesocosm facility “SURF” in 2023 to study changes in the SML over the course of a phytoplankton bloom for one month. During the experiment, we collected samples for dissolved amino acids (DAA) and dissolved combined carbohydrates (DCCHO) from the SML and the underlying water (ULW). Overall, concentrations of DAA and DCCHO were enriched in the SML compared to the ULW by a factor of 2.88 ± 1.16 and 2.68 ± 1.47, respectively. The highest enrichment factors for DCCHO and DAA occurred a few days after the peak of the phytoplankton bloom. Particularly high enrichment factors were calculated for the polar amino acids arginine (4.67 ± 2.64), glutamic acid (4.31 ± 2.24), and tyrosine (4.46 ± 2.92). However, nonpolar amino acids leucine and phenylalanine showed enhanced enrichment factors as well. Extremely high enrichment with factors were observed for glucose (8.79 ± 8.30), while other DCCHO only showed slight enrichment. Our results point towards a strong effect on the surface activity of polar and freshly produced, very labile DOM. Investigating variations in the biomolecular composition of the SML in relation to potential source dynamics further enhances our understanding of biogeochemical and climate-relevant processes in the SML, such as air-sea gas exchange.

How to cite: Karnatz, J., Barthelmess, T., Ribas-Ribas, M., Lehners, C., Wurl, O., and Engel, A.: Enrichment of Dissolved Organic Matter in the Sea Surface Microlayer During a Phytoplankton Bloom – Preliminary Results from a Mesocosm Study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20162, https://doi.org/10.5194/egusphere-egu25-20162, 2025.

EGU25-20597 | ECS | Orals | OS3.1

VSFG Based Surfactant Coverage Index - A Feasible Approach to Assess the Effect of the SML on Air-Sea Gas Exchange? 

Falko Schäfer, Florian-David Lange, Kristian Laß, and Gernot Friedrichs

The sea surface microlayer (SML) acts as a biogeochemical and (photo)chemical reactor. It is enriched with surfactants that modulate the physico-chemical properties of the interface. As such, the SML reduces the formation of capillary waves and thus turbulent air-sea gas exchange.

In recent years, the surface sensitive methods of Vibrational Sum Frequency Generation (VSFG) and Langmuir through compression isotherms (LT) have been used to characterize the state of the SML on the nanoscale. Here, we give a brief overview of the results obtained during the last decade, reporting on a variety of experiments ranging from (i) artificial laboratory experiments with model wet and dry surfactants (Triton X-100 and DPPC), (ii) semi-natural large-scale mesocosm experiments (SURF facility in Wilhelmshaven, Germany, 2023), and (iii) the analysis of natural samples. These include samples from a study targeting slick versus non-slick conditions (near Helgoland island, Germany, 2024), year-long time-series measurements at Boknis Eck Time series Station as well as during the Baltic GasEX campaign (Eckernförde Bay, Germany, 2009-2019). In this context, we have derived a surface coverage index as a proxy parameter to reduce the spectral VSFG information to a single parameter in order to enable correlation with other biogeochemical and physical variables, including surfactant activity based on AC voltammetry and wave damping data from previous studies.

We hypothesize that gas exchange reduction can be constrained by a surfactant coverage threshold. Working out solid correlation of biogeochemical parameters with surfactant coverage would help to better model the influence of the SML on large-scale air-sea gas exchange based on their climatologies.

How to cite: Schäfer, F., Lange, F.-D., Laß, K., and Friedrichs, G.: VSFG Based Surfactant Coverage Index - A Feasible Approach to Assess the Effect of the SML on Air-Sea Gas Exchange?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20597, https://doi.org/10.5194/egusphere-egu25-20597, 2025.

EGU25-466 | ECS | Posters on site | BG1.3

Effects of N fertilization on soil chemistry dynamics in Ferralsols of the High Potential Maize Zone, Kenya  

Kevin Churchil Oluoch, Abigael Otinga, Ruth Njoroge, Scholar Mutua, Turry Ouma, Phillip Agredazywczuk, Matti Barthel, Johan Six, Sonja Leitner, Collins Oduor, and Eliza Harris

Nitrogen-based inorganic fertilizers have been crucial in crop production globally. For a long time, SSA agriculture has been characterised by low fertilizer use and negative nutrient balances. However, recently fertilizer use has increased drastically. Unfortunately, increased use of synthetic N fertilizers alters soil properties directly and indirectly, and N losses to the ecosystem contribute to environmental degradation and climate change. Limited studies have focused on the effect of increased N application rates on agricultural soils in the tropical highlands. It is crucial to investigate and understand N flows in tropical soils to predict potential ecological impacts of increased synthetic N-fertilizer use while meeting the food demand in SSA.

This study aimed to investigate the effects of increasing N rates on soil N dynamics, chemical properties and N use efficiency in maize-monocrop systems in the tropical highlands of the Rift Valley region, Kenya. A field experiment consisting of six N-fertilizer rates (0, 25, 50, 75, 100 and 125 kg N ha-1) in triplicate was set up in Eldoret, Kenya. Soil samples were collected at depths of 0-20, 20-40 and 40-60 cm throughout the maize cropping season and analysed for mineral N (NH4+-N and NO3--N), soil organic carbon and pH. Results indicate a significant change in the soil chemistry due to fertilisation. The response magnitude varied across the three soil depths. For instance, NO3- -N increased with increased N application rate, which peaked at 14 (55.81 mg kg-1) and 42 (34.99 mg kg-1) days after treatment application in the top 20 cm and 20-40 cm depths, respectively. Similar trends were also observed in the NH4+-N concentration across different depths, with high N application rates tending to exhibit relatively high concentrations compared to treatments with lower N rates. We also observed a considerable decline in soil pH for plots treated with N fertilizer in the first 14 days, which then stabilized and rose gradually throughout the maize growing stages. However, the lower fertilizer plots tended to have higher pH in contrast to the other treatments. There was also a consistent increase in soil organic carbon (SOC), with slight fluctuations, throughout the cropping season.  

These results indicated low mineral N movement below the effective root zone depth during the active growth phase of the crop. Thus, a clear indicator of increased plant uptake and implies a reduced risk of loss through leaching in Ferralsols. We also expect that meteorological conditions coupled with crop phenological processes to play a significant role in the soil chemistry variability, as exhibited by the differences in response to the treatments. We will therefore consider crop phenological processes and how they influence soil nutrient cycles. The results of this study will help to inform sustainable N use in maize cropping systems and further improve understanding of N cycle in tropical soils.  

How to cite: Oluoch, K. C., Otinga, A., Njoroge, R., Mutua, S., Ouma, T., Agredazywczuk, P., Barthel, M., Six, J., Leitner, S., Oduor, C., and Harris, E.: Effects of N fertilization on soil chemistry dynamics in Ferralsols of the High Potential Maize Zone, Kenya , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-466, https://doi.org/10.5194/egusphere-egu25-466, 2025.

EGU25-880 | ECS | Orals | BG1.3

Insights into the sources of precursor and formation pathways of particulate NO3- during paddy-residue burning period through dual isotope proxies 

Chandrima Shaw, Ritwick Mandal, Atinderpal Singh, Prasanta Sanyal, and Neeraj Rastogi

Particulate nitrate (pNO3-) and its precursor gas nitrogen oxide (NOx) are among the most significant reactive nitrogen species in the atmosphere. NOx emissions over the Indian sub-continent especially the Indo-Gangetic Plain (IGP) have increased rapidly over the past decades. NOx, an atmospheric gaseous pollutant, plays important roles in the formation of tropospheric ozone, recycling of hydroxyl radicals (OH), etc. It also serves as a precursor to pNO3- formation. This has significant implications for air quality, climate, and human health. Rapid accumulation of pNO3- can also increase PM load by aiding in secondary aerosol formations. Identification of the major sources of NOx and the formation pathways of pNO3- is crucial for improving the accuracy of air quality models and effective mitigation strategies. In the atmosphere, pNO3- is known to form mainly via four distinct pathways: (P1) oxidation of NO2 by OH in gas phase, (P2) hydrolysis of N2O5 on existing aerosols, (P3) reaction between NO3 radicals and VOCs, and (P4) reaction of NO3 radical and ClO. However, studies on the sources and formation pathways of pNO3- are limited pertaining to the Indian subcontinent as well as the globe. Dual isotopes (δ15N and δ18O) of pNO3- are an excellent tool to understand the formation mechanisms and sources of pNO3- precursor (NOx) in the atmosphere. In this study, diurnal samples of PM2.5 were collected over a semi-urban site (Patiala) in the IGP during a large-scale paddy residue burning period (October-November). Dual isotopes (δ15N and δ18O) of pNO3- along with other major ions were measured. Average δ18O and δ15N of pNO3- were 57.2 ± 8 ‰and -1.9 ± 5 ‰, respectively. Significant diurnal differences in δ18O-NO3- and δ15N-NO3- were observed. δ15N-NO3- and δ18O-NO3- were -5.0 ± 2.4‰, 52.1 ± 6.2‰ and -0.13 ± 5.7‰, 60.0 ± 8.4‰ during day and night-time respectively. Enriched δ15N-NO3- during night-time was due to enhanced gas-particle partitioning owing to lower temperature. A significant negative correlation between Nitrate Oxidation Ratio (NOR), and temperature further supported the above statement. Stable isotope mixing model (MixSIAR) was used to estimate the contribution of different pathways to pNO3- formation and sources. The major pathways contributing to the formation of pNO3-  were  P1(OH)  (~ 92%) followed by P2 (N2O5) (~ 5%). P3 (VOCs) and P4 (ClO) had negligible contributions of ~1.3 and ~1.5% respectively. Relative contributions of P1 and P2 during day and night-time were calculated. P1 and P2 contributed to 95% and 5%, and 77% and 23% during day and night-time respectively. Presence of pNO3- formed via P1 during night-time could be due to the higher lifetime of pNO3- compared to sampling duration. Source apportionment showed biomass burning (32%) and traffic exhaust (35%) were the major contributors followed by combustion (18%) and soil emissions (15%) during the study period. Our study, first of its kind over India, is important for elucidating the formation mechanism of pNO3- from its precursor gas. Such studies are helpful in planning and developing mitigation strategies aiming to reduce NOx pollution over a specific region. 

How to cite: Shaw, C., Mandal, R., Singh, A., Sanyal, P., and Rastogi, N.: Insights into the sources of precursor and formation pathways of particulate NO3- during paddy-residue burning period through dual isotope proxies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-880, https://doi.org/10.5194/egusphere-egu25-880, 2025.

EGU25-1042 | ECS | Orals | BG1.3

Investigating the sensitivity of modelled nitrogen inputs in the Mediterranean to dry deposition parameters 

André Barreirinha, Sabine Banzhaf, Michael Russo, Markus Thürkow, Martijn Schaap, and Alexandra Monteiro

There are several nitrogen-sensitive areas in Europe, some more sensitive than others, and the Mediterranean climate zone is where many of the highly sensitive areas are. One of these areas is Portugal, where very few studies focus on this issue. The lack of infrastructure to monitor nitrogen concentrations and deposition in the country, as well as policies to enforce nitrogen emission reductions, poses a challenge, as ammonia is the most critical pollutant to fulfil Portugal's future emission goals.
Currently, modelling is the only cost-effective option to effectively study nitrogen deposition in the Mediterranean. Due to the extent of agriculture in these areas, nitrogen (N) deposition assessments have been conducted for many years in other countries, such as the Netherlands and Germany, using Chemistry Transport Models (CTMs) to assess the dry deposition of reduced and oxidised N. Among these CTMs, LOTOS-EUROS is regarded as one of the most advanced models that includes a compensation point parametrization for ammonia. However, applying this model to a Mediterranean area requires some adaptation since its deposition parameters are mostly based on studies from North-Western Europe. Since vegetation parameters influence the surface resistance of gas-phase deposition, and this resistance is crucial for gas deposition, using these models in climates different from where they were initially developed will likely lead to inaccurate results. Due to this, there is a need for a CTM that better represents different climate zones. 
Here, we use a new version of the LOTOS-EUROS model incorporating a three-tiered vegetation approach. The three tiers considered are Tier 1—climate zones; Tier 2—land use classes; and Tier 3—vegetation type. This method incorporates 140 combinations of land use and vegetation types, allowing us to differentiate the Mediterranean from the standard temperate climate by changing vegetation parameters.
With this study, we aim to adapt and enhance the dry deposition module of LOTOS-EUROS by including specifications for the Mediterranean climate and vegetation. To achieve this goal, sensitivity runs were performed for multiple vegetation and climate-specific parameters to assess which are the most influential variables for the study region. Then, the most sensitive parameters were analysed to understand the variations.
This work found that adapting the maximum stomatal conductance is highly prone to introduce changes in the modelled deposition fluxes and concentrations of oxidised and reduced nitrogen and ozone. Maximum and minimum vapour pressure deficit and maximum, optimal and minimum temperature were also among the most susceptible to cause impacts in the model results over the Mediterranean. Also, the start and end of the growing season greatly impacted the modelled deposition fluxes since the growing season starts earlier and finishes later in the Mediterranean. Hence, adapting the deposition parameters to the Mediterranean climate and vegetation significantly impacts the modelled concentration and deposition fluxes of oxidised and reduced nitrogen compounds and ozone.

How to cite: Barreirinha, A., Banzhaf, S., Russo, M., Thürkow, M., Schaap, M., and Monteiro, A.: Investigating the sensitivity of modelled nitrogen inputs in the Mediterranean to dry deposition parameters, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1042, https://doi.org/10.5194/egusphere-egu25-1042, 2025.

EGU25-1143 | ECS | Posters on site | BG1.3

Emissions of ammonia and nitrogen dioxide over the Iberian Peninsula estimated with satellite observations 

Daniel Helm, Enrico Dammers, Carla Gama, Martijn Schaap, and Alexandra Monteiro

Anthropogenic emissions of reactive nitrogen in Europe have increased significantly over the last two centuries. A large proportion of this reactive nitrogen is released into the atmosphere in the form of ammonia (NH3), which is generated from livestock farming activities and fertilizer use, and in the form of oxides of nitrogen (NOX) generated from the combustion of fossil fuels. 

The atmospheric deposition of reactive nitrogen can adversely impact ecosystems and biodiversity. This is particularly relevant to the Iberian Peninsula where ecosystems that have a low threshold for eutrophication, and are therefore highly sensitive to nitrogen levels, are found. 

In-situ measurements of reactive nitrogen species in this region are sparse and those that are available are measurements of NO2 concentrations and in some cases intermittent measurements of NHX & NOY wet deposition. This limitation in the availability of deposition data gives rise to a dearth of knowledge and a high degree of uncertainty in ascertaining the budget of nitrogen species in this region. 

Several approaches have been developed to estimate emissions of NO2 and NH3 utilizing earth observation. Here we present the application of a multi-gaussian plume inversion method in combination with satellite observations of NH3 from the Cross-Track Infrared Sounder instrument and observations of NO2 from the TROPOMI sensor to validate concentration distributions simulated by the LOTOS-EUROS chemistry transport model. 

Initially, a steady-state inversion scheme was applied over the Iberian Peninsula to derive spatial-temporal emission fields and evaluate these against inventory emissions and existing spatial and temporal distributions. An analysis of these results shows variations between the spatial distribution of inventory emissions and those obtained from the satellite observations. Then, the resulting emission fields are used within the LOTOS-EUROS model to simulate the concentration and deposition fields which will be evaluated with in-situ data. 

How to cite: Helm, D., Dammers, E., Gama, C., Schaap, M., and Monteiro, A.: Emissions of ammonia and nitrogen dioxide over the Iberian Peninsula estimated with satellite observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1143, https://doi.org/10.5194/egusphere-egu25-1143, 2025.

EGU25-1792 | Orals | BG1.3

Determining the origin of nitrogen deposition in nature areas 

Roy Wichink Kruit, Kasper Brandt, Albert Bleeker, and Wim van der Maas

Nitrogen policy in the Netherlands has a long history. Since the 70’s of the last century, various measures have been implemented in an attempt to reduce emissions of different nitrogen compounds. A few examples of a wide range of measures implemented since then are the introduction of catalytic converters removing nitrogen oxides from fossil fuel burning, shallow injection of manure into the soil reducing ammonia emissions to air and lowering of the manure application rates. In 2019, the European High Court judged that the Dutch nitrogen policy with respect to nitrogen deposition onto protected nature areas was not in accordance with the European Habitats Directive. All infrastructural developments came to a halt: building houses, roads, etc. stopped. With a new Minister on Nitrogen in place since 2021, the focus became a drastic reduction of nitrogen emissions to get the nitrogen deposition below the nitrogen critical loads for 74% of the protected (Natura 2000) nature areas, which is laid down in a nitrogen law. This requires a drastic change in activities in and around these nature areas, mainly (but not exclusively) focusing on the agricultural sector. This because the contribution to the total nitrogen deposition of this sector is on average 50% in the Netherlands. To help policymakers take measures as efficiently as possible, RIVM has developed a tool that maps the origin of the nitrogen deposition in each nature area. In this presentation, the tool will be presented and it will be shown how the tool can help the government, provinces and other stakeholders to take dedicated regional measures to reduce the nitrogen emissions and eventually reduce the nitrogen deposition in nature areas.

How to cite: Wichink Kruit, R., Brandt, K., Bleeker, A., and van der Maas, W.: Determining the origin of nitrogen deposition in nature areas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1792, https://doi.org/10.5194/egusphere-egu25-1792, 2025.

EGU25-1999 | ECS | Orals | BG1.3

Contrasting physico-chemical and oxidative relationships to thalli nitrogen and metal ion contents in Usnea spp. and Hypotrachyna spp. from Himalayan forests of Nepal. 

Suman Prakash Pradhan, Hirendra Bista, Bishal Lamsal, Bishnu Prasad Pandey, Chitra Bahadur Baniya, Ajinkya Deshpande, Subodh Sharma, and Mark A Sutton

South Asian nations are facing the challenge of increasing nitrogen pollution with the Indo-Gangetic Plain having some of the highest levels of atmospheric ammonia pollution globally. However, there is a lack of in-country research to evaluate the possible impact of nitrogen-related pollutants on South Asian biodiversity. In the Himalayas, there is an opportunity to utilize lichens from natural habitats to establish field-based references for better future tracking of changes in ecosystem health relevant to the wider South Asian region. In this study, we assessed the natural chemical variability of two lichens (Usnea spp. and Hypotrachyna spp.) based on thallus nitrogen and metal ion contents along with their physico-chemical and oxidative responses in two 1-km long transects from two forests of Nepal representing local gradients. Our results revealed a moderate concentration of total Kjeldalh nitrogen (0.36-0.98 % DM in Chandragiri, KTM and 0.57-2.04 % DM in Ghorepani, ACA), as well as ammonium (40.42-159.84 mg/L in Chandragiri, KTM and 80.60-280.64 mg/L in Ghorepani, ACA) and considerable amount of metal ions in both lichens, though with the highest values for lichens collected from the Ghorepani, ACA (from Western Nepal). A noteworthy background concentration of atmospheric ammonia was also observed at both sites. The highest variation in physico-chemical responses, such as electrical conductivity, chlorophyll content, chlorophyll degradation, chlorophyll fluorescence, and phenolic content was observed in the lichens from the same area, consistent with the higher levels of air pollution. Moreover, there appeared to be associated impacts on oxidative responses such as radical scavenging and catalase activities. Furthermore, the metal ions in the lichen thalli were found to originate from both anthropogenic and natural sources in Chandragiri, KTM and few of the metal ions were deposited from long-range transport mechanisms in Ghorepani, ACA, which signifies the diverse sources of pollution in the study areas. The sampling line-wise variation in thallus chemistry signifies the local pollution gradient in both sites. Further, environmental covariables (slope, elevation, crown settings, wind pattern) were observed to affect the lichen abundance and accumulation of nitrogen and metal ions. In comparison, Hypotrachyna spp. showed greater potential to accumulate pollutants and variability in physico-chemical and oxidative responses. From this study, we conclude that a range of physico-chemical and biochemical responses of the target lichens can be used as proxies for the bioindication of nitrogen and metal ion pollution to assess lichen’s health and ecological functioning. Wider studies covering large spatial extent and cellular mechanisms of lichen response are now recommended to fully understand the functional biology explaining contrasting responses between lichen species in different geographic settings of Nepal and South Asia.

 

Keywords: Lichens; Bioindicators; Pollution; Ecosystem; Reference

How to cite: Pradhan, S. P., Bista, H., Lamsal, B., Pandey, B. P., Baniya, C. B., Deshpande, A., Sharma, S., and Sutton, M. A.: Contrasting physico-chemical and oxidative relationships to thalli nitrogen and metal ion contents in Usnea spp. and Hypotrachyna spp. from Himalayan forests of Nepal., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1999, https://doi.org/10.5194/egusphere-egu25-1999, 2025.

EGU25-2297 | Posters on site | BG1.3

Acidification of European croplands by nitrogen fertilization: Consequences for carbonate losses, and soil health 

Kazem Zamanian, Ruhollah Taghizadeh-Mehrjardi, Jingjing Tao, Lichao Fan, Sajjad Raza, Georg Guggenberger, and Yakov Kuzyakov
Soil acidification is an ongoing problem in intensively cultivated croplands due to inefficient and excessive nitrogen (N) fertilization. We collected high-resolution data comprising 19,969 topsoil (0–20 cm) samples from the Land Use and Coverage Area frame Survey (LUCAS) of the European commission in 2009 to assess the impact of N fertilization on buffering substances such as carbonates and base cations. We have only considered the impacts of mineral fertilizers from the total added N, and a N use efficiency of 60 %. Nitrogen fertilization adds annually 6.1 × 107 kmol H+ to European croplands, leading to annual loss of 6.1 × 109 kg CaCO3. Assuming similar acidification during the next 50 years, soil carbonates will be completely removed from 3.4 × 106 ha of European croplands. In carbonate-free soils, annual loss of 2.1 × 107 kmol of basic cations will lead to strong acidification of at least 2.6 million ha of European croplands within the next 50 years. Inorganic carbon and basic cation losses at such rapid scale tremendously drop the nutrient status and production potential of croplands. Soil liming to ameliorate acidity increases pH only temporarily and with additional financial and environmental costs. Only the direct loss of soil carbonate stocks and compensation of carbonate-related CO2 correspond to about 1.5 % of the proposed budget of the European commission for 2023. Thus, controlling and decreasing soil acidification is crucial to avoid degradation of agricultural soils, which can be done by adopting best management practices and increasing nutrient use efficiency. Regular screening or monitoring of carbonate and base cations contents, especially for soils, where the carbonate stocks are at critical levels, are urgently necessary.

How to cite: Zamanian, K., Taghizadeh-Mehrjardi, R., Tao, J., Fan, L., Raza, S., Guggenberger, G., and Kuzyakov, Y.: Acidification of European croplands by nitrogen fertilization: Consequences for carbonate losses, and soil health, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2297, https://doi.org/10.5194/egusphere-egu25-2297, 2025.

EGU25-3079 | Orals | BG1.3

Trends of inorganic nitrogen deposition in European forests during the period 2000-2020 

Arne Verstraeten, Andreas Schmitz, Aldo Marchetto, Nicholas Clarke, Anne Thimonier, Char Hilgers, Anne-Katrin Prescher, Till Kirchner, Karin Hansen, Tamara Jakovljević, Carmen Iacoban, Wim de Vries, Bernd Ahrends, Henning Meesenburg, Gunilla Pihl Karlsson, Per Erik Karlsson, and Peter Waldner

The input of nitrogen (N) into forests through atmospheric deposition has been determined for the main forest types within the ICP Forests Level II monitoring network and the Swedish Throughfall Monitoring Network (SWETHRO) since the 1990s from measured concentrations in continuously collected precipitation (bulk deposition) and throughfall (below tree canopy) samples. Recently, aggregated data sets have been created, containing gap-filled monthly and annual bulk and throughfall depositions (including stemflow in beech stands) for more than 500 forest stands. Total deposition was calculated from throughfall deposition accounting for canopy exchange. Here, we present trends for throughfall deposition of inorganic N, including ammonium (NH4+-N) and nitrate (NO3--N), for plots with a complete time series, during the period 2000-2020 and in the first and last decade separately. Furthermore, we highlight and discuss spatial trends of total inorganic N deposition across Europe.

How to cite: Verstraeten, A., Schmitz, A., Marchetto, A., Clarke, N., Thimonier, A., Hilgers, C., Prescher, A.-K., Kirchner, T., Hansen, K., Jakovljević, T., Iacoban, C., de Vries, W., Ahrends, B., Meesenburg, H., Pihl Karlsson, G., Karlsson, P. E., and Waldner, P.: Trends of inorganic nitrogen deposition in European forests during the period 2000-2020, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3079, https://doi.org/10.5194/egusphere-egu25-3079, 2025.

EGU25-3928 | Posters on site | BG1.3

Synchronized N2O/CH4/H2O/NH3 plume mobile measurement system based on low-power open-path laser analyzers 

Songtao Hu, Weihao Shen, Ruisheng Jiang, Daniel Wilson, Ting-Jung Lin, and Yin Wang

In recent years, vehicle-based, multiple-gas mobile sensing platforms have been developed and extensively utilized for greenhouse gases (GHGs) and air pollutant emission studies. Closed-path analyzers are currently the primary equipment used for plume observations. However, the closed-path approach, poses sampling challenges for the species such as water vapor (H2O) and ammonia (NH3) that readily adsorb and desorb from the instrument inlets, tubings, and optical cells. Due to the different adsorption characteristics of each gas, the plume signals generated during the sampling process may become desynchronized. In addition, many mobile systems are deployed on fuel-powered vehicles, which emit exhaust that can contaminate the detected plume signals. These issues can increase the complexities in subsequent data processing tasks.

This work reports the field deployment of a multiple trace gas plume sensing platform, equipped with open-path N2O, CH₄, H2O and NH₃ quantum-cascade laser analyzers (model HT8500, HT8600P, HT8700, respectively) with a 10 Hz sampling time resolution. The plume monitoring system with a total power consumption of no more than 150W allows it to be easily driven by an electric vehicle. Utilizing the open-path N2O/CH4/H2O/NH3 gas analyzers eliminates the need for a pressure-controlled enclosed gas cell, the associated tubing systems, and power- hungry pump. The ambient air flows unrestricted through the optical path, enabling analyzers to achieve high temporal resolution, high response rates, and reduced sampling artifacts and power consumption compared to their closed-path gas analyzer counterparts. This open-path configuration not only eliminates the influence of exhaust emission signals from vehicles using fossil fuel engines, but also achieves perfect plume synchronization, which is crucial for the real-time identification of diffuse sources using correlations between different molecules in measured plumes.

The mobile platform has been field deployed in different field experiments including livestock farms, ammonia plants, cold storage facilities, wastewater treatment plants, and urban traffic roads in China. Our study has identified a substantial increase in ammonia concentrations adjacent to rivers, with an average increment of ~37 ppb relative to a few ppb background concentration. We observed that the peak methane concentration near a wastewater treatment plant reached 7539 ppb. Furthermore, the ratio of methane plume signal intensity to ammonia plume signal intensity in the vicinity of industrial areas is ~10, as opposed to non-industrial areas where this ratio is significantly reduced. The synchronized plume significantly enhances the efficiency of extracting effective plume data from the raw signals acquired from different gas analyzers.

How to cite: Hu, S., Shen, W., Jiang, R., Wilson, D., Lin, T.-J., and Wang, Y.: Synchronized N2O/CH4/H2O/NH3 plume mobile measurement system based on low-power open-path laser analyzers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3928, https://doi.org/10.5194/egusphere-egu25-3928, 2025.

Nitrogen holds a crucial place in maintaining the sustainability of the food-energy-water (FEW) nexus, essential pillars underpinning human society. Its vital role spans across food production, energy generation, and the preservation of water quality. Here based on CHANS model, we show that comprehensive nitrogen management strategies offer the dual benefits of satisfying China's food requirements and boosting nitrogen energy production from straw by 1 million tonnes (26%) compared to the baseline year of 2020. Simultaneously, these strategies could lead to a reduction of 8 million tonnes (-31%) in nitrogen fertilizer usage, a decrease of 3.8 million tonnes (-46%) in nitrogen-induced water pollution, and a halving of water consumption in agriculture, all relative to 2020 levels. These transformative changes within the FEW nexus could result in national societal gains of around US$140 billion, against a net investment of just US$8 billion. This emphasizes the cost-effectiveness of such strategies and highlights their significant potential in assisting China to meet multiple sustainable development goals, especially those related to hunger relief, clean energy advancement, and the protection of aquatic ecosystems.

How to cite: Chen, B.: Managing nitrogen to achieve sustainable food-energy-water nexus in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4076, https://doi.org/10.5194/egusphere-egu25-4076, 2025.

EGU25-4177 | ECS | Orals | BG1.3

Validation and uncertainty quantification of three state-of-the-art ammonia surface exchange schemes using NH3 flux measurements in a dune ecosystem 

Tycho Jongenelen, Margreet van Zanten, Enrico Dammers, Roy Wichink Kruit, Arjan Hensen, Leon Geers, and Jan Willem Erisman

Deposition of reactive nitrogen causes detrimental environmental effects, including biodiversity loss, eutrophication, and soil acidification. Measuring and modeling the biosphere-atmosphere exchange of ammonia, the most abundant reduced nitrogen species, is complex due to its high reactivity and solubility, often leading to systematic discrepancies between model predictions and observations. This study aims to determine whether three state-of-the-art exchange schemes for NH3 can accurately model NH3 exchange in a dune ecosystem and detect factors causing the uncertainties in these schemes. The selected schemes are DEPAC by Van Zanten et al. (2010), and the schemes by Massad et al. (2010) and Zhang et al. (2010). Validation against one year of gradient flux measurements revealed that the Zhang scheme represented the NH3 deposition at Solleveld best, whereas the DEPAC scheme overestimated the total deposition while the Massad scheme underestimated the total deposition. Yet, none of these schemes captured the emission events at Solleveld, pointing to considerable uncertainty in the compensation point parameterization and possibly in the modeling of NH3 desorption processes from wet surface layers. The sensitivity analysis further reinforced these results, showing how uncertainty in essential model parameters in the external resistance (Rw) and compensation point parameterization propagated into diverging model outcomes. These outcomes underscore the need to improve our mechanistic understanding of surface equilibria represented by compensation points, including the adsorption-desorption mechanism at the external water layer. Specific recommendations are provided for future modeling approaches and measurement setups to support this goal.

How to cite: Jongenelen, T., van Zanten, M., Dammers, E., Wichink Kruit, R., Hensen, A., Geers, L., and Erisman, J. W.: Validation and uncertainty quantification of three state-of-the-art ammonia surface exchange schemes using NH3 flux measurements in a dune ecosystem, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4177, https://doi.org/10.5194/egusphere-egu25-4177, 2025.

EGU25-5842 | Orals | BG1.3

Periodic Cicada Mass Mortality Events Drive Microbial-Mediated Gas Pulses from Forest Soils 

Ryan Mushinski, Megan Purchase, Richard Phillips, Jonathan Raff, Amy Phelps, Elizabeth Huenupi, and Jennifer Lau

Mass emergence of periodic cicadas (Magicicada spp.) represents a unique ecosystem disturbance with potential impacts on forest soil biogeochemistry and greenhouse gas emissions. During the 2021 Brood X emergence in Indiana, USA, we investigated how cicada emergence and subsequent decomposition affected soil microbial communities and their production of nitrous oxide (N2O) and ammonia (NH3). Using a combination of field measurements and controlled laboratory experiments, we discovered that the interface between cicada carcasses and soil surfaces creates hotspots of enhanced microbial nutrient cycling, leading to significant pulses of N2O and NH3 after approximately 10-15 days. Our study revealed that dissimilatory nitrate reduction to ammonia (DNRA) was the primary mechanism driving these emissions, evidenced by increased abundance of DNRA taxa on cicada carcass surfaces (the necrobiome) coinciding with peak gas fluxes. Notably, the abundance of Serratia marcescens, a bacteria capable of both chitin degradation and DNRA, was significantly positively associated with N2O pulses. Analysis of 16S rRNA amplicon sequencing data showed distinct microbial community compositions between soil and cicada necrobiome samples, with significantly higher abundances of chitinolytic and DNRA taxa in the necrobiome. Time series decomposition experiments demonstrated that soil respiration rates and nitrogen cycling were significantly enhanced in cicada-amended soils. Quantitative PCR revealed that bacterial ammonia oxidisers dominated over archaeal counterparts in soil samples, while the cicada necrobiome was characterised by high abundances of heterotrophic nitrifiers. The emergence tunnels created by cicadas also influenced soil conditions, potentially creating microsites that favour DNRA over conventional denitrification. While individual emergence events may contribute relatively small amounts of nitrogen compared to annual atmospheric deposition, the predictable nature and geographic extent of cicada emergences suggest they may represent an overlooked yet significant contributor to forest nitrogen cycling and greenhouse gas emissions. Our findings provide new insights into the complex microbiological mechanisms driving biogeochemical pulses following mass mortality events and highlight the need to consider periodic ecosystem disturbances in climate change models.

How to cite: Mushinski, R., Purchase, M., Phillips, R., Raff, J., Phelps, A., Huenupi, E., and Lau, J.: Periodic Cicada Mass Mortality Events Drive Microbial-Mediated Gas Pulses from Forest Soils, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5842, https://doi.org/10.5194/egusphere-egu25-5842, 2025.

EGU25-6623 | ECS | Posters on site | BG1.3

Trade-offs between crop yield, soil organic carbon and greenhouse gas emissions under reduced tillage and rainfall exclusion 

Antonios Apostolakis, Paulina Englert, Oliver Lindunda Daka, Stefan Siebert, and Ana Meijide

Reduced tillage is often considered as an agroecological practice that promotes soil organic carbon (SOC) sequestration in the topsoil, offering potential for climate change mitigation. However, effective mitigation requires a comprehensive understanding of trade-offs among SOC stocks, greenhouse gas emissions, and crop yields. As climate change alters carbon and nitrogen cycling, these trade-offs must be evaluated under current and experimentally induced extreme conditions to assess the effectiveness of reduced tillage in a changing climate. In this study, we measured crop yields, soil carbon stocks and soil CO2 and N2O fluxes in a conventional tillage (CT) vs. reduced tillage (RT) field trial in central Germany. The long-term trial runs since 1970 in a field with Luvisol soil (73% silt, 15% clay, and 6.6 pH). The mean annual precipitation is 611±120 mm and the mean annual temperature is 9.6±0.7°C. The field trial follows a randomized block design and consists of 16 plots: eight under CT with inversion ploughing to a depth of 27-30 cm, and eight under RT with non-inversion harrowing to a depth of 7-10 cm. In 2022-23 and in 2023-24 we cultivated winter wheat and winter barley respectively. In February 2023, rain-out shelters (area =2 m × 2 m) designed to intercept 50% of the precipitation were installed in half of the plots, and we initiated the soil flux measurements with static chambers over permanently installed rings and portable gas analyzers. We measured crop yields in both years, and SOC in samples from 0-90 cm at 10 cm intervals sampled in August 2023. SOC traits were examined with by-size fractionation to particulate and mineral-associated organic matter and an incubation experiment with an automated respirometer. Winter wheat yield did not differ between tillage and precipitation treatments but, in the second year of our experiment, winter barley yield was lower under rainfall exclusion than ambient precipitation in the RT fields only (50% precipitation: 0.26±0.05 kg m-2 vs. 100% precipitation: 0.52±0.02 kg m-2). Regarding SOC, we found that fields under RT had higher stocks in the 0-10 cm depth than under CT (RT: 1.93±0.03 kg m-2 vs. CT: 1.53±0.02 kg m-2), but the opposite occurred in the 20-30 cm depth (RT: 1.16±0.04 kg m-2 vs. CT: 1.58±0.06 kg m-2). Comparing SOC stocks at 0-90 cm, there was no difference between the two tillage systems. Field soil N2O fluxes did not differ significantly between tillage and precipitation treatments when considering block, plot and date as random effects. In contrast, field soil CO2 fluxes were significantly lower in RT than CT fields under ambient precipitation but this did not result in higher SOC stocks under RT. Rainfall exclusion led to higher soil CO2 fluxes both in the RT (in average, 50%: 32.0±1.0 mg CO2-C m-2 h-1 vs. 100%: 30.6±0.9 mg CO2-C m-2 h-1) and CT (in average, 50%: 30.1±1.1 mg CO2-C m-2 h-1 vs. 100%: 24.2±0.7 mg CO2-C m-2 h-1) fields. Based on the above, RT seems to have no climate change mitigation potential in a productive fine textured soil of temperate central Europe.

How to cite: Apostolakis, A., Englert, P., Daka, O. L., Siebert, S., and Meijide, A.: Trade-offs between crop yield, soil organic carbon and greenhouse gas emissions under reduced tillage and rainfall exclusion, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6623, https://doi.org/10.5194/egusphere-egu25-6623, 2025.

EGU25-6740 | ECS | Orals | BG1.3

Dynamics of N2O emissions from Amazonian tropical peat forest and partitioning N-processes using 15N isotopes. 

Mohit Masta, Fahad Ali Kazmi, Mikk Espenberg, Jaan Pärn, Kaido Soosaar, and Ülo Mander

Tropical peatlands are crucial for global nitrogen (N) cycling because they store large amounts of carbon and N. This study, conducted in November 2023, investigated the dynamics of N2O emissions from Amazonian peatland forests in Peru. It focused specifically on two peatland forest sites in Iquitos: the Quistococha and Zungarococha forests. We conducted static chamber gas measurements to assess soil greenhouse gas (GHG) fluxes. Additionally, we took soil samples for physical and chemical properties and soil microbiome (DNA & RNA). In order to investigate the source processes for N2O production and consumption, we applied 15N isotopes as tracers in soil. We also took samples for natural abundance of 15N in N2O gas. Our results indicate that both forests exhibited different trends in soil GHG fluxes and N substrates. Quistococha had higher levels of soil nitrate and ammonium compared to Zungarococha, which correlated with increased N2O emissions from Quistococha. A similar pattern was observed for CO2 emissions, with Quistococha producing higher levels than Zungarococha. Contrastingly, Zungarococha had higher soil moisture levels, which aligned with its lower N2O emissions. This forest also showed greater soil N2 emissions, suggesting the potential for complete denitrification. However, this site was also a significant source of CH4 emissions due to its higher soil moisture, which supports methanogenic activity. Overall, the two sites demonstrated distinct behaviors: Quistococha was a source of N2O and CO2, influenced by intermediate soil moisture. Zungarococha emitted higher levels of CH4 and N2 due to its high soil moisture conditions. The patterns in N2O fluxes are further supported by 15N isotopic mapping, correlating N2O emissions with their source processes. The site preference values fall within the denitrification zone at Zungarococha and the nitrification zone, with some hybrid processes in Quistococha.  The microbiome analyses show similar results, with denitrifying microbes dominating the Zungarococha soil and nitrifying microbes dominating the Quistococha soil.

How to cite: Masta, M., Kazmi, F. A., Espenberg, M., Pärn, J., Soosaar, K., and Mander, Ü.: Dynamics of N2O emissions from Amazonian tropical peat forest and partitioning N-processes using 15N isotopes., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6740, https://doi.org/10.5194/egusphere-egu25-6740, 2025.

Soil organic matter (SOM) consists of carbon and nitrogen, both of which can contribute to the production of nitrous oxide (N2O). Currently, there is ample focus on increasing soil carbon content as a strategy for climate mitigation. Yet, the role of SOM on N2O production is poorly understood. We will present field flux N2O measurements from a hillslope cultivated to cereals with a natural gradient in SOM, pH and soil moisture. Additionally, eight rain exclusion shelters (~50% drought) were installed along the gradient, and N2O fluxes were measured both under 50% reduced and normal rainfall conditions. N2O fluxes have been measured for two growing seasons and will be presented alongside with soil and yield characteristics.

How to cite: Dörsch, P. and Kjær, S. T.: Influence of soil organic matter and reduced rainfall on nitrous oxide emissions along a cultivated hillslope , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7923, https://doi.org/10.5194/egusphere-egu25-7923, 2025.

EGU25-8269 | Posters on site | BG1.3

Decreasing N deposition leads to significant decrease in foliar N concentrations in forest trees 

Inken Krüger, Andreas Schmitz, Catrin Stadelmann, and Tanja Sanders

Despite reduction of nitrogen emissions, deposition in German forests remain high. Eutrophication of ecosystems thus remains an important issue of scientific and socio-political interest. Here we analyse data from 78 intensive forest monitoring (Level II) sites operated by the forest research institutes of the German federal states as part of the ICP Forests network (International Co-operative Programme on Assessment and Monitoring of Air Pollution Effects on Forests). In the 2013-2022 period, mean annual bulk open field (inorganic + organic) deposition was between 4.4 and 13.5 kg N ha-1 a-1. Over the past twenty years, N deposition decreased by about 40 % which corresponds to a decrease of 2.5 % per year compared to the deposition in 2010. The decrease in N-NO3 (-3.1 % per year) was slightly higher than the decrease in N-NH4 (-2.7 %). Organic N deposition decreased by only 0.7 % per year. Canopy budget models show that N deposition (wet + dry + occult) to forest sites was between 10 and 31 kg N ha-1 a-1 over the same period.

The deposition data is used for reporting duties such as the German federal states’ core indicators of environmental quality (LIKI) and for scientific research e.g. to evaluate changes in biodiversity, dynamics of nutrient cycles and ensuing vulnerability of ecosystem services, or effects on tree vitality. We used the data to assess the impact of N deposition on foliar N concentrations, an import indicator of tree nutrition status. Tree nutrition influences vitality and trees’ resilience to climate extremes. A deterioration of foliar nutrients has been observed in forest ecosystems across Europe. At the German Level II sites, all main tree species (European beech, Norway spruce, Scots pine, sessile and pedunculate oak) show a significant decrease in foliar N concentration of 0.2-0.3 % per year. Besides nitrogen deposition, the reduction has been linked to various environmental factors, including increasing temperatures and changing precipitation patterns, as well as, the increase in atmospheric CO2 concentrations. At the spatial scale, nutrient availability can be explained by various site conditions such as parent material. Nonetheless, weak positive but significant relationships between mean foliar N and total N deposition for beech, oak, and pine for the 2013-2022 time period show that atmospheric deposition can explain part of the spatial variability between forest sites. The results indicate the importance of assessing deposition, trophy classes, and climate conditions at the same sites to fully understand their interaction.

How to cite: Krüger, I., Schmitz, A., Stadelmann, C., and Sanders, T.: Decreasing N deposition leads to significant decrease in foliar N concentrations in forest trees, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8269, https://doi.org/10.5194/egusphere-egu25-8269, 2025.

EGU25-8306 | ECS | Posters on site | BG1.3

Investigating Nitrous Oxide Pathways and Soil Carbon-Nitrogen Interactions Using Isotopic Techniques to Mitigate Greenhouse Gas Emission 

Sobia Bibi, Barira Shoukat Hafiza, Wolfgang Wanek, Magdeline Vlasimsky, Mariana Rabello, Maria Heiling, Gerd Dercon, Sandén Taru, Spiegel Adelheid, and Rebecca Hood-Nowotny

Effective management of carbon (C) and nitrogen (N) in agricultural soils is crucial for mitigating greenhouse gas (GHG) emissions, particularly nitrous oxide (N2O) and carbon dioxide (CO2). This study investigates innovative dual C and N isotope-based methods to explore the mechanisms driving N2O and CO2 production and their potential mitigation, while maintaining soil fertility. By applying selectively labelled fertilizers with labelled in both fractions (15NH4NO3 or NH415NO3) the microbial transformations of N in soil are traced, allowing for the identification of conditions that promote N2O production or its reduction to the environmentally benign N gas (N2).

The impact of different labile and recalcitrant C sources on N cycling and GHG emissions is investigated by applying 13C-labelled maize-derived plant litter and biochar. The interaction between labile-C (e.g., plant litter) and recalcitrant C (e.g., biochar) with N in soils plays a critical role in regulating microbial processes and, consequently, GHG emissions. Plant litter, as a labile C source, stimulates microbial activity, (i) enhancing N-cycling and potentially increasing N2O emissions or, alternatively, (ii) stimulating microbial inorganic N immobilization thereby reducing N availability to gaseous and hydrological N loss processes. In contrast, recalcitrant C, such as biochar, provides a stable C form with long term C storage potential in soils. Biochar with its large specific surface area is recognized for its ability to sorb inorganic N such as ammonium and nitrate, reducing its availability for microbial processes that produce N2O and thereby may mitigate soil N2O emissions. However, how C inputs and N availability influence each other and affect microbial processes linked to GHG emissions remains poorly understood.

To address these challenges, a large-scale incubation study was initiated using soils sampled from a field experiment in Grabenegg, Austria, conducted by, The University of Natural Resources and Life Sciences, Vienna (BOKU) and Austrian Agency for Health and Food Safety, Vienna (AGES). One experimental soil was amended with NPK fertilizer, while the other received both NPK and hardwood- derived biochar since 2022. Soil samples were collected from the upper 10 cm of the root zone in October 2024 and used in a laboratory mesocosm experiment to trace litter-C and biochar-C processing and their effects on soil inorganic N cycling using 15N and 13C isotope tracing and isotope pool dilution measurements. Key measurements, including emissionsof 15N2O, 15N2, and 13CO2, 13C tracing into particulate organic 13C, mineral-associated organic 13C, and microbial biomass 13C and, 15N tracing in, mineral-N (15NH4, 15NO3) and microbial 15N will be performed at various intervals over one month, and data evaluated using numerical modelling. Findings from this study will greatly contribute to optimizing climate-smart soil management practices aimed at reducing GHG emissions from soil while maintaining its fertility.  

How to cite: Bibi, S., Hafiza, B. S., Wanek, W., Vlasimsky, M., Rabello, M., Heiling, M., Dercon, G., Taru, S., Adelheid, S., and Hood-Nowotny, R.: Investigating Nitrous Oxide Pathways and Soil Carbon-Nitrogen Interactions Using Isotopic Techniques to Mitigate Greenhouse Gas Emission, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8306, https://doi.org/10.5194/egusphere-egu25-8306, 2025.

EGU25-9733 | ECS | Posters on site | BG1.3

Nitrogen transformation mediated by artificial root exudates derived from young alder and English oak trees 

Novalia Kusumarini, Iseult Lynch, Liam Cox, and Sami Ullah

Root exudates account for up to 17% of the carbon fixed from photosynthesis and are allocated belowground, where they significantly influence microbial communities that drive nutrient cycling, particularly nitrogen in the rhizosphere. Root C exudation for nitrogen acquisition may differ between tree types. This study aimed to investigate how root exudates from English oak (Quercus robur) influence nitrogen cycling in rhizosphere soils compared to soils under alder (Alnus glutinosa). We hypothesized that oak root exudates would prime faster N transformation, given that alder tree roots host nodules for biological nitrogen fixation and thus will not invest exudate C in nitrogen acquisition. We experimented to measure gross and net nitrogen mineralization rates in soils subjected to simulated oak- and alder-specific carbon exudation rates. The study was designed using three artificial root exudate concentrations: 0, 77, and 359 µg C g⁻¹ soil day⁻¹ for alder, and 0, 187, and 814 µg C g⁻¹ soil day⁻¹ for oak. Soils were collected from the top 15 cm of the mineral layer from a four-year-old monoculture plantation of oak and alder trees in Staffordshire, England. The artificial root exudates were based on the actual root exudate rates from alder and oak trees collected during the Summer of 2022 and Spring of 2023 and contained carbohydrates, amino acids, and organic acids. Nitrogen transformation responses in the incubated soils were measured on days 15 and 30. On day 15, half of the soils were recovered from the incubation chambers and subjected to 15N-N tracer addition to determine gross N mineralization. The study revealed that higher concentrations of root exudate significantly (p<0.001) enhanced microbial activity. This was evidenced by increased soil respiration (21-fold in the oak simulation and 10-fold in the alder), microbial biomass carbon (3-fold in both tree species), and microbial biomass nitrogen (6-fold in oak and 2-fold in alder simulations) compared to the control after 30 days of incubation. These changes contributed to a 282% increase in total dissolved nitrogen in the oak and a 140% increase in the alder simulations. Root carbon inputs altered both gross and net mineralization and nitrification rates. Higher exudate concentrations over longer incubation periods elevated gross mineralization rates by up to 20-fold in the oak but reduced by up to fivefold in the alder compared to controls. Net mineralization rates increased with exudate concentration in both species. In gross nitrification, oak exudates enhanced tenfold, while alder exudates increased eightfold compared to controls after 15 days. Gross mineralization strongly correlated with net mineralization (R²oak=0.92, R²alder=0.76) but showed weaker correlations with net nitrification (R²oak = 0.30, R²alder = –0.47). Oak root exudates exhibited higher responses across gross mineralization (lnRR=3.08), net mineralization (lnRR=2.50), and gross nitrification (lnRR=1.57) compared to alder. Our results demonstrate that higher oak exudation rates enhanced nitrogen cycling compared to alder, underscoring the importance of species-specific traits in shaping carbon allocation strategies and nutrient cycling in the rhizosphere. This research highlights the critical role of root exudation in regulating soil nutrient dynamics and has broader implications for forest management.

How to cite: Kusumarini, N., Lynch, I., Cox, L., and Ullah, S.: Nitrogen transformation mediated by artificial root exudates derived from young alder and English oak trees, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9733, https://doi.org/10.5194/egusphere-egu25-9733, 2025.

EGU25-9997 | ECS | Orals | BG1.3

Trade-off analysis of conventional and organic crop rotations under current and future climate scenarios in Finland 

Roberta Calone, Elena Valkama, Marco Acutis, Alessia Perego, Marco Botta, and Simone Bregaglio

Maintaining agricultural productivity while reducing soil organic carbon (SOC) loss, greenhouse gas emissions and groundwater contamination is a major challenge for European agriculture. Organic farming practices are expected to improve soil health and have increased their share of European cropland, but their effects on soil biogeochemical properties, biodiversity and nitrogen dynamics are mixed. This study uses the process-based ARMOSA crop model to assess the impact of conventional and organic farming practices on yield, SOC stock, nitrate (NO3) leaching, and nitrous oxide (N2O) emissions in both crop and livestock farms.

The research was carried out using simulations under current and projected future climate conditions in the South Savo region of Finland, which is characterised by a subarctic climate (Köppen-Geiger classification). The soil type was loamy sand (sand 76%, clay 4%, silt 20%) with a SOC content of 3.5%, a carbon-to-nitrogen ratio of 17, and a pH of 6.2 in the top 30 cm of the soil.

Five-year crop rotations that reflect prevalent practices in the area were designed for both crop and livestock production systems. Crop production rotations included cereals (with fodder peas in organic management), oilseed rape, and grass. Livestock farm rotations featured two years of cereals followed by a three-year fescue and timothy meadow (including clover in organic management). Nine scenarios were simulated to explore residue management and fertilisation strategies. Conventional systems used mineral fertilisers alone or combined with slurry. Organic systems used slurry, green manure, and a commercial organic fertiliser.

To evaluate the productivity and the environmental impact of these rotations, a fuzzy logic-based trade-off analysis was employed for each climate scenario. This analysis quantifies the trade-offs between crop yield, N2O emissions, NO3 leaching, and SOC stock changes. The result is a composite index known as the ∑ommit index. This index rates these trade-offs on a scale from 0 (poor) to 1 (excellent).  To accommodate diverse evaluation criteria, alternative versions of this trade-off analysis were implemented. Each version varies the weightings assigned to the trade-off components to mirror the perspectives and priorities of different representative stakeholder categories.

Using the ∑ommit index to evaluate a five-year rotation, rather than analysing individual cropping cycles, offers a significant advantage. This approach takes into account the interconnected effects of each cycle and its interactions with preceding and subsequent cycles. By considering these cumulative effects, the index provides a more comprehensive view of the trade-off dynamics during crop transitions. This holistic perspective is essential for making informed decisions about sustainable farming practices and long-term crop rotation strategies.

How to cite: Calone, R., Valkama, E., Acutis, M., Perego, A., Botta, M., and Bregaglio, S.: Trade-off analysis of conventional and organic crop rotations under current and future climate scenarios in Finland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9997, https://doi.org/10.5194/egusphere-egu25-9997, 2025.

EGU25-10246 | ECS | Orals | BG1.3

Global net cooling effects of anthropogenic reactive nitrogen: the unneglectable roles of short-lived nitrogen components 

Cheng Gong, Hanqin Tian, Hong Liao, Sian Kou-Giesbrecht, Nicolas Vuichard, Yan Wang, and Sönke Zaehle and the NMIP2 contributors

Anthropogenic activities have substantially enhanced the loadings of reactive nitrogen (Nr) in the Earth system since pre-industrial times, contributing to widespread eutrophication and air pollution. Increased Nr can also influence global climate through a variety of effects on atmospheric and land processes but the cumulative net climate effect is yet to be unravelled. Here we show that anthropogenic Nr causes a net negative direct radiative forcing of −0.34 [−0.20, −0.50] W m−2 in the year 2019 relative to the year 1850. This net cooling effect is not only as a result of the increased terrestrial carbon sequestration, but also led by short-lived Nr components and the associated atmospheric chemical reactions, including increased aerosol loading and reduced methane lifetime induced by nitrogen oxide (NOx). Such cooling effect is not offset by the warming effects of enhanced atmospheric nitrous oxide (N2O) and ozone (O3). However, despite the significant climate impacts of the short-lived nitrogen components, in particular, NOx, the associated soil biogeochemical processes remain poorly constrained, thus leading to varied responses to N fertilizer application as well as the estimates of global soil emissions among different approaches. Our results highlight the urgent necessities to integrate knowledge between atmospheric chemistry and soil biogeochemistry to improve the understanding of the Nr climatic effects.

How to cite: Gong, C., Tian, H., Liao, H., Kou-Giesbrecht, S., Vuichard, N., Wang, Y., and Zaehle, S. and the NMIP2 contributors: Global net cooling effects of anthropogenic reactive nitrogen: the unneglectable roles of short-lived nitrogen components, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10246, https://doi.org/10.5194/egusphere-egu25-10246, 2025.

EGU25-10603 | ECS | Orals | BG1.3

Landscape fluxes and dry deposition velocity of ammonia near a cattle feedlot using flux gradient approach 

Qingmei Wang, Thomas K. Flesch, and Deli Chen

Concentrated animal feeding operations (CAFOs) are emission hotspots of ammonia (NH3). The NH3 emitted from these hotspots can be locally recaptured by the surrounding vegetation, mainly due to dry deposition. This deposition can either have beneficial fertilizing effects for N-limited ecosystems or pose adverse impacts on sensitive ecosystems. However, there is a lack of direct measurements of NH3 deposition near hotspots. We conducted two field campaigns to investigate the landscape NH3 fluxes over the barley (winter), lentil (winter), and fallow (summer) fields adjacent to an intensive beef cattle feedlot in southeast Australia. The flux measurements were segregated into periods when the measurement location was upwind of the feedlot or downwind. Upwind of the feedlot, we observed upward fluxes (surface emissions) over the fallow and barley sites with daily means (± standard error) of 0.16 ± 0.02 and 0.007 ± 0.012 μg NH3 m-2 s-1, and downward fluxes (deposition) over the lentil site with a daily mean of -0.022 ± 0.007 μg NH3 m-2 s-1. These measurements indicated the NH3 compensation point for barley was approximately 6.2 μg m-3 (equivalent to the background atmospheric NH3 concentration), and the NH3 compensation point for lentils was lower than 3.4 μg m-3. Downwind of the feedlot, we observed downward fluxes at all sites with daily means of -0.57 ± 0.09 μg NH3 m-2 s-1 for the barley site, -1.26 ± 0.17 μg NH3 m-2 s-1 for the lentil site, and -0.58 ± 0.12 μg NH3 m-2 s-1 for the fallow site; the mean deposition velocities over the barley, lentil, and fallow sites were 0.74, 0.82 and 0.78 cm s-1. Based on the frequency of upwind and downwind periods, we estimate that the accumulated N inputs to the barley, lentil and fallow fields during each campaign were 4.5, 14.8 and 4.3 kg N ha-1, indicating that the deposition of NH3 emitted from the feedlot serves as a significant source of N input to its adjacent fields. Our study can provide valuable information on NH3 exchange between vegetation and atmosphere, and extend our understanding of the fate of NH3 emitted from hotspots.

How to cite: Wang, Q., Flesch, T. K., and Chen, D.: Landscape fluxes and dry deposition velocity of ammonia near a cattle feedlot using flux gradient approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10603, https://doi.org/10.5194/egusphere-egu25-10603, 2025.

EGU25-11361 | Posters on site | BG1.3

Standardization of a resistance model for the calculation of nitrogen deposition in the updated German standard VDI 3782-5 

Ulf Janicke, Sabine Banzhaf, Christian Brümmer, Thomas Gauger, Thomas Krämerkämper, Helmut Lorentz, Klaus Maßmeyer, Karsten Mohr, Alexander Moravek, Wolfgang J. Müller, Joachim Namyslo, Julia Nickel, Andreas Prüeß, Beat Rihm, Martijn Schaap, Andreas Schmitz, Andreas Tilgner, and Alfred Trukenmüller

The German standard VDI 3782-5 "Deposition Parameters" (German/English, www.vdi.de) provides deposition velocities and washout rates for various gaseous substances and particles. It is applied in local and mesoscale dispersion modelling, for example in the context of the German regulation on Air Quality Control (TA Luft). The current version of the standard dates from 2006. It is based on findings from a limited number of studies that led to the implementation of relatively simple descriptions and only rough estimates of atmospheric nitrogen deposition. The standard is currently undergoing a rigorous scientific revision by the authors on behalf of the VDI.

The updated standard will specify, among others, a model for the calculation of surface resistances, including compensation points for NH3. The model is based on DEPAC (RIVM, Netherlands) and implemented in Java program (JDepac). JDepac allows parameter variations and time series calculations. Input parameters include date and time, geographical location, land use, meteorological data and, for NH3, information on current and past loads. Default options are provided for missing input. Output quantities are, among others, resistances, deposition velocities, and deposition fluxes of NH3, NO, NO2, HNO3, SO2, O3, Hg and particles.

JDepac is compared to various deposition measurements and results from mesoscale models. For NH3, effects of the compensation point on the resulting deposition velocities are investigated. JDepac is used to calculate temporal averages of deposition velocities for different land use classes. In combination with dispersion calculations, effective deposition velocities are derived from the calculated deposition fluxes and concentrations. These simpler parameters are straightforward to apply in local dispersion modelling. JDepac itself allows more sophisticated calculations and can be coupled to dispersion and chemical transport models.

The updated standard VDI 3782-5 and its OpenSource tool JDepac are intended to serve as a state-of-the art, practical, and transparent reference for both local and mesoscale calculations of nitrogen deposition. In addition, the standard contains descriptions for the calculation of deposition velocities and washout rates of particles, the calculation of deposition probabilities for Lagrangian particle models, and the effects of drop displacement in wet deposition.

The updated standard is expected to serve as a useful tool for example in the decision process of facility planning and its licensing procedure conducted by local authorities, which is especially critical for the impact assessment on ecosystems under the EU Habitats Directive. In addition, the updated standard is expected to support the harmonization of air pollution modelling within the implementation of the new (2024) EU Ambient Air Quality Directive.

How to cite: Janicke, U., Banzhaf, S., Brümmer, C., Gauger, T., Krämerkämper, T., Lorentz, H., Maßmeyer, K., Mohr, K., Moravek, A., Müller, W. J., Namyslo, J., Nickel, J., Prüeß, A., Rihm, B., Schaap, M., Schmitz, A., Tilgner, A., and Trukenmüller, A.: Standardization of a resistance model for the calculation of nitrogen deposition in the updated German standard VDI 3782-5, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11361, https://doi.org/10.5194/egusphere-egu25-11361, 2025.

EGU25-11640 | ECS | Posters on site | BG1.3

Rhizobia inoculation to mitigate nitrous oxide (N2O) emissions from UK grasslands and herbal leys under intercropping systems. 

Katie Weir, Christopher Williamson, Tom Williams, and Fotis Sgouridis

N2O is a potent greenhouse gas, with ~300 times the warming potential of carbon dioxide.  The current trajectory for N2O emissions follows the highest warming RCP8.5 scenario, with agriculture accounting for ~70% of global emissions.  As demand for food and livestock feed is expected to increase, mitigation measures which reduce agricultural N2O emissions and simultaneously increase nitrogen use efficiency (NUE) are urgently required to limit warming below the 2°C target set by the Paris Agreement.

The promotion of biological nitrogen fixation (BNF) in crop and forage systems via the incorporation of legumes has been advocated as a N2O mitigation strategy because it reduces synthetic N fertiliser application and increases NUE.  However, novel strategies suggest that in addition to BNF, manipulation of the soil microbiota could hold the key to N2O mitigation.  Soybean studies have successfully identified strains of symbiotic N-fixing rhizobia which can reduce N2O because they possess the gene encoding for nitrous oxide reductase (nosZ).  The potential of N2O-reducing (NosZ+) rhizobia inoculums could therefore be critical to agricultural N2O emission mitigation; however, few studies have explored other legume-rhizobia associations for NosZ+ strains.  Most notable is the complete lack of research on permanent grassland ecosystems, which cover 40% of global land surface and account for 54% of global N2O emissions.

This study aims to investigate the potential of clover-rhizobia associations to mitigate N2O emissions from UK grasslands and herbal leys under intercropping systems.  Soils from five different land uses were sampled from FarmED (agroecology demonstration farm) and Pudlicote Farm in the Cotswolds, UK: unfertilised permanent pasture, unfertilised clover/grass sward, herbal ley (1st and 5th year) and conventionally farmed winter wheat.  Native rhizobia present in the soil samples were selected by the growth and nodulation of Red Clover (Trifolium pratense) plants.  Rhizobia extracted from the harvested root nodules were cultured on yeast mannitol agar to isolate individual strains.  Strains then underwent gDNA extraction and whole-genome sequencing using the Illumina NovoSeq X platform to determine the presence of the nosZ gene.  Biogeochemical analysis of the soils was related to the presence/absence of the nosZ gene to infer potential genotype environmental controls.

Finally, identified NosZ+ strains will undergo a phenotype assessment using a soil-plant-atmosphere mesocosm experiment, whereby N2O emissions from clover plants inoculated with NosZ+ strains will be monitored. Control strains; Rhizobium leguminosarum bv.trifolii T117 (nosZ+) and T132 (nosZ-) were obtained from the MIAE collection (INRAE, France) and will be tested alongside Bradyrhizobium diazoefficiens G49 (nosZ+) (soybean specific strain) and the identified native strains. The overall aim of the study is to create a rhizobia inoculum able to reduce N2O emissions when included in the intercropping sequence of leys and pastures, thus contributing to Net Zero global strategies.

How to cite: Weir, K., Williamson, C., Williams, T., and Sgouridis, F.: Rhizobia inoculation to mitigate nitrous oxide (N2O) emissions from UK grasslands and herbal leys under intercropping systems., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11640, https://doi.org/10.5194/egusphere-egu25-11640, 2025.

EGU25-11830 | ECS | Orals | BG1.3

The role of tree pollen in forest nitrogen cycling: A laboratory perspective 

Ivan Limić, Samuel Bodé, Pascal Boeckx, Marijn Bauters, Johan Neirynck, Nicolas Bruffaerts, Stribor Marković, Elena Gottardini, and Arne Verstraeten

Pollen is a critical component of the nitrogen (N) cycle in forests, but its role in N uptake, release and transformation during precipitation events remains poorly understood, contributing to uncertainties in N deposition estimates. In the frame of the COST Action CLEANFOREST a laboratory experiment was conducted to assess the biochemical activity of tree pollen and its effects on N compounds in precipitation. Pollen from green alder (Alnus viridis), pedunculate oak (Quercus robur), European beech (Fagus sylvatica), silver birch (Betula pendula), Scots pine (Pinus sylvestris) and Norway spruce (Picea abies) was suspended in a synthetic nitrate (NO₃-) solution isotopically labelled with ¹⁵N under non-sterilized conditions and two sterilization treatments: addition of (i) thymol and (ii) a broad-spectrum antibiotic mixture (PSA) containing penicillin, streptomycin, and amphotericin B. Over one week, water samples were analysed daily for NO₃-, nitrite (NO₂-), ammonium (NH₄⁺) and total dissolved nitrogen (TDN) from which dissolved organic nitrogen (DON) was calculated. The results showed significant NO₃- removal from the solution in broadleaved species, particularly oak, beech, and alder, in all treatments, but most clearly in the non-sterilized treatment. Most species showed a significant decrease in DON during the first two-three days, in all treatments, but especially in the sterilized (PSA) treatment, which was subsequently converted into NH₄⁺ (mineralization). The use of 15N as a tracer clearly shows that the labelled N was actively taken up by the pollen in both the non-sterilized and PSA-treated samples. Notably, pollen from all tree species, predominantly the broadleaves, enzymatically transformed extracellular NO₃- into NO₂-, highlighting its active role in the N cycle. These findings offer valuable insights into N release, uptake, and transformation during precipitation events and reveal important interactions between pollen and microorganisms. The differences observed between sterilized and non-sterilized treatments underline the significant influence of microbial activity on N conversion. By expanding our understanding of canopy-level N processes, this research contributes to improving N deposition models and introduces innovative approaches to studying the forest N cycle. Further studies are essential to clarify the mechanisms by which pollen and microbial communities influence N transformations at ecosystem scales.

Keywords: Broadleaves; Conifers; Pollen; ¹⁵N; Ammonium; Nitrate; Nitrite

How to cite: Limić, I., Bodé, S., Boeckx, P., Bauters, M., Neirynck, J., Bruffaerts, N., Marković, S., Gottardini, E., and Verstraeten, A.: The role of tree pollen in forest nitrogen cycling: A laboratory perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11830, https://doi.org/10.5194/egusphere-egu25-11830, 2025.

Global changes caused by anthropogenic activities are altering the cycling of nitrogen (N) in terrestrial ecosystems. For example, droughts of increasing frequency and severity can stimulate large emission pulses of nitrous oxide (N2O; a powerful greenhouse gas) when dry soils wet up. Further, increased fire frequency can favor the colonization of novel pyrophilous or “fire-loving” fungi on soils with the capacity to produce N2O, yet N2O isotopic ranges have been characterized in few fungal species, making generalizations difficult. To better understand how global changes are altering the N cycle, we studied drylands in southern California that can experience >6 months without rain, burned experimental “pyrocosms” to assess impacts of fire severity on soil biogeochemistry, and used a culture collection of pyrophilous fungi isolated from wildfire-burned soils to characterize their δ15N2Obulk,δN218Obulk, and δ15N2OSP values. Despite the hot and dry conditions known to hinder denitrification, isotope tracers and natural abundance isotopologues of N2O indicated NO3- was reduced within 15 minutes of wetting dry desert soils and that N2O reduction to N2 occurred. In post-fire environments, we found that while N2O isotope values for Neurospora discreta and Fusarium tricinctum closely matched literature values when grown with NO2-, Aspergillus fumigatus, Coniochaeta hoffmannii, Holtermaniella festucosa, and R. columbienses did not. Further, Fusarium sp. δ15N2Obulk and δN218Obulk values fell outside literature-derived values when grown with NO3-. Overall, we find that despite the hot and dry conditions known to make denitrification thermodynamically unfavorable in many drylands, denitrifiers can endure through hot and dry summers and are key to producing the surprisingly large N2O emissions when dry desert soils wet up. Further, we find that novel pyrophilous fungi present an opportunity to further characterize the isotopic composition of N2O as well as the factors controlling fungal denitrification as ecosystems are impacted by global changes.

How to cite: Homyak, P.: Drought, wildfires, and “fire-loving” fungi effects on ecosystem nitrogen cycling: Understanding global change effects on denitrification using N2O isotopologues, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12451, https://doi.org/10.5194/egusphere-egu25-12451, 2025.

EGU25-12860 | Orals | BG1.3

Impact of wet nitrogen deposition on soil nitrogen emissions in West African ecosystems 

Claire Delon, Corinne Galy-Lacaux, Dominique Serça, Money Ossohou, Moussa Zouré, Sébastien Barot, Xavier Le Roux, Ousmane Ndiaye, Silué Siélé, Adjon Kouassi, Eric Gardrat, Maria Dias-Alves, and Océane Lenoir

Human activities such as fertilization of agricultural lands and human-induced biomass burning strongly impact nitrogen (N) dynamics and losses, with many consequences on the environment. The quantification of N budgets (N inputs and outputs) between the surface and the atmosphere is a prerequisite to understand the N biogeochemical cycle, i.e. how N is transferred from the atmosphere to the biosphere, through the soil and back to the atmosphere from surface emissions. Sub Saharan Africa (SSA) is characterized by an increase in demography, with strong impacts on biodiversity, and on the sustainability of human activities including agriculture. In Africa, the increase in demography and the associated increased fertilizer inputs (to supply growing food and energy demands) will lead to increased emissions from amended soils, which will in turn increase atmospheric N deposition and induce feedbacks to the ecosystems and the atmosphere.

In this context, the NitroAfrica project (2023-2026) is designed to study the impact of N wet deposition on the soil – plant – atmosphere continuum. We make the hypothesis that changes of wet N deposition in West African ecosystems over the 21th centuries will induce important changes in biogenic emissions from the ecosystems to the atmosphere with impacts on regional atmospheric chemistry and further N deposition. Indeed, increasing trends of N wet deposition has already been observed, especially in the NH4+ form. Three ecoclimatic zones in West Africa are studied, in Guinean (Lamto, Côte d’Ivoire), Sudanese (Korhogo, Côte d’Ivoire) and Sahelian (Dahra, Senegal) zones, where solutions with different NH4+/NO3- partition are used to mimic the increase in N wet deposition.

Results on N (N2O, NO) and CO2 emissions from soils from plots amended with solutions as well as control plots will be presented. N wet deposition fluxes from recent years will also be presented within the context of existing long-term studies on N wet deposition. This comparison is particularly relevant for the Lamto station where the International Network to study Deposition and Atmospheric chemistry in Africa (INDAAF) is based and provides long-term data since 1995.

This study contributes to fill in the lack of studies in SSA, and to understand the processes involved in N emissions and deposition in tropical regions.

How to cite: Delon, C., Galy-Lacaux, C., Serça, D., Ossohou, M., Zouré, M., Barot, S., Le Roux, X., Ndiaye, O., Siélé, S., Kouassi, A., Gardrat, E., Dias-Alves, M., and Lenoir, O.: Impact of wet nitrogen deposition on soil nitrogen emissions in West African ecosystems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12860, https://doi.org/10.5194/egusphere-egu25-12860, 2025.

EGU25-14072 | Orals | BG1.3

Hotspots and hot moments of DNRA in the Vadose Zone of Agricultural Croplands  

Jun Shan, Xiaomin Wang, and Xiaoyuan Yan

High nitrogen (N) input in intensive cropping systems has resulted in significant nitrate (NO₃⁻) accumulation in agricultural soils of China. However, despite substantial N input (500-600 kg ha-1 y-1) in the Taihu Lake region, NO₃⁻ accumulation in soils and groundwater therein remains minimal with the mechanisms behind are unclear. Here, we investigated the spatiotemporal distribution and activity of dissimilatory nitrate reduction to ammonium (DNRA), anaerobic ammonium oxidation (anammox), and denitrification, and the associated microbial communities—in the vadose zones of rice-wheat, vegetable, and orchard fields of the Taihu Lake region. Results revealed NO₃⁻ content decreased progressively with soil depth, while NH₄⁺ levels increased, particularly in deeper soil layers. DNRA emerged as the primary pathway for NO₃⁻ reduction, contributing to over 50% of NO₃⁻ removal, especially in the 50–190 cm depth range. Seasonal variations indicated that DNRA activity was highest during spring and autumn, with lower rates observed in winter and summer. DNRA significantly contributed to NH₄⁺ accumulation, with rates strongly positively correlated with NH₄⁺ content, especially in rice-wheat rotation fields characterized by high OC/ NO₃⁻ ratios. Interestingly, DNRA rates were significantly negatively correlated with groundwater N₂O concentrations and the N₂O/(N₂ + N₂O) ratios. Microbial community analysis revealed that the nrfA gene, a marker for DNRA, exhibited higher diversity compared to genes related to denitrification. Additionally, the abundance of DNRA-specialist microbes was positively associated with DNRA rates, particularly in deep layer soils, emphasizing the role of microbial community composition in shaping DNRA activity. These findings demonstrate that DNRA plays a crucial role in facilitating NH₄⁺ accumulation, attenuating NO₃⁻ accumulation, and mitigating N₂O emission in the vadose zone of agricultural croplands in the Taihu Lake region.

How to cite: Shan, J., Wang, X., and Yan, X.: Hotspots and hot moments of DNRA in the Vadose Zone of Agricultural Croplands , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14072, https://doi.org/10.5194/egusphere-egu25-14072, 2025.

EGU25-14338 | ECS | Posters on site | BG1.3

Estimating the Tipping Point between N2O Emissions and C Sequestration in Soil using the DNDC v. CAN Model 

Meng Kong, Huan Liu, Diego Abalos, Brian B. Grant, Ward N. Smith, Azhar Zhartybayeva, Johannes L. Jensen, Jørgen Eriksen, and Christian Dold

Increasing the grassland proportion in the crop rotation has been considered as an effective approach to sequester carbon (C) in the soil. However, its climate mitigation benefits may be overestimated because the associated impact of long-term C sequestration on nitrous oxide (N2O) emissions remains uncertain. Mechanistic models, such as the DeNitrification and DeComposition model (DNDC v. CAN 9.5.0), are used to simulate changes in soil organic carbon (SOC) and N2O emissions. This provides the opportunity to estimate future emission trends and to enhance our understanding of the interactions between SOC and N2O emissions under different levels of grass/clover proportion in arable crop rotations. We hypothesize that increases in N2O emissions will offset the benefits from the increased SOC over time. The objectives of this study are to (1) calibrate and validate the DNDC model, and (2) estimate and predict the potential tipping point at which the negative climate forcing of N2O emissions offsets the benefits of C sequestration over long-term timescales. For this, we used long-term measurements of biomass, SOC, and N2O emissions from two crop rotations with either two or four years of grass-clover in a six-year rotation in Denmark. Preliminary results showed that the DNDC model simulated crop biomass production with fair to high accuracy as indicated by an index of agreement (d) of 0.98, a Nash-Sutcliffe efficiency (NSE) of 1, and a normalized root mean square error (nRMSE) of less than 30%. The simulated biomass was slightly underestimated as shown by a negative mean bias error (MBE). Conversely, the simulations for N2O fluxes and SOC exhibited poorer agreement, with d-values below 0.7 and nRMSE exceeding 30%. These findings suggest that while the DNDC model effectively predicts crop growth, including annual crops and grass/clover ley, its ability to simulate SOC and N2O fluxes requires substantial improvement. Our future efforts will focus on refining and optimizing model parameters for SOC and N2O, with an emphasis on calibration to enhance the model performance and the capacity to predict management-induced long-term dynamics under future climate scenarios. Results of these updated model simulations will be shown at the conference.

How to cite: Kong, M., Liu, H., Abalos, D., Grant, B. B., Smith, W. N., Zhartybayeva, A., Jensen, J. L., Eriksen, J., and Dold, C.: Estimating the Tipping Point between N2O Emissions and C Sequestration in Soil using the DNDC v. CAN Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14338, https://doi.org/10.5194/egusphere-egu25-14338, 2025.

Atmospheric nitrogen (N) deposition is a significant driver of global change and disrupts the carbon and nitrogen cycles in ecosystems. Volatile Organic Compounds (VOCs) emitted by plants play an important role in regional air quality and the carbon cycle. This study investigates the effects of different forms and doses of N deposition on Biogenic Volatile Organic Compounds (BVOCs) emissions, photosynthesis, growth, and non-structural carbohydrate (NSC) accumulation in the widespread subtropical bamboo species-Moso bamboo (Phyllostachys edulis). A pot experiment was conducted with three N doses: 100 kg(N)·hm⁻²·a⁻¹ (L1), 200 kg(N)·hm⁻²·a⁻¹ (L2), and 0 kg(N)·hm⁻²·a⁻¹ (L0), using ammonium N (AN), nitrate N (NN), and a mixed N form (AN+NN). Dynamic headspace sampling was used to assess the effects of N deposition on BVOC emissions and the relationships between N deposition, photosynthesis, plant growth, and NSC distribution throughout the growing season.

The results indicated that N deposition increased BVOC emissions, with the highest emissions occurring under NN treatment at L1 during March and June. Isoprene (ISO) emissions were significantly enhanced under AN treatment, with L2 doses increasing ISO emissions by 99.20% compared to L1. The AN+NN treatment resulted in higher ISO emissions at L2, with increases of 76.02% and 141.69% compared to AN and NN alone, respectively. N form and dose also influenced photosynthetic pigments, with the highest total chlorophyll content observed under AN+NN at L1. Photosynthetic parameters, including net photosynthetic rate (Pn), stomatal conductance (Gs), and carboxylation efficiency (CE), were significantly higher under L1 compared to L0. A positive correlation was found between chlorophyll content and VOC emissions, with Pn, Gs, and CE strongly correlating with ISO emissions. Growth responses varied by N form. AN+NN treatment significantly promoted the growth of Phyllostachys edulis, particularly in above-ground biomass, while AN inhibited root and whip growth. Biomass of leaves and culms was significantly higher under L1 treatment, with increases of 85.60% and 38.14%, respectively, compared to L0 under AN treatment. Soluble sugar content in leaves, culms, and roots was highest at L1, with decreases observed as the N dose increased. Soluble sugars in leaves, culms, and buds increased by 24.85%, 24.92%, and 21.20% under L1 compared to L0. Starch content in leaves and culms increased initially but declined under higher N doses. AN and NN treatments at L2 reduced starch content in leaves and culms, with significant reductions observed in both N forms.

NSC content was positively correlated with ISO emissions, especially for soluble sugars. Total NSC content and soluble sugars were also positively correlated with BVOC emissions, suggesting that NSCs play a key role in plant responses to environmental stress. In conclusion, N deposition—particularly in mixed forms (AN+NN)—enhances BVOC emissions, especially ISO emissions, promotes biomass accumulation, and improves photosynthetic capacity. Lower N doses support higher ISO emissions and NSC accumulation. This study highlights that appropriate levels of N deposition can support bamboo growth and improve resilience to atmospheric changes.

How to cite: Li, L., Jiang, M., and Wang, X.: Effects of nitrogen deposition on VOCs emission and its relationship with photosynthesis, growth, accumulation and distribution of NSC in Moso bamboo tree (Phyllostachys edulis) , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14982, https://doi.org/10.5194/egusphere-egu25-14982, 2025.

EGU25-15249 | ECS | Posters on site | BG1.3 | Highlight

Changing patterns of global nitrogen deposition driven by socio-economic development 

Jianxing Zhu, Guirui Yu, and Qiufeng Wang

Advances in manufacturing and trade have reshaped global nitrogen deposition patterns, yet their dynamics and drivers remain unclear. Here, we compile a comprehensive global nitrogen deposition database spanning 1977–2021, aggregating 52,671 site-years of data from observation networks and published articles. This database show that global nitrogen deposition to land is 92.7 Tg N in 2020. Total nitrogen deposition increases initially, stabilizing after peaking in 2015. Developing countries at low and middle latitudes emerge as new hotspots. The gross domestic product per capita is found to be highly and non-linearly correlated with global nitrogen depositiondynamic evolution, and reduced nitrogen deposition peaks higher and earlier than oxidized nitrogen deposition. Our findings underscore the need for policies that align agricultural and industrial progress to facilitate the peak shift or reduction of nitrogen deposition in developing countries and to strengthen measures to address NH3 emission hotspots in developed countries.

How to cite: Zhu, J., Yu, G., and Wang, Q.: Changing patterns of global nitrogen deposition driven by socio-economic development, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15249, https://doi.org/10.5194/egusphere-egu25-15249, 2025.

EGU25-15354 | ECS | Orals | BG1.3

The effect of drought and rewetting on nitrogen cycling and nitrous oxide emissions in a controlled experiment with different cover crop species 

Pauliina Turunen, Anne Viinikainen, Markku Koskinen, Asko Simojoki, Kristiina Karhu, and Mari Pihlatie

Cover crops are recognized as a climate-smart agricultural practice that increases soil organic carbon content (SOC). As carbon (C) and nitrogen (N) cycles are coupled, an increase in SOC can impact the N cycle and nitrous oxide (N2O) emissions. Another major driver affecting N cycling and N2O emissions is soil moisture. With the increasing risk of summer droughts and wetter conditions during the off-season in Northern Europe, it is important to understand how drying-wetting and agricultural practices together affect N cycling and N2O emissions.

To address this knowledge gap, we conducted a pot experiment with clay soil in controlled greenhouse conditions simulating summer drought with bare soil pots and oats sown either alone, with Italian ryegrass, or with alfalfa as plant treatments. The pots were initially watered to 70% degree of saturation to ensure that the plants start to grow, after which half the pots were let dry to 40% degree of saturation. The plants were grown for 36 days. At the end of the growth period, soil N2O emissions were measured over three days. Following this, the pots were sampled destructively, and total N in plants, roots, and soil, as well as mineral N in soil, were analysed. Additionally, a follow-up pool-dilution incubation experiment using 15N-labelling with bare soil and soil previously covered with oats was conducted to study the effect of moisture content and rewetting on gross N transformation rates.

Contrary to our expectations, the results from the pot experiment showed that N2O emissions in the plant treatments were higher in drought conditions than in moist conditions. This does not support our results from a cover crop field trial where reduced rainfall did not affect N2O emissions during the growing season. However, during off-season reduced rainfall in the field led to higher N2O emissions. Preliminary results from the incubation indicated lower N2O emissions under drought conditions, with increased emissions upon rewetting and the highest emissions under moist conditions. The presence of plants decreased soil N2O emissions in both experiments, but the plant species did not affect the emissions nor the total mineral N content in soil. As expected, in the pot experiment, total mineral N content in soil was higher in drought conditions than in moist soil as well as in bare soil compared with soil with growing plants. Results on the effects of drought and plants on gross N transformations during the incubation experiment with 15N labelling will be presented later.

How to cite: Turunen, P., Viinikainen, A., Koskinen, M., Simojoki, A., Karhu, K., and Pihlatie, M.: The effect of drought and rewetting on nitrogen cycling and nitrous oxide emissions in a controlled experiment with different cover crop species, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15354, https://doi.org/10.5194/egusphere-egu25-15354, 2025.

EGU25-15383 | Orals | BG1.3

Mechanisms of soil emissions of NO and HONO produced by ammonia-oxidizing bacteria during drying 

Bettina Weber, Stefanie Maier, Jens Weber, Diego Leiva, Min Zhou, Xiaoyong Qian, Ulrich Pöschl, Yafang Cheng, Hang Su, and Minsu Kim

Nitric oxide (NO) and nitrous acid (HONO) are important reactive atmospheric trace gases. As part of the nitrogen (N) cycle, ammonia oxidizing nitrifiers in soils are recognized as key producers of these gases, impacting near-surface nitrogen oxide (NOx = NO + NO2) and ozone (O3) concentrations. The nitrification process results in the production of nitrite (NO2-), subsequently protonated in the liquid phase to form HONO, and NO, which are both emitted as gases. However, there is limited understanding of the coupled processes causing the simultaneous emission NO and HONO from drying soils incorporating ammonia oxidizing nitrifiers. Here, we combined experimental in-vitro studies of ammonia-oxidizing bacteria with a mechanistic modelling approach to investigate the mechanisms triggering gaseous NO and HONO emissions. We found out that several abiotic processes, such as NO auto-oxidation, Fe2+ catalysis, and soil moisture dynamics crucially influence the overall emission as well as the partitioning of reactive N. This, in turn, impacts the hydroxyl radical (OH) budget and soil N retention. Modelling allowed us to elucidate the interactions between biological and environmental processes under varying soil hydration conditions for different field scenarios, such as the effects of fertilization. This analysis suggests potential strategies for effectively managing the release of soil-derived NOx and OH emissions.

How to cite: Weber, B., Maier, S., Weber, J., Leiva, D., Zhou, M., Qian, X., Pöschl, U., Cheng, Y., Su, H., and Kim, M.: Mechanisms of soil emissions of NO and HONO produced by ammonia-oxidizing bacteria during drying, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15383, https://doi.org/10.5194/egusphere-egu25-15383, 2025.

EGU25-15466 | Posters on site | BG1.3

Cover crop diversity and summer drought increase off-season N2O emissions from Finnish agricultural soil  

Mari Pihlatie, Pauliina Turunen, Markku Koskinen, Asko Simojoki, Anne Viinikainen, Osmo Virta, and Jussi Heinonsalo

The use of cover crops in agriculture is one of the climate-smart practices that have multiple benefits, such as increasing SOC, reducing N losses, and increasing biodiversity. Still the question whether cover crops and their diversity increase resilience against drought, and how the combined effects of cover crops, their diversity and drought affect N2O emissions, remain largely unknown. We study the combined effects of cover crop diversity and drought on cropland (oat) greenhouse gas emissions and belowground C and N processes in a field plot trial. The effect of drought on soil and crop C and N dynamics and greenhouse gas (CO2, N2O) emissions is studied with rainout shelters that remove 50% of incoming precipitation. The CO2 and N2O emissions are measured with the manual dark chamber method twice a week during the growing season and once a week during off-season, soil temperature and water content are measured continuously, and soil is sampled for mineral N and total C and N analysis seasonally.

The preliminary results show that reduced rainfall decreases CO2 emissions but does not affect N2O emissions significantly during the growing season. During off-season, reduced rainfall increases both CO2, and particularly N2O emissions irrespective of cover crop diversity treatments. During growing season there is a tendency of higher N2O emissions from diverse cover crop treatments compared to oat only treatment, and during off-season, a higher cover crop diversity significantly increases N2O emissions. Overall and in all treatments, off-season N2O emissions dominate the annual N2O balance. Our results highlight the need to include off-season measurements to the annual N2O balance estimation, and when assessing the effects of cover crops and future climate change scenarios such as summer drought on annual N2O emissions.

 

How to cite: Pihlatie, M., Turunen, P., Koskinen, M., Simojoki, A., Viinikainen, A., Virta, O., and Heinonsalo, J.: Cover crop diversity and summer drought increase off-season N2O emissions from Finnish agricultural soil , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15466, https://doi.org/10.5194/egusphere-egu25-15466, 2025.

EGU25-16227 | ECS | Orals | BG1.3

Phosphorus addition impacts on soil nitrogen dynamics in a subtropical plantation 

Huijun Ye, Huiying Lin, Muhammed Mustapha Ibrahim, Leiru Chen, Yang Liu, Roland Bol, and Enqing Hou

Human activities have globally increased atmospheric nitrogen (N) deposition, which has enhanced the risk of ecosystem N losses. Phosphorus (P), as a macroelement required for life, is closely linked to the biogeochemical cycle of N. Therefore, quantifying how soil N cycle responds to different P supply levels is important. Here we examined the responses of soil N dynamics to altered P supply using a P addition experiment (+0, +25, +50, +100 kg P ha−1 yr−1) in an evergreen broadleaf mixed plantation in subtropical China. We found that P addition led to a more open soil N cycle in the forest ecosystem. The primary source of N2O emissions in the study plots was fungal denitrification, which accounted for 41%-52% of the total N2O emissions, based on δ18O-N2O, δ15Nα-N2O, δ15Nbulk-N2O and SP measurements. Nitrogen loss by gas or water and N assimilation by plants were found to be coupled processes at +25 kg P ha−1 yr−1 addition level. The δ15N-NO3 and δ18O-NO3 values in runoff and leaching water from different depths were all depleted from −10‰ to +0‰ in the wet season. This result indicates that soil N has a short residence time and rapid NO3-N loss in the forest ecosystem, and with fewer nitrogen conversions according to the isotope fractionation theory. These observed varied responses of soil N transformation, gaseous loss, and liquid loss to different P supply levels provide new insights into our understanding of N-P relationships in broadleaf forest plantations.

How to cite: Ye, H., Lin, H., Ibrahim, M. M., Chen, L., Liu, Y., Bol, R., and Hou, E.: Phosphorus addition impacts on soil nitrogen dynamics in a subtropical plantation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16227, https://doi.org/10.5194/egusphere-egu25-16227, 2025.

EGU25-17098 | ECS | Posters on site | BG1.3

Microbial nitrogen cycling in wetland forests with varying management statuses across Europe 

Laura Kuusemets, Kaido Soosaar, Maarja Öpik, Mika Aurela, Aldis Butlers, Laura Escarmena, Jyrki Jauhiainen, Sari Juutinen, Rana Kanaan, Tuula Larmola, Andis Lazdiņš, Ülo Mander, José Miguel Sánchez Pérez, Sílvia Poblador, Francesc Sabater, Sabine Sauvage, Thomas Schindler, Liisa Ukonmaanaho, and Mikk Espenberg

Temperature and oxygen content in soil are the well-known drivers of macronutrient cycling, as they influence the overall conditions that regulate microbial metabolism. However, the more detailed underlying aspects affecting nutrient cycling remain insufficiently understood.

This study focuses on different wetland forest types across Europe, aiming to investigate N cycling processes, the spatial distribution of N cycling genes and the linkage with soil greenhouse gas (GHG) emissions and relevant environmental parameters. The study sites were located in Finland, Estonia, and Latvia in Northern Europe, as well as in France and Spain in Southern Europe. The Northern Europe sites consisted of drained peatlands with varying management statuses, while the Southern Europe ones were alluvial forests. Soil samples were collected from three depths (0-10, 10-20, 20-40 cm) in autumn 2023, analysed using quantitative polymerase chain reaction (qPCR), and sequenced to assess processes and communities. In all samples, soil physico-chemical parameters were also determined and simultaneously with soil sampling, in-situ GHG emission measurements were done all as a part of Horizon Europe ALFAwetlands project.  

Preliminary results of the quantification of N cycle genes revealed differences in the microbiome across wetland forest types in Europe. Ammonia-oxidizing archaea appeared to be the primary nitrifiers in the soils of the study sites, compared to ammonia-oxidizing bacteria. The alluvial forest soils revealed a higher genetic potential for the DNRA (Dissimilatory Nitrate Reduction to Ammonium) process in soil. The abundance of genes responsible for the comammox process—complete ammonia oxidation by a single microorganism—was also higher in the soils of the alluvial forests. In the rewetted peatland forest of Latvia, the soil exhibited a greater genetic potential for denitrification and DNRA processes compared to the drained peatland forests. The further analyses will be exploring the links between N cycle genes, GHG emissions, and soil physico-chemical properties.

 

 

How to cite: Kuusemets, L., Soosaar, K., Öpik, M., Aurela, M., Butlers, A., Escarmena, L., Jauhiainen, J., Juutinen, S., Kanaan, R., Larmola, T., Lazdiņš, A., Mander, Ü., Sánchez Pérez, J. M., Poblador, S., Sabater, F., Sauvage, S., Schindler, T., Ukonmaanaho, L., and Espenberg, M.: Microbial nitrogen cycling in wetland forests with varying management statuses across Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17098, https://doi.org/10.5194/egusphere-egu25-17098, 2025.

EGU25-17316 | Posters on site | BG1.3

The GreenEO Project: Satellite-Based Services to Support Sustainable Land Use Practices Under the European Green Deal 

Paul Hamer, Lise Marie Frohn, Camilla Geels, Jesper Christensen, Bruce Rolstad Denby, David Simpson, Nicholas Hutchings, Susana Lopez-Aparicio, Philipp Schneider, Tuan-Vu Cao, Isadora Jiminez, Thais Fontenelle, Ronald van der A, Bas Mijling, Jieying Ding, Isabel Trigo, Jean-Christophe Calvet, Joanne Schante, Thomas Judes, and Leonor Tarrason and the GreenEO Consortium

We present a new Horizon Europe project titled GreenEO (2025-2029) as well as findings based on advances in modelling within the Nordic Nature & Nitrogen (Nordic Council of Ministers, 2021-2024) and the SEEDS (Horizon 2020, 2021-2023) projects. The ambition of GreenEO is to support governance approaches for the implementation of EU’s Green Deal. The implementation of which will rely on accessible, actionable environmental data for policymaking and monitoring. Success will be dependent on the usage of the latest observational data as well as on the level of uptake of these data by end-users. GreenEO addresses this by using observations from the Sentinel and newest meteorological (MTG and Metop-SG) satellites, and through co-creation with users of high-resolution services and novel indicators to directly meet user needs.

GreenEO will specifically address the environmental impacts of nitrogen deposition and advance the state of knowledge on this topic within the context of supporting the EU’s Green Deal and its ambition for protecting biodiversity.

Current data on nitrogen emissions, deposition, and biodiversity impacts are inconsistent and lack sufficient spatial resolution. GreenEO will therefore try to advance the state of knowledge in three areas:

  • Using advanced satellite data, data assimilation, modeling, and ancillary data, GreenEO will estimate high-resolution nitrogen emissions (NH3, NOx). These high-resolution emissions will then be used in turn as a basis for modelling downstream impacts.
  • GreenEO will advance the state of the art for nitrogen deposition modelling using findings from previous projects (Nordic Nature & Nitrogen and SEEDS projects). A bi-directional flux parameterization (Wichink-Kruit et al., 2012) was added to three regional scale air quality models (DEHM, MATCH, and EMEP) within the Nordic Nature and Nitrogen project. The findings were that this approach did not lead to consistent improvements in ambient concentration and flux modelling without commensurate improvements in land cover and vegetation data. For instance, bi-directional fluxes were shown to be highly sensitive to leaf area index (LAI) due to the dominating pathway being through external leaf water. Work within the SEEDS project to derive improved estimates of LAI by combining satellite observations of LAI in a land surface model using data assimilation, will serve as a basis for improving estimates of the bi-directional depositional fluxes of reactive nitrogen.
  • GreenEO will combine these methods and data with regional scale air quality models (DEHM and EMEP) in order to model the distribution of nitrogen deposition with high accuracy. Specific attention will be paid to deposition within vulnerable habitats. Via this approach, GreenEO will improve the estimation of nitrogen deposition and critical load exceedances in vulnerable ecosystems. Collaborating with stakeholders, we will link these outputs to biodiversity indicators, like plant species richness and butterfly indices, to create a nitrogen sensitivity index. This will identify high-recovery areas and support sustainable agricultural practices.

Wichink Kruit, R. J., Schaap, M., Sauter, F. J., van Zanten, M. C., and van Pul, W. A. J.: Modeling the distribution of ammonia across Europe including bi-directional surface-atmosphere exchange, Biogeosciences, 9, 5261–5277, https://doi.org/10.5194/bg-9-5261-2012, 2012.

How to cite: Hamer, P., Frohn, L. M., Geels, C., Christensen, J., Denby, B. R., Simpson, D., Hutchings, N., Lopez-Aparicio, S., Schneider, P., Cao, T.-V., Jiminez, I., Fontenelle, T., van der A, R., Mijling, B., Ding, J., Trigo, I., Calvet, J.-C., Schante, J., Judes, T., and Tarrason, L. and the GreenEO Consortium: The GreenEO Project: Satellite-Based Services to Support Sustainable Land Use Practices Under the European Green Deal, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17316, https://doi.org/10.5194/egusphere-egu25-17316, 2025.

EGU25-17830 | Orals | BG1.3

Increasing soil nitrous acid emissions driven by climate and fertilization change aggravate global ozone pollution 

Yanan Wang, Qinyi Li, Ivonne Treb, Yurun Wang, Chuanhua Ren, Alfonso Saiz-Lopez, Likun Xue, and Tao Wang

Soil microbial nitrous acid (HONO) production is an important source of atmospheric reactive nitrogen that affects air quality and climate. However, long-term global soil HONO emissions driven by climate change and fertilizer use have not been quantified. Here, we derive the global soil HONO emissions over the past four decades and evaluate their impacts on ozone (O3) and vegetation. Results show that climate change and the increased fertilizer use enhanced soil HONO emissions from 9.4 Tg N in 1980 to 11.5 Tg N in 2016.  Chemistry-climate model simulations show that soil HONO emissions increased global surface O3 mixing ratios by 2.5% (up to 29%) and vegetation risk to O3, with increasing impact during 1980s-2016 in low-anthropogenic-emission regions. With future decreasing anthropogenic emissions, the soil HONO impact on air quality and vegetation is expected to increase. We thus recommend consideration of soil HONO emissions in strategies for mitigating global air pollution.

How to cite: Wang, Y., Li, Q., Treb, I., Wang, Y., Ren, C., Saiz-Lopez, A., Xue, L., and Wang, T.: Increasing soil nitrous acid emissions driven by climate and fertilization change aggravate global ozone pollution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17830, https://doi.org/10.5194/egusphere-egu25-17830, 2025.

Reactive nitrogen (N) deposition presents significant environmental challenges in India, where approximately 24% of the land is forested and agriculture plays a vital role in the economy. As a major contributor from South Asia—a global reactive nitrogen emissions hotspot—India's policy actions, or inactions, have far-reaching implications. Despite ongoing clean air initiatives, the scientific community has largely neglected the effects of reactive nitrogen deposition on terrestrial ecosystems. This study aims to compile and assess the current research status on reactive nitrogen deposition in India, underscoring its importance given the country's unique geography and agricultural reliance.

The study will provide indirect estimations of reactive nitrogen deposition based on nitrogen concentration measurements from various regions across the country. While wet deposition studies offer a broader understanding, research on dry deposition remains limited. Recent efforts, such as the South Asia Nitrogen Hub project led by CEH UK, have studied the forest ecosystem to explore the impact of reactive nitrogen on lichens. However, comprehensive data on reactive nitrogen deposition across diverse ecosystems is still lacking.

This research seeks to identify existing gaps and stimulate discussion on future research directions essential for the effective management of reactive nitrogen in India's varied ecosystems. By addressing these issues, we aim to inform policy and practice to mitigate the adverse effects of reactive nitrogen deposition while promoting sustainable development in the region.

 

How to cite: Singh, S.: Reactive Nitrogen Deposition in India: Impacts on Terrestrial Ecosystems and Current Research Status, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17857, https://doi.org/10.5194/egusphere-egu25-17857, 2025.

EGU25-18103 | Posters on site | BG1.3

Atmospheric nitrogen deposition in Switzerland 

Mario Meier, Zaida Ehrenmann, and Eva Seitler

Increased atmospheric nitrogen (N) deposition into sensitive ecosystems is leading to soil acidification, nutrient imbalances and biodiversity losses. Therefore, N depositions were quantified throughout Switzerland in 2000, 2014, 2019 and 2024 measuring the concentrations of seven different inorganic N compounds in wet and dry gravitational as well as in dry non-gravitational deposition. For data collection passive (diffusion tubes and bulk sampler) and active sampling systems (denuder and filter sampler) were used. From the obtained measurement data, N depositions were calculated. The wet and dry gravitational deposition was obtained directly from the bulk samples. The dry non-gravitational deposition was calculated using the inferential method. By summing up the gravitational and non-gravitational N deposition, the total N deposition was obtained and compared to the critical loads for N (CLN). The results show that N inputs in Switzerland are largely around or above the CLN, regardless of the sensitive ecosystems considered. Considerable exceedances have been found near intensive agriculture. In the long-term comparison, a decrease in oxidized N components was observed. However, the total N deposition remained stable over time. The most important processes for the N deposition are the precipitation and the dry deposition of ammonia (NH3). In summary, the atmospheric N inputs into sensitive ecosystems in Switzerland are largely too high and therefore further measures to reduce N emissions are necessary.

We would like to thank to the Swiss Federal Office for the Environment (FOEN), Swiss Federal Institute for Forest, Snow and Landscape Research (WSL), Ostluft, the Swiss cantons and the University of Basel for financial support of the measurement campaigns. A special thank goes to the Swiss Federal Laboratories for Materials Science and Technology (EMPA) for the valuable cooperation.

How to cite: Meier, M., Ehrenmann, Z., and Seitler, E.: Atmospheric nitrogen deposition in Switzerland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18103, https://doi.org/10.5194/egusphere-egu25-18103, 2025.

EGU25-18590 | Orals | BG1.3 | Highlight

Dutch and EU consumption-based assessments of nitrogen losses throughout the global food system 

José M. Mogollón, Nicolas Navarre, and Kevin Kevin Morgan-Rothschild

The modern global food system is the largest driver of nitrogen imbalances across the world. These problems are exacerbated by excessive and resource-intensive food demand prone to large amounts of loss and waste throughout the food system. Increasing international trade is shifting the burden and upstream nitrogen demand and downstream eutrophication impacts beyond national borders and moving beyond the safe regional boundaries for their presence in the environment. To better understand drivers and solutions to close nitrogen loops, we use the global food input-output model FABIO, which monitors the movement of biomass and the land utilized across global supply chains, encompassing 191 countries, and 130 agricultural and food products. We couple FABIO to nitrogen crop demand, livestock manure management systems, and agricultural surpluses to assess the consumption-based drivers for nitrogen emissions stemming from the agricultural system. A substantial amount of nitrogen losses can be attributed to traded commodities especially toward high-income nations. We further show how policy measures in a high-income nation (the Netherlands) related to the taxation of meat and carbon emissions from the food sector can lead to significant reduction of manure application (up to 20 kt N/yr) and nitrogen losses (over 1 kt N/yr) on a global scale. However, as the Dutch food system relies heavily on manure, there may be a concomitant increase in the need for synthetic fertilizers to account for the significant drop in manure of nearly (14 kt N/yr). We provide similar scenarios for various, more ambitious dietary changes (e.g. the EAT-Lancet diet) at the EU level that can help ameliorate global nitrogen losses, focusing in areas sensitive to terrestrial and aquatic eutrophication and acidification.

How to cite: Mogollón, J. M., Navarre, N., and Kevin Morgan-Rothschild, K.: Dutch and EU consumption-based assessments of nitrogen losses throughout the global food system, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18590, https://doi.org/10.5194/egusphere-egu25-18590, 2025.

EGU25-18703 | ECS | Orals | BG1.3

Effects of long-term nitrogen addition on changes in the functional composition of microbial communities after long-term N addition in a temperate beech forest 

Carme López Sánchez, Àngela Ribas, Rossella Guerreri, Jiesi Lei, Yunfeng Yang, Jizhong Zhou, and Stefania Mattana

Forests are integral to maintaining planetary health, serving as biodiversity reservoirs, carbon sink, and regulators of nutrient cycles, yet their capacity to sustain these functions is increasingly disrupted by global changes. Among them, the rise in atmospheric nitrogen (N) deposition, resulting from anthropogenic emissions of reactive N compounds during fertilizer production and fossil fuel combustion, occurs across terrestrial ecosystems and can alter microbial communities’ functional composition and diversity.

In this study, we evaluate the effects of long-term N fertilisation (simulating an increase in N deposition) on the taxonomic and functional diversity of soil microbial communities in a mature beech forest in Northern Italy. The experiment started in 2015, and it includes control (only ambient deposition, N0) and soil N addition (30 kg ha-1 yr-1, N30) each replicated in 3 plots. Soil biochemical variables including Nitrogen (N), Carbon (C) and Phosphorus (P) content and soluble ions were characterized for both treatments. In addition, GeoChip 5.0S, a microarray technology, was used to characterize the taxonomic and functional diversity of microbial communities.

Although no changes were detected in soil physicochemical characteristics between N30 and N0, there was a significant increase in the taxonomic richness and diversity (Shannon-Weiver and Simpson indices) in the fertilized plots. Moreover, the relative abundance of some functional genes related to the N, C and sulphur (S) cycles were significantly increased in N30 plots, whereas P cycling genes showed no significant changes between treatments. Preliminary results suggest a probable increase in the denitrification and assimilatory and dissimilatory nitrate reduction processes of the N-added soil microbiome. In addition, the results suggest an increase of both the C fixation and C degradation pathways in N30 plots. The higher stimulation of C degradation cycling genes in comparison to C fixation cycling genes, could be explained by the promotion of plant growth and the consequent increase in rhizosphere secretions and C input to the soil after N addition.

This study contributes to the description of microbial community dynamics and the resulting changes in soil biogeochemical processes in forests under increased N deposition conditions.

How to cite: López Sánchez, C., Ribas, À., Guerreri, R., Lei, J., Yang, Y., Zhou, J., and Mattana, S.: Effects of long-term nitrogen addition on changes in the functional composition of microbial communities after long-term N addition in a temperate beech forest, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18703, https://doi.org/10.5194/egusphere-egu25-18703, 2025.

EGU25-18764 | Orals | BG1.3

Biochar as a sustainable amendment in fertilized agricultural soils; insights and trade-offs among nitrogen kinetics, carbon sequestration, and greenhouse gas emissions. 

Georgios Giannopoulos, Elpida Pasvadoglou, George Kourtidis, Eugenio Diaz-Pines, Fotis Sgouridis, Anne Boos, Glykeria Duelli, Vassileios Tzanakakis, Vassilis Aschonitis, George Arampatzis, and Ioannis Anastopoulos

Under European and International policies, organic soil amendments are highly promoted as a cost-efficient solution to improve soil C, quality, and agrosystem sustainability. Inorganic N application is an essential agronomic practice to increase and secure crop yields, however, its long-term application has led to serious environmental problems including deterioration of soil organic C, enhanced greenhouse gas emissions, and an overall decline in environmental quality. Consequently, the co-application of organic and inorganic fertilizers is advocated as a more effective and environmentally friendly fertilization regime. This study aims, to decipher the short-term N kinetics in agricultural soils amended with organic, inorganic, and a combined application of N fertilizer, with and without biochar, and to assess the trade-off balance of soil C and greenhouse gas emissions. Therefore, we investigated the short-term (90 d) soil N dynamics of sandy soil mesocosms (2 Kg) receiving municipal sewage sludge (MSS) amendments (50 t/ha), urea-N fertilization (U; 200 kg/ha), a combined application (MSS+U), without and with biochar (1.5% w/w). An unamended soil mesocosm was included as a control. The addition of urea-N (U), municipal sewage sludge (MSS), and their combined application (MSS+U) increased the availability of soil NH4+ by 3x, 5x and 12x times, relative to the control, respectively. Interestingly, we observed a tremendous release of soil NO2- only in the urea treatment (U; 128 mg kg-1), and not in the other remaining treatments. Throughout the incubation approx. 12.7x, 13.4x, and 19.7x more soil NO3- was observed for the U, MSS, and MSS+U treatment, relative to the control, respectively. Where biochar was applied, an approx. 40% reduction in soil available NO2- andNO3- was observed. Considering the gaseous emissions of CO2 and N2O, that are generally products of soil respiration, nitrification, and denitrification, the addition of MSS and its co-application (MSS+U), enhanced soil CO2 by 2.4x and 2.4x, and by 13.6x and 16.9x for soil N2O emissions, respectively. Though biochar addition reduced cumulative CO2 emissions by 24%, for all treatments except the control. Although biochar addition decreased cumulative N2O emission by 65% in the U, it had no effect on cumulative N2O emission for MSS and the combined treatment (MSS+U). Fertilization by U did not affect much soil CO2 (526 mg CO2-C kg-1) and N2O (1258 μg N2O-N kg-1) emissions when compared to the unamended soil treatment (C). The MSS+U reduced the N2O emission factor, by 5x when compared to MSS treatment, however, it was well above the IPPC emission factor of 1%. Municipal sewage sludge is a source of C, though we observed that MSS (74%) and the combined treatment (MSS+U, 96%) enhanced the CO2-equivalent emissions, indicating a complete loss of the added organic C through greenhouse gas emissions. Considering our key question, whether co-application of inorganic, and organic fertilizer with biochar is a double-edged sword, we conclude that co-application should be carefully evaluated case per case, as it affects several key soil parameters differently, and therefore we should seek new ways to minimize gaseous losses thus to improve sustainability in agrosystems.

How to cite: Giannopoulos, G., Pasvadoglou, E., Kourtidis, G., Diaz-Pines, E., Sgouridis, F., Boos, A., Duelli, G., Tzanakakis, V., Aschonitis, V., Arampatzis, G., and Anastopoulos, I.: Biochar as a sustainable amendment in fertilized agricultural soils; insights and trade-offs among nitrogen kinetics, carbon sequestration, and greenhouse gas emissions., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18764, https://doi.org/10.5194/egusphere-egu25-18764, 2025.

EGU25-19141 | Posters on site | BG1.3

Long-term variations in nitrate leaching from ICP Forests Level II plots 

Peter Waldner, Stephan Raspe, Stefan Fleck, Lothar Zimmermann, Paul Schmidt-Walter, Carmen Iacoban, Bruno De Vos, Nathalie Cools, Heleen Deroo, Elena Vanguelova, Zoran Galic, Athanassios Bourletsikas, Henning Meesenburg, Tim Schütt, Lena Wohlgemuth, Kai Schwärzel, Katrin Meusburger, and Tiina Nieminen

Forests in Europe have been exposed to an increase in atmospheric deposition of nitrogen in the second half of the 20th century that potentially lead to nitrogen saturation and elevated leaching of nitrogen from forest soils potentially impacting water quality of drinking water resources. Nitrogen dynamics of forests, however, are complexe and still not fully understood.

Atmospheric deposition, soil solution, meteorology, soils, as well as stand and site characteristics have been continuously measured and analysed at several hundred intensive monitoring plots of the Level II plot network of the International Cooperative Programme on Assessment and Monitoring of Air Pollution Effects on Forests for many years.

We used the hydrological model LWFBrook90R to calculate water fluxes through the soils of these sites and calculated nitrogen input with atmospheric deposition and output fluxes with percolating soil water. We found high long-term variations on parts of the plots. Some of these variation patterns are in the time range of changes in the tree stands, e.g. mortality and subsequent biomass decomposition. We will discuss relations of found nitrate leaching patterns with nitrogen saturation indicators suggested in literature. 

How to cite: Waldner, P., Raspe, S., Fleck, S., Zimmermann, L., Schmidt-Walter, P., Iacoban, C., De Vos, B., Cools, N., Deroo, H., Vanguelova, E., Galic, Z., Bourletsikas, A., Meesenburg, H., Schütt, T., Wohlgemuth, L., Schwärzel, K., Meusburger, K., and Nieminen, T.: Long-term variations in nitrate leaching from ICP Forests Level II plots, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19141, https://doi.org/10.5194/egusphere-egu25-19141, 2025.

EGU25-19168 | ECS | Orals | BG1.3

Atmospheric reactive nitrogen and its dry deposition regimes under anthropogenic influence: Insights from intensive and long-term monitoring in Switzerland 

Jun Zhang, Ali Waseem, Andrea Baccarini, Ghislain Motos, Christoph Hüglin, Siyao Yue, Benjamin Brem, Leila Simon, Lubna Dada, Kalliopi Violaki, Martin Gysel, Jay Slowik, and Athanasios Nenes

Excessive nitrogen deposition from anthropogenic activities poses significant challenges to ecosystems and air quality.1 The atmospheric deposition of ammonium and nitrate plays a critical role in regulating ecosystem productivity and driving particulate matter formation, with impacts that vary across spatial and temporal scales.

In this study, high time-resolution measurements of gas-phase nitric acid (HNO3) and ammonia (NH3), as well as particulate nitrate and ammonium were conducted at an agricultural site in Switzerland. These measurements were complemented by 15 years of long-term monitoring data at the same site, providing a comprehensive record of changes in atmospheric gas and aerosol species over time. Aerosol pH was estimated using the ISORROPIA thermodynamic model2 and evaluated using a well-established approach based on the agreement between observed and predicted partition ratios of nitrogen species. The intensive measurement shows that the diurnal cycles of HNO3 and NH3 partitioning exhibited distinct patterns. HNO3 tended to partition into the particle phase during the night, driven by cooler temperatures, while NH3 remained predominantly in the gas phase throughout the day and night, regulated by high aerosol pH characteristics at the sampling site.

The dry deposition regimes of HNO3 and NH3 were investigated in relation to aerosol liquid water content and acidity following the approach of Nenes et al. (2021).3 The findings indicate that NH3 deposition is rapid, meaning it tends to deposit near its sources, raising concerns about its localized ecological impacts. Aerosol mass formation was found to be primarily sensitive to HNO3 concentrations. Long-term monitoring data spanning 15 years revealed that reduction in SO2 emissions did not lead to increases in aerosol pH owing to the buffering effect of NH3 in the NH3-rich environment. The decline in sulfate concentration has driven a clear shift in aerosol mass sensitivity, transitioning from NH3-sensitive to NH3 -insensitive regime. Comparative measurements at forested sites in Switzerland provide further insight into the diurnal cycle of aerosol pH and reactive nitrogen deposition, highlighting the influence of anthropogenic activities on nitrogen dynamics across different ecosystems. These findings show the complex interplay between rapidly fluctuating diurnal aerosol acidity and reactive nitrogen deposition, offering important reference for designing effective pollutant mitigation strategies.

References:

(1) Wim de Vries.: Impacts of nitrogen emissions on ecosystems and human health: A mini review, Current Opinion in Environmental Science & Health, 2021, 21:100249, DOI: 10.1016/j.coesh.2021.100249. 

(2) Fountoukis, C. and Nenes, A.: ISORROPIA II: a computationally efficient thermodynamic equilibrium model for K+–Ca2+–Mg2+–NH4+–Na+–SO42−–NO3–Cl–H2O aerosols, Atmospheric Chemistry and Physics, 7, 4639–4659, DOI:10.5194/acp-7-4639-2007, 2007.

(3) Nenes, A., Pandis, S. N., Kanakidou, M., Russell, A. G., Song, S., Vasilakos, P., and Weber, R. J.: Aerosol acidity and liquid water content regulate the dry deposition of inorganic reactive nitrogen, Atmospheric Chemistry and Physics, 21, 6023–6033 DOI:10.5194/acp-21-6023-2021, 2021.

How to cite: Zhang, J., Waseem, A., Baccarini, A., Motos, G., Hüglin, C., Yue, S., Brem, B., Simon, L., Dada, L., Violaki, K., Gysel, M., Slowik, J., and Nenes, A.: Atmospheric reactive nitrogen and its dry deposition regimes under anthropogenic influence: Insights from intensive and long-term monitoring in Switzerland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19168, https://doi.org/10.5194/egusphere-egu25-19168, 2025.

EGU25-19982 | Orals | BG1.3

Cycling of nitrogen in soil organic matter pools in grasslands as influenced by land use intensity and soil diversity 

Steffen A. Schweizer, Anne Böhm, Julia Kepp, Ralf Kiese, Narda L. Pacay-Barrientos, Elisabeth Ramm, Michael Schloter, Ingo Schöning, Marion Schrumpf, Stefanie Schulz, and Michael Dannenmann

Soil organic matter (SOM) provides crucial storage for carbon but also contains a majority of soil nitrogen. Land use intensity (LUI) may affect the particulate and mineral-associated SOM pools having repercussions on the carbon and nitrogen storage and cycling. Soil organic matter dynamics and composition plays a key role for the extent of these processes, yet its interactions remain poorly understood preventing targeted mitigation measures for carbon and nitrogen-related soil functions. Here we provide insights investigating how LUI and soil properties affect the storage of carbon and nitrogen in functional SOM pools in the topsoil (0-30 cm) of grassland soils across three different regions in Germany. Furthermore, we present a conceptual framework integrating biological, mineral, and organic nitrogen pools to disentangle nitrogen cycling processes and their interactions with organic matter dynamics.

Across the land use intensity gradient, we isolated particulate organic matter (POM), which is part of  in the >20 μm fraction, and mineral associated organic matter (MOM) in the <20 μm fraction. Random forest and mixed model analysis showed that LUI did not significantly affect SOM storage, but led to reduced C/N ratios in POM and MOM, driven by increased N fertilization intensity. Rather than land use intensity, soil properties, such as clay and iron oxide content, and soil type diversity exerted most influence on SOM.

To reconcile the influences of soil properties on soil nitrogen cycling, we provide a novel conceptual framework integrating organic matter stabilization mechanisms, microbial N uptake and release as necromass, as well important processes catalyzed by the soil microbiome including  biological nitrogen fixation pathways. Our integrative nitrogen cycling framework stimulates different disciplines towards a new perception of the nitrogen cycle in unlocking multiple organic nitrogen pools as mediated by soil type and climatic conditions.

How to cite: Schweizer, S. A., Böhm, A., Kepp, J., Kiese, R., Pacay-Barrientos, N. L., Ramm, E., Schloter, M., Schöning, I., Schrumpf, M., Schulz, S., and Dannenmann, M.: Cycling of nitrogen in soil organic matter pools in grasslands as influenced by land use intensity and soil diversity, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19982, https://doi.org/10.5194/egusphere-egu25-19982, 2025.

EGU25-20072 | ECS | Orals | BG1.3

Nitrate in water: Understanding the sources using δ15N and δ18O values 

Manoj Jakhar and Prasanta Sanyal

Nitrogen is a crucial component of nutrient dynamics in the environment and exists in multiple oxidation states. Nitrate (NO3-) is the most stable form of all the reactive nitrogen species and has a higher residence time in groundwater. Sources of nitrate include mainly fertilizers, sewage, manure, soil organic matter, and rain. In a country like India, where agriculture covers an area of about 60% of the total land and population with 2nd rank globally, contributes a huge fertilizer and sewage component to the environment. Also, nitrate in groundwater deteriorates the potable water quality. So, optimization of nitrogen use and sources estimation of nitrate in groundwater and surface water is very essential. Hindon River basin in the western Indo-Gangetic plain provides an opportunity to study nitrate dynamics in a huge populated and extensive agricultural area. Nitrate concentration in groundwater has been found from 0.1 ppm to 80 ppm, far apart from the permissible limit. Pre-monsoon groundwater shows higher nitrate concentration than that of post-monsoon groundwater at most of the places suggesting the dilution effect of rainwater after monsoon. Fluctuations in δ15N and δ18O values seasonally suggest a rapid change in contribution of nitrate source in groundwater. Contribution from each source of nitrate was estimated by Stable Isotope Mixing Models in R (SIMMR). As the dual isotope plot shows denitrification trend, the actual fertilizers contribution shifted towards manure and sewage end members evidenced by higher sewage and manure contributions (60-75% in pre and post-monsoon respectively) need to be optimized for sustainability.

How to cite: Jakhar, M. and Sanyal, P.: Nitrate in water: Understanding the sources using δ15N and δ18O values, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20072, https://doi.org/10.5194/egusphere-egu25-20072, 2025.

EGU25-20384 | ECS | Posters on site | BG1.3

Nitrous oxide emissions in natural and managed wetlands across Europe 

Thomas Crestey-Chury, Romain Darnajoux, Rana Kanaan, Mika Aurela, Aldis Butlers, Tom De Dobbelaer, Laura Escarmena, Laure Gandois, Jyrki Jauhiainen, Sari Juutinen, Tuula Larmola, Ülo Mander, Sílvia Poblador, Maud Raman, Fransesc Sabater, Thomas Schindler, Kaido Soosaar, Liisa Ukonmaanaho, and José-Miguel Sánchez-Pérez and the French team (CRBE)

Wetlands play a complex role as both sources of greenhouse gases (GHGs) and carbon sinks, making it essential to understand their dynamics and effects on biodiversity. The increasing pressures from climate change and human activities can disrupt the natural balance of these ecosystems, potentially resulting in elevated GHG emissions. The intricate abiotic and biotic interactions that govern these processes remain poorly understood. Therefore, there is an urgent need to enhance our understanding of the factors influencing GHG production in wetlands and to improve our capacity to model these emissions on a larger scale. In this study, we investigated the emissions of N2O, CO2 and CH4, with a particular focus on N2O, which is primarily produced through the microbial process of denitrification, and for which a satisfactory large-scale model formulation is lacking. The objective of this study was to evaluate these GHG emissions under optimal conditions for denitrification and to identify unifying abiotic factors. To achieve this, we selected contrasting study sites that varied by wetland type and climate zone, thereby gathering extensive data essential for our modelling efforts.

The research was conducted across multiple wetland sites involved in the ALFAwetlands project (https://alfawetlands.eu/), a European initiative dedicated to the study and restoration of both natural and managed wetlands. A total of 21 sites were selected across five European countries, encompassing a range of climate zones from Mediterranean to arctic. These included floodplains, alluvial forests, drained forests, peatlands, and mountain peatlands (with four sites each in France and Spain, three in Belgium, and five each in Finland and Estonia). For each location, three core samples (10 cm depth and 10 cm diameter) were collected and stored in the dark at 4°C prior to conducting mesocosm experiments. The samples were then placed in a custom-designed “GHG-aquacosm”, which simulates the effect of flooding on wetlands soils. During the experiments, soil cores were submerged in heated water enriched with nitrate. GHG emissions, soil moisture, and soil temperature were continuously monitored until stabilization or end of emission.

While CO2 and CH4 emissions were recorded, they have not yet been analysed, as this study primarily focuses on N2O emissions. The results indicated that N2O emissions varied significantly based on wetland type and initial soil water content. Drained forests, located in cool sub-arctic regions in Finland, demonstrated the highest N2O fluxes, ranging from 500 to 2000 µmol/m²·h. In contrast, floodplains and peatlands in Belgium and Estonia showed the lowest fluxes, between 5 and 150 µmol/m²·h. Significant variability was noted even among replicates, highlighting the considerable spatial heterogeneities of soils. Additionally, N2O emissions began immediately after nitrate addition, and for most sites ended 30 to 40 hours after, indicating the short temporal scale of N2O production and the challenges associated with in situ measurement. Ongoing data analysis and measurements are focused on further elucidating the spatial and temporal heterogeneities of denitrification processes, with the goal of effectively incorporating these factors into our modelling efforts.

How to cite: Crestey-Chury, T., Darnajoux, R., Kanaan, R., Aurela, M., Butlers, A., De Dobbelaer, T., Escarmena, L., Gandois, L., Jauhiainen, J., Juutinen, S., Larmola, T., Mander, Ü., Poblador, S., Raman, M., Sabater, F., Schindler, T., Soosaar, K., Ukonmaanaho, L., and Sánchez-Pérez, J.-M. and the French team (CRBE): Nitrous oxide emissions in natural and managed wetlands across Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20384, https://doi.org/10.5194/egusphere-egu25-20384, 2025.

EGU25-21215 | ECS | Orals | BG1.3

Does nitrogen deposition affect plant community stability–area relationships? The role of biodiversity, area, and seasonal N addition 

Yuqiu Zhang, Carly J. Stevens, Weiyu Lu, Xu Chen, Zhengru Ren, and Yunhai Zhang

Nitrogen (N) deposition generally reduces the temporal stability of plant community (community stability) across spatial scales. Theory predicts that community stability increases with sampling area, leading to a positive community stability–area relationship (CSAR). However, because atmospheric N deposition exhibits a temporal pattern, little is known about how the responses of community stability differ under seasonal N deposition, or whether seasonal N deposition alters the CSAR and its underlying mechanisms. Understanding this is crucial for assessing multi-scale ecological sustainability under global change. We conducted an experiment with N input during autumn, winter, or the growing season in a temperate grassland. Based on six years of survey data across nested spatial scales ranging from 0.01 to 16 m2, we explored the potential impacts of seasonal N enrichment on the CSAR. Our results showed that community stability increased with sampling area, regardless of N addition. Each of the three seasonal N inputs caused a significant reduction in the CSAR intercept, while N addition in winter or the growing season also reduced the CSAR slope. Biodiversity had a stronger effect than area in maintaining the positive CSAR, and mediated the relationship between area and stability. High biodiversity preserved community stability by maintaining population stability and compensatory dynamics. By validating and extending the CSAR theory under seasonal N input, our research showed that N input in winter or the growing season caused a greater reduction in plant community stability at larger spatial scales. As global N deposition continues to increase, small-scale studies may undervalue the adverse impact of N input on stability, while large-scale studies based only on N input during the growing season may overestimate this effect. These findings highlight the need to consider both spatial scales and seasonality of N deposition for accurately predicting ecosystem responses to atmospheric N deposition.

How to cite: Zhang, Y., Stevens, C. J., Lu, W., Chen, X., Ren, Z., and Zhang, Y.: Does nitrogen deposition affect plant community stability–area relationships? The role of biodiversity, area, and seasonal N addition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21215, https://doi.org/10.5194/egusphere-egu25-21215, 2025.

AS3 – Atmospheric Composition, Chemistry and Aerosols

EGU25-138 | Posters on site | AS3.1

Aerosol Monitoring at the Western Arabian Peninsula and North region of KSA (NEOM). 

Illia Shevchenko, Yoshihide Wada, and Georgiy Stenchikov

Deserts are the primary source of atmospheric dust. Covering over one-third of the Earth’s land surface, deserts play a pivotal role in influencing planetary albedo and dust dynamics.
The Arabian Peninsula is one of the world’s largest dust source regions. It is also affected by natural and anthropogenic pollution of African, Asian, and European origin. As the Arabian Peninsula is highly under-sampled, we have since 2012 established and maintained aerosol monitoring sites at King Abdullah University of Science and Technology (KAUST), as well as in the North-Western part of the Arabian Peninsula, and the Red Sea coast.
The sites incorporate the following instrumentation:
1.
Two CIMEL sun photometers operational since 2012 as a part of the NASA Aerosol Robotic NETwork (AERONET), providing aerosol parameters, reporting data to the NASA Goddard website (http://aeronet.gsfc.nasa.gov/cgi-bin/type_piece_of_map_opera_v2_new).
2.
Hand-held sun photometer (Microtops II). The data are reported to the NASA Maritime Network (http://aeronet.gsfc.nasa.gov/new_web/maritime_aerosol_network.html).
3.
Micro Pulse Lidar (MPL) operating as a part of the NASA MPLNET (http://kimura.gsfc.nasa.gov/site--‐page?site=Kaust). Monitoring the vertical distribution of Aerosols.
4.
We measure aerosol deposition rates on a monthly basis using passive samplers in different several locations (KAUST, 2015-2023; Al Wajh Lagoon, 2021-2022; DUBA & Tabuk,2022 -2023; NEOM project area (NESTOR; ENOWA), 2024 - now)
5.
Mineralogical analysis of deposited aerosols by X-ray diffractometry (XRD)
6.
Measured particle size distributions using Mastersizer3000.
In this study we conduct an analysis of the combined effects of natural and anthropogenic pollution on air quality, climate, and application of renewable energy across the Arabian Peninsula, providing a scientific foundation for model calibration in this region.
Here we report on the data sets collected in 2021- 2025:

KAUST campus site: Two dust deposition samplers, AERONET, MPL

Al Wajh Lagoon site: Nine dust deposition samplers

Duba site: Two dust deposition samplers

Tabuk site: Two dust deposition samplers

NEOM, NESTOR Project: Two dust deposition samplers
These data sets, in combination with the available satellite observations, were integrated into the meteorology-chemistry-aerosol model, WRF-Chem, to quantify the aerosol environmental impacts and support environmental decision-making in the region.

How to cite: Shevchenko, I., Wada, Y., and Stenchikov, G.: Aerosol Monitoring at the Western Arabian Peninsula and North region of KSA (NEOM)., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-138, https://doi.org/10.5194/egusphere-egu25-138, 2025.

EGU25-516 | ECS | Posters on site | AS3.1

Sensitivity of Phase Partitioning of Inorganic Aerosols to pH and ALWC In Northwestern Indo-Gangetic Plain 

Swati Joshi, Chandrima Shaw, Neeraj Rastogi, and Atinderpal Singh

Keywords:   Inorganic ions, ISOROPIIA-II, Sensitivity regime, ALWC, pH

Abstract

The Indo-Gangetic Plain (IGP) is one of the world’s most critical aerosol pollution hotspots, experiencing severe air quality degradation during the transition from summer to cooler months. Enhanced aerosol loading arises from a complex interplay of meteorological conditions, anthropogenic activities, and the region’s unique topography. Fine-mode aerosols, particularly those containing inorganic nitrate, chloride, and ammonium, significantly impact atmospheric chemistry and air quality over this region. The interaction between aerosol, liquid water content (ALWC), and pH is a key determinant of gas-particle partitioning for these species, influencing their atmospheric residence times and depositional velocities. This study presents real-time measurements of inorganic ions (NH4+, SO42--, Cl-, Na+, Mg2+, Ca2+, K+, NO3-) and major gases (SO2, HCl, HONO, HNO3, NH3) in ambient air by deploying the MARGA-R (Monitor for AeRosols and Gases in Ambient Air, Metrohm) instrument during the post-monsoon to winter transition in the Northwestern IGP region, with a focus on the role of temperature, ALWC, and pH in gas-particle partitioning. Using the thermodynamic model ISORROPIA-II, aerosol pH and ALWC were determined and applied in a mathematical framework to elucidate the interactions between inorganic aerosols and major gaseous species and to identify the chemical domains (sensitivity regimes) where aerosol particulate matter is sensitive to NH3 and HNO3. Results illustrate that pH and ALWC conditions during the study period predominantly favoured the partitioning of nitric acid (HNO₃) into particulate nitrate (NO₃⁻). Conversely, ammonium (NH₄⁺) remained mainly in its gaseous form as ammonia (NH₃) over the study site. This distinct partitioning behaviour implies that NH₃ tend to stay localized near their source regions, whereas NO₃⁻ has a greater potential for long-range transport, depending on environmental parameters controlling its mobility and deposition. These findings underscore the critical role of region-specific meteorological processes and shifting source profiles from post-monsoon to winter in influencing secondary inorganic aerosol dynamics. This knowledge offers valuable insights for designing effective pollution mitigation strategies tailored to the unique characteristics of the IGP, emphasizing the importance of considering not just the mass concentration of species but also their sensitivities.

How to cite: Joshi, S., Shaw, C., Rastogi, N., and Singh, A.: Sensitivity of Phase Partitioning of Inorganic Aerosols to pH and ALWC In Northwestern Indo-Gangetic Plain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-516, https://doi.org/10.5194/egusphere-egu25-516, 2025.

EGU25-1326 | ECS | Orals | AS3.1

Sensitivity studies on cloud droplet number enhancement from the co-condensing NH3, HNO3, and organic vapours in Hyytiälä, Finland 

Yu Wang, Judith Kleinheins, Beiping Luo, Claudia Marcolli, Thomas Peter, Ying Chen, Gang Chen, and Ulrike Lohmann

Semi-volatile compounds (organics, nitrate, chloride, ammonium) are ubiquitous in atmospheric aerosols and usually contribute over 50% to the fine aerosol mass worldwide. Their gas precursors (organics, HNO3, HCl, NH3) can co-condense with water vapour as an extra source of aerosol particle growth when ambient relative humidity (RH) increases, therefore facilitating hygroscopic growth under sub-saturated conditions and activation to cloud condensation nuclei (CCN). Yet, the attribution of co-condensing semi-volatile compounds to the CCN activation is poorly understood.

Topping et al. (2013) developed a cloud parcel model to simulate the co-condensation effect of organics and sensitivities to key influencing factors (e.g. aerosol concentration, updraft velocity) for the first time. Building on Topping’s study, we further developed a cloud parcel model that simulates co-condensation for both organic and inorganic compounds. We used in-situ observations of gas and aerosols from SMEAR II Hyytiälä Forestry Field Station in Finland as input and quantified co-condensation for inorganics, organics, and their combination. Evaporation losses of particulate semi-volatile compounds in the sampling and non-ideality of organics are also considered.

In Hyytiälä, the inclusion of co-condensing semi-volatile compounds to CCN activation is sensitive to the updraft velocity (0.003 – 5 m s-1) and assumed volatility distribution and non-ideality of organics. The volatility distribution of organics is highly uncertain but important because it relates the amount of organic gas precursors with measured mass concentration in the condensed phase. Topping et al. (2013) simulated co-condensation of organic compounds with volatility bins up to C* = 10-3 μg m-3, saturation mass concentration of organics in condensed phase. To understand the role of more volatile bin C* = 10-4 μg m-3 which is usually considered too volatile for co-condensation, we modified volatility basis set of Topping et al (2013) by adding an extra bin C* = 10-4 μg m-3. We found that the bin C* = 10-4 μg m-3 can play a large role in CCN activation when temperature decreases, resulting in a 30% higher cloud droplet number concentration (CDNC), consistent with Heikkinen et al. (2024). For the combined co-condensation of organics and inorganics increase CDNC by up to 52% with bin C* = 10-4 μg m-3 compared to 40% without the bin. The semi-volatile compounds evaporated by ~10% due sampling losses, dryer tubes, and outdoor-indoor temperature changes before detection by the instrument, which should be considered in the total organic mass estimate. Non-ideality of the system is important for considering the co-condensation effect realistically. Assuming ideality, co-condensation is overestimated by 100% in CDNC. The combined enhancement in CDNC of inorganic and organic species goes beyond the sum of individual effects and should be further constrained and properly estimated in models.

Reference:

Heikkinen et al. (2024), Cloud response to co-condensation of water and organic vapors over the boreal forest, Atmos. Chem. Phys., 24(8), 5117-5147.

Topping, D., P. Connolly, and G. McFiggans (2013), Cloud droplet number enhanced by co-condensation of organic vapours, Nature Geoscience, 6, 443.

How to cite: Wang, Y., Kleinheins, J., Luo, B., Marcolli, C., Peter, T., Chen, Y., Chen, G., and Lohmann, U.: Sensitivity studies on cloud droplet number enhancement from the co-condensing NH3, HNO3, and organic vapours in Hyytiälä, Finland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1326, https://doi.org/10.5194/egusphere-egu25-1326, 2025.

EGU25-1895 | Posters on site | AS3.1

Core-shell morphology of PM2.5 from three Northeast Asian cities: Its role in reactive uptake  

Mijung Song, Changjoon Seong, Ying Li, Zhijun Wu, Ji Yi Lee, and Atsushi Matsuki

Aerosol particle morphology plays a pivotal role in atmospheric processes, particularly heterogeneous chemistry. This study investigates phase transitions and corresponding morphologies of PM2.5 particles collected from three Northeast Asian cities: Seoul, Beijing, and Noto. The samples, representing both polluted and clean environments, were predominantly organic-rich. Observations reveal that PM2.5 particles underwent distinct phase transitions with varying relative humidity (RH), often forming complex three-phase systems. Under ambient conditions, particles predominantly existed in two-liquid or three-phase states, with fully homogeneous or non-liquid states being rare. The organic-rich outer phase serves as a diffusion barrier, limiting the reactive uptake of N₂O₅, especially at lower RH when organic materials become more viscous. These findings will be presented.

How to cite: Song, M., Seong, C., Li, Y., Wu, Z., Lee, J. Y., and Matsuki, A.: Core-shell morphology of PM2.5 from three Northeast Asian cities: Its role in reactive uptake , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1895, https://doi.org/10.5194/egusphere-egu25-1895, 2025.

EGU25-2187 | ECS | Orals | AS3.1

Development of a Dual-Beam Optical Trap for Monitoring Water Uptake and Activation of Single Aerosol Particles 

Aleksandr Odelskii, Svitlana Malashevych, Alexander Logozzo, and Thomas Preston

The microphysical properties of natural and anthropogenic aerosols play a crucial role in cloud formation, particularly in water uptake and droplet activation. Köhler's theory provides a framework for predicting the critical supersaturation at which a droplet activates, combining the effects of solute-induced water vapour reduction and surface curvature. While effective for inorganic compounds, the theory inaccurately predicts water uptake in droplets containing organic species. Models incorporating surfactant effects offer potential improvements but require robust experimental data for validation. At the same time, conventional ensemble measurements average over droplet size and compositional heterogeneities, obscuring critical single-particle behaviours.

To address these limitations, we present a dual-beam optical trap for studying droplet activation in single aerosol particles. The setup uses counter-propagating laser beams to stably trap individual particles, enabling precise size and refractive index measurements via Cavity-Enhanced Raman Spectroscopy. A specially designed cell, featuring cooling and heating sections, establishes controlled temperature and relative humidity/supersaturation gradients, enabling the investigation of droplet growth under defined conditions. Additionally, the setup is equipped with a high-speed camera to monitor the activation and subsequent growth of droplets, allowing real-time visualization of growth dynamics. By systematically isolating individual particles and monitoring their behaviour, this technique avoids the averaging effects inherent to ensemble methods, providing high-resolution data critical for validating and refining models of organic aerosol activation.

How to cite: Odelskii, A., Malashevych, S., Logozzo, A., and Preston, T.: Development of a Dual-Beam Optical Trap for Monitoring Water Uptake and Activation of Single Aerosol Particles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2187, https://doi.org/10.5194/egusphere-egu25-2187, 2025.

EGU25-2290 | Posters on site | AS3.1

Source apportionment of aerosol ammonium in the urban boundary layer of Beijing from tower-based observations 

Libin Wu, Peng Wang, Hong Ren, and Pingqing Fu

Ammonium (NH4+) is an important component of PM2.5, and atmospheric NH4+ mainly comes from secondary reactions of NH3. It significantly impacts air pollution, radiative forcing, and human health. Source apportionment of NH4+ can help improve air quality through emission reductions. Previous studies have primarily focused on ground-level aerosols, and understanding the vertical characteristics of atmospheric NH4+ in the atmospheric boundary layer can deepen our understanding of the sources and transport processes of NH3/NH4+, enhancing the accuracy of atmospheric model simulations. In this study, we collected PM2.5 samples at 8, 120, and 260 m from the 325-meter meteorological tower at the Institute of Atmospheric Physics, Chinese Academy of Sciences (Beijing, China), conducted stable isotope analyses and source apportionment of atmospheric aerosol NH4+ in summer and winter. The summer results show that the concentration of NH4+ rises and its δ15N decreases as the sampling height increases, indicating that regional transport, especially from agricultural sources of NH3/NH4+ in the North China Plain, has a greater impact on high-altitude NH4+ in Beijing. The source apportionment results from the stable isotope mixing model “MixSIAR” show that agricultural sources contribute 47% to NH4+ in ground-level PM2.5, and this increases to 51~56% at higher altitudes. Comparing the observational results with atmospheric chemistry modeling suggests that non-agricultural NH3 emissions in Beijing may be significantly underestimated. Compared to summer, the vertical characteristics in winter are more complex. Still, overall, the concentration of NH4+ increases with height, indicating that both local emissions and regional transport contribute significantly to NH4+, with local emissions having a greater impact near the ground. Combustion-related NH3 emissions, including fossil fuel sources, NH3 slip, and biomass burning, contribute 60% to atmospheric NH4+ during heavily polluted days in winter, exceeding the contributions from volatilization-related NH3 emissions, including livestock breeding, N-fertilizer application, and human waste. In contrast, volatilization-related NH3 emissions dominate on clean days. Biomass burning, especially bioapplication (combustion and use of straw and firewood), may be an important NH3 source that has been overlooked. The study also used atmospheric chemical models to compare the effects of different emission reduction strategies on air pollution control. Compared to reducing a single pollutant (NH3), the simultaneous reduction of NH3 and other pollutants has a more significant effect on lowering PM2.5 concentrations. To improve air quality, future policies could consider implementing simultaneous emission reductions of NH3 and other pollutants for air pollution control.

How to cite: Wu, L., Wang, P., Ren, H., and Fu, P.: Source apportionment of aerosol ammonium in the urban boundary layer of Beijing from tower-based observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2290, https://doi.org/10.5194/egusphere-egu25-2290, 2025.

             Cement is an essential material for construction, but cement manufacturing factories are concentrated in areas where the raw materials are produced and the manufacturing process requires a large amount of energy. In Republic of Korea, a total of 50,237 tonnes in 2023 are produced at 13 manufacturing plants composed of 9 cement companies. Among these 13 plants, 6 are located in Gangwon-do Province. The cement production process generates a large amount of pollutants, including nitrogen oxides, sulfur oxides, and fine dust, causing various environmental issues and complaints from local residents in the surrounding areas near by the cement manufacturing factories.

In Republic of Korea, the proportion of using waste materials (especially plastic waste) as an alternative fuel instead of anthracite coal has been increasing recently. Additionally, the nitrogen oxide emission limit for cement manufacturing plants is set at 270 ppm (for facilities installed before 2007), which is much alleviated level than the 70 ppm limit for waste incineration plants (with a capacity of 2 tonnes per hour or more).

             Nitrogen oxides emitted into the atmosphere can act as precursor substances for acid rain, and they can also convert into fine dust (<PM 2.5) through photochemical reactions, potentially affecting the concentration of fine particulate matter in the air. The high concentrations of nitrogen oxides emitted from cement manufacturing facilities can impact the fine dust concentration in Gangwon-do Province, where these facilities are concentrated.

             Therefore, the objectives of this study are as follows: First, to calculate the proportion and amount of waste materials (specifically plastic waste) used as fuel in the cement manufacturing process; second, to examine the impact of nitrogen oxides on the fine dust (<PM 2.5) generation characteristics in Gangwon-do Province, considering the conversion rate of nitrogen oxides into fine dust; and third, to evaluate the proportion of fine dust attributable to nitrogen oxides. Using these results, the study aims to assess how much the fine dust concentration can be reduced by tightening the nitrogen oxide emission limit for cement plants to the level of waste incineration plants, and to propose policy alternatives to the government and Gangwon-do Province.

 

Acknowledgments

"This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)"

How to cite: Lee, N.-S., Jung, M., and Park, J.-S.: The impact of nitrogen oxides emitted from cement manufacturing facilities on the PM 2.5 concentration in the atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2440, https://doi.org/10.5194/egusphere-egu25-2440, 2025.

 New particle formation (NPF) event happened in the planetary boundary layer contribute more than 60% of ultrafine particles (UFP), which impact the could condensation nuclei (CCN) and the climate. This study retrieved the Particle Number Size Distribution (PNSD) and its relationship with Planetary Boundary Layer Height (PBLH), as well as nucleation mode aerosols trajectories during NPF events in three major Chinese cities: Beijing (BJ), Guangzhou (GZ), and Shanghai (SH). The observation periods include July 2017 to October 2019 (408 effective observation days), November 2019 to March 2020 (127 effective observation days), and April to June 2020 (44 effective observation days) for BJ, GZ, and SH, respectively. The results show that BJ exhibits the highest Number Concentration (PNC) at 2.05 × 10⁶ cm⁻³, while GZ records the highest NPF frequency at 25.98% GZ during the Covid 19 lockdown. In contrast, SH has the lowest PNC at 6.27 × 10⁵ cm⁻³ and the lowest NPF frequency (18.87%). An increase in the PBLH reduces the survival parameter (P), thereby promoting the occurrence of NPF events. A high nucleation-mode PNC also promotes the occurrence of NPF events. The sources of PNSD at the three cities exhibit distinct trajectories on NPF days. The main source of pollutants in BJ is Mongolia, located to the northwest. In GZ, the contribution mainly comes from Jiangxi and Fujian provinces to the northeast, while in SH, the source lies to the northwest. NPF frequencies consistently exceed 25%, predominantly in the northern regions of each site, indicating higher NPF levels in the north compared to the south. This research provides valuable insights for developing strategies to manage the atmospheric environment.

How to cite: Hu, H.: New insights into the boundary layer revolution correlation with new particle formation characteristic in megacities of China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2447, https://doi.org/10.5194/egusphere-egu25-2447, 2025.

EGU25-3447 | ECS | Posters on site | AS3.1

Atmospheric Dispersion Assessment of Fine Particulate Matter Precursors from Landfills Using the Gaussian Plume Model 

Minseon Park, Hyunjun Park, Namhoon Lee, Minjung Jung, and Hui-Young Yun

Landfills emit a variety of pollutants in both gaseous and liquid phases during the final disposal of waste. Among the gaseous pollutants, hydrogen sulfide (H2S), primarily generated during anaerobic decomposition, oxidizes in the atmosphere to form sulfur oxides (SOx) and contributes as a precursor to particulate matter (PM2.5) formation. While hydrogen sulfide (H2S) can affect local air quality during its atmospheric transport and oxidation, there is a lack of research on the quantitative evaluation of the atmospheric movement and oxidation processes of hydrogen sulfide (H2S) emitted from landfills.

Thus, this study aims to predict the emission of hydrogen sulfide (H2S) through elemental analysis of landfill waste, calculate the conversion to sulfur oxides (SOx), and then assess the impact on local air quality by modeling the diffusion of sulfur oxides (SOx) using the Gaussian plume model.

The sulfur (S) content in waste samples was measured using an elemental analyzer (vario-MARCO), and the potential for hydrogen sulfide (H2S) generation was calculated based on these measurements. Using chemical formulas, the amount of sulfur converted into sulfur oxides (SOx) was estimated. The horizontal and vertical diffusion coefficients (σy, σz) of the converted sulfur oxides (SOx) were determined using the Pasquill-Gifford empirical formula. The diffusion of sulfur oxides (SOx) was then modeled using the Gaussian plume model in Python, up to a distance of 1 km from the emission source.

By utilizing the Gaussian plume model, this study evaluates the conversion and diffusion of hydrogen sulfide from landfills into sulfur oxides and their impact on local air quality. The findings can provide a basis for landfill emission management and the formulation of air pollution reduction policies. Future research should verify the accuracy of the model by comparing the results with real-time air concentration data.

 

Acknowledgment

"This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)"

How to cite: Park, M., Park, H., Lee, N., Jung, M., and Yun, H.-Y.: Atmospheric Dispersion Assessment of Fine Particulate Matter Precursors from Landfills Using the Gaussian Plume Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3447, https://doi.org/10.5194/egusphere-egu25-3447, 2025.

EGU25-3830 | Orals | AS3.1

Processes governing new particle formation over croplands and urban influenced central USA and effects of entrainment mixing on cloud chemistry and formation of secondary organic aerosols 

Manish Shrivastava, Jie Zhang, Rahul Zaveri, Bin Zhao, Jeffrey Pierce, Samuel O' Donnell, Jerome Fast, Brian Gaudet, John Shilling, Alla Zelenyuk, Benjamin Murphy, Havala Pye, Qi Zhang, Justin Trousdell, Qi Chen, Steve Krueger, Raymond Shaw, and Mikhail Ovchinnikov

In forested regions around the world, biogenic emissions have been reported to be key drivers of new particle formation (NPF) that contribute to about half the budget of global cloud condensation nuclei (CCN). However, over the central U.S., far from forests and influenced by croplands and urban emissions, the processes driving NPF and CCN are not well understood. Using detailed regional model simulations using WRF-Chem, we show that acid-base reactions including sulfuric acid and dimethyl amines (DMA) are key nucleation drivers at the SGP site during two simulated days in the springtime. We also show that anthropogenic extremely low volatility organics (ELVOCs) formed by the oxidation of anthropogenic VOCs in the atmosphere are critical for explaining the observed particle growth. Conversely, simulated non-NPF days at SGP are characterized by low-level clouds, which reduce photochemical activity, sulfuric acid, and ELVOC concentrations, thereby explaining the lack of NPF. At the Bankhead National Forest (BNF) site the southeastern U.S., we show that nucleation rates are limited by availability of sulfuric acid in this forested area. Our study highlights the large potential heterogeneities in nucleation and particle growth mechanisms between forested and urban/farmland-influenced areas that need to be verified with new BNF measurements.

Additionally, we simulate droplet-resolved cloud chemistry and the interactions between turbulence and cloud chemistry using a one-dimensional explicit mixing parcel model (EMPM-Chem) to simulate how isoprene epoxydiol secondary organic aerosol (IEPOX-SOA) formation evolves in individual cloud droplets within rising cloudy parcels in the atmosphere. We find that as subsaturated air is entrained into and turbulently mixed with the cloud parcel, cloud droplet evaporation causes a reduction in droplet sizes, which leads to corresponding increases in per droplet ionic strength and acidity. Increased droplet acidity in turn greatly accelerates the kinetics of IEPOX-SOA formation. Our results provide key insights into single-cloud-droplet chemistry, suggesting that entrainment mixing may be an important process that increases SOA formation in the real atmosphere.

How to cite: Shrivastava, M., Zhang, J., Zaveri, R., Zhao, B., Pierce, J., O' Donnell, S., Fast, J., Gaudet, B., Shilling, J., Zelenyuk, A., Murphy, B., Pye, H., Zhang, Q., Trousdell, J., Chen, Q., Krueger, S., Shaw, R., and Ovchinnikov, M.: Processes governing new particle formation over croplands and urban influenced central USA and effects of entrainment mixing on cloud chemistry and formation of secondary organic aerosols, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3830, https://doi.org/10.5194/egusphere-egu25-3830, 2025.

EGU25-4600 | Orals | AS3.1 | Highlight

Advancing aerosols in Earth system modeling with artificial intelligence 

Po-Lun Ma, Andrew Geiss, Matthew Christensen, Meng Huang, Yi Qin, Balwinder Singh, Michael Pritchard, Hugh Morrison, Sam Silva, Daniel Rothenberg, and Sungduk Yu

The representations of aerosol and aerosol-cloud interactions (ACI) in conventional Earth system models are overly simplified due to computational constraints. These simple process representations limit the models’ predictive power as they contribute to significant errors in various parts of the simulated climate system. To address this challenge, we developed neural networks to replace aerosol and ACI processes (optics, activation, and precipitation) in the U.S. Department of Energy’s Energy Exascale Earth System Model (E3SM). These neural networks are trained on high-fidelity-high-resolution data and achieve remarkably high accuracy in offline tests. When implemented in E3SM, robust tests and guardrails are needed to ensure that the model produces correct and stable simulations and that their computational cost is low enough so that multi-year global simulations are possible. The hybrid E3SM produces a much more accurate characterization of aerosol and ACI, which leads to a very different climate simulation. To evaluate E3SM, an observationally based emulator has also been developed for understanding aerosol’s role in modulating various atmospheric features across scales in the real world. We highlight that the new hybrid approach, combining physics and artificial intelligence, provides ample opportunities for advancing understanding and predictability of the role of aerosols in the Earth system.

 

How to cite: Ma, P.-L., Geiss, A., Christensen, M., Huang, M., Qin, Y., Singh, B., Pritchard, M., Morrison, H., Silva, S., Rothenberg, D., and Yu, S.: Advancing aerosols in Earth system modeling with artificial intelligence, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4600, https://doi.org/10.5194/egusphere-egu25-4600, 2025.

EGU25-5023 | ECS | Orals | AS3.1

Increasing aerosol emissions from boreal biomass burning exacerbate Arctic warming 

Qirui Zhong, Nick Schutgens, Sander Veraverbeke, Guido van der Werf, and Shu Tao

The Northern Hemisphere boreal region is undergoing rapid warming, leading to an upsurge in biomass burning. Previous studies have primarily focused on greenhouse gas emissions from these fires, whereas the associated biomass burning aerosols (BBAs) have received less attention. Here we use satellite-constrained modelling to assess the radiative effect of aerosols from boreal fires on the climate in the Arctic region. We find a substantial increase in boreal BBA emissions associated with warming over the past two decades, causing pronounced positive radiative effects during Arctic summer mostly due to increased solar absorption. At a global warming level of 1 °C above current temperatures, boreal BBA emissions are projected to increase 6-fold, further warming the Arctic and potentially negating the benefits of ambitious anthropogenic black carbon mitigation. Given the high sensitivity of boreal and Arctic fires to climate change, our results underscore the increasingly relevant role of BBAs in Arctic climate.

How to cite: Zhong, Q., Schutgens, N., Veraverbeke, S., van der Werf, G., and Tao, S.: Increasing aerosol emissions from boreal biomass burning exacerbate Arctic warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5023, https://doi.org/10.5194/egusphere-egu25-5023, 2025.

EGU25-5435 | ECS | Posters on site | AS3.1

Quantitative analysis of indoor CO2 and PM levels during violin performance in a music practice room 

Cian-Han Chen, Wei-Chieh Huang, and Hui-Ming Hung

Indoor air quality significantly impacts public health as high CO2 levels impair cognition, and elevated particulate matter (PM) increases respiratory diseases. Music practice rooms, often enclosed spaces where musicians spend extended time, are seldom assessed for air quality. This study investigates CO2 and PM levels during violin practice in a music practice room using home-built low-cost air quality box (AQB) systems. Without ventilation, CO2 levels increase nearly linearly, frequently exceeding the 1000 ppm threshold. Simulations of CO2 profiles retrieve the exhaled minute volume of (9 ± 0.7) × 10-3 m3 min-1 person-1 for the violinist. The PM levels vary across five experiments, influenced by factors such as music tempo, rosin, and bow. In the simulation of PM profiles, the deposition rate constants are evaluated as 2.3×10-2, 2.6×10-2, and 9.8×10-2 min-1 for PM1, PM1-2.5, and PM2.5-10, respectively, higher than the gravitational deposition rate constants likely due to advection and turbulence. Smaller particles show higher deposition ratios due to their lower inertia. A model accounting for a decreasing PM generation rate over time, linked to rosin consumption during playing, offers improved prediction accuracy. This variation in rosin is further corroborated by scanning electron microscopy images. Infrared spectroscopy further identified functional groups of rosin and bow hair as factors affecting PM levels across experiments. Additional tests in a room with external circulation systems suggest strategies to maintain low CO2 and PM levels. These findings highlight the importance of adequate ventilation and proper material maintenance to mitigate CO2 and PM levels, thereby improving indoor air quality in music practice rooms to provide healthier environments for musicians, enhancing their well-being and performance.

How to cite: Chen, C.-H., Huang, W.-C., and Hung, H.-M.: Quantitative analysis of indoor CO2 and PM levels during violin performance in a music practice room, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5435, https://doi.org/10.5194/egusphere-egu25-5435, 2025.

This study integrates long-term data from the Surface Particulate Matter Network (SPARTAN) and the Aerosol Robotic Network (AERONET) to analyze the relationship between aerosol chemical composition and optical properties across 14 globally distributed sites. SPARTAN provides filter-based measurements of PM2.5 chemical species, including ammoniated sulfate (AS), ammonium nitrate (AN), fine soil (FS), and black carbon (BC). In contrast, AERONET offers column-based remote sensing optical data, such as aerosol optical depth (AOD), fine mode fraction (FMF), and single scattering albedo (SSA). By applying a collocation methodology to harmonize the SPARTAN and AERONET datasets, we conducted a detailed investigation of aerosol behavior using data collected from 2016 to 2023. Notable differences in aerosol optical properties were observed according to the mass differences and mass ratios of these chemical components. For FS, an increase in its mass led to decreases in dSSA and FMF, with changes of 0.0045 and 0.033 per 1 µg/m³, respectively. For non-absorbing components like AS and AN, an increase in their mass ratio consistently increased SSA across all wavelengths. This relationship was further supported by grouping data by PM2.5/AOD categories, revealing a correlation coefficient as high as 0.69. This integrated approach bridges the gap between column-based optical properties and surface-level chemical measurements, providing novel insights into aerosol classification and behavior. The findings underscore the importance of combining SPARTAN and AERONET datasets to enhance the understanding of aerosol dynamics and atmospheric impacts.

 

This work was supported by a grant from the National Institute of Environment Research (NIER), funded by the Ministry of Environment (MOE) of the Republic of Korea (Grant Number NIER-2021-03-03-007) and the Korea Meteorological Administration Research and Development Program under Grant RS-2024-00404042.

How to cite: Eom, S., Kim, J., and Park, S. S.: Bridging Surface and Column Perspectives: Insights into Aerosol Chemical Composition and Optical Properties from SPARTAN and AERONET Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5464, https://doi.org/10.5194/egusphere-egu25-5464, 2025.

Dust aerosols are a major component of atmospheric aerosols, impacting climate systems and human health. In Asia, dust storms pose significant threats to air quality and public health, particularly in China, Korea, and Japan. Additionally, dust deposition in China's coastal regions supplies trace elements and nutrients that influence microbial communities, affecting marine productivity. Over the Tibetan Plateau, dust reduces snow and ice albedo, accelerating glacial melting. Given these impacts, understanding the sources and contributions of dust aerosols is crucial. Therefore, we focused on typical regions in Asia—North China, Southeast China, the Korea-Japan region, the East China Sea, and the Tibetan Plateau—and selected four primary dust source regions: Eastern Central Asia (ECA), Western Central Asia (WCA), West Asia-South Asia (WA-SA), and North Africa-Middle East (NA-ME).

Previous studies on tracing the sources of airborne dust have largely relied on back-trajectory analysis. However, simply using the number of air mass trajectories passing over a desert to determine dust sources can lead to an overestimation of the relative contribution from source regions. This method, which did not consider the dust load in the transported air masses, resulted in an inaccurate evaluation of the desert-source contribution to the study regions. To address this issue, we present a novel algorithm for source-tracing of airborne dust (STAD), which incorporates satellite and reanalysis-based estimates to more precisely track dust activity and provide a more accurate quantification of source contributions. Overall, ECA emerges as the dominant source of dust affecting East Asia. In regions such as North China and the Korea-Japan area, ECA accounts for 60%-70% of dust transport, with WCA contributing around 20%. In Southeast China and the East China Sea, ECA still plays a major role, contributing 40%-50% of the dust. The Tibetan Plateau, as a dust transit hub in the Northern Hemisphere, has a complex dust source composition. The airborne dust at high altitudes over the Tibetan Plateau shows considerable spatial variation and primarily comes from desert clusters in ECA, WCA, and WA-SA. The Karakum, Taklimakan, and Thar deserts are significant sources of high-altitude airborne dust in the northwest, northeast, and southwest regions of the TP, with average mass loadings (mg m⁻²) contributing rates of 42.2% (32.9), 49.6% (48.3), and 16.4% (32.1), respectively.

This research lays a solid foundation for future studies on the role of dust aerosols in the Asian climate system, including their impacts on water cycles, weather patterns, and long-term environmental changes, providing crucial insights for developing effective mitigation strategies.

How to cite: Tang, J. and Wang, T.: Dominant Remote Sources and Their Potential Contributions to Airborne Dust over Typical Asian Regions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5540, https://doi.org/10.5194/egusphere-egu25-5540, 2025.

EGU25-5719 | ECS | Posters on site | AS3.1

ATMOMACCS: Predicting atmospheric compound properties 

Linus Lind, Hilda Sandström, and Patrick Rinke

Aerosol formation is a complex process involving numerous molecules, whose identities and environmental variations remain largely uncharted (Bianchi et al., 2019). Computational simulations and property prediction tools have emerged to identify compounds likely to participate in the particle formation process (Elm et al., 2020). In recent years, predictive machine learning models for saturation vapor pressure and partition coefficient estimation have achieved impressive accuracy, with mean absolute errors within one order of magnitude (Besel et al., 2023; Lumiaro et al., 2021); an advancement that enables the categorization of molecules into different volatility regions. However, the interpretability of these models in molecular sciences is often limited unless the molecular descriptor used is easily interpretable. Another challenge is that atmospheric molecules possess unique characteristics that may be overlooked by standard molecular representations developed in other chemical domains (Sandström et al., 2024). We hypothesize that combining sufficiently informative and interpretable descriptors with modern machine learning methods, chemical insight of these largely unknown chemical spaces can be gained in a data-driven way.

In this contribution, we introduce a new interpretable molecular descriptor, ATMOMACCS, specifically tailored to atmospheric molecules. We demonstrate its competitive performance in predicting various thermodynamic properties, such as saturation vapor pressure, vaporization enthalpy, partition coefficients, and glass-transition temperature, equaling or surpassing published results for four distinct atmospheric molecular datasets (Besel et al., 2023; Wang et al., 2017; Ferraz-Caetano et al., 2024; Li et al., 2020). Our descriptor is based on enumerating atmospherically relevant structural motifs, making it readily interpretable for atmospheric chemists. Additionally, in our approach, we analyze the relative importance of these motifs with Shapley Additive Explanations (SHAP) values (Lundberg & Lee, 2017), providing insight into the performance improvements observed. Notably, from this analysis, we found that explicitly counting the number of carbon atoms is particularly important for property prediction, though less so for water-gas phase partition coefficients. Moreover, the analysis shows that general structural motifs are roughly equally important as motifs specific to atmospheric organic chemistry, and the combinations of these two types of motifs were pivotal for predictive performance.

Our molecular descriptor, ATMOMACCS, can serve as a vital tool for advancing data-driven atmospheric science, addressing the need for more customized and accurate modelling in the field. Furthermore, the descriptor’s inherent interpretability and its strong performance in thermodynamic property prediction, with machine learning, show promise for further research in atmospheric chemistry.

This work was supported by the VILMA (Virtual laboratory for molecular level atmospheric transformations) centre of excellence funded by the Academy of Finland under grant 346377.

 

Besel, V. et al. (2023). Sci. Data 10, 1–11.

Bianchi, F et al. (2019). Chem. Rev. 119, 3472–3509.

Elm, J. et al. (2020) J. Aerosol Sci. 149, 105621.

Ferraz-Caetano, J. et al. (2024). Chemosphere, 359, 142257

Li, Y. et al. (2020). Atmos. Chem. Phys. 20, 8103–8122.

Lumiaro, E. et al. (2021). Atmos. Chem. Phys. 21, 13227–13246.

Lundberg, S. M. and Lee S.-I. (2017). Curran Associates Inc. 30, 9781510860964.

Sandström, H. et al. (2024). Adv. Sci. 11, 2306235.

Wang, C. et al. (2017).  Atmos. Chem. Phys. 17, 7529–7540.

How to cite: Lind, L., Sandström, H., and Rinke, P.: ATMOMACCS: Predicting atmospheric compound properties, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5719, https://doi.org/10.5194/egusphere-egu25-5719, 2025.

EGU25-6156 | ECS | Orals | AS3.1

Simulated photochemical response to observational constraints on aerosol vertical distribution over North China 

Xi Chen, Ke Li, Ting Yang, Xipeng Jin, Lei Chen, Yang Yang, Shuman Zhao, Bo Hu, Bin Zhu, Zifa Wang, and Hong Liao

The significance of Aerosol-photolysis interaction (API) in photochemistry has been emphasized by studies utilizing box models and chemical transport models. Some of them noted that API is closely related to aerosol vertical distributions. However, few studies have considered the actual aerosol vertical distribution when evaluating API due to the lack of observations and the substantial uncertainties in simulation. Herein, we used lidar and radiosonde observations with the GEOS-Chem model to quantify the response of photochemistry to observational constraints on aerosol vertical distribution across different seasons in North China. The underestimation of aerosol optical depth (AOD) in lower layers and the overestimation in upper layers were revised. Vertically, photolysis rates changed following AOD, showing 33.4%–73.8% increases at the surface. Ozone increased by an average of 0.9 ppb and 0.5 ppb in winter and summer and the default API impact on ozone reduced by 36%–56%. The weaker response in summer can be related to the compensatory effects of stronger turbulence mixing in the boundary layer. Besides, the underestimation of ozone levels in winter was improved by 8.5%. PM2.5 increased by 0.8 µg m−3 in winter and 0.2 µg m−3 in summer due to the promotion of photochemistry and increased more during pollution, with a maximum daily change of 16.5 µg m−3 at Beijing station in winter. The weakened API enhanced nitric acid (HNO3) formation by increasing the atmospheric oxidizing capacity (13.7% for OH radical) in high NOx emission areas and this helps explain the strong response of PM2.5in winter.

How to cite: Chen, X., Li, K., Yang, T., Jin, X., Chen, L., Yang, Y., Zhao, S., Hu, B., Zhu, B., Wang, Z., and Liao, H.: Simulated photochemical response to observational constraints on aerosol vertical distribution over North China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6156, https://doi.org/10.5194/egusphere-egu25-6156, 2025.

EGU25-6321 | ECS | Orals | AS3.1

Integrating Simulations and Observations: A Foundation Model for Estimating Aerosol Mixing State Index 

Fei Jiang, Zhonghua Zheng, Hugh Coe, David Topping, Nicole Riemer, and Matthew West

The aerosol chemical mixing state refers to the distribution of chemical components within individual aerosol particles, which affects their physical properties and interactions with the environment, such as light absorption, cloud formation, and potential health impacts. Accurate estimations of aerosol chemical mixing states are crucial for assessing both climate and health impacts. While particle-resolved models can track changes in aerosol compositions, they often struggle to capture real-world mixing states due to limitations in input data quality, such as emission inventories used in simulations.

In this study, we developed a deep learning foundation model based on particle-resolved simulations and fine-tuned it with limited observational data. The process-guided fine-tuned model improved R² by 300% compared to a fully data-driven baseline, effectively mitigating the challenges posed by sparse observational data and uncertainties model simulations.

Our approach enables dynamic estimations of aerosol mixing states in real-world environments, offering scalability and continuous learning.

How to cite: Jiang, F., Zheng, Z., Coe, H., Topping, D., Riemer, N., and West, M.: Integrating Simulations and Observations: A Foundation Model for Estimating Aerosol Mixing State Index, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6321, https://doi.org/10.5194/egusphere-egu25-6321, 2025.

EGU25-6515 | ECS | Orals | AS3.1

Size-fractionation of airborne particulate matter: chemical properties, distribution and health risk assessment – a one year study in Slovenia, Central Europe 

Anja Ilenič, Marija Đurić, Radmila Milačič Ščančar, Alenka Mauko Pranjić, and Janez Ščančar

The behavior and toxicity of particulate matter (PM) is primarily influenced by particle size and chemical composition, with fine (PM2.5) and ultrafine particles (PM0.1) posing the greatest health risks due to their deep respiratory penetration ability and enhanced adsorption capacity. While most studies focus on a single pollutant type – either organic or inorganic − using high-volume air samplers positioned far from areas commonly used by local commuters (e.g. rooftops), data on the multi-pollutant chemical composition of nanoparticles (PM1 or smaller) and their impacts on active commuters in urban environments remains scarce. A ground-level sampling device utilising a low-volume cascade system was employed to collect and fractionate PM-bound metal(oid)s and polycyclic aromatic hydrocarbons (PAHs), including in nanoparticles, over the course of one year in five urban areas across Slovenia, Europe. In the collected samples, metal(oid)s and PAHs were determined by inductively coupled plasma mass spectrometry following microwave-assisted acid digestion, and gas chromatography mass spectrometry after solvent extraction with mechanical shaking. The highest concentrations of metal(oid)s were predominantly found in PM10 (As, Cr, Ni, Pb) and PM<0.1 (Cd, Pd, Pt, Sb) fraction. High-molecular weight PAHs (BaA, BaP, BbF, BghiP, Ch, IP) were more abundant in PM10, while low-molecular weight PAHs (Fl, Na, Pa, P) were more prevalent in finer fractions. The highest concentrations of pollutants across all fractions and locations were consistently observed during the winter months. The contaminants investigated primarily originated from anthropogenic activities, particularly those associated with traffic emissions and biomass burning. Given that pollutants bound to the smallest airborne particles are the most harmful, it is essential to enhance pollution control measures and risk assessment strategies by addressing various PM fractions, including nano-sized particles.

How to cite: Ilenič, A., Đurić, M., Milačič Ščančar, R., Mauko Pranjić, A., and Ščančar, J.: Size-fractionation of airborne particulate matter: chemical properties, distribution and health risk assessment – a one year study in Slovenia, Central Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6515, https://doi.org/10.5194/egusphere-egu25-6515, 2025.

EGU25-6788 | ECS | Orals | AS3.1

Exploring the Role of Highly Oxygenated Organic Molecules in New Particle Formation Events with Explainable Artificial Intelligence 

Federica Bortolussi, James Brean, Shawon Barua, Avinash Kumar, Alexandra Karppinen, Siddharth Iyer, Hilda Sandström, Zongbo Shi, Roy Harrison, Patrick Rinke, and Matti Rissanen


New particle formation (NPF) is a significant source of atmospheric aerosols. The formation rate (J) quantifies the rate at which new particles form, and can be empirically determined from the particle number size distribution (PNSD). However, identifying the specific causes of NPF in urban areas remains challenging.
It is believed that in urban environments, most NPF occurs through the clustering of sulfuric acid (H2SO4) with bases. However, in a chamber study, it was observed that also the clustering of H2SO4 with highly oxygenated organic molecules (HOMs) may greatly promote NPF (Riccobono, 2014, Science, 344(6185), 717-721).

This research project employs AI data-driven approaches to predict J and examine the role of HOMs in NPF events.
The data were collected in August 2022 in two close sites in Leipzig, Germany: an urban background (Leibniz Institute for Tropospheric Research) and a roadside (Eisenbahnstraße). The data include HOMs, H2SO4, and bases from the nitrate CIMS, PNSD measurements, pollutants such as BC, and meteorological variables. Previous research indicated a higher concentration of OOMs at the roadside (Brean, 2024, Environ. Sci. Technol. 58, 10664−10674), suggesting its potential impact on J.

Preliminary results show that our data-driven model successfully predicted J values on a logarithmic scale with a mean absolute error of 0.33 at the urban background site and 0.63 at the roadside. Further analysis reveals the most significant contributors to predicting J, indicating that alongside H2SO4, various HOMs play a crucial role.

How to cite: Bortolussi, F., Brean, J., Barua, S., Kumar, A., Karppinen, A., Iyer, S., Sandström, H., Shi, Z., Harrison, R., Rinke, P., and Rissanen, M.: Exploring the Role of Highly Oxygenated Organic Molecules in New Particle Formation Events with Explainable Artificial Intelligence, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6788, https://doi.org/10.5194/egusphere-egu25-6788, 2025.

Aerosols exert a significant influence on the Earth's radiative balance. Black carbon (BC), a potent light-absorbing aerosol primarily generated from incomplete combustion of fossil fuels, biofuels, and biomass, has garnered substantial global research attention due to its substantial impact on regional and global climate change. However, long-term trends in aerosols in the western North Pacific remain poorly understood. Located at 2862 meters above sea level on Lulin Mountain in central Taiwan (23.47°N, 120.87°E), the Lulin Atmospheric Background Station (LABS) stands as the sole high-altitude background station in this region. Operational since the spring of 2006, LABS has been continuously monitoring the impact of various air pollutants through long-range transport. This study utilized continuous real-time measurements of PM10 (2006-2016), PM2.5 (2013-2020), and BC (2008-2020) collected at LABS using two tapered element oscillating microbalances (TEOM 1405) and an aethalometer (AE-31) to investigate their temporal variations, characteristics, and key controlling factors. Correlation analysis was employed to assess the influence of meteorological parameters on their monthly/seasonal burdens. The multi-year annual mean mass concentrations of PM10, PM2.5, and BC were determined to be 9.2, 7.2, and 0.4 µg m-3, respectively. Concentration-weighted trajectory analyses identified northern peninsular Southeast Asia and mainland China as major long-distance source regions for all aerosols at LABS, particularly during spring (March-May) and the northeast monsoon season (October-November), respectively. A slight downward trend in the mass concentrations of ambient aerosols was observed at LABS. This decline may be attributed to a decrease in biomass burning emissions from peninsular Southeast Asia, recent energy policy changes in China, and alterations in regional atmospheric boundary layer dynamics.

How to cite: Pani, S. K. and Lin, N.-H.: Long-term monitoring of ambient aerosols at a subtropical high-altitude mountain site in the western North Pacific, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9126, https://doi.org/10.5194/egusphere-egu25-9126, 2025.

Atmospheric particles impact our climate and adversely affect air quality and human health (IPCC, 2022; Pozzer et al., 2023). Molecular emissions in the atmosphere can react with ozone and radicals, forming a diverse array of organic compounds that can drive particle formation (Bianchi et al., 2019). However, due to the vast number of potential reactions and precursors, the identities of many of these particle-forming products remain largely unknown. Electron ionization mass spectrometry (EI-MS) is a widely used tool for identifying organic compounds in aerosol particle samples (Franklin et al., 2022; Worton et al., 2017; Hamilton et al., 2004). High-confidence identification relies on matching recorded EI-MS spectra to reference spectra in mass spectral libraries, which contain reference data for known compounds (Laskin et al., 2018). However, the identification of many atmospheric compounds is limited by a lack of reference data for these species (Nozière et al., 2015; Sandström et al., 2024).

In this presentation, I will introduce a simulated reference mass spectrometry dataset for atmospheric organic compounds. Using quantum chemistry and machine learning-based EI-MS simulation tools (Wei et al., 2019; Koopman & Grimme, 2021), we have simulated mass spectra for organic atmospheric compounds from the Master Chemical Mechanism (MCM v3.2, http://mcm.leeds.ac.uk/MCM, Wang et al., 2017). This simulated mass spectral dataset will be made publicly available to support future efforts to identify atmospheric organic compounds and advance our understanding of organic particle formation processes.

 

This work was supported by the VILMA (Virtual laboratory for molecular level atmospheric transformations) centre of excellence funded by the Research Council of Finland under grant 346377.

 

Bianchi, F., et al. (2019). Chemical Reviews, 119, 3472–3509.

Franklin, E. B., et al. (2022). Atmospheric Measurement Techniques, 15, 3779–3803.

Hamilton, J. F., et al. (2004). Atmospheric Chemistry and Physics, 4, 1279–1290.

IPCC. (2022). Climate Change 2022: Impacts, Adaptation, and Vulnerability. Cambridge University Press.

Koopman, J., & Grimme, S. (2021). Journal of the American Society for Mass Spectrometry, 32, 1735–1751.

Laskin, J., et al. (2018). Analytical Chemistry, 90, 166–189.

Nozière, B., et al. (2015). Chemical Reviews, 115, 3919–3983.

Pozzer, A., et al. (2023). GeoHealth, 7, 24711403.

Sandström, H., et al. (2024). Advanced Science, 11, 2306235.

Wang, C., et al. (2017). Atmospheric Chemistry and Physics, 17, 7529–7540.

Wei, J. N., et al. (2019). ACS Central Science, 5, 700–708.

Worton, D. R., et al. (2017). Analyst, 142, 2395–2403.

How to cite: Sandström, H. and Rinke, P.: Towards Atmospheric Compound Identification: A Reference Library of Simulated Electron Ionization Mass Spectra, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10129, https://doi.org/10.5194/egusphere-egu25-10129, 2025.

EGU25-10154 | ECS | Posters on site | AS3.1

Advancements in the incorporation of complex soot morphology within atmospheric sciences 

Baseerat Romshoo, Thomas Müller, Sascha Pfeifer, Jorge Saturno, Andreas Nowak, Yifan Yang, Ajit Ahlawat, Gazala Habib, Arun S. Babu, Anil Madariya, Andrea Cuesta, Shravan Deshmukh, Jaikrishna Patil, Tobias Michels, Marius Kloft, and Mira Pöhlker

Soot, also commonly known as black carbon (BC) aerosol, is an important short-lived climate forcer. Although global anthropogenic BC emissions from fossil fuel combustion are expected to decrease, BC remains a significant concern in air pollution hotspots in Asia and Africa. Estimates of the global black carbon direct radiative forcing are still subject to considerable uncertainties, ranging from 0.20 to 0.42 Wm⁻². To reduce these uncertainties, it is crucial to improve the representation of the complex soot morphology in simulations of their optical properties and global models. We have investigated various aspects of the optical properties of morphologically complex soot particles, including field and laboratory measurements, and optical simulations of BC as ‘realistic’ fractal aggregates. Investigations conducted in Delhi, a highly polluted urban environment in Asia, confirmed that fractal morphology is important in reducing the overestimation of aerosol light absorption by commonly used light simulation models by 10 to 80%.

To address the computationally expensive nature of fractal simulations, we propose a new metric known as the morphology index (MI). Additionally, to reduce the computational burden of optical simulations of fractal BC particles, we developed a fast and accurate machine learning-based tool for predicting the optical properties of BC fractal aggregates. We have highlighted the importance of the lack of representation of complex soot particles in global models, and offer methods to facilitate their integration into the atmospheric science community.

How to cite: Romshoo, B., Müller, T., Pfeifer, S., Saturno, J., Nowak, A., Yang, Y., Ahlawat, A., Habib, G., Babu, A. S., Madariya, A., Cuesta, A., Deshmukh, S., Patil, J., Michels, T., Kloft, M., and Pöhlker, M.: Advancements in the incorporation of complex soot morphology within atmospheric sciences, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10154, https://doi.org/10.5194/egusphere-egu25-10154, 2025.

EGU25-11092 | ECS | Posters on site | AS3.1

A Reduced Ordel Model for Aerosol Coagulation 

Oscar Jacquot, Virginie Ehrlacher, Tony Lelievre, and Karine Sartelet

Aerosol coagulation is a significant process regarding the dynamics of aerosols in the atmosphere. This process leads to an evolution of the size distribution of aerosols over time induced by particle collisions, and is described by Smoluchowski equation [1].
Accurate numerical simulations of this process are computationally demanding by typical discretization methods [2]. We investigate the effectiveness of the reduced basis method [3] to provide accurate but less demanding simulations, by constructing a reduced order subspace included within the reference high-dimensional space used to provide high fidelity simulations.
We also provide residual-based a posteriori error estimates [4] which enable certification of results up to a given error tolerance. We obtain efficient online model and error estimates as their online computational cost only scale with the reduced dimension, and not the dimension of the high-fidelity model.
By careful design of reduced subspaces we ensure that some properties of the high fidelity operator, such as mass conservation [5], are also preserved by reduced order models.

[1] M. V. Smoluchowski. Drei vortage uber diffusion, brownsche bewegung und koagulation von kolloidteilchen. Physik, 17, 557–585, 1916
[2] E. Debry, and B. Sportisse. Solving aerosol coagulation with size-binning methods. Applied Numerical Mathematics, 57(9), 1008–1020, 2007
[3] A. Quarteroni, et al. Reduced Basis Methods for Partial Differential Equations. Springer Cham. 2015
[4] M. Grepl, and A. Patera, A Posteriori Error Bounds for Reduced-Basis Approximations of Parametrized Parabolic Partial Differential EquationsESAIM: Mathematical Modelling and Numerical Analysis, 39(1), 157-181, 2005
[5] F. Filbet, and P. Laurençot. Mass-conserving solutions and non-conservative approximation to the Smoluchowski coagulation equation. Archiv der Mathematik, 83(6), 558-567, 2004

How to cite: Jacquot, O., Ehrlacher, V., Lelievre, T., and Sartelet, K.: A Reduced Ordel Model for Aerosol Coagulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11092, https://doi.org/10.5194/egusphere-egu25-11092, 2025.

EGU25-11298 | Orals | AS3.1

Rising alkali-to-acid ratios in the atmosphere may correspond to increased aerosol acidity 

Guangjie Zheng, Hang Su, Ruilin Wan, Xiaolin Duan, and Yafang Cheng

Aerosol acidity (or pH) is one central parameter in determining the health, climate and ecological effects of aerosols. While it is traditionally assumed that the long-term aerosol pH levels are determined by the relative abundances of atmospheric alkaline to acidic substances (referred to as RC/A hereinafter), we observed contrasting pH - RC/A trends at different sites globally, i.e., rising alkali-to-acid ratios in the atmosphere may unexpectedly lead to increased aerosol acidity. Here, we examined this apparently counter-intuitive phenomenon using the multiphase buffer theory. We show that the aerosol water content (AWC) set a pH “baseline” as the peak buffer pH, while the RC/A and particle-phase chemical compositions determine the deviation of pH from this baseline within the buffer ranges. Therefore, contrasting long-term pH trends may emerge when RC/A increases while AWC or nitrate fraction decreases, or vice versa. Our results provided a theoretical framework for a quantitatively understanding the response of aerosol pH to variations in SO2, NOx versus NH3 and dust emissions, offering broad applications in studies on aerosol pH and the associated environmental and health effects.

How to cite: Zheng, G., Su, H., Wan, R., Duan, X., and Cheng, Y.: Rising alkali-to-acid ratios in the atmosphere may correspond to increased aerosol acidity, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11298, https://doi.org/10.5194/egusphere-egu25-11298, 2025.

EGU25-11354 | Posters on site | AS3.1

An Improved Representation of Organic Aerosol Composition and Atmospheric Evolution in the EC-Earth3-AerChem model 

Stelios Myriokefalitakis, Stelios Kakavas, Marios Chatziparaschos, Vlassis Karydis, Alexandra Tsimpidi, Orfeas Karathanasopoulos, Lars Nieradzik, Maria Kanakidou, and Spyros N. Pandis

Organic compounds can constitute roughly half of the sub-micron aerosol mass in the troposphere, necessitating an accurate representation of organic aerosol (OA) in Earth system models (ESMs) to better capture aerosol-climate feedbacks. The secondary fraction of OA (SOA), however, formed through the oxidation of various volatile organic compounds (VOCs) from both natural and anthropogenic sources, complicates the description of OA in ESMs. Most ESMs either assume a non-volatile SOA produced with a constant yield from known precursors or provide a simplistic depiction of its volatility derived from biogenic VOCs, treating the primary fraction of OA (POA) as non-reactive and non-volatile. This approach often fails to accurately reproduce observed OA atmospheric measurement. On the other hand, biological materials such as bacteria, fungal spores, and various fragments released by living organisms into the atmosphere have been widely identified as part of the super-micron OA mass, which most ESMs also inadequately represent.

In the context of the H.F.R.I. project REINFORCE, we focus on improving the representation of atmospheric composition in Earth System Models (ESMs). We present simulations using the volatility basis set (VBS) approach to represent SOA formation, along with incorporating the organic fraction of bioaerosols. These developments are implemented in the state-of-the-art ESM, EC-Earth version 3, which includes interactive aerosols and atmospheric chemistry (EC-Earth3-AerChem). A lite version of the well-documented aerosol module ORACLE, which allows for relatively limited computing resource consumption, has been coupled to the CTM component of EC-Earth3-AerChem to calculate the partitioning and chemical evolution of POA vapors and their changes in volatility. The formation of SOA from semivolatile organic compounds (SVOCs) and intermediate-volatility organic compounds (IVOCs) has been added to the existing SOA formation scheme from biogenic VOCs in the model. Moreover, the three main types of bioaerosols—bacteria, fungal spores, and pollen grains—have been implemented into the model based on interactive bioaerosol schemes that depend on ecosystem types, the leaf area index (LAI), and various meteorological parameters. Bioaerosols in EC-Earth3-AerChem can also be transferred to the soluble aerosol coarse mode due to atmospheric aging processes. Overall, our efforts aim to bridge the gap between model simulations and observations, thereby enhancing our understanding of OA climate impacts.

How to cite: Myriokefalitakis, S., Kakavas, S., Chatziparaschos, M., Karydis, V., Tsimpidi, A., Karathanasopoulos, O., Nieradzik, L., Kanakidou, M., and Pandis, S. N.: An Improved Representation of Organic Aerosol Composition and Atmospheric Evolution in the EC-Earth3-AerChem model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11354, https://doi.org/10.5194/egusphere-egu25-11354, 2025.

EGU25-12803 | Orals | AS3.1

Role of Low-Volatility Oxygenated Organic Molecules in Urban Aerosol Nucleation in Houston, Texas  

Shan-Hu Lee, Lee Tiszenkel, James Flynn, and Alana Dodero

Atmospheric new particle formation (NPF) is an extremely complex chemical process that produces aerosols directly from gas phase species, impacting air quality, human health, and climate. Observations have shown frequent NPF in polluted urban areas even with high preexisting aerosols, but it is unclear how low-volatility oxygenated organics contribute to urban aerosol nucleation. Urban NPF studies in Chinese megacities show that urban nucleation takes place from sulfuric acid and dimethylamine, yet the measured aerosol nucleation rates cannot be explained with sulfuric acid and dimethylamine alone. There are abundant oxygenated organic molecules (OOM) in Chinese megacities, but these OOMs primarily form from oxidation reactions of aromatic compounds and the majority of OOMs contain nitrates and the volatilities of OOMs are not sufficiently low enough to be able to nucleate. To understand the role of low-volatility OOMs in urban aerosol nucleation, we conducted comprehensive measurements of NPF precursors in Houston, the 4th most populated and polluted urban site in the United States. Our observations, together with numerical parameterizations constrained by the in-situ measured chemical precursors and based on the algorithms provided by the chamber experiments, show that rapid nucleation and growth of freshly formed clusters can be explained by the measured sulfuric acid, base, and low-volatility OOMs (with saturation vapor concentrations in the low or extremely volatility ranges). The chemical composition analysis of OOMs, together with F0AM box model simulations incorporated with the Master Chemical Mechanism, show that under the urban Houston conditions, OOMs form oxidation from both biogenic and anthropogenic VOCs, and autoxidation and dimerization of organic peroxides are not suppressed by NOx. Our findings thus contrast with previous urban studies mostly made in Chinese megacities, demonstrating the distinctively different roles of organics in urban aerosol nucleation under different urban settings due to different emission profiles and chemical compositions of air pollutants. Given rapid global urbanization and increasing emissions of emerging chemical pollutants in the United States and Europe, this multicomponent nucleation process will be crucial for mitigating air pollution in the evolving urban climate.

How to cite: Lee, S.-H., Tiszenkel, L., Flynn, J., and Dodero, A.: Role of Low-Volatility Oxygenated Organic Molecules in Urban Aerosol Nucleation in Houston, Texas , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12803, https://doi.org/10.5194/egusphere-egu25-12803, 2025.

EGU25-13343 | Posters on site | AS3.1

Characterization of Aerosols for Stratospheric Solar Radiation Management 

Svitlana Malashevych, Aleksandr Odelskii, Alexander Logozzo, and Thomas Preston

Understanding the properties of aerosols under stratospheric conditions is of particular importance for applications in solar radiation management. Aerosols have the potential to influence the Earth's radiative balance by stratospheric aerosol injection (SAI), which increases albedo and enhances the reflection of solar radiation back into space. By investigating the optical properties of various aerosol types under different environmental conditions, we aim to explore materials for SAI that exhibit albedo-enhancing potential while maintaining stability in the stratosphere.

We have developed an optical trapping system with counter-propagating laser beams coupled with cavity-enhanced Raman spectroscopy to monitor the physical properties of single aerosol particles. This technique, supported by bulk measurements, enables us to determine the wavelength-dependent refractive index under different temperature and relative humidity parameters. Our specially designed optical system allows for rapid changes in temperature and relative humidity using a movable platform while maintaining a stable gradient within the cell reproducing stratospheric conditions. Our findings contribute to a deeper understanding of the suitability of aerosols for climate mitigation strategy and the broader effects of their deployment.

How to cite: Malashevych, S., Odelskii, A., Logozzo, A., and Preston, T.: Characterization of Aerosols for Stratospheric Solar Radiation Management, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13343, https://doi.org/10.5194/egusphere-egu25-13343, 2025.

Atmospheric soot and organic particles from fossil fuel combustion and biomass burning modify Earth’s climate through their interactions with solar radiation and through modifications of cloud properties by acting as cloud condensation nuclei and ice nucleating particles. Recent advancements in understanding their individual properties and microscopic composition have led to heightened interest in their microphysical properties. This review article provides an overview of current advanced microscopic measurements and offers insights into future avenues for studying microphysical properties of these particles. To quantify soot morphology and ageing, fractal dimension (Df) is a commonly employed quantitative metric which allows to characterize morphologies of soot aggregates and their modifications in relation to ageing factors like internal mixing state, core-shell structures, phase, and composition heterogeneity. Models have been developed to incorporate Dfand mixing diversity metrics of aged soot particles, enabling quantitative assessment of their optical absorption and radiative forcing effects. The microphysical properties of soot and organic particles are complex and they are influenced by particle sources, ageing process, and meteorological conditions. Furthermore, soluble organic particles exhibit diverse forms and can engage in liquid-liquid phase separation with sulfate and nitrate components. Primary carbonaceous particles such as tar balls and soot warrant further attention due to their strong light absorbing properties, presence of toxic organic constituents, and small size, which can impact human health. Future research needs include both atmospheric measurements and modeling approaches, focusing on changes in the mixing structures of soot and organic particle ensembles, their effects on climate dynamics and human health.

How to cite: Li, W.: Microphysical Properties of Atmospheric Soot and Organic Particles: Measurements, Modeling, and Impacts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14445, https://doi.org/10.5194/egusphere-egu25-14445, 2025.

EGU25-15947 | ECS | Posters on site | AS3.1

The heterogeneous reaction of HNO3 and HCl with CaCO3 in the context of stratospheric aerosol injection and its impact on stratospheric ozone 

Célia Paolucci, Sandro Vattioni, Beiping Luo, Thomas Peter, Arnold Müller, Christof Vockenhuber, and Markus Ammann

Lack of action in climate change mitigation is driving research on solar radiation modification via stratospheric aerosol injection (SAI), i.e., the injection of aerosols or their precursors into the stratosphere to increase Earth’s albedo, inducing global cooling. The idea evolved from observations of the cooling effect of large volcanic eruptions, which emitted SO2 into the stratosphere. Therefore, SAI research mainly focused on sulfur dioxide (SO2) injection, the main precursor of H2SO4 aerosols. However, SO2 injection could lead to adverse side effects such as stratospheric ozone depletion, stratospheric heating, and sizable effects on the large-scale atmospheric circulation. Recent studies suggested that injection of solid particles such as calcite (CaCO3), alumina (Al2O3) and diamond (C) instead of SO2 could reduce some of these adverse side effects. However, the expected improvements are subject to large uncertainties. Heterogeneous chemistry on solid aerosols in the stratosphere can increase ozone depletion by moving passive chlorine reservoir species such as HCl or ClONO2 into their active, ozone depleting form (e.g., ClO). Furthermore, alkaline materials such as CaCO3 are subject to acid-base reactions resulting in an uptake of acidic gases which could impact stratospheric ozone. We constrain some of these uncertainties by experimental work on heterogeneous chemistry of CaCO3 in presence of gaseous HCl, HNO3, and H2SO4 under near-stratospheric conditions. Single crystalline CaCO3 {001} and {104} faces were exposed to controlled gas mixtures closely above either a binary HNO3/H2SO4 or HCl/H2SO4 solution, or a ternary HNO3/HCl/H2SO4 solution for several days. Fixed temperature ranging between -20°C and -60°C were investigated, reaching lower temperature conditions than in previous experiments. Various Relative Humidities (RH) were as well probed. Elastic Recoil Detection Analysis (ERDA), an ion beam analysis technique to obtain elemental concentration depth profile of up to 300 nm, was used to observe surface reaction and diffusion in the material. Uptake coefficients were calculated from these observations. This work presents a path forward for climate intervention research and more specifically for more reliably assessing the impact of SAI of solid particles on stratospheric ozone.

How to cite: Paolucci, C., Vattioni, S., Luo, B., Peter, T., Müller, A., Vockenhuber, C., and Ammann, M.: The heterogeneous reaction of HNO3 and HCl with CaCO3 in the context of stratospheric aerosol injection and its impact on stratospheric ozone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15947, https://doi.org/10.5194/egusphere-egu25-15947, 2025.

Data driven tools are emerging across all domains, largely held under the banner of AI. This includes developments at the interface between academic research and policy implementation. Data science, as a much broader discipline, also requires us to consider the supporting ecosystem of infrastructure and principles that underpin data access and sustainability. The research community is now constantly demonstrating more potential applications within air quality research, from molecular through to global scales. Likewise, the gap between air quality and health research is closing through demonstrable applications of data science approaches.

Alongside this, the UKs Natural Environment Research Council (NERC) Digital Solutions programme is funding a new national facility to connect environmental data with users in the public and private sector, covering health and climate use cases. Taking the unusual approach of asking what end-users may need, in this presentation we present outcomes from workshops held across the UK. We find remaining challenges centre around access and sustainable delivery and discuss the cultural dependencies on the research community. With a focus around the rapidly evolving pace of AI, we present several overarching developments including work on using Large Language Models (LLMs) to improve search and discovery of air quality data.

 

 

How to cite: Topping, D. and Kingston, R.: Building a new national facility to connect the UK’s environmental data holdings with end-users across multiple sectors: a case study on linking air quality and health data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16046, https://doi.org/10.5194/egusphere-egu25-16046, 2025.

EGU25-17174 | ECS | Posters on site | AS3.1

Impact of Aircraft Emissions on Ultrafine Particles Sulfate Content around Frankfurt/Main international Airport 

Truong Thi Huyen, Dominik van Pinxteren, Florian Ungeheuer, Alexander Vogel, and Hartmut Herrmann

Numerous studies have been reported that airport is an important source of ultrafine particles (UFPs, Dp ≤ 100 nm), potentially affecting the health of nearby residents. This study measured UFPs at the Frankfurt/Main international airport as well as in three locations (Raunheim, Schwanheim and Riedberg) at about 5 to 15 km from the airport. Cascade impactors (NanoMOUDI, TSI Inc.) collected UFPs in the size fractions of 56-100, 32-56, 18-32, and 10-18 nm on aluminum substrates during different seasons, allowing the observation of ground-level transport of UFPs. Before the campaign, three models of nanoMOUDI used in this study were collocated at the Goethe University (Riedberg campus) to compare data consistency. Inorganic ions, in particular sulfate, were then analyzed to determine the contribution of sulfur dioxide and sulfuric acid nucleation to the UFP mass concentration. Preliminary results indicate that the sampling efficiencies at UFP stages differed between the three applied impactor models and correction factors might need to be applied for more accurate concentration comparison. The measurements at the Frankfurt/Main international airport during Autumn 2023 showed highest concentrations of sulphate in the 32-56 nm size range, at approximately 40 ng m-3, followed by 56-100 nm, 18-32 nm at ~18 and ~8 ng m-3, respectively, and the lowest concentration was in the 10-18 nm range at ~2 ng m-3. In the measurement campaigns in 2024, the preliminary results show mostly lower average sulfate concentrations in the UFP range at the sites more distant from the airport, ranging from ~ 2 ng m-3 to ~20 ng m-3. Similar relative variations across the UFP size range were observed at the two sites of Raunheim (mostly upwind of the airport) and Riedberg (~ 15 km away from the airport). The highest sulfate concentrations were found in the size range of 56-100 nm and the lowest concentration in the size range of 10-18 nm in both locations. The lowest sulfate concentration was also observed in the 10-18 nm size range in the samples collected at Schwanheim, the sampling site located closer and mostly downwind of the airport. However, the peak sulfate concentration was found in the size range of 32-56 nm, more similar to the relative profile observed directly on the airport. Next to emissions from aircraft engines, the difference in the peak concentration of sulfate may be influenced by several other factors, such as wind direction or other local emissions in the sampling sites. Detailed comparisons of UFP sulfate concentrations together with considerations of local meteorological conditions during the sampling periods will be presented in this contribution.

How to cite: Thi Huyen, T., van Pinxteren, D., Ungeheuer, F., Vogel, A., and Herrmann, H.: Impact of Aircraft Emissions on Ultrafine Particles Sulfate Content around Frankfurt/Main international Airport, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17174, https://doi.org/10.5194/egusphere-egu25-17174, 2025.

Atrazine is a selective synthetic triazine herbicide that is primarily used for the management of weeds in corn. Despite being banned in the EU in 2004, it is still used in large quantities globally. Numerous studies have demonstrated adverse effects of atrazine on organisms, particularly its role as an endocrine disruptor causing reproductive dysfunction in vertebrates.1 The occurrence, effects and fate of atrazine in soil and water has been well studied. However, a less investigated pathway for the spread of pesticides is through the atmosphere. Via long-range atmospheric transport (LRAT) pesticides can be transported to pristine environments.2,3

To investigate atmospheric concentrations of atrazine, particulate matter (PM2.5) samples were collected at the rural background station Taunus Observatory, Germany. The collected filters underwent liquid extraction, enrichment, and analysis using high-performance liquid chromatography - high resolution mass spectrometry. Samples from April 2021 to May 2022 were analyzed in two-week increments. For a more detailed examination one intensive two-week period was analyzed. Using the FLEXible PARTicle Lagrangian transport and dispersion model (FLEXPART)4 we identified source regions of atrazine.

The analysis successfully quantified atrazine in PM2.5 samples. Concentrations showed seasonal variation, with high concentrations observed in May and June, corresponding to typical agricultural application periods in the Northern Hemisphere. These results suggest that atrazine detected in the atmosphere is linked to recent usage rather than legacy contamination and wind-driven resuspension from soil.  A simple partitioning calculation suggests that atrazine primarily partitions into the partice phase, especially at higher altitudes, which may extend its atmospheric half-life facilitating its potential for LRAT. Backward trajectory modeling indicated that low atrazine concentrations were associated with air masses originating from Europe, whereas higher concentrations corresponded to transatlantic transport from North America.

Our study confirms the presence of atrazine in PM and provides evidence of its LRAT from regions where it is still in use. These results highlight the need for revising pesticide risk assessments accounting for the potential extension of pesticides atmospheric half-life in the condensed phase.5

 

 (1) Rohr, J. R.; McCoy, K. A. A qualitative meta-analysis reveals consistent effects of atrazine on freshwater fish and amphibians. Environmental health perspectives 118, 20–32, 2010.

(2) Mayer, L.; Degrendele, C.; Šenk, P.; Kohoutek, J.; Přibylová, P.; Kukučka, P.; Melymuk, L.; Durand, A.; Ravier, S.; Alastuey, A.; et al. Widespread Pesticide Distribution in the European Atmosphere Questions their Degradability in Air. Environmental science & technology 58, 3342–3352, 2024.

(3) Thurman, E. M.; Cromwell, A. E. Atmospheric Transport, Deposition, and Fate of Triazine Herbicides and Their Metabolites in Pristine Areas at Isle Royale National Park. Environ. Sci. Technol. 34, 3079–3085, 2000.

(4) Bakels, L.; Tatsii, D.; Tipka, A.; Thompson, R.; Dütsch, M.; Blaschek, M.; Seibert, P.; Baier, K.; Bucci, S.; Cassiani, M.; et al. FLEXPART version 11: improved accuracy, efficiency, and flexibility. Geosci. Model Dev. 17, 7595–7627, 2024.

(5) Socorro, J.; Durand, A.; Temime-Roussel, B.; Gligorovski, S.; Wortham, H.; Quivet, E. The persistence of pesticides in atmospheric particulate phase: An emerging air quality issue. Scientific reports 6, 33456, 2016.

How to cite: Vogel, A., Saur, F., and Jesswein, M.: Detection of the Herbizide Atrazine in PM2.5 at a Rural Background Station in Germany: Evidence of Long-Range Atmospheric Transport, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17251, https://doi.org/10.5194/egusphere-egu25-17251, 2025.

Long-Term Variability of Air Pollutants in the Indo-Gangetic Plain: Drivers, Trends, and Hotspots

Abhishek Saxena

Saxenaabhishek85@gmail.com

This study examines seasonal, monthly, and yearly trends of sulfur dioxide (SO₂), black carbon (BC), carbon monoxide (CO), ozone (O₃), fine particulate matter (PM2.5), and methane (CH₄) across the Indo-Gangetic Plain (IGP) from 2010 to 2024 using MERRA-2 Reanalysis data (0.5° x 0.625° resolution). Elevated concentrations of SO₂, BC, CO, PM2.5, and CH₄ are observed during winter and post-monsoon months due to thermal inversions, stagnant conditions, and emissions from biomass burning and agriculture, while O₃ peaks during summer due to photochemical activity.

Yearly trends show declines in SO₂ and PM2.5 due to emission controls, while BC, CO, and CH₄ remain stable, and O₃ increases slightly with rising precursor emissions. The western IGP, particularly Punjab and Haryana, is identified as a hotspot for SO₂, BC, CO, PM2.5, and CH₄ in post-monsoon, with O₃ hotspots prevalent in summer. Correlations among pollutants vary seasonally, with stronger links in winter and weaker ones during monsoon. These findings highlight the need for targeted, multi-pollutant mitigation strategies tailored to seasonal and regional pollution dynamics in the IGP.

 

 

How to cite: Saxena, A.: Long-Term Variability of Air Pollutants in the Indo-Gangetic Plain: Drivers, Trends, and Hotspots, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17261, https://doi.org/10.5194/egusphere-egu25-17261, 2025.

EGU25-17364 | ECS | Orals | AS3.1

Atmospheric black carbon mass absorption cross-section: a literature review 

Jorge Saturno, Joel C. Corbin, John Backman, Konstantina Vasilatou, Ernest Weingartner, Krzysztof Ciupek, Thomas Müller, Babu Suja Arun, Griša Močnik, Luka Drinovec, Konstantinos Eleftheriadis, and Eija Asmi

Black carbon (BC) aerosol particles are emitted by the incomplete combustion of carbonaceous fuels. These particles absorb solar radiation and BC-dominated aerosol mixtures with low single scattering albedo have a positive radiative forcing, thus heating the atmosphere. Radiative transfer models make use of the BC mass absorption cross section (MACBC) to derive the radiative forcing of BC given a certain particle mass concentration. Freshly emitted BC has a MAC value of 8 ± 1 m2/g at 550 nm (Bond et al., 2013). However, MAC can increase as aerosols age in the atmosphere due to increase in particle coating. This is the so-called lensing effect, which leads to MACBC observations of up to 15 m2/g at 550 nm (Li et al., 2022; Savadkoohi et al., 2024). The effect of coatings and the evolution of MACBC with ageing have been and still are a matter of intense scientific discussions.

The determination of MACBC is carried out in the lab and in the field using various methods for light absorption and BC mass measurement. The most common techniques for absorption measurement include filter-based attenuation measurements, whereas the most common technique for mass measurement is thermo-optical analysis, which quantifies elemental carbon mass (EC; EN 16909:2017). The development of more accurate techniques with operational and scientific advantages for both light absorption and BC mass quantification has led to more reliable MACBC field measurements, allowing researchers to have a clearer picture of how atmospheric ageing and regional conditions affect the optical properties of BC.

In this study, we have reviewed 63 publications that provide atmospheric MACBC values and present the results in terms of aerosol type, measurement technique, regional variability, and how interpretation of results using these factors can help the community to use the appropriate MAC in models. We provide guidance and perspectives for future studies and how the literature on MACBC can be exploited and interpreted in order to improve radiative models that include BC.

References

 Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T., DeAngelo, B. J., Flanner, M. G., Ghan, S., Kärcher, B., Koch, D., Kinne, S., Kondo, Y., Quinn, P. K., Sarofim, M. C., Schultz, M. G., Schulz, M., Venkataraman, C., Zhang, H., Zhang, S., … Zender, C. S. (2013). Bounding the role of black carbon in the climate system: A scientific assessment. Journal of Geophysical Research: Atmospheres, 118(11), 5380–5552. https://doi.org/10.1002/jgrd.50171

Hanyang Li & Andrew A. May (2022) Estimating mass-absorption cross-section of ambient black carbon aerosols: Theoretical, empirical, and machine learning models, Aerosol Science and Technology, 56:11, 980-997, https://doi.org/10.1080/02786826.2022.2114311

Savadkoohi, Marjan, Marco Pandolfi, Cristina Reche, Jarkko V. Niemi, Dennis Mooibroek, Gloria Titos, David C. Green, et al. (2023) The Variability of Mass Concentrations and Source Apportionment Analysis of Equivalent Black Carbon across Urban Europe. Environment International 178: 108081. https://doi.org/10.1016/j.envint.2023.108081.

How to cite: Saturno, J., Corbin, J. C., Backman, J., Vasilatou, K., Weingartner, E., Ciupek, K., Müller, T., Arun, B. S., Močnik, G., Drinovec, L., Eleftheriadis, K., and Asmi, E.: Atmospheric black carbon mass absorption cross-section: a literature review, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17364, https://doi.org/10.5194/egusphere-egu25-17364, 2025.

EGU25-17482 | Orals | AS3.1

Measurement of ultrafine Particles (2 to 800 nm) in the Rhein-Main area with a special Emphasis on Airport Emissions 

Manuel Granzin, Lena Große Schute, Diana Rose, Florian Ditas, Joachim Curtius, and Andreas Kürten

In recent years, the importance of ultrafine particle (UFP) measurements has increased significantly, particularly due to their adverse health effects. For this reason, it is important to further investigate and characterise strong UFP sources, especially in densely populated urban and suburban areas, to shed more light on their impact on local air quality. Former studies have already shown that highly frequented airports are a major source of UFPs (Hudda et al. 2014, Keuken et al. 2015); these studies further showed that even over long distances of up to 10 km downwind of the airport, UFP concentrations are significantly elevated. In this study, we deployed a variety of instruments to characterise the UFPs from Frankfurt Airport (FRA) in the densely populated Rhein-Main area. Size and concentration levels over a size range from 2-800 nm were measured at three different locations which are located 4, 8, and 15 km away from the airport, respectively. Overall, the measurements were conducted over a duration of 6 months. As a result, we found that aerosol emissions from the airport dominate the aerosol population of the neighbouring districts (up to a distance of at least 15 km) to a great extent. This can be seen when comparing particle number concentrations downwind of the airport versus urban background levels. The average diurnal particle number concentration at the closest measurement station with a distance of 4 km from the airport is elevated by almost a factor of 6 during the airport operating hours (05:00 – 23:00) compared to the urban background when the wind is arriving from the airport. Additionally, we found that the particle number concentration of diameters above 3 nm is up to a factor of 5 to 6 higher than the fraction above 10 nm, indicating that a large fraction of aircraft aerosol emissions is below 10 nm in size and therefore remains mostly undetected by standardised UFP measurements. This suggests that the particle burden can be significantly underestimated when only focussing on particles larger than 10 nm. In the presentation a detailed analysis of the measured results at the three different stations will be presented. The analysis focuses on the dependence of the diurnal pattern of the aerosol size distribution as a function of the origin of the air masses (wind direction). This way, airport emissions can be distinguished from other traffic emissions and the urban background. Furthermore, we present direct evidence that landing airplanes can contribute significantly to the smallest measurable particles < 10 nm. Overall, we conclude that for a full assessment of the negative health effects of UFP emissions it is important to (1) increase the number of monitoring stations, especially in areas with strong sources such as airports and (2) lower the size of the smallest particles that are detected from 10 to 3 nm, in order to determine the UFP concentrations and health risks more realistically.

How to cite: Granzin, M., Große Schute, L., Rose, D., Ditas, F., Curtius, J., and Kürten, A.: Measurement of ultrafine Particles (2 to 800 nm) in the Rhein-Main area with a special Emphasis on Airport Emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17482, https://doi.org/10.5194/egusphere-egu25-17482, 2025.

EGU25-18595 | Orals | AS3.1

Impact of nanostructure on hygroscopicity and reactivity of fatty acid atmospheric aerosol proxies. 

Christian Pfrang, Adam Milsom, Ben Woden, Maximilian Skoda, Yizhou Su, Andy Ward, Andy Smith, Adam Squires, and Ben Laurence

Atmospheric aerosol hygroscopicity and reactivity play key roles in determining the aerosol’s fate and are strongly affected by its composition and physical properties. Fatty acids are surfactants commonly found in organic aerosol emissions. They form a wide range of different nanostructures dependent on water content and mixture composition. We follow nano-structural changes in mixtures frequently found in urban organic aerosol emissions, i.e. linoleic acid (LOA), oleic acid (OA), sodium oleate and fructose, during humidity change and exposure to the atmospheric oxidant ozone. Small-Angle X-ray Scattering (SAXS) was employed (Milsom et al., 2024) to derive the hygroscopicity of each nanostructure by measuring time- and humidity-resolved changes in nano-structural parameters. We found that hygroscopicity is directly linked to the specific nanostructure. Reaction with ozone revealed a clear nanostructure-reactivity trend, with notable differences between the individual nanostructures investigated. Simultaneous Raman microscopy complementing the SAXS studies revealed the persistence of oleic acid even after extensive oxidation. Our findings demonstrate that self-assembly of fatty acid nanostructures can significantly impact water uptake and chemical reactivity, thus directly affecting the atmospheric lifetime of these materials.

Another focus of our studies are one-molecule thin layers of LOA and their behaviours when exposed to ozone in multi-component films at the air–water interface (Woden et al., 2024). LOA’s two double bonds allow for ozone-initiated autoxidation, a radical self-oxidation process, as well as traditional ozonolysis. Neutron reflectometry was employed to follow the kinetics of these films in real time in a temperature-controlled environment. We oxidised deuterated LOA (d-LOA) as a monolayer, and in mixed two-component films with either oleic acid (h-OA) or its methyl ester, methyl oleate (h-MO), at room temperature and atmospherically more realistic temperatures of 3 ± 1 °C. We found that the temperature change did not notably affect the reaction rate which was similar to that of pure OA. Kinetic multi-layer modelling using our Multilayer-Py package showed that neither temperature change nor introduction of co-deposited film components alongside d-LOA consistently affected oxidation rates, but the deviation from a single process decay behaviour (indicative of autoxidation) at 98 ppb is clearest for pure d-LOA, weaker for h-MO mixtures and weakest for h-OA mixtures. As atmospheric surfactants will be present in complex, multi-component mixtures, it is important to understand the reasons for these different behaviours even in two-component mixtures of closely related species. Our work demonstrates that it is essential to employ atmospherically realistic ozone levels as well as multi-component mixtures to understand LOA behaviour at low O3 in the atmosphere. Residue formation may be affected by the temperature change, potentially impacting on the persistence of the organic character at the surface of aqueous droplets. Our findings could have impacts on both urban air quality (e.g. protecting harmful urban emissions from atmospheric degradation and therefore enabling their long-range transport), and climate (e.g. affecting cloud formation), with implications for human health and wellbeing.

Milsom et al., Atmos. Chem. Phys., 2024, 24, 13571–13586, DOI: 10.5194/acp-24-13571-2024, 2024.

Woden et al., Faraday Discuss., 2024, DOI: 10.1039/D4FD00167B.

How to cite: Pfrang, C., Milsom, A., Woden, B., Skoda, M., Su, Y., Ward, A., Smith, A., Squires, A., and Laurence, B.: Impact of nanostructure on hygroscopicity and reactivity of fatty acid atmospheric aerosol proxies., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18595, https://doi.org/10.5194/egusphere-egu25-18595, 2025.

EGU25-19425 | ECS | Orals | AS3.1

Investigating Organic-Mineral Core-Shell Aerosols: A Study of Hydroxyl Radical Oxidation 

Megan Poole, Andy Ward, and Martin King

Aerosols significantly influence air quality, climate, and health. Specifically, aerosols can influence climate directly though scattering/absorbing and indirectly in their capacity of cloud condensation nuclei. Aerosols exist in the atmosphere in different morphologies (e.g. core-shell) which can as a result can affect their scattering properties. This study explores the Mie scattering of an organically coated mineral aerosol when exposed to an atmospherically significant oxidant: Hydroxyl radical, OH∙.

Figure 1. Laser tweezer trap with annotated optical pathway.

Atmospheric oxidation by OH∙ can cause changes to an organic particle’s optical properties. Utilising a combination of Optical Tweezers and Mie Spectroscopy (figure 1) the significance of exposure to OH∙ has on both homogenous and coated aerosols can be studied. These techniques were used since they enable the manipulation and analysis of individual aerosol particles (~1 µm radii) in a controlled environment. OH∙ was generated in situ, due to its short lifetime, through the mechanism outlined in equation 1.

(eq.1)

From Mie theory we know that the movement of Mie resonance peaks indicate a change in the optical properties of the levitated particle. Said changes can be attributed to loss of organic material and/or shift in refractive index (indicating a chemical change in the organic sample).

Figure 2. Line graph illustrating the movement of a single peak from the recorded Mie spectra (peak shift) over time whilst the optically levitated particle is exposed to OH∙.

 

Results are measured in terms of the shifting of Mie resonance peaks and show that real urban atmospheric coatings react with OH∙, and that reaction is to a significant scale (-1.23 nm / 60 minutes) as seen in figure 2. Woodsmoke yielded no significant reaction (figure 2). Squalane thin films reacted significantly, presenting a peak shift of -5.73 nm / 60 minutes and was repeatable (figure 2). The homogenous squalane droplets also showed significant change. Overall, it has been determined that for the squalane and real urban organic samples form a core-shell morphology with silica. Furthermore, these thin films present a negative shift in peak position indicating a significant loss of material when exposed to OH∙. Therefore, it can be concluded that OH∙ results in alteration of the optical properties of organic thin films, and this observable behaviour can be considered to an order of magnitude that should be accounted for in atmospheric radiative forcing calculations, however future work is required to model this with detail.

This work was supported by the Natural Environment Research Council and the ARIES Doctoral Training Partnership [grant number NE/S007334/1], NERC grant NE/T00732X/1, with additional support from STFC's Central Laser Facility for access at the Research Complex at Harwell.

How to cite: Poole, M., Ward, A., and King, M.: Investigating Organic-Mineral Core-Shell Aerosols: A Study of Hydroxyl Radical Oxidation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19425, https://doi.org/10.5194/egusphere-egu25-19425, 2025.

EGU25-19589 | ECS | Orals | AS3.1

Global inversions of black carbon emissions using TM5-MP coupled with CTDAS 

Angelos Gkouvousis, Nikos Gialesakis, Alexis Drosos, Ioannis Maris, and Maria Kanakidou

Black Carbon (BC) aerosol is a major short-lived climate forcer which plays a significant role in both atmospheric warming and air quality. BC is emitted during incomplete combustion during fossil fuel combustion, biomass burning and domestic heating but its emission fluxes estimate remains uncertain. The accurate representation of BC fluxes and its atmospheric fate in climate models is crucial for understanding BC contribution to climate change. This study aims to optimize the total BC emissions, using as starting point the emission inventories provided by CMIP6 for both anthropogenic and biomass burning sources. For this, a data assimilation global 3-d modeling system was used together with filter and aethalometer measurements of BC worldwide. The assimilation system used is the forward chemistry and transport model TM5-MP combined with the Carbon Tracker Data Assimilation Shell (CTDAS) that utilizes an Ensemble Kalman filter data assimilation method. The TM5-MP model simulates atmospheric chemistry and aerosol microphysics using the M7 module in the global atmosphere driven by ERA-5 meteorology and running with a 2ox3o horizontal resolution and 25 hybrid levels up to 0.1 hPa. The efficiency of the optimisation method is evaluated by comparing the forward simulations with the aerosol optical depth observations from the AERONET network before and after the emission optimization.

How to cite: Gkouvousis, A., Gialesakis, N., Drosos, A., Maris, I., and Kanakidou, M.: Global inversions of black carbon emissions using TM5-MP coupled with CTDAS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19589, https://doi.org/10.5194/egusphere-egu25-19589, 2025.

EGU25-19876 | Orals | AS3.1

Multiseasonal aerosol pH variations between boundary layer and free tropospheric airmasses in the East Mediterranian during the CleanCloud CHOPIN Campaign 

Athanasios Nenes, Carolina Molina, Romanos Foskinis, Olga Zografou, Maria Gini, Kostantinos Granakis, Prodromos Fetfatzis, Christos Mitsios, Alexandros Papayannis, and Konstatinos Eleftheriadis

Atmospheric acidity is a major aerosol parameter that influences atmospheric chemistry, nutrient availability and deposition rates, aerosol formation and growth rates, nutrient availability, aerosol toxicity and the ability of aerosol to nucleate ice crystals and cloud droplets. Aerosol acidity depends on the concentration and volatility of precursor gases/bases, the amount of non-volatile cations (such as Ca, K, Mg), sulfate, temperature and humidity. Understanding how aerosol acidity changes between airmasses and its vertical evolution from moist, warm boundary layer conditions (close to source regions), into the dry, cold and clean free tropospheric air is highly unconstrained from observations. High altitude mountaintop sites observations offer a unique opportunity to address this uncertainty, as observations required to constrain aerosol pH can be carried out for extensive periods of time, and can sample both free tropospheric and boundary layer air from a variety of sources and over different seasons.

This study addresses the need for vertical profiling of aerosol pH by utilizing the extensive dataset available from the CleanCloud CHOPIN field campaign (https://go.epfl.ch/chopin-campaign) at Mount Helmos, Greece from Fall 2024 to Spring 2025. pH is calculated with the ISORROPIA-Lite thermodynamic model applied to the aerosol chemical composition and gas-phase NH3 measurements carried out at the Helmos Hellenic Atmospheric Aerosol and Climate Change ((HAC)²) station (2314 m a.s.l.) at mount Helmos. Airmass origin is identified through a series of chemical and turbulence metrics (to identify when observations correspond to boundary layer or free tropospheric conditions) and backtrajectory analysis when the site is residing in the free troposphere. We observed a clear daily pH cycle at the site, with lower pH values between 7 am and 1 pm, where the airmass is predominantly influenced by free tropospheric air. Higher pH values tend to be observed in the afternoon when ammonia associated with anthropogenic emissions from nearby urban and agricultural activities reached the station, which together with higher humidity and ammonia levels end up reducing acidity. Seasonal variations and the influences of dust episodes, biomass burning and temperature are all analyzed to determine "characteristic" acidity levels associated with each airmass type and infleunce. We then conclude by discussing the implications of the acidity levels for nutrient availability and deposition in each regime, and discuss the ability of models to reproduce the observed acidity patterns.

How to cite: Nenes, A., Molina, C., Foskinis, R., Zografou, O., Gini, M., Granakis, K., Fetfatzis, P., Mitsios, C., Papayannis, A., and Eleftheriadis, K.: Multiseasonal aerosol pH variations between boundary layer and free tropospheric airmasses in the East Mediterranian during the CleanCloud CHOPIN Campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19876, https://doi.org/10.5194/egusphere-egu25-19876, 2025.

Air pollution, responsible for the deaths of 7 million people annually, stands as one of the most significant environmental challenges of our time. Among its components, particulate matter (PM) is a key parameter that demands close monitoring due to its adverse effects on human health and its direct and indirect impacts on climate change. The Eastern Mediterranean region, including Turkey, experiences higher levels of warming compared to other areas at the same latitude, making it one of the most climate-vulnerable regions globally. In this context, addressing air pollution, identifying pollutant levels and sources, and implementing mitigation strategies are essential for combating climate change effectively.

In Turkey, the iron and steel industry contributes approximately 7% of the nation’s total greenhouse gas emissions. Within the framework of the European Green Deal and Border Carbon Adjustment Mechanism, the green transformation of this sector is crucial. However, the specific pollutants released into ambient air from this industry and their impacts on human health remain inadequately addressed, particularly for the province of Karabük, where approximately 4 million tons of iron and steel are produced annually. Developing science-based air quality action plans for Karabük requires a comprehensive understanding of the region’s air pollution levels.

This study analyzed fine (PM2.5) and coarse (PM10-2.5) particulate matter samples collected from an air quality monitoring station located in Safranbolu, a tourist hub in Karabük. The sampling periods spanned from August 7 to September 3, 2021, and from November 9 to December 28, 2021. The samples were analyzed using various analytical techniques to determine major ions, elements, and elemental carbon/organic carbon (EC/OC). The findings revealed the urgent need for targeted air pollution reduction measures in Safranbolu to protect both public health and the region's touristic appeal, while addressing the environmental impact of Turkey's largest iron and steel industry based in Karabük.

This study highlights the critical importance of integrating scientific insights into policy and action to reduce air pollution and foster sustainable development in one of Turkey's most industrialized regions.

How to cite: Güllü, G., Aslanoglu, Y., and Ozturk, F.: Air Quality Assessment in Safranbolu (Karabük): A Critical Step Towards Combating Air Pollution in Turkey's Steel Industry Hub, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20059, https://doi.org/10.5194/egusphere-egu25-20059, 2025.

EGU25-647 | ECS | Posters on site | AS3.2

Chemical Analysis and Source Apportionment of Particulate-Bound Polycyclic Aromatic Hydrocarbons (PAHs) in Northeast India 

Pratibha Vishwakarma, Pradhi Rajeev, and Tarun Gupta

Particulate-bound Polycyclic Aromatic Hydrocarbons (PAHs) are recognized as critical pollutants due to their significant health impacts on both human and animal life. This study analyzed 16 PAHs identified by the United States Environmental Protection Agency (USEPA) in PM2.5 samples collected from Jorhat, India, during the winter months (January to March 2020). Alongside examining the temporal variability of these compounds, the research also evaluated the influence of meteorological factors, including temperature, wind speed, relative humidity, and planetary boundary layer (PBL) height, on PAHs concentrations.
The findings revealed that ambient air temperature and PBL height have a more pronounced effect on PAHs concentrations compared to other meteorological parameters during the winter season. The average total PAH concentration during the study period was 157.2 ± 127.7 ng/m³, with a clear dominance of high molecular weight PAHs over low molecular weight ones. Among the 16 PAHs studied, benzo(b,j)fluoranthene was identified as the most abundant compound, contributing 27.26% to the total PAHs concentration, followed by dibenzo(a,h)anthracene at 10.37%.
Source identification was conducted using isomeric PAHs ratio analysis, which highlighted crop residue burning, vehicular emissions, and coal and wood combustion as the primary sources of PAHs emissions in Jorhat. A comparative analysis with other northern Indian cities revealed that vehicular emissions are a common contributor across all locations. However, there are distinct regional variations in source contributions. For instance, in Kolkata, PAHs emissions are significantly influenced by wood and coal combustion, while biomass burning is a notable contributor in Amritsar. In contrast, the primary sources of PM2.5-bound PAHs in Jorhat are crop residue burning and coal/wood combustion, distinguishing it from the other cities studied.
This research emphasizes the importance of identifying regional emission sources to develop targeted strategies for mitigating PAHs pollution and protecting public health.

How to cite: Vishwakarma, P., Rajeev, P., and Gupta, T.: Chemical Analysis and Source Apportionment of Particulate-Bound Polycyclic Aromatic Hydrocarbons (PAHs) in Northeast India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-647, https://doi.org/10.5194/egusphere-egu25-647, 2025.

EGU25-2486 | Orals | AS3.2

pH, ionic strength and sulfate influence the aqueous nitrate-mediated photooxidation of green leaf volatiles 

Theodora Nah, Yuting Lyu, Taekyu Joo, Ruihan Ma, Mark Kristan Espejo Cebello, Tianye Zhou, Shun Yeung, Cheuk Ki Wong, Yifang Gu, and Yiming Qin

Green leaf volatiles (GLVs) are biogenic C5 to C6 unsaturated oxygenated organic compounds that are emitted when vegetation is exposed to herbivores, pathogens, or harsh weather conditions. Increased GLV emissions when vegetation is subjected to biotic and abiotic stresses can lead to GLVs contributing substantially to the local secondary organic aerosol (SOA). GLVs can dissolve into atmospheric aqueous phases (e.g., aqueous aerosols, cloud and fog droplets), where they can be oxidized by aqueous oxidants. Aqueous SOA (aqSOA) mass yields as high as 88 % from aqueous reactions have been reported in previous studies, but these previous studies were mostly conducted under dilute aqueous conditions mimicking aqueous cloud/fog droplets. Little is currently known about the aqueous oxidation of GLVs under more concentrated aqueous aerosol-like conditions.  Here, we investigated the nitrate-mediated photooxidation of four GLVs, cis-3-hexen-1-ol, trans-2-hexen-1-ol, trans-2-penten-1-ol, and 2-methyl-3-buten-2-ol, focusing on the effects of pH, ionic strength, and sulfate on the reaction kinetics and aqSOA mass yields under cloud/fog-like vs. aqueous aerosol-like conditions. Our results showed that the aqueous reaction medium conditions governed the effects that pH, ionic strength, and sulfate had on the reaction kinetics and aqSOA mass yields. Higher reaction rates were observed at lower pH under dilute cloud/fog-like conditions, which could be attributed to the pH-dependent formation of reactive species from nitrate photolysis. Ionic strength and sulfate had insignificant effects on the reaction rates. In contrast, under concentrated aqueous aerosol-like conditions, higher reaction rates were observed at higher pH, and at higher ionic strength and sulfate concentration. Many of these differences could be attributed to sulfur-containing radicals produced from sulfate photolysis participating in the reactions of GLVs under aqueous aerosol-like conditions, but not in cloud/fog-like conditions. Nevertheless, similar aqSOA mass yield trends were observed for cloud/fog-like and aqueous aerosol-like conditions. Higher aqSOA mass yields were measured, likely due to increased production of oligomers from RO2· and RO· combination reactions as a result of the higher concentrations of GLVs reacted. Higher aqSOA mass yields were measured at lower pH, likely a result of increased production of low volatility products from acid-catalyzed reactions. Lower aqSOA mass yields were measured at higher ionic strength and sulfate concentration, likely due to the increased importance of fragmentation pathways in the reactions of GLVs with sulfur-containing radicals formed from sulfate photolysis. These results provide new insights that can be used in modeling studies of the atmospheric fates of GLVs and their contributions to the SOA budget.

How to cite: Nah, T., Lyu, Y., Joo, T., Ma, R., Cebello, M. K. E., Zhou, T., Yeung, S., Wong, C. K., Gu, Y., and Qin, Y.: pH, ionic strength and sulfate influence the aqueous nitrate-mediated photooxidation of green leaf volatiles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2486, https://doi.org/10.5194/egusphere-egu25-2486, 2025.

EGU25-2587 | ECS | Posters on site | AS3.2

Revisiting the global atmospheric glyoxal budget: updates in secondary production pathways and evaluations against satellite observations 

Aoxing Zhang, Tzung-May Fu, Yuhang Wang, Enyu Xiong, and Yumin Li

Glyoxal (CHOCHO) serves as a critical marker for the oxidation capacities of volatile organic compounds (VOCs) and acts as a precursor to secondary organic aerosols. Nonetheless, the sources and chemical reaction pathways of glyoxal have not been updated, which results in global simulations underestimating the observed concentrations of glyoxal. We have enhanced the representation of glyoxal sources and sinks through laboratory experiments, a comprehensive MCM chemical scheme, and diverse observational data. Within the GEOS-Chem chemical transport model, the revised glyoxal parameterizations reduced the model's underestimation from 80% (72%~85%) to 17% (5%~32%), compared with TROPOMI satellite retrievals. This advancement is attributed to the increased glyoxal yield from isoprene photooxidation (from 5% to 15%) and the incorporation of a glyoxal source over the marine boundary layer (78 Tg/yr). Following the inclusion of the marine source, the global burden of glyoxal augmented by a factor of 1.4, signifying enhanced oxidation over the remote ocean. This investigation elucidates an improved global budget of glyoxal, underscoring the necessity to refine the photochemical processes of biogenic OVOCs and to address the oxidation states of OVOCs in remote oceanic regions.

How to cite: Zhang, A., Fu, T.-M., Wang, Y., Xiong, E., and Li, Y.: Revisiting the global atmospheric glyoxal budget: updates in secondary production pathways and evaluations against satellite observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2587, https://doi.org/10.5194/egusphere-egu25-2587, 2025.

EGU25-2702 | ECS | Orals | AS3.2

Long-term Observations of Volatile Organic Compounds at a Regional Background Site in the Eastern Mediterranean Affected by Middle Eastern Air Masses  

Anchal Garg, Maximilien Desservettaz, Aliki Christodoulou, Theodoros Christoudias, Vijay Punjaji Kanawade, Tujia Jokinen, Jean Sciare, and Efstratios Bourtsoukidis

Volatile Organic Compounds (VOCs) play a key role in the formation of tropospheric ozone and secondary aerosols, influencing air quality, climate, and human health. Originating from both biogenic and anthropogenic sources, their volatile nature enables long-range transport, with oxidation products impacting distant regions. The island of Cyprus, located at the intersection of Europe, Asia, and Africa, experiences complex air mass dynamics that transport diverse VOC emissions and their oxidation products, making it a key site for studying regional air quality. However, VOC observations in the Eastern Mediterranean and Middle East region (EMME) are often constrained by the short duration of measurement campaigns and a narrow focus on specific species, resulting in a significant data gap. In this study, we employed a Proton Transfer Reaction–Time-of-Flight Mass Spectrometer (PTR-ToF-MS 4000; Ionicon Analytik, Austria) to perform continuous, high-resolution measurements of VOCs from April 2022 to June 2024 at the Cyprus Atmospheric Observatory (CAO-AMX; 35.038692° N, 33.057850° E; 532 m above mean sea level). This site represents regional background concentrations while providing valuable insights into local emission sources, including significant contributions of biogenic emissions originating from the Troodos mountain forest. We analyzed over 70 VOC species, classifying them into chemical groups such as aromatics, alcohols, aldehydes, ketones, and oxygenated VOCs. By examining their distinct seasonal and diurnal variations along with the origins of the sampled air masses, we derive valuable information about their regional and local emission dynamics and their respective impact on atmospheric chemistry. Additionally, we compared the measured VOC mixing ratios with simulations from a coupled atmospheric chemistry model (WRF-Chem) to comprehensively evaluate the model’s performance and its ability to reproduce the observed VOC variability. We find that while regional biogenic sources are reasonably well captured by the simulations, significant discrepancies for oxygenated VOCs suggest the presence of uncharacterized VOC sources in the Middle East. This work offers a unique, long-term perspective on the role of VOCs in shaping air quality in the EMME region, supporting efforts to mitigate air pollution and address climate change impacts. 

How to cite: Garg, A., Desservettaz, M., Christodoulou, A., Christoudias, T., Kanawade, V. P., Jokinen, T., Sciare, J., and Bourtsoukidis, E.: Long-term Observations of Volatile Organic Compounds at a Regional Background Site in the Eastern Mediterranean Affected by Middle Eastern Air Masses , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2702, https://doi.org/10.5194/egusphere-egu25-2702, 2025.

EGU25-3072 | Posters on site | AS3.2

Anthropogenic influence on terpene concentrations in urban air in Helsinki, Finland: Insights from wintertime measurements 

Heidi Hellén, Toni Tykkä, Elli Suhonen, Jarkko Niemi, Topi Rönkkö, Hilkka Timonen, and Arnaud Praplan

Recent studies suggest significant anthropogenic contributions to terpene concentrations in urban air. However, differentiating between biogenic and anthropogenic sources is not clear.  In this study, we measured terpenes in a street canyon in Helsinki during cold winter months (mean temperature < 0 °C), when biogenic emissions were expected to be negligible. Monoterpenes were detected at mean concentrations of approximately 200 ng/m³, which is over ten times lower than the mixing ratios of aromatic hydrocarbons. Despite their lower abundance, monoterpenes contributed significantly to local atmospheric chemistry due to their high reactivity with hydroxyl radicals, nitrate radicals, and ozone. This reactivity, coupled with their high secondary organic aerosol (SOA) formation potential, highlights the important role of anthropogenic terpene emissions in SOA formation and urban air quality.

How to cite: Hellén, H., Tykkä, T., Suhonen, E., Niemi, J., Rönkkö, T., Timonen, H., and Praplan, A.: Anthropogenic influence on terpene concentrations in urban air in Helsinki, Finland: Insights from wintertime measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3072, https://doi.org/10.5194/egusphere-egu25-3072, 2025.

EGU25-3522 | ECS | Orals | AS3.2

An Urban Emission Inventory Approach for Source Specific Atmospheric Chamber Studies 

Yizhen Wu and the SAPHIR-CHANEL Campaign team

Urban pollution poses one of the largest threats to human health worldwide. A significant portion of this pollution is secondary, formed through atmospheric chemical reactions of emitted trace gases, with secondary organic aerosol (SOA) and ozone (O₃) being major contributors to health impacts in urban areas. While decades of air quality regulations have significantly reduced motor vehicle emissions of organic compounds that are precursors to secondary pollution, recent focus has shifted to understudied urban sources such as volatile chemical products (VCPs) and cooking emissions. These sources are complicated and challenging to replicate in chamber experiments, which typically focus on single-compound scenarios, thus limiting their comparability to real-world urban environments.

In this study, we utilized emission inventories and developed an approach to reduce the number of compounds that represent each urban source, including VCPs, gasoline, diesel, and cooking, by generating chemical fingerprints representing 80% of the overall reactivity and SOA formation potential of each urban source. These fingerprint solutions were then injected into the atmospheric simulation chamber SAPHIR to explore their potential for SOA and O₃ formation. We conducted experiments simulating each source at various NOx exposures, as well as mixed systems to simulate the urban atmosphere of US and European cities. Finally, we contextualize our findings by comparing them with data from the Atmospheric Emissions and Reactions Observed from Megacities to Marine Areas (AEROMMA) mission, offering insights into the dynamics of urban air pollution.

How to cite: Wu, Y. and the SAPHIR-CHANEL Campaign team: An Urban Emission Inventory Approach for Source Specific Atmospheric Chamber Studies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3522, https://doi.org/10.5194/egusphere-egu25-3522, 2025.

EGU25-3769 | Orals | AS3.2

Monoterpene and sesquiterpene emissions increase with forest degradation and land use change in the Amazon Arc of Deforestation 

Eliane Gomes Alves, Michelle Robin, Leonardo Maracahipes-Santos, Tyeen Taylor, Ana Paula Faggiani, Antônio Carlos Silveiro da Silva, Darlisson Nunes da Costa, Nadav Bendavid, Paulo Brando, Jonathan Williams, Joseph Byron, Johanna Schüttler, and Christoph Hartmann

Biogenic Volatile Organic Compounds (BVOCs) are primarily emitted into the atmosphere by plants. These compounds serve various functions, including cellular protection and defense at the leaf level, chemical signaling between and within plants, and regulation of large-scale biogeochemical processes, such as influencing atmospheric chemistry and contributing to aerosol formation. The Amazon Forest is the major source of BVOCs to the global atmosphere.  Over the past four decades, multiple studies have measured BVOC concentrations in the air, mainly focusing on central Amazonia. However, while there is much to be investigated in undisturbed forests, the Amazon is already undergoing changes in land use and climate, particularly in the Amazon Arc of Deforestation. These changes may affect BVOC emissions and associated processes at the biosphere-atmosphere interface in ways that are not yet fully understood. In this light, this study aimed to identify and quantify the main BVOCs emitted by trees and crops in a changing Amazon region. We measured the above-canopy BVOC concentrations and leaf-level BVOC emissions from crops (cotton and corn) and dominant tree species in a mosaic of disturbed forest fragments and agricultural fields in southeastern Amazonia during the wet and dry seasons of 2023. Surprisingly, our results revealed that monoterpene and sesquiterpene emissions were higher than isoprene emissions for most trees and crops. When we compared the same tree species across a gradient of forest degradation, we found that monoterpene and sesquiterpene emissions were up to three times higher in the most degraded forest areas. Furthermore, with a leaf temperature curve experiment, we observed that at 45°C, the amount of recently assimilated carbon emitted in the form of isoprene, monoterpenes, and sesquiterpenes were up to 35%, 5%, and 23%, respectively - suggesting that plants were losing a high amount of carbon to cope with the heat stress. In contrast to leaf-level measurements, our ambient air measurements indicated that monoterpene and sesquiterpene concentrations were significantly lower than isoprene concentrations during both the wet and dry seasons, indicating that the atmosphere in this region is very reactive and that only leaf-level measurements are likely to give us a true measure of monoterpene and sesquiterpene emissions. Yet, interestingly, sesquiterpene concentrations were higher in the dry season than in the wet season, supporting the leaf-level results showing that increased heat and drought may lead to higher emissions of sesquiterpenes. This may have occurred either because plants emit more monoterpenes and sesquiterpenes in response to stress or due to changes in plant species composition resulting from forest degradation and land use changes. This study presents the first observations of BVOCs conducted in the Amazon Arc of Deforestation at both the leaf and canopy levels. The observed shift in emissions towards monoterpenes and sesquiterpenes is likely modifying atmospheric chemical and physical processes and the carbon balance in this already changing Amazon region. This makes it crucial to include these changes in air quality and Earth system modeling. 

How to cite: Gomes Alves, E., Robin, M., Maracahipes-Santos, L., Taylor, T., Faggiani, A. P., Silveiro da Silva, A. C., Nunes da Costa, D., Bendavid, N., Brando, P., Williams, J., Byron, J., Schüttler, J., and Hartmann, C.: Monoterpene and sesquiterpene emissions increase with forest degradation and land use change in the Amazon Arc of Deforestation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3769, https://doi.org/10.5194/egusphere-egu25-3769, 2025.

EGU25-4097 | ECS | Posters on site | AS3.2

The Air Quality Impacts of the Bio-Based Solvent Cyrene 

James D'Souza Metcalf, Ruth Winkless, Claudiu Roman, Salome Raymond, Cecilia Arsene, Romeo Olariu, James Sherwood, Iustinian Bejan, and Terry Dillon

Solvents have long been recognized as one of the principal sources of waste from the chemical industry, particularly from fine chemical manufacturing.1,2 While neoteric solvents with minimal atmospheric impact such as supercritical fluids and ionic liquids show promise for some applications, most processes remain dependent on organic solvents. As a result, the last two decades have seen a rapid increase in the development and deployment of bio-derived and biodegradable “green” solvents.3 Design processes for such solvents pay close attention to solvent performance, human and environmental toxicity, and process-scale safety, however the impact of new “green” solvents on the chemistry of the atmosphere remains largely unexplored. As increasingly strict  regulation brings traditional sources of VOC emissions under control solvents have emerged as the largest anthropogenic source of non-methane VOCs.4 It is therefore crucial that we expand our understanding of the atmospheric ramifications of this growing and diversifying class of emissions.

This work is a collaboration between green materials chemists and atmospheric scientists. Our interdisciplinary approach to solvent selection and development involves rigorous experimental and in silico testing of both solvent performance and environmental impact as VOCs. Herin we will discuss the atmospheric chemistry of the bio-derived solvent Cyrene (dihydrolevoglucosenone, C6H8O3). Our investigation into this unique, bicyclic multifunctional oxygenate covers its two primary atmospheric breakdown routes. Chamber experiments to determine OH kinetics and aerosol yields, quasi-gas-phase measurement of UV cross sections and fast flow investigations into photolysis quantum yields. Results will be presented in the context of Structure-Activity Relationship (SAR) calculations and other predictive tools, with impacts assessed via estimations of atmospheric lifetime and photochemical ozone creation potential. 

The chamber experiments carried out as part of this work are part of a Transnational access project that is supported by the European Commission under the Horizon 2020 – Research and Innovation Framework Programme, H2020-INFRAIA-2020-1, ATMO-ACCESS Grant Agreement number: 101008004

(1)          Constable, D. J. C.; Dunn, P. J.; Hayler, J. D.; Humphrey, G. R.; Leazer, Jr., J. L.; Linderman, R. J.; Lorenz, K.; Manley, J.; Pearlman, B. A.; Wells, A.; Zaks, A.; Zhang, T. Y. Key Green Chemistry Research Areas—a Perspective from Pharmaceutical Manufacturers. Green Chem 2007, 9 (5), 411–420. https://doi.org/10.1039/B703488C.

(2)          Bryan, M. C.; Dunn, P. J.; Entwistle, D.; Gallou, F.; Koenig, S. G.; Hayler, J. D.; Hickey, M. R.; Hughes, S.; Kopach, M. E.; Moine, G.; Richardson, P.; Roschangar, F.; Steven, A.; Weiberth, F. J. Key Green Chemistry Research Areas from a Pharmaceutical Manufacturers’ Perspective Revisited. Green Chem. 2018, 20 (22), 5082–5103. https://doi.org/10.1039/C8GC01276H.

(3)          Jordan, A.; Hall, C. G. J.; Thorp, L. R.; Sneddon, H. F. Replacement of Less-Preferred Dipolar Aprotic and Ethereal Solvents in Synthetic Organic Chemistry with More Sustainable Alternatives. Chem. Rev. 2022, 122 (6), 6749–6794. https://doi.org/10.1021/acs.chemrev.1c00672.

(4)          Lewis, A. C.; Hopkins, J. R.; Carslaw, D. C.; Hamilton, J. F.; Nelson, B. S.; Stewart, G.; Dernie, J.; Passant, N.; Murrells, T. An Increasing Role for Solvent Emissions and Implications for Future Measurements of Volatile Organic Compounds. Philos. Trans. R. Soc. Math. Phys. Eng. Sci. 2020, 378 (2183), 20190328. https://doi.org/10.1098/rsta.2019.0328.

How to cite: D'Souza Metcalf, J., Winkless, R., Roman, C., Raymond, S., Arsene, C., Olariu, R., Sherwood, J., Bejan, I., and Dillon, T.: The Air Quality Impacts of the Bio-Based Solvent Cyrene, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4097, https://doi.org/10.5194/egusphere-egu25-4097, 2025.

EGU25-4126 | ECS | Posters on site | AS3.2

Improved isoprene emission estimates from MEGAN and comprehensive modeling of BVOCs driven aerosol dynamics in the Boreal forests 

Manuel Bettineschi, Giancarlo Ciarelli, Arineh Cholakian, and Federico Bianchi

Accurate representation of biogenic volatile organic compound (BVOC) emissions is critical for understanding their role in atmospheric chemistry and secondary organic aerosol (SOA) formation. In this study, we present an improved framework for modeling biogenic emissions, using the latest version of the Model of Emissions of Gases and Aerosols from Nature (MEGAN). We used domain-specific tree cover data, species distributions (retrieved from the Natural Resources Institute Finland website), and species-specific emission factors, and we recalculated isoprene emission factors tailored to the Finnish boreal region. These modifications were implemented in MEGAN and integrated into the WRF-CHIMERE chemistry transport model, enabling a more accurate simulation of biogenic emissions. We perform simulations over the summer period for the year 2017, 2018, and 2019.

These simulations reveal a significant reduction in bias for both isoprene emissions as well as concentrations when compared to observations at the Hyytiälä and Pallas stations. Additionally, we introduced a detailed canopy correction (sensitivity simulation) to account for the effects of forest canopy on the vertical and horizontal transport of BVOCs. These adjustments additionally reduced the bias in modeled isoprene concentrations when compared to observations. 

The enhanced representation of BVOC emissions and the effects of canopy on dispersion resulted in improvements in the modeled dynamics of SOA formation and transportation, emphasizing the importance of ecosystem-specific modifications in emission models and the inclusion of forest canopy correction in chemical transport models.

Our findings show that the vanilla versions of MEGAN version 3.2 without modification is insufficient to accurately represent isoprene emissions, at least in the European boreal forest ecosystem. High-resolution, domain-specific vegetation data are essential to capture the variability in tree cover, species distribution, and emission factors, ensuring the reliability of modeled biogenic emissions and their impacts on atmospheric chemistry.

How to cite: Bettineschi, M., Ciarelli, G., Cholakian, A., and Bianchi, F.: Improved isoprene emission estimates from MEGAN and comprehensive modeling of BVOCs driven aerosol dynamics in the Boreal forests, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4126, https://doi.org/10.5194/egusphere-egu25-4126, 2025.

EGU25-5154 | ECS | Posters on site | AS3.2

Modelling taxonomic biodiversity driven effects on regional air quality using the new chemical mechanism URMELL 

Marie Luttkus, Erik Hoffmann, Andreas Tilgner, Ina Tegen, Hartmut Herrmann, and Ralf Wolke

Air quality is a globally pressing issue as it poses a major threat for human health and ecosystems. Non-methane volatile organic compounds (NMVOCs) are highly reactive substances and known for their impact on the HOx (OH + HO2) and NOx (NO + NO2) budget. Important air pollutants such as ozone and particulate matter (PM) in terms of secondary organic aerosols (SOA) result from the chemical oxidation of NMVOCs. NMVOCs comprise a variety of anthropogenic and biogenic compounds with highly complex and interwoven interrelations. Therefore, it is key to capture these interdependencies for any air quality model assessment. Here we emphasize the importance of considering taxonomic biodiversity for regional air quality modeling by integrating the most common European tree species (116 tree classes) into the model framework COSMO-MUSCAT. This has major impacts on modeled biogenic NMVOC emissions and the tropospheric oxidizing capacity which is also impacting the chemical degradation of anthropogenic VOCs. To entangle these complex interdependencies the new chemical mechanism URMELL (short for: Urban and Remote cheMistry modELLing) was developed. URMELL comprises an extended chemical treatment of major anthropogenic (e.g. aromatics) and biogenic (e.g. isoprene) NMVOCs. By maintaining reaction products with multiple functional groups as possible SOA precursors, URMELL enables a direct and explicit SOA approach and considers HOx/NOx regime shifts creating a multitude of individual SOA species. URMELL simulates higher contributions of non- and lower volatile isoprene and aromatic products. Unexpected high concentrations of non-volatile aromatic SOA products are reached in remote spruce forests, away from the emission sources.

How to cite: Luttkus, M., Hoffmann, E., Tilgner, A., Tegen, I., Herrmann, H., and Wolke, R.: Modelling taxonomic biodiversity driven effects on regional air quality using the new chemical mechanism URMELL, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5154, https://doi.org/10.5194/egusphere-egu25-5154, 2025.

EGU25-6459 | ECS | Posters on site | AS3.2

Air Quality Impact of a “Green” Solvent – Ethyl Lactate  

Salome Usakuhyel Raymond, James D'Souza Metcalf, Claudiu Roman, Cecilia Arsene, Romeo Olariu, Helen Sneddon, Iustinian Bejan, and Terry Dillon

Organic solvents play an important role in industry,  but as the world progresses towards net-zero, their synthesis and end-of-life have become critical areas of research. Most traditional solvents are toxic, petrochemically derived and contribute significantly to chemical waste. Additionally, they have significant impact on air quality because of their role as volatile organic compounds (VOCs), able to fuel atmospheric cycles that generate ozone (O3) and other harmful gases.1 While VOC emissions from many sectors are decreasing, emissions from solvents are on the rise.2 Notable research efforts focus on developing “green” solvents that are sustainable, renewable, and less toxic but little is known about their air impact.

This research focuses on a promising solvent, ethyl lactate, a bioderived ester from glucose, relevant in various industries. The work addresses the air quality research gap by studying its atmospheric behaviour including its lifetime, photochemical ozone creation potential, and gas-phase breakdown routes.

To achieve these objectives, this work employs methods such as Pulsed Laser Photolysis–Laser Induced Fluorescence for direct OH decay kinetics, UV-vis. spectroscopy for absorption cross-sections and calculating photolysis rate coefficients, and relative rate OH kinetics experiments carried out at an Atmospheric Simulation Chamber (ESC-Q-UAIC facility, CERNESIM centre, Romania).

Relative rate kinetic studies in the atmospheric chamber estimated the kOH(296K)for ethyl lactate as (2.8 ± 0.5) x 10-12 cm3 molecule−1 s−1. Using a mean tropospheric [OH]3, the lifetime with respect to OH was estimated to be 4 days. Other preliminary experiments have revealed small UV absorption cross-sections (310 – 350 nm). Further investigations are ongoing to refine and improve on these results and so determine air quality impacts.

Keywords: green, volatile organic compound emissions, air quality impact

The atmospheric chamber results presented in this work is part of a Transnational access project that is supported by the European Commission under the Horizon 2020 – Research and Innovation Framework Programme, H2020-INFRAIA-2020-1, ATMO-ACCESS Grant Agreement number: 101008004.

References

1            M. E. Jenkin, R. Valorso, B. Aumont, A. R. Rickard and T. J. Wallington, Atmos. Chem. Phys., 2018, 18, 9297–9328.

2            A. C. Lewis, J. R. Hopkins, D. C. Carslaw, J. F. Hamilton, B. S. Nelson, G. Stewart, J. Dernie, N. Passant and T. Murrells, Philos Trans A Math Phys Eng Sci, 2020, 378, 20190328.

3            J. Lelieveld, S. Gromov, A. Pozzer and D. Taraborrelli, Atmospheric Chemistry and Physics, 2016, 16, 12477–12493.

How to cite: Raymond, S. U., D'Souza Metcalf, J., Roman, C., Arsene, C., Olariu, R., Sneddon, H., Bejan, I., and Dillon, T.: Air Quality Impact of a “Green” Solvent – Ethyl Lactate , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6459, https://doi.org/10.5194/egusphere-egu25-6459, 2025.

EGU25-7373 | ECS | Posters on site | AS3.2

Cloud-Aerosol Chemistry Observations at Whiteface Mountain: Organic Acids and the Growing Importance of Ammonium 

Archana Tripathy, Christopher Lawrence, Sara Lombardo, Paul Casson, Rudra Patel, Lily Hammond, Kathleen DeMarle, Richard Brandt, Scott McKim, James Schlemmer, James Schwab, Haider Khwaja, Mirza Hussain, Liz Yerger, Phil Snyder, Dan Kelting, William May, and Sara Lance

Organic compounds are vital to atmospheric chemistry, with clouds playing a key role in their formation and transformation. Di-carboxylic organic anions, such as oxalate, act as tracers for aqueous-phase chemical processes. This study presents summer measurements of three organic acids (formic, acetic, oxalic), inorganic anions, and cations in cloud water, aerosol, and cloud droplet residual samples obtained 2018-2024 from the summit of Whiteface Mountain (WFM), a forested site in the Adirondack Mountains of northern New York State. Contributions of these acids to dissolved organic carbon (DOC), ion balance, and acidity are assessed in both cloud and aerosol samples. The current study builds on prior studies linking oxalate-to-DOC ratios with ozone concentrations, from which inferences have been made about biogenic volatile organic carbon (BVOC) contributions to secondary organic aerosol (SOA) formation, and we present new insights based on comparisons between cloud water and aerosol phases. We further expand upon the findings of Lawrence et al. (2023), which showed that more than half of the cloud water samples at WFM exhibit excess ammonium (i.e. exceeding sulfate plus nitrate concentrations) in recent years, by evaluating the relationship between excess ammonium and organic acids in both the cloud and aerosol phases.  These findings provide new insights into multi-phase chemistry and SOA formation processes at a remote forested site downwind of many natural and anthropogenic sources, and a site frequently influenced by wildfire smoke.

How to cite: Tripathy, A., Lawrence, C., Lombardo, S., Casson, P., Patel, R., Hammond, L., DeMarle, K., Brandt, R., McKim, S., Schlemmer, J., Schwab, J., Khwaja, H., Hussain, M., Yerger, L., Snyder, P., Kelting, D., May, W., and Lance, S.: Cloud-Aerosol Chemistry Observations at Whiteface Mountain: Organic Acids and the Growing Importance of Ammonium, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7373, https://doi.org/10.5194/egusphere-egu25-7373, 2025.

EGU25-8208 | Posters on site | AS3.2

VOC fluxes of a subarctic mountain birch forest 

Albert Egea Guevara, Thomas Holst, Cleo L. Davie-Martin, Jolanta Rieksta, Amy Smart, Riikka Rinnan, and Roger Seco

Biogenic volatile organic compounds (BVOCs) play a significant role in the interactions between the biosphere and the atmosphere, but their impact in northern latitudes is difficult to quantify due to a lack of measurements and modeling studies.

We present here the findings from our latest field campaigns in a mountain birch forest near Abisko (Northern Sweden), where we used Proton Transfer Reaction–Time of Flight–Mass Spectrometry (PTR–TOF–MS) and the Eddy Covariance technique to measure the ecosystem-scale fluxes of BVOCs during 3 growing seasons (2021, 2022, and 2023), to understand the diel cycle of these emissions. Furthermore, our study aims to observe and model the impact of herbivore insect defoliation on the gas exchange of the forest, caused by a caterpillar outbreak during our 2023 campaign.

How to cite: Egea Guevara, A., Holst, T., Davie-Martin, C. L., Rieksta, J., Smart, A., Rinnan, R., and Seco, R.: VOC fluxes of a subarctic mountain birch forest, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8208, https://doi.org/10.5194/egusphere-egu25-8208, 2025.

EGU25-8957 | ECS | Orals | AS3.2

Uronium CIMS: Robust high-pressure positive mode ion attachment chemical ionization mass spectrometry via X-ray-assisted sublimation of urea 

Henning Finkenzeller, Aleksei Shcherbinin, Netta Vinkvist, Hans-Jürg Jost, Fariba Partovi, Jyri Mikkilä, Jussi Kontro, Nina Sarnela, Juha Kangasluoma, and Matti Rissanen

The chemical diversity in the varied spectrum of atmospheric trace gases requires to combine different ionization approaches to enable comprehensive mass spectrometric analysis. Ion-molecule reactors (IMR) at high pressure generally enable better detection limits, due to a larger reaction time, but are also more prone to matrix effects (e.g., dependency on humidity). For the ionization of low polarity volatile organic compounds (VOCs), positive mode chemical ionization (e.g. PTR, low IMR pressure) has been found to be more suitable than negative mode ionization (e.g., NO3-, I-, Br-), but humidity dependency and other matrix effects of unselective reagent ions need to be constrained e.g. by reduction of IMR pressure. More selective reagent ions such as ammonium and aminium have been previously proposed for more sensitive and soft ionization. However, they are reactive, toxic, and difficult to control.

Inspired by these challenges, we demonstrate uronium as an efficient and robust reagent cation for the ionization of VOCs at high IMR pressures. Urea, a solid chemical safe to humans with a negligible vapor pressure under normal circumstances, is sublimated from the solid phase under x-ray irradiation, which also subsequently forms the uronium ion. We determine the calibration factors for VOCs, amines, and DMSO under different humidities in calibration experiments, interpret the ionization efficiencies using theory, and show results of test measurements of different chemical systems. Beyond the favorable sensitivities allowing detection at the low ppq level - attainable due to uronium’s applicability at high IMR pressure and a tendency to form remarkably strongly bound ion-molecule clusters – and low susceptibility to humidity changes, the marked benefit of uronium CIMS lies in the trivial handling of the reagent supply and long-term stability of the ion production system. The combination of favorable performance and easy handling render uronium CIMS promising to become a go-to method for ultra-sensitive positive mode chemical ionization.

How to cite: Finkenzeller, H., Shcherbinin, A., Vinkvist, N., Jost, H.-J., Partovi, F., Mikkilä, J., Kontro, J., Sarnela, N., Kangasluoma, J., and Rissanen, M.: Uronium CIMS: Robust high-pressure positive mode ion attachment chemical ionization mass spectrometry via X-ray-assisted sublimation of urea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8957, https://doi.org/10.5194/egusphere-egu25-8957, 2025.

EGU25-8986 | Orals | AS3.2

Beyond constitutive plant BVOCs: modelling emissions from litter, permafrost soil, forest management and stress disturbance 

Jing Tang, Twan van Noije, Zhenqian Wang, Paul A. Miller, Zhanzhuo Chen, John Bergkvist, Ross Petersen, and Riikka Rinnan

Earth system models have incrementally integrated the climate effects of biogenic volatile organic compounds (BVOCs). Currently, the global estimate stands at less than 1 PgC/year, considering only the emissions from actively growing plants while neglecting other sources of BVOCs and emissions from plants under stress.

Based on process understanding from various empirical data, this study extends beyond modelling plant BVOCs to include BVOC emissions from multiple ecosystem components, including litterfall, soil, forest management, and stress disturbance, into the dynamic vegetation model LPJ-GUESS. We will present four case studies in which these emissions are accounted for and compared with leaf constitutive emissions, highlighting their dynamic contributions to the ecosystem's total BVOC budget.

Furthermore, LPJ-GUESS previously simulated only isoprene and monoterpene emissions from plants, and this study further extends the model to consider all major BVOC compound groups (with a total of 150 compound species specified). We have dynamically coupled the LPJ-GUESS modelled BVOC emissions into the atmospheric chemistry and transport module TM5 within the European Earth System Model EC-Earth to assess the atmospheric impacts. We will also showcase the modelled impacts of BVOC emissions on atmospheric variables based on the coupled EC-Earth runs. The modelling framework provides an essential tool for integrating various ecosystem processes to understand BVOC emission dynamics and further assess the associated climate impact mechanically.

How to cite: Tang, J., van Noije, T., Wang, Z., Miller, P. A., Chen, Z., Bergkvist, J., Petersen, R., and Rinnan, R.: Beyond constitutive plant BVOCs: modelling emissions from litter, permafrost soil, forest management and stress disturbance, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8986, https://doi.org/10.5194/egusphere-egu25-8986, 2025.

EGU25-9422 | ECS | Orals | AS3.2

Insight from VOC flux measurements on managing air quality in cities 

Xianjun He, Bin Yuan, Yibo Huangfu, Sihang Wang, Xiaoxiao Zhang, and Thomas Karl

Managing ozone remains one of the most pressing and significant environmental challenges across megacities. Numerous studies suggest that biogenic emissions of volatile organic compounds (VOCs) play a key role in ozone formation in urban areas, yet direct evidence remains limited due to the complexity of the sources, sinks, and chemistry of biogenic VOCs. In the summer of 2021, we conducted VOC flux measurements in Beijing, a megacity in China, using the eddy covariance technique. We analyzed VOC flux data using positive matrix factorization allowing to identify prominent urban VOCs emission sources. Our findings highlight the decreasing importance of vehicle-related emissions for VOCs, while the demand for eliminating emissions from volatile chemical products has been increasing. Meanwhile, we discovered that more than half of the OH reactivity of the VOC flux originates from urban vegetation, underscoring the often-overlooked role of urban forests in air pollution. Surprisingly, the strong influence of biogenic emissions in Beijing largely governs the temperature dependence of ozone concentrations, aligning with the OH reactivity from VOC flux. This leads to ozone pollution episodes predominantly occurring on high-temperature days, when biogenic emissions, particularly isoprene, are substantially enhanced. Our study calls for a greater attention from air quality managers to the regulation of emissions from urban vegetation.

How to cite: He, X., Yuan, B., Huangfu, Y., Wang, S., Zhang, X., and Karl, T.: Insight from VOC flux measurements on managing air quality in cities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9422, https://doi.org/10.5194/egusphere-egu25-9422, 2025.

EGU25-9860 | Orals | AS3.2

VOCentinel - a novel solution for automated real-time monitoring of atmospheric VOCs 

Markus Müller, Klaus Winkler, Andreas Herburger, Martin Graus, and Jens Herbig

Volatile Organic Compounds (VOCs), emitted by both biogenic and anthropogenic sources, play a crucial role in atmospheric processes and significantly affect air quality. Despite their importance, routine monitoring of VOCs poses challenges due to limitations in time-resolution, labor intensity, long-term stability, and compound-specific identification capabilities. Proton-transfer-reaction mass-spectrometry (PTR-MS) is widely used for detecting VOCs with high time-resolution and stability. However, as a soft chemical ionization method, it primarily identifies chemical compositions rather than specific compounds. Acquiring additional chemical information through alternative ionization methods remains labor-intensive, making it impractical for long-term VOC monitoring.

Here, we introduce an innovative solution to streamline these time-consuming tasks with the push of a button for key atmospheric VOCs. This new VOC monitor “VOCentinel” leverages Selective-Reagent-Ion (SRI) PTR-MS combined with Automatic Measurement and Evaluation (AME), integrating recent technological advancements in PTR-MS, such as fast switching of reagent ions, extended volatility range (EVR) surface treatment, active humidity control, and automatic pattern matching, alongside IONICON's extensive experience in robust industrial monitoring. Essentially, five ionization modes sequentially ionize specific atmospheric VOCs within one minute, and the resulting mass spectra are immediately analyzed for chemical composition using a pattern matching algorithm. Automatic quality control ensures optimal instrument performance.

We will present a comprehensive characterization of the VOCentinel, emphasizing its long-term stability, and share initial results from VOC measurements in Innsbruck, Austria. Using isoprene as an example - an important biogenically emitted VOC often subject to chemical interferences in PTR-MS measurements - we demonstrate the system’s ability to automatically measure, evaluate, and correctly quantify compounds with isobaric and/or isomeric interferences.

How to cite: Müller, M., Winkler, K., Herburger, A., Graus, M., and Herbig, J.: VOCentinel - a novel solution for automated real-time monitoring of atmospheric VOCs, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9860, https://doi.org/10.5194/egusphere-egu25-9860, 2025.

EGU25-10238 | ECS | Posters on site | AS3.2

Underestimated Formaldehyde Emission from Residential Coal Combustion in North China 

Min Zhao, Lin Li, Hengqing Shen, and Likun Xue

Atmospheric formaldehyde (HCHO) plays a critical role in atmospheric radical budgets and secondary formation of ozone and particulate matter. However, HCHO is known to be significantly underestimated by regional air quality models, which indicates an incomplete understanding of HCHO origins and limits our comprehension of its atmospheric roles and implications. In this study, we revealed that direct emissions of HCHO from wintertime residential coal combustion in north China has been significantly underestimated in current emission inventories, based on field measurements. We observed high values of HCHO (up to 9.4 ppbv) at a typical rural site in Qingdao, north China, which exhibited a diurnal variation pattern with a double-peak distribution in the morning and late afternoon. During the morning peak period, HCHO showed a stronger correlation with SO2 and NO, while HCHO strongly correlated with CO, NO2 and biomass burning indicators (levoglucosan, K+, Cl-) during the late afternoon peak period. The diurnal variation of HCHO aligns well with the combustion activities of residents, which are dominated by coal combustion in the morning and biomass burning in the evening, implying the potentially significant contributions of residential combustion emissions to ambient HCHO. We then conducted source apportionment using the Positive Matrix Factorization (PMF) method and confirmed the significant contributions of residential biomass burning and residential coal combustion to observed HCHO. Using the Minimum R Squared (MRS) method, we further calculated the HCHO emission ratios from the two combustion-related sources. We further calculated HCHO emission from residential combustion sectors in widely used emission inventories, such as EDGER, MEIC, MIX and REAS. However, HCHO emissions from residential combustion sectors exhibit large discrepancies among these emission inventories, with the maximum estimate provided by MEIC and the minimum estimate by EDGAR. When we calculated HCHO emissions from residential coal combustion sector and residential biomass burning sector separately, HCHO emissions from residential biomass burning sector were well estimated, while HCHO emissions from residential coal combustion sector were significantly underestimated by an order of magnitude. Using current emission inventory, HCHO was significantly underestimated by CMAQ modeling compared with field measurements. After updating the HCHO emissions from residential coal combustion based on field results, modeled HCHO concentrations significantly increased (over 100%), which further enhanced the atmospheric oxidation capacity and secondary organic formation. Our findings highlight the necessity to revisiting the HCHO emission from residential coal combustion sector in current emission inventory, especially in north China.

How to cite: Zhao, M., Li, L., Shen, H., and Xue, L.: Underestimated Formaldehyde Emission from Residential Coal Combustion in North China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10238, https://doi.org/10.5194/egusphere-egu25-10238, 2025.

EGU25-10519 | ECS | Posters on site | AS3.2

Gas-phase Experiments on the Reactivity and Fate of Short-Chain Fatty Acid Ethyl Ester Derivatives 

Finja Löher, Nicola Carslaw, and Terry J Dillon

Fatty acid ethyl esters (FAEEs) are a class of aroma chemicals that occur naturally in numerous plants and are known for their fruity odour. They are commonly added to food items, cosmetics, scented air fresheners, and cleaners to provide flavour or fragrance, to enhance sweetness perception, or to intensify other aromas. Additionally, they are potentially suitable as solvents and advanced biofuels and could help reduce dependence on fossil fuels.

FAEEs are therefore widely used in both indoor and outdoor environments. If the side chain is short, FAEEs are highly volatile and prone to be present in the ambient air. Especially in indoor environments with poor ventilation, cumulative human exposure can be substantial. In the gas phase, the main loss processes of FAEEs are likely the reactions with OH radicals and photolysis. Rate coefficients and photolysis parameters for these processes determine the atmospheric lifetime of the FAEEs and the degree to which indoor-outdoor-exchange is possible, as well as the production rate of potentially harmful secondary products. However, detailed knowledge of the degradation mechanisms and kinetics is scarce for many FAEEs.

Here, we report experimental data on the OH radical reactions and photolytic properties of ethyl butyrate and several branched derivatives (ethyl 2-methylbutyrate, ethyl isovalerate, isopropyl butyrate). Results are discussed in terms of their potential impact on air quality both indoors and out.

How to cite: Löher, F., Carslaw, N., and Dillon, T. J.: Gas-phase Experiments on the Reactivity and Fate of Short-Chain Fatty Acid Ethyl Ester Derivatives, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10519, https://doi.org/10.5194/egusphere-egu25-10519, 2025.

EGU25-10782 | Orals | AS3.2

Impacts of oxygenated organic compounds on photochemical air pollution in coastal Hong Kong 

Zhe Wang, Lirong Hui, Yang Xu, Yi Chen, Yao Chen, and Xin Feng

Oxygenated organic compounds are key reactive pollutants that significant impact air quality and human health. They play critical roles in tropospheric photochemistry and oxidation capacity, profoundly influencing radical cycling and O3 formation. Despite their importance, the precise quantification of these compounds remain a significant challenging. Here we present a comprehensive field study of volatile organic compounds (VOCs) and oxygenated VOCs in the coastal atmosphere of Hong Kong, employing a combination of real-time online mass spectrometry and offline sampling methods. The measurements revealed the substantial abundance of OVOCs and their significant contributions (~50%) to photochemical reactivity and O3 formation potential. Further observation-based modeling analysis were performed to quantify the impacts of these reactive organic species on photochemistry and the formation of secondary pollutants. The results demonstrated that the OVOCs related reactions can contribute to 30-65% of peroxy radical formation and recycling, thereby enhancing daytime O3 formation. This highlights the pivotal role of OVOCs in photochemical pollution and air quality. Our results provide quantitative insights into the formation and impacts of oxygenated reactive organics, highlighting their pivotal roles in photochemical pollution and air quality. These findings are essential for improving air quality models and developing effective pollution control strategies, particularly in coastal urban environments.

How to cite: Wang, Z., Hui, L., Xu, Y., Chen, Y., Chen, Y., and Feng, X.: Impacts of oxygenated organic compounds on photochemical air pollution in coastal Hong Kong, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10782, https://doi.org/10.5194/egusphere-egu25-10782, 2025.

EGU25-11696 | Posters on site | AS3.2

Ozone and Secondary Organic Aerosol Formation Potential from Native Tree Species in Atlantic Forest Remnants of Southeastern Brazil under Anthropogenic Influence 

Silvia Ribeiro de Souza, Bruno Ruiz Brandão da Costa, Fernanda Anselmo-Moreira, Alex do Nascimento, Eduardo Luiz Martins Catharino, Patrícia Menezes Ferreira Rodrigues, Tarcísio Ferreira Martins, Michael Staudt, Kátia Mazzei, Cláudia Maria Furlan, Manon Rocco, Agnès Borbon, and Adalgiza Fornaro

Biogenic volatile organic compounds (BVOCs) play a crucial role in urban air quality by contributing to ground-level ozone (O₃) and secondary organic aerosol (SOA) formation. While forests help mitigate air pollution, BVOC emissions can interact with anthropogenic pollutants, exacerbating air pollution. These emissions are influenced by seasonality and urbanization, affecting both their rates and chemical compositions [1]. In the Metropolitan Area of São Paulo (MASP), the Atlantic Forest provides a valuable opportunity to study these interactions, but current research is limited [2].

This study assessed BVOC emissions from four native Atlantic Forest species —Alchornea sidifolia (AS), Casearia sylvestris (CS), Guarea macrophylla (GM), and Machaerium nyctitans (MN) —across two forest reserves exposed to different pollution levels. Sampling was conducted at the less polluted Morro Grande Forest Reserve (RMG) and the more urbanized Matão-IAG Forest during the dry (August–September 2023) and rainy (January–February 2024) seasons.

Six replicates per species were analyzed. Branches were cut and placed in water to prevent embolism, and BVOCs were collected using a dynamic enclosure system for 1h. Volatiles were trapped on Tenax cartridges, desorbed using thermal desorption, and analyzed via gas chromatography-mass spectrometry. Ozone formation potential (OFP) and SOA formation potential (SOAP) were calculated using emission rates (ER, µg g⁻¹ h⁻¹), Maximum Incremental Reactivity (MIR), and Fractional Aerosol Coefficients (FACs).

Among the species studied, no isoprene emitters were identified. Sesquiterpenes (SQTs) dominated the emissions. During the dry season at RMG, CS presented the highest OFP (23.44 µg g⁻¹ h⁻¹), driven by elevated SQT emissions. MN ranked second (4.89 µg g⁻¹ h⁻¹) due to high 3-hexen-1-ol emissions, followed by GM (2.91 µg g⁻¹ h⁻¹) and AS (1.96 µg g⁻¹ h⁻¹). At Matão-IAG, CS remained the top contributor but with reduced OFP. AS rose to second place (2.40 µg g⁻¹ h⁻¹), surpassing GM (2.05 µg g⁻¹ h⁻¹). During the rainy season, CS still led (3.26 µg g⁻¹ h⁻¹) at RMG, followed by GM (2.10 µg g⁻¹ h⁻¹), AS (1.65 µg g⁻¹ h⁻¹), and MN (1.50 µg g⁻¹ h⁻¹). Similar trends were observed at Matão-IAG, with CS (2.74 µg g⁻¹ h⁻¹) leading, followed by AS (2.23 µg g⁻¹ h⁻¹), GM (1.99 µg g⁻¹h⁻¹), and MN (0.51 µg g⁻¹ h⁻¹). SOAP trends mirrored OFP. CS consistently had the highest SOAP, particularly at RMG during the dry season (213.30 µg g⁻¹ h⁻¹). GM (19.98 µg g⁻¹ h⁻¹) and AS (17.93 µg g⁻¹ h⁻¹) followed while MN had minimal contributions (1.89 µg g⁻¹ h⁻¹). At Matão-IAG, AS surpassed GM during the rainy season (18.93 vs. 15.63 µg g⁻¹ h⁻¹). Overall, OFP and SOAP exhibited site- and season-dependent variations, declining during the rainy season. CS, as the highest emitter, warrants careful consideration in reforestation planning.

Keywords: BVOCs, São Paulo, Atlantic Forest


Acknowledgements: Funded by Biomasp+ Project - FAPESP (20/07141-2) and, conducted at the Laboratory of Plant-Atmosphere Interaction (LABIAP), Environmental Research Institute of São Paulo.

References
[1] dos Santos et al. 2022. Science of the Total Environment, 824, 153728.
[2] Anselmo-Moreira et al. 2025. Urban Forestry & Urban Greening, 104, 128645.

How to cite: de Souza, S. R., Ruiz Brandão da Costa, B., Anselmo-Moreira, F., do Nascimento, A., Martins Catharino, E. L., Menezes Ferreira Rodrigues, P., Ferreira Martins, T., Staudt, M., Mazzei, K., Furlan, C. M., Rocco, M., Borbon, A., and Fornaro, A.: Ozone and Secondary Organic Aerosol Formation Potential from Native Tree Species in Atlantic Forest Remnants of Southeastern Brazil under Anthropogenic Influence, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11696, https://doi.org/10.5194/egusphere-egu25-11696, 2025.

EGU25-12518 | Orals | AS3.2 | Highlight

Evaluating the emissions and chemistry of understudied VOC sources using observations from field and laboratory studies. 

Matthew Coggon and the AEROMMA and SAPHIR Team

Oxygenated volatile organic compounds (oVOCs) emitted from non-vehicular sources, such as volatile chemical products (VCPs) and cooking, are important contributors to the total anthropogenic VOCs observed in urban regions. Models typically underrepresent oVOC emissions compared to observations and the chemical reactions that describe oVOC oxidation are often missing or misrepresented in chemical mechanisms. Here, we present multi-year efforts to update atmospheric models to better reflect the emissions and chemistry of oVOC sources. We leverage measurements from multiple ground campaigns to update emissions inventories, then use models with updated oVOC chemistry to understand how these emissions react in the atmosphere. We compare these observations to laboratory simulations of urban air conducted in the SAPHIR chamber during the Household Chemicals Amplifying Urban Aerosol Pollution (CHANEL) experiment. We demonstrate how we are using these models to better understand the detailed chemical measurements conducted in urban areas during the 2023 Atmospheric Emissions and Reactions from Megacities to Marine Areas (AEROMMA) aircraft campaign. We will discuss what implications these updates may have on model simulations of ozone production in megacities like Los Angeles, CA.

How to cite: Coggon, M. and the AEROMMA and SAPHIR Team: Evaluating the emissions and chemistry of understudied VOC sources using observations from field and laboratory studies., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12518, https://doi.org/10.5194/egusphere-egu25-12518, 2025.

EGU25-12883 | ECS | Posters on site | AS3.2

The Role of Oxygenated Organosulfates in Mixed Biogenic and Anthropogenic New ParticleFormation 

Lee Tiszenkel, Vignesh Vasudevan Geetha, Jonas Elm, Daniel Bryan, and Shanhu Lee

New particle formation (NPF) from the interactions between biogenic and anthropogenic precursors is responsible for a large portion of the sub-micron particle loadings observed in the atmosphere. Previous observations of aerosol chemical composition in these environments have found that organosulfates form in the particle phase. However, it is not clear how organosulfates form and how they contribute to the formation and growth of new particles.  We present the results of laboratory studies of NPF in a mixed organic/inorganic system including α-pinene, isoprene, sulfur dioxide and ozone in a fast flow reactor. Highly-oxidized organic compounds, organosulfates and sulfuric acid clusters were measured online with nitrate high-resolution time-of-flight (HRToF) CIMS at the end of the flow tube. Additionally, newly formed particles were collected on filters for offline analysis of their chemical composition with an ultra- performance liquid chromatography-electrospray ionization Orbitrap mass spectrometer (UPLC/(-)ESI-Orbitrap MS). There was a significant amount of oxygenated organosulfates in the particle phase, which is consistent with our previous studies. We also detected significant amounts of gas-phase organosulfates in the experimental system and found that their contribution to nucleation rates depends on the molecular size, precursor compound, and O:C ratio within the oxygenated organosulfate compound. We present detailed formation mechanisms of oxygenated organosulfates determined through MS/MS fragmentation analysis and quantum chemical modelling. Currently, parameterizations of atmospheric NPF sum the contributions of each individual chemical precursor as a separate process. Our observations demonstrate that chemical interactions of precursors in the gas and particle phase must be considered in NPF parameterizations to predict particle formation and growth in biogenic environments with transported sulfur plumes, or urban environments with abundant monoterpenes and isoprene.

How to cite: Tiszenkel, L., Vasudevan Geetha, V., Elm, J., Bryan, D., and Lee, S.: The Role of Oxygenated Organosulfates in Mixed Biogenic and Anthropogenic New ParticleFormation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12883, https://doi.org/10.5194/egusphere-egu25-12883, 2025.

EGU25-13021 | Posters on site | AS3.2

Volatile organic compound measurements in an urban coastal environment impacted by oil refinery emissions 

Rodrigo Seguel, Nicole Zárate, Charlie Opazo, Lucas Castillo, Felipe Céspedes, Roberto Quezada, Gerardo Alvarado, and Ricardo Muñoz

This study aims to evaluate the reliability of volatile organic compound (VOC) detection and identification in complex coastal terrains in Central Chile. In this zone, frequent complaints by residents prompted a new National Ambient Air Quality Standard for benzene in 2023, set at 0.9 ppbv (nmol mol-1). The monitoring site is located in Concón City, near an oil refinery where we combine a Proton Transfer Reaction Time of Flight Mass Spectrometry (PTR–TOF–MS), a Gas Chromatograph coupled with a Flame Ionization Detector (GC-FID) and meteorological observations.  

We utilized a PTR-TOF-MS (Ionicon Analytik GmbH) to assign monoisotopic masses to specific VOCs. The mass resolution (m/Δm full width at half maximum) was typically ~1000 for benzene (toluene) at m/z 79.054 (93.070). To measure the PTR’s sensitivity, we calibrated the instrument by a multipoint calibration, ranging from 0.5 to 8 ppbv, using a self-made dilution system, ultra-high-purity nitrogen and gas mixture of 8 VOCs (Apel-Riemer Environmental, Inc.). The sensitivity and limit of detection (LoD) for benzene (toluene) determined at a measurement frequency of 1 Hz was 38 cps ppbv-1 (30 cps ppbv-1) and 0.20 ppbv (0.30 ppbv).

Our initial PTR measurements in the zone indicated the worst air quality conditions occurred early in the morning due to unfavorable ventilation. Therefore, we will use the parallel measurements of the PTR and the GC (from Jan to Sep 2025) to evaluate the instrument responses during short and intense VOC spikes, considering the rapid meteorological changes such as wind speed and direction and the evolution of the marine boundary layer height (estimated with a ceilometer). In addition, we will use the intercomparison data to assess the fragmentation among other interferences.

How to cite: Seguel, R., Zárate, N., Opazo, C., Castillo, L., Céspedes, F., Quezada, R., Alvarado, G., and Muñoz, R.: Volatile organic compound measurements in an urban coastal environment impacted by oil refinery emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13021, https://doi.org/10.5194/egusphere-egu25-13021, 2025.

EGU25-13080 | Orals | AS3.2

Advancements in the Detection and Monitoring of VOCs 

Jan Wozniak, Keren Drori, Russell Chedgy, Chris Rella, Kai Skog, and Gregor Lucic

In recent years, there has been increasing interest in monitoring Volatile Organic Compounds (VOCs) in the ambient atmosphere. VOCs in the atmosphere can lead to dangerous levels of ozone, impacting human health and degrading ecosystems. Further, many VOCs are themselves considered highly toxic at parts-per-billion (ppb) and even parts-per-trillion (ppt) levels, potentially causing respiratory problems and contributing to elevated cancer risk in affected populations. More recently, the EPA has proposed more stringent fence line monitoring requirements for six critical air toxics: benzene, ethylene oxide, chloroprene, 1,3-butadiene, vinyl chloride, and ethylene dichloride.

 

In response to this growing need for high-performance, field-deployable VOC analyzers, Picarro has developed Broad Band Cavity Ring-Down Spectroscopy (BB-CRDS), a laser-based technology that is capable of quantifying a wide variety of VOCs in real time (< 5 seconds) at ppb and ppt levels. This analyzer is capable of simultaneously measuring ten or more compounds, selected from our growing library of nearly 500 characterized species, which includes both VOCs and common inorganics like H2O, CO2, CH4, N2O, and NH3. It is simple to operate, and it can be deployed in harsh environments with little to no consumables. We demonstrate the design and performance of these analyzers, presenting substantial advancements for air quality management and regulatory compliance.

How to cite: Wozniak, J., Drori, K., Chedgy, R., Rella, C., Skog, K., and Lucic, G.: Advancements in the Detection and Monitoring of VOCs, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13080, https://doi.org/10.5194/egusphere-egu25-13080, 2025.

EGU25-13407 | ECS | Orals | AS3.2

Gas-particle partitioning and yield of organic nitrate under different VOC, NOx, and oxidation conditions 

Farhan Ramadzan Nursanto, Quanfu He, Sophia van de Wouw, Annika Zanders, Willem S. J. Kroese, Roy Meinen, Robert Wegener, Max Gerrit Adam, Benjamin Winter, René Dubus, Lukas Kesper, Franz Rohrer, Rupert Holzinger, Thorsten Hohaus, Georgios I. Gkatzelis, Maarten C. Krol, and Juliane L. Fry and the SAPHIR-CHANEL 2024

Particulate nitrate is a major aerosol component worldwide that acts as a reservoir of urban nitrogen oxides (NOx=NO+NO2). Chemical reactions of NOx with volatile organic compounds (VOCs) will form organic nitrates that undergo gas-particle partitioning and therefore may influence the lifetime and transport of nitrogen compounds, impacting their deposition on ecosystems.

In this study, we use data collected in chamber experiments and in ambient air to investigate how emission profiles and ambient conditions affect the gas-particle partitioning and the yield of organic nitrate. Chamber studies during the SAPHIR-CHANEL campaign show that monoterpenes, higher NOx, and reactions with the nitrate radical in the absence of light favor the formation of organic nitrate in urban NOx-VOC mixtures. Similar results are found at a continuous monitoring site in rural central Netherlands where the type of organic nitrate during pollution episodes depends on the airmass source and the corresponding VOC and NOx profiles. By combining results from chamber and ambient measurements, we provide new insights into atmospheric organic nitrate chemistry.

How to cite: Nursanto, F. R., He, Q., van de Wouw, S., Zanders, A., Kroese, W. S. J., Meinen, R., Wegener, R., Adam, M. G., Winter, B., Dubus, R., Kesper, L., Rohrer, F., Holzinger, R., Hohaus, T., Gkatzelis, G. I., Krol, M. C., and Fry, J. L. and the SAPHIR-CHANEL 2024: Gas-particle partitioning and yield of organic nitrate under different VOC, NOx, and oxidation conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13407, https://doi.org/10.5194/egusphere-egu25-13407, 2025.

EGU25-13574 | Orals | AS3.2

Long-term Trends in Organic Carbon Concentrations within Cloud Water and Precipitation Samples in the Northeastern United States  

Sara Lance, Christopher Lawrence, Archana Tripathy, Paul Casson, Phil Snyder, Georgia Murray, Desneiges Murray, Adam Wymore, Bill McDowell, Michelle Shattuck, James Shanley, John Campbell, Mark Green, Eric Apel, Rebecca Hornbrook, Alan Hills, Elizabeth Yerger, and Dan Kelting

Recent research at Whiteface Mountain, one of the few remaining sites in the U.S. where long-term cloud water chemistry research has continued to the present day, has revealed a doubling in cloud water organic carbon concentrations since measurements began in 2009. This dramatic increasing trend was an unexpected result, which requires further investigation. The present study attempts to verify these results using additional independent datasets from within the region and explores potential driving factors behind the observed organic carbon trends. Through evaluation of measurements from four additional sites in the north eastern U.S., each with long-term measurements of organic carbon concentrations within bulk cloud water or wet deposition samples, we show that there is strong evidence for a regional increasing trend in organic concentrations within aqueous atmospheric samples. These results provide further context behind the growing inorganic ion imbalance observed in wet deposition samples collected across the eastern U.S. and Canada, as identified in a separate study published in 2021. We discuss hypotheses for the potential driving factors behind the increasing organic carbon trends observed, including increased biomass burning influence, increased biogenic emissions and a changing chemical regime characterized by relatively high concentrations of reactive nitrogen chemical species.

How to cite: Lance, S., Lawrence, C., Tripathy, A., Casson, P., Snyder, P., Murray, G., Murray, D., Wymore, A., McDowell, B., Shattuck, M., Shanley, J., Campbell, J., Green, M., Apel, E., Hornbrook, R., Hills, A., Yerger, E., and Kelting, D.: Long-term Trends in Organic Carbon Concentrations within Cloud Water and Precipitation Samples in the Northeastern United States , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13574, https://doi.org/10.5194/egusphere-egu25-13574, 2025.

EGU25-15281 | Orals | AS3.2

Sources of Oxygenated Organic Molecules and Their Impacts on Organic Aerosol in China 

Bin Zhao, Dejia Yin, Shuxiao Wang, Yicong He, and Neil Donahue

Oxygenated organic molecules (OOMs), the oxidation products of organic precursors with low volatility and a high oxygen atom number, are an important driver of new particle formation (NPF) and secondary organic aerosols (SOA) formation. The sources and formation processes of OOMs are highly complicated, especially in populous regions (e.g., China) with diverse emissions of anthropogenic and biogenic precursors. However, current models fail to capture OOM formation from different precursors due to the absence of important reaction pathways (e.g., autoxidation, dimerization) and the oversimplified treatment of the oxidation of semi-volatile and intermediate-volatility precursors (I/SVOCs). In this work, we develop a Precursor-resolved Integrated two-dimensional Volatility Basis Set (I2D-VBS) model framework, which simulates the multi-generational ageing of organic emissions in the full volatility range on a precursor level and explicitly tracks irregular radical reactions, including autoxidation, dimerization, and RO isomerization followed by accelerated autoxidation. The parameterizations within the Precursor-resolved I2D-VBS are optimized by simulating chamber and flow-tube experiments measuring OOMs and SOA formed from individual precursors. We then incorporate the Precursor-resolved I2D-VBS in the CMAQ chemical transport model and simulate OOM formation in China. The CMAQ/I2D-VBS model successfully reproduced OOM concentrations at various sites across China, achieving accuracy within ±40% for total OOM concentrations and within a factor of 2 for volatility-binned OOM concentrations. The model results reveal that over 60% of total OOM concentrations are from I/SVOC in China; nevertheless, for extremely low-volatility OOMs (logC*<=-5) that are important for initial particle growth, ~60% of them are from anthropogenic VOCs in the North China Plain and ~80% of them are from biogenic VOCs in Southeast China. Multi-generational OH oxidation is the reaction pathway contributing most to OOM formation (>70%), followed by autoxidation (~20%). Overall, OOMs contribute around half of SOA concentrations in China, highlighting the critically important role of OOMs in SOA formation.

How to cite: Zhao, B., Yin, D., Wang, S., He, Y., and Donahue, N.: Sources of Oxygenated Organic Molecules and Their Impacts on Organic Aerosol in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15281, https://doi.org/10.5194/egusphere-egu25-15281, 2025.

EGU25-15473 | ECS | Posters on site | AS3.2

Source and sink of volatile organic compounds over snow surface 

Yan Yang, Xinxin Li, Wenjia Zhao, Tao Wang, Qianjie Chen, and Jianhuai Ye

Snow can serve as both a source and a sink for atmospheric volatile organic compounds (VOCs), as well as a surface for their oxidation. However, the influence of snow on the distribution and fate of VOCs at the surface level remains largely unclear. To address this, we conducted a field campaign in a suburban site of Northeast China, from January to March 2024. VOCs were collected using sorbent cartridges at three different heights (i.e., 2.2 m above snow, at snow surface, and 0.1 m below snow surface), over five daily time intervals, including 7:00 to 10:00, 10:00 to 13:00, 13:00 to 16:00, 16:00 to 19:00, and 19:00 to 7:00 the following day. A total of 48 VOCs, out of 89 in the standards, were detected and quantified due to their relatively low concentrations. These included 16 alkanes, 3 alkenes, 14 aromatics, and 15 halogenated hydrocarbons, measured using thermal desorption-gas chromatography-mass spectrometry (TD-GC-MS). Alkanes and aromatics were the most abundant VOC species, exhibiting a diurnal pattern with lower concentrations during the day and higher concentrations at night. The vertical profiles of VOCs indicated that snow could serve as a source for certain species, such as monoterpenes, and as a sink for others, such as aromatics. The corresponding emission rates and deposition velocities were calculated. The findings from this study enhance the understanding of snow-atmosphere interactions and provide critical insights into the role of snow in influencing surface-level VOC distributions and their associated atmospheric processes.

How to cite: Yang, Y., Li, X., Zhao, W., Wang, T., Chen, Q., and Ye, J.: Source and sink of volatile organic compounds over snow surface, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15473, https://doi.org/10.5194/egusphere-egu25-15473, 2025.

EGU25-15481 | ECS | Orals | AS3.2

BVOC fluxes and concentrations at a boreal forest site in Sweden: an overview of long-term observations at ICOS Norunda and the impacts of forest clear-cutting on BVOC emissions 

Ross Petersen, Cheng Wu, Claudia Mohr, Riikka Rinnan, Thomas Holst, Erica Jaakkola, Radovan Krejci, and Janne Rinne

Vegetation is the major source of volatile organic compounds (VOCs) in the atmosphere, which affect both air quality and climate. Long-term ecosystem-level data on biogenic VOC (BVOC) emissions, however, are limited. This limits assessment of impacts of short-term landscape-scale disturbances like clear-cutting, and seasonal-scale and interannual variation of emissions of boreal forests.

Here we present an overview of BVOC concentration and flux measurements and results spanning several years, leading up to the summer 2022 clear-cutting of a boreal forest located at the ICOS (Integrated Carbon Observation System) and ACTRIS (Aerosol, Clouds, and Traces Gases Research Infrastructure) station Norunda (located at 60°05′N, 17°29′E, ca. 30 km north of Uppsala) in Sweden. This managed boreal forest, between 80 and 120 years old, primarily consisted of a mix of Scots pine (Pinus sylvestris) and Norway spruce (Picea abies). Beginning in summer 2020, BVOC mixing ratios were measured using a Vocus proton-transfer-reaction time-of-flight mass spectrometer (Vocus PTR-ToF-MS) (Tofwerk AG, Thun, Switzerland). These Vocus measurements (at 10 Hz) were collected at 35 m on the station flux tower to determine BVOC fluxes using the eddy-covariance method. During several intensive BVOC sampling periods in 2020 and 2022, hourly adsorbent samples were also collected, at 37 and 60 m, for subsequent GC-MS analysis to determine compound-speciated BVOC concentrations. These samples were additionally used to estimate the changes in the fluxes of speciated monoterpene (MT) compounds using the surface-layer-gradient (SLG) and modified Bowen-ratio (MBR) methods.

Our results indicate a large variety of VOC compounds being emitted by the forest system, including among them terpenoids - e.g., isoprene, monoterpenes (MTs) and sesquiterpenes (SQTs). The most common MT compounds emitted were α-pinene and Δ3-carene. During the 2022 clearcut, MT emissions increased by more than an order of magnitude during active-cutting, with persisting MT emission increases from clearcut residue which continued for several months. In comparison, many BVOCs lacking storage reservoirs in plant tissues (e.g., isoprene) were relatively unaffected by active-cutting. Fluxes and the mixture of speciated MT compounds observed before, during, and post-cut are compared, and the additional total and speciated MT emissions due to clear-cutting are estimated. For context, in Sweden 69% of total land cover is forest, of which 84% is productive forest for clear-cut forestry (~58% of total land cover). From Swedish forestry information of yearly absolute timber removal and on-site residue volumes following typical clearcuts, we find that current Swedish boreal forest MT emission inventory estimates may be significantly underestimated.

How to cite: Petersen, R., Wu, C., Mohr, C., Rinnan, R., Holst, T., Jaakkola, E., Krejci, R., and Rinne, J.: BVOC fluxes and concentrations at a boreal forest site in Sweden: an overview of long-term observations at ICOS Norunda and the impacts of forest clear-cutting on BVOC emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15481, https://doi.org/10.5194/egusphere-egu25-15481, 2025.

EGU25-15710 | Orals | AS3.2

Emerging diversity of volatile organic compounds from freshwater and marine ecosystems 

Riikka Rinnan, Ellen Slater, Riley Hughes, Yinghuan Qin, Mehrshad Foroughan, Isabelle Laurion, Genevieve Chiapusio, Michael Steinke, Lauri Laakso, Heidi Hellén, Kaisa Kraft, Jukka Seppälä, Kajsa Roslund, Jesper Riis Christiansen, and Thomas Holst

The chemical diversity of volatile organic compound (VOC) emissions from terrestrial vegetation is relatively well understood, while research on VOC emissions from freshwater and marine systems has largely focused on dimethyl sulfide (DMS) and isoprene. Through VOC concentration measurements in water samples, and VOC flux measurements using floating chambers and the direct eddy covariance (EC) technique we aim to evaluate aquatic ecosystems as sources of VOCs. Here, we present selected case studies that demonstrate the need to consider other VOCs beyond DMS and isoprene when assessing aquatic sources of atmospheric VOCs.

A survey of depth-specific VOC concentrations in water from four Alpine lakes in France showed that VOC concentrations were highest either at the deep chlorophyll maximum or at the surface. The VOC composition profiles differed between depths and lakes. In another study, we assessed net emissions of VOCs from three ponds in a rewetted peatland forest in Denmark. Again, the three ponds showed differences in the quantity and diversity of their emission profiles. Over 100 chemical species were detected, including acetone, acetaldehyde, isoprene, other terpenoids, and hydrocarbons. The most eutrophic and acidic pond had highest emission rates but lower VOC diversity compared to the alkaline ponds.

The VOC emission rates and compositions also vary over time, depending on the balance between VOC production, consumption, and emission rates, driven by both biotic and abiotic factors. Our EC flux measurements on Utö Island in the Baltic Sea show strong seasonal variation in marine VOC emissions, which can be coupled to the biomass and phenology of the phytoplankton as well as to environmental factors.

We highlight the emerging diversity of VOC emissions from aquatic ecosystems. These emissions need to be better quantified to assess their atmospheric fate and implications.

How to cite: Rinnan, R., Slater, E., Hughes, R., Qin, Y., Foroughan, M., Laurion, I., Chiapusio, G., Steinke, M., Laakso, L., Hellén, H., Kraft, K., Seppälä, J., Roslund, K., Riis Christiansen, J., and Holst, T.: Emerging diversity of volatile organic compounds from freshwater and marine ecosystems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15710, https://doi.org/10.5194/egusphere-egu25-15710, 2025.

EGU25-16045 | ECS | Orals | AS3.2

Plant volatile emissions experiments with coniferous and broadleaf tree seedlings: the impact of extreme events and future climate scenarios 

Simone M. Pieber, Ugo Molteni, Na Luo, Markus Kalberer, Celia Faiola, and Arthur Gessler

Biogenic volatile organic compounds (BVOC) are a highly complex and highly diverse set of chemicals emitted into the atmosphere by the Earth's biosphere. They affect atmospheric composition of trace gases such as the mixing ratios of methane, carbon monoxide, and tropospheric ozone through their atmospheric oxidation. Atmospheric oxidation products also lead to formation of atmospheric aerosol, which plays a crucial role in defining Earth's radiative balance and impacts air quality.  

Further increases in the average global temperature are expected for the following decades, with warmer and dryer conditions for Alpine regions. Warm winters appear to lead to earlier leaf-out. This may put trees at higher risk of late frost in spring. Thus, in addition to long-term changes in abiotic factors (temperature, water availability), the frequency of stress and double-stress events, such as a late spring frost and an extreme summer drought occurring in the same year, is expected to increase. How trees respond to such changes in abiotic factors and to abiotic (double) stress regarding their BVOC emissions composition and quantities is critical in understanding how atmospheric chemistry and SOA properties may be impacted.  

During the summer of 2022, we studied the impact of elevated temperatures (heat), reduced water availability (drought), extreme events (early spring frost) and double stress (early spring frost followed by extreme summer drought) on tree seedlings i.) BVOC precursors in plant tissues (i.e., secondary metabolites) and ii.) BVOC gas-phase emissions. To this end, i.) we developed an analytical method for extraction and chromatographic separation of secondary metabolites from plant tissues, and ii.) we designed and built a novel plant chamber for BVOC gas-phase measurements online with a PTR-ToF-MS and offline with thermodesorption-GC-MS. We will present comprehensive results from experiments with Scots Pine, Beech, and Oak seedlings under various abiotic stress conditions. Our findings provide crucial insights for improving estimations of future BVOC emissions and their atmospheric impacts.

How to cite: Pieber, S. M., Molteni, U., Luo, N., Kalberer, M., Faiola, C., and Gessler, A.: Plant volatile emissions experiments with coniferous and broadleaf tree seedlings: the impact of extreme events and future climate scenarios, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16045, https://doi.org/10.5194/egusphere-egu25-16045, 2025.

EGU25-16150 | ECS | Posters on site | AS3.2

Improving BVOC emission estimation with high-resolution tree species mapping in urban areas 

Linqiang Ma and Jianhuai Ye

Biogenic volatile organic compounds (BVOCs) are critical precursors of atmospheric secondary pollutants, posing challenges to urban air quality management and public health. Current methodologies for estimating BVOC emissions, largely based on plant functional types (PFTs), lack the spatial and taxonomic precision required for urban landscapes characterized by diverse and heterogeneous vegetation. This limitation introduces significant uncertainties, particularly in highly developed urban areas. To address this gap, this study proposes the development of a high-resolution tree species classification dataset by utilizing remote sensing, machine learning, or in situ data integration techniques. By integrating this dataset with existing emission models, the research aims to quantify the discrepancies between species-level and PFT-based BVOC emission estimates, with a specific focus on urban areas. The species-level data is observed to yield higher emission estimates, highlighting the importance of fine-scale classification for accurately capturing emission dynamics. Additionally, this study analyzes the spatial distribution of BVOCs across urban and peri-urban gradients and assesses the implications of BVOC emissions on the formation of ozone. The findings are expected to provide suggestions for urban vegetation management, supporting the design of evidence-based strategies to mitigate air pollution and enhance urban sustainability.

How to cite: Ma, L. and Ye, J.: Improving BVOC emission estimation with high-resolution tree species mapping in urban areas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16150, https://doi.org/10.5194/egusphere-egu25-16150, 2025.

EGU25-16682 | ECS | Posters on site | AS3.2

Breaking Calibration Barriers: Quantifying Oxidation Products in Chamber and Field Measurements via Voltage Scanning 

Milan Roska, Chelsea Stockwell, Lu Xu, Matthew M. Coggon, Kelvin Bates, Caroline Womack, Carsten Warneke, and Georgios I. Gkatzelis and the CHANEL Campaign 2024

Quantification of intermediate oxidation products is critical for understanding urban emissions and secondary pollution. Ammonium chemical ionization mass spectrometry is established as a detection method for a wide range of functionalized gas-phase compounds. However, conventional calibration methods are reaching their limits.

In this work, we use Voltage Scanning as a novel approach to estimate the detection sensitivity for uncalibrated compounds by comparing their dissociation patterns to patterns of well-calibrated gas standards. We performed extensive characterization and optimization of the method in laboratory experiments to determine optimal conditions at a high time resolution. We implement the method in experiments in the SAPHIR simulation chamber and onboard the NASA DC8 research aircraft. This enables the quantification of a substantial number of the oxygenated organic compounds that have not been previously quantified. We highlight the potential of Voltage Scanning as a powerful tool to further advance our understanding of urban air pollution for field studies, but also in simulation chamber experiments, moving a step closer to achieving carbon closure.

How to cite: Roska, M., Stockwell, C., Xu, L., Coggon, M. M., Bates, K., Womack, C., Warneke, C., and Gkatzelis, G. I. and the CHANEL Campaign 2024: Breaking Calibration Barriers: Quantifying Oxidation Products in Chamber and Field Measurements via Voltage Scanning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16682, https://doi.org/10.5194/egusphere-egu25-16682, 2025.

EGU25-17927 | Posters on site | AS3.2

Identifying volatile organic compounds at a rural site in the Italian Po Valley 

Nora Zannoni, Luca D'Angelo, Alice Cavaliere, Marco Paglione, Julia David, Mario Simon, Alexander Vogel, and Angela Marinoni

Volatile organic compounds (VOCs) released into the atmosphere by natural and anthropogenic sources play a key role in atmospheric processes. They can react with atmospheric oxidants leading to secondary organic aerosols and tropospheric ozone, with effects on air pollution, human health and climate.

The Po Valley, located in the North of Italy is a densely populated area influenced by intense agricultural, industrial and urban-related activities, suffering among the worst air pollution in Europe. Although efforts aimed at characterizing the chemical and physical processes influencing aerosols and other atmospheric pollutants have been conducted over the last decades, very little is known about the precursor organic chemical species emitted in this region.

Volatile organic compounds in the mass range 0-400 amu were measured for three weeks in October 2023 at a rural site in Schivenoglia (MN), in central Po Valley, using a Vocus CI-ToF (chemical ionization time of flight) 2R mass spectrometer (Tofwerk, Switzerland). During the measuring campaign, the site was influenced by contrasting meteorological conditions, warm and colder temperatures as well as biomass burning events and the application of manure to fertilize the fields. Over 1000 peaks, corresponding to volatile molecules and their possible fragments were detected in the measured mass spectra. Among the detected peaks, about 500 were tentatively associated to a chemical identity. The concentrations of the identified species are discussed in function of their variability with time, meteorological conditions, and emission sources, in order to elucidate the atmospheric processes influencing VOC concentrations in the Po valley.

How to cite: Zannoni, N., D'Angelo, L., Cavaliere, A., Paglione, M., David, J., Simon, M., Vogel, A., and Marinoni, A.: Identifying volatile organic compounds at a rural site in the Italian Po Valley, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17927, https://doi.org/10.5194/egusphere-egu25-17927, 2025.

Volatile chemical products (VCPs) are increasingly recognized as significant sources of volatile organic compounds (VOCs) in urban atmospheres, potentially serving as key precursors for secondary organic aerosol (SOA) formation. This study investigates the formation and physicochemical transformations of VCP-derived SOA, produced through ozonolysis of VOCs evaporated from a representative room deodorant air freshener, focusing on the effects of aerosol evaporation on its molecular composition, light absorption properties, and reactive oxygen species (ROS) generation. Following aerosol evaporation, solutes become concentrated, accelerating reactions within the aerosol matrix that lead to a 42% reduction in peroxide content and noticeable browning of the SOA. This process occurs most effectively at moderate relative humidity (∼40%), reaching a maximum solute concentration before aerosol solidification. Molecular characterization reveals that evaporating VCP-derived SOA produces highly conjugated nitrogen-containing products from interactions between existing or transformed carbonyl compounds and reduced nitrogen species, likely acting as chromophores responsible for the observed brownish coloration. Additionally, the reactivity of VCP-derived SOA was elucidated through heterogeneous oxidation of sulfur dioxide (SO2), which revealed enhanced photosensitized sulfate production upon drying. Direct measurements of ROS, including singlet oxygen (1O2), superoxide (O2•–), and hydroxyl radicals (OH), showed higher abundances in dried versus undried SOA samples under light exposure. Our findings underscore that drying significantly alters the physicochemical properties of VCP-derived SOA, impacting their roles in atmospheric chemistry and radiative balance.

How to cite: Zhou, L., Liang, Z., Qin, Y., and Chan, C. K.: Evaporation-Induced Transformations in Volatile Chemical Product-Derived Secondary Organic Aerosols: Browning Effects and Alterations in Oxidative Reactivity, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18690, https://doi.org/10.5194/egusphere-egu25-18690, 2025.

EGU25-18770 | ECS | Posters on site | AS3.2

Characterization of Volatile Organic Compounds in the Arctic Atmosphere: Insights from High-Resolution Measurements of VOCs at Villum Research Station 

Varun Kumar, Christel Christoffersen, Rossana Bossi, and Henrik Skov

Atmospheric volatile organic compounds (VOCs) influence air quality and climate by participating in chemical reactions that convert them into low-volatility species. These species can contribute to the formation of new particles or condense onto existing aerosol mass. In the presence of NOx, VOC reactions also lead to the production of ground-level ozone. Despite their significance, measurements of VOCs in remote regions such as the Arctic remain scarce, leaving critical gaps in our understanding of their sources, sinks, and chemistry in these pristine environments.

To address this, we conducted field measurements of atmospheric VOCs at the Villum Research Station in northern Greenland from 20 July to 15 August 2024 using proton transfer reaction mass spectrometry (PTR-MS). By employing a high-resolution instrument (PTR-ToF MS 8000; Ionicon Analytik GmbH, Innsbruck, Austria), we identified a broader range of atmospheric VOCs compared to earlier studies at the same site that used a lower-resolution instrument.

In this study, we focus on the concentration levels, chemical family compositions, and source characteristics of VOCs using the positive matrix factorization (PMF) model. We further analyze variations in VOC levels based on back-trajectory data, providing insights into the transport and transformation of these compounds in the Arctic atmosphere. Our findings have important implications for understanding VOC-related atmospheric chemistry in remote regions and their role in Arctic air quality and climate processes.

How to cite: Kumar, V., Christoffersen, C., Bossi, R., and Skov, H.: Characterization of Volatile Organic Compounds in the Arctic Atmosphere: Insights from High-Resolution Measurements of VOCs at Villum Research Station, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18770, https://doi.org/10.5194/egusphere-egu25-18770, 2025.

EGU25-19882 | ECS | Posters on site | AS3.2

Cloud processing of isoprene in the presence of NOx 

Anouck Chassaing, Ilona Riipinen, Roman Bardakov, Claudia Mohr, Francesca Salteri, Imad El Haddad, and Wei Huang

Recent studies show the important role of isoprene in new particle formation (NPF) in the outflow of convective clouds. The oxidation of isoprene combined with low temperatures and low condensation sink yields organic vapours with very low volatility, promoting nucleation (Bardakov et al. 2024, Shen et al. 2024).

This study focuses on the transport of isoprene from low altitudes to the upper troposphere, by convective updrafts. In-cloud isoprene concentration is affected by microphysical mechanisms (uptake by cloud droplets, mixing) and chemical reactions (e.g., OH oxidation). Previous observational and modeling studies have highlighted the survivability of isoprene during transport overnight  due to its high volatility (Bardakov et al. 2024, Murphy et al., 2015). If oxidation can occur inside the convective cloud during the diurnal updraft, further chemical reactions could take place, altering the volatility of the organic vapours present. This would affect the uptake and therefore change the availability of precursors reaching the outflow. NOx, formed during convection due to lightning, could react with isoprene oxidation products to form isoprene nitrates.

We designed a one-month experimental campaign using the smog chamber and the rotating wetted-wall flow reactor (WFR) at PSI. The experimental set up is shown in Figure 1. The isoprene oxidation products are formed in the chamber in the presence of UV lights after the injection of isoprene and HONO (produces OH and NOx) . We varied the oxidation times (OH exposure levels) in the chamber in order to produce first- and second- generation oxidation products (case 1 and 2, respectively). Then, the chamber is used as a reservoir of vapours with the lights off. The vapours are continuously injected into the WFR for 5 hours. In addition, water is injected into the WFR, where due to rotation a microfilm on the inner wall is created. Cases 1 and 2 are carried out either in the absence of light around the WFR (only aqueous uptake), or in the presence of UVB lights, leading to simultaneous aqueous uptake and photochemistry. Another aspect of the experiment is to study the temperature dependence of the aqueous uptake of isoprene oxidation products. The experiment is carried out at 20°C as well as at 5°C in the absence of the light.

Multiple online instruments are deployed in the experiments: two mass spectrometers, Vocus 2R PTR-TOF-MS (proton-transfer-reaction time-of-flight mass spectrometry) and Vocus AIM (Adduct Ionization Mechanism), as well as gas monitors (O3, NO, NO2, NOx) and an SMPS (Scanning mobility particle sizer). 

Figure 1. Schematic of the experimental set-up.

The preliminary analysis shows the dominant presence of MVK/MACR, C4H6O, and isoprene hydroxy nitrates, C5H9NO4 (Figure 2). We will characterize the uptake and chemistry behaviours of the organic vapours under different conditions.

Figure 2. Time series of organic vapours measured with the VOCUS 2R PTR for case 1 at 20°C. Purple shading area indicates chamber measurements.

Grant Agreement number: 101008004.
Grant number: 101073026.

Bardakov, R. et al., (2024) Geophys. Res. Letters, 51
Murphy, B. N. et al., (2015) J. Geophys. Res. Atmos.,120
Shen et al., (2024) Nature, 636

How to cite: Chassaing, A., Riipinen, I., Bardakov, R., Mohr, C., Salteri, F., El Haddad, I., and Huang, W.: Cloud processing of isoprene in the presence of NOx, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19882, https://doi.org/10.5194/egusphere-egu25-19882, 2025.

EGU25-20688 | ECS | Posters on site | AS3.2

Urban emissions fate towards secondary aerosol formation; a chamber study 

Sana Farhoudian, Rabbia Asgher, Shawon Barua, Avinash Kumar, and Matti Rissanen

In recent decades, the proliferation of megacities in developed regions has been paralleled by rapid urbanization across the globe, particularly in developing nations. This trend has led to an increasing number of individuals residing in urban areas, where they face significant air pollution challenges stemming from vehicles and cooking emissions.

It is widely recognized that these sources emit substantial quantities of volatile, semi-volatile, and intermediate-volatility organic compounds (VOCs, SVOCs, and IVOCs), which contribute to considerable secondary organic aerosol (SOA) production. Notable SOA formation has been documented in multiple urban settings, resulting in the generation of carcinogens linked to severe health issues such as lung cancer. Once VOCs are released into the ambient atmosphere, they undergo oxidation, partition between gas and particle phases, and ultimately integrate into primary and secondary organic aerosols (POAs and SOAs), thereby introducing uncertainties into health risk assessments.

Recently, volatile chemical products (VCPs) have emerged as significant unconventional contributors to SOA, particularly as traditional emissions, such as those from vehicle exhausts, are mitigated. A large portion of VCP emissions aligns with urban air quality measurements, both indoors and outdoors. In the U.S., VCPs now represent an increasing share of VOC emissions in urban centers and remain largely unregulated concerning their SOA formation. A comprehensive mass balance indicates that VCPs—including pesticides, coatings, printing inks, adhesives, cleaning products, and personal care items—account for approximately half of fossil fuel VOC emissions in industrialized cities. Furthermore, studies have highlighted that human exposure to carbonaceous aerosols, previously dominated by transportation-related sources, is now shifting towards emissions from VCPs.

In this study, chamber experiments were conducted for various VOC precursors during both daytime and nighttime under different conditions, including a range of NOx levels (low, medium, and high) and the impact of biogenic factors on aerosol yields and composition. Additionally, a low NOx future scenario was explored, assuming reductions in emissions from incomplete combustion alongside a continued rise in global urban population density.

To investigate the oxidation reactions occurring during these experiments, a multi-scheme chemical ionization inlet (MION2, Karsa Inc.) paired with an Orbitrap mass spectrometer (Exploris 240, ThermoFisher) was utilized in the atmospheric simulation chamber. Both nitrate (NO3-) and ethylenediamine (EDA+) reagent ions were employed to ionize the oxidation products, forming corresponding adduct ions.

The oxidation processes yielded a diverse array of highly oxygenated organic molecules (HOM), which are recognized precursors for SOA formation. The various conditions explored in this study enhance our understanding of how gas-phase oxidation influences SOA generation in both polluted and non-polluted urban environments.

How to cite: Farhoudian, S., Asgher, R., Barua, S., Kumar, A., and Rissanen, M.: Urban emissions fate towards secondary aerosol formation; a chamber study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20688, https://doi.org/10.5194/egusphere-egu25-20688, 2025.

EGU25-20718 | Posters on site | AS3.2

Analysis of twenty years (2004–2023) observation of non-methane hydrocarbons in a subtropical coastal environment 

Bernhard Rappenglück, Morshad Ahmed, and Mateen Ahmad

A twenty-year (2004–2023) trend analysis of marine background air was conducted to explore potential changes in non-methane hydrocarbons (NMHCs) emissions and atmospheric oxidation capacity using the Propylene Equivalent (Propy-Equiv) concentration. The focus was on C2-C6 NMHCs including alkanes, aromatics, acetylene, and isoprene, as those were most frequently found in the air samples. During wintertime, least impacted by photochemical impacts, a clear increase in n-pentane was observed from 2004 to 2023 (2.07 ± 2.26 % year-1) (statistically significant). Ethane (-3.82 ± 8.65 % year-1) and n-butane (-1.35 ± 15.62 % year-1) decreased from 2004 to 2008, but this was not statistically significant, but a statistically significant increase was then observed until 2023 (ethane: 1.05 ± 0.51 % year-1; n-butane: 1.09 ± 1.26 % year-1). Iso-pentane decreased (-4.25 ± 1.91 % year-1) steadily from 2004 to 2011 (statistically significant), then remained constant but with increased variability until 2023 (0.28 ± 2.49 % year-1). Propane increased (5.51 ± 23 1.35 % year-1) from 2004 to 2014 (statistically significant) and decreased thereafter until 2023 (-3.63 ± 3.91 % year-1). Acetylene (-1.67 ± 0.51 % year-1), benzene (-2.43 ± 0.14 % year-1), and i-butane (-0.58 ± 25 0.25 % year-1) showed a steady decreasing (statistically significant) trend from 2004 to 2023. The increasing ethane trend for the last 15 years is due to global oil and natural gas extraction, especially in the US, which began in mid-2009. Improvements in gasoline technologies are causing the decline of acetylene and benzene trends. The slower than expected decreasing trend of acetylene mixing ratio might have been offset by the impact of biomass burning emissions. Other NMHCs show varying trends indicating the merge of different emission sources and strengths in separate time periods. During the summertime, 80–90% Propy-Equiv concentration is due to isoprene, with a statistically significant increasing trend (0.45 ppbC/year) between 2004 and 2023. This increase is largely due to rising temperatures (1.58 ± 0.14 ◦C) leading to increased isoprene emissions (20 ± 1.6%).

How to cite: Rappenglück, B., Ahmed, M., and Ahmad, M.: Analysis of twenty years (2004–2023) observation of non-methane hydrocarbons in a subtropical coastal environment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20718, https://doi.org/10.5194/egusphere-egu25-20718, 2025.

EGU25-21187 | ECS | Posters on site | AS3.2

Coupling Measurements of Biogenic Volatile Organic Compounds and Ozone Reactivity in the Field 

Lara Dunn, Joe Acton, Roberto Sommariva, Julia Lehman, and William Bloss

The concentration and fate of ozone in the troposphere is dependent on the ratio of volatile organic compounds (VOCs) and NOx gases emitted from both anthropogenic and biogenic sources. The biosphere emits over 1,000 Tg of VOCs annually, over half of which come from vegetation. The ‘fingerprint’ of chemical compounds emitted varies greatly both between and within vegetative species. This fingerprint is greatly influenced by the environmental conditions an individual plant is exposed to.  In a changing climate, rising atmospheric CO2 concentration is expected to significantly change the quantity and variation of BVOC emissions from vegetation; and thus, the fate of tropospheric O3 concentrations.

This study uses a coupled deployment of a Total Ozone Reactivity System (TORS) and Proton-Transfer-Reaction Mass-Spectrometer (PTR-MS)

At BIFoR FACE (Birmingham Institute for Forest Research Free Air Carbon Dioxide Enrichment) under both ambient and elevated CO2 to assess the impact of rising CO2 on both BVOC emissions and ozone chemistry. Our results show a clear diurnal trend with key ozone reactive BVOCs and ozone reactivity. Interestingly, our study showed a variation in morning and afternoon activity, with isoprene and monoterpene emissions predominantly in the afternoon, with a variation of both BVOC emission and ozone reactivity profile seen in the mornings.

How to cite: Dunn, L., Acton, J., Sommariva, R., Lehman, J., and Bloss, W.: Coupling Measurements of Biogenic Volatile Organic Compounds and Ozone Reactivity in the Field, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21187, https://doi.org/10.5194/egusphere-egu25-21187, 2025.

EGU25-853 | ECS | Posters on site | AS3.3

Chemical Characterization and source apportionment of PM2.5 over an upwind site of Delhi during Biomass Burning and Diwali Festival period  

Vasu Singh, Dilip Ganguly, Jaswant Rathore, Sagnik Dey, and Shahzad Gani

Each year Delhi experiences extremely poor air quality in the post-monsoon season due to large scale stubble burning in the upwind states of Punjab and Haryana, excessive firecracker uses during the Diwali festival, and unfavorable meteorological conditions such as shallow inversions over emission sources. Numerous studies have reported severe haze episodes in Delhi, often linking them to long-range transport of biomass burning aerosols from these upwind regions. In the present study, we investigate the variability in chemical composition of  non-refractory PM2.5 using a Time-of-Flight Aerosol Chemical Speciation Monitor (ToF-ACSM) and black carbon (BC) aerosols using an Aethalometer AE31 at an upwind side of Delhi-NCR in Sonipat, Haryana (28.9° N, 77.1° E) during the stubble burning period and Diwali time (25 Oct 2023 to 15 Nov 2023). We quantified the mass concentrations of biomass burning tracer species, such as levoglucosan, mannosan, and potassium (K+), along with other chemical constituents. The daily average concentrations of levoglucosan, mannosan and K+ in NR-PM2.5 were 1.28 ± 1.27, 0.02 ± 0.01 and 5.38±4.57 μg m−3, respectively. Preliminary analysis indicates higher concentration of biomass burning tracers, carbonaceous aerosols, and secondary inorganic aerosols during nighttime as compared to daytime. The daily average mass concentrations of Organics are 108±48.5 and 70.2±49.7 μg m−3, and BC are 18.8±86.0 μg m−3 and 24.0±10.2 μg m−3 during biomass burning and Diwali festival period, respectively. Additionally, we are conducting source apportionment analysis using models such as Positive Matrix Factorization (PMF) to identify various sources contributing to PM2.5 concentrations over the region. More results with greater details will be presented.

How to cite: Singh, V., Ganguly, D., Rathore, J., Dey, S., and Gani, S.: Chemical Characterization and source apportionment of PM2.5 over an upwind site of Delhi during Biomass Burning and Diwali Festival period , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-853, https://doi.org/10.5194/egusphere-egu25-853, 2025.

EGU25-2937 | Posters on site | AS3.3

Influence of Salting Out and Organic Nitrogen on Mixed Amino Acid Aerosol Cloud-Nucleating Ability 

Nahin Ferdousi-Rokib, Kotiba A. Malek, Kanishk Gohil, Kiran R. Pitta, Dabrina D. Dutcher, Timothy M. Raymond, Miriam A. Freedman, and Akua A. Asa-Awuku

Aerosols are present as complex organic-inorganic mixtures within our atmosphere, resulting in particles presenting phase separated morphology. Mixed organic-inorganic aerosols can be predominantly found in nascent sea spray aerosols (SSA). When these aerosols are exposed to supersaturated conditions (>100% RH), the water uptake ability of the aerosols vary based on the composition of the mixture. Previous studies have characterized phase separated systems through the determination of an average oxygen to carbon (O/C) ratio where liquid-liquid phase separation (LLPS) reaches its limit. The hygroscopicity of complex mixtures presenting LLPS was previously studied through the measurement of CCN activity within a 2-methylglutaric (2-MGA)/ammonium sulfate (AS) binary system and a 2-MGA/AS/sucrose ternary system; both studies correlated water-uptake abilities to O/C and surface tension. However, little is known about the influence of solubility of the third component on phase separation of a ternary mixture containing 2-MGA/AS. Additionally, the water-uptake properties of mixtures containing nitrogen containing compounds, such as amino acids, are not well defined. Amino acids are a major component of SSA and can contribute to aerosol hygroscopicity. Therefore, it is undetermined if O/C alone is an acceptable parameter for the estimation of solubility and hygroscopicity of complex amino acid mixtures. To improve our understanding of LLPS within aerosol mixtures and factors influencing its presence, three ternary systems were studied – a leucine system (2-MGA/AS/leucine), valine system (2-MGA/AS/valine), and proline system (2-MGA/AS/proline). For each system, the CCN activity of mixture compositions with varying O/C ratios and compositions was measured using a Cloud Condensation Nuclei Counter (CCNC) at 0.375% to 1.667% SS. For all mixtures, the single hygroscopic parameter κ was calculated. Experimental κ-results demonstrated increased hygroscopic activity as the amino acid became more soluble in the order of leucine<valine<proline. Experimental κ results were compared against four theoretical models; three of the theoretical models included were Köhler theory, O/C LLPS with surface tension (O/C LLPS-ST) and a newly developed model, X/C LLPS with surface tension (X/C LLPS-ST). For this study, a new parameter considering O/C and nitrogen to carbon (N/C) X/C, was introduced as a parameterization for solubility. The O/C LLPS-ST model was adapted to consider X/C for subsequent estimations of κ. A fourth theoretical model took a weighted average of the O/C LLPS-ST and X/C LLPS-ST models. The study provides an improved understanding of amino acid aerosol mixtures’ water uptake abilities through the introduction of a new parameter and model. As a result, the study is able to show varied N/C contribution to the system based on the structure of the amino acid as well as a method to improve current abilities to predict hygroscopicity of these complex, nitrogen-containing aerosol mixtures.

How to cite: Ferdousi-Rokib, N., Malek, K. A., Gohil, K., Pitta, K. R., Dutcher, D. D., Raymond, T. M., Freedman, M. A., and Asa-Awuku, A. A.: Influence of Salting Out and Organic Nitrogen on Mixed Amino Acid Aerosol Cloud-Nucleating Ability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2937, https://doi.org/10.5194/egusphere-egu25-2937, 2025.

EGU25-3242 | ECS | Orals | AS3.3

Global impacts of organic aerosol phase state 

Yumin Li and Colette Heald

Organic aerosol (OA) in the atmosphere can exist in liquid, semi-solid, or solid states, influenced by molecular properties and environmental conditions. However, regional and global models typically assume OA to be only in a liquid phase. Recent studies underscore that OA can present in a semi-solid or even solid state in low-temperature, dry environments. Under such conditions, increased viscosity can impede heterogeneous reaction rates by reducing diffusion. We develop a novel phase state scheme within the GEOS-Chem global model, enabling real-time simulation of OA phase states from various sources under diverse environmental conditions. Subsequently, we investigate the effects of OA phase states on heterogeneous chemical processes, including gas-particle partitioning, reactive uptake, and ice particle nucleation. Finally, our simulated OA concentrations are evaluated against global vertical profiles from aircraft observations. Our simulations indicate that on a global scale, viscosity is higher in polar regions compared to tropical regions and increases with altitude, with little to no liquid phase present above 500 hPa. Additionally, anthropogenic secondary OA (SOA) exhibits greater viscosity than biogenic SOA, hydrophobic primary OA (POA), and hydrophilic POA. The increased viscosity leads to slower gas-phase partitioning and uptake processes, thereby reducing near-source concentrations and increasing concentrations in remote areas. Considering solid-phase OA as heterogeneous ice nuclei enhances OA removal. Overall, our simulations demonstrate that incorporating phase state effect results in a reduction of OA concentrations, particularly for the more viscous SOA.

How to cite: Li, Y. and Heald, C.: Global impacts of organic aerosol phase state, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3242, https://doi.org/10.5194/egusphere-egu25-3242, 2025.

EGU25-3899 | Orals | AS3.3

Formation and aging of nitrogen-containing organic aerosol 

Ru-Jin Huang, Lu Yang, Wei Huang, and Yi Liu

Nitrogen-containing organic aerosol, consisting of nitroaromatics, N-heterocyclic compounds, and organic nitrates, are a group of key species in organic aerosol affecting aerosol optical properties and nitrogen cycle. The formation and aging of nitrogen-containing organic aerosol, however, are still not well understood hindering our understanding on their atmospheric evolution and impacts. In this study, nitrate-mediated photooxidation of some important nitroaromatics in atmospheric aqueous phase under different pH and temperature conditions were investigated. The dynamic changes in light absorption of nitroaromatics were measured, the photolysis rates and oxidation products as well as the aging processes were characterized. Besides nitroaromatics, the nighttime formation processes of secondary organic nitrates were investigated based on size-resolved measurements with a soot particle long-time-of-flight aerosol mass spectrometer. It was found that aqueous processing played an important role in the nighttime formation of particulate secondary organic nitrates in large size particles, especially in fog-rain days. In addition, N-heterocyclic compounds from aqueous-phase reaction of dicarbonyls with amines and ammonium under different pH were also studied. We identified for the first time 155 new N-heterocyclic compounds and their formation pathways were characterized.

How to cite: Huang, R.-J., Yang, L., Huang, W., and Liu, Y.: Formation and aging of nitrogen-containing organic aerosol, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3899, https://doi.org/10.5194/egusphere-egu25-3899, 2025.

EGU25-4424 | Posters on site | AS3.3

Integrating Observations and Model Simulations to Uncover Chemical and Physical Drivers of Organic Aerosol Composition in Urban Taiwan 

Feng Chen, Hui-Ming Hung, Ping-Wen Tsai, and Charles C.-K. Chou

This study investigates the composition, sources, and transformation processes of organic aerosols (OA) in Xitun, a near-industrial urban area in Taichung City, Taiwan, during a field measurement campaign in November 2023. Using a real-time Aerosol Mass Spectrometer (AMS) combined with Positive Matrix Factorization analysis, five organic aerosol components are identified: hydrocarbon-like OA (HOA), aged hydrocarbon-like OA (aged-HOA), semi-volatile oxygenated OA (SV-OOA), low-volatility oxygenated OA (LV-OOA), and background species. Oxygenated OA (OOA), primarily comprising secondary organic aerosol (SOA) formed through the oxidation of gas-phase precursors, accounted for 43–60% of the total OA mass, while HOA and aged-HOA, mainly derived from primary organic aerosol (POA) emitted by traffic and industrial sources, contributed approximately 30% of the total OA mass. To simulate OA evolution, a two-box model is developed, incorporating physical processes, including advection and entrainment, which are characterized using CO concentration simulations. The results align closely with those from the Community Multiscale Air Quality (CMAQ) model. With the physical processes well-constrained, the chemical processes are added to the model to quantify the chemical production and loss of selected volatile organic compounds (VOCs) and the formation of semi-volatile organic compounds (SVOCs) species, distinguishing between anthropogenic and biogenic VOC sources contributing to SOA formation. The oxidation rates of OA will be further determined through model simulations constrained by AMS observations. This study offers valuable insights into the sources, oxidation processes, and evolution of organic aerosols, providing a basis for comprehensive modeling approaches and enhancing our understanding of their impacts on air quality and human health.

How to cite: Chen, F., Hung, H.-M., Tsai, P.-W., and Chou, C. C.-K.: Integrating Observations and Model Simulations to Uncover Chemical and Physical Drivers of Organic Aerosol Composition in Urban Taiwan, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4424, https://doi.org/10.5194/egusphere-egu25-4424, 2025.

This study investigates the fluorescent properties of the water-soluble organic aerosol (WSOC) in PM2.5 and PM10 from the city of Karlsruhe, Germany. Major fluorescent components were identified by excitation–emission matrix spectroscopy with parallel factor analysis in this study. The lower humification index (HIX) value of PM2.5 and PM10 (0.72 ± 0.13, 0.77 ± 0.06), together with lower biological index (BIX) value of PM2.5 and PM10 (0.85 ± 0.07, 0.84 ± 0.06) and fluorescence index (FI) value of PM2.5 and PM10 (1.34 ± 0.16, 1.32 ± 0.06) showed that fluorescent source of WSOC influenced by the primary aerosol’s emissions (such as vehicles emission and heating) and natural dust (such as road and building contributions). The fluorescent components identified of the water-soluble organic aerosol show that Component 1 (Ex < 240/Ex = 323 nm, Em = 408 nm) and Component 2 (Ex = 248/362 nm, Em = 469 nm) can be identified as Highly oxygenated humic-like substance (HULIS) components. Component 3 (Ex <240 nm, Em = 363 nm) is associated with biomass burning with less-oxygenated HULIS component and Component 4 (Ex = 242/269 nm, Em = 311 nm) is substances from multiple sources of mixtures. Relative contribution of Highly oxygenated HULIS components (Component 1 & Component 2) in heating period (52.7%) is lower than in non-heating period (67.6%); Biomass burning with less-oxygenated HULIS component (Component 3) had the highest contribution (41%) in winter and the phenol- and naphthalene-like component (Component 4) had lower contributions and in different periods.

How to cite: Wang, X. and Norra, S.: Chemical composition and source identification of fluorescent components in water-soluble organic carbon in the city of Karlsruhe, Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5118, https://doi.org/10.5194/egusphere-egu25-5118, 2025.

EGU25-5301 | Posters on site | AS3.3

Volatility and Atomic Ratio of Aromatic Secondary Organic Aerosol: Effects of Aging and Alkyl Substituents 

Ho-Jin Lim, Jun-Hyun Park, Jooyong Lim, Atta Ullah, and Seonghyun Kim

Vaporization enthalpy (ΔHv) is an essential thermodynamic parameter that governs the phase transitions of organic compounds, linking their volatility to their temperature-dependent gas–particle partitioning. Secondary organic aerosol (SOA) was produced by the photooxidation of aromatic volatile organic compounds (VOCs) using a newly developed Teflon flow reactor. SOA volatility was assessed using a thermodenuder and parametrized using a kinetic mass transfer model. This study examined the effects of aging on the SOA volatility, chemical composition, and mass yield volatility. Variations in the ΔHv values of SOA driven from different aromatic VOCs were linked to the chemical structure of their aromatic precursors. Elevated hydroxyl exposures increased the oxygen to carbon ratio of SOA, while ΔHv remained relatively consistent, likely due to fragmentation offsetting the effects of increased oxidation. SOA yields were influenced by the degree of alkyl substitution and the chain length of alkyl substituents in the aromatic VOCs.

How to cite: Lim, H.-J., Park, J.-H., Lim, J., Ullah, A., and Kim, S.: Volatility and Atomic Ratio of Aromatic Secondary Organic Aerosol: Effects of Aging and Alkyl Substituents, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5301, https://doi.org/10.5194/egusphere-egu25-5301, 2025.

EGU25-5620 | ECS | Orals | AS3.3

Modeling the role of extremely low-volatile organic compounds in β-caryophyllene secondary organic aerosol formation 

Yijie Shi, Florian Couvidat, and Karine Kata-Sartelet

Sesquiterpene emitted from nature is the main precursor for secondary organic aerosol (SOA) formation. β-caryophyllene (BCA) is the most common sesquiterpene. Autoxidation of BCA oxidation products may lead to the rapid formation of extremely low-volatile organic compounds (ELVOCs), and it could be one of the dominant SOA formation pathways. However, until now the BCA SOA formation mechanisms are missing an autoxidation pathway. In this work, we develop a semi-explicit peroxy radical autoxidation mechanism for the production of ELVOCs from the oxidation of BCA with two major oxidants (O3 and NO3) under dark conditions and couple it to the Master Chemical Mechanism (MCMv3.3.1). Here, SOA originating from BCA is simulated under varying environmental conditions (temperature, humidity, and NOx levels) reported in several BCA chamber experiments. Simulations are performed with the SSH-Aerosol model accounting for multiphase chemistry, ELVOC nucleation, and condensation/evaporation. Our mechanism demonstrates a very good agreement between the modeled and observed SOA mass concentrations and size distribution.

How to cite: Shi, Y., Couvidat, F., and Kata-Sartelet, K.: Modeling the role of extremely low-volatile organic compounds in β-caryophyllene secondary organic aerosol formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5620, https://doi.org/10.5194/egusphere-egu25-5620, 2025.

EGU25-5677 | ECS | Posters on site | AS3.3

High-resolution, seasonal studies of carbon sources in atmospheric dust in Gliwice, using the radiocarbon method 

Alicja Ustrzycka, Natalia Piotrowska, Maksymilian Jędrzejowski, Marzena Kłusek, and Anna Mainka

From October 2024 to October 2025, the Gliwice Radiocarbon Laboratory is carrying out a project titled “High-resolution, seasonal studies of carbon sources in atmospheric dust using the radiocarbon method” (project number 2024/08/X/ST10/00655) funded by the National Science Centre (NCN).

The aim of the pilot study is to analyse radiocarbon concentration in atmospheric dust samples collected in Gliwice with weekly (autumn-winter) and two-week (spring-summer) resolution. Based on the results, we want to determine the seasonal contribution of different carbon emission sources.

Air pollution has a very negative impact on the human cardiorespiratory system including reducing resistance to bacterial or viral infections [1]. Particulate matter is a major contributor to overall air pollution. It consists of solid and liquid particles suspended in the atmosphere. Particularly dangerous are PM10, PM2.5 and PM1, which refers to particles smaller than 10 μm, 2.5 μm and 1 μm in diameter, respectively.

Gliwice (50°17′37.1′′ N 18°40′54.9′′ E) is located in southern Poland, within the Silesian Voivodeship in the industrial region of Upper Silesian conurbation. Upper Silesia is a densely populated and highly industrialized region of Poland. However, due to the high levels of air pollution, the Silesian region has the shortest life expectancy, as well as the highest rates of premature births and genetic birth defects in Poland [2].

Radiocarbon (14C) is one of three isotopes of carbon. It is the only one that undergoes radioactive decay (with a half-life of 5730 years), so its concentration in organic matter is closely related to its decay time. Burning fuels releases two types of carbon into the air: modern carbon (from burning biomass) and fossil carbon (from burning fossil fuels). Fossil fuels were formed from organic matter millions of years ago, so the concentration of radiocarbon in them is much lower than in biomass.

One of the methods used to determine the concentration of 14C is Accelerator Mass Spectrometry (AMS). Accelerator mass spectrometry is a highly sensitive method for counting carbon atoms and may be precise method of identifying carbon sources in atmospheric PM [3].

[1] M. Urrutia-Pereira, C. A. Mello-da-Silva, and D. Solé, COVID-19 and air pollution: A dangerous association?, Allergologia et Immunopathologia, vol. 48, no. 5, pp. 496–499, 2020, doi: 10.1016/j.aller.2020.05.004.

[2] E. Brągoszewska and A. Mainka, Impact of Different Air Pollutants (PM10, PM2.5, NO2, and Bacterial Aerosols) on COVID-19 Cases in Gliwice, Southern Poland, IJERPH, vol. 19, no. 21, p. 14181, 2022, doi: 10.3390/ijerph192114181.

[3] G. Zhang, J. Liu, J. Li, P. Li, N. Wei, and B. Xu, Radiocarbon isotope technique as apowerful tool in tracking anthropogenic emissions of carbonaceous air pollutants and greenhouse gases: A review, Fundamental Research, vol. 1, no. 3, pp. 306–316, 2021, doi: 10.1016/j.fmre.2021.03.007.

How to cite: Ustrzycka, A., Piotrowska, N., Jędrzejowski, M., Kłusek, M., and Mainka, A.: High-resolution, seasonal studies of carbon sources in atmospheric dust in Gliwice, using the radiocarbon method, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5677, https://doi.org/10.5194/egusphere-egu25-5677, 2025.

EGU25-8441 | Orals | AS3.3

Understanding the sources and formation of organic aerosol in Delhi using non-target analysis  

Jacqueline Hamilton, Daniel Bryant, Andrew Rickard, Beth Nelson, Will Drysdale, James Hopkins, James Lee, James Cash, Ben Langford, Eiko Nemitz, Shivani Shivani, and Ranu Gadi

Exposure to PM2.5 is the leading environmental risk to healthin India, where the National Capital Territory of  Delhi experiences annual mean concentrations of ~110 μg m-3. During the post-monsoon season, severe air pollution events are frequent, with extreme levels exceeding 1000 µg  m−3. A large fraction of PM2.5 in Delhi is organic aerosol (OA) derived from a wide range of primary and secondary sources. Recent studies investigating the composition and sources of OA in Delhi using online aerosol mass spectrometry (AMS), followed by positive matrix factorisation have highlighted the dominance of primary sources over secondary production during the very polluted post monsoon period. These studies suggest the resolved traffic and burning-related sources were the largest contributors, however, significant oxidised organic aerosol is present across most of the year, and the dominant sources of this material cannot be resolved using this approach.

 

High-resolution mass spectrometry (HRMS) allows detailed investigation of the molecular complexity of OA composition. Previous studies have focussed on key tracers of specific OA sources such as biomass burning or biogenic volatile organic compound oxidation. However, targeted analysis reveals a biased and incomplete picture of the chemical composition which limits our ability to detect emerging pollutants. Here we harness recent advances in the analysis of complex environmental samples via non-target analysis (NTA), coupled with advanced suspect screening and a novel semi-quantification method to investigate the complex composition of OA within Old Delhi during the post-monsoon period of 2018. Using high time resolution filter sampling and an automated analysis workflow, the temporal evolution of the OA  could be studied. Hierarchical cluster analysis of this high resolution data identified six separate OA factors. Two factors peaked at night and were dominated by primary oxidised traffic and wood combustion emissions. The other four factors peaked during the day and could be linked to different types of secondary organic aerosol that peak under different oxidative and meteorological conditions. These species showed different temporal profiles to the oxidised factors, MO-OOA and LO-OOA, measured using AMS, providing novel insights into the sources and factors that control local SOA production in Delhi. This offline NTA approach provides complementary information to the online AMS observations, while only requiring the deployment of a filter sampler to the observation location.

How to cite: Hamilton, J., Bryant, D., Rickard, A., Nelson, B., Drysdale, W., Hopkins, J., Lee, J., Cash, J., Langford, B., Nemitz, E., Shivani, S., and Gadi, R.: Understanding the sources and formation of organic aerosol in Delhi using non-target analysis , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8441, https://doi.org/10.5194/egusphere-egu25-8441, 2025.

EGU25-9109 | ECS | Posters on site | AS3.3

Freezing atmospheric organic nucleation: A matrix isolation study 

Vincent Enders, Dennis F. Dinu, Hinrich Grothe, Maren Podewitz, Markus Tischberger, and Dominik Stolzenburg

New particle formation (NPF) is the largest source of atmospheric aerosols with respect to their number and has a large impact on the global climate and human health. During this process, low-volatility vapors form stable molecular clusters, which subsequently grow through the condensation of additional molecules. Inorganic acids such as sulfuric acid or iodic acid are often the main drivers of clustering. While organic molecules contribute significantly to the growth processes, it remains unclear at what stage they start to contribute to NPF, i.e., the exact clustering routes of organic or organic-inorganic mixtures are unknown. This is in part due to the fact that current state-of-the-art mass spectroscopic methods only provide compositional information and not information on the actual structure of the molecular clusters or the functionalization of the growing nanoparticles. However, ultimately, the interaction between functional groups defines the properties of the molecular clusters [1].

Here, we use matrix isolation Fourier transform infrared spectroscopy (MI-FTIR) as a new tool to investigate the formation of molecular clusters. It was previously demonstrated [2,3] that MI-FTIR is a reliable tool for studying small molecular clusters' structure. In the present work, we investigate organic precursor vapors, their oxidation products, and newly formed clusters as stabilized in inert noble-gas matrices. Due to cryogenic temperatures, rotational transitions are suppressed, making the identification of the cluster constituents and the molecular structure of the cluster easier compared to conventional gas-phase FTIR.

The current study focuses on NPF involving α-pinene, a monoterpene that is recognized to be rapidly convertible to extremely low volatile organic compounds (ELVOC). Spectra of α-pinene and first-order oxidation products from α-pinene, such as pinic and pinonic acid, isolated in noble gas matrices are presented. The infrared absorption bands are compared to calculations based on density functional theory (DFT), as specific bands can be associated with the presence of multimers in the matrix. This gives insights into potential cluster formation pathways and can be used to benchmark the most widely used DFT approaches with experimental data. Altogether, we demonstrate that our MI-FTIR setup provides a new approach to NPF studies, complementing mass spectrometry-based measurements.

References:

[1]: Stolzenburg, D. et al. Atmospheric nanoparticle growth. Rev. Mod. Phys. 95, 045002 (2023).

[2]: Köck, E.-M. et al. Alpha-Carbonic Acid Revisited: Carbonic Acid Monomethyl Ester as a Solid and its Conformational Isomerism in the Gas Phase Chem. Eur. J. 26, 285 (2020).

[3]: Dinu, D. F. et al. Increase of Radiative Forcing through Midinfrared Absorption by Stable CO 2 Dimers? J. Phys. Chem. A 126, 2966–2975 (2022).

How to cite: Enders, V., Dinu, D. F., Grothe, H., Podewitz, M., Tischberger, M., and Stolzenburg, D.: Freezing atmospheric organic nucleation: A matrix isolation study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9109, https://doi.org/10.5194/egusphere-egu25-9109, 2025.

The formation, degradation, and physical properties of organic aerosol (OA) constituents strongly depend on multiphase chemical kinetics. Gas-phase oxidation of OA precursors has been extensively investigated in recent decades. However, laboratory kinetic data on the aqueous-phase oxidation of the organics are scarce. As a result, the aging of organics in cloud droplets and deliquescent aerosols is commonly simplified in model simulations. In studies that aim to characterize the constituents and the phase state of organics specifically, this limitation may be overcome by introducing reactions based on structure-activity relationships (SAR). In models with sophisticated gas-phase oxidation and partitioning schemes, organics of various sizes and oxidation states are present in the condensed phase. Thus, an oxidation mechanism for hundreds of species needs to be constructed. However, manual mechanism development is time-consuming and error-prone. The use of new or updated SAR methods may lead to different dominant reaction routes, further increasing the required time investment. Alternatively, various SAR methods can be combined in a code framework in order to automatically generate self-contained mechanisms for a given list of compounds, within seconds. Updates of the SARs can be implemented in the underlying code framework.
In this study, we construct and apply a mechanism generator for the application in global model simulations. It focuses on the chemical processing in aqueous media such as cloud droplets and deliquescent aerosols. The generator is developed in conjunction with the MESSy model. As a result, the output of the generator is fined-tuned to be used with the MESSy submodels. However, mechanisms can be generated without MESSy by user input of molecule structures. This feature is intended to simplify the wide range application of the generator results. Molecular structure input is given by SMILES strings and output can be generated in either SMILES or InChI-Key format. Currently, the generator is restricted to a predefined set of input molecule types. This is due to the limitations of the available SARs. The generator considers the following reaction types: 1) OH-oxidation 2) photolysis 3) hydrolysis of nitrates and 4) peroxy-radical reactions. Minor reaction pathways are neglected to minimize the effect of the new chemistry on model performance.
An aqueous-phase mechanism for the most water-soluble organics has been generated and used to simulate aerosol and cloud chemistry within MESSy. Test simulations with the expanded aqueous-phase mechanism revealed a change in the distribution of aerosol constituents. The results suggest that in aerosols larger organics are efficiently degraded and the average molecular size of organics is smaller. However, the change in aerosol mass by outgassing of organics is less pronounced than expected. The mechanism generator does not construct phase-partitioning "reactions" as the respective constants are missing. Thus, in the generated mechanism solely compounds that have a predefined partitioning may outgas. Consequently, future developments will focus on the estimation of partitioning constants upon generation of a novel molecule. In general, the range of application of the generator may be extended for further reactions.

How to cite: Wieser, F. and Taraborrelli, D.: Mechanism generation for aqueous-phase oxidation of organics: development and application for global model simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9174, https://doi.org/10.5194/egusphere-egu25-9174, 2025.

EGU25-9180 | Posters on site | AS3.3

Modelling aerosol chamber experiments with kinetic gas-to-particle partitioning of organic molecules under humid conditions 

Duong H. Do, Astrid Kerkweg, and Domenico Taraborrelli

The partitioning of organic vapors between the gas and the condensed phase is a crucial process influencing the formation of organic aerosol (OA). Investigating the key factors affecting  partitioning is quite challenging because of the disparate range and variability of atmospheric conditions (temperature, relative humidity, precursors etc.). Therefore, the combination of chamber experiments and chemical box models allows for investigating a specific OA formation via gas-aerosol partitioning under controlled experimental conditions. On this basis, we have developed a novel multiphase chemical box model, the so-called MESSy DWARF, to simulate chamber experiments. MESSy DWARF is part of the MESSy (Modular Earth Submodel System) modeling framework. This allows the box model to utilize the full range of process parameterizations  available in MESSy, which originally have been designed for global atmospheric chemistry simulations. 

Here, we present a MESSy DWARF application to simulate a chamber experiment for studying gas-to-particle partitioning of organic molecules under humid conditions. The kinetic partitioning scheme is based on the Schwartz mass transfer coefficient and is governed by the liquid water content (LWC) and water solubility. Losses of organic vapors to the walls have been included. To assess the kinetic partitioning of the model, we selected an experiment of alpha-pinene photooxidation with the presence of ammonium sulfate seeds at 50 % relative humidity. This experiment was conducted in SAPHIR-STAR, an indoor continuous glass tank chamber at Forschungszentrum Jülich. The model simulations emphasize the significance of LWC for organic aerosol concentration. Thus, the model has been expanded to include capabilities for estimating LWC from aerosol number counts and inorganic mass concentrations and the wet radius. LWC is calculated as the difference between the average wet and dry volumes of the particles. The volume of dry particles is estimated by use of either densities or grow factors of solute components.

The analysis of the model results indicates a correlation between NO-levels and water solubility of alpha-pinene oxidation products. As the level of NO decreases, the reaction pathways of the organic peroxy radicals shift towards the production of species bearing carboxyl and hydro(pero)xyl functional groups. The enhanced production of water-soluble products is consistent with the observed increase in organic mass at low NO. The preliminary success in simulating the multiphase chamber experiment indicates the potential for further model applications.

How to cite: Do, D. H., Kerkweg, A., and Taraborrelli, D.: Modelling aerosol chamber experiments with kinetic gas-to-particle partitioning of organic molecules under humid conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9180, https://doi.org/10.5194/egusphere-egu25-9180, 2025.

EGU25-9506 | Orals | AS3.3

Oxygenated organic molecules (OOMs) in the megacities of east China 

Wei Nie, Yuliang Liu, Chao Yan, and Aijun Ding

Oxygenated organic molecules (OOMs) are critical intermediates connecting the oxidation of volatile organic compounds (VOCs) and the formation of secondary organic aerosol (SOA). However, directly measuring these intermediate vapors presents significant challenges, particularly in megacity areas, due to their exceedingly low concentrations and complex compositional diversity. Since 2018, we have been monitoring OOMs at the SORPES station in Nanjing, eastern China, using a nitrate-CI-APi-ToF. To manage and simplify the complex mass spectra, we employed both binPMF and sub-range binPMF techniques prior to peak fitting, successfully identifying over 2,000 distinct OOM molecules with high accuracy. We also developed a framework to identify probable precursors of the detected OOMs. Our findings indicate that the oxidation of anthropogenic VOCs primarily drives OOM formation across most seasons, contributing approximately 40% each from aromatic compounds and aliphatic hydrocarbons, mainly alkanes. During summer, however, the oxidation of biogenic VOCs significantly contributes OOM production. The irreversible condensation of these OOMs substantially contributes to the growth of newly formed particles and the generation of SOA, particularly under warmer season and highly polluted conditions.

How to cite: Nie, W., Liu, Y., Yan, C., and Ding, A.: Oxygenated organic molecules (OOMs) in the megacities of east China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9506, https://doi.org/10.5194/egusphere-egu25-9506, 2025.

EGU25-10433 | ECS | Posters on site | AS3.3

Causes of the unremitting high ambient levels of PM10 in a suburban background site in NE Spain 

Anna Canals-Angerri, Marta Via, Rosa Lara, Andrés Alastuey, Maria Cruz Minguillón, Marco Pandolfi, Barend L. van Drooge, and Xavier Querol

Atmospheric PM10 and benzo(a)pyrene (BaP) concentrations in Manlleu (NE Spain) have remained high from 2008–2023, frequently exceeding EU limit/target values, and reaching BaP levels up to six times higher than urban averages in Spain. Furthermore, PM speciation campaigns were carried out in 2013, 2014-2015, 2016-2017 and 2021-2022. Chemical mass closure for autumn-winter showed a consistent PM10 composition for the different PM speciation campaigns, comprising 46–53% organic matter (OM), 18–26% secondary inorganic aerosol (SIA), 13–23% mineral matter (MM), and 5-9% elemental carbon (EC). Trend analysis revealed very light decrease and constant concentrations for PM10 and BaP, respectively over the study period, emphasizing the need for compliance with current and forthcoming EU air quality directives, the last aiming to halve PM10 limit values. Source apportionment of samples of the sporadic campaigns identified biomass burning (BB, 17.5 µg m-3, 48%) and MM and industry (16.3 µg m-3, 44%) as the main autumn-winter PM10 contributors, with high SIA concentrations attributed to several factors, including high ammonia (NH3) emissions. Local topography and meteorological conditions contribute to aggravate PM10 pollution. While metal concentrations have decreased since 2013, suggesting reduced industrial emissions, persistently high OM and EC concentrations indicate ongoing issues with BB emissions from domestic, commercial, and agricultural sources. Online analysis of black carbon (BC) and non-refractory PM1 components during winter 2016–2017 confirmed domestic and commercial BB as the primary sources of the BB contributions. These findings highlight the need of the implementation of more effective measures in reducing BB and agricultural/farming NH3 emissions. This study highlights the relevance of these issues for similar towns, the probable unremitting problem over the last decade, and the necessity of enhanced monitoring in small cities and policy actions to meet air quality standards under the new EU directive.

How to cite: Canals-Angerri, A., Via, M., Lara, R., Alastuey, A., Minguillón, M. C., Pandolfi, M., van Drooge, B. L., and Querol, X.: Causes of the unremitting high ambient levels of PM10 in a suburban background site in NE Spain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10433, https://doi.org/10.5194/egusphere-egu25-10433, 2025.

EGU25-10922 | Orals | AS3.3 | Highlight

Occurrence of a “forever chemical” in the atmosphere above pristine Amazon Forest 

Ivan Kourtchev, Bruna G. Sebben, Sebastian Brill, Cybelli, G.G. Barbosa, Bettina Weber, Rosaria R. Ferreira, Flávio Augusto Farias D'Oliveira, Cléo Q. Dias-Junior, Olalekan A.M. Popoola, Jonathan Williams, Christopher Pöhlker, and Ricardo H.M. Godoi

Per- and polyfluoroalkyl substances (PFAS), often referred to as "forever chemicals", are a class of man-made, extremely stable chemicals, which are widely used in industrial and commercial applications. Exposure to some PFAS is now known to be detrimental to human health. By virtue of PFAS long residence times, they are widely detected in the environment, including remote locations such as the Arctics, where the origin of the PFAS is poorly understood. It has been suggested that PFAS may be transported through contaminated waters, leading to accumulation in coastal areas, where they can be aerosolised via sea spray, thereby extending their geographical distribution far beyond their original source regions. The aim of this work is to investigate, for the first time, whether "forever chemicals" could be transported to areas considered to be pristine, far from coastal sites. This study was performed at the Amazonian Tall Tower Observatory (ATTO), a unique remote site situated in the middle of the Amazon rainforest, where a restricted PFAS, perfluorooctanoic acid (PFOA), was observed with concentrations reaching up to 2 pg/m3. A clear trend of increasing concentration with sampling height was observed and air masses from the south over Manaus had the highest concentrations. Atmospheric lifetime estimations, removal mechanisms supported by measurements at two heights (320 and 42 m above the rainforest), and concentration spikes indicated a long-range transport of PFOA to pristine Amazon rainforest. Potential sources, including industrial activities in urban areas, were explored, and historical fire management practices considered. This research presents the first measurements of PFAS in the atmosphere of Amazon rainforest. Remarkably, even in this remote natural environment, appreciable levels of PFAS can be detected. This study provides valuable insights into the long-range transport of the anthropogenic "forever chemical" into a remote natural ecosystem and should raise awareness of potential environmental implications.

 

How to cite: Kourtchev, I., Sebben, B. G., Brill, S., Barbosa, C. G. G., Weber, B., Ferreira, R. R., D'Oliveira, F. A. F., Dias-Junior, C. Q., Popoola, O. A. M., Williams, J., Pöhlker, C., and Godoi, R. H. M.: Occurrence of a “forever chemical” in the atmosphere above pristine Amazon Forest, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10922, https://doi.org/10.5194/egusphere-egu25-10922, 2025.

EGU25-11178 | ECS | Posters on site | AS3.3

Synthesis and Characterization of Organic Peroxides from Monoterpene-derived Secondary Organic Aerosol 

Kangwei Li, Zhensen Zheng, Julian Resch, and Markus Kalberer

Organic peroxides are health-relevant organic components in secondary organic aerosols (SOA), which is also a major compound class substantially contributing to SOA mass. However, their molecular identification and characterization in SOA is highly challenging and uncertain. Ozonolysis of alkenes is known to produce reactive intermediates ─ stabilized Criegee intermediates, and their subsequent bimolecular reactions with various carboxylic acids can form α-acyloxyalkyl hydroperoxides (AAHPs), which is considered a major class of organic peroxides in SOA. Here we use this knowledge to synthesize a number of atmospherically relevant AAHPs through liquid-phase ozonolysis from either α-pinene or 3-carene in the presence of ten different carboxylic acids. These AAHPs with diverse structures are identified individually by liquid chromatography coupled with high-resolution mass spectrometry (LC-HRMS). AAHPs were previously thought to decompose quickly in aqueous environment such as cloud droplets, but we demonstrate here that AAHPs hydrolysis rates are highly compound-dependent with rate constants differing by 2 orders of magnitude. Some synthesized AAHPs were further identified via targeted analysis in monoterpene SOA samples collected from laboratory flowtube experiments.

Another focus of this study is to expand the molecular identification ability of organic peroxides in SOA, which goes beyond peroxide standards. Iodide is known to selectively react with peroxides, and their kinetics are fundamentally determined by the structures of individual peroxides. We extrapolate this knowledge and develop a novel analytical strategy for molecular characterization of organic peroxides in SOA via iodometry kinetic experiments using LC-HRMS. Through non-targeted analysis, more than 300 organic peroxides are identified in α-pinene SOA with unprecedented accuracy of their chemical formula. Their reactivity with iodide is highly compound-dependent and can vary 4 orders of magnitude. Our study improves the molecular-level identification and understanding of organic peroxides in SOA, offering numerous opportunities for further investigation into their formation chemistry, atmospheric transformation, and health impact.

How to cite: Li, K., Zheng, Z., Resch, J., and Kalberer, M.: Synthesis and Characterization of Organic Peroxides from Monoterpene-derived Secondary Organic Aerosol, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11178, https://doi.org/10.5194/egusphere-egu25-11178, 2025.

EGU25-11510 | ECS | Orals | AS3.3

Non-target screening ice-core analysis reveals changes in the atmospheric organic aerosol composition between the pre-industrial and industrial periods 

Francois Burgay, Daniil Salionov, Thomas Singer, Anja Eichler, Sabina Brutsch, Theo Jenk, Alexander Vogel, Tatyana Papina, Sasa Bjelic, and Margit Schwikowski

Organic aerosols constitute up to 90% of submicron aerosol mass, playing a crucial role in influencing the Earth’s radiative forcing by absorbing and scattering incoming solar radiation, as well as acting as cloud condensation nuclei. To unravel the complexity of organic aerosol (OA) chemical composition, recent analytical advances, such as high-resolution mass spectrometry and the development of non-target screening (NTS) workflows, have been applied to present-day atmospheric aerosol samples. However, for a better understanding on how human activities have influenced OA chemistry, it is essential to unravel its changes between the pre-industrial and industrial periods.

In this study, we present the first application of a novel NTS method to an ice core from the Belukha glacier (Russian Federation), covering the period from 1800 to 1980 CE. A total of 398 molecules were identified, mainly secondary organic aerosol tracers (SOA), such as mono- and di-carboxylic acids. Since the 1950s, we observed a shift in the atmospheric aerosol composition, characterized by the appearance of organic molecules—such as nitrogen-containing compounds—that result from increased atmospheric reactions with anthropogenic NOx or direct emissions. Additionally, we recorded a significant increase in the oxygen-to-carbon ratio (+3%) and the average carbon oxidation state (+18%) of the detected compounds compared to the pre-industrial period, suggesting an increased oxidative capacity of the atmosphere, associated with enhanced tropospheric ozone concentrations.

This work demonstrates the potential of NTS ice-core studies for extending the reconstruction of OA chemical composition prior to the advent of direct instrumental monitoring, providing valuable contributions to the atmospheric aerosol community. 

How to cite: Burgay, F., Salionov, D., Singer, T., Eichler, A., Brutsch, S., Jenk, T., Vogel, A., Papina, T., Bjelic, S., and Schwikowski, M.: Non-target screening ice-core analysis reveals changes in the atmospheric organic aerosol composition between the pre-industrial and industrial periods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11510, https://doi.org/10.5194/egusphere-egu25-11510, 2025.

EGU25-11592 | ECS | Orals | AS3.3

Decadal Trends in Atmospheric Aerosols: Insights into PM1 Composition, Seasonal Variability, and Source Apportionment in Central Europe 

Samira Atabakhsh, Laurent Poulain, Alessandro Bigi, Martine Collaud Coen, Mira Pöhlker, and Hartmut Herrmann

Particulate matter (PM) is a major climate-forcing agent and significantly impacts air quality. To grasp how environmental policies and climate change impact atmospheric aerosols, long-term measurements are vital, especially for organic aerosol (OA) and black carbon (BC). OA represents a large portion of aerosol mass, while BC has the strongest direct radiative forcing effect. State-of-the-art equipment like the Aerosol Chemical Speciation Monitor (ACSM) and the Multi-Angle Absorption Photometer (MAAP) help to identify OA and BC sources, respectively. Since 2012, an ACSM and a MAAP have operated at the ACTRIS-TROPOS research station in Melpitz, Germany, enabling a decade-long study of aerosol composition and OA sources for PM1 from September 2012 to August 2022.

To analyse these trends, a rolling Positive Matrix Factorization (PMF) approach was applied and implemented in SoFi Pro software (Datalystica Ltd., Villigen, Switzerland). The Melpitz station's strategic location allows for the study of particle composition changes typical of both Western and Eastern Europe (Spindler et al., 2010). This improves our understanding of emissions and the effects of air quality regulations on PM1 chemical species in these regions. The results reveal high PM1 mass concentrations were associated with eastern air masses across all meteorological seasons. However, the relative contributions of individual chemical components varied depending on the season and the origin of the air mass. Expanding on Atabakhsh et al. (2023) work, which analyzed a 12-month dataset, this study identified five OA factors: three associated with primary organic sources—hydrocarbon-like OA (HOA), biomass burning OA (BBOA), and coal combustion OA (CCOA)—and two oxygenated OA factors—more-oxidized OOA (MO-OOA) and less-oxidized OOA (LO-OOA). Trend analysis using a pre-whitening method (Collaud Coen et al., 2020) revealed a statistically significant annual decrease of -4.59% y-1 in total PM1 mass over the decade, driven by decreases in nitrate (-1.10% y-1) and equivalent BC (eBC) (-1.3% y-1) concentrations. However, HOA showed a minor decline (-0.25% y-1) under eastern air masses, BBOA increased by +0.94% y-1 during summer, and CCOA showed a modest increase (+0.27% y-1) in western air masses. The OOA factors showed declining trends in eastern air masses (-1.52% and -1.09% y-1), indicating improvements in the emissions of secondary aerosol precursors.

This study provides a comprehensive analysis of seasonal variability, source apportionment, and trends of PM1 components in Central Europe. It highlights differences in air masses from Eastern and Western Europe, providing insights into regional air quality regulations and sources of atmospheric aerosols.

References:

Atabakhsh, S., et al. (2023) Atmospheric Chem. Phys., 842.

Collaud Coen, et al. (2020) Atmos. Meas. Tech., 178.

Spindler, G., et al. (2010) Atmos. Environ., 44, 164-173

How to cite: Atabakhsh, S., Poulain, L., Bigi, A., Collaud Coen, M., Pöhlker, M., and Herrmann, H.: Decadal Trends in Atmospheric Aerosols: Insights into PM1 Composition, Seasonal Variability, and Source Apportionment in Central Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11592, https://doi.org/10.5194/egusphere-egu25-11592, 2025.

EGU25-12699 | ECS | Orals | AS3.3

Insufficient mass spectrometric detection of synthesized hydroperoxy acids from α-pinene ozonolysis 

Markus Tischberger, Maximilian Kaiser, Hinrich Grothe, Marco Lair, Melanie Opacak, David Schachamayr, and Dominik Stolzenburg

Alpha-pinene is one of the most studied precursor molecules for new particle formation (NPF). It was shown that RO2 radicals formed by α-pinene ozonolysis can undergo autoxidation to rapidly form highly oxygenated molecules (HOMs) (Bianchi et al, 2019). These HOMs are hypothesized to often contain hydroperoxide (C-O-O-H) functionalization. As the functionalization of molecules influences their vapor pressure, it is an important factor when modeling the formation and growth of new aerosol particles (Stolzenburg et al, 2022).

Authentic standards of α-pinene derived HOMs are sparse. While some research groups have achieved the synthesis of HOM-dimers (see, e.g., Kenseth et al, 2023), monomeric HOM compounds with the significant hydroperoxide functionalization are still not available commercially (Mettke et al, 2022). There is an urgent need to investigate the detection of these compounds in the widely used chemical ionization mass spectrometers, as their charging efficiencies remain largely unknown (Alage et al, 2024).

In this work, we report the synthesis of two α-pinene derived molecules containing hydroperoxy-acid (C(O)-O-O-H) groups, verified by H- and C-NMR techniques. We characterized the synthesized standards using an Orbitrap mass spectrometer with electrospray ionization and NO3- based chemical ionization at atmospheric pressure. We demonstrate that both ionization methods result in much higher signals of the corresponding carboxylic acids. This indicates a rapid destruction of the hydroperoxy acids during the ionization process.

Our results imply that HOMs formed via the autoxidation of α-pinene might often not be correctly quantified with different mass spectrometric techniques. As especially the chemical ionization using NO3- is widely used in atmospheric studies related to NPF, this could result in huge discrepancies when atmospheric process rates (such as nucleation and growth rates of newly formed particles) are derived from gas-phase measurements.

References:

Alage, S. et al (2024), Atmos. Meas. Techn., 17(15), 4709-4724, https://doi.org/10.5194/amt-17-4709-2024

Bianchi, F. et al (2019), Chem. Rev., 119(6), 3472–3509, https://doi.org/10.1021/acs.chemrev.8b00395

Kenseth, C. M. et al (2023), Science, 382(6672), 787-792, https://doi.org/10.1126/science.adi0857

Mettke, P. et al (2022), Atmosphere, 13(4), 507, https://doi.org/10.3390/atmos13040507

Stolzenburg, D. et al (2022), J. Aerosol Sci., 166, 106063, https://doi.org/10.1016/j.jaerosci.2022.106063

How to cite: Tischberger, M., Kaiser, M., Grothe, H., Lair, M., Opacak, M., Schachamayr, D., and Stolzenburg, D.: Insufficient mass spectrometric detection of synthesized hydroperoxy acids from α-pinene ozonolysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12699, https://doi.org/10.5194/egusphere-egu25-12699, 2025.

EGU25-13005 | ECS | Orals | AS3.3

Oxygenated Organic Molecules in Newly Formed Biogenic Particles: Molecular Structures and Formation Pathways 

Vignesh Vasudevan-Geetha, Lee Tiszenkel, Robin Russo, Daniel Bryant, and Shan-Hu Lee

Oxygenated organic molecules (OOMs) formed from oxidation of anthropogenic and volatile organic compounds VOCs are essential ingredients for atmospheric new particle formation (NPF) and secondary organic aerosol formation. There is a large variety of OOM compounds, but currently, for the vast majority of OOMs, their molecular structures and formation pathways are largely unknown. Here, we made detailed chemical analysis of gas- and aerosol-phase OOMs produced from a-pinene ozonolysis,  using a high-resolution time-of-flight chemical ionization mass spectrometer (HrTOF-CIMS) attached to the filter inlet for gas and aerosol (FIGAERO), as well as an ultrahigh-performance liquid chromatography-electrospray ionization Orbitrap mass spectrometer (UPLC/(-)ESI-Orbitrap MS). Based on LC and MS/MS fragmentation ions, we identified isomer molecular structures and chemical formation pathways. For C19H30O5, one isomer forms in the particle phase via aldol condensation, whereas another isomer forms via esterification. Two isomers of C16H26O6 form via decarboxylation from different C17H26O8 isomers. Thus, our experimental results with detailed chemical speciation show that OOM NPF precursors also form in the particle phase. Currently, parameterizations for the growth of newly formed particles are based on the gas-to-particle conversion of low-volatility OOMs formed in the gas phase. Our study demonstrates that particle-phase formation pathways of OOMs should also be considered for the growth of new particles in the atmosphere.

How to cite: Vasudevan-Geetha, V., Tiszenkel, L., Russo, R., Bryant, D., and Lee, S.-H.: Oxygenated Organic Molecules in Newly Formed Biogenic Particles: Molecular Structures and Formation Pathways, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13005, https://doi.org/10.5194/egusphere-egu25-13005, 2025.

EGU25-13194 | ECS | Posters on site | AS3.3

Formaldehyde as a SOA Indicator: Regional and Temporal Variability 

Fiona Román de Miguel, Nick Schutgens, and Qirui Zhong

Formaldehyde, a short-lived species, is used as an indicator of secondary organic aerosol (SOA) formation due to its involvement in the chemical reactions that produce SOA. While formaldehyde is emitted during fires, observed concentrations in regions like the Amazon are often too high to be explained solely by combustion, suggesting additional sources. Previous research has shown that during the 2010 fire season in the Amazon, SOA was found to account for 52% of total organic aerosol (OA) emissions, highlighting the importance of SOA in the region's aerosol budget.

In this study, we extend this previous work by analyzing satellite observations of formaldehyde, aerosol optical depth (AOD), and single scattering albedo (SSA) across multiple years. We examine whether higher formaldehyde concentrations, indicative of more active SOA formation, continue to correlate with higher AOD and SSA, suggesting increased SOA mass and the presence of non-absorbing aerosols.

Also, we investigate whether these relationships hold in other regions, such as Southern Africa, where SOA contributions to OA emissions were found to be lower. Additionally, we explore the temporal variability of the formaldehyde-AOD-SSA correlation, assessing whether these associations are consistent across different fire seasons and years. This analysis aims to uncover potential temporal trends in SOA formation dynamics and better understand the regional and inter-annual variability of these relationships.

How to cite: Román de Miguel, F., Schutgens, N., and Zhong, Q.: Formaldehyde as a SOA Indicator: Regional and Temporal Variability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13194, https://doi.org/10.5194/egusphere-egu25-13194, 2025.

EGU25-13516 | ECS | Orals | AS3.3

Understanding the Importance of the H-Abstraction Channel in HOM Formation from OH Oxidation of α-pinene 

Hui Wang, Hongru Shen, Yarê Baker, Rongrong Wu, Sungah Kang, Annika Zanders, Defeng Zhao, Sören R. Zorn, and Thomas F. Mentel

Secondary organic aerosols (SOA) can affect global climate change and air quality. Explaining the formation of highly oxygenated organic molecules (HOM) is important due to their vital role in SOA formation. α-pinene as the most abundant monoterpene can react rapidly with oxidants (e.g. OH radicals and O3) and peroxy radicals (RO2) undergo fast unimolecular reactions to form HOM. For the reaction with the important daytime hydroxyl radical, previous studies (Shen et al., 2022; Luo et al., 2023) have shown that the H-abstraction pathway, which initially appears to be a minor reaction channel (~10%), contributes significantly to the HOM formation during the early stages of monoterpene oxidation reactions. However, the importance of the H-abstraction channel under different environmentally relevant conditions is unknown.

Our study focused on the OH oxidation reactions of a-pinene under different NOx and OH exposure conditions. The experiments were conducted in the Jülich Saphir STAR (Stirred atmospheric tank Reactor) chamber. The photolysis of hydrogen peroxide was used as OH source to ensure pure OH radical reactions without interference of ozone reactions. A multi-scheme chemical ionization inlet (MION) was coupled to an APi-Long-TOF-MS to characterize HOM. An increased mass fraction of H-abstraction pathway-related HOM (C10H15Ox and C10H15NOx) were observed among all HOM containing 10 C-atoms, with 0.7% at NO levels of ~0 ppb, 6% at 0.03 ppb NO, 22% at 1.0 ppb NO, and 31% at 2.2 ppb NO. Time series of these H-abstraction related HOM show a fast increase within the first minute after initiating reactions, which corresponds to direct formation from H-abstraction instead of secondary oxidation of accumulated pinonaldehyde. This could be explained by accelerated formation of alkoxy radicals promoted by RO2 radicals and NO reactions. Similar results were observed under OH exposure ranging from 1×106 to 1.3×107 molecule cm-3. Our study here shows the importance of the H-abstraction channel for the formation of HOM from OH oxidation of a-pinene, further emphasizing the role of NOx.

  Luo, H., Vereecken, L., Shen, H., Kang, S., Pullinen, I., Hallquist, M., Fuchs, H., Wahner, A., Kiendler-Scharr, A., Mentel, T. F., and Zhao, D.: Formation of highly oxygenated organic molecules from the oxidation of limonene by OH radical: significant contribution of H-abstraction pathway, Atmospheric Chemistry and Physics, 23, 7297-7319, 10.5194/acp-23-7297-2023, 2023.

  Shen, H. A.-O., Vereecken, L. A.-O. X., Kang, S. A.-O., Pullinen, I. A.-O., Fuchs, H. A.-O., Zhao, D. A.-O., and Mentel, T. A.-O.: Unexpected significance of a minor reaction pathway in daytime formation of biogenic highly oxygenated organic compounds, 2022.

 

How to cite: Wang, H., Shen, H., Baker, Y., Wu, R., Kang, S., Zanders, A., Zhao, D., Zorn, S. R., and Mentel, T. F.: Understanding the Importance of the H-Abstraction Channel in HOM Formation from OH Oxidation of α-pinene, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13516, https://doi.org/10.5194/egusphere-egu25-13516, 2025.

EGU25-14134 | ECS | Orals | AS3.3

Photochemical Aging Enhances the Viscosity of Biomass Burning Organic Aerosol 

Nealan Gerrebos, Lyle Browning, Sepehr Nikkho, Julia Zaks, Changda Wu, and Allan Bertram

Biomass burning organic aerosols (BBOA) are a major contributor to organic aerosols in the atmosphere. Viscosity is an important property of BBOA, as it influences many of the processes it is involved in in the atmosphere; this includes but is not limited to particle growth rates, reaction and mixing rates, and cloud condensation nucleation. As BBOA is transported through the troposphere, it undergoes photochemical aging due to reactions with atmospheric oxidants such as OH and O3. Recently it has been shown that the viscosities of some aerosols can be enhanced through atmospheric aging processes. However, research on the influence of atmospheric aging on BBOA is still limited.We used a Potential Aerosol Mass oxidative flow reactor (185 nm mode) to expose BBOA to high concentrations of OH and O3, simulating the equivalent of 1 to 8 days in the troposphere.  We measured the viscosity of the photochemically aged BBOA with the poke-flow viscometry technique, and found that aging increased the viscosity of BBOA. After 1 day of aging, the viscosity of BBOA increased by several orders of magnitude. However, further aging up to 8 days saw a less dramatic increase in viscosity, with no noticeable increase between 5 days and 8 days. We also measured the carbon oxidation state of the BBOA with high-resolution aerosol mass spectrometry, and the trend in increasing oxidation state reflected the trend in viscosity. This suggests that the most dramatic changes in the physicochemical properties of BBOA occur within the first days or hours of aging, after which oxidation becomes a less significant aging mechanism. These results have implications for how the aging and eventual fate of BBOA should be treated in models. 

How to cite: Gerrebos, N., Browning, L., Nikkho, S., Zaks, J., Wu, C., and Bertram, A.: Photochemical Aging Enhances the Viscosity of Biomass Burning Organic Aerosol, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14134, https://doi.org/10.5194/egusphere-egu25-14134, 2025.

EGU25-14487 | ECS | Posters on site | AS3.3

Spatial distribution and Source Apportionment of Organic Nitrogen in PM2.5 over Northeast Asia 

Ju Young Kim, Xu Yu, Jian Zhen Yu, Yong Pyo Kim, and Ji Yi Lee

Nitrogen-containing compounds constitute up to 77% of the molecular species in organic aerosols (OA), contributing approximately 40% to the total OA mass. Despite this significant abundance, research on characterizing organic nitrogen (ON) in particulate matter with an aerodynamic diameter of 2.5 micrometers or less (PM2.5) has predominantly focused on water-soluble ON (WSON) or specific subgroups due to the complexity of ON and challenges in identifying its diverse sources. Beyond its abundance, ON plays an essential role in new particle formation, secondary organic aerosol (SOA) formation, and serves as a major atmospheric source of reactive nitrogen, potentially disrupting the global nitrogen cycle.
This study aimed to investigate the spatial distribution and source apportionment of ON in PM2.5 across four sites in Northeast Asia. PM2.5 samples were collected daily for one month in the fall of 2023 from Ulaanbaatar (Mongolia), Beijing (China), Seoul, and Seosan (South Korea). ON concentrations were measured using a simultaneous ON and inorganic nitrogen (IN) detection system, consisting of a thermal aerosol carbon analyzer and a chemiluminescence NOx analyzer (Yu et al., 2021). The average concentrations were 0.35 ± 0.17 μgN/m³ in Ulaanbaatar, 0.22 ± 0.12 μgN/m³ in Beijing, 0.20 ± 0.08 μgN/m³ in Seoul, and 0.28 ± 0.10 μgN/m³ in Seosan, corresponding to 39 ± 15%, 21 ± 15%, 23 ± 12%, and 23 ± 11% of total aerosol nitrogen in PM2.5, respectively. The correlation analysis of water-soluble organic carbon (WSOC) and water-insoluble organic carbon (WISOC) in PM2.5 with ON showed that in Ulaanbaatar ON correlated well only with WISOC, in Seoul only with WSOC, and in Beijing and Seosan with both WSOC and WISOC. The correlation analysis between IN and ON revealed the strongest relationship in Beijing, followed by Seoul, Seosan, and Ulaanbaatar. Since IN generally originates from secondary formation, the strong ON-IN correlation suggests that they may largely share common formation pathways or precursors, or that IN indirectly facilitates ON formation by providing reactive precursors through photochemical processes. Overall, it can be inferred that primary emissions, such as coal combustion, are the main source of ON in Ulaanbaatar, resulting in water-insoluble, lipid-like characteristics. In Seoul, ON likely originates from a combination of primary emissions and secondary formation. In Beijing, secondary formation, particularly IN-associated chemical reactions, appears to be the dominant source. In Seosan, primary emissions, particularly those linked to WSOC, such as biomass burning, are the primary contributors.

                                    

Acknowledgement

This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute (KEITI) funded by the Ministry of Environment (MOE).

 

References

Yu, X., Li, Q., Ge, Y., Li, Y., Liao, K., & Huang, X. H. (2021). Environmental Science & Technology, 55(17), 11579–11589.

How to cite: Kim, J. Y., Yu, X., Yu, J. Z., Kim, Y. P., and Lee, J. Y.: Spatial distribution and Source Apportionment of Organic Nitrogen in PM2.5 over Northeast Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14487, https://doi.org/10.5194/egusphere-egu25-14487, 2025.

EGU25-14850 | Posters on site | AS3.3

Explicit simulation of chemical composition, size distribution and cloud condensation nuclei of the secondary organic aerosol from α-pinene oxidation 

Zhen Song, Chenqi Zhang, Hongru Shen, Thomas Mentel, and Defeng Zhao

Secondary organic aerosol (SOA), formed by oxidation of volatile organic compounds and gas-particle partitioning, account for a large proportion of atmospheric submicron aerosol mass, and hence have a significant impact on clouds and global climate. The impact depends on the concentration and the cloud condensation nuclei (CCN) activity of SOA. CCN activity of SOA is determined by its particle size and hygroscopicity parameter (κ) characterizing the properties of different chemical composition. Despite a number of chamber studies on SOA formation and its CCN activity, few studies have simulated particle size and chemical composition of SOA and thus CCN concentration based on explicit chemical mechanism. To bridge this gap, in this study we used the box model PyCHAM to explicitly simulate the α-pinene ozonolysis reaction in an atmospheric reaction chamber, and compared the simulated SOA mass and number concentrations, chemical composition, particle size distribution, κ and CCN concentration with experimental measurements. In general, the simulation underestimated SOA mass concentration  and overestimated oxygen-to-carbon (O:C) and hydrogen-to-carbon (H:C), indicating the potential role of particle-phase reactions in SOA formation. The simulated SOA number concentration, particle nucleation and subsequent growth agreed well with measurement, whereas the geometric mean diameter was slightly overestimated, which partly due to the simplified microphysical processes like coagulation in the model. Moreover, the simulated κ and CCN concentration were also in consistent with measurements. This study reveals the key chemical processes that may influence SOA formation, as well as the importance of considering detailed chemical composition and particle size distribution for CCN simulations based on the explicit chemical mechanism.

How to cite: Song, Z., Zhang, C., Shen, H., Mentel, T., and Zhao, D.: Explicit simulation of chemical composition, size distribution and cloud condensation nuclei of the secondary organic aerosol from α-pinene oxidation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14850, https://doi.org/10.5194/egusphere-egu25-14850, 2025.

EGU25-15491 | ECS | Posters on site | AS3.3

Nonlinear Formation of Secondary Organic Aerosol from Biogenic VOC Mixtures 

Jianhuai Ye, Yanchen Li, Yiming Qin, Yifang Gu, Xiaoyu Hu, Yaying Wang, and Baohua Cai

Secondary organic aerosol (SOA) plays a significant role in air quality, climate, and human health. SOA produced from the oxidation of biogenic volatile organic compounds (VOCs) in the presence of reactive nitrogen species constitutes a major fraction of ambient organic aerosol. This study investigates the nonlinear effects of mixed biogenic VOC systems, including monoterpenes and sesquiterpenes, on the yield, chemical composition, and volatility of SOA. Smog chamber experiments show that SOA yields for mixtures are reduced compared to single-component systems, likely due to interactions among C10 and C15 RO2 radicals. High-resolution mass spectrometry identifies unique chemical species specific to the mixed-component system, while volatility analysis reveals that sesquiterpene-derived compounds and monoterpene-sesquiterpene cross-reaction products dominate. Model simulations using the Master Chemical Mechanism reveal substantial discrepancies between predicted and experimentally observed SOA yields and volatility. These findings highlight the complexity of SOA formation from VOC mixtures, emphasizing the need to incorporate nonlinear precursor interactions into atmospheric chemistry and air quality models.

How to cite: Ye, J., Li, Y., Qin, Y., Gu, Y., Hu, X., Wang, Y., and Cai, B.: Nonlinear Formation of Secondary Organic Aerosol from Biogenic VOC Mixtures, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15491, https://doi.org/10.5194/egusphere-egu25-15491, 2025.

EGU25-15702 | ECS | Orals | AS3.3

Seasonal analysis of organic aerosol composition resolves anthropogenic and biogenic sources at a rural background station in central Europe 

Markus Thoma, Franziska Bachmeier, Karina Knauf, Julia David, Mario Simon, and Alexander Lucas Vogel

Introduction

Fine particulate matter (PM2.5) has a major impact on the climate1 and can affect human health.2 Though the major fraction of submicron PM is from organic compounds,3 their sources or organic precursor vapours, their atmospheric oxidation mechanisms and cross-reactions with inorganic trace gases remain unknown and are the focus of ongoing research. Volatile organic compounds of biogenic and anthropogenic origin can be oxidised in the atmosphere.4 The oxidation leads to a higher functionality, which reduces the volatility of the products, hence gas-to-particle conversion contributes to the formation of secondary organic aerosol (SOA) particles.2

 

Methods

From August 2021 to August 2022, we sampled PM2.5 glass fiber filters with a high-volume sampler for 12 hours at a rural background monitoring station. We measured the sample extracts in full scan MS with data dependent tandem mass spectrometry on a high-resolution hybrid quadrupole-Orbitrap mass spectrometer (Q Exactive Focus). Analytes were ionized with a heated electrospray ionisation source. For separation we used a ultra-high-performance liquid chromatography (Vanquish Flex) on a reversed phase column. To identify known and unknown compounds we used non-target analysis (Compound Discoverer 3.3), implementing fragmentation spectra search with mzCloud and the aerosolomics database. Hierarchical cluster analysis (HCA) and concentration-weighted trajectories (CWT) supports the interpretation of the results.   

 

Results

The HCA groups the 6,080 detected compounds into two main clusters. Based on the chemical composition we interpret the compounds therein as of biogenic and anthropogenic origin. Sample clustering shows a clear seasonal cycle of the SOA mass and its chemical composition. During summer the SOA is dominated by biogenic compounds indicating a strong local influence of the vegetation. Anthropogenic compounds are relatively enriched during colder conditions with strong transport of air pollution during singular events. CWT show the air mass origins of these pollution events and allow for an interpretation of potential sources such as coal-fired power plants in eastern Germany and eastern Europe during stable, warm and dry weather conditions in Europe.

Our top-down approach could be valuable for understanding the variability and complexity of SOA processes and origins, helping to estimate anthropogenic influences on SOA formation, and thus for validating the anthropogenic aerosol forcing in Earth system models.

 

Literature

  • 1. Shrivastava, M. et al. Recent advances in understanding secondary organic aerosol: Implications for global climate forcing. Rev. Geophys. 55, 509–559 (2017).
  • 2. Fan, W. et al. A review of secondary organic aerosols formation focusing on organosulfates and organic nitrates. Journal of Hazardous Materials 430, 128406 (2022).
  • 3. Jimenez, J. L. et al. Evolution of Organic Aerosols in the Atmosphere. Science 326, 1525–1529 (2009).
  • 4. Atkinson, R. & Arey, J. Atmospheric Degradation of Volatile Organic Compounds. Chem. Rev. 103, 4605–4638 (2003).

 

How to cite: Thoma, M., Bachmeier, F., Knauf, K., David, J., Simon, M., and Vogel, A. L.: Seasonal analysis of organic aerosol composition resolves anthropogenic and biogenic sources at a rural background station in central Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15702, https://doi.org/10.5194/egusphere-egu25-15702, 2025.

EGU25-16078 | Orals | AS3.3

Aerosol Cloud Interactions in a Nitrogen-dominated Atmosphere (CAINA) – first highlights from AIDA cloud chamber studies  

Ulrike Dusek, Jinglan Fu, Harald Saathoff, Willem Kroese, Rupert Holzinger, Juliane Fry, and Hengjia Ou and the the CAINA team

The goal of the CAINA project is to investigate multiple aspects of aerosol-cloud interactions under high concentrations of reactive nitrogen. The CAINA project is a consortium project (7 PhD students) that combines in-situ and remote sensing observations of aerosols and clouds with high-resolution modeling to study the formation of CCN, cloud chemistry, and aerosol effects on clouds under high reactive nitrogen concentrations. This is chemical regime is starting to emerge in many regions on the globe following the strong reduction of SO2 emissions and consequently particulate sulfate concentrations. The presentation will give a short overview of the whole CAINA project and focus mainly on the results from 2 campaigns that were conducted at the AIDA cloud chamber to study the formation of aqueous SOA (AqSOA) under high reactive nitrogen concentrations.

The CAINA-AIDA campaigns are among the first experiments that investigate the influence of inorganic compounds on AqSOA formation under atmospherically relevant conditions, as opposed to more common bulk solution and flow-tube experiments. Seed aerosol consisting of inorganic salts (NaCl, NH4NO3, (NH4)2SO4) were nebulized as aqueous solution into the 84.5 m3 AIDA chamber at 90% RH. Subsequently, secondary organic aerosol (SOA) was generated from various precursors (a-pinene, limonene, isoprene) to study aqSOA formation for several hours under dark and irradiated conditions, followed by a cloud activation of ~ 8 min. The chemical composition of the organic gas and particle phase were characterized by high-resolution mass spectrometry, using both Iodide-CIMS and PTR-MS based techniques.

First results show that SOA mass yields are strongly enhanced at 90% RH compared to dry conditions, e.g. for a factor of more than 3 for the a-pinene experiments. This coincides with changes in chemical mass spectra, which are drastic for isoprene and more moderate for a-pinene. In the case of a-pinene, considerably higher concentrations of dicarboxylic acids and water-soluble oxidation products, such as DTAA, can be observed at 90% compared to dry conditions. At 90% RH the chemical composition of the SOA depends more strongly on the type of inorganic seed particle than at dry conditions. Particularly, nitrogen containing compounds as well as oxalic and malonic acid concentrations are clearly enhanced in NH4NO3 containing solutions compared to NaCl. A control experiment using NaCl seeds, where NH3 and NOx were added in the gas phase, gives a first indication that some of these compounds are preferentially formed in the liquid phase, but others in the gas phase with subsequent partitioning into the liquid phase. The effects of UV illumination and subsequent cloud activation on SOA composition will be also be presented.

How to cite: Dusek, U., Fu, J., Saathoff, H., Kroese, W., Holzinger, R., Fry, J., and Ou, H. and the the CAINA team: Aerosol Cloud Interactions in a Nitrogen-dominated Atmosphere (CAINA) – first highlights from AIDA cloud chamber studies , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16078, https://doi.org/10.5194/egusphere-egu25-16078, 2025.

EGU25-16087 | Orals | AS3.3

Isoprene nitrates drive new particle formation in Amazon’s upper troposphere 

Martin Heinritzi, Lisa Beck, Sarah Richter, Marcel Zauner-Wieczorek, Lianet Hernández Pardo, Thomas Klimach, Konstantinos Barmpounis, Nidhi Tripathi, Akima Ringsdorf, Philip Holzbeck, Clara Nussbaumer, Hartwig Harder, Jonathan Williams, Horst Fischer, Christopher Pöhlker, Anna Possner, Mira Pöhlker, Ulrich Pöschl, Jos Lelieveld, and Joachim Curtius

For several decades intense new particle formation (NPF) events have been observed by aircraft measurements in the upper tropical troposphere (UTT) (Brock et al. 1995, Weigel et al. 2011, Williamson et al. 2019). These events typically occur above 8 km altitude in the outflow of mesoscale convective systems. The resulting particles can grow further and be transported downwards where they enhance cloud condensation nuclei (CCN) levels over large geographic areas in the tropics. However, the chemical mechanism driving these events remained unclear, as no direct measurements of the involved low-volatility gaseous precursors were possible.

Here, we present in-situ aircraft observations taken on board the High Altitude LOng Range (HALO) aircraft (operated by the German Aerospace Center, DLR) over the Amazon rainforest with the goal of deciphering the chemical mechanism behind NPF in the UTT. The measurements were taken during the CAFE Brazil campaign in December 2022/January 2023, where HALO was stationed in Manaus, Brazil. The aircraft was equipped with a comprehensive suite of instruments measuring both gas- and particle-phase properties. To detect low volatility organic compounds, we operated a purpose-built nitrate Chemical Ionization Mass spectrometer (CIMS).

We show that isoprene nitrates drive new particle formation after sunrise in the upper tropospheric outflow of mesoscale convective systems (Curtius et al. 2024). Isoprene (C5H8) is carried from the boundary layer to high altitudes within deep convective cells, while NOx is produced in these cells via lightning. After sunrise, oxidation of isoprene by OH is initiated, as well as photolytic conversion of NO2 to NO, which leads to the formation of second generation isoprene nitrates. At the cold temperatures in the upper tropical troposphere (around -60 °C) these molecules have sufficiently low saturation vapour pressure to drive strong new particle formation events, leading to several tens of thousands of particles per cubic centimetre. We find that this process happens frequently over the Amazon at high altitude (>8 km) and might have far reaching consequences for tropical aerosol and CCN production.

We also compare our results with recent findings from the CLOUD experiment (Shen et al. 2024), which studied the capability of isoprene to nucleate at low temperature conditions and find good agreement between field and laboratory measurements.

 

 

 

References:

Brock C. A., et al. (1995), Science, 270, 1650-1653

Weigel, R, et al. (2011), Atmos. Chem. Phys., 11, 9983-10010

Williamson, C. J., et al. (2019). Nature, 574(7778), 399-403.

Curtius, J, et al. (2024). Nature, 636(8041), 124-130.

Shen, J, et al. (2024). Nature, 636(8041), 115-123.

How to cite: Heinritzi, M., Beck, L., Richter, S., Zauner-Wieczorek, M., Hernández Pardo, L., Klimach, T., Barmpounis, K., Tripathi, N., Ringsdorf, A., Holzbeck, P., Nussbaumer, C., Harder, H., Williams, J., Fischer, H., Pöhlker, C., Possner, A., Pöhlker, M., Pöschl, U., Lelieveld, J., and Curtius, J.: Isoprene nitrates drive new particle formation in Amazon’s upper troposphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16087, https://doi.org/10.5194/egusphere-egu25-16087, 2025.

EGU25-17091 | ECS | Posters on site | AS3.3

Characterization of cooking aerosol through an ensemble of measurements targeting chemical composition, physical properties and oxidative potential. 

Iasonas Stavroulas, Jesus Yus-Diez, Marta Via, Kristina Glojek, Luka Drinovec, Manousos Ioannis Manousakas, André Prévôt, and Griša Močnik

Cooking, one of key human activities, has been known to contribute significantly to ambient aerosol in both the indoor and outdoor settings. In certain urban environments, cooking Organic Aerosol (OA) have been documented to drive outstanding smog events. On the other hand, more research is necessary on induced health effects by such aerosol. A controlled, cooking and grilling experiment was performed in June 2024 in an effort to physically and chemically characterize cooking aerosol and derive estimations on their oxidative potential. Along the way, the response of the Aerosol Chemical Speciation Monitor (ACSM) to direct cooking emissions was assessed, while reference single source mass spectra were acquired, to be used as an important aid for constraining algorithms performing source apportionment of ambient aerosol. Various cooking conditions (gas vs charcoal grill, frying pan) were tested on different types of food (vegetables, steaks, burgers, chicken, fish, fries, etc). The experimental setup included an ACSM, a 7-wavelength filter-based absorption photometer (AE-33 aethalometer), a Scanning Mobility Particle Sizer (SMPS) providing number size distributions and filter sampling of PM2.5 aerosol to perform off line detailed composition analysis and oxidative potential estimates.

                Acquired OA mass spectra presented similarities, being dominated by prominent signals at m/z = 41, 43, 55 and 57, linked to the fragmentation of alkyls and specifically the CnH2n+1 and CnH2n-1 ion series. All cooking spectra acquired, share the common feature of an m/z = 55 over m/z = 57 contribution ratio (i.e. f55/f57) well above unity. The contribution of significant signal at m/z = 60, a typical tracer of the fragmentation of levoglucosan, related to the pyrolysis of cellulose was evident in the mass spectra of charcoal grilled food. Interestingly non negligible, nevertheless low contributions at m/z = 60, were also found for food cooked on a gas burner grill. Grilling vegetables yields pronounced contributions at higher m/z values (e.g. for m/z =67, 69, and 71). The largest contribution at m/z = 44 in the mass spectrum, was observed when sampling aerosol from burning the residual fat from a heated pan.

Acknowledgement: This work is supported by the European Union's Horizon Europe research and innovation programme under the Marie Skłodowska-Curie Postdoctoral Fellowship Programme, SMASH co-funded under the grant agreement No. 101081355. The SMASH project is co-funded by the Republic of Slovenia and the European Union from the European Regional Development Fund.

How to cite: Stavroulas, I., Yus-Diez, J., Via, M., Glojek, K., Drinovec, L., Manousakas, M. I., Prévôt, A., and Močnik, G.: Characterization of cooking aerosol through an ensemble of measurements targeting chemical composition, physical properties and oxidative potential., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17091, https://doi.org/10.5194/egusphere-egu25-17091, 2025.

EGU25-17234 | ECS | Posters on site | AS3.3

Distribution of jet engine oil emissions in the urban surroundings of Germany's largest airport 

Florian Ungeheuer, Dominik van Pinxteren, and Alexander L. Vogel

Numerous studies have identified airports as key sources of ultrafine particles (UFPs – aerodynamic diameter <100 nm) [1] [2] [3] [4], yet the chemical composition and formation mechanisms of these particles remain poorly understood. In a previous study we characterized the organic chemical composition of aviation-related UFPs by non-targeted screening and identified jet engine oils as a significant contributor [5]. Besides quantifying the mass contribution of jet oils to ambient UFPs originating from Frankfurt International Airport, we were able to show the new-particle formation ability of jet engine oils by laboratory based thermodenuder-experiments, using a common synthetic lubrication oil [6].

Here, we show the spatial distribution of jet engine oil emissions emerging from Frankfurt Airport, which is the largest airport in Germany.  We conducted a quantitative analysis of two different types of synthetic esters which are used as base stock in jet engine oils to monitor their prevalence in the region. Hence, we collected particles with diameters <100 nm at five different locations around the airport with varying distances to the airport grounds. We sampled UFPs on aluminium-filters using multiple 13-stage cascade impactor systems (Nano-MOUDI) in the direct vicinity of the airport runways and up to a distance of 20 km. Collection took place in summer and winter periods to observe a possible seasonal variability and at three stations in parallel to monitor the simultaneous spatial extent and wind direction dependence. In parallel to filter sampling, the particle size distribution was monitored to determine the size-resolved total particle mass. Quantitative characterization of UFPs in the size ranges 10–18 nm, 18–32 nm, 32–56 nm and 56-100 nm was performed by external calibration applying liquid chromatography (UHPLC) separation, followed by heated electrospray ionization (HESI) and mass analysis using a high-resolution Orbitrap mass spectrometer (HRMS). The two homologous ester series of pentaerythritol- (C25-40H44-74O8) and trimethylolpropane (C26-36H48-68O6) esters were quantified by external calibration using one ester compound (C29H52O8). Since different types of Nano-MOUDI samplers (NanoMOUDI Model 115; NanoMOUDI-II 122R & 125R) were in use, we compared their sampling efficiency for each stage in order to make later corrections. Over a period of two weeks, we collected parallel filter samples at the same station and compared the collected engine oil mass accordingly. Results indicate that aircraft engine oils are detectable across the full UFP size range, with the highest concentrations observed at airport grounds in the 32-56 nm particle size fraction. Sulfate concentrations show a similar picture regarding the size distribution. To accurately account for these variations in size fractions, it is crucial to consider the differing collection efficiencies as these can vary significantly depending on the sampler model and design.

[1] Habre, R., et al. (2018) Environ. Int., 118, 48–59.

[2] Fushimi, A., et al. (2019) Atmos. Chem. Phys., 19, 6389–6399.

[3] Stacey, B., (2019) Atmos. Environ., 198, 463–477.

[4] Rivas, I., et al. (2020) Environ. Int., 135, 105345.

[5] Ungeheuer, F., et al. (2021) Atmos. Chem. Phys., 21, 3763–3775.

[6] Ungeheuer, F., et al. (2022) Commun Earth Environ 3, 319.

How to cite: Ungeheuer, F., van Pinxteren, D., and L. Vogel, A.: Distribution of jet engine oil emissions in the urban surroundings of Germany's largest airport, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17234, https://doi.org/10.5194/egusphere-egu25-17234, 2025.

EGU25-17378 | ECS | Posters on site | AS3.3

Molecular representation of benzene SOA for 3D modelling  

Aurélien Le Bayon, Zhizhao Wang, Victor Lannuque, Florian Couvidat, Raluca Ciuraru, and Karine Sartelet

Aromatic compounds account for a significant proportion of anthropogenic volatile organic compounds emissions, and their atmospheric ageing is a key driver of the formation and growth of organic aerosols. In this study, the benzene oxidation scheme extracted from the Master Chemical Mechanism (MCM) 3.3.1 was revised and improved by the implementation of several new oxidation pathways, including multigeneration oxidation, peroxy radical rearrangement, formation of di-bridged species and autoxidation. These updates lead to the formation of various compounds that can partition into organic and aqueous aerosol phases. Comparisons to chamber experiments of benzene and phenol oxidation show that the addition of these pathways provides a better representation of the formation (aerosol mass yields) and chemical composition of secondary organic aerosols.

While near-explicit schemes provide greater details, their computational complexity makes them difficult to directly implement in chemistry-transport models. To address this, the near-explicit scheme of benzene is reduced using the GENerator of Reduced Organic Aerosol Mechanisms (GENOA) algorithm under representative atmospheric conditions. Using reduction strategies and evaluation criteria, GENOA trains and reduces the SOA mechanism under atmospheric conditions commonly encountered over Europe. The trained benzene SOA mechanism preserves the main characteristic of the near-explicit mechanism (e.g., chemical pathways, molecular structures of crucial compounds, the effect of non-ideality and hydrophilic/hydrophobic partitioning of aerosols), with a size (in terms of reaction and species numbers) that is manageable for three-dimensional aerosol modelling (e.g., regional chemical transport models).

How to cite: Le Bayon, A., Wang, Z., Lannuque, V., Couvidat, F., Ciuraru, R., and Sartelet, K.: Molecular representation of benzene SOA for 3D modelling , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17378, https://doi.org/10.5194/egusphere-egu25-17378, 2025.

EGU25-17649 | Orals | AS3.3

Volatility of molecular components of aPinene SOA modulated by inorganic seed composition 

David Bell, Natasha Garner, Jens Top, Jun Zhang, Francesca Salteri, Andre Prevot, Katherine Kolozsvari, Andrew Ault, Sabine Lüchtrath, Markus Ammann, and Imad El Haddad

The effective saturation vapor concentration (Log C*eff) of a molecule represents an important variable that governs the ability of molecule to nucleate new particles and partition into pre-existing aerosols. Thus, the saturation vapor concentration affects the chemical composition and the mass yields of ambient aerosol, ultimately affecting air pollution and climate.1 The determination of saturation vapor concentration is straight forward for small molecules, and those readily synthesized. However, the oxidation of volatile organic compounds creates a complex mixture of molecules, which is not easily separated to determine their saturation vapor concentration. Furthermore, SOA can often be mixed with other particles, containing species such as inorganic salts (e.g., ammonium sulfate) or mineral dust, impacting the non-ideality of the aerosols.

 

A thermal denuder coupled to a scanning mobility particle sizer (TD-SMPS) has been employed to determine the saturation vapor concentration of single component systems.2 However, the lack of chemical resolution prevents its applicability to determine the saturation vapor concentration of more complex organic mixtures such SOA.3 Consequently, considerably uncertainties still exists regarding the saturation vapor concentration of ambient SOA components. To address this issue, here we deployed an extractive electrospray ionization mass spectrometer (EESI-MS) coupled with a TD-SMPS (hence TD-SMPS+EESI) to provide molecular formula separation of complex mixtures together with their saturation vapor concentrations.4 We performed measurements on a complex mixture of known species (PEG-300) to demonstrate the ability to extract the saturation vapor concentration. We have generated SOAs derived from the ozonolysis of α-pinene in an atmospheric simulation chamber to extract their C*eff’s under three conditions: without seeds present, with ammonium sulfate seeds, and with a mixed iron/ammonium sulfate seeds. The presence of seed modulates the extracted C*eff values from SOA samples, suggesting there are non-ideal interactions between the underlying seed. Further, the presence of iron in the seed significantly exacerbates these non-ideal interactions, which indicates that knowing the underlying seed composition is important for understanding C*eff.

References:

 

(1) Ciarelli, G.; Haddad, I. E.; Bruns, E.; Aksoyoglu, S.; Möhler, O.; Baltensperger, U.; Prévôt, A. S. H. Constraining a hybrid volatility basis-set model for aging of wood-burning emissions using smog chamber experiments: A box-model study based on the VBS scheme of the CAMx model (v5.40). Geosci. Model Dev. 2017, 10 (6), 2303-2320. DOI: 10.5194/gmd-10-2303-2017.

(2) Kostenidou, E.; Karnezi, E.; Kolodziejczyk, A.; Szmigielski, R.; Pandis, S. N. Physical and Chemical Properties of 3-Methyl-1,2,3-butanetricarboxylic Acid (MBTCA) Aerosol. Environmental Science & Technology 2018, 52 (3), 1150-1155. DOI: 10.1021/acs.est.7b04348.

(3) Cappa, C. D.; Wilson, K. R. Multi-generation gas-phase oxidation, equilibrium partitioning, and the formation and evolution of secondary organic aerosol. Atmos. Chem. Phys. 2012, 12 (20), 9505-9528. DOI: 10.5194/acp-12-9505-2012.

(4) Bell, D. M.; Zhang, J.; Top, J.; Bogler, S.; Surdu, M.; Slowik, J. G.; Prevot, A. S. H.; El Haddad, I. Sensitivity Constraints of Extractive Electrospray for a Model System and Secondary Organic Aerosol. Analytical Chemistry 2023, 95 (37), 13788-13795. DOI: 10.1021/acs.analchem.3c00441.

 

How to cite: Bell, D., Garner, N., Top, J., Zhang, J., Salteri, F., Prevot, A., Kolozsvari, K., Ault, A., Lüchtrath, S., Ammann, M., and El Haddad, I.: Volatility of molecular components of aPinene SOA modulated by inorganic seed composition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17649, https://doi.org/10.5194/egusphere-egu25-17649, 2025.

EGU25-18823 | ECS | Orals | AS3.3

Sensitivity of Cloud Microphysics to BVOC-Induced Aerosol Growth Over Boreal Forests 

Léo Faivre, Peter Tunved, Radovan Krejci, Paul Bowen, Tuukka Petäjä, Theodore Khadir, Daniel G. Partridge, and Liine Heikkinen

This study explores how the evolution of aerosol size distribution and chemical composition, driven by exposure to biogenic volatile organic compounds (BVOCs), influences cloud microphysics over the boreal forests of Southern Finland. Aerosol properties were derived from eight years of particle number size distribution (PNSD) and chemical composition measurements collected at the SMEAR II station. These data were categorized based on the time air masses spent traversing forested regions (Time Over Land, ToL), calculated using 97-hour HYSPLIT back trajectories. ToL was divided into 5-hour bins, and the median PNSD and aerosol composition for each bin were used to drive simulations with the PseudoAdiabatic bin-micRophySics University of Exeter Cloud parcel model (PARSEC).

The boreal forest emits biogenic volatile organic compounds (BVOCs) into the atmosphere, where these compounds undergo various oxidation processes. These reactions influence the growth and composition of atmospheric particles, ultimately contributing to the formation of secondary organic aerosols (SOA). Our simulation results show that with longer ToL, aerosols exhibit increased particle size and higher organic mass fractions. These changes significantly affect simulated cloud droplet activation and subsequent microphysical processes. PARSEC simulations revealed that the fraction of activated particles—cloud droplets relative to total aerosols—increases with both ToL and updraft velocity. However, for high ToL conditions (>3 days), the maximum supersaturation plateaus, particularly at stronger updraft velocities (>1 m/s), even as the activated fraction continues to increase. Moreover, once ToL exceeds one day, the albedo of clouds stabilizes rapidly, underscoring the importance of the initial 30-hour period in modulating the local climate.

While these observations provide insights into the coupling of aerosols and cloud properties, additional complexities remain. For instance, the impact of cloud droplet collisions, coalescence, and entrainment on cloud microphysics along ToL trajectories will be further discussed, highlighting their role in shaping cloud lifetime and albedo feedbacks.

By focusing on clean-sector air masses to minimize anthropogenic influences, this work underscores the critical interplay between BVOC-driven aerosol evolution and cloud microphysics. These findings emphasize the need to account for dynamic aerosol changes over boreal forests in climate models, particularly under conditions where BVOCs drive efficient SOA formation. Expanding our understanding of these interactions is essential for accurately representing the contribution of boreal forest ecosystems to local and regional climate systems.

How to cite: Faivre, L., Tunved, P., Krejci, R., Bowen, P., Petäjä, T., Khadir, T., Partridge, D. G., and Heikkinen, L.: Sensitivity of Cloud Microphysics to BVOC-Induced Aerosol Growth Over Boreal Forests, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18823, https://doi.org/10.5194/egusphere-egu25-18823, 2025.

EGU25-19500 | ECS | Posters on site | AS3.3

New particle formation from alpha pinene and trace sulfuric acid in the CERN CLOUD chamber 

Eva Sommer, Joao Almeida, Mario Simon, Lucìa Caudillo-Plath, Wenjuan Yu, Heikki Junninen, Zhensen Zheng, Bernhard Judmaier, Jiali Shen, Lubna Dada, and Jasper Kirkby and the CLOUD Collaboration

New particle formation (NPF) contributes to about half of all cloud condensation nuclei worldwide (Gordon et al. 2017) and plays a critical role in understanding anthropogenic climate change (IPCC, 2021). A keymechanism driving atmospheric NPF is acid-base nucleation, primarily involving anthropogenic sulfuric acid and ammonia (Kirkby, 2023). Nonetheless, oxygenated organic molecules (OOM), produced from oxidation of terpenes like alpha-pinene (Kirkby et al. 2016) or  – in the upper troposphere –  isoprene (Shen et al. 2024), can drive rapid particle nucleation in the complete absence of sulfuric acid, a process known as pure biogenic nucleation.

Shen et al. (2024) found that that the addition of trace amounts of sulfuric acid to isoprene-driven NPF enhanced the nucleation rates up to 100-fold. However, so far, a synergistic effect of sulfuric acid with alpha-pinene OOM (AP-OOM) has not been reported.

This study focuses on measurements from the CERN CLOUD chamber, examining NPF from alpha-pinene in the presence of trace sulfuric acid concentrations ranging from 104 to 106 cm−3, levels that are commonlyfound in pristine regions. Experiments were conducted at -10°C and +5°C, typical of the cool boundary layer of boreal forest regions, and in the absence of any base vapors such as ammonia or amines.

Gas-phase concentrations were monitored using various CI-Time-Of-Flight mass spectrometers (Nitrate-CIMS, Fusion PTR, STOF PTR-MS, FIGAERO), while naturally charged nucleating clusters were analyzed using an APi-TOF. Aerosol particle distributions were characterized with an array of particle measurement instruments (scanning PSM, CPC, NAIS, nSMPS, lSMPS, DMA-Train). Nucleation and growth rates were determined under varying concentrations of alpha-pinene OOMs and sulfuric acid.

This study presents nucleation and growth rates from AP-OOM in the presence of trace sulfuric acid and compares the rates with those from pure AP-OOM and pure sulfuric acid, respectively.

 

Gordon, H. et al. (2017) Causes and importance of new particle formation in the present-day and preindustrial atmospheres. J. Geophys. Res. Atmos. 122, 8739-8760.

IPCC (2021) Climate Change 2021 – The Physical Science Basis: Working Group I Contribution to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change. Cambridge University Press.

Kirkby, J. et al. (2016) Ion-induced nucleation of pure biogenic particles. Nature 533, 521-526.

Kirkby, J. et al. (2023) Atmospheric new particle formation from the CERN CLOUD experiment. Nature Geoscience 16, 948-957.

Shen, J. et al. (2024) "New particle formation from isoprene under upper-tropospheric conditions." Nature 636.8041, 115-123.

How to cite: Sommer, E., Almeida, J., Simon, M., Caudillo-Plath, L., Yu, W., Junninen, H., Zheng, Z., Judmaier, B., Shen, J., Dada, L., and Kirkby, J. and the CLOUD Collaboration: New particle formation from alpha pinene and trace sulfuric acid in the CERN CLOUD chamber, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19500, https://doi.org/10.5194/egusphere-egu25-19500, 2025.

EGU25-19513 | Posters on site | AS3.3

Bipolar FUSION PTR-TOF Mass Spectrometer: Advantages of Multiple Reagent Ions to Characterize Oxidation and Secondary Organic Aerosol Formation  

Markus Sebastian Leiminger, Andreas Klinger, Hannah Beckmann, Martin Graus, Tobias Reinecke, and Markus Müller

Aerosol particles significantly impact Earth’s climate, air quality, and human health. Secondary Organic aerosols (SOA) present a major fraction of the particulate mass in the troposphere. Due to the involved processes ranging from molecular to particle scales, SOA remains a complex topic with a continuing need of method and instrument development. 

Proton-transfer-reaction mass spectrometry (PTR-MS) is a well established technique for the characterization of SOA and its precursors. More advanced instruments like the recently introduced FUSION PTR-TOF feature positive selective reagent ions like H3O+ for quantitative measurements of the widest range of organic compounds or NH4+ for soft adduct ionization that enables the detection of highly oxidized compounds. Complemented by NO+ and O2+  ionization mode, this instrument covers the detection of the vast majority of organic and inorganic compounds. However, the measurement of certain inorganic compounds like SO2, H2SO4, other small inorganic acids and organic acids still poses a challenge utilizing only positive reagent ions.

To close this gap, the FUSION PTR-TOF was upgraded with bipolar electronics, enabling operation in negative ion mode using negative reagent ions such as CO3- which provides enhanced selectivity for acids and volatile inorganic compounds, including SO2, HNO3, H2SO4, and halogenated compounds.

In this work we focus on limonene, a monoterpene emitted by plants and widely used in consumer products. It is of particular interest due to its high aerosol yield and structural features like endocyclic and exocyclic double bonds, which influence its oxidation pathways. To study limonene oxidation and its contribution to SOA formation on a molecular level, a laminar flow oxidation reactor was set up. This reactor allows for a controlled oxidation of limonene with oxidants like OH or ozone with residence times of up to 15 min that is sufficient for SOA formation. Limonene and its volatile oxidation products were monitored in real-time with a FUSION PTR-TOF and the particle phase was measured with a CHARON particle inlet for a direct detection of SOA constituents. Based on these measurements we will highlight the benefits and limitations of complementary ionization modes of the new Bipolar FUSION PTR-TOF. CO3- proves to be highly selective to the formed acids and effectively captures products like pinonic acid with virtually no fragmentation significantly simplifying data interpretation. Sequentially ionizing with H3O+, NH4+, NO+, and CO3- primary reagent ion modes allows for capturing the complete picture of the formation process from precursor to SOA.

How to cite: Leiminger, M. S., Klinger, A., Beckmann, H., Graus, M., Reinecke, T., and Müller, M.: Bipolar FUSION PTR-TOF Mass Spectrometer: Advantages of Multiple Reagent Ions to Characterize Oxidation and Secondary Organic Aerosol Formation , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19513, https://doi.org/10.5194/egusphere-egu25-19513, 2025.

EGU25-19908 | ECS | Posters on site | AS3.3

Application example of a novel untargeted LC-UHRMS processing approach for the analysis of organic aerosols 

Niklas Karbach, Anna Breuninger, Alexander Vogel, and Thorsten Hoffmann

Atmospheric organic aerosol contains unique information about the origin, reaction regimes and the atmospheric conditions of the air mass that is sampled. Extracting the maximum amount of information from every sample can be a challenging task. Traditional targeted analysis of a few selected compounds is not up to the task. Therefore, untargeted analysis is becoming increasingly popular for analyzing complex atmospheric aerosol samples.

This poster presents an in-house developed specialized software that allows to analyze full-scan / AIF MS measurements that were previously too complex for direct human interpretation. In contrast to traditional measurements, this mode provides the maximum amount of information about the sample without any unnecessary restrictions, allowing to create digital databases of complete organic aerosol samples. With continuous improvement of the analysis program, this allows to utilize data of samples that were measured today to be used in the future for other projects and to be analyzed with different methods and programs. The custom software can convert such full-scan / AIF LC-UHRMS data into a human readable format and visualize the data in a comprehensive way. Utilizing this approach allows to capture the maximum amount of data in a single measurement reducing both manual labor and device utilization.

How to cite: Karbach, N., Breuninger, A., Vogel, A., and Hoffmann, T.: Application example of a novel untargeted LC-UHRMS processing approach for the analysis of organic aerosols, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19908, https://doi.org/10.5194/egusphere-egu25-19908, 2025.

Limonene is an abundant and highly reactive monoterpene that forms secondary organic aerosol (SOA) in the atmosphere. Limonene SOA from emerging anthropogenic sources, e.g., volatile chemical products, can deteriorate air quality in developed cities, yet the impacts may vary depending on its chemical properties. During the CHANEL campaign, atmospheric oxidation of limonene was simulated in the 270 m3 SAPHIR chamber to study the influence of reaction conditions and timescales on the molecular-level chemical composition of SOA. Different combinations of hydroxyl (OH.), nitrate (NO3.) and ozone (O3) oxidants were used in medium NOx for investigating day- and night-time oxidation conditions with each experiment spanning 10 – 12 hours. The SOA was transmitted from the chamber directly to an Ionicon CHARON-FUSION time-of-flight mass spectrometer that was operated in both H3O+ and ammonium (NH4+) modes with a periodic ion-switching measurement protocol. A positive matrix factorization approach was implemented via Source Finder (SoFi) to constrain the relative prominence of organic species in aerosol composition at different stages of each experiment. SOA evolved over several hours, yet with oxygenated species (CxHyOz) constituting 70 – 80% of the mass spectra that were dominated by compounds containing 5 – 10 carbon and 2 – 6 oxygen atoms. For daytime oxidation (OH+O3), C9H14O4 and C9H14O5 species were highly prominent in SOA formed immediately after the first precursor injection. The C9-species group also dominated peak SOA concentrations during night-time conditions. These were followed by O5 and O6-containing species that dominated the daytime tests after 4 – 5 hours of initial injection. After 7 – 8 hours, the molecular distribution looked considerably similar to that of SOA formed in O3-only oxidation tests with delayed appearance of C8H12O5 and C8H14O5 species that were likely multigenerational oxidation products. These observations suggest that properties of limonene SOA may continue to evolve over several hours following emissions and could influence their environmental impacts.

How to cite: Khare, P. and the CHANEL team: Detailed Molecular Characterization of Limonene Secondary Organic Aerosol Under Varying Oxidation Conditions and Reaction Timescales at the SAPHIR Chamber during CHANEL campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20142, https://doi.org/10.5194/egusphere-egu25-20142, 2025.

EGU25-372 | ECS | Posters on site | AS3.5

Continuous Detection of Pathogenic Bioaerosol Using Antibody Labelled Magnetic Beads and Flow Cytometry 

Pia Karbiener, Battist Utinger, and Markus Kalberer

Biogenic aerosols play a key role in various infectious diseases, like COVID-19 (virus) and Tuberculosis (bacteria). This fact makes detecting and characterizing bioaerosol, especially the pathogenic kind, crucial for human health. Traditional surveillance (via agar plates or PCR) of pathogenic bioaerosol is time and/or labor intensive. As staff in health-related sectors like hospitals is already limited, rapid and automated pathogenic bioaerosol monitoring is of dire need.

In this proof of concept study, we build and test a continuous pathogenic bioaerosol sampler and detector. The set-up consists of three main parts. In a first step (Collection phase), the bioaerosol is sampled via a particle into liquid sampler. This bioaerosol liquid flow is mixed continuously with antibodies for the relevant pathogen species, which are conjugated to magnetic nanobeads. From here the bioaerosol-antibody-bead flow is transported into a column, containing magnetic spheres. There the bioaerosol of interest is captured (Selection phase), stained and then released separately to be analyzed in a flow cytometer (Detection phase).

We are currently working to connect all three successfully tested phases into one continuous, automated, and autonomous instrument for pathogenic bioaerosol monitoring.

How to cite: Karbiener, P., Utinger, B., and Kalberer, M.: Continuous Detection of Pathogenic Bioaerosol Using Antibody Labelled Magnetic Beads and Flow Cytometry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-372, https://doi.org/10.5194/egusphere-egu25-372, 2025.

EGU25-986 | ECS | Posters on site | AS3.5

Investigation on meteorological dependency of airborne bacterial communities enriched with pathogens over Eastern Himalayas 

Shahina Raushan Saikh, Antara Pramanick, Md Abu Mushtaque, and Sanat Kumar Das

Airborne bacteria have a significant role in structural variation of atmospheric microorganisms with limited knowledge about their composition and geographical distribution, which demands high attention to understand their effect on human health and climate change, as their substantial temporal variation depends on local meteorological conditions. Current study presents composition, diversity, and variability of airborne bacterial loading over the Eastern Himalayas in India. A long-term airborne bacterial sampling is carried out within Bose Institute campus, situated at Darjeeling (27.03°N, 88.26°E, 2200m amsl) from January 2022 to September 2023. Samples are collected for eight hours duration, three times a day at 15m above the ground over sampling site. Illumina NextSeq platform is used to analyze V3-V4 regions of 16S rRNA gene in airborne bacterial samples using bacterium-specific primers. Total 88 samples are being investigated and categorized into four groups according to seasons: winter (temperature = 7±3ºC, relative humidity (RH) = 88±7%), pre-monsoon (15±2ºC, 87±10%), monsoon (17±1ºC, 97±3%), and post-monsoon (13±4ºC, 91±8%). About one-fourth (349 bacterial genera) population of airborne bacterial genera are present throughout the year, implying as background of Eastern Himalayan atmosphere. Human pathogens like Aeromonas, hydrophila, Acinetobacter lwoffii, Staphylococcus aureus, and Staphylococcus epidermis, responsible for gastroenteritis, endocarditis, respiratory, skin, and urinary tract infections are dominating in the atmosphere over Eastern Himalayas. Airborne bacterial loading varies significantly during different seasons with maximum concentration during pre-monsoon (Total cell count = 4.6±2.1 cells.m-3, OTUs = 597±343, Genera = 189±76, Shannon diversity index = 4.1±1.0), followed by post-monsoon (4.2±1.6 cells.m-3, 492±299, 171±65, 4.1±0.5), monsoon (3.8±1.3 cells.m-3, 332±171, 122±58, 3.4±1.0), and winter (3.6±1.7 cells.m-3, 239±87, 105±37, 3.4±0.8). Two distinct groups of beta diversities have been noticed over Eastern Himalayas during pre-monsoon & monsoon and post-monsoon & winter seasons, indicating similar bacterial populations. Eastern Himalayan airborne bacteria exhibit a strong dependency on temperature (r= -0.90, p<0.001) during seasonal changes from winter to pre-monsoon and post-monsoon to winter. Wind (r= 0.80, p<0.01) plays a significant role in the diversity of pre-monsoon season by transporting desert dust from western India, having highly diverse bacteria, and introducing unique pathogenic bacteria responsible for respiratory and skin infections over Eastern Himalayas.

How to cite: Saikh, S. R., Pramanick, A., Mushtaque, M. A., and Das, S. K.: Investigation on meteorological dependency of airborne bacterial communities enriched with pathogens over Eastern Himalayas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-986, https://doi.org/10.5194/egusphere-egu25-986, 2025.

EGU25-2600 | ECS | Posters on site | AS3.5

Photochemistry of Atmospheric Bioaerosols 

Palina Bahdanovich, Kevin Axelrod, Andrey Khlystov, and Vera Samburova

The chemistry and atmospheric fate of biological aerosols (bioaerosols) have been largely unexplored, despite their significant contribution to atmospheric particulate matter and organic carbon. Although bioaerosols are typically larger than anthropogenic aerosols, up to 100 µm, they can be transported over long distances and thus affect cloud physics (CCN, IN) and play a role in atmospheric chemical reactions. Studies have found that bioaerosols are expected to increase in concentration due to rapid climate change. For example, pollen concentrations are anticipated to increase by 21% and the pollen season length to increase by 21 days. Further, increases in instances and intensities of harmful algal blooms are already being observed. Due to the growing importance of bioaerosols in the atmosphere and climate, the goal of this study was to determine the effects of simulated atmospheric aging on bioaerosol functional groups and polarity. Water extracts of bioaerosols, lodgepole pine pollen and spirulina algae, were aged in a Suntest CPS solar simulator for 24 hours, under simulated solar radiation and in the presence of  H2O2 to promote oxidation with OH radicals. Proton Nuclear Magnetic Resonance Spectroscopy(1H-NMR) and Fourier-Transform Infrared Spectroscopy (FTIR) analyses were performed for fresh and aged bioaerosol extracts. FTIR results show an increase in polarity of both bioaerosols after aging with simulated solar radiation, up to 30.9% in pollen and 27.5% in algae, whereas 1H-NMR results are more complex, and a clear polarity increase was not observed. To our knowledge, this is the first study to analyze the effects of atmospheric aging on the chemistry of bioaerosols.

How to cite: Bahdanovich, P., Axelrod, K., Khlystov, A., and Samburova, V.: Photochemistry of Atmospheric Bioaerosols, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2600, https://doi.org/10.5194/egusphere-egu25-2600, 2025.

EGU25-4339 | Posters on site | AS3.5

Assessing indoor fungal spore health impacts with real-time detection technologies 

Ian Crawford, Hao Zhang, David Topping, Nurul Bintinazarudin, and Martin Gallagher

Bioaerosols are ubiquitous airborne microorganisms comprised of bacteria, fungi, pollen, virus and their constituents. Fungi have been associated with negative health effects ranging in severity from allergic reactions to asthma and serious infection, where susceptible individuals are at greater risk of life-threatening health outcomes resulting from exposure. While airborne fungi are abundant indoors, their airborne concentrations and source fluxes are poorly characterized due to the low temporal resolution of traditional offline sampling methods, limiting our understanding of key emission drivers in critical microenvironments and their impacts on air quality. 

There is a critical need to better characterize background fungal aerosol concentrations across a range of indoor microenvironments to build representative emission baselines to explore exposure assessment. Here we demonstrate the utility of emerging real-time detection methods across several indoor microenvironments to characterize the concentrations of key aeroallergenic fungi at high time resolution. 

In this study, Multiparameter Bioaerosol Spectrometer (MBS) and Plair Rapid E+ UV-LIF real-time bioaerosol spectrometers were deployed in University Place, a large multifunctional public space within the University of Manchester campus, over a 4-week period.  The single particle fluorescence and morphological data from the spectrometers was leveraged via cutting edge supervised and unsupervised machine learning approaches to yield 5-minute timeseries of key bioaerosol classes to investigate the impacts of human activity on emissions. Follow up studies with an MBS also investigated emissions within a large lecture theatre over several days and a busy thoroughfare within the Manchester Museum located on campus. 

Clear trends relating to the general movements of people through the microenvironments were observed, with notable increases in fungal aerosols correlating to a maximum in footfall and occupancy. Interestingly large, rapidly decaying spikes in concentration were observed in University Place around the hour, corresponding with a high flux of people through the building as they attend lectures or use other facilities. Crucially, these characteristic emission features would not be evident from sample integrations typical of offline sampling.  

The work presented here demonstrates the utility of real-time detection approaches to assess bioaerosol impact on indoor air quality and exposure. The use of specialised supervised learning training data focused on indoor bioaerosol composition in conjunction with high resolution, multiparameter UV-LIF spectrometers provides excellent high temporal resolution datasets to interrogate bioaerosol emission mechanisms and evaluate impacts on air quality, informing mitigation strategies and regulatory controls. 

How to cite: Crawford, I., Zhang, H., Topping, D., Bintinazarudin, N., and Gallagher, M.: Assessing indoor fungal spore health impacts with real-time detection technologies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4339, https://doi.org/10.5194/egusphere-egu25-4339, 2025.

EGU25-7168 | Posters on site | AS3.5

Artificial Intelligence for Pollen and Spore Detection, Forecasting and Human Health (AIPS) 

Francis Pope, Gordon Allison, Katie Brown, Alison Buckley, Ian Crawford, Philippa Douglass, Anna Hansell, Rob MacKenzie, Emma Marczylo, Sophie Mills, Lucy Neil, Jack Satchwell, Fiona Symon, David Topping, and Hao Zhang

Pollen and fungal spores are important for human health in both outdoor and indoor environments. They are linked to several respiratory illnesses which range in severity from minor to deadly. Better detection and forecasting of pollen and fungal spores would allow for interventions to be developed that would reduce their risk to human health. 

The current methodologies available for the detection of pollen and fungal spores are either expensive or time consuming, and often both. This hugely limits their use. For example, the UK Met Office currently only has available 11 regulatory grade sites for pollen monitoring from which their pollen forecast is based upon. This equates to about one regulatory pollen monitoring station per 11 million people in the UK. Similarly, regulatory agencies lack cheap methodologies to detect fungal spores in both outdoor and indoor locations. A cheaper, more agile detection method would much increase the UK's capacity for the detection and forecasting of pollen and fungal spores. 

The AIPS project has combine several rapidly developing technologies. It brings together a distributed internet-of-things (IoT) sensor arrays in combination with regulatory grade equipment and artificial intelligence (AI) techniques. The IoT sensors measure the size distribution of the small particles that are present within the air. The sources and compositions of these particles are many and varied. Atmospheric particles include bioaerosols that are composed of fragments from the biosphere, including pollen and fundal spores. Finding these bioaerosols within the much larger populations of other atmospheric aerosols, is like finding a needle in a haystack. Fortunately for this project, pollen and fungal spores have well defined sizes that are distinct to the background aerosol which makes detection possible. AI approaches will use machine learning algorithms to classify the pollen and fungal spore species of interest and generate approaches to detect them in real time. The results are then compared to regulatory grade equipment to assess the skill of the low-cost approach.  This real time detection will allow for data-driven real-time forecasts of the pollen and spore species of interest.

The presentation will provide an overview of the AIPS project, and discuss the efficacy and applicability of the new AI and IoT tools with respect to bioaerosol detection and forecasting needs.

How to cite: Pope, F., Allison, G., Brown, K., Buckley, A., Crawford, I., Douglass, P., Hansell, A., MacKenzie, R., Marczylo, E., Mills, S., Neil, L., Satchwell, J., Symon, F., Topping, D., and Zhang, H.: Artificial Intelligence for Pollen and Spore Detection, Forecasting and Human Health (AIPS), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7168, https://doi.org/10.5194/egusphere-egu25-7168, 2025.

EGU25-10456 | Posters on site | AS3.5

A case study based on bioaerosol emissions from farmland and animal houses 

Zhuo Chen, Emily Matthews, Ian Crawford, Jonathan West, Michael Flynn, David Topping, Martin Gallagher, and Hugh Coe

Bioaerosols encompass a diverse range of airborne particles such as viruses, bacteria, fungal spores, pollen, and various fragments related to plants and animals. Bioaerosols through their extensive involvement in surface-atmosphere physic-chemical reactions affect the stability of the biosphere, climate change, and human health. To accurately measure bioaerosols and provide early warning of exposure, a range of real-time bioaerosol detection instruments have been developed that can rapidly identify bioaerosol species through techniques such as fluorescence spectroscopy, holography and light scattering. In this work we deployed a Multiparameter Bioaerosol Spectrometer (MBS), a UVLIF and morphological single particle spectrometer,  as part of a pilot experiment at the Rothamsted North Wyke Farm Platform (NWFP). Analysis of the MBS measurements was used to assess the contributions of biofluorescent aerosol emitted from local farmyards and animal housing compared with the surrounding environment. Preliminary analysis of the data shows that the expected distinct bioaerosol diurnal concentration pattern experienced significant perturbations induced by the nearby animal house emissions. Concentrations in general were higher during morning and nighttime periods and displayed more stable patterns in the afternoon indicative of activities. Bioaerosol sizes ranged from Dp = 0.5 to 5 µm and were dominated by specific fluorescent clusters clearly dependent on the emission source. These data will be examined in more detail using laboratory training data sets to inform AI algorithms to further discriminate bioaerosol classes.

 
 

How to cite: Chen, Z., Matthews, E., Crawford, I., West, J., Flynn, M., Topping, D., Gallagher, M., and Coe, H.: A case study based on bioaerosol emissions from farmland and animal houses, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10456, https://doi.org/10.5194/egusphere-egu25-10456, 2025.

Primary biological aerosol particles (PBAPs) significantly affect human health and aerosol-cloud-climate interactions. Fluorescent aerosol particles (FAPs), detected using light/laser-induced fluorescence (LIF) instruments, serve as a crucial proxy for understanding the concentration and size distribution of PBAPs and the factors that influence their variability in the atmosphere. This study systematically evaluates FAPs collected from field measurements worldwide and simulates their concentrations on a global scale using machine learning algorithms, incorporating comprehensive global weather, climate and emissions data. The simulated global concentration reveals spatial variations in size and concentration, with heightened annual mean concentration predominantly observed in the tropics and the Asia region. The post-hoc Shapley Additive Explanation (SHAP) method indicates that the spatio-temporal patterns of FAPs concentrations and size distributions are primarily driven by anthropogenic emissions in urban regions, while weather factors are more closely linked to variations in oceanic and rural areas. Notably, certain non-biological emissions (e.g., dust and black carbon) exhibit strong correlations with FAPs, particularly in densely populated areas and the Arctic region. Overall, this study underscores the significant role of anthropogenic emissions in shaping simulated FAP concentrations on a global scale and provides guidance for future investigations into FAP concentrations in unexplored regions.

How to cite: Miao, Y. and Lee, P. K. H.: Global Modeling of Fluorescent Aerosol Particles with Machine Learning Reveals Potential Regional Anthropogenic Impacts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16487, https://doi.org/10.5194/egusphere-egu25-16487, 2025.

EGU25-17236 | Posters on site | AS3.5

Testing the generation of fungal spore aerosols with a new atomization setup 

Elias Graf, Haruna Gütlin, Erny Niederberger, Philipp Burch, and Tomke Musa

To study bioaerosols under controlled conditions, aerosol chambers equipped with aerosol generators have been used for a long time. However, the method used for generation can change the constitution and properties of the bioaerosol produced, including the biological integrity of fungal spores, bacteria or airborne viruses. The properties of a bioaerosol in turn influence the results of detection, enumeration and identification methods downstream (Pogner et al., 2024). Recent developments of automatic bioaerosol monitors equipped with AI-based identification algorithms require simple and reliable generation of bioaerosols in the laboratory to collect  data for the machine learning trainings.

Figure 1 View into the SAG chamber through the window at the front, containing a petri dish with a fungal colony.

The Swisens Aerosol Generator (SAG) is an atomizer for efficient and gentle aerosolization of fungal spores, as well as other dry biological materials, for measurement with the SwisensPoleno and other instruments. The SAG principle is based on the design described by Lee et al. (2010), with improvements for better controllability and a higher yield. It consists of a chamber, shown in Figure 2, in which the petri dishes and other materials are placed. Pressured air, generated by a separate air supply unit, is led to a nozzle inside the chamber and directed over the biological materials. The horizontal air stream detaches the fungal spores into the air of the chamber, which can then be taken in by the instrument to measure the content.

 

Figure 2 Left: Aerosol chamber with HEPA filter at the top for clean air supply. Right: Air supply unit with digital flow meter, flow controls and air filter.

The structure and quantity of aerosolized particles is highly dependent on the fungi species, its growth stage and success, as well as the airflow onto the petri dish. Measurements with Cladosporium cladosporioides (Tested by Pogner et al. (2024) with SAG prototype) created, for example, numerous data of agglomerated spores and mycelium parts besides single spores, whereas Alternaria alternata constantly generated single spores in high numbers. With the SAG the process and the efficiency of fungal spores aerosolization can be improved, making it a new tool besides other fungal spore aerosols generation methods. This opens more opportunities to choose the best means of aerosolization depending on the fungal species and required particles.

 

References:

Lee, Jun Hyun, Gi Byung Hwang, Jae Hee Jung, Dae Hee Lee, und Byung Uk Lee. 2010. «Generation characteristics of fungal spore and fragment bioaerosols by airflow control over fungal cultures». Journal of Aerosol Science 41 (3): 319–25. https://doi.org/10.1016/j.jaerosci.2009.11.002.

Pogner, Clara-E, Elias Graf, Erny Niederberger, und Markus Gorfer. 2024. «What do spore particles look like - use of real-time measurements and holography imaging to view spore particles from four bioaerosol generators». Aerosol Science and Technology 58 (7): 1–17. https://doi.org/10.1080/02786826.2024.2338544.

How to cite: Graf, E., Gütlin, H., Niederberger, E., Burch, P., and Musa, T.: Testing the generation of fungal spore aerosols with a new atomization setup, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17236, https://doi.org/10.5194/egusphere-egu25-17236, 2025.

EGU25-18207 | ECS | Posters on site | AS3.5

UAV-based aerosol and VOC measurements above a spruce forest canopy in Lower Austria 

Florian Wieland, Matthäus Rupprecht, Peter J. Wlasits, Jürgen Gratzl, Pascal Langer, Vanessa Treml, Jordan Horral, Cayden Smedley, Regina Hanlon, David Schmale III, and Hinrich Grothe

Forests are increasingly recognized as significant sources of biogenic aerosols, impacting air quality and climate. However, understanding the distribution and transport of these aerosols within and above forest canopies remains a challenge. This study investigates the vertical profiles of aerosol and volatile organic compound (VOC) concentrations above a spruce forest in Lower Austria using a novel analytical instrument packages on Uncrewed Aerial Vehicles (UAV).

In our campaign we used multiple UAVs outfitted with various air quality sensors to monitor aerosol concentrations above natural and managed forests. Here, we describe the use of a drone aerosol analytics package consisting of a volatile organic compounds (VOC) sensor, a portable optical particle spectrometer (POPS), and an environmental sensor module to investigate particle emissions at different heights above a spruce forest within Wienerwald in Lower Austria. This package was compared to simultaneous measurements with other drone-based and ground-based systems, including optical particle counters (OPCs) and impingers.

Preliminary results showed higher particle number concentrations across all size channels (0.115 – 3.370 µm) at near-canopy altitudes (<5m above the canopy) compared to measurements at higher altitudes (> 5m above the canopy). Furthermore, our results point towards a height dependence of VOC concentrations, where VOC concentrations strongly decrease with increasing height.  Future work aims to use drone-based aerosol measurements above forest canopies to assist in gauging forest health, such as identifying early warnings of attack by pathogens or insects.

How to cite: Wieland, F., Rupprecht, M., Wlasits, P. J., Gratzl, J., Langer, P., Treml, V., Horral, J., Smedley, C., Hanlon, R., Schmale III, D., and Grothe, H.: UAV-based aerosol and VOC measurements above a spruce forest canopy in Lower Austria, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18207, https://doi.org/10.5194/egusphere-egu25-18207, 2025.

EGU25-898 | ECS | Orals | AS3.6

Which INPs and secondary ice processes are necessary to accurately model a warm Arctic mixed-phase cloud?  

Hannah Frostenberg, Jessie Creamean, Camille Mavis, Luis Santos, Erik S. Thomson, Annica M. L. Ekman, and Luisa Ickes

The phase of low-level clouds plays a crucial role in their interaction with radiation, particularly in the Arctic.  Despite the Arctic's notably clean air, characterized by low aerosol and ice nucleating particle (INP) concentrations, cloud ice can still be observed at relatively warm sub-zero temperatures. 

We present a modeling closure analysis of an Arctic low-level mixed-phase cloud observed during the 2023 ARTofMELT (Atmospheric rivers and the onset of sea ice melt) campaign using the large eddy simulation model MIMICA. Comprehensive measurements of INPs and aerosols were taken at the surface, within, and above the cloud. By combining modeling and observations, we will explore which aerosol population was necessary to aid in the formation of ice within the cloud. 

The minimum observed in-cloud temperature was -8 °C, with ice present throughout the cloud’s lifetime. The highest temperature at which INPs were detected was -13 °C, with an INP concentration of approximately 1.6e-4 /L. Our findings indicate that observed INP concentrations alone are insufficient to produce a significant amount of ice in the model. This suggests the need for other processes like secondary ice formation and INP recycling, or a possible misrepresentation of microphysical processes in the model. By utilizing the model and including these missing processes, we aim to determine the necessary INP concentrations and properties, as well as the secondary ice mechanisms, to account for the observed ice. This includes analyzing the importance of local versus long-range transported aerosols and primary versus secondary ice production. 

How to cite: Frostenberg, H., Creamean, J., Mavis, C., Santos, L., Thomson, E. S., Ekman, A. M. L., and Ickes, L.: Which INPs and secondary ice processes are necessary to accurately model a warm Arctic mixed-phase cloud? , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-898, https://doi.org/10.5194/egusphere-egu25-898, 2025.

EGU25-2169 | ECS | Posters on site | AS3.6

Improved Formulation of Snow Fragmentation during Collision with Hail/ Graupel based on Field Observation at Jungfraujoch 

Freddy Paul, Martanda Gautam, Deepak Waman, Sachin Patade, Ushnanshu Dutta, Christoffer Pichler, Marcin Jackowicz-Korczynski, and Vaughan Phillips

Secondary Ice Production (SIP) has been ascribed to the formation of new ice particles from preexisting ones. Fragmentation of ice particles during collision is one among the known SIP processes. Some of the studies have used theoretical formulation of this SIP processes in the cloud micro-physics scheme of numerical atmospheric models. However, there has been a lack of observational data for better understanding of the SIP process. This study reports fragmentation of naturally falling snow  during their collision with graupel/hail particles based on the observation at Jungfraujoch, a mountain pass in the Alps located about 3.4 km above mean sea level. The study used a  specially designed portable chamber to observe the fragmentation of snow particles outdoor. Based on the observational study, we optimised the theoretical formulation for the prediction of number of fragments arising from the collision between non-dendritic snow and hail/graupel. The observations show an average number of fragments per collision of about 5. The study improved the prediction of SIP through fragmentation compared to our original theoretical formulation, for snow in the non-dendritic regime of temperatures less than -170C.

How to cite: Paul, F., Gautam, M., Waman, D., Patade, S., Dutta, U., Pichler, C., Jackowicz-Korczynski, M., and Phillips, V.: Improved Formulation of Snow Fragmentation during Collision with Hail/ Graupel based on Field Observation at Jungfraujoch, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2169, https://doi.org/10.5194/egusphere-egu25-2169, 2025.

EGU25-2825 | ECS | Posters on site | AS3.6

Life cycle of ice-nucleating particles in an Arctic cold air outbreak 

Erin Raif, Paul Field, Benjamin Murray, and Kenneth Carslaw

Ice-nucleating particles (INPs) can modulate the cloud-phase feedback, where the albedo of mixed-phase clouds increases in a warming climate. Mid-to-high latitude shallow cloud systems such as cold-air outbreaks (CAOs) are particularly important for cloud-phase feedbacks and sensitive to INPs. While previous studies have looked at the impact of INP concentration on CAOs, few studies have considered the life cycle of INPs in cold-air outbreaks, and the consequences for cloud albedo.

To understand how INPs are processed in CAOs, we are performing regional modelling of a CAO observed over the Norwegian Sea during the 2022 Arctic Cold Air Outbreak field campaign. Airborne INP measurements during this CAO revealed a reduction in INP concentration as the CAO developed despite the addition of sea-spray aerosol downstream in the outbreak (Raif, et al. 2024). We will test the hypothesis that INPs in air flowing into Arctic CAOs initially overwhelms local surface sources of aerosol, but are removed through precipitation processes as air moves south.

To do this, we are using the UK Met Office Unified Model with a new two-moment microphysics scheme utilising two-way interaction between cloud and aerosol tracers. Using in-situ measurements of aerosol and INPs, we will test the sensitivity of CAO development to the entrainment of INPs, removal of INPs through precipitation and redistribution of INPs after sublimation/evaporation.

Reference: Raif, et al. (2024). High ice-nucleating particle concentrations associated with Arctic haze in springtime cold-air outbreaks, Atmos. Chem. Phys. https://doi.org/10.5194/acp-24-14045-2024

How to cite: Raif, E., Field, P., Murray, B., and Carslaw, K.: Life cycle of ice-nucleating particles in an Arctic cold air outbreak, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2825, https://doi.org/10.5194/egusphere-egu25-2825, 2025.

EGU25-3750 | ECS | Orals | AS3.6

Surface topography and ice nucleation activity of alkali feldspar 

David Andreas Heuser, Michael Hagn, Johanna Seidel, Elena Petrishcheva, Rainer Abart, and Alexei Kiselev

Alkali feldspar undergoes a variety of phase transformations during cooling from magmatic crystallization leading to increasing ordering of Al and Si on the tetrahedrally coordinated lattice sites and to grain-internal microstructures such as twins and exsolution lamellae and associated surface topography. Both, Al-Si ordering as well as the specific surface topography may contribute to the extraordinary ice nucleation activity of alkali feldspar. We studied seven natural alkali feldspars ranging from homogeneous and featureless gem-quality sanidine with disordered Al-Si to hydrothermally altered microcline with ordered Al-Si, several generations of exsolution lamellae and micropore-rich regions associated with domains of hydrothermal albitization. (010) and (001) cleavage plates were produced from each feldspar sample and mounted in a cooling stage. Then an array of 7nl droplets of ultra-pure water was applied and cooled at 2 K/min. Droplet freezing events were recorded with an infrared camera.

The highest freezing temperatures are observed on (010) cleavage plates of K-rich (XK=0.94) microcline that exhibits 1-8 µm wide albite exsolution lamellae and 20-100 µm wide microporous regions along cracks related to hydrothermal albitization. In contrast, featureless (001) plates of gem-quality sanidines show freezing at over 10 K lower temperatures. The enhanced ice nucleation activity is tentatively ascribed to Si-Al ordering [1] and to heterogeneous ice nucleation on the surface features related to the grain-internal microstructures [2]. Which one of the two factors is more important is still unresolved.

 

[1] Franceschi G., Conti A., Lezuo L., Abart R.,  Mittendorfer F., Schmid M., Diebold U. (2023) How Water Binds to Microcline Feldspar (001), J. Phys. Chem. Lett., Vol. 15, 1, 15–22, https://doi.org/10.1021/acs.jpclett.3c03235

[2] Kiselev, A., Keinert, A., Gaedeke, T., Leisner, T., Sutter, C., Petrishcheva, E., Abart, R. (2021) Effect of chemically induced fracturing on the ice nucleation activity of alkali feldspar. Atmospheric Chemistry and Physics, 21 (15): 11801-11814, DOI 10.5194/acp-21-11801-2021

How to cite: Heuser, D. A., Hagn, M., Seidel, J., Petrishcheva, E., Abart, R., and Kiselev, A.: Surface topography and ice nucleation activity of alkali feldspar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3750, https://doi.org/10.5194/egusphere-egu25-3750, 2025.

EGU25-4346 | ECS | Posters on site | AS3.6

How do volcanic eruptions effect cloud hydrometeor properties?A case study of the Raikoke eruption 2019 

Melina Sebisch, Fatemeh Zarei, Julia Bruckert, and Corinna Hoose

One of the major causes for uncertainties in atmospheric modelling are aerosol-cloud-interactions as stated in the IPCC report WG1 in 2021. The aerosols available in the atmosphere can act as cloud condensation nuclei (CCNs) or ice nucleating particles (INPs) and thereby have a direct effect on cloud formation and properties. The investigation of those effects is not easy since these properties also depend on other atmospheric conditions such as the synoptic state. In volcanic eruptions the emitted aerosols are a local perturbation in the atmospheric aerosol distribution independent of synoptic conditions. The volcanic aerosols such as SO2 reacting to sulfuric acid or volcanic ash can act as CCNs and INPs respectively. Simulations with and without the eruption can be compared to directly quantify the effect of the volcanic aerosols on cloud properties. The simulations with an eruption can be compared to obervational data to verify the simulation results and improve the simulation setup.

In the presented work, the eruption of the Raikoke volcano in 2019 has been simulated using the ICOsahedral Nonhydrostatic model (ICON) and the module for Aerosols and Reactive Trace gases (ART) in limited area mode with up to 2.5 km horizontal resolution. The simulated area contains both the location of the eruption and a large cloud system consisting of liquid, mixed-phase and ice clouds. The eruption is modelled using the module fplume, a dynamics driven model predicting the vertical distribution of the emitted aerosols at the source. An ice nucleation parameterization specific for volcanic ash derived in laboratory experiments by Umo et al. (2021) for heterogeneous freezing has been implemented in the model.

First preliminary results will be shown with a focus on cloud hydrometeor properties of mixed-phase and ice clouds. Due to the location of the volcanic plume above the low liquid clouds it is found that ice crystal properties are more affected than liquid hydrometeors. The results using the ice nucleation parameterization by Umo et al. are compared to the commonly used parameterization for mineral dust particles by Ullrich et al. (2017). By specifically enabling aerosol-radiation and aerosol-cloud interactions seperately the direct and indirect impact of the eruption on the radiation balance will be quantified.

How to cite: Sebisch, M., Zarei, F., Bruckert, J., and Hoose, C.: How do volcanic eruptions effect cloud hydrometeor properties?A case study of the Raikoke eruption 2019, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4346, https://doi.org/10.5194/egusphere-egu25-4346, 2025.

EGU25-4383 | Posters on site | AS3.6

Comparing ice-nucleating particles in extensive stratiform clouds 

Heike Wex, Kevin Ohneiser, Markus Hartmann, Anja Hardt, Anna J. Miller, Zamin A. Kanji, Jan Henneberger, Katharina Baudrexl, and Patric Seifert

In the Southwest of Germany and the North of Switzerland, there is a wind known as Bise, roughly blowing from Northeast. Associated with this wind, an extensive and long-living stratiform cloud deck can form in the winter months.

For this study, measurements were done at two different locations, both protruding above the surrounding landscape: Hohenpeißenberg (47.801°N,11.009°E, elevation 950m, station of the German Weather Service DWD, ~ 50km southwest of Munich) and Eriswil (47.071°N,7.873°E, elevation 920m, ~ 60 km southwest of Zurich). During a Bise situation, there is typically a stratus cloud at and between both locations, with winds blowing roughly from Hohenpeißenberg to Eriswil. During two Bise periods in January and February 2024, we collected aerosol particles onto polycarbonate filters at both sites. Sampling was conducted with a Digitel low-volume sampler. Sampling time was 12 hours for each filter, with a flow rate of 25 l/min. Collected filters were examined for their INP (Ice Nucleating Particle) concentrations with well-established offline methods at TROPOS.

When the Bise cloud was present at both Hohenpeißenberg and Eriswil, INP spectra at both locations were very similar. In January (Bise-1), temperatures in the boundary layer were below 0°C, and INP spectra did not show a high fraction of INPs with biogenic origin. In February (Bise-2), temperatures in the boundary layer had already risen to be constantly above 0°C. Much higher INP concentrations were observed for the whole INP spectra during Bise-2. This increase was particularly strong for freezing temperatures above -12°C, caused by additional heat labile INPs of biogenic origin. The difference in INP concentrations between the two Bise situations may at least partially originate in INP removal through ice nucleation with subsequent precipitation formation during Bise-1 which did not occur during Bise-2.

During Bise-1, there was a phase when at Hohenpeißenberg the inversion decreased in altitude by a few hundred meters. With this, the measurement site protruded above the Bise cloud, while at the same time the temperature at the ground in Hohenpeißenberg increased from -10°C to just below 0°C. Meanwhile, the Bise cloud was still present at Eriswil. While INP spectra had been similar at Hohenpeißenberg and Eriswil when both sites were in the Bise cloud, during this phase of more than a day, INP spectra at Hohenpeißenberg showed much higher concentrations and additional heat labile INPs. The changed conditions reflect the situation in the free troposphere, and we suggest the free troposphere as a source for INPs for the Bise clouds.

How to cite: Wex, H., Ohneiser, K., Hartmann, M., Hardt, A., Miller, A. J., Kanji, Z. A., Henneberger, J., Baudrexl, K., and Seifert, P.: Comparing ice-nucleating particles in extensive stratiform clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4383, https://doi.org/10.5194/egusphere-egu25-4383, 2025.

EGU25-4998 | Orals | AS3.6

On the abundance and sources of biological aerosol serving as ice nuclei in the high Arctic 

Paul Zieger, Gabriel Pereira Freitas, and Julia Kojoj and the Arctic-Bioaerosol-INP-Team

Aerosols significantly influence Arctic cloud properties, affecting radiative balance and climate dynamics. Among them, ice-nucleating particles (INPs) are particularly impactful, as they nucleate ice at higher temperatures than homogeneous freezing, altering cloud radiative properties and lifetimes. Primary biological aerosol particles (PBAPs), a subset of aerosols of biological origin, have garnered attention due to their abundance and widespread presence. PBAPs may influence clouds more than previously recognized, particularly in the Arctic, where aerosol-cloud interactions are crucial for regional climate regulation. Understanding the sources, seasonality, and mechanisms of PBAP-induced cloud microphysics is critical, especially as Arctic environmental changes potentially amplify or mitigate these interactions.

Here, we present an overview of recent observational and experimental evidence linking PBAPs to INPs and their subsequent impact on cloud phase and radiative properties. Observations across diverse Arctic regions from Ny-Ålesund (Svalbard) to the central Arctic Ocean over the pack ice will be presented.  Through a synthesis of multi-year and expedition-based studies using a wide range of experimental and modelling approaches, we provide evidence linking fluorescent PBAPs to INPs, and their yearly dominance in the high-temperature regime. Our results show that PBAPs are closely associated with heat-labile high-temperature INPs, especially during the biologically active summer and early fall seasons. Concentrations of fluorescent PBAPs range from 10-3 to 10-1 L-1, peaking in summer when biological activity and terrestrial vegetation are at their height (Freitas et al., 2023). PBAP were also for the first time directly observed in-situ within cloud residuals (dried cloud particles) using single-particle fluorescence spectroscopy and electron microscopy coupled to a ground-based counterflow virtual impactor inlet. Seasonal cloud observations linked their presence to a possible influence on the prevalence of mixed-phase clouds during warm months (Freitas et al., 2024).

While the sources of fluorescent PBAP over Svalbard are mainly suggested to be of regional and terrestrial origin, over the Arctic Ocean, marine sources emerge as significant contributors to fluorescent PBAP emissions, particularly during ice-free periods in biologically productive areas. At the North pole, air parcel trajectory analysis, combined with ocean productivity reanalysis, links episodic fluorescent PBAP and high temperature INP events to biologically active regions (Kojoj et al., 2024). 

Our findings underscore the critical role of PBAPs acting as INP and in determining the phase and radiative properties of low-level Arctic MPCs. This work has important implications for improving the representation of Arctic aerosol sources - especially of biological origin - and their interactions in climate models. As the Arctic undergoes profound transformations in its hydrological and biogeochemical cycles, it is essential to understand the sources and characteristics of PBAPs and their links to INPs in order to better predict future cloud and climate dynamics in this sensitive region.

References:

Freitas et al. Nature Communications 14.1 (2023): 5997. https://doi.org/10.1038/s41467-023-41696-7

Freitas et al. Atmospheric Chemistry and Physics 24.9 (2024): 5479-5494. https://doi.org/10.5194/acp-24-5479-2024

Kojoj et al. Tellus. Series B, 76.1 (2024): 47-70. https://doi.org/10.16993/tellusb.1880

How to cite: Zieger, P., Pereira Freitas, G., and Kojoj, J. and the Arctic-Bioaerosol-INP-Team: On the abundance and sources of biological aerosol serving as ice nuclei in the high Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4998, https://doi.org/10.5194/egusphere-egu25-4998, 2025.

EGU25-5737 | ECS | Orals | AS3.6

Fluorescent fungal spores as a major contributor to ice nucleating particles in the European sub-Arctic 

Jürgen Gratzl, Alexander Böhmländer, Ottmar Möhler, Eija Asmi, Sanna Pätsi, Annika Saarto, Clara-E. Pogner, David Brus, Konstantinos Matthaios Doulgeris, Dominik Stolzenburg, Florian Wieland, and Hinrich Grothe

Primary biological aerosol particles (PBAPs), including fungal spores, bacteria and pollen grains, are widely distributed in the atmosphere. Some PBAPs are highly efficient ice nucleating particles (INPs), but their impact on atmospheric ice formation is currently uncertain. PBAPs have been associated with INPs that are active at high sub-zero temperatures and may contribute disproportionally high  in places with little anthropogenic influence, such as the high Arctic [1] and in the boreal forest [2].

This study investigates PBAPs and INPs in the pristine Finnish sub-Arctic at the Pallas supersite from September 2022 to September 2023. To study PBAPs, we combine measurements of highly fluorescent aerosol particles (HFAPs) with the Wideband Integrated Bioaerosol Sensor (WIBS) [3], fungal spore counts from a Hirst-type volumetric sampler and eDNA sequence analysis from filter samples. We compare PBAPs to INP measurements over a wide temperature range using the Portable Ice Nucleation Experiment (PINE) [4] and the Ice Nucleation Spectrometer of the Karlsruhe Institute of Technology (INSEKT) [2].

We found a strong seasonal trend of a subset of HFAPs with maximum concentrations in summer and an abrupt and strong decrease with snow cover. Together with an exponential relationship with temperature, this suggests locally emitted bioaerosols. The measured bioaerosols show a positive correlation with INPs active over a wide activation temperature range (-31°C - -8°C). An exceptionally high correlation (r=0.94, p<0.001) was found for INPs active above -13.5°C, showing that WIBS is a powerful tool to predict INP concentrations in biologically dominant environments. Comparison of WIBS data with fungal spore counts indicates the fungal nature of the biological INPs. eDNA analysis revealed a much higher fungal biodiversity than the visually identified spore counts with most of the species belonging to Basidiomycota. Although we found some species known for ice nucleation (e.g. Penicillium_sp, Aspergillus_sp) the ice nucleation of most of the fungi detected has not yet been tested. Future work could contribute to the knowledge of the exact fungal species that dominate the INP population in the sub-Arctic.

This work was supported by ATMO-ACCESS under the ID ATMO-TNA-4-0000000069 and by the FFG under the Project Lab on a Drone (888109).

[1] Pereira Freitas, G. et al. (2023) Nat Commun, 14, 5997

[2] Schneider, J. et al. (2021) Atmos Chem Phys, 21, 3899- 3918

[3] Gratzl, J. et al. (2025), Earth Syst Sci Data (submitted)

[4] Möhler, O. et al. (2021). Atmos Meas Tech. 14(2), 1143-1166.

How to cite: Gratzl, J., Böhmländer, A., Möhler, O., Asmi, E., Pätsi, S., Saarto, A., Pogner, C.-E., Brus, D., Doulgeris, K. M., Stolzenburg, D., Wieland, F., and Grothe, H.: Fluorescent fungal spores as a major contributor to ice nucleating particles in the European sub-Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5737, https://doi.org/10.5194/egusphere-egu25-5737, 2025.

EGU25-6371 | ECS | Orals | AS3.6

A laboratory study of secondary ice production from collisions between supercooled raindrops and ice particles 

Rachel James, Jonathan Crosier, and Paul Connnolly

As part of the CERTAINTY project, we present results from our laboratory study of secondary ice production (SIP) from collisions between supercooled raindrops and more massive ice particles, building on our previous proof-of-concept work (James et al., 2021) with a refined experimental setup for improved quantification.

In mixed phase clouds, ice formation can occur via two pathways: primary ice formation, via ice nucleating particles, or secondary ice production (SIP). Observations in both shallow and deep convective clouds often show ice concentrations that exceed those predicted by primary ice nucleation by several orders of magnitude. However, parameterisations of SIP mechanisms remain poorly constrained due to limited laboratory data.

One proposed SIP mechanism involves collisions between supercooled raindrops and more massive ice particles, where secondary drops may form during impact, with some freezing to create secondary ice. Our previous work (James et al., 2021) demonstrated the viability of this SIP mechanism, and showed that approximately 30 % of the secondary drops froze under a limited set of conditions.  Building on this, we have refined our experimental setup to reduce uncertainties in the freezing fraction of secondary drops by elevating the ice particle to allow the splashing to occur freely, without interference of a flat surface used in our previous experiments. We also explore a broader range of supercooled water drop diameters, ice particle sizes, impact velocities and temperatures to better reflect cloud conditions.

Finally, we incorporate our updated results into a parcel model with bin microphysics for idealised clouds, which previously used our earlier results (James et al. 2023), to demonstrate the impact this improved quantification in conjunction with other SIP mechanisms.

References
James, R. L., Phillips, V. T. J., and Connolly, P. J. (2021), Secondary ice production during the break-up of freezing water drops on impact with ice particles, Atmos. Chem. Phys., 21, 18519–18530, https://doi.org/10.5194/acp-21-18519-2021.
James, R. L., Crosier, J., and Connolly, P. J. (2023), A bin microphysics parcel model investigation of secondary ice formation in an idealised shallow convective cloud, Atmos. Chem. Phys., 23, 9099–9121, https://doi.org/10.5194/acp-23-9099-2023.

How to cite: James, R., Crosier, J., and Connnolly, P.: A laboratory study of secondary ice production from collisions between supercooled raindrops and ice particles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6371, https://doi.org/10.5194/egusphere-egu25-6371, 2025.

EGU25-6935 | ECS | Posters on site | AS3.6

Ice Nucleation Abilities and Chemical Characteristics of Laboratory-Generated and Aged Biomass Burning Aerosol 

Jie Chen, Fähndrich Martin Othmar Jakob, Aristeidis Voliotis, Huihui Wu, Sara Aisyah Syafira, Osayomwanbor Oghama, Nadia Shardt, Nicolas Fauré, Xiangrui Kong, Gordon Mcfiggans, and Zamin A. Kanji

Biomass burning aerosols (BBA) significantly contribute to the global aerosol burden, thereby influencing air quality and global climate. The chemical properties and ice nucleation activity of BBA remain poorly constrained due to the heterogeneity of biomass sources and the complexity of atmospheric aging processes. This study comprehensively investigates the chemical composition and ice nucleation of BBA generated from laboratory-controlled burns using various biomass types and burning conditions. Both freshly emitted and photochemically aged BBA exhibit distinct and reproducible chemical compositions. However, the ice nucleation activity of BBA shows substantial variability at mixed-phase cloud temperatures and cannot be predicted by the chemical variability of the organic and inroganic carbon content. This indicates that the carbonaceous components of BBA are not a predictor for ice nucleation activity of BBA.  Using laboratory data, we further evaluate the impact of BBA on atmospheric ice nucleation based on particulate matter mass concentration and equivalent spherical diameter. The estimated ice nucleating particle concentrations from laboratory-produced BBA are lower than those observed during BBA pollution in field studies. We hypothesize that the discrepancy likely arises from the co-lofting of mineral particles during real-world biomass burning events, such as ash or soil particles. These particles, which are absent in our experiments but abundant in field observations, may be an important source of atmospheric INPs, rather than carbonaceous-rich particles from combustion. The role of mineral particles in the INP concentrations of BBA is not quantified in this study, further research to address co-lofting of mineral particles with BBA is encouraged.  

How to cite: Chen, J., Martin Othmar Jakob, F., Voliotis, A., Wu, H., Aisyah Syafira, S., Oghama, O., Shardt, N., Fauré, N., Kong, X., Mcfiggans, G., and A. Kanji, Z.: Ice Nucleation Abilities and Chemical Characteristics of Laboratory-Generated and Aged Biomass Burning Aerosol, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6935, https://doi.org/10.5194/egusphere-egu25-6935, 2025.

EGU25-8753 | Posters on site | AS3.6

The Impact of Atmospheric Photochemistry on Marine Aerosols: Ice Nucleation and Droplet Activation 

Najin Kim, Ahmed Abdelmonem, Nsikanabasi Silas Umo, Robert Wagner, Larissa Lacher, Ottmar Möhler, Hao Li, Harald Saathoff, Kyung Hwan Kim, Do-Hyeon Park, Chanwoo Ahn, Dong Hwi Kim, Un Hyuk Yim, Seong Soo Yum, and Sun Choi

Oceans cover more than 70% of the Earth’s surface and are a critical component of global climate system. Sea spray aerosols (SSAs), derived from ocean surfaces, represent a unique and significant source of ice nucleating particles (INPs) and cloud condensation nuclei (CCN), yet their contribution to cloud processes remains poorly understood, with substantial uncertainties surrounding their role in climate systems. To address this gap, we investigate the atmospheric photochemical effects on marine aerosols and their implications for ice nucleation and droplet activation through controlled laboratory experiments.

Our study utilizes two key experimental systems: the AIDAd (Aerosol Interactions and Dynamics in the Atmosphere) cloud chamber and PINE (Portable Ice Nucleation Experiment). AIDAd, with its temperature-controlled walls capable of simulating temperature range from +30 °C to −55 °C and tropospheric cooling rates up to 10 °C min⁻¹, allows for precise investigations of aerosol-cloud interactions. PINE measures INP concentrations under mixed-phase cloud conditions at temperatures ranging from −10 °C to −38 °C.

For our experiments, marine aerosols were generated from three distinct seawater samples collected from diverse oceanic regions: the Indian Ocean, the South China Sea, and Jangmok Port (Korea). These samples capture the variability of natural marine environments and provide a comprehensive basis for understanding the effects of geographical and biological diversity on aerosol properties. These samples underwent photochemical treatment using a custom-built solar radiation simulator to replicate atmospheric conditions. The irradiated aerosols are subsequently analyzed using the AIDAd chamber and PINE, and further chemical analysis are done to evaluate changes in composition and ice nucleation potential.

This study provides critical insights into the interplay between marine aerosol sources, photochemistry, and cloud formation. By integrating data from AIDAd and PINE, we aim to unravel the mechanisms underlying ice nucleation and droplet activation of marine aerosols under simulated atmospheric conditions. Our findings will contribute to reducing uncertainties in the representation of marine aerosol-cloud interactions in climate models, enhancing our understanding of their role in the Earth's climate system.

How to cite: Kim, N., Abdelmonem, A., Umo, N. S., Wagner, R., Lacher, L., Möhler, O., Li, H., Saathoff, H., Kim, K. H., Park, D.-H., Ahn, C., Kim, D. H., Yim, U. H., Yum, S. S., and Choi, S.: The Impact of Atmospheric Photochemistry on Marine Aerosols: Ice Nucleation and Droplet Activation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8753, https://doi.org/10.5194/egusphere-egu25-8753, 2025.

EGU25-9444 | Posters on site | AS3.6

Aging of feldspar ice nucleation particles immersed in water: the loss of ice-nucleation efficiency of mineral particles in clouds. 

Albert Verdaguer, Júlia Canet, Laura Rodríguez, Maite Garcia-Valles, Galit Renzer, Mischa Bonn, and Konrad Meister

The challenges of global warming and climate change demand climate models with accurate projections to effectively plan adaptation and mitigation strategies. However, significant uncertainties persist in current climate models. One key uncertainty involves the behavior of mixed-phase clouds, which consist of supercooled droplets and ice crystals. The dynamics between the phases within these clouds are critical to understanding precipitation and cloud albedo, both of which influence the regulation of global warming [1].

Aerosol particles capable of nucleating ice, known as ice-nucleating particles (INPs), play a vital role in these mixed-phase dynamics. Numerous studies have examined how materials' surface properties modify water structure at the interface, modifying their ice nucleation activity [2]. Among the various INPs present in the atmosphere, feldspars have garnered substantial attention over the past decade due to their high nucleation efficiency. This efficiency has been shown to be affected by felspar surface properties such as surface chemistry, structure or morphology [3]

In this presentation, we will share our analysis of feldspar samples collected from various mines in Europe and Africa, focusing on the evolution of their ice-nucleation efficiency after prolonged immersion in water. Using droplet-freezing assay experiments, we identified different categories of ice-nucleation sites, utilizing an analytical method developed by our team [4]. We investigated the evolution of these site families over time in water, finding that some sites disappeared while others remained stable.X-ray diffraction studies show that the feldspar samples used in the previous tests undergo weathering and evolve to stable mineral and/or amphipathic phases under new conditions. Our results demonstrate that feldspar particles within clouds can undergo transformations when immersed in water droplets, altering their ice-nucleation efficiency over timescales of just a few weeks.

[1]“Ice-Nucleating Particles That Impact Clouds and Climate: Observational and Modeling Research Needs” S. M. Burrows et al. Rev. Geophys. 60 (2) e2021RG000745 (2022)

[2]” Water at surfaces and interfaces: From molecules to ice and bulk liquid.” T.K. Shimizu, S. Mayer, A. Verdaguer, J.J. Velasco-Velez, M. Salmeron. Progress in Surface Science 4, 87(2018).

[3]“Pores Dominate Ice Nucleation on Feldspars” E. Pach and A. Verdaguer J. Phys. Chem. C 123, 34, 20998–21004, (2019)

[4] “HUB: A method to model and extract the distribution of ice nucleation temperatures from drop-freezing experiments” I. de Almeida Ribeiro, K. Meister, V. Molinero, Atmospheric Chemistry and Physics, 23 (10), 5623-5639, (2023)

 

How to cite: Verdaguer, A., Canet, J., Rodríguez, L., Garcia-Valles, M., Renzer, G., Bonn, M., and Meister, K.: Aging of feldspar ice nucleation particles immersed in water: the loss of ice-nucleation efficiency of mineral particles in clouds., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9444, https://doi.org/10.5194/egusphere-egu25-9444, 2025.

EGU25-13737 | Posters on site | AS3.6

A new instrument for measuring ice-nucleating particles in the free troposphere and at temperatures relevant for cirrus formation: development and first applications 

Ottmar Möhler, Pia Bogert, Alexander Böhmländer, Nicole Büttner, Joachim Curtius, Larissa Lacher, Jann Schrod, and Romy Ullrich

A minor and strongly temperature-dependent fraction of atmospheric aerosols, called Ice Nucleating Particles (INPs), is known to impact the weather and climate systems by inducing the formation of ice in mixed-phase and cirrus clouds. There is increasing evidence that INPs not only induce the formation of precipitation in particular over continental areas, but also have an important impact on the radiative properties of a number of cloud types throughout the troposphere. For cirrus formation, the abundance and types of INPs play important roles in the interplay between heterogeneous and homogeneous ice nucleation pathways, leading to either net cooling or heating of cirrus clouds in the global climate system.

During the previous years, the new instrument PINEair was developed for measuring INPs at cirrus formation temperatures between -40°C and -65°C and ice supersaturations of up to about 100%. The new instrument can be operated both onboard research aircrafts or at high altitude mountain stations. It is based on the PINE (Portable Ice Nucleation Experiment) instrument, which was developed for laboratory experiments on ice nucleation processes and for automated operation during longer-term INP monitoring activities in the field. PINEair is developed and optimized for direct sampling in the free troposphere.

This contribution will explain the working principle of the new instrument, describe the development and setup of the prototype version, discuss the results of first INP measurements both in the laboratory and at a high-altitude mountain station, and outlines the next steps for building the final aircraft-based version of PINEair.

How to cite: Möhler, O., Bogert, P., Böhmländer, A., Büttner, N., Curtius, J., Lacher, L., Schrod, J., and Ullrich, R.: A new instrument for measuring ice-nucleating particles in the free troposphere and at temperatures relevant for cirrus formation: development and first applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13737, https://doi.org/10.5194/egusphere-egu25-13737, 2025.

EGU25-13928 | ECS | Posters on site | AS3.6

Do bioaerosols or mineral dust dominate the global population of ice-nucleating particles? 

Marios Chatziparaschos, Stelios Myriokefalitakis, Nikos Kalivitis, Nikos Daskalakis, Athanasios Nenes, Maria Gonçalves Ageitos, Montserrat Costa-Surós, Carlos Pérez García-Pando, Mihalis Vrekoussis, and Maria Kanakidou

Ice processes in mixed-phase clouds (MPC) are a key source of uncertainty in climate predictions due to complex aerosol-cloud interactions. This study improves a global chemistry-transport model by incorporating advanced laboratory-based parameterizations to assess the contributions of diverse ice nucleating particle (INP) sources: mineral dust (K-feldspar and quartz), marine primary organic aerosols (MPOA), and terrestrial primary biological aerosol particles (PBAP). The results reveal distinct roles for each source: PBAP dominate ice formation at lower altitudes in warmer conditions, particularly in tropical regions and during the Northern Hemisphere summer. Dust-derived INP prevail at high altitudes across all seasons, especially in polar regions and colder temperatures, while MPOA-derived INPs are most influential at low altitudes in the Southern Hemisphere, notably in subpolar and polar areas. The model achieves its highest predictive accuracy when dust and marine aerosols are treated as independent sources of INP, while PBAP, though significant for warm-temperature ice nucleation at low altitudes, contribute less to improving model-observation agreement. These findings underscore the need for explicitly representing dust, marine, and biological aerosols as distinct contributors to ice formation in climate models, offering a pathway to more accurate predictions of cloud processes and their impacts on climate systems.

How to cite: Chatziparaschos, M., Myriokefalitakis, S., Kalivitis, N., Daskalakis, N., Nenes, A., Gonçalves Ageitos, M., Costa-Surós, M., Pérez García-Pando, C., Vrekoussis, M., and Kanakidou, M.: Do bioaerosols or mineral dust dominate the global population of ice-nucleating particles?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13928, https://doi.org/10.5194/egusphere-egu25-13928, 2025.

EGU25-15357 | Orals | AS3.6

Polysaccharides - Important Constituents of Ice Nucleating Particles of Marine Origin 

Roland Schrödner, Susan Hartmann, Brandon Hassett, Markus Hartmann, Manuela van Pinxteren, Khanneh Wadinga Fomba, Frank Stratmann, Hartmut Herrmann, Mira Pöhlker, and Sebastian Zeppenfeld

Ice formation processes influence the radiative properties, precipitation formation and consequently cloud life time in these mixed-phase clouds. Primary ice formation is enabled by so-called ice nucleating particles (INPs). In remote marine regions such as the Southern Ocean, where INP concentrations are naturally low (McCluskey et al., 2018; Tatzelt et al., 2022), discrepancies to atmospheric observations in the representation of cloud phase with strong biases in radiative effects were identified in atmospheric models (Vergara-Temprado et al., 2018). To improve atmospheric models, a better understanding of INP sources, such as sea spray aerosol, INP properties and a physical-sound INP description are needed.

Ice nucleating macromolecules (INMs), that are produced by marine microorganisms, have been described to potentially enter the atmosphere as part of sea spray aerosol (DeMott et al., 2016; Wilson et al., 2015). While INMs produced from terrestrial micro- and more complex organisms could be attributed to e.g. specific proteins and polysaccharides (e.g., Dreischmeier et al., 2017, Frohlich-Nowoisky et al., 2015), we are lacking knowledge about the chemical identity of INMs from the marine biosphere. A polysaccharidic nature of marine INMs is likely as free glucose, a degradation product of polysaccharides and non-ice active monosaccharide, scales with ice activity of Arctic surface seawater (Zeppenfeld et al., 2019).

In this study, we present polysaccharides produced from aquatic eukaryotic microorganisms (incl. thraustochytrid, yeast, filamentous fungus) as relevant ice nucleating macromolecules (INMs) originating from the marine biosphere. In these and samples using polysaccharide standards, it could be shown that normalization by the polysaccharide mass in the sample harmonizes the freezing spectra across different microorganism and standard samples. We parameterized polysaccharidic INMs based on classical nucleation theory and applied this parameterization on global model simulations. A comparison with currently available atmospheric INP observations over the oceans demonstrates a 44% contribution of polysaccharidic INMs to the total marine INPs in the temperature range from -15 °C to -20 °C (Fig. 1). The importance of polysaccharidic INMs is highlighted for remote marine regions.

 

DeMott, P.J., et al. (2016). Proceedings of the National Academy of Sciences 113, 5797-5803.

Dreischmeier, K., et al. (2017). Scientific Reports 7.

Frohlich-Nowoisky, J., et al. (2015). Biogeosciences 12, 1057-1071.

McCluskey, C.S., et al. (2018). Geophysical Research Letters 45, 11989-11997.

Tatzelt, C., et al. (2022). Atmospheric Chemistry and Physics 22, 9721-9745.

Vergara-Temprado, J., et al. (2018). Proceedings of the National Academy of Sciences 115, 2687-2692.

Wilson, T.W., et al. (2015). Nature 525, 234-+.

Zeppenfeld, S., et al. (2019). Environmental Science & Technology 53, 8747-8756.

How to cite: Schrödner, R., Hartmann, S., Hassett, B., Hartmann, M., van Pinxteren, M., Fomba, K. W., Stratmann, F., Herrmann, H., Pöhlker, M., and Zeppenfeld, S.: Polysaccharides - Important Constituents of Ice Nucleating Particles of Marine Origin, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15357, https://doi.org/10.5194/egusphere-egu25-15357, 2025.

EGU25-16405 | ECS | Posters on site | AS3.6

Sensitivity studies on secondary ice processes using detailed microphysics scheme 

Noémi Sarkadi and István Geresdi

Ice formation in clouds occurs over a wide temperature range (-5°C to -40°C) during primary and secondary ice formation. In most clouds, primary ice formation (PIP) is generated by ice-forming aerosol particles (INP) through heterogeneous nucleation. Observations show that the concentration of ice crystals often exceeds the concentration of available active ice nuclei. This suggests that ice crystals can be generated by secondary processes (SIP). In contrast to PIP, the range of possible processes for SIP is not yet fully understood.

The aim of this study is to identify what are the dominant SIP mechanisms at different environmental conditions, such as temperature, liquid water content, primary ice formation and different CCN and INP concentrations.

At the current state of the research we have performed numerical experiments to study the impact of the different ice splintering mechanisms (due the freezing of the water drops; ice – ice collision and Hallett-Mossop process) at different environmental conditions. A detailed microphysics scheme (University of Pécs-NCAR Bin scheme) implemented in a 2D kinematic framework were used to perform the numerical experiments.  

How to cite: Sarkadi, N. and Geresdi, I.: Sensitivity studies on secondary ice processes using detailed microphysics scheme, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16405, https://doi.org/10.5194/egusphere-egu25-16405, 2025.

EGU25-16421 | ECS | Posters on site | AS3.6

Fragmentation in Collisions of Snow with Graupel/Hail: New Formulation fromField Observations 

Martanda Gautam, Deepak Waman, Sachin Patade, Akash Deshmukh, Freddy Paul, Paul Smith, Aaron Bansemer, Marcin Jackowicz-Korczynski, and Vaughan Phillips

Secondary ice production (SIP) is believed to be responsible for the majority of ice particles observed in precipitating clouds with temperatures above −36°C, based on various field observations from both aircraft and ground-based studies worldwide. One known mechanism of SIP is the fragmentation of ice particles during collisions. This process has been explored using a theoretical model, which has been incorporated into the microphysical schemes of some atmospheric models, where it has been shown to significantly influence cloud glaciation and radiative properties. However, there has been a lack of experimental field studies, particularly those involving naturally falling snowflakes, to better understand this specific SIP mechanism. This study presents the first field measurements of fragmentation during collisions between naturally falling snowflakes and graupel/hail particles, using a newly designed portable chamber deployed outdoors in northern Sweden. Based on these field observations, we refined the existing model for predicting the number of fragments produced by collisions between snow and graupel/hail. The data revealed that, on average, dendritic snowflakes (3–12 mm) produced about 12 fragments per collision, while nondendritic snowflakes (1–3 mm) produced around 1 fragment. This represents an increase in predicted fragment numbers compared to our original model published in 2017. The updated fragmentation model for ice–ice collisions can now be integrated into atmospheric models’ microphysical schemes.

How to cite: Gautam, M., Waman, D., Patade, S., Deshmukh, A., Paul, F., Smith, P., Bansemer, A., Jackowicz-Korczynski, M., and Phillips, V.: Fragmentation in Collisions of Snow with Graupel/Hail: New Formulation fromField Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16421, https://doi.org/10.5194/egusphere-egu25-16421, 2025.

EGU25-16438 | ECS | Posters on site | AS3.6

Dependence of ice nucleation activity on mineralogy and particle size of surface dust from Morocco and Iceland in immersion freezing mode. 

Sebastian Vergara Palacio, Agnesh Panta, Andreas Baer, Adolfo González-Romero, Xavier Querol, Konrad Kandler, Carlos Pérez García-Pando, Corinna Hoose, and Martina Klose

Mineral dust is one of the most abundant types of aerosol particles in the atmosphere, playing a crucial role in various atmospheric processes. A key interaction within clouds is its ability to produce ice-nucleating particles (INPs), influencing cloud properties such as phase, lifetime, and water content. The efficiency of mineral dust as INPs depends on factors such as mineralogy, composition, and particle size. This study investigates the role of particle size and mineralogy in INP efficiency, contrasting Morocco and Iceland, i.e. a mid- and a high-latitude dust sources by using developed parameterizations in ICON-ART.

For this purpose, we used experimental results obtained with the AIDA chamber and the INSEKT freezing assay. The experiments tested ice production in immersion freezing mode for samples from Morocco and Iceland with different size distributions including large particles (greater than 10 µm in diameter). Our analysis revealed notable differences in INP efficiency for the two source locations. The ice nucleation active surface site (INAS) density indicated no significant size dependence for Moroccan samples. In contrast, Icelandic samples exhibited a subtle size dependence, with larger particles showing slightly reduced activity. This behavior was linked to the dust mineralogical composition, specifically the presence of pyroxene. For Icelandic samples, the pyroxene relative volume fraction decreases with increasing particle size, which correlates with the observed reduction in INP activity.

Based on these insights, we developed a new INAS density parameterization for Icelandic dust and proposed a modification to the equation used to compute INAS density to represent the variation in the efficiency of ice nucleation activity at different diameters. We then used this new parameterization in the ICON-ART model to test the impact of a different ice nucleation efficiency of Icelandic dust on a regional scale. By using ICON-ART global dust distributions were simulated and surface dust was used as input for the new parameterizations at different temperatures, recreating typical field experiments on ice nucleation.

This study underscores the importance of characterizing both mineralogical composition and its size dependence when developing parameterizations for INP activity. Our results challenge the assumption that larger particles are always more efficient INPs in immersion freezing mode, as their efficiency is linked not only to their large surface areas but also to their mineralogical composition, which can vary for different sizes. Additionally, size distribution shapes should be considered as another factor influencing INP concentration as the abundance of particles at different diameters might determine the efficiency of the sample.

How to cite: Vergara Palacio, S., Panta, A., Baer, A., González-Romero, A., Querol, X., Kandler, K., Pérez García-Pando, C., Hoose, C., and Klose, M.: Dependence of ice nucleation activity on mineralogy and particle size of surface dust from Morocco and Iceland in immersion freezing mode., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16438, https://doi.org/10.5194/egusphere-egu25-16438, 2025.

EGU25-16455 | ECS | Orals | AS3.6

Modelling Ice Nucleating Particles from High-Latitude Sources to Reproduce Arctic In Situ Concentrations 

Anderson Da Silva, Louis Marelle, Rémy Lapere, and Jean-Christophe Raut

Ice nucleating particles (INPs) are crucial for the formation and evolution of ice-containing clouds, particularly in the Arctic, where INPs are scarce. Their influence on the radiative budget and its evolution in a warming climate remains an active area of research. INP sources in the Arctic are diverse, ranging from long-range transported mineral dust to local marine biological particles. However, their representation in regional and global models remains uncertain.

In this study, we implement emissions of marine primary organic aerosols (MPOAs) and high-latitude dust in the WRF-Chem chemistry-transport model. Using a set of offline ice nucleation schemes, we evaluate the contributions of different aerosol species to INP production. Model outputs are compared with in situ INP measurements from recent Arctic campaigns, assessing the performance of nucleation schemes in terms of particle concentrations.

Modeled MPOAs appear to be a major source of INP, but only because the model strongly overestimates organic aerosols. While certain nucleation schemes successfully reproduce baseline observed INP concentrations, they fail to capture the occasional sharp drops observed in freezing temperature. By incorporating Lagrangian dispersion modelling, we demonstrate that in-cloud removal of efficient INP along the likely transport pathways of INPs may account for the observed reductions in concentrations. Building on this insight, we implement, in WRF-Chem, new INP emission schemes sensitive to online nucleation processes during atmospheric transport. These updated tracers show improved agreement with in situ INP observations, offering new perspectives for more accurate representation of Arctic INPs in models.

How to cite: Da Silva, A., Marelle, L., Lapere, R., and Raut, J.-C.: Modelling Ice Nucleating Particles from High-Latitude Sources to Reproduce Arctic In Situ Concentrations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16455, https://doi.org/10.5194/egusphere-egu25-16455, 2025.

EGU25-18611 | ECS | Posters on site | AS3.6

An Investigation of the Validity of Secondary Ice Production Parameterizations in WRF in an Orographic Environment with Preliminary Data From CHOPIN 

Ali Waseem, Paraskevi Georgakaki, Nicole Clerx, Romanos Foskinis, Carolina Molina, Maria Gini, Anne-Claire Billault-Roux, Paul Zieger, Konstantinos Eleftheriadis, Alexis Berne, and Athanasios Nenes

Mixed-phase clouds play a key role in weather and climate and are a major challenge to model accurately in models. Nevertheless, considerable progress on modeling microphysical processes in mixed-phase clouds, such as primary and Secondary Ice Production (SIP) has led to systematic improvements in model performance.

Here, we use the Weather Research and Forecasting (WRF) model with the EPFL/FORTH cloud microphysical scheme improvements (Georgakaki et al., 2024) to simulate weather, cloud formation and precipitation events sampled during the Cleancloud Helmos OrograPhic sIte experimeNt (CHOPIN) campaign during the Fall of 2024 to Spring of 2025. CHOPIN takes place at Mount Helmos in the Peloponnese, Greece, an ideal location for studying aerosol-cloud interactions in orographic mixed-phase clouds.

The performance of SIP parameterizations in WRF are evaluated by (i) comparing model outputs to meteorological data from both a fixed weather station and radiosondes, (ii) comparing the model's ability to capture boundary layer dynamics using atmospheric trace gasses as a proxy, and (iii) the model's ability to capture cloud formation using reflectivity from a Ka-band (35 GHz) radar, by comparing the output of a forward operator (radar simulation) from the modeled cloud fields. Through the modelling of various days between October 2024 and December 2024, as well as a clustering analysis of the radar reflectivities, the capabilities of using SIP parameterizations in WRF are assessed with respect to particular cloud regimes. We see that distinct improvements are seen in the simulated fields, particularly for the clusters associated with cloud fields that are developed and regional in nature.

How to cite: Waseem, A., Georgakaki, P., Clerx, N., Foskinis, R., Molina, C., Gini, M., Billault-Roux, A.-C., Zieger, P., Eleftheriadis, K., Berne, A., and Nenes, A.: An Investigation of the Validity of Secondary Ice Production Parameterizations in WRF in an Orographic Environment with Preliminary Data From CHOPIN, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18611, https://doi.org/10.5194/egusphere-egu25-18611, 2025.

EGU25-20340 | ECS | Orals | AS3.6 | Highlight

Vertical transport and segregation of ice nucleating particles in deep convective clouds 

Jonas Schaefer, Sarah Grawe, Hans-Christian Clemen, Johannes Schneider, Bruno Wetzel, Stephan Mertes, Daniel Sauer, Jennifer Wolf, Johanna Mayer, Laura Tomsche, Roland Schrödner, Silvia Henning, Tina Jurkat-Witschas, Christiane Voigt, Helmut Ziereis, Theresa Harlaß, Mira Pöhlker, and Frank Stratmann

Ice nucleating particles (INP) play a crucial role in shaping Earth's weather and climate by influencing cloud properties and precipitation behavior. However, their abundance in the free troposphere and transport mechanisms remain poorly characterized. INP sources are generally at ground level and large-scale atmospheric vertical motion, which could lift INP from the ground into the free troposphere is often accompanied by cloud formation. The fate of INP in clouds, whether they are lifted up or washed out, is still mostly unclear.

During the HALO aircraft campaign CIRRUS-HL in June and July 2021, aerosol particles and cloud particle residuals were collected on filters using the airborne High-volume flow aERosol particle filter sAmpler (HERA). Offline laboratory analysis of these filters yield immersion mode INP concentrations. Here we present a case study with which we investigate the vertical transport and cloud processing of INP in deep convective clouds (DCC) by analyzing residuals in clouds and aerosol particles in cloud-free inflow and outflow of  DCC.

Our results show that INP active above -15°C are diminished in anvil cirrus cloud particle residuals, while INP active below -20°C are found in high concentrations in DCC outflow air. We propose that precipitation formation wash out INP active at high temperatures, while INP active at low temperatures are efficiently transport upwards into the upper troposphere with ambient temperatures below -40°C, i.e., far below the INP immersion freezing temperature. With that, DCC outflow INP concentration are at least two order of magnitude above typical upper tropospheric/lower stratospheric INP concentrations derived throughout the CIRRUS-HL campaign.

This study provides new insights into the vertical transport and cloud processing of INP in the free troposphere with implications for balance between heterogeneous and homogeneous freezing in cirrus clouds.

How to cite: Schaefer, J., Grawe, S., Clemen, H.-C., Schneider, J., Wetzel, B., Mertes, S., Sauer, D., Wolf, J., Mayer, J., Tomsche, L., Schrödner, R., Henning, S., Jurkat-Witschas, T., Voigt, C., Ziereis, H., Harlaß, T., Pöhlker, M., and Stratmann, F.: Vertical transport and segregation of ice nucleating particles in deep convective clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20340, https://doi.org/10.5194/egusphere-egu25-20340, 2025.

EGU25-20540 | Orals | AS3.6

 A new parameterization for simulating global ice-nucleating particle concentrations based on long-term  measurements with a network of expansion chambers  

Benjamin Murray, Ross Herbert, Carslaw Ken, Tarn Mark, Daily Martin, Möhler Ottamr, Lacher Larissa, Böhmländer Alex, Büttnar Nicole, Hiranuma Naruki, Pantoya Aiden, Freney Evelyn, Planche Céline, Canzi Antoine, and Tian Ping

The most important milestone in a mixed-phase cloud’s life is the initiation of ice. If we cannot sufficiently capture this process in weather and climate models then it is unlikely that the cloud’s properties and evolution will be accurately represented. Here we focus on improving the representation of ice-nucleating particles (INPs), which are the fundamental link between aerosols and primary ice production in mixed-phase clouds.

We use a newly collated dataset of 20 campaigns from across the northern hemisphere using Portable Ice Nucleation Experiment (PINE) instruments together with nudged simulations of the UK Earth System Model, which includes a modal aerosol microphysics model. We use 30,000 collocated PINE measurements and output from the UK Earth System Model to derive a new parameterization that links the full dust size distribution to an INP concentration. We base the functional shape of the parameterization assuming the presence of a mineral component and a biogenic ice-nucleating component, which is consistent with recent understanding.

The new parameterization reproduces 80% of the 30,000 PINE measurements within a factor of 2 and 96% within a factor of 10, and UKESM simulations correctly represent many of the short term synoptic events seen in the PINE time series. The new parameterization also performs considerably better than alternative parameterizations. The analysis shows that the INP concentrations are correlated with the dust surface area but cannot be explained by the mineral component (K-feldspar) alone. The new parameterization is consistent with the spread of laboratory derived activity for mineral soils that contain biogenic material, suggesting a biogenic ice-nucleating component associated with dust is prevalent throughout the northern hemisphere.

How to cite: Murray, B., Herbert, R., Ken, C., Mark, T., Martin, D., Ottamr, M., Larissa, L., Alex, B., Nicole, B., Naruki, H., Aiden, P., Evelyn, F., Céline, P., Antoine, C., and Ping, T.:  A new parameterization for simulating global ice-nucleating particle concentrations based on long-term  measurements with a network of expansion chambers , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20540, https://doi.org/10.5194/egusphere-egu25-20540, 2025.

EGU25-970 | ECS | PICO | CL4.14

Studies to Control Resuspension of Dust from Playgrounds 

Umangi Mehta, V.S. Vamsi Botlaguduru, Manaswita Bose, and Virendra Sethi

Dust resuspension from playgrounds can be a major contributor to urban air pollution. To address this issue, mitigation strategies such as the use of windscreens, water sprinkling, and dust suppressants have been reported in literature (Dong et al., 2007; Jeon et al., 2021; Taylor et al., 2015). However, the effectiveness of these measures is dependent on the soil type, wind patterns affected by green cover and surrounding. This study aims to provide insights into the effectiveness of different dust control strategies and offer potential solutions for widespread application in urban playgrounds. Laboratory-scale experiments were conducted to evaluate the influence of particle size distribution, wind speed and moisture content on dust resuspension from three different soil types. Numerical simulations will be performed to simulate the wind patterns that influence dust resuspension for a selected playground in Mumbai.

How to cite: Mehta, U., Botlaguduru, V. S. V., Bose, M., and Sethi, V.: Studies to Control Resuspension of Dust from Playgrounds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-970, https://doi.org/10.5194/egusphere-egu25-970, 2025.

EGU25-1057 | ECS | PICO | CL4.14

Dust Aerosol and Water Vapor Radiative Effects: A Multi-Campaign Analysis of ASKOS and ORCESTRA/PERCUSION Over the Atlantic 

Dimitra Kouklaki, Alexandra Tsekeri, Anna Gialitaki, Kyriakoula Papachristopoulou, Panagiotis-Ioannis Raptis, Bernhard Mayer, Claudia Emde, Silke Groß, Eleni Marinou, Vassilis Amiridis, and Stelios Kazadzis

Aerosols significantly attenuate solar radiation and influence atmospheric thermodynamic stability, particularly over regions like the Atlantic, impacting Earth's energy budget and climate through radiative heating or cooling. Quantifying these effects is challenging due to aerosol diversity and complexity. For desert dust particles, the difficulty lies in defying their optical properties and accurately monitoring their extensive distribution.

This study aims to assess the radiative effects of dust aerosols and water vapor (WV), and their impact on atmospheric heating rates, by adopting non-spherical particle shapes and their intrinsic microphysical and optical properties during severe dust events. To achieve this, ground-based, airborne, and satellite observations are employed along with Radiative Transfer (RT) modeling, and more precisely the libRadtran RT package (Mayer and Kylling, 2005; Emde et al., 2016). The study utilizes data from two experimental campaigns – ASKOS and ORCESTRA/PERCUSION – both conducted in the Atlantic region during peak trans-Atlantic dust transport periods, in summers of 2022 and 2024.

In the frame of the ASKOS ESA Joint Aeolus Tropical Atlantic Campaign (JATAC), we utilized ground-based remote sensing and airborne in-situ observations, including solar radiation and airborne meteorological profiles. Microphysical properties from UAVs, MOPSMAP (Gasteiger and Wiegner, 2018) and TAMUdust2020 (Saito et al., 2021) scattering databases were used to derive dust optical properties considering a mixture of spheroidal and irregular-hexahedra shapes. Multi-wavelength lidar measurements contributed to the validation of the optical properties and dust vertical distribution. RT simulations incorporated WV concentration, to investigate dust-WV-solar radiation interactions under clear sky conditions. The simulated broadband shortwave radiation was, finally, compared with the ground-based solar radiation measurements.

A second case study was performed, leveraging ORCESTRA/PERCUSION campaign (https://orcestra-campaign.org/percusion.html) synergistic airborne measurements. This campaign incorporated a comprehensive suite of airborne instruments, providing, amongst others, radiation measurements, meteorological profiles, and extensive lidar measurements. Radiation at the top of the atmosphere (TOA) from the EarthCARE ESA mission supported comprehensive closure studies at TOA and at aircraft level.

Acknowledgements

This research was financially supported by the PANGEA4CalVal project (Grant Agreement 101079201) funded by the European Union, the CERTAINTY project (Grant Agreement 101137680) funded by Horizon Europe program and the AIRSENSE project which is part of Atmosphere Science Cluster of ESA’s EO Science for Society programme. DK, ΑΤ, ΚP, PR and SK would like to acknowledge COST Action HARMONIA (International network for harmonization of atmospheric aerosol retrievals from ground-based photometers), CA21119, supported by COST (European Cooperation in Science and Technology).

References

Mayer, B., Kylling, A.: Technical note: The libRadtran software package for radiative transfer calculations - description and examples of use. Atmos. Chem. Phys., 5(7), 1855–1877, 2005.

Emde, C., et al.: The libRadtran software package for radiative transfer calculations (version 2.0.1), Geoscientific Model Development, 9(5), 1647–1672, 2016.

Gasteiger, J. and Wiegner, M.: MOPSMAP v1.0: a versatile tool for the modeling of aerosol optical properties, Geosci. Model Dev., 11, 2739–2762, https://doi.org/10.5194/gmd-11-2739-2018, 2018.

Saito, M., et al.: A comprehensive database of the optical properties of irregular aerosol particles for radiative transfer simulations, J. Atmos. Sci., in press, https://doi.org/10.1175/JAS-D-20-0338.1, 2021.

 

 

How to cite: Kouklaki, D., Tsekeri, A., Gialitaki, A., Papachristopoulou, K., Raptis, P.-I., Mayer, B., Emde, C., Groß, S., Marinou, E., Amiridis, V., and Kazadzis, S.: Dust Aerosol and Water Vapor Radiative Effects: A Multi-Campaign Analysis of ASKOS and ORCESTRA/PERCUSION Over the Atlantic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1057, https://doi.org/10.5194/egusphere-egu25-1057, 2025.

EGU25-1247 | ECS | PICO | CL4.14

Vertical Profiling of Dust Layers in the Eastern Mediterranean: Sources, Dynamics, and Impacts 

Irina Rogozovsky, Albert Ansmann, Kevin Ohneiser, Holger Baars, Ronny Engelmann, Julian Hofer, and Alexandra Chudnovsky

Dust pollution is a critical environmental challenge with far-reaching impacts on climate and health. Despite its significance, no unified methodology exists for identifying dust-contaminated days, leading to inconsistencies across disciplines. The most widely used approaches often rely on ground-based measurements to classify dust events. However, these methods may overlook lofted dust layers. We used a ground-based lidar system to detect and classify dust layers and compared the results to widely adopted methods. Surprisingly, at least 50% of dust-contaminated days identified by lidar were missed by traditional surface-based methods. This gap underscores the critical role of vertical profiling in accurately capturing dust presence, which is vital for improving health impact studies and climate models. Our results highlight the challenges of distinguishing between anthropogenic and natural dust events using only ground-based measurements, as many measurement approaches classify mixed aerosols as dust, potentially leading to biased exposure estimates. In addition, vertical profiling and layering data revealed distinct pollution configurations in the Eastern Mediterranean (EM) region, ranging from purely anthropogenic layers to complex mixtures of marine aerosols, anthropogenic pollution, and desert dust. Results reveal that dust layers in the EM often extend vertically up to 10 km, with depths reaching 6.3 km. We used air masses back trajectory analysis to identify the source of particles for each layering type, and found 2 distinct dust sources, North African mostly pure dust and Middle Eastern dust with anthropogenic component. Finally, we analysed the uncertainties of the conventional satellite-derived AOD measurements. It was found the presence of lofted dust layers or mixed aerosols challenge the retrieval accuracy, gaining crucial insights into the limitations of satellite-derived AOD in representing complex atmospheric environments, especially in dust dominated regions. The holistic approach applied in our study is essential for understanding the dynamic interplay between pollution sources and atmospheric interactions, particularly in regions like the EM, which serve as a crossroads for diverse aerosol types.

How to cite: Rogozovsky, I., Ansmann, A., Ohneiser, K., Baars, H., Engelmann, R., Hofer, J., and Chudnovsky, A.: Vertical Profiling of Dust Layers in the Eastern Mediterranean: Sources, Dynamics, and Impacts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1247, https://doi.org/10.5194/egusphere-egu25-1247, 2025.

EGU25-2589 | PICO | CL4.14

Can we infer a mineralogical signature of dust hot spots using EMIT hyperspectral data? 

Paul Ginoux, Philip G. Brodrick, Maria Gonçalves Ageitos, Greg S. Okin, Carlos Pérez Garcia-Pando, David R. Thompson, and Robert O. Green

With more than 20 years of MODIS twice daily global measurements, dust hot spots have been
located using the extrema of frequency of occurrence of Dust Optical Depth (DOD) derived from
MODIS Deep Blue aerosol products. We know that these hot spots have a geomorphological signature (cf. Prospero et al., 2002; Baddock et al., 2016) but does it also imply that they have a mineralogical signature? This is important to know as mineralogy controls the sign and amplitude of dust interactions with the Earth's climate systems, in particular in terms of radiative forcing, ice cloud formation, rain water acidity, snow albedo, ocean bio-geochemistry. By overlaying over the dust hot spots, the soil mineralogy retrieved from the hyperspectral instrument NASA-JPL Earth Surface Mineral Dust Source Investigation (EMIT) over almost 3 years, our presentation will show that mineralogical content of dust hot spots is region specific.

How to cite: Ginoux, P., Brodrick, P. G., Gonçalves Ageitos, M., Okin, G. S., Pérez Garcia-Pando, C., Thompson, D. R., and Green, R. O.: Can we infer a mineralogical signature of dust hot spots using EMIT hyperspectral data?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2589, https://doi.org/10.5194/egusphere-egu25-2589, 2025.

EGU25-3373 | ECS | PICO | CL4.14

Analysis of PM2.5 Impacts from Agricultural Vinyl Waste Treatment Processes and Uncollected Waste 

Hyunjun Park, Minseon Park, Namhoon Lee, and Hui-Young Yun

The treatment of agricultural plastic waste is a critical source of fine dust (PM2.5) emissions, contributing significantly to air pollution. Uncollected plastic waste, predominantly subjected to open-air incineration, exacerbates this issue, underscoring the need for comprehensive management strategies.

This study aims to predict PM2.5 emissions from agricultural plastic waste treatment processes and quantify the contribution of uncollected plastic waste to air pollution, providing a novel analysis of the relative environmental impact of these two waste management pathways. Using the CAPSS model and process-specific emission factors, PM2.5 emissions from shredding, crushing, and sorting processes were estimated based on the annual average agricultural plastic waste generation of 314,000 tons from 2016 to 2021.

Predicted PM2.5 emissions per ton of treated waste were 0.00012 kg, 0.00075 kg, and 0.00043 kg for shredding, crushing, and sorting processes, respectively. By 2030, cumulative emissions from these processes are expected to reach 25.09 kg, 156.84 kg, and 89.92 kg. In contrast, uncollected vinyl waste subjected to open-air incineration is estimated to generate approximately 725,779.45 kg of PM2.5 by 2030, a figure nearly 2,600 times higher than emissions from treated waste.

The findings highlight the disproportionate environmental impact of uncollected vinyl waste compared to treated waste. This study underscores the urgency of improving collection rates and optimizing treatment processes for agricultural vinyl waste. Policy recommendations include expanding treatment facilities, fostering private-sector recycling initiatives, and enforcing stricter regulations on open-air incineration to mitigate fine dust emissions effectively. Future research should explore the comprehensive evaluation of waste management systems and the development of advanced technologies for reducing PM2.5 emissions.

Acknowledgments

This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)

How to cite: Park, H., Park, M., Lee, N., and Yun, H.-Y.: Analysis of PM2.5 Impacts from Agricultural Vinyl Waste Treatment Processes and Uncollected Waste, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3373, https://doi.org/10.5194/egusphere-egu25-3373, 2025.

EGU25-4448 | ECS | PICO | CL4.14

Detection of seasonal-specific potential source areas of mineral dust on Crete (Greece) based on isotope measurements and mineralogical investigations 

Simon Bitzan, Cécile L. Blanchet, Georgios E. Christidis, Kerstin Schepanski, and Fabian Kirsten

The Sahara is the Earth’s largest dust source, producing dust plumes that impact the whole planet. The eastern Mediterranean is one of the areas significantly affected by Saharan dust and its deposition.
The geochemical and mineralogical composition of the deposited mineral dust particles depend on their source area and on spatiotemporal variability of the source areas.
Although being of great importance for local soil formation and soil distribution, the impact of changes in dust provenance has not been extensively studied in the eastern Mediterranean. Thus, further research is required to characterize dust deposition fluxes, transport trajectories and the geochemical and mineralogical composition of deposited mineral dust.
Modelled trajectories of dust events provide good insights on aeolian transport routes, but if larger distances are covered over land, the exact source area of the deposited material cannot be traced with certainty. The question also arises as to whether the composition of the mineral dust deposited differs due to spatial sorting and thus its influence on the deposition area.
In order to gain insight into the dynamics of dust deposited on Crete, we present results from eight passive deposition traps (marble samplers) that were installed in western Crete at various sites around the Lefka Ori mountains. Monthly sampling was performed between March 2023 and June 2024, which provides us a unique temporal and spatial coverage.
Here we used a multi-proxy fingerprinting approach including Nd-Sr isotopic composition, mineralogy and grain-size distribution. The isotope analyses show a temporal shift in the potential source areas over the year, but no significant spatial differences. This spatial homogeneity in the isotopic signature of deposited dust suggests a minor influence of local inputs, which are characterized by distinct geological contexts, which is confirmed by the mineralogy. Samples with a coarser and well-sorted grain-size distribution likely track larger dust events, as a relatively larger proportion originates from the same source. The aim is to combine the results and thus to highlight and classify the intensity of influence of different source areas on the soil development of western Crete. In the long term, an analysis of back-tracking trajectories is to be carried out and combined with the results of the isotope analyses, which we expect to improve the informative value of the potential source areas.

How to cite: Bitzan, S., Blanchet, C. L., Christidis, G. E., Schepanski, K., and Kirsten, F.: Detection of seasonal-specific potential source areas of mineral dust on Crete (Greece) based on isotope measurements and mineralogical investigations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4448, https://doi.org/10.5194/egusphere-egu25-4448, 2025.

EGU25-4494 | PICO | CL4.14

Unraveling Late Quaternary Climate Dynamics: Insights from the Velika Vrbica Loess-Palaeosol Sequence, Wallachian Basin 

Zoran Perić, Cathal Ryan, Warren Thompson, Milica Radaković, Petar Krsmanović, Helena Alexanderson, and Slobodan Marković

The Velika Vrbica loess-palaeosol sequence (LPS) in northeastern Serbia, located at the westernmost boundary of the Wallachian Basin, provides a high-resolution terrestrial archive of palaeoenvironmental changes spanning Marine Isotope Stages (MIS) 3 to MIS 1. This study integrates optically stimulated luminescence (OSL) dating, magnetic susceptibility (χ), and mass accumulation rates (MAR) to reconstruct climatic and environmental dynamics over the last ~41,000 years. The OSL chronology reveals consistent loess deposition from ~41 ka to 3 ka, with peak accumulation rates during MIS 3 and late MIS 2. Notably, MARs are higher during the interstadial MIS 3 compared to the Last Glacial Maximum (MIS 2), challenging conventional models that associate intensified dust deposition solely with colder glacial phases. This pattern highlights the influence of regional factors such as sediment source proximity, wind dynamics, and variations in sediment trapping efficiency. The χ record highlights fluctuations in pedogenesis and aeolian activity, which broadly correspond to climatic oscillations captured in the NGRIP δ¹⁸O ice core record. These global cold periods align with intensified dust deposition, but substantial MAR values observed during warmer interglacial phases suggest that sedimentation processes in southeastern Europe were influenced by additional, localized drivers. The Velika Vrbica LPS captures detailed environmental responses to Dansgaard-Oeschger (D-O) events, marked by rapid warming and subsequent cooling phases. These responses reflect the sensitivity of southeastern Europe to abrupt climatic shifts and reveal the nuanced relationship between global climatic drivers and regional environmental processes. Notably, the sandy layer deposited between ~32 ka and ~15 ka reflects intensified palaeowind activity during the Last Glacial Maximum, further illustrating the interplay between climate and sedimentation dynamics. Comparison with other LPSs in southeastern Europe highlights the distinct depositional patterns of Velika Vrbica, with pronounced MAR peaks during MIS 3 and considerable variability during MIS 2. These findings diverge from the widely accepted model of loess formation, emphasizing the importance of site-specific factors and regional climatic influences. For example, while most models predict lower dust input during interglacial periods, the Velika Vrbica LPS records substantial dust deposition even during MIS 3 interstadials. This challenges established paradigms and underscores the complexity of loess formation processes in dynamic semi-arid environments. By integrating high-resolution geochronological data with sedimentological and palaeoclimatic analyses, this research provides critical insights into late Quaternary climate dynamics in southeastern Europe. The Velika Vrbica LPS not only enhances our understanding of the region’s environmental history but also contributes to refining global models of loess deposition and dust dynamics. These findings emphasize the need for further site-specific investigations to disentangle the interplay between global climate systems and local environmental processes, thereby advancing our understanding of past climatic variability and its implications for future environmental changes.

How to cite: Perić, Z., Ryan, C., Thompson, W., Radaković, M., Krsmanović, P., Alexanderson, H., and Marković, S.: Unraveling Late Quaternary Climate Dynamics: Insights from the Velika Vrbica Loess-Palaeosol Sequence, Wallachian Basin, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4494, https://doi.org/10.5194/egusphere-egu25-4494, 2025.

EGU25-4612 | ECS | PICO | CL4.14

Westerly jet variations over East Asia since the Last Glacial Maximum: Evidence from Asian dust records in the Mariana Trench  

Yanning Wu, Yifeng Liu, Tao Wu, Chun-Feng Li, Wancang Zhao, Taoran Song, and Liyan Tian

The seasonal migration of the westerly jet (WJ) over East Asia is recognized as a substantial factor in the historical climate of the region, especially regarding spatial and temporal variability of regional rainfall and the dust cycle in the Northern Hemisphere. However, the evolution of East Asian WJ since the Last Glacial Maximum (LGM) remains debated. To enhance our understanding, we investigate the changes in Asian dust sources in sediments from the southern Mariana Trench utilizing trace elements and Sr-Nd isotopes.

According to the geochemical analyses, the eolian dust from the Taklimakan desert is the major dust source to the southern Mariana Trench during most of the LGM. Nevertheless, the Mongolian Gobi Desert became the dominant dust contributor during partial periods of the early LGM. This result can be attributed to changes in the timing of the seasonal WJ transition and the meridional distribution of the WJ. During the LGM, low boreal summer insolation kept the WJ axis south of the Tibetan Plateau throughout the year, which should be accompanied by broad meridional distribution of the WJ affecting mid-to-high latitudes. However, extensive Northern Hemisphere ice sheets prevented the occurrence of the WJ over mid-to-high latitudes. Therefore, the WJ mainly transported the Taklimakan dust. The smaller ice sheets in the early LGM than in the late LGM allowed the WJ to appear over the Mongolian Gobi Desert, favoring the local dust export.

During the mid-Holocene, the trench received a mixed contribution of the Taklimakan and the Mongolian Gobi dust. Strong boreal summer insolation during this period caused the WJ axis to frequently shift to a southwest-northeast orientation and an earlier seasonal WJ transition. This facilitated the transport of dust from both deserts. In the late Holocene, the Taklimakan desert became the dominant dust source, due to a reoriented WJ axis with a west-east orientation and a delayed seasonal transition driven by declining boreal summer insolation.

How to cite: Wu, Y., Liu, Y., Wu, T., Li, C.-F., Zhao, W., Song, T., and Tian, L.: Westerly jet variations over East Asia since the Last Glacial Maximum: Evidence from Asian dust records in the Mariana Trench , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4612, https://doi.org/10.5194/egusphere-egu25-4612, 2025.

EGU25-4644 | ECS | PICO | CL4.14

Intermediate-mode mineral dust aerosols efficiently scatter solar radiation 

Chen Cui, Pengfei Tian, Binrui Wang, and Wenfang Wang

Dust aerosols emitted naturally into the atmosphere play a crucial role in the climate system by scattering and absorbing radiation, which may alter regional aerosol radiative forcing. Aerosol size distributions exhibit a widespread trimodal pattern globally, and the presence of this trimodal distribution affects the scattering properties of the aerosol population. Here, we identify an intermediate mode in the African dust aerosol size distribution, previously overlooked, located between the fine and coarse modes. In regions with high dust loads, dust particles undergo physical processes, including surface fragmentation due to external forces, generating fine fragments with a characteristic size of approximately 0.6 µm. These fragments exhibit strong scattering properties, with a scattering efficiency factor roughly five times that of the fine mode, making them significant contributors to regional cooling effects. However, in recent years, the concentration of the intermediate mode has been gradually decreasing due to regional economic development and desert management, impacting both regional and global environmental and climate effects. This study provides new insights into dust aerosol emissions and improves the parameterization of dust in global climate models. These findings are crucial for enhancing the accuracy of global climate simulations and better quantifying the impact of dust aerosols on the climate.

How to cite: Cui, C., Tian, P., Wang, B., and Wang, W.: Intermediate-mode mineral dust aerosols efficiently scatter solar radiation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4644, https://doi.org/10.5194/egusphere-egu25-4644, 2025.

EGU25-4775 | PICO | CL4.14

Paleoclimate informed simulations for constraining aerosol radiative effects 

Samuel Albani, Natalie M. Mahowald, Longlei Li, Douglas S. Hamilton, and Jasper F. Kok

Aerosol radiative effects are still one of the major sources of uncertainty in terms of a quantitative understanding of climate changes across time scales, despite many advances in the field. Yet, paleodata databases offer the opportunity to constrain to some extent past natural aerosol emissions, allowing to account for aerosol radiative effects in a more realistic way in simulations with Earth System Models, at least from the point of view of amounts and spatial distributions of different aerosol species.

Here we first present the results of simulations conducted with CESM1.0 using paleodust constrained emissions for different equilibrium climate states, then broaden our discussion on the importance of historical and paleoclimate aerosol radiative effects, considering the published literature. We estimated that preindustrial to present-day aerosol radiative effects are affected by emission uncertainties that are just as large as model spread uncertainties (2.8 W m−2). We advocate that more efforts are put into improving and expanding existing paleodata collections and that those available should be taken into account when assessing uncertainties related to aerosol radiative effects. In particular we propose a new intercomparison project (AERO-HISTMIP) that compares outcomes when using multiple emission pathways in CMIP historical simulations.  

How to cite: Albani, S., Mahowald, N. M., Li, L., Hamilton, D. S., and Kok, J. F.: Paleoclimate informed simulations for constraining aerosol radiative effects, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4775, https://doi.org/10.5194/egusphere-egu25-4775, 2025.

EGU25-5652 | ECS | PICO | CL4.14

From Sahara Desert to Ukraine: an integrated study of mineral dust transport 

Yuliia Yukhymchuk, Gennadi Milinevsky, Vassyl Danylevsky, Philippe Goloub, Xuhui Gao, and Xuanyi Wei

In April 2024, the transport of mineral dust from the Sahara Desert was observed over Ukraine. This phenomenon, unusual for the region, resulted in reduced visibility, "red rain," degraded air quality, and altered atmospheric aerosol properties over Kyiv. To better understand the impact of this event, sun photometers and modeling efforts were used to analyze the changes in aerosol characteristics and the atmospheric influence of mineral dust transport. Observations from the AERONET Kyiv station indicated significant changes in aerosol characteristics. Specifically, there was an increase in aerosol optical depth (AOD) and coarse-mode AOD, while the Angstrom exponent (AE) and fine-mode AOD showed a decline. Cluster analysis of these parameters revealed temporal patterns and correlations between the observed changes. The size distribution analysis highlighted the dominant influence of coarse particles. Additionally, the single scattering albedo (SSA) and refractive index values were affected, reflecting the presence of mineral dust compared to typical conditions. The GEOS-Chem chemical transport model further indicated changes in mineral dust concentrations, suggesting its notable impact on Ukraine's territory. Additionally, the HYSPLIT model was utilized in this study to analyze backward trajectories of air masses, providing crucial information about their movement before reaching the territory of Ukraine and identifying their origins.

How to cite: Yukhymchuk, Y., Milinevsky, G., Danylevsky, V., Goloub, P., Gao, X., and Wei, X.: From Sahara Desert to Ukraine: an integrated study of mineral dust transport, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5652, https://doi.org/10.5194/egusphere-egu25-5652, 2025.

EGU25-5908 | ECS | PICO | CL4.14

Towards Convection-Resolving Dust Emission Modelling 

Pascal Kunze, Matthias Faust, Kerstin Schepanski, and Ina Tegen

Dust emissions are closely associated with wind speed and are affected by a variety of meteorological drivers and factors that have effects across different spatial and temporal scales. Global or regional atmospheric dust models employing parameterized convection often encounter difficulties in accurately replicating observed dust emissions. Recent investigations by Garcia-Carreras et al. (2021) have demonstrated significant discrepancies when modeling Northern African dust emissions across various grid scales using either parametrized convection or resolved convection. In order to further clarify the influence of model resolution on dust emissions, an investigation was conducted employing surface winds from two different model studies: the coarse-resolution CMIP-6 model intercomparison study [Eyring et al. (2016)] with parameterized convection and the high-resolution ICON model  simulation that was part of the DYAMOND project [Stevens et al. (2019)], which was computed with explicit convection. Two different dust products were computed using the modelled surface winds: the Dust Uplift Potential (DUP) derived from wind data and an offline dust emission model based on Tegen et al. (2002), which incorporates soil and vegetation effects to simulate dust emission fluxes utilizing gridded surface wind fields. The dust emissions from the different models are evaluated across various source regions, including Northern Africa, the Arabian Peninsula, Central Asia, the Gobi Desert, and the Taklamakan Desert. Convective events such as haboobs particularly necessitate explicit modeling at convection-resolving resolution, which is e.g an important cause of dust emissions in the southern Sahara in northern hemisphere summer. Other local wind systems can be discerned by both high and low-resolution models, albeit at varying magnitudes. In the Gobi region, there is negligible impact of model resolution on dust emissions. These findings could inform further research on modeling dust emission and  transport by providing a basis for improved dust emission parameterizations in large-scale models.

How to cite: Kunze, P., Faust, M., Schepanski, K., and Tegen, I.: Towards Convection-Resolving Dust Emission Modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5908, https://doi.org/10.5194/egusphere-egu25-5908, 2025.

EGU25-6183 | ECS | PICO | CL4.14

Meteorological Drivers of East Asian dust activity in spring 2001-2022 

Feifei Mu and Stephanie Fiedler

East Asian dust storms from the Gobi and the Taklamakan Desert occur frequently in spring. Dust aerosols influence climate through effects on radiation and clouds, and impair air quality with impacts on human health. However, large uncertainties in model simulations of dust aerosols persist. An estimation of the relative contributions of different meteorological drivers to dust activities can help to improve the representation of dust storms in models.

Mongolian cyclones, which form East of the Altai-Sayan Mountains, are important for dust-emitting winds in the Gobi Desert. Utilizing an automated detection algorithm of extratropical cyclones and multiple datasets for dust aerosol for 2001–2022, the contribution of Mongolian cyclones to East Asian dust emission and dust optical depth is quantitatively estimated (Mu and Fiedler). The results highlight that springtime dust storms in East Asia are primarily associated with a low-pressure system over Mongolia. Mobile Mongolian cyclones explain almost half of the total spring dust emission amount of the Gobi Desert. The calculated relative contributions of Mongolian cyclones to dust emissions in the Gobi Desert are similar from two different products, despite differences in the physical parameterization schemes for dust emission, number and location of the prescribed potential dust sources, and in the absolute dust emission amount by a factor ten. Dust emissions in the Gobi Desert and dust aerosol optical depth in the region downwind have decreased in the past decades, with Mongolian cyclones contributing to reductions of 10%-18% decade-1 and 11%--15% decade-1, respectively. The reduction of dust emissions and dust aerosol optical depth is at least in part explained by weaker and fewer Mongolian cyclones over time. 

Mongolian cyclones may also affect the dust activity in the Taklamakan Desert to the west of the Gobi Desert. The passage of the Mongolian cyclone in mid-March 2021 has led to a cold air intrusion into the Taklamakan Desert. The cold air favored the nighttime near-surface temperature inversion. The stable stratification near the surface allows the development of Nocturnal Low-Level Jets (NLLJs). The breakdown of NLLJs results in a strengthening of near-surface winds, which are sufficiently strong for dust emissions in many parts of the Taklamakan Desert (Mu et al., 2023). The Taklamakan dust was elevated by deep mixing and transported eastwards by prevailing mid-level westerlies, impacting air quality primarily in western China. Ongoing work addresses the link of cyclones and NLLJs in the Taklamakan Desert from the climatological perspective.

References:

Mu, F., Luiz, E.W., Fiedler, S., 2023. On the dynamics and air-quality impact of the exceptional East Asian dust outbreak in mid-March 2021. Atmos. Res. 292, 106846.
Mu, F. and Fiedler, S., in review. How much do atmospheric depressions and Mongolian cyclones contribute to East Asian spring dust activities?

How to cite: Mu, F. and Fiedler, S.: Meteorological Drivers of East Asian dust activity in spring 2001-2022, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6183, https://doi.org/10.5194/egusphere-egu25-6183, 2025.

EGU25-6741 | ECS | PICO | CL4.14

The contribution of haboobs to the dust direct radiative effect 

Andreas Baer, Rumeng Li, and Martina Klose

Mineral dust is the most abundant type of atmospheric aerosol in terms of mass. Dust models at non-storm resolving resolutions are usually able to capture the dust load on diurnal or longer-term average, but perform worse in capturing its diurnal variability. A main reason for this deficit is the fact that phenomena smaller than the grid size cannot be represented and are therefore lacking in the simulations. A major dust-event type that can only be represented at single-digit kilometer resolution are haboobs – intense dust storms created by the cold-pool outflow of moist convection. Haboobs mostly occur during the afternoon and thus their representation in models at storm resolving resolutions increases dust emissions during the afternoon hours, especially in regions where haboobs typically occur. As a significant amount of global dust emissions can be attributed to haboobs, their impact, e.g. on interactions of dust aerosol with radiation, on the continental to global scale is of special interest.

Here we investigate the contribution of haboobs to the direct radiative effect (DRE) of dust through their modulation of the dust diurnal cycle and vertical and horizontal distributions. For this purpose, we performed a set of annual simulations of the year 2020 using the ICON-ART model at 5km and 80km grid resolution for a domain covering North Africa and the Arabian Peninsula, as these regions are strong dust sources and haboob hotspots. A radiation multiple call scheme in ICON-ART was used to assess the DRE from a single simulation. We analyze differences in DRE and the vertical and horizontal dust distribution between the simulations and link them to the spatial distribution of haboob occurrence in the high-resolution simulation.

By assessing the impact of haboobs on the radiation balance of the earth, we aim to contribute to evaluating the benefits of storm-resolving simulations on a global scale with online treatment of aerosols; and to test the importance of representing meso-scale phenomena for quantification of dust-climate impacts.

How to cite: Baer, A., Li, R., and Klose, M.: The contribution of haboobs to the dust direct radiative effect, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6741, https://doi.org/10.5194/egusphere-egu25-6741, 2025.

EGU25-7106 | ECS | PICO | CL4.14

Another one traps the dust: Central Svalbard Lake sediments track 8,000 years of High Arctic wind strength 

Zofia Stachowska, Willem G. M. van der Bilt, Mateusz C. Strzelecki, and Jan Kavan

The Arctic warms faster than any other region on Earth. As sea ice diminishes in response, wind speeds increase due to reduced drag over open waters. Lake sediments offer valuable records of these processes and their relation to past climate change through the deposition of wind-blown grains and elements. This study reconstructs 8,000 years of Arctic eolian activity using laminated sediments from closed Lake Dunsappietjørna on the Svalbard archipelago. The site faces North Atlantic Westerlies as well as Easterly winds. By integrating geochemical (X-Ray Fluorescence – XRF), visual (Computed Tomography – CT and Scanning Electron Microscope – SEM), and granulometric (End Member Modeling Analysis – EMMA) fingerprints in a geostatistical (Principal Component Analysis – PCA) framework, we link clastic lacustrine input to sediment sources in the catchment, and unravel the imprint of Westerly and Easterly wind systems throughout the Holocene.

How to cite: Stachowska, Z., van der Bilt, W. G. M., Strzelecki, M. C., and Kavan, J.: Another one traps the dust: Central Svalbard Lake sediments track 8,000 years of High Arctic wind strength, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7106, https://doi.org/10.5194/egusphere-egu25-7106, 2025.

The 2.3-million-year grain-size records of detrital components from IODP Site U1430 in the East (Japan) Sea illustrate the influence of East Asian Winter Monsoon variations on Asian dust transport and deposition. Dust transport was driven by two distinct wind systems: low-level northwesterly winter monsoon winds and upper-level westerlies. Using end-member (EM) modeling of grain-size distributions, five EMs were identified: fine-mode dust transported by upper-level westerlies (EM1), coarse-mode dust carried by northwesterly surface winds (EM2), and marine tephra components (EM3, EM4, EM5). After excluding marine tephra contributions, a refined dust-size distribution model was developed, focusing on EM1 and EM2. The cyclic patterns and amplitudes of dust-size variations at Site U1430 closely align with size records from the Chinese Loess Plateau (CLP), where sedimentation is predominantly influenced by northwesterly surface winds. This agreement suggests that dust deposition at Site U1430 was similarly controlled by the intensity of these winds, rather than upper-level westerlies. Additionally, variations in loess size across the CLP and modern dust observations indicate that vertical and lateral sorting processes during atmospheric transport contributed to the finer dust sizes recorded at Site U1430. These findings highlight the critical role of surface wind intensity and atmospheric sorting in shaping long-term dust deposition patterns in the East (Japan) Sea. 

How to cite: Jang, J.-H., Bahk, J.-J., and Lee, D. E.: IODP Site U1430 Asian Dust Size Records in the East (Japan) Sea Since the Early Pleistocene: The Role of Northwesterly Surface Winds and Upper Westerlies , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7600, https://doi.org/10.5194/egusphere-egu25-7600, 2025.

EGU25-8292 | ECS | PICO | CL4.14

Saharan dust deposition in the eastern Mediterranean Sea: ballasting agent or fertilizer? 

Anouk van Boxtel, Addison Rice, Gert J. de Lange, Francien Peterse, and Jan-Berend Stuut

Dust deposition can increase the strength of the biological pump through fertilizing and ballasting effects of the deposited dust, in particular in (ultra-)oligotrophic oceans such as the eastern Mediterranean Sea (EMS). However, dust characteristics, such as nutrient content and bioavailability, organic-matter content, and grain-size distribution, and thus its fertilizing and ballasting potential, can vary between dust events.

Here, we present a long-term (1999-2011), high-resolution (14-21 days) sediment-trap record of dust fluxes, dust grain-size distributions, and fluxes of plant leaf waxes at 500, 1500, and 2500m water depth to assess seasonal and interannual variation in the amount and characteristics of dust deposited in the EMS.

We find that dust events mainly occur during late spring and summer, although their exact timing and magnitude varies between years. Differences in grain-size distribution and plant wax content between dust events indicate that the provenance, transportation, and/or deposition mode of the dust varied between events. The dust events archived in the sediment traps are preceded by atmospheric dust transport, indicated by increased Aerosol Optical Depth (AOD) values recorded by satellites in the weeks before dust fluxes increase. However, several major atmospheric dust outbreaks observed by satellites do not appear in the sediment trap record. This indicates that not all material that passes the EMS through the atmosphere is actually deposited on the sea surface and/or reaches the traps at larger water depths.

Most dust events in the sediment traps can be traced through the water column, indicating relatively rapid vertical export. The dust events coincide with increases in organic carbon flux, supporting the proposed role of dust in the biological pump through ballasting. However, while coarse-grained dust is consistently transferred to the deepest trap, regardless of the absolute flux, finer-grained dust is primarily detected in the upper trap. We will use our dataset to further investigate whether export of fine-grained dust is also linked to ballasting or is mediated by productivity in the surface ocean through the formation of organic aggregates and fecal pallets, either as a result of dust fertilization or natural processes.

How to cite: van Boxtel, A., Rice, A., de Lange, G. J., Peterse, F., and Stuut, J.-B.: Saharan dust deposition in the eastern Mediterranean Sea: ballasting agent or fertilizer?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8292, https://doi.org/10.5194/egusphere-egu25-8292, 2025.

EGU25-8963 | PICO | CL4.14

Evaluating the impact of improved dust representation and atmospheric iron chemistry in marine primary production and subsurface iron stocks  

Joan Llort, Elisa Bergas-Massó, Raffaelle Bernardello, Valentina Sicardi, Maria Gonçalves Ageitos, Carla Pons, Stelios Myriokefalitakis, and Carlos Pérez García-Pando

The impact of dust deposition on the fertilisation of marine ecosystems has been studied for decades. Despite the relevance of this air-sea interaction, aerosol chemical transformation, deposition over the ocean, and the eventual influence on ocean biogeochemistry (including carbon export) are poorly represented in most Earth System Models (ESM). For instance, the deposition of soluble iron (the chemical iron forms that phytoplankton can uptake) is often estimated in ESM as a constant fraction of deposited dust. This type of simplistic formulation underrepresents the interannual and spatial variability of the aeolian input of nutrients in marine ecosystems. 

In this work, we present a reconstruction of global ocean biogeochemistry for the last 30 years, where we evaluate the impact of newly produced iron deposition fields derived from the state-of-the-art atmospheric model EC-Earth3-Fe, which explicitly resolves the mineralogy of dust sources, includes a detailed representation of the atmospheric Fe dissolution processes and accounts for the contribution of other sources of Fe, such as anthropogenic combustion and biomass-burning. When compared to a standard run using climatological atmospheric inputs and constant dissolution rates the new simulation shows a contrasted response of marine primary production where production increases above 10% in large areas of the Pacific and the South Atlantic, while other smaller regions show an equivalent decrease. 

We also analysed the impact of the monthly resolved historical reconstruction of dust deposition (i.e., atmospheric model forced with observed meteorology) on the primary production’s interannual variability. Results showed no immediate impact of dust deposition variability on marine primary production. However, we found a replenishment of the subsurface stock of dissolved iron associated with the increase in dust deposition over the Equatorial Atlantic, the Indian Ocean and the subtropical Pacific. As this subsurface stock is one of the main seasonal inputs of iron through winter vertical mixing, it can induce delayed responses in marine ecosystems. Ongoing work is evaluating this hypothesis and comparing the simulated vertical distribution of dissolved iron in the water column against observations acquired by the GEOTRACES program.

In this presentation, we will also describe the efforts made in the new project BIOTA to understand how changes in aerosol transformation and deposition interact with the projected increase in upper ocean stratification, potentially enhancing the relative importance of aeolian nutrient inputs.

How to cite: Llort, J., Bergas-Massó, E., Bernardello, R., Sicardi, V., Gonçalves Ageitos, M., Pons, C., Myriokefalitakis, S., and Pérez García-Pando, C.: Evaluating the impact of improved dust representation and atmospheric iron chemistry in marine primary production and subsurface iron stocks , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8963, https://doi.org/10.5194/egusphere-egu25-8963, 2025.

EGU25-8965 | ECS | PICO | CL4.14

Photovoltaic production in West Africa: Impact of dust and water footprint of cleaning operations 

Amy Tamunoibinyemiem Banigo, Benoit Hingray, Louise Crochemore, Béatrice Marticorena, and Sandrine Anquetin

To achieve universal electricity access and comply with Paris Agreement, one large-scale objective of the Economic Community of West African States (ECOWAS) is the deployment of +8 to +20 GWp of solar energy systems by 2030 (IRENA, 2018). ECOWAS is located south of the Saharan region and close to the Bodélé depression, which has been observed to have the largest atmospheric dust production activity on Earth (Isaacs et al., 2023). Once deposited on panels, dust reduces the transmission of solar radiation to the panels and, consequently, the energy production (Sarver et al., 2013). Annual losses of solar energy production of up to 54% have been observed in the region due to dust (Chanchangi et al., 2022). These production losses can be mitigated by regularly cleaning solar panels. In West Africa, cleaning operations commonly use water but many areas are water-scarce. It is thus important to ensure that water resources are not further strained by water cleaning operations associated with the expected large-scale deployment of solar energy systems in the region.

In the present work, we aim to assess the water footprint of different cleaning strategies of virtual solar plants in the ECOWAS region. A first step towards this aim consists in regionally assessing how dust would accumulate on Photovoltaic (PV) panels and, in turn, what the associated production losses would be. We present a dust accumulation model allowing to simulate, over a long time period and across the region, the temporal sub daily variations of dust accumulation on virtual PV panels. The model uses as input the particulate matter concentration of different particle sizes. Dust data from the CAMS and MERRA2 reanalyses are considered. Both datasets are first compared to observations of regional particulate matter concentration available from a set of four stations from the INDAAF network. CAMS data were found to better agree with observations (> 0.8 correlation for a 1-week temporal resolution). Time series of dust accumulation simulated from CAMS data were then compared to time series of dust deposit observations available for the same four INDAAF stations. Results show fair agreement but highlight significant differences, likely due to uncertainties in various variables and model assumptions. Lastly, simulated accumulated dust amounts are used as input to a PV soiling loss model to derive the transmission reduction and the mean PV production losses for different cleaning operation strategies.

References

Chanchangi et al., 2022. Soiling mapping through optical losses for Nigeria. Renewable Energy, 197, 995–1008. https://doi.org/10.1016/j.renene.2022.07.019

IRENA (2018), Renewable Energy Statistics 2018, The International Renewable Energy Agency, Abu Dhabi.

Isaacs et al., 2023. Dust soiling effects on decentralized solar in West Africa. Applied Energy, 340, 120993. https://doi.org/10.1016/j.apenergy.2023.120993

Sarver et al.,2013. A comprehensive review of the impact of dust on the use of solar energy: History, investigations, results, literature, and mitigation approaches. Renewable and Sustainable Energy Reviews, 22, 698–733. https://doi.org/10.1016/j.rser.2012.12.065

How to cite: Banigo, A. T., Hingray, B., Crochemore, L., Marticorena, B., and Anquetin, S.: Photovoltaic production in West Africa: Impact of dust and water footprint of cleaning operations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8965, https://doi.org/10.5194/egusphere-egu25-8965, 2025.

EGU25-9134 | PICO | CL4.14

Coordinated vertical tandem-profiling of a Saharan dust intrusion over Central Europe on 20 June 2024 based on balloon-borne soundings from two different sites. 

Ralf Weigel, Konrad Kandler, Monika Scheibe, Katie Smith, Luis Valero, Luca K. Eichhorn, Sina Jost, Kristin Röck, Sonja Gisinger, Alexandre Baron, Troy Thornberry, Adrienne Jeske, and Holger Tost

When favourable synoptic conditions prevail, desert dust is transported from North Africa to Central Europe. Between June 19 and 21, 2024, air from North and Northwest Africa spread from Algeria across the south-coast of France with predicted dust load > 1200 mg m-2 over an area limited by the Rhone Valley, extending to the coasts of Belgium and the Netherlands. The intrusion reached as far as the Skagerrak and the Kattegat and stretched across parts of Poland and the Czech Republic to the Aegean Sea and Greece, and it entirely covered Italy. On June 20, 2024, time-coordinated balloon-borne vertical soundings were carried out over Germany from two locations: 1) at 13:18 CEST from Oberpfaffenhofen (OPH - near Munich) and 2) at 14:15 CEST from Spielberg (SPb - near Frankfurt/Main, in the framework of “TPChange”, DFG TRR301) with the aim to analyse the same (intermediately transported) air mass. The SPb balloon payload included (a. o.) a radiosonde (RS41 SGP by VAISALA), a set of dual-stage impactors to perform particle sampling for offline physico-chemical analyses, and optical particle counters (OPC) such as the Portable Optical Particle Spectrometer (POPS). The OPH payload consisted of an OPC-N3 (by Alphasense) and the RS41 SGP.

Qualitative agreement was obtained from the independent profiles: from 1.5 km to 4.8 km height, a layer of increased particle number concentration (N) with 100 to 1000 cm-3 stands out from the background (N < 20 cm-3) in the vertical profile for particles with a diameter (Dp) from 0.14 µm to 2.6 µm (POPS-detected sized range). While below ~ 4.5 km (OPH) and ~ 4.8 km (SPb), the relative humidity (RH) remains below 87 %, the region of particle enhancement is effectively capped by a cloud layer (RH exceeding 100 %) of about 200 m vertical thickness above ~ 4.5 km (OPH) and ~ 4.8 km (SPb), respectively. Aloft, N drops abruptly and temporarily reaches background values < 20 cm-3. The impactor sample taken throughout passage of the particle layer showed considerable presence of mineral dust (generally > 75 % of all particles collected), the largest of which have estimated Dp of 10 µm and smallest Dp were estimated with 0.1 µm. Admixtures of sea salt (particle fraction Dp > 500nm) and sulphates (fraction Dp < 500 nm) were also identified. We will present more specific microphysical properties of the mineral dust aerosol, including morphology and chemical composition, and discuss these in the context of the atmospheric conditions at both measurement sites.

How to cite: Weigel, R., Kandler, K., Scheibe, M., Smith, K., Valero, L., Eichhorn, L. K., Jost, S., Röck, K., Gisinger, S., Baron, A., Thornberry, T., Jeske, A., and Tost, H.: Coordinated vertical tandem-profiling of a Saharan dust intrusion over Central Europe on 20 June 2024 based on balloon-borne soundings from two different sites., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9134, https://doi.org/10.5194/egusphere-egu25-9134, 2025.

EGU25-9264 | PICO | CL4.14 | Highlight

The shadow of the wind: photovoltaic power generation under Europe's dusty skies 

György Varga, Fruzsina Gresin, András Gelencsér, Adrienn Csávics, and Ágnes Rostási

The impact of the Sahara dust storm events on photovoltaic power generation in Europe will be presented. In recent years, driven by global sustainability, climate and energy security objectives, photovoltaic power generation has been expanding worldwide, with a particular focus on the European continent. We are also witnessing a change in the frequency and intensity of Saharan dust storm events. Atmospheric particulate matter significantly reduces irradiance through its direct and indirect effects, with energy flux changes sometimes having serious economic and security of supply implications. 

In a diverse energy mix, which varies significantly from state to state, weather-dependent renewable generation must be forecasted to meet the delicate balancing needs of electricity supply, which poses a major challenge to the system operator. Analysis of the accuracy of the forecasts has shown that this is subject to significant errors and that the magnitude of these errors is larger during dust storm events than during non-dust storm situations. In the photovoltaic power generation data series of the southern (Portugal, Spain, France, Italy, Greece) and central European (Hungary) countries  presented here, we characterise episodes where atmospheric dust caused irradiance and electricity production to deviate significantly from the predicted levels.

Key Takeaways:

(1) The influence of atmospheric particulate matter is substantial for both photovoltaic (PV) production and generation forecasting. This effect is likely more pronounced with meridional (south-north) dust transport due to a steeper thermal gradient, which intensifies cloud formation processes through warm air advection and increased fine-grained particulate mass.

(2) Accurate PV production forecasts cannot be achieved using coarse-resolution aerosol climatology data without aerosol-cloud coupling. Instead, calculations should integrate up-to-date dust load data and relevant cloud physics relationships.

(3) The quantities of atmospheric dust, the dynamics of its transport, and the mineralogical and physical properties (such as grain size and shape) of the dust are not well understood. These factors have diverse impacts on cloud formation processes, necessitating further research for better comprehension.

(4) Due to climate change and the inherent variability of the climate system, forecasts are made under fluctuating hydrometeorological and atmospheric conditions, which inherently carry uncertainties. These errors are expected to become more significant with increasing PV capacity, thus managing them will require expanding electricity storage capacities alongside more precise forecasts.

The research was supported by the NRDI projects FK138692 and by the Sustainable Development and Technologies National Programme of the Hungarian Academy of Sciences (FFT NP FTA). This work has been implemented by the National Multidisciplinary Laboratory for Climate Change (RRF-2.3.1-21-2022-00014) project within the framework of Hungary's National Recovery and Resilience Plan supported by the Recovery and Resilience Facility of the European Union.

How to cite: Varga, G., Gresin, F., Gelencsér, A., Csávics, A., and Rostási, Á.: The shadow of the wind: photovoltaic power generation under Europe's dusty skies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9264, https://doi.org/10.5194/egusphere-egu25-9264, 2025.

EGU25-10547 | PICO | CL4.14

Dust emission from dust sources in Iceland: Insights from the High-Latitude Dust Experiment in summer 2021 

Kerstin Schepanski, Konrad Kandler, Mara Montag, Kilian Schneiders, Agnesh Panta, Adolfo González-Romero, Cristina González-Flórez, Martina Klose, Xavier Querol, Andrés Alastuey, Jesús Yus-Díez, Sylvain Dupont, Pavla Dagsson-Waldhauserová, and Carlos Pérez García-Pando

Mineral dust is one of the most prominent natural aerosols and is almost ubiquitous in the atmosphere, where it substantially interacts, modulates and alter atmospheric processes. Although research on dust aerosol is carried out since many decades by means of different approaches and techniques, knowledge on mineral dust emitted at high latitudes or in cold climate regions is still limited despite its pivotal impact on polar environments. Within a warming climate, dust emitted from sources located in cold climate zones is expected to increase due to the retreat of the ice sheets and increasing melting rates. Therefore, and for its extensive impacts on different aspects of the climate system, a better understanding of the atmospheric dust cycle at high latitudes/cold climates in general, and the spatio-temporal distribution of dust sources in particular, are essential.

We will present results from the HiLDA measurement campaign which took place in summer 2021 in the Dyngjusandur in Iceland. The measurements were set up to observe dust concentration variability across the Dyngjusandur and near-source dust transport areas in order to eventually conclude on the variability in dust source emissivity. We have measured aerosol size distributions and meteorological parameters distributed over different dust source areas at high temporal resolution for a period of eight weeks in summer 2021 and spring 2022. During this time, we observed a couple of intense dust events as well as background conditions. Ultimately, the analysis of our measurement data addresses the complex web of interactions which is defined by the variability of dust source characteristics and wind speed distribution in concert. Findings from this study contribute to the understanding of dust emission in cold climate regions and its spatio-temporal variability, which is essential with respect to the quantification of dust-associated feedbacks in the Earth system.

How to cite: Schepanski, K., Kandler, K., Montag, M., Schneiders, K., Panta, A., González-Romero, A., González-Flórez, C., Klose, M., Querol, X., Alastuey, A., Yus-Díez, J., Dupont, S., Dagsson-Waldhauserová, P., and Pérez García-Pando, C.: Dust emission from dust sources in Iceland: Insights from the High-Latitude Dust Experiment in summer 2021, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10547, https://doi.org/10.5194/egusphere-egu25-10547, 2025.

EGU25-11653 | PICO | CL4.14

Earth Observations and Atmospheric Dust: unveiling Atlantic Ocean deposition 

Jan-Berend Stuut, Emmanouil Proestakis, Vassilis Amiridis, Carlos Pérez Garcia-Pando, Svetlana Tsyro, Jan Griesfeller, Antonis Gkikas, Thanasis Georgiou, Maria Gonçalves Ageitos, Jeronimo Escribano, Stelios Myriokefalitakis, Elisa Bergas Masso, Enza Di Tomaso, Sara Basart, and Angela Benedetti

The global ocean is a key component to the Earth’s climate system, absorbing atmospheric energy in excess and exchanging as a sink climate-relevant gases with the atmosphere. More specifically, through the uptake of atmospheric CO2 and acting as carbon storage, through the processes of biological pump and solubility pump, helps to mitigate anthropogenic CO2 increase. Moreover, the ocean enables phytoplankton photosynthesis, impacts ocean color, light penetration into deeper layers, and sea surface temperature, eventually modulating weather and resulting to feedback effects on climate. However, primary production highly depends on the spatial distribution of input nutrients from the atmosphere, with iron (Fe) availability the most important limiting factor for phytoplankton growth. Across the open ocean, the principal source of Fe is considered atmospheric mineral dust, transported over distances of thousands of kilometers prior removal through wet deposition or gravitational settling.

The present study provides quantification of the amount of atmospheric dust deposited into the broader Atlantic Ocean. Based on Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) routine observations on atmospheric dust, the primary instrument onboard Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO), and meridional and zonal wind components provided by the European Centre for Medium-Range Weather Forecasts (ECMWF) reanalysis (ERA5), the atmospheric dust fluxes and the dust deposited component across the tans-Atlantic transits are estimated. On the basis of more than sixteen years (12/2006-11/2022) of Earth Observations, and for the Atlantic Ocean region extending between latitudes 60°S and 40°N, the annual-mean amount of deposited dust is estimated at 274.79 ± 31.64 Tg, of which 243.98 ± 23.89 Tg is deposited into the North Atlantic Ocean and 30.81 ± 10.49 Tg into the South Atlantic Ocean. Moreover, a negative statistically significant decreasing trend in dust deposition into the Atlantic Ocean for this period is revealed, characterized by slope -13.35 Tg yr-1 and offset 306.97 Tg.

The climate data record is evaluated against high quality sediment-trap measurements of deposited lithogenic material implemented as reference dataset, demonstrating the protentional of the established dataset to be used in a wide range of applications, including filling geographical and temporal gaps in sediment-trap measurements, aiding model simulation evaluations, uncovering physical processes in the dust cycle from emission to deposition, and enhancing our understanding of dust's biogeochemical impacts on ocean ecosystems, as well as its effects on weather and climate.

 

Acknowledgements

This research was supported by the Dust Observation and Modelling Study (DOMOS) under ESA contract number 4000135024/21/I-NB. Emmanouil Proestakis acknowledges support by the AXA Research Fund for postdoctoral researchers under the project entitled “Earth Observation for Air-Quality – Dust Fine-Mode (EO4AQ-DustFM)”.

How to cite: Stuut, J.-B., Proestakis, E., Amiridis, V., Pérez Garcia-Pando, C., Tsyro, S., Griesfeller, J., Gkikas, A., Georgiou, T., Gonçalves Ageitos, M., Escribano, J., Myriokefalitakis, S., Bergas Masso, E., Di Tomaso, E., Basart, S., and Benedetti, A.: Earth Observations and Atmospheric Dust: unveiling Atlantic Ocean deposition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11653, https://doi.org/10.5194/egusphere-egu25-11653, 2025.

EGU25-12087 | ECS | PICO | CL4.14

From fine to giant: Multi-instrument assessment of the particle size distribution of emitted dust during the J-WADI field campaign 

Hannah Meyer, Martina Klose, Konrad Kandler, Sylvain Dupont, and Carlos Pérez García-Pando and the J-WADI Team

Mineral dust, a key component of Earth’s aerosols, impacts atmospheric processes and climate. Emitted from dry soil, these particles travel long distances, influencing atmospheric radiation, cloud dynamics, and biogeochemical cycles. Dust effects are size-dependent. Larger particles, for example, tend to warm the atmosphere, whereas smaller ones (diameter dp < 2.5 µm) typically cool it. Understanding dust transport and impacts requires detailed particle size distribution (PSD) data at emission, but measurements are sparse and larger particles (dp > 10 µm) are understudied due to low concentrations and sampling challenges.

The Jordan Wind Erosion and Dust Investigation (J-WADI) campaign, conducted in September 2022 near Wadi Rum, Jordan, provides the platform for this study, in which we characterize the PSD at emission, focusing on super-coarse (10 < dp ≤ 62.5 µm) and giant (dp > 62.5 µm) particles. This study is the first to comprehensively characterize the size distribution of mineral dust directly at the emission source, covering diameters between 0.4 and 200 µm. Using a suite of aerosol spectrometers, the overlapping size ranges enabled systematic intercomparison and validation across instruments, improving PSD reliability and addressing challenges in detecting larger particles, such as inlet efficiencies or size range restrictions.

Results show significant PSD variability over the course of the campaign. During periods with friction velocities (u*) above 0.25 ms⁻¹, super-coarse and giant particles were observed, with concentrations increasing with u*. These large particles account for about two-thirds of the total mass during the campaign, with contributions of 90% during an active emission event, emphasizing the importance of including super-coarse and giant particles in PSD analyses. A prominent mass concentration peak was observed near 50 µm. While particle concentrations for dp < 10 µm show strong agreement among most instruments, discrepancies appear for larger dp due to reduced instrument sensitivity at the size range boundaries and sampling inefficiencies. Despite these challenges, physical samples collected using a flat-plate sampler largely confirm the PSDs derived from aerosol spectrometers.

These findings advance the characterization of PSD over a large size range at emission sources and lay the foundation to further improve our understanding of the mechanisms facilitating super-coarse and giant dust particle emission and transport.

How to cite: Meyer, H., Klose, M., Kandler, K., Dupont, S., and Pérez García-Pando, C. and the J-WADI Team: From fine to giant: Multi-instrument assessment of the particle size distribution of emitted dust during the J-WADI field campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12087, https://doi.org/10.5194/egusphere-egu25-12087, 2025.

EGU25-13198 | PICO | CL4.14

Giant Particle Size Distribution and Composition Near and In Dust Sources 

Konrad Kandler, Agnesh Panta, Mara Montag, Melanie Eknayan, Hannah Meyer, Martina Klose, Kerstin Schepanski, Cristina González-Flórez, Adolfo González-Romero, Andres Alastuey, Pavla Dagsson Waldhauserová, Xavier Querol, and Carlos Pérez García-Pando

Mineral dust is one of the key players in the Earth’s atmosphere with respect to climate and atmospheric nutrient transport. Dust spans a large size range of particle diameters, reaching from around 100 nm to more than 100 µm. While it has been assumed for a long time that the super-coarse (10 - 62.5 µm) and giant (> 62.5 µm) particles are not widely dispersed from the sources, more recent observations show that they can travel on a regional up to even intercontinental scale. Owing to the negligence and difficulty in measurement, not much information is available on this dust size range.

In the present work we have collected dust by means of a simple flat-plate deposition sampler and analyzed the collected material with electron microscopy and X-ray fluorescence, yielding information on particle size distributions and elemental composition. Samples were collected during intensive field campaigns of the FRAGMENT project in Morocco in 2019, a joint field campaign with the HiLDA project in Iceland in 2021, and the Jordan Wind erosion And Dust Investigation (J-WADI) in 2022. During all campaigns, severe dust conditions were observed with mass concentrations ranging into the tens of milligrams per cubic meter.

All observed number size distributions have in common a decrease towards submicron particles and a monotonic decrease with increasing particle size starting from 5 µm diameter. Both features are in general corroborated by online size distribution measurements in the overlap region, while the decrease towards smaller particle sizes is enhanced in the deposition sampling, most probably linked to the lower deposition speed of these particle sizes. The mean size distribution observed in Iceland has relatively more larger particles, followed by Jordan and lastly Morocco. Besides modes at around 1 µm and 5 µm, in Morocco a tertiary mode at around 70 µm in diameter gets pronounced. Mineral composition was estimated for each particle from the elemental composition. Morocco and Jordan have a similar composition with a slightly higher amount of Ca-accreted and feldspar particles in Jordan and more illite-/muscovite-like ones in Morocco. Expectedly, the composition of Icelandic dust is different, with volcanic glass, feldspars, and pyroxene/amphibole-like particles dominating. Comparing the coarse (sub-10-µm) with the super-coarse/giant (>10 µm) size range, we observe in the hot deserts less calcite for the larger particles as a common feature. The trend of a decreasing relative contribution of Fe-rich particles starting at the submicron range continues. In Iceland, we see the dominance of glassy particles still increase with increasing particle size. A big change in composition between these size classes is not observed unlike, for example, in previous measurements in Morocco, which showed a strong increase of quartz-like particles for the giant particle range. That indicates a considerable small-scale variability in freshly emitted dust plumes, dependent on their source.

How to cite: Kandler, K., Panta, A., Montag, M., Eknayan, M., Meyer, H., Klose, M., Schepanski, K., González-Flórez, C., González-Romero, A., Alastuey, A., Dagsson Waldhauserová, P., Querol, X., and Pérez García-Pando, C.: Giant Particle Size Distribution and Composition Near and In Dust Sources, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13198, https://doi.org/10.5194/egusphere-egu25-13198, 2025.

EGU25-13655 | ECS | PICO | CL4.14

Modelling of Dust Emissions from Agricultural Sources in Europe 

Matthias Faust, Robert Wagner, Ralf Wolke, Steffen Münch, Roger Funk, and Kerstin Schepanski

Mineral dust emissions from arable land are a significant environmental concern. Fugitive dust emissions commonly arise during mechanical activities such as tilling and harvesting, while aeolian emissions occur from sparsely vegetated cropland, particularly during the transitional phases between fresh tillage and substantial vegetation growth and hence coverage of the bare soil. Suspended in the atmosphere, dust aerosol particles originating from arable land suposedly affect human health, reduce air quality, and can economically impact agricultural productivity due to soil degradation and reduced yields.

Agricultural dust emissions are often overlooked in coupled atmosphere-aerosol models, perhaps due to the complex conditions that lead to emissions. Fugitive emissions are highly variable, influenced by unpredictable human activities, while aeolian emissions require accurate descriptions of vegetation dynamics during transitional periods.

To address these gaps, we developed modelling strategies to simulate both fugitive and aeolian emissions. Fugitive emissions were analysed using a Lagrangian particle dispersion model designed to capture the turbulent mixing of dust particles in the atmospheric boundary layer. A case study based on measured tilling emissions demonstrated how atmospheric stratification can limit or amplify dust plumes and their range of transport.

For aeolian emissions, a new parameterisation was implemented in the atmosphere-aerosol model COSMO-MUSCAT, utilising high-resolution satellite data to represent vegetation cover. We tested our model for a dust emission event in Poland in 2019, where the model showed good agreement with satellite observations and ground-based measurements.

Ultimately, our modelling efforts provide insights into the dynamics, spatial distribution, and broader impacts of agricultural dust emissions, contributing to a more comprehensive understanding of their role in the atmosphere.

How to cite: Faust, M., Wagner, R., Wolke, R., Münch, S., Funk, R., and Schepanski, K.: Modelling of Dust Emissions from Agricultural Sources in Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13655, https://doi.org/10.5194/egusphere-egu25-13655, 2025.

EGU25-16684 | ECS | PICO | CL4.14

Enhancing Aerosol Modeling: Integrating the Mineralogy of Mineral Dust into ECHAM_HAMMOZ 

Elisabeth Hofmann, Robert Wagner, and Kerstin Schepanski

Dust aerosols are a key component of the climate system due to their interactions with radiation, their influence on atmospheric chemistry, and their role in biogeochemical cycles. Despite this importance, many climate models treat mineral dust particles as a homogeneous entity, overlooking their inherent variability regarding mineralogical composition. In reality, dust aerosols consist of fine particles entrained by wind from sparsely vegetated soil surfaces, originating from geographically diverse regions of the Earth and shaped by local climate and geological conditions. These particles are a complex mixture of various mineralogies with distinct size distributions.

In this study, we discuss the global distribution of mineral dust aerosol concentrations with regard to the dust particles’ mineralogical composition, using the atmosphere-aerosol model ECHAM-HAMMOZ (ECHAM6.3.0-HAM2.3-MOZ1.0). The model has been enhanced by integrating 12 minerals derived from the database of Journet et al. (2014), as modified by Gonçalves Ageitos et al. (2023). This implementation allows for a more detailed representation of the mineralogical diversity of atmospheric dust aerosols as a function of soil mineralogy at the contributing dust source areas. The results of the model simulations are evaluated against observational data in order to assess the model's accuracy and performance with regard to the representation of the mineralogical composition of dust aerosol plumes.

This work highlights the importance of incorporating mineralogical diversity in climate models to better understand the role of dust aerosols in the Earth system.

 

  • Gonçalves Ageitos, María & Obiso, Vincenzo & Miller, Ron & Jorba, Oriol & Klose, Martina & Dawson, Matt & Balkanski, Yves & Perlwitz, Jan & Basart, Sara & Tomaso, Enza & Escribano, Jerónimo & Macchia, Francesca & Montané Pinto, Gilbert & Mahowald, Natalie M & Green, Robert O & Thompson, David & Pérez García-Pando, Carlos. (2023). Modeling dust mineralogical composition: sensitivity to soil mineralogy atlases and their expected climate impacts. Atmospheric Chemistry and Physics. 23. 8623-8657. 10.5194/acp-23-8623-2023.

  • Journet, E., Balkanski, Y., and Harrison, S. P.: A new data set of soil mineralogy for dust-cycle modeling, Atmos. Chem. Phys., 14, 3801–3816, https://doi.org/10.5194/acp-14-3801-2014, 2014.

How to cite: Hofmann, E., Wagner, R., and Schepanski, K.: Enhancing Aerosol Modeling: Integrating the Mineralogy of Mineral Dust into ECHAM_HAMMOZ, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16684, https://doi.org/10.5194/egusphere-egu25-16684, 2025.

EGU25-16882 | ECS | PICO | CL4.14

Magnetic minerals in atmospheric Saharan dust  

Iida Kostamo, Johanna Salminen, Anu Kaakinen, Outi Meinander, Antti Penttilä, and Karri Muinonen

Atmospheric dust is an important component of the global climate system. It has large-scale effects on the planetary radiation budget, the albedo of snow/ice, and biogeochemical cycles. Despite this, particularly the magnetic minerals in atmospheric dust have been poorly described in aerosol models. The absorption effects of magnetic particles can be comparable to black carbon, they promote ice nucleation and therefore play a role in cloud formation, and they increase the input of iron into ocean ecosystems. We aim to contribute to characterizing these dust particles and their source areas, long-range transport, and scattering effects.  

The research material consists of Saharan dust deposited on snow in Finland, collected as an extensive citizen science campaign by the Finnish Meteorological Institute during 2021. The first results regarding the dust samples were published by Meinander et al. (2023). The multidisciplinary study showed that the dust originated from the Sahara and the Sahel regions (south of Sahara), based on the magnetic properties of the particles, and the System for Integrated modeLling of Atmospheric coMposition (SILAM) model. The results form the basis for the present project.  

A detailed magnetic characterization of the dust samples is one of the main objectives. Identifying properties such as the types and grain sizes of the magnetic particles is crucial in indicating the source area of the dust and improving the light scattering and absorption models of dust. Magnetic measurements, including initial susceptibility with two frequencies, anhysteretic remanence, and isothermal remanence, have been carried out for a set of 47 dust samples. The preliminary results are in good agreement with the previously published magnetic analyses (Meinander et al. 2023), showing signs of the presence of both Saharan and anthropogenic dust.  

In the future, the scattering and absorption of light by the dust particles will be studied both experimentally and theoretically. The existing numerical methods will be extended for the treatment of magnetic particles, particularly. 

 

Meinander, O., Kouznetsov, R., Uppstu, A. et al. African dust transport and deposition modelling verified through a citizen science campaign in Finland. Sci Rep 13, 21379 (2023). https://doi.org/10.1038/s41598-023-46321-7 

How to cite: Kostamo, I., Salminen, J., Kaakinen, A., Meinander, O., Penttilä, A., and Muinonen, K.: Magnetic minerals in atmospheric Saharan dust , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16882, https://doi.org/10.5194/egusphere-egu25-16882, 2025.

EGU25-17479 | ECS | PICO | CL4.14

A 21-year evaluation of MODIS Aerosol Optical Depth retrievals during Icelandic dust events 

Sam Poxon, Matthew Baddock, and Joanna Bullard

The wind-blown entrainment, transportation, and deposition of mineral dust originating in the high latitudes plays a significant role in atmospheric, cryospheric, marine and terrestrial environments at the regional scale. However, the intermittent nature of dust events occurring over broad spatial scales is difficult to capture from field studies alone. Remote sensing datasets are well-suited to overcoming some of these spatial limitations, and while they have been effectively used to characterise and understand dust activity across the major global hotspots, they lack application in high latitude dust regions. The use of surface observations of dust, such as those recorded at meteorological stations, is an important step in assessing the value of data retrieved from space. Meteorological observations have an established application in monitoring wind erosion and dust activity at broad spatial and temporal scales, however their use as a comparative method for evaluating data retrieved from remote sensing remains under explored.

This research presents the first systematic comparison of remotely-sensed data and ground-based present weather dust codes for a high latitude region, using Iceland as a case study. Remote sensing datasets including Aerosol Optical Depth, Angstrom Exponent and Single Scattering Albedo are derived from the MODIS Level-2 Aerosol Product at 10 km resolution, has and have been evaluated against coded present weather reports of dust obtained from 23 Icelandic meteorological stations for the study period 2001 – 2022. Preliminary analysis indicates that Aerosol Optical Depth is elevated for dust constrained days which allows some inference about the seasonality of dust activity.  Further comparative testing of ground-based and remotely-sensed data may create opportunities for better understanding the opportunities and limitations associated with remote sensing of high latitude dust activity in regions where ground-based data are not available.

How to cite: Poxon, S., Baddock, M., and Bullard, J.: A 21-year evaluation of MODIS Aerosol Optical Depth retrievals during Icelandic dust events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17479, https://doi.org/10.5194/egusphere-egu25-17479, 2025.

EGU25-20931 | ECS | PICO | CL4.14

Is there a link between modelled mineral dust hematite content and lidar measured intensive optical properties? 

Sofía Gómez Maqueo Anaya, Dietrich Althausen, Julian Hofer, Moritz Haarig, Ulla Wandinger, Bernd Heinold, Ina Tegen, Matthias Faust, Holger Baars, Albert Ansmann, Ronny Engelmann, Annett Skupin, Birgit Hesse, and Kerstin Schepanski

Mineral dust aerosols are composed of a complex mixture of various minerals that vary by source region. Notably, the iron oxide fraction differs yielding to differences in the dust absorbing properties in the UV-VIS spectrum due to changes in the imaginary parts of the complex refractive index.

This study investigates whether variations in the Saharan dust’s iron oxide content have led to measurable variations in the backscattering properties of dust particles, which is indicated by laboratory measurements and theoretical models. This work combines modelled mineralogical data using the regional dust model COSMO-MUSCAT with vertically resolved lidar measurements conducted in Cabo Verde, located in the tropical Atlantic Ocean off the west coast of Northern Africa.

The results include comparisons between the modelled iron oxide content and lidar resolved intensive optical properties, such as the lidar ratio (extinction-to-backscattering ratio), the backscatter-related Ångström exponent (ÅE), and the particle depolarization ratio. Dust plumes were analysed over two northern hemispheric summer campaign periods in 2021 and 2022. The findings reveal that the strongest correlations were observed between the modelled iron oxide mineral content and the backscatter-related ÅE. This supports the idea that variations in dust iron oxide content influence this intensive optical property at UV-VIS wavelengths, even though the backscatter-related ÅE is regarded to indicate mainly the particle size.

This study provides a framework for further exploring the influence of a varying hematite content on the backscattering properties of dust in the UV-VIS wavelength range. Establishing certainty with regards to dust optical properties, particularly at these wavelengths, is essential for improving calculations of dust radiative impact.

How to cite: Gómez Maqueo Anaya, S., Althausen, D., Hofer, J., Haarig, M., Wandinger, U., Heinold, B., Tegen, I., Faust, M., Baars, H., Ansmann, A., Engelmann, R., Skupin, A., Hesse, B., and Schepanski, K.: Is there a link between modelled mineral dust hematite content and lidar measured intensive optical properties?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20931, https://doi.org/10.5194/egusphere-egu25-20931, 2025.

Microplastics (MP) have emerged as pervasive pollutants, present in environments ranging from urban centers to remote areas worldwide. While research has largely concentrated on aquatic and terrestrial systems, the study of microplastics in airborne particles is a comparatively new and evolving domain. In particular, investigating the risks of inhaling nano- and microplastic particles is critical, as fine particulate matter (PM) with aerodynamic diameters under 10 µm (PM10) is recognized for its substantial potential to impact human health.

This study presents the development and optimization of methodologies for identifying and quantifying microplastic content in PM10 samples. Critical aspects of the workflow include the selection of appropriate filter materials in sampling, such as quartz fibre filters (QFF) and steel mesh filters, chosen for their minimal interference with subsequent analytical techniques. Sampling durations were optimized to ensure sufficient microplastic proportion while avoiding filter overloading.

Pre-treatment protocols were carefully designed to isolate microplastics from the complex atmospheric particulate matter matrix, enabling compatibility with Raman microscopy. These protocols incorporate chemical digestion steps tailored to reduce organic matter while preserving polymer integrity and use density separation with heavy salt solutions to effectively remove inorganic contaminants like mineral dust.

Methodological improvements were validated through controlled experiments, demonstrating reliability in detecting microplastics including particles below 10 microns. The study also addresses the challenges in applying automated Raman microscopy for rapid identification and quantification. Issues such as background interference, polymer-specific spectral variability, and the need for optimized machine learning algorithms to classify microplastic types are explored, highlighting advancements and limitations in automation.

In parallel, the study employs a mass-based analytical technique, pyrolysis gas chromatography/mass spectrometry (pyrolysis GC/MS), to complement particle-based findings. Results from this approach underline the importance of selecting appropriate quantification parameters, such as calibration standards and sampling subsets, to ensure accurate mass-specific data.

To contextualize findings, a comparative analysis was conducted to evaluate microplastic concentrations and polymer characteristics in PM10 samples collected from urban and rural locations. This comparison of the results raises the opportunity to evaluate the spatial variability of microplastic pollution and the influence of local and regional activities, providing valuable insights into the sources, dispersal mechanisms, and environmental impact of airborne microplastics.

How to cite: Schumacher, M. and Fischer, D.: Raman Microscopy and Pyrolysis GC/MS for Comprehensive Analysis of PM10 Microplastics: Method Development and Urban-Rural Comparison, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-299, https://doi.org/10.5194/egusphere-egu25-299, 2025.

EGU25-1448 | ECS | Posters on site | AS3.8

Airborne microplastic radiative effects: a sensitivity study 

Felix Goddard, Stefania Glukhova, Eric Le Ru, Cameron McErlich, Catherine Hardacre, and Laura Revell

Microplastics and nanoplastics are recognised as common airborne pollutants, capable of being transported over large distances and altering the radiative properties of the atmosphere, with implications for global climate. Work in recent years has provided new constraints on many aspects of the spatial and temporal distribution of airborne plastics and their physical and optical properties. Using these updated findings, we perform simulations with the HadGEM3-GA7.1 atmospheric model to investigate the sensitivity of the direct radiative effect of airborne microplastics to these factors. Our ERF estimates range from -0.89 to +0.63 mW m-2 assuming an average surface concentration of 1 MP particle per cubic meter. We show that the sign of the radiative forcing depends on the colour of microplastic particles, and that the abundance of nanoplastics has the strongest influence on the magnitude of their radiative effect, emphasising the importance of experimental work to constrain the micro- and nanoplastic size distribution.

How to cite: Goddard, F., Glukhova, S., Le Ru, E., McErlich, C., Hardacre, C., and Revell, L.: Airborne microplastic radiative effects: a sensitivity study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1448, https://doi.org/10.5194/egusphere-egu25-1448, 2025.

EGU25-1526 | ECS | Posters on site | AS3.8

The effects of sediment properties on the aeolian abrasion and surface characteristics of microplastics 

Lucrecia Alvarez Barrantes, Joanna E Bullard, Sam Davis, Cheryl McKenna Neuman, Patrick O’Brien, Paul Roach, and Zhaoxia Zhou

Microplastics (< 5 mm diameter) are significant environmental contaminants whose small sizes and low densities facilitate transport by wind.  Transport by wind erosion alongside soils or sediments results in mechanical abrasion of the plastic surfaces which can alter their physical and chemical properties.  This paper using laboratory simulations to determine the effects of up to 216 hours of aeolian abrasion on polyethylene microplastics by angular, sub-rounded and rounded mineral sediments.  During the abrasion process the mineral particles break down producing small fragments which adhere to the microplastic surfaces altering their surface roughness and chemistry.  With increasing duration of abrasion the microplastic surface becomes coated with mineral fragments changing the dominant surface element from carbon to oxygen and silicon reflecting the composition of the erodents. The coating develops more rapidly when microplastics are abraded with angular sediments as these produce a lot of small fragments within the first 1-2 hours.  However, after > 200 hours of abrasion all the erodents had similar effects.  A model of microplastic surface change is presented in which the plastic cracks and fractures, then flattens alongside the increasing density of sediment fragment cover.  Surface changes may affect the ability of the plastics to transport airborne contaminants.

How to cite: Alvarez Barrantes, L., Bullard, J. E., Davis, S., McKenna Neuman, C., O’Brien, P., Roach, P., and Zhou, Z.: The effects of sediment properties on the aeolian abrasion and surface characteristics of microplastics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1526, https://doi.org/10.5194/egusphere-egu25-1526, 2025.

EGU25-1543 | ECS | Orals | AS3.8

Global climate model development: Adding microplastics to the UK Earth System Model 

Cameron McErlich, Catherine Hardacre, Felix Goddard, Nikos Evangeliou, and Laura Revell

Airborne microplastics, an emerging class of anthropogenic aerosols, are small and lightweight, allowing them to remain suspended in the atmosphere for extended periods of time. Their detection in remote locations (such as Antarctica) and in high-altitude cloud water raises questions about their potential impacts on climate systems. As global climate models do not routinely include airborne microplastics as an aerosol species, the full consequences of microplastics on climate remain uncertain. To investigate these impacts, we have incorporated micro- and nanoplastics (MnP) as a new aerosol species within GLOMAP-mode, the aerosol scheme used in the United Kingdom Chemistry & Aerosols (UKCA) component model of the UK Earth System Model (UKESM). MnP have been implemented in GLOMAP-mode alongside the existing aerosol species of sulfate, black carbon, organic carbon, sea salt and dust.  Microplastics can be emitted into UKESM as both fragments and fibres. MnP are added to the Aitken (5 – 50 nm), accumulation (50 - 500 nm), coarse (> 500 nm) and super-coarse (> 2500 nm) modes. Emissions are sourced from an observationally-derived dataset with global spatial coverage. MnP are initially emitted in insoluble modes but can transition to soluble modes through the accumulation of organic material on their surfaces, enabling them to act as CCN. Airborne microplastics in UKSEM transported and can be removed from the atmosphere by both dry and wet deposition processes. We present preliminary results using the new microplastics scheme, which has been run for both microplastics fragments and fibres. Our novel microplastic scheme is a significant advancement in modelling airborne microplastics and lays the groundwork for understanding their impact on climate and the wider Earth system.

How to cite: McErlich, C., Hardacre, C., Goddard, F., Evangeliou, N., and Revell, L.: Global climate model development: Adding microplastics to the UK Earth System Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1543, https://doi.org/10.5194/egusphere-egu25-1543, 2025.

EGU25-2806 | Posters on site | AS3.8

Microplastic Distibution and Magnetic Susceptibility in Size-Fractionated Road Dust from Warsaw: Environmental Implications. 

Małgorzata Kida, Sylwia Dytłow, and Sabina Ziembowicz

Road dust samples were collected in Warsaw, the capital of Poland and assessed both as a whole (“all”) and after separation into five size fractions: (1–0.8 mm, “0.8”), (0.8–0.6 mm, “0.6”), (0.6–0.4 mm, “0.4”), (0.4–0.2 mm, “0.2”), and (below 0.2 mm, “<0.2”). RD is composed of the “0.4” and “0.8” fractions, which contribute the most to the total mass, whereas “<0.2” and “0.2,” have a lower overall contribution.

The qualitative and quantitative analysis of microplastics (MPs) in various fractions of road dust revealed the presence of materials such as acrylonitrile butadiene styrene (ABS), polyamide, naturally occurring polyamide, polymethyl methacrylate (PMMA), polytetrafluoroethylene (PTFE), polyurethane (PU), polyvinyl chloride (PVC), and rubber. The largest quantities were observed for polypropylene and rubber, while the smallest quantities of MPs were recorded in the largest analyzed fraction of dust, "0.8". Conversely, the highest number of MPs, amounting to 51,660 particles, was noted in the smallest fraction, "<0.2," in sample WAW4. An increasing trend in the number of MPs was observed with decreasing particle size in samples WAW1 and WAW4. Plastic particles can pose significant environmental risks, not only due to their presence but also because of the additives used in plastics manufacturing. The road dust samples were analyzed for bisphenol A and phthalic acid esters, which act as plasticizers. Four phthalates were detected: dimethyl phthalate (DMP), dibutyl phthalate (DBP), bis(2-ethylhexyl) phthalate (DEHP), and di-n-octyl phthalate (DNOP). The highest concentrations were recorded for DBP and DEHP, reaching 48.72 µg/g and 37.59 µg/g, respectively, in sample WAW2 for the "<0.2" fraction. A strong correlation was found between MPs and DEHP in samples WAW1 and WAW4, indicating the release of this contaminant from plastics. For the other contaminants, no significant correlations were observed, suggesting diverse sources of these substances in the analyzed samples.Magnetic susceptibility analysis reveals the highest values in the “<0.2” fraction, with bulk samples showing intermediate levels and coarser fractions generally lower. An exception is observed at WAW1, where the “0.8” fraction exhibits the highest χ.

Strong Pearson coefficients were obtained  between χ  and DEHP (0.78), DBP (0.96), and BPA (0.89) for WAW2. For WAW3, the best correlation with  χ was observed for DEHP (0.89), whereas for WAW4, an excellent correlation was found between MPs (0.97) and DBP (0.9). For the finest fractions “0.2” and “<0.2”, strong correlations were observed between χ, DBA and DBP (ranging from 0.8 to 0.9). Such a result may indicate a good prospect for using χ for the preliminary assessment of DBA and BPA concentrations in fine fractions of RD.

Acknowledgment
This research was funded in whole by the National Science Centre (Poland), grant number 2021/43/D/ST10/00996. This work was supported by a subsidy from the Polish Ministry of Education and Science for the Institute of Geophysics, Polish Academy of Sciences. 

How to cite: Kida, M., Dytłow, S., and Ziembowicz, S.: Microplastic Distibution and Magnetic Susceptibility in Size-Fractionated Road Dust from Warsaw: Environmental Implications., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2806, https://doi.org/10.5194/egusphere-egu25-2806, 2025.

EGU25-6787 | Orals | AS3.8 | Highlight

Plastic burning: An important global source of atmospheric nanoplastic particles 

Arthur Chan, Hongru Shen, Lin Kong, Michael Tawadrous, Xing Wang, Jonathan Abbatt, Man Nin Chan, and Alex Lee

Small nano-sized plastic particles can enter the atmosphere and be transported globally from source areas to remote regions. In contrast to secondary nanoplastic emissions, plastic materials exposed to high temperatures can emit large amounts of nanoplastics directly into the atmosphere. However, very little is known about emission rates and physical and chemical characteristics of these particles. In this work, we conducted laboratory smoldering experiments to simulate smoldering emissions of PVC, PP, LDPE, PET and PS. We measured the chemical composition using aerosol mass spectrometry show that both polymeric materials (characteristic of nanoplastics) and thermo-oxidation products are emitted in submicron particles. Based on the emission factors measured, we estimate that plastic waste burning and building fires can contribute roughly 0.5–5 megatons per year of nanoplastics, which exceeds emissions from oceans, and comparable to tire wear.

The chemical fate of these particles was also examined by exposing the particles to atmospheric oxidants. We observe that these particles can age at appreciable rates under simulated oxidation conditions, on the order of days to weeks. These rates are similar to that of organic aerosol. This extent of oxidation in the atmosphere has strong implications on their hygroscopicity and their atmospheric fate, suggesting extensive oxidation prior to their deposition. Our laboratory studies provide mechanistic understanding for modeling atmospheric processes of nanoplastic particles and quantitative information for estimating atmospheric burden from plastic burning.

How to cite: Chan, A., Shen, H., Kong, L., Tawadrous, M., Wang, X., Abbatt, J., Chan, M. N., and Lee, A.: Plastic burning: An important global source of atmospheric nanoplastic particles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6787, https://doi.org/10.5194/egusphere-egu25-6787, 2025.

EGU25-7251 | Orals | AS3.8 | Highlight

Are we underestimating microplastic emissions from agricultural soils? 

Sujith Ravi and Sanjay Mohanty

Agricultural management practices significantly influence the the emission of particulate matter into the atmosphere, which is a key component of air quality indicators. In particular, agricultural soils in drylands, which constitute ~40% of Earth's terrestrial surface, are highly vulnerable to emissions via accelerated wind erosion because of factors such as increased aridity, recurrent droughts, crop failures, lack of irrigation, and unsustainable soil management practices. These lands are often subjected to large-scale biosolid application, irrigation with reclaimed (grey) water, and plastic mulching to meet the growing demand for water and to reduce reliance on fossil fuel-intensive fertilizers. However, these practices could significantly increase microplastics in the topsoil. Wind can transport these microplastic particles beyond agricultural systems, potentially carrying adsorbed contaminants such as per- and polyfluoroalkyl substances (PFAS). To evaluate inhalation exposure risks, it is crucial to understand the extent of microplastic pollution and the mechanisms driving their resuspension from agricultural soils. To investigate microplastic emission potential, we used a combination of wind tunnel studies and laboratory experiments on biosolid-amended agricultural soils. Our findings reveal that inhalable microplastics are preferentially entrained and enriched through two primary mechanisms: (1) the accelerated emission of fine plastic particles under wind conditions that are lower than those required for initiating movement of background soil particles (direct suspension without saltation), and (2) the generation and resuspension of fine plastic particles resulting from the abrasion of larger plastic fragments or soil-plastic aggregates by sand grains (saltation-induced suspension). We developed a theoretical framework to explain this preferential transport, attributing it to the low density and reduced interparticle forces between microplastics and soil. Our findings suggest that current methods and models for fugitive dust emissions may underestimate the particulate matter emission potential of amended soils. This is due to limitations in detecting fine particles during sampling and the inadequate representation of plastic entrainment mechanisms (e.g., suspension without saltation) in existing dust emission models. To illustrate this, we demonstrated that over 85% of wind events above bare soil surface exceed the threshold velocity required to mobilize microplastics of a specific size, while only 20% of these events surpass the threshold velocity for background soil particles. Given that fine microplastics may adsorb contaminants from agricultural soils, their preferential entrainment by wind could lead to a concentration of these contaminants in airborne dust, posing potential environmental and health risks.

How to cite: Ravi, S. and Mohanty, S.: Are we underestimating microplastic emissions from agricultural soils?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7251, https://doi.org/10.5194/egusphere-egu25-7251, 2025.

EGU25-7749 | Orals | AS3.8

Airborne microplastic concentrations in remote coastal environments 

Joel Rindelaub, Jennifer Salmond, Wenxia Fan, and Gordon Miskelly

While plastics have been detected in remote locations across the planet, there remains uncertainty in the mechanisms governing global microplastic transport. The transfer of plastic pollution from the marine environment to the air via crashing waves may be a significant avenue of atmospheric microplastic entrainment. In this study, sampling was conducted at coastal locations in Aotearoa New Zealand, a remote region near the Southern Ocean that does not contain high levels of plastic production. Results from both active and passive sampling, in conjunction with air parcel back trajectory analysis, indicated that local atmospheric microplastic concentrations were derived from the marine environment. The use of pyrolysis GC/MS allowed for the determination of airborne mass concentrations of seven different polymers, finding that airborne microplastic levels at remote coastal areas were similar to those previously reported at urban sampling locations. These results highlight the significance of the air-ocean interface in relation to long range microplastic transport, and further work relating to the impacts on climate – such as in the Southern Ocean region – and to local health are warranted.

How to cite: Rindelaub, J., Salmond, J., Fan, W., and Miskelly, G.: Airborne microplastic concentrations in remote coastal environments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7749, https://doi.org/10.5194/egusphere-egu25-7749, 2025.

EGU25-8428 | ECS | Posters on site | AS3.8

Atmospheric microplastic measurements reconciliation with emission estimates: A Lagrangian approach 

Ioanna Evangelou, Nikolaos Evangeliou, and Andreas Stohl

Microplastics (MPs), defined as particles measuring between 1 μm and 5 mm, originate from the fragmentation of larger plastic materials or are produced intentionally. These particles have attracted considerable attention in aquatic, terrestrial, and marine environments. Despite the pivotal role played by the atmosphere in the global transport and dispersion of MPs, there is a paucity of data concerning their atmospheric abundance and deposition. Additionally, the existing measurements exhibit substantial variability, and global estimates of total MP emissions tend to reflect significant inconsistencies based on the estimation method.

This study seeks to address these gaps by reconciling current measurement data with estimated emission fluxes through a detailed analysis of source-receptor relationships that link emissions, atmospheric concentrations, and deposition measurements. To establish these source-receptor relationships, we employ the Lagrangian particle dispersion model FLEXPART, considering various shapes and sizes of microplastics. Back trajectory analysis is utilized to elucidate the sources of MPs in distinct geographical regions. Three MP emission inventories, estimated with different methods, are combined with the back trajectory output to yield the simulated values at the measurement locations.

For the geographical region of Europe, around 50% of the simulated MP concentration values agree with the measured values within a factor of 10, while only 5% of the simulated deposition is in a 10-factor range of the deposition data. A clear overprediction of the modeled values indicates that the available emissions may be lower, that the transport and scavenging scheme of the model should be reconsidered, or that the measuring and identification methodologies are coming with substantial errors. We emphasize that a uniform sampling protocol should be created to achieve reliable and comparable data, and more efforts should be made to create bottom-up emission inventories based on relevant emission factors and proxies.

How to cite: Evangelou, I., Evangeliou, N., and Stohl, A.: Atmospheric microplastic measurements reconciliation with emission estimates: A Lagrangian approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8428, https://doi.org/10.5194/egusphere-egu25-8428, 2025.

EGU25-8481 | Posters on site | AS3.8

Atmospheric Dry and Wet Deposition of Microplastics in an Urban Area and a Remote Island: Year-Round Consecutive Monthly Observations 

Yun-Jung Ji, Seung-Kyu Kim, Zhexi Tian, Min-Jae Seong, Jun-Hyuk Shin, Chan-Yeong Je, Eun-Seo Jeong, and Un-Hyuk Yim

Atmospheric transport and deposition are key processes in the global spread of microplastics (MPs). However, field-based observational data are limited, and the dynamics of MP transport and deposition are still insufficiently understood. This study aimed to identify the effects of long-range transport and urbanization by comparing identical time-series data on atmospheric MP deposition between an urban city (Seoul, SE; ~10 million residents) and a remote region (Baengnyeong Island, BI; located on the Yellow Sea). In 2023, atmospheric MP deposition samples were simultaneously collected from both regions during the same period every month. Each sample was continuously collected using selective air deposition samplers to separate dry (DD) and wet deposition (WD). A total of 48 samples, comprising 12 pairs of DD and WD from each site, were analyzed for MPs (≥20 µm). Both sites exhibited a lower trend in total deposition (TD; sum of DD and WD) flux of MPs during the summer compared to other seasons, suggesting that MP deposition was influenced by atmospheric stability and monsoon scouring effects. Despite similar monthly pattern, TD flux of MPs was 3.5 times higher at SE (271±155 n/m²/day) than at BI (77.1±76.4 n/m²/day), with significant differences between the two regions for all monthly samples (paired t-test; p<0.01) except for March, supporting the emission effect from local sources in urban area. In March, which was marked by the dominance of westerly winds from eastern China and the highest aerosol (PM10) concentrations at both BI and SE, MP-TD fluxes recorded the highest at BI (311 n/m2/day) and the second highest at SE (330 n/m2/day) among those observed at each site. The March-MP flux increased by 6.3-fold (BI) and 1.6-fold (SE) compared to other months, with a larger increase in BI compared to PM10 (2.4-fold vs. 2.3-fold), indicating stronger trans-boundary transport at the remote regions. Major five polymers accounted for 94.4% (BI) and 84.2% (SE) of MPs, with the most weathering-prone PP dominating (69.0% and 59.3%), indicating fugitive input from aged plastics. WD was 10 (BI) and 5 (SE) times more efficient in MP deposition than DD, but contributed only 47% (BI) and 36% (SE) to monthly TD due to limited precipitation. Although fragment-shaped MPs prevailed in TDs of both BI (88.6%) and SE (94.9%), higher fiber proportion in WD than DD (14.2% vs. 8.2% in BI and 5.8% vs. 3.7% in SE) represented susceptible precipitation-scavenging potential of fibers. However, higher proportion of fibers in TD of BI (10.7%) than of SE (4.5%), with significant differences (p<0.01) between the two regions, suggests that fibers are more likely to survive long-distance transport. Our findings help improve the uncertainties in global MP dispersion and budget.

Acknowledgement: This work was supported by 'Land/Sea-based input and fate of microplastics in the marine environment' of Korea Institute of Marine Science & Technology Promotion (KIMST) funded by the Ministry of Oceans and Fisheries, Republic of Korea (20220357), and was also partially supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIT) (No. RS-2024-00356940).

How to cite: Ji, Y.-J., Kim, S.-K., Tian, Z., Seong, M.-J., Shin, J.-H., Je, C.-Y., Jeong, E.-S., and Yim, U.-H.: Atmospheric Dry and Wet Deposition of Microplastics in an Urban Area and a Remote Island: Year-Round Consecutive Monthly Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8481, https://doi.org/10.5194/egusphere-egu25-8481, 2025.

EGU25-10405 | ECS | Posters on site | AS3.8

A Comparative Examination of Atmospheric Models for Studying Airborne Micro- and Nanoplastic Pollution 

Thies Hamann, Peter Braesicke, Jan Bumberger, and Lennart Schüler

The apparent omnipresence of plastic waste is a serious global issue. The question of micro- and nanoplastics pollution in the environment has been more widely addressed in recent years, and its occurrence in the oceans, freshwater systems, air, soil and various organisms has been well documented [1]. This widespread pollution not only threatens ecosystems it also raises concerns about potential impacts on human health [2]. Alongside the well-studied transport pathway in marine and freshwater systems, micro- and nanoparticles can also be distributed via airborne pathways [1]. In-situ sampling sites provide only in-direct evidence of some possible pathways. Thus, the use of atmospheric models to study atmospheric pathways of different classes of micro- and nanoplastics can give valuable insights into the atmospheric redistribution and possible sources. Various models can be used to describe the behaviour of airborne particles. Trajectory models, like HYSPLIT [3], trace the path of an air parcel with low computational effort, excluding the effect of diffusion and turbulence. In contrast, the weather forecast model ICON and its aerosol and reactive trace gases module ART account for these factors [4], describing the status and the development of the atmosphere in more detail. Using the data of nanoplastic in-situ measurements at a remote sampling site in the high-altitude Alps [5] and the combination of HYSPLIT backwards and ICON-ART forwards simulations, the two model types are compared and characterized, exploring their potential and limitations in describing airborne micro- and nanoplastic particle distributions and revealing potential pathways and attributing possible source regions.

 

[1] Allen, Steve, et al. "Micro (nano) plastics sources, fate, and effects: What we know after ten years of research." Journal of Hazardous Materials Advances 6 (2022): 100057.
[2] Lehner, Roman, et al. "Emergence of nanoplastic in the environment and possible impact on human health." Environmental science & technology 53.4 (2019): 1748-1765.
[3] Stein, Ariel F., et al. "NOAA’s HYSPLIT atmospheric transport and dispersion modeling system." Bulletin of the American Meteorological Society 96.12 (2015): 2059-2077.
[4] Rieger, Daniel, et al. "ICON-ART 1.0–a new online-coupled model system from the global to regional scale." Geoscientific Model Development Discussions 8.1 (2015): 567-614.
[5] Materić, Dušan, et al. "Nanoplastics transport to the remote, high-altitude Alps." Environmental Pollution 288 (2021): 117697.

How to cite: Hamann, T., Braesicke, P., Bumberger, J., and Schüler, L.: A Comparative Examination of Atmospheric Models for Studying Airborne Micro- and Nanoplastic Pollution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10405, https://doi.org/10.5194/egusphere-egu25-10405, 2025.

EGU25-11340 | ECS | Posters on site | AS3.8

Physical and Chemical Characterisation of Nanoplastic Aerosol  

Peter J. Wlasits and Paul M. Winkler

Physical and Chemical Characterisation of Nanoplastic Aerosol

Peter J. Wlasits1, and Paul M. Winkler1

1 Faculty of Physics, University of Vienna, Vienna, Austria

 

Mass production of plastic products has led to an environmental problem on global scale. Consequently, an increasing number of studies has investigated the impact of micro- and nanoplastics on the environment in recent years (e. g. Amobonye et al., 2021). As a consequence of their small sizes, nanoplastic particles undergo long range atmospheric transport and deposit in remote regions (Materić et al., 2021; 2022). Hence, measurement techniques capable of accurately detecting nanoplastic aerosol are urgently needed.

The presented project, funded by the Austrian Science Fund (FWF) [10.55776/PAT5114323], relies on the controlled generation of nanoplastic particles from gas-to-particle conversion (Wlasits et al., 2022). The aforementioned generation method enables process level studies under well-defined laboratory conditions.

Accordingly, nanoplastic aerosols will be generated by exposing selected macroplastics to thermal stress in a tube furnace (Wlasits et al., 2022). Aerosol particles will then be size selected using a differential mobility analyser and subsequently fed into detectors for physical and chemical analysis. The chemical composition of the generated particles will be investigated using an atmospheric pressure interface time-of-flight mass spectrometer, capable of analysing particles of both polarities simultaneously. Prior to mass analysis particles will undergo thermal decomposition and ionisation. Physical characterisation will be performed using the Size Analysing Nuclei Counter (SANC), an expansion-type condensation particle counter providing nucleation probabilities as a function of the saturation ratio (Wlasits et al., 2023).

In summary, the outlined project is based on a comprehensive experimental approach combining physical and chemical information about nanoplastic aerosol. New insights on the influence of nanoplastic particles on cloud formation will be gained and the potential use of condensation techniques for nanoplastic detection will be investigated.

 

References

Amobonye, A., Bhagwat, P. , Raveendran, S., Singh, S., and Pillai, S., Microbiol., 12, 768297, 2021, doi:10.3389/fmicb.2021.768297.

Materić, D., Ludewig, E., Brunner, D., Röckmann, T., and Holzinger, R., Environ. Pollut., 288, 117697, 2021, doi:10.1016/j.envpol.2021.117697.

Materić, D., Kjær, H. A., Vallelonga, P., Tison, J.-L., Röckmann, T., and Holzinger, R., Environ. Res., 208, 112741, 2022, doi:10.1016/j.envres.2022.112741.

Wlasits, P. J., Stoellner, A., Lattner, G., Maggauer, K., and Winkler, P. M., Aerosol Sci. Technol., 56 (2), 176–185, 2022, doi:10.1080/02786826.2021.1998339.

Wlasits, P. J., Konrat, R., and Winkler, P. M., Environ. Sci. Technol., 57 (4), 1584–1591, 2023, doi:10.1021/acs.est.2c07643.

How to cite: Wlasits, P. J. and Winkler, P. M.: Physical and Chemical Characterisation of Nanoplastic Aerosol , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11340, https://doi.org/10.5194/egusphere-egu25-11340, 2025.

EGU25-11439 | ECS | Posters on site | AS3.8

Quantifying the detachment dynamics of microplastic car tire-wear particles using a deep learning framework in a laboratory wind tunnel. 

Bashir Olasunkanmi Ayinde, Wolfgang Babel, Johannes Olesch, Seema Agarwal, Daniel Wagner, Anke Nölscher, and Christoph Thomas

Traffic-related microscale particles, including passenger car tire-wear particles (PCTWPs), are recognised as one of the primary sources of microplastic pollution. While the chemical composition, shape characterisation, and emission rates of these non-exhaust traffic emission have received some attention, their detachment behaviour from surfaces into the air after deposition remains poorly understood. Their irregular, elongated shapes and relative orientation to the near-surface airflows pose significant challenges which influence aerodynamic performance. Moreover, the effect of their spatial deposition pattern at detachment needs to be studied as it may be relevant for potential particle-particle blockages and impacts. Owing to the multifactorial nature of drivers controlling the detachment process which may not lend itself to simple multi-linear correlation, we use a state-of-the-art deep learning (DL) based instance segmentation model, named You Only Look Once version 8 nano (YoloV8n) to detect, segment, characterise, and resolve particle detachment in high-resolution imagery from wind tunnel experiments. Three different PCTWP seeding approaches, namely tipping, sieving, and fabricated pressurised methods were evaluated and compared to identify the optimal method for uniform particle distribution with minimal agglomerates on substrates. The fabricated pressurised seeding method was selected as the optimal technique adopted for subsequent detachment experiments. PCTWPs were deposited onto glass surfaces and exposed to evolving, turbulent flow conditions. The model performance was evaluated using a variety of statistical quantities from the DL model including precision, recall, Intersection over Union (IoU) and dice coefficient metrics. The resolved detachment was analysed under two different transient conditions, subject to flow evolution, using PCTWPs with various size distributions (50µm - 220µm). For each condition, eight replicates were conducted to ensure statistical reliability. The analysis was performed as a function of time and friction velocity. Our results revealed that PCTWPs exhibit a median threshold fluid friction velocity at 0.46m/s for detachment, which is notably higher than that of polyethylene beads of 0.13 m/s for particles of the same size cohort. This highlights the significant role of local variations in the balance of forces and particle shape plays a crucial role in influencing detachment potential.

How to cite: Ayinde, B. O., Babel, W., Olesch, J., Agarwal, S., Wagner, D., Nölscher, A., and Thomas, C.: Quantifying the detachment dynamics of microplastic car tire-wear particles using a deep learning framework in a laboratory wind tunnel., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11439, https://doi.org/10.5194/egusphere-egu25-11439, 2025.

EGU25-11924 | Posters on site | AS3.8

Atmospheric microplastics emissions estimation and uncertainty quantification using Gibbs sampler 

Ondřej Tichý, Václav Košík, Václav Šmídl, and Nikolaos Evangeliou

This study quantifies microplastics based on atmospheric concentration measurements, achieved by optimizing the measurements against the theoretical output of an atmospheric transport model. The core of our contribution is addressing the severe ill-posedness of this inverse problem, as the solution space for spatial-temporal emissions is much larger than the number of available measurements. For regularization of the inverse problem, we assume that microplastics sources follow patterns from agriculture, dust, road dust, and ocean emissions. The emissions are mapped to measurements using source-receptor sensitivity relations, forming an optimization problem. To rigorously estimate emissions and precisely quantify the associated uncertainties, we developed a hierarchical prior model, whose parameters are estimated using a Gibbs sampler. Our results show that the estimates are significantly uncertain, with standard deviations often being about the same size as the mean values. We conclude that uncertainties are reasonably quantified considering the issue related to the microplastics measurements and modeling.

Acknowledgment:

This research has been supported by the Czech Science Foundation (grant no. GA24-10400S).

How to cite: Tichý, O., Košík, V., Šmídl, V., and Evangeliou, N.: Atmospheric microplastics emissions estimation and uncertainty quantification using Gibbs sampler, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11924, https://doi.org/10.5194/egusphere-egu25-11924, 2025.

EGU25-12448 | ECS | Orals | AS3.8

Potential Influence of Microplastics on Cloud Formation through Heterogeneous Ice Nucleation 

Teresa M. Seifried, Sepehr Nikkho, Aurelio Morales Murillo, Lucas J. Andrew, Gurcharan Uppal, Cameron Varcoe, Steven N. Rogak, Edward R. Grant, and Allan K. Bertram

Recent studies highlight the environmental threat of microplastic pollution, both in waterways and as airborne particles.1,2 Airborne microplastics may affect climate by influencing cloud formation and precipitation through heterogeneous ice nucleation.3,4 In addition, if microplastics are effective at nucleating ice, their lifetime may be influenced by ice nucleation followed by precipitation. Yet, the role of microplastics as ice-nucleating particles and their impact on cloud ice formation remains largely unknown.

Here, we present evidence of ice nucleation in the immersion freezing mode induced by various microplastics. Specifically, two polypropylene samples and one polyethylene terephthalate sample exhibited heterogeneous freezing with median temperatures of -20.9°C, -23.2°C, and -21.9°C, respectively, while the water background froze at -25.8°C. The number of ice nucleation sites per surface area, ns(T), ranged from 10-1 to 104 cm-2 within a temperature range of -15 to -25°C, similar to volcanic ash and fungal spores. Following exposure to ozone or a combination of UV light and ozone, mimicking atmospheric aging, the ice nucleation activity either decreased or remained unchanged.5

In addition, we investigated the ice nucleation ability of tire wear particles, which are classified as microplastics and are considered a dominant type of urban airborne microplastics.6 Tire wear aerosols were generated by running a truck on a dynamometer to simulate real-world driving conditions. Aerosols were collected on Nuclepore filters and tested for freezing activity, revealing freezing temperatures above the water background.

Our freezing data suggest that microplastics including tire wear samples may promote ice formation in cloud droplets. In addition, based on a comparison of our freezing results and previous simulations using a global transport model, ice nucleation by microplastics will impact their long-range transport to faraway locations and global distribution.

 

References:

1. Dris, R.; Gasperi, J.; Rocher, V.; Saad, M.; Renault, N.; Tassin, B. Microplastic Contamination in an Urban Area: A Case Study in Greater Paris. Environ. Chem. 2015, 12 (5), 592–599.

2. Allen, S.; Allen, D.; Baladima, F.; Phoenix, V. R.; Thomas, J. L.; Le Roux, G.; Sonke, J. E. Evidence of Free Tropospheric and Long-Range Transport of Microplastic at Pic Du Midi Observatory. Nat. Commun. 2021, 12 (1), 7242.

3. Ganguly, M.; Ariya, P. A. Ice Nucleation of Model Nanoplastics and Microplastics: A Novel Synthetic Protocol and the Influence of Particle Capping at Diverse Atmospheric Environments. ACS Earth Space Chem. 2019, 3 (9), 1729–1739.

4. Aeschlimann, M., Li, G., Kanji, Z.A. and Mitrano, D.M. Potential impacts of atmospheric microplastics and nanoplastics on cloud formation processes. Nat. Geosci. 2022, 15(12), 967-975.

5. Seifried, T.M., Nikkho, S., Morales Murillo, A., Andrew, L.J., Grant, E.R. and Bertram, A.K. Microplastic particles contain ice nucleation sites that can be inhibited by atmospheric aging. Environ. Sci. Technol. 2024, 58(35), 15711-15721.

6. Evangeliou, N., Grythe, H., Klimont, Z., Heyes, C., Eckhardt, S., Lopez-Aparicio, S. and Stohl, A. Atmospheric transport is a major pathway of microplastics to remote regions. Nat. Commun., 2020, 11(1), 3381.

How to cite: Seifried, T. M., Nikkho, S., Morales Murillo, A., Andrew, L. J., Uppal, G., Varcoe, C., Rogak, S. N., Grant, E. R., and Bertram, A. K.: Potential Influence of Microplastics on Cloud Formation through Heterogeneous Ice Nucleation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12448, https://doi.org/10.5194/egusphere-egu25-12448, 2025.

EGU25-13014 | ECS | Posters on site | AS3.8

Quantification of wind-driven MP mobilisation potential in semi-arid regions in Kazakhstan using wind tunnel experiments 

Steve Utecht, Miriam Marzen, Moritz Koza, Tobias Schütz, Gerd Schmidt, Kanat Akshalov, Johannes B. Ries, and Roger Funk

The northeastern steppe landscape of Kazakhstan, with its loess soils, flat terrain, and erosive climate, is highly susceptible to aeolian processes, which can lead to extensive and variable soil mobilisation and deposition. Although agricultural activity has been low in recent decades, the introduction of modern practices has intensified agriculture, potentially leading to greater plastic emissions from irrigation and plant growth and protection systems. Despite extensive global research on microplastics (MP, <5 mm in size) in natural systems, their transport and deposition via aeolian processes, as well as their production and input rates on agricultural land in continental climate zones, have received little attention to date.

In this study, wind-driven MP mobilisation was quantified by on-farm experiments on two sites, with Zhelezinka on Haplic Kastanozem soil, and Shortandy on Haplic Chernozem soil. While both sites are for agricultural use, the management differs in terms of soil tillage, fertilizer input, pest management, and irrigation. A portable boundary layer wind tunnel was applied for five 15-minute tests with a wind speed of 14 m s⁻¹. This accounts for an average wind speed that occurs in this region for an average of six hours per year, representing relatively extreme conditions used to assess the overall potential for wind-driven MP mobilisation at the study sites. Samples were collected using an aluminium wedge trap, covering approximately 1% of the tunnel mouth's area, and were characterised using confocal micro-Raman spectroscopy.

The total results reveal 2.24 g min⁻¹ mobilised soil material at Shortandy and 14.52 g min⁻¹ at Zhelezinka, with MP mobilisation of 0.01 g min⁻¹ (89 MP items) and 0.14 g min⁻¹ (1206 MP items), respectively. The detected MP varied in shape (fragments and fibres) and size, with all detections having diameters smaller than 150 μm. Greater variability in MP types, predominantly fragments (PPSU, PP, PE, PMMA), was observed at Zhelezinka. In contrast, Shortandy showed fewer MP mobilisation, with only one plastic type (PA) identified and a more balanced distribution between fragments and fibres compared to Zhelezinka. The overall fragment-to-fibre ratio is 31:1. The differences in MP mobilisation between the sampling sites can be explained by varying land use durations and intensities. The study highlights that wind erosion can make a significant contribution to the local and regional distribution of MP in the northeastern steppe of Kazakhstan.

How to cite: Utecht, S., Marzen, M., Koza, M., Schütz, T., Schmidt, G., Akshalov, K., Ries, J. B., and Funk, R.: Quantification of wind-driven MP mobilisation potential in semi-arid regions in Kazakhstan using wind tunnel experiments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13014, https://doi.org/10.5194/egusphere-egu25-13014, 2025.

EGU25-13643 | ECS | Posters on site | AS3.8

Occupational Exposure to Elevated Levels of Inhalable Microplastics in Plastic and Fiber Factory Workers 

Guyu Peng, Mikko Mikko Poikkimäki, Maija Leppänen, Tomi Kanerva, Dušan Materić, and Thorsten Reemtsma

Micro(nano)plastics enter the human body mainly through inhalable and oral uptake, and the fraction below 20 μm can penetrate biological membranes, accumulate in tissues, and induce cytotoxicity and inflammation. While inhaled indoor air may be a primary source of exposure, concentrations are potentially higher in occupational settings in the plastic and fiber factories. Here, external exposure to inhalable microplastics <100 µm was studied in four industrial workplaces: two non-woven fabric production factories, and two different plastics recycling facilities located in Finland and Spain. Air samples were collected from the worker breathing zone and stationary measurements during various production tasks. For comparison, urban aerosols were assessed in two urban locations in Finland and in France. Inhalable microplastics in the aerosol samples were analyzed using FTIR (Fourier-transform infrared microscopy) imaging and Raman spectroscopy equipped with automated particle analysis and identification algorithms. In addition, total particle number concentration (PNC, 20 – 700 nm) were measured in parallel. PNC varied between the workplaces and tasks, ranging from 2000 to 50000 #/cm3. Aerosols in the plastic recycling factory predominantly contained PS, ABS, PP, PE and EVA particles at elevated concentration, averaging 2000 #/m3 for the inhalable fraction (<100 µm) and 1500 #/m3 for the thoracic and respirable fraction (<10 µm), based on FTIR imaging and Raman analyses. In non-woven fabric manufacturing facilities, inhalable microplastics were dominated by PET fibers, along with PA, PP and PE particles. The median size of inhalable microplastics ranged from 23 – 40 µm in occupational aerosols. Inhalable microplastics in aerosols from the 4 factories ranked among the highest concentrations reported to date, indicating elevated health risks for exposed workers. These novel findings from the validation of sampling and analytical strategies underscore the significance in reducing airborne microplastic emissions and mitigating inhalation exposure, especially in occupational settings.

How to cite: Peng, G., Mikko Poikkimäki, M., Leppänen, M., Kanerva, T., Materić, D., and Reemtsma, T.: Occupational Exposure to Elevated Levels of Inhalable Microplastics in Plastic and Fiber Factory Workers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13643, https://doi.org/10.5194/egusphere-egu25-13643, 2025.

EGU25-13857 | ECS | Posters on site | AS3.8 | Highlight

Do Microplastics Contribute to the Total Number Concentration of Ice Nucleating Particles? 

Daria Tatsii, Blaž Gasparini, Ioanna Evangelou, Silvia Bucci, and Andreas Stohl

Microplastics (MPs) can be transported into clouds, where they can affect formation and properties of clouds by acting as ice-nucleating particles (INPs), indirectly influencing the global climate.
However, MPs have not been considered contributors to total INP concentrations.
In this study, we quantify road traffic-related (i.e. from tire wear, brake wear, road markings and polymer-modified bitumen) MP number concentrations and estimate their contribution to total INP concentrations using the atmospheric transport model FLEXPART.
To do this, we provide two possible global road traffic-related MP emissions scenarios.
We find that MPs can disperse throughout the entire troposphere and reach regions with low natural ice nucleating particle concentrations.
Under a high emissions scenario, ice-active MPs can contribute from about 0.1% to more than 40% of the total INP number under immersion freezing conditions in some areas of the tropics, while under cirrus conditions, their contribution can be up to about 7% over the tropical Pacific and up to about 20% over East Antarctica.
Our results suggest that in regions where other effective INPs are rare, ice-active MP concentrations may be sufficient to trigger heterogeneous ice nucleation of ice crystals in mixed-phase or cirrus clouds, especially when concentrations of other effective INPs (mineral dust, marine particles, or bioaerosols) are low or absent.
These results underscore the potential role of MPs in cloud formation and highlight the need to reduce uncertainties in MP emissions and their fate in the atmosphere as plastic production and use continue to grow.

How to cite: Tatsii, D., Gasparini, B., Evangelou, I., Bucci, S., and Stohl, A.: Do Microplastics Contribute to the Total Number Concentration of Ice Nucleating Particles?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13857, https://doi.org/10.5194/egusphere-egu25-13857, 2025.

EGU25-14538 | Orals | AS3.8

A Multi-Platform Study on Atmospheric Deposition Flux of Microplastics in the East Sea (Sea of Japan) 

Jongcheon Won, Andrew Loh, Joon Geon An, Donghwi Kim, and Un Hyuk Yim

The atmosphere is recognized as one of the major pathways for microplastics (MPs) transport from land to the ocean. Reducing uncertainties in deposition flux estimates requires an integrated approach that combines temporal variability, evaluated through long-term monitoring at a fixed station, and spatial variability, assessed through mobile observations. In this study, the deposition flux and pollution characteristics of atmospheric microplastics in the East Sea were analyzed through long-term monitoring at a fixed station (Ulleung Island) and mobile observations conducted via a research vessel (R/V Onnuri). From November 2022 to October 2023, the total deposition flux of MPs measured at the fixed station ranged from 43 to 991 n/m²/day, with an average of 209 ± 281 n/m²/day. The average fluxes of dry and wet deposition were 119 ± 165 n/m²/day and 89 ± 120 n/m²/day, respectively. Although dry deposition exhibited a higher average flux than wet deposition, the difference was not statistically significant. Fragments (67.2%) accounted for the majority of MP shape, with the most common size range being 20-100 μm (72.9%). The dominant polymers identified were polypropylene (32.4%), followed by polyester (30.1%) and polyethylene (15.3%). Cluster-mean back trajectory analysis revealed that MPs in the East Sea originated not only from nearby marine sources but also from distant terrestrial air masses. The spatial distribution of MP deposition measured using a mobile platform showed a decreasing deposition flux with increasing distance from land. Smaller MPs were more frequently detected farther from land, along with a higher proportion of fibrous PES. These mobile observation results were consistent with those of MPs observed at a fixed station. These findings are expected to reduce uncertainties in estimating the atmospheric input of MPs into the ocean.

Acknowledgements

This research was supported by 'Land/Sea-based input and fate of microplastics in the marine environment' of Korea Institute of Marine Science & Technology Promotion (KIMST) funded by the Ministry of Oceans and Fisheries, Republic of Korea (RS-2022-KS221604).

How to cite: Won, J., Loh, A., An, J. G., Kim, D., and Yim, U. H.: A Multi-Platform Study on Atmospheric Deposition Flux of Microplastics in the East Sea (Sea of Japan), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14538, https://doi.org/10.5194/egusphere-egu25-14538, 2025.

High-resolution TD-PTR-MS as a novel analytical technique for nanoplastic detection – quantification in high-altitude glacial snow samples
Milena Latz1, Alasdair J Gill2, Robin Milner2, Dušan Materić1
1Helmholtz Centre for Environmental Research Leipzig, Permoserstr. 15, 04318 Leipzig/DE
2www.high-level-route.com
On the Haute Route – a known 19th century mountaineering route from Chamonix (France) to Zermatt (Switzerland), snow samples were taken on high-altitude glacial levels (2364-3734 m). Analyzing samples from less travelled areas allows for a general picture of current effects of human-made plastic pollution beyond our urban scope. In these remote regions, environmental pollution is mainly airborne and distributed via winds. In this case, especially small plastic particles of sizes <1 µm (nanoplastics) can be easily transported through the atmosphere and even reach remote places. Nanoplastic particles pose a large threat, not only to the ecosystem, but also to human health. Being carried by the air, these small particles can enter our respiratory system via inhalation, accumulate, and even introduce harmful substances such as chemicals, viruses, or bacteria into our system. In order to  further study current pollution levels and the effects on human health, an increased research in this field is necessary. To achieve this, glacial surface samples were analyzed for nanosized plastic particles via high-sensitivity TD-PTR-MS. Seven different plastic types (PE, PP, PS, PVC, PET, TWP, PTFE) were successfully detected.
TD-PTR-MS is a novel analytical method established for the detection of nanoplastics. While analysis of one sample can already be achieved in 15 min without lengthy preliminary steps, sample processing involves a more extensive pipeline. Both qualitive and semi-quantitative analysis of our environmental sample allowed for a detailed insight into plastic pollution in remote areas. Further analysis of the generated data through atmospheric particle dispersion modelling subsequently enables an outlook on the origins of plastic pollution detected.
The presented results were made possible through a citizen-science project in collaboration with the High Level Route Expedition (HLR-2022, https://www.high-level-route.com/). Especially in the field of environmental research, sample collection can be both a costly and time-intensive task. Moreover, travelling to remote, high-altitude areas can be dangerous for scientists lacking the necessary mountaineering training. Collaborations like these allow for safe, effective, and fast sampling at multiple sites at once, highlighting the importance of citizen-science projects for current research. With the promising results of the previous project in mind, we are introducing the Global Atmospheric Plastic Survey (GAPS, https://gaps2024.com/). This sampling project collaborates with mountaineers from across the world, generating data on plastic pollution on high-altitude remote regions worldwide. In this work, we can already report preliminary results from remote glaciers in Bolivia and the Tian Shen mountain range.

How to cite: Latz, M.: High-resolution TD-PTR-MS as a novel analytical technique for nanoplastic detection– quantification in high-altitude glacial snow samples, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16816, https://doi.org/10.5194/egusphere-egu25-16816, 2025.

EGU25-17157 | Orals | AS3.8

Can we identify the dominant sources of atmospheric microplastic? 

Silvia Bucci, Daria Tatsii, Ioanna Evangelou, and Andreas Stohl

Despite the increasing numbers of observations of atmospheric microplastic (MP), including at the poles, the marine boundary layer, clouds, high mountains snow, and the atmospheric fallout of densely populated areas, the identification of the main sources of emissions in the atmosphere remains complicated. Their emissions are still not well characterized and there are high uncertainties in the attempts of estimating their relative contributions. In this work, we apply to atmospheric microplastic observations a widespread method for source apportionment of air pollutants, based on Lagrangian modelling. We will specifically use the latest version of the state-of-the-art model, FLEXPART-v11 (Bakels et al., 2024), which incorporates the ability to simulate the transport patterns of irregular particles, such as fibers. These particles are characterized by higher drag coefficients (Tatsii et al., 2023) compared to the values typically assumed in conventional settling schemes, usually based on the assumption of spherical particles. The method will be applied to different time series of microplastic concentrations from literature, including data from Thermal Desorption - Proton Transfer Reaction - Mass Spectrometry (TD-PTR-MS) describing the total mass of MP, and data from micro-Raman and Fourier transform infrared spectroscopy (FT-IR), which instead provides information on particles counts, size, shape and composition. Among the results, the analysis suggests that ocean sources may be dominant in certain regions of the free troposphere, and that the total microplastic atmospheric emissions are not directly related to the population density, as instead often assumed.

References:

Bakels, L., Tatsii, D., Tipka, A., Thompson, R., Dütsch, M., Blaschek, M., Seibert, P., Baier, K., Bucci, S., Cassiani, M., Eckhardt, S., Zwaaftink, C. G., Henne, S., Kaufmann, P., Lechner, V., Maurer, C., Mulder, M. D., Pisso, I., Plach, A., . . . Stohl, A. (2024). Flexpart version 11: Improved accuracy, efficiency, and flexibility. Geoscientific Model Development, 17, 7595–7627.  https://doi.org/10.5194/gmd-17-7595-2024

Tatsii, D., Bucci, S., Bhowmick, T., Guettler, J., Bakels, L., Bagheri, G., & Stohl, A. (2023). Shape matters: Long-range transport of microplastic fibers in the atmosphere. Environmental Science Technology.  https://doi.org/10.1021/acs.est.3c08209

How to cite: Bucci, S., Tatsii, D., Evangelou, I., and Stohl, A.: Can we identify the dominant sources of atmospheric microplastic?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17157, https://doi.org/10.5194/egusphere-egu25-17157, 2025.

EGU25-17574 | ECS | Posters on site | AS3.8

POLARSENSE: Polar Online Airborne Nano and Microplastic Sensing and Environmental Monitoring 

Liam Kelleher, Steve Allen, Dusan Materic, Gijsbert Breedveld, and Stefan Krause

 

We present an automated tool for long-term sampling of nano and microplastics (NMP) and associated chemicals in remote areas, addressing a critical need for cost-effective, high-temporal-resolution data collection. A major challenge in NMP research is overcoming the financial and time constraints of intensive sampling campaigns.

To address this, we deployed two devices in the Arctic at the Ny-Ålesund research base, focusing on enhancing understanding of polar NMP distribution and transport mechanisms. The auto-sampling system utilises active air sample containers, NanoTank’s, to collect airborne particles through percolation in a liquid trap. Stepper motors, linear actuators, and controllers enable the movement of NanoTanks for automated collection of time-series samples at set intervals.

The first systems were deployed in October 2024, and the collected samples will be analysed by pyrolysis gas chromatography mass spectrometry (pyGC/MS) for nanoplastics, Raman spectroscopy for microplastics, and Liquid Chromatography/Tandem Mass Spectrometry (LC/MS/MS) for persistent organic pollutant analysis (PFAS focus).

This setup alleviates the need for porous filters that can clog given varied exposure levels. Our system will help to expand the capabilities of atmospheric research and allow us to increase our datasets and understanding of temporal and spatial distributions of NMP.

How to cite: Kelleher, L., Allen, S., Materic, D., Breedveld, G., and Krause, S.: POLARSENSE: Polar Online Airborne Nano and Microplastic Sensing and Environmental Monitoring, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17574, https://doi.org/10.5194/egusphere-egu25-17574, 2025.

EGU25-18591 | Orals | AS3.8 | Highlight

Atmospheric transport dynamics of microplastic fibres 

Joanna Bullard, Lucrecia Alvarez Barrantes, Cheryl McKenna Neuman, and Patrick O'Brien

Microplastics have been identified in most terrestrial areas of Earth including rural, remote and isolated locations where the only likely source is through atmospheric transport and deposition.  To date there has been limited attention paid to the fundamentals of microplastic transport by wind, and in particular, the similarities and differences between the motion of mineral grains and microplastic particles within boundary layer flows.  These fundamentals are key to future modelling of mineral-microplastic interaction in the atmosphere.  This research examines the dynamics of microplastic entrainment and transport by wind, focusing on fibres which are one of the most common shapes associated with aeolian systems.  A series of particle tracking velocimetry (PTV) experiments was conducted in a boundary layer wind tunnel to determine how nylon fibres (4 mm length) travel through the air and interact with the ground surface. The high-speed camera images show that the silhouette area presented to the wind has a high degree of temporal variability for fibres, as compared to sedimentary particles, affecting the fluid drag (e.g. form versus skin friction), translational versus rotational energy, and lift.  The motion of plastic particles in the flow follows a variety of different patterns, including end-over-end cartwheeling and horizontal transport with the long-axis oriented flow parallel. The progression of an airborne plastic particle through different motion types (a "lifecycle") appears to be orderly, despite a wide variability in the length of time spent in each particular motion type. Travelling across a mobile sand bed, microplastic fibres are observed to dislodge and cause the ejection of sand particles suggesting they can contribute to the development of the saltation cloud and may have the potential to reduce the threshold velocity for sand transport.

How to cite: Bullard, J., Alvarez Barrantes, L., McKenna Neuman, C., and O'Brien, P.: Atmospheric transport dynamics of microplastic fibres, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18591, https://doi.org/10.5194/egusphere-egu25-18591, 2025.

Microplastics (MPs) are ubiquitous, persistent pollutants that are harmful to human and reported in various environmental compartments like air, water, soil and biota. Owing to its hydrophobicity, MPs can adsorb chemicals like plasticizers, additives and flame retardants that can impart oxidative stress when inhaled. In this study, the MPs concentration in particulate matter (PM) was investigated for Tiruchirappalli, a rapidly growing city in Tamil Nadu. The study focuses on the PM bound MPs in outdoor and indoor environments through the collection of active PM10 samples and atmospheric depositions, respectively. The results showed that PM10 concentration at the monitoring sites were in the range of 28.17±6.4 μg/m3 to 43.67±6.3 μg/m3. The MPs in PM samples were extracted and viewed under Fluorescence microscope using Nile Red staining. The results indicated only a little difference in MP concentration among the monitoring sites (30.27±13.6 particles/m3 at residential area (L1) and 32.69±7.27 particles/m3 at industrial area (L2)). It was noteworthy that majority of MPs identified in PM10 samples were fragments and only a few fibres were noticed. This indicated the prevalence of MPs formed from degradation of plastic debris. The mean size of MPs was estimated to be 2.75 μm, showing the aerodynamic nature of the MPs in smaller sizes. MPs were found to be more prevalent in indoor atmospheric depositions (L1: 666 particles/m2/day; L2:727 particles/m2/day) than outdoor air. This study emphasizes the need for comprehensive understanding of the characteristics and sources of indoor and outdoor MPs so that appropriate mitigation strategies can be formulated.      

How to cite: Mohan V, L. and Raja, S.: Airborne microplastics distribution in indoor and outdoor environments of a rapidly growing city in South India , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19123, https://doi.org/10.5194/egusphere-egu25-19123, 2025.

EGU25-1201 | Orals | AS3.9 | Highlight

Near-future rocket launches could slow ozone recovery 

Laura Revell, Michele Bannister, Tyler Brown, Timofei Sukhodolov, Sandro Vattioni, John Dykema, Dave Frame, John Cater, Gabriel Chiodo, and Eugene Rozanov

Rocket emissions damage the stratospheric ozone layer, which protects life from harmful solar radiation. To understand if significant ozone losses could occur as the launch industry grows, we examine two scenarios of industry aspirations. Our ‘ambitious’ scenario (2,040 launches/year) leads to a -0.29% depletion in annual-mean, near-global total column ozone, relative to a simulation with no rocket launches. Antarctic springtime ozone decreases by 3.9%. Our ‘conservative’ scenario (884 launches/year) leads to a -0.17% annual depletion; current licensing rates suggest this scenario may be exceeded sooner than 2030. Ozone losses are mostly driven by the reactive chlorine produced from solid rocket motor propellant, and black carbon which is emitted from most propellants in contemporary use. The ozone layer is slowly healing from the effects of anthropogenic CFCs, yet ozone abundances are still 2% lower than those measured prior to the onset of CFC-induced ozone depletion. Our results demonstrate that ongoing and frequent rocket launches could delay ozone recovery. Action is needed now to ensure that future growth of the launch industry and ozone protection are mutually sustainable.

How to cite: Revell, L., Bannister, M., Brown, T., Sukhodolov, T., Vattioni, S., Dykema, J., Frame, D., Cater, J., Chiodo, G., and Rozanov, E.: Near-future rocket launches could slow ozone recovery, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1201, https://doi.org/10.5194/egusphere-egu25-1201, 2025.

EGU25-1262 | ECS | Posters on site | AS3.9

Middle Atmosphere Climatology using LIDAR for the evaluation of atmospheric conditions during man-made object reentry 

Nicolas Tufel, Philippe Keckhut, and Alain Hauchecorne

Atmospheric reentry impact on the atmosphere is an increasingly important topic today as the number of objects entering the atmosphere continues to rise (e.g. nanosats, cubesats, missiles, …) Modelling the way those artificial objects both enter the atmosphere and disaggregate requires precise knowledge of the medium conditions (e.g. temperature, density, …) However,current atmospheric models like MSIS 2.0 or ERA-5 reanalyses have been proven to lack accuracy at higher altitudes, limiting their use for this application. Therefore, this study aims at proposing an updated middle-atmospheric climatology using the NDACC and our Rayleigh LIDAR. We evaluate the bias between LIDAR observations and models (MSIS 2.0 and ERA 5), and explore the impact of mesospheric events on the temperature climatology. We also demonstrate how both the general daily variability and the input of some extreme events can influence the density and temperature at those altitudes. Climatologies were developed using 40 years of Lidar data, then compared to a climatology obtained with the calling of models. MSIS 2.0, while reliable in terms of seasonal trends, is less accurate daily: it shows high biases with the lidar at high altitudes (1.25% at 60 km, up to 6% at 80km). The European Climate and Weather Forecast model ERA-5 agrees with the lidar at 98.9% in the upper stratosphere but shows a larger statistical bias of 7 to 10% in the mesosphere. We removed extreme events  such as Sudden Stratospheric Warmings (SSWs), Mesospheric Inversion Layers (MILs) and Double Stratopause (DSs) to create a “Steady-State” Climatology at different lidar stations. Observing the densities corresponding to the temperature profiles, we could evaluate the annual mean density in the OHP and the impact of those different events on the mean density profile. Density disturbances caused by SSWs and MILs were quantified, revealing deviations of up to 12% and 25%, respectively, from MSIS density profiles, with impacts spanning 10–20 km in altitude. Our study provided important basis for the study of atmospheric reentry. Re-actualisation of temperature and density above lidar station and expected bias for the most commonly used middle-atmosphere model will help set the ground for future evaluation of heating, ablation and trajectory computation in this medium.

How to cite: Tufel, N., Keckhut, P., and Hauchecorne, A.: Middle Atmosphere Climatology using LIDAR for the evaluation of atmospheric conditions during man-made object reentry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1262, https://doi.org/10.5194/egusphere-egu25-1262, 2025.

EGU25-2816 | Posters on site | AS3.9

Space sustainability through atmosphere pollution? De-orbiting, atmosphere-blindness and planetary environmental injustice 

Urs Schaefer-Rolffs, Patrick Flamm, Daniel Lambach, Claudia Stolle, and Vitali Braun

Space debris is a major issue for space safety. In this context, there is a growing norm of disposal of orbital debris through atmospheric re-entry. The few existing studies, including our own modelling, agree that the projected exponential growth of satellites in Low-Earth Orbits (LEO) may come at the expense of damaging the integrity of the middle and upper atmosphere, with potentially unforeseeable consequences. We argue that sustainable LEO management requires overcoming what we call 'atmosphere-blindness': the limited understanding of the connections between space and the Earth system through orbital disposal practices and their impacts on the atmosphere. In our view, it is thus crucially important to undertake more interdisciplinary research on the issue of de-orbiting, as it is not merely a technical environmental problem, but also an inherently political matter of environmental justice on a planetary scale.

How to cite: Schaefer-Rolffs, U., Flamm, P., Lambach, D., Stolle, C., and Braun, V.: Space sustainability through atmosphere pollution? De-orbiting, atmosphere-blindness and planetary environmental injustice, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2816, https://doi.org/10.5194/egusphere-egu25-2816, 2025.

EGU25-3801 | Posters on site | AS3.9

Recent Observations of Rocket Exhaust Effects on the Ionosphere 

Michael Mendillo, Jeffrey Baumgardner, Joei Wroten, and Carlos Martinis

In 1973, the launch of Skylab created a ~50% depletion in the daytime ionosphere over the N. Atlantic Ocean that lasted for hours. This effect was discovered in the data being routinely gathered by radio receivers monitoring the Total Electron Content (TEC) using the Faraday rotation of a signal from the ATS-3 geostationary satellite. This “ionospheric hole” was created by the H2O and H2 in the rocket exhaust reacting with the ambient O+ in the F region. This reaction is ~2 orders of magnitude faster than the “normal” reaction between O+ and the ambient O2. Subsequent rocket launches were studied to confirm this process. Dedicated rocket launches were also used to create steep density gradients to study ionospheric instabilities near the magnetic equator. Today, rockets are being launched at an ever increasing rate (~2 launches/week), some of them causing ionospheric holes. The launches of Starlink group 6 from Florida de-orbit over the McDonald Observatory where Boston University has an All-sky Imager (ASI) dedicated to observing the optical emissions from the ionosphere. The de-orbit burns release H2O and CO2, both of which create an ionospheric hole with a concurrent burst of 630.0nm airglow. This airglow is bright enough (~ 10kR) to be seen with the unaided eye, and has been documented by citizen scientists. The resulting hole is also seen on GPS TEC maps of the region. Several examples of the de-orbit burns observed with the ASI at McDonald are shown.

How to cite: Mendillo, M., Baumgardner, J., Wroten, J., and Martinis, C.: Recent Observations of Rocket Exhaust Effects on the Ionosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3801, https://doi.org/10.5194/egusphere-egu25-3801, 2025.

EGU25-3866 | ECS | Posters on site | AS3.9

Modeling the atmospheric transport and possible radiative impact of alumina aerosols emitted from the projected increase in annual satellite reentry emissions. 

Christopher Maloney, Robert Portmann, Martin Ross, and Karen Rosenlof

The recent uptick in rocket launch rates, as well as the proposal of large low earth orbit satellite constellations (LLC’s) has renewed interest into how space traffic might impact Earth’s climate. One issue, the potential atmospheric response to a significant increase in aerosols released into the lower mesosphere/upper stratosphere during satellite reentry, remains under studied. It is predicted that if all proposed LLC’s are implemented, the total number of satellites in low earth orbit (LEO) will balloon from ~5,000 to over 60,000 individual satellites by as early as 2040. The corresponding annual emissions of metallic aerosol from satellite reentry is also expected to increase and approach 10 Gg/year. This reentry emission source would be on the same scale as the naturally occurring meteoric mass flux which is estimated to fall between 8 Gg and 20 Gg per year. Little is currently known about what type of exotic aerosols may be released during satellite ablation, but a significant portion of the aerosol population may be aluminum. Reentering LEO satellites are expected to completely vaporize in the mesosphere, and the subsequent vapor cloud will cool and coalesce into metallic aerosol roughly between 60km and 70km. As a result, aluminum aerosol could be rapidly transported into the stratosphere by atmospheric circulation and oxidize into aluminum oxide (Al2O3). Past studies have shown how Al2O3 released by solid rocket motors in the stratosphere can impact heterogeneous chemistry and thus ozone. Additionally, not much work looking at the radiative impact from Al2O3 aerosols in the stratosphere has been conducted. Here we present results from a study which focuses on the radiative impacts and atmospheric transport of hypothetical Al2O3 emissions from satellite reentry. The WACCM6 global model coupled with the CARMA sectional model was run with a 10 Gg/year mass flux of Al2O3 between 60 km and 70 km. We simulate multiple reentry patterns and aerosol size distributions. Our results show that reentry Al2O3 begins to accumulate in the polar region of both hemispheres on a time frame of months to two years, depending on the reentry location and aerosol size. Additionally, anomalous longwave cooling near the stratopause may lead to as large as 1.5 K temperature anomalies in the high latitude stratosphere and perturb the strength of the stratospheric polar vortex by as much as 10%. Due to modeling limitations, the work presented here does not consider important interactions between metallic reentry aerosol and stratospheric chemistry, but our results provide a first order approximation of the potential atmospheric response to an increased influx of satellite reentry aerosol.

How to cite: Maloney, C., Portmann, R., Ross, M., and Rosenlof, K.: Modeling the atmospheric transport and possible radiative impact of alumina aerosols emitted from the projected increase in annual satellite reentry emissions., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3866, https://doi.org/10.5194/egusphere-egu25-3866, 2025.

EGU25-4460 | ECS | Orals | AS3.9

Modelling impacts of ablated space debris on atmospheric aerosols  

Joanna Egan, Wuhu Feng, Daniel Marsh, and John Plane

Around 10% of Junge layer sulphuric acid droplets have been measured to contain metals from ablated space debris. Some metals – Al, Li, Cu, Ni, Mn etc. – already exceed natural background levels from cosmic dust that has ablated in the mesopause region. The effect of these metals on the stratosphere is not yet known, and space debris input has been projected to increase by more than an order of magnitude in the next 15 years. It is therefore vitally important to determine the level of re-entering space debris that will cause significant changes to atmospheric aerosols and stratospheric chemistry, in particular to the ozone layer.  Our calculations predict that the primary component of space debris particles (SDPs) will be aluminium hydroxide (Al(OH)3), which is expected to polymerise rapidly to form nano-particles and react with atmospheric HCl. The resulting complex is predicted to have a photolysis rate ~10 000 times faster than that of gas-phase HCl, and so Cl concentrations and therefore destruction of ozone by chlorine radicals are expected to increase. 

Here we present preliminary results of a modelling study using a sectional aerosol model within an Earth system model (Whole Atmosphere Community Climate Model with the Community Aerosol and Radiation Model for Atmospheres, WACCM-CARMA).  We simulate the transport of SDPs and meteoric smoke particles (MSPs) produced by condensation of Fe and Mg silicates from ablated cosmic dust. The particles grow by coagulation and deposition of sulphuric acid through 28 size bins (0.34 nm to 1.6 µm radius). The SDPs and MSPs are initially injected in concentrations consistent with current models and observations (7.9 t d-1 MSPs and 0.96 t d-1 SDPs) to assess the transport and lifetimes of the particles in the atmosphere. The effect of increasing the mass of SDPs in line with future increases in space travel is also simulated. The maximum possible impact of SDPs on stratospheric chemistry is then estimated from the available SDP surface area and assuming upper limits for unmeasured physico-chemical parameters. 

How to cite: Egan, J., Feng, W., Marsh, D., and Plane, J.: Modelling impacts of ablated space debris on atmospheric aerosols , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4460, https://doi.org/10.5194/egusphere-egu25-4460, 2025.

EGU25-4490 | ECS | Orals | AS3.9

Origins of stratospheric particles through an updated automated classification: revisiting the 1981-2020 period of the NASA Cosmic Dust Collections 

Quentin Taupin, Jérémie Lasue, Anni Määttänen, and Michael Zolensky

Every year, from 2000 to 8000 tons of natural extraterrestrial meteoroids are ablated in our atmosphere in the form of aerosols, estimated as a fraction of the total mass of incoming meteoroids. In 2019, the corresponding number for anthropogenic materials was estimated at about 263 tons, originating from launches and re-entries of rocket bodies, satellites, and space debris [1]. These injections of anthropogenic materials raise concerns about their effects on the Earth’s atmosphere such as ozone depletion, radiative forcing  and other unknow effects [2], [3], [4]. Furthermore, the anthropogenic injections are expected to increase significantly due to the rapid increase in launch rates and number of mega-constellations planned for the coming years. Indeed, there have been more satellites launched in the last 6 years than between 1957 and 2018 [5] and these numbers are set to grow, especially in the low Earth orbit region located below 2000 km [6].

However, large uncertainties remain about the evolution of the proportion and origins of these injected anthropogenic particles. This work attempts to reduce these uncertainties by further exploring the compositions of stratospheric particles collected in situ by the NASA Cosmic Dust program over 40 years.

Since 1981, the NASA Johnson Space Center (JSC) has been collecting dust particles from the lower stratosphere with airborne collectors during specific campaigns and published ~5500 preliminary analyses in the “Cosmic Dust Catalogs”. Each preliminary analysis is based on Scanning Electron Microscopy (SEM) images, some morphological characteristics and X-ray Energy-Dispersive Spectrometry (EDS) composition. The particles are then classified into four main groups: Cosmic, Terrestrial Contaminant Natural, Terrestrial Contaminant Artificial and Aluminum Oxide Sphere. Nevertheless, at least 20% of them remain ambiguously classified. The recent digitalization of all the published catalogs gives us the opportunity to explore their composition using multivariate analysis techniques such as Principal Component Analysis, and automatic clustering of the EDS spectra for classification. Nonlinear projected maps of the EDS composition can help visualize the classification of the particles [7]. The compositional clusters obtained can be used to identify the origin of each particle and constrain the atmospheric injection of each material. The temporal variations of the different compositions injected will be assessed and additional EDS data taken on meteorites and natural minerals will be included in the analysis to define natural material references.

In the future, this work will be complemented with new EDS spectra, SEM images and Raman spectroscopy of selected old samples and post-2020 collected samples curated at NASA JSC in Houston.

 

[1] Schulz and Glassmeier, Advances in Space Research, 2021. DOI: 10.1016/j.asr.2020.10.036

[2] Ferreira et al., Geophysical Research Letters, 2024. DOI: 10.1029/2024GL109280

[3] Jones et al., Journal of Geophysical Research, 1995. DOI: 10.1029/95JD01539

[4] Ross and Sheaffer, Earth’s Future, 2014. DOI: 10.1002/2013EF000160

[5] McDowell, « Jonathan’s Space Report », Accessed: Jan. 2025. https://planet4589.org/space/log/launch.html

[6] Gaston et al., Frontiers in Ecology and the Environment, 2023. DOI: 10.1002/fee.2624

[7] Lasue et al., Meteoritics & Planetary Science, 2010. DOI: 10.1111/j.1945-5100.2010.01059.x

How to cite: Taupin, Q., Lasue, J., Määttänen, A., and Zolensky, M.: Origins of stratospheric particles through an updated automated classification: revisiting the 1981-2020 period of the NASA Cosmic Dust Collections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4490, https://doi.org/10.5194/egusphere-egu25-4490, 2025.

The space industry is currently growing more rapidly than during any earlier time period since the beginning of the space age. Large low Earth orbit (LEO) satellite constellations and reusable liquid natural gas (LNG) fueled launch vehicles will change the scope and character of spaceflight. Satellite launches have increased four-fold in the past decade and are projected to grow even more quickly in coming decades. Given this explosive growth of the space industry, we need to understand combustion emissions from rockets and vaporization emissions from reentering space debris and how they will impact the global atmosphere. In particular, there may be changes to the stratospheric ozone chemistry as a result of space industry emissions into the middle atmosphere. At present, impacts are small, but evidence of metals that can only come from rocket stages and satellites have been detected in stratospheric aerosols, with an estimate that 10% of stratospheric aerosols contain species that can only originate from rocket stage/satellite ablation. Current rates of reentry particles are a few Gg/yr, but are projected to be over 10 Gg/year by 2030. Although modeled heating rates produced by reentry aluminum particles are small, they are statistically significant, and, as the number of objects in LEO are projected to increase, that impact will grow with time. Future work will attempt to estimate the impact of heterogeneous chemistry on reentry particles. Well quantifying impacts will require information on reentry scenarios, rocket plume chemistry and reentry vaporization debris characterization. Measurements, via laboratory experiments, remote sensing of launches and reentry, and in situ sampling are all needed to fully characterize space industry impacts on the atmosphere. This presentation will give an overview on what has been accomplished so far, and address what is needed to better characterize the impacts (and uncertainties) on the ozone layer from a growing space industry.

How to cite: Rosenlof, K.: Rocket Launches and Satellite Re-Entry: Potential Issues and the Need for Additional Modeling and Measurements , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4564, https://doi.org/10.5194/egusphere-egu25-4564, 2025.

EGU25-6158 | Posters on site | AS3.9

What do we know about the chemistry of spacecraft constituent metals in the Lower Mesospehere-Upper Stratosphere? 

Juan Carlos Gomez Martin, Antonio Jesus Ocaña, John Plane, and Juan Diego Carrillo-Sanchez

A large number of low earth orbit satellites are projected in the coming decades, which has led to concerns about environmental impacts of demised spacecraft. The current flux of anthropogenic aluminium vapours entering the Earth’s atmosphere is estimated to be already 10 times larger than the natural flux from meteoroids.
Metals ablated from meteoroids between 80 and 110 km react with atmospheric constituents in the mesosphere forming meteor smoke particles, which are transported by the global circulation to the stratosphere, where they entrain sulfuric acid aerosols and modify their properties. Metals ablated from demised spacecraft at ~60 km have a similar fate: Recent aircraft-based measurements show that 10% of stratospheric aerosols contain metals from re-entering satellites and rocket stages.
In this presentation I will give an overview of what we know about the gas-phase chemistry of spacecraft-relevant metals in the lower mesosphere-stratosphere. Based on this incomplete knowledge, I will speculate about the possible pathways of anthropogenic metals towards stratospheric aerosol and I will highlight uncertainties and experimental/theoretical work that needs to be carried out in order to address them. In particular, I will discuss preliminary results obtained with a modified version of the Meteor Ablation Simulator on the ablation of aluminium particles and the subsequent gas-phase chemistry of aluminium.

How to cite: Gomez Martin, J. C., Ocaña, A. J., Plane, J., and Carrillo-Sanchez, J. D.: What do we know about the chemistry of spacecraft constituent metals in the Lower Mesospehere-Upper Stratosphere?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6158, https://doi.org/10.5194/egusphere-egu25-6158, 2025.

EGU25-6252 | ECS | Orals | AS3.9

An update of space waste matter injection into the atmosphere 

Leonard Schulz, Karl-Heinz Glassmeier, Adam Mitchell, Daniel Murphy, John M. C. Plane, and Ferdinand Plaschke

In the last 5 years, the mass of human-made objects like satellites or rocket stages launched into orbit has strongly risen due to the implementation of satellite mega-constellations and generally increased space activity. Besides the well-known problems of on-orbit space debris and ground impacts, this means a strong increase of the human-made mass re-entering Earth’s atmosphere. Upon reentry, this space waste ablates in the atmosphere, injecting matter in form of aerosols and vapor. Murphy et al. (PNAS, 2023, Vol. 120, No. 43, e2313374120) detected remnants of such material in stratospheric aerosol particles. Thus, there is the concrete possibility of environmental effects due to space waste matter injection like ozone depletion or increased cloud nucleation (Mitchell et al., Understanding the Atmospheric Effects from Spacecraft Re-entry, Whitepaper, 2024). In order to understand what the exact effects on the atmosphere are, first, the amount and element-wise composition of the injected material has to be known. In this context, we present updated annual injection estimates compared to the first comprehensive estimation in Schulz and Glassmeier, 2021 (Advances in Space Research, 2021, 67 (3), 1002-1025) taking into account launch and re-entry databases, used spacecraft materials, as well as the observational data from the stratosphere. We present estimates of the overall injected mass as well as of specific elements. This data can serve as a baseline for modelling efforts and help steer towards the most promising future research.

How to cite: Schulz, L., Glassmeier, K.-H., Mitchell, A., Murphy, D., Plane, J. M. C., and Plaschke, F.: An update of space waste matter injection into the atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6252, https://doi.org/10.5194/egusphere-egu25-6252, 2025.

EGU25-7114 | Orals | AS3.9

Metals from spacecraft reentry in the stratosphere 

Daniel Murphy, Michael Lawler, Gregory Schill, and Leonard Schulz

Measurements of aerosol particles in the stratosphere show that metals that were vaporized during the reentry of rocket boosters and satellites accumulate in the stratosphere. These metals are incorporated into natural sulfuric acid particles in the stratosphere. With the rapidly increasing number of spacecraft reentry events, in the coming decades a majority of sulfuric acid particles in the stratosphere could contain novel metals from spacecraft in addition to the meteoric metals that are already present.

Over 20 elements from reentry were detected in stratospheric particles. We are able to quantify the relative amounts of a number of these metals, including lithium, aluminum, copper, and lead. For the EGU meeting we will also present results on several more metals such as titanium, niobium, molybdenum, silver, and tin. These atmospheric measurements can be compared to inventories of the elemental composition of spacecraft.

These metal-containing particles are found in the same air that contains the ozone layer. The addition of materials from spacecraft might affect heterogeneous chemistry in the ozone layer or change ice nucleation in polar stratospheric clouds.

How to cite: Murphy, D., Lawler, M., Schill, G., and Schulz, L.: Metals from spacecraft reentry in the stratosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7114, https://doi.org/10.5194/egusphere-egu25-7114, 2025.

EGU25-9526 | Orals | AS3.9

DLR Initiative S3D: Advancing Space Sustainability and Sustainable Development 

Jascha Wilken, Moritz Herberhold, Volker Maiwald, Matthias Nützel, Anja Schmidt, and Martin Sippel

The German Aerospace Center (DLR) has launched the S3D initiative, aimed at advancing the assessment and enhancement of sustainability in space activities. While recent years have seen growing attention to the environmental impacts of spacecraft and launch vehicles, S3D seeks to extend this perspective by integrating economic and social dimensions, transitioning from traditional Life Cycle Assessment (LCA) to a more comprehensive Life Cycle Sustainability Assessment (LCSA). A practice that is already established in other industries.

In addition to developing an LCSA process tailored for space activities, this initiative places particular emphasis on the impact of launch vehicle emissions in the upper atmosphere. This focus is driven by significant knowledge gaps and the potential for these emissions to be a major contributor to the climate impact of space transport activities. Substantial uncertainties remain with regard to the exact chemical composition of the exhaust, the post-combustion processes within the plume as well as the formation of particles such as black carbon. Moreover, there is a critical lack of data on the atmospheric effects of these gas and particle emissions at higher altitudes. To address these challenges, S3D will leverage the expertise of specialized DLR institutes in space systems, aerothermodynamics, propulsion, and atmospheric sciences to better characterize launch emissions and their atmospheric impacts.

This presentation will introduce the S3D initiative, outline the methodological approaches under development, and present initial findings on the exhaust profiles of various launch vehicle designs, along with progress toward creating a comprehensive exhaust inventory for 2024.

How to cite: Wilken, J., Herberhold, M., Maiwald, V., Nützel, M., Schmidt, A., and Sippel, M.: DLR Initiative S3D: Advancing Space Sustainability and Sustainable Development, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9526, https://doi.org/10.5194/egusphere-egu25-9526, 2025.

EGU25-13478 | ECS | Posters on site | AS3.9

Reducing the Environmental Impacts of Rocket Launch Emissions through Launch Parameter Variations 

Helena McDonald, Sebastian Eastham, and Raymond Speth

Increasing rocket launch rates in the last decade have prompted concerns over their environmental impacts. Launch vehicles are unique among anthropogenic pollution sources for directly emitting pollutants at all levels of the atmosphere. These high-altitude emissions have distinct – and poorly understood – consequences; emissions such as water vapor and black carbon aerosols have longer lifetimes in the stratosphere and thus a longer window for climate and ozone impacts. 

Accurately estimating launch emissions is an outstanding problem in launch vehicle research, complicated further by diverse combustion products which vary according to propellant type. We create unique emissions profiles for representative launches with equivalent payloads to LEO for three different propellants: RP1/LOx, CH4/LOx, and LH2/LOx. Using the GEOS-Chem High-Performance (GCHP) chemical transport model, we simulate an array of launch scenarios reflecting different choices of launch site, propellant, and launch season in a global three-dimensional atmosphere. 

We evaluate the impact of launch hemisphere by comparing launches at the same latitude in the Northern and Southern hemispheres, and show a greater ozone impact in southern-hemisphere launches. We simulate a range of launch sites across the northern hemisphere and show substantial variance in high-altitude ozone formation as a function of latitude. We show a several percent larger increase in stratospheric ozone for summer launches than in winter. Finally, we see net ozone column increase with RP1 and CH4 fuelled launches but net decrease with LH2, which we posit suggests black carbon is the dominant force in high-altitude ozone formation as a response to rocket launches. 

Using these results, we synthesize a variety of impact mitigation strategies for a given rocket launch and estimate the potential harm reduction across a variety of metrics: global ozone column changes, radiative forcing, surface air quality, and population exposure to fine particulate matter. These findings could be used to inform future developments in the launch industry, from selecting and researching fuel types for future launch vehicles, to choosing locations for future launch sites, and even optimal utilization rates for existing launch sites. 

How to cite: McDonald, H., Eastham, S., and Speth, R.: Reducing the Environmental Impacts of Rocket Launch Emissions through Launch Parameter Variations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13478, https://doi.org/10.5194/egusphere-egu25-13478, 2025.

EGU25-14035 | Orals | AS3.9

In situ observations of a kerosene-fueled rocket plume sampled during SABRE 2023 

Troy Thornberry, Joshua Schwarz, Karen Rosenlof, Martin Ross, Ming Lyu, Eleanor Waxman, Colin Gurganus, Glenn Diskin, Gordon Novak, Adam Ahern, Charles Brock, Paul Bui, Georgia Michailoudi, Rajesh Poudyal, Mike Robinson, and Drew Rollins

Rocket launches and space debris from reentries are the only direct anthropogenic emission sources above ~20 km in the atmosphere. Space launch activities, and consequently these emissions, are expected to grow by an order of magnitude in just the next decade. Modeling the impact of rocket emissions on the stratosphere requires accurate specification of exhaust composition profiles that depend on rocket propellant types (fuels) and operational and design parameters. Global models predict that black carbon (BC) is the most significant radiative forcing component in both kerosene (RP-1) and liquefied natural gas (LNG, methane) fueled rocket exhaust, although these emissions have never been measured from a rocket in flight. Validation of rocket combustion models, in turn, requires comprehensive in situ composition data from rocket plumes at stratospheric altitudes where near-field hot plume chemistry is expected to weaken.

In February 2023, the NOAA SABRE mission, using a NASA WB-57F aircraft, obtained in situ plume composition data (H2O, SO2, NO, NO2, NOy, HONO, CO, CO2, BC, particle concentration) just above the tropopause from a kerosene-fueled rocket launched from Cape Canaveral, FL. The nighttime plume (not visible to the aircrew) was intercepted twice using a predetermined search pattern flown by the WB-57F. Measured ratios of emissions constituents reveal potentially surprising clues about near-field exhaust chemistry and kerosene engine BC emission in the lowermost stratosphere. The plume data acquired here, while limited, demonstrate the utility of such measurements toward resolving key questions about rocket emissions, and the SABRE 2023 flight experience suggests ways to improve plume sampling (e.g., need for plume direction finding capability) for future stratospheric rocket emission studies.

How to cite: Thornberry, T., Schwarz, J., Rosenlof, K., Ross, M., Lyu, M., Waxman, E., Gurganus, C., Diskin, G., Novak, G., Ahern, A., Brock, C., Bui, P., Michailoudi, G., Poudyal, R., Robinson, M., and Rollins, D.: In situ observations of a kerosene-fueled rocket plume sampled during SABRE 2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14035, https://doi.org/10.5194/egusphere-egu25-14035, 2025.

EGU25-15071 | ECS | Orals | AS3.9

Development and assessment of space launch and re-entry emission inventories for atmospheric modelling 

Jan-Steffen Fischer, Stefanos Fasoulas, Matthias Nützel, and Anja Schmidt

The space sector has experienced significant growth in recent years, with rocket launch rates increasing by over 20% since 2019. In its 2022 Scientific Assessment of Ozone Depletion the World Meteorological Organization cautions that future increases in launch rates, the adoption of new propellants like hydrogen and methane, and emissions from reentering objects could significantly influence future ozone levels . Therefore, the creation and evaluation of emission inventories of space activities, which can be used in atmospheric chemistry modelling, is of particular importance. Here we present two open-source tools developed at the University of Stuttgart. 1) Launch Emission Assessment Tool (LEAT), and 2) Re-entry Emission Assessment Tool (REAT), and discuss the underlying models and assumptions. Furthermore, we compare results obtained with LEAT to previously published emission inventories.

LEAT enables the calculation of a launch trajectory based on basic launcher data and calculates emissions such as CO, H2O and NO either using emission indices or by calculating the engine and afterburning emissions. The model accounts for the different flight states and environmental conditions based on a chemical equilibrium model. This makes it possible to distinguish between emissions stemming from different fuel systems and those from different flight paths.

REAT enables the calculation of emissions from re-entering objects. The interaction with the atmosphere is simulated using emission indices or a chemical equilibrium model depending on atmospheric conditions.

Both tools enable us to create detailed high-resolution 3-D emission inventories, which can readily be used in chemistry-climate models in order to assess the atmospheric and climatic effects of launcher and re-entry emissions. Furthermore, by using existing emission inventories a comparison can be made with literature. We also assess and discuss underlying model assumptions and parameter and model uncertainties as well as measures required to reduce uncertainties related to the emission inventories.

How to cite: Fischer, J.-S., Fasoulas, S., Nützel, M., and Schmidt, A.: Development and assessment of space launch and re-entry emission inventories for atmospheric modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15071, https://doi.org/10.5194/egusphere-egu25-15071, 2025.

EGU25-17301 | ECS | Posters on site | AS3.9

Defining the environmental impacts of satellite megaconstellation missions in a rapidly growing space sector 

Connor Barker, Eloise Marais, and Sebastian Eastham

Emissions from the space industry are rapidly increasing due to surges in rocket launches and the amount of mass re-entering the Earth’s atmosphere. Satellite megaconstellations (SMCs) are a key contributor to this growth, representing a fifth of rocket launches and a quarter of object re-entries in 2020-2022. These activities release air pollutant emissions throughout the atmosphere, including in upper atmospheric layers where turnover rates are very slow. This results in extremely effective stratospheric ozone depletion and radiative forcing. Of the approximately 7500 satellites in low-Earth orbit (LEO), 75% belong to satellite megaconstellations, with 60,000 additional SMC satellites expected to be launched in the next decade. Despite this anticipated growth, the environmental impacts of SMC emissions lack characterization and are under regulated. Here we implement a recently published 3-D, global inventory of space industry emissions into a computational model to determine the impacts on stratospheric composition and radiative forcing from a decade of SMC missions. The inventory comprises emissions up to 80 km from all SMC and non-SMC rocket launches and spacecraft re-entries during the onset of the megaconstellation era (2020-2022). The emission species include gaseous nitrogen oxides (NOx≡NO), water vapour (H2O), carbon monoxide (CO), and chlorine species (Cly≡HCl+Cl2+Cl), and particulate black carbon (BC) and alumina (Al2O3). We project the emissions to 2029 based on linear growth in SMC and non-SMC launch propellant consumption and re-entry mass. We use the GEOS-Chem 3-D model of atmospheric composition coupled to a radiative transfer model to simulate the response of atmospheric composition and radiative forcing to these emissions. We include a standard GEOS-Chem simulation of externally mixed aerosols and an updated simulation where BC and Al2O3 undergo prompt uptake to abundant stratospheric sulfate aerosols (SSA), as evidenced by observations from a recent aircraft campaign. We find a global stratospheric ozone loss of 0.03% (0.072 DU) from launch and re-entry emissions at the end of the decade. This is much smaller than stratospheric ozone loss attributable to surface sources (~2% in 2022). Depletion due mostly to Cly from solid rocket motors is concentrated in the northern midlatitude upper stratosphere. SMC missions are responsible for 13% of this ozone depletion, as solid fuel represents <1% of rocket fuel used by SMC missions from 2020-2022. Uptake of aerosol emissions to SSA results in nearly complete removal of wintertime stratospheric BC and Al2O3 concentrations and a summertime peak. This process greatly reduces the positive radiative forcing by stratospheric BC, resulting in stratospheric ozone depletion as the dominant forcing process and an overall negative forcing. Space industry emissions from all mission types result in radiative forcing of -3.38 mW m-2 at the top of the atmosphere in summer 2029, with -0.59 mW m-2 from SMC missions.  At the tropopause, there is a net negative radiative flux from all missions (-1.64 mW m-2) and SMC missions (-0.35 mW m-2). Current work includes conducting sensitivity simulations to quantify the impact of uncertainties in properties and chemical pathways of aerosol emissions on our results to inform future field and experimental studies.

How to cite: Barker, C., Marais, E., and Eastham, S.: Defining the environmental impacts of satellite megaconstellation missions in a rapidly growing space sector, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17301, https://doi.org/10.5194/egusphere-egu25-17301, 2025.

EGU25-18151 | ECS | Orals | AS3.9

Designing a mission concept for atmospheric plume measurements during a rocket launch event 

Andreas Marsing, Christiane Voigt, Anke Roiger, Matthias Nützel, Hiroshi Yamashita, Anja Schmidt, Tiziana Bräuer, Justin Hardi, Leon Lober, Sebastian Karl, Margaux Duperray, and Valère Girardin

The frequency of space launches has increased dramatically as costs plummet and demand rises with the advent of use cases (such as mega constellations or larger-scale exploration). This increase in launch cadence is enabled by reusable launchers, whose technology is progressing in Europe. They provide enhanced material efficiency while adding complexity to flight paths, burn patterns and more. There is, however, a notable gap in observational evidence regarding emissions and their subsequent atmospheric effects, especially for liquid or hybrid solid/liquid propellants.

We present ongoing work within the ESA project FIREWALL (Facilitate Inquiry of Rocket Emission impact With Atmosphere Lower Layers) that aims to design a mission concept for measuring emission and plume properties during the takeoff and return of current or near-future launch vehicles. It leverages expertise in the fields of ground observations at the launch site, airborne in-situ measurements with different available platforms like aircraft, balloons or sounding rockets, satellite remote sensing of contrails or trace gases, as well as plume and global atmospheric modelling. Thereby the major atmospheric burn events of a modern launcher shall be captured in unprecedented extent and detail to better quantify their atmospheric effects.

This innovative atmospheric science mission brings together experts from the fields of atmospheric measurements with space launch system operators and airspace authorities. Additionally, input will be provided by experts in plume thermodynamics and chemistry modelling, trajectory and dispersion modelling as well as weather forecasting. The gathered mission concept devises a recipe to operate a comprehensive suite of measurement platforms and instruments at a scheduled rocket launch event, including a list of objectives and requirements as well as a comprehensive risk assessment.

How to cite: Marsing, A., Voigt, C., Roiger, A., Nützel, M., Yamashita, H., Schmidt, A., Bräuer, T., Hardi, J., Lober, L., Karl, S., Duperray, M., and Girardin, V.: Designing a mission concept for atmospheric plume measurements during a rocket launch event, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18151, https://doi.org/10.5194/egusphere-egu25-18151, 2025.

EGU25-20347 | Posters on site | AS3.9

Atmospheric and climate effects of NOx emissions from Aviation and Rocket launches 

Wuhu Feng, Yuwen Li, Martyn Chipperfield, John Plane, Daniel Marsh, Joanna Egan, Shuijie Chang, Alexandru Rap, Weiyu Zhang, Alexander Archibald, Tyler Brown, Laura Revell, Alfonso Saiz López, Jean-Paul Booth, and Douglas Kinnison

There have been long concerns on the potential environmental impact of aviation, which is the second biggest source of transport greenhouse gas emissions after road transport. Direct emissions from aviation accounted 3.8% of total CO2 emissions, which is estimated to contribute ~3.5% to the anthropogenic effective radiative forcing of climate (IPCC). The environmental impact of emissions from space launches is currently receiving much attention due to the space industry being one of the fastest growing global economic sectors. Since the first assessment of the impact of rocket emissions by Cicerone and Stedman (1974), there have been many developments in rockets and modelling. Rocket emissions can inject significant quantities of gases and particles into the atmosphere (including chlorine compounds HCl, H2O, CO2, NOx, H2, Al2O3 and black carbon), potentially affecting ozone depletion, the dynamics of the atmosphere, and climate change. Feng et al. (2023) have investigated stratospheric ozone depletion due to the presence of small satellites (e.g., CubeSats) with an iodine propulsion system to keep them in orbit. They have shown that an increase in the number of small satellite launches could cause substantial ozone depletion in the Antarctic.

In this work, we have incorporated the up-to-date aviation emission inventories (Teoh et al., 2024) and rocket emissions (Brown et al., 2023) into a state-of-the-art global chemistry-climate model (NCAR’s Community Earth System Model, CESM2) to explore how aviation and rocket emissions affect the stratospheric ozone layer and climate once the gases and particulates are injected into the atmosphere. The model includes dynamics, transport, aerosol microphysics, photochemistry, radiation, emissions, and their influences on stratospheric ozone depletion. We have carried out many model experiments in CEMS2 using different configurations (free running, specific-dynamic versions of Whole Atmosphere Community Climate Model) with different chemistry and NOx emissions scenarios from aircraft and rocket emissions (from zero NOx emissions, released NOx emission inventories and up to 100 times NOx emissions) to assess the atmospheric changes induced by these emissions under historical and future scenarios.

How to cite: Feng, W., Li, Y., Chipperfield, M., Plane, J., Marsh, D., Egan, J., Chang, S., Rap, A., Zhang, W., Archibald, A., Brown, T., Revell, L., Saiz López, A., Booth, J.-P., and Kinnison, D.: Atmospheric and climate effects of NOx emissions from Aviation and Rocket launches, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20347, https://doi.org/10.5194/egusphere-egu25-20347, 2025.

EGU25-21651 | Orals | AS3.9

 The European Space Agency’s approach towards environmental impact assessment in the atmosphere: Lessons learned, knowledge gaps and roadmap 

Lorenz Affentranger, Adam Mitchell, Enrico Tormena, Valere Girardin, Sara Morales Serrano, and Jeroen Van den Eynde

The European Space Agency (ESA) through the Clean Space Office has approached the assessment of the environmental performance of its activities by applying Life Cycle Assessment (LCA) since the early 2010’s. ESA through its Green Agenda (EGA) has put sustainability as one of its key pillars aiming at reducing the environmental impacts of ESA projects. The assessments of the three traditional space, launch and ground segments have been instrumental in the creation of the ESA LCA Handbook and Database which are being applied systematically to its missions. Nevertheless, significant knowledge gaps remain, particularly in understanding the intricate interactions between launcher exhaust emissions and spacecraft demise with the upper layers of the atmosphere—critical steps in the life cycle assessment process. This work will present the growing necessity to better understand the potential environmental impacts at all altitudes, the current challenges of including atmospheric impacts into LCA thinking and ESA’s consolidated efforts to address key knowledge gaps. In addition to addressing areas of uncertainty, this paper will detail ongoing activities and outline how ESA plans to enhance awareness and implement measures to mitigate the environmental impacts of space activities.

How to cite: Affentranger, L., Mitchell, A., Tormena, E., Girardin, V., Morales Serrano, S., and Van den Eynde, J.:  The European Space Agency’s approach towards environmental impact assessment in the atmosphere: Lessons learned, knowledge gaps and roadmap, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21651, https://doi.org/10.5194/egusphere-egu25-21651, 2025.

EGU25-974 | ECS | Posters on site | AS3.10

Label-free Ambient Pollen Identification and Classification Using Total Internal Reflection Microscopy and Deep Learning 

Sachin Dhawan, Anuj Saxena, Anand Kumar, Mukesh Khare, and Dalip Singh Mehta

Ambient pollen identification and classification using traditional label-dependent methodologies is often time-consuming and prone to errors. Conventional methods such as bright field (BF) microscopy and including labeled techniques provide low-contrast and low signal-to-noise ratio images of pollens.  These techniques are also associated with high noise due to the complex nature of ambient samples.  Numerous other label-free techniques such as phase contrast, and quantitative phase imaging have been applied for ambient pollen imaging; however, these imaging methods provide better contrast images but the identification of pollens in ambient samples is very difficult due to the heterogeneous nature of ambient particles as it contains particulate matter, fungal spores, mold spores, and other ambient particles. To address these limitations, the current work employs a label-free novel application of total internal reflection (TIR) phenomenon. When the light beam undergoes TIR at an optical interface, an evanescent field is generated over the interface where the samples are prepared. The generated evanescent field illuminates the sample upto a certain depth (~500nm) only, which helps to avoid the background noise and gives high-contrast images with high SNR. TIR imaging enhances the optical properties of ambient pollen by emphasising surface and near-surface features, providing remarkable contrast in ambient pollen images. The study used TIR imaging, enabling non-invasive, no-sample preparation and precise identification of pollen in ambient samples, even with high background concentration of ambient particles.  It also allows better visualization of pollen boundary and additional surface features such as the polarity and aperture patterns. Additionally, the CNN-based deep-learning model is used for pollen detection, significantly advancing ambient pollen analysis. The model demonstrates strong performance, with a high F1 score for detecting pollen (0.83) and a well-balanced overall performance (F1 score of 0.77 for all classes). The confusion matrix shows excellent classification accuracy, especially for the pollen class. The model’s mean average performance is 76.7% across all classes at a threshold of 0.5, indicating good performance. Preliminary results demonstrate the model's robust performance, even when handling complex ambient samples with high ambient concentrations of other ambient particles. Pollen monitoring is crucial due to the scarcity of comprehensive data on airborne pollen, which impacts public health. The application of TIR microscopy combined with automated analysis offers a label-free, real-time, and field-deployable solution for addressing challenges in airborne particle monitoring. These results highlight the novel potential of TIR microscopy with deep learning as a method for precise, effective, and scalable pollen monitoring.

How to cite: Dhawan, S., Saxena, A., Kumar, A., Khare, M., and Mehta, D. S.: Label-free Ambient Pollen Identification and Classification Using Total Internal Reflection Microscopy and Deep Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-974, https://doi.org/10.5194/egusphere-egu25-974, 2025.

EGU25-2508 | Posters on site | AS3.10

Scaling Down Modelled Airborne Birch and Grass Pollen Levels 

Willem W. Verstraeten, Nicolas Bruffaerts, Rostislav Kouznetsov, Mikhail Sofiev, and Andy Delcloo

Allergenic airborne pollen in Europe affect the health of a quarter of the adult population and a third of all children badly. Due to climate change even more people might suffer from pollen allergies in the future. If timely information on forthcoming pollen episodes is available, however, mitigation measures can be taken for easing off the allergy symptoms. This requires forecasting systems at the scale of the citizens that may alert people who are vulnerable for these pollen. In order to achieve this, we aim at providing modelled and forecasted airborne birch and grass pollen levels near the surface at the one by one kilometer scale.

The pollen transport model SILAM (System for Integrated modeLling of Atmospheric coMposition) is used as backbone for modelling and forecasting airborne birch and grass pollen in Belgium. SILAM is driven by ECMWF ERA5 meteorology in a bottom-up emission approach. The dynamic vegetation component in the pollen transport model is determined by pollen emission source maps which have to be ingested every pollen season in the model. To date, these maps have 0.10° x 0.10° and 0.05° x 0.05° gridcells for birch trees and grasses, respectively. Here, we combine monthly MODIS Land Surface Temperature (LST) data on a one by one kilometer grid with vegetation maps from earlier research on top of a pollen footprint analysis. We apply daily pollen footprints produced by SILAM running in a 3-day backward mode for five locations in Belgium, coupling the fraction of air to the pollen levels monitored by the devices of the aerobiological network. The down-scaled pollen emission source maps are then applied into SILAM in the forward mode to obtain modelled birch and grass pollen concentrations near the surface for Belgium more tailored towards the scale of citizens.

Preliminary analysis indicates that late winter/early spring MODIS LST is a good proxy of the severity of the grass pollen season. The added value of LST for the birch pollen season is small. By ingesting the new maps with down-scaled pollen emissions sources into SILAM and by comparing modelled and measured time series for the 2013-2018 pollen seasons a substantial improvement (up to 210% increase in R² values for grass pollen) is found for the monitoring stations, especially at the North Sea side. This can be mainly attributed to a better separation between sea and land characteristics in the 0.01 x 0.01° grid of the pollen emission source maps compared to the coarser native gridcells.

How to cite: Verstraeten, W. W., Bruffaerts, N., Kouznetsov, R., Sofiev, M., and Delcloo, A.: Scaling Down Modelled Airborne Birch and Grass Pollen Levels, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2508, https://doi.org/10.5194/egusphere-egu25-2508, 2025.

EGU25-3092 | Orals | AS3.10

Hydrometeorological drivers of Cupressaceae pollen rupture in southeastern Spain 

José María Moreno, Francisco Aznar, Luis Negral, and Stella Moreno

The rupture of Cupressaceae pollen grains significantly affects allergenic exposure and depends on specific hydrometeorological factors. This study analysed the main meteorological variables influencing pollen rupture in three cities in southeastern Spain during two pollen seasons (2019-2020 and 2020-2021). Using data from the Aerobiological Network of the Region of Murcia and standardised sampling methods (EN 16868), the study quantified total pollen concentrations, disrupted pollen (DP) levels and percentage of disrupted pollen (DPP).

The results reveal that the main factors influencing pollen rupture are related to water, specifically relative humidity and precipitation. Higher relative humidity levels were positively correlated with increased DP and DPP, indicating that relative humidity triggers structural changes in pollen grains. Precipitation showed a dual effect, simultaneously promoting pollen swelling and disruption while reducing airborne concentrations due to its wash-out effect. The influence of relative humidity aligns with the reproductive mechanisms of Cupressaceae, which rely on hydration for pollen tube formation. The percentage of disrupted pollen was significantly higher during periods of high relative humidity, with always positive correlations.

Statistical analyses confirmed that geographical characteristics and bioclimatic indices had a limited influence compared to localised factors such as urban ornamental flora and specific hydrometeorological conditions. Differences between the cities studied were also explored using hierarchical clustering dendrograms. These visualisations highlighted different clustering patterns based on pollen concentration and meteorological variables, highlighting the importance of localised urban vegetation management in influencing allergenic risks.

The results showed the dual role of precipitation in influencing airborne allergen exposure. This duality highlights the importance of considering both weather conditions and urban planning strategies to mitigate health risks. Management of ornamental Cupressaceae in urban areas, combined with monitoring of high relative humidity periods, could significantly reduce allergen exposure.

The integration of aerobiological and meteorological data networks provides a robust framework for allergen risk forecasting. Such systems can provide real-time alerts to vulnerable populations, especially during high pollen seasons. A better understanding of factors such as relative humidity and rainfall will improve public health responses and inform sustainable urban development policies.

How to cite: Moreno, J. M., Aznar, F., Negral, L., and Moreno, S.: Hydrometeorological drivers of Cupressaceae pollen rupture in southeastern Spain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3092, https://doi.org/10.5194/egusphere-egu25-3092, 2025.

Allergic rhinitis affects half a billion people globally, including a fifth of the Australian population. In Canberra, the nation’s capital, more than 1 in 3 people suffer from the disease and this can cause significant negative impacts on community wellbeing as well as the local economy. Thunderstorm Asthma events have also been recorded and have led to increasing public and government concern with regard to improving our responses to thunderstorm asthma and other environmental drivers of respiratory morbidity and mortality. Over the last decade the Canberra Pollen Monitoring Program has been monitoring airborne allergenic pollen and fungal spores in Canberra on a daily basis. These records of airborne pollen are beginning to provide a historical lens to create pollen taxa calendars, estimate the pollen season length and variability, and to provide the basis for forecast evaluation.

In this presentation we provide the latest information on the seasonal nature of the most significant airborne tree pollen, herb pollen and spore types for Canberra, Australia. The development of a citizen science approach designed to provide the public with daily airborne allergenic pollen information while allowing users to give feedback on their hay fever symptoms, is also providing insights into the impact of airborne pollen on people in the region. We also consider why Canberra is a hotspot for allergic rhinitis in Australia and discuss how pollen and spore exposure is likely to be altered by future climate change and rapid urban development.

How to cite: Haberle, S. and Keaney, B.: A decade of airborne pollen monitoring in an allergic rhinitis hotspot of Australia: insights into how climate change and urban development are altering pollen seasons and human wellbeing., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3390, https://doi.org/10.5194/egusphere-egu25-3390, 2025.

Approximately 20-30% of the European population suffers from pollen allergies, imposing an economic burden of 50 to 150 billion euros annually. Traditional pollen monitoring methods, which rely on manual counting, face significant limitations, including a delay of 3 to 9 days between data collection and the availability of results. This lag hampers timely allergy management and forecasting.

Recent advancements in technology, particularly the use of artificial intelligence and automated systems, have revolutionized the field, enabling real-time detection of pollen and other large bioaerosols. These innovations offer a significant leap forward in the accuracy, speed, and efficiency of pollen monitoring.

Since its inception in 2018, the EUMETNET AutoPollen Programme has united a diverse group of experts and stakeholders to address all aspects of the information chain, from instrument certification and calibration all the way to estimating impacts and disseminating products to end-users. A notable achievement of the programme includes an international study that compared various combinations of monitoring devices and particle identification algorithms. This study successfully identified several viable solutions for operational, real-time bioaerosol observations, paving the way for practical implementation across Europe.

The ongoing collective effort aims to establish a robust European network for real-time pollen and fungal spores monitoring. This network will significantly enhance allergy management by providing timely and accurate data, improve forecasting capabilities, and support further scientific research. Ultimately, it will expand access to reliable, real-time information, benefiting end users and contributing to a healthier and better-informed society.

How to cite: Meurville, M. P.: EUMETNET AutoPollen: establishing a European network for automatic bioaerosol detection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3533, https://doi.org/10.5194/egusphere-egu25-3533, 2025.

EGU25-4712 | ECS | Orals | AS3.10

Intercomparison studies and potential of pre-load algorithms for training and validating automated sampling systems in aerobiology 

Qasim Farooq, Rocío López-Orozco, Moises Martínez-Bracero, Carmen Galán, and José Oteros

Background: Monitoring airborne pollen measurements depends on accurate and reproducible pollen recognition and analysis. The traditional volumetric Hirst method for pollen monitoring is based on European standards. This method demands skilled technicians, and it is a time-consuming process. Furthermore, this method has a 5–10 days delay in the data reported. To overcome these problems, a transition from manual to modern automatic methodologies is needed.  A Hirst-type trap has been used as a baseline and maintains historical time sequences of measured data to validate automatic samplers.

Methods: We compared both three-hourly and daily data of selected pollen types: Cupressus, Fraxinus, Pinaceae, Platanus, Poaceae, and Quercus, detected with a Hirst-type trap with a parallel retrieved concentration from three different automatic samplers: Pollen Sense APS-330, Hund BAA-500, and Swisens Poleno Jupiter. The pollen measurement campaign was conducted from 01 January 2024 to 03 June 2024 in Córdoba under the Mediterranean climate. The automatic samplers are based on different sampling and analysis methods, such as imaging-based identification, fluorescence spectroscopy and/or holographic imaging. We calculated Pearson's linear correlation coefficients (r) and daily ratio among Hirst and automatic measurements. 

Results: These results indicates the statistical significant differences between Hirst and automatic samplers (p ≤ 0.001) with strong correlation coefficient (r) for APS-330 data with r > 0.74 (3h) and r > 0.89 (daily) for Quercus, r > 0.77 (3h) and r >0.83 (daily) for Cupressus, and r > 0.65 (3h) and r > 0.70 (daily) for Poaceae ; the Hund BAA-500 data shows r > 0.63 (3h) and r > 0.84 (daily) for Cupressus, r > 0.55 (3h) and r > 0.56 (daily) for Poaceae at statistically highly significant (p ≤ 0.001), and for Platanus at moderately significant (p ≤ 0.01) with r > 0.50 (daily) and non-significant (p > 0.05) with r > 0.13 (3h). As with Swisens Poleno Jupiter, the weak correlation results with  r > 0.61 (3h) and r > 0.85 (daily) (p ≤  0.001) for Platanus, r > 0.38 (3h) and r > 0.67 (daily)  (p ≤ 0.001) for Poaceae, and r > 0.17 (3h) (p ≤ 0.001) and r > 0.36 (daily) (p ≤ 0.01) for Quercus. The average daily ratio for APS-330 was 2.31, for Hund BAA-500 was 2.77, and for Swisens Poleno Jupiter was 3.18.

Conclusion: This research study gives first insights into the Mediterranean environment. The results are from the pre-loaded algorithms and the companies did not include southern categories (e.g. Olea, Morus), which could lead to false positivity for already trained categories. We observed comparable concentrations provided by Hirst and both APS-330 and Hund BAA-500. The concentrations are not similar due to different measuring techniques of automatic samplers, we always noted a similar distribution curve, taking into account the use of scaling factors for the application of a homogenization index. However, further intercomparison studies, in particular, after the training of local categories and refinement of the algorithms based on digital reference datasets (DRD), the automatic samplers would show potential.

Keywords: Automated biomonitoring; Validation; Intercomparison studies; Airborne pollen

How to cite: Farooq, Q., López-Orozco, R., Martínez-Bracero, M., Galán, C., and Oteros, J.: Intercomparison studies and potential of pre-load algorithms for training and validating automated sampling systems in aerobiology, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4712, https://doi.org/10.5194/egusphere-egu25-4712, 2025.

EGU25-11529 | Orals | AS3.10

Method for calibration of bioaerosol monitors based on reference pollen aerosols and imaging-based Lagrangian particle tracking as reference: the case of the Swisens Poleno 

Stefan Horender, Christina Giannakoudaki, Reto Abt, Kevin Auderset, Benoît Crouzy, Sophie Erb, Oguzhan Erdogdu, Elias Graf, Kenjiro Iida, Erny Niederberger, Langying Ou, Hiromu Sakurai, Julia Schmale, Christian Wälchli, and Konstantina Vasilatou

Several automated pollen monitors have recently become available, most using conventional and/or machine-learning algorithms to detect pollen and classify their taxa. An international intercomparison campaign was organised by the EUMETNET AutoPollen Programme and the ADOPT COST Action in Munich (March–July 2021) (Maya-Manzano et al. 2023). The study showed that some automatic systems, especially those that have built-in correction factors to compensate for losses of sampling, detection and classification, agreed with the averaged pollen concentration of four manual Hirst-type measurements. The manual pollen counting method, relying on human operators, is still used today due to a lack of traceable metrological standards for pollen monitoring. Additionally, existing reference particle counters have been validated up to particle sizes around 20 µm only (Vasilatou et al. 2022). In this study, we evaluated the shake-the-box particle tracking/detection algorithm (Novara et al. 2023) to serve as a reference measurement of particle number concentration. A volume is illuminated with an expanded light sheet produced by a double-pulse laser, and four calibrated double-frame cameras record images of the particles inside this volume. The algorithm determines the position and velocity of each particle, allowing the measurement of particle number concentration directly in the air without sampling inlets that could influence the measurement.

Particle tracking was validated against the Inkjet Aerosol Generator at the Japanese National Metrology Institute NMIJ and the reference optical particle counter at METAS using an 11-D spectrometer (Grimm GmbH, Germany) as a transfer standard and size-certified polystyrene particles. Expanded uncertainties (coverage factor k=2) were 24 %, 10 %, and 7 % for particle sizes 15 μm, 20 μm, and 26 μm, respectively. The good agreement among the three methods shows that the shake-the-box particle tracking method can be applied as a reference for particle number concentration.

We used a laboratory-based method for characterising the performance of bioaerosol monitors as a whole unit (hardware plus identification algorithms) using the particle tracking method and, in a separate experiment, freshly sampled pollen. Experiments were carried out with the SwisensPoleno Jupiter, which combines light scattering, inline digital holography and ultraviolet laser-induced fluorescence with machine learning to classify different particles. For a pollen grain to be measured, it must be sampled, detected and correctly classified.  Each stage is subject to particle losses, leading to a measurement efficiency below 100 %. Particle tracking measurements of pollen (Pinus, Zea Mays) resulted in an average counting efficiency of about 43 %, neglecting particle losses in the Sigma-2 sampling head and issues with the classification of particles. The unit-to-unit variability of the Poleno instruments was 30 % based on measurement with three units. Independent experiments with Alnus glutinosa, Betula pendula and Corylus avellana showed that the major source of losses, however, originates from the pollen classification algorithm, which is trimmed to best correlate with Hirst measurements (currently the defacto reference for pollen monitoring). This highlights the need for an independent, standardised method for evaluating classifier losses.

How to cite: Horender, S., Giannakoudaki, C., Abt, R., Auderset, K., Crouzy, B., Erb, S., Erdogdu, O., Graf, E., Iida, K., Niederberger, E., Ou, L., Sakurai, H., Schmale, J., Wälchli, C., and Vasilatou, K.: Method for calibration of bioaerosol monitors based on reference pollen aerosols and imaging-based Lagrangian particle tracking as reference: the case of the Swisens Poleno, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11529, https://doi.org/10.5194/egusphere-egu25-11529, 2025.

EGU25-12519 | Posters on site | AS3.10

Assessing Associations Between Pollen Resilience Index Forecast Values and Allergic Health Symptoms Induced by Aeroallergens 

Ingrida Sauliene, Laura Sukiene, Gintautas Daunys, Ruta Dubakiene, Odilija Rudzeviciene, and Edvinas Stonevicius

Pollen is one of the primary aeroallergens that negatively impacts human health during the vegetation period. Studies have demonstrated that air pollution and meteorological factors influence the severity of airborne pollen load and modify its effects on health. The Pollen Resilience Index (PRI) is a five-point index developed by integrating CAMS air pollution and pollen forecast data within a framework of legal and scientific thresholds and Humidex index values. It ranges from 1 (no health effects observed in sensitive individuals) to 5 (pollen exposure, combined with environmental factors, causes adverse health effects). The forecasted PRI values indicate the potential severity of pollen exposure under varying environmental conditions.

In this study, we aimed to validate the PRI using retrospective, anonymised data collected from users of the PASYFO mobile application. The dataset comprised 9,472 symptom reports related to eye, nose, and lung symptoms from 247 participants. These responses were analysed to determine how PRI values correspond with symptom reporting. Sensitivity to airborne irritants and individuals’ ability to tolerate these effects varied considerably and were limited by personal health conditions, reporting habits, and symptom intensity. This variation introduced uncertainty into the results, complicating statistical analysis.

Our analysis revealed a strong and consistent tendency for participants to report symptoms when the PRI exceeded a value of 1. Specifically, as the PRI increased, the proportion of respondents reporting symptoms also rose. This effect was most prominent for eye and nose symptoms. For example, when the PRI was 1, 21.3% of participants reported eye and 31.1% reported nose symptoms. At the maximum PRI value of 5, the proportion of individuals reporting eye symptoms increased to 42.6%, while nose symptoms were reported by 58.7% of participants. Common symptoms, such as eye itching, watering, redness, runny nose, and sneezing, showed the most significant increase in reporting under higher PRI conditions. The effect on lung-related symptoms was less pronounced, although their reporting also increased with higher PRI levels. Respiratory symptoms, including shortness of breath and coughing, rose by less than 7% even under the worst conditions (PRI = 5). This suggests that while pollen exposure affects respiratory health, its correlation with lung symptoms is less direct compared to eye and nose symptoms.

Among the various types of pollen, Betula (birch) and Alnus (alder) were most closely associated with the development of allergic symptoms. This highlights the significance of specific pollen types in exacerbating allergic reactions. The findings underscore the value of using the PRI as a predictive tool to assess the potential health risks posed by aeroallergens and to help mitigate their impact on sensitive individuals. Our research demonstrates the effectiveness of integrating air quality, weather, and pollen data to create a tool for predicting the health impacts of aeroallergens.

This research was funded by the LMTLT agreement No. S-MIP-19-53 and supported by EO4EU, funded by the Horizon Europe RIA Programme under Grant Agreement No. 101060784.

How to cite: Sauliene, I., Sukiene, L., Daunys, G., Dubakiene, R., Rudzeviciene, O., and Stonevicius, E.: Assessing Associations Between Pollen Resilience Index Forecast Values and Allergic Health Symptoms Induced by Aeroallergens, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12519, https://doi.org/10.5194/egusphere-egu25-12519, 2025.

EGU25-12813 | Posters on site | AS3.10

A 43 years-long European pollen reanalysis for alder, birch, and olive 

Mikhail Sofiev and Julia Palamarchuk and the SILAM modelling team and European Pollen Reanalysis data providers

Airborne pollen released by plants during their flowering season can cause significant allergic symptoms impairing public health, especially if accompanied with air pollutants and/or weather phenomena (e.g., high temperature). Apart from the public health-related motivation, information on pollen in the air can be useful to monitor biodiversity, follow species migration, habitat degradation, etc. Systematic knowledge about continental-scale pollen distribution patterns is hard to obtain due to tedious manual observation methods used through decades and limited modelling experience and maturity level.

The European Pollen Reanalysis v.1.1 (EPR) is the first 43 year-long reanalysis of pollen seasons for three major allergenic tree genera in Europe: alder (Alnus), birch (Betula), and olive (Olea). The EPR has been created by the atmospheric composition model SILAM driven by the European meteorological reanalysis ERA5. SILAM predicted a Europe-wide dispersion pollen for 1980–2022. For each year, an extended 4-dimensional variational data assimilation was applied assimilating in-situ observations of aerobiological networks of 34 European countries. The assimilated variable was the total seasonal emission of pollen grains. Therefore, the EPR assimilation constitutes an inverse dispersion problem solution realized as an annual correction factor to the mean pollen production. The EPR is positioned as an input for health- and climate- related studies, biodiversity monitoring, etc.

How to cite: Sofiev, M. and Palamarchuk, J. and the SILAM modelling team and European Pollen Reanalysis data providers: A 43 years-long European pollen reanalysis for alder, birch, and olive, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12813, https://doi.org/10.5194/egusphere-egu25-12813, 2025.

EGU25-13392 | Posters on site | AS3.10

The European infrastructure for real-time monitoring of bioaerosols: collaborative solutions of AutoPollen Programme and SYLVA project 

Yuliia Palamarchuk, Mikhail Sofiev, Bernard Clot, Evgeny Kadansev, and Annika Saarto

The presence of aerosols of biological origin in the atmosphere is one of the key factors affecting the quality of human life on a daily basis. The spread and diversity of bioaerosols are heavily influenced by anthropogenic activity and significantly modulated by changing climate. A constantly growing number of allergy sufferers in Europe sets new demands to available information about the aeroallergen sources and their evolution. The existing monitoring activities and practices for bioaerosol observations are very fragmented and country specific. Limited access to the highly demanding manual counts slows down cross-disciplinary research and development of prevention measures (effective strategies) to minimize the environmental bioaerosol impact. At the same time, the recent technological progress in the automatic particle counters paved the way to the volunteering consolidation of European aerobiologists to establish and to drive the EUMETNET AutoPollen Programme (www.autopollen.ne). The extremely active collaboration within AutoPollen set a solid background for the dedicated innovative project SYLVA (A SYstem for reaL-time obserVation of Aeroallergens, https://sylva.bioaerosol.eu). Development of the standards and guidelines for the aeroallergen measurements within AutoPollen and technological solutions within SYLVA (newly created and updated and verified existing solutions) are integrated in a complex synergy of the prototype of European network and infrastructure for the real-time monitoring of bioaerosols.

How to cite: Palamarchuk, Y., Sofiev, M., Clot, B., Kadansev, E., and Saarto, A.: The European infrastructure for real-time monitoring of bioaerosols: collaborative solutions of AutoPollen Programme and SYLVA project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13392, https://doi.org/10.5194/egusphere-egu25-13392, 2025.

EGU25-14796 | Posters on site | AS3.10

Betula pollen observation: integration of automated device records into long-term datasets 

Laura Šukienė, Ingrida Šaulienė, Edvinas Stonevičius, Lukas Vaitkevičius, and Gintautas Daunys

Technological progress and the timely availability of Earth Observation (EO) data have rapidly changed pollen research. Innovative solutions enable the development of instruments for airborne pollen identification, and integrating an increasing amount of remotely acquired EO data improves pollen forecasts. Nowadays, data about pollen in the air are available from different types of devices. Pollen data gathered using Hirst-type volumetric spore traps is especially valuable as they are long-term and can be used to evaluate climate peculiarities. The air samples were collected over 20 years. Meanwhile, data on pollen spread has recently been monitored using more sophisticated devices. The new generation devices collect data about airborne pollen automatically in near real-time. Multiple statistical methods are essential in data homogenisation, especially when integrating heterogeneous data to handle long-term observation challenges. This study aims to demonstrate the feasibility of statistical methods used to integrate records about airborne pollen from automated devices into long-term data collected with Hirst-type volumetric spore traps.

The research is based on 20 years of Betula pollen data (2005-2024) collected with a Hirst-type trap (so-named manual data) and the short-term pollen data from SwisensPoleno Mars records (so-named automatic data) covered by several years. Both devices are operational and located in Vilnius, Lithuania. Overlapping datasets from 2022 to 2024 were used in this research. We chose the data modelling pathway to assess the integration of automated device records with long-term data. Several statistical modelling approaches were tested: simple linear regression, polynomial multiple regression, generalised additive model, Prophet model, random forest model and their combinations.

Multivariate polynomial regression enables the estimation of non-linear relationships and local data heterogeneity. Heterogeneity in local pollen data records can be caused by peculiarities of flowering time and/or local weather patterns, which require models to evaluate differences. Generalized Additive Model (GAM’s) handless non-linear and seasonal patterns of airborne pollen. The Prophet model concept was also applied to estimate long-term trends and seasonality of datasets. Statistical data analysis of long-term Betula pollen data was used to make corrections to the data collected by the automatic devices and to compare the corrected bias with the observational data to assess the performance and applicability of the methods. Considering variations in mean bias error (MBE), mean absolute error (MAE) and root mean square error (RMSE), the tested models were demonstrated to highlight different causal pathways for the inconsistency between the long-term manual data and the short-term automatic data. The knowledge gained is valuable for integrating observational data into current forecasting tools, such as PASYFO, which forecasts allergy symptoms, as well as homogenising heterogeneous airborne pollen data.

This research is supported by the projects EO4EU and SYLVA, funded by the Horizon Europe RIA Programme under Grant Agreements No. 101060784 and No. 101086109.

How to cite: Šukienė, L., Šaulienė, I., Stonevičius, E., Vaitkevičius, L., and Daunys, G.: Betula pollen observation: integration of automated device records into long-term datasets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14796, https://doi.org/10.5194/egusphere-egu25-14796, 2025.

EGU25-15510 | Orals | AS3.10

Forecasting the Onset of Cupressus Flowering in the Mediterranean Region  

Pilvi Siljamo, Mikhail Sofiev, and Yuliia Palamarchuk

Cypress species and other members of the Cupressaceae family are widespread evergreen trees and shrubs, commonly used as ornamental plants. Some species, such as Mediterranean cypress (Cupressus sempervirens), Arizona cypress (Cupressus arizonica), and prickly juniper (Juniperus oxycedrus), widespread in Mediterranean, cause significant allergic reactions. This study aimed to develop a phenological model for Southern and Central Europe to predict the timing of cypress pollen release, enabling integration into atmospheric models for pollen dispersion forecasts. 

A key challenge is the microscopic similarity of all Cupressaceae pollen grains, which prevents species-level identification. Consequently, pollen observations report total Cupressaceae counts, complicating phenological modeling of allergenic species. 

For early-flowering species, thermal time models, such as growing degree days (GDD) or growing degree hours (GDH), are suitable. These models require defining a heat accumulation start date, a temperature threshold, and the cumulative heat required for flowering. Geographic variability and ornamental planting further influence flowering patterns, even between neighbouring locations. 

Pollen data were obtained from the European Aeroallergen Network (EAN), and temperature data from the ERA5 reanalysis dataset. Testing three start dates of the accumulation revealed that the autumn equinox was too early, while January 1st was too late, as J. oxycedrus and C. arizonica may flower before the new year. November 30th was optimal for detailed analysis. GDD/GDH was calculated using thresholds of 0°C, 1°C, 2°C, and 5°C, with normalized GDH (nGDH) yielding the most accurate results. 

When flowering onset was defined as 5% of the seasonal pollen index (SPI), the median GDH requirements ranged from 0.06–0.15 nGDH0 (SD 0.01–0.05) to 0.01–0.06 nGDH5 (SD 0–0.02). A 5°C threshold was too high leading to insufficient heat accumulation sensitivity, while 0°C was too low due to higher variability between years. Thresholds of 1°C and 2°C provided optimal accuracy with moderate inter-annual variability, making them suitable for forecasting the flowering onset. 

 

How to cite: Siljamo, P., Sofiev, M., and Palamarchuk, Y.: Forecasting the Onset of Cupressus Flowering in the Mediterranean Region , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15510, https://doi.org/10.5194/egusphere-egu25-15510, 2025.

EGU25-17983 | Posters on site | AS3.10

Bridging Automatic and Manual Pollen Monitoring: A Path Towards Homogenized Long-Term Time Series 

Mária Lbadaoui-Darvas, Regula Gehrig, Ingrida Sauliene, Laura Sukiene, and Jose Oteros

The measurement of pollen concentrations began in the 1960s, initiated by medical doctors seeking to address allergenic concerns. Historically, pollen monitoring networks relied on the manual identification of daily samples collected on tapes in Hirst-type traps using optical microscopy. This approach persisted until a recent paradigm shift towards automatic, in situ monitoring solutions.

The new generation of automatic measurement systems employs advanced techniques, such as automated microscopy (e.g., BAA 500) or digital holography combined with fluorescence measurements (Swisens Poleno). These are augmented by AI-based identification algorithms, enabling real-time pollen monitoring with temporal resolutions of at least one hour. However, manual and automatic measurement systems exhibit different sampling efficiencies for various pollen species, stemming from disparities in instrumentation characteristics such as flow rates, identification and data processing methods, and temporal resolution. This technological transition has introduced a discontinuity in the historical pollen concentration time series, which are crucial for forecasting models.

In this study, we analyze and compare manual and automatic pollen concentration time series from the Swiss national pollen monitoring network for four major allergenic pollen types: alder, birch, grasses, and oak—species significant across different regions of Europe. Data from 2022 to 2024, collected simultaneously using both methods in rural and urban settings in Switzerland, are evaluated. Machine learning regression algorithms (Random Forest, GRNN) are leveraged to establish a transfer function that relates automatic and manual pollen data. The model incorporates environmental variables likely to influence pollen concentrations, including temperature, wind velocity, elevation, and particulate matter (PM) concentrations.

How to cite: Lbadaoui-Darvas, M., Gehrig, R., Sauliene, I., Sukiene, L., and Oteros, J.: Bridging Automatic and Manual Pollen Monitoring: A Path Towards Homogenized Long-Term Time Series, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17983, https://doi.org/10.5194/egusphere-egu25-17983, 2025.

EGU25-18305 | Posters on site | AS3.10

Pollen, fungal spore and fluorescent particle concentrations during long-range transport events at the Sonnblick Observatory (3106m asl) 

Julia Burkart, Silvia Bucci, Karen Kölzer, Andreas Stohl, Bernadett Weinzierl, Elke Ludewig, and Maximilian Bastl

The recent rise of automatic and online instrumentation for bioaerosol research has stirred the interest from diverse scientific communities and more and more monitoring stations are installed worldwide. Providing a higher time resolution, the automatic instruments promise novel insights into atmospheric processes and distribution patterns of bioaerosols. While most stations are situated well within the atmospheric boundary layer and in populated areas, we will present data from a high alpine research station, the Sonnblick Observatory, located at 3106 m asl. Such measurements at high altitudes, far away from local sources and in atmospheric regions where clouds form, are rare.

From April 2023, a SwisensPoleno Jupiter was installed at the Sonnblick Observatory alongside a manual Hirst-type pollen trap. The SwisensPoleno Jupiter is an online aerosol monitor that obtains scattered light, two holographic images and fluorescence signals of single aerosol particles. With the Hirst-type pollen trap, the particles are collected on a sticky tape and are later examined manually under a microscope, identifying pollen and fungal spores by visual inspection. For pollen, 30 percent of the tape surface and for fungal spores 10 percent is analyzed, which exceeds the requirements of the current European standard for pollen monitoring. The increased detection area for pollen takes in account the lower concentrations which are expected at high altitudes.

In a first step, time series of concentrations and fractions of fluorescent particles (as a proxy for bioaerosols) obtained from the SwisensPoleno Jupiter were analyzed to identify particularly interesting time periods and seasonal patterns. The time series of fluorescent particles show a clear increase in the concentrations and fractions of fluorescent particles over the course of the season from early spring to summer (fluorescent fraction: 0.2 in April; 0.6 in June).

In a second step, we focused on selected time periods where FLEXPART simulations indicate long-range transport of air masses such as from the Saharan region. For these periods, we took a closer look at the fluorescence properties of the particles together with the holographic images. In a previous laboratory study, we obtained representative fluorescence signals for three classes of bioaerosol particles: pollen, fungal spores and plant debris. We use these data in combination with pollen and spore counts from the Hirst-type trap to characterize the selected events and compare them with periods with stagnant conditions and stronger local influence.

How to cite: Burkart, J., Bucci, S., Kölzer, K., Stohl, A., Weinzierl, B., Ludewig, E., and Bastl, M.: Pollen, fungal spore and fluorescent particle concentrations during long-range transport events at the Sonnblick Observatory (3106m asl), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18305, https://doi.org/10.5194/egusphere-egu25-18305, 2025.

EGU25-18361 | ECS | Orals | AS3.10

Atmospheric spore content of the grapevine pathogenic fungi Plasmopara viticola and Botrytis cinerea in Mediterranean vineyards 

Guillermo Muñoz Gómez, Eduardo Jiménez Jiménez, Beatriz Lara Espinar, Rosa María Rodriguez-Arias, Jesús Rojo Úbeda, María Fernández González, Francisco Javier Rodríguez Rajo, Federico Fernández González, and Rosa Pérez Badia

Grapevine (Vitis vinifera L.) cultivation is one of the oldest, most widespread and important crops in the world. Downy mildew and grey mould are fungal diseases caused by the oomycete Plasmopara viticola and the ascomycete Botrytis cinerea, respectively. These diseases have a serious negative impact on viticulture, reducing the quantity and quality of harvests. Monitoring of variables affecting the environment-host-pathogen system in important viticulture areas is necessary for the control and prevention of these diseases. The aim of this study was to analyse the dynamics and behaviour of the atmospheric content of P. viticola and B. cinerea spores, as well as their relationship with different meteorological variables and the phenology of the grapevine.

The study was conducted between May and November 2023 in a vineyard belonging to the land of the Designation of Origin Uclés, D.O Uclés, located in the west of Cuenca province (Castilla-La Mancha region, central Spain). The area has a dry Mediterranean climate. Aerobiological sampling was carried out using a Hirst volumetric spore trap placed 2 metres above the ground in a vineyard of the Syrah grape cultivar. Samples were prepared and analysed following the methodology established by the Spanish Aerobiology Network. Phenological sampling was carried out weekly on 20 Syrah grapevines close to the spore trap, using an adaptation of the BBCH scale. Meteorological data were obtained from the Spanish Meteorological Agency (AEMET). The relationship between spore concentrations and meteorological variables was analysed using Spearman's non-parametric correlation test and Principal Component Analysis (PCA). Furthermore, an intradiurnal analysis of spore concentration was carried out.

A total of 894 spores/m3 of B. cinerea and 758 spores/m3 of P. viticola were obtained during the studied period. For B. cinerea, the daily peak spore concentration was on 18 October with 54 spores/m3, for P. viticola it was on 13 November with 74 spores/m3. The phenological stages with the highest daily spore concentrations for both pathogens were flowering, ripening and senescence of the grapevine. The spore concentration of both pathogens is positively influenced by relative humidity (RH), while temperature variables (mean, maximum and minimum) have a negative influence. Intradiurnal analysis showed that the highest spore concentrations occurred between midday (11:00-12:00) and early afternoon (16:00-17:00).

Flowering and ripening are critical stages for the development of these diseases. High temperatures and drought, characteristic of the summer period in areas with a dry Mediterranean climate, inhibit sporulation. However, diseases can develop before and after this period, when conditions are favourable. Progress in the knowledge of the environment-host-pathogen system in these areas will help to decide the most appropriate times for the application of phytosanitary treatments.

This work has been funded by the Ministry of Education, Culture and Sports of the JCCM, through the project SBPLY/21/180501/000172 and by the University of Castilla-La Mancha (UCLM) through the project 2022-GRIN-34507 and a pre-doctoral contract to Guillermo Muñoz-Gómez of the “Plan Propio I+D+I” of the UCLM.

How to cite: Muñoz Gómez, G., Jiménez Jiménez, E., Lara Espinar, B., Rodriguez-Arias, R. M., Rojo Úbeda, J., Fernández González, M., Rodríguez Rajo, F. J., Fernández González, F., and Pérez Badia, R.: Atmospheric spore content of the grapevine pathogenic fungi Plasmopara viticola and Botrytis cinerea in Mediterranean vineyards, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18361, https://doi.org/10.5194/egusphere-egu25-18361, 2025.

EGU25-19020 | ECS | Posters on site | AS3.10

Performance of the Swisens Poleno automatic air-flow cytometer in Nordic conditions 

Evgeny Kadantsev, Julia Palamarchuk, Rostislav Kouznetsov, and Mikhail Sofiev

Real-time air-flow cytometry, a technique for analysing microparticles suspended in the air, has advanced rapidly with the development of state-of-the-art automatic monitors. This study presents results obtained using measurements from the Swisens Poleno cytometer, which, in our case, were processed using a pollen recognition algorithm primarily trained to identify species typical of Southern Finland.

The algorithm performed remarkably well under laboratory conditions, achieving an overall accuracy of nearly 90%. Most misclassifications involved pollen grains from species within the same pollen family, an understandable outcome given their morphological similarities. However, applying the classification model to environmental measurements collected under real atmospheric conditions revealed additional challenges. The most significant issue was the occurrence of false positive recognitions, where the algorithm mistakenly identified particles as pollen that could not realistically be present in the air at the time of measurement. This discrepancy was identified through parallel measurements conducted with a manually operated Hirst-type pollen trap. To address this, previously neglected fluorescence signal was integrated into the algorithm, which partially mitigated the issue. We present a comparison of pollen concentrations measured by the Poleno cytometer, using the improved recognition algorithm, and the manual trap across multiple seasons and locations in Northern Europe. While the correlation between the two methods was slightly lower than expected based on laboratory results, it reached approximately 0.85 for the main pollen species in bi-hourly measurement intervals. Additionally, we demonstrate the device’s reliability under the harsh weather conditions of Arctic winters.

How to cite: Kadantsev, E., Palamarchuk, J., Kouznetsov, R., and Sofiev, M.: Performance of the Swisens Poleno automatic air-flow cytometer in Nordic conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19020, https://doi.org/10.5194/egusphere-egu25-19020, 2025.

EGU25-19841 | ECS | Posters on site | AS3.10

Advancing eDNA analysis techniques of atmospheric bioaerosol samples  

Julija Salokas, Svetlana Sofieva-Rios, Jussi Paatero, Eija Asmi, Ari Karppinen, and Mikhail Sofiev
Primary biological aerosols in the Earth atmosphere, including pollen, fungal spores, bacteria and viruses, constitute a substantial fraction of aerosols and are actively dispersed by winds over large distances. The composition of bioaerosols is determined by vegetation composition at the surface and influenced by seasonal shifts, weather patterns, and can be modulated by air pollution levels.  

Aerial microbes, which make up less than 1% of airborne entities, have often been overlooked due to challenges in traditional monitoring methods, such as culturing and microscopy. Metagenomics has addressed this gap, allowing for the exploration of species diversity through DNA extraction and culture-independent analyses. This approach is particularly pertinent for understanding enigmatic aerosols, such as pollen, where accurate DNA extraction is essential for precise metagenomic studies, microbial profiling, and aeroallergen detection. Long-read DNA sequencing technologies, such as PacBio and Oxford Nanopore, have transformed biodiversity studies by providing much more comprehensive and accurate genetic information. These technologies produce reads that can cover entire genes or genomes, making them invaluable for studying complex ecosystems. In the field of bioaerosols, long-read sequencing can help to identify new species, detect genetic diversity, and enhance our understanding of microbial community functions, also simplifying the task of genome assembly.  

Metagenomic studies of the atmospheric bioaerosols face challenges due to low concentration of biological material in the air in comparison with water and soil. Overcoming this roadblock, one has to use high-volume samplers (expensive and difficult as well) and/or a highly sensitive and precise procedure of the sample treatment and sequencing. Here the second challenge is addressed by presenting an eDNA analysis procedure applicable to atmospheric samples with moderate-to-low amount of biological material. 

How to cite: Salokas, J., Sofieva-Rios, S., Paatero, J., Asmi, E., Karppinen, A., and Sofiev, M.: Advancing eDNA analysis techniques of atmospheric bioaerosol samples , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19841, https://doi.org/10.5194/egusphere-egu25-19841, 2025.

EGU25-19857 | ECS | Posters on site | AS3.10

A glance into specie composition of biological aeroallergens: metagenomic approach 

Svetlana Sofieva-Rios, Anders Stangel, and Mikhail Sofiev

Environmental metagenomic air samples contain a large amount of information that can be unraveled with a suitable toolkit. Among numerous objectives, taxonomic identification and relative abundance estimation are one of the key points of interest in metagenomic DNA analysis. This type of analysis for large sequence datasets requires considerable computing resources with the publicly available bioinformatic software and pipelines optimized for analysis of next generation sequencing data and often targeting only bacteria. The SYLVA-DNA-classifier is a pipeline developed to efficiently and accurately classify large quantities of 3rd generation sequencing data among all kingdoms, with a special focus on plants and fungi, as best known aeroallergens.

How to cite: Sofieva-Rios, S., Stangel, A., and Sofiev, M.: A glance into specie composition of biological aeroallergens: metagenomic approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19857, https://doi.org/10.5194/egusphere-egu25-19857, 2025.

EGU25-20504 | ECS | Posters on site | AS3.10

Detection of pollen and biomass burning particles using laser- induced aerosol fluorescence and in situ techniques during the PERICLES campaign 2023 in Switzerland 

Marilena Gidarakou, Alexandros Papayannis, Kunfeng Gao, Panagiotis Gidarakos, Benoît Crouzy, Romanos Foskinis, Sophie Erb, Cuiqi Zhang, Gian Lieberherr, Maxime Hervo, Michael Rösch, Martine Collaud Coen, Branko Sikoparija, Zamin Kanji, Bernard Clot, Bertrand Calpini, and Athanasios Nenes

The Payerne lidaR and Insitu detection of fluorescent biomass burning and dust partiCLES and their cloud impact (PERICLES) campaign (May - June 2023) took place at the rural site of Payerne, Switzerland (46.82o N, 6.94o E, 491 m a.s.l.), at the premises of MeteoSwiss station. PERICLES aimed to understand the spatio-temporal variability of different types of bioaerosols (biomass burning, pollen, dust, etc.) in the Planetary Boundary Layer and aloft (typically up to 2-5 km asl.) and their role in cloud formation. As bioaerosols play a crucial role in cloud formation and on human health, there is strong need to characterize them, both at ground level and aloft. Recently, elastic and fluorescence lidars have become important tools for characterizing bioaerosols’ types. In this study, we used a synergy of in-situ and laser remote sensing instrumentation to discriminate between pollen, dust and biomass burning bioparticles and evaluate their role in cloud formation. Biomass burning particles originated from long-range wildfires in Canada and near-range ones in Germany. High concentrations of pollen were recorded by in situ instruments (Hirst-type volumetric trap, Swisens Poleno and WIBS 5 NEO) at ground level. The EPFL elastic-laser induced fluorescence (LIF) lidar was used to provide vertical profiles of the aerosol elastic (baer) and fluorescence backscatter (bF) coefficients, along with the fluorescence capacity factor (GF), during the study period. Typical values of bF ranged from 1.5 to 8.5 x10-4 Mm-1 sr-1, while GF took values between 1-8 x 10-4. A 32-channel spectrometer detected the bioaerosol fluorescence lidar signals aloft (from ground up to 1-1.5 km height). Application of machine learning algorithms we were able to determine the percentage distribution of various pollen types (e.g. Dactylis glomerata, Quercus robur, Fagus Sylvatica and Betula pendula), which correlate well with ground-level pollen data and number concentrations of ice-nucleating particles (INPs).

How to cite: Gidarakou, M., Papayannis, A., Gao, K., Gidarakos, P., Crouzy, B., Foskinis, R., Erb, S., Zhang, C., Lieberherr, G., Hervo, M., Rösch, M., Collaud Coen, M., Sikoparija, B., Kanji, Z., Clot, B., Calpini, B., and Nenes, A.: Detection of pollen and biomass burning particles using laser- induced aerosol fluorescence and in situ techniques during the PERICLES campaign 2023 in Switzerland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20504, https://doi.org/10.5194/egusphere-egu25-20504, 2025.

EGU25-21463 | ECS | Posters on site | AS3.10

Detection of bioparticles by synergy of depolarisation-LIF lidars supported by in situ measurements at the high alpine station of Helmos, Greece, during the CHOPIN campaign 2024 

Alexandros D. Papayannis, Marilena Gidarakou , Romanos Foskinis  , Christos Mitsios , Carolina Molina  , Kaori Kawana , Kalliopi Violaki , Olga Zografou , Maria Gini , Prodromos Fetfatzis, Konstantinos Granakis , Paul Zieger, Aiden Jönsson, Mika Kommpula, Konstantinos Eleftheriadis, Eugenia Giagka, Marios-Andreas Zagklis, and Athanasios Nenes

The Cleancloud Helmos OrograPhic site experimeNt (CHOPIN) campaign took place in autumn 2024 at a unique high-altitude location at Mount Helmos, Greece (38.0oN, 22.2oE) ideal for targeted studies of aerosol-cloud interactions (ACI) due to its strategic location, serving as a crossroad for different aerosol transport paths. This unique position allows the detection of a wide range of particles like wildfire smoke, continental polluted, marine and mineral dust from Sahara, as well as bioparticles (pollen, bacteria, fungal spores) from near- and long-range sources. State-of-the-art laser remote sensing and in situ instrumentation was implemented at Mount Helmos at two level heights: 1700 m (remote sensing instrumentation) and 2314 m a.s.l. (in situ instrumentation) to characterize the incoming air masses in terms of their bioparticle content and study the role of bioparticles in cloud formation. In this study we will focus on data obtained by two lidar systems: the two-wavelength (532 -parallel and cross depolarization and 1064 nm) depolarization aerosol lidar system (AIAS), and the NTUA/EPFL/FORTH 4-wavelength elastic-Raman-laser induced fluorescence (LIF) lidar system (ATLAS-NEF) to provide vertical profiles of aerosol optical properties (extinction and backscatter coefficients and lidar ratio at 355 nm, backscatter Ångström exponents at 355/532nm, 532/1064 nm, particle depolarisation lidar ratio at 532 nm), water vapor mixing ratio, fluorescence capacity and fluorescence backscatter coefficients at 470 nm. We present cases of Saharan dust intrusions with increased values of the aerosol backscatter coefficient and high particle depolarization ratios (δ532 ~0.20-0.25) and increased values of lidar ratios (LR~40-55 sr), high numbers of ice-nucleation particles (INPs) obtained with a PINE instrument and strong signals obtained at the 3 channels of the Wideband Integrated Bioparticles Sensor (WIBS) operating at the (HAC)2 station indicate the presence of bioparticles able to enhance cloud formation.

How to cite: Papayannis, A. D., Gidarakou , M., Foskinis  , R., Mitsios , C., Molina  , C., Kawana , K., Violaki , K., Zografou , O., Gini , M., Fetfatzis, P., Granakis , K., Zieger, P., Jönsson, A., Kommpula, M., Eleftheriadis, K., Giagka, E., Zagklis, M.-A., and Nenes, A.: Detection of bioparticles by synergy of depolarisation-LIF lidars supported by in situ measurements at the high alpine station of Helmos, Greece, during the CHOPIN campaign 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21463, https://doi.org/10.5194/egusphere-egu25-21463, 2025.

EGU25-21470 | ECS | Orals | AS3.10

Evaluating the capture efficiency of fungal spores with automatic monitors: the case of BAA500 (Hund GmbH) 

Mónica González-Alonso, Matúš Žilka, Carsten Schmidt-Weber, and Jeroen Buters

Although bioaerosol particles are invisible to our eyes, they have a big impact in human life. Already at the beginning of the past century, the first attempts to detect the airborne pathogens causing damages in crops took place (Hirst, 1994), leading to the development of the Hirst trap (Hirst, 1952). From the agriculture field, the use of this trap jumped to the medical field, being used to monitor pollen and spores for the allergy patients. Since then, the use of manual pollen traps has spread around the world (Buters et al., 2018). However, the lack of experts and the laborious work of counting spores with a bright field microscope due to their small size and high numbers, has led to a scarcity of data on airborne fungal spores as compared to pollen. 

Recently, automatic monitors have been developed and are able to identify pollen in the air (Buters et al., 2022). Some automatic monitors have proven to perform well in pollen identification (Maya-Manzano et al., 2023) and are being used in official monitoring networks (Oteros et al., 2020, Sauvageat et al., 2020, Tešendić et al., 2020). These devices have brought a new opportunity to the identification of other bioaerosols, i.e., fungal spores. 

One of such instruments is the BAA500 (Hund GmbH). This instrument is designed as a cascade impactor. The air is sucked at high speed and particles between 4-80 µm arrive to a sticky plate at the end, where they are photographed with a camera attached to a microscope. Then, a software based in convolutional neural networks identifies the particles. The Validation tool (https://validation.pollenscience.eu/) is a quality control tool that allows to see the particles detected by the monitor. Within these images, we have confirmed that fungal spores are being captured by the device. However, a closer examination to evaluate their capture efficiency has not been done yet. 

In order to test the efficiency of the BAA500 in the capture of fungal spores, we collocated a Hirst trap next to an automatic monitor for five months (from May to October 2024) and compared the concentration of 5 fungal spore types, comprising a wide size range challenging the detection lower and upper limits of the instrument: Ganoderma, Cladosporium, Polythrincium, Epicoccum and Alternaria.

First results show that small (R2= 0.02, 0,08) and big (R2= 0.39) spores are under captured by the automatic device as compared to the Hirst trap, probably due to their size being in the limits of the cascade impactor, whereas medium-size spores correlate nicely with Hirst concentrations, showing a correlation of R2= 0.69 and 0.76. These results confirm the potential of the BAA500 to be used as fungi monitor for medium-size spores. Spores with a size close to the detection limit will need a scaling factor.

How to cite: González-Alonso, M., Žilka, M., Schmidt-Weber, C., and Buters, J.: Evaluating the capture efficiency of fungal spores with automatic monitors: the case of BAA500 (Hund GmbH), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21470, https://doi.org/10.5194/egusphere-egu25-21470, 2025.

EGU25-21490 | Orals | AS3.10

The influence of local particles on classifier performance for pollen monitoring 

Andreas Schwendimann, Yanick Zeder, Kilian Koch, Elias Graf, Erny Niederberger, Elena Gottardini, Antonella Cristofori, Fabiana Cristofolini, and Magdalena Widmann

Pollen detection through automatic instruments has significantly improved over the recent years. Hirst-type traps start to be complemented with automatic instruments throughout Europe. Instead of the traditional identification of airborne pollen particles using light microscopy, data of the particles is collected and subsequently analysed by an AI-classifier. As an airflow-cytometer, SwisensPoleno instruments capture a fingerprint of each particle in-flight. Holography images, as well as fluorescence spectral data, as for SwisensPoleno Jupiter, are collected to classify measured pollen grains flowing through the device in real-time. Labelled datasets of each pollen-type of interest are required for the training of a new classifier. These are generated by collecting fresh and pure pollen from plants and aerosolizing it directly into a SwisensPoleno instrument under controlled conditions. 

New classifiers are evaluated by correlating concentrations determined by the automatic instrument with daily concentrations of co-located Hirst-type traps. To evaluate the performance of classifiers throughout Europe, multiple sites in different countries are assessed. Using results of the latest pollen classifier “Swisens (2025)”, based on holography images and fluorescence spectra, we show here how different locations of the SwisensPoleno and different input data can affect the resulting correlations to Hirst data, as well as the Mean Absolute Error (MAE). Differences in performance are expected between sites which are far apart, due to many factors such as differing geography, local climatic conditions and flora. Bad performance may arise from unknown interfering particles, only abundant at one specific site, and thus not included in the training datasets.

Our results demonstrate that this effect can also occur at a sub-regional scale, in sites only 30 km apart (Figure 1A), installed with the same instrument, and analysing data with the same classifier. Fraxinus pollen concentrations for P48 (Bolzano, Italy) correlate very well with a co-located Hirst (Figure 1B); that isn’t true for P46 (San Michele all’Adige, Italy), where strong interference from other particles is present during late May and beginning of June (Figure 1C). Interfering particles, similar to the target taxa, require site specific fine-tuning, e.g. in form of additional filters specifically excluding the interfering particles. In conclusion, while automatic pollen detection instruments show great promise in improving accuracy and efficiency, our findings highlight the importance of site-specific adaptations to address geographic and environmental variability, ensuring reliable performance across diverse locations.

 

How to cite: Schwendimann, A., Zeder, Y., Koch, K., Graf, E., Niederberger, E., Gottardini, E., Cristofori, A., Cristofolini, F., and Widmann, M.: The influence of local particles on classifier performance for pollen monitoring, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21490, https://doi.org/10.5194/egusphere-egu25-21490, 2025.

EGU25-21517 | Orals | AS3.10 | Highlight

Airborne Pollen Trends during the 3 last decades in Spain  

Carmen Galan and Jose Oteros and the Pollen team

Airborne pollen significantly impacts air quality, human health, and ecosystems. Monitoring pollen trends is critical for understanding these effects, especially as pollen allergies affect millions of persons globally, reducing respiratory health and life quality. Pollen data provide relevant information about the impacts of climate change on vegetation, with shifts in flowering timing serving as indicators of ecological responses. These trends are also vital for forecasting agricultural yields, particularly in Mediterranean climates where water availability and temperature are increasingly erratic.

This study examines flowering timing and intensity trends for 12 anemophilous taxa across 12 locations in the Iberian Peninsula from 1994 to 2023. Using data from Hirst pollen monitoring method, we calculated annual trends in several flowering date indicators (e.g. peak pollen day, start of flowering, duration of pollen season) and other indicators for pollen production (e.g. peak daily pollen concentration or seasonal pollen integral). Statistical analyses assessed linear trends, comparing variations among woody and herbaceous taxa, as well as regional differences between Mediterranean and more temperate areas.

The date of maximum flowering advanced by an average of -0.054 days/year, with species-specific variations ranging from -4.2 (Amaranthaceae) to +7.3 days/year (Fraxinus). Woody taxa, especially those flowering in winter or early spring, exhibited varied responses. For instance, in some locations, Cupressus showed a slight delay with an average of -0.16 days/year, while Betula displayed a more marked delay, averaging -0.33 days/year. These delays are likely linked to insufficient chilling requirements in warm winters. Herbaceous taxa, such as Poaceae, advanced their flowering by an average of -0.13 days/year, equivalent to 1.3 days/decade, reflecting their sensitivity to rising temperatures and altered water availability. Notably, Rumex experienced a marked delay in flowering of -0.48 days/year, while Urticaceae advanced by +0.42 days/year.

Seasonal pollen integral displayed contrasting trends. Tree species such as Olea (average increase: +377.83 pollen grains/year, max: +1193.99 pollen grains/year in Jaén), Quercus (+180.81 pollen grains/year, max: +594.15 pollen grains/year in Córdoba), and Cupressus (+174.55 pollen grains/year, max: +853.45 pollen grains/year in Granada) showed significant increases. Conversely, certain herbaceous taxa, such as Poaceae (-11.89 pollen grains/year, min: -158.79 pollen grains/year in Badajoz), Amaranthaceae (-10.81 pollen grains/year, min: -30.07 pollen grains/year in Málaga) and Rumex (-6.67 pollen grains/year, min: -24.85 pollen grains/year in Badajoz), showed declining pollen loads, particularly in Mediterranean regions heavily affected by drought. In contrast, some taxa like Platanus displayed moderate increases averaging +101.11 pollen grains/year, demonstrating the complexity of pollen production responses to climatic variables.

Trends were not homogeneous across Spain. Southern regions exhibited more pronounced changes in flowering timing and intensity, aligning with greater climatic extremes. The observed trends in flowering timing and intensity underscore the complex ecological responses to climate change. Warming winters delay flowering in some taxa due to insufficient chilling, while rising temperatures and CO2 levels could have driven increased pollen production in others, particularly in trees, but not so clear evidence in herbaceous. These findings highlight the need for continued pollen monitoring to mitigate the health impacts of allergenic pollen and to adapt agricultural practices to changing climatic conditions.

How to cite: Galan, C. and Oteros, J. and the Pollen team: Airborne Pollen Trends during the 3 last decades in Spain , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21517, https://doi.org/10.5194/egusphere-egu25-21517, 2025.

EGU25-354 | ECS | Posters on site | AS3.11

Distributional characteristics and causes of single-layer stratiform clouds in the Southeastern Pacific Ocean 

Ximing Deng, Yong Han, Chunsong Lu, Xinxin Xie, Yurong Zhang, Tianwei Lu, Li Dong, and Qicheng Zhou

Single-layer stratocumulus clouds (Sc), as the most common cloud system for stratiform clouds, plays an important role in global radiative balance due to their duration and extensive coverage. However, there are still substantial uncertainties in their formation and radiative forcing, creating significant challenges for accurately assessing cloud-climate feedbacks in climate models. In this paper, we use the Cloudsat 2B-CLDCLASS-LIDAR product to distinguish them from other cloud types, and investigate their formation causes and radiative effects with the ERA5 datasets and the 2B-FLXHR-LIDAR. The results show that (1) the single-layer Sc exhibits obvious seasonal variation in the spatial distribution, which is closely related to the distribution of whole-layer humidity (TCWV) and Lower Tropospheric Stability (LTS). Different aerosol concentrations alter the effects of TCWV and LTS. (2) the Cloud Fraction (CF) of the single-layer Sc showed an upward trend during January 2007-December 2010. It is believed that the CF interannual variations of the single-layer Sc are related to the monthly temperature and humidity anomalies in the middle and lower layers of the atmospheric troposphere. (3) CF has a larger impact on shortwave radiative forcing than on longwave, but its effect depends on the cloud geometric thickness (CGT). When the cloud layer is thin (61<CGT<941m), the CF enhances the cloud shortwave and longwave radiative forcing, resulting in a regional cooling effect (slope_CERnet=-1.2756); the thick cloud layer (941–1820m) will inhibit both radiation forcings, leading to a warming effect (slope_CERnet=3.0932). These findings will help improve the simulation of cloud radiative forcing, thereby reducing uncertainties in climate change assessments.

 
 
 
 
 
 
 
 
 
 
 
 
 
 
 
 
 
 

How to cite: Deng, X., Han, Y., Lu, C., Xie, X., Zhang, Y., Lu, T., Dong, L., and Zhou, Q.: Distributional characteristics and causes of single-layer stratiform clouds in the Southeastern Pacific Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-354, https://doi.org/10.5194/egusphere-egu25-354, 2025.

EGU25-387 | ECS | Posters on site | AS3.11

Exploring the hidden role of aerosols in altering the Indian Summer Monsoon rainfall variability through cloud modification 

Arya Vettikkattu Babu Nair, Moumita Bhowmik, Rituparna Chowdhury, Anupam Hazra, and Suryachandra A Rao

In recent years, the scientific community has placed growing emphasis on the impact of aerosols on the Indian Summer Monsoon (ISM) system. The ISM, the world’s strongest monsoon system, delivers approximately 80% of India’s annual rainfall from June to September, sustaining ecosystems, agriculture, and millions of livelihoods. The Indian subcontinent, with its diverse geography, dense population, and industrial zones, is a major source of aerosols through short-range and long-range transportation. Aerosols are instrumental in the process of cloud formation, functioning as cloud condensation nuclei (CCN) and ice nuclei (IN), which are vital for the formation and evolution of cloud hydrometers. Numerous possible mechanisms by how aerosols influence rainfall have been suggested by recent research on the direct radiative effects of aerosols. However, the microphysical impact of aerosols on monsoonal rainfall in the Indian Summer Monsoon Region (ISMR) remains largely unexplored. Indian summer monsoon rainfall is influenced by the large-scale circulation and different monsoon drivers. The large-scale driver modulates clouds and indicates the sign of seasonal mean ISM rainfall anomalies and the role of aerosols are secondary. Our current understanding of both the direction and magnitude of aerosol-cloud interaction (ACI), which induced changes in rainfall is insufficient. Furthermore, changes in thermodynamic and climatic circumstances, precipitation types, their vertical distribution in the atmosphere, cloud and dynamics all have a significant impact on the ACI and give feedback to ISM rainfall. In this context, we will carry out a comprehensive analysis of  multi-satellite observations and numerical model simulations  to examine the role of aerosol on cloud properties and precipitation susceptibility. The analysis of multi-satellite data reveals considerable spatial and vertical variability of dust aerosols over the ISM region. Increased dust activity can modify the monsoon cloud system, leading to significant changes in the microphysics of both the liquid and ice phases over the ISM region. The process analysis of ACI is crucial for accurately predicting monsoonal rainfall and will help resolve discrepancies in aerosol-cloud-rainfall interactions between models and observations. While more aerosols tend to reduce the cloud drop size and delay the warm rain, during the Indian summer monsoon, this is overcome by invigoration in higher moisture environments and cold-rain processes. The observational and modeling studies will be helpful for in depth understanding the role of aerosols and their interactions with clouds on the hydrological cycle by modifying the cloud properties and monsoon intraseasonal oscillations. The process studies must be beneficial for the realistic parameterization of cloud processes in the NWP model and can provide a pathway for increasing the grid point ISM rainfall skill through fundamental basic research on cloud microphysical processes.

How to cite: Vettikkattu Babu Nair, A., Bhowmik, M., Chowdhury, R., Hazra, A., and Rao, S. A.: Exploring the hidden role of aerosols in altering the Indian Summer Monsoon rainfall variability through cloud modification, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-387, https://doi.org/10.5194/egusphere-egu25-387, 2025.

Aerosol susceptibility (AS) is a parameter describing the sensitivity of cloud properties (such as increasing albedo and decreasing precipitation) to increasing aerosol concentrations. It has been shown that AS of shallow warm clouds decreases monotonically but remains positive with increasing condensation nuclei (CN) concentration. However, the presence of ice in the mixed-phase cloud may disrupt such susceptibility. We investigated the effect of ice-phase processes on AS by applying the WRF model with an aerosol-sensitive cloud microphysical scheme running in 1 km resolution. The type of low clouds investigated are the boundary-layer-topped clouds (BLTC) occurring frequently over the Northwest Pacific Ocean in winter. Aerosol sensitivity is examined by applying a wide range of CN concentration and ice nucleation rates, with the latter mimicking ice nuclei effects.

Our simulation results show that, with ice in the cloud, AS weakens and does not decrease monotonically with increasing CN concentration. The weakening of AS is due to the more efficient snow formation through the Wegener-Bergeron-Findeisen (WBF) process, which becomes stronger with more numerous cloud drops (increasing CN). Stronger snow production also enhanced graupel initiation. However, the riming growth of graupel tends to be inhibited under high CN conditions. Such a seesaw effect disrupted the monotonic trend of AS. We also found that CN and ice-phase processes can affect cloud coverage, which, in turn, gives feedback to the overall AS of all-sky albedo.

How to cite: Chen, J.-P. and Wu, C.-K.: Ice-Phase Influence on Aerosol Susceptibility in Wintertime Marine Boundary-Layer Clouds over Northwest Pacific Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1182, https://doi.org/10.5194/egusphere-egu25-1182, 2025.

EGU25-1291 | ECS | Posters on site | AS3.11

Distinct structure, radiative effects, and precipitation characteristics of deep convection systems in the Tibetan Plateau compared to the tropical Indian Ocean 

Yuxin Zhao, Jiming Li, Deyu Wen, Yarong Li, Yuan Wang, and Jianping Huang
Using spaceborne lidar and radar observations, this study identifies deep convection systems (DCSs), including deep convection cores (DCCs) and anvils, over the Tibetan Plateau (TP) and tropical Indian Ocean (TO) and finds that DCSs over the TP are less frequent, exhibiting narrower and thinner DCCs and anvils compared to those over the TO. The thinner DCCs over the TP exert weaker radiative cooling effects at the top of atmosphere (TOA) compared to the TO. But, the shortwave TOA cloud radiative effect (CRE) of TP anvils is stronger than that of the TO possibly due to more densely packed cloud tops over the TP. It results in a stronger TOA CRE of DCSs over the TP than that of TO. In particular, the longwave CRE of DCSs over the TP is notably greater at surface and low-level atmosphere due to the distinct lower temperature and less water vapour. The width of DCSs shows a positive correlation with wind shear and atmospheric instability, and the underlying mechanisms are discussed. We also find that the impact of aerosols on cloud top heights and precipitation displays significant discrepancies between the two regions. It is because that the aerosol invigoration effect is less efficient on the TP DCSs, mainly attributed to the significantly colder cloud base. Due to competition between invigoration and direct/semi-direct radiative effects of aerosols, the correlation between precipitation and aerosols over the TP is not obvious. However, precipitation in the TO experiences invigoration followed by suppression with increasing aerosols, due to the dominance of aerosol radiative effects and enhancement entrainment under polluted conditions.

How to cite: Zhao, Y., Li, J., Wen, D., Li, Y., Wang, Y., and Huang, J.: Distinct structure, radiative effects, and precipitation characteristics of deep convection systems in the Tibetan Plateau compared to the tropical Indian Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1291, https://doi.org/10.5194/egusphere-egu25-1291, 2025.

EGU25-1885 | Posters on site | AS3.11

Submicron-size aerosol scavenging by electro-collection and ice nucleation 

Vladan Vučković, Dragana Vujović, Darko Savić, and Lazar Filipović

In this study, we investigated how submicron aerosol particles (APs) are scavenged by cloud droplets and raindrops, including the effects of ice nucleation on these particles. We used an original two-moment aerosol scheme, which contains the prognostic equations for the number and mass of APs in the air and in all types of hydrometeors. This scheme was integrated into a three-moment microphysics scheme within a three-dimensional, non-hydrostatic Advanced Regional Prediction System (ARPS) model (Vučković et al. 2022, 2023).

We analyzed the scavenging of APs through electroscavenging processes, which involve Coulomb interactions with raindrops and both Coulomb and image charge interactions with cloud droplets. We assumed a Boltzmann charge distribution of aerosols, while cloud droplets and raindrops can possess either positive or negative charges in an amount that depends on their surface area. The kernels calculated for discrete bins of APs and droplets/drops are incorporated into the bulk microphysical scheme.

Ice nucleation on the APs is also considered a scavenging mechanism. This approach allows us to analyse how these processes impact the number and mass of APs in the atmosphere, hydrometeors, and those washed out by precipitation. Our results indicate that electroscavenging is the dominant process for medium to large submicron APs, whereas Brownian diffusion primarily affects smaller particles. Nucleation scavenging caused by depositional nucleation on atmospheric particles (APs) is identified as the primary mechanism for nucleation scavenging involving APs. This process is especially significant for reducing mass, while it plays a lesser role in decreasing the number of APs in the atmosphere.

Electrostatic collection by cloud droplets and raindrops enhance the scavenging of APs regardless of their charge sign, and the presence of image charges on cloud droplets further increases this collection. Increasing the charge on hydrometeors correlates with a greater number and mass of aerosol particles removed. The sign of the charge is less significant: our findings show that even when droplets are uncharged, the collection efficiency is still high. Depositional nucleation scavenging is identified as the most important mechanism for reducing the mass of APs (Vučković et al. 2024).

This approach provides valuable insights into the redistribution of APs between the atmosphere, hydrometeors and precipitation. The results are applicable to issues related to air pollution, cloud modification, and climate modelling.

 

Acknowledgement: This research was supported by the Science Fund of the Republic of Serbia, No. 7389, Project Extreme weather events in Serbia - analysis, modelling and impacts” – EXTREMES

 

References

 

Vučković, V., D. Vujović, and A. Jovanović, 2022: Aerosol parameterisation in a three-moment microphysical scheme: Numerical simulation of submicron-sized aerosol scavenging. Atmos Res, 273, 106148, https://doi.org/10.1016/j.atmosres.2022.106148.

Vučković, V., D. Vujović, and D. Savić, 2023: Influence of electrostatic collection on scavenging of submicron-sized aerosols by cloud droplets and raindrops. Aerosol Science and Technology, 57, https://doi.org/10.1080/02786826.2023.2251551.

Vučković, V., D. Vujović, D. Savić, and L. Filipović, 2024: Impact of electro-collection and ice nucleation on aerosol scavenging. Aerosol Science and Technology, https://doi.org/10.1080/02786826.2024.2441289.

How to cite: Vučković, V., Vujović, D., Savić, D., and Filipović, L.: Submicron-size aerosol scavenging by electro-collection and ice nucleation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1885, https://doi.org/10.5194/egusphere-egu25-1885, 2025.

EGU25-1987 | ECS | Posters on site | AS3.11

Assessment of the Cloud Seeding Efficiency over Tom Green County Texas, USA 

Marya Al Homoud, Stavros-Andreas Logothetis, Yosra SR Elnaggar, and Ashraf Farahat

The efficiency of cloud seeding in enhancing precipitation is a subject of active debate within the scientific community. This work examines the impacts of cloud seeding in changing cloud properties and dynamics over Tom Green County in West Texas, USA, from 2015 to 2020. Several cloud categories including small, large, and type B are considered. The effect of cloud-seeding missions in changing clouds’ lifetime, area, volume, and precipitation mass is investigated. The results show that the average increase in the lifetime of small, large, and type B is 53.6, 27, and 3.5%, respectively, while the average area increased by 47.1, 27.5, and 5.0% respectively, and their average volume increased by 63.6, 33, and 5.6% respectively. A significant increase in the precipitation mass of the small, large, and type B clouds is observed after the seeding missions. From 2015 to 2020, the precipitation rates in seeded clouds are higher than the unseeded clouds. Comparing precipitation rates during the 2015–2020 cloud-seeding campaigns to the period from 2010 to 2014 before the campaigns shows no trend of increasing precipitation except during 2015 and 2016.

How to cite: Al Homoud, M., Logothetis, S.-A., SR Elnaggar, Y., and Farahat, A.: Assessment of the Cloud Seeding Efficiency over Tom Green County Texas, USA, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1987, https://doi.org/10.5194/egusphere-egu25-1987, 2025.

EGU25-2046 | ECS | Posters on site | AS3.11

 Urban-Rural differences in characteristics for Shallow Clouds observed over Chennai, a tropical megacity in India 

Sougat Kumar Sarangi, Chandan Sarangi, Niravkumar Patel, Saleem Ali, Athira Karimpuzha Ramadas, Anouksha Hemanth, and Sanjay Kumar Mehta

Shallow clouds significantly influence the Earth's radiative balance by modulating incoming and outgoing shortwave radiation. The formation and characteristics of shallow clouds are closely coupled with the land-atmosphere interactions and hence urbanization can have a distinct impact on the occurrence of shallow clouds. This study investigates the occurrence and radiative properties of shallow clouds using simultaneous observations of mini–Micro-Pulsed Lidar (MPL), pyranometers and a network of sky imager over Chennai. These observations span over four sites across Chennai, representing a mix of urban and semi-urban microenvironments, during the months of January and February. Largely, shallow clouds are having a mean cloud base height of 800-1000 m and a mean cloud thickness of 250-300 m. Mean cloud radiative forcing (CRF) of -200 W/m², confirms the strong cooling effect of shallow clouds. The diurnal variation of hourly averaged cloud fraction (CF) shows a peak of 0.3 around 10:00AM, followed by a gradual decline, consistent with the lifecycle of shallow clouds driven by local meteorological conditions, including temperature and humidity fluctuations. A strong negative correlation (r = -0.95) was observed between CF and CRF, highlighting enhanced cooling effects of shallow clouds with increasing CF. The detailed differences in CRF, CF and cloud albedo from the three additional sites spanning the urban to rural transect across the city will be discussed. Observational findings will provide valuable empirical data for refining cloud-climate interactions over urban environments in northeast monsoon region.

How to cite: Kumar Sarangi, S., Sarangi, C., Patel, N., Ali, S., Karimpuzha Ramadas, A., Hemanth, A., and Kumar Mehta, S.:  Urban-Rural differences in characteristics for Shallow Clouds observed over Chennai, a tropical megacity in India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2046, https://doi.org/10.5194/egusphere-egu25-2046, 2025.

EGU25-2136 | ECS | Orals | AS3.11

Impact of Land Use Changes during Agricultural Cycles on AOD Trends over the Indo-Gangetic Plain during Last Two Decades 

Rohit Kumar Singh and Achanta Naga Venkata Satyanarayana

Rapid urbanization and industrialization lead to significant changes in land use and land cover (LULC), particularly in agricultural activities over the Indo-Gangetic Plain (IGP), which in turn impacts the distribution of aerosol loading. In the present study, climatological and spatio-temporal trends of aerosol optical depth (AOD) and aerosol sources are investigated over the IGP region from 2001 to 2022. Climatological analysis of the AOD over the upper, central, and lower IGP regions was conducted using satellite-based MODIS data. LULC analysis over the IGP region during the study period showed a significant increase in crop land and built-up area, mainly replacing the vegetation. It is hypothesized that changes in LULC patterns, especially the expansion of cropland and crop residue burning (CRB), are major drivers of aerosol trends. The results reveal significant AOD increases, particularly in the lower IGP, which experienced extensive vegetation loss replaced by cropland, intensifying CRB and aerosol emissions. In contrast, the upper IGP exhibited reduced CRB activity and even declining AOD trends during the second half of the study period (2012–2022), indicating improved air quality. The findings highlight a direct relationship between LULC changes, CRB, and AOD trends, emphasizing the need for sustainable agricultural practices and emission control measures to mitigate aerosol pollution and improve air quality across the IGP.

How to cite: Kumar Singh, R. and Satyanarayana, A. N. V.: Impact of Land Use Changes during Agricultural Cycles on AOD Trends over the Indo-Gangetic Plain during Last Two Decades, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2136, https://doi.org/10.5194/egusphere-egu25-2136, 2025.

EGU25-2203 | Orals | AS3.11

Surface-tension lowering of aerosols by organics in urban atmospheres: implication to cloud condensation nuclei prediction 

Tianyi Fan, Jingye Ren, Chenxi Liu, Zhanqing Li, Jieyao Liu, Yele Sun, Yuying Wang, Xiaoai Jin, and Fang Zhang

Surface-active organics lower the aerosol surface tension (σs/a), leading to enhanced cloud condensation nuclei (CCN) activity and potentially exerting impacts on the climate. Quantification of σs/a is mainly limited to laboratory or modeling work for particles with selected sizes and known chemical compositions. Inferred values from ambient aerosol populations are deficient. In this study, we propose a new method to derive σs/a by combining field measurements made at an urban site in northern China with the κ-Köhler theory. The results present new evidence that organics remarkably lower the surface tension of aerosols in a polluted atmosphere. Particles sized around 40 nm have an averaged σs/a of 53.8 mN m-1, while particles sized up to 100 nm show σs/a values approaching that of pure water. The dependence curve of σs/a with the organic mass resembles the behavior of dicarboxylic acids, suggesting their critical role in reducing the surface tension. The study further reveals that neglecting the σs/a lowering effect would result in lowered ultrafine CCN (diameter < 100 nm) concentrations by 6.8% to 42.1% at a typical range of supersaturations in clouds, demonstrating the significant impact of surface tension on the CCN concentrations of urban aerosols.

How to cite: Fan, T., Ren, J., Liu, C., Li, Z., Liu, J., Sun, Y., Wang, Y., Jin, X., and Zhang, F.: Surface-tension lowering of aerosols by organics in urban atmospheres: implication to cloud condensation nuclei prediction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2203, https://doi.org/10.5194/egusphere-egu25-2203, 2025.

This study investigates the hydro-climatic changes in the Central-South Asia and Tibetan Plateau (CSATP) region under two future scenarios: high greenhouse gas emissions (SSP5-8.5) and the combined impact of greenhouse gases with stratospheric aerosol intervention (SAI). Using model simulations, we analyze key variables such as total water storage (TWS), temperature (TMP), precipitation (PCP), real evapotranspiration (RET), soil moisture (SM), and leaf area index (LAI) over the historical period (1985–2014) and the future period (2071–2100). The SSP5-8.5 scenario projects a significant increase in temperature, RET, precipitation extremes, and reductions in TWS, SM, and LAI, reflecting the adverse effects of unmitigated global warming. Conversely, the SSP5-8.5+SAI scenario demonstrates the potential to moderate these impacts. SAI reduces temperature anomalies and precipitation extremes while stabilizing RET, SM, and LAI levels. Results reveal region-specific responses; for instance, in the Tibetan Plateau, significant temperature and precipitation variability reductions are observed under SAI, highlighting its role in mitigating climate extremes. Similarly, soil moisture and TWS exhibit more stable trends under SAI than in the SSP-only scenario, underscoring its effectiveness in counteracting warming-induced drying trends. Overall, the findings underscore the critical role of SAI in alleviating the adverse hydro-climatic impacts of greenhouse gas emissions. While SAI does not entirely negate these impacts, it provides a viable pathway for reducing extremes and fostering climate stability in vulnerable regions. This study contributes to understanding the implications of climate engineering as a complementary strategy for climate adaptation in the CSATP region.

How to cite: Hussain, I., Hussain, A., and Rezaei, A.: Future hydro-climatic changes in Central-South Asia and Tibetan Plateau in response to global warming and stratospheric aerosol intervention scenarios, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2246, https://doi.org/10.5194/egusphere-egu25-2246, 2025.

EGU25-2298 | ECS | Posters on site | AS3.11

Resources on SRM Science for New Researchers 

Sam Kaufmann, Jean-François Lamarque, and Alex Wong

There is a recognized urgent need for broadening and coordinating access to scientific information regarding Solar Radiation Modification (SRM) to support evidence-based decision making. To build such capacity, the research community has expressed the need for accessible and searchable metadata about modeling studies of SRM and associated impacts.

For this purpose, we have put together a prototype for a Repository, which is an extensive collection of peer-reviewed articles of Earth System Models (ESMs) simulations whose outputs have been used by impacts studies, and impacts studies that have used ESM data outputs. In its current version, the repository offers a list of peer-reviewed journal articles, with specific meta-data such as specific information on climate models, scenarios or impact targets used to simulate SRM, in order to enable users with the ability to identify the most relevant studies to their own research. The repository is accompanied by a Guide targeted at new entrants to the field, such as graduate students and established researchers conducting their first SRM studies. The Guide offers a narrative description of ESM experiments available for SRM impacts research today and reviews current limitations, uncertainties, and gaps that remain unaddressed. These resources will be freely available online.

How to cite: Kaufmann, S., Lamarque, J.-F., and Wong, A.: Resources on SRM Science for New Researchers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2298, https://doi.org/10.5194/egusphere-egu25-2298, 2025.

The 26th United Nations Climate Change Conference (COP26) proposes to limit global warming to <1.5 °C above pre-industrial levels until 2030 and aligns CO2 emissions with net-zero by 2050. To achieve this goal, it is crucial to replace fossil fuels with renewable and clean energy sources. Among the various renewable energy sources, solar energy undoubtedly stands out as an attractive option. Future meteorological conditions and emission reductions are expected to impact on solar energy potential. Consequently, the Weather Research and Forecasting model with chemistry (WRF-Chem) was applied to current (2016–2020) and future (2046–2050) under the shared socio-economic pathways (SSP) 2–4.5 scenario to investigate the impact of future meteorological conditions and emission reductions on solar energy potential. The evaluation of the WRF-Chem demonstrates satisfactory performance in capturing most meteorological and chemical variables at a climatological scale. However, the model underestimates 2 m temperature while overestimating 2 m specific humidity and 10 m wind speed, with mean bias (MB) of -0.1°C, 1.4 g kg-1, and 0.8 m s-1, respectively. Additionally, the WRF-Chem overestimates PM2.5, with normalized mean bias (NMB) of -20%. The model underestimates cloud fraction and precipitation caused by the limitation in the cloud microphysical parameterization. The model well reproduced the solar energy distribution in China, with R of 0.76 and NMB of -3%. Looking ahead, the future annual average solar energy increases by 2.2, 0.1, 2, 4.1, 1.9, and 2.9 W m-2 for China, Beijing-Tianjin-Hebei, Fenwei Plain, Yangtze River Delta, Pearl River Delta, and Sichuan Basin, respectively. The future annual average photovoltaic potential increase by 1–4% in these regions. This increase is primarily attributed to the increase in solar energy resulting from emission reductions (4.7, 5.1, 5.0, 4.7, 3.2, and 6.1 W m-2), which outweighs the decrease caused by meteorological conditions (2.5, 5.0, 2, 4.1, 1.9, and 2.9 W m-2). Hence, emission reduction plays a vital role in promoting solar energy utilization.



How to cite: Gao, Y., Zhang, Y., and Zhang, M.: Assessment of future solar energy potential changes under the shared socio-economic pathways scenario 2–4.5 with WRF-chem: The roles of meteorology and emission, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2412, https://doi.org/10.5194/egusphere-egu25-2412, 2025.

EGU25-2559 | ECS | Orals | AS3.11

Regional to global impacts of boreal biomass burning emissions changes: a multi-model study 

Zosia Staniaszek, Bjørn Samset, Marianne T Lund, and Annica Ekman

Wildfire activity in boreal regions is changing, due to climate change and other anthropogenic drivers. Given the high climate sensitivity of the Arctic and boreal regions, it is important to explore the impacts of these changes. There are also region-specific impacts of biomass burning particular to high latitude regions, such as black carbon (BC) deposition on snow. While many sources of atmospheric pollutions are being mitigated, fires are emerging as a growing contributor to poor air quality, both locally to the fire emissions source and across wider regions.

Here we investigate the climate and atmospheric impacts of several idealised biomass burning perturbations, focusing on aerosols. We present initial results from a new set of multi-model experiments (including CESM2, NorESM2 and EC-Earth), where biomass burning emissions are perturbed in several idealised experiments. The species concerned are: BC, SO4, organic carbon, SO2, DMS, and secondary organic aerosol precursors. We first perturb all boreal biomass burning emissions, and then smaller regions of interest individually (boreal North America, East Siberia and West Siberia). These experiments use 2005-2014 as a baseline period, and use the sum of this period as the perturbation, giving an approximately x10 perturbation in the regions of interest, in both fixed SST (30 years) and coupled (200 years) simulations. The strength and location of the aerosol changes studied here (when comparing aerosol optical depth) are comparable to the recent trends in aerosols between 2015-2024 and 2005-2014.

We will present the modelled atmospheric composition response both globally and in the focus regions described above, including teleconnections to other regions. This includes aerosol optical depth, aerosol absorption, and a breakdown by aerosol species. We will also highlight the climate response to the biomass burning perturbations, including effective radiative forcing (ERF) and fully-coupled climate response estimates.

How to cite: Staniaszek, Z., Samset, B., Lund, M. T., and Ekman, A.: Regional to global impacts of boreal biomass burning emissions changes: a multi-model study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2559, https://doi.org/10.5194/egusphere-egu25-2559, 2025.

EGU25-2741 | ECS | Posters on site | AS3.11

Role of aerosols in modulating the convection over the South China Sea associated with boundary layer clouds during boreal winter 

Ushnanshu Dutta, Chung-Kai Wu, and Jen-Ping Chen

During the winter monsoon, a high-pressure ridge extends from Siberia to the northern South China Sea (SCS). This system brings northeasterly cold air, which rises over the warm sea surface of the SCS, causing atmospheric instability and frequent convection over the region. This continental cold-air outbreak also forms cloud streets over the northwestern Pacific. In this study, we investigated the effects of aerosol-cloud interactions over the upstream northwestern Pacific (e.g., the East China Sea) on convective activity in the downstream tropical area (e.g., the South China Sea). To achieve this, we selected two distinct cases associated with boundary layer clouds and conducted sensitivity experiments using different aerosol types—such as anthropogenic or continental, oceanic, and mixed aerosols—to simulate convection characteristics over the SCS. For our analysis, we employed the aerosol-sensitive National Taiwan University (NTU) multimoment microphysical scheme coupled with the Weather Research and Forecasting (WRF) model. Our results indicate that the thermal and moisture properties of the winter cold-air mass reaching the SCS and tropical oceans can be significantly influenced by anthropogenic aerosols produced over the East Asian continent. We also examined variations in orographic rainfall patterns over different regions, such as northeastern Taiwan and coastal Vietnam, in relation to these boundary layer clouds and their sensitivity to the choice of aerosol types. This study highlights the importance of using a multimoment microphysical scheme capable of accounting for diverse aerosol types to improve simulation accuracy with the WRF model.

Keywords: Aerosol-cloud interaction, South China Sea, Boundary layer clouds, WRF

How to cite: Dutta, U., Wu, C.-K., and Chen, J.-P.: Role of aerosols in modulating the convection over the South China Sea associated with boundary layer clouds during boreal winter, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2741, https://doi.org/10.5194/egusphere-egu25-2741, 2025.

EGU25-2980 | ECS | Posters on site | AS3.11

Constrained changes in future diurnal cloud pattern cause stronger ocean warming and radiation imbalance 

Yang zhao, Jiming Li, Shanshan Wang, Yuan Wang, and Yang Wang

Diurnal cloud pattern (DCP) determines total clouds’ impacts on Earth’s radiation balance in one day and is sensitive to climate change. Changes in DCP affect diurnal cycle of radiation and temperature, leading to obvious impacts on vegetation growth and human health, but with less attention and large projection spread. Here we show that future changes in cloud is significantly linked to present-day clouds’ climatology, reducing uncertainty by 60%-70% over typical regions. Under warming climate, various long-term trends in cloud fraction (CF) at different times determine the DCP changes. There are largely decreased noon and lightly changed night CF for most land, while distinct CF reduction at all times but more sever in the afternoon for ocean. Therefore, maritime (continental) area has enhanced (attenuate) amplitude, i.e., daily cloud variation rate, and more (less) shift of DCP. These DCP changes with significant CF deviation would reduce net cloud radiative (cooling) effect, amplifying surface warming. Especially, tremendous daily net radiative warming (exceeding 100 Wh/m2) occurs in extensive midlatitude ocean domain due to remarkable afternoon CF reduction.

How to cite: zhao, Y., Li, J., Wang, S., Wang, Y., and Wang, Y.: Constrained changes in future diurnal cloud pattern cause stronger ocean warming and radiation imbalance, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2980, https://doi.org/10.5194/egusphere-egu25-2980, 2025.

EGU25-3245 | ECS | Orals | AS3.11

Investigating a double moment, fully coupled aerosol-cloud model over the Amazon 

Joseph Carton-Kelly, Anthony Jones, and Paul Field

We have developed a double moment aerosol model appropriate for numerical weather prediction (NWP) within the Met Office’s Unified Model framework. Our aerosol model (Sol-Insol) is fully coupled to a double moment cloud microphysics model (CASIM) permitting aerosol-cloud interactions to be resolved at high-resolution. As a test we investigate how our setup performs against traditional ACI parametrizations used for NWP by comparing model results to observations from the Café-Brazil field campaign over the Amazon. Our simulations contribute to the CleanCloud model intercomparison project (MIP) aimed at improving aerosol-cloud interactions across timescales. As a case study, we use 14th January 2023, a date selected due to HALO aircraft observations being recorded alongside a pronounced mesoscale squall line.

The MIP protocol sets out 3 regional domains surrounding the ATTO site - a 6.6km resolution grid over the Northern part of South America into Central America, a 3.3km resolution grid inside this and then a 1.6km resolution grid covering the Amazon. Three model configurations were selected to isolate the impacts of aerosol on cloud and precipitation: a control run with no aerosol scheme, fixed cloud CDNC and a Cooper ICNC vs T relation (CONTROL); a coupled aerosol-cloud run with arbitrary initialised aerosols (ARB-AER); and a coupled aerosol-cloud run with aerosol initialised to CAMS reanalysis data (CAM-AER).

We constrain the simulated aerosol, cloud and radiation properties using a range of co-located satellite, surface (ATTO) and air (HALO) observations. Our results show that initialising the aerosol to CAMS reanalysis concentrations leads to slightly improved results relative to CONTROL while ARB-AER performs significantly worse when looking at observed top of the atmosphere radiation, highlighting the high sensitivity of cloud to ambient aerosol. Further experiments comparing ground and flight observations to model metrics help to support the conclusion that CAM-AER is performing better than ARB-AER and highlights potential improvements to NWP hydro-forecasts from using realistic aerosol properties.

How to cite: Carton-Kelly, J., Jones, A., and Field, P.: Investigating a double moment, fully coupled aerosol-cloud model over the Amazon, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3245, https://doi.org/10.5194/egusphere-egu25-3245, 2025.

EGU25-3333 | Posters on site | AS3.11

Towards Understanding Biases in Cloud Radiative Effects Simulated in E3SMv3 

Yuying Zhang, Shaocheng Xie, Ryutaro Christopher Terai, Wuyin Lin, Jean-Christophe Golaz, Meng Zhang, Yun Qian, and Qi Tang

This study systematically evaluates clouds and their radiative impacts in the newly released U. S. Department of Energy (DOE)’s Energy Exascale Earth System Model (E3SM) version 3 using both satellite data and the DOE Atmospheric Radiation Measurement (ARM) program’s ground-based measurements. The comparison is done by utilizing the Cloud Feedback Model Intercomparison Project (CFMIP) Observation Simulator Package (COSP) and the ground-based lidar and radar simulator package, the Earth Model Column Collaboratory (EMC^2), to improve the model-observation cloud comparison. The use of detailed ARM cloud observations is to better diagnose the strengths and deficiencies of E3SM through process-level understanding. Compared to its earlier versions, E3SMv3 has significantly updated its atmospheric physical parameterizations including noticeable improvements in representing cloud and convective processes. These include the use of the Predicted Particle Properties (P3) scheme for stratiform clouds to improve the treatment of ice microphysical processes and aerosol-cloud interactions and a more sophisticated two-moment bulk cloud microphysics scheme for the Zhang-McFarlane (ZM) deep convection. In addition, mesoscale heating from organized convection is added on top of the ZM deep convective heating. The interactions of deep convection with its environment are enhanced. Several carefully defined sensitivity tests are conducted by tuning off each of the major changes relevant to clouds and convection to isolate their individual impacts on simulation of clouds. Detailed results will be presented in the meeting.

How to cite: Zhang, Y., Xie, S., Terai, R. C., Lin, W., Golaz, J.-C., Zhang, M., Qian, Y., and Tang, Q.: Towards Understanding Biases in Cloud Radiative Effects Simulated in E3SMv3, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3333, https://doi.org/10.5194/egusphere-egu25-3333, 2025.

EGU25-3346 | ECS | Posters on site | AS3.11

Air Mass Patterns for Deep Convective Clouds over Poland in the first and second generation Meteosat retrievals 

Izabela Wojciechowska and Andrzej Kotarba

Deep Convective Clouds (DCCs) are associated with severe weather, where ‘severity’ refers to the potential negative impact of weather systems on human safety and the economy. As a natural hazard, convective storms need to be incorporated into mitigation plans, which is particularly important for mid-latitudes. Additionally, in a warming climate, extreme events are expected to occur more frequently. Motivated by the lack of DCC-focused air mass studies, this work evaluates how changes in circulation (air mass location and transport) relate to DCC activity over Poland.

The two generations of Meteosat observations provide a unique data record for studying the atmosphere and climate variability over Europe since the 1980s. Meteosat data enable the detection and, in a basic form, the tracking of DCCs, but the monitoring is limited to the lifetime of DCCs. While Meteosat data allow for the tracking of DCCs to some extent, identifying and following the air mass associated with their formation is not feasible using Meteosat data alone. One approach to overcoming this obstacle is to track air parcel transport in the atmosphere—i.e., calculating air parcel trajectories.

In this research, we identify cases of Deep Convective Clouds over Poland using the bi-spectral threshold method for DCC detection, which assesses differences in Brightness Temperature (BT) between infrared and water vapor channels. Our analysis is based on Meteosat Visible Infra-Red Imager (MVIRI) and Spinning Enhanced Visible Infra-Red Imager (SEVIRI) retrievals from the summer season of 2005. Thereafter, for each observation time, we determine which cells of a 0.25°×0.25° grid over Poland can be classified as having DCCs present and calculate the backward trajectory of the air mass for the center of each grid cell. For tracking purposes, we use the HYbrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model, a widely recognized tool developed by the National Oceanic and Atmospheric Administration (NOAA) Air Resources Laboratory. The study examines air mass patterns associated with deep convective clouds forming over Poland and addresses the question: What are the dominant air mass sources and transport pathways leading to the formation of DCCs over Poland?

This research was funded by the National Science Centre of Poland. Grant no. UMO-2023/49/N/ST10/00366.

How to cite: Wojciechowska, I. and Kotarba, A.: Air Mass Patterns for Deep Convective Clouds over Poland in the first and second generation Meteosat retrievals, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3346, https://doi.org/10.5194/egusphere-egu25-3346, 2025.

EGU25-3708 | Orals | AS3.11

On the Processes Determining the Slope of Cloud-Water Adjustments in Non-Precipitating Stratocumulus 

Fabian Hoffmann, Yao-Sheng Chen, and Graham Feingold

Cloud-water adjustments are a part of aerosol-cloud interactions, affecting the ability of clouds to reflect shortwave radiation by processes altering the vertically integrated cloud water content L in response to changes in the droplet concentration N. In this study, we utilize a simple entrainment parameterization for mixed-layer models to determine entrainment-mediated cloud-water adjustments in non-precipitating stratocumulus. At lower N, L decreases due to an increase in entrainment in response to an increase in N suppressing the stabilizing effect of evaporating precipitation (virga) on boundary layer dynamics. At higher N, the cessation of cloud-droplet sedimentation sustains more liquid water at the cloud top, and hence stronger preconditioning of free-tropospheric air, which increases entrainment with N. Overall, cloud-water adjustments are found to weaken distinctly from dln(L)/dln(N) = -0.48 at = 100 cm-3 to -0.03 at = 1000 cm-3, indicating that a single value to describe cloud-water adjustments in non-precipitating clouds is insufficient. Based on these results, we speculate that cloud-water adjustments at lower N are associated with slow changes in boundary layer dynamics, while a faster response is associated with the preconditioning of free-tropospheric air at higher N.

How to cite: Hoffmann, F., Chen, Y.-S., and Feingold, G.: On the Processes Determining the Slope of Cloud-Water Adjustments in Non-Precipitating Stratocumulus, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3708, https://doi.org/10.5194/egusphere-egu25-3708, 2025.

EGU25-3965 | Posters on site | AS3.11

Aerosol-cloud interactions near cloud base deteriorating the haze pollution in East China 

Ximeng Qi, Caijun Zhu, Liangduo Chen, Xuguang Chi, Jiaping Wang, Guangdong Niu, Shiyi Lai, Wei Nie, Yannian Zhu, Xin Huang, Tom V. Kokkonen, Tuukka Petäjä, Veli-Matti Kerminen, Markku Kulmala, and Aijun Ding

Atmospheric aerosols not only cause severe haze pollution, but also affect climate through changes in cloud properties. However, during the haze pollution, aerosol-cloud interactions are not well understood due to a lack of in-situ observations. In this study, we conducted simultaneous observations of cloud droplet and particle number size distribution, together with supporting atmospheric parameters, from ground to cloud base in East China using a high-payload tethered airship. We found that high concentrations of aerosols and cloud condensation nuclei were constrained below cloud, leading to the pronounced “Twomey effect” near the cloud base. The cloud inhibited the pollutants dispersion by reducing surface heat flux and thus deteriorated the near-surface haze pollution. Satellite retrievals matched well with the in-situ observations for low stratus clouds, while were insufficient to quantify aerosol-cloud interactions for other cases. Our results highlight the importance to combine in-situ vertical and satellite observations to quantify the aerosol-cloud interactions.

How to cite: Qi, X., Zhu, C., Chen, L., Chi, X., Wang, J., Niu, G., Lai, S., Nie, W., Zhu, Y., Huang, X., Kokkonen, T. V., Petäjä, T., Kerminen, V.-M., Kulmala, M., and Ding, A.: Aerosol-cloud interactions near cloud base deteriorating the haze pollution in East China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3965, https://doi.org/10.5194/egusphere-egu25-3965, 2025.

EGU25-4280 | ECS | Orals | AS3.11

Indian Summer Monsoon Response to Regional Aerosol Emission Changes: RAMIP insights 

Ankit Bhandekar, Bryan Lawrence, Luke Abraham, Fiona O’Connor, and Chris Maynard and the RAMIP Team

Anthropogenic aerosol emissions are projected to decline significantly by 2050, with major implications for regional climate. However, unlike greenhouse gases, aerosol impacts are spatially heterogeneous and can influence climate both near emission sources and through remote teleconnections. This is particularly important for the Indian monsoon system, where both local and remote aerosol changes can significantly affect precipitation patterns.

Using the Regional Aerosol Model Intercomparison Project (RAMIP) framework, we examine how local and remote aerosol emission changes influence Indian climate across both pre-monsoon and monsoon seasons. Our analysis employs 10-member ensembles from multiple CMIP6-era models to compare three experiments: Global, South Asian, and East Asian aerosol reductions relative to a high-emission baseline (SSP3-7.0). This experimental design allows us to isolate and quantify the distinct impacts of regional emission changes. Initial results reveal that global aerosol reductions lead to more widespread and intense precipitation changes compared to regional reductions alone, with South Asian aerosol reductions largely mirroring the global response pattern while East Asian emissions play an additional role in modulating monsoon circulation. The Western Ghats and Indo-Gangetic Plains show particularly strong responses. We find significant inter-model diversity in the spatial patterns and magnitudes of these changes, highlighting key areas of uncertainty in aerosol-monsoon interactions. Through detailed analysis of circulation patterns and moisture transport, we investigate the mechanisms driving these precipitation responses and their implications for future climate projections.

Our findings provide insights into the complex relationship between regional aerosol emissions and monsoon dynamics, with important implications for both climate prediction and air quality management in South Asia.

How to cite: Bhandekar, A., Lawrence, B., Abraham, L., O’Connor, F., and Maynard, C. and the RAMIP Team: Indian Summer Monsoon Response to Regional Aerosol Emission Changes: RAMIP insights, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4280, https://doi.org/10.5194/egusphere-egu25-4280, 2025.

EGU25-4312 | ECS | Posters on site | AS3.11

Impacts of reductions in non-methane short-lived climate forcers on future droughts 

Tianhui Zhou and Massimo Bollasina

Droughts, prolonged periods of deficient precipitation and heightened evapotranspiration, pose severe threats to water resources, ecosystems, and socioeconomic well-being worldwide. While previous research has established that the continuous growth of greenhouse gas (GHG) emissions is a primary driver of global warming and the associated intensification of the hydrological cycle, the role of non-methane near-term climate forcers (NTCFs), including anthropogenic aerosols, in modulating drought risk remains less clearly understood. In particular, the complex interplay between aerosol-induced radiative cooling and greenhouse warming can produce non-linear drought responses at regional scales, notably in arid and semi-arid regions.

In this study, we employ seven Earth System Models (ESMs) participating in the Phase 6 of the Coupled Model Intercomparison Project (CMIP6) to investigate the specific contributions of NTCFs emission reduction to the evolution of drought characteristics (i.e., frequency, duration, and severity) under the SSP3-7.0 scenario. Droughts are identified by using the Standardized Precipitation Evapotranspiration Index (SPEI) at multiple timescales (3, 6, and 12 months). 

Results reveal considerable spatial heterogeneity in the responses of drought metrics. Reductions in NTCFs generally lead to cooler temperatures and, in many tropical and mid-latitude regions, enhanced precipitation. For parts of southern Africa and South America, these changes translate into fewer and shorter droughts under the SSP3-7.0-lowNTCF scenario compared to SSP3-7.0. By contrast, arid and semi-arid regions such as the Sahara and West Asia exhibit a worsening of drought conditions—drought events become more frequent, severe, and prolonged. These outcomes indicate that aerosol-related cooling and its impact on atmospheric circulation may, in some regions, help maintain or strengthen rainfall, so that reducing aerosols can inadvertently diminish that effect and exacerbate water deficits. Indeed, our multi-model ensemble suggests heightened water stress in the Sahara and West Asia under the SSP3-7.0-lowNTCF scenario, underscoring how local feedbacks and large-scale circulation patterns can alter the hydrological response to emission mitigation.

Overall, our findings highlight the non-linear and regionally dependent effects of NTCF mitigation on drought risk. In many regions, curtailing aerosol and ozone-precursor emissions offers co-benefits for air quality and climate adaptation by decreasing drought likelihood; however, arid and semi-arid areas may face more severe drought outcomes.

How to cite: Zhou, T. and Bollasina, M.: Impacts of reductions in non-methane short-lived climate forcers on future droughts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4312, https://doi.org/10.5194/egusphere-egu25-4312, 2025.

Aerosol perturbations primarily affect albedo (Bellouin et al., 2019) by scattering a fraction of insolation back into space. Specifically, aerosol emissions enhance cloud formation and cloud cover, which directly increase albedo.

To investigate this effect, we analyze CMIP6 data from a set of experiments conducted using models with robust aerosol modules. Our focus is on variables such as cloud droplet number concentration, which reflect aerosol emissions, and cloud fraction, as well as their correlation with the shortwave radiative flux at the top of the atmosphere.

To achieve this, we apply a Random Forest Regression to the dataset, enabling a more precise quantification of the impact of aerosol-cloud interactions on the atmosphere’s radiative balance

How to cite: Clement, N.:  Impact of aerosol-cloud interaction on aerosol effective radiative forcing revealed by a Random Forest Regression over CMIP6 data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5943, https://doi.org/10.5194/egusphere-egu25-5943, 2025.

EGU25-6015 | Orals | AS3.11

Distinct climate responses to regional aerosol emissions 

Laura Wilcox, Bjørn Samset, Camilla Stjern, and Robert Allen and the RAMIP Team

Anthropogenic aerosol emissions have had a major influence on global climate over the industrial era, counteracting some of the warming and precipitation increases due to rising greenhouse gas concentrations. These greenhouse gas driven changes are now rapidly being unmasked, through a range of national and regional policies aimed at improving air quality. However, unlike greenhouse gases, aerosol emissions have strongly regional response patterns, and influence the climate both near to, and far from emission sources. These regional influences have to date not been quantified in a consistent, multi-model framework.

Here, we present results from the Regional Aerosol Model Intercomparison Project (RAMIP). Ten CMIP6 era models have performed 10- member ensemble simulations investigating the climate response to aerosol emissions, separately, from South Asia, East Asia, Africa and the Middle East, and Europe and North America. All RAMIP experiments are based on two CMIP6-era SSPs: SSP3-7.0 (strong GHG increases, minimal aerosol reductions) and a hybrid SSP370-126aer (anthropogenic emissions of SO2, organic carbon, and black carbon are rapidly reduced following SSP1-2.6, either globally or regionally).

We find a rapid surface warming in response to aerosol reductions, and strong precipitation increases, but with marked regional differences in the magnitude of the response. While there are many robust responses, strong inter-model differences in the pattern and strength of the responses in some regions highlights where aerosol related uncertainty is large in the near-future.

We discuss the linearity of the effective radiative forcing and climate responses from regional aerosol perturbations, and demonstrate that emission location is key to the amplitude and extent of the response. In particular, emission changes in East Asia and North America and Europe have a larger global temperature impact than those over South Asia due to their influence on Pacific clouds. This initial analysis demonstrates the need for aerosol awareness in the design of future scenario ensembles, and in climate risk and impact studies both near to and far from aerosol emission sources.

How to cite: Wilcox, L., Samset, B., Stjern, C., and Allen, R. and the RAMIP Team: Distinct climate responses to regional aerosol emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6015, https://doi.org/10.5194/egusphere-egu25-6015, 2025.

EGU25-6060 | Orals | AS3.11 | Highlight

Strong contribution of SO2 emissions reductions from China to global warming intensification since 2010 

Bjorn H. Samset, Laura J. Wilcox, and Robert J. Allen and the RAMIP team

The rate of global warming has seemingly increased since around 2010, relative to the previous 30-year period, leading up to the recent strong records in global surface temperature anomalies set in 2023 and 2024. Concurrently, Chinese emissions of SO2 have dropped dramatically as a consequence of strong national air quality policies. This has, in turn, led to marked reductions in atmospheric sulphate aerosol loadings over, and downwind from, the Chinese mainland, as well as strong improvements in air quality. To date, the contribution of Chinese emissions reductions to the intensification of global warming, through unmasking of greenhouse gas driven climate change, has however not been quantified.

Here, we use simulations from the Regional Aerosol Model Intercomparison Project (RAMIP) to investigate the climate response to strong reductions in Chinese SO2 emissions, closely analogous to real-world changes since 2010. We use 10-member ensembles of fully coupled simulations from ten CMIP6 era Global Climate Models, to quantify the global and regional, seasonally resolved influences on temperature and precipitation in a total of 100 ensemble members.

Overall, we find a warming due to recent reductions in SO2 emissions from China of 0.07 ± 0.05 ºC. Assuming that this has happened since 2010 leads to a warming rate of 0.05 ºC / decade. Recent observations of global surface temperature anomalies indicate a warming rate increase of 0.07 ºC / decade, when filtered for the effects of interannual variability in sea surface temperature patterns. Hence, our results indicate a strong contribution of aerosol emissions reductions to this elevated warming rate. This conclusion is supported by the geographical pattern of elevated warming, as well as correspondence between modelled and observed top-of-atmosphere radiative imbalance changes.

How to cite: Samset, B. H., Wilcox, L. J., and Allen, R. J. and the RAMIP team: Strong contribution of SO2 emissions reductions from China to global warming intensification since 2010, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6060, https://doi.org/10.5194/egusphere-egu25-6060, 2025.

EGU25-6413 | Posters on site | AS3.11

Simulation of Biomass Burning Events and Their Atmospheric Effects: A Study with WRF-Chem 

Douglas Lima de Bem, Vagner Anabor, Luiz Angelo Steffenel, Leonardo Brenner, Mauro Morichetti, and Umberto Rizza

In the Southern Hemisphere, regions in South America are recognized as significant sources of carbonaceous aerosols, which are produced by biomass burning. This type of burning typically occurs during the winter months, predominantly in the region known as the "Deforestation Arc," often associated with the expansion of agricultural and livestock production areas in Brazil.  Given the limited number of observations in this region, numerical modeling becomes essential for analyzing and accurately representing biomass burning events. In this context, the purpose of this study is to discretize the atmospheric behavior during fire events across South America by utilizing the Weather Research and Forecasting with Chemistry (WRF-Chem) model, thereby assessing the impact of these carbonaceous aerosols on cloud microphysics throughout the region. 

For this study, WRF-Chem version 4.3.1 was employed. The simulation began on September 28, 2007, and ended on October 3, 2007, using ERA5 fields to provide the initial and boundary conditions with a spatial resolution of 0.25°. The domain covered the South American region. Two simulations were conducted: the first, referred to as the control simulation (CTRL), had the coupling between aerosols, radiation, and cloud microphysics turned off, while the second, the fully coupled simulation (CPL), enabled both couplings. This approach facilitates a subsequent analysis to distinguish the role of aerosols on radiative properties and quantify the effects of coupling. For the analysis, precipitation fields, radiation components, and hydrometeor composition were evaluated in both simulations. This approach provides insights into the influence of biomass-burning aerosols on atmospheric processes and their role in modifying cloud microphysics and radiative balance.

How to cite: Lima de Bem, D., Anabor, V., Steffenel, L. A., Brenner, L., Morichetti, M., and Rizza, U.: Simulation of Biomass Burning Events and Their Atmospheric Effects: A Study with WRF-Chem, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6413, https://doi.org/10.5194/egusphere-egu25-6413, 2025.

EGU25-6953 | ECS | Orals | AS3.11

Sub-Saharan African Precipitation Responses to Aerosol Emission Changes 

Catherine Toolan, Andrew Turner, and Joe Adabouk Amooli and the RAMIP Team

Precipitation changes over sub-Saharan Africa linked to remote aerosol emissions have severely impacted agriculture, ecosystems, and livelihoods historically in the region. Established links between aerosol emissions and precipitation responses impact future projections of sub-Saharan precipitation, which remain uncertain due to differences in model representations of aerosol, aerosol-precipitation interactions, and unclear future aerosol emission pathways. Ongoing large reductions in aerosol emissions from East Asia, combined with uncertainty in future aerosol emissions for India and Africa, indicate that aerosol changes are likely to play an important role in African climate in the near-term future.
In this presentation, we identify regional African precipitation responses to local and remote aerosol emission changes, and establish mechanisms behind them. We focus on responses in the East and West African monsoons, including changes to the intensity, timing, spatial pattern, and variability of rainfall. We also demonstrate the sensitivity of the responses to aerosol emission region, to determine whether local or remote emission changes dominate rainfall responses on seasonal timescales. Using the Regional Aerosol Model Intercomparison Project experiments, we quantify the role of regional aerosol emission changes in near-term African precipitation responses. This allows us to determine the aerosol emission regions which dominate the African precipitation responses, while also exploring sensitivities to absorbing and scattering species of aerosol emissions.
Current analysis has determined that reductions in global aerosol emissions cause West Africa to become significantly hotter and wetter, with a northward shift in precipitation found in some models; this change is strongest along the coastline in most models, though there is considerable diversity in the magnitude of modelled responses.
This work highlights the role of changing aerosol emissions on African precipitation patterns, providing essential information for near-term climate adaptation strategies.

How to cite: Toolan, C., Turner, A., and Adabouk Amooli, J. and the RAMIP Team: Sub-Saharan African Precipitation Responses to Aerosol Emission Changes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6953, https://doi.org/10.5194/egusphere-egu25-6953, 2025.

EGU25-7034 | ECS | Orals | AS3.11

 Estimation of turbulence dissipation rate within shallow cumulus using airborne Particle Image Velocimetry 

Yewon Kim, Eberhard Bodenschatz, and Gholamhossein Bagheri

Accurately estimating cloud microphysics is crucial for reducing uncertainties in weather and climate models. A particular challenge is capturing the interactions between the cloud microphysics and turbulence. The pervasive shallow cumulus clouds over tropical oceans play a critical role in the Earth’s energy budget, making their study crucial for understanding atmospheric dynamics. In this context, the EUREC4A field campaign, conducted over the Atlantic Ocean close to Barbados from January to February 2020, gathered approximately 200 hours of unique observational data from these clouds [1]. The data was collected by two Max Planck CloudKites deployed from ships. A subset of this data includes Particle Image Velocimetry (PIV) and holographic measurements taken within clouds, providing unique insight into cloud dynamics. To our knowledge, our data represent the first application of airborne PIV in atmospheric clouds and provide an unprecedented opportunity to link cloud turbulence and microphysics.

In this study, we explore the feasibility and accuracy of estimating high-resolution turbulence energy dissipation rates within clouds based on the PIV data. We used the approximate 100k PIV image pairs from both precipitating and non-precipitating clouds collected during the EUREC4A campaign. We employed several established dissipation rate estimating methods, including the second-order structure function method [2] and the 2D gradient method used in the field of planar PIV [3, 4]. The turbulence energy dissipation rate across different cloud types (or flight segments) observed during the campaign is computed.

In addition, we have performed a detailed comparative analysis of the dissipation rate estimated with different techniques, including a 1- and 3-dimensional pitot tube. We also investigate the two-dimensional spatial distribution of cloud droplets and its correlation with turbulence features. We believe that these findings will improve our understanding of turbulence in shallow cumulus clouds and its impact on their formation and evolution.

 

References

[1] Bony, S., Stevens, B., Ament, F., Bigorre, S., Chazette, P., Crewell, S., ... & Wirth, M. EUREC 4 A: A field campaign to elucidate the couplings between clouds, convection and circulation., Surveys in Geophysics, 38, 1529–1568 (2017).

[2] Schröder, M., Bätge, T., Bodenschatz, E., Wilczek, M., & Bagheri, G. Estimating the turbulent kinetic energy dissipation rate from one-dimensional velocity measurements in time., Atmospheric Measurement Techniques, 17, 2, 627-657 (2024).

[3] Tanaka, T. & Eaton, J. K. A correction method for measuring turbulence kinetic energy dissipation rate by PIV: Validated by random Oseen vortices synthetic image test., Experiments in Fluids, 42, 6, 893-902 (2007).

[4] Verwey, C., & Birouk, M. Dissipation rate estimation in a highly turbulent isotropic flow using 2D-PIV. Flow., Turbulence and Combustion, 109, 3, 647-665 (2022).

How to cite: Kim, Y., Bodenschatz, E., and Bagheri, G.:  Estimation of turbulence dissipation rate within shallow cumulus using airborne Particle Image Velocimetry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7034, https://doi.org/10.5194/egusphere-egu25-7034, 2025.

EGU25-7303 | Orals | AS3.11

Advancing understanding and predictability of aerosol effective radiative forcing due to structural uncertainty in an Earth system model 

Po-Lun Ma, Jerome Hast, Andrew Geiss, Mohammad Taufiq Hassan Mozumder, Meng Huang, Yi Qin, Mingxuan Wu, Rahul Zaveri, Kai Zhang, Litai Kang, Roger Marchand, Vincent Larson, Hugh Morrison, Bin Zhao, Casey Wall, and Yu Yao

Earth system models struggle to accurately simulate aerosol’s interactions with weather and climate. This is largely attributed to structural uncertainty including insufficient process representation and model resolution due to limited computer power, and model tuning has become a low-cost remedy for improving performance. With unprecedented computational capability, improved understanding, modern software, and novel machine learning algorithms, high-resolution Earth system modeling with accurate and yet expensive process representations has become possible. In this study, we quantify the impacts of longstanding structural uncertainty on aerosol effective radiative forcing (ERF) by incorporating much more sophisticated process representations in U.S. Department of Energy’s Energy Exascale Earth System Model (E3SM). The ERF associated with aerosol-cloud interactions is further decomposed into the Twomey effect, liquid water path (LWP) adjustment, and cloud fraction adjustment using a satellite-based radiative kernel so that the impacts of each new process representation on aerosol ERF can be evaluated against observations. We find that while increasing model resolution to kilometer scale changes aerosol ERF by 30%, model physics representations (aerosol mixing assumption, condensational growth, secondary organic and sulfate aerosol formation, aerosol optics, aerosol activation, emission, giant aerosol, chemistry, warm rain process, and aerosol-turbulence coupling) contributes to a factor-of-two variation in aerosol ERF. As opposed to model tuning, this approach improves understanding and increases confidence in simulations as they are traceable to physics. Furthermore, even though the model’s total aerosol ERF or the Twomey effect alone can be brought to agree well with satellite estimate, significant biases in LWP and cloud fraction adjustments remain, highlighting the importance of improving aerosol interactions with cloud macrophysics in the model.

How to cite: Ma, P.-L., Hast, J., Geiss, A., Hassan Mozumder, M. T., Huang, M., Qin, Y., Wu, M., Zaveri, R., Zhang, K., Kang, L., Marchand, R., Larson, V., Morrison, H., Zhao, B., Wall, C., and Yao, Y.: Advancing understanding and predictability of aerosol effective radiative forcing due to structural uncertainty in an Earth system model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7303, https://doi.org/10.5194/egusphere-egu25-7303, 2025.

EGU25-7763 | ECS | Orals | AS3.11

Aerosols exacerbating the heterogeneity of precipitation vertical structures 

Yue Sun and Chuanfeng Zhao

The vertical structures of precipitation serve as a direct link between clouds and surface precipitation, reflecting the processes of cloud and precipitation formation and development. However, their significance remains debatable, particularly concerning the aerosol effects on these structures. We utilize data from PM2.5 station measurements and the GPM 2A DPR to investigate the impact of aerosols on the vertical structure of precipitation and its microphysical characteristics.

Our findings show that the raindrop size in cold-topped (storm top height more than freezing level) precipitation exhibits three distinct trends from the storm top height to the surface: raindrop size decreases or shows no significant change in the upper layers, increases rapidly in the middle layers, and slightly decreases in the lower layers. Based on the observed turning points in raindrop size changes, we conducted a study on the influence of aerosols on the vertical structure of precipitation.

This study reveals phenomena different from previous views. Conventional wisdom suggests that higher and more extensive cloud development leads to greater surface precipitation intensity. However, our results indicate that for local cold-topped convective precipitation, the correlation between storm top height and precipitation rate at different altitudes decreases gradually with decreasing altitude. Absorbing aerosols are identified as a significant factor exacerbating the heterogeneity of precipitation vertical structures.

Within clouds, aerosols act as cloud condensation nuclei (CCN), influencing the growth of cloud droplets and ice crystals through microphysical effects. The competition between latent heat released and evaporative cooling initially increases storm top height but subsequently reduces it. Above the freezing level, precipitation rates and raindrop sizes remain highly consistent with storm top height. Below the freezing level, however, the vertical structure of precipitation is altered by evaporation. Larger raindrops and higher proportions of absorbing aerosols enhance evaporation, leading to a complex relationship where surface precipitation rates first decrease and then increase with increasing aerosol concentration. This response to aerosol is almost opposite to that observed above the freezing level.

This indicates that aerosols significantly exacerbate the heterogeneity of precipitation vertical structures through both microphysical and radiative effects.

How to cite: Sun, Y. and Zhao, C.: Aerosols exacerbating the heterogeneity of precipitation vertical structures, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7763, https://doi.org/10.5194/egusphere-egu25-7763, 2025.

Maritime stratocumulus clouds play a crucial role in Earth’s climate system by reflecting incoming solar radiation. The optical and microphysical properties of stratocumulus are determined by the droplet size distribution (DSD), commonly characterized by the mean droplet radius and relative dispersion. In this study, we identify distinct droplet evolution regimes within the stratocumulus-topped boundary layer (STBL) by tracking individual droplets in large-eddy simulations coupled with Lagrangian cloud microphysics. Two dominant regimes emerge: the adiabatic growth regime, dominated by droplet activation and condensation in the updraft, and the entrainment and descent regime. Droplets in the adiabatic growth regime follow consistent trajectories, with increasing mean droplet radius and decreasing relative dispersion. In the entrainment and descent regime, however, droplets follow diverse pathways: Droplets directly affected by entrainment and mixing at the cloud top show signs of inhomogeneous mixing, with some droplets completely evaporating, while droplets following the downdrafts without being directly affected by entrainment and mixing exhibit smoother changes in microphysical properties, resembling homogeneous mixing, indicating that such mixing-like signatures can arise from the large-scale STBL dynamics rather than mixing alone. This study underscores the complexity of droplet evolution within stratocumulus and highlights the need to distinguish between microphysical processes and large-scale dynamics when interpreting observed or simulated mixing-related microphysical properties.

How to cite: Lim, J.-S. and Hoffmann, F.: Regimes of Droplet Size Distribution Evolution in Stratocumulus: From Adiabatic Growth to Entrainment and Mixing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8044, https://doi.org/10.5194/egusphere-egu25-8044, 2025.

EGU25-8549 | ECS | Posters on site | AS3.11

Wind-induced aerosol transport and associated precipitation enhancement over South - East Asia 

Sebastian Joy, Sreenath Avaronthan Veettil, and Madhu Vazhathottathil

As the most populous and rapidly developing region, Asia has garnered significant attention regarding the anthropogenic influence on the atmospheric composition, climate, and hydrological cycle. Air pollution due to industrialization and urbanization is a local issue; however, its influence may go beyond regional scales due to large-scale atmospheric circulations along with the transport and evolution of particles. In this study, we investigated the impact of atmospheric circulation on regional air quality and its associated influence on regional precipitation. The datasets used for the analysis are the Cloud and the Earth’s Radiant Energy System (CERES – MODIS) and MERRA-2 Aerosol Optical Depth (AOD), Tropical Rainfall Measuring Mission (TRMM) rainfall and ERA-5 wind components for the years 2000 - 2019. The eastward drift of aerosol, along with the wind patterns, is observed. Also, the impacts of the long-range transport of natural and anthropogenic aerosols, as well as dust particles originating from the surrounding land masses, on the deepening of marine clouds and precipitation are evident over Southeast Asia. Moreover, the frequency and intensity of rain events exhibit modulation in response to the aerosol type and through their transport and interaction with clouds, and their vertical profile mainly by its impact on atmospheric heating. The Indian Ocean and Maritime Continent experience significant variability in both precipitation and AOD, reflecting the strong influence of the Madden-Julian Oscillation (MJO) in these regions. This highlights the importance of MJO in modulating aerosol distribution, which can further influence radiative forcing and local weather patterns. Understanding this coupling is critical for assessing regional air quality, hydrological cycles, and climate variability in tropical regions affected by the MJO.

How to cite: Joy, S., Avaronthan Veettil, S., and Vazhathottathil, M.: Wind-induced aerosol transport and associated precipitation enhancement over South - East Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8549, https://doi.org/10.5194/egusphere-egu25-8549, 2025.

EGU25-8614 | ECS | Orals | AS3.11

Mechanisms of surface solar irradiance variability under broken clouds 

Wouter Mol and Chiel van Heerwaarden

Surface solar irradiance variability is present under all broken clouds, but the patterns, magnitude of variability, and mechanisms behind it vary greatly with cloud type. Most radiative transfer models do not resolve the observed variability, primarily due to limiting radiative transport to two streams (up and down) to save computation time. From observations, we selected a diverse set of surface solar irradiance patterns under various cloud types and modelled these cloud types in combination with a Monte Carlo ray tracer for accurate 3D radiative transfer. Stratus, altocumulus, and cumulus growing into cumulonimbus are among the studied cloud types. The goal of these experiments is to understand through which mechanisms various cloud types generate observed patterns of irradiance variability. 

The results show that we can capture the essence in four mechanisms. We find that for optically thin (optical thickness  <  6) clouds, scattering in the forward direction dominates. In cloud fields with enough optically thin area, such as altocumulus, "forward escape" alone can drive areas of irradiance enhancement of over 50 % of clear-sky irradiance.  For flat, optically thick clouds (optical thickness > 6), irradiance is instead scattered diffusely downward ("downward escape"), and (extreme) enhancements are thus found directly below the cloud rather than in the direction along the solar angle. For vertically structured clouds, "side escape" dominates domain-averaged diffuse irradiance enhancement until anvil clouds form and start shading the updraft.  Lastly, under optically thick cloud cover, surface albedo enhances downward radiative fluxes due to multiple scattering between surface and cloud. This both brightens shadows and contributes 10 to 60 % of the total irradiance enhancement in sunlit areas for respectively low (0.2) to high (0.8) albedo. 

With these four mechanisms, we provide a framework for understanding the vast diversity and complexity found in surface solar irradiance and cloudiness. Such a framework can guide the development of parameterizations that capture 3D solar irradiance effect at a fraction of the computational cost of 3D radiative transfer models, for example.

How to cite: Mol, W. and van Heerwaarden, C.: Mechanisms of surface solar irradiance variability under broken clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8614, https://doi.org/10.5194/egusphere-egu25-8614, 2025.

EGU25-8619 | ECS | Posters on site | AS3.11

Unveiling the hidden heating layer at the top of stratocumuli 

Kenneth Chan, Stefan A. Buehler, Juan Pedro Mellado, and Manfred Brath

High-resolution simulations such as direct numerical simulations (DNS) are imperative to resolve the metre-scale variability in the stratocumulus-topped boundary layer (STBL). Previous research has considered the liquid water path (LWP) as a proxy for the longwave radiative transfer, to simplify the expensive radiative transfer calculations. However, the contribution to the radiative fluxes from the absorptive gases is thereby neglected. Utilising the line-by-line radiative transfer model ARTS, we show that the cloud top radiative cooling is underestimated by 30% in earlier simulations that employed the LWP parametrisation. Moreover, we identify a layer warming at 2.5 K h-1 with thickness of merely about 5 m directly above the cloud top, which we call the cloud top inversional heating layer (CTIHL), the warming in which is attributed to the clear sky radiative effect. About the cloud top inversion, the absorptive gases, predominantly water vapour and carbon dioxide, exchange heat locally due to the strong temperature gradient. The clear sky radiative warming is compensated in the cloud layer by the cloud top radiative cooling due to the liquid water, resulting in the minimal thickness of the CTIHL, which poses challenge for observations. We investigate the environmental factors which modulate the strength of the CTIHL. It is determined that the warming magnitude of the CTIHL is sensitive to the strength of the inversion and water vapour content, but less to the concentration of carbon dioxide.

How to cite: Chan, K., Buehler, S. A., Mellado, J. P., and Brath, M.: Unveiling the hidden heating layer at the top of stratocumuli, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8619, https://doi.org/10.5194/egusphere-egu25-8619, 2025.

EGU25-8750 | ECS | Posters on site | AS3.11

How will climate change impact fog and low clouds in the Namib desert? 

Alexandre Mass, Hendrik Andersen, and Jan Cermak

In this contribution, a statistical model built on observations (ERA5, SEVIRI) is used with climate model data from the Coupled Model Intercomparison Project Phase 6 (CMIP6) to estimate the cloud-system responses to climate change in the Namib desert.

Fog, which is the most relevant non-rainfall water source for plants and animals in the coastal parts of the Namib Desert, may become increasingly important for local ecosystems as regional climate simulations predict a warmer and drier climate for southern Africa in the future. However, projecting changes in fog using global circulation models (GCMs) or even regional climate models (RCMs) is challenging because these numerical models often cannot resolve, or have yet to incorporate, many processes that drive fog development.

A statistical model is developed to predict fog and low cloud (FLC) occurrence in the Namib region by combining reanalysis products with satellite data. Assuming that the relationships learned by the statistical model in the current climate remain valid in the future, this model can utilize climate model outputs from CMIP6 as predictors to estimate changes in FLCs in the region.

It is found that under low-emission scenarios like SSP1-2.6, FLC cover remains mostly constant. In contrast, higher-emission scenarios such as SSP3-7.0 project a decrease in FLC cover by up to 10%, with this decline accelerating around 2050.

How to cite: Mass, A., Andersen, H., and Cermak, J.: How will climate change impact fog and low clouds in the Namib desert?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8750, https://doi.org/10.5194/egusphere-egu25-8750, 2025.

EGU25-8938 | ECS | Posters on site | AS3.11

How 3D cloud radiative effects are influenced by microphysics of low-level clouds 

Irene Elisa Bellagente and Fabian Senf

Key words: Cloud Radiative Effects (CRE), Three-Dimensional Radiative Transfer, ICON, MYSTIC, Low-Level Clouds, Cloud Microphysics


Abstract: The microphysical properties of low-level clouds play a critical role in influencing threedimensional (3D) cloud radiative effects (CRE), yet significant uncertainties and approximations persist in their parametrizations. Our research investigates how detailed microphysical parameterizations and high-resolution simulations can advance the representation of 3D CREs. We intend to establish a thorough framework for examining cloud-radiation interactions by integrating regional and local simulations with data from extensive observational campaigns. As a first step towards this objective, we present preliminary results from nested simulations of the ICON model at hectometer resolution, targeting specific low-level cloud regimes over the Lindenberg Observatory in Germany. Cloud microphysics is simulated with a two-moment microphysical scheme. The 3D cloud radiative effects are estimated from the application of the 3D radiative transfer model MYSTIC in offline mode. The resulting model data are extensively evaluated against observed ground-based radiation fluxes and cloud radar data. We discuss how spatial cloud heterogeneity and microphysical complexity significantly modulate the deviations between 1D and 3D CRE estimates. By integrating high-resolution simulations with advanced observational datasets, this work provides critical insights into the mechanisms driving cloud radiative effects and their representation in climate models. Ultimately, this project will lay the foundations for refining parameterizations of cloud feedbacks and enhancing the realism of atmospheric radiation schemes.

How to cite: Bellagente, I. E. and Senf, F.: How 3D cloud radiative effects are influenced by microphysics of low-level clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8938, https://doi.org/10.5194/egusphere-egu25-8938, 2025.

Aerosol-cloud interactions are complex processes that contribute significantly to uncertainties in predicting global climate. Cloud droplet formation is influenced by factors such as the hygroscopicity of soluble aerosol particles, aerosol processing within clouds, aerosol particle number concentration, and updraft velocity. Accurately understanding these factors is crucial for better representing cloud droplet numbers on a global scale. Updraft velocity is characterized by the probability density function (PDF) of the vertical velocity distribution. Earth system models (ESMs) typically assume a constant standard deviation (σw) for the vertical velocity PDF (van Noije et al. 2021; Mulcahy et al. 2020). However, this assumption may be inaccurate, as it has been shown that the σw exhibits significant diurnal variability (Bougiatioti et al. 2020). In this study, we implemented the turbulent kinetic energy (TKE) calculations to OpenIFS cycle 48r1 (OIFS48r1) following Bastak Duran et al. (2018). In addition, we implemented Morales and Nenes (2014) activation parameterization (M&N) to OIFS48r1 including the TKE to calculate the σw instead of using a constant σw for the vertical velocity PDF. OIFS48r1 is derived from the Integrated Forecasting System (IFS) developed by European Centre for Medium-Range Weather Forecasts (ECMWF) and it will be the main atmospheric model used in the newest version of European Community ESM (EC-Earth 4). First, we investigated the effects of using constant σw values of 0 and 0.8 m/s on the TKE-derived σw and their impact on column averaged cloud droplet number concentrations. The results showed that using σw of 0 m/s led to very low droplet numbers, as weaker updraft variability resulted in smaller supersaturations, causing fewer particles to activate. On the other hand, using σw of 0.8 m/s produced stronger activation, particularly in regions with high aerosol particle number concentrations. When using the TKE-derived σw, the differences in droplet numbers compared to the activation scheme with σw of 0.8 m/s were minimal. Next, we compared the monthly column-averaged and boundary-layer (BL) average number of activated particles obtained from the TKE-derived σw activation routine with the pre-existing Abdul-Razzak and Ghan (2000) activation parameterization (AR&G). The results showed that the AR&G scheme produced stronger activation than the M&N scheme, both in terms of the total column average and the BL-averaged regions. One of the reasons for this difference could be due to the activation calculations in the M&N scheme, which are only performed in areas where clouds are present, while in the AR&G scheme, activation is calculated for every gridbox.

How to cite: Holopainen, E. and Nenes, A.: Aerosol processes and activation in OpenIFS cycle 48r1 portable global aerosol-climate and weather prediction model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9397, https://doi.org/10.5194/egusphere-egu25-9397, 2025.

Satellite sensors provide global monitoring of cloud properties, such as cloud effective radius and cloud optical thickness, which have been extensively used to quantify the radiative forcing due to aerosol-cloud interactions. These cloud properties are simultaneously retrieved from a pair of reflectance measurements using a bi-spectral retrieval algorithm. However, the algorithm’s solution space is limited, and retrievals often fail when observations fall outside this space. Upon analyzing five years of quality-constrained liquid-cloud pixels observed by MODIS aboard Aqua, we find that a significant 10% of cloudy pixels experience retrieval failure, primarily because the observations correspond to an effective radius exceeding MODIS’s upper retrieval limit of 30 µm. The omission of these cloudy pixels introduces a sampling bias in aggregated mean gridded cloud properties, affecting, among other things, radiative forcing calculations. To address this, we restore the failed cloud retrievals in MODIS using two reconstruction algorithms: (1) a conservative approach that assigns a fixed minimum effective radius to failed pixels, and (2) a realistic approach that uses extreme effective radius distributions from spaceborne radar measurements. Our findings reveal that MODIS-derived cloud droplet number concentration is positively biased, while liquid water path is negatively biased. Accounting for this bias increases the magnitude of cloud water adjustments, highlighting the crucial need to expand the solution space in MODIS and similar sensors.

How to cite: Choudhury, G. and Goren, T.: Sampling bias from satellite retrieval failure of cloud properties and its implications for aerosol-cloud interactions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9585, https://doi.org/10.5194/egusphere-egu25-9585, 2025.

EGU25-9604 | ECS | Orals | AS3.11

RCEMIP-ACI: Aerosol-Cloud Interactions in a Multimodel Ensemble of Radiative-Convective Equilibrium Simulations  

Guy Dagan, Susan C. van den Heever, Philip Stier, Tristan H. Abbott, Christian Barthlott, Jean-Pierre Chaboureau, Stephan de Roode, Jiwen Fan, Blaž Gasparini, Corinna Hoose, Fredrik Jansson, Gayatri Kulkarni, Gabrielle Leung, Thara Prabhakaran, David M. Romps, Denis Shum, Mirjam Tijhuis, Chiel C. van Heerwaarden, Allison Wing, and Shan Yunpeng

Aerosol-cloud interactions are a persistent source of uncertainty in climate research. This study presents findings from a model intercomparison project examining the impact of aerosols on clouds and climate in "cloud-resolving" Radiative-Convective Equilibrium (RCE) simulations. Specifically, 11 different models conducted RCE simulations under varying aerosol concentrations, domain configurations, and sea surface temperatures (SSTs). We analyze the response of domain-mean cloud and radiative properties to imposed aerosol concentrations across different SSTs. Additionally, we explore the potential impact of aerosols on convective aggregation and large-scale circulation in large-domain simulations.

 

The results reveal that the cloud and radiative responses to aerosols vary substantially across models. However, a common trend across models, SSTs, and domain configurations is that increased aerosol loading tends to suppress warm rain formation, enhance cloud water content in the mid-troposphere, and consequently increase mid-tropospheric humidity and upper-tropospheric temperature, impacting static stability. The warming of the upper troposphere can be attributed to reduced entrainment effects due to the higher environmental humidity in the mid-troposphere. However, examining high percentiles of vertical velocities at the mid troposphere do not demonstrate convective invigoration. In large-domain simulations, where convection tends to self-organize, aerosol loading does not influence self-organization but tends to reduce the intensity of large-scale circulation forming between convective clusters and dry regions. This reduction in circulation intensity can be explained by the increase in static stability.      

How to cite: Dagan, G., van den Heever, S. C., Stier, P., Abbott, T. H., Barthlott, C., Chaboureau, J.-P., de Roode, S., Fan, J., Gasparini, B., Hoose, C., Jansson, F., Kulkarni, G., Leung, G., Prabhakaran, T., Romps, D. M., Shum, D., Tijhuis, M., van Heerwaarden, C. C., Wing, A., and Yunpeng, S.: RCEMIP-ACI: Aerosol-Cloud Interactions in a Multimodel Ensemble of Radiative-Convective Equilibrium Simulations , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9604, https://doi.org/10.5194/egusphere-egu25-9604, 2025.

The Arctic is experiencing a faster warming, known as the Arctic amplification, but climate projections are still uncertain due to the aerosol-cloud interactions (ACI). The impact of aerosols on glaciation temperature, acting as ice nucleating particles, is poorly understood, especially for aerosols from long-range transport. During transport, physico-chemical properties of aerosols evolve due to aging, complicating the quantification of their role.

This study considers satellite observations from POLDER and MODIS instruments with atmospheric chemistry model (GEOS-Chem) and reanalysis datasets (ERA5) to investigate the influence of aerosols on cloud properties and glaciation temperatures. Carbon monoxide (CO) is employed as a passive tracer to aerosols from combustion sources. GEOS-Chem is used to distinguish between biomass burning (BB) and anthropogenic (ANT) emissions and further identify the source regions of air parcels. Spatial and temporal co-localization of cloud, aerosol, and environmental parameter datasets is performed to assess the interplay between meteorological parameters and aerosol properties on cloud properties and on the glaciation process.

Our analysis reveals distinct impacts of aerosols from BB and ANT sources on the glaciation temperature. Preliminary results indicate that pollution plumes from BB are associated with an increase or decrease of about 1.7°C of the glaciation temperature depending on the source region, while ANT pollution plumes suggest an increase of the glaciation temperature between 1.5°C and 2.8°C depending on the transport of air parcels before interacting with the clouds. This work highlights the necessity of considering transport-induced changes in aerosol properties to improve our understanding of the ACI and Arctic climate dynamics.

How to cite: Coopman, Q. and Riedi, J.: Understanding the Impact of Aerosol Transport on the cloud glaciation temperature in the Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9656, https://doi.org/10.5194/egusphere-egu25-9656, 2025.

EGU25-10008 | Posters on site | AS3.11

Insights into aging of biomass burning aerosols based on satellite observations and trajectory modelling 

Manu Anna Thomas, Abhay Devasthale, and Michael Kahnert

Aerosols from biomass burning significantly impact human health, climate and society. These particles can be both natural and human-induced sources. While wildfires are considered a natural source, seasonal burning of agricultural fields before planting is an example for anthropogenic sources. With increasing global temperatures, the frequency and intensity of wildfires are escalating. Despite their importance, our understanding of these aerosols and their accurate representation in global emission inventories remain inadequate. The current estimates of the global direct radiative forcing of these aerosols range from net cooling to net warming in climate models. This shows how little we know about these aerosols and the chemical transformation they undergo as they age when they are advected farther away from the source regions. The optical properties of these biomass burning aerosols depends on the type of vegetation that is burnt, the type of burning and the prevailing meteorological conditions. Hence, in this study, we attempt to evaluate their optical properties at the source and also, as they are transported away from their source and age.

Here, we use MODIS data to locate the fires in Africa and we chose those fires based on the percentage of area burnt and the fire intensity. A trajectory model, HYSPLIT, is run to get the trajectory of the fire plumes. These trajectories are then collocated with the CALIPSO tracks to estimate the optical properties of these aerosols as they age away from the source regions.

 

How to cite: Thomas, M. A., Devasthale, A., and Kahnert, M.: Insights into aging of biomass burning aerosols based on satellite observations and trajectory modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10008, https://doi.org/10.5194/egusphere-egu25-10008, 2025.

EGU25-10728 | Orals | AS3.11

When Co-Variability Mimics Causal Aerosol-Cloud Interactions in Satellite Data 

Tom Goren, Goutam Choudhury, Jan Kretzschmar, and Isabel McCoy

Relationships between variables derived from satellite observations can be interpreted as causal connections between explanatory and response variables. When physical processes support the observed relationship, it appears more likely to represent a true causal link. A notable example is the observed relationship between liquid water path and droplet number concentration in marine low clouds, which aligns with the physical mechanisms involved. However, a closer examination reveals that the observed relationships may actually be driven by co-variability between meteorological conditions and aerosol levels, reflecting the climatological evolution of stratocumulus clouds. We therefore suggest that the aerosol influence on marine low clouds should be separated into two pathways: (1) the influence of background aerosol levels on the clouds' climatology, which overlays the co-variability, and (2) the causal response, as seen in the case of ship tracks.

How to cite: Goren, T., Choudhury, G., Kretzschmar, J., and McCoy, I.: When Co-Variability Mimics Causal Aerosol-Cloud Interactions in Satellite Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10728, https://doi.org/10.5194/egusphere-egu25-10728, 2025.

EGU25-10796 | Orals | AS3.11

Convective clouds over the Amazon rainforest – aerosol dependence and microphysical features 

Mira L. Pöhlker, Baseerat Romshoo, Oliver Lauer, Jyothirbindu Maddali, Philipp Liznerski, Alice Henkes, Johannes Quaas, Patric Seifert, Tom Gaudek, Bruno Meller, Subha Raj, Luiz Machado, Micael Cecchini, Rachel Albrecht, Samira Atabakhsh, Paulo Artaxo, Yifan Yang, Arun Babu Suja, Maris Kloft, and Christopher Pöhlker

The Amazon rainforest plays an important role in global climate systems, particularly in regional precipitation patterns, atmospheric circulation, and Earth's energy balance. Convective systems in this region are intricately linked to these broader climatic processes. Through a combination of ground-based, satellite, and aircraft observations, we find that Amazonian convective clouds are particularly sensitive to aerosol concentrations, being highly aerosol-limited. This study explores the relationship between cloud droplet concentrations and ambient aerosol particles, both within the Amazon and in broader regions, evaluating various parameterizations commonly used in global climate models. Machine learning methods were used to capture the relationships between various aerosol, cloud, and meteorological parameters in the Amazon rainforest. To gain deeper insight into the microphysical processes within individual clouds, we examine the evolution of the cloud droplet effective radius (rₑ) as a function of cloud temperature (T), looking into the vertical structure of deep convective cumulus clouds. 

How to cite: Pöhlker, M. L., Romshoo, B., Lauer, O., Maddali, J., Liznerski, P., Henkes, A., Quaas, J., Seifert, P., Gaudek, T., Meller, B., Raj, S., Machado, L., Cecchini, M., Albrecht, R., Atabakhsh, S., Artaxo, P., Yang, Y., Babu Suja, A., Kloft, M., and Pöhlker, C.: Convective clouds over the Amazon rainforest – aerosol dependence and microphysical features, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10796, https://doi.org/10.5194/egusphere-egu25-10796, 2025.

EGU25-11812 | Orals | AS3.11

Machine Learning derived CCN concentrations provide better constraints on the first aerosol indirect effect than aerosol optical properties 

Jens Redemann, Lan Gao, Emily Lenhardt, Sharon Burton, Ewan Crosbie, Marta Fenn, Richard Ferrare, Johnathan Hair, Chris Hostetler, Amin Nehrir, Taylor Shingler, Brian Cairns, and Armin Sorooshian

The first indirect effect of aerosols on cloud reflectivity, primarily through changes in cloud droplet number concentration (Nd) or effective radius (Reff), remains one of the most uncertain components of anthropogenic radiative forcing. The strength of the first aerosol indirect effect (AIE) is quantified using relationships between aerosol proxies and Nd/Reff. For large-scale assessments, these relationships have historically been observed via satellites and serve as critical constraints for climate models calculating radiative forcing from aerosol-cloud interactions (ACIs). They have often relied on observations of aerosol optical depth or aerosol index, which are column-integrated proxies for Cloud Condensation Nuclei (CCN) concentration that may not be directly relevant for studying ACIs. Additionally, these proxies are influenced not only by particle concentration but also by size distribution, composition, and relative humidity. Since CCN represents only a fraction of the aerosol size distribution, there may not always be an obvious correlation between CCN and optical properties, introducing uncertainties in estimating indirect effects when using aerosol optical properties.

To address this issue, we developed a machine learning approach to estimate the vertical profile of CCN concentration at 0.4% supersaturation using airborne High Spectral Resolution Lidar Generation-2 (HSRL-2) data and collocated in situ CCN, the latter as truth to train a neural network model. Reanalysis data were used to enhance model performance. Our algorithm predicts vertically resolved CCN concentration within a mean relative uncertainty of 20% and is applicable to EarthCARE/ATLID measurements.  Utilizing this new CCN product derived from the full suite of HSRL-2 extinction and backscatter measurements and reanalysis data of relative humidity and temperature in ACTIVATE (Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment) along with collocated cloud properties retrieved from Research Scanning Polarimeter data, we investigate the first AIE over the western North Atlantic Ocean. Our preliminary findings indicate that the new CCN product consistently constrains the relationships between CCN and Nd/Reff, for a wide range of cloud liquid water paths. The separation of indirect effects for different aerosol types indicates the expected differences in aerosol properties relevant for ACI. Overall, our approach using ML-derived CCN yields tighter constraints and physically more plausible insights into ACIs than vertically-resolved aerosol extinction, vertically-resolved aerosol index (extinction multiplied by Angstrom exponent), or column-integrated aerosol optical depth. We will conclude our presentation by illustrating that the aerosol vertical distribution and hygroscopic growth characteristics are the primary reasons why aerosol optical properties are inadequate for directly constraining the first AIE in the western North Atlantic Ocean.

How to cite: Redemann, J., Gao, L., Lenhardt, E., Burton, S., Crosbie, E., Fenn, M., Ferrare, R., Hair, J., Hostetler, C., Nehrir, A., Shingler, T., Cairns, B., and Sorooshian, A.: Machine Learning derived CCN concentrations provide better constraints on the first aerosol indirect effect than aerosol optical properties, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11812, https://doi.org/10.5194/egusphere-egu25-11812, 2025.

EGU25-13039 | ECS | Posters on site | AS3.11

UAV-Based Insights into Cloud Particle Size Distributions from the CHOPIN Campaign 

Alkistis Papetta, Anna Voß, Marine Goret, Leo Håkansson, Konstantinos Michailidis, Spyros Bezantakos, George Biskos, Maria Kezoudi, Nikos Mihalopoulos, Jean Sciare, and Franco Marenco

Clouds play an important role in the Earth’s climate through well-established mechanisms, such as their interactions with solar radiation and their role in precipitation. However, their influence on future climate projections remains highly uncertain. One of the key challenges is the understanding of aerosol-cloud interactions in studying clouds, as aerosols can serve as cloud condensation nuclei.  Aerosols can have significant variability across both space and time. While in situ measurements provide precise data for a small atmospheric volume—just a few cubic centimetres—they may not accurately reflect the spatial (horizontal and vertical) variability of aerosol characteristics and therefore do not give accurate statistical information on the average cloud state and its variability.

Airborne observations offer the capability of sampling a larger volume of the atmosphere and therefore give a more comprehensive understanding of clouds.This study highlights UAV-based observations of particle size distributions both inside and outside clouds, conducted during the #CHOPIN (CleanCloud Helmos Orographic Site Experiment) campaign. As part of this campaign, the Unmanned Systems Research Laboratory (USRL) of the Cyprus Institute deployed light Unmanned Aircraft Systems at Mt. Helmos, Greece, from October 11 to November 1, 2024, providing valuable data for the study of clouds and their interactions with aerosols. This is one of the few times USRL/CYI reported observations aerosol-cloud interaction flights.

The #CHOPIN campaign, conducted in collaboration with NCSR Demokritos and FORTH/EPFL, was hosted at the Kalavryta Ski Center with a base altitude for the UAS takeoffs and landings of ~1.7 km ASL. The campaign aimed to improve the understanding of aerosol-cloud interactions and to evaluate remote sensing algorithms and models. Located in a rapidly changing "climate hotspot" at the intersection of various air masses, Mount Helmos is particularly sensitive to environmental changes, with interactions between wildfire smoke, pollution, sea salt, and Saharan dust. This unique setting provides an ideal location to study the dynamics of aerosol-cloud interactions.

During the campaign, several flights were performed inside and outside clouds operating in a horizontal area of approximately ~16km² and providing vertical profiles of particle size distribution from the ground up to 3.5 km ASL. We will focus on the cloud observations and the derivation of particle and droplet size distributions from UAV-based optical particle counters. These observations provide a good dataset for improving cloud-resolving models and for comparison with fixed station observations.

How to cite: Papetta, A., Voß, A., Goret, M., Håkansson, L., Michailidis, K., Bezantakos, S., Biskos, G., Kezoudi, M., Mihalopoulos, N., Sciare, J., and Marenco, F.: UAV-Based Insights into Cloud Particle Size Distributions from the CHOPIN Campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13039, https://doi.org/10.5194/egusphere-egu25-13039, 2025.

EGU25-13393 | ECS | Posters on site | AS3.11

A Holistic Investigation of Cloud Droplet Formation Representation in General Circulation Models 

Jamie Knight, Megan Haslum, Paul Bowen, Edward Bearman, and Daniel Partridge

Atmospheric aerosol particles are essential to Earth’s climate, serving as the nuclei for cloud droplet formation. The process of cloud droplet formation directly links aerosols and clouds, thereby influencing cloud properties (e.g., albedo and lifetime). Model estimates of effective radiative forcing suggest a net cooling effect from aerosol-cloud interactions (–0.84 W m‑2), but the wide range of values (–1.45 to –0.25 W m‑2) has hindered future climate projections (Masson-Delmotte et al., 2021).

Aerosol activation in general circulation models (GCMs) is parameterised, with the Abdul-Razzak & Ghan (2000; ARG) scheme used in the Unified Model for its efficiency, while the Morales Betancourt & Nenes (2014; MN) scheme represents a recent addition. These parameterisations are based on adiabatic cloud parcel model theory and estimate the maximum supersaturation (Smax) from which the cloud droplet number concentration (Nd) is derived. We will demonstrate that an improved GCM representation of cloud droplet formation is vital for constraining estimates of the climatic effect of aerosol-cloud interactions using a three-step holistic framework:

  • Direct comparison of parameterisations against an efficient cloud parcel model

In this study the DiffeRential Evolution Adaptive Metropolis (DREAM) Markov Chain Monte Carlo algorithm (Vrugt et al., 2009) is used to compare predictions of Smax and Nd from the ARG and MN schemes with those from the Pseudo-Adiabatic bin-micRophySics university of Exeter Cloud parcel model (PARSEC), using model input parameters selected near-randomly from predefined prior ranges that reflect those used in GCMs. These comparisons show that ARG underestimates both Smax and Nd relative to PARSEC (both by up to ~60%), while MN, to a lesser extent, overpredicts both values. Crucially for future climate projections, we identify differences in model sensitivity to input parameters (e.g., updraft velocity), and parameter combinations, between the parameterisations and PARSEC.

  • Offline evaluation against in-situ observations

The DREAM algorithm is applied within an inverse modelling framework to perform Nd closure experiments, using data from three marine aircraft campaigns that span updraft- and number-limited regimes. The results show that, compared to PARSEC, both ARG and MN often fail to match observed Nd, with ARG significantly underestimating Nd. Our framework reveals parameter sensitivities and correlations, offering insights for refining models and guiding future measurement campaigns.

  • Online evaluation – exploring the Southern Ocean albedo bias

GCM predictions of cloud albedo in the Southern Ocean are significantly underestimated relative to observations (Mulcahy et al., 2018). Here, PARSEC has been integrated into the UK Met Office climate model, allowing the first online evaluation of existing aerosol activation parameterisations. Importantly, we quantify the impact of cloud droplet formation representation on the observed Southern Ocean albedo bias.

Finally, we will discuss the implications of our findings from (1-3) for the effectiveness of current aerosol activation parameterisations for geoengineering via marine cloud brightening.

(1) Masson-Delmotte, et al., 2021, DOI:10.1017/9781009157896.001, (2) Abdul-Razzak, H. and Ghan, S. J., 2000, DOI: 10.1029/1999JD901161, (3) Morales Betancourt, R. and Nenes, A, 2014, DOI: 10.5194/gmd-7-2345-2014, (4) Vrugt, J. A., et al., 2009, DOI:10.1515/IJNSNS.2009.10.3.273, (5) Mulcahy, J, P., et al., 2018, DOI: 10.1029/2018MS001464.

How to cite: Knight, J., Haslum, M., Bowen, P., Bearman, E., and Partridge, D.: A Holistic Investigation of Cloud Droplet Formation Representation in General Circulation Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13393, https://doi.org/10.5194/egusphere-egu25-13393, 2025.

EGU25-13932 | ECS | Orals | AS3.11

A Closer Look into Shallow Cumulus Clouds: Investigating Cloud Microphysics and Droplet Clustering Using the Max Planck Cloudkite+ 

Birte Thiede, Michael L. Larsen, Oliver Schlenczek, Freja Nordsiek, Eberhard Bodenschatz, and Gholamhossein Bagheri

We present the findings from our in-situ holographic measurements conducted in shallow cumulus clouds, using the tethered aerostat Max Planck CloudKite (MPCK) during the EUREC4A campaign. The MPCK+ instrument is equipped with a holographic system sampling cloud droplets  8µm diameter or larger in a 10cm^3 three-dimensional volume every 12cm. This unprecedentedly small inter-sample spacing for holographic measurements is achieved by combining two variables: the high sampling frequency of our MPCK+ holographic setup, set at 75 Hz, and the low true airspeed of the aerostat.

The microphysical characteristics of clouds, such as droplet concentration, size distribution and liquid water content can be calculated with sub-meter spatial resolution. This allows us to obtain a detailed horizontal snapshot of a cloud's microphysics. The three-dimensional nature of holographic droplet data also allows a direct calculation of the radial distribution function (RDF), and the high measurement cadence of the MPCK+ data invites a spatially localized investigation of cloud droplet clustering.

We present an overview of our holographic data showcasing the structure of shallow cumulus clouds as well as an analysis of cloud droplet clustering in a short horizontal cloud snapshot.

How to cite: Thiede, B., Larsen, M. L., Schlenczek, O., Nordsiek, F., Bodenschatz, E., and Bagheri, G.: A Closer Look into Shallow Cumulus Clouds: Investigating Cloud Microphysics and Droplet Clustering Using the Max Planck Cloudkite+, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13932, https://doi.org/10.5194/egusphere-egu25-13932, 2025.

EGU25-13980 | Orals | AS3.11

Africa’s climate response to stratospheric aerosol injection materials 

Romaric C. Odoulami, Trisha D. Patel, Timofei Sukhodolov, Temitope S. Egbebiyi, Sandro Vattioni, Gabriel Chiodo, Christopher J Lennard, Babatunde J. Abiodun, and Mark G New

This study assessed Africa’s climate response to different injection materials for stratospheric aerosol geoengineering (SAG) using simulations from the SOCOLv4 model, which provides a set of SAG simulations following the G6sulfur experiment in the Geoengineering Multi-model Intercomparison Project (GeoMIP). We analysed four SAG experiments, which used four injection materials (sulfur, alumina, calcite, and diamond) referred to as G6sulfur, G6alumina, G6calcite, and G6diamond, respectively. The SAG experiments used a high-emission pathway (SSP5-8.5) as baseline in which each material was injected into the equatorial stratosphere to keep global warming levels similar to an intermediate emission pathway (SSP2-4.5). We assessed Africa’s climate response to these SAG materials by quantifying the end-of-century (2080-2099) mean changes in minimum and maximum temperatures and precipitation relative to SSP2-4.5. Our findings suggest that all injection materials show a cooling potential by keeping annual and seasonal minimum and maximum temperatures below SSP2-4.5 across most parts of the continent. Maximum and minimum temperatures could decrease the most between 10°S and 10°N, along the Guinean coast of west Africa and parts of Central Africa, by up to -2°C and -4°C, respectively. This SAG-induced cooling remains partial over north Africa where a residual warming of about 1°C could persist at the end of the century relative to the SSP2-4.5, irrespective of the injection material. On the other hand, the impact on precipitation is less linear and spatially heterogeneous. However, SAG could reverse the SSP5-8.5 projected mean continental and regional (especially over Central Africa) increases in annual and seasonal precipitation, inducing a dryer future under SAG across the continent, irrespective of the injection material. Our results further suggest that, relative to SSP2-4.5, G6alumina could cause the largest precipitation decrease and G6diamond the slightest decrease at the end of the century. In summary, our results show that irrespective of the injection material, SAG could significantly decrease temperatures across Africa, however lower warming and drying could still be achieved under SSP2-4.5, over parts of Africa.

How to cite: Odoulami, R. C., Patel, T. D., Sukhodolov, T., Egbebiyi, T. S., Vattioni, S., Chiodo, G., Lennard, C. J., Abiodun, B. J., and New, M. G.: Africa’s climate response to stratospheric aerosol injection materials, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13980, https://doi.org/10.5194/egusphere-egu25-13980, 2025.

EGU25-14185 | ECS | Posters on site | AS3.11

Effects of the Sea Salt Aerosol On an Idealized Tropical Cyclone Microphysics Using a Bulk Method 

Xuancheng Liu, Ruyan Chen, Lulin Xue, and Sisi Chen

Sea Salt Aerosols (SSA) constitute a primary component of atmospheric aerosols over the ocean, playing an important role in Earth's radiation balance, cloud formation, and precipitation processes. These aerosols serve as significant cloud condensation nuclei for marine clouds, with their production influenced by wind speed, sea temperature, and salinity, and are directly emitted from the sea surface via sea spray. Their strong hygroscopic nature allows them to maintain water content even under unsaturated conditions, thereby impacting heat flux, atmospheric water vapor content, cloud droplet water content, and precipitation intensity. Current research either focuses on the effects of SSA emission fluxes on water vapor and heat flux under diverse marine meteorological conditions, often neglecting the microphysical processes of SSA as hydrometeors, or employs computationally intensive microphysical schemes that are not readily applicable in practice. This study calculates SSA emission fluxes based on sea surface temperature and wind speed, applying a computationally efficient bulk parameterization approach for SSA microphysical processes. The methodology is integrated with the WRF numerical model to examine the influence of SSA microphysical processes on the microphysics of tropical cyclones under idealized conditions, with a focus on cloud formation and precipitation processes.

How to cite: Liu, X., Chen, R., Xue, L., and Chen, S.: Effects of the Sea Salt Aerosol On an Idealized Tropical Cyclone Microphysics Using a Bulk Method, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14185, https://doi.org/10.5194/egusphere-egu25-14185, 2025.

The western North Pacific Subtropical High (WNPSH) significantly influences East Asian weather. In the Northwest Pacific where sea‐salt aerosols (SSAs) are abundant and the large‐scale environment is dominated by the dry subsidence of the WNPSH during summer, inhomogeneous SSAs form as a product of the environment. However, the extent to which inhomogeneous SSAs affect the WNPSH remains unclear. This study investigates the radiative effects of SSAs through numerical simulations, revealing a novel mechanism for the strengthening of the WNPSH. The results demonstrate that inhomogeneous SSAs enhance the WNPSH by generating diabatic cooling in the upper troposphere and associated unstable subsidence motion. Further considering the radiative hysteresis effects of inhomogeneous SSAs, the WNPSH further strengthens under the combined dynamic and thermodynamic influences associated with upper‐level radiative cooling. Inhomogeneous SSAs not only enhance the WNPSH but also influence the location where the central area of high pressure intensifies.

How to cite: Shu, S.: Inhomogeneous Sea‐Salt Aerosols—A New StrengtheningMechanism for the Western North Pacific Subtropical High, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14328, https://doi.org/10.5194/egusphere-egu25-14328, 2025.

EGU25-14843 | ECS | Orals | AS3.11

Can evaporative cooling of water droplets play a role in enhancing ice formation at moderately supercooled cloud boundaries? 

Puja Roy, Robert M. Rauber, Larry Di Girolamo, Sisi Chen, Lulin Xue, and Sarah A. Tessendorf

Cloud droplet temperature is an important parameter influencing cloud microphysical and radiative processes. The supercooled droplet temperature and lifetime impact cloud ice and precipitation formation via homogeneous freezing and activation of ice-nucleating particles through contact and immersion freezing. While most observational and modeling studies often assume droplet temperature to be almost equal to the ambient temperature (Ta), this assumption may not always be valid, particularly when droplets experience strong relative humidity (RH) gradients at cloud boundaries.

This study investigates the evolution of temperature and lifetime of evaporating, supercooled cloud droplets considering initial droplet radius (r0) and temperature (Tr0), and environmental relative humidity (RH), ambient temperature (Ta), and pressure (P). The time (tss) required by droplets to reach a lower steady-state temperature (Tss) after sudden introduction into a new subsaturated environment, the magnitude of ΔT = Ta - Tss, and droplet survival time (tst) at Tss are calculated. The temperature difference (ΔT) is found to increase with Ta, and decrease with RH and P. ΔT values are typically 1–5 K lower than Ta, with highest values (~10.3 K) for very low RH, low P, and Ta closer to 0°C. Results show that tss is < 0.5 s over the range of initial droplet and environmental conditions considered. Tss of the evaporating droplets can be approximated by the environmental thermodynamic wet-bulb temperature. Radiation was found to play a minor role in influencing droplet temperatures, except for larger droplets in environments close to saturation. The implications for ice nucleation in cloud-top generating cells and near cloud edges are discussed. Using Tss instead of Ta in widely used parameterization schemes could lead to enhanced number concentrations of activated ice-nucleating particles (INPs), by a typical factor of 2–30, with the greatest increases (>100) coincident with low RH, low P, and Ta closer to 0°C. The findings corroborate the hypothesized mechanism of potential enhancement of ice nucleation at cloud boundaries, such as cloud-top generating cells and for ambient temperatures close to 0°C. The importance of using accurate droplet temperatures to improve existing primary ice nucleation parameterization schemes, especially in sub-saturated environments, is highlighted.

The impacts of droplet evaporative cooling on droplet lifetimes are compared with Maxwellian pure diffusion-limited evaporation approach under similar conditions. For higher RH and larger droplets, droplet lifetimes can increase by more than 100 s compared to those with droplet cooling ignored. Larger droplets (r0 ~ 30–50 µm) can survive at Tss for about 5 s to over 10 min, depending on the subsaturation of the environment. The impacts of droplet evaporative cooling on evolution of drop size distributions, using high-resolution direct numerical simulations of moderately supercooled mixed-phase cloud boundaries, are discussed.

How to cite: Roy, P., Rauber, R. M., Di Girolamo, L., Chen, S., Xue, L., and Tessendorf, S. A.: Can evaporative cooling of water droplets play a role in enhancing ice formation at moderately supercooled cloud boundaries?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14843, https://doi.org/10.5194/egusphere-egu25-14843, 2025.

EGU25-15228 | ECS | Posters on site | AS3.11

Constraining aerosol–cloud radiative forcing using present-day observations 

Hailing Jia, Willem Kroese, Johannes Quaas, Bastiaan van Diedenhoven, and Otto Hasekamp

The anthropogenic perturbation to cloud droplet number concentration (ΔlnNd) can be derived from the Nd-to-aerosol sensitivity in the present day (PD) (ßPD), and the anthropogenic perturbation to aerosol from the pre-industrial (PI) to PD. A key assumption in this process is that the PD aerosol-Nd relationship is indicative of the actual sensitivity of Nd to anthropogenic perturbation to aerosol, i.e., the PI-to-PD sensitivity (ßPI-PD). This assumption holds true only when using the cloud condensation nuclei at cloud base (CCNb) as the CCNb-Nd relationship is not dependent on aerosol regime. However, due to the difficulty in obtaining CCNb at a large scale, in practice one has to use proxies for the CCNb, which makes the above assumption less likely to hold. By combining multiple satellite observations, reanalysis, and AeroCom simulations, this study evaluates the performances of all existing proxies, and then constrain the radiative forcing from aerosol–cloud interactions (RFaci) by selecting ‘good’ proxies.

To assess whether a proxy-Nd relationship is aerosol-regime dependent, we propose a 'hemispheric contrast' approach, using the Northern and Southern Hemispheres to mimic the PD and PI aerosol environments, respectively. Under the same meteorological background, the hemispheric contrast in Nd at a certain aerosol amount serves as a measure of the aerosol-regime dependency. The results show that aerosol optical depth (AOD) exhibits the strongest dependency, followed sequentially by aerosol index (AI), sulfate burden (SO4C), surface sulfate mass (SO4S) and CCN burden (CCNc), and finally surface CCN (CCNS).

We further calculate the biases in RFaci caused by using ßPD instead of ßPI-PD in an ideal model world, based on the AeroCom model outputs. The results suggest that CCNS has the smallest bias (+3%), followed by AI, SO4S and CCNc with positive biases of ~+25%. The AOD and SO4C show the largest biases, with values of –60% and +80%, respectively.  Assuming CCNs would give the true RFaci, the biases in observation-based RFaci can be thus inferred, which turn out to be of similar magnitude to those in the model world. This gives us the confidence that true RFaci is likely around –0.68 W m-2 (ocean only).

How to cite: Jia, H., Kroese, W., Quaas, J., van Diedenhoven, B., and Hasekamp, O.: Constraining aerosol–cloud radiative forcing using present-day observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15228, https://doi.org/10.5194/egusphere-egu25-15228, 2025.

EGU25-15271 | ECS | Posters on site | AS3.11

Predicting Modal Aerosol Chemical Composition for Improved CCN Closure: A Boreal Forest Case Study 

Rahul Ranjan, Liine Heikkinen, Maura Dewey, Annica M. L. Ekman, Daniel Partridge, Lauri Ahonen, Tuukka Petäjä, Pasi P. Aalto, Krista Luoma, and Ilona Riipinen

Boreal forests are a significant natural source of aerosol particles. As anthropogenic emissions are expected to decline in the future, the relative contribution of boreal forest aerosols to cloud formation is likely to grow. Understanding the cloud-forming potential of these particles and accurately representing their effects in climate models is essential for assessing aerosol-cloud interactions. Previous research has highlighted the importance of aerosol particle number size distribution in predicting cloud condensation nuclei (CCN) concentrations, often outweighing uncertainties in overall aerosol composition. However, online measurement techniques typically provide data on total sub-micron particulate mass, without resolving chemical composition by size—a limitation that affects the accuracy of CCN predictions.

To address this limitation, we applied k-Köhler theory to evaluate how well observed and predicted CCN concentrations align, while simultaneously estimating size-resolved chemical composition. This approach leveraged an extensive dataset from the Hyytiälä research station in southern Finland, encompassing aerosol size distribution, CCN concentrations, and sub-micron aerosol composition derived from the Aerosol Chemical Speciation Monitor (ACSM) and an aethalometer. By exploring combinations of Aitken and accumulation mode compositions—expressed as mass fractions of organics, ammonium sulfate, and black carbon—we identified the composition that minimized prediction errors, achieving what we term "inverse CCN closure."

Our analysis of five years of data revealed distinct patterns in aerosol composition: inorganic compounds were enriched in the accumulation mode, while organics dominated the Aitken mode. This finding underscores the critical role of low-volatility organics in enabling the growth of newly-formed particles to CCN-relevant sizes, alongside the influence of aged aerosols from distant industrial sources and cloud-processed sulfate in the accumulation mode. Moreover, Aitken-mode particles were shown to contribute, sometimes substantially, to CCN concentrations in this boreal forest environment. These results highlight the necessity of investigating compositional differences between Aitken and accumulation mode particles to refine CCN predictions further. The uncertainty in the estimated modal aerosol chemical composition, stemming from measurement errors, will be quantified and presented.

This work was supported by the European Union’s Horizon 2020 research and innovation programme through the project FORCeS (grant agreement No. 821205) and the INTEGRATE project, funded by the European Research Council Consolidator Grant (No. 865799). Göran Gustafsson foundation is also gratefully acknowledged for financial support. Additional support for the SMEAR II station was provided by the University of Helsinki through ACTRIS-HY.

 

 

How to cite: Ranjan, R., Heikkinen, L., Dewey, M., Ekman, A. M. L., Partridge, D., Ahonen, L., Petäjä, T., Aalto, P. P., Luoma, K., and Riipinen, I.: Predicting Modal Aerosol Chemical Composition for Improved CCN Closure: A Boreal Forest Case Study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15271, https://doi.org/10.5194/egusphere-egu25-15271, 2025.

EGU25-15296 | ECS | Posters on site | AS3.11

Clouds' Clout on the Aerosol Size Distribution - Modelling Detailed Chemical Processing 

Levin Rug, Willi Schimmel, Fabian Hoffmann, and Oswald Knoth

Clouds have, by introducing the liquid phase as a chemical reaction chamber, the ability to change the aerosol size distribution. In as short as 40 minutes, the mass of an aerosol particle can increase by an order of magnitude due to chemical processing, with commensurate impacts on the precipitation efficiency and cloud optical properties. To study the chemical processing of aerosols in clouds, we developed the Chemical Mechanism Integrator (Cminor), a new, open-source, stand-alone Fortran environment for particle-based simulation of chemical multiphase mechanisms. Cminor employs advanced mathematical techniques tailored to heavily exploit the structure of chemical kinetic systems, multiple aqueous phases, and efficient evaluation of rate constants. Cminor uses the idea of Lagrangian cloud microphysics, i.e., computational particles, each representing a multitude of identical particles (e.g., aerosol particles of specific chemical composition). In addition to chemistry, Cminor predicts the activation of aerosol particles to cloud droplets and their subsequent growth by condensation, which enables us to directly investigate some impacts of the processed aerosol size distribution on cloud microphysics. While Cminor is currently applied in an adiabatic parcel framework, in which the influence of chemical processing on the aerosol size distribution is reliably captured, it will be coupled to a three-dimensional large-eddy simulation model shortly, which allows us to investigate the interactions of atmospheric chemistry, dynamics, and cloud physics with an unprecedented degree of detail.

How to cite: Rug, L., Schimmel, W., Hoffmann, F., and Knoth, O.: Clouds' Clout on the Aerosol Size Distribution - Modelling Detailed Chemical Processing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15296, https://doi.org/10.5194/egusphere-egu25-15296, 2025.

EGU25-15483 | ECS | Orals | AS3.11

Evidence of Anthropogenic Aerosols Impacts on the Southwestern U.S. Droughts since 1980 

Yan-Ning Kuo, Flavio Lehner, Isla Simpson, Clara Deser, Adam Phillips, Matthew Newman, Sang-Ik Shin, Spencer Wong, Julie Arblaster, and Hanjun Kim

The freshwater resources of the Southwestern United States (SWUS) largely depend on wintertime precipitation, which has declined since 1980. During this period, the tropical Pacific sea surface temperature (SST) has exhibited a multi-decadal La Niña-like trend, inducing a teleconnection that reduces SWUS precipitation. However, the extent to which this SST trend is driven by internal variability (i.e., natural fluctuations) versus anthropogenic radiative forcings remains uncertain. This study explores two aspects of the impact of anthropogenic aerosols on the Pacific sector and their influence on the wintertime SWUS precipitation trend. First, we demonstrate that the La Niña-like SST trend is partially forced by anthropogenic aerosols, as evidenced by simulations from the Community Earth System Model version 2 (CESM2) large ensemble and its single-forcing large ensemble. This forced La Niña-like SST trend, in turn, drives a decline in SWUS precipitation through its teleconnection. Second, we show that the teleconnection pattern associated with internal Pacific decadal variability during the post-1980 period differs from the pre-industrial condition. Specifically, using a hierarchy of model simulations, we find that even under El Niño-like SST trends, there is a tendency toward a North Pacific anticyclonic circulation trend and reduced SWUS precipitation during post-1980 — contrary to the canonical El Niño teleconnection. This unintuitive yet robust circulation change arises from nonadditive responses to tropical mean warming and radiative effects from anthropogenic aerosols. As the forced SWUS precipitation decline combines with anthropogenic warming, the post-1980 period exhibits the most rapid SWUS soil moisture drying among past and future periods of similar length. Although future projected El Niño-like warming and aerosol emission reductions could potentially reverse the precipitation trend, these changes are unlikely to mitigate the currently projected drought risk in the region.

How to cite: Kuo, Y.-N., Lehner, F., Simpson, I., Deser, C., Phillips, A., Newman, M., Shin, S.-I., Wong, S., Arblaster, J., and Kim, H.: Evidence of Anthropogenic Aerosols Impacts on the Southwestern U.S. Droughts since 1980, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15483, https://doi.org/10.5194/egusphere-egu25-15483, 2025.

EGU25-16293 | ECS | Orals | AS3.11

Anthropogenic aerosol-induced changes in radiative forcing and temperature over the Mediterranean 

Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, and Prodromos Zanis

Since the 1980s, the increase in greenhouse gases and the decrease in anthropogenic aerosols (AA) over Europe and the Mediterranean (MED), driven by air pollution control policies, along with anthropogenic land-use changes, have been linked to the enhanced regional warming trend in the MED, particularly during boreal summer (JJA). However, the effect of AA changes on the temperature trend over this region requires further investigation. This study examines temperature changes attributed to AA over the MED during the historical period (1850-2014) with respect to changes in effective radiative forcing (ERF) based on experiments from 11 CMIP6 Earth System Models. The transient shortwave ERF due to AA is assessed using the “histSST” and “histSST-piAer” experiments, which share the same historical forcings driven by prescribed sea surface temperatures and sea ice from the corresponding coupled models except that “histSST-piAer” uses pre-industrial aerosol precursor emissions from the year 1850. Shortwave ERFs due to aerosol-radiation interactions and aerosol-cloud interactions, as quantified by the approximate partial radiative perturbation (APRP) method,  present a negative peak in 1965-1984 relative to 1850 over the MED region (multi-model means of -2.17±0.82 W m-2 and -3.08±1.85 W m-2, respectively), exhibiting trends towards less negative values in recent past (1995-2014) relative to the 1965-1984 period (changing by 0.94±0.37 W m-2 and 0.51±1.02 W m-2, respectively). Furthermore, we quantify the response in near-surface air temperature (monthly mean, and daily maximum and minimum) caused by AA on an annual and seasonal basis using the “historical” and “hist-piAer” experiments, which are driven by historical forcings except that “hist-piAer” uses fixed pre-industrial AA and aerosol precursor emissions. Consistent with the negative ERF changes, we find a surface cooling of -1.23±0.56 K in the 1965-1984 period relative to 1850 on an annual basis. During 1995-2014 there is an annual mean increase of 0.25±0.36 K relative to 1965-1984 pointing towards an amplification of warming due to AA reduction. The regional surface warming in 1995-214 relative to 1965-1984 is more prominent in JJA (0.26±0.34 K) than in boreal winter (0.18±0.57 K) as models show lower agreement on the sign of change during wintertime. Similar results are derived for maximum and minimum temperatures regarding the magnitude and the trend of changes over the MED region.

This work is implemented within the research project REINFORCE (impRovEments in the simulation of aerosol clImate liNkages in earth system models: From glObal to Regional sCalEs) in the framework of HFRI call “Basic Research Financing (Horizontal Support of all Sciences)” under the National Recovery and Resilience Plan “Greece 2.0” funded by the European Union – NextGenerationEU (HFRI; project no. 15155).

How to cite: Kalisoras, A., Georgoulias, A. K., Akritidis, D., Allen, R. J., Naik, V., and Zanis, P.: Anthropogenic aerosol-induced changes in radiative forcing and temperature over the Mediterranean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16293, https://doi.org/10.5194/egusphere-egu25-16293, 2025.

EGU25-16348 | ECS | Orals | AS3.11

Impact of Asian aerosols on the summer monsoon strongly modulated by regional precipitation biases 

Zhen Liu, Massimo Bollasina, and Laura Wilcox

Attributing variations in the Asian summer monsoon to aerosol forcing is crucial for reducing uncertainties in future regional water availability projections. This is essential for effective risk management and adaptation planning in this densely populated region. However, accurately simulating the monsoon remains a significant challenge for climate models due to persistent biases, which compromise their reliability in attributing anthropogenic influences. In this study, we analyze a set of climate model experiments to uncover the connection between these biases and the monsoon’s response to Asian aerosols, focusing on the underlying physical mechanisms, including large-scale circulation changes. The impact of aerosols on monsoon precipitation and circulation is strongly shaped by a model's ability to represent the spatio-temporal variability in climatological monsoon winds, clouds, and precipitation across Asia. This variability modulates the magnitude and efficacy of aerosol–cloud–precipitation interactions, a key component of the total aerosol response. Our findings reveal a strong interplay between South Asia and East Asia monsoon precipitation biases, with their relative dominance significantly influencing the overall monsoon response. Notably, there is a sharp contrast between aerosol-driven changes during early and late summer, which can be attributed to the opposing signs and seasonal evolution of biases in these two regions. Realistically simulating the progression of large-scale atmospheric circulation is essential to fully capture the aerosol impact across Asia. These insights have significant implications for improving the understanding and reducing inconsistencies in model responses to aerosol changes over Asia, both in historical simulations and future projections.

How to cite: Liu, Z., Bollasina, M., and Wilcox, L.: Impact of Asian aerosols on the summer monsoon strongly modulated by regional precipitation biases, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16348, https://doi.org/10.5194/egusphere-egu25-16348, 2025.

EGU25-16380 | ECS | Posters on site | AS3.11

The Cloud-Aerosol Transition Zone from Satellite and Ground-Based Lidar Observations 

Jaume Ruiz de Morales, Josep Calbó, Josep-Abel González, Hendrik Andersen, Jan Cermak, Julia Fuchs, and Yolanda Sola

One of the main uncertainties in future climate projections is the cloud and aerosol contribution to the Earth’s radiative budget. The imprecise distinction between these aggregates of particles in suspension, combined with the transition zone within the cloud-aerosol continuum, further complicate the study of their radiative and climatic effects. Despite their importance, observations of the cloud-aerosol transition zone (TZ), particularly its vertical distribution, remain limited.

This study addresses this gap using a Vaisala CL31 ceilometer located at Girona (Spain), and the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) instrument on the CALIPSO satellite. For the ceilometer, we conducted a sensitivity analysis of backscatter and signal-to-noise ratio thresholds used for cloud detection in the Cloudnetpy algorithm from ACTRIS Cloudnet and considered as TZ all those cases where varying those thresholds (from relaxed to a strict situation) changed cloud detection. The CALIOP data was processed by applying several filters to avoid artifacts, and identifying the TZ as the atmospheric layers within the no-confidence range (NCR) of the CAD score, as well as the Cirrus fringes (CAD = 106). Such methodologies enabled the assessment of the vertical distribution and frequency of clouds, aerosols, and the TZ.

Overall, results indicate a gradual transition in backscatter retrievals from cloud to cloud-free, where suspended particles detected near cloud boundaries induced higher backscatter values than those found further away. From the local perspective, we observed a 9.3% (with an uncertainty range of 5.4─20%) variation in cloud occurrence attributed to TZ conditions. When analyzing the whole backscatter profile, we found as many TZ conditions as cloudy values, remarking the importance of TZ vertical frequency. Furthermore, the analysis of TZ occurrence in height and time in Girona revealed that these conditions tend to concentrate below 800 m during night periods. However, annual height-hour distributions showed remarkable seasonal variability. From the global perspective, TZ layers’ optical characteristics showed three main TZ groups:  1. Cluster 1, layers with properties between high-altitude ice clouds and aerosols (e.g. wispy cloud fragments); 2. Cluster 2, layers with properties between water clouds and aerosols at lower altitudes (e.g. hydrated aerosols); 3. Layers classified as Cirrus fringes. The TZ conditions were found worldwide, appearing in 9.5% of all profiles and comprising 6.4% of the filtered layers. The Cluster 1 and Cirrus fringes layers predominate near the ITCZ and in mid-latitudes. In contrast, Cluster 2 is more frequent over the oceans in the central West African and East Asian coasts where elevated smoke and dusty marine aerosols are common. Both ground-based and satellite approaches highlight the significant ubiquity and vertical frequency of the TZ.

How to cite: Ruiz de Morales, J., Calbó, J., González, J.-A., Andersen, H., Cermak, J., Fuchs, J., and Sola, Y.: The Cloud-Aerosol Transition Zone from Satellite and Ground-Based Lidar Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16380, https://doi.org/10.5194/egusphere-egu25-16380, 2025.

EGU25-16481 | Orals | AS3.11

Reconciling aerosol-cloud interactions through multiscale observations, modeling, and statistical techniques 

Harri Kokkola, Sami Romakkaniemi, Annele Virtanan, Daniel Partridge, Sara Blichner, Tero Mielonen, Silvia Calderón, Muhammed Irfan, Antti Lipponen, Timo Virtanen, Eemeli Holopainen, Pekka Kolmonen, Prithvi Raj Jallu, Dmitri Moisseev, Bernd Mom, and Antti Arola

Aerosol-cloud interactions remain one of the largest uncertainties in quantifying anthropogenic impacts on climate, particularly through their influence on cloud liquid water path (LWP), cloud droplet number concentration (CDNC), and cloud susceptibility to aerosol perturbations. This presentation synthesizes insights from satellite observations, large-eddy simulations, global climate models, long-term in-situ observations, and advanced statistical analyses to address biases and uncertainties in these interactions. Satellite-based studies often report a decreasing LWP with increasing CDNC, yet retrieval errors and natural spatial variability can mask positive LWP adjustments, leading to an underestimation of the cooling effects of aerosol-cloud interactions. Large-eddy simulations of marine stratocumulus clouds reveal that assumptions of adiabaticity and spatial variability in cloud properties contribute to biases in satellite-derived LWP-CDNC relationships. However, with careful case selection and well-defined meteorological conditions, satellite-based estimations can be improved. Building on these findings, global climate modeling and machine learning analyses highlight the importance of updraft velocity and aerosol size distributions in shaping the CCN-CDNC relationship. Advanced methods such as Elastic Net Regression isolate these confounding factors, refining susceptibility estimates and enhancing consistency with physical expectations. Further, long-term in-situ observations of aerosols and clouds at high-latitude locations reveal that the susceptibility of CDNC to CCN is significantly higher for low-level stratiform clouds than suggested by global oceanic satellite data. This implies stronger aerosol radiative forcing than current satellite-based estimates assume. Comparisons with Earth system models reveal large inter-model variability in susceptibility, driven by differences in sub-grid scale updraft velocities and aerosol size distributions. Even models with relatively accurate susceptibility values exhibit unrealistic underlying physics, highlighting areas for improvement in model representation. Lastly, combining satellite, reanalysis, and in-situ ACTRIS observations, we evaluate the roles of aerosol size distributions and updrafts in warm cloud formation, bridging gaps between microphysical processes and large-scale variability. This comprehensive approach emphasizes the need for integrating multi-platform observations with advanced modeling and statistical methods to reduce biases and improve the fidelity of aerosol-cloud interaction estimates. These advancements are crucial for more accurately quantifying aerosol radiative forcing and its implications for climate prediction.

How to cite: Kokkola, H., Romakkaniemi, S., Virtanan, A., Partridge, D., Blichner, S., Mielonen, T., Calderón, S., Irfan, M., Lipponen, A., Virtanen, T., Holopainen, E., Kolmonen, P., Raj Jallu, P., Moisseev, D., Mom, B., and Arola, A.: Reconciling aerosol-cloud interactions through multiscale observations, modeling, and statistical techniques, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16481, https://doi.org/10.5194/egusphere-egu25-16481, 2025.

EGU25-17097 | Orals | AS3.11

Long lived dusts from low latitudes may dominate primary ice production in polar regions 

Ross Herbert, Stephen Arnold, Benjamin Murray, and Ken Carslaw

For most regions of the world, the availability of mineral dust particles drives the production of primary ice in mixed-phase clouds. The mineral dust acts as an ice nucleating particle (INP), which facilitates the freezing of supercooled cloud droplets at higher temperatures than in its absence (~ -38C). Mixed-phase clouds are ubiquitous in the polar regions, but are far from the world’s primary sources of dust emissions in the tropics and subtropics. Secondary sources from high-latitude sources exist but do not fully explain observations of relatively high INP concentrations during the full annual cycle.

In this study we identify a previously overlooked source of low-latitude dust: those from long-lived dusts in smaller size modes that have been in the atmosphere for up to 5 months. Using simulations of the UK Earth System Model (UKESM), we find that although fresh dust contributes most of the dust mass in the polar regions, the INP contribution is weighted towards the older dust particles. In some regions, dust older than 90 days contributes over 50% of the total dust-sourced INP concentration. This occurs due to changes in the dust population size distribution, and has important implications. Close to primary dust sources, the INP concentration is dependent on the super-micron particles, whereas far from the source (i.e. the polar regions and remote oceans) the INP concentration is dependent on the smaller, older, sub-micron particles.

How to cite: Herbert, R., Arnold, S., Murray, B., and Carslaw, K.: Long lived dusts from low latitudes may dominate primary ice production in polar regions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17097, https://doi.org/10.5194/egusphere-egu25-17097, 2025.

EGU25-17259 | ECS | Orals | AS3.11

Investigating Secondary Ice Production effects on wintertime orographic clouds using the Regional Atmospheric Modelling System (RAMS) 

Ioannis Chaniotis, Paraskevi Georgakaki, Platon Patlakas, Romanos Foskinis, Nicole Clerx, Carolina Molina, Maria Gini, Paul Zieger, Konstantinos Eleftheriadis, Alexis Berne, Alexandros Papayannis, Mika Komppula, Helena Flocas, and Athanasios Nenes

In recent years, there has been a breakthrough in the identification and description of various secondary ice production (SIP) mechanisms that affect mixed-phase clouds. However, SIP is in general not described well in climate and mesoscale models, which leads to notable biases in the representation of warm mixed-phase clouds in terms of ice content, ice number concentration and cloud structure. In this study, the Integrated Community Limited Area Modelling System (ICLAMS) has been utilized to examine the formation and evolution of wintertime orographic clouds over Mt. Helmos, Greece. ICLAMS is a special version of the Regional Atmospheric Modelling System (RAMS). In addition to the Hallett-Mossop process, already included in the model, two additional SIP mechanisms are implemented, a) collisional break-up of ice particles and b) droplet shattering. Model results are evaluated against in-situ and remote sensing observations collected during the CleanCloud CHOPIN campaign (https://go.epfl.ch/chopin-campaign) at Mt. Helmos in the Peloponnese, Greece during Fall 2024 to Spring 2025. Remote sensing (wind lidar and cloud radar) data are used to evaluate model performance, through the application of forward operators (cloud radar simulator) and comparison with radar reflectivity and turbulence parameters. The mesoscale model simulations indicate that SIP enhances aggregation and results in clouds with increased ice crystal number concentrations, aligning more closely with observed distributions. Among the SIP mechanisms, collisional break-up is identified as the dominant contributor to simulated SIP rates, underscoring its critical role in accurately representing orographic mixed-phase clouds.

How to cite: Chaniotis, I., Georgakaki, P., Patlakas, P., Foskinis, R., Clerx, N., Molina, C., Gini, M., Zieger, P., Eleftheriadis, K., Berne, A., Papayannis, A., Komppula, M., Flocas, H., and Nenes, A.: Investigating Secondary Ice Production effects on wintertime orographic clouds using the Regional Atmospheric Modelling System (RAMS), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17259, https://doi.org/10.5194/egusphere-egu25-17259, 2025.

This research attempts to reassess, using observation and latest literature studies, the importance of anthropogenic aerosol changes over the past 6000 years to present on regional and global climate forcings and its strong impact on the rate of climate change. Recent research studies (Hansen et al. 2023 & 2025) reveals that a better assimilation of higher aerosol forcing can help to explain the Holocene (temperature) conundrum (a stable Holocene climate, while greenhouse concentrations increased). Such an aerosol forcing has strong impact on paleo- and present climate change.

To this day, pre-industrial anthropogenic aerosol forcing sources remain, including harmful slash and burn agriculture and biomass cooking. But regulations and technologies for aerosol mitigation are present and in the pipeline. 

This contributes to regional and global forcing changes, combined with mitigation from industrial aerosol sources like coal plant desulphurisation and notably, since the implementation of stringent sulphur regulations by the International Maritime Organization (IMO) in 2015 and 2020, mitigation of aerosols and aerosol cloud interactions over the dark (low albedo), relatively cold oceans, which act as the primary planetary heat sink of Earth’s Energy Imbalance. More strict regional sulphur regulations will soon come into effect.

Recent forcing estimates from IMO regulations vary widely, from only 0.08 W/m² based on a simple climate model (Hausfather & Forster 2023 using FaIR) to up to 0.50 W/m² based on observations (Hansen et al. 2025). Our analysis, based on NASA CERES satellite data, reveals that the active shipping region of the North Atlantic (20-60N) has experienced a 4-year averaged increase in Absorbed Solar Radiation of 3.0 W/m² and a regional Net flux increase of 1.4 W/m² since 2014, with estimated impacts on regional warming, extreme weather and on the Atlantic Meridional Overturning Circulation (AMOC).

These rapid reductions in aerosol (precursor) emissions combined with a high greenhouse gas (GHG) forcing (currently about +4 W/m² above 1750) may lead to regional, and potentially global, aerosol termination shocks, whereby the reduction of aerosols in absence of GHG reductions increases the rate of warming by >0.2°C/dec. And latest observations are already signalling a potential earlier than anticipated approach to climate tipping points (incl. coral reef die-off; AMOC slow down; and reducing Amazon rainforest and boreal forest carbon sinks), with underestimated climate sensitivities.

Because strong scientific uncertainties remain, we highlight the necessity, from a precautionary principle perspective, to urgently re-evaluation of regional and global climate models to better acknowledge and incorporate these aerosol changes and for policymakers to prepare for scenarios where previously considered 'safe' pathways might accelerate towards dangerous climate thresholds. 

For mitigation, we advocate for policies that consider the full lifecycle impacts of emissions, including the unintended consequences of pollution control measures.

 

How to cite: Simons, L. and Dufournet, Y.: The Case for a Pre-industrial Aerosol Forcing and Impacts of Cleaner Air on Regional Climate Change: Urgent Call for Precautionary Mitigation and Adaptation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17621, https://doi.org/10.5194/egusphere-egu25-17621, 2025.

EGU25-18015 | ECS | Orals | AS3.11

Quantification of aerosol influence on day-to-day mesoscale variability of shallow convection 

Hauke Schulz, Robert Wood, and Bjorn Stevens

A major uncertainty in the cloud-feedback to a warming climate can be attributed to shallow convection in the trades. With recent advances in observational and computational resources, the potential impact of the mesoscale organization of these clouds became apparent. While the processes leading to the mesoscale organization are not resolved in current climate models, observations of these features and more importantly their interaction with different scales became available through field campaigns like EUREC4A.

This study quantifies the ability of large-domain large-eddy simulations to represent the observed mesoscale variability in cloudiness. By using forward operators to mimic the observations, we show that the stratiform cloud amount and precipitation frequency remain challenging to simulate at hectometre resolutions. Despite these challenges, the simulations show a similar sensitivity in cloud distribution to environmental conditions.

By perturbing the 41 days simulation with a 13-fold increase in CCN concentration we quantify the sensitivity of the mesoscale cloud organisation to changes in precipitation and show the strong influence on the cold-pool driven cloud formations. We further emphasise the importance to correctly represent the mesoscale processes in climate simulations by showing that changes in cloud-radiative effects due to aerosol changes vary day-by-day with varying contributions from changes in cloud albedo and cloud fraction.

How to cite: Schulz, H., Wood, R., and Stevens, B.: Quantification of aerosol influence on day-to-day mesoscale variability of shallow convection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18015, https://doi.org/10.5194/egusphere-egu25-18015, 2025.

EGU25-18206 | ECS | Posters on site | AS3.11

Retrieving Microphysical Properties of Arctic and Mediterranean clouds using a synergy of remote sensing and in situ instrumentation 

Romanos Foskinis, Nicole Clerx, Carolina Molina, Christos Mitsios, Kaori Kawana, Marilena Gidarakou, Prodromos Fetfatzis,  Maria I. Gini,  Olga Zografou,  Konstantinos Granakis,  Stefano Decesari, Marco Paglione, Paul Zieger, Aiden Jönsson, Kalliopi Violaki, Anne-Claire Marie Billault-Roux, Lu Zhang, Varun Kumar, Thierry Podvin, Gaël Dubois, Mika Komppula, Lise Lotte Sørensen, Bjarne Jensen, Christel Christoffersen, Silvia Henning, Sven-Erik Gryning, Andreas Massling, Henrik Skov, Ulas Im, Konstantinos Eleftheriadis, Alexandros Papayannis, Alexis Berne, and Athanasios Nenes

Aerosol-Cloud Interactions (ACI) play an important role in the hydrological cycle and are strong modulators of cloud radiative forcing and climate. Nevertheless, they remain poorly understood and constrained despite decades of research, because many processes and feedbacks are highly uncertain and are challenging to describe in regional and global climate models. Even less understood is the role of natural aerosol and ACI in a post-fossil future, where anthropogenic emissions is vastly reduced but emerging “natural” aerosol sources modulated by anthropogenic climate change (biomass burning, bioaerosols, dust) will dominate. The CleanCloud project aims to address these uncertainties and as part of its activities carries out major observational field campaigns at climate hot spots (Arctic, Mediterranean) to better constrain ACI processes, and, evaluate, improve and develop new remote sensing algorithms for studying aerosols, clouds and ACI.

The first CleanCloud campaign was based at the Villum Research Station (81.6° N, 16.6° W) in North Greenland, with in-situ and remote sensing measurements, and consisted of two phases, one during the spring (16 March – 13 April) and one during summer (16 July – 13 August) of 2024, in collaboration with the NASA ARCSIX aircraft mission. The second campaign, named “Cleancloud Helmos OrograPhic site experimeNt (CHOPIN)”, is ongoing and is anticipated to last for 6 months, starting from 1 October at Mt.Helmos (38.0o N, 22.2o E) in the Peloponnese, Greece. A series of in situ and remote sensing measurements were distributed at 6 sites along the lee side of Mt. Helmos, 4 at the Kalavrita ski Center’s parking lot (altitude ~ 1690 m), 1 at the foothills (altitude ~ 1747 m) and the Helmos Hellenic Atmospheric Aerosol and Climate Change station ((HAC)2) at the mountaintop (altitude ~ 2314 m) constrain almost every aspect of the aerosols, clouds and their interaction in the region – and especially in the orographic clouds that form at the (HAC)2 station.

Here, we present results from these two campaigns to examine the cloud (e.g., droplet number concentration & size) and aerosol microphysical characteristics (size distribution, CCN concentrations, chemical composition, bioaerosol number concentration and type) and cloud-scale dynamical forcing (vertical velocity) to understand their contribution to ACI processes. Radiosondes to derive the vertical structure of the atmosphere, Lidar systems and sun photometers were used to determine the presence of aerosol amount, their altitude and type (bioaerosol, dust, pollution, biomass burning) as well as the aerosol optical and columnar microphysical properties, Doppler lidars for turbulence and cloud-scale dynamics, radars to obtain the microphysical properties of the clouds, and finally satellites to retrieve the spatio-temporal evolution of the clouds. Additionally, in the case of CHOPIN campaign, cloud probes and cloud samplers were used to perform in-cloud sampling and to obtain the cloud microphysical properties. Thus, the use of this synergistic approach enables us to perform closure studies and to improve our current retrievals to predict cloud properties. These extensive field campaigns will aid in developing new ACI-related retrieval algorithms, development/improvement of parameterizations, and the ESA EarthCARE calibration/validation activities.

How to cite: Foskinis, R., Clerx, N., Molina, C., Mitsios, C., Kawana, K., Gidarakou, M., Fetfatzis, P., Gini,  . I., Zografou,  ., Granakis,  ., Decesari,  ., Paglione, M., Zieger, P., Jönsson, A., Violaki, K., Billault-Roux, A.-C. M., Zhang, L., Kumar, V., Podvin, T., Dubois, G., Komppula, M., Sørensen, L. L., Jensen, B., Christoffersen, C., Henning, S., Gryning, S.-E., Massling, A., Skov, H., Im, U., Eleftheriadis, K., Papayannis, A., Berne, A., and Nenes, A.: Retrieving Microphysical Properties of Arctic and Mediterranean clouds using a synergy of remote sensing and in situ instrumentation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18206, https://doi.org/10.5194/egusphere-egu25-18206, 2025.

EGU25-18210 | ECS | Orals | AS3.11

Combining spaceborne observations of CCN, INP, and cloud development for assessing ACI in liquid and ice-containing clouds 

Fani Alexandri, Felix Müller, Goutam Choudhury, Torsten Seelig, Peggy Tesche-Achtert, and Matthias Tesche

Last year, we presented the Cloud-by-Cloud (CxC) approach for studying aerosol-cloud interactions (ACI) through a combination of observations with polar-orbiting and geostationary satellites. Specifically, cloud-relevant aerosol concentrations at cloud level are matched to individual clouds that are observed throughout their life time.

The methodology has now been applied to 11 years of data from MSG-SEVIRI and the CALIPSO lidar over Europe and northern Africa. The resulting data set of several thousand matched aerosol-cloud cases provides a first satellite-based assessment of ACI in warm and cold clouds in which the aerosol component is expressed in actual number concentrations of cloud condensation nuclei (nCCN) and ice nucleating particles (nINP) at cloud level. We present findings of the aerosol impact on cloud droplet number concentration, effective radius, liquid water path and cloud phase for different aerosol types and discuss differences to the conventional data-aggregation approach in which aerosols are expressed through aerosol optical depth.

How to cite: Alexandri, F., Müller, F., Choudhury, G., Seelig, T., Tesche-Achtert, P., and Tesche, M.: Combining spaceborne observations of CCN, INP, and cloud development for assessing ACI in liquid and ice-containing clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18210, https://doi.org/10.5194/egusphere-egu25-18210, 2025.

EGU25-18274 | ECS | Posters on site | AS3.11

Novel measures for diagnosing and evaluating entrainment-mixing in warm and mixed-phase clouds using airborne, in situ measurements 

John Dalessandro, Robert Wood, Peter Blossey, and Greg McFarquhar

Multiple methods using in situ observations exist to evaluate cloud microphysical characteristics associated with entrainment-mixing. These include comparing average drop sizes with drop concentrations, comparing these quantities weighted by their adiabatically derived values, as well as computing theoretically derived mixing parameters (e.g., Damköhler number [Dimotakis 2005] and transition length scale [Lehmann et al. 2009]). Although multiple methods exist to quantify entrainment-mixing, observational studies often incorporate a number of these methods due to a wide range of variability in the methods’ output. Further, multiple uncertainties exist when computing these parameters, ranging from required assumptions for determining adiabatic values to sampling limitations preventing the diagnosis of the entrained air’s humidity. For these reasons, most observational studies only evaluate a select number of flight legs due to the diligent analysis required case-by-case.

To compensate for such discrepancies, we introduce a novel method to diagnose the presence of entrainment by using the variance of drop concentrations on the order of ~100 m as a proxy variable. Drop concentrations are acquired using a commonly deployed cloud droplet probe (CDP) at ~10 m spatial resolutions. These basic factors allow for the dissemination of entrainment-mixing characteristics amongst hundreds of hours of cloud measurements acquired during numerous field campaigns.

Findings using this proxy variable suggest that the greatest ice crystal sizes in low-level mixed-phase clouds over the Southern Ocean are found in cloud samples associated with relatively weak entrainment (D’Alessandro and McFarquhar 2023). The methodology is further developed to evaluate how drop size distributions evolve in the presence of entrainment-mixing, revealing greater frequencies of inhomogeneous (homogeneous) mixing associated with high (low) aerosol environments and non-precipitating (precipitating) clouds in subtropical marine environments (D’Alessandro et al. submitted). Occurrence frequencies of inhomogeneous and homogenous mixing are approximately similar amongst four field campaigns, which sampled cloud regimes ranging from low-level warm and mixed-phase marine clouds to terrestrial, convective clouds. Additionally, the methodology in conjunction with measurements from the HOLODEC probe suggest the potential of droplet growth in the “bottleneck” size range (diameters ~25–50 µm) in the presence of entrainment.

 

Bibliography

D’Alessandro, J. J., and G. M. McFarquhar, 2023: Impacts of Drop Clustering and Entrainment-Mixing on Mixed Phase Shallow Cloud Properties Over the Southern Ocean: Results From SOCRATES. Journal of Geophysical Research: Atmospheres, 128, e2023JD038622, https://doi.org/10.1029/2023JD038622.

D’Alessandro, J. J., R. Wood, and P. N. Blossey, submitted: Evaluating entrainment-mixing characteristics through direct comparisons of drop size distributions using in situ observations from ACE-ENA. J. Atmos. Sci.

Dimotakis, P. E., 2005: TURBULENT MIXING. Annual Review of Fluid Mechanics, 37, 329–356, https://doi.org/10.1146/annurev.fluid.36.050802.122015.

Lehmann, K., H. Siebert, and R. A. Shaw, 2009: Homogeneous and inhomogeneous mixing in cumulus clouds: Dependence on local turbulence structure. Journal of the Atmospheric Sciences, 66, 3641–3659, https://doi.org/10.1175/2009JAS3012.1.

 

How to cite: Dalessandro, J., Wood, R., Blossey, P., and McFarquhar, G.: Novel measures for diagnosing and evaluating entrainment-mixing in warm and mixed-phase clouds using airborne, in situ measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18274, https://doi.org/10.5194/egusphere-egu25-18274, 2025.

EGU25-18461 | ECS | Posters on site | AS3.11

Cloud observations over Limassol, Cyprus using CLOUDNET facilities 

George Kotsias, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, and Patric Seifert

This study utilizes the results of the Cyprus Cloud Aerosol and Radiation Experiment (CyCARE) campaign that took place in Limassol, Cyprus, during the period October 2016 - March 2018. The cloudnet target classification scheme was followed for the retrieval of cloud geometrical and microphysical properties and a climatological statistical analysis was applied for the investigation of cloud seasonal variability and characteristics. Of the total number of 1,338,785 available vertical profiles 440,377 (33%) were found to contain hydrometeors. The applied statistical analysis revealed that, in the presence of clouds, ice phase has appeared in 86% of the cases, mixed phase was identified in 43% of the cases, and liquid phase was observed in 42% of the cases. Precipitation (drizzle or rain) occurred in 28% of the cases. The seasonal analysis showed that clouds over Limassol during the study period are more frequent during the winter season (60%) followed by spring (22%) and autumn (17%). The most frequent cloud type is mixed phased clouds (354,440 profiles), followed by pure ice clouds (251,402) and liquid phase clouds (125,838). Concerning the cloud geometrical characteristics, cloud base height ranged from a median value of 1478 m for liquid precipitable clouds during winter to 9803 m for ice clouds during summer. Cloud top height varied from a median value of 1977 m for liquid precipitable clouds during winter to 10271 m for ice clouds during summer. Cloud vertical thickness ranged from a median of 249 m for liquid clouds during spring to 5519 m for mixed phase precipitable clouds during spring. Since June 2024 a new permanent ground-based remote sensing station, namely Cyprus Aerosol Remote sensing Observatory  (CARO), has been established in Limassol and the continuous observations will be used in future aerosol-cloud interaction relevant studies in the region of eastern Mediterranean.

Acknowledgements

The authors acknowledge the ‘EXCELSIOR’: ERATOSTHENES: EΧcellence Research Centre for Earth Surveillance and Space-Based Monitoring of the Environment H2020 Widespread Teaming project (www.excelsior2020.eu). The ‘EXCELSIOR’ project has received funding from he European Union’s Horizon 2020 research and innovation programme under Grant Agreement No 857510, from the Government of the Republic of Cyprus through the Directorate General for the European Programmes, Coordination and Development and the Cyprus University of Technology. This study was supported by the ATARRI Horizon Europe Widespread Twinning Project. ATARRI receives funding from the European Union’s Horizon Europe Twinning Call (HORIZON-WIDERA-2023-ACCESS-02) under the grant agreement No 101160258.

How to cite: Kotsias, G., Mamouri, R.-E., Nisantzi, A., and Seifert, P.: Cloud observations over Limassol, Cyprus using CLOUDNET facilities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18461, https://doi.org/10.5194/egusphere-egu25-18461, 2025.

EGU25-18479 | Posters on site | AS3.11

Anthropogenic aerosol effects on convective clouds and precipitation in global km-scale simulations with ICON-HAM-lite  

Philip Stier, Philipp Weiss, Sadhitro De, Maor Sela, and William Jones

Aerosol effects on convective clouds and precipitation mediated via radiative and microphysical perturbations remain highly uncertain. Microphysical perturbations are generally not included in current climate models due to the simplified representation of convective clouds in existing parameterisations. Progress has been made through regional cloud resolving modelling; however, such simulations often neglect energy and water budget constraints and the coupling to larger scales. The emergence of global km-scale climate models provides a significant opportunity to advance our understanding of aerosol-convection interactions, but the inclusion of prognostic aerosols has been limited previously by their high computational demands.

Here we present results from global km-scale atmospheric model simulations using ICON coupled to HAM-lite, a new reduced complexity aerosol model derived from the microphysical aerosol scheme HAM, suitable for global km-scale simulations [Weiss et al., GMD Discussions, 2024]. Performing aerosol perturbation experiments with pre-industrial and present-day aerosol emissions allows us to isolate anthropogenic aerosol effects on convective clouds and precipitation globally. As a first step, we compare simulated perturbations in terms of radiative (aerosol optical depth) and microphysical (cloud droplet number concentrations) against a set of observationally constrained idealised perturbations [Herbert et al., ACP Discussions, 2024]. This will allow us to put simulated cloud and precipitation responses in the simulations in the context of the perturbation strength.

Comparison of our global km-scale simulations with prognostic aerosols with idealised simulations with prescribed aerosols [Herbert et al., 2024] provides a first insight into the effect of simulating global aerosols at the km-scale. Ultimately, this work offers a new way to study anthropogenic aerosol effects on convective clouds and precipitation globally, including microphysical and radiative perturbations, the diurnal cycle of convection, the coupling to the global circulation and regional climate.

How to cite: Stier, P., Weiss, P., De, S., Sela, M., and Jones, W.: Anthropogenic aerosol effects on convective clouds and precipitation in global km-scale simulations with ICON-HAM-lite , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18479, https://doi.org/10.5194/egusphere-egu25-18479, 2025.

EGU25-18569 | Posters on site | AS3.11

High-Resolution Insights from the Max Planck CloudKite During EUREC4A 

Gholamhossein Bagheri, Freja Nordsiek, Oliver Schlenczek, Birte Thiede, Yewon Kim, Venecia Chavezmedina@ds.mpg.de, Mike Larsen, Marcel Schroeder, and Eberhard Bodenschatz

We present the first results from the Max Planck CloudKite (MPCK) measurements conducted during the EUREC4A campaign in 2020, targeting shallow cumulus clouds in the trade wind regions near Barbados. The MPCK is a 250 m³ tethered balloon stabilized with a kite, capable of carrying up to 100 kg of scientific payload in no-wind conditions or heavier payloads in windy conditions, reaching altitudes of up to 2 km above ground level. During EUREC4A, we performed airborne measurements of cloud microphysics and turbulence using the MPCK+ instrument box, which combines fast inline holography with Particle Image Velocimetry (PIV) to resolve micrometer-scale features. The low true airspeed of the tethered balloon, combined with the high sampling frequencies of our imaging setups—15 Hz for PIV and 75 Hz for holography—provided unprecedented detail into the dynamics of shallow cumulus clouds. To date, we have analyzed over 300,000 holograms and 100,000 PIV images acquired during the campaign. Our analysis spans the structure of these clouds from their edges to their cores. We present results on droplet clustering, void formations, the influence of turbulence, and the mechanisms of entrainment and mixing. As clouds remain a major source of uncertainty in climate and weather models, we believe these findings represent a significant step forward in understanding cloud dynamics and their broader implications for atmospheric processes. 

How to cite: Bagheri, G., Nordsiek, F., Schlenczek, O., Thiede, B., Kim, Y., Chavezmedina@ds.mpg.de, V., Larsen, M., Schroeder, M., and Bodenschatz, E.: High-Resolution Insights from the Max Planck CloudKite During EUREC4A, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18569, https://doi.org/10.5194/egusphere-egu25-18569, 2025.

EGU25-18825 | ECS | Orals | AS3.11

Simulating shipping impacts on clouds in a high-resolution weather model 

Anna Tippett, Edward Gryspeerdt, and Paul Field

Aerosol-cloud interactions remain a significant source of uncertainty in our understanding of climate change. Ship emissions provide a unique natural experiment, artificially brightening clouds through the injection of aerosols that act as cloud condensation nuclei. These "ship tracks" offer a valuable opportunity to evaluate the impacts of aerosols on clouds. Comparing satellite observations of aerosol-cloud interactions with model simulations is often challenging. Direct case studies of natural experiments, such as those involving ship tracks, allow for more precise investigation of the representation of physical processes in models, enabling a clearer assessment of where models succeed or fail. Such simulations are also critical for evaluating the potential of marine cloud brightening as a climate intervention strategy.  

In this study, we simulate ship tracks using the UK Met Office Unified Model in km-scale resolution. By incorporating real ship locations and representing ships as moving aerosol sources within a two-moment cloud microphysics and coupled aerosol scheme, we successfully reproduce the cloud droplet number concentration of observed ship tracks for a specific day in a hindcast (relative to observations). Direct comparisons between these simulated tracks and MODIS satellite observations reveal differences in the model’s ability to represent the magnitude and timescales of cloud and precipitation processes, such as the LWP adjustments to aerosols and the width/depth of the resultant ship tracks. These comparisons shed light on the requirements for accurately simulating ship tracks. 

To further investigate the representation of aerosol-cloud interactions within models, we examine the sensitivity of aerosol impacts to grid resolution. This analysis addresses a critical question for scaling high-resolution simulations to global climate models (GCMs): Can small-scale constraints (such as ship tracks) reliably constrain the parametrisations of large-scale models? We explore whether the scaling of aerosol effects from high resolution models to GCM resolutions are linear or if saturation and concentration effects must be considered. The findings from this study contribute to improving the representation of aerosol-cloud interactions in models and enhancing our understanding of their role in climate systems. 

How to cite: Tippett, A., Gryspeerdt, E., and Field, P.: Simulating shipping impacts on clouds in a high-resolution weather model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18825, https://doi.org/10.5194/egusphere-egu25-18825, 2025.

EGU25-19341 | Orals | AS3.11

Fluorescent primary bioaerosol particle measurements in mixed phase cloud residuals at Mount Helmos, Greece 

Aiden Jönsson, Paul Zieger, Konstantinos Eleftheriadis, Maria Gini, Kaori Kawana, Athanasios Nenes, Carolina Molina, Prodromos Fetfatzis, Romanos Foskinis, Julia Asplund, Lea Haberstock, and Kouji Adachi

The partitioning between liquid- and ice-phase cloud water content can have a substantial impact on the cloud’s radiative effect and on precipitation. This partitioning is expected to change on average with global warming due to warmer temperatures, more atmospheric moisture, and different cloud nucleating particle distributions, which then feed back into the changing climate. Changes in mixed phase clouds (MPCs)  are difficult to predict due to the complexity of microphysical processes that determine cloud phase partitioning and the uncertainty of future aerosol emissions, both natural and anthropogenic. The characteristics of MPCs are particularly sensitive to the availability of ice-nucleating particles (INPs), which are generally few in number relative to overall aerosol concentrations. Primary bioaerosol emissions are understood to be important to INP availability, making these aerosols and the processes affecting them critical to understanding how clouds and precipitation might change with global warming and with different anthropogenic emissions.

The CleanCloud project under which this research is conducted targets these aerosols and MPCs in order to improve our understanding and climate predictions of a post-aerosol drawdown and warmer world with different natural aerosol sources. We present preliminary observations from the CleanCloud Helmos Orographic SIte Experiment (CHOPIN) campaign targeting primary bioaerosols at the Helmos Hellenic Atmospheric Aerosol Climate Change Station (HAC2) on Mount Helmos in the Peloponnese peninsula, southern Greece, carried out between October 2024 and April 2025. At an altitude of 2314 m, atmospheric conditions at HAC2 are at times within the planetary boundary layer and otherwise more representative of the free troposphere. During wintertime at this altitude, MPCs can be frequently observed at HAC2. We employed a ground-based counterflow virtual impactor (GCVI; Brechtel Industries) in order to sample clouds and observe cloud residuals using a multiparameter bioaerosol spectrometer (MBS; CAIR, University of Herefordshire), scanning electrical mobility spectrometer (SEMS; Brechtel Industries), and a portable ice nucleation experiment (PINE; EPFL). Samples were also taken for offline analysis with transmission electron microscopy (TEM; MRI-JMA).

We present a preliminary overview of fluorescent primary bioaerosol particle (fPBAP) measurements at HAC2 in both cloud residuals and whole air as part of the CHOPIN campaign. We relate these to observed INP concentrations measured by the PINE, and to cloud properties measured by a fog monitor (FM120; DMT, Inc.) and a ground-based fog and aerosol sensor (GFAS; DMT, Inc.).

How to cite: Jönsson, A., Zieger, P., Eleftheriadis, K., Gini, M., Kawana, K., Nenes, A., Molina, C., Fetfatzis, P., Foskinis, R., Asplund, J., Haberstock, L., and Adachi, K.: Fluorescent primary bioaerosol particle measurements in mixed phase cloud residuals at Mount Helmos, Greece, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19341, https://doi.org/10.5194/egusphere-egu25-19341, 2025.

EGU25-19417 | ECS | Orals | AS3.11

Short time-scale evolution of aerosol-cloud interactions 

Vishnu Nair and Edward Gryspeerdt

The difficulty in establishing causality between stratocumulus cloud droplet number concentration (Nd) and liquid water path (LWP) is well established. Recent studies on the satellite observations of the development of clouds over short time scales to examine the role of Nd perturbations in LWP variations demonstrated that LWP evolved differently depending on the initial Nd. This highlighted the need to consider the temporal development rather than the instantaneous measurements.

Here we characterise the dependence of this short timescale behaviour on the local meteorological environment, with aerosol production, entrainment from the free troposphere and wet scavenging all acting to modify the Nd. Many of these effects act to further steepen the Nd–LWP relationship and obscure the causal Nd impact on LWP. The multi-dimensional process space to represent stratocumulus is reduced to the two-dimensional Nd-LWP state space. The role of different physical processes is investigated and process-level fingerprints are extracted in this space.

How to cite: Nair, V. and Gryspeerdt, E.: Short time-scale evolution of aerosol-cloud interactions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19417, https://doi.org/10.5194/egusphere-egu25-19417, 2025.

EGU25-19436 | Orals | AS3.11

Influence of free tropospheric aerosols on the microphysical properties of a coupled low-level cloud in the central Arctic: a case study from the ARTofMELT expedition.  

Roman Pohorsky, Radiance Calmer, Berkay Dönmez, Ian Brooks, Heather Guy, Lea Haberstock, Julia Kojoj, Nicolas Fauré, Sonja Murto, Camille Mavis, Jessie Creamean, Michael Tjernström, Paul Zieger, and Julia Schmale

Low-level mixed-phase clouds (LLMPCs) containing both ice and supercooled liquid water are ubiquitous in the Arctic and play a crucial role for radiative fluxes. Mixed-phase clouds are inherently instable due to the competition over water between ice crystals and liquid droplets. The persistence of LLMPCs in the Arctic is challenging to reproduce in models, which affects predictions of the energy budget. These challenges stem from current uncertainties related to the complex web of interactions between aerosol particles, cloud microphysics, atmospheric (thermo-)dynamics and surface processes. These uncertainties can be partly attributed to the scarcity of detailed observations of aerosol characteristics and cloud microphysical properties as well as their interactions within clouds.

LLMPCs highly depend on the presence of aerosol particles acting as cloud condensation nuclei (CCN) or ice nucleating particles (INPs). In the Arctic, where aerosol concentrations can be very low, small changes in aerosol properties (e.g., size, chemical composition, hygroscopicity) can significantly impact the radiative properties and lifetime of LLMPCs. Accurate knowledge of aerosol characteristics at cloud level and their influence on cloud properties is crucial for improving the representation of clouds and their radiative behavior.

To address the need for more observations of aerosols and cloud properties at cloud level, a tethered-balloon equipped with the Modular Multiplatform Compatible Air Measurements System (MoMuCAMS) was deployed from the Swedish icebreaker Oden during the Atmospheric River and onset of sea ice melt (ARTofMELT) expedition. The expedition took place in the Fram Strait during the transition from spring to summer (May – June) in 2023. In total, 23 flights up to 645 m above mean sea level were performed, collecting unique and detailed measurements of aerosol and cloud droplet size distributions from 8 nm to 50 µm, below, inside and above LLMPCs. A key aspect addressed with the measurements is how boundary layer and free tropospheric aerosols contribute to the formation of clouds.

Results from of a case study examining the data collected from three consecutive flights through a single cloud layer located between roughly 150 and 350 meters above the surface will be presented. A combination of in situ vertical and surface-based measurements with remote sensing data and modeling studies is used to understand to what extent aerosols from below and above the cloud contribute to the formation of cloud droplets. Results indicate that the cloud is coupled to the surface and profiles of particle number size distributions show a homogenous distribution between the surface and the cloud. A comparison between estimated CCN concentrations below and above the cloud and observed cloud droplet number concentrations suggests however, that entrainment of aerosol from the free troposphere is needed to produce the amount of droplets observed.

These observations suggest that also when clouds are coupled to the surface, a different and significant source of CCN and INPs can feed the cloud from above, which is then not observable from surface-based measurements. This can have important implications for the representation of cloud microphysical and radiative properties based solely on surface-based observations.

How to cite: Pohorsky, R., Calmer, R., Dönmez, B., Brooks, I., Guy, H., Haberstock, L., Kojoj, J., Fauré, N., Murto, S., Mavis, C., Creamean, J., Tjernström, M., Zieger, P., and Schmale, J.: Influence of free tropospheric aerosols on the microphysical properties of a coupled low-level cloud in the central Arctic: a case study from the ARTofMELT expedition. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19436, https://doi.org/10.5194/egusphere-egu25-19436, 2025.

An understanding of aerosol-cloud interactions is key to many areas of climate science due to the diversity of mechanisms by which clouds interact with the Earth’s climate. One such area of growing interest is Climate Intervention – deliberately altering the climate to counteract anthropogenic Climate Change. Many Climate Intervention techniques concern aerosol-cloud interactions in some way, Marine Cloud Brightening (MCB) – whereby aerosols are injected into the marine boundary layer to increase the albedo of low clouds – does in particular. Developing a comprehensive understanding of MCB requires modelling across all scales. The focus of this work is modelling with large-eddy simulations (LES) and parcel models, performing a variety of experiments such as step forcing and continuous injection of aerosols in different models of the same class. Most the LES experiments have been performed in MONC (Met Office NERC Cloud) and compared to DALES (Dutch Atmospheric LES). Model intercomparison is key to understanding MCB; thus far there is disagreement among LES models over some important details of MCB, such the impact of small injected aerosols on the entrainment of dry air. It is hoped that better comparison of models can address this.

How to cite: Smith, W. M.: Modelling marine cloud brightening in large-eddy simulation and parcel model intercomparison projects, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19507, https://doi.org/10.5194/egusphere-egu25-19507, 2025.

EGU25-20156 | ECS | Orals | AS3.11

Vertical Structure of Deep Convective Clouds and Their Large Radiative Warming Masked by Background Water Clouds 

Zengxin Pan, Jianhua Yin, Fan Liu, Lin Zang, Feiyue Mao, and Daniel Rosenfeld

Deep convective clouds (DCCs) are crucial in the Earth’s energy budget. Although the abundant DCC-generated ice-phase anvil and cirrus theoretically have a warming effect, the reported observations of their cloud radiative effect (CRE) by previous studies are unexpectedly negative. Here, based on five years of global satellite data analysis, we find that the apparent contradiction between theory and observations resulted from neglecting the radiative contribution of background underlying clouds based on active and passive satellite observations. The probability of underlying clouds vertically below the anvils is up to 2/3. They can contribute up to 70% of the observed total shortwave cooling effect when they fully overlap with anvils. After excluding the effect of underlying clouds, most of the anvil CRE changes sign from negative to positive, increasing by over +25 W/m2, especially over land. This revelation suggests a substantially underestimated warming effect of DCC anvils and cirrus in previous observations. Also, it may imply an underestimated aerosol-driven positive radiative forcing on DCC, which has been estimated as neutral previously.

How to cite: Pan, Z., Yin, J., Liu, F., Zang, L., Mao, F., and Rosenfeld, D.: Vertical Structure of Deep Convective Clouds and Their Large Radiative Warming Masked by Background Water Clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20156, https://doi.org/10.5194/egusphere-egu25-20156, 2025.

EGU25-20175 | Orals | AS3.11

The Role of Deep Convection in Modulating LNOx and Boundary Layer-Upper Troposphere Exchange in the Amazon 

Rachel I. Albrecht, W. Isabella Valenti, Lucas Camargo, Thibaut Dauhut, Christelle Barthe, Micael Cecchini, Marco Franco, Axel Ventre, Carolina Monteiro, Lianet Pardo, Francisco Alcinei, Lemoel de Brito, Cleo Quaresma Dias Júnior, Hartwig Harder, Joachim Curtius, Mira Pöhlker, Christopher Pöhlker, Paulo Artaxo, and Luiz Machado

Lightning-produced nitrogen oxides (LNOx) represent a key source of reactive nitrogen in the Amazon, yet their role in regional atmospheric chemistry and transport remains poorly constrained. Beyond their role in ozone production, LNOx is a key driver of new aerosol particle formation in the upper troposphere, with earlier studies linking this process to the outflow of deep convective clouds and a downward flux of aerosol particles during precipitation events. However, recent findings highlight that ozone injections driven by LNOx from convective processes also play a crucial role in triggering in-situ particle bursts in the boundary layer. Both upper tropospheric aerosols and boundary layer particle bursts may play a pivotal role in supplying cloud condensation nuclei, promoting the development of green-ocean clouds and precipitation in the Amazon.

This study investigates the interplay between deep convective processes and LNOx production, emphasizing the vertical transport of gases and aerosols between the boundary layer and upper troposphere. Using data from the GoAmazon, ACRIDICON-CHUVA and CAFE-Brazil experiments, ATTO project, radar, satellite and lightning observations, we evaluate the temporal and spatial scales of NOx and ozone enrichment following deep convection activity. Time series of NOx and ultrafine particles are analyzed to identify peaks associated with potential LNOx emissions, contextualized with precipitation structure, divergence, mass flux at the cloud top, and lightning events. We intercompare radar-derived wind profiles and echo top heights from cloud and wind profiler radars at ATTO to determine the vertical range of mass detrainment. The height of the detrainment layer (HDL) is identified by correlating the divergence profiles with the distribution of radar reflectivity and ice water content within the anvil and convective cores. Echo tops exceeding the level of neutral buoyancy, derived from atmospheric soundings, are also used to assess the extent of vertical mass transport, with particular attention to anvil echo tops and convective tops surpassing this level. Ice water content within the anvil is used as a proxy for mass detrainment, applying a correction for ice fall speed to estimate the detrainment range. This proxy is then applied to 3D scanning radars over the Amazon. 

For the storms analyzed, all of them demonstrated enhanced ozone and NOx concentrations during downdrafts. The HDL is calculated to be near 11 km, with the detrainment range spanning 8 to 18 km. Over 15% of anvil echo tops extended beyond the neutral level of buoyancy of 16 km, and convective tops reached altitudes above 18 km. The results suggest that deep convection not only redistributes NOx and ozone but also alters the oxidative capacity and particle formation potential of the regional atmosphere. This work highlights the need to incorporate detailed convective processes into atmospheric models to improve predictions of chemical budgets and their implications for climate and air quality in tropical environments.

How to cite: Albrecht, R. I., Valenti, W. I., Camargo, L., Dauhut, T., Barthe, C., Cecchini, M., Franco, M., Ventre, A., Monteiro, C., Pardo, L., Alcinei, F., de Brito, L., Quaresma Dias Júnior, C., Harder, H., Curtius, J., Pöhlker, M., Pöhlker, C., Artaxo, P., and Machado, L.: The Role of Deep Convection in Modulating LNOx and Boundary Layer-Upper Troposphere Exchange in the Amazon, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20175, https://doi.org/10.5194/egusphere-egu25-20175, 2025.

EGU25-20598 | Posters on site | AS3.11

Multiseasonal measurements of ice-nucleating particle (INPs) levels and their drivers in the Easter Mediterranean during the CHOPIN field campaign 

Kaori Kawana, Romanos Foskinis, Aiden Jönsson, Marilena Gidarakou, Carolina Molina, Christos Mitsios, Maria Gini, Prodromos Fetfatzis, Alexandros Papayannis, Paul Zieger, Konstantinos Eleftheridadis, and Athanasios Nenes

 Ice formation in mixed-phase clouds is a critical component of their evolution and impacts on the hydrological cycle and climate. Nevertheless, their quantification and link to different aerosol sources (dust, biological particles) and impact of atmospheric aging leads to considerable uncertainty in their description in atmospheric models. Observations at high altitude mountaintop sites can provide a way to alleviate this uncertainty, as observations can be carried out for extensive periods of time, and can sample both free tropospheric and boundary layer air from a variety of sources and over different seasons – and their associated INP levels.

 Motivated by the above, we conducted the long-term observation at the top of the Mount Helmos (2314 m above sea level) for 6 months during the Cleancloud Helmos OrograPhic sIte experimeNt (CHOPIN) champaign, as part of the CleanCloud project. The INP concentrations were observed using a Portable Ice Nucleation Experiment (PINE) at -15°C and -25°C. We will discuss the characterization and drivers of INP changes between -15°C and -25°C, as well as cloud events and seasonal variations during fall, winter, and early spring. Additionally, we will discuss the controlling factors for INP activation in combination with other concurrent observations such as aerosol size distribution, fluorescent particle concentrations and shape, biological particle concentrations and speciation (e.g., flow cytometry) and laser remote sensing (elastic-Raman-fluorescence lidar), backtrajectory analysis, and in-situ aerosol chemical composition. We will evaluate the ability of existing parameterizations to capture the INP levels – and their link to aerosol type and origin – and examine whether aged INP (characterized by their airmass type, and acidity levels) tend to exhibit different INP activity compared to more freshly emitted particles.

How to cite: Kawana, K., Foskinis, R., Jönsson, A., Gidarakou, M., Molina, C., Mitsios, C., Gini, M., Fetfatzis, P., Papayannis, A., Zieger, P., Eleftheridadis, K., and Nenes, A.: Multiseasonal measurements of ice-nucleating particle (INPs) levels and their drivers in the Easter Mediterranean during the CHOPIN field campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20598, https://doi.org/10.5194/egusphere-egu25-20598, 2025.

EGU25-20619 | Posters on site | AS3.11

Regime Classification and AI-Enhanced Causal Analysis of Aerosol-Cloud Interactions Based on Long-Term Observations 

Yangang Liu, Yaohui Su, Tao Zhang, Kashif Anwar, and Weijia Liu

Despite decades of research and progress, climate models still suffer from large uncertainty in estimated aerosol indirect effects and large discrepancy with observations. Understanding of aerosol-cloud interactions (ACI) and their representation in climate models still pose vital challenges even for the simplest of all clouds – warm liquid clouds. In particular, different, even opposite, results have been reported in different studies of both the first and second aerosol indirect effects, awaiting physical explanation. This study conducts systematic classification of ACI regimes by analyzing decade-long surface-based measurements collected by the U.S. Department of Energy’s Atmospheric Radiation Measurement (ARM) facility under the frame of Twomey vs anti-Twomey and Albrecht vs. anti-Albrecht effects. Inspection of confounding factors (e.g., vertical motion, entrainment, decoupling, and stability) and potential micro-macro interactions will also made to provide physical understanding of the occurrence of the different ACI regimes, together with  AI-based causal analysis.

How to cite: Liu, Y., Su, Y., Zhang, T., Anwar, K., and Liu, W.: Regime Classification and AI-Enhanced Causal Analysis of Aerosol-Cloud Interactions Based on Long-Term Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20619, https://doi.org/10.5194/egusphere-egu25-20619, 2025.

The quantification of aerosol-induced radiative forcing remains a significant challenge in climate modeling, primarily due to the complex interplay of aerosol and clouds in a warming world. Traditional approaches often rely on either bottom-up process-based models, difficult to constrain against present-day observations, or top-down methods that lack the ability to capture the underlying processes accurately.

Here, we present an approach that combines both bottom-up process-based constraints and top-down energetic constraints of aerosol forcing and cloud feedbacks simultaneously to achieve a more comprehensive understanding of aerosol impacts on clouds and the climate. We generate one million samples of parametric uncertainty of aerosol forcing and cloud feedback and estimate the historic temperatures they would have produced using an impulse-response model. Both the temperature trajectories and the associated microphysical properties (such as the hemispheric contrast in cloud droplet number concentration) can then be compared to observations simultaneously.

Applying the new method to the Community Atmosphere Model v6, we infer narrower parameter ranges for key process parameters, a reduced effective radiative forcing of -1.08 [-1.29 – -0.77] Wm-2, and hence 66% more precise future projections.

How to cite: Watson-Parris, D.: Integrating Bottom-Up Process-Based Constraints with Top-Down Energetic Constraints of Historic Warming for More Accurate Future Projections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21790, https://doi.org/10.5194/egusphere-egu25-21790, 2025.

EGU25-597 | ECS | Orals | AS3.13

Unveiling the Impact of Lightning-induced NOx on Air Quality Over India 

Subhojit Ghoshal Chowdhury, Dilip Ganguly, and Sagnik Dey

Nitrogen oxides (NOx = NO + NO₂) are significant air pollutants that pose direct health risks and drive the formation of secondary pollutants such as ozone (O₃) and fine particulate matter (PM₂.₅). While NOx emissions have declined in regions like Europe and the United States (Schneider et al., 2015), the South Asia has experienced a sharp increases, exacerbating air quality challenges. Despite regulatory efforts to curb anthropogenic NOx emissions, the contribution of natural NOx sources, particularly lightning, remains poorly understood. This study explores the role of lightning-induced NOx (LNOx) in shaping the NOx budget and its implications for air quality across the Indian subcontinent.

Focusing on the pre-monsoon (March-May) season, when deep convective activity is at its peak, we analyzed high-resolution lightning data from the Lightning Imaging Sensor (LIS) to identify periods of intense activity. Using the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem), we simulated LNOx emissions by varying NO emissions per lightning flash (200–800 mol) to quantify its contribution accurately. Sensitivity experiments were conducted to isolate the impact of LNOx on atmospheric composition. Our results reveal that lightning significantly alters surface concentration of NO₂ and O₃. At lightning-strike locations, surface NO₂ levels increased by up to 0.5 ppb/day, though reductions of ~0.25 ppb were observed in certain areas due to complex chemical interactions. O3concentrations showed enhancements of up to 1.5 ppb/day, driven by NOx- fueled ozone production. Although, these numbers are small compared to anthropogenic contributions, it may have significant impacts on human exposure. Additionally, we observed a notable increase in hydroxyl radical (OH) concentrations across the atmosphere, highlighting the role of LNOx in modulating oxidative capacity. Stratosphere-troposphere exchange processes further influenced surface levels of NO₂, O₃, and OH.

As climate change intensifies deep convective activity, the contribution of LNOx to air quality is expected to grow. This study underscores the need to incorporate LNOx as a significant natural source in air quality models and policymaking efforts to develop effective strategies for mitigating air pollution in the region.

How to cite: Ghoshal Chowdhury, S., Ganguly, D., and Dey, S.: Unveiling the Impact of Lightning-induced NOx on Air Quality Over India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-597, https://doi.org/10.5194/egusphere-egu25-597, 2025.

EGU25-1752 | Posters on site | AS3.13

Air pollution-fire weather interaction in diverse regions 

Xin Huang, Zilin Wang, Ke Ding, Lian Xue, and Aijun Ding

Wildfires pose a substantial threat to human lives, destroy infrastructure, disrupt economic activity, and damage ecosystem services. Weather and climate conditions, including air temperature, humidity, wind, and precipitation, play crucial roles in determining the intensity and persistence of wildfires, as well as the dispersion and transport of smoke plumes. In turn, aerosols emitted from biomass burning are capable of influencing meteorology via aerosol-radiation interaction or aerosol-cloud interaction. However, there has been limited attention paid to the intricate interplay between smoke aerosol pollution, fire weather, and wildfire emissions. Our studies highlight the significance of synoptic-scale feedback in driving extreme wildfires across diverse fire-prone landscapes, including the United States, southeastern Asia, and even the Siberian region. We found that meteorological feedback induced by smoke aerosols can modify near-surface wind speed, air dryness, and rainfall and thus worsen air pollution by enhancing wildfire emissions and weakening dispersion. The intricate interactions among wildfires, smoke aerosol, and fire weather form a positive feedback loop that substantially increases air pollution exposure.

How to cite: Huang, X., Wang, Z., Ding, K., Xue, L., and Ding, A.: Air pollution-fire weather interaction in diverse regions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1752, https://doi.org/10.5194/egusphere-egu25-1752, 2025.

The co-polluted days by ozone (O3) and PM2.5 (particulate matter with an aerodynamic equivalent diameter of 2.5 μm or less) (O3–PM2.5PDs) were frequently observed in the Beijing–Tianjin–Hebei (BTH) region in warm seasons (April–October) of 2013–2020. We applied the 3-D global chemical transport model (GEOS- Chem) to investigate the chemical and physical characteristics of O3–PM2.5PDs by composited analyses of such days that were captured by both the observations and the model. Model results showed that, when O3–PM2.5PDs occurred, the concentrations of hydroxyl radical and total oxidant, sulfur oxidation ratio, and nitrogen oxidation ratio were all high, and the concentrations of sulfate at the surface were the highest among all pollution types. We also found unique features in vertical distributions of aerosols during O3–PM2.5PDs; concentrations of PM2.5 decreased with altitude near the surface but remained stable at 975–819 hPa. Process analyses showed that sec- ondary aerosols (nitrate, ammonium, and sulfate) had strong chemical productions at 913–819 hPa, which were then transported downward, resulting in the quite uniform vertical profiles at 975–819 hPa on O3–PM2.5PDs. The weather patterns for O3–PM2.5PDs were characterized by anomalous high-pressure system at 500 hPa as well as strong southerlies and high RH at 850 hPa. The latter resulted in the strong chemical productions around 850 hPa on O3–PM2.5PDs. The physical and chemical characteristics of O3–PM2.5PDs are quite different from those of polluted days by either O3 alone or PM2.5 alone and have important implications for air quality management.

How to cite: Dai, H. and Liao, H.: Composited analyses of the chemical and physical characteristics of co-polluted days by ozone and PM2.5 over 2013-2020 in the Beijing–Tianjin–Hebei region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1769, https://doi.org/10.5194/egusphere-egu25-1769, 2025.

Brown carbon (BrC) has been recognized as an important light-absorbing carbonaceous aerosol, yet understanding of its influence on regional climate and air quality has been lacking, mainly due to the ignorance of regional coupled meteorology-chemistry models. Besides, assumptions about its emissions in previous explorations might cause large uncertainties in estimates. Here, we implemented a BrC module into the WRF-Chem model that considers source-dependent absorption and avoids uncertainties caused by assumptions about emission intensities. To our best knowledge, we made the first effort to consider BrC in a regional coupled model. We then applied the developed model to explore the impacts of BrC absorption on radiative forcing, regional climate, and air quality in East Asia. We found notable increases in aerosol absorption optical depth (AAOD) in areas with high OC concentrations. The most intense forcing of BrC absorption occurs in autumn over Southeast Asia, and values could reach around 4 W m–2. The intensified atmospheric absorption modified surface energy balance, resulting in subsequent declines in surface temperature, heat flux, boundary layer height, and turbulence exchanging rates. These changes in meteorological variables additionally modified near-surface dispersion and photochemical conditions, leading to changes of PM2.5 and O3 concentrations. These findings indicate that BrC could exert important influence in specific regions and time periods. A more in-depth understanding could be achieved later with the developed model.

How to cite: Gao, M. and Wang, F.: Brown Carbon in East Asia: Seasonality, Sources, and Influences on Regional Climate and Air Quality, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1921, https://doi.org/10.5194/egusphere-egu25-1921, 2025.

EGU25-2318 | Orals | AS3.13

iDust - The deep integration of dust and numerical weather prediction for renewable energy applications 

Xi Chen, Mei Chong, Shian-Jiann Lin, Zhi Liang, Paul Ginoux, and Yuan Liang

The increasing demand for renewable energy highlights the importance of accurate dust process forecasting in regions with abundant wind and solar resources, as it can create significant value for the sector. However, leading real-time operational global numerical weather prediction (NWP) models often lack dust modules due to computational resource limitations and application scenarios. Current 'Near-Real-Time' dust forecasting services can only run after the completion of NWP, failing to meet the timeliness requirements for reporting power generation plans to the power grids. This work proposes a global dust-weather integrated (iDust) model development paradigm, incorporating dust modules into the dynamical core. Utilizing approximately one-eighth of additional computing power extends the global 12 km resolution NWP with dust prediction capabilities. To evaluate the forecasting capabilities of iDust, a comparative study is conducted with the ECMWF CAMS forecast and NASA MERRA2 reanalysis, including verifications over China during March to May in 2023, as well as three extreme dust events. The results demonstrate that iDust has better intensities and timings than its counterparts in dust storm forecasting. Using iDust, the global 12-km 10-day hourly dust storm forecast simulation initiated at 00UTC can obtain results by 06UTC, enabling timely forecasting of severe dust storms with concentrations exceeding 1000 μg/m3 on a global scale. iDust's novel capability can fill the urgent forecasting needs of the renewable energy industry for extreme dust weather conditions, promoting the goal of the green energy transition.

How to cite: Chen, X., Chong, M., Lin, S.-J., Liang, Z., Ginoux, P., and Liang, Y.: iDust - The deep integration of dust and numerical weather prediction for renewable energy applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2318, https://doi.org/10.5194/egusphere-egu25-2318, 2025.

EGU25-2322 | ECS | Posters on site | AS3.13

Extreme heat and drought have amplified the adverse effects of dust events across Eurasia 

Wei Wang and Mengmeng Li

Dust aerosols are critical in global climate change and air quality. In the context of global warming, dust emissions are projected to increase in certain dry areas. Utilizing a 40-year dataset of dust records and reanalysis data, along with satellite aerosol products, this study investigates the driving effects of extreme weather conditions on dust emissions and the magnification of their adverse impacts across Eurasia. Analysis reveals an overall upward trend (averaging 0.9 days decade1) in dust event frequency in Central East Asia over the past four decades, and a rapid increase (averaging 0.28 days yr1) in dust event occurrences in Mongolia. The study elucidates the influence of key meteorological factors—such as high temperatures, strong winds, low precipitation levels, reduced soil moisture, and diminished NDVI index—on the frequency of dust events across various regions. Particularly, temperature is identified as the dominant driver of the abrupt escalation in dust frequency observed in Middle East (R=0.30), Mongolia between 1994 and 2003 (R=0.62), and northern China (R=0.51). The analysis further indicates a substantial rise of dust events associated with extreme high temperatures accompanied by droughts over the past 40 years. It was also observed that the meteorological conditions, downwind air pollutants, and aerosol optical depth anomalies for dust events compounded by extreme high temperatures and droughts were considerably higher than those for typical dust events. Generalized additive machine learning models was employed to validate the driving impact of extreme weather on Eurasian dust events and the exacerbation of their adverse effects. These findings underscore that the increasing frequency of extreme weather events due to climate warming significantly amplifies the climate impacts and health risks posed by dust aerosols.粉尘气溶胶对全球气候变化和空气质量至关重要。在全球变暖的背景下,预计某些干旱地区的粉尘排放量将增加。利用40年的沙尘记录和再分析数据集,以及卫星气溶胶产品,本研究调查了极端天气条件对欧亚大陆沙尘排放的驱动作用及其不利影响的放大。分析表明,近40年来,中亚地区沙尘事件频次总体呈上升趋势(平均0.9 d /年 1 ),蒙古地区沙尘事件频次快速增加(平均0.28 d /年 1 )。研究阐明了高温、强风、低降水、土壤水分减少、NDVI指数降低等关键气象因素对不同区域沙尘事件发生频率的影响。特别是,温度被认为是中东(R=0.30)、蒙古(R=0.62)和中国北方(R=0.51)沙尘频率急剧上升的主要驱动因素。分析进一步表明,在过去40年里,与极端高温和干旱相关的沙尘事件大幅增加。在极端高温和干旱条件下,沙尘事件的气象条件、顺风空气污染物和气溶胶光学深度异常明显高于典型沙尘事件。采用广义加性机器学习模型验证了极端天气对欧亚沙尘事件的驱动作用及其不利影响的加剧。这些发现强调,气候变暖导致的极端天气事件日益频繁,大大放大了沙尘气溶胶造成的气候影响和健康风险。

How to cite: Wang, W. and Li, M.: Extreme heat and drought have amplified the adverse effects of dust events across Eurasia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2322, https://doi.org/10.5194/egusphere-egu25-2322, 2025.

Extreme weather becomes more frequent with global warming. The compound heatwave and drought (CHWD) events can intensify their individual environmental and societal impacts and cause disastrous threats. Abnormally high concentrations of surface ozone (O3), were usually observed during CHWD worldwide, while vegetation-atmosphere interactions further complicate the response of ozone to CHWD by influencing BVOC emissions and stomatal deposition processes. Using ERA5 data and major heatwave and drought indicators, the trend of heatwave and CHWD in summer in northern hemisphere during 1960-2023 was analyzed. We then used the online regional meteorology-chemistry model (WRF/Chem) to explore the effects of soil wilting point and dry deposition algorithms on the simulated vegetation-atmosphere feedback processes, as well as their impact on ozone pollution under CHWD. Results show that CHWD events have frequently engulfed many parts of the Northern Hemisphere, which is 3−5 times higher than in past decades. Under the influence of CHWD, more ozone pollution may be caused, especially in Europe, with a 35% increase in ozone concentrations during CHWD. The simulation results show that the increase of isoprene emission promoted the formation of ozone in CHWD summer, while the emission of isoprene is inhibited under drought conditions, mainly concentrated in the area with rich vegetation. Although the reduction of isoprene emissions during droughts inhibits ozone production, the ozone concentration of CHWD in summer is still higher, and high temperature plays a leading role. The wilting point from International Food Policy Research Institute (IFPRI) and Wesely-NoahMP dry deposition algorithms can more accurately describe the vegetation-atmosphere feedback process.

How to cite: lu, Y. and li, M.: Vegetation-atmosphere feedback during compound heatwave and drought aggravates the ozone pollution in northern Hemisphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2368, https://doi.org/10.5194/egusphere-egu25-2368, 2025.

The impact of aerosol-meteorology feedback on the effectiveness of emission reduction for PM2.5: A modeling case study in Northern China

 

Meigen Zhang, Jing He, and Yi Gao

State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China

 

The quantification of the effectiveness of anthropogenic emission control measures is crucial for future air quality policies. Meteorology plays a vital role in haze pollution, and the interactions between aerosol and meteorology have been widely studied. However, it is not fully clear how aerosol-meteorology feedback affects the effectiveness of emission reduction for PM2.5, which limits our ability of optimizing anti-pollution policies. Here, with the two-way atmospheric chemical transport model WRF-Chem, the effects of aerosol-meteorology feedback on the effectiveness of emission reduction for PM2.5 during a winter severe haze event in 2016 over the Northern China Plain (NCP) are studied. In the more polluted area of NCP (MP_NCP) during the daytime, 20% emission reduction over NCP increases near-surface downward shortwave radiation by 4.62 W/m2, 2 m temperature by 0.08 C, boundary layer height by 7.19 m and reduces 2 m relative humidity by 0.31% and thereby alleviates worsened meteorological conditions caused by aerosol effect. As a result, in MP_NCP, 20% emission reduction without aerosol-meteorology feedback leads to a decrease of 40.49 μg/m3 of near-surface PM2.5 and the above meteorological changes decrease near-surface PM2.5 concentration by 7.82 μg/m3, indicating that aerosol-meteorology feedback strengthens the effectiveness of emission reduction by 19%. In the less polluted area (LP_NCP), aerosol effect induced meteorological changes decrease PM2.5 concentration by 7.57 μg/m3 and 20% emission reduction without aerosol-meteorology feedback leads to a decrease of 13.15 μg/m3 in near-surface PM2.5. This reveals a remarkable enhancement of 58% in the effectiveness of emission reduction, which is much larger than that in MP_NCP. Such difference can be attributed to the presence of more clouds in LP_NCP, where the decrease in liquid water path, along with the increase in the planetary boundary layer height, jointly contributes to the PM2.5 decrease. Moreover, the effect of aerosol-meteorology feedback on the effectiveness of emission reduction for PM2.5 is nonlinear. With increasing PM2.5 concentration, the aerosol-meteorology feed back induced PM2.5 reduction first increases and then stabilizes once the PM2.5 concentration exceeds 350 μg/m3. This study can provide reference for air pollution control strategies.

 

Keywords: Emission reduction, Aerosol-meteorology feedback, WRF-Chem

How to cite: Zhang, M., He, J., and Gao, Y.: The impact of aerosol-meteorology feedback on the effectiveness of emission reduction for PM2.5: A modeling case study in Northern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2637, https://doi.org/10.5194/egusphere-egu25-2637, 2025.

Heatwaves, defined as prolonged periods of excessively hot weather, are increasingly recognized as a public threat due to their significant impact on human health and the environment. While the intrinsic impact of heatwaves on public health and the environment is well-recognised, a growing interest is emerging in the impact that these extreme weather events have on air pollution. Moreover, climate change has increased the frequency and intensity of these events raising concern about the potential impact on air pollution, and in particular on O3 levels. While the positive correlation between O3 and Temperature has been extensively analysed worldwide and in different time scales, the underpinning processes, their occurrence and their combination are still unclear. The summer of 2019 in the UK offers a compelling case study, as three distinct heatwave events occurred, characterized by record-breaking temperatures, including a peak of 38.7°C, and widespread O3 exceedances across both urban and rural areas. This study uses the WRF-Chem chemistry-transport model to simulate the entire summer of 2019, focusing on heatwave events and their influence on O3 formation. The analysis identifies key meteorological and chemical drivers, such as temperature, VOC emissions, and stagnation of air masses, which exacerbate O3 levels during the heat waves. The results indicate that the increased presence of biogenic isoprene played a significant role in O3 formation, particularly during heatwaves, with urban areas experiencing higher peaks due to a combination of temperature, emissions, and weak air movement.  With the frequency and intensity of heatwaves increasing due to climate change, our findings underscore the importance of considering both anthropogenic and natural emissions in future air quality management to protect public health.

How to cite: Mazzeo, A. and Hossaini, R.: Chemical and meteorological drivers of Ozone extremes during the heatwave of summer 2019 in the UK. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2810, https://doi.org/10.5194/egusphere-egu25-2810, 2025.

Biomass burning (BB) is one of the largest sources of trace gases and primary carbonaceous particles in the global troposphere, posing great impacts on air quality and regional climate. Accurate quantification of BB emissions is vital for assessing its environmental and climate impacts. However, there are still large uncertainties in current BB emission inventories due to poorly characterized emission rates under different combustion states. The fixed emission factor (EF) instead of varying EF associated with different combustion efficiencies may be the reason for the bias. Here, based on satellite-retrieved carbon dioxide (CO2) and carbon monoxide (CO), the modified combustion efficiency (MCE) is derived for fire-prone regions in Africa. The monthly and inter-annual variability of MCE shows a good correlation with meteorological variables such as relative humidity. Therefore, variable EF was established based on its statistical relationship with MCE for different fire-emitted species. Application of such MCE-dependent EF in the global climate-chemistry model can greatly improve the performance of wildfire smoke pollution during the fire season, indicated by an increase of 31% in aerosol optical depth (AOD) and a 50% reduction in normalized mean bias compared with AOD observations. The study elucidates the critical role of meteorology in BB emission estimates and highlights the importance of implementing a dynamic fire emission inventory in response to meteorological conditions.

How to cite: Fang, X. and Wang, Z.: Variation of Modified Combustion Efficiency and Its Impact on Biomass Burning Emission Estimation in Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3433, https://doi.org/10.5194/egusphere-egu25-3433, 2025.

EGU25-3439 | ECS | Posters on site | AS3.13

Modeling the Effects of Vegetation and Snow on Dust Storm over the Gobi Desert 

Yueting Hao and Xin Huang

The Gobi Desert is a prominent dust source in Asia, where the dust storm is severe and features great interannual and seasonal variability. Previous studies have found land surface variation plausibly plays an important role in the occurrence and intensity of dust storms. However, the quantitative estimation and numerical description in current models are still limited. Here, a comprehensive study utilizing multiple observations and modeling methods to assess the influence of vegetation and snow on dust was conducted. We found that Gobi deserts exhibit substantial monthly and interannual variability in dust storms, which shows a close connection with vegetation and snow. To quantitatively understand the impact of vegetation and snow cover on dust emissions and also to better characterize such effects in numerical models, we introduced a high-resolution dynamic dust source function that incorporates the effects of vegetation and snow on erodibility. The new parameterization noticeably improved dust-related simulations, including aerosol optical thickness and PM10 concentrations, and provided insights into the distinct effects of vegetation and snow on dust emissions. This study sheds light on the effects of vegetation and snow on dust storms over the Gobi Desert, highlighting the importance of dynamic representation of time-varying surface properties in dust simulation.

How to cite: Hao, Y. and Huang, X.: Modeling the Effects of Vegetation and Snow on Dust Storm over the Gobi Desert, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3439, https://doi.org/10.5194/egusphere-egu25-3439, 2025.

EGU25-3923 | ECS | Posters on site | AS3.13

Convective injection into stratospheric intrusions alters tropopause chemical structure 

Zhixiong Chen, Jane Liu, Xiushu Qie, Valerie Thouret, Jianchun Bian, Dan Li, Zhixuan Bai, Xian Xiao, Xugeng Cheng, Mengmiao Yang, Lei Shu, and Jingming Chen

Tropopause chemical structure (TCS) is influenced by the stratosphere-troposphere exchange (STE) and plays a role in Earth’s climate. Yet, this role is still not fully resolved in East Asia where active STE and high anthropogenic emissions coexist. Using airborne measurements of trace gases including O3, CO and H2O, we reveal the variations in TCS during two consecutive cut-off lows (COL), an important trigger of STE. We demonstrate the important roles of two-way STE and long-range transport processes in delivering natural and anthropogenic signatures in the TCS. The former COL case shows a normal pattern of TCS, consisting of stratospheric and tropospheric air and mixture of them. The latter, as a novel type of STE, exhibits an anomalous and complex structure, due to the deep convective injection into stratospheric intrusions, and advection of remote marine air. The distinct mixture of stratospheric air and anthropogenic pollution alters the TCS, with a horizontal and vertical scale estimated to be 200 km and 1 km, respectively. Moreover, air of maritime origins is also identified there, which is convectively transported and strongly dehydrated during the long-range transport. Such a complex TCS can produce unique chemical environments modulating cloud physics and atmospheric radiation. From a climatological perspective, events of these anomalous airmasses are nonnegligible in terms of their frequency and chemical impact revealed by multi-year observations. These new insights advance our understanding of the mixing of natural and anthropogenic species that shapes the TCS in East Asia, and have implications for climate change.

How to cite: Chen, Z., Liu, J., Qie, X., Thouret, V., Bian, J., Li, D., Bai, Z., Xiao, X., Cheng, X., Yang, M., Shu, L., and Chen, J.: Convective injection into stratospheric intrusions alters tropopause chemical structure, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3923, https://doi.org/10.5194/egusphere-egu25-3923, 2025.

EGU25-3995 | ECS | Orals | AS3.13

Relating satellite NO2 tropospheric columns to near-surface concentrations: implications from ground-based MAX-DOAS NO2 vertical profile observations 

Bowen Chang, Haoran Liu, Chengxin Zhang, Chengzhi Xing, Wei Tan, Qihua Li, Xiangguang Ji, Qihou Hu, and Cheng Liu

Given the significant environmental and health risks associated with near-surface nitrogen dioxide (NO2), machine learning is frequently employed to estimate near-surface NO2 concentrations (SNO2) from satellite-derived tropospheric NO2 column densities (CNO2). However, data-driven methods often face challenges in explaining the complex relationships between these variables. In this study, the correlation between CNO2 and SNO2 is examined using vertical profile observations from China’s MAX-DOAS network. Cloud cover and air convection substantially weaken (R = −0.68) and strengthen (R = 0.71) the CNO2-SNO2 correlation, respectively. Meteorological factors dominate the correlation (R2 = 0.58), which is 31% stronger in northern regions than in the southwest. Additionally, anthropogenic emissions impact SNO2, while topographical features shape regional climate patterns. At the Chongqing site, the negative impacts of unfavorable meteorological conditions, high emissions, and basin topography lead to significant contrasts and delays in daily CNO2 and SNO2 variations. This study enhances understanding of the spatial and temporal dynamics and influencing mechanisms of CNO2 and SNO2, supporting improved air quality assessments and pollution exposure evaluations.

How to cite: Chang, B., Liu, H., Zhang, C., Xing, C., Tan, W., Li, Q., Ji, X., Hu, Q., and Liu, C.: Relating satellite NO2 tropospheric columns to near-surface concentrations: implications from ground-based MAX-DOAS NO2 vertical profile observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3995, https://doi.org/10.5194/egusphere-egu25-3995, 2025.

EGU25-4100 | Posters on site | AS3.13

Superimposed effects of typical local circulations and aerosol–radiation interaction on heavy haze 

Yue Peng, Hong Wang, Xiaoye Zhang, Zhaodong Liu, and Wenjie Zhang

Although China’s air quality has substantially improved in recent years due to the vigorous emissions reduction, the Beijing–Tianjin–Hebei (BTH) region, especially its central and southern plains at the eastern foot of the Taihang Mountains, has been the most polluted area in China, with persistent and severe haze in winter. Combining meteorology–chemistry coupled model simulations and multiple observations, this study explored the causes of several heavy haze events in this area in January 2017, focusing on local circulations related to mountain terrain. The study results showed that on the weather scale, the configuration of the upper, middle, and lower atmosphere provided favorable weather and water vapor transport conditions for the development of haze pollution. Under the weak weather-scale systems, local circulation played a dominant role in the regional distribution and extreme values of PM2.5. Influenced by the Taihang and Yanshan mountains, vertical circulations and wind convergence zone were formed between the plain and mountain slopes. The vertical distribution of pollutants strongly depended on the intensity and location of the circulation. The circulation with high intensity and low altitude was more unfavorable for the vertical and horizontal diffusion of near-surface pollutants. More importantly, we found that the aerosol–radiation interaction (ARI) significantly amplified the impacts of local vertical circulations on heavy haze by two mechanisms. First, the ARI strengthened the vertical circulations at the lower levels, with the zonal wind speeds increasing by 0.3–0.8m s−1. Meanwhile, the ARI could cause a substantial downward shift in the vertical circulations (∼100 m). Second, the ARI weakened the horizontal diffusion of pollutants by reducing the westerly winds and enhancing wind convergence and southerly winds. Under these two mechanisms, pollutants could only recirculate in a limited space. This superposition of the typical local circulation and the ARI eventually contributed to the accumulation of pollutants and the consequent deterioration of haze pollution in the region.

How to cite: Peng, Y., Wang, H., Zhang, X., Liu, Z., and Zhang, W.: Superimposed effects of typical local circulations and aerosol–radiation interaction on heavy haze, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4100, https://doi.org/10.5194/egusphere-egu25-4100, 2025.

EGU25-4164 | ECS | Posters on site | AS3.13

Modeling Study on the spatiotemporal distribution of global atmospheric brown carbon 

Zijian Jiang and Zhe Wang

    Brown carbon (BrC), a certain type of organic carbon (OC) with light-absorbing ability at visible and near-ultraviolet spectrum, pays an important role in the Earth's radiation budget and atmospheric warming. It is primarily produced through the incomplete combustion of biomass and fossil fuels, as well as the formation of secondary organic aerosols. Recent laboratory and field studies have identified a class of BrC known as dark brown carbon which exhibits black carbon (BC)-like properties and strong absorbing ability, with k value between 0.2 to 0.4 in the visible spectrum. However, few modeling studies have taken dark brown carbon into account, leading to  an underestimation of its direct radiative forcing on the climate system.

    In this study, we utilized the global-regional nested transport model, the Aerosol and Atmospheric Chemistry Model of the Institute of Atmospheric Physics (IAP-AACM), to simulate global brown carbon distribution. Following previous studies, we classified brown carbon into four categories based on its absorptivity: very weak brown carbon, weak brown carbon, moderate brown carbon, and dark brown carbon. Using the mass ratio of BrC/OC in the published paper, we constructed emission inventories for anthropogenic and biomass burning from EDGAR_v8.1 and GFED_v4.1, respectively, and assigned each emission source to one of the four BrC categories based on its absorptive properties. The model simulations were performed at a 1° × 1° resolution for both winter and summer in 2022 by coupling physical and chemical modules including dry deposition, wet scavenging, secondary formation, and aging. Model results were compared with AERONET and satellite-based aerosol absorption optical depth (AAOD), showing reasonable agreement.

    This research includes dark brown carbon from biomass burning and secondary BrC from aromatic secondary organic aerosol (SOA). The Volatility Basis Set (VBS) scheme was employed to simulate SOA formation. The results indicate that secondary BrC contributes approximately 2% ~ 8% to global BrC absorption. Dark brown carbon accounts for 2% ~ 14% BrC concentrations, but contributes 47% ~ 88% to global BrC absorption. These findings highlight the significant role of dark brown carbon in solar absorption and its potential impact on the Earth's radiative forcing.

How to cite: Jiang, Z. and Wang, Z.: Modeling Study on the spatiotemporal distribution of global atmospheric brown carbon, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4164, https://doi.org/10.5194/egusphere-egu25-4164, 2025.

EGU25-4618 | ECS | Posters on site | AS3.13

Asian dust storm performing the role in surface ozone reduction 

Keqin Tang, Yunjiang Zhang, Nan Li, and Xinlei Ge

Natural dust storms significantly contribute to air pollution by elevating atmospheric particle levels. These dust storms also influence atmospheric photochemical processes through surface reactions on dust particles. In this study, we conduct a quantitative analysis of the impact of dust aerosols on near ground ozone in China, integrating multiple observations with advanced modeling techniques. Our findings reveal a notable reduction in regional average ozone concentrations (1.8 – 12.0 ppbv) in 12 dust storm events during 2016 to 2023, compared to scenarios with minimal or no dust influence. The critical drivers of the ozone decline include interactions between dust aerosols and ozone, the relevant radicals and radiation, as well as adverse meteorological conditions. Among these factors, dust aerosols are estimated to account for 24±13% of the observed ozone reduction. Furthermore, heterogeneous removal pathways, such as the direct uptake of ozone and the adsorption of dinitrogen pentoxide (N₂O₅) and hydroperoxyl radicals (HO₂) by dust aerosols, are identified as the crucial mechanisms contributing to ozone depletion. These findings underscore the complex chemistry of dust-mediated processes, which profoundly influence tropospheric photochemical cycles and amplify ozone sensitivity in volatile organic compound (VOC)-limited atmospheric environments.

How to cite: Tang, K., Zhang, Y., Li, N., and Ge, X.: Asian dust storm performing the role in surface ozone reduction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4618, https://doi.org/10.5194/egusphere-egu25-4618, 2025.

EGU25-4747 | ECS | Posters on site | AS3.13

Impacts of Sea-Land Breeze on the Ozone Pollution under varied synoptic weather patterns in the Pearl River Delta, China 

Chenxi Liu, Haichao Wang, and Shaojia Fan

Ground-level ozone (O₃) pollution has become a critical environmental issue in coastal urban areas, driven by rapid global urbanization. Sea-land breeze (SLB) circulation plays a key role in this process. However, the combined effects of SLB and synoptic-scale weather systems on O₃ pollution remain poorly understood. Most existing studies focus on individual events or short-term periods, lacking a systematic analysis of how mesoscale SLB interacts with larger-scale weather patterns to influence O₃ concentrations.This study investigates the impacts of SLB on O₃ pollution in the Pearl River Delta (PRD), a densely populated coastal region in southern China. Using 28 years of observational data and ERA5 reanalysis datasets, we analyze the spatial and temporal variability of SLB and its interactions with synoptic-scale winds in shaping O₃ distributions. Additionally, a random forest model is applied to quantitatively assess the contributions of SLB to O₃ variations under different meteorological conditions.This research provides a systematic framework for understanding the mesoscale-synoptic coupling processes that drive O₃ pollution in coastal cities. The findings highlight the critical role of SLB in regulating regional air quality and offer a solid scientific basis for designing effective mitigation strategies in similar coastal urban regions worldwide.

How to cite: Liu, C., Wang, H., and Fan, S.: Impacts of Sea-Land Breeze on the Ozone Pollution under varied synoptic weather patterns in the Pearl River Delta, China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4747, https://doi.org/10.5194/egusphere-egu25-4747, 2025.

Wildfires and dust storms are two major environmental hazards that significantly degrade air quality and pose severe risks to human health and ecosystems. These events often occur simultaneously, forming compound extreme events that can have amplified impacts compared to individual occurrences. This study aimed to investigate the mechanisms linking wildfires and dust pollution, analyze the spatiotemporal distribution and trends of their co-occurrence, and examine the global inequality in exposure to these compound events, all using a combination of satellite data, reanalysis datasets, and environmental variables.

We first explored the underlying mechanisms by which wildfires contribute to dust pollution. This included investigating how wildfires disturb vegetation and soil, and how changes in land cover interact with meteorological factors such as wind speed and direction to produce and transport dust. Using satellite-based aerosol optical depth (AOD) and dust optical depth (DOD) data (e.g., MODIS, IASI), as well as environmental variables such as soil moisture, vegetation cover, and wind data, we aimed to understand the physical and chemical processes that link wildfire activity to increased dust emissions.

The second part focused on analyzing the spatiotemporal distribution of the co-occurrence of wildfires and dust storms. We examined the geographical overlap of these events over recent decades, identifying regions where the co-occurrence of wildfires and dust storms is most frequent. By analyzing multi-year satellite and reanalysis data, we also explored interannual variations in the frequency of these compound events and assess how their co-occurrence has changed over time.

Finally, we investigated the global inequality in exposure to the combined air pollution resulting from co-occurring wildfires and dust storms. By mapping the spatial distribution of these compound events, we identified regions and populations that were disproportionately affected, particularly in areas with high vulnerability. We analyzed the exposure levels based on socioeconomic and demographic factors, highlighting how vulnerable populations in certain regions face a higher risk of respiratory and cardiovascular diseases due to these compounded pollution events. This part of the study aimed to shed light on the unequal burden of wildfire-dust compound events and provides insights into the need for targeted mitigation and health interventions.

Our study seeks to provide a comprehensive understanding of the interactions between wildfires and dust storms, and the compounded environmental and health impacts they have. The results will contribute to the development of effective mitigation strategies, improve public health outcomes, and inform policies aimed at reducing the exposure and risks associated with these extreme events.

How to cite: Yang, Q.: Unequal Environmental and Health Impacts of Co-occurring Wildfires and Dust Events: Mechanisms, Spatiotemporal Distribution, and Exposure Inequality, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4931, https://doi.org/10.5194/egusphere-egu25-4931, 2025.

EGU25-5542 | ECS | Posters on site | AS3.13

Impacts of northward typhoons on autumn haze pollution over North China Plain 

Ke Ding and Haoxian Lin

Although air quality in China has improved substantially over recent years, haze pollution events still occur frequently, especially over the North China Plain (NCP). Previous studies showed that typhoons are conducive to regional pollution events in eastern China; however, the underlying mechanism and quantitative understanding of the typhoons' impact on haze pollution remain unclear there. Here, based on ground-based and satellite observations, reanalysis data, and model simmulations, we show that northward typhoons approaching China are essential for autumn haze pollution over NCP. Elevated relative humidity levels and enhanced pollution accumulation, caused by northward typlhoons and the corresponding high-pressure systems, are responsible for the pollution enhancements over NCP. Compared with episodes without typhoon influence,cities near Taihang and Yan Mountain suffer from heavier haze pollution when typhoons approach, with PM2.5 concentrations increasing from 87.1 to 106.4 ug m-3. More water vapor from the Yellow and Bohai Seas and pollutants from eastern China are transported to these cities by typhoon-induced southeasterly wind anomalies, facilitating the chemical formation of aerosols there. In addition, by the block of mountains, these southeasterly wind anomalies also lead to stronger local accumulation over cities and an elevation of pollutants along themountains. What is more, with the implementation of emission reduction, the relative changes of PM2.5 concentrations between typhoon-induced episodes and no-typhoon episodes increase. This work highlights the importance of understanding the impact of synoptical weather on PM2.5 transport, accumulation, and formation processes in haze pollution mitigation in eastern China.

How to cite: Ding, K. and Lin, H.: Impacts of northward typhoons on autumn haze pollution over North China Plain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5542, https://doi.org/10.5194/egusphere-egu25-5542, 2025.

EGU25-6166 | Orals | AS3.13

A key role of wildfires in the association between droughts and PM2.5 air pollution 

Hyung Joo Lee, Min Young Shin, and Na Rae Kim

This study investigates the role of wildfires in elevating ambient PM2.5 concentrations during droughts in California, U.S., from 2006 to 2020. While previous research has explored individual relationships between droughts, wildfires, and PM2.5 concentrations, a comprehensive analysis integrating all these components is lacking. This study employs a multi-tiered statistical approach to estimate each relationship among droughts, wildfires, and PM2.5 concentrations and to quantify the contribution of wildfires to the association between droughts and PM2.5 air pollution. During the study period, PM2.5 concentrations increased by 1.47 µg/m3 [standard error (SE)= 0.10] on average as drought conditions worsened by 1 unit of the Standardized Precipitation Evapotranspiration Index (SPEI). Drought-related PM2.5 increases were greater during wildfire days [3.29 µg/m3 (SE= 0.36)] than during non-wildfire days [0.97 µg/m3 (SE= 0.08)] per unit decrease in SPEI. During wildfire days, the drought-related PM2.5 increase substantially diminished from 3.29 µg/m3 (p< 0.0001) to -0.10 μg/m3 (p= 0.1307) after adjusting for wildfire-induced PM2.5 concentrations. Furthermore, the likelihood of PM2.5 exceedance days increased by 198% per unit decrease in SPEI due to wildfires during droughts. These findings demonstrate that the increase in drought-related PM2.5 concentrations is largely attributable to wildfire-induced PM2.5. Understanding the role of wildfires is crucial for air quality management and preparedness for future extreme events in the era of climate change.

How to cite: Lee, H. J., Shin, M. Y., and Kim, N. R.: A key role of wildfires in the association between droughts and PM2.5 air pollution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6166, https://doi.org/10.5194/egusphere-egu25-6166, 2025.

Brown carbon (BrC) from anthropogenic activities and wildfires significantly impacts atmospheric processes through its sunlight absorption properties. This study aims to constrain the understanding of BrC's light absorption using multiple observations and models, providing a comprehensive assessment of its environmental implications. Anthropogenic sources and wildfires release BrC with distinct characteristics, influencing regional and global aerosol optical properties. By integrating field measurements, laboratory analyses, satellite products, and climate models, this research quantifies BrC's absorption across different spectral ranges and evaluates its contribution to radiative forcing. The results highlight the need for refined models to accurately represent BrC's complex behavior and improve predictions of its impacts on climate and air quality. This abstract presents the methodology, findings, and future directions for constraining BrC's sunlight absorption.

How to cite: Lin, G.: Constraining Sunlight Absorption of BrC from Anthropogenic Sources and Wildfires with Multiple-type Observations and Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7557, https://doi.org/10.5194/egusphere-egu25-7557, 2025.

Biomass burning (BB) emission inventories are often used to understand the interactions of aerosols with weather and climate. However, large uncertainties exist among current BB inventories, so the choice of inventories can greatly affect model results. To quantify the differences among BB emission inventories and reveal their reasons, we compared carbon monoxide (CO) and organic carbon (OC) emissions from seven major BB regions globally from 2013 to 2016. The current inventories are based on two basic approaches: (1) bottom-up approach, which establishes inventories based on observed surface data, and (2) top-down approach, which based on the release rate of radiative energy from vegetation burning. In this study, we selected mainstream bottom-up inventories Fire INventory from NCAR 1.5 (FINN1.5) and Global Fire Emissions Database version 4s (GFED4s), and the top-down inventories Quick Fire Emissions Dataset 2.5 (QFED2.5) and VIIRS-based Fire Emission Inventory version 0 (VFEI0). We find that the total global CO emissions fluctuate between 252 and 336 Tg and the regional bias is even larger, which can be up to six times. Dry matter is responsible for most of the regional variation in CO emissions (50–80 %), with emission factors accounting for the remaining 20–50 %. Uncertainties in dry matter often come from biases in the calculation of bottom fuel consumption and burned area, which are closely related to vegetation classification methods and fire detection products. In the tropics, peatlands contribute more fuel loads and higher emission factors than grasslands. At high latitudes, as cloud fraction increases, the bias between burned area (or fire radiative power) increases by 20 %. In addition, due to the corrected emission factors in QFED2.5, global BB OC emissions have higher variability, fluctuating between 14.9 and 42.9 Tg.

Finally, we applied the four sets of BB emission inventories to the Community Atmosphere Model version 6 (CAM6) and compared the model results with observations. Our results suggest that the simulations based on the GFED4s agree best with the MOPITT-retrieved CO. We also compared the simulation results with satellite or ground-based measurments, such as Moderate Resolution Imaging Spectroradiometer (MODIS) AOD and AErosol RObotic NETwork (AERONET) AOD. Our results reveal that there is no global optimal choice for the BB inventories, but we give certain inventory recommendations based on different study areas and spatiotemporal scales. This study has implications for reducing the uncertainties in emissions or improving BB emission inventories in further studies.

How to cite: Lou, S., Hua, W., and Huang, X.: Diagnosing uncertainties in global biomass burning emission inventories and their impact on modeled air pollutants, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7871, https://doi.org/10.5194/egusphere-egu25-7871, 2025.

EGU25-7898 | ECS | Orals | AS3.13

Impact of extreme weather induced BOVCs on O3 formation in China 

Nan Wang and Fumo Yang

As pollution control efforts in China continue to deepen, the role of natural processes, such as vegetation emissions, in air pollution has become increasingly significant. Climate warming, coupled with the growing frequency of extreme weather events like high temperatures, droughts, and typhoon peripheries, intensifies the emission of biogenic volatile organic compounds (BVOCs) from vegetation. The interaction between natural emissions and urban anthropogenic pollutants contributes to the escalation of ozone photochemical pollution. This study aims to explore the relationship between BVOC emissions and ozone pollution at both climate and weather scales through numerical simulations. Additionally, leveraging large-scale environmental data and machine learning techniques, the research will investigate the drivers of isoprene emissions and their impact on urban air quality.

How to cite: Wang, N. and Yang, F.: Impact of extreme weather induced BOVCs on O3 formation in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7898, https://doi.org/10.5194/egusphere-egu25-7898, 2025.

EGU25-8633 | ECS | Orals | AS3.13

Why did PM2.5 pollution persist in the Pearl River Delta, South China during the El Niño–La Niña transition despite emission reductions? 

Kun Qu, Xuesong Wang, Yu Yan, Xipeng Jin, Ling-Yan He, Xiao-Feng Huang, Xuhui Cai, Jin Shen, Zimu Peng, Teng Xiao, Mihalis Vrekoussis, Maria Kanakidou, Guy Brasseur, Nikos Daskalakis, Limin Zeng, and Yuanhang Zhang

PM2.5 pollution poses a serious threat to human health, making its mitigation a priority for policymakers. Over the last decade, air quality control measures have led to significant reductions in PM2.5 concentrations across China. However, meteorological changes driven by variations in the climate system can offset these effects and even exacerbate PM2.5 pollution. During the cold seasons (autumn and winter) of 2015-2017, PM2.5 pollution persisted in the Pearl River Delta (PRD), South China, despite rapid emission reductions both in the PRD and its upwind regions. This period coincided with a notable transition in ENSO state, from a very strong El Niño in 2015 to a weak-to-moderate La Niña in 2017. Through meteorological analysis and WRF/CMAQ simulations, this study investigates the connection between this climate transition and persisted PM2.5 pollution in the PRD. Comparisons of meteorological conditions during the three cold seasons align with previously reported El Niño and La Niña effects: Precipitation and polluted-day humidity reached the highest in the El Niño year (2015), while a northerly wind anomaly was observed in the La Niña year (2017). These meteorological changes weakened local PM2.5 production but enhanced PM2.5 transport to the PRD in the three cold seasons, as indicated by changing contributions to PM2.5 in the WRF/CMAQ simulations: The contributions of local emissions declined from 30% in 2015 to 22% in 2017, while the contributions of upwind emissions rose from 48% to 56%. Although emission reductions contributed to lower polluted-day PM2.5 concentration in the PRD by -5.7 µg/m3 in 2015-2016 and -2.7 µg/m3 in 2016-2017, this effect was outweighed by the influence of meteorological changes, which resulted in its reduction of -6.1 µg/m3 in 2015-2016 and increase of +10.7 µg/m3 in 2016-2017. Three-year changes in PM2.5 sulfate were mainly attributed to emission reduction in the upwind regions, while these in PM2.5 nitrate were linked to varying transport contributions under meteorological changes. This study indicates that to effectively mitigate PM2.5 pollution in the PRD, targeted strategies that focus on local or upwind emissions under varying meteorological conditions should be adopted.

Acknowledgement: This work was supported by the National Key Research and Development Program of China (grant No. 2018YFC0213204),the National Science and Technology Pillar Program of China (grant No. 2014BAC21B01), the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany´s Excellence Strategy (University Allowance, EXC 2077, University of Bremen) and co-funded DFG-NSFC Sino-German Air-Changes project (grant no. 448720203).

How to cite: Qu, K., Wang, X., Yan, Y., Jin, X., He, L.-Y., Huang, X.-F., Cai, X., Shen, J., Peng, Z., Xiao, T., Vrekoussis, M., Kanakidou, M., Brasseur, G., Daskalakis, N., Zeng, L., and Zhang, Y.: Why did PM2.5 pollution persist in the Pearl River Delta, South China during the El Niño–La Niña transition despite emission reductions?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8633, https://doi.org/10.5194/egusphere-egu25-8633, 2025.

Ozone (O3) concentration in the regional atmosphere of South China were shown to increase, but the recent variations in the context of dramatic emissions fluctuations remain unknow. In contrast to the overall increase determined elsewhere, O3 at a regional background site in South China decreased at a surprisingly high rate of -2.79 ppbv yr-1 during 2018-2023, which has not been seen before and was unlikely to be explained by the COVID-19 lockdowns. Significant reductions in O3 were only observed in summer and autumn. Three statistical methods were used to eliminate the impacts of meteorological variations on O3 trends, which were shown not to be the main cause of the O3 reduction. With the 2017 emission inventories (EIs), the Weather Research and Forecasting model coupled with Community Multiscale Air Quality (WRF-CMAQ) well reproduced the O3 in August 2018. Sensitivity tests indicated that meteorological variations explained at most half of the O3 reduction rate. Despite the significant drop in cargo throughput at Hong Kong (HK) terminals, ship emissions made a higher contribution to O3 in August 2023 than in the same period of 2018. The unexplained O3 decrease was likely due to reduced anthropogenic emissions in mainland China and HK. Simulations with a simple extrapolation based on the 2017 EIs did show that emission changes in the neighboring Pearl River Delta led to a decrease in O3. However, updated emissions are needed to clearly understand the effects of local and regional emission changes.

How to cite: Lyu, X.: What drove the rapid ozone reduction at a background site in South China during 2018-2023?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9564, https://doi.org/10.5194/egusphere-egu25-9564, 2025.

EGU25-9896 | ECS | Orals | AS3.13

Projected changes and implications of surface ozone pollution in India under changing climate and emission scenarios 

Anagha Kunhimuthappan Suresan and Jayanarayanan Kuttippurath

Surface ozone (SurfO3) pollution poses significant challenges to air quality, public health and agriculture worldwide. In a scenario of rising anthropogenic emissions, increasing temperature and altered atmospheric compositions exacerbate SurfO3 production in hotspots of pollution, leading to an ozone-climate penalty that could offset gains from emission reduction measures. This study explores projected changes in SurfO3 under the Aerosol and Chemistry Model Intercomparison Project (AerChemMIP) simulations of the Coupled Model Intercomparison Project phase-six (CMIP6), focusing on their implications for agriculture in India. We analyse the simulations from the United Kingdom Earth System Model version1 at low (-LL) resolution (UKESM 1-0-LL) and Geophysical Fluid Dynamics Laboratory Earth System Model version 4 (GFDL-ESM 4) models, following the anthropogenic emission trajectory of the shared socio-economic pathway (SSP)3–7.0 high emission scenario with pre-defined climate (SSP370pdSST) and changing climate (SSP370SST). Climate-induced increases in SurfO3 is observed in the rabi (December–February) and late-kharif (OctoberNovember) seasons, whereas early to mid-kharif (June–September) season show a reduction in SurfO3 in India. Increasing trend in climate change-induced SurfO3(0.03–0.08 ppbv yr-1) is evident in the Indo-Gangetic Plain (IGP), the breadbasket of India, during most seasons, and in central India during post-kharif and rabi seasons. This suggests that, even if the precursor emission remains at the current level, climate change alone could contribute to the increase in SurfO3 in the highly polluted regions of south Asia by 2050. Furthermore, the IGP region, one of the most fertile agricultural regions in South Asia, is likely to face significant challenges due to increasing SurfO3, which exacerbates crop yield losses, particularly for rabi wheat. This situation is concerning, as IGP comprises of about 27% of the total cultivated area and contributes significantly (about 50% of the total food consumed in the country) to the national agricultural production in India. Therefore, the study emphasise the need for targeted mitigation strategies, particularly for CH4, VOCs and NOx, to mitigate the dual challenges of climate change and SurfO3 pollution.

Keywords: Surface ozone, Climate change, AerChemMIP, Ozone-climate penalty, Agriculture, IGP

How to cite: Kunhimuthappan Suresan, A. and Kuttippurath, J.: Projected changes and implications of surface ozone pollution in India under changing climate and emission scenarios, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9896, https://doi.org/10.5194/egusphere-egu25-9896, 2025.

EGU25-10924 | ECS | Orals | AS3.13

Complex Ozone-Temperature Relationship in the North China Plain Under Heat Extremes 

Zhenjiang Yang, Ke Li, and Hong Liao

The North China Plain is one of the most heavily polluted regions in the world in terms of surface ozone pollution, and experiences frequent extreme summer heat waves. Concurrently, extreme heat events—capable of triggering severe ozone episodes—are becoming increasingly frequent, suggesting a growing challenge for ozone air quality control in a warming climate. In this study, we utilize the long-term surface measurements to show that, in the North China Plain, ozone-temperature relationship has two distinct regimes of ozone suppression (OS) vs. non-OS in June months, with a regime shift occurring around 2020. The observed OS can be well captured by the GEOS-Chem model and a machine learning model based on meteorological data only; our analysis indicates that OS is primarily driven by different circulation patterns rather than by the previously identified chemical and emissions processes. Furthermore, although the GEOS-Chem successfully captures the shift from OS to no-OS around 2020, the observed non-OS in NCP was strongly underestimated by the model. Using an improved version of GEOS-Chem, we quantify the potential importance of meteorological factors, changes in anthropogenic emissions, and chemical drivers. The results show that at extremely high temperatures, temperature-dependent emission processes such as soil NOx and anthropogenic VOCs contribute significantly to the ozone temperature slope during no-OS. Whereas the reduction of anthropogenic emissions is unfavorable for the occurrence of no-OS, the contribution of NOx-producing processes (e.g., PAN decomposition) is amplified at high temperatures due to a shift in ozone production control from NOx-limited to VOC-limited conditions.

How to cite: Yang, Z., Li, K., and Liao, H.: Complex Ozone-Temperature Relationship in the North China Plain Under Heat Extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10924, https://doi.org/10.5194/egusphere-egu25-10924, 2025.

EGU25-12236 | ECS | Orals | AS3.13

Understanding the influence of particle growth on air quality and local climate in megacity 

Wei Du, Yele Sun, Jian Zhao, Lubna Dada, Yuying Wang, Xueshun Chen, Zhanqing Li, Yingjie Zhang, Fei Hu, Tom Kokkonen, Veli-Matti Kerminen, and Markku Kulmala

New particle formation (NPF) is a process in which gaseous molecules in the atmosphere cluster together to form aerosol particles [1]. These particles contribute significantly to the total number of aerosols in the atmosphere, further influencing air quality and climate [2]. The environmental and climate effects of NPF largely depend on the particle growth (NPG) process; however, it remains poorly understood, especially in urban [3]. In this study, we performed simultaneous measurements of particle number size distributions (PNSD) and chemical compositions at the ground and at 260 m based on the 325 m meteorological tower in urban Beijing. By comparing the NPG process at the two heights, we provide new insights into the interactions between boundary layer dynamics and NPG in megacity [4, 5].
Our results show that although NPG occurred at both heights, significant differences of NPG between 260 m and the ground level were observed in megacity. When vertical diffusion is sufficient, gaseous precursors from the surface could be transported to higher altitudes. The lower temperature and higher relative humidity aloft promoted gas-to-particle conversion, leading to stronger particle growth at higher altitudes. As a result, higher particle concentrations accompanied by stronger hygroscopicity led to >20% higher NPF-induced cloud condensation nuclei (CCN) formation aloft. However, when vertical mixing was suppressed, gaseous pollutants tended to accumulate near the surface. These pollutants then contributed to particle growth at ground level, exacerbating atmospheric haze pollution near ground. This, in turn, further reduced the boundary layer height. The valuable results provided novel information of the interactions between boundary layer dynamics and new particle growth, enhancing our understanding on the climate and environmental effects of NPF.
1.    Kulmala, M., et al., Direct Observations of Atmospheric Aerosol Nucleation. Science, 2013. 339(6122): p. 943-946.
2.    Kerminen, V.-M., et al., Atmospheric new particle formation and growth: review of field observations. Environmental Research Letters, 2018. 13(10): p. 103003.
3.    Stolzenburg, D., et al., Atmospheric nanoparticle growth. Reviews of Modern Physics, 2023. 95(4).
4.    Du, W., et al., A 3D study on the amplification of regional haze and particle growth by local emissions. npj Climate and Atmospheric Science, 2021. 4(1): p. 1-8.
5.    Du, W., et al., Impacts of enhanced new-particle growth events above urban roughness sublayer on cloud condensation nuclei. One Earth, 2024.

How to cite: Du, W., Sun, Y., Zhao, J., Dada, L., Wang, Y., Chen, X., Li, Z., Zhang, Y., Hu, F., Kokkonen, T., Kerminen, V.-M., and Kulmala, M.: Understanding the influence of particle growth on air quality and local climate in megacity, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12236, https://doi.org/10.5194/egusphere-egu25-12236, 2025.

The paper presents the air pollutant measurements and the spatial variation of air pollutants in Lhasa to reflect the characteristics of the air pollutants in a typical high-altitude city. According to the research, five-year measurements of air pollutants at 6 sites in Lhasa, were analyzed from January 2013 to December 2017. Within this period, the average pollutant concentration was highest for O3, at about 65.24 μg/m3, followed by PM10, with an average of 58μg/m3. The lowest concentration was found for SO2, with an average of 9.258 μg/m3; additionally, the concentrations of surface ozone were higher in spring (100.73μg/m3) than in winter (49.00μg/m3). O3 concentrations are greater in the spring and summer and clearly peaked at 12 and 6 PM. The NOx concentration peaked in the winter and rise sharply between 9:00-11:00 and 22:00-01:00.Air pollutants at all the 6 sites in Lhasa generally displayed similar patterns of both diurnal and monthly variations, indicating the mixed atmospheric environment and the overall effect of the meteorological conditions in the city.

The air quality in Lhasa is better than in other Chinese provincial capitals because it has lower concentrations of all air pollutants except O3. The vegetation index is also one of the key factors affecting the concentration of pollutants. The highest correlation with the vegetation index was found to be with PM10 (-0.91), followed by PM2.5 and SO2, with correlation coefficients of -0.74 and -0.68, respectively. The vegetation index has a strong impact on the pollutants in Lhasa city, and areas with sparse vegetation and a dry climate usually result in higher atmospheric ozone loads. We suggested that underscoring the need for targeted interventions to enhance green spaces and mitigate the adverse effects of climate on air quality.

How to cite: Zhuoga, D., Jun, D., Duo, B., and Zhuoma, L.: Pollution characteristics of ozone and atmospheric particulate matter during 2013-2017 associated with meteorological factors in Lhasa, Tibet, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12257, https://doi.org/10.5194/egusphere-egu25-12257, 2025.

EGU25-16683 | ECS | Orals | AS3.13

Analyzing the Environmental Impact of Thermal Power Plants on Air Pollution across Taiwan. 

Szu Tung Yao and Christina W. Tsai

Air pollution is a high-profile issue that causes precipitation acidification, water pollution, and building corrosion, negatively affecting human respiratory health. As technology gradually digitalizes, the rise in electricity demand may exacerbate pollution, further impacting the environment and public health. The process of electricity generation emits significant amounts of air pollutants like SO₂, NOₓ, O₃, CO, PM₁₀, and PM₂.₅, which cause acid precipitation and smog that can potentially threaten public health. Among various methods of generating electricity, the thermal power-based method has the most significant impact on air pollution, accounting for 70% of the total, primarily through gas-fired and coal-fired power. To comprehend the environmental impact of electricity generation by the government-operated Taiwan Power Company, this study concentrates on identifying the relationship between electricity consumption, air pollutants, and hydro-meteorological factors. To achieve this aim, two data-driven methods are employed: (1) Complete Ensemble Empirical Mode Decomposition with Adaptive Noise (CEEMDAN), an improved version of Empirical Mode Decomposition (EMD), to extract long-term trends from non-stationary, non-linear data (2) Time-dependent Intrinsic Correlation (TDIC) to visualize and quantify the correlation, illustrating the degree of relationship between two time-series data sets. The CEEMDAN algorithm will decompose data into several Intrinsic Mode Functions (IMF) and one long-term trend of data. Those IMFs represent the changing data in different time scales. Subsequently, this research utilizes each IMF to reconstruct signals and generate wind rose diagrams. With the wind rose diagram, this research can analyze multi-scale distribution properties of wind direction and wind speed that can explore the changing trends of the wind field. By decoding these relationships, this research can better examine the degree of thermal power generation impacts on air pollution and how wind direction disperses air pollutants, providing a high-risk mapping to avoid human activities. Based on Taiwan's geographical address surrounded by the sea, this study can encompass the impacts of anthropogenic factors and natural factors, like monsoons, on air pollution, achieving a more comprehensive analysis. Moreover, integrating these findings and policy implementation enables more sustainable resource management and decision-making.

How to cite: Yao, S. T. and Tsai, C. W.: Analyzing the Environmental Impact of Thermal Power Plants on Air Pollution across Taiwan., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16683, https://doi.org/10.5194/egusphere-egu25-16683, 2025.

The El Niño-Southern Oscillation (ENSO) significantly affects the interannual variability of tropospheric ozone, but the quantitative contributions from individual processes and how the ozone-ENSO response will change in the future remain unclear. In this study, we apply the GEOS-Chem global chemical transport models to quantify the contribution of transport, chemistry, and biomass burning to ozone variability in different ENSO phases, evaluate the ability of different climate-chemistry models (CCMs) in the Coupled Model Intercomparison Project Phase 6 (CMIP6) in capturing the present-day ozone-ENSO response, and examine the future changes in such response. GEOS-Chem model simulation over 2005-2020 largely reproduces the ozone-ENSO response observed by the Ozone Monitoring Instrument (OMI) and Microwave Limb Sounder (MLS) instrument, including the instantaneous decrease (increase) in tropospheric ozone column (TCO) over tropical eastern (western) Pacific in the El Niño phase, and the delayed responses (3-9 months lagged behind the Nino 3.4 index) in South America and Africa. The combined effects of transport, chemistry, and biomass burning emissions explain 94%~98% of the variability of TCO in tropical Pacific during ENSO. Changes in transport patterns dominate the overall tropospheric ozone-ENSO response, by increasing TCO by 0.8 DU (53% of the total variability) in western Pacific region and decreasing TCO by 2.2 DU (92%) in the eastern Pacific region during the El Niño condition relative to the normal periods. Changes in atmospheric temperature, water vapor, and cloud cover reduce ozone in the lower and middle troposphere (500-800 hPa) in the eastern Pacific by 2.0 ppbv, comparable to the transport induced ozone decrease of 3.8 ppbv. Biomass burning emissions cause an averaged ozone increase of 0.8 DU in Indonesia during El Niño and 0.7 DU in Brazil during La Niña. We find that five out of ten CCMs in CMIP6 can reproduce the historical ozone-ENSO response in 1980-2014. Interactive tropospheric chemistry and accurate representation of vertical circulation in ENSO phases are vital for the CCMs to capture the ozone-ENSO response. These models with successful skills consistently indicate that the ozone-ENSO response will increase by approximately 20% by the end of the 21st century, driven by the strengthening anomalous circulation and high water vapor concentration in ENSO phases in a warming climate. These results are critical for understanding climate-chemistry interactions and for improving future ozone projection.

How to cite: Li, J., Wang, H., Fan, Q., and Lu, X.: Tropospheric ozone responses to the El Niño-Southern Oscillation (ENSO): quantification of individual processes and future projections from multiple chemical models , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16719, https://doi.org/10.5194/egusphere-egu25-16719, 2025.

EGU25-17363 | Posters on site | AS3.13

Role of Bay of Bengal cyclone  in unusual aerosol loading and fog events over the Kerala regions 

Komban Arun, Manguttathil Gopalakrishnan Manoj, Kuttikulangara Ahana, and Karathazhiyath Satheesan

Atmospheric conditions show significant variations during cyclone advancement and landfall in tropical regions. Here, we investigate the unusual fog event over the Kerala region associated with the Mandous cyclone (December 6-10, 2022) in the Bay of Bengal (BoB). This study also investigates the variations in atmospheric aerosol loading and its potential source identification. Before the landfall of cyclone Mandous, there was a significant increase in aerosol concentration over the Kerala region. Changes in prevailing wind patterns due to BoB cyclones lead to long-range transport of aerosols from the Indo-Gangetic Plain (IGP) and Rajasthan region to the South Indian region. The changes in meteorological parameters during these days are analyzed. Previous studies reported increased aerosol concentration during cyclone formation, but such events still need to be reported in the Kerala region. Unusual fog events in the Kerala region are associated with this increased aerosol loading. From the HYSPLIT back trajectory analysis, it is evident that particulate matter (PM2.5) has been brought to the Kerala region from multiple places in South Asia during these days. The IGP region contributes the majority of the transported aerosols. The average PM2.5 mass concentration over the Kerala region shows a sharp increase during these days. Mandous form in winter (December), and the PBL height is low during this season. From analysis, it is clear that all meteorological parameters favor fog formation. The increased loading of atmospheric aerosol and moisture to the Kerala region during the study period was associated with the formation of the Mandous cyclone. Low ventilation coefficient values imply less vertical mixing and a stable atmosphere. So, these conditions lead to the observed abnormal fog events over the Kerala region. This kind of event is rare in South Indian regions but significantly impacts air quality and human health. Large-scale transport during cyclones increases the concentration of PM2.5 in the south Indian region, leading to a poor Air Quality Index (AQI), significantly affecting human health.

How to cite: Arun, K., Manoj, M. G., Ahana, K., and Satheesan, K.: Role of Bay of Bengal cyclone  in unusual aerosol loading and fog events over the Kerala regions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17363, https://doi.org/10.5194/egusphere-egu25-17363, 2025.

EGU25-17376 | ECS | Orals | AS3.13

Climate Response to a Decade of Anthropogenic Emission Changes (2013-2023) 

Xiaochun Wang, Bin Zhao, Gregory Faluvegi, Yanning Zhang, Wen Yi, Drew Shindell, and Shuxiao Wang

Global emission patterns have changed significantly in the past decade as regions around the world started various reduction policies, notably marked by China's Air Pollution Prevention and Control Action Plan and IMO's regulations on shipping emissions. However, the climate response to these regional emission changes has not been fully quantified. Using two climate models (CESM2 and GISS), we conducted 80-year simulations and analyzed the last 70 years to study the radiative effects of emission changes during 2013-2023. Through designed 4 experiments using ABaCAS EI, CMIP6, and SEIM shipping emission inventories, we separated the climate impacts from three main sources: China, regions outside China, and global shipping emissions. We then used the FaIR model to evaluate their temperature responses.

Our model simulations show remarkable consistency in top-of-atmosphere radiative changes despite differences in aerosol-cloud interaction parameterizations. The total effective radiative forcing (ERF) is approximately 0.15 W/m², with China's emission changes contributing the largest forcing (0.06-0.07 W/m²), followed by other regions (0.04-0.05 W/m²) and shipping (0.04-0.05 W/m²). Spatial analysis reveals significant positive forcing (>2 W/m²) over East Asia (20°N-45°N, 100°E-125°E) with notable downstream effects. CESM2, with its higher resolution, shows stronger aerosol transport signals over the Pacific, while GISS exhibits weaker signals in regions far from sources.

While both models differ in simulating cloud-aerosol interactions, CESM2's more detailed aerosol and cloud microphysics schemes and stronger aerosol-cloud-radiation coupling capture more transport and indirect effects, though the result also has larger uncertainties. In the North Pacific region, both CESM2 and GISS simulate strong positive radiative forcing change, showing significant radiative anomalies consistent with CERES satellite observations of outgoing shortwave radiation changes during 2013-2023. Our results indicate that China's emissions, through downwind transport, contribute more to these radiative changes than shipping emissions.

The FaIR model results suggest that China's emission reductions have led to approximately 0.025°C warming, while global emission changes have contributed about 0.05°C. We also evaluated potential future temperature trends based on temperature response functions. These findings improve our understanding of how regional emission changes affect the global climate system and highlight the importance of coordinated emission reduction strategies across regions and sectors, considering the role of both continental and maritime emissions in global radiative forcing patterns and their implications for future climate policies.

How to cite: Wang, X., Zhao, B., Faluvegi, G., Zhang, Y., Yi, W., Shindell, D., and Wang, S.: Climate Response to a Decade of Anthropogenic Emission Changes (2013-2023), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17376, https://doi.org/10.5194/egusphere-egu25-17376, 2025.

EGU25-18288 | ECS | Orals | AS3.13

Meteorological Drivers of Compound Atmospheric Events Associated with High Mortality Rates in Spain 

Ginés Garnés-Morales, Pedro Jiménez-Guerrero, Salvador Gil-Guirado, Ester García-Fernández, Leandro Segado-Moreno, Eloisa Raluy-López, and Juan Pedro Montávez

Many studies have demonstrated the relationship between extreme meteorological events and air pollution with increased mortality. However, only a few studies attribute mortality excesses to compound events, where meteorological causes overlap with elevated atmospheric pollutant levels. In this work, we present a study on mortality excesses in Spain, air pollution, and their relationship with atmospheric circulation. Daily mortality rate data at a provincial level is used for the summer season for the period 2015-2022.

First, mortality extremes were categorized and related to preceding extreme atmospheric conditions. The results show that most mortality extremes are preceded by extreme atmospheric conditions, with a time lag that depends on the season and the variable considered. For instance, in Madrid during summer, the variables explaining mortality include temperature (minimum and maximum), ozone (O3), particulate matter (PM10), and their combinations. Influences from previous days are significant for more than 50% of cases, with a median lag of three days for ozone, two days for temperature, and one day for PM10, and deviations ranging from 1 to 3 days.

Once all days potentially associated with mortality extremes were identified, they were classified into different atmospheric circulation types (CTs) based on sea-level pressure (SLP), temperature at 850 mb, and geopotential height at 500 mb. This classification uses daily average fields derived from ERA5 reanalysis over a domain encompassing the entire Iberian Peninsula. For each identified CT, average fields of temperature, O3, and PM10 were calculated using CAMS reanalysis data. Additionally, the efficiency of each CT in all provinces was assessed. The results indicate that most situations leading to mortality extremes are associated with upper-level ridges, with the position and inclination of the ridge axis determining regional differences in the efficiency on mortality rates across the Iberian Peninsula.

 

Acknowledgments: The authors acknowledge Grant PID2020-115693RB-I00 funded by MCIN/AEI/ 10.13039/501100011033

How to cite: Garnés-Morales, G., Jiménez-Guerrero, P., Gil-Guirado, S., García-Fernández, E., Segado-Moreno, L., Raluy-López, E., and Montávez, J. P.: Meteorological Drivers of Compound Atmospheric Events Associated with High Mortality Rates in Spain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18288, https://doi.org/10.5194/egusphere-egu25-18288, 2025.

The health impacts of air pollution and temperature variations are of increasing concern, particularly in urban environments where emissions and population densities are high. Short-term exposure to pollutants such as sulfur dioxide (SO₂), nitrogen dioxide (NO₂), suspended particulate matter (SPM), and oxidants (Ox) has been linked to adverse health outcomes, including increased rates of cardiovascular and respiratory diseases. Additionally, temperature fluctuations, especially during extreme weather conditions, exacerbate the vulnerability of populations to these pollutants, contributing to excess mortality.

Japan, with its diverse climate and urban landscape, presents a unique case for studying the interactions between air pollution, temperature, and mortality. Hiroshima, located in a temperate climate, and Sapporo, in a colder region, offer contrasting environments to examine the seasonal and regional variations in these associations. This study investigates the short-term associations between temperature, air pollutants (SO₂, NO₂, suspended particulate matter (SPM), and oxidants (Ox)), and mortality in Hiroshima and Sapporo, Japan, from January 1, 2012, to December 31, 2019. Using a time-stratified case-crossover study design, we examine the impacts on cardiovascular, respiratory, and general mortality, focusing on gender- and age-specific differences. Seasonal variations, comparing summer and winter periods, and different emission levels across the study period are also considered. By analyzing these interactions, this study aims to deepen the understanding of how short-term environmental factors and pollution levels influence health outcomes in urban populations, contributing to targeted public health interventions in Japan.

How to cite: Marggraf, C., Huang-Lachmann, J.-T., Hashizume, M., and Ng, C. F. S.: Short-Term Associations Between Temperature, Air Pollutants (SO₂, NO₂, SPM, Ox), and Mortality in Hiroshima and Sapporo, Japan (2012–2019): Age and Gender-Specific Differences Across Seasons, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19665, https://doi.org/10.5194/egusphere-egu25-19665, 2025.

EGU25-20017 | ECS | Orals | AS3.13

Understanding Drivers of Extreme Ozone Events: A Sensitivity Study with WRF-Chem 

Leandro Segado-Moreno, Juan Pedro Montávez, Ginés Garnés-Morales, Eloisa Raluy-López, and Pedro Jiménez-Guerrero

Extreme weather events, such as stagnation conditions and heatwaves, are known to exacerbate hazardous air quality situations by promoting the accumulation and persistence of pollutants like ozone (O3) in the near-surface environment. In particular, during the summer over the Iberian Peninsula (IP), extreme O3 values often exceed the 180 µg/m3 threshold, significantly impacting air quality and public health. While meteorological factors like high temperatures and radiation are important drivers of these events, classifying them based solely on synoptic weather patterns fails to capture the full scope of the risks involved. Even when events are classified under the same synoptic category, O3 concentration can vary greatly. This implies that variability is not only due to direct meteorological influences, but also other factors related to transport, previous concentrations or processes linked to surface conditions can modify emissions of compouds that affect O3 formation. In this regard, biogenic volatile organic compound (BVOC) emissions from vegetation can significantly influence O3 formation in a complex and non-linear way. The amount and type of vegetation, as well as the available soil moisture, modulate these emissions.

In this study, we conducted sensitivity experiments using the Weather Research and Forecasting model coupled with chemistry (WRF-Chem, version 4.6.0) to explore how factors like soil moisture and vegetation amount influence extreme O3 events over the IP. We first performed simulations varying leaf area index (LAI) and soil moisture (SM) by multiplying the original fields of SM (all layers) and LAI by a factor ranging from 0.25 to 2. The results indicate that decreasing  the available soil water (-50%) increases BVOCs emission rates (20% spatial and temporal average), which is reflected in an increase in daily maximum O3 concentrations (10%). On the other hand, increasing the vegetation (50 %) leads to an increase in BVOC emission rates (10%), as well as in O3 concentrations (up to 10 %). The combined experiments exacerbated the changes, although most of the time they are smaller than the sum of the isolated experiments. 

Regional Climate Models (RCMs) often use climatological variables to characterize vegetation. Some studies show that differences in vegetation fraction with respect to climatological values can reach up to 40% over the IP. We performed a series of simulations of extreme O3 occurrences, employing both observed and climatological values of vegetation. Preliminary results indicate that such differences in vegetation moderately modify final O3 concentrations, in most cases obtaining better agreement with observations. 

Acknowledgements: Project PID2020-115693RB-I00 funded by MCIN/ AEI /10.13039/501100011033

How to cite: Segado-Moreno, L., Montávez, J. P., Garnés-Morales, G., Raluy-López, E., and Jiménez-Guerrero, P.: Understanding Drivers of Extreme Ozone Events: A Sensitivity Study with WRF-Chem, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20017, https://doi.org/10.5194/egusphere-egu25-20017, 2025.

EGU25-3629 | ECS | Posters on site | AS3.16

Rapid Ash Removal in the 2022 Hunga Volcano Plume: The Role of Aerosol Microphysical Processes 

Simran Chopra, Julia Bruckert, and Gholamali Hoshyaripour

The record-breaking January 2022 Hunga eruption raised questions regarding the large amount of water vapor (150 Tg) reaching the stratosphere and the surprisingly less amount of ash detected. The emission of such large amount of water vapor in numerical models poses its own challenges and limitations. From ground-based estimates of emitted ash, the emitted fine ash is estimated to be around 17-34 Tg, however, only up to 1-2 Tg was present in the atmosphere which indicates an extremely fast removal of ash. This study investigates the role of various aerosol dynamical processes and hence, the accelerated removal of ash particles. This is done through emission of ash, water vapor, SO2 and NaCl in the ICOsahedral Nonhydrostatic model with Aerosols and Reactive Tracers (ICON-ART). Three possible pathways of faster growth and consequently, removal of particles, are explored in this study. These include (1) ash particle growth due to coagulation with sea salt and further growth by water owing to the highly hygroscopic nature of sea salt, (2) fast wet aggregation of particles during the plume rise, and (3) activation of particles to large hydrometeors.  The results emphasize the importance of including sea salts emission along with ash and SO2 in modelling studies and the subsequent effects on aerosol dynamical processes. 

How to cite: Chopra, S., Bruckert, J., and Hoshyaripour, G.: Rapid Ash Removal in the 2022 Hunga Volcano Plume: The Role of Aerosol Microphysical Processes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3629, https://doi.org/10.5194/egusphere-egu25-3629, 2025.

EGU25-3642 | Posters on site | AS3.16

Radiative forcing and stratospheric ozone changes due to major forest fires and recent volcanic eruptions including Hunga Tonga 

Christoph Brühl, Matthias Kohl, Jos Lelieveld, Landon Rieger, and Michelle Santee

Using the chemistry-climate model EMAC with nudged tropospheric meteorology, we show that organic carbon injected into the stratosphere through forest fire-related pyro-cumulonimbi enhances heterogeneous chlorine activation due to enhanced solubility of HCl in particles containing organic acids and a larger aerosol surface area. After the 2019/2020 Australian mega-bushfires, the upward transport of the pollution plume led to enhanced ozone depletion in the Southern hemispheric lower stratosphere, in agreement with AURA-MLS satellite observations. It reduced total ozone in 2020 and 2021 by up to 28 DU around 70oS, accompanied by a dynamic reduction in August 2020 from the lofting of smoke-filled vortices, reaching 24 DU (total about 40 DU near 65oS). The eruption of Hunga Tonga in January 2022 led to a reduction of total ozone in the entire Southern hemisphere, exceeding 10 DU south of about 55oS in Austral spring of 2022 and 2023. The water vapor injection by the volcano modified only the vertical distribution of ozone loss.
The absorbing aerosol from the combined Australian and Canadian forest fire emissions in 2019/2020 caused the largest perturbation in stratospheric optical depth (e.g., seen in OSIRIS data) since the eruption of Pinatubo. It changed the instantaneous stratospheric aerosol forcing -derived at the top of  the atmosphere- from -0.2 W/m2 to +0.3 W/m2 in January 2020. In January 2022, the remaining effect was about 0.05 W/m2, reducing the negative forcing by volcanoes. The computed global aerosol radiative forcing caused by the Hunga Tonga eruption in 2022 was about -0.12 W/m2, decreasing to -0.06 W/m2 by December 2023, dominated by the change in stratospheric sulfate aerosols. The positive forcing of the injected water vapor was small (in agreement with other models). 

How to cite: Brühl, C., Kohl, M., Lelieveld, J., Rieger, L., and Santee, M.: Radiative forcing and stratospheric ozone changes due to major forest fires and recent volcanic eruptions including Hunga Tonga, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3642, https://doi.org/10.5194/egusphere-egu25-3642, 2025.

EGU25-3677 | ECS | Orals | AS3.16

Assessing the stratospheric temperature response to volcanic sulfate injections: insights from a multi-model framework 

Katharina Perny, Pavle Arsenovic, Christoph Brühl, Sandip Dhomse, Ales Kuchar, Anton Laakso, Graham Mann, Ulrike Niemeier, Giovanni Pitari, Ilaria Quaglia, Harald Rieder, Takashi Sekiya, Timofei Sukhodolov, Simone Tilmes, Claudia Timmreck, and Daniele Visioni

Volcanic sulfate injections into the stratosphere following major eruptions are able to modulate climate, as demonstrated by the well-documented 1991 Mt. Pinatubo eruption. Understanding the climate response to such events is critical, especially in the context of potential solar radiation management strategies to counteract climate change. An important part of volcanic impact on the atmospheric system originates from volcano-induced lower stratospheric heating that leads to changes in stratospheric circulation and transport and possibly in stratosphere-troposphere coupling and regional tropospheric circulation. Previous modeling studies have shown diverse results concerning these effects, partly due to model uncertainties and differences in simulation setup or study design, such as prescribed aerosols and/or chemistry, while the feedbacks between these system components were shown to be significant.

This study evaluates the tropical stratospheric temperature response to the Mt. Pinatubo eruption using eight global models with interactive aerosol microphysics. All models adhered to the Historical Eruptions SO2 Emission Assessment (HErSEA) protocol under the Interactive Stratospheric Aerosol Model Intercomparison Project (ISA-MIP). We focus on the uncertainties related to initial SO2 emission amounts and injection heights. Results reveal that while models exhibit consistent sensitivity to initial SO2 amounts and injection heights, the magnitude and extent of the stratospheric temperature response vary. By comparing model outputs and observations, this study enhances our understanding of individual model performances and the current multi-model uncertainty range and provides critical insights for future climate impact assessments of volcanic eruptions.

How to cite: Perny, K., Arsenovic, P., Brühl, C., Dhomse, S., Kuchar, A., Laakso, A., Mann, G., Niemeier, U., Pitari, G., Quaglia, I., Rieder, H., Sekiya, T., Sukhodolov, T., Tilmes, S., Timmreck, C., and Visioni, D.: Assessing the stratospheric temperature response to volcanic sulfate injections: insights from a multi-model framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3677, https://doi.org/10.5194/egusphere-egu25-3677, 2025.

EGU25-6342 | Posters on site | AS3.16

Will the climate response to volcanic eruptions change in the future? 

Claudia Timmreck, Shih-Wei Fang, Johannes Meuer, Johann Jungclaus, Christopher Kadow, and Hauke Schmidt

In the future, in a warmer world due to anthropogenic greenhouse gas forcing, the impact of natural forcing on climate could change dramatically.  However, it is not yet clear how strong a volcanic forcing as in the early 19th century will affect future climate. Previous studies show both an amplification of the surface cooling response, mainly due to an increase in upper ocean stability, and a weakening of the volcanic-induced surface cooling in a future climate state due to a reduced effective volcanic aerosol radiative forcing.

To assess how different climate states affect the climate response to volcanic forcing, we have performed MPI-ESM ensemble experiments under historical, 4xCO2 and present-day conditions with volcanic forcing equivalent to that of the early 19th century.  On these simulations, we have also tested explicable artificial intelligence methods to see if they are able to achieve a similar skill for specific fingerprints in the temperature record when the boundary conditions are very different from the present, as in the case of a 4xCO2 scenario.

We find that different changes in Arctic sea ice cover and northern hemisphere winter sea level pressure are induced by the same volcanic forcing under distinct climate states, while the large-scale average temperature response shows no significant differences.  The volcanic fingerprint in the surface temperature pattern is similar for all climate states for large volcanic eruptions in the first post-volcanic year, while the background state becomes relevant afterwards, as well as for smaller eruptions

How to cite: Timmreck, C., Fang, S.-W., Meuer, J., Jungclaus, J., Kadow, C., and Schmidt, H.: Will the climate response to volcanic eruptions change in the future?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6342, https://doi.org/10.5194/egusphere-egu25-6342, 2025.

EGU25-10357 | Orals | AS3.16

Modulation of the Northern Polar Vortex by the Hunga Tonga-Hunga Ha’apai Eruption and Associated Surface Response 

Ales Kuchar, Timofei Sukhodolov, Gabriel Chiodo, Andrin Jörimann, Jessica Kult-Herdin, Eugene Rozanov, and Harald Rieder

The January 2022 eruption of Hunga Tonga-Hunga Ha’apai (HTHH) injected unprecedented amounts of water vapour (WV) and sulfur dioxide (SO2) into the stratosphere, significantly impacting the Earth's climate system. Utilizing the Earth System Model SOCOLv4, this study investigates the dynamical implications of the middle-atmosphere disturbances caused by HTHH. A novel dynamical pathway linking water-rich volcanic eruptions to surface climate was identified. The excess stratospheric WV led to significant anomalies in atmospheric circulation, particularly influencing the Northern Hemisphere polar vortex (PV). The findings highlight the potential for such eruptions to modulate the stratospheric PV and subsequent surface climate through altered temperature gradients and weakened polar-night jets, contributing to sudden stratospheric warmings (SSWs). Furthermore, we explain the mechanism dependency on model-projected forcing and its relation to identified biases common also in other chemistry-climate models.

How to cite: Kuchar, A., Sukhodolov, T., Chiodo, G., Jörimann, A., Kult-Herdin, J., Rozanov, E., and Rieder, H.: Modulation of the Northern Polar Vortex by the Hunga Tonga-Hunga Ha’apai Eruption and Associated Surface Response, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10357, https://doi.org/10.5194/egusphere-egu25-10357, 2025.

Various sets of metrics have been used to rank the performance of CMIP6 models for a variety of purpose.

Here we present a potential set of metrics that would simplify a similar ranking for the purpose of evaluating the skill of climate models with a fully resolved stratosphere, including dynamics, chemistry, and aerosol microphysics in representing perturbations to stratospheric composition, such as past volcanic eruptions, as a first step to determine the reliability in future cases such as new volcanic eruptions or Stratospheric Aerosol Intervention.

Our purpose is to find metrics that include available observations of large and medium volcanic eruptions, such as Mt. Pinatubo in 1991, and that also consider the uncertainties in past retrievals, and that are representative of models skills across time (i.e. considering not just the initial plume development, but also the e-folding time and ultimate fate of the aerosol cloud) and space. We include metrics that consider aerosol spatial distribution, local and global size distribution and chemical properties through surface area density.

Our set of metrics could be of great use as more models in CMIP7 start including prognostic aerosols schemes and higher tops, and could inform future strategies for better observations of the stratospheres, as well as identify necessary variables to be requested by CMIP as part of the data requests prioritization for the Atmosphere Working Group.

How to cite: Visioni, D. and Quaglia, I.: Developing a set of simple metrics to evaluate the performance of models with interactive stratospheric aerosols, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10745, https://doi.org/10.5194/egusphere-egu25-10745, 2025.

EGU25-11701 | ECS | Orals | AS3.16

Self-lofting and radiative forcing of stratospheric aerosol from major wildfires and how it compares to volcanic eruptions 

Raphaël Lebrun, Yevgeny Derimian, François Ravetta, Jérôme Bureau, and Sergey Khaykin

Caused by intense wildfires, Pyrocumulonimbus generate vigorous convective updrafts that inject biomass burning plumes into the stratosphere. Due to the absorption of solar radiation by carbonaceous aerosols, these plumes are uplifted by radiative heating, up to 35 km altitude, which prolongs their stratospheric residence time. In this study we model the self-lofting of these stratospheric plumes as well as their radiative impact.

In the first step, we focus on the physical properties of these plumes and the radiative modeling of their self-lofting. Measurement-based determination of the Single Scattering Albedo (SSA) for stratospheric aerosols is however a challenging task. We thus attempt to constrain the SSA using a combination of radiative transfer modeling and observations from both ground-based and CALIPSO space-borne lidars, as well as use of OMPS-LP extinction profiles. The DIScrete Ordinate Radiative Transfer (DISORT) model, as part of Atmospheric Radiative Transfer Database for Earth Climate Observation (ARTDECO) numerical tool is employed to reproduce the observed self-lofting rate of the plume for varying properties of the plume. We find that the aerosol optical depth and the geometrical thickness of the plume are crucial parameters to model the self-lofting. We also take into account the variations of the underlying cloud cover and surface albedo to better model the self-lofting mechanism.

In the second step, having assessed the SSA, we estimate the radiative forcing induced by these plumes at the top and the bottom of the atmosphere. This method is applied to the Pacific Northwest Event (PNE) wildfire outbreak in August 2017 and the Australian New Year Super Ourbreak (ANYSO) in 2019/20. The results are then compared with previous studies. Finally, we compare the radiative forcing efficiencies of stratospheric smoke with that of stratospheric aerosols from moderate volcanic eruption on local and global scales.

How to cite: Lebrun, R., Derimian, Y., Ravetta, F., Bureau, J., and Khaykin, S.: Self-lofting and radiative forcing of stratospheric aerosol from major wildfires and how it compares to volcanic eruptions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11701, https://doi.org/10.5194/egusphere-egu25-11701, 2025.

EGU25-12390 | Posters on site | AS3.16

ENSO response to tropical volcanic eruptions: the role of the season 

Francesco S.R. Pausata and David Zanchettin

Stratospheric volcanic aerosol can have major impacts on the global climate. However, these impacts are eruption specific, as they critically depend on the characteristics of the eruption, such as magnitude, location and timing. Towards understanding these criticalities, only a handful of studies have either assessed the effects of eruptions at distinct times throughout the year or the location of eruption. To our knowledge, no study has hitherto considered the combined of the timing and location of an eruption. Here we investigate variations in the impact of volcanic eruptions linked on the timing of the eruption in relation to the seasons of the year and the location (Northern or Southern Tropical eruption), focusing on ENSO dynamics. In doing so, we use the Norwegian Earth System Model (NorESM) to perform a set of sensitivity experiments in which the tropical volcanic eruptions are set to go off at the beginning of each season. These experiments are meant to shed light on the role of the season in shaping the ENSO response to volcanic eruption, elucidating the nuanced role of volcanic forcing in modulating ENSO variability and enhancing our predictive capabilities of this influential climate phenomenon. In our contribution, we will describe first results from our experiments showing how boreal spring and summer Northern Tropical eruptions lead to El Niño-like conditions in the winter of the eruption, followed by strong La Niña conditions. On the other hand, boreal fall and winter eruptions causes a weak La Niña on the first 6-8 months, followed by El Niño conditions in the winter after the eruption. For Southern Tropical eruptions the response is muted and only fall and winter eruptions show El Niño conditions in the second winter of the eruption. To better understand the different responses, we will also interpret the model results within the framework of a simple delayed oscillator of ENSO.

How to cite: Pausata, F. S. R. and Zanchettin, D.: ENSO response to tropical volcanic eruptions: the role of the season, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12390, https://doi.org/10.5194/egusphere-egu25-12390, 2025.

EGU25-12721 | ECS | Orals | AS3.16

Unveiling volcanic forcing through lunar eclipses: past, present and future perspectives 

Lucas Boissel, Sébastien Guillet, Charlie Hureau, Franck Lavigne, and Salem Dahech

Explosive volcanic eruptions inject substantial quantities of sulfur gases into the atmosphere significantly influencing global temperatures and hydrological cycles. The formation of sulfate aerosols in the stratosphere following such eruptions can give rise to unusual optical phenomena, including solar dimming, red twilight glows, reddish solar halos, and dark total lunar eclipses. Recently, lunar eclipses have emerged as a valuable tool for reconstructing past stratospheric turbidity and refining the dating of major volcanic eruptions (Guillet et al., 2023).

This study presents a preliminary reconstruction of stratospheric aerosol optical depth (SAOD) from 1600 to 1850 CE, based on descriptions of 80 lunar eclipses documented in over 1,000 historical sources from across Europe. The reconstructed SAOD dataset was compared with bipolar ice core records (Sigl et al., 2015), model-derived aerosol optical depth (Toohey and Sigl, 2017), and climate reconstructions.

Our findings reveal that the darkest lunar eclipses of the past 400 years – occurring in 1601, 1642, 1696 and 1816 – correspond to the largest volcanic eruptions recorded in ice cores and align with significant cooling events in the Northern Hemisphere. This study highlights the potential of lunar eclipse observations to complement ice core data, providing additional, robust information to refine global stratospheric aerosol databases, which are essential for future climate modeling.

This contribution will also discuss plans to extend the dataset to the present day and address the inherent limitations and uncertainties associated with the methodology.

 

References:

Guillet, S., et al. (2023). Lunar eclipses illuminate timing and climate impact of medieval volcanism. Nature, 616, 90–95.

Sigl, M., et al. (2015). Timing and climate forcing of volcanic eruptions for the past 2,500 years. Nature, 523, 543–549.

Toohey, M., Sigl, M. (2017). Volcanic stratospheric sulfur injections and aerosol optical depth from 500 BCE to 1900 CE. Earth Syst. Sci. Data, 9, 809–831.

How to cite: Boissel, L., Guillet, S., Hureau, C., Lavigne, F., and Dahech, S.: Unveiling volcanic forcing through lunar eclipses: past, present and future perspectives, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12721, https://doi.org/10.5194/egusphere-egu25-12721, 2025.

EGU25-12900 | ECS | Posters on site | AS3.16

The Impact of 2022 Hunga Tonga-Hunga Ha’apai (Hunga) Eruption on Stratospheric Circulation and Climate 

Simchan Yook, Susan Solomon, and Xinyue Wang

     The Hunga Tonga-Hunga Ha’apai (Hunga) volcanic eruption in January 2022 injected a substantial amount of water vapor and a moderate amount of SO2 into the stratosphere. Both satellite observations in 2022 and subsequent chemistry-climate model simulations forced by realistic Hunga perturbations reveal large-scale cooling in the Southern Hemisphere (SH) tropical to subtropical stratosphere following the Hunga eruption. This study analyzes the drivers of this cooling, including the distinctive role of anomalies in water vapor, ozone, and sulfate aerosol concentration on the simulated climate response to the Hunga volcanic forcing, based on climate simulations with prescribed chemistry/aerosol. Simulated circulation and temperature anomalies based on specified-chemistry simulations show good agreement with previous coupled-chemistry simulations and indicate that each forcing of ozone, water vapor, and sulfate aerosol from the Hunga volcanic eruption contributed to the circulation and temperature anomalies in the Southern Hemisphere stratosphere. Our results also suggest that 1) the large-scale stratospheric cooling during the austral winter was mainly induced by changes in dynamical processes, not by radiative processes, and that 2) ozone’s radiative feedback contributed to the prolonged cold temperature anomalies in the lower stratosphere (~70 hPa level) and hence to long lasting cold conditions of the polar vortex.

How to cite: Yook, S., Solomon, S., and Wang, X.: The Impact of 2022 Hunga Tonga-Hunga Ha’apai (Hunga) Eruption on Stratospheric Circulation and Climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12900, https://doi.org/10.5194/egusphere-egu25-12900, 2025.

EGU25-13646 | Posters on site | AS3.16

Changes in the spectral composition of surface solar radiation under the presence of stratospheric aerosols: a case study for the Pinatubo eruption 

Ilias Fountoulakis, Stergios Misios, Anna Gialitaki, Antonis Gkikas, Vassilis Amiridis, Anna Kampouri, Dimitra Kouklaki, Andreas Kazantzidis, Kostas Eleftheratos, Konstantinos Kourtidis, Samuel Rémy, Bernhard Mayer, and Christos S. Zerefos

The presence of aerosols in the stratosphere alters the spectral shape, the amount and the spatial distribution of the solar light that reaches the Earth surface. Such changes in surface solar radiation have been discussed in a few studies, but the role of the underlying tropospheric aerosol layer in the presence of stratospheric aerosols has not been considered. In this study we investigate the changes in the direct and global spectral surface solar irradiances following the extremely intense volcanic eruption (VEI=6) of Mount Pinatubo (15°N, 120°E) in June 1991. The eruption of Mount Pinatubo ejected massive loads of sulphate and ash particles into the stratosphere, which covered the entire globe after three weeks and then remained in the stratosphere for several months. In the aftermath, major perturbations of the stratospheric ozone layer and the near-surface temperature have been documented. Here, we provide model-derived stratospheric aerosol optical properties, constrained by ground-based and airborne remote sensing and in-situ data, to the radiative transfer model libRadtran to calculate the spectral surface solar irradiance in the wavelength range 350 – 750 nm. Radiative transfer simulations have been performed for two European sites where in situ measurements of the aerosol extinction profile were available a few months after the eruption, assuming different concentrations and types of tropospheric aerosols present in the atmosphere along with the overlying stratospheric volcanic layers, as well as different solar zenith angles. Changes in the spectral composition and the distribution of surface solar radiation in the considered spectral range play a key role in many biological processes (e.g., photosynthesis), as well as in solar energy production. Thus, our results provide insights on how such processes could be impacted after future volcanic eruptions or under solar radiation modification scenarios.

Acknowledgements: This work has been supported by the action titled “Support for upgrading the operation of the National Network for Climate Change (CLIMPACT II)”, funded by the Public Investment Program of Greece, General Secretary of Research and Technology/Ministry of Development and Investments.  

How to cite: Fountoulakis, I., Misios, S., Gialitaki, A., Gkikas, A., Amiridis, V., Kampouri, A., Kouklaki, D., Kazantzidis, A., Eleftheratos, K., Kourtidis, K., Rémy, S., Mayer, B., and Zerefos, C. S.: Changes in the spectral composition of surface solar radiation under the presence of stratospheric aerosols: a case study for the Pinatubo eruption, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13646, https://doi.org/10.5194/egusphere-egu25-13646, 2025.

EGU25-13842 | ECS | Orals | AS3.16

Stratospheric Aerosol layer responses to volcanic and wildfire perturbations 

Alexandre Baron, Katie Smith, Elizabeth Asher, Parker Case, Peter Colarco, Emrys Hall, Patrick Cullis, Nicolas Mastromonaco, Alex Fritz, Stephanie Evan, Jerome Brioude, Jean-Marc Metzger, Matthew Martinsen, Darryl Kuniyuki, David Nardini, Penny Smale, Ben Liley, Richard Querel, and Troy Thornberry

The stratospheric aerosol layer plays a critical role in the climate system and is often disrupted by natural phenomena such as volcanic eruptions and extreme wildfire events. These perturbations differ significantly in their injection magnitude, aerosol mass, composition, and the altitude of material deposition. When coupled with the dynamic and chemical state of the stratosphere, these factors produce varied responses in the aerosol layer’s optical and microphysical properties.

Quantifying microphysical responses in detail requires reliable in situ observations, such as those provided by the NOAA Balloon Baseline Stratospheric Aerosol Profiles (B2SAP) network. Spanning latitudes from 72°N to 90°S and capturing data from the surface to approximately 28 km, regular B2SAP soundings monitor the stratospheric aerosol background and the evolution of perturbations over time and space. The Portable Optical Particle Spectrometer (POPS) in the B2SAP payload measures aerosol number and  size distribution, variables crucial for understanding stratospheric aerosol microphysics and refining satellite retrievals of aerosol extinction and effective radius.

In this study, we leverage data collected by B2SAP since its inception in 2019, encompassing a range of perturbations from moderate to large volcanic eruptions and extreme wildfire events, including the 2019–2020 Australian wildfires. We compare in situ observations to satellite-derived measurements, examining differences in aerosol extinction and effective radius. Additionally, we interpret POPS size distribution data alongside NASA GEOS Chemistry Climate Model outputs, providing insights into the processes driving the observed variability in stratospheric aerosol responses.

How to cite: Baron, A., Smith, K., Asher, E., Case, P., Colarco, P., Hall, E., Cullis, P., Mastromonaco, N., Fritz, A., Evan, S., Brioude, J., Metzger, J.-M., Martinsen, M., Kuniyuki, D., Nardini, D., Smale, P., Liley, B., Querel, R., and Thornberry, T.: Stratospheric Aerosol layer responses to volcanic and wildfire perturbations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13842, https://doi.org/10.5194/egusphere-egu25-13842, 2025.

EGU25-14519 | ECS | Posters on site | AS3.16

State dependence of stratospheric aerosol chemistry-climate impacts in GFDL-ESM4.1 

Shipeng Zhang, Vaishali Naik, Larry Horowitz, and Yuchao Gao

Projecting the chemistry-climate effects of stratospheric aerosols within general circulation models (GCMs) requires simulating multiple coupled processes, which are subject to large uncertainties. Here, we utilize an updated version of the GFDL Earth System Model (GFDL-ESM4.1) with an interactive representation of the stratospheric sulfur cycle to explore the state dependence of stratospheric aerosol chemistry-climate impacts in GFDL-ESM4.1. Understanding this state dependence is crucial for assessing the volcanic chemistry-climate impacts under global warming and is beneficial for evaluating the effectiveness of stratospheric aerosol injection as a geoengineering approach.

We first conduct a baseline simulation from 1989 to 2014, driven by observed sea-surface temperature and sea ice, and including volcanic emissions of sulfur into the stratosphere. Then, we perform sensitivity simulations with sea surface temperature uniformly increased or decreased by 4K to examine the chemistry-climate impacts of stratospheric aerosols under warmer and cooler climate conditions. Our results show that stratospheric aerosol optical depth (SAOD) and burden are sensitive to surface temperature, in our simulations with prescribed volcanic injection heights. In a warmer climate, the accelerated Brewer-Dobson Circulation causes a rapid decay of stratospheric sulfate lifetime and lower SAOD in the 3 years following a the Mt. Pinatubo eruption. The warmer climate also produces a continuously lower SAOD during periods without major eruptions. Changes in SAOD from major eruptions are more sensitive to warming (approximately -11%/K) than to cooling (approximately -5%/K) from the baseline climate. Moreover, the lower SAOD from major eruptions is compensated by higher natural aerosol emissions under a warmer climate, buffering the changes in total AOD. Combined changes—decreased SAOD, albedo feedback, and increased natural aerosols emissions—result in an increase of clear-sky shortwave radiative effect by up to ~2.8 W/m2 in a warmer climate compared to the baseline. We will also explore the follow-on effects on ozone chemistry from the sensitivity of stratospheric aerosols to surface temperature in GFDL-ESM4.1. These results highlights the importance of the interactive sulfur cycle approach in GCMs.

How to cite: Zhang, S., Naik, V., Horowitz, L., and Gao, Y.: State dependence of stratospheric aerosol chemistry-climate impacts in GFDL-ESM4.1, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14519, https://doi.org/10.5194/egusphere-egu25-14519, 2025.

EGU25-15396 | Posters on site | AS3.16 | Highlight

Can Reanalysis Datasets Show Unprecedented Stratospheric Water Vapor After the Hunga Tonga-Hunga Ha’apai Eruption? 

Yang Li, Xin Zhou, Wenhui Zhang, Chaochao Gao, Quanliang Chen, and Wuhu Feng

The 2022 Hunga Tonga-Hunga Ha'apai (HTHH) volcanic eruption injected around 150 Tg water vapor into the stratosphere. Using Microwave Limb Sounder (MLS) water vapor measurement, this study provides the first evaluation of the HTHH-induced stratospheric water vapor (SWV) products revealed by the ERA5, MERRA2 and M2-SCREAM reanalyses. Results show that ERA5 and MERRA2 underestimate the SWV mass compared to MLS observations, while M2-SCREAM shows good consistency not only in the magnitude but also in the transport and depletion details. M2-SCREAM also perform well in the estimation of the long-term trend of SWV mass, while ERA5 and MERRA2 both overestimate the trend, suggesting the potential value of M2-SCREAM in estimating the long-term climatic influence of HTHH eruption. The extent to which the assimilation of SWV contributes to the significant discrepancies observed between M2-SCREAM and ERA5 as well as MERRA2 offers valuable insights for enhancing the numerical simulation of reanalyses.

How to cite: Li, Y., Zhou, X., Zhang, W., Gao, C., Chen, Q., and Feng, W.: Can Reanalysis Datasets Show Unprecedented Stratospheric Water Vapor After the Hunga Tonga-Hunga Ha’apai Eruption?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15396, https://doi.org/10.5194/egusphere-egu25-15396, 2025.

EGU25-16379 | ECS | Posters on site | AS3.16

Radiative Effects of Hunga Volcanic Eruption in the Middle Atmosphere: A Model and Observation-Based Analysis 

Alistair Bell, Gunter Stober, Guochun Shi, Hanli Liu, and Axel Murk

The 2022 Hunga volcanic eruption, which injected approximately 150 Tg of water vapour directly into the stratosphere, was an unprecedented event and provided a basis for a multitude of middle atmospheric studies. Changes in water vapour in the stratosphere and above affect the chemical composition of the middle atmosphere, the heating and cooling rates in this region, and the longwave downwelling fluxes at the surface.

In this study, we focus on the radiative impact of the changes in the water vapour mixing ratio at two locations where continuous profiling of water vapour has been performed using high-spectral-resolution microwave radiometers. The radiative transfer schemes included in the Whole Atmosphere Community Climate Model (WACCM-X (SD)) are compared to a line-by-line radiative transfer scheme from the Atmospheric Radiative Transfer Simulator (ARTS) to assess the accuracy of these radiative transfer schemes in analysing differences in heating rates and fluxes in the middle atmosphere.

How to cite: Bell, A., Stober, G., Shi, G., Liu, H., and Murk, A.: Radiative Effects of Hunga Volcanic Eruption in the Middle Atmosphere: A Model and Observation-Based Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16379, https://doi.org/10.5194/egusphere-egu25-16379, 2025.

EGU25-16471 | Posters on site | AS3.16

The dependence of tracer transport on grid refinement 

Ulrike Niemeier, Luis Kornblueh, and Andrea Schneidereit

The lifetime of sulphur in the strartosphere depends on volcanic emission parameters and aerosol microphysical processes, as well as on particle transport. These processes interact and determine the particle size and optical depth of the volcanic cloud.
While tracer transport, via advection and turbulence, affects mixing and dilution, it feeds back onto the aerosol concentration and the microphysical processes.  At the same time, the aerosols absorb terrestrial radiation, which heats the stratospheric aerosol layer and affects transport. Thus, all processes interact, feedback to each other and determine the concentration and particle size of the aerosol.
 
To disentangle the role of aerosol microphysical processes and heating from the role of transport in aerosol evolution, we introduced a passive tracer. This allows us to determine the impact of the grid size on stratospheric dynamics and tracer transport.  Therefore, we added emissions of the gas SF6 (sulphur hexafluoride) to ICON-XPP. SF6 is inert in the troposphere and lower stratosphere and is emitted in industrial production. This allows us to compare the simulated distribution of SF6 with observations.

Comparison with observations allows us to better understand the transport processes in the model. Important for the transport of a volcanic cloud is the velocity of the vertical transport in the tropical pipe or the meridional transport to higher latitudes. Since previous studies have shown a dependence of the transport in the tropical pipe on the model grid, we have performed simulations with different horizontal and vertical resolutions to determine the role of the grid. We had to tune the model for the different resolutions. In the process, we obtained different dynamical states in the lower tropical stratosphere, the region of the quasi-biennial oscillation (QBO). For example, we got only easterly or only westerly jets in the lower tropical stratosphere. These different jets allow us to see the effect of the QBO on the transport of SF6.

 

How to cite: Niemeier, U., Kornblueh, L., and Schneidereit, A.: The dependence of tracer transport on grid refinement, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16471, https://doi.org/10.5194/egusphere-egu25-16471, 2025.

The release of stratospheric aerosols from major volcanic eruptions induces large-scale global and regional climate impacts through radiative perturbations. The extent of these impacts depends on the season, aerosol-cloud distribution, the height reached by the ejections, and the latitude of the eruption, causing symmetrical and asymmetrical forcing. Previous studies have linked some severe Sahel drought conditions during the 20th century from two to four seasons of post-eruption feedback. However, a detailed analysis of the causal mechanism through the complex teleconnections driving changes of the African monsoon and its atmospheric dynamics in response to the volcanic eruption is yet to be addressed. Besides, the interest in the deliberate stratospheric injection of sulfate aerosols as a Solar Radiation Management (SRM) technique has increased due to the difficulties of limiting the global mean temperature to 1.5 or 2.0 °C above the Pre-industrial level. This implies the need to investigate the associated hydro-climate changes in response to such climate change solution techniques across Africa. In this study, we explore the response of the African monsoon and its driving teleconnections changes to past volcanic eruptions to better understand the potential climate impacts of future eruptions and even further to the proposed SRM geoengineering. Since larger and wider varieties of eruptions occurred in the last millennium compared to the 20th century, we use the past millennium's natural external volcanic forcings as an analog to explore the dynamics feature and associated teleconnections of the African monsoon. We rely on the varied experimental simulation outputs of the state-of-the-art Earth System Models that participated in the sixth phase of the Coupled Model Intercomparison Project (CMIP6). More specifically, we use the models that simulated the past millennium (PMIP4; Jungclaus et al., 2017), volcanic forcing experiments (VolMIP; Zanchettin et al., 2016), and stratospheric aerosol geoengineering experiments (GEOMIP; Jones et al., 2021). Overall, the analyzed responses from the modelling perspective provide an overview of the impact of volcanic forcings across Africa in the past, present, and future climates.

How to cite: Arthur, F. and Boateng, D.: The response of African monsoons to the symmetric and asymmetric Volcanic eruptions in past and future climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16818, https://doi.org/10.5194/egusphere-egu25-16818, 2025.

EGU25-17973 | ECS | Posters on site | AS3.16

Sensitivity of Monsoon Onset to Idealised Volcanic Forcing 

Shreyas Iyer, Moritz Guenther, Chetankumar Jalihal, and Claudia Timmreck

Large volcanic eruptions are a source of climate variability, affecting global temperatures and precipitation. The hydrology of the Indian monsoon region is particularly sensitive to volcanic forcing. Previous studies have focused on the seasonal mean response of the Indian monsoon to eruptions. Here, we investigate the changes to the onset of the monsoon, which is an important characteristic that impacts the water budget of the region. Using large Earth System ensemble simulations with idealised model eruptions that inject 40 Tg of sulphur into the stratosphere at varying latitudes, we observe changes in onset date by a few weeks compared to an unforced case. We find that the date of onset of the Indian summer monsoon is strongly dependent on the eruption latitude. Our results show a delayed (advanced) Indian monsoon onset for a Northern (Southern) Hemispheric eruption. However, the internal variability of the monsoon system also influences the onset. We find that existing mechanisms linking internal variability to monsoon onset are insufficient to explain the onset changes observed due to volcanic forcings. Based on the Low-Level Jet (LLJ) and ITCZ frameworks, we propose a new mechanism of monsoon onset variation due to volcanic eruptions. We show that not just a strengthening LLJ, but also an increased moisture flux into the Indian monsoon region triggers an earlier onset.

How to cite: Iyer, S., Guenther, M., Jalihal, C., and Timmreck, C.: Sensitivity of Monsoon Onset to Idealised Volcanic Forcing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17973, https://doi.org/10.5194/egusphere-egu25-17973, 2025.

EGU25-18228 | ECS | Orals | AS3.16

 The impact of the 2022 Hunga water-rich eruption on polar stratospheric clouds, chlorine activation and ozone depletion 

Saffron Heddell, Martyn Chipperfield, Sandip Dhomse, Graham Mann, Wuhu Feng, Masaru Yoshioka, and Xin Zhou

The Hunga eruption, January 2022, injected ~150 Tg of water vapour into the sub-tropical mid-stratosphere, unprecedented in the satellite era. The effects of the Hunga water vapour on the heterogeneous chemistry in the Antarctic stratosphere did not occur in the 2022 season, with the vortex edge a barrier to transport to high southern latitudes, until vortex break-up. Here, we analyse chlorine activation and ozone loss impacts starting with the 2023 vortex, and find these effects were not uniform throughout the vortex, and were limited by widespread mid-winter dehydration that occurs in the Antarctic each year, mainly in the colder “vortex core” region, via ice-containing polar stratospheric clouds (PSCs).  

Heterogeneous, chlorine-activating reactions on PSC surfaces play a key role in polar stratospheric ozone depletion and the formation of the seasonal Antarctic ozone hole. Stratospheric water vapour is one of the key factors in PSC formation; thus, the water vapour enhancement from Hunga is likely to impact PSC occurrence and therefore may increase the ozone depletion. However, the effects may vary between different regions of the vortex. The core region experiences the lowest temperatures, frequently reaching the threshold for ice PSCs, and the most extensive dehydration (in the lower stratosphere) over much of the vortex season. In contrast, the edge region is more sunlit, less cold, and experiences less extensive dehydration than the core, meaning there is scope for different chemical impacts in this region. Overall, the Hunga eruption offers a unique opportunity to test our understanding of how a large-scale increase in water vapour impacts polar ozone, and how the vortex structure influences the timing and magnitude of the effects.

Here we use the TOMCAT three-dimensional chemical transport model to investigate the impacts of the Hunga water vapour on Antarctic stratospheric ozone and associated heterogeneous chlorine reactions, comparing the 2023 and 2024 Antarctic vortex seasons. We find that the enhanced water vapour raised PSC formation temperatures, resulting in earlier formation and, consequently, an earlier onset of the heterogeneous chemistry and chlorine activation. However, it is evident that the vortex structure has some influence on the impact. Compared to a control simulation without Hunga, the effect on the edge region occurs throughout the PSC season, whereas the core, due to effective dehydration, experiences large differences at the beginning and end of the season, with minimal differences in between.

We will also briefly summarise the impact of Hunga water vapour on Arctic springtime ozone in recent years, including 2025. The effect of Hunga in the Arctic has so-far been limited by the timing of the water transport (2022/23) and a series of stratospheric warming events (SSWs) (2023/24). However, the 2024/25 Arctic winter began colder than usual in December/January. Therefore, effects of the Hunga water vapour may be more pronounced during this Arctic winter subject to any warming events still to come.

How to cite: Heddell, S., Chipperfield, M., Dhomse, S., Mann, G., Feng, W., Yoshioka, M., and Zhou, X.:  The impact of the 2022 Hunga water-rich eruption on polar stratospheric clouds, chlorine activation and ozone depletion, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18228, https://doi.org/10.5194/egusphere-egu25-18228, 2025.

The stratospheric aerosol layer is a key component of the climate system through its impact on radiation, chemistry and climate. While satellite observations have observed this layer for more than 4 decades through solar occultation, limb scatter and lidar techniques, we still lack in situ measurements to fully understand how its spatial and temporal evolution vary through the influence of multiple sources. Long-term balloon measurements of stratospheric aerosols are available mostly at mid-latitudes and do not cover the tropics, a key region that largely affects the supply and the transport of stratospheric aerosols at global scales. Our team has deployed at multiple locations including Australia, India, Brazil since the past decade to study the impacts of volcanic eruptions, the Asian monsoon and PyroCbs on the stratosphere through in situ measurements. Leveraging on this experience, we believe that the next step is to conduct regular balloon-borne observations through a new network, the Balloon Network for stratospheric aerosol Observation (BalNeO). During this presentation, we will describe the overall objectives of BalNeO and show some preliminary results.

How to cite: Vernier, J.-P.: Balloon Network for stratospheric aerosol Observations (BalNeO): A new network to monitor the stratosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18647, https://doi.org/10.5194/egusphere-egu25-18647, 2025.

EGU25-18827 | ECS | Posters on site | AS3.16

Winter Warming in Northern Eurasia Following the 1783 Laki Volcanic Eruption 

Linshan Yang, Chaochao Gao, and Fei Liu

        Northern Eurasian winter warming (NEWW) is reported both in the observation and reconstruction following major tropical volcanic eruptions. However, current climate models struggle to accurately simulate this warming phenomenon, posing challenges to fully understand and validate this distinct climate response amidst the general trend of volcano-induced global cooling. Here we show that, the persistent volcanic cloud from summer to late autumn and the associated warming of the mid-latitude stratosphere plays a pivotal role in triggering NEWW. The role of winter aerosols is demonstrated by sensitivity simulations with updated volcanic forcing of the 1783 Icelandic Laki eruption, supported by two recently available temperature reconstructions, and reversely verified by model results of various eruptions without substantial cold season aerosol loadings. The abnormal mid-latitude stratospheric warming enhances the meridional temperature gradient, strengthens the polar vortex, alters both horizontal and vertical energy redistribution that contributed to NEWW. The findings help to reconcile the model-observation discrepancy of post-eruption winter climate responses, and point to the critical role of stratosphere-troposphere coupling in responding and redistributing the radiative perturbation.

How to cite: Yang, L., Gao, C., and Liu, F.: Winter Warming in Northern Eurasia Following the 1783 Laki Volcanic Eruption, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18827, https://doi.org/10.5194/egusphere-egu25-18827, 2025.

EGU25-18860 | ECS | Posters on site | AS3.16

Investigating the Climatic Impacts of Volcanic Eruptions over Eurasia and MENA Using the MIROC6 Coupled Climate Model 

Muhammad Mubashar Dogar, Shingo Watanabe, and Masatomo Fujiwara

Tropical volcanic eruptions are significant drivers of climate variability, inducing North Atlantic Oscillation (NAO)-like circulation changes that lead to high-latitude Eurasian winter warming and amplified cooling in the Middle East and North Africa (MENA). However, recent studies have raised concerns about the robustness of this post-eruption NAO-like response, suggesting that its regional impacts on Eurasia and MENA could be linked to coexisting El Niño-like variability rather than volcanic-induced NAO variability. To address this gap, this study utilizes the high-top MIROC6 coupled model to examine the roles of NAO and ENSO in shaping regional climate dynamics over MENA following tropical volcanic events. Our findings reveal that post-eruption winter responses are primarily driven by NAO, with El Niño-like conditions amplifying MENA cooling but not initiating it. In summer, volcanic aerosols weaken the Hadley circulation's updraft branch (i.e., ITCZ), leading to tropical warming and drying, with further amplification by ENSO interactions. These results validate MIROC6's effectiveness in simulating volcanic impacts and offer critical insights for interpreting climate models and informing post-eruption climate policies.

How to cite: Dogar, M. M., Watanabe, S., and Fujiwara, M.: Investigating the Climatic Impacts of Volcanic Eruptions over Eurasia and MENA Using the MIROC6 Coupled Climate Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18860, https://doi.org/10.5194/egusphere-egu25-18860, 2025.

EGU25-19434 | ECS | Posters on site | AS3.16

Climate Responses to Volcanic Eruption Clusters in the North Atlantic Under Different Boundary Conditions 

Deepashree Dutta, Peter Hopcroft, Francesco Muschitiello, Laurits Andreasen, Thomas Aubry, Xu Zhang, Claudia Timmreck, and Davide Zanchettin

Volcanic eruptions release aerosols into the stratosphere, which can trigger a wide range of climate responses across different temporal and spatial scales. However, the physical processes through which volcanic forcing leads to long-term global and regional cooling remain inadequately explored. Specifically, the climate responses following a series of intense volcanic eruptions before the Holocene remain insufficiently understood. The conditions during such past climates were vastly different from today’s, suggesting that potential amplifying feedbacks may also have differed. Using fully glacial, deglacial and pre-industrial boundary conditions, we conducted a suite of experiments with the Hadley Centre Coupled Model Version 3 and the Max Planck Institute's Earth System Model, forced with idealised volcanic eruption clusters, to investigate the long-term post-eruption sea surface temperature and sea ice responses in the North Atlantic. We find more intense and longer-lasting cooling in the subpolar North Atlantic in the fully glacial state compared to the other climate states. We explore the physical processes driving this cooling and how differences in the representation of upper-ocean conditions across the two climate models lead to model-dependent results.

How to cite: Dutta, D., Hopcroft, P., Muschitiello, F., Andreasen, L., Aubry, T., Zhang, X., Timmreck, C., and Zanchettin, D.: Climate Responses to Volcanic Eruption Clusters in the North Atlantic Under Different Boundary Conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19434, https://doi.org/10.5194/egusphere-egu25-19434, 2025.

EGU25-19899 | Posters on site | AS3.16

Diabatic Heating Rates and Mesoscale Vortices in Stratospheric Volcanic Plumes: Insights from the 2022 Hunga and 2019 Raikoke plumes 

Aurélien Podglajen, Duc Dung Tran, Pasquale Sellitto, Clair Duchamp, Bernard Legras, William Randel, and Jon Starr

Following the eruptions of Raikoke in 2019 and Hunga in 2022, it was recently discovered that stratospheric volcanic plumes may feature specific mesoscale dynamics. First, they undergo important vertical motions, a descent for the Hunga plume [e.g., 1,2], a self-lofting for the Raikoke plume [e.g., 3]. Second, they tend to self-organize into mesoscale anticyclonic circulations. This behavior dramatically affects the dispersion of the plumes and their climate impacts. While it is clear that they arise due to significant diabatic heating anomalies, a quantitative estimate of the radiative heating rates and their link with the vertical motions of the plumes is currently lacking .

In this study, we use offline radiative transfer calculations with a broad-band radiative transfer model to quantify the anomalous stratospheric heating rates resulting from a localized volcano-induced perturbation. The calculations are forced using particle optical properties and water vapor concentrations in the Hunga and Raikoke plumes observed from a suite of space-borne sensors including the spaceborne Lidar CALIOP. We explore the sensitivity of the heating rates to various plume properties, including altitude and composition. Their consequences on mesoscale organization are discussed in light of idealized mesoscale plume simulations [4].

 

References

[1] Sellitto, P., Podglajen, A., Belhadji, R. et al. The unexpected radiative impact of the Hunga Tonga eruption of 15th January 2022. Commun Earth Environ 3, 288 (2022). https://doi.org/10.1038/s43247-022-00618-z

[2] Legras, B., Duchamp, C., Sellitto, P., Podglajen, A., Carboni, E., Siddans, R., Grooß, J.-U., Khaykin, S., and Ploeger, F.: The evolution and dynamics of the Hunga Tonga–Hunga Ha'apai sulfate aerosol plume in the stratosphere, Atmos. Chem. Phys., 22, 14957–14970, https://doi.org/10.5194/acp-22-14957-2022, 2022.

[3] Khaykin, S.M., de Laat, A.T.J., Godin-Beekmann, S. et al. Unexpected self-lofting and dynamical confinement of volcanic plumes: the Raikoke 2019 case. Sci Rep 12, 22409 (2022). https://doi.org/10.1038/s41598-022-27021-0

[4] Podglajen, A., Legras, B., Lapeyre, G., Plougonven, R., Zeitlin, V., Brémaud, V., et al. (2024) Dynamics of diabatically forced anticyclonic plumes in the stratosphere. Quarterly Journal of the Royal Meteorological Society, 150(760), 15381565. https://doi.org/10.1002/qj.4658

How to cite: Podglajen, A., Tran, D. D., Sellitto, P., Duchamp, C., Legras, B., Randel, W., and Starr, J.: Diabatic Heating Rates and Mesoscale Vortices in Stratospheric Volcanic Plumes: Insights from the 2022 Hunga and 2019 Raikoke plumes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19899, https://doi.org/10.5194/egusphere-egu25-19899, 2025.

EGU25-19929 | ECS | Posters on site | AS3.16

 Impact of the April 2024 Ruang volcanic eruption on the Asian Tropopause Aerosol Layer: insights from Balloon measurements 

Hazel Vernier, Neeraj Rastogi, Nicolas Dumelie, Jean-Paul Vernier, Lilian Joly, Gwenael Berthet, and Rohit Meena

Stratospheric aerosols play a crucial role in Earth's radiative balance and atmospheric chemistry. Their sources and properties are influenced by various factors, including volcanic eruptions, biomass burning (PyroCbs), and the Asian Tropopause Aerosol Layer (ATAL). The ATAL, a prominent feature of the Asian Summer Monsoon (ASM), extends from the eastern Mediterranean across India to western China at altitudes of 13-18 km.

Recent volcanic eruptions have significantly impacted the stratosphere, with varying characteristics such as the magnitude and altitude of the eruption, the injected mass, and the resulting aerosol composition. These eruption characteristics, combined with the dynamics of the Asian Monsoon Anticyclone (AMA), and the pre-existing chemical state of the ATAL, contribute to complex and diverse aerosol properties within this region.

The Balloon measurement campaign of the ATAL (BATAL) project utilizes balloon-borne instruments to investigate the optical, physical, and chemical properties of the ATAL. Since its inception a decade ago, BATAL has employed optical particle counters, balloon-borne radiosondes, and aerosol collectors to characterize ATAL aerosols. These measurements are further complemented by satellite and ground-based lidar observations to enhance our understanding of aerosol sources and transport mechanisms. Understanding the different sources of stratospheric aerosols over Asia is critical to differentiate the impacts of anthropogenic and natural aerosols on the climate and monsoon hydrological cycle. 

In the summer of 2024, after a four-year hiatus due to the COVID-19 pandemic, the BATAL project resumed measurements in India. Our observations revealed a complex scenario where the UTLS was influenced by both the ATAL and the transport of aerosols from the Ruang volcanic eruption, which occurred in April 2024. By analyzing data from a suite of instruments, including balloon-borne optical particle counters, backscatter sondes, and aerosol samplers. This analysis will enable us to compare the characteristics of ATAL and volcanic aerosols and discuss the implications of these findings for understanding their combined impact on the atmosphere.

 

How to cite: Vernier, H., Rastogi, N., Dumelie, N., Vernier, J.-P., Joly, L., Berthet, G., and Meena, R.:  Impact of the April 2024 Ruang volcanic eruption on the Asian Tropopause Aerosol Layer: insights from Balloon measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19929, https://doi.org/10.5194/egusphere-egu25-19929, 2025.

"Radiative" or "rapid" adjustments refer to the climate system's responses to an instantaneous radiative forcing, which are independent of surface temperature changes. They occur on timescales from hours to months or even longer, making it difficult to distinguish them from feedbacks. Despite variations in definitions, understanding these processes is essential for advancing climate modeling.

Volcanic eruptions, which introduce scattering aerosol to the stratosphere, serve as natural experiments for studying short-term adjustments. However, the gradual global spread of aerosols during a volcanic eruption complicates analysis. To address this, we took a stepwise approach, starting with idealized model simulations, gradually increasing complexity and finally comparing model results with satellite measurements of the Mt. Pinatubo eruption in 1991. We analyzed data of the abrupt-solm4p experiment from the Cloud Feedback Model Intercomparison Project (CFMIP) within the 6th Coupled Model Intercomparison Project (CMIP6). This experiment simulates a 4% reduction in the solar constant. Additionally, we analyzed an MPI-ESM 1.2 model experiment with both absorbing and non-absorbing stratospheric aerosol layers, using fixed and fully coupled sea surface temperatures. Moreover, results from the volc-pinatubo-full experiment of the CMIP6 Volcanic MIP (VolMIP) were considered, simulating a Pinatubo like eruption, but initializing it from different years of the control run to account for climate variability. Finally, model results were compared to ERA5 reanalysis data of the Pinatubo eruption in 1991.

This study focused on changes in climate variables, cloud properties, and radiative fluxes during the first year after the onset of forcing. All model experiments were initialized on January 1st as the start of forcing, while ERA5 data was used from January 1st, 1992, onwards, since volcanic forcing from the Mt. Pinatubo eruption was strongest at that point.

Results show rapid cooling in the troposphere, especially over Antarctica and the Southern Hemisphere. In contrast, the stratosphere warms significantly when absorbing aerosol is present in the stratopshere. These temperature changes affect the jet streams, as well as the polar night jet, leading to a disruption of the polar vortex and consequently increased surface temperature in the Arctic. Within the first month, the troposphere cools faster than the ocean surface, reducing vertical stability and increasing relative humidity over the ocean. Conversely, over land in the tropics, the opposite effect occurs, influencing land-sea circulation.

How to cite: Lange, C. and Quaas, J.: Rapid adjustments after volcanic eruptions - A stepwise approach towards a better understanding of short-term adjustments in climate models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20169, https://doi.org/10.5194/egusphere-egu25-20169, 2025.

EGU25-20238 | ECS | Orals | AS3.16

Sulfur isotopes and tephra geochemistry in identifying the volcanic sources of mystery, climate forcing eruptions preserved in ice cores 

Helen Innes, William Hutchison, Celeste Smith, Patrick Sugden, and Andrea Burke

Ice cores provide the best record of volcanic sulfate aerosol emissions in the pre-satellite era, which are used in model simulations to understand the past and future climate hazards of volcanic stratospheric injection. However, the vast majority of ice core recorded events used in climate models are not attributed to known eruptive sources. Therefore, it is necessary to make assumptions of source latitude, plume height, and stratospheric sulfur loading – all variables which impact the climate forcing of an eruption. This is even the case for relatively recent eruptions recorded in ice during the post-industrial era, where cold conditions were experienced by global societies, but no historical records of the culprit eruptions exist.

Using a multi-pronged approach that combines high time resolution sulfur isotope analysis of deposited aerosols and geochemical analysis of microscopic ash particles in polar ice cores, these eruption characteristics can be better constrained. We demonstrate how this multi-method approach has recently aided the investigations into several volcanic eruptions recorded in polar ice cores which are associated with periods of notable climate cooling in the Common Era, including the mysterious 1831 CE eruption. These efforts will improve the volcanic forcing used in model simulations of the climate over the last 2000 years.

How to cite: Innes, H., Hutchison, W., Smith, C., Sugden, P., and Burke, A.: Sulfur isotopes and tephra geochemistry in identifying the volcanic sources of mystery, climate forcing eruptions preserved in ice cores, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20238, https://doi.org/10.5194/egusphere-egu25-20238, 2025.

EGU25-20342 | Posters on site | AS3.16

Nonlinear precipitation and temperature response to large low-latitude eruptions spanning the last two millennia 

Dana Raiter, Zachary McGraw, and Lorenzo Polvani

We ask whether the temperature and precipitation response to large, low-latitude volcanic eruptions is a linear function of the eruption magnitude, as measured by the mass (in Teragrams) of sulfur injected in the lower stratosphere (TgS).  Consider the last 2,000 years, magnitudes of climatically interesting eruptions range from roughly 10 TgS from the 1991 Pinatubo and the 1883 Krakatau eruptions, to nearly 30 TgS for the 1815 eruption, to almost 60 TgS for the largest event, the 1257 Samalas eruption.  To span this entire range, we simulate eruptions of 5, 10, 20, 40, 80 and 160 TgS, using a state-of-the art climate model with a well-resolved stratosphere.  For each eruption magnitude we run a 20-member ensemble of 10-year-long simulations.

We confirm earlier studies, and find that the response is linear up to 20 TgS.  However, for eruptions of 40 TgS and above, our analysis reveals a clear nonlinear relationship between eruption magnitude and climate response.  We also find important differences between the responses in temperature and precipitation: while the temperature response saturates after 40 TgS, the precipitation response continues to increase in magnitude albeit at a reduced rate.  Furthermore, we find that the controlling mechanisms driving the precipitation response are different for the weakest and strongest events.  For small eruptions the precipitation anomalies are primarily driven by the cooling surface temperatures (slow response), while for the largest eruptions they are dominated by the absorption of longwave radiation by the volcanic aerosols which warms the lower stratosphere (fast response).

How to cite: Raiter, D., McGraw, Z., and Polvani, L.: Nonlinear precipitation and temperature response to large low-latitude eruptions spanning the last two millennia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20342, https://doi.org/10.5194/egusphere-egu25-20342, 2025.

EGU25-21360 | Posters on site | AS3.16

Exploring stratospheric aerosol radiative forcing using the SASKTRAN radiative transfer framework 

Matthew Toohey, Taran Warnock, Daniel Zawada, and Adam Bourassa

The radiative forcing associated with stratospheric aerosol is often diagnosed using coupled general circulation models. The radiation codes within such models are state-of-the-art, but contain simplifications in order to optimize computational efficiency and make it feasible to perform simulations on climate-relevant time scales. Calculating radiative forcing using different radiative transfer techniques is useful to validate results from GCMs, and explore sensitivities to parameters that are not easily modified in such models. Here, we report on progress toward quantifying global stratospheric aerosol radiative forcing using the SASKTRAN radiative transfer framework, which has a rich heritage in the context of the retrieval of aerosol and gas species from limb scattered radiation. SASKTRAN is coupled to the Easy Volcanic Aerosol (EVA) forcing generator, allowing for realistic but adjustable stratospheric aerosol properties in global or single column radiative transfer calculations. Simulations are used to assess the impact of multiple scattering on the global radiative forcing, and its dependence on location and aerosol perturbation magnitude. We also assess the impact of using the simplified scattering parameters used as input to most GCMs (extinction, single scattering albedo and asymmetry factor) compared to using the full Mie scattering phase function computed from a given aerosol size distribution.

How to cite: Toohey, M., Warnock, T., Zawada, D., and Bourassa, A.: Exploring stratospheric aerosol radiative forcing using the SASKTRAN radiative transfer framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21360, https://doi.org/10.5194/egusphere-egu25-21360, 2025.

EGU25-59 | ECS | Orals | AS3.17

Variability and long-term changes in tropical cold-point temperature 

Mona Zolghadrshojaee, Susann Tegtmeier, Sean M. Davis, Robin Pilch Kedzierski, and Leopold Haimberger

The tropical tropopause layer (TTL) serves as a crucial boundary for air exchange between the troposphere and stratosphere, influencing the chemical composition and radiative balance of the lower stratosphere. Specifically, the cold-point tropopause, where air parcels undergo final dehydration, plays a key role in determining stratospheric water vapor content, which has significant implications for the global energy budget.

Our research utilizes Global Navigation Satellite System – Radio Occultation (GNSS-RO) and radiosonde data to investigate long-term changes in cold-point temperature and their impact on water vapor trends. We present evidence of a shift from pre-2000 cooling to post-2000 warming in TTL and lower stratospheric temperatures. Between 2002 and 2023, the cold point exhibits significant warming trends, reaching up to 0.7 K per decade during boreal winter and spring, with pronounced longitudinal asymmetries. These trends are strongest over the Atlantic and weakest over the central Pacific and are anti-correlated with upper tropospheric temperature trends. Our analysis shows a decrease in the seasonal cycle of cold-point temperature by ∼7%, driving a corresponding reduction of 6% in the seasonal cycle of water vapor at 100 hPa. This decrease of the water vapor seasonal cycle is transported upwards weakening the amplitude of the well-known stratospheric tape recorder signal.

Our findings are reproduced by reanalysis data (ERA5, JRA-55, MERRA-2), which accurately capture the spatial and seasonal variations in temperature trends. The reanalyses also highlight an important connection between TTL temperatures and tropical upwelling with a pre-2000 increase in tropical upwelling consistent with observed cold-point cooling and a post-2000 decrease in upwelling consistent with observed cold-point warming.

How to cite: Zolghadrshojaee, M., Tegtmeier, S., M. Davis, S., Pilch Kedzierski, R., and Haimberger, L.: Variability and long-term changes in tropical cold-point temperature, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-59, https://doi.org/10.5194/egusphere-egu25-59, 2025.

EGU25-474 | ECS | Posters on site | AS3.17

Stratosphere to troposphere transport of ozone over South America during the SouthTRAC campaign 

Charlie Opazo, Rodrigo Seguel, Laura Gallardo, Roberto Rondanelli, Björn-Martin Sinnhuber, Florian Obersteiner, Jörn Ungermann, and Peter Hoor

Stratosphere-troposphere exchange (STE) plays a key role in the tropospheric ozone budget. In extratropical latitudes, ozone transport from the stratosphere occurs mainly through the development of cut-off lows and tropopause folds. However, chemical measurements in the free troposphere and between the upper troposphere and lower stratosphere (UTLS) are remarkably sparse in the southern hemisphere compared with the northern hemisphere. In this context, the Southern Hemisphere Transport, Dynamics, and Chemistry (SouthTRAC) campaign was conducted between September and November 2019. One of its key objectives was to investigate dynamical and chemical processes in the UTLS over South America, using the High Altitude and LOng Range (HALO) research aircraft for in situ and remote measurements. This study analyzes the impact of a cut-off low (7-13 September 2019) on free tropospheric ozone, which extended from subpolar to subtropical latitudes using ozone (O3), water vapor (H2O), methane (CH4), carbon monoxide (CO) and nitric acid (HNO3) measured by HALO instrumentation. These measurements were complemented with ozonesondes launched from Ushuaia, Argentina (54.8°S, 68.3°W) and Marambio, Antarctica (64.2°S, 56.6°W) and included surface ozone measured at Cerro Tololo, Chile (30.2°S, 70.8°W) at 2200 m above sea level.

The observations revealed complex ozone structures during the evolution of the cut-off low between 65°S-30°S. The 9 September flight recorded O3 mixing ratios up to 100 nmol mol-1 above 8 km altitude over Río Grande, Argentina (53.78°S, 67.75°W). In contrast, the sonde in Ushuaia recorded 30 nmol mol-1 above 10 km. The difference observed between these sites was due to the formation of a tropopause fold, which transported O3-rich air into lower levels. The increases in O3 measured in the free troposphere were accompanied by consistent increases in HNO3 (a stratospheric tracer) and decreases in CO and H2O (tropospheric tracers). In addition, on 12 September, O3 levels at Cerro Tololo, where the diurnal O₃ cycle is nearly absent, experienced a sharp increase of approximately 13 nmol mol-1, sustained for nearly 24 hours. This O3 increase was accompanied by low relative humidity (<20%). Furthermore, we used trajectory analysis to link these changes in O3 with this stratospheric intrusion. Overall, this study highlights the linkage between subpolar and subtropical latitudes, emphasizing the importance of STE processes in southern hemisphere atmospheric chemistry and the need for more highly resolved chemical profiles in the region.

How to cite: Opazo, C., Seguel, R., Gallardo, L., Rondanelli, R., Sinnhuber, B.-M., Obersteiner, F., Ungermann, J., and Hoor, P.: Stratosphere to troposphere transport of ozone over South America during the SouthTRAC campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-474, https://doi.org/10.5194/egusphere-egu25-474, 2025.

EGU25-610 | ECS | Posters on site | AS3.17

Comparing simulated polar stratospheric clouds in the UKESM with CALIOP satellite data  

Isabelle Sangha, Andrew Orr, Luke Abraham, Hua Lu, Michael Pitts, Lamont Poole, and Michael Weimer

Polar stratospheric clouds (PSCs) play a fundamental role in depleting stratospheric ozone. Heterogeneous reactions on their surfaces increase the concentration of active chlorine, which can catalytically destroy ozone and prolong ozone depletion by denitrifying and dehydrating the stratosphere. However, parametrisations of PSC formation is poorly included in global chemistry-climate models due to the complexity of the microphysical processes involved in PSC particle formation. This limits our ability to project the future recovery of the stratospheric ozone and the resulting climate impacts.

In this work, the representation of PSCs in the UK Earth System Model (UKESM) has been improved by refining the particle formation schemes to 1) kinetically determine the growth of nitric acid trihydrate particles rather than using a thermodynamic assumption, and 2) include the growth of supercooled ternary solution particles through the uptake of nitric acid rather than using a sulphate aerosol climatology. To validate these changes, the simulated PSCs are converted into optical properties and evaluated against satellite data. Here, a comparison of the results from the new PSC scheme in the UKESM with the observations from the satellite-borne Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) is presented. Whether the changes to the formation parameterisation improve the model’s ability to accurately simulate PSCs both temporally and spatially in the Northern and Southern hemisphere is assessed and the effect on stratospheric denitrification in the model is examined.

How to cite: Sangha, I., Orr, A., Abraham, L., Lu, H., Pitts, M., Poole, L., and Weimer, M.: Comparing simulated polar stratospheric clouds in the UKESM with CALIOP satellite data , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-610, https://doi.org/10.5194/egusphere-egu25-610, 2025.

EGU25-1407 | ECS | Posters on site | AS3.17

Impact of the 1994–1997 Temporary Decrease in Northern Hemisphere Stratospheric Methane on the 1990s Methane Trend 

Yuanyuan Han, Shentao Li, Xinlong Tan, Wenyan Guo, Wuhu Feng, Xin Li, Feiyang Wang, and Fei Xie

Methane (CH4) ranks as the second most significant anthropogenic greenhouse gas following carbon dioxide (CO2). It originates from a wide range of surface sources and subsequently enters the stratosphere through the tropical tropopause. In line with the observed positive trend in tropospheric CH4, stratospheric CH4 has shown an overall increase in the long-term trend. However, contrary to the continuous increase in tropospheric CH4, stratospheric CH4 exhibits a temporal decrease in the Northern Hemisphere middle to upper stratosphere during short-time periods. This study investigates the causes behind the decreasing trend of stratospheric CH4 in the Northern Hemisphere from 1991 to 2000. We find that the extreme decrease of stratospheric CH4 from July 1994 to May 1997 contributes to the overall decreasing trend of CH4 from 1991 to 2000. This extreme decrease is attributed to the weakened meridional component of the residual circulation. The weakened meridional component attenuates the transport of CH4-rich air from the low-latitude lower stratosphere to the mid-latitude middle and upper stratosphere, leading to the observed decrease in CH4. It is further found that the smallest SST gradient in the North Pacific and adjacent regions is identified as a significant factor contributing to the weakened residual circulation and the decrease in CH4. Simulations by a chemistry-climate model support the results.

How to cite: Han, Y., Li, S., Tan, X., Guo, W., Feng, W., Li, X., Wang, F., and Xie, F.: Impact of the 1994–1997 Temporary Decrease in Northern Hemisphere Stratospheric Methane on the 1990s Methane Trend, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1407, https://doi.org/10.5194/egusphere-egu25-1407, 2025.

EGU25-1676 | ECS | Posters on site | AS3.17

Mechanistic evaluation of reanalysis composition and circulation in the Asian monsoon tropopause layer 

Shenglong Zhang and Jonathon S. Wright

Changes in stratospheric water vapor and other constituents have important radiative and chemical impacts on climate. Here, we use Aura Microwave Limb Sounder (MLS) satellite observations and five meteorological and composition-focused reanalyses to examine covariations of water vapor, ozone, and carbon monoxide (CO) within the dynamical and thermodynamic environment of the tropopause layer (147–68 hPa) above the Asian summer monsoon (ASM). All reanalyses capture the thermal environment near the tropopause well and largely capture the climatological distributions and seasonal cycles of water vapor, along with the seasonal ‘ozone valley’ and convective enhancement of CO above the monsoon. The primary balance is between advective hydration and cold trap dehydration near the cold point; however, data assimilation effects are of the same order as the leading balance and therefore cannot be neglected. Applying principal component analysis to both vertical and horizontal variations of water vapor, we identify three leading modes of deseasonalized variability. The first mode, which consists of regional-scale moist or dry anomalies on the interannual scale, is decomposed into a linear trend over 2005–2021 and detrended interannual variability. The spatial pattern and sign of the linear trend in tropopause-layer water vapor over this period differ between Aura MLS and the reanalyses despite a consistent increasing trend. Signatures of interannual variability are otherwise largely consistent, except for ozone in the Japanese Reanalysis for Three-Quarters of a Century (JRA-3Q), which assimilates only total column ozone. Detrended interannual variability in water vapor can be attributed mainly to the pre-monsoon influence of the quasi-biennial oscillation. The second mode features dry or moist anomalies centered in the northeastern and southwestern quadrants of the anticyclone coupled with weaker opposing anomalies in the southeast, while the third mode features a horizontal dipole oriented east-to-west. The second and third modes vary on subseasonal scales and often occur in quadrature, representing the propagation of quasi-biweekly waves across the monsoon domain. The overall consistency between Aura MLS and reanalysis-derived modes of variability in UTLS water vapor in this region is a promising sign that atmospheric reanalyses are increasingly able to capture the processes controlling water vapor near the tropopause.

How to cite: Zhang, S. and Wright, J. S.: Mechanistic evaluation of reanalysis composition and circulation in the Asian monsoon tropopause layer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1676, https://doi.org/10.5194/egusphere-egu25-1676, 2025.

EGU25-2047 | Posters on site | AS3.17

Significant Response of Methane in the Upper Troposphere to Subseasonal Variability of the Asian Monsoon Anticyclone 

Mengchu Tao, Sihong Zhu, Zhaonan Cai, Yi Liu, Liang Feng, Sangmu Pubu, Zhongshui Yu, and Junji Cao

Substantial methane (CH4) emissions in Asia are efficiently transported to the upper troposphere through the monsoon dynamical system, which forms a remarkable seasonal CH4 enhancement in the upper troposphere. Using a chemical transport model GEOS-Chem driven by surface optimized CH4 flux, the CH4 enhancement over the Asian monsoon region is explored as a combined effect of the monsoon dynamical system and regionally increased emissions during late monsoon season. The spatial distributions of CH4 at the upper troposphere show strong subseasonal variability, which is closely tied to the east-west oscillation of Asian monsoon anticyclone (AMA). Besides, the AMA patterns influence the vertical structure of methane. The AMA center around 80°E favors the upward transport from north India and Bangladesh while the AMA center around 105°E favors the source from southwest China transported to the upper troposphere. The AMA center over the Iranian Plateau suppresses the vertical transport and favors the horizontal redistribution. According to our model sensitivity study, the differences in the upper tropospheric CH4 anomalies caused by large-scale circulation is 1-2 times of that caused by regional surface emissions. Our research highlights the complex interaction between monsoon dynamics and surface emissions to determine the upper tropospheric methane.

How to cite: Tao, M., Zhu, S., Cai, Z., Liu, Y., Feng, L., Pubu, S., Yu, Z., and Cao, J.: Significant Response of Methane in the Upper Troposphere to Subseasonal Variability of the Asian Monsoon Anticyclone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2047, https://doi.org/10.5194/egusphere-egu25-2047, 2025.

EGU25-2225 | ECS | Orals | AS3.17

Changes in the convective transport into the upper troposphere due to climate change 

Adrienne Jeske and Holger Tost

The atmospheric temperature and moisture profiles have changed given the rapid increases in the sea surface temperature in the past decades. This has implications for the stability of the atmosphere and therefore for the frequency, intensity and other characteristics of atmospheric moist convection and convective transport of water vapour and trace species. The latter is of high relevance to the composition of the upper troposphere and lower stratosphere.
We performed a historical simulation with the global chemistry climate model EMAC (ECHAM/MESSy Atmospheric Chemistry) from 1979 to 2020 and investigated the changes in convective properties and transport. Within EMAC, the convective exchange matrix is applied to quantify and track the convective transport. This tool connects the transport of air masses between all model levels due to convection and enables the analysis of convective transport features and their changes disentangled from other processes.
Deep convection is reaching higher in the decade from 2011 to 2020 in comparison to 1980 to 1989. This is strongly correlated with an increase in the tropopause height. Thereby, the convective mass fluxes increased in the upper troposphere, but the overall strength of the convection did not change. Deep convection occurs less frequently in the more recent period. This leads in total to a decrease in the transport from the boundary air to the upper troposphere on average from 2011 to 2020 compared to the reference period at the beginning of the simulation time. We will present these trends and their dependence on the choice of the convection parameterisation and the nudging of the meteorological conditions.

How to cite: Jeske, A. and Tost, H.: Changes in the convective transport into the upper troposphere due to climate change, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2225, https://doi.org/10.5194/egusphere-egu25-2225, 2025.

EGU25-2797 | ECS | Orals | AS3.17

Evaluating the impact of tropopause definitions on long-lived tracer distributions in the exUTLS 

Sophie Bauchinger, Tanja Schuck, Andreas Zahn, Harald Bönisch, Hans-Christoph Lachnitt, and Andreas Engel

Aircraft measurement campaigns such as IAGOS-CARIBIC and HALO missions are invaluable sources of long-lived trace gas observations in the extratropical Upper Troposphere and Lower Stratosphere (exUTLS). The simultaneous measurement of multiple substances enables a comprehensive characterisation of sampled air masses.

To contextualize these observations, the use of dynamic coordinate systems - where measurements are for example presented relative to the tropopause - is highly beneficial. The tropopause itself can be defined from several perspectives, including differences in chemical composition, dynamical parameters, or temperature gradients between the troposphere and stratosphere.

In this study, we examine how different tropopause definitions influence the climatology of long-lived tracer substance observations. We investigate how effective filtering of tropospheric and stratospheric air masses can homogenise measurements of long-lived tracers and therefore decouple atmospheric dynamics from long-term trends and seasonalities. Meteorological parameters used in this analysis are obtained from ERA5 reanalysis data sets, which have been subsampled along the flight tracks.

Our findings indicate that the thermal tropopause results in larger variability in bins around the tropopause. Different potential-vorticity thresholds result in vertically displaced distributions but similar trends around the tropopause. Chemical tropopauses, while effective in differentiating between the troposphere and stratosphere, show significant limitations in their sensitivity towards the surface.

How to cite: Bauchinger, S., Schuck, T., Zahn, A., Bönisch, H., Lachnitt, H.-C., and Engel, A.: Evaluating the impact of tropopause definitions on long-lived tracer distributions in the exUTLS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2797, https://doi.org/10.5194/egusphere-egu25-2797, 2025.

EGU25-3216 | ECS | Orals | AS3.17

Interannual variability of the Asian Summer Monsoon Anticyclone 

Oleh Kachula, Bärbel Vogel, and Gebhard Günther

Definition of the boundaries of the Asian summer monsoon anticyclone (ASMA) is a known challenge that highly impacts the information about the anticyclone's behavior and affects the study of its interannual variability. We present a novel method based on the absolute vortex moments that defines the ASMA boundaries by solving an optimization problem. The results show climatology (1980–2023), interannual variability, start and end dates range and the duration of the anticyclone peak phase calculated with help of the defined method. In addition, three individual years – 2017, 2022 and 2023 are highlighted during which StratoClim, ACCLIP and PHILEAS campaigns took place respectively. The interannual analysis is based on the anticyclone's centroid latitude and longitude, excess kurtosis, angle, aspect ratio and using 4 isentropic surfaces: 350, 370, 390 and 410K. The work determined correlation of the centroid position of the anticyclone with a set of month lag ENSO considering the whole year equatorial pacific sea surface temperature anomalies (DJF–NDJ) using ONI index. The ASMA centroid latitude is negatively correlated with 5-month lag ENSO ( ∼ -0.6) when the anticyclone is still in its formation phase and then the correlation starts to decline when the anticyclone enters its peak phase.

How to cite: Kachula, O., Vogel, B., and Günther, G.: Interannual variability of the Asian Summer Monsoon Anticyclone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3216, https://doi.org/10.5194/egusphere-egu25-3216, 2025.

EGU25-3680 | ECS | Orals | AS3.17

Understanding Boreal Summer UTLS Water Vapor Variations in Monsoon Regions: A Lagrangian Perspective 

Hongyue Wang, Mijeong Park, Mengchu Tao, Cristina Peña-Ortiz, Nuria Pilar Plaza, Felix Ploeger, and Paul Konopka

Water vapor in the Upper Troposphere and Lower Stratosphere (UTLS) plays a crucial role in climate feedback by influencing radiation, chemistry, and atmospheric dynamics. The amount of water vapor entering the stratosphere is sensitive to cold point temperatures (CPT), making Northern Hemisphere summer monsoons more favorable for transporting water vapor into the stratosphere. This study uses a Lagrangian method to reconstruct water vapor over the Asian (ASM) and North American (NAM) monsoons, investigating their contributions to stratospheric water vapor. The Lagrangian method tracks air parcels and identifies the coldest temperature along each trajectory, contrasting with local methods that rely on vertical temperature profiles. The reconstructed water vapor fields are validated against satellite observations from SAGE III/ISS and NASA’s Aura MLS. SAGE III/ISS shows stronger moisture enhancements than MLS, but both datasets reveal similar water vapor anomalies within the ASM and NAM anticyclones. Although the Lagrangian method is dry-biased compared to observations, it effectively reconstructs UTLS water vapor (correlation coefficient ~0.75), capturing moist anomalies in the ASM but performing less well in the NAM. Our analysis shows that, rather than local conditions, large-scale cold point tropopause temperatures in the vicinity of the monsoons primarily drive the moisture anomalies, with NAM water vapor significantly influenced by long-range transport from South Asia. Some convection-related processes, such as east-west shifts within the ASM, are not fully captured due to unresolved temperature variability in ERA5 and missing ice microphysics. Despite biases and computational challenges, the Lagrangian method provides valuable insights into UTLS water vapor transport.

How to cite: Wang, H., Park, M., Tao, M., Peña-Ortiz, C., Pilar Plaza, N., Ploeger, F., and Konopka, P.: Understanding Boreal Summer UTLS Water Vapor Variations in Monsoon Regions: A Lagrangian Perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3680, https://doi.org/10.5194/egusphere-egu25-3680, 2025.

The Asian summer monsoon (ASM) is one of the most important events of the northern winter hemisphere. It represents an effective pathway of tropospheric air originating from the south-Asian continent into the upper troposphere (UT), which is to date only partially understood and quantified.

Through Rossby wave breaking events large filaments of ASM air are transported westward into the mid-latitudes, where they are mixed into the lower stratosphere (LS). The composition of the UTLS, especially with respect to radiatively active trace gas species, is a key factor for the global climate, which the ASM affects directly.

During the PHILEAS (Probing High Latitude Export of Air from the Asian Summer Monsoon) campaign in later summer 2023 a filament of ASM outflow was measured with the airborne limb imager GLORIA on board the German research aircraft HALO on two consecutive days. The edge of the filament was imaged in 3-D during the first flight and its outflow based on CLaMS trajectory calculations was revisited inside a second 3-D retrieval on the following day. The chemical composition of the filamented air was measured in the five different trace gas species water vapor, ozone, peroxyacetyl nitrate (PAN), nitric acid and carbon tetrachloride with unprecedented 3-D spatial resolution unique to the GLORIA instrument. The filament contains a strong tropopause fold, which perturbs its dynamical structure.

We present the tomographic retrievals of the matching flights. We are able to identify the different types of air from their chemical composition using a novel classification method based on mixture models, and are able to resolve the spatial structure of both the filament and the mixing process on the mesoscale. By revisiting the outflow of the filament we are able to directly measure the change in chemical composition and are able to determine and quantify the different possible pathways during mixing. We are able to uniquely link the different types of air to different regions of origin.

GLORIA is an airborne demonstrator for the European Space Agency Earth Explorer 11 candidate CAIRT, currently selected for Phase A. GLORIA observations offer an outlook on how exploring global processes in the UTLS would be possible using CAIRT.

How to cite: Kaumanns, J. and the GLORIA Team: Analysing mixing processes in tomographically imaged filaments of Asian Monsoon outflow during the PHILEAS campaign using computer vision, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4335, https://doi.org/10.5194/egusphere-egu25-4335, 2025.

EGU25-4817 | ECS | Orals | AS3.17

Stratosphere-Troposphere Exchange during a Typhoon event: A Lagrangian approach. 

Massimo Martina, Anahí Villalba Pradas, and Petr Šácha

The characterization of the stratosphere-troposphere exchange (STE) is fundamental to its role in the global atmospheric budget of chemical constituents. The troposphere-to-stratosphere transport can inject anthropogenic pollutants from the Earth’s surface into the stratosphere, changing its chemical composition and influencing the radiative processes. For instance, the Asian Tropopause Aerosol Layer, with a main known pathway via the Asian summer monsoon, has been shown to have a radiative cooling effect on the surface. Here we propose a previously underreported potential pathway contributing to STE via tropical cyclones, typhoons in particular. We focus on one episode of a typhoon crossing over the Philippines, which is located in the highly polluted Eastern Asia-Western Pacific region.  A case study for typhoon Molave (2020), combining a Lagrangian modeling tool with the Weather Research and Forecasting model (FLEXPART-WRF), demonstrates that the typhoon can result in rapid transport of pollutants from the surface to the upper troposphere-lower stratosphere (UTLS) region, inducing strong STE. Using a Lagrangian model, it has been possible to characterize the intensity of the air intrusion from the boundary layer to the free troposphere and stratosphere by computing their residence times. Furthermore, we try to disentangle the role of convection, orographic lifting, and gravity waves inducing this type of rapid transport. Overall, our study indicates that typhoon episodes can play an important, intermittent and previously insufficiently considered role in STE, influencing emerging topics of the highest importance such as the long-range dispersion of microplastics.

How to cite: Martina, M., Villalba Pradas, A., and Šácha, P.: Stratosphere-Troposphere Exchange during a Typhoon event: A Lagrangian approach., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4817, https://doi.org/10.5194/egusphere-egu25-4817, 2025.

EGU25-6027 | ECS | Posters on site | AS3.17

Vertical Variability of Relative Humidity and Its Relation to Cirrus Clouds in the Extratropical UTLS 

Yun Li, Susanne Rohs, Armin Afchine, Nicole Spelten, Christian Rolf, Nicolas Emig, Heiko Bozem, Peter Hoor, Dieter Schell, and Andreas Petzold

Small changes in the equilibrium between water vapor and cirrus clouds in the upper troposphere and lower stratosphere (UTLS) can strongly influence atmospheric radiative forcing. Relative humidity with respect to ice (RHice) is a key parameter governing the formation and life cycle of cirrus clouds.

We present RHice measurements in the UTLS over the North Sea and Germany during the TPEx Learjet campaign (7–20 June 2024), conducted from Hohn, Germany, as part of the TPChange research program. Two IAGOS capacitive hygrometers (ICHs) were deployed: one mounted on the Learjet fuselage and the other on an AIRTOSS (AIRcraft Towed Sensor Shuttle) trailing approximately 70–180 m below the aircraft. This setup enabled the resolution of fine vertical structures of RHice that cannot be captured by weather and climate models.

By combining ICH RHice measurements with ECMWF ERA5 cloud ice water content along flight paths, we distinguish between cirrus and non-cirrus conditions, corroborated by the NIXE cloud probe onboard. Additionally, we examine the fine vertical structure of RHice across the extratropical tropopause and its relationship with cirrus clouds. These findings enhance our understanding of cirrus cloud occurrence and variability in this sensitive region, providing valuable insights for improving their representation in climate models.

How to cite: Li, Y., Rohs, S., Afchine, A., Spelten, N., Rolf, C., Emig, N., Bozem, H., Hoor, P., Schell, D., and Petzold, A.: Vertical Variability of Relative Humidity and Its Relation to Cirrus Clouds in the Extratropical UTLS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6027, https://doi.org/10.5194/egusphere-egu25-6027, 2025.

 Age of stratospheric air is a well established metric for the stratospheric transport circulation. Rooted in a robust theoretical framework, this approach offers the benefit of being deducible from observations of trace gases. Given potential climate-induced changes, observational constraints on stratospheric circulation are crucial. In the past two decades, scientific progress has been made in three main areas: (a) Enhanced process understanding and the development of process diagnostics led to better quantification of individual transport processes from observations and to a better understanding of model deficits. (b) The global age of air climatology is now well constrained by observations thanks to improved quality and quantity of data, including global satellite data, and through improved and consistent age calculation methods. (c) It is well established and understood that global models predict a decrease in age, that is, an accelerating stratospheric circulation, in response to forcing by greenhouse gases and ozone depleting substances. Observational records now confirm long-term forced trends in mean age in the lower stratosphere. However, in the mid-stratosphere, uncertainties in observational records are too large to confirm or disprove the model predictions. Continuous monitoring of stratospheric trace gases and further improved methods to derive age from those tracers will be crucial to better constrain variability and long-term trends from observations. Future work on mean age as a metric for stratospheric transport will be important due to its potential to enhance the understanding of stratospheric composition changes, address climate model biases, and assess the impacts of proposed climate geoengineering methods.

How to cite: Garny, H. and the Age of Air ISSI Team: A review on Age of Stratospheric Air: Progress on Processes, Observations, and Long-Term Trends, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6029, https://doi.org/10.5194/egusphere-egu25-6029, 2025.

EGU25-6351 | ECS | Orals | AS3.17

CH4 emission reductions and removal slow stratospheric O3 recovery and highlight importance of chlorine and N2O mitigation 

James Weber, Maisie Wright, Bill Collins, Keith Shine, Fiona O'Connor, Gerd Folberth, Paul Griffiths, and Sam Abernethy

Reducing methane emissions is critical for restricting global surface temperature increases. However, methane also influences stratospheric ozone, and its recovery, via chemical and radiative processes. Using the state-of-the-art methane emission-driven capability in the fully coupled United Kingdom Earth System Model (UKESM), we examine the impact of methane emission reductions and methane removal of varying magnitude and timing on stratospheric ozone recovery in the 21st Century under climate scenarios with high (SSP3-7.0) and low (SSP1-2.6) surface warming. Despite beneficial reductions to surface temperatures and surface ozone, reducing methane emissions slows, and in some cases even prevents, the recovery of total column ozone (TCO). This is driven by reduced ozone production in the troposphere and lower stratosphere and by increased destruction in the mid and upper stratosphere by compounds derived from nitrous oxide (N2O) and halocarbons. This suggests that for methane emission reductions to be universally beneficial, they must be accompanied by continued efforts to reduce emissions of N2O and halocarbons.         

 

How to cite: Weber, J., Wright, M., Collins, B., Shine, K., O'Connor, F., Folberth, G., Griffiths, P., and Abernethy, S.: CH4 emission reductions and removal slow stratospheric O3 recovery and highlight importance of chlorine and N2O mitigation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6351, https://doi.org/10.5194/egusphere-egu25-6351, 2025.

EGU25-6597 | Orals | AS3.17

A chemical mechanism explaining the observed wintertime HCl in the Antarctic vortex 

Jens-Uwe Grooß, Rolf Müller, John N. Crowley, and Michaela I Hegglin

It is well established that the drastic ozone loss in the Antarctic stratosphere, commonly known as the ozone hole, is caused by gas-phase and heterogeneous processes.  Chemistry models generally reproduce observed ozone depletion reasonable well.  However, models have been unable to reproduce observations of rapid HCl loss at the beginning of the polar winter.  Here we examine the impact of the heterogeneous reaction between Cl2O2 and HCl to form HOOCl and its subsequent photolysis on chlorine compounds. A chemical mechanism with these reactions added is able to clearly better reproduce the observed temporal development of the chlorine compounds HCl, ClONO2, ClO, and HOCl in the polar vortex lower stratosphere. The proposed chemical mechanism does moderately increase the chemical ozone column depletion, about 10\% in the lower stratospheric vortex core in September. Laboratory measurements of the proposed reactions are needed to confirm this mechanism.

How to cite: Grooß, J.-U., Müller, R., Crowley, J. N., and Hegglin, M. I.: A chemical mechanism explaining the observed wintertime HCl in the Antarctic vortex, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6597, https://doi.org/10.5194/egusphere-egu25-6597, 2025.

Recent increases in global anthropogenic ammonia emissions have yet to be fully quantified in terms of impacts on atmospheric particle formation, cloud microphysical properties, and climate. We employ the EMAC global climate-chemistry model, including recently published multi-component new particle formation (NPF) parameterisations from the CERN CLOUD experiment, to investigate the impact of anthropogenic ammonia on upper tropospheric processes. Our simulations show that convective transport significantly enhances ammonia-driven NPF and particle growth at these altitudes, leading to an average increase in particle number concentrations by up to 2000 cm⁻³ and a doubling of cloud condensation nuclei (CCN) concentrations over regions with high ammonia emissions. In simulations without anthropogenic ammonia, aerosol composition in the upper troposphere is dominated by sulphate and organic species rather than ammonium nitrate. Furthermore, anthropogenic ammonia emissions contribute to an increase in aerosol optical depth by up to 90%, producing a pronounced radiative forcing pattern: cooling in the Northern Hemisphere and warming in the Southern Hemisphere. These results underscore the critical role of ammonia emissions in aerosol composition in the upper troposphere and the global radiative forcing of climate.

How to cite: Xenofontos, C.: Anthropogenic Ammonia's Impact on Upper Tropospheric Aerosol Composition and Climate Forcing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6744, https://doi.org/10.5194/egusphere-egu25-6744, 2025.

EGU25-7145 | Orals | AS3.17

Multiscale Dynamical Processes Shaping a Mixing Line 

Andreas Dörnbrack, Peter Hoor, Paola Rodriguez Imazio, and Hans-Christoph Lachnitt

The paper discusses multiscale dynamical processes shaping a mixing line in the upper troposphere/lower stratosphere (UTLS). It focuses on aircraft observations above southern Scandinavia during a mountain wave event and how they can be analyzed based on dynamic variables and the trace gases N2O and CO. This study aims to identify the irreversible component of the stratosphere-troposphere exchange. It was shown that the overall shape of the mixing line is determined by the large-scale and mesoscale atmospheric conditions in the UTLS. Especially, the wide range of Θ values along the flight tracks causes a compact, almost linear tracer-tracer relation between N2O and CO. Only motion components with scales less than 4 km lead to the observed scattering along the mixing line. The anisotropic and patchy nature of the observed turbulence is responsible for this scatter in N2O and CO. The turbulence analysis reveals different scaling laws for the power spectra upstream, over the ridge and downstream of the mountains that lead to energy dissipation and irreversible mixing. The study suggests that turbulence dynamics may follow a cycle starting with 3D homogeneous isentropic turbulence upstream, transitioning to anisotropic turbulence over the ridge and further downstream. This transition is attributed to an interplay between turbulent eddies and internal gravity waves.

How to cite: Dörnbrack, A., Hoor, P., Rodriguez Imazio, P., and Lachnitt, H.-C.: Multiscale Dynamical Processes Shaping a Mixing Line, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7145, https://doi.org/10.5194/egusphere-egu25-7145, 2025.

EGU25-7476 | ECS | Posters on site | AS3.17

Retention During Freezing of Raindrops 

Martanda Gautam, Jackson Seymore, Moritz Hey, Alexander Theis, Karoline Diehl, Stephan Bormann, Subir K Mitra, and Miklós Szakáll

Understanding the interaction between freezing processes and the vertical movement of trace gases into the upper atmosphere during intense convection is essential for analyzing the distribution of aerosol precursors and their impact on the climate. We conducted experimental studies in a cold room with freely suspended raindrops (2 mm diameter) using an acoustic levitation setup. For the first time, we examined how freezing affects the retention of organic species, using silver iodide as the ice nucleating agent. Through quantitative chemical analysis, we calculated the retention coefficient, which represents the proportion of a chemical species that remains in the ice phase relative to its concentration prior to freezing. We measured the retention coefficients of nitric acid, formic acid, acetic acid, and 2-nitrophenol as individual compounds, as well as in binary and complex mixtures. Our findings indicate that physical properties have a greater influence on overall retention than chemical properties in the case of the larger raindrops we studied. Therefore, nearly all substances are completely retained during the freezing process in rain-sized drops, even those with low Henry’s law constants. An ice shell forms within 4.8 milliseconds after freezing begins, and this ice shell formation is the key factor preventing the expulsion of dissolved substances from the drop.

How to cite: Gautam, M., Seymore, J., Hey, M., Theis, A., Diehl, K., Bormann, S., Mitra, S. K., and Szakáll, M.: Retention During Freezing of Raindrops, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7476, https://doi.org/10.5194/egusphere-egu25-7476, 2025.

EGU25-7598 | Posters on site | AS3.17

The STRIVE Earth System Explorer Mission Concept 

Lyatt Jaeglé, Jun Wang, Luke Oman, and Matt DeLand and the STRIVE Science Team

We will present the Stratosphere Troposphere Response using Infrared Vertically-resolved light Explorer (STRIVE) mission concept, which was recently selected for a competitive Phase A Concept Study within NASA's 2023 Earth System Explorers Program. STRIVE fills a critical need for high vertical resolution profiles of temperature, ozone, trace gases, and aerosols in the upper troposphere and stratosphere with near-global horizontal sampling. The goal of STRIVE is to understand the processes controlling the composition and dynamics of the upper troposphere and stratosphere, thus constraining their critical influence on the predictability of weather, climate, the ozone layer, and air quality.

STRIVE will carry two synergistic instruments: a limb-scanning imaging Dyson spectrometer retrieving profiles of temperature, trace gas concentrations, aerosol extinction, and cloud properties during day and night; and a dual-spectral multi-directional limb profiling radiometer retrieving detailed aerosol properties during day. STRIVE will measure infrared radiation emitted and scattered from the atmospheric limb to provide profiles of temperature, O3, H2O, CH4, N2O, CFCs, CO, NO2, HNO3, ClONO2, N2O5, HCN, cloud top height, polar stratospheric clouds, and aerosol properties with fine vertical resolution (1 km) and unparalleled horizontal sampling (>400,000 profiles each day). STRIVE has the novel ability to resolve small-scale vertical structures of atmospheric composition and temperature, enabling new insights into the processes of troposphere-stratosphere interactions. STRIVE will provide unique observations necessary to inform and evaluate next-generation global Earth system models in the upper troposphere and stratosphere.

How to cite: Jaeglé, L., Wang, J., Oman, L., and DeLand, M. and the STRIVE Science Team: The STRIVE Earth System Explorer Mission Concept, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7598, https://doi.org/10.5194/egusphere-egu25-7598, 2025.

EGU25-7998 | ECS | Orals | AS3.17

Comparative Analysis of Transport Trace Gases in High-Resolution Simulations from ICON-ART and IFS Models 

Achraf Qor-el-aine, Stefan Versick, and Anna Agusti-Panareda

The CATRINE (Carbon Atmospheric Tracer Research to Improve Numerics and Evaluation) project, financed by the European Union, is a ground-breaking initiative aiming at improving the accuracy and dependability of atmospheric tracer transport models. The European Centre for Medium-Range Weather Forecasts (ECMWF) coordinates CATRINE, which brings together an interdisciplinary team of atmospheric scientists, climate researchers, and computational modelers to address significant challenges in emissions monitoring and carbon cycle knowledge. This investigation focuses on high-resolution global simulations of key atmospheric constituents—carbon dioxide (CO₂), methane (CH₄), and carbon monoxide (CO)—using two state-of-the-art numerical frameworks: the ICOsahedral Nonhydrostatic Atmospheric Model with aerosol and reactive trace gas capabilities (ICON-ART) and the Integrated Forecasting System (IFS) to advance our understanding of trace gas transport dynamics and improve numerical modelling techniques.

The study implements sophisticated modelling approaches within both frameworks, leveraging ICON-ART's innovative unstructured triangular grid system based on a spherical icosahedron, which facilitates flexible grid refinement and incorporates a height-based terrain-following coordinate system with smooth level vertical coordinate implementation. The ART module, coupled online with ICON, enables detailed simulation of aerosols and trace gases, encompassing their emissions, transport, and removal processes throughout the troposphere and stratosphere. In parallel, the investigation examines the IFS framework, renowned for its global numerical weather prediction capabilities, as well as atmospheric composition/air quality monitoring and prediction as part of the Copernicus Atmosphere Monitoring Service (CAMS).

The methodology employs high-resolution global simulations focused on trace gas transport processes, with particular emphasis on the upper troposphere/lower stratosphere (UTLS) region. The validation framework integrates observational data from the DCOTSS (Dynamics and Chemistry of the Summer Stratosphere) flight campaigns to evaluate model performance across various atmospheric phenomena. Also, the analysis examines deep convective overshooting event as characteristic cases where rapid vertical transport significantly modifies UTLS composition, altering mixing ratios of CO₂, CH₄, CO, and other trace species. Statistical analyses quantify model performance in representing these complex transport processes and their effects on atmospheric composition across multiple spatial and temporal scales.

The comparative analysis reveals distinct characteristics in how ICON-ART and IFS represent transport processes, particularly during deep convective events and associated overshooting phenomena. These findings contribute substantial methodological advances to atmospheric sciences, with direct implications for improving our understanding of UTLS dynamics, enhancing emissions monitoring capabilities, and supporting more accurate climate change assessments. The research establishes a comprehensive framework for future investigations of atmospheric transport processes, particularly in regions of complex dynamical interactions such as the UTLS region.

How to cite: Qor-el-aine, A., Versick, S., and Agusti-Panareda, A.: Comparative Analysis of Transport Trace Gases in High-Resolution Simulations from ICON-ART and IFS Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7998, https://doi.org/10.5194/egusphere-egu25-7998, 2025.

EGU25-8181 | ECS | Posters on site | AS3.17

Cirrus related diabatic processes and impact on ExTL structure 

Nicolas Emig, Armin Afchine, Heiko Bozem, Chun Hang Chau, Peter Hoor, Philipp Joppe, Daniel Kunkel, Hans-Christoph Lachnitt, Yun Li, Annette Miltenberger, and Johannes Schneider

The extratropical transition layer (ExTL), located above the extratropical tropopause, is an atmospheric region characterized by vertical gradients in atmospheric composition, transitioning between tropospheric and deeper stratospheric properties. Since the tropopause constitutes a mixing barrier under adiabatic conditions, the existence of the ExTL is evidence of diabatic processes influencing this atmospheric region.

Although not usually thought to occur above the tropopause, cirrus clouds can be the cause of diabatic processes via radiative and latent (microphysical) effects. Here we present two cases of cirrus occurrence above the extratropical tropopause captured during the AIRTOSS-ICE (2013) and TPEx (2024) campaigns. The observational data include simultaneous in situ measurements on two platforms in different altitudes, allowing for the calculation of vertical gradients of potential temperature (static stability) and other quantities. The measurements are supported by ERA5 reanalysis data as well as Lagrangian analyses of ICON (Icosahedral Nonhydrostatic) model simulations which yield contributions from different diabatic processes to the evolution of air masses.

The results of the AIRTOSS-ICE case suggest long residence times of the cirrus in stratospheric air as well as substantial differences in static stability between in- and outside the cirrus. The second case confirms the earlier observations and extends the simultaneous in situ measurements to ozone mixing ratios. Our findings underline the importance of diabatic cloud processes for the thermodynamic structure of the ExTL and potential cross tropopause exchange.

How to cite: Emig, N., Afchine, A., Bozem, H., Chau, C. H., Hoor, P., Joppe, P., Kunkel, D., Lachnitt, H.-C., Li, Y., Miltenberger, A., and Schneider, J.: Cirrus related diabatic processes and impact on ExTL structure, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8181, https://doi.org/10.5194/egusphere-egu25-8181, 2025.

EGU25-8337 | ECS | Posters on site | AS3.17

Understanding Convective Transport Through Transit and Turnover Timescales 

Chun-Wen Wang, Zhengzhao Johnny Luo, and Hui-Ming Hung

Deep convection plays a crucial role in atmospheric transport, yet the associated vertical transport characteristics and timescales remain insufficiently understood. This study investigates the transport dynamics of tropical deep convection by analyzing two key timescales: transit time, the average duration for chemical species to travel from the boundary layer to the upper troposphere, and turnover time, the average residence time of chemical species in the upper troposphere. The transit time considers the parcel taken through different pathways, represented mathematically by the Green function. This calculation requires integrating over all possible pathways and times, adding complexity. In contrast, the turnover time is derived from a more straightforward mass-balance approach, depending solely on the difference in mixing ratios between the upper troposphere and the boundary layer. Using observations from the CONvective TRansport of Active Species in the Tropics (CONTRAST) experiment conducted from January to February 2014, this study estimated transit and turnover times by analyzing mixing ratio differences of trace gaseous species between the boundary layer and the upper troposphere in relation to their atmospheric lifetimes. The mean transit time was determined to be 8.4 days, while the mean turnover time was 9.3 days, indicating a remarkable similarity despite their distinct physical interpretations. This close correspondence suggests a robust consistency between the efficiency of vertical transport and upper-tropospheric residence characteristics of species within deep convective systems. These findings might indicate the simpler mass-balance residence time could be applied to represent the convection processes and offer a foundation for quantifying the impact of chemical species on the warming efficiency through convective transport.

How to cite: Wang, C.-W., Luo, Z. J., and Hung, H.-M.: Understanding Convective Transport Through Transit and Turnover Timescales, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8337, https://doi.org/10.5194/egusphere-egu25-8337, 2025.

EGU25-8559 | ECS | Orals | AS3.17

Evidence of Tropospheric Uplift into the Stratosphere via the Tropical Western Pacific Cold Trap 

Xiaoyu Sun, Katrin Müller, Mathias Palm, Christoph Ritter, Denghui Ji, Tim Balthasar Röpke, and Justus Notholt

Understanding air mass sources and transport pathways in the Tropical Western Pacific (TWP) is crucial for determining the origins of atmospheric constituents in the stratosphere. This study uses lidar and ballon observations in Koror, Palau, and trajectory simulations to study the upward transport pathway over the TWP in the upper troposphere and lower stratosphere (UTLS). During northern hemisphere winter, the region experiences the highest relative humidity with respect to ice (RHi) and the lowest temperatures (<185 K) at 16–18 km, and is called the "cold trap".  These conditions lead to water vapor condensation, forming thin cirrus clouds. Latent heat released during cloud formation drives the ascent of air masses.

A case study in December 2018 shows a subvisible cirrus cloud layer (optical depth < 0.03) measured by lidar, coinciding with high supersaturation (RHi > 150%) observed by radiosonde. Trajectories initiated from the cloud layers confirm that air masses ascend slowly from the troposphere into the stratosphere primarily during northern hemisphere winter. In contrast, lidar measurements show similar cloud layers during a summer case (August 2022) with warmer temperatures and drier conditions, where air descends after cloud formation indicated by the forward trajectory. Among all cirrus clouds observed in December and August, 46% of air masses rise above 380 K after cloud formation in December, compared to only 5% in August, possibly influenced by the Asian summer monsoon. These findings underscore the importance of the cold trap in driving air mass transport and water vapor transformations in the UTLS.

How to cite: Sun, X., Müller, K., Palm, M., Ritter, C., Ji, D., Röpke, T. B., and Notholt, J.: Evidence of Tropospheric Uplift into the Stratosphere via the Tropical Western Pacific Cold Trap, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8559, https://doi.org/10.5194/egusphere-egu25-8559, 2025.

EGU25-8747 | Orals | AS3.17

Cold-point tropopause temperature bias modulated by equatorial waves: a reanalysis intercomparison 

Robin Pilch Kedzierski, Sean Davis, Susann Tegtmeier, Krzysztof Wargan, and Martin Weissmann

The tropical Cold-point tropopause temperature (CPT) is a prominent climate variable: it effectively controls the amount of water vapor entering the stratosphere by freeze-drying the air masses that cross through the tropopause near the equator.

GNSS radio-occultation measurements (GNSS-RO) provide global coverage of temperature profiles with high vertical resolution, making possible the monitoring of the CPT evolution outside of the few tropical regions covered by radiosondes. Reanalyses are all known to have a modeled CPT that is on average too warm, compared to GNSS-RO measurements. The reanalysis warm CPT biases maximize near the Equator, hinting at a possible role of equatorial waves.

Observed equatorial CPT shows spectral peaks coinciding with equatorial wave dispersion curves, i.e. it is modulated by the equatorial waves that propagate through the equatorial tropopause. However, to date the warm biases in reanalysis CPT have only been studied from a systematic and zonal-mean perspective, without accounting for equatorial wave presence.

 

In the present study, we bridge this gap by showing how the reanalysis warm CPT bias varies relative to the phase of equatorial waves. Reanalysis datasets (ERA5, ERA-Interim, JRA55, CFSR and MERRA-2, all with CPT from model levels) are inter-compared to multi-mission GNSS-RO for the years 2007-2018. Equatorial waves are filtered from a 5° x 5° daily grid – the best resolution that GNSS-RO data density permits reliably for 2007-2018 – onto which the reanalyses CPTs are interpolated for a 1-to-1 comparison.

A common feature among all reanalysis datasets is as follows: within an equatorial wave’s cold phase, reanalysis CPT biases markedly increase – sometimes by over 1K on top of the average warm bias. The opposite happens within the warm phase of the wave: the bias decreases. This can be explained by the stronger vertical temperature gradients around the colder equatorial CPTs, and the atmospheric models of the reanalyses increasingly struggling there.

There is an important caveat to the above: a time-space scale-dependence, where smaller-scale and faster equatorial waves modulate CPT reanalysis bias more. Mixed Rossby-Gravity waves show this behavior most clearly, Kelvin waves about half the magnitude, and equatorial Rossby wave modulation of CPT reanalysis bias is even weaker but still apparent. In contrast, the large-scale and slow-moving MJO does not show any of this bias modulation.

 

Current work is on validating Inertia-Gravity wave results which may contain significant proportions of noise. Analysis of assimilation increments of CPT in the reanalyses shows data assimilation cooling the modeled CPT – enhancing the gradients around it – in all datasets.

How to cite: Pilch Kedzierski, R., Davis, S., Tegtmeier, S., Wargan, K., and Weissmann, M.: Cold-point tropopause temperature bias modulated by equatorial waves: a reanalysis intercomparison, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8747, https://doi.org/10.5194/egusphere-egu25-8747, 2025.

EGU25-9313 | Orals | AS3.17

Fine scale structure of the tropopause region as measured during the TPEx mission 

Peter Hoor and the The TPEx team

The extratropical transition layer of (ExTL) has been recognized about 20 years ago as part of the upper troposphere / lower stratosphere (UTLS) of the extratropics, which shows the chemical characteristics of both, the stratosphere and the troposphere. Its composition is to a large extent dominated by rapid transient small scale dynamical processes, driven by mid-latitude synoptics. The dynamical processes may include frontal uplift and shear at the tropopause , convection and gravity wave breaking, all in sum leading to turbulence and mixing. As a result gradients of tracer, moisture, and aerosol are highly perturbed on small scales and cross tropopause exchange may occur.

Here we report on a novel measurement approach during June 2024 with a double platform airborne approach targeting small scale variability in the UTLS. This allowed for simultaneous measurements of ozone, humidity and aerosol size distribution on two platforms, which provide information on the vertical gradients of these quantities. The gradients of ozone and aerosol number concentration show a surprisingly high variability in the UTLS and at the tropopause highlighting the importance of small scale processes for the composition of the tropopause region. The measurements were complemented by surface-based and balloon-borne observations at one surface site and comprehensive forecasts including forward trajectories based on ICON forecast data as well as ECMWF forecast data.

We will present highlights from the mission including convective overshoots deep into the LMS at high latitudes, probing of convective outflow and mixing at the tropopause, as well as cirrus occurrence in the stratosphere.

The mission was a central part of the collaborative research center TPChange (The tropopause region in a changing atmosphere).

How to cite: Hoor, P. and the The TPEx team: Fine scale structure of the tropopause region as measured during the TPEx mission, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9313, https://doi.org/10.5194/egusphere-egu25-9313, 2025.

EGU25-9737 | Orals | AS3.17

Tracking air mass history with respect to convective mixing - a SOUTHTRAC example 

Holger Tost, Adrienne Jeske, Linda Smoydzin, and Peter Hoor

The composition of the upper troposphere is determined by both the tropospheric transport times causing near surface air to be transported away from the emission sources as well as the dynamics of the atmosphere, including exchange with the stratosphere. Atmospheric convection and the associated tracer transport lead to rapid mixing of air masses given the strong up- and downdrafts in convective clouds, both in the tropics and the midlatitudes.

However, determining the impact of convection on a sampled air mass is rather difficult from an experimental point of view, as the mixing ratios of short lived compounds can originate from one individual or several convective mixing events. For that purpose, we use global simulation results using parameterised convection and driven by re-analysis data for the period of the SOUTHTRAC campaign.
We sample the output from the convective exchange matrix, i.e., a novel diagnostic for convective transport, on backward trajectories for aircraft measurements and therefore can identify the contribution of near surface air to the UTLS composition. Additionally, we analyse the time evolution of the air mass and the convective events to estimate the contribution of observed trace gases to the total composition in an temporally integrated point of view, which allows to also estimate the chemical degradation of compounds given their individual chemical lifetimes. Overall, this study which is within the framework of the TPChange project, consequently leads to a better understanding of the composition of the upper troposphere and potential injections into the lower stratosphere.

How to cite: Tost, H., Jeske, A., Smoydzin, L., and Hoor, P.: Tracking air mass history with respect to convective mixing - a SOUTHTRAC example, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9737, https://doi.org/10.5194/egusphere-egu25-9737, 2025.

EGU25-10043 | ECS | Posters on site | AS3.17

Observed perturbation of stratospheric chemical composition caused by wildfires smoke vortices 

Loïc Vieille, Fabrice Jégou, Gwenaël Berthet, Clair Duchamp, and Bernard Legras

The increasing severity and duration of forest fire seasons, exemplified by the Canadian fires of 2017 (Pacific Northwest Event) and the Australian fires of 2019-2020 (Australian New Year's event), have highlighted the significant impact of these events on the stratosphere. Through intense pyrocumulonimbus activity, these fires injected large quantities of gases, biomass burning products, and other pollutants into the stratosphere.  During both fires, a unique phenomenon was observed, i.e. the formation of vortex structures in the stratosphere.

Theses vortex structures confined the injected mixture of gases and aerosols, transporting them over weeks in the case of the Canadian fires and months for the Australian fires. These vortices caused localized disturbances in stratospheric chemical composition and triggered specific chemical reactions.

This study focuses on the localized impact created by these vortices, particularly their role in ozone depletion. By confining and transporting biomass combustion products, these vortex structures created conditions for unique chemistry. Data from the Microwave Limb Sounder (MLS) and the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) revealed substantial increases in water vapor and biomass burning tracers, including CO, CH₃Cl, HCN, and CH₃OH. Simultaneously, significant depletions were observed in critical stratospheric reservoirs such as HNO₃, ClONO₂, and HCl. This was accompanied by a marked decrease in ozone mixing ratios with respect to unperturbed conditions, initially associated with injection of ozone-poor tropospheric air but maintained throughout the course of the vortices, questioning about the occurrence of potential ozone destruction through heterogeneous chemical processes, even if no direct evidence of chlorine activation is observed.

Similarities in the chemical content are clearly highlighted for these two events. While this analysis sheds light on the impact of these vortices on stratospheric chemistry, further investigations are necessary to explore the role of organic compounds in the observed ozone depletion and to better understand the broader implications of increasingly severe wildfire events on atmospheric composition and dynamics.

How to cite: Vieille, L., Jégou, F., Berthet, G., Duchamp, C., and Legras, B.: Observed perturbation of stratospheric chemical composition caused by wildfires smoke vortices, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10043, https://doi.org/10.5194/egusphere-egu25-10043, 2025.

EGU25-10853 | ECS | Posters on site | AS3.17

Are springtime Arctic ozone concentrations predictable from wintertime observations? 

Jessica Kult-Herdin, Harald Rieder, and Ales Kuchar

How to cite: Kult-Herdin, J., Rieder, H., and Kuchar, A.: Are springtime Arctic ozone concentrations predictable from wintertime observations?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10853, https://doi.org/10.5194/egusphere-egu25-10853, 2025.

EGU25-11148 | ECS | Posters on site | AS3.17

Evidence of gravity wave contribution to vertical shear and mixing in the lower stratosphere: a WISE case study 

Madhuri Umbarkar, Peter Hoor, Cornelis Schwenk, Annette Miltenberger, Thorsten Kaluza, Hans-Christoph Lachnitt, and Daniel Kunkel

Atmospheric gravity waves (GWs) play a crucial role in the dynamics of the middle atmosphere, transporting energy and momentum and substantially influencing the atmospheric energy budget. In the upper troposphere and lower stratosphere (UTLS), the composition is shaped by horizontal transport, vertical transport associated with convective systems and warm conveyor belts (WCBs), as well as turbulent mixing. GWs can drive cross-isentropic fluxes of trace gases through turbulence generation; however, their role in enhancing shear and turbulent mixing within the extratropical transition layer (ExTL) remains poorly understood.

This study investigates the characteristics and dynamics of GWs generated near an extratropical cyclone using observations from the WISE (Wave-driven ISentropic Exchange) campaign over the North Atlantic on 23 September 2017, supported by ERA-Interim and ERA5 reanalysis data. Additionally, convection-permitting simulations with the ICOsahedral Non-hydrostatic (ICON) model were conducted on a global and two higher resolution nested domains. The tracer observations reveal fine scale structures around the tropopause which are embedded in a region affected by the WCB ascent, inertia gravity waves, a mesoscale modifications in the tropopause structure.

These GWs propagate through highly sheared flows above the jet stream, perturbing background wind shear and static stability, creating conditions conducive to turbulent mixing in the lowermost stratosphere (LMS). The observed significant correlation between GW-induced absolute momentum flux and enhanced small-scale shear confirms their role in driving potential turbulence and facilitating trace gas exchange in the lower stratosphere. Bands of low Richardson number, indicative of potential turbulence, suggest regions prone to clear air turbulence (CAT).

Our findings underscore the critical role of GWs in enhancing vertical wind shear and facilitating turbulent mixing in the LMS, thereby contributing to the formation of the ExTL. These results highlight the necessity of accurately representing GWs in atmospheric models to improve predictions of clear-air turbulence and associated mixing in the UTLS.

How to cite: Umbarkar, M., Hoor, P., Schwenk, C., Miltenberger, A., Kaluza, T., Lachnitt, H.-C., and Kunkel, D.: Evidence of gravity wave contribution to vertical shear and mixing in the lower stratosphere: a WISE case study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11148, https://doi.org/10.5194/egusphere-egu25-11148, 2025.

EGU25-12700 | ECS | Posters on site | AS3.17

Towards Measuring the Uptake of HCl to Organic Aerosol Proxies Under Stratospheric Conditions 

Corey Pedersen, David Verbart, and Frank Keutsch

Stratospheric aerosols have long been known to directly impact ozone concentrations through heterogeneous chemistry involving halogen and nitrogen oxide species. While these aerosols are commonly assumed to consist entirely of sulfate, measurements have revealed a significant organic fraction in the ambient lower stratosphere. Additionally, wildfires like the 2019-2020 Australian wildfires have injected large quantities of organic aerosol (OA) and gas-phase organics into the stratosphere. Satellite observations following the Australian wildfires found that chlorine species were markedly perturbed, and ozone loss had occurred. These perturbations cannot be explained based on the heterogeneous chemistry of sulfate aerosol, demonstrating the need for an improved understanding of stratospheric aerosol heterogeneous chemistry. Despite the widespread presence of OA in the stratosphere, virtually no laboratory experiments have been performed to constrain the interaction of OA with halogen and nitrogen oxide species under stratospheric conditions. The uptake of HCl to OA is particularly important because it is a possible loss pathway of Cly and a precursor to the chlorine activation reaction of ClONO2 + HCl. Here I present the development of an aerosol flow reactor to study the uptake of HCl to OA proxies to improve our understanding of stratospheric chlorine and, by extension, ozone chemistry.

How to cite: Pedersen, C., Verbart, D., and Keutsch, F.: Towards Measuring the Uptake of HCl to Organic Aerosol Proxies Under Stratospheric Conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12700, https://doi.org/10.5194/egusphere-egu25-12700, 2025.

EGU25-12886 | Orals | AS3.17

Two-dimensional observations of dichloromethane-rich air masses transported from the Asian summer monsoon region across the North Pacific 

Wolfgang Woiwode, Jens-Uwe Grooß, Valentin Lauther, Sören Johansson, Jörn Ungermann, Tom Neubert, Andreas Engel, Peter Hoor, and Martin Riese and the GLORIA, CLaMS, HAGAR, and GhOST Teams

Dichloromethane (CH2Cl2) is known to be emitted by industrial processes and suspected to be capable of delaying the recovery of the stratospheric ozone layer significantly. A rapid rise of its global emissions over the last decades, with the majority being located in East and South East Asia, is documented in the literature. We present unique observations of CH2Cl2-rich air masses over the North Pacific, Canada and Alaska by the infrared limb imager GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere). During the boreal summer of 2023, GLORIA was deployed aboard the German research aircraft HALO (High Altitude and LOng Range Research Aircraft) in the framework of the PHILEAS campaign (Probing High Latitude Export of Air from the Asian Summer Monsoon). Two-dimensional vertical cross-sections of CH2Cl2 derived from GLORIA observations in August and September 2023 show large plumes with high mixing ratios of typically up to ~300 pptv far away from their anticipated source regions. Up to 450 pptv are observed locally, which corresponds to ~700% of the northern hemispheric background in that season. Air masses with high CH2Cl2 mixing ratios are detected in the free troposphere and moderately enhanced mixing ratios are observed partly also in the tropopause region. Using backward trajectories and simulations by the Chemical Lagrangian Model of the Stratosphere (CLaMS), the transport pathways and timescales of the observed air masses are analysed. Our analysis suggests that East Asia is a major source region of the observed air masses. Together with the model data and in situ observations by HAGAR-V (High Altitude Gas AnalyzeR-V) and GhOST (Gas chromatograph for Observational Studies using Tracers), the GLORIA observations provide new insights into the long-range transport of CH2Cl2-rich airmasses from the Asian Summer Monsoon region. GLORIA is an airborne demonstrator for the ESA Earth Explorer 11 candidate CAIRT (Changing-Atmosphere Infra-Red Tomography explorer), which is currently in the final selection round and would provide new opportunities to study a multitude of ozone- and climate-relevant trace species continuously.

How to cite: Woiwode, W., Grooß, J.-U., Lauther, V., Johansson, S., Ungermann, J., Neubert, T., Engel, A., Hoor, P., and Riese, M. and the GLORIA, CLaMS, HAGAR, and GhOST Teams: Two-dimensional observations of dichloromethane-rich air masses transported from the Asian summer monsoon region across the North Pacific, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12886, https://doi.org/10.5194/egusphere-egu25-12886, 2025.

EGU25-13178 | ECS | Posters on site | AS3.17

How ENSO affects ozone, RHi and transport dynamics at the UTLS above Palau and the Tropical West Pacific 

Tim Röpke, Katrin Müller, Ingo Wohltmann, and Markus Rex

The Upper Troposphere/Lower Stratosphere (UT/LS) above the Tropical West Pacific (TWP) is an important pathway into the global stratosphere, influencing stratospheric chemistry and atmospheric dynamics overall. Its composition and dynamics are subject to both seasonal and inter-annual variations like El Niño Southern Oscillation (ENSO). We have studied the effects of ENSO on the composition and transport dynamics of the UT/LS using the variables ozone and relative humidity over ice (RHi). The analysis is based on measurements, made at the Palau Atmospheric Observatory (PAO) from 2016 until 2024 using ECC ozone sondes with Vaisala RS92/RS41 radiosondes (Müller et al., 2024a). The PAO is located on the island-state of Palau (7.3° N, 134.5° E); in the tropical warm pool and is part of the Southern Hemisphere ADditional OZone (SHADOZ) network. 

We found that the UT/LS (14-18.5 km) tends to be drier and more ozone-rich during El Niño, compared to La Niña. During El Niño the ascending branch of the Walker Circulation is weakened, resulting in the suppression of local convection and thus less uplift of humid, ozone poor air-masses and accumulation of ozone in the UT/LS. Using Lagrangian-Backtrajectories, calculated with the Lagrangian Chemistry and Transport Model ATLAS (Wohltmann et al., 2009; Wohltmann et al., 2019) we further identified where the air-parcels were last mixed in a convective cell on their way to Palau. We found that under El Niño conditions, during winter and spring the distribution for this point of last mixing shifts eastward with the ascending branch of the Walker Circulation. This is in contrast to summer and autumn, where the point of last mixing distribution shifts northward, with the transport path taking an anticyclonic route from Asia to Palau, indicating the dominant influence of the Asian-Summer-Monsoon (ASM) over the typical El Niño pattern.

We conclude that ENSO is an important mode of variability for the composition and transport dynamics of the UT/LS. However, the seasonal differences for El Niño conditions highlight the importance of the ASM in this region during summer and autumn.

How to cite: Röpke, T., Müller, K., Wohltmann, I., and Rex, M.: How ENSO affects ozone, RHi and transport dynamics at the UTLS above Palau and the Tropical West Pacific, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13178, https://doi.org/10.5194/egusphere-egu25-13178, 2025.

EGU25-13614 | Orals | AS3.17

The role of mesoscale structures in the disturbance of the stratosphere by two major events in 2020 and 2022 

Bernard Legras, Aurélien Podglajen, Clair Duchamp, Pasquale Sellitto, Richard Siddans, Elisa Carboni, and Redha Belhadji

High-explosivity volcanic eruptions and extreme-intensity fires can inject pollutants into the upper troposphere and stratosphere (UTS), generating persistent disturbances of its composition and of the stratospheric aerosol layer, affecting the radiative balance and the climate system on a global scale.

We focus on two recent events, the largest known plume generated by a forest fire on 2020 new year in Australia (AF) with an amplitude comparable to a large volcanic eruption and the Hunga submarine eruption in January 2022, which has generated the largest stratospheric disturbance since the Pinatubo eruption. Its plume has been exceptional by its altitude reach 58 km and the massive injection of water vapour (10% instantaneous increase in the stratosphere).

In both cases, we take advantage of the large number and diversity of spaceborne instruments to analyze and revisit the properties of the stratospheric plumes, in particular the role of confinement in mesoscale structures dynamically induced from the radiative forcing. In the case of the AF, rising anticyclonic smoke vortices were formed by shortwave absorption and maintained compact for several months during which the confinement maintained the high concentration in aerosol and an anomalous chemical composition with a persisting moist air depleted in ozone. The ozone anomaly in the ozone column is also partly dynamical due to the fast rising motion of the vortices when they cruise in the high latitude summer stratosphere. In the case of the Hunga eruption, condensing water vapour was first essential to get rid of most of the ashes during the first hours following the eruption. The strong emission of the remaining water vapour in the stratosphere generated a pair of rapidly descending structures, also anticyclonic, that eventually broke after about a couple of weeks but were essential in maintaining a confinement able to convert SO2 to sulfates at an unprecedented rate. Such compact structures are in fact expected in any plume submitted to localized internal warming or cooling. The confinement process is discussed in relation with the various estimates of SO2 and sulfate, in particular a mesoscale resolving product with IASI which shows the fast conversion to sulfate in mesoscale structures. The longer-term impact is diagnosed with SAGE III, showing how the rapid growth led to larger than usual aerosols with a sharper distribution, differing from other eruptions and providing large radiative impact in spite of the relatively small amount of emitted SO2. In passing, these unusual characters are the main reason of the dispersion of measurements of limb scattered instruments for this event. We show on the contrary that the SAGE III measurements are in very good agreements with the CALIOP estimates of extinctions for the isolated plume.

How to cite: Legras, B., Podglajen, A., Duchamp, C., Sellitto, P., Siddans, R., Carboni, E., and Belhadji, R.: The role of mesoscale structures in the disturbance of the stratosphere by two major events in 2020 and 2022, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13614, https://doi.org/10.5194/egusphere-egu25-13614, 2025.

EGU25-13843 | ECS | Orals | AS3.17

Widespread influence of aerosol from the Asian summer monsoon throughout the extratropical lower stratosphere 

Franziska Köllner and Oliver Eppers and the PHILEAS team

Motivated by the limited knowledge of how much the extratropical UTLS region is influenced by the Asian summer monsoon (ASM) outflow, we conducted the aircraft-based mission PHILEAS (Probing High Latitude Export of air from the Asian Summer Monsoon). The mission took place in August/September 2023, operating from Oberpfaffenhofen (Germany) and Anchorage (Alaska). The research aircraft HALO was equipped with a comprehensive suite of in-situ and remote-sensing instruments for aerosol and gas analysis. 

We performed vertically-resolved submicron aerosol composition measurements up to a potential temperature of 400 K (~14.5 km altitude) by using the ERICA aerosol mass spectrometer. Our analysis identifies particulate ammonium nitrate and organic compounds as prevalent throughout the extratropical lower stratosphere. The mass concentrations are comparable to those in remote continental regions. The presence of this pollution aerosol is linked to the ASM convection, followed by subsequent isentropic northward transport in the stratosphere. Global simulations with the ECHAM/MESSy Atmospheric Chemistry model (EMAC) suggest that this transport pathway persists from July to September and recurs annually. Even after the ASM dissipates in September, the particulate ammonium remains widespread in the stratosphere, with broad implications for stratospheric aerosol composition and heterogeneous chemistry.

How to cite: Köllner, F. and Eppers, O. and the PHILEAS team: Widespread influence of aerosol from the Asian summer monsoon throughout the extratropical lower stratosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13843, https://doi.org/10.5194/egusphere-egu25-13843, 2025.

EGU25-13848 | ECS | Posters on site | AS3.17

Clear air turbulence induced tracer mixing in the UTLS using Chemistry-Climate Model EMAC 

Chun Hang Chau, Peter Hoor, and Holger Tost

The Earth's radiation budget could be affected by the distribution of the chemical composition in the upper troposphere/lower stratosphere (UTLS). Bi-directional stratosphere-troposphere exchange is one of the processes affecting the UTLS chemistry. This exchange could be e.g., facilitated by clear air turbulence (CAT), as it leads to diabatic mixing of chemical tracers between stratosphere and troposphere. Chemistry climate models usually ignore such small scale processes. In order to examine its importance, we developed a new submodel CAT for the climate chemistry model EMAC to parameterize the turbulent tracer mixing in the UTLS. The mixing scheme uses a 2-layer mixing algorithm based on turbulence diagnostics including the widely used Ellrod index and a newly introduced MoCATI. The model results show that the new mixing scheme could lead to a significant difference of the UTLS radiative active tracer gases in a climatological time scale. We also compared the results of the CAT submodel in EMAC with the turbulent mixing scheme of the non-hydrostatic regional model COSMO to investigate the impact of the turbulent mixing on a smaller spatial and temporal scale. The result shows that the new scheme could mix tracer significantly near the tropopause as the COSMO mixing scheme. The implementation of the new CAT submodel could allow further research on the long term climatic impact of turbulent mixing in the UTLS such as radiative budget or ozone destructive substances.

How to cite: Chau, C. H., Hoor, P., and Tost, H.: Clear air turbulence induced tracer mixing in the UTLS using Chemistry-Climate Model EMAC, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13848, https://doi.org/10.5194/egusphere-egu25-13848, 2025.

EGU25-14762 | ECS | Orals | AS3.17

A new method to quantify tracer dispersion in the upper troposphere 

Louis Rivoire, Sebastian Eastham, Arlene Fiore, Jezabel Curbelo, Joseph Palmo, and Justin Finkel

Public attention has been captured by urban pollution and wildfire smoke plumes and their adverse impacts on air quality and public health even far downstream of their origin. Downwind impacts depend on the rate at which these plumes dissipate. However, quantifying this rate using chemical transport models has proven difficult because numerical diffusion systematically overestimates plume dilution. This bias affects our understanding of non-linear chemistry, chemistry-climate coupling, as well as surface impacts. We therefore seek to constrain the rate at which an emitted mass of pollutant is diluted in the upper troposphere, by combining observations with model simulations.

The first step towards our goal is to track plumes in satellite retrievals. The task is daunting: plumes deform, split, and merge, and are at times obscured by clouds or simply out of satellites' sight. In addition, the standard practice of defining plumes as regions with pollutant concentrations greater than a preset threshold is rendered ineffective by the very dilution we aim to quantify: the threshold should change over time to reflect plume dilution, but at what rate?

To address these issues, we propose a new plume definition that incorporates both pollutant ('chemical') data and meteorological ('dynamical') data. Our approach views a plume as a collection of pollutant-enriched air masses, where each air mass is a region bounded by dynamical barriers. Because dilution is slow across such barriers, the envelope of the 'chemical-dynamical' plumes thus defined provides a spatial constraint on dilution processes. By tracking ‘chemical-dynamical’ plumes over time using Lagrangian tools, we aim to more accurately define the volume relevant to quantifying the dilution of the pollutant mass.

We present a proof of concept for our approach using simulated carbon monoxide and meteorological fields archived from the GEOS Chemical Forecast system. We show that our plume-tracking method a) reduces sensitivity to the choice of pollutant concentration threshold to define plumes, and b) can overcome the coverage limitations of pollutant data retrieved by satellite instruments. Overall, our new method represents a promising step towards quantifying tracer dilution using observations as a primary source of information.

How to cite: Rivoire, L., Eastham, S., Fiore, A., Curbelo, J., Palmo, J., and Finkel, J.: A new method to quantify tracer dispersion in the upper troposphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14762, https://doi.org/10.5194/egusphere-egu25-14762, 2025.

EGU25-15106 | ECS | Posters on site | AS3.17

Observation of biomass burning aerosol from Canada in a warm conveyor belt outflow event over Europe during TPEx 

Philipp Joppe, Johannes Schneider, Jonas Wilsch, Heiko Bozem, Anna Breuninger, Joachim Curtius, Nicolas Emig, Peter Hoor, Daniel Kunkel, Hans-Christoph Lachnitt, Isabel Kurth, Yun Li, Annette Miltenberger, Sarah Richter, Christian Rolf, Cornelis Schwenk, Nicole Spelten, Holger Tost, Alexander Vogel, and Stephan Borrmann

The chemical composition, especially of aerosol particles, in the extratropical upper troposphere and lower stratosphere (exUTLS) plays a crucial role in the radiation budget of the atmosphere. This composition is affected by large-scale dynamics in the stratosphere and troposphere, and additionally by small-scale processes. The effects of aerosol particle number concentration as well as the chemical composition in the extratropical lowermost stratosphere (exLMS) are a major research topic in recent years. The measurements presented in this study were taken during the TPEx campaign (Tropopause composition gradients and mixing Experiment) in summer 2024 over the North Sea and northern Germany. In addition to aerosol and trace gas measurements taken on the main platform, a Learjet 35A, we make use of partly redundant aerosol and trace gas measurements on a fully automated sensor shuttle towed by the aircraft (TOSS; towed sensor shuttle), which yield information about the vertical distribution of the measured quantities. The aim of this study is to describe the process of warm conveyor belt (WCB) uplift as source for aerosol particles in the exLMS. Although WCBs are typically associated with cloud formation and efficient precipitation formation, we were able to observe transported aerosol originating at lower altitudes in the outflow. In more detail, we present the observation of a small-scale streamer of polluted biomass burning (BB) air masses which most probably originate from forest fires over Canada. Trajectory analyses indicate that the aerosol is transported within the lowest 2 km above the surface across the Atlantic towards Europe where it undergoes the moist uplift and consequent mixing into the exLMS. The TOSS below the aircraft allows for obtaining in-situ temperature gradients over a vertical scale of 200 m. In particular potential temperature gradients show a change, presumably caused by a potential radiative warming effect of the observed BB aerosol. We compared this observation with a 1D-radiation simulation, for which the measured chemical composition as well as the size distribution of the aerosol particles were used as input parameters.

How to cite: Joppe, P., Schneider, J., Wilsch, J., Bozem, H., Breuninger, A., Curtius, J., Emig, N., Hoor, P., Kunkel, D., Lachnitt, H.-C., Kurth, I., Li, Y., Miltenberger, A., Richter, S., Rolf, C., Schwenk, C., Spelten, N., Tost, H., Vogel, A., and Borrmann, S.: Observation of biomass burning aerosol from Canada in a warm conveyor belt outflow event over Europe during TPEx, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15106, https://doi.org/10.5194/egusphere-egu25-15106, 2025.

EGU25-15894 | ECS | Posters on site | AS3.17

Influence of convection over East Asia on the chemical composition of the Asian Tropopause Aerosol Layer inferred from airborne aerosol mass spectrometry 

Oliver Eppers, Franziska Köllner, Oliver Appel, Philipp Brauner, Fatih Ekinci, Sergej Molleker, Antonis Dragoneas, Warren Smith, Rej Ueyama, Silvia Bucci, Bernard Legras, Christina Williamson, Johannes Schneider, and Stephan Borrmann

The Asian tropopause aerosol layer (ATAL) is a feature occurring within the anticyclone of the Asian summer monsoon in the UTLS region between 13 and 18 km. This aerosol layer can have significant implications for the Earth’s radiative budget (Vernier et al., 2015) and the chemistry of the stratosphere depending on its chemical composition. So far, ammonium nitrate, organics and sulfate have been identified as the main particle compounds found in the ATAL (Appel et al., 2022). High emissions of ammonia in northern India play a crucial role for the formation of ammonium nitrate in the ATAL (Höpfner et al., 2019). However, the effect of different origin regions on the chemical composition of the ATAL remains unclear.

Here, we present a comparison between aircraft-based measurements above India and Nepal during the StratoClim campaign in summer 2017 and above the Western Pacific during the ACCLIP campaign in summer 2022. For both airborne missions, the chemical composition of aerosol particles was measured using the hybrid aerosol mass spectrometer ERICA (ERC instrument for chemical composition of aerosols; Hünig et al., 2022; Dragoneas et al., 2022). In addition, the air mass origin was determined based on kinematic backward trajectories combined with satellite-derived convective cloud top altitudes.

Our results from the non-refractory particle composition measurements reveal a larger contribution of organics and sulfate and less ammonium nitrate mass fractions during the ACCLIP mission compared to the StratoClim measurements. Combining the ERICA results and the trajectory-based product of air mass history, the differences could be explained by a large contribution from east Asian sources. In 2022, the monsoon anticyclone extended further to the northeast compared to the climatological mean. Thus, our results suggest the convection above eastern China with high emissions of SO2 and volatile organic compounds as driver of the observed changes in the ATAL composition.

 

References:

Appel, O., Köllner, F., Dragoneas, A., et al.: Chemical analysis of the Asian tropopause aerosol layer (ATAL) with emphasis on secondary aerosol particles using aircraft-based in situ aerosol mass spectrometry, Atmos. Chem. Phys., 22, 13607–13630, https://doi.org/10.5194/acp-22-13607-2022, 2022.

Dragoneas, A., Molleker, S., Appel, O., et al.: The realization of autonomous, aircraft-based, real-time aerosol mass spectrometry in the upper troposphere and lower stratosphere, Atmos. Meas. Tech., 15, 5719–5742, https://doi.org/10.5194/amt-15-5719-2022, 2022.

Höpfner, M., Ungermann, J., Borrmann, S. et al.: Ammonium nitrate particles formed in upper troposphere from ground ammonia sources during Asian monsoons. Nat. Geosci., 12, 608–612, https://doi.org/10.1038/s41561-019-0385-8, 2019.

Hünig, A., Appel, O., Dragoneas, A., et al.: Design, characterization, and first field deployment of a novel aircraft-based aerosol mass spectrometer combining the laser ablation and flash vaporization techniques, Atmos. Meas. Tech., 15, 2889–2921, https://doi.org/10.5194/amt-15-2889-2022, 2022.

Vernier, J. -P., Fairlie, T. D., Natarajan, M., et al.: Increase in upper tropospheric and lower stratospheric aerosol levels and its potential connection with Asian pollution. J. Geophys. Res. Atmos., 120: 1608–1619. doi: 10.1002/2014JD022372, 2015.

How to cite: Eppers, O., Köllner, F., Appel, O., Brauner, P., Ekinci, F., Molleker, S., Dragoneas, A., Smith, W., Ueyama, R., Bucci, S., Legras, B., Williamson, C., Schneider, J., and Borrmann, S.: Influence of convection over East Asia on the chemical composition of the Asian Tropopause Aerosol Layer inferred from airborne aerosol mass spectrometry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15894, https://doi.org/10.5194/egusphere-egu25-15894, 2025.

EGU25-16298 | ECS | Orals | AS3.17

Fractal Characteristics and Seasonal Variations of Ice-SupersaturatedRegions (ISSRs) in the Tropopause Region 

Helena Schuh, Peter Spichtinger, and Philipp Reutter

Ice supersaturated regions (ISSRs) are area in the upper troposphere and lower stratosphere (UTLS) where relative humidity (RH) with respect to ice exceeds 100%. These regions are critical for the formation of cirrus clouds and contrails. While the impact of ISSRs on the planetary radiation balance is small to negligible, the thin cirrus clouds and aircraft induced contrail cirrus formed within them have a large radiative impact. Understanding the characteristics of ISSRs, including their geometry and seasonal variability, is essential for improving atmospheric models. While ISSR path-length statistics have been studied, their geometric properties, particularly fractal characteristics, and their seasonal variability remain largely unexplored.

We identify ISSRs using ERA5 reanalysis data spanning from 2010 to 2020 at three pressure levels. An area-perimeter method is employed to compute fractal dimensions. The results reveal slopes equaling fractal dimensions with high coefficients of determination, strongly suggesting that ISSRs in the UTLS exhibit fractal behavior. A seasonal cycle in both dimension and total count of observed ISSRs was verified on both hemispheres. We hypothesize that this is caused by the seasonal variation of convective and frontal activity.

We further analyzed the latitudinal and longitudinal spans of ISSRs and the path lengths of modeled flights along common IAGOS flight routes. The results of the latitudinal and longitudinal spans suggest two distinct formation processes for ISSRs.

How to cite: Schuh, H., Spichtinger, P., and Reutter, P.: Fractal Characteristics and Seasonal Variations of Ice-SupersaturatedRegions (ISSRs) in the Tropopause Region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16298, https://doi.org/10.5194/egusphere-egu25-16298, 2025.

EGU25-16726 | ECS | Orals | AS3.17

Microphysical properties and trace gas signatures of a convective overshoot observed over Sweden during the TPex campaign 

Patrick Konjari, Christian Rolf, Martina Krämer, Armin Afchine, Nicole Spelten, Nicolas Emig, Philipp Joppe, Heiko Bozem, and Peter Hoor

Convective overshoot can result in irreversible mixing of air from the troposphere into the stratosphere, thereby influencing the radiation balance of this climate-sensitive region by altering greenhouse gas concentrations, particularly water vapor, and inducing ice and aerosol particles into the stratosphere. This study examines the cloud microphysical properties and trace gas signatures associated with a convective overshoot event observed during the TPex (TropoPause composition gradients and mixing Experiment) campaign in June 2024 over southern Sweden. While recent investigations have predominantly focused on convective overshoots related to air masses of (sub)tropical origin, this particular event took place during a cold air outbreak characterized by low tropopause altitudes (9 km; with temperatures around -55°C).

For the study, microphysical data collected in-situ during Tpex aboard a Learjet by NIXE-CAPS (New Ice eXpEriment - Cloud and Aerosol Particle Spectrometer) and trace gas measurements, including water vapor and ozone, were utilized. The findings reveal that ice particles were transported into the lower stratosphere, up to 1.5 km above the tropopause. At this altitude, a pronounced stratospheric ozone concentration of approximately 800 ppbv and a notable tropospheric water vapor concentration (~40 ppmv) were recorded, the latter being twice as high as background levels at the same height. This substantial injection of tropospheric air was linked to gravity wave breaking, and subsequently irreversible mixing near the overshooting top.

To gain deeper insight into the development of the overshoot, a forward trajectory analysis was conducted, and the evolution of cloud ice microphysical properties along the trajectories was simulated using the CLaMS (Chemical Lagrangian Model of the Stratosphere) model.

How to cite: Konjari, P., Rolf, C., Krämer, M., Afchine, A., Spelten, N., Emig, N., Joppe, P., Bozem, H., and Hoor, P.: Microphysical properties and trace gas signatures of a convective overshoot observed over Sweden during the TPex campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16726, https://doi.org/10.5194/egusphere-egu25-16726, 2025.

EGU25-18146 | Posters on site | AS3.17

How representative are turbulence diagnostic statistics on seasonal time scales? 

Thorsten Kaluza, Paul Williams, David Schultz, Geraint Vaughan, and Timothy Banyard

The current state of knowledge about the occurrence of turbulence in the upper troposphere and lower stratosphere (UTLS) is linked to our understanding of the underlying atmospheric instabilities, the reliability of diagnostics for identifying them in gridded numerical model data, and the availability of measurements to validate the theoretical approach. Although advances in observational coverage and model resolution have led to ongoing reevaluation of the predictive accuracy of turbulence diagnostics, their climatological characteristics, and the alignment with measurement-based climatologies, these aspects are seldom examined together within individual studies using the same datasets. This separation has left room for the interpretation of model-based turbulence maps as a key source for turbulence statistics in the free atmosphere.

We present a climatology of upper tropospheric relativ turbulence frequency maps from several hundred million automated EDR turbulence reports from commercial aircraft between January 2017 and September 2024, made available by the NOAA MADIS ACARS (National Oceanic and Atmospheric Administration – Meteorological Assimilation Data Ingest System – Aircraft Communications Addressing and Reporting System) archive. Sampling biasses in the archived data are taken into account by analyzing only consistently reported turbulence intensities along regularly sampled flight tracks. 

The relative frequency maps of observed turbulence indicate distinct large-scale maxima over the northern hemisphere winter storm tracks, whereas North America exhibits minimum turbulence frequencies across broad areas. Additional maxima are evident along tropical flight routes over the Atlantic and Pacific. The 99th percentile of the Richardson number derived from ERA5 reanalysis data as one key diagnostic shows good agreement with the measurements on seasonal scales, whereas the Ti1 index indicates a distinct northward shift of the storm track maxima as the predominant feature. Linking the seasonal signals with the local forecast precision and probability of detection shows high variability across all longitudes and latitudes, which resolves the apparent contradiction between highest-ranking overall classification skill of the Ti1 index and low agreement with observations on seasonal timescales. 

How to cite: Kaluza, T., Williams, P., Schultz, D., Vaughan, G., and Banyard, T.: How representative are turbulence diagnostic statistics on seasonal time scales?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18146, https://doi.org/10.5194/egusphere-egu25-18146, 2025.

EGU25-18470 | ECS | Orals | AS3.17

Turbulent fractions in the Tropical Tropopause Layer using STRATEOLE-2 long-duration balloon measurements 

Flore Juge, Richard Wilson, and Albert Hertzog

The Tropical Tropopause Layer (TTL) is a gateway for momentum fluxes and atmospheric components to the global stratosphere. The dynamical processes in the TTL remain challenging to characterize, particularly at turbulent length scales, and are still poorly understood. Current estimates of turbulence frequency and intensity vary considerably between observations in this region, although they are crucial for designing efficient and accurate model parameterizations.

 

Quasi-Lagrangian in situ measurements of thermodynamic parameters and GPS are obtained from STRATEOLE-2 long-duration balloons drifting at isopycnal level around 20 km altitude during several months over the equator. The balloons' vertical oscillations around their density equilibrium position in a stratified environment allow us to estimate local vertical gradients in temperature, pressure and winds. From these estimates we evaluate Richardson numbers, which enable us to characterize the flow as turbulent or laminar during each flight, and thus to estimate turbulent fractions. 

 

Various methods were tested to evaluate local gradient estimates that can be applied directly to the detection of turbulent episodes. For example, using the envelope defined by the local extrema of the time series, we estimate instantaneous local gradients from the ratio of the variables amplitude to the vertical displacement amplitude. This approach enables the reconstruction of temperature and wind increments time series. By calculating correlations between observed and reconstructed increments, we show that our gradients are quite consistent, especially for shear winds estimates. 

 

We deduce the turbulent fraction from the ratio of the mean lifetime of turbulent episodes to the mean interval between two successive ones. Additionally, we describe the distribution of these estimates. 

How to cite: Juge, F., Wilson, R., and Hertzog, A.: Turbulent fractions in the Tropical Tropopause Layer using STRATEOLE-2 long-duration balloon measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18470, https://doi.org/10.5194/egusphere-egu25-18470, 2025.

EGU25-19003 | Orals | AS3.17

Observed zonally and meridionally resolved trends in lapse rate tropopause temperature and height over the past two decades 

Florian Ladstädter, Matthias Stocker, Sebastian Scher, and Andrea K. Steiner

The tropopause is a sensitive indicator of both radiative and dynamic changes in the atmospheric climate system. This study presents an analysis of lapse-rate tropopause (LRT) trends using remote-sensing satellite data for the period 2002-2023. The evaluation of trends is performed using GNSS radio occultation satellite measurements, which are particularly well suited for observing the temperature in the tropopause region with high vertical resolution and global coverage. In addition, GNSS radio occultation provides long-term stable measurements that allow robust detection of tropopause trends. Our results indicate pronounced zonal and meridional variations in LRT temperature trends, with  certain regions exhibiting significant warming while others show no substantial trends. In particular, the tropics show LRT warming but no trend in LRT height. Additionally, we observe distinct seasonal patterns of trends in LRT temperature and height, with particularly pronounced trends in the Pacific region in the Northern Hemisphere winter. A spatially and seasonally resolved view of LRT trends is thus required for a complete picture of the changes in the tropopause region.

How to cite: Ladstädter, F., Stocker, M., Scher, S., and Steiner, A. K.: Observed zonally and meridionally resolved trends in lapse rate tropopause temperature and height over the past two decades, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19003, https://doi.org/10.5194/egusphere-egu25-19003, 2025.

EGU25-19101 | ECS | Orals | AS3.17

Long-term Changes in the Thermodynamic Structure and the Mass of the Lowermost Stratosphere Comparing Five Modern Reanalyses 

Franziska Weyland, Peter Hoor, Daniel Kunkel, Thomas Birner, Katharina Turhal, and Felix Plöger

The mass of the lowermost stratosphere (LMS) is an important characteristic of the thermodynamic structure of the lower stratosphere. From a scientific perspective, long-term LMS mass changes illustrate the combined effect of tropopause pressure trends, tropical width trends and temperature changes in the tropical tropopause region. Further, understanding LMS mass trends can improve our knowledge of lower stratospheric ozone and water vapor trends that, despite their radiative importance, are still insufficiently understood. From a technical perspective, comparing LMS mass trends across reanalyses reveals consistencies and discrepancies between the data sets.

 

We examine long term trends in LMS mass using five modern reanalyses – ERA5, ERA-Interim, MERRA-2, JRA-55 and JRA3Q – for the time period 1979–2019. The focus is on changes after the year 1998, marking the anticipated beginning of stratospheric ozone recovery. The trend analysis is performed with a dynamic linear regression model (DLM).

 

All reanalyses consistently show decreasing tropopause pressure in the tropics and the Northern Hemisphere (NH) extratropics. This is reflected in a robust LMS mass decrease in the NH when a fixed isentrope of 380K is used as upper boundary, i.e. to approximate the tropical tropopause. However, we show that a fixed isentrope is an inadequate approximation of the upper LMS boundary for long-term studies, as the tropical tropopause also exhibits a trend. Therefore, we propose dynamically varying upper boundaries linked to the tropical tropopause potential temperature, accounting for this trend. In ERA5, ERA-Interim and MERRA-2, the dynamical upper boundaries are able to partly compensate for the tropopause rise in the NH. In contrast, the LMS mass decrease in the NH is enhanced by the dynamical upper boundaries in JRA-55 and JRA3Q. This is due to opposing absolute temperature trends in the tropical tropopause region across the reanalyses.

How to cite: Weyland, F., Hoor, P., Kunkel, D., Birner, T., Turhal, K., and Plöger, F.: Long-term Changes in the Thermodynamic Structure and the Mass of the Lowermost Stratosphere Comparing Five Modern Reanalyses, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19101, https://doi.org/10.5194/egusphere-egu25-19101, 2025.

EGU25-19191 | ECS | Orals | AS3.17

A Source of Clear-Air Turbulence? Tracking Gravity Wave Formation in Inertially Unstable Regions 

Timothy P. Banyard, David M. Schultz, Geraint Vaughan, B. Helen Burgess, Thorsten Kaluza, and Paul D. Williams

Turbulence was responsible for 71% of all weather-related aviation accidents and incidents in the US between 2000–2011 [1], leading to structural damage, injuries, and US$200 million in unforeseen costs for airlines each year [2]. With only 14% of turbulence encounters being attributable to convection [3], clear-air turbulence (CAT) is a leading cause of these encounters and thus poses a major risk to travellers.

A variety of dynamical mechanisms can be responsible for CAT, including shear instabilities, inertial instabilities, and gravity waves; however, differentiating between the distinct roles of each mechanism when more than one is present remains difficult. In fact, it is the precise evolution of these atmospheric instabilities and waves, and their potential for generating CAT, which remain uncertain in our current scientific understanding.

In this study, we investigate the relationship between CAT and gravity waves, with a specific focus on tracking the formation of these waves around regions of inertial instability. Previously, [4] showed the emission of inertia–gravity waves following the release of inertial instability using idealised model simulations. Here, we use the WRF model to consider some real-world examples of where regions of low potential vorticity (PV) in the vicinity of the jet stream are associated with inertia–gravity waves. We track the waves as they propagate and investigate whether the causal link found by Thompson and Schultz can be observed in more realistic simulations.

We present results from several case studies exhibiting this behaviour, identifying the sources of the gravity waves observed in simulations. The characteristics of these waves will be compared to those in the idealised model simulations, and gravity-wave parameters will be calculated. Finally, we widen our analysis by examining the broader upstream pattern that contributes to the development of the initial inertial instabilities and explore the different regimes under which these phenomena occur.

References:
[1] Gultepe, I. et al. (2019), "A review of high impact weather for aviation meteorology." Pure and Applied Geophysics, 176, pp.1869–1921.
[2] Williams, J. K. (2014), "Using random forests to diagnose aviation turbulence." Machine Learning, 95, pp.51-70.
[3] Meneguz, E., Wells, H. and Turp, D. (2016), "An automated system to quantify aircraft encounters with convectively induced turbulence over Europe and the Northeast Atlantic." Journal of Applied Meteorology and Climatology, 55(5), pp.1077-1089.
[4] Thompson, C. F. and Schultz, D. M. (2021), "The release of inertial instability near an idealized zonal jet." Geophysical Research Letters, 48(14), e2021GL092649.

How to cite: Banyard, T. P., Schultz, D. M., Vaughan, G., Burgess, B. H., Kaluza, T., and Williams, P. D.: A Source of Clear-Air Turbulence? Tracking Gravity Wave Formation in Inertially Unstable Regions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19191, https://doi.org/10.5194/egusphere-egu25-19191, 2025.

EGU25-19811 | ECS | Posters on site | AS3.17

Observations of water vapor in the UT/LS of unprecedented accuracy with non-equilibrium corrected frost point hygrometers 

Yann Poltera, Beiping Luo, Frank G. Wienhold, and Thomas Peter

We present a new retrieval protocol for chilled mirror hygrometer measurements under rapidly changing humidity conditions that enables balloon-borne frost point measurements in the upper troposphere/lower stratosphere of unprecedented accuracy. Chilled mirror hygrometers measure the frost point (or dew point) of air by quantifying the degree of saturation of the air with respect to the condensed phases of water (ice or liquid water). To this end, they attempt to determine the thermodynamic equilibrium of the condensate with the vapor phase by measuring the mirror reflectance, which changes with the thickness of the condensate. In the rapidly changing environment along the balloon trajectory, however, the adjustment of the mirror temperature to the new equilibrium point leads to frequent, damped overshoots or non-equilibrium errors. For the Cryogenic Frost Point Hygrometer (CFH), a balloon-borne chilled mirror instrument of reference quality, we (i) identify points in time along the balloon trajectory when the mirror is in true equilibrium with the gas phase, which we term ‘Golden Points’, and (ii) correct the measurements for non-equilibrium conditions between these Golden Points. For (i), we identify the points where the mirror reflectance assumes an extreme value, i.e. a maximum or a minimum. At these extreme points, the CFH mirror temperature represents the frost point with an accuracy better than 0.2 K (resulting from the uncertainties of the mirror temperature sensor and the precise timing of the Golden Points along the sounding profile). These accurately determined frost points can be used to detect and correct offsets, biases and time-lag errors in other humidity sensors flown together with CFH on the same balloon payload, such as the thin-film capacitive hygrometer of the Vaisala RS41 radiosonde. In the middle stratosphere (~ 28 km), a frost point uncertainty of 0.2 K corresponds to < 4 % uncertainty (2-σ) in H2O mixing ratio which includes the 0.3 hPa uncertainty of the RS41 radiosonde GPS-based pressure measurement. At lower altitudes, the uncertainty is even less. For (ii), we compute the time-derivative of the mirror reflectance, which is proportional to the non-equilibrium error. The proportionality factor is related to a property of the mirror condensate, which we term ‘morphological sensitivity’, and allows correction of the CFH non-equilibrium data. The sensitivity constant is determined using an a-priori reference, such as the RS41 radiosonde humidity measurements after they have been time-lag and bias-corrected by means of (i), or the Golden Points interpolation in situations where Golden Points occur frequently enough (< 50 m) and the non-equilibrium error between Golden Points is large enough (> 0.5 K). This procedure paves the way for H2O mixing ratio and relative humidity observations of unprecedented accuracy (< 4 % at 250 m vertical resolution) in the UT/LS. We showcase this novel measurement strategy and design philosophy on chilled mirror hygrometers with low global warming potential coolant, DIA-CFH (i.e., CFH using a mixture of dry ice and alcohol as coolant) and PCFH (thermoelectric coolant), flown in 2023-2024 over the central European alpine region as part of the Swiss H2O Hub project.

How to cite: Poltera, Y., Luo, B., Wienhold, F. G., and Peter, T.: Observations of water vapor in the UT/LS of unprecedented accuracy with non-equilibrium corrected frost point hygrometers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19811, https://doi.org/10.5194/egusphere-egu25-19811, 2025.

EGU25-19950 | ECS | Orals | AS3.17

Stratospheric Water Vapor Affecting Atmospheric Circulation 

Edward Charlesworth and Felix Plöger

A consistent result of climate model simulations is the moistening of the stratosphere. Many models show their strongest changes in stratospheric water vapor in the extratropical lowermost stratosphere, a change which could have substantial climate feedbacks (e.g. Banerjee et al. 2019). 

However, models are also heavily wet-biased in this region when compared to observations (Keeble et al. 2020), presenting some uncertainty on the robustness of these model results. In this study, we examine this wet bias, showing that it is consistent across various models. We present the results of applying a fully-Lagrangian transport scheme (CLaMS) within the EMAC climate model, showing that water vapor distributions from the modified model are very similar to observations.

Addionally, we describe the sensitivity of the atmospheric circulation in the stratosphere and troposphere to the abundance of water vapor in the lowermost stratosphere, including the mechanism by which this occurs, and show that the related effects on atmospheric circulation are of similar magnitude as climate change effects.

How to cite: Charlesworth, E. and Plöger, F.: Stratospheric Water Vapor Affecting Atmospheric Circulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19950, https://doi.org/10.5194/egusphere-egu25-19950, 2025.

EGU25-20209 | ECS | Orals | AS3.17

Importance of the representation of aerosol wet scavenging for aviation aerosol transport 

Nicolas Février, Didier Hauglustaine, and Nicolas Bellouin

Aircraft engines emit aerosols and aerosol precursor gases, mostly black carbon (soot) and sulfur dioxide, which remain longer in the atmosphere than aerosols emitted at the surface. Long-range transport during that long residence time means that aviation aerosols may interact with clouds far from the main flight corridors. The radiative forcing of interactions between aviation aerosols and clouds is so uncertain that even its uncertain range is unknown. Its quantification relies on climate models, where aerosol concentrations and long-range vertical and horizontal transport are strongly affected by wet scavenging, which can be parameterized in different ways with several tunable parameters. One could assume that the representation of wet scavenging is of secondary importance for the simulated residence time of aviation aerosols, because they are emitted high above precipitating clouds. In this work, we use the LMDZ-OR-INCA climate model to investigate the impact of three different scavenging parameterizations on total and aviation aerosol distributions, using regional and seasonal vertical profiles measured during the ATom and HIPPO airborne campaigns to evaluate the performances of the different parameterizations. Results confirm that the residence time and the mass budgets of black-carbon, sulfates and nitrates from all sources are significantly influenced by the scavenging scheme. Moreover, the skill of a scavenging parameterization to simulate vertical aerosol concentration profiles depends on geographical location, altitude and season, although no parametrizations are consistently better than the others. Unexpectedly, the scavenging parameterizations also affect aviation aerosol concentrations at flight cruise levels: although scavenging rates are small, residence time are long so differences accumulate. Near-surface aerosol concentrations, which are mainly due to Landing and Take-off Operations (LTO), are also affected by the choice of a wet scavenging parameterization. Results suggest it may be possible to design a new scavenging routine for LMDZ-OR-INCA model to better represent the long-range transport of aviation aerosols and reduce uncertainties in aviation aerosol-cloud interaction radiative forcing.

How to cite: Février, N., Hauglustaine, D., and Bellouin, N.: Importance of the representation of aerosol wet scavenging for aviation aerosol transport, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20209, https://doi.org/10.5194/egusphere-egu25-20209, 2025.

EGU25-20453 | ECS | Posters on site | AS3.17

The Organic Contribution to Stratospheric Aerosol Particles Collected during the SABRE 2023 Campaign 

Sophie Abou-Rizk, Yaowei Li, Zezhen Cheng, Swarup China, Zhenli Lai, Xena Mansoura, Gregory Vandergrift, Nurun Nahar Lata, Ashfiqur Rahman, Troy Thornberry, John Dykema, and Frank Keutsch

Stratospheric aerosols play a critical role in the chemistry of the atmosphere and the climate through heterogeneous chemistry and radiative forcing. While sulfate aerosols in the stratosphere are relatively well-studied, the organic component of stratospheric aerosols remain poorly understood, despite their potential to impact climate and chemistry.

The Stratospheric Aerosol processes, Budget, and Radiative Effects (SABRE) 2023 campaign employed high-altitude aircraft (WB-57) with a payload designed to better characterize stratospheric aerosols. We used a cascade impactor (Mini-MOUDI 135, MSP) to collect aerosol particles between 0.18-3.2 μm aerodynamic diameter for offline analysis. Here we highlight the effectiveness of Computer-Controlled Scanning Electron Microscopy with Energy Dispersive X-ray (CCSEM-EDX) and Scanning Transmission X-ray microscopy paired with near-edge X-ray absorption fine structure (STXM-NEXAFS) to determine stratospheric aerosol composition and morphology. These properties can help constrain aerosol effects on radiative forcing and ozone chemistry. CCSEM-EDX is used to analyze the morphological and elemental properties of atmospheric aerosols on the single particle basis. STXM-NEXAFS uses carbon K-edge spectra to categorize individual stratospheric aerosols into organic carbon, elemental carbon, and inorganic content, which can be used to investigate the mixing state, morphology, and carbon functional group distribution. Preliminary findings from nanospray Desorption Electrospray Ionization (nano-DESI) further reveal molecular-level organic aerosol composition. We show comparative analysis across multiple flights, distinguishing between polar vortex and non-polar vortex air. Finally, we explore the implications of these findings for assessing the chemical and radiative properties of stratospheric aerosols, advancing our understanding of their role in Earth’s atmosphere. 

How to cite: Abou-Rizk, S., Li, Y., Cheng, Z., China, S., Lai, Z., Mansoura, X., Vandergrift, G., Lata, N. N., Rahman, A., Thornberry, T., Dykema, J., and Keutsch, F.: The Organic Contribution to Stratospheric Aerosol Particles Collected during the SABRE 2023 Campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20453, https://doi.org/10.5194/egusphere-egu25-20453, 2025.

In this paper, we estimate the adiabatic cooling and warming in the MLT utilizing the SABER CO2 VMR displacement from the global mean. This confirms that the summer mesopause temperature is largely controlled by adiabatic cooling instead of any absorptive heating or chemical heating. Because the adiabatic cooling is dynamically driven by waves from below, the summer polar mesopause is mostly sensitive to the changes in the stratosphere and mesosphere, for example, Sudden Stratospheric Warmings (SSWs) and polar vortex. And it well explains that the Aeronomy of Ice In the Mesosphere (AIM) satellite did not observe solar cycle responses in PMCs over the latest solar cycles. Unlike UV radiative heating in the upper atmosphere, dynamical cooling and mesosphere dynamics may have a complex relationship with the solar cycle. The paper also reveals a previously overlooked layer of adiabatic warming in summer and cooling in winter in the lower thermosphere due to downwelling and upwelling. Because this process is embedded in the thermosphere where mean temperature rises sharply driven by diffusive heating (or heat conduct from the upper thermosphere), it is not obvious without removing the global mean temperature. The mesosphere is the opposite, being lacking of strong heating sources. The heating layer (~100 K) in the summer lower thermosphere is substantial. Auroral heating also occurs in the magnetic polar lower thermosphere. How the adiabatic heating and cooling in the polar lower thermosphere interacts with auroral heating and the Joule heating driven adiabatic heating and cooling during geomagnetic active times warrants further investigations.   

How to cite: Yue, J. and Wang, N.: Estimation of Adiabatic Cooling and Warming in the Mesosphere and Lower Thermosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-185, https://doi.org/10.5194/egusphere-egu25-185, 2025.

EGU25-786 | ECS | Posters on site | ST3.3

Stratosphere, Stratopause, and Lower Mesosphere in the JRA-55and JRA-3Q reanalyses: Insights and Discrepancies 

Celia Pérez Souto, Juan A. Añel, Aleŝ Kuchař, and Laura de la Torre

The representation of the stratosphere in reanalyses is crucial for various issues such as atmospheric transport, sudden stratospheric warmings, the polar vortex, and studying the impact of climate change. High-top and latest reanalyses are designed with the aim of being able to reproduce the high stratosphere better than previous generation of low-top reanalyses, thus being better equipped to capture issues such as elevated stratopause events.

In this study, we examine how various variables behave in both reanalyses, JRA-55 and JRA-3Q, showing notable differences when comparing various parameters such as correlations and trends. We show that JRA3Q exhibit substantial differences in their representation of the middle and upper stratosphere compared to its predecessors or ERA5.1. Different latitudinal bands have been compared for this purpose. For instance, negative correlations in stratopause height have been observed in the subtropical zone between both reanalyses. Moreover, negative correlations with JRA-3Q and high correlations with JRA-55 have been observed when compared with observational data from MLS (Microwave Limb Sounder), on board of AURA satellite. Also, we compare our results with SABER (Sounding of the Atmosphere using Broadband Emission Radiometry) data, allocated in TIMED (Thermosphere Ionosphere Mesosphere Energetics Dynamics) satellite.

How to cite: Pérez Souto, C., Añel, J. A., Kuchař, A., and de la Torre, L.: Stratosphere, Stratopause, and Lower Mesosphere in the JRA-55and JRA-3Q reanalyses: Insights and Discrepancies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-786, https://doi.org/10.5194/egusphere-egu25-786, 2025.

EGU25-3199 | ECS | Orals | ST3.3

Resolved Gravity Waves in High-Resolution Nested UA-ICON Simulations Compared to Mesospheric Observations of the VortEx Campaign 

Yanmichel A. Morfa Avalos, Markus Kunze, Tarique A. Siddiqui, Christoph Zuelicke, Claudia C. Stephan, Claudia Stolle, Irina Strelnikova, Gerd Baumgarten, Robin Wing, Michael Gerding, Toralf Renkwitz, Mohamed Mossad, Gerald A. Lehmacher, Sebastian Borchert, and Jorge Luis Chau

We conducted high-resolution nested simulations over Andøya, Norway (ALOMAR) with UA-ICON to be co-analyzed with mesospheric measurements collected during the NASA Vorticity Experiment (VortEx) sounding rocket campaign in March 2023. The UA-ICON model was configured with 180 vertical levels, a model top at 150 km, and a global horizontal resolution of R2B7 (~20 km). One-way nesting was applied to achieve progressively finer resolutions of R2B8 (~10 km), R2B9 (~5 km), R2B10 (~2.5 km), and R2B11 (~1.25 km). For the global domain (~20 km horizontal resolution), the dynamic situation during the campaign is specified (specified dynamics, SD) by nudging to ECMWF operational analyses up to an altitude of 50 km. At resolutions finer than 5 km, UA-ICON resolves a significant portion of the gravity wave (GW) spectrum. Consequently, GW and convective parameterizations were disabled to isolate the effects of resolved GWs. Observational data from the campaign include wind measurements from the rocket flight, along with temperature and wind profiles up to ~80 km from the Rayleigh-Mie-Raman (RMR) lidar, and horizontal wind fields from the MF Saura and SIMONe Norway radar systems. We present and discuss initial results from comparisons between the simulations and the observations collected during the VortEx campaign. UA-ICON spectra exhibit the characteristic frequency spectrum of gravity waves, following the $\omega^{-2}$ relationship, validated by the observed Lidar spectrum. The simulations align well with observations, demonstrating UA-ICON's effectiveness in studying MLT dynamics.

How to cite: Morfa Avalos, Y. A., Kunze, M., Siddiqui, T. A., Zuelicke, C., Stephan, C. C., Stolle, C., Strelnikova, I., Baumgarten, G., Wing, R., Gerding, M., Renkwitz, T., Mossad, M., Lehmacher, G. A., Borchert, S., and Chau, J. L.: Resolved Gravity Waves in High-Resolution Nested UA-ICON Simulations Compared to Mesospheric Observations of the VortEx Campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3199, https://doi.org/10.5194/egusphere-egu25-3199, 2025.

EGU25-3334 | Orals | ST3.3

Impact of Weak and Strong Polar Vortices in the Northern and Southern Hemispheres on Solar-Migrating Semidiurnal Tides in the lower thermosphere using UA-ICON model simulations 

Claudia Stolle, Akash Kumar, Yosuke Yamazaki, Nicholas M. Pedatella, Markus Kunze, Claudia C. Stephan, Tarique A. Siddiqui, and M. V. Sunil Krishna

The coupling between the stratosphere and the mesosphere-lower thermosphere (MLT) has been known for several years. Its investigation was further pushed during the deep minimum of solar cycle 24 when the upper atmosphere was less affected by solar and geomagnetic forcing and by variability due to atmospheric forcing from below became more significant in observations. Another aspect supporting the understanding of the vertical atmosphere coupling has been the increased availability of globally distributed observations and of sophisticated general circulation models reaching up to the thermosphere.    

A negative correlation between the strength of the northern stratospheric polar winter vortex and solar-migrating semidiurnal tides (SW2) in winds at around 100 km altitude has been derived recently by Pedatella and Harvey (2022) based on 38 years of SD-WACCM-X model data. Observational evidence of this correlation was provided shortly afterwards by Kumar et al. (2023) using 26 years of geomagnetic observations of the equatorial electrojet, the latter being largely driven by thermospheric winds.

In this study, we have used a 60-year free-run simulation by the upper atmospheric extension of the ICOsahedral Non-hydrostatic (UA-ICON) general circulation model to explore the influence of northern hemisphere (NH) and southern hemisphere (SH) stratospheric polar vortex variability on the MLT. This study also elucidates the response of SW2 in MLT winds to variations in the strength of polar vortices. A weak NH polar vortex is associated with an increase in SW2, while a strong NH vortex results in a decrease in SW2. The response of SW2 to changes in the strengths of the SH polar vortex is similar, although considerably weaker. The NH polar vortex variability can explain around 40 − 50% of the variability in the SW2 during NH winter. The SH polar vortex, however, accounts for only a small fraction of the variability (up to ∼ 5%) in SW2, highlighting hemispheric differences in the response to stratospheric polar vortex variability.

References:

Kumar, S., Siddiqui, T. A., Stolle, C. and Pallamraju, D., Impact of strong and weak stratospheric polar vortices on geomagnetic semidiurnal solar and lunar tides. Earth Planets Space, 75, 52, https://doi.org/10.1186/s40623-023-01810-x, 2023.

Pedatella, N.M. and Harvey, V. L., Impact of strong and weak stratospheric polar vortices on the mesosphere and lower thermosphere. Geophys. Res. Lett. 49, e2022GL098877. https://doi.org/10.1029/2022GL098877, 2022.

How to cite: Stolle, C., Kumar, A., Yamazaki, Y., Pedatella, N. M., Kunze, M., Stephan, C. C., Siddiqui, T. A., and Krishna, M. V. S.: Impact of Weak and Strong Polar Vortices in the Northern and Southern Hemispheres on Solar-Migrating Semidiurnal Tides in the lower thermosphere using UA-ICON model simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3334, https://doi.org/10.5194/egusphere-egu25-3334, 2025.

Several studies have shown the importance of solar tides for the dynamics in the MLT region. The solar tidal modes generated
in the troposphere and stratosphere increase in amplitude as they propagate vertically, transporting energy and momentum
to higher layers and enhancing layer mixing. The energy and momentum deposition by wave breaking alters the angular
momentum and kinetic energy budget and forces the global circulation in the MLT.


The majority of observations of solar tides have been derived from satellite data. Temperature and wind measurements from
satellites in geostationary orbits have been successfully used to derive tidal amplitudes around the equator. At higher latitudes,
however, the temporal resolution of the derived data product is limited by the orbital geometry of the satellites. With a revis-
iting time of several hours, the data set must be sampled over long periods to derive spectral components with periods of 8,
12, or 24 hours. In contrast, ground-based observations provide a comparably high time resolution of 0.5-1 hours, which is
suitable for investigating the short-time variability of solar tides. Observations of tidal amplitudes derived from ground-based
measurements using meteor radar systems, LIDARs, and microwave radiometers, are reported but are rare.


TEMPERA-C is a newly developed fully polarimetric ground-based microwave radiometer for temperature observations in the middle atmo-
sphere. It is designed to measure the four Stokes components of the Zeeman-split fine structure emission line of oxygen at 53
GHz. Compared to single polarized instruments, TEMPERA-C has an increased altitude coverage for temperature retrievals
with an upper limit of 60 km. By resolving the Zeeman-split emission line with a digital correlator with high frequency
resolution, retrievals of magnetic field features are possible. However, the calibration of a fully polarimetric instrument is more
complex than in the case of single polarization.


For a test campaign, TEMPERA-C measured continuously from March to November 2024 at the Jungfraujoch high-altitude
research station. In my presentation, I will focus on how thermal tides and other wave modes can be derived from this dataset.
I will also introduce the instrument, present a simplified calibration method, and discuss the influence of the Earth’s magnetic
field on the measured spectra.

How to cite: Krochin, W., Stober, G., and Murk, A.: Thermal tide observations from ground-based measurements of the Zeeman-split emission lines of oxygen at 53 GHz, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3786, https://doi.org/10.5194/egusphere-egu25-3786, 2025.

EGU25-3889 | Posters on site | ST3.3

Stratospheric contraction under Climate Intervention by Sulfate Aerosol Injection 

Juan Antonio Añel, Juan Carlos Antuña-Marrero, Susana Bayo-Besteiro, Celia Pérez-Souto, and Laura de la Torre

Anthropogenic CO2 emissions cause the Earth's Stratosphere to contract because of radiative cooling of the layer, lowering of the stratopause, heating of the troposphere, and rising of the tropopause.
Stratospheric sulphate aerosol injection (SAI) has been proposed over the years as a potential climate intervention technique to counteract some of the impacts of climate change. Many of the impacts of such interventions on the tropospheric climate have been studied; however, the impacts on the stratosphere are not so well studied.
Here, we present results from model simulations on the impact of SAI on the current trend of stratospheric contraction, using data from the Geoengineering Large Ensemble Project (GLENS). Our results show that in GLENS simulations, SAI can counteract part of the stratosphere contraction while the whole stratosphere moves down.

How to cite: Añel, J. A., Antuña-Marrero, J. C., Bayo-Besteiro, S., Pérez-Souto, C., and de la Torre, L.: Stratospheric contraction under Climate Intervention by Sulfate Aerosol Injection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3889, https://doi.org/10.5194/egusphere-egu25-3889, 2025.

EGU25-4006 | Orals | ST3.3

The neutral October effect in the lower mesosphere simulated by different models 

Vivien Wendt and Helen Schneider

The October effect is long known as a sharp decrease in the amplitude of radio waves with Very Low Frequency (VLF) reflected in the D-region (60-90km). However, the mechanism of the October effect is unclear until today. Recent studies show that neutral atmosphere dynamics might cause the October effect. Simultaneously with the October effect in the ionized D-region, there is a warming in the lower mesosphere, which we call the neutral October effect and which cannot be observed in spring, resulting in a spring-fall asymmetry. This spring-fall asymmetry is reproduced by MERRA-2 in years after 2005 only when satellite observations are assimilated in the mesosphere. Other models like WACCM-X, ERA5 and GAIA also have difficulties reproducing this asymmetry. Only CMAM30 can reproduce the neutral October effect. A modelling study and various analysis techniques are used to investigate the mechanism of the neutral October effect in the neutral atmosphere. Based on our results we assume that the onset of the planetary wave activity and westward gravity wave drag after the quiet summer season induces a poleward and downward motion resulting in the observed warming in the lower mesosphere. 

How to cite: Wendt, V. and Schneider, H.: The neutral October effect in the lower mesosphere simulated by different models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4006, https://doi.org/10.5194/egusphere-egu25-4006, 2025.

EGU25-4603 | ECS | Posters on site | ST3.3

Polar ozone anomalies, radiative effects, and their connection to mesospheric tidal dynamics during extreme events 

Guochun Shi, Hanli Liu, Alexander Kozlovsky, Njål Gulbrandsen, Dimitry Pokhotelov, Mark Lester, Masaki Tsutsumi, Kun Wu, and Gunter Stober

Continuous ozone measurements above Ny-Ålesund, Svalbard (79°N, 12°E), using the ground-based microwave radiometer GROMOS-C, effectively capture the daily, seasonal, and interannual variability of polar ozone in the middle atmosphere. In this study, we analyze observed ozone changes during sudden stratospheric warming (SSW) events and compare the measurements with Aura/MLS satellite data and WACCM-X simulations. Results reveal the formation of a double-ozone layer in the stratosphere and lower mesosphere following the onset of SSW events, with ozone levels increasing by approximately 50% relative to the background value. Ozone absorbs solar UV radiation, contributing to radiative heating in the stratosphere and mesosphere. To further explore the impact of radiative ozone processes on mesospheric tide variability during SSWs, we extract diurnal (DT), semidiurnal (SDT), and terdiurnal (TDT) tidal components from zonal and meridional wind measurements recorded by meteor radars at three high-latitude stations: Sodankylä (67.37°N, 26.63°E), Tromsø (69.58°N, 19.22°E), and Svalbard (78.99°N, 15.99°E). The analysis reveals connections between tidal amplitude anomalies and radiative effects of ozone in the polar regions during SSW events. Additionally, we investigate the response of polar ozone to the May 2024 superstorm using Aura/MLS measurements and MERRA-2 reanalysis data. The results highlight a rapid and significant stratospheric ozone response following the superstorm and provide quantitative insights into the impact of such extreme events on ozone variability and UV radiation. This study underscores the critical role of ozone radiative processes in polar atmospheric dynamics and their modulation by extreme events, including SSWs and solar storms.

How to cite: Shi, G., Liu, H., Kozlovsky, A., Gulbrandsen, N., Pokhotelov, D., Lester, M., Tsutsumi, M., Wu, K., and Stober, G.: Polar ozone anomalies, radiative effects, and their connection to mesospheric tidal dynamics during extreme events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4603, https://doi.org/10.5194/egusphere-egu25-4603, 2025.

EGU25-4750 | ECS | Posters on site | ST3.3

Investigation of Polar Mesospheric Summer Echoes observed with the EISCAT VHF radar 

Ines Seeliger, Devin Huyghebaert, Yoshihiro Yokoyama, and Ingrid Mann

Polar mesospheric summer echoes (PMSE) are strong radar echoes that can be observed in the mesosphere. They form at altitudes between 80 and 90 kilometres during summer in high and middle latitudes, when temperatures are low enough for ice particles to form. PMSE come from coherent scattering from irregularities in the electron density and are observed when the spatial structures of the electron density are at half the radar wavelength. It is assumed that ice particles are spatially structured by the neutral air turbulence and that via their surface charge they influence the electron density. The formation of PMSE depends on atmospheric characteristics such as turbulence, electron density and electron diffusivity. The size and lifetime of the ice particles which are involved in the formation of PMSE vary with height.

We investigate the properties of PMSE using selected data of EISCAT VHF observations made between 2010 and 2021. The observations were made using the Manda experiment, which is suitable for observing the mesosphere and the lower ionosphere; the observations have a time resolution of several seconds. The EISCAT real-time graphics software is used to determine the spectra at altitudes of 80-90 km.

Using a Gaussian fit, we determine the spectral width, Doppler shift and received echo strength and use thresholds for these parameters to classify PMSE. We present an analysis of these properties, their variation with the height, the characteristics of gravity waves seen in PMSE, and the correlation between spectral width and amplitude.

How to cite: Seeliger, I., Huyghebaert, D., Yokoyama, Y., and Mann, I.: Investigation of Polar Mesospheric Summer Echoes observed with the EISCAT VHF radar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4750, https://doi.org/10.5194/egusphere-egu25-4750, 2025.

EGU25-5252 | Orals | ST3.3

Climatology of Mesosphere and Lower Thermosphere Residual Circulations and Mesopause Height Derived From NASA TIMED/SABER Observations  

Liying Qian, Ningchao Wang, Jia Yue, Wenbin Wang, Martin Mlynczak, and James Russell III

In the mesosphere and lower thermosphere (MLT) region, residual circulations driven by gravity wave and tidal breaking/dissipation significantly impact constituent distribution and the height and temperature of the mesopause.  Distributions of CO2 can be used as a proxy for the residual circulations. NASA TIMED Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) CO2 volume mixing ratio (VMR) and temperature measurements from 2003 to 2020 are used to study the monthly climatology of MLT residual circulations and mesopause heights. Our analyses show that (a) mesopause height strongly correlates with the CO2 VMR vertical gradient during solstices; (b) mesopause height has a discontinuity at midlatitude in the summer hemisphere, with a lower mesopause height at mid-to-high latitudes as a result of adiabatic cooling driven by strong adiabatic upwelling; (c) residual circulations have strong seasonal variations at mid- to high latitudes, but they are more uniform at low latitudes; and (d) the interannual variability of the residual circulations and mesopause heights is larger in the Southern Hemisphere (SH; 4–5 km) than in the Northern Hemisphere (NH; 0.5–1 km).

How to cite: Qian, L., Wang, N., Yue, J., Wang, W., Mlynczak, M., and Russell III, J.: Climatology of Mesosphere and Lower Thermosphere Residual Circulations and Mesopause Height Derived From NASA TIMED/SABER Observations , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5252, https://doi.org/10.5194/egusphere-egu25-5252, 2025.

EGU25-5564 | Orals | ST3.3

CMIP7 solar forcing – evaluation of solar impacts with UA-ICON 

Markus Kunze, Miriam Sinnhuber, Alexander Siebelts, Astrid Kerkweg, Kerstin Hartung, Bastian Kern, and Patrick Jöckel

The ICOsahedral Non-hydrostatic model (ICON) framework is the open-source numerical weather prediction and climate model jointly developed by the German Weather Service (DWD), the Max-Planck Institute of Meteorology (MPI-M), Deutsches Klimarechenzentrum (DKRZ), the Karlsruhe Institute of Technology (KIT), and the Center for Climate Systems Modeling (C2SM). A consolidated climate setup with interactive ocean, land surface and atmosphere is being developed and tested. However, while ICON's basic setup includes monthly varying solar TSI and SSI forcing, the ability to prescribe higher-frequency UV irradiances and energetic particle precipitation (EPP) to change atmospheric composition has not been considered.

The upper atmosphere extension of ICON (UA-ICON) is currently a modelling framework allowing the analysis of dynamic phenomena from the ground to the lower thermosphere (150 km). Implementing varying solar forcing and interactive chemistry is expected to hugely influence the thermal structure and composition in the mesosphere/lower thermosphere (MLT).

Updated historical forcing datasets for the 7th phase of the Coupled Model Intercomparison Project (CMIP7) are now available for evaluation. These include daily varying spectral solar irradiance (SSI), total solar irradiance (TSI), and ion pair production rates for solar protons, cosmic rays, and medium-energy electrons to model EPP. Implementing these solar forcing data and the interactive chemistry is still ongoing work, and we present the first results of this effort, focusing on the MLT and UA-ICON.

How to cite: Kunze, M., Sinnhuber, M., Siebelts, A., Kerkweg, A., Hartung, K., Kern, B., and Jöckel, P.: CMIP7 solar forcing – evaluation of solar impacts with UA-ICON, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5564, https://doi.org/10.5194/egusphere-egu25-5564, 2025.

EGU25-6290 | Posters on site | ST3.3

Statistical analysis of Multistatic meteor radar observations 

Gunter Stober, Alan Liu, Alexander Kozlovsky, Diego Janches, Erin Dawkins, Loretta Pearl Poku, Zichun Qiao, Masaki Tsutsumi, Mark Lester, Njål Gulbrandsen, Satonori Nozawa, Johan Kero, Tracy Moffat-Griffin, and Nicholas Mitchell

Multistatic meteor radar networks have become a valuable tool to study the spatial and temporal variability of mesosphere/lower thermosphere winds. Combined with advanced and tomographic analysis such as the 3DVAR+DIV or VVP algorithm it is possible to infer spectral information related to the horizontal wavelength and the temporal spectrum. Here we present a statistical analysis of almost 5 years of observations recorded with the Nordic Meteor Radar Cluster and CONDOR. Our initial results show a seasonal variability of the spectral slopes for different spatial scales indicating a reduced gravity wave activity during the spring for the Northern hemispheric data. Furthermore, we find a transition from a k-3 to a k-5/3 slope for spatial scales around 150 kilometers. Zonal wavelength spectra at CONDOR exhibit a less clear seasonal pattern compared to the Nordic Meteor Radar Cluster.   

How to cite: Stober, G., Liu, A., Kozlovsky, A., Janches, D., Dawkins, E., Pearl Poku, L., Qiao, Z., Tsutsumi, M., Lester, M., Gulbrandsen, N., Nozawa, S., Kero, J., Moffat-Griffin, T., and Mitchell, N.: Statistical analysis of Multistatic meteor radar observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6290, https://doi.org/10.5194/egusphere-egu25-6290, 2025.

EGU25-7102 | Orals | ST3.3

Studies to Resolve a Persistent Upper Atmospheric Mystery 

Alexander Kutepov, Artem Feofilov, Ladislav Rezac, and Konstantinos Kalogerakis

The year 2025 marks the 55th anniversary of Paul Crutzen’s brilliant hypothesis that collisions of the carbon dioxide molecules with oxygen atoms is the dominant process responsible for excitation of the bending vibrational mode of carbon dioxide and, thus, the resulting 15-µm infrared (IR) emission from vibrationally excited CO2 provides a remote sensing window into the temperature profiles, energy budget, and thermal balance of the upper atmosphere. The O + CO2 problem has remained open for the past five decades due to unacceptably large discrepancies between the laboratory measurements of the rate constant for this process, its values retrieved from space-based observations, and the rate constant values used in general circulation models (GCMs) for estimating CO2 cooling of the mesosphere and lower thermosphere (MLT).

 

We have been actively engaged in research efforts to address this problem by revisiting its different aspects, including theoretical analysis, atmospheric modeling, and laboratory experiments investigating the processes leading to the generation of the 15-µm emission in the Earth’s MLT region. This report discusses our recent progress on this topic. We will present non-local thermodynamic equilibrium (non-LTE) modeling calculations on the MLT 15-µm cooling using our recently published, optimized version of the Accelerated Lambda Iteration for Atmospheric Radiation and Molecular Spectra (ALI-ARMS) research code [Kutepov and Feofilov, 2024]. Detailed comparisons of these results with the parameterizations of this cooling used in GCMs and remote sensing by space-based observations will be discussed.

 

This research is supported by grants from the US National Science Foundation (AGS-2312191/92, AGS-2125760) and NASA (80NSSC21K0664).

 

References

Kutepov, A. and Feofilov, A., 2024. New routine NLTE15µmCool-E v1. 0 for calculating the non-local thermodynamic equilibrium (non-LTE) CO2 15 µm cooling in general circulation models (GCMs) of Earth’s atmosphere. Geoscientific Model Development, 17(13), 5331-5347.

How to cite: Kutepov, A., Feofilov, A., Rezac, L., and Kalogerakis, K.: Studies to Resolve a Persistent Upper Atmospheric Mystery, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7102, https://doi.org/10.5194/egusphere-egu25-7102, 2025.

We present analysis of the chemical and dynamical variability in the mesosphere and lower thermosphere (MLT) during the 2018-2019 sudden stratospheric warming (SSW) as simulated by the high resolution (~25 km horizontal and 0.1 scale height vertical resolution) version of the Whole Atmosphere Community Climate Model with thermosphere-ionosphere eXtension (WACCM-X). The WACCM-X simulations make use of new capabilities, including the spectral element dynamical core and the ability to constrain the lower atmosphere meteorology in WACCM-X at high-resolutions. Compared to standard resolution (~200 km horizontal and 0.25 scale height vertical resolution) WACCM-X simulations, the high-resolution simulations are in better agreement with Thermosphere Ionosphere Mesosphere Energetics Dynamics-Sounding of the Atmosphere using Broadband Emission Radiometry (TIMED-SABER) and Atmosphere Chemistry Experiment-Fourier Transform Spectrometer (ACE-FTS) observations. In particular, the high-resolution simulations better reproduce the Northern Hemisphere middle-high latitude winds in the MLT. The downward transport of nitric oxide (NO) following the SSW is also better reproduced in the high-resolution simulations. The results demonstrate the importance of capturing mesoscale processes for accurately simulating the chemistry and dynamics of the MLT.      

How to cite: Pedatella, N., Harvey, V. L., Liu, H., and Datta-Barua, S.: High resolution simulations of the chemistry and dynamics in the mesosphere and lower thermosphere during the 2018-2019 sudden stratosphere warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7273, https://doi.org/10.5194/egusphere-egu25-7273, 2025.

EGU25-7418 | Orals | ST3.3

Climatologies of MLT winds and waves retrieved from long-term radar observations and GCMs 

Dimitry Pokhotelov, Gunter Stober, Ales Kuchar, Huixin Liu, Han-Li Liu, and Christoph Jacobi

Long-term observations of mesospheric-lower thermospheric winds from six meteor radars located at middle and polar latitudes in both hemispheres, covering two recent solar cycles, are analysed to construct climatologies of atmospheric tides and gravity waves (GWs). The obtained climatologies of diurnal and semidiurnal tides and GWs are compared to numerical simulations using three general circulation models (GCMs), namely the Ground-to-topside model of Atmosphere and Ionosphere for Aeronomy (GAIA), the Whole Atmosphere Community Climate Model eXtension - Specified Dynamics (WACCM-X-SD), and the Upper Atmosphere ICOsahedral Non-hydrostatic (UA-ICON) model. Despite of generally good agreement with radar observations, there are substantial differences between the GCMs in reproducing key features of the MLT dynamics, e.g., the hemispheric zonal summer wind reversal. The differences are attributed in particular to sub-grid parameterisations of GWs in GCMs.

How to cite: Pokhotelov, D., Stober, G., Kuchar, A., Liu, H., Liu, H.-L., and Jacobi, C.: Climatologies of MLT winds and waves retrieved from long-term radar observations and GCMs, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7418, https://doi.org/10.5194/egusphere-egu25-7418, 2025.

EGU25-7659 | Orals | ST3.3

Effects of nonmigrating diurnal tides on the Na layer in the mesosphere and lower thermosphere 

Jianfei Wu, Wuhu Feng, Xianghui Xue, Daniel Marsh, and John Plane

Neutral metal layers such as Na, Mg, and Fe occur in the Earth's mesosphere and lower thermosphere (80-120 km) region due to the ablation of cosmic dust. These layers provide important tracers of chemical and dynamical processes within this region. Nonmigrating diurnal tides are persistent global oscillations in atmospheric fields (e.g., wind, temperature, and density) with a period of 24 hours and nonsynchronous propagation with the sun. A complex combination of tidal forcing, chemistry, and photochemistry drives the diurnal cycle of these meteoric atoms. However, the mechanism behind their diurnal variation is not yet fully understood.

The influence of nonmigrating diurnal tides on Na layer variability in the mesosphere and lower thermosphere regions is investigated for the first time using data from the Optical Spectrograph and InfraRed Imaging System (OSIRIS) on the Odin satellite and Specified Dynamics Whole Atmosphere Community Climate Model (SD-WACCM) with metal chemistry. The Na density from OSIRIS exhibits a clear longitudinal variation indicative of the presence of tidal components. Similar variability is seen in the SD-WACCM result. Analysis shows a significant relationship between the nonmigrating diurnal tides in Na density and the corresponding temperature tidal signal. Below 90 km, the three nonmigrating diurnal tidal components in Na density show a significant positive correlation with the temperature tides. Conversely, the phase mainly indicates a negative correlation above 95 km. Around the metal layer peak, the response of the Na density to a 1 K change in tidal temperature is estimated to be 120 cm−3.

How to cite: Wu, J., Feng, W., Xue, X., Marsh, D., and Plane, J.: Effects of nonmigrating diurnal tides on the Na layer in the mesosphere and lower thermosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7659, https://doi.org/10.5194/egusphere-egu25-7659, 2025.

EGU25-8365 | ECS | Posters on site | ST3.3

Comparison of Volume Velocity Processing (VVP) and 3DVAR+DIV Algorithms for Deriving 3D Wind Fields in the Mesosphere and Lower Thermosphere  with Meteor Radar Observations.  

Loretta Pearl Poku, Gunter Stober, Alan Liu, Alexandre Kozlovski, Diego Janches, Erin Dawkins, Zishun Qiao, Masaki Tsutsumi, Njål Gulbrandsen, Satonori Nozawa, Mark Lester, Johan Kero, Nicholas Mitchell, and Tracy Moffat-Griffin

Accurate estimation of three-dimensional wind fields in the mesosphere and lower thermosphere (MLT) is crucial for understanding atmospheric dynamics and variability, however, it has been a longstanding challenge in atmospheric science. Particularly, the retrieval of vertical wind, due to the inherent biases in meteor radar observations resulting from geometric and observational limitations. This challenge has to be addressed as the vertical wind plays a key role in the dynamical processes in the global atmosphere, such as the vertical transport of momentum and energy which incorporates the global meridional circulation. Volume Velocity Processing (VVP) and the 3DVar+DIV algorithms are two advanced retrieval methodologies which have been applied to estimate vertical winds and their variabilities, mitigating the biases and improving the accuracy of wind estimations. These approaches have recently demonstrated significant progress in overcoming the longstanding challenge.
The VVP method derives three-dimensional winds by employing coordinate transformations and nonlinear constraints on the observed radial velocities of the meteor radars. Its design is emphasized on high spatial resolution, making it particularly effective for localized studies of wind variability. The 3DVAR+DIV algorithm integrates radial velocity data into a variational framework that minimizes a cost function while adhering to physical constraints such as the continuity equation. This approach ensures a physically consistent wind field and allows for the calculation of additional atmospheric diagnostics, including horizontal divergence and vorticity. While both methods provide robust solutions for addressing vertical wind biases, their respective implementations capabilities offer unique advantages.
This study seeks to compares these two cutting-edge methodologies; VVP and the 3D-Var+DIV algorithms using data the Nordic Meteor Radar Cluster (NORDIC), a dense multistatic radar network in the Northern Hemisphere, to uncover their ability to estimate 3D wind fields and mitigate vertical wind biases in MLT as well as their potential in advancing understanding of atmospheric dynamics. Algorithm implementation and testing are being conducted to ensure both methods operate optimally within the same dataset, enabling a fair and direct comparison. Key aspects of the comparison will include vertical wind retrieval accuracy, spatial resolution, diagnostic capabilities, and computational efficiency. The anticipated outcomes of this study will provide valuable insights into the relative strengths and weaknesses of the VVP and 3DVAR+DIV methods. While the VVP method is expected to excel in capturing spatially detailed wind patterns, the 3DVAR+DIV algorithm may offer enhanced physical consistency and diagnostic functionality. This study aims to contribute to advancing retrieval techniques and enhance the accuracy of atmospheric models and improve our understanding of MLT dynamics. Such advancements are crucial for refining predictions of global weather and climate systems, particularly in the context of long-term atmospheric monitoring and modeling.

How to cite: Poku, L. P., Stober, G., Liu, A., Kozlovski, A., Janches, D., Dawkins, E., Qiao, Z., Tsutsumi, M., Gulbrandsen, N., Nozawa, S., Lester, M., Kero, J., Mitchell, N., and Moffat-Griffin, T.: Comparison of Volume Velocity Processing (VVP) and 3DVAR+DIV Algorithms for Deriving 3D Wind Fields in the Mesosphere and Lower Thermosphere  with Meteor Radar Observations. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8365, https://doi.org/10.5194/egusphere-egu25-8365, 2025.

EGU25-10859 | Posters on site | ST3.3

Recent observations of Lithium atoms in the middle atmosphere by lidar 

Michael Gerding, Robin Wing, Josef Höffner, Jan Froh, and Gerd Baumgarten

Ablating meteoroids form a well-known layer of metal atoms in the middle atmosphere between about 80 km and more than 100 km altitude. Some of these metals, like sodium, iron, potassium, or calcium, have been observed for decades by lidar. They are now often used for resonance lidar measurements of temperature and winds or as tracers of the middle atmosphere dynamics and the coupling with the ionosphere. Atomic lithium has rarely been observed so far because the natural abundance is very low, as is the lidar backscatter signal. Early observations in the late 1970s above southern France revealed a number density of only a few atoms per cubic centimeter, but have been suspended about 45 years ago. While lithium has a low abundance in meteoroids, it has a much higher share in space debris, i.e. satellites and upper rocket stages re-entering into the atmosphere. This makes lithium an important target for space-debris research in the mesosphere / lower thermosphere. We have set up a Li resonance lidar in 2024 at our site at Kühlungsborn/Germany (54°N, 21°E). We will show first results on the atomic Li abundance in the middle atmosphere after a 45-year observational gap, including some record-high concentrations, and describe our new lidar for regular Li monitoring.

How to cite: Gerding, M., Wing, R., Höffner, J., Froh, J., and Baumgarten, G.: Recent observations of Lithium atoms in the middle atmosphere by lidar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10859, https://doi.org/10.5194/egusphere-egu25-10859, 2025.

EGU25-11190 | Orals | ST3.3

The Impact of Geomagnetic Storms on Antarctic Stratospheric Ozone: Modelling Study Based on the WACCM-D  

Shujie Chang, Zhenfeng Chen, John M.C.Plane, Martyn P.Chipperfield, Daniel R.Marsh, Wuhu Feng, and Yuanzi Zhang

Geomagnetic storms can lead to energetic particle precipitation (EPP), which increase ionization levels in the atmosphere, enhancing NOx/HOx concentrations, thus destroying ozone in the polar mesosphere and stratosphere. There has been many studies to study the impact of solar proton on ozone, but the contributions of solar proton and energetic electron precipitation under different space weather especially geomagnetic storms events to the changes in middle/upper atmospheric in different seasons are not well quantified. It is also important to study long term changes in ozone due to solar activities including geomagnetic storms to understand how they affect global climate and atmospheric chemical processes.

In this work, we have carried out long term simulations (1980-2019) using the Whole Atmosphere Community Climate Model (WACCM), with detailed D-region (60-90 km) chemistry. The model uses a specific-dynamic version with nudging of Modern-Era Retrospective analysis for Research and Applications (MERRA-2) reanalysis. First, we have made comprehensive model validations using various satellite measurements, which shows the model with detailed D region ion-nuetral chemistry has better performance in reproducing some key neutral chemical species (e.g., NOx, HOx, HNO3 etc) affected by EPP. In order to highlight how different geomagnetic storms events (strong or quite conditions) affected stratospheric ozone in different seasons, we use a composite analysis method. Interestingly, The ozone loss is more noticeable in summer than in winter. Surprisingly, ozone changes usually become more noticeable after one month. To investigate the impact of medium energy electron (MEE, 30-1000 keV) precipitation on the middle and upper atmosphere, several model sensitivity experiments have been made. Results shows MEE has a significant impact in the mesosphere with small contribution to stratosphere ozone depletion (2-5% in the Antarctic winter).

How to cite: Chang, S., Chen, Z., M.C.Plane, J., P.Chipperfield, M., R.Marsh, D., Feng, W., and Zhang, Y.: The Impact of Geomagnetic Storms on Antarctic Stratospheric Ozone: Modelling Study Based on the WACCM-D , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11190, https://doi.org/10.5194/egusphere-egu25-11190, 2025.

EGU25-11666 | Orals | ST3.3

EPP-climate link by reactive nitrogen polar winter descent: Science studies for the EE11 candidate mission CAIRT 

Stefan Bender, Bernd Funke, Manuel Lopez Puertas, Maya Garcia-Comas, Gabriele Stiller, Thomas von Clarmann, Michael Höpfner, Björn-Martin Sinnhuber, Miriam Sinnhuber, Quentin Errera, Gabriele Poli, Jörn Ungermann, Peter Preusse, Sebastian Rhode, Hanli Liu, and Nick Pedatella

Polar winter descent of NOy produced by energetic particle precipitation (EPP) in the mesosphere and lower thermosphere affects polar stratospheric ozone by catalytic reactions. This, in turn, may affect regional climate via radiative and dynamical feedbacks. NOy observations by MIPAS/Envisat during 2002--2012 have provided observational constraints on the solar-activity modulated variability of stratospheric EPP-NOy.

ESA’s Earth Explorer 11 candidate Changing Atmosphere Infra-Red Tomography (CAIRT) will observe the atmosphere from about 5 to 115 km with an across-track resolution of 30 to 50 km within a 500 km wide field of view. CAIRT will provide NOy and tracer observations from the upper troposphere to the lower thermosphere with unprecedented spatial resolution. We present the science studies using WACCM-X high resolution model runs simulating modelling a Sudden Stratospheric Warming event to assess its potential to advance our understanding of the EPP-climate link and to improve upon the aforementioned constraints in the future.

How to cite: Bender, S., Funke, B., Lopez Puertas, M., Garcia-Comas, M., Stiller, G., von Clarmann, T., Höpfner, M., Sinnhuber, B.-M., Sinnhuber, M., Errera, Q., Poli, G., Ungermann, J., Preusse, P., Rhode, S., Liu, H., and Pedatella, N.: EPP-climate link by reactive nitrogen polar winter descent: Science studies for the EE11 candidate mission CAIRT, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11666, https://doi.org/10.5194/egusphere-egu25-11666, 2025.

EGU25-12527 | ECS | Posters on site | ST3.3

Decadal Trends of Non-Migrating Eastward-Propagating Diurnal Tides in the MLT Region  

Sovit Khadka, Federico Gasperini, and Hanli Liu

Vertically propagating tides and other waves of tropospheric origin are leading drivers of long-term variability and dynamical coupling in the ionosphere-thermosphere-mesosphere (ITM) system. This study explores the decadal trends, variability, and coupling of the dominant non-migrating eastward-propagating diurnal (DE) tides in the mesosphere and lower thermosphere (MLT) region. The non-migrating tides are excited by differential solar heating, deep tropospheric convection over the tropics releasing latent heat, and nonlinear interactions between migrating tides and planetary-scale waves. These tides are important for understanding the complex interplay between upward-propagating waves of lower atmospheric origin and the coupling between terrestrial weather and space weather across different atmospheric layers on various timescales.

Utilizing long-term temperature observations from the Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) in the MLT region, and simulated results from the Whole Atmosphere Community Climate Model with Thermosphere and Ionosphere Extension (WACCM-X), we identify decadal trends in DE tidal amplitudes and phases over the past 22 years (2002-2023). During the course of vertical propagation, the competing role of DE tides in the modulation of the E-region dynamo will be examined, which ultimately impacts the space weather of the ionosphere. This analysis also evaluates the impacts of the solar cycle (SC), quasi-biennial oscillation (QBO), semiannual oscillations (SAO), and El Niño–Southern Oscillation (ENSO) on non-migrating diurnal tides. The observed trends are further examined in the context of simulation results from WACCM-X to understand the physical mechanisms that transmit long-term variability from the lower atmosphere into the ITM system. This study emphasizes the importance of understanding long-term trends in tidal waves to advance knowledge of the interconnections between terrestrial and space weather processes across different spatial and temporal scales and for improving predictive models of upper atmospheric conditions, which are crucial for mitigating space weather impacts on modern technologies.

How to cite: Khadka, S., Gasperini, F., and Liu, H.: Decadal Trends of Non-Migrating Eastward-Propagating Diurnal Tides in the MLT Region , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12527, https://doi.org/10.5194/egusphere-egu25-12527, 2025.

EGU25-13155 | ECS | Posters on site | ST3.3

High-resolution Analysis of Evolving Mesospheric KHI at Poker Flat 

Jessica Norrell, Katrina Bossert, Jessica Berkheimer, Richard L Collins, and Jintai Li

The dynamics of the mesopause and lower thermosphere region are vital to understanding the transition from gravity wave breaking to the generation of turbulence, higher order waves, and instabilities. However, these features are unresolved in global-scale models. We present a case study of small-scale gravity waves and kelvin Helmholtz instabilities using ground-based instruments, which include the collocated sodium resonance lidar and hydroxyl imager at the Poker Flat Research Range. These observations provide insight into gravity wave and instability interaction and evolution. The combination of data from both instruments is used to develop a three-dimensional understanding of wave packets on 31 March 2022. 

How to cite: Norrell, J., Bossert, K., Berkheimer, J., Collins, R. L., and Li, J.: High-resolution Analysis of Evolving Mesospheric KHI at Poker Flat, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13155, https://doi.org/10.5194/egusphere-egu25-13155, 2025.

EGU25-13463 | ECS | Posters on site | ST3.3

Vertical Gravity Wave Coupling Combining Ground and Satellite Based Measurements 

Sophie Phillips and Katrina Bossert

Gravity waves are influential drivers of the ionosphere-thermosphere (I-T) region. Gravity waves perturb background neutral and ion densities, temperatures, and winds. The dissipation of gravity waves in this region also leads to drag on background winds, altering the mean wind and circulation. There remain limited capabilities for measurements in the lower thermosphere despite the important role that gravity waves play in the dynamics of this region. Additionally, understanding sources of gravity waves in the thermosphere is important for improving thermospheric models. This study seeks to investigate wave coupling from the stratosphere to the I-T region over Alaska by combining both ground and satellite-based data sources. The Scanning Doppler Imager in Poker Flat Research Range (-147W, 65N) obtains zonal and meridional wind speeds in the red line emission, 630.0nm, which occurs near 250km in altitude. The Atmospheric Infrared Sounder uses 4.3-micron CO2 emissions to derive brightness temperature perturbations in the stratosphere. The Poker Flat Incoherent Scatter Radar provides information regarding gravity wave associated travelling ionospheric disturbances in altitude and time. We use wavelet analysis to acquire wave information in the different atmospheric regions, and determine gravity wave propagation conditions in the stratosphere and mesosphere using MERRA-2 reanalysis data to further determine gravity wave sources. 

How to cite: Phillips, S. and Bossert, K.: Vertical Gravity Wave Coupling Combining Ground and Satellite Based Measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13463, https://doi.org/10.5194/egusphere-egu25-13463, 2025.

EGU25-13733 | Posters on site | ST3.3

ICON/MIGHTI as a Nightglow Probe of the Atomic Oxygen Green Line 

Konstantinos S. Kalogerakis, Daniel Matsiev, and Stefan Noll

The objective of the Michelson Interferometer for Global High-Resolution Thermospheric Imaging (MIGHTI) instrument aboard NASA’s Ionospheric Connection Explorer (ICON) satellite was to determine altitude profiles of the wind and temperature in the Earth’s upper atmosphere [1]. The winds were obtained from the Doppler shift of the measured atomic oxygen green and red line emissions at 557.7 nm and 630.0 nm [2], respectively, and the temperatures derived from the measured molecular oxygen Atmospheric band emission [3].

Our study aims to broaden the scientific impact of the MIGHTI instrument, advance knowledge of the nightglow emissions, and improve retrievals of nighttime atomic oxygen by using the intensities of the emissions measured by MIGHTI. Accurate nighttime O-atom densities are required for modeling the chemistry and energy budget of the upper atmosphere. Just as important, a detailed understanding of the relationship between atmospheric composition and the intensity of observed nightglow emissions is essential for modeling and understanding gravity wave propagation and dissipation.

We recently performed a radiometric calibration of the ICON/MIGHTI signals by comparisons with flux-calibrated astronomical sky spectra. This report will describe our efforts to investigate the calibrated 557.7-nm atomic oxygen green line emission measurements during the ICON/MIGHTI era, characterize its climatology, and determine atomic oxygen profiles.

This work is supported by the NASA GOLD-ICON Guest Investigators Program Grant 80NSSC22K0172 and the NASA Heliophysics (LNAPP) Program Grant 80NSSC23K0694.

[1] Immel et al., Space Sci. Rev. 219(41), 1-26 (2023).

[2] Englert et al., Space Sci. Rev. 219(3), 27 (2023).

[3] Stevens et al., Space Sci. Rev. 218(8), 67 (2022).

How to cite: Kalogerakis, K. S., Matsiev, D., and Noll, S.: ICON/MIGHTI as a Nightglow Probe of the Atomic Oxygen Green Line, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13733, https://doi.org/10.5194/egusphere-egu25-13733, 2025.

EGU25-13773 | ECS | Orals | ST3.3

Observing Mesospheric Gravity Waves with NASA’s AWE Mission and Correlating to GNSS TEC Maps 

Jaime Aguilar Guerrero, Björn Bergsson, Sehin Mesfin, Pavel Inchin, Matthew Zettergren, Ludger Scherliess, Yucheng Zhao, and Dominique Pautet

The Atmosphere Waves Experiment (AWE) is a NASA mission launched on November 9, 2023, and installed on the International Space Station (ISS). Its primary goal is to detect and characterize atmospheric gravity waves (AGWs) by measuring Earth’s mesospheric hydroxyl (OH) airglow with its key instrument, the Advanced Mesospheric Temperature Mapper (AMTM). Since its deployment, AWE has been quantifying the seasonal and regional variability of AGWs, investigating their occurrence and potential sources, and enabling the assessment of their broader impact on the atmosphere by comparing measurements at different altitudes by other instruments. AWE has collected extensive imagery and temperature data capturing distinct mesospheric phenomena, including mesospheric bores, signatures of a hurricane, and instability- and convection-driven disturbances. These observations are now publicly available for the first several months of the mission. In this work, we compare AWE’s dataset to total electron content (TEC) maps derived from GNSS data processed by the System for Rapid Analysis of Ionospheric Dynamics (S-RAID) (Inchin et al., 2023), which analyzes data from approximately 2,700 stations across the continental United States (CONUS). S-RAID applies common bandpass filters to isolate traveling ionospheric disturbances (TIDs) with periods shorter than two hours. By comparing AWE’s measurements at the approximate OH airglow height of 87 km with the GNSS data at an average ionospheric pierce point (IPP) of 300 km, we identify wave parameters and potentially determine which signatures correspond to upward-propagating gravity waves. These signals, in turn, can be traced back to various tropospheric sources, such as those mentioned above.

How to cite: Aguilar Guerrero, J., Bergsson, B., Mesfin, S., Inchin, P., Zettergren, M., Scherliess, L., Zhao, Y., and Pautet, D.: Observing Mesospheric Gravity Waves with NASA’s AWE Mission and Correlating to GNSS TEC Maps, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13773, https://doi.org/10.5194/egusphere-egu25-13773, 2025.

The underlying physics of the Turbopause, from approximately 80-120 km, remains one of the most poorly understood topics in aeronomy today. However, the composition and dynamics of this region have a profound impact on the local and global climatological behavior of the thermosphere-ionosphere system. A detailed understanding of this region is critical to modern general circulation models and accurately predicting high-altitude weather systems within the mesosphere and lower thermosphere (MLT), which can have a detrimental effect on space and ground-based products. To improve our understanding of the Turbopause we propose the first modern measurements of O, O2 , N2, NO, CO2, H2O, O3, and Ar spanning an altitude of 80 to 120 km. To achieve this, we present the Mass Spectrometry of the Turbopause Region (MSTR) program, a NASA HTIDES-funded technology development effort led by Orion Space Solutions (OSS) in partnership with the Southwest Research Institute (SwRI). MSTR is a novel, compact Cryogenically cooled Time-Of-Flight Mass Spectrometer (CTOF-MS) designed to integrate with a variety of aerospace platforms, including sounding rockets, small satellites, and advanced payloads. The flight prototype has a current SWAP of approximately 61 x 27 x 9 centimeters (volume: ~14800 cm3), 8 kg, and 20 to 25 W. MSTR is capable of sampling both ion and neutral elements and has demonstrated a resolving power at full width, half maximum of better than 3500 (predicted 5000), and a mass capability of 2u to 1500u. For integration with low-altitude sounding rockets, the instrument features an integrated 3D printed, liquid helium subcooled nosecone, to reduce and collapse the impinging bow shock experienced during supersonic flight. The MSTR CTOF-MS and cryogenic nosecone have undergone laboratory characterization and TRL advancement. The scientific objectives of the MSTR instrument are to provide simultaneous, in-situ, measurements of the chemistry and structure of the Turbopause as a function of altitude. The MSTR team plans to operate coincidentally with SABER overflights and ground-based LIDAR measurements to characterize the transport of NO across the Turbopause and compare measured CO2 profiles to those retrieved by remote IR radiometry. Ultimately, the MSTR instrument hopes to improve our understanding of the complex temporal-spatial dynamics of the Turbopuase and MLT and provide valuable data to validate global circulation models.

How to cite: Anderson, L., Miller, G., Blase, R., and Fish, C.: In-Situ Sounding of the Chemistry and Dynamics of the Turbopause: The Development of a Novel Cryogenic Time-Of-Flight Mass Spectrometer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13929, https://doi.org/10.5194/egusphere-egu25-13929, 2025.

EGU25-14547 | Posters on site | ST3.3

Nonlinear Interactions of Mesospheric Planetary-Scale Waves: Seasonal Variations and Association with Sudden Stratospheric Warmings 

Maosheng He, Jeffrey M. Forbes, Gunter Stober, Christoph Jacobi, Guozhu Li, Libo Liu, and Jiyao Xu

This study utilizes meteor radar observations gathered over nine years at two longitudes and 52°N latitude to explore planetary-scale waves in mesospheric winds. By analyzing zonal wavenumbers across various time scales—specifically multi-day, near-24-hour, 12-hour, and 8-hour periods—we were able to distinguish normal modes (NMs) from other planetary waves (PWs), identify migrating and non-migrating tides, and uncover a range of novel nonlinear interactions.

Our statistical analysis revealed that multi-day oscillations were predominantly associated with NMs, which exhibit distinct seasonality in both period and wavenumber, and show a statistical correlation with sudden stratospheric warmings (SSWs). Notably, April featured a prominent 6-day NM (zonal wavenumber 1), followed by a dominance of 4- and 2-day NMs (wavenumbers 2 and 3, respectively) through June. From July to October, we observed peaks in 2-, 4-, and 6-day NMs (zonal wavenumbers 3, 2, and 1, respectively).

Our insights into seasonal variations are based on observational determinations of frequency and zonal wavenumber, in contrast to satellite observations that often use fixed frequencies and wavenumbers to fit individual waves. The statistical link between NMs and SSWs provides significant input to the ongoing debate on this topic. Additionally, for the first time, we identified frequency and zonal wavenumber matching in over ten secondary waves resulting from nonlinear interactions among NMs (16-, 10-, and 6-day), tides (diurnal, semidiurnal, and terdiurnal, both migrating and non-migrating), and stationary planetary waves (SPWs).

Among these interactions, three novel categories were identified: (1) interactions between terdiurnal tides and planetary waves, (2) interactions between stationary and traveling planetary waves, and (3) interactions between non-migrating tides and planetary waves. These interactions with SPWs help explain our finding that the amplitudes of non-migrating tides exceed those of the corresponding migrating tides, particularly evident in the winter diurnal tide and the summer terdiurnal tide. These non-migrating signatures stand out as notable exceptions, as migrating components generally dominate diurnal, semidiurnal, and terdiurnal tides throughout most of the year.

How to cite: He, M., Forbes, J. M., Stober, G., Jacobi, C., Li, G., Liu, L., and Xu, J.: Nonlinear Interactions of Mesospheric Planetary-Scale Waves: Seasonal Variations and Association with Sudden Stratospheric Warmings, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14547, https://doi.org/10.5194/egusphere-egu25-14547, 2025.

EGU25-14797 | Orals | ST3.3

The Atmospheric Waves Experiment (AWE) 

Ludger Scherliess, Mike Taylor, P.-Dominique Pautet, Yucheng Zhao, Burt Lamborn, Harri Latvakoski, Greg Cantwell, Pedro Sevilla, Erik Syrstad, Jeff Forbes, Steve Eckermann, Dave Fritts, Diego Janches, Hanli Liu, and Jonathan Snively

NASA’s Atmospheric Waves Experiment (AWE) mission is a Heliophysics Small Explorers Mission of Opportunity designed to investigate how terrestrial weather affects space weather, via small-scale atmospheric gravity waves (AGWs) produced in Earth’s atmosphere. Following its launch to the International Space Station (ISS) in November 2023, AWE began a 2-year mission to explore the global distribution of AGWs, study the processes controlling their propagation throughout the upper atmosphere, and estimate their impacts on the ionosphere – thermosphere – mesosphere (ITM) system. The AWE science instrument consists of the Advanced Mesospheric Temperature Mapper (AMTM) — a wide field-of-view Shortwave Infrared (SWIR) imager that quantifies gravity wave-induced temperature disturbances in the hydroxyl (OH) airglow layer, which lies near the mesopause at ~87 km altitude. The AMTM’s four identical telescopes make continuous nighttime observations of the P1(2) and P1(4) emission lines of the OH (3,1) band and the Q1(1) emission line in the OH (2,0) band, as well as the atmospheric background, from which the OH layer temperature is derived. AWE images are collected once per second, co-added, and processed into temperature swaths using correction algorithms derived from ground calibration test results. Global coverage of the OH layer is provided about every four days, which enables regional and seasonal studies, as well as characterization of AGW ‘hot spots.’ This paper will present an overview of the AWE mission and discuss initial science results.

How to cite: Scherliess, L., Taylor, M., Pautet, P.-D., Zhao, Y., Lamborn, B., Latvakoski, H., Cantwell, G., Sevilla, P., Syrstad, E., Forbes, J., Eckermann, S., Fritts, D., Janches, D., Liu, H., and Snively, J.: The Atmospheric Waves Experiment (AWE), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14797, https://doi.org/10.5194/egusphere-egu25-14797, 2025.

EGU25-15306 | ECS | Orals | ST3.3

From data to discovery: understanding tropical middle stratospheric ozone variability through causal inference 

Evgenia Galytska, Birgit Hassler, Fernando Iglesias-Suarez, Martyn Chipperfield, Sandip Dhomse, Wuhu Feng, Jakob Runge, and Veronika Eyring

Ozone (O3) plays a critical role in the atmosphere by absorbing harmful ultraviolet solar radiation and also shaping the thermal structure and dynamics of the stratosphere. Variability in O3 levels is driven by a complex interplay of factors, including long-term climate change, the abundance of ozone-depleting substances (ODSs), and non-linear interactions between transport and chemical processes. Changes in tropical stratospheric O3 are particularly intricate due to a strong altitude dependence (WMO, 2022). In the tropical middle stratosphere, a region characterized by strong O3 production and loss, during the early 2000s satellite measurements revealed an unexpected decline in O3. Since then, O3 levels in this region have increased again, but the underlying mechanisms driving such variability remain insufficiently understood, highlighting the need to investigate further the processes driving O3 concentrations.

In this study, we show the pivotal role of causal inference in disentangling the complex chemical-dynamical influences on O3 behavior in the narrower region of the tropical (10°S-10°N) middle (10 hPa) stratosphere. Causal inference can add significant value to traditional statistical methods by inferring causal relationships, distinguishing genuine causal links from spurious correlations, and quantifying their strength. The framework integrates qualitative physical knowledge through a causal graph applied to satellite observations and state-of-the-art 3-D chemical-transport model (CTM) TOMCAT simulations. By leveraging causal inference, we provide robust insights into the drivers of O3 fluctuations and showcase the method’s potential for uncovering causal relationships in stratospheric chemistry-dynamics interactions. To validate this approach, we first construct a simplified toy model that reproduces major chemical-dynamical interactions in tropical middle stratospheric O3 that are based on the NOx (=NO + NO2) catalytic ozone destruction cycle and stratospheric dynamics via stratospheric residual velocity w*. Using this toy model, we demonstrate that causal discovery reproduces the connections between w*, nitrous oxide (N2O), nitrogen dioxide (NO2), and O3 in the tropical middle stratosphere. This successful application establishes a foundation for extending causal effect estimation to observed and modelled chemical processes, including their time lags. We split the periods 2004-2018 into two subperiods (i.e. 2004-2011 when O3 concentrations declined, and 2012-2018 when O3 concentrations increased in the tropical middle stratosphere) to demonstrate differences in the w*-N2O connection that drives distinct O3 behaviors. Additionally, a process-oriented analysis of different Quasibiennial oscillation (QBO) regimes, combined with bootstrap aggregation, reveals robust patterns in chemical-dynamical interactions. These results highlight the potential of causal inference as a transformative tool for advancing our understanding of stratospheric O3 variability and its response to dynamic forcing.

World Meteorological Organization (WMO). Scientific Assessment of Ozone Depletion: 2022, GAW Report No. 278, 509 pp.; WMO: Geneva, 2022.

How to cite: Galytska, E., Hassler, B., Iglesias-Suarez, F., Chipperfield, M., Dhomse, S., Feng, W., Runge, J., and Eyring, V.: From data to discovery: understanding tropical middle stratospheric ozone variability through causal inference, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15306, https://doi.org/10.5194/egusphere-egu25-15306, 2025.

EGU25-16063 | ECS | Orals | ST3.3

Analyzing the MLT region with mass spectrometers 

Rico Fausch, Audrey Vorburger, and Peter Wurz

The mesosphere and lower thermosphere (MLT) region is a key transition zone between Earth’s lower and upper atmospheres, where energetic processes, wave dynamics, and chemical reactions converge. Understanding the temperature and chemical composition in this region is crucial for interpreting processes at higher altitudes. Despite the MLT’s importance in mediating couplings between the lower and upper atmosphere, direct in-situ measurements are inherently challenging due to the low-density, high-altitude, and high-speed environment. However, recent advances in compact, high-sensitivity mass spectrometers offer novel opportunities to investigate some of the most pressing open questions in MLT research. In this work, we highlight how state-of-the-art mass spectrometry can address uncertainties in key processes governing the composition and temperature of the MLT. We outline how measurements of species such as atomic and molecular oxygen, molecular nitrogen, trace metals from meteoric or anthropogenic sources, and reactive radicals can inform MLT models. Our goal is to provide data that will enable the integration of mass spectrometry findings into a range of models, including regional and global climate models, that incorporate long-term measurements, potentially revealing hidden trends in chemical composition and temperature. Such temperature drifts could be indicative of climate change affecting this region of the atmosphere as well.

How to cite: Fausch, R., Vorburger, A., and Wurz, P.: Analyzing the MLT region with mass spectrometers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16063, https://doi.org/10.5194/egusphere-egu25-16063, 2025.

The influence of solar activity on the coupled magnetosphere-ionosphere-neutral atmosphere system has significant impact on middle atmosphere climate chemistry. It is now considered a driver for influencing the concentration of chemical species such as Nitric Oxide (NO) which can act catalytically to deplete ozone. This is important as its removal in the stratosphere alters the temperature distribution of the atmosphere, leading to major consequences for the environment, such as hindering plant growth and disrupting ecosystems. We present a multi-instrumental study which combines satellite measurements linking the energy transfer from energetic particle precipitation (EPP) into the upper atmosphere to the formation of nitric oxide in the mesosphere via the “direct effect” and stratosphere via the “indirect effect”. The former is characterised by an enhanced and localised stream of NO in the path of the particles traveling through the atmosphere. The “indirect effect” is a secondary enhancement due to the transport of the NO generated by the direct effect into the stratosphere via atmospheric processes such as the residual circulation, zonal winds and the polar vortex.

The study utilises the Solar Occultation For Ice Experiment (SOFIE) dataset, extending the work by Smith-Johnson et al. (2017), to determine the relative change in NO density over the solar cycle from 2008 to 2019. We have also been able to determine the average response of NO within the mesosphere and stratosphere as a result of geomagnetic storms between 2008 and 2014, through application of a Superposed Epoch Analysis. This demonstrates a strong direct feature at the onset of the storms in both hemispheres. However, the indirect response varies, extending lower into the stratosphere in the southern hemisphere than the northern hemisphere. This analysis is complemented by field aligned currents derived by the Active Magnetosphere and Planetary Electrodynamics Response Experiment (AMPERE) to analyse the variability in the NO density following periods of intense geomagnetic activity and associated EPP. This will provide a greater understanding of the energy transfer and coupling mechanisms between the magnetosphere, Mesosphere and Lower thermosphere regions (MLT) and the middle atmosphere and offer insights on the impacts of space weather on Earth’s climate. 

How to cite: Coulson, R., Wright, D., and Milan, S.: Investigating the impact of energetic particle precipitation on middle atmosphere climate chemistry using high altitude measurements of NO in conjunction with AMPERE., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16772, https://doi.org/10.5194/egusphere-egu25-16772, 2025.

EGU25-19358 | ECS | Posters on site | ST3.3

Modelling and validation of small-scale variability of the MLTI using WACCM-RR over Scandinavia 

Marcin Kupilas, Daniel Marsh, Tracy Moffat-Griffin, Corwin Wright, Andrew Kavanagh, John Plane, and Peter Lauritzen

The ability of Earth system models to forecast the behaviour of the mesosphere/lower thermosphere/ionosphere (MLTI) system lags far behind that of other atmospheric regions, hindering prediction capability of the whole atmosphere. A better understanding of the nature and causes of MLTI variability, which is currently poorly understood, can address this problem. In this work we present results from the Whole Atmosphere Community Climate Model with regional refinement (WACCM-RR) which has been employed to resolve what would normally be subgrid-scale gravity waves that give rise to variability on timescales from hours to days and length scales from several to several hundred kilometres. We focus our studies over high-latitude Scandinavia, the most instrumented region on Earth for MLTI studies, where we resolve down to 1/8° horizontal resolution, approximately 14 km, and study small-scale variability of temperature, horizontal/vertical winds, electron density and key atmospheric constituents such as O, NO and O3. The modelled variability is compared to WACCM simulations without regional refinement (global 1° resolution) and observations from instruments over Scandinavia such as EISCAT, NIPR and AMTM. This study will allow us to identify in-situ and external variability drivers and correlate them to local and global processes and coupled interactions between the atmospheric layers. This work is thus a step towards determining predictable variability of small-scale features in the MLTI, pushing beyond current limitations in forecasting the whole atmosphere.

How to cite: Kupilas, M., Marsh, D., Moffat-Griffin, T., Wright, C., Kavanagh, A., Plane, J., and Lauritzen, P.: Modelling and validation of small-scale variability of the MLTI using WACCM-RR over Scandinavia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19358, https://doi.org/10.5194/egusphere-egu25-19358, 2025.

EGU25-20108 | Orals | ST3.3

The Activity of Atmospheric Turbulence in the MLT 

Cunying Xiao

The Mesosphere and Lower Thermosphere (MLT) act as a critical region for the propagation and dissipation of atmospheric waves, such as gravity waves, tides, and planetary waves, playing a significant role in the global atmospheric circulation system. These waves, particularly gravity waves, dissipate and break in the MLT, converting their energy into turbulence and generating localized turbulent structures. The turbulence produced in turn can modulate wave propagation, with part of the dissipated energy potentially re-exciting new waves. Atmospheric turbulence in the MLT significantly influences the transport of energy, momentum, and matter, making it a key mechanism for understanding the coupling across the entire atmospheric system. The studies of MLT atmospheric turbulence can also promote the fine modeling of the middle and upper atmosphere.

By integrating ground-based MF radar observations over (39.4°N, 116.7° E) with TIMED/SABER satellite data, we investigated the variations of atmospheric turbulence energy dissipation rate (ε) and the turbopause, as well as their relationship with atmospheric wave dynamics in the MLT region. Results show that the atmospheric ε is modulated by different periods at different altitudes. The ε is subject to 12 h and 24 h periodic variations. The 12 h periodic variation is more obvious at higher altitudes than the 24 h periodic variation at lower altitudes with the dividing layer at about 90 km. Advanced analysis of turbopause are based on the total wave variations based on SABER/TIMED. We first propose a new method for identifying the wave-turbopause by employing the conservation of energy principle, and introducing an energy index to delineate the turbopause layer’s boundaries. This method defines a set of parameters including the lower boundary height, upper boundary height, turbopause height, and turbopause layer thickness. Applying this method to long-term SABER data over Beijing, we find that the turbopause layer exhibits distinct seasonal and interannual variations. The average heigh of lower boundary is 69 km, and the average heigh of upper boundary is 94 km. Global characteristics of the turbopause layer are provided, which are quite valuable to enhancing our further atmospheric modeling and empirical studies.

How to cite: Xiao, C.: The Activity of Atmospheric Turbulence in the MLT, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20108, https://doi.org/10.5194/egusphere-egu25-20108, 2025.

EGU25-20552 | ECS | Orals | ST3.3

Re-evaluation of inter-annual variability using lidars Temperature extending over several decades of observation 

Pedro Da Costa, Philippe Keckhut, and Alain Hauchecorne

Rayleigh lidars, in particular as part of the NDACC (Network for the Detection of Atmospheric Composition Change) network, have been observing the stratosphere and mesosphere (also known as the 'middle atmosphere' (MA)) with excellent vertical resolution for many years. Data from the lidars at the Observatoire de Haute-Provence (1978-2024), Table Mountain in California (1989-2024), Mauna Loa in Hawaii (2000-2024), Hohenpeissenberg (1987-2024) and Kühlungsborn (2012-2024) in Germany, Rio Grande in Argentina (2017-2024) and Réunion Island (1994-2024) have made it possible to obtain a unique dataset of temperature profiles between 30 and 80 km. This dataset makes it possible to establish a climatology of MA at several latitudes and over several decades.

Seasonal variations are represented by annual and semi-annual sinusoids. The behaviour of the amplitudes is similar at all sites: stable in the stratosphere, a decrease at the stratopause followed by a constant increase in the mesosphere; the opposite is true for the biannual amplitude, with a slight increase followed by stagnation in the mesosphere. The strength of the annual amplitudes measured at mid-latitudes is about 6 K in the stratosphere, with a decrease to 2 K in the stratopause, followed by an increase to 16 K in the mesosphere. These amplitudes are halved at tropical sites.

The temporal extent of the data series also allows us to analyse the response of the atmosphere to variations in solar activity, showing that these can cause variations of up to 3 K. The influence of the QBO (Quasi-Biennial Oscillation) produces variations that can exceed variations of about 1 K. There is also a general cooling of the atmosphere. We also observe a general cooling of the AM, which varies from site to site: for example, Reunion Island records a cooling of up to 3 K/decade in the mesosphere, while the Haute-Provence site measures a cooling of 1.5 K/decade.

These lidars have also been used to validate measurements made by limb observations from space. The main objective of this study is therefore to provide complete climatologies of the middle atmosphere from several points on the globe, in order to ensure continuity between several successive limb targeting missions. The production of temperature profiles from experiments such as GOMOS or OMPS shows that it is possible to obtain excellent precision in the measurement of temperature profiles. As the observations are made at different times of the day, atmospheric tides must also be taken into account.

How to cite: Da Costa, P., Keckhut, P., and Hauchecorne, A.: Re-evaluation of inter-annual variability using lidars Temperature extending over several decades of observation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20552, https://doi.org/10.5194/egusphere-egu25-20552, 2025.

EGU25-2784 | ECS | Orals | AS3.19

Bridging the Scale Gap: Non-Equilibrium Phase Changes in Contrail Formation 

Katharina Tegethoff and Jessie R. Smith

Contrails formed in aircraft exhaust plumes are a significant contributor to aviation’s climate impact; however, the physical processes driving their formation are not yet fully understood. This presentation focuses on advancing our understanding of non-equilibrium phase change phenomena, including homogeneous and heterogeneous condensation, liquid-to-solid transitions, and interphase momentum transfer, which are central to contrail formation. 

The investigation is based on numerical methods of 3D RANS for non-ideal fluid flow and combined with well-established models in the field of steam turbines to describe the formation of a dispersed phase during phase change. Non-equilibrium thermodynamic principles are used to model nucleation and droplet growth, complemented by detailed representations of heterogeneous condensation and ice formation. The resulting approach is applied to simulate the flow behind an aircraft engine under upper tropospheric conditions. While capturing polydispersed size distributions of the dispersed phases and accounting for interphase momentum transfer, it enables a comprehensive investigation of contrail formation processes. 

By assessing the influence of non-equilibrium effects on the validity of established approaches such as the Schmidt-Appleman Criterion, the presented method aims to bridge the gap between atmospheric-scale contrail models and detailed, small-scale physics of engine exhaust flows. In future work, these approaches could be used to explore how engine specifications, operational conditions, and fuel types shape the early stages of contrail formation. 

How to cite: Tegethoff, K. and Smith, J. R.: Bridging the Scale Gap: Non-Equilibrium Phase Changes in Contrail Formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2784, https://doi.org/10.5194/egusphere-egu25-2784, 2025.

EGU25-2948 | Posters on site | AS3.19

WRF Configuration for Prediction of Aircraft-Induced Cirrus Formation 

Bonnie Valant-Weiss, William Deal, J. Eric Klobas, Aaron Swanson, and Bruce Hauss

Northrop Grumman Corporation (NGC), in partnership with NASA’s Jet Propulsion Laboratory (JPL), is developing modeling capabilities for the prediction of Aircraft-Induced Cirrus (AIC) cloud generation by commercial aviation operators. This work is in support of the United States Department of Energy’s (DOE) Advanced Research Projects Agency – Energy (ARPA-E) Predictive Real-time Emissions Technologies Reducing Aircraft Induced Lines in the Sky (PRE-TRAILS) program. Leveraging NGC knowledge and flight test data on contrail prediction and formation, NGC is developing the Contrail Avoidance System (CAS) to prevent the formation of AIC by enabling aircraft to identify and avoid Ice Super Saturated Regions (ISSRs) in real time. The two key components of this work are development of a new instrument, JPL’s Y-band Temperature and Humidity Profiler (YTHP), and prediction of contrail formation and evolution to AIC using a fusion of NGC’s existing Contrail Prediction Model and the Weather Research and Forecasting (WRF) numerical weather prediction model.

YTHP is an aircraft-mounted submillimeter-wave spectroradiometer that will retrieve vertical profiles of atmospheric temperature and moisture in front of an aircraft. As part of the PRE-TRAILS program, we plan 12 flight test missions in which the YTHP sensor and our operational contrail-avoidance tools will be characterized and validated. Ground observers will track the onset and evolution of persistent contrails using photometrically calibrated cameras.

We will use WRF as a cloud-resolving regional model for the spatial domain covering the flight testing of YTHP. Our long-term modeling goals are to develop a method to insert recently created contrails into the WRF simulation to predict the evolution of contrails to persistent cirrus, and to show how assimilation of YTHP profiles improves that prediction capability. These efforts support the project goal of integrating the YTHP sensor onto aircraft, allowing flight crews to proactively respond to ISSR in the flight path minutes prior to the formation of contrails that would otherwise become AIC.

We will present results of our initial modeling work, which is aimed at assessing WRF performance for simulating ISSRs that cause persistent contrails/AIC. Our studies will include comparison of WRF ISSR representation to contrail formation flight test data previously gathered by NGC.  We will also present comparisons of WRF ISSR results with areas of AIC visible in satellite images.

How to cite: Valant-Weiss, B., Deal, W., Klobas, J. E., Swanson, A., and Hauss, B.: WRF Configuration for Prediction of Aircraft-Induced Cirrus Formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2948, https://doi.org/10.5194/egusphere-egu25-2948, 2025.

EGU25-3653 | ECS | Orals | AS3.19

Reducing Climate Impact through Formation Flying: A Refined Approach to Contrail Simulation and Wake Vortex Analysis 

Judith Pauen, Simon Unterstrasser, and Anton Stephan

Given the significant environmental impacts associated with global aviation, this sector must transition towards being more climate-friendly. Emissions from CO2 and NOx contribute substantially to climate change, while contrails also have a high negative impact. The establishment of formation flight configurations involving two or more passenger aircraft can support the reduction of the climate footprint, without the need for revolutionary technological improvements. By retrieving the energy generated from the wake vortex of the leading aircraft, subsequent aircraft experience reduced induced drag, thereby decreasing fuel consumption and emission (e.g., -5% CO2 and  -15% NOx). As a consequence of atmospheric saturation effects, this approach also reduces the impact of contrails, resulting in an overall reduction in climate impact of approximately 25%. 
The evolution of contrails depends on the dynamics of the wake vortices, as the aircraft exhaust and the resulting contrail ice crystals are captured within the wake vortex system and transported downwards. When flying in formation, the wake vortex system of the leading aircraft is affected by the interference with the wing and fuselage of the following aircraft. The complex interaction between the four wake vortex tubes requires a realistic modeling of the wake vortex dynamics behind a formation configuration. However, existing simulations have been limited to idealized scenarios.
To address this limitation, we develop a novel, refined and more realistic initialization method for our early contrail simulations. Firstly, we conduct RANS-LES simulations with two wings flying in formation, followed by the extraction of a velocity field downstream of the second wing. Subsequently, we initialize our early contrail simulations using this velocity field. This approach will be compared with previous analytical methods and with the contrail behavior of individual aircraft to quantify the potential for climate impact mitigation.
The work is performed as part of the EU project GEESE, which aims to demonstrate the operational feasibility of commercial formation flights over the North Atlantic and continental European airspace.

How to cite: Pauen, J., Unterstrasser, S., and Stephan, A.: Reducing Climate Impact through Formation Flying: A Refined Approach to Contrail Simulation and Wake Vortex Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3653, https://doi.org/10.5194/egusphere-egu25-3653, 2025.

EGU25-3698 | ECS | Orals | AS3.19

The potential role of lubrication oil in contrail formation 

Josef Zink, Simon Unterstrasser, and Tina Jurkat-Witschas

Contrail cirrus clouds contribute significantly to the climate impact of aviation. This impact depends non-linearly on the number of ice crystals formed in nascent contrails. For conventional kerosene combustion, ice crystals primarily form on soot particles emitted from the engine. However, in scenarios with reduced or no soot emissions (such as hydrogen combustion) other particles in the exhaust plume become relevant. Lubrication oil is one potential source of such particles.
Modern aircraft engines rely on lubrication systems to cool and lubricate rotating components such as bearings. When lubrication oil escapes into the environment—whether controlled or uncontrolled—it can become a source of volatile ultrafine particles. In the hot exhaust plume, the oil may evaporate and upon cooling of the plume nucleate new particles. Even if only a small amount of oil (on the order of a few milliliters per hour) forms new particles, the oil particle numbers can exceed the soot particle numbers of conventional engines if the resulting particles are only a few nanometers in size.
Although it is unclear to this point in how far this process occurs in the exhaust, this numerical study explores the potential role of oil particles in contrail ice crystal formation. By investigating many different scenarios, we study their activation behavior and importance compared to other ice-forming particles. The findings indicate that oil particles could substantially contribute to ice crystal formation in soot-poor or hydrogen combustion scenarios. While in-situ flight measurements are necessary to evaluate their actual formation, number, and size distribution, the study highlights the need to minimize oil particle emissions in aircraft exhaust as part of the transition to more sustainable aviation technologies.

How to cite: Zink, J., Unterstrasser, S., and Jurkat-Witschas, T.: The potential role of lubrication oil in contrail formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3698, https://doi.org/10.5194/egusphere-egu25-3698, 2025.

EGU25-4258 | ECS | Posters on site | AS3.19

Modeling the impact of aviation fuel hydrogen and sulfur content on contrail properties: insights and implications 

Ziming Wang, Andreas Marsing, Christiane Voigt, Dennis Piontek, Simon Kirschler, Kai Widmaier, and Luca Bugliaro

Contrail cirrus represents the most significant warming component within the total aviation impact on climate, suspected to exceed even the effects of aviation CO2 emissions. It remains to be shown that regulating hydrogen and sulfur content in aviation kerosene could help to reduce the climate impact from CO2 and from contrails, in order to allow for a science-based jet fuel standardization. Hence, this study conducts a model-based scenario analysis of the climate impact of the European fleet in 2019, exploring different levels of aromatic and sulfur reductions in fossil fuel-based kerosene as short-term mitigation measures.

Using the Lagrangian plume model CoCiP within the open-source pycontrails package, we simulate contrail properties and energy forcing (EF) for a reference fleet using Jet-A1 fuel (13.8% hydrogen content) over Europe in 2019. For scenarios with increased hydrogen content (13.8%–15.4%, in 0.2% increments), reductions in non-volatile particulate matter (nvPM) emissions and changes in contrail properties—such as initial ice particle number, persistent contrail formation, age, optical depth, contrail coverage, and EF—are quantified. In parallel, sulfur content scenarios—including high and ultralow levels with increased and reduced soot activation fractions, as well as zero sulfur—are analyzed, to estimate the impact of sulfur-mediated elevated or reduced activation of aerosol into water droplets.

The reference simulations compare well to previous studies. Furthermore, results show that increasing hydrogen content from 13.8% to 15.2% (the theoretical maximum) enhances the potential for persistent contrail formation from 13% by 6%, but reduces nvPM emission index from 1.22 x 1015 kg-1 by 61%, contrail age from 2.37 h by 20%, contrail optical depth from 0.12 by 24%, and contrail cirrus coverage from 0.67% by 34%. This leads to a reduction in total EF by up to by 52%. The high sulfur scenario increases contrail EF by up to 10%, while the ultralow scenario reduces EF by up to 14%. The simulation of the zero-sulfur content scenario represents the potential lower limit and serves as a pre-study for hydrogen combustion. These findings, part of the European Fuel Standard project by the European Union Aviation Safety Agency, demonstrate how improving fuel composition can mitigate aviation climate impact. These results  highlight the potential of hydroprocessed and ultra-low sulfur kerosene as near-term solutions, providing actionable insights and implications for the development of aviation fuel standardization.

How to cite: Wang, Z., Marsing, A., Voigt, C., Piontek, D., Kirschler, S., Widmaier, K., and Bugliaro, L.: Modeling the impact of aviation fuel hydrogen and sulfur content on contrail properties: insights and implications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4258, https://doi.org/10.5194/egusphere-egu25-4258, 2025.

EGU25-4596 | Orals | AS3.19

ContrailBench: evaluating the performance of contrail models 

Kevin McCloskey, Vincent Meijer, Luc Busquin, Jerome Busquin, Denis Vida, Tom Dean, and Scott Geraedts

The development of effective contrail warming mitigation strategies requires the ability to accurately model contrail formation. This is a challenging problem for a number of reasons, including high uncertainty in the humidity data which is a key component of such models. Observational datasets can be used to constrain and improve contrail formation models. Here we present an analysis of existing contrail models on the task of predicting whether a contrail will be observed in a collection of observational datasets (collectively termed 'ContrailBench'). The observational datasets include one based on Ref [1] using automated contrail detections from the GOES-16 satellite and an automated contrail attribution algorithm, another based on Ref [2] which detects contrails using GOES-16 and uses knowledge of the altitude from LIDAR measurements to attribute them to flights, and a third dataset based on Global Meteor Network ground-based camera imagery [3] with automated contrail detection and high-confidence attribution to the flights that formed them. Different downstream applications require different properties from contrail models, so we evaluate the contrail models based on their performance in both ‘high-recall’ mode (which prioritizes identifying all the flights which make contrails) as well as in ‘high-precision’ mode (which prioritizes minimizing the number of flights incorrectly predicted as forming a contrail). We find that models using raw ERA5 weather reanalysis data perform poorly on all metrics, but the use of machine learning to correct the weather data can lead to improvement.

 

[1] A. Sarna et al, “Benchmarking and improving algorithms for attributing satellite-observed contrails to flights”, https://doi.org/10.5194/egusphere-2024-3664

[2] V. Meijer, thesis, “Satellite-based Analysis and Forecast Evaluation of Aviation Contrails”

[3] D. Vida et al, “The Global Meteor Network – Methodology and first results” https://doi.org/10.1093/mnras/stab2008

How to cite: McCloskey, K., Meijer, V., Busquin, L., Busquin, J., Vida, D., Dean, T., and Geraedts, S.: ContrailBench: evaluating the performance of contrail models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4596, https://doi.org/10.5194/egusphere-egu25-4596, 2025.

EGU25-6481 | ECS | Orals | AS3.19

Contrail Cirrus Climate Effects for Hydrogen-Propelled Aircraft 

Susanne Pettersson, Daniel Johansson, and Tomas Grönstedt

Introducing hydrogen as an aviation fuel offers a promising pathway to significantly mitigate the climate impact of the aviation sector. While this transition demands substantial technological advancements and logistical transformations, hydrogen combustion produces zero CO₂ emissions. However, significant uncertainties remain regarding the non-CO₂ effects of hydrogen-powered aviation, particularly the impact of contrails cirrus. For conventional aircraft, contrail cirrus— the later stages of condensation trails—are estimated to exert an effective radiative forcing comparable to that of CO₂ emissions.

This study models contrail cirrus and their radiative forcing associated with hydrogen combustion. Using a theoretical framework for ice particle formation and a modified version of the CoCiP (Contrail Cirrus Prediction) model for contrail development and radiative forcing, we address key uncertainties specific to hydrogen combustion. These uncertainties include fuel burn, which depends on aircraft and engine design, and the characterization of the exhaust. Unlike conventional jet fuel combustion, which relies primarily on soot particles as condensation nuclei, hydrogen exhaust lacks soot, shifting the role of nucleation to entrained ambient aerosols and lubrication oil particles.

First, to address fuel burn variability, we model three tube-and-wing hydrogen-powered aircraft (short-, medium-, and long-range) with 2050 technology assumptions for realistic fuel flow estimates. Second, given the limited availability of empirical data of lubrication oil and the potential to optimize size and quantity in the exhaust through future engine designs, we evaluate the impact of lubrication oil particles on contrail cirrus by varying particle size distributions.

Our results show a consistent reduction in contrail cirrus radiative forcing across all lubrication oil particle size distributions when realistic hydrogen fuel flow is assumed. The largest reductions are observed in cases with larger mean particle radius and smaller variance. These findings provide insights into the potential for hydrogen-powered aviation to reduce the climate impact of contrail cirrus and highlight opportunities to steer engine design for further mitigation.

How to cite: Pettersson, S., Johansson, D., and Grönstedt, T.: Contrail Cirrus Climate Effects for Hydrogen-Propelled Aircraft, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6481, https://doi.org/10.5194/egusphere-egu25-6481, 2025.

EGU25-7019 | Orals | AS3.19

A high-fidelity physics-based approach towards contrail and contrail cirrus persistence and longevity  

Miad Yazdani, Tom Dean, Elli Daw, and Peter deBock

We present a brief outcome of our research with focus on recently developed persistence modeling framework referred to as AP3 “Accuracy Preserving Physics-based Persistence” model. The purpose of this framework is to predict the evolution of contrail to contrail cirrus and cirrus cloud over the course of >12hrs with preserved accuracy from the formation throughout its lifetime. The model captures nucleation of ice on  particles through Gibbs-Free-Energy (GFE)-based classical nucleation theory (CNT) and accounts for particles coating and morphology on their nucleation propensity, which allows a physics-based representation of the dynamics of ice formation and growth post-sublimation. Other features of the model include,  a DNS-based subgrid model for cloud-turbulence interaction, a source-based approach to account the impact of the cloud on surrounding atmospheric flow and a computationally efficient approach to track the cloud in earth-frame. AP3 is the learning machine for the PIML forecaster that is being developed as part of the ARPA-e CONFIRMMS program.

How to cite: Yazdani, M., Dean, T., Daw, E., and deBock, P.: A high-fidelity physics-based approach towards contrail and contrail cirrus persistence and longevity , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7019, https://doi.org/10.5194/egusphere-egu25-7019, 2025.

EGU25-7191 | ECS | Orals | AS3.19

Persistent contrails simulated in 0D models may experience premature evaporation compared to equivalent simulations in 2D models 

Caleb Akhtar Martínez, Sebastian Eastham, and Jerome Jarrett

Observing contrail cirrus from satellites is challenging because of their low optical depth and large coverage. There is hence widespread reliance on contrail models to consider the periods in which contrails are too optically thin to be observable remotely. The lack of observational data for aged contrails means that contrail model validation relies on intercomparison, which is largely still missing in the literature. To address this, we compare CoCiP, the most used contrail model, to APCEMM, a 2D contrail model, under parametrized meteorological conditions. We show that APCEMM contrails persist for much longer than the equivalent CoCiP contrails, that the lifetime optical depth (a proxy for climate impact) in APCEMM is higher than that in CoCiP, and that the sensitivity of the lifetime optical depth to the relative humidity of the ice supersaturated layer is opposite between the models. These observations are explained by considering the contrail evolution in each model: CoCiP only simulates the fallstreak (the period in which the precipitation plume of the contrail has not reached the subsaturated layer), whereas APCEMM simulations exhibit behavior beyond this. Since post-fallstreak behavior has been seen in large eddy simulations and accounts for ~90 % of the APCEMM lifetime optical depth, our findings have significant implications for both global climate predictions and optimized contrail avoidance. Consequently, we call for the development of contrail models using new methodologies and for the increased collection of in situ observational data for aged contrails to robustly validate late lifetime behavior of contrail models.

How to cite: Akhtar Martínez, C., Eastham, S., and Jarrett, J.: Persistent contrails simulated in 0D models may experience premature evaporation compared to equivalent simulations in 2D models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7191, https://doi.org/10.5194/egusphere-egu25-7191, 2025.

EGU25-7230 | ECS | Orals | AS3.19

Evaluating Forecasts for Navigational Contrail Avoidance 

Thomas Dean, Tristan Abbot, Zebediah Engberg, Nick Masson, Roger Teoh, Marc Stettler, and Marc Shapiro

Navigational avoidance as a contrail mitigation strategy has the potential to reduce the climate impact of aviation by as much as half. The effective implementation of avoidance strategies requires forecasts of the state of the upper troposphere and lower stratosphere that are stable (consistent across a range of lead times) and accurate (true to reality). However, the optimal criteria for evaluating whether a contrail forecasting system is sufficiently stable and accurate remain unclear. Here, we argue that forecast stability is best evaluated holistically by asking whether estimated decreases in contrail warming, for a given set of flight trajectories and deviations, are consistent across forecasts with different lead times. We use real-world flight trajectories taken from operational ADS-B datasets and deviations generated using aircraft performance models with a contrail-aware trajectory optimization routine to evaluate the stability of contrail predictions based on ECMWF IFS HRES forecasts. We find a high degree of stability with contrail warming reduced by over 80% even with lead times as long as 48 hours, sufficient to enable pre-tactical contrail avoidance at the flight planning stage. Finally, we show that we obtain large reductions in contrail warming despite frequent pointwise differences in the locations of ice supersaturated regions across forecast cycles because forecasts agree on the broad regions where ice supersaturation occurs.

How to cite: Dean, T., Abbot, T., Engberg, Z., Masson, N., Teoh, R., Stettler, M., and Shapiro, M.: Evaluating Forecasts for Navigational Contrail Avoidance, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7230, https://doi.org/10.5194/egusphere-egu25-7230, 2025.

EGU25-7440 | Orals | AS3.19

Physics-informed Machine Learning (PIML)-guided Contrails Formation Prediction 

Soumalya Sarkar, Sudeepta Mondal, and Miad Yazdani

Contrail cirrus is estimated to be responsible for more than 50% of aviation induced climate forcing to date. However operational contrail avoidance is currently not possible due to the inability to predict exactly when and where a persistent contrail will form, and how that translates into radiative forcing. This research presents how to construct a high-accuracy physics-informed machine learning (PIML) models based on engine and weather variables to predict contrails formation parameters such as visibility, onset, and plumes’ optical depth as a function of distance from the aircraft. The approach is based on nonintrusive PIML model with low compute need at inference, making it ideal for onboard deployment. Based on a comprehensive sensitivity and feature importance study of the PIML model, this work demonstrates that spatial variation of plumes’ optical depth and as a result, the onset probability and location of contrails formation are only sensitive to a handful of engine and weather variables.

How to cite: Sarkar, S., Mondal, S., and Yazdani, M.: Physics-informed Machine Learning (PIML)-guided Contrails Formation Prediction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7440, https://doi.org/10.5194/egusphere-egu25-7440, 2025.

EGU25-7550 | Posters on site | AS3.19

Enhanced Predictive Modeling and Validation of Persistent Contrails 

Saikat Ray Majumder

We present recent work in modeling the impact of the aviation industry on contrail formation and its subsequent effect on global warming by utilizing the Contrail Cirrus Prediction Model (CoCiP) with comprehensive 2019 airline data. This approach offers an in-depth, fleet-level perspective, revealing the influence on global energy forcing due to various factors including, but not limited to aircraft market class, operator region, and origin-destination pairs. Our analysis extends to a comparative study with results derived from our internally developed machine-learning (ML) emulator, the Hybrid Contrail Prediction (HyCoP) modeling framework. The HyCoP framework is designed to harness the power of physics-based CoCiP simulation data alongside satellite image-based ground truth observations to accurately predict persistent contrail formation. Central to this innovative framework is the Bayesian Deep Neural Network (BDNN) classifier. HyCoP is being developed to integrate aircraft engine-specific features, enhancing the standard inputs traditionally used in the CoCiP model. Furthermore, we detail our rigorous validation efforts for these contrail models. We employ geostationary satellite (GOES) images and data from flight campaigns such as 2023 ecoDemonstrator and 2024 Contrail Optical Depth Experiment (CODEX) to ensure the accuracy and reliability of our predictions. Our presentation includes the current status of our comprehensive start-to-end validation pipeline, which detects and tracks contrails and attributes them to their originating aircraft. This holistic approach underscores our commitment to advancing the understanding of contrail impacts on climate change through cutting-edge predictive modeling and thorough validation methodologies.

How to cite: Ray Majumder, S.: Enhanced Predictive Modeling and Validation of Persistent Contrails, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7550, https://doi.org/10.5194/egusphere-egu25-7550, 2025.

EGU25-8217 | ECS | Orals | AS3.19

Modeling the formation of contrails produced by SAF emissions 

Margaux Vals, Nicolas Bonne, Ismael Ortega, Katharina Seeliger, Charles Renard, Christiane Voigt, Daniel Sauer, Raphael Märkl, Rebecca Dischl, Stefan Kaufmann, Theresa Harlass, Andreas Marsing, Anke Roiger, Emmanuel Greslin, and Amandine Roche

Alternative aviation fuels represent a promising approach to reduce contrails climate effect. In the frame of VOLCAN (“VOL avec Carburants Alternatifs Nouveaux”) project (DGAC funding, collaboration with AIRBUS, Safran Aircraft Engines and DLR, financed by Neofuels), the influence of Sustainable Alternative Fuels (SAF) composition on exhaust plumes emission, and therefore on contrails, is investigated using the 1D detailed microphysical code MoMiE (Modèle Microphysique pour Effluents) developed at ONERA1,2. The VOLCAN measurement campaigns have been able to provide estimations of ice particle number emission indexes within contrails formed by different fuel types (classical kerosene Jet A-1 and biofuel HEFA) and different combustion modes (“rich” and “lean” burn). These are complementing the observations obtained for Sustainable Alternative Fuels with Emission and “CLimate Impact of alternative Fuels” (ECLIF) campaigns3,4, recently compared to the results of the “Aerosol and Contrail Microphysics” (ACM) model developed at the University of Albany5.

In its most recent version ONERA’s code MoMiE has been adapted to Sustainable Alternative Fuels (SAF)2. It includes heterogenous freezing with soot activation by sulfur and organic species, as well as homogeneous freezing of liquid droplets of hydrated sulfates and organics, accounting for the competition between both nucleation modes. Chemiionization, brownian coagulation of particles, ice sublimation and condensation are also represented. The code computes the different aerosols distributions (size and number) of sulfates, organics, dry soot, activated soot, and ice particles, homogeneously (no solid nucleus) and heterogeneously (soot solid nucleus) formed.

The work proposed here aims first at presenting and analyzing the results obtained with the model in comparison to some of the VOLCAN measurements. The sensitivity of contrail formation to the different fuel types, combustion modes and emission characteristics, as ion emission index, which is known to play a significant role in the coagulation process, are studied. The model is also confronted to the ECLIF measurements3,4 and the microphysics model results from University of Albany5. Advancement and results of this study will be presented and discussed during the conference.

1Vancassel X. et al., Numerical simulation of aerosols in an aircraft wake using a 3D LES solver and a detailed microphysical model, International Journal of Sustainable Aviation, 2014

2Rojo C. et al., Impact of alternative jet fuels on aircraft-induced aerosols, Fuel, 2014

3Voigt C. et al., Cleaner burning aviation fuels can reduce contrail cloudiness, communications earth & environment, 2021

4Märkl R. S. et al., Powering aircraft with 100% sustainable aviation fuel reduces ice crystals in contrails, Atmospheric Chemistry and Physics, 2024

5Yu F. et al., Revisiting Contrail Ice Formation: Impact of Primary Soot Particle Sizes and Contribution of Volatile Particles, Environmental Science & Technology, 2024

How to cite: Vals, M., Bonne, N., Ortega, I., Seeliger, K., Renard, C., Voigt, C., Sauer, D., Märkl, R., Dischl, R., Kaufmann, S., Harlass, T., Marsing, A., Roiger, A., Greslin, E., and Roche, A.: Modeling the formation of contrails produced by SAF emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8217, https://doi.org/10.5194/egusphere-egu25-8217, 2025.

Condensation trails from aviation have been shown to have a significant contribution to the total radiative impact of civil aviation. Consequently, their observation and modelling is an active field of research, so is the design of strategies to reduce the climate impact of aviation by avoiding contrail formation. However, the radiative efficacy of contrails in warming the climate is not well understood and constrained. Only a handful of studies have provided estimates of this key quantity so far. To better understand the impact of contrails on the climate, we developped a new parameterisation of contrails, cirrus clouds and ice supersaturation in the ICOLMDZ atmospheric general circulation model. This parameterisation is evaluated by estimating the value of radiative forcing of linear contrails and contrails evolving in cirrus clouds.

ICOLMDZ is the global atmospheric component of the IPSL-CM Earth System Model, actively and historically involved in the CMIP exercises. The standard version of ICOLMDZ is found to poorly represent cirrus clouds, and does not simulate ice supersaturated regions, which is a prerequisite for the formation of contrails. These regions are thermodynamically unstable, thus their modelling required a substantial revamp of the current parameterisation of cirrus clouds, which assumes thermodynamic equilibrium at all times. A new subgrid parameterisation that allows for ice supersaturation in both clear and cloudy sky was developped and implemented in ICOLMDZ.

This new parameterisation has then been adapted to simulate the effect of contrails and is used to assess the radiative forcing of contrails for a typical year, and a comparison with other state-of-the-art parameterisations in global climate models has been made. It will be used to estimate the efficacy of contrails to warm the Earth, using an ensemble of weakly nudged climate simulations with and without contrails.

How to cite: Borella, A., Boucher, O., and Vignon, É.: Modelling the climate effects of aviation in the ICOLMDZ climate model: From parameterising cirrus clouds and ice supersaturated regions to quantifying the radiative impact of contrails, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8888, https://doi.org/10.5194/egusphere-egu25-8888, 2025.

Cirrus clouds play a crucial role in regulating Earth’s radiation balance, with human activities altering their coverage and thus exerting a positive radiative forcing on the climate system. Among these, condensation trails left by planes, known as contrails, can persist into contrail cirrus which are nearly indistinguishable from natural cirrus. Their forcing constitutes most of the non-CO2 impact of the aviation sector, but its quantification remains very uncertain. Adjustments to radiative forcing are particularly poorly known, with estimates from a single climate model, where adjustments in natural cirrus counteract more than half of the initial radiative forcing.

We quantify the climate adjustments that follow abrupt, global transformation of water vapour in ice-supersaturated regions (ISSRs) into cirrus clouds. Using a new method based on ensembles of simulations with the French LMDZ atmospheric general circulation model, we analyse atmospheric and surface climate responses over a four-day period. We quantify the time constants of the ice water response, and its modulation of the initial radiative forcing. Preliminary results suggest that adjustments counteract 70% of the initial forcing within 4 hours.

Working with an simulation ensemble allows us to quantify a statistically significant behaviour of the adjustments and their time constants. Our findings enhance our understanding of the impact of contrails on climate and hold important implications for future climate modelling and prediction.

How to cite: Juvin-Quarroz, J.: On Short-Term Climate Adjustments Following Abrupt Cirrus Cloud Formation from ISSR, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8923, https://doi.org/10.5194/egusphere-egu25-8923, 2025.

EGU25-9027 | Orals | AS3.19

Global climate modelling of contrails cirrus from current and alternative fuel aircraft 

Alexandru Rap, Weiyu Zhang, Timmy Francis, Piers Forster, and Wuhu Feng

Contrail cirrus is estimated to be responsible for the largest and the most uncertain aviation effective radiative forcing (ERF) term. With the aviation sector’s commitment to reach net-zero emissions by 2050, there is a stringent need to better understand and constrain this term. A key challenge in reducing its associated uncertainty comes from the very limited number of climate models able to simulate contrail cirrus.

In this work we present results from two new contrail cirrus parameterisations for the UK Met Office Unified Model (UM), one based on the existing contrail scheme within the Community Atmosphere Model (CAM) and the other based on the prognostic contrail scheme developed for the ECHAM model. We find substantial differences in the simulated contrail coverage (up to a factor of 3) and radiative forcing (up to a factor of 8) caused by model differences in ice supersaturation and cloud microphysics schemes, together with existing uncertainty in contrail cirrus optical depth. Using the CAM model, we also quantify the change in the contrail cirrus climate impact due to switching to alternative fuels, such as sustainable aviation fuel (SAF), liquid hydrogen, and fuel cells. We find that the use of liquid hydrogen and fuel cells will likely lead to a substantial increase (up to 70%) in contrail cover compared to kerosene and SAF. However, our simulations indicate that despite this increase in coverage, the reduction in aerosol emissions associated with alternative fuels will lead to an overall reduction in contrail cirrus ERF.

We suggest that future work should focus on better constraining contrail cirrus optical properties (in particular for alternative fuels), and on improved representation of ice supersaturation and contrail microphysical processes in models.

How to cite: Rap, A., Zhang, W., Francis, T., Forster, P., and Feng, W.: Global climate modelling of contrails cirrus from current and alternative fuel aircraft, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9027, https://doi.org/10.5194/egusphere-egu25-9027, 2025.

EGU25-9035 | ECS | Orals | AS3.19

High-resolution simulations of contrails from hydrogen-powered aircraft 

Annemarie Lottermoser and Simon Unterstrasser

The transition to climate-friendly aviation necessitates the development of new propulsion technologies to replace conventional kerosene combustion engines. Hydrogen (H₂) propulsion is widely regarded as a promising and environmentally sustainable alternative. A key aspect of creating climate-friendly aviation involves evaluating the climate impact of contrails, which significantly contribute to aviation’s non-CO₂ effects. This study examines the properties of contrails produced by H₂-powered aircraft, with a particular focus on comparing them to contrails generated by conventional kerosene combustion. Using high-resolution simulations performed with the EULAG-LCM model—a large-eddy simulation (LES) model with fully coupled particle-based ice microphysics—we analyze individual contrails throughout their entire lifecycle. This includes the interaction of young contrails with the downward moving wake vortices and their evolution into contrail-cirrus over several hours.
Previous simulations of early contrail evolution during the vortex phase and the subsequent contrail-cirrus transition have extensively explored variations in meteorological and aircraft-related parameters. However, these studies have been limited to contrails from kerosene combustion.
To assess the impact of H₂ propulsion on contrail evolution, we adjust two key input parameters: increasing the water vapor emission and varying the number of initial ice crystals. Additionally, we expand the atmospheric scenarios to include higher ambient temperatures, accounting for the fact that H₂ contrails can form in warmer conditions where ice crystal formation in kerosene plumes is not possible (assuming the same droplet characteristics in both cases).
We analyze H₂ contrail evolution in various atmospheric scenarios, finding that wake vortices cause significant ice crystal loss through adiabatic heating. This loss is less pronounced with fewer initial ice crystals but increases at ambient temperatures above 225 K. In the subsequent contrail-cirrus phase, we focus on the evolution of the contrail total extinction, which serves as a proxy for relative changes in the contrail’s radiative effect. Our results demonstrate that factors such as the initial ice crystal number, ambient temperature, and relative humidity strongly influence the contrail lifecycle, while increased water vapor emissions (immanent to H2 propulsion) have a secondary effect.
This work contributes to the collaborative effort of the German Aerospace Center (DLR) and Airbus in assessing the climate impact of H2 contrails.

How to cite: Lottermoser, A. and Unterstrasser, S.: High-resolution simulations of contrails from hydrogen-powered aircraft, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9035, https://doi.org/10.5194/egusphere-egu25-9035, 2025.

EGU25-9076 | ECS | Posters on site | AS3.19

A novel Contrail Detection Algorithm for the Meteosat Second Generation satellite 

Vanessa Santos Gabriel, Luca Bugliaro, and Christiane Voigt

Contrail cirrus is estimated to be the largest contributor to global effective radiative forcing from aviation, surpassing even aviation CO2 emissions in their impact. One promising mitigation strategy is contrail avoidance by rerouting flights to avoid regions where warming contrails can persist. These regions are forecast with numerical contrail models fed with weather prediction model output. Satellite imagery presents a good opportunity to evaluate both the models and the success of the mitigation strategy.

An automatic contrail detection algorithm was implemented by Mannstein et al. (1999) for a polar orbiting satellite with high spatial resolution (≈ 1 km and used two thermal channels in the atmospheric window). Since then, it has been adapted to the Meteosat Second Generation (MSG) satellite because geostationary satellites have the big advantage of high temporal coverage of a large area. However, its lower spatial resolution (≥ 3 km) is a challenge for contrail detection. In recent years AI algorithms have been presented for the American geostationary GOES-R/S satellites (spatial resolution ≥ 2 km). In this study, a new improved contrail detection algorithm for MSG is proposed based on image processing.

To establish a new detection algorithm a labeled dataset was compiled. This labeled dataset contains 140 MSG images with data from the years 2013-2018 and 2023-2024. This data volume is very suitable to develop and evaluate an algorithm with a classical approach, would however not be sufficient to train an AI based algorithm. The data covers the whole MSG disk with a wide distribution of satellite viewing angles, cloud cover, number of contrails in the image and other properties. Each image was labeled by three individuals, and a common contrail mask was established as the consensus of the labelers. Based on this dataset, a new detection algorithm was developed. Making use of the spectral information of MSG, an image is created as input for the algorithm where contrail visibility is enhanced. The algorithm takes advantage of several new techniques compared to Mannstein et al. (1999). In addition to the contrail mask, uncertainty information is provided.

This new algorithm for contrail detection in MSG images demonstrates superior performance compared to the previous algorithm for MSG based on the Mannstein approach with a probability of detection higher than 70%. The contrail detection algorithm can now be employed for generating datasets to evaluate contrail models as well as to assess the success of contrail mitigation strategies such as flight path alteration. Thanks to this classical image processing approach, in the future the algorithm can be adapted to other satellites like Meteosat Third Generation.

How to cite: Santos Gabriel, V., Bugliaro, L., and Voigt, C.: A novel Contrail Detection Algorithm for the Meteosat Second Generation satellite, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9076, https://doi.org/10.5194/egusphere-egu25-9076, 2025.

EGU25-9774 | Posters on site | AS3.19

RANS simulations for contrail formation modelling 

Jhaswantsing Purseed, Grégoire Pont, Jean-Paul Romeo, Jérôme Huber, Lucile Arsicaud, Catherine Mackay, and Charles Renard

Condensation trails (contrails) are ice clouds formed at high altitudes as a result of water-vapour condensing and freezing on soot particles and sulphate aerosols which are present in the aircraft engine plumes (case of soot-rich combustion with kerosene [1]). Under favourable atmospheric conditions such as ice supersaturated regions, i.e., low temperatures and high humidities with respect to ice, these contrails can persist for up to several hours while covering large areas. The latter is especially important when considering the climate impacts of the aviation emissions as the radiative forcing from persistent contrails and contrail-cirrus is one of the major contributors [2]. 

Therefore, improving the understanding of the underlying physics of contrail is of utmost importance for the development of mitigation solutions. The process of formation and early evolution of the ice crystals occurs within the first few seconds which is often referred to as the jet phase. As such, Computational Fluid Dynamics (CFD) serves as an important tool in studying the near-field wake of the aircraft. In this study, we use a Reynolds-Averaged Navier Stokes (RANS) CFD solver, named FLUSEPA [3], to simulate the exhaust of the Common Research Model (CRM) [4] engine up to 500 m behind the engine (focusing on the mixing of the plume and not the ice crystal formation). FLUSEPA is a solver developed by Ariane Group for launcher propulsion. Furthermore, we consider an engine powered by hydrogen combustion consequently emitting about 2.6 times more water-vapour mass than a kerosene-powered engine. Note that for a hydrogen-powered engine, depending on the design choices, ice crystals would most likely form on a combination of ambient aerosols and/or soluble NOx particles. 

 

The RANS solver is used to simulate an idealised configuration of an isolated engine. This allows us to validate the dynamics of the jet in the axial direction. We briefly describe the methodologies used so as to obtain the plume’s dilution as a function of the axial position which can then be used by an offline microphysics model to simulate ice crystal formation. Finally, we vary physical and numerical parameters relevant to contrail formation to identify their role on the dilution factor. 

 

References

 

[1]  Yu, Fangqun, et al. "Revisiting contrail ice formation: Impact of primary soot particle sizes and contribution of volatile particles." Environmental Science & Technology 58.40 (2024): 17650-17660.

[2] Lee, David S., et al. "The contribution of global aviation to anthropogenic climate forcing for 2000 to 2018." Atmospheric environment 244 (2021): 117834.

[3] Pont, Grégoire, and Pierre Brenner. "High order finite volume scheme and conservative grid overlapping technique for complex industrial applications." Finite Volumes for Complex Applications VIII-Hyperbolic, Elliptic and Parabolic Problems: FVCA 8, Lille, France, June 2017 8. Springer International Publishing, 2017.

[4] Vassberg, John, et al. "Development of a common research model for applied CFD validation studies." 26th AIAA applied aerodynamics conference. 2008.

How to cite: Purseed, J., Pont, G., Romeo, J.-P., Huber, J., Arsicaud, L., Mackay, C., and Renard, C.: RANS simulations for contrail formation modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9774, https://doi.org/10.5194/egusphere-egu25-9774, 2025.

The steady increase in global air traffic demand has led to a corresponding rise in contrail radiative forcing, contributing significantly to effective radiative forcing (ERF). Contrails, formed when hot exhaust gases from jet engines mix with cold, humid ambient air, have a warming effect that can surpass the CO₂ emissions of aviation in the short term. While contrail mitigation strategies often focus on adjustments to cruise altitudes and flight trajectories, less attention has been given to the impact of climb and descent phases, and particularly their effects on cruise phases for short- and medium-range flights. This study explores the contrail mitigation potential of these flight phases, providing a comprehensive analysis of their contribution to contrail formation, and associated operating costs.

Contrail persistence depends on atmospheric conditions within ice-supersaturated regions (ISSRs), primarily occurring at typical cruising altitudes. However, the dynamics of the initial climb and final descent phases should only occasionally allow for contrails to form, and much less for persistence to occur, primarily due to higher temperatures at low altitudes. When transitioning through vertical layers of ISSRs, some contrails may however still form, though a quantification of this phenomenon is lacking. Thus, by leveraging simulations conducted with an air traffic simulator embedded in a climate-chemistry model (EMAC/AirTraf), this study investigates contrail formation during these phases, narrowing this gap. By incorporating these overlooked flight segments, we aim to provide a more accurate estimate of contrail prevalence.

A critical aspect of the analysis involves quantifying the impact of climb and descent phases on contrail length and operating costs. By grouping simulations based on flight length for a set of European flights, this study elucidates differences in contrail distances and cost estimated using fuel consumption. In order to investigate this, the flights are first analysed using an airport to airport trajectory, optimised using different objectives such as contrail distance minimum, fuel optimal, and multi-objective (fuel-contrail). For airport to airport, it assumes that these flights entirely occur at cruise altitude. The next step uses more realistic trajectories, considering a cruise phase bounded by climbing and descending phases, using the same optimisation options. The direct impact of climb and descent in terms of contrail distance is observed from the difference between the original trajectory (airport-airport) and the cruise only trajectory. Next using the cruise only trajectory determined with the standard entry/exit points, also known as standard instrument departures (SID) and standard instrument arrivals (STAR), together with the separate impact of ascent/descent, the overall climate impact reduction potential can be determined for a more realistic flight path, using algorithmic climate change functions (ACCF).

By applying this method, we expect to identify the potential contribution of climb and descend to the contrail climate impact for a given flight. By extension, this would indicate the relevance of climb/descent phases in contrail mitigation potential studies, regardless of chosen optimiser, and moreover, the differences arising in the mitigation potential as a function of flight length. 

How to cite: Stefanidi, A., Yin, F., and Grewe, V.: Assessing Contrail Mitigation Potential Through Initial Climb and Final Descent Phase Analysis: A Comparison of Short- and Medium-Range Flights Within Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9779, https://doi.org/10.5194/egusphere-egu25-9779, 2025.

EGU25-10666 | Posters on site | AS3.19

Simulating the climate benefit of contrail reduction through targeted SAF in 2030 at Copenhagen airport 

Roland Eichinger, Katrin Dahlmann, Volker Grewe, Benedict Enderle, Sven Maertens, Shravana Kumar, Christian Weder, Wolfgang Grimme, and Leon Müller

To reduce the considerable climate effect of aviation, the ReFuelEU aviation regulation obliges all aviation fuel suppliers to provide increasing amounts of sustainable aviation fuel (SAF) to EU airports in the coming years and decades. SAF primarily reduces aviation CO2 life-cycle emissions, but also the contrail climate effect. As SAF on average contains less aromatics, SAF-fueled aircraft emit less particulate matter, leading to lower ice crystal number concentrations with larger ice crystals in the formed contrails. In consequence, this reduces the overall contrail climate effect, as the contrails are optically thinner and less persistent. In contrast to the CO2 emissions of a flight, which are directly proportional to the fuel use, the contrail climate effect
is highly variable from flight to flight. Hence, SAF allocation to specific flights can maximise climate mitigation efforts for certain amounts of SAF, especially as long as SAF supply is limited and production capacities are still about to be scaled up.
Within the ALIGHT project, Copenhagen Airport (CPH) works towards the introduction of sustainable aviation solutions for the future. For this, one important component is knowledge on the climate-optimal SAF distribution to the flights at CPH, which we here estimate using the climate surrogate model AirClim. For the purpose, we have refined the SAF parameterisation with regard to the particulate matter reduction through SAF and use a wing span parameterisation to account for the aircraft type. The study particularly targets year 2030, as the 6% SAF mandate then is still expected to allow large climate benefits through targeted SAF use and there is still time for infrastructural adaptions. We quantify the additional climate benefit for all flights departing from CPH through targeted SAF use in those flights with the largest contrail climate effect to fuel use ratio instead of distributing it uniformly to all flights. For this, we assess the optimal SAF blending ratio, analyse various climate metrics and time horizons and cluster the flights with regard to their mean latitudes and aircraft types. The results of this study lay the ground for a complete cost-benefit analysis taking into account all aspects of infrastructure at CPH to assess practical feasibility.

How to cite: Eichinger, R., Dahlmann, K., Grewe, V., Enderle, B., Maertens, S., Kumar, S., Weder, C., Grimme, W., and Müller, L.: Simulating the climate benefit of contrail reduction through targeted SAF in 2030 at Copenhagen airport, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10666, https://doi.org/10.5194/egusphere-egu25-10666, 2025.

EGU25-11011 | Posters on site | AS3.19

HYDEA Project Work Package 6: Contrail modeling for hydrogen combustion. 

Catherine Mackay, Lucile Arsicaud, Jhaswantsing Purseed, Simon Unterstrasser, Josef Zink, Kamila Roszkiewicz, Tomasz Iglewski, and Nicolas Bonne

Aviation emissions contribute to climate change, one of the key contributors being contrail cirrus clouds. The importance of this impact is strongly dependent on their properties . 

A condensation trail - or contrail - is composed of ice crystals which form behind the aircraft engine exhaust at high altitudes when local weather conditions are favorable. The formation is also influenced by the engine technology and operating conditions, and by the fuel type. The contrail persists and evolves as long as it remains in an ice supersaturated region, a local atmospheric air mass characterized by a low temperature and a humidity level that is saturated versus ice. Only persistent contrails are considered as having a climate effect.

Hydrogen propulsion is considered as one promising technology to reduce aviation’s climate impact, in line with the European Green Deal and Clean Aviation Strategic Research and Innovation Agenda (SRIA). In this context, the EU-funded HYDEA project proposes a robust and efficient technology maturation plan for H2 propulsion. 

The formation of contrail ice crystals in an aircraft plume is mainly driven by the interaction of three physical phenomena: the dynamics in the engine exhaust, chemical transformations of effluents and microphysical processes.

The main assumptions when moving from a kerosene to a H2 fueled propulsion system are that there will be no soot particles in the jet exhaust, and an increased water vapour emission compared to kerosene. New modelling chains are required to understand how, in this case, ice crystals are formed and they evolve.

The models under development will be presented along with the assumptions being made. In HYDEA Work Package 6, two H2 contrail models using complementary methods are under development, using the Common Research Model [1]. The ONERA model using the 3D model CEDRE for both jet and vortex phases simulation provides a high-fidelity engine and aeroplane representation. The DLR model uses a Lagrangian Cloud Module box model approach with particle-based microphysics providing a high-fidelity microphysical representation with a simplified geometry. This ingests jet exhaust CFD data provided by Airbus and GEAP. The latest scientific developments and assumptions being incorporated in the models are discussed.

[1] Development of a Common Research Model for Applied CFD Validation Studies: J. Vassberg, M. Dehaan, M. Rivers & R. Wahls. 26th AIAA Applied Aerodynamics Conference 2012, June 2012, Hawaii, United States. https://doi.org/10.2514/6.2008-6919.

How to cite: Mackay, C., Arsicaud, L., Purseed, J., Unterstrasser, S., Zink, J., Roszkiewicz, K., Iglewski, T., and Bonne, N.: HYDEA Project Work Package 6: Contrail modeling for hydrogen combustion., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11011, https://doi.org/10.5194/egusphere-egu25-11011, 2025.

EGU25-11045 | Orals | AS3.19

Influence of tail plan vortices on contrail vortex and dissipation phase 

Nicolas Bonne and Remy Annunziata

Contrails are ice clouds formed by both the aircraft emissions and the water content of the atmosphere. Under specific atmospheric conditions, contrails can persist for several hours. During this time, these human made clouds perturb the energy balance of the atmosphere. It has been shown in [1] that contrails are the main contribution of non CO2 radiative forcing due to aviation. There effective radiative forcing is estimated to be about twice the one from the CO2 emitted by the aircrafts; however, this value remains uncertain.

Contrails climatic impact is usually studied either by a dedicated parametrization in global climate model [2] or using a Gaussian model [3]. In both kinds of model, contrails are initialized once the dynamic of the aircraft can be neglected (about 7.5 min after the aircraft). Therefore, it is important to have the best parametrization of contrails at this stage of contrail’s life. To study contrails up to 7.5 minutes usually two different kinds of simulations are made. The first one covering the contrail formation (known as jet phase), and another one looking at the dissipation of the wing tip vortices (vortex and dissipation phases). Their formation is studied using RANS simulation [4] or with 0D models run on streamlines of a previous LES simulation of a single jet [5]. Then the results are injected in the vortex phase simulation ([6],[7]). When only a jet simulation is used, the wing tip vortices are initialized with two Lamb-Oseen vortices scaled based on the lift of the aircraft. However, a recent study [8] has shown some differences in terms of dilution between a simulation initialized based on a RANS solution and the analytical solution. This has be explained by 4 vortex instabilities which triggers shorter waves than the so called crow instabilities [9] as shown in [10].

In this study, we test the influence of the tail plan vortices on contrails characteristics assuming different tail plan vortices strength in order to see the dependency of the aircraft equilibrium on contrail.

[1] Lee et al. (2021). The contribution of global aviation to anthropogenic climate forcing for 2000 to 2018. Atmospheric environment

[2] Burkhardt et al. (2010). Global modeling of the contrail and contrail cirrus climate impact. Bulletin of the American Meteorological Society

[3] Schumann  (2012). A contrail cirrus prediction model. Geoscientific Model Development

[4] Khou et al. (2015). Spatial simulation of contrail formation in near-field of commercial aircraft. Journal of Aircraft

[5] Bier et al. (2022). Box model trajectory studies of contrail formation using a particle-based cloud microphysics scheme. Atmospheric Chemistry and Physics

[6] Paoli et al. (2013). Effects of jet/vortex interaction on contrail formation in supersaturated conditions. Physics of Fluids

[7] Unterstrasser et al. (2014). Dimension of aircraft exhaust plumes at cruise conditions: effect of wake vortices. Atmospheric Chemistry and Physics

[8] Bouhafid et al. (2024). Combined Reynolds-averaged Navier-Stokes/Large-Eddy Simulations for an aircraft wake until dissipation regime. Aerospace Science and Technology

[9] Crow (1970). Stability theory for a pair of trailing vortices. AIAA journal

[10] Fabre et al. (2000). Stability of a four-vortex aircraft wake model. Physics of Fluids,

How to cite: Bonne, N. and Annunziata, R.: Influence of tail plan vortices on contrail vortex and dissipation phase, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11045, https://doi.org/10.5194/egusphere-egu25-11045, 2025.

EGU25-11289 | ECS | Posters on site | AS3.19

Highly-resolved simulations of contrail formation generatedby fuel cell-propelled aircraft 

Dennis Hillenbrand and Simon Unterstrasser

Aviation emissions are estimated to contribute approximately 3.5% of the global anthropogenic effective radiative forcing [3]. The goal to reduce this forcing can only be realized by a combination of measures including also new propulsion technologies. Aircraft powered by fuel cells operated with hydrogen are one promising future technology as they avoid both CO2 and NOx emissions. Additional to the reduction of these emissions generating strong contrail-cirrus has to be avoided to reduce the overall radiative forcing due to aviation emissions. Therefore it is important to investigate the contrail properties from fuel cell aircraft since they may significantly differ from current aircraft.
The number of ice crystals formed in the first few seconds of the exhaust is crucial for the radiative impact of the evolving contrail-cirrus. Among other effects the changed dynamics behind the propellers and the expected higher moisture-to-temperature ratio of the fuel cell exhaust will alter the number of formed ice crystals compared to classical jet combustion exhausts. Additional nucleation processes become important due to larger supersaturation values during the cooling of the plume. We will present the influence of these processes and different fuel cell setups on the number of formed ice crystals after the formation phase.
We simulate the formation of contrails by means of the Lagrangian Cloud Module (LCM) with detailed particle-based microphysics. To avoid computational overload we use a 0-D offline approach: suitably averaged data from a priori 3D CFD simulations of the exhaust dilution are used as input in the 0D LCM box model. This model has been used in recent studies for contrail formation simulations of a classical turbo-fan aircraft with kerosene or hydrogen combustion [1, 2]. During this work the LCM model has been adapted and extended to enable the simulation of contrail formation behind fuel cell powered aircraft. The model was applied and results are shown.
This work contributes to the collaborative effort of DLR and Airbus in assessing the climate impact of H2 contrails.

How to cite: Hillenbrand, D. and Unterstrasser, S.: Highly-resolved simulations of contrail formation generatedby fuel cell-propelled aircraft, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11289, https://doi.org/10.5194/egusphere-egu25-11289, 2025.

EGU25-11345 | ECS | Posters on site | AS3.19

A Global Aviation Emission Inventory of Contrail-Processed nvPM Particles 

Kexin Qiu, Roger Teoh, Marc Stettler, Masaru Yoshioka, Paul Field, Benjamin Murray, and Alex Rap

The largest uncertainties in current estimates of the aviation contribution to anthropogenic climate forcing are associated with aerosol-cloud interactions, particularly the role of soot, i.e., non-volatile particulate matter (nvPM), as the ice-nucleating particle (INP). Contrail processing, where ice crystals form on aircraft-emitted nvPM particles and subsequently release these particles back into the atmosphere after sublimation, influences their ice nucleation efficiency. However, to date, no aircraft emission inventory includes contrail-processed aerosol particles. In this study, we present the first comprehensive global aircraft emission inventory of contrail-processed nvPM particles, based on robust contrail simulations from the CoCiP (Contrail Cirrus Prediction) model and GAIA, a high-resolution real-life aircraft emissions inventory for the years 2019–2021. Our results show that aviation emitted a total of 2.83 × 1026 nvPM particles in 2019, with reductions of 48% and 41% in 2020 and 2021, respectively, due to COVID-19. During this period, the proportion of contrail-processed particles remained relatively consistent, with a slight reduction from 15% annually in 2019 to around 13% in 2020 and 2021. Approximately 75% of contrail-processed nvPM particles were processed by short-lived contrails. Spatially, the highest absolute concentrations of contrail-processed particles occurred over Europe and North America, while regions like the Arctic and North Atlantic exhibited the largest relative percentages due to favourable contrail formation conditions. Vertically, contrail-processed particles were primarily concentrated between 7 and 17 km, becoming increasingly dominant with altitude. Future work will focus on using this inventory in global climate models to estimate the impact of contrail processing on aviation aerosol-cloud interactions, contributing to reducing the uncertainties in aviation’s climate impact assessments.

How to cite: Qiu, K., Teoh, R., Stettler, M., Yoshioka, M., Field, P., Murray, B., and Rap, A.: A Global Aviation Emission Inventory of Contrail-Processed nvPM Particles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11345, https://doi.org/10.5194/egusphere-egu25-11345, 2025.

EGU25-11372 | Posters on site | AS3.19

Ground-based installations at the Haute Provence Observatory (OHP) to monitoring and study condensation trails 

Abdanour Irbah, Philippe Keckhut, Dunya Alraddawi, Florian Mandija, and Olivier Liandrat

Cloud formation can also result from human activity, such as aircraft condensation trails, or contrails. They are created by the release of water vapor and soot from aircraft. Contrails can then change shape rapidly after forming, and then persist in the atmosphere for varying lengths of time. They will persist in the atmosphere if the air is super-saturated with ice, i.e. when the height of aircraft is in the upper troposphere. They can then evolve into cirrus clouds if the thermodynamic conditions of the atmosphere are favourable. These cloud-like contrails will therefore have environmental consequences that need to be understood to be included in climate models as non-CO2 contributions. These are the main motivations that led us to the establishment of ground facilities at the Haute Provence Observatory (OHP south of France) to observe and study condensation trails. They are mainly composed of a Lidar, radiosondes and two sets of fisheye cameras recording hemispherical images of the sky in the visible and thermal infrared for nighttime observations. The Global Horizontal Irradiance (GHI) of the Sun and some meteorological data on ground are also recorded together with the images. We will first describe in detail the instrumentation currently installed on the ground and operational for contrail monitoring. We will then present a case of a contrail recorded on March 21, 2024 at OHP and detail all the processing steps, from its detection to its analysis, including the identification of the aircraft trajectory in the images and the expansion of the contrail it leaves.

How to cite: Irbah, A., Keckhut, P., Alraddawi, D., Mandija, F., and Liandrat, O.: Ground-based installations at the Haute Provence Observatory (OHP) to monitoring and study condensation trails, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11372, https://doi.org/10.5194/egusphere-egu25-11372, 2025.

EGU25-11650 | Orals | AS3.19

1D/2D radiative forcing modelling of a contrail using a Monte-Carlo approach 

Etienne Terrenoire, Mattéo Roch, Jean-Michel Lamet, and Lionel Tessé

Contrails affect the radiative balance of the Earth climate (Lee et al., 2021). The representation of contrails characteristics and evolution into climate model remains highly challenging due to the complexity of the microphysical and chemical processes involved into the formation of contrails. The high sensitivity of contrails Radiative Forcing (RF) to the contrails morphology and composition in terms of ice crystal shape, number and size as well as surface temperature and albedo leads to major uncertainty when the RF of contrails is evaluated. In this paper, contrails RF has been modelled using the CEDRE-ASTRE Monte Carlo solver (Tessé and Lamet, 2011) for 1D and 2D idealized representations of a contrail in an atmospheric column (0 - 120 km). The role of the microphysical contrail characteristics have been evaluated using a multiple run sensitivity analysis to key parameters in the determination of contrails RF such as ice crystal size, ice water content, surface albedo and emissivity. A critical analysis of the results is made with comparable studies using different codes (Wolf et al., 2023) and will be detailed in the presentation.

 

References

 

Lee, D.S., Fahey, D.W., Skowron, A., Allen, M.R., Burkhardt, U., Chen, Q., Doherty, S.J., Freeman, S., Forster, P.M., Fuglestvedt, J., Gettelman, A., De León, R.R., Lim, L.L., Lund, M.T., Millar, R.J., Owen, B.,Penner, J.E., Pitari, G., Prather, M.J., Sausen, R., Wilcox, L.J., The contribution of global aviation to anthropogenic climate forcing for 2000 to 2018, Atmospheric Environment, 2021, 244.

Tessé L. and Lamet J.-M., Radiative Transfer Modeling Developed at ONERA for Numerical Simulations of Reactive Flows, AerospaceLab, ed. 2, https://aerospacelab.onera.fr/en/Radiative-Transfer-Modeling-Developed, 2011.

Wolf, K., Bellouin, N., and Boucher, O.: Sensitivity of cirrus and contrail radiative effect on cloud microphysical and environmental parameters, Atmos. Chem. Phys., 23, 14003–14037, https://doi.org/10.5194/acp-23-14003-2023, 2023.

How to cite: Terrenoire, E., Roch, M., Lamet, J.-M., and Tessé, L.: 1D/2D radiative forcing modelling of a contrail using a Monte-Carlo approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11650, https://doi.org/10.5194/egusphere-egu25-11650, 2025.

EGU25-11993 | ECS | Orals | AS3.19

Modelling contrail cirrus using a double-moment cloud microphysics scheme in the UK Met Office Unified Model 

Weiyu Zhang, Paul Field, Piers Forster, and Alexandru Rap

Aviation currently contributes approximately 3.5% to the anthropogenic effective radiative forcing (ERF) on climate, with contrail cirrus being the largest contributor, accounting for twice the impact of aviation CO2 emissions. However, the latest assessment of aviation's climate impact highlights significant uncertainty of around 70% in contrail cirrus ERF estimates due to process-related uncertainties. Recent research also highlights the critical role of cloud microphysical schemes in representing contrail microphysical and optical properties in climate models.

In this study, we implement a contrail parameterisation in the double-moment cloud microphysics scheme, Cloud AeroSol Interacting Microphysics (CASIM), within the UK Met Office Unified Model (UM). This enables the UM to represent the high number concentration of young contrails, which is critical for the simulation of contrail cirrus evolution and climate impacts. We use a contrail cluster model experiment to evaluate the simulated contrail cirrus evolution, demonstrating that the CASIM modelled changes in several key contrail characteristics are consistent with previous modelling and observation studies. Our analysis indicates that contrails retain a high ice crystal number concentration for a several hours, while contrail ice water content increases during the early stage of the lifecycle before gradually decreasing. In addition, as the contrail cluster descends due to sedimentation, there is an increase in both contrail ice number concentration and water content below flight levels.

We also perform a series of regional simulations over a European domain (i.e. around 35°N-58° N and 10°W-22°E) using the AEDT air traffic inventory. We find that the regional mean contrail cirrus ERF over Europe simulated in our model compares well with estimates from other climate models. Our study highlights the critical role of using a double-moment cloud microphysics scheme when simulating contrails in global climate models. In contrast, results using the UM with a single moment cloud microphysics scheme fails to capture the high ice particle number concentration in young contrails, resulting in unrealistic ERF estimates. Future work with CASIM-UM should focus on estimating contrail cirrus ERF over other regions with high air traffic to provide a more comprehensive understanding of aviation climate impact. In addition, future work should also investigate how the use of alternative fuels affects ice crystal number concentrations, contrail lifetime, microphysical and optical properties. 

How to cite: Zhang, W., Field, P., Forster, P., and Rap, A.: Modelling contrail cirrus using a double-moment cloud microphysics scheme in the UK Met Office Unified Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11993, https://doi.org/10.5194/egusphere-egu25-11993, 2025.

EGU25-12684 | Posters on site | AS3.19

Understanding contrail formation in the near-field of modern turbofan engines 

Manas Madasseri Payyappalli, Feijia Yin, and Arvind Gangoli Rao

Contrails are formed when the hot exhaust from the core of the engine mixes with the relatively cold ambient. Traditionally, contrail formation and its persistence is predicted using the Schmidt-Appleman (SA) criterion, which is a simple thermodynamic model developed based on the engine exhaust and ambient conditions. However, the formation of contrails is a complex multi-physics problem which lies at the intersection of thermodynamics, fluid mechanics, and physical chemistry, and is strongly dependent on engine conditions and atmospheric variables. 

This being said, for modern turbofans with different engine architectures, the competing thermal and flow-field characteristics of the core jet, bypass jet, and ambient conditions play vital role in the formation of contrails in the near-field. We use RANS CFD modelling approaches to understand the macrophysical nature of contrail formation in different turbofan engines. Thermodynamic theories and analyses on the flow physics are utilized to understand the underlying mechanisms leading to contrail formation. The study finds interesting relations between the bypass ratios of the engines and potential contrail forming regions. Regions in the exhaust plume where contrails are likely to form is thus strongly dependent on the bypass ratio, or in other words, the flow-field mixing is found as an important deciding factor in contrail formation. The results are compared with the prediction from the SA criterion and the limitations and advantages of both approaches are discussed in detail. As outlook, we plan to extend this work by implementing microphysics models to complement the macrophysics results. 

How to cite: Madasseri Payyappalli, M., Yin, F., and Gangoli Rao, A.: Understanding contrail formation in the near-field of modern turbofan engines, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12684, https://doi.org/10.5194/egusphere-egu25-12684, 2025.

EGU25-13300 | ECS | Posters on site | AS3.19

Ground Cameras with ADS-B Data for High-Resolution Contrail Detection & Attribution  

Vasha DuTell, Olivier Kigotho, Shrenik Borad, Robert Pless, Prashanth Prakash, Ian Waitz, and Bill Freeman

Aircraft contrails are a significant contributor to aviation-induced climate effects, but attributing individual contrails to specific aircraft remains a challenge, especially when relying solely on satellite data. Satellite imagery offers extensive coverage but is limited by temporal and effective spatial resolution due to the large imaging distance. We propose a methodology that integrates freely available ground-based webcams, with ADS-B flight data to detect and attribute contrails to specific flights. 

We project flight trajectories from ADS-B data with latitude-longitude-altitude coordinates into the ground camera frame of reference using camera extrinsics pre-calculated from geographic points of reference. We then use a contrail segmentation method based on Canny edge detection and curve fitting to identify contrails in the frame of reference of the ground camera, capitalizing on the ground camera’s proximity and high framerate to attribute detected contrails to flights. Detected contrails can also be projected from ground camera space to satellite perspective, enabling the direct comparison between ground camera and satellite-based detection and attribution methods. With higher-accuracy ground-camera based attribution, we also enable the validation of more challenging satellite-based contrail attributions.

By leveraging the proximity of ground cameras for higher effective spatial resolution and their continuous capture for higher temporal resolution, our system addresses key limitations of satellite data. Our framework lays the groundwork for improved understanding of contrail creation, lifecycle, persistence, and more reliable monitoring of aviation-induced climate impacts. This method has the potential to enhance and validate operational contrail monitoring and avoidance and improve the integration of ground-based observations with satellite-based methods.

How to cite: DuTell, V., Kigotho, O., Borad, S., Pless, R., Prakash, P., Waitz, I., and Freeman, B.: Ground Cameras with ADS-B Data for High-Resolution Contrail Detection & Attribution , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13300, https://doi.org/10.5194/egusphere-egu25-13300, 2025.

EGU25-13450 | ECS | Orals | AS3.19

Influence of Fuel Sulfur Content and nvPM Emissions on Contrail Formation: A CFD-Microphysics Approach 

Francois Garnier, Sébastien Cantin, and Mohamed Chouak

A CFD-microphysics coupling approach is presented for accurately predicting the formation and evolution of ice crystals originating from soot and volatile particles in the near-field of a turbofan engine. This method integrates an online Eulerian–Lagrangian coupling based on 2D axisymmetric unsteady Reynolds-Averaged Navier–Stokes equations to simulate exhaust plume dynamics. The framework incorporates tabulated chemistry (including 60 reactions, 22 reactive species, and 29 non-reactive species) and a detailed ice microphysics model. The model accounts for complex multicomponent interactions, including soot surface activation, condensation of organic vapors and sulfur species (H₂SO₄, SO₃), and the scavenging of sulfuric acid-water droplets by soot surfaces.

The analysis examines the effects of varying ambient temperatures, fuel sulfur content, and soot particle concentrations on ice crystal formation, which will be discussed in detail.

As a result, the figure compares the spatial distributions of plume particles, focusing on the effects of ambient temperature and fuel sulfur content. Specifically, it examines the spatial distribution of soot particles in three states: dried (black), activated (blue points), and frozen (cyan points). The comparison is presented for two scenarios:
a) ambient temperatures of 212 K and 218.8 K at a sulfur content of 700 ppm, and
b) sulfur contents of 700 ppm and 20 ppm at an ambient temperature of 218.8 K.

a)

b)

How to cite: Garnier, F., Cantin, S., and Chouak, M.: Influence of Fuel Sulfur Content and nvPM Emissions on Contrail Formation: A CFD-Microphysics Approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13450, https://doi.org/10.5194/egusphere-egu25-13450, 2025.

EGU25-14010 | ECS | Orals | AS3.19

Assessment of Exhaust Plume Microphysics for Quantification of Contrail Climate Impacts 

Marcos Logrono, Cyprien Jourdain, Adam Boies, Prakash Prashanth, Raymond Speth, and Sebastian Eastham

Current estimates of the climate impacts of aviation condensation trails (contrails) are highly uncertain, primarily due to limited observational data and inconsistencies among different contrail models. However, contrails are thought to contribute substantially to the overall climate impacts of aviation, even at the lower end of the estimated uncertainty. One potential mitigation strategy is to reduce ice-forming emissions through advancements in fuel and engine technology. However, our current understanding of the sensitivities of contrail formation and radiative forcing to engine design variables and fuel properties is limited. Initial studies show that the early plume microphysics modeling (EPM) in contrail models such as the Aircraft Plume Chemistry, Emissions, and Microphysics Model (APCEMM) do not sufficiently capture the role of various emission species. These limitations include lack of representation of ice formation through homogeneous freezing of volatile aerosols, the effect of chemi-ions on aerosol coagulation, and a simplified treatment of nvPM and their activation.

To address these gaps, we aim to improve the existing EPM by including first principle-based modeling, supported by experimental results. In particular, the physics of condensation at the single-particle level is key to determining the transition towards ice crystals. This study investigates the role of nvPM activation via sulfates and organics, as well as the role of pore condensation and freezing, in contrail formation.  The presence of sulfuric precursors can promote the activation of initially hydrophobic soot particles. Such particles have complex fractal shapes that include regions with high surface energy associated with open nano-and micro-pores, favoring the nucleation of critical water droplets. First results have shown that liquid fills the gaps between the primary particles of soot aggregates to form pendular rings which can develop even in a low saturation environment (Sr<1). The model used in the present study captures the realistic internal mixing of soot aggregates, from the activation up to heavy coating states, e.g., soot cores hosted within spherical droplets. The properties of the growing aerosols are measured throughout, including their size, density, and mass, as well as their optical signature, and will be communicated within APCEMM.

In addition, the effect of chemi-ions on aerosol coagulation will be considered. Implementing these microphysical considerations into the EPM, we can capture the soot-rich to soot-poor continuum of ice formation and test the impact of desulfurized fuel as well as low-soot emission indices on long term contrail evolution and the associated radiative forcing through APCEMM. With this work we hope to quantify the relative importance of various engine design parameters and fuel types to contrail formation, evolution, and, subsequently, climate impacts.

How to cite: Logrono, M., Jourdain, C., Boies, A., Prashanth, P., Speth, R., and Eastham, S.: Assessment of Exhaust Plume Microphysics for Quantification of Contrail Climate Impacts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14010, https://doi.org/10.5194/egusphere-egu25-14010, 2025.

EGU25-14302 | Orals | AS3.19

Stochastic modeling of contrail formation 

Roberto Paoli and Justin Rigal

Contrails and contrail cirrus are the largest contributors of aviation radiative forcing, yet the exact quantification of their global impact remains far more uncertain compared to other sources, such as direct CO2 emissions. This uncertainty involves all phases of contrail lifetime –from formation until dilution in the free atmosphere. It is known for example that aircraft induce persistent contrails when flying in ice-supersaturated regions by providing condensation nuclei (soot particles or liquid aerosols) onto which ice nucleates and accumulates. These processes are strongly non-linear and also depend on the atmospheric conditions and engine setup among other parameters. Since it is not possible to explore the effects of all these parameters using detailed modeling such as 3D large-eddy simulations, low or mid-fidelity modeling approaches have been used in the literature with mixed success. In an effort to assist industry and modelers with design tools and flight trajectories definition, we developed an efficient computational method based on Reynolds Average Navier Stokes (RANS) simulations coupled to a stochastic model that captures the essence of jet turbulent mixing and the microphysical processes occurring in the plume. The method is validated for pure mixing using existing database of jet flow experiments and simulations, and it is then applied to contrail formation by activating simple ice microphysical models.

How to cite: Paoli, R. and Rigal, J.: Stochastic modeling of contrail formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14302, https://doi.org/10.5194/egusphere-egu25-14302, 2025.

EGU25-15429 | Posters on site | AS3.19

Addressing Uncertainty and Rerouting Strategies in Aviation Climate Impact Assessments 

Daniel Johansson, Christian Azar, Susanne Pettersson, Thomas Sterner, Marc Stettler, and Roger Teoh

Aviation causes climate effects through both long-lived CO₂ emissions and short-lived but highly uncertain contrail cirrus. The radiative forcing (RF) of contrail cirrus is spatially and temporally very heterogeneous. This study evaluates the costs and benefits of rerouting by incorporating estimates of the social cost of CO₂ and contrail cirrus, applied to nearly half a million flights over the North Atlantic (Johansson et al., 2024). We estimate contrail cirrus formation and RF uncertainty for individual flights using CoCIP and the 10-member ERA5 ensemble from the European Centre for Medium-Range Weather Forecasts (ECMWF) (Teoh, 2022), alongside additional assumptions on forcing and efficacy uncertainty.

We explore the potential climate benefits of rerouting flights to avoid contrail formation, weighing additional fuel burnt against reduced contrail RF. Our results highlight that while rerouting can contribute to climate mitigation, its attractiveness depends on the probability that each rerouting case delivers a net climate benefit. For instance, with a 50% probability threshold (i.e., the median) that a net climate benefit is obtained, 33–35% of flights are beneficial to reroute with a 1% fuel penalty, depending on the social cost assumptions. This proportion decreases to 28–33% for a 5% fuel penalty. Raising the probability to 80% that a net climate benefit is achieved lowers the fraction of flights beneficial to reroute to 27–29% for a 1% fuel penalty and 22–27% for a 5% fuel penalty, where the ranges depend on the social cost assumptions.

In this presentation, we provide further insights from the analysis and present an analysis of the value of improved contrail forcing predictability for more effective climate impact mitigation strategies.

References

Johansson, D. J. A., Azar, C., Pettersson, S., Sterner, T., Stettler, M., & Teoh, R. (2024, May 14). The social costs of aviation: Comparing contrail cirrus and CO2. Research Square Preprints. https://doi.org/10.21203/rs.3.rs-4329434/v1

Teoh, R., Schumann, U., Gryspeerdt, E., Shapiro, M., Molloy, J., Koudis, G., Voigt, C., & Stettler, M. E. J. (2022). Aviation contrail climate effects in the North Atlantic from 2016 to 2021. Atmospheric Chemistry and Physics, 22(22), 10919–10935. https://doi.org/10.5194/acp-22-10919-2022

How to cite: Johansson, D., Azar, C., Pettersson, S., Sterner, T., Stettler, M., and Teoh, R.: Addressing Uncertainty and Rerouting Strategies in Aviation Climate Impact Assessments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15429, https://doi.org/10.5194/egusphere-egu25-15429, 2025.

EGU25-15580 | ECS | Posters on site | AS3.19

Modelling of contrail climate effects with the AviTeam and the CoCiP model 

Kentaro Indo

Currently, contrails and the induced contrail cirrus are estimated to have the strongest contribution to global warming from the aviation sector. However, the uncertainty is still large, primarily because the characteristics of contrails are strongly dependent on the atmospheric conditions at cruise altitude. Therefore, to accurately estimate the climate forcing effects of contrails, both atmospheric data and aircraft activity data must be of high quality and resolution.

The recent deployment of ADS-B transponders on aircraft has provided a new open source of aircraft activity data. The AviTeam, developed by Klenner et al. (2022), uses the ADS-B data to produce spatially and temporarily explicit emission inventories. In our work (Indo, 2024), we couple the AviTeam with the Contrail Cirrus Prediction (CoCiP) model (Schumann, 2012) to simulate the evolution of contrails from a sample of domestic flights in Norway in 2019. The results show the expected pattern of seasonal variability, with the winter (December, January and February) and autumn (September, October and November) months accounting for 81% of the annual total contrail energy forcing. Similarly, the hours between 18:00 and 06:00 were responsible for 93% of the total daily contrail energy forcings. Additionally, it is found that 2% of the flights were responsible for 80% of the annual total contrail energy forcing. Comparing our results with the literature, we also deduce that short-haul flights have significantly less contrail energy forcing per km than long-haul flights, the latter of which typically cruise in higher altitudes and are more likely to fly at night. Thus, our work reveals the specific characteristics of contrails produced by domestic flights in Norway, and also underlines the value of geospatially and temporarily explicit emissions modelling tools such as the AviTeam for modelling contrail climate forcings. Our findings also suggest that flight scheduling could be used as a tool to mitigate contrail climate forcing effects.

 

References

Klenner, J., Muri, H., and Strømman, A. H. (2022). High-resolution modeling ofaviation emissions in Norway. Transportation Research Part D: Transport and Environment, 109:103379. https://www.sciencedirect.com/science/article/pii/S1361920922002073.

Indo, K. (2024). Modelling of contrail climate effects with the AviTeam and the CoCiP model [master’s thesis]. https://hdl.handle.net/11250/3155585.

Schumann, U. (2012). A contrail cirrus prediction model. Geoscientific Model Development, 5(3):543–580. https://gmd.copernicus.org/articles/5/543/2012/.

How to cite: Indo, K.: Modelling of contrail climate effects with the AviTeam and the CoCiP model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15580, https://doi.org/10.5194/egusphere-egu25-15580, 2025.

EGU25-15625 | Posters on site | AS3.19

Uncertainties in contrail modelling of high impact regions 

Kai Widmaier, Dennis Piontek, Simon Kirschler, Roger Teoh, Marc E.J. Stettler, and Christiane Voigt

Aviation impacts Earth’s climate by the formation of contrails, where the largest fraction of the total atmospheric impact is caused by only a small fraction of flights. Forecasting of high impact regions which are likely to produce strongly warming contrails can be achieved with the Lagrangian plume model CoCiP (Contrail cirrus Prediction tool). The model calculates the instantaneous energy forcing per meter flight distance (EFm) during a contrails’ lifetime. It can be operated in two modes: Either along specific flight trajectories or on a 4D grid over an extended area. Simulations depend on meteorological input data and information on aircraft type, heading and contrail overlap. In this study we analyse the impact of these input parameters on the EFm and assess the spatial uncertainty of high-impact regions.

We use the pycontrails open-source implementation of CoCiP to simulate the potential contrail occurrence on a grid over Europe multiple times. We successively vary i) the aircraft type across an ensemble of the 10 most common types, ii) the heading from northward to eastward and iii) the meteorology across the 10-member ensemble of ECMWF ERA5 data for 2019. Additionally, we simulate the contrail formation from historical flight trajectories in 2019 provided by the Global Aviation emissions Inventory based on ADS-B (GAIA), both with and without accounting for contrail radiative interactions.

The standard deviation in EFm is largest for the aircraft ensemble, followed by the meteorology ensemble. This reveals that the aircraft type has significant impact on the climate effect from contrails. Within the aircraft ensemble, 26% of high-impact grid points are agreed upon by all ensemble members, whereas 8% are considered as high impact by only one member. The radiative interaction between contrails leads to a reduction in EFm by 2%, with a stronger effect during night than during daytime. In areas of high air traffic density, the reduction increases up to 5%.

Our results help to assess uncertainties in the prediction of contrail-sensitive airspaces and of individual flights necessary for operational contrail avoidance.

How to cite: Widmaier, K., Piontek, D., Kirschler, S., Teoh, R., Stettler, M. E. J., and Voigt, C.: Uncertainties in contrail modelling of high impact regions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15625, https://doi.org/10.5194/egusphere-egu25-15625, 2025.

EGU25-16019 | ECS | Orals | AS3.19

Numerical investigation of installation effects on condensation trail evolution during the vortex phase. 

Remy Annunziata, Nicolas Bonne, François Garnier, and Marc Massot

Condensation trails (contrails) contribute significantly to the non-CO₂ climate impacts of aviation, with their effect estimated to be up to twice that of CO₂ emissions (Lee et al., 2021). Under specific atmospheric conditions, contrails can persist for several hours, potentially spanning tens of hours. To develop effective strategies for mitigating their climate impact, it is essential to investigate the processes that underlie their formation and evolution.

The formation and evolution of contrails are influenced by various factors, including the aircraft generating them (Unterstrasser et al., 2014). A recent study by Saulgeot et al. (2023) demonstrated that engine position affects the radiative properties of induced contrails. However, this analysis was based on a 2D assumption and initiated calculations at the onset of the vortex phase. Building on and extending this work, we present a 3D numerical study of contrail evolution during the vortex phase for different engine positions. Large-Eddy Simulations (LES) are initialized using Reynolds-Averaged Navier-Stokes (RANS) simulations conducted in the near-field of a realistic aircraft geometry, representative of a Boeing 777.

Three distinct engine positions are analyzed: one at 34% of the wingspan (typical of B-777 or A-320), another at 60% (outboard engine of a B-747), and a more academic configuration at 80%. The latter position aligns the propulsive jet with the wingtip vortex position, as predicted by elliptical wing loading theory, and represent the optimal configuration in the 2D study. Initialization involves extruding a slice of the RANS domain, obtained from prior simulations, onto the LES domain over a length corresponding to the wavelength of Crow instabilities, using the methodology developed by Bouhafid et al. (2024). This approach allows for the simulation of both contrail formation and its subsequent evolution over longer timescales. Microphysical processes, including soot-induced condensation, are modeled using an Eulerian approach (Khou et al., 2015). The simulations will extend up to 5 minutes after the effluent is ejected from the engine.

Simulation results reveal distinct aerodynamic behaviors, particularly in the lifetime of vortex dipoles, which are influenced by variations in jet proximity to wingtip vortices. These differences affect the resulting plumes, influencing both their spatial dispersion and the microphysical properties within them. As a result, the three configurations show variations in ice crystal radii and survival rates. These differences, in turn, impact the optical properties of the contrails, particularly their optical thickness.

How to cite: Annunziata, R., Bonne, N., Garnier, F., and Massot, M.: Numerical investigation of installation effects on condensation trail evolution during the vortex phase., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16019, https://doi.org/10.5194/egusphere-egu25-16019, 2025.

EGU25-16151 | ECS | Orals | AS3.19

Probability of Successful Avoidance of Persistent Contrails 

Wessel Kruin, David Faleiros, Feijia Yin, and Volker Grewe

Contrails are estimated to have one of the largest contributions to aviation’s effective radiative forcing [1]. Fortunately, potential operational and technical measures have been identified to mitigate contrail induced warming. A promising mitigation strategy is to avoid persistent contrail formation through optimised flight trajectories. However, employing such a strategy is currently hampered by the large uncertainties involved in predictions for persistent contrail formation. This uncertainty introduces a risk of unsuccessful or unnecessary detours, resulting in needless extra emissions and fuel burn. Policymakers need to know the magnitude of this risk to carry out mitigation strategies effectively. Yet, estimates of persistent contrail formation are often provided in a deterministic manner, lacking quantifications of uncertainty. Furthermore, earlier studies that do quantify uncertainty often introduce an assumed or simplified uncertainty or propagate a limited scope of uncertainty sources (e.g., [2]). Therefore, instead of simple binary outputs (persistent/non-persistent), this work constructs an approach to quantify the probability of persistent contrail formation for flight waypoints, regarding a wider scope of realistically quantified uncertainty sources than done before.

To quantify the uncertainty of meteorological parameters, we employ the method of Bayesian Model Averaging (BMA) [3]. Using BMA, modelled weather data from ECMWF Reanalysis v5 (ERA5) is calibrated with data from the IAGOS measurement campaign [4]. The calibration process overcomes the bias and under dispersiveness of ERA5 and constructs probability distributions for humidity, temperature and wind. Relevant uncertainties related to the aircraft and its performance are quantified using the variance of these parameters among different estimates of their value.

The obtained uncertainties are propagated to obtain the probability that the condition for contrail formation, the Schmidt-Appleman criterion, is satisfied for waypoints along a flight. Further in the contrail development, we assess the chance that a formed contrail survives the wake downwash phase, to quantify the likeliness of contrail persistence. Moreover, we produce a probabilistic result for potential contrail cirrus coverage (PCC), a parameter representing the fractional area of a grid box in which contrail cirrus can persist once they have been formed. The approach is applied to real flights over the North Atlantic in 2019, from the perspective of an airliner when planning flights for persistent contrail avoidance. We intend to verify the hypothesis that the presented approach reduces the risk of failed avoidance of persistent contrail formation with respect to an approach using binary estimates of contrail persistence.

[1] Lee, D.S. et al. (2021) ‘The contribution of global aviation to anthropogenic climate forcing for 2000 to 2018’, Atmospheric Environment, 244, p. 117834.

[2] Platt, J.C. et al. (2024) ‘The effect of uncertainty in humidity and model parameters on the prediction of contrail energy forcing’, Environmental Research Communications, 6(9), p. 095015.

[3] Raftery, Adrian E., et al. (2005) ‘Using Bayesian model averaging to calibrate forecast ensembles’, Monthly weather review, 133.5, p. 1155-1174.

[4] Petzold, A. et al. (2015) ‘Global-scale atmosphere monitoring by in-service aircraft – current achievements and future prospects of the European Research Infrastructure IAGOS’, Tellus B: Chemical and Physical Meteorology, 67(1), p. 28452.

How to cite: Kruin, W., Faleiros, D., Yin, F., and Grewe, V.: Probability of Successful Avoidance of Persistent Contrails, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16151, https://doi.org/10.5194/egusphere-egu25-16151, 2025.

EGU25-16836 | ECS | Orals | AS3.19

Operational feasibility of contrail avoidance by flight trajectory adaptation: first insights from the German 100-flights-trial 

Simon Kirschler, Dennis Piontek, Marlin Juchem, Alexander Lau, Devaiah Nalianda, Leon B. Schymura, Julian Solzer, Christoph Todt, Kai Widmaier, Zarah Zengerling, and Christiane Voigt

Over the past few decades, research has increasingly revealed the significant impact of non-CO2 emissions from aviation on global warming, with estimates suggesting they may account for as much or even more than the sector's entire CO2 footprint. While aviation produces various non-CO2 emissions, contrail cirrus is identified as one of the most significant contributor to aviation's climate impact. Whereas CO2 emissions linearly correlate to fuel consumption, this is not the case for contrail cirrus effects, making them more challenging to measure and mitigate. This highlights the importance of addressing contrail cirrus effects alongside CO2 and other emission reduction efforts in the aviation industry's pursuit of climate neutrality.

Here, we present first insights from the 100-flights-trial, a contrail avoidance demo trial by the German Aerospace Center (DLR) and the aviation industry tasked by the German federal government. In this trial, aircraft were actively rerouted (pre-tactical) to avoid airspaces with potential warming contrail cirrus formation. Existing models and tools were used to integrate the planning and execution of contrail avoidance flights into the flight operations processes. The analysis presented utilizes real flight data from 25 contrail avoidance flights operated by TUIfly which is then further analyzed using a modelling workflow consisting of DLR’s Trajectory Calculation Module (TCM), the Contrail Cirrus Prediction (CoCiP) model from the open-source pycontrails library, and ECMWF ERA5 reanalysis data. By comparing the originally planned trajectory, the contrail-optimized planned trajectory and the actual flown flight trajectory for each flight, we are able to quantify the effects of mitigation on parameters such as flight time, fuel consumption and the radiation effect of contrails. The methods developed may also be used to investigate the potential of the mitigation strategy and the impact on operational aspects like delay and fuel consumption. In addition, feasibility is considered with regard to airspace restrictions, optional direct routings, but also bad weather. We demonstrate through the implementation of contrail avoidance strategies that there is potential to achieve substantial reductions in the climate impact of contrails at a relatively low cost with comparable flight times. In addition, the choice of climate metric is shown to have little influence on the evaluation of the flights.

How to cite: Kirschler, S., Piontek, D., Juchem, M., Lau, A., Nalianda, D., Schymura, L. B., Solzer, J., Todt, C., Widmaier, K., Zengerling, Z., and Voigt, C.: Operational feasibility of contrail avoidance by flight trajectory adaptation: first insights from the German 100-flights-trial, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16836, https://doi.org/10.5194/egusphere-egu25-16836, 2025.

EGU25-17034 | ECS | Orals | AS3.19

Accurate Contrail Simulation In the Jet and Vortex Phases by Combining Space- and Time-Developing Paradigms 

Denis-Gabriel Caprace, Matthieu Duponcheel, and Philippe Chatelain

Accurate simulation of contrail formation requires to capture the crucial nucleation of ice crystals in the jet phase and their evolution through the vortex phase. During these phases, the dynamics are largely dominated by the engine exhaust jets and the aircraft wake vortices, with turbulent fluctuations that drive the mixing of the hot gases with ambient air. The mixing influences the history of the thermodynamic quantities seen by all ice crystals and may therefore affect their final number concentration and size distribution after the demise of the aircraft wake.
 
A challenge in the simulation of spatially developing aircraft plumes lies in their extremely high aspect ratios, with a length of up to hundreds of kilometers and a cross-sectional dimension of hundreds of meters at most. To bring the computational expenses within a reasonable range, it is customary to simulate the jet and vortex phases separately. The former can be done in a space-developing paradigm. In contrast, the latter usually exploits a space-time analogy to limit the extent of the computational domain, allowing the plume to be aged in a time-developing manner. As a potential limitation of such a segregated approach, the initial condition of the vortex simulations often involves arbitrary assumptions on the velocity field and on the particle distribution. We propose to reconcile the two approaches using a technique to carefully transfer information between space- and time-developing paradigms while maintaining consistency in the momentum balance and particle distributions.
 
This study relies on Large Eddy Simulation performed with the Vortex Particle-Mesh method augmented with a simple ice microphysics model that tracks Lagrangian ice tracers and accounts for condensational growth and sublimation. We present the method itself together with the technique to transform space-developing results into a time-developing initial condition. We then consider a notional twin-engine aircraft with regular Jet fuel. The plume is first simulated in a space-developing manner in a domain of 100 wingspans in length. This case, considered the reference, is compared to time-developing simulations with various initial conditions, using either the presented technique or arbitrary assumptions. We assess the variability in ice crystal properties at the end of the vortex phase from these time-developing simulations and discuss the possible implications for the propagation of uncertainty into the contrail diffusion and dispersion phases.

How to cite: Caprace, D.-G., Duponcheel, M., and Chatelain, P.: Accurate Contrail Simulation In the Jet and Vortex Phases by Combining Space- and Time-Developing Paradigms, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17034, https://doi.org/10.5194/egusphere-egu25-17034, 2025.

EGU25-17191 | ECS | Orals | AS3.19

Comparing high-fidelity LES of early contrail formation with ground-based images 

Raúl Quibén Figueroa, Tânia Ferreira, Catherine Gorlé, and Manuel Soler Arnedo

Contrails have been identified as a principal contributor to aviation’s impact on the atmospheric radiative balance. However, considerable uncertainties remain regarding their effects, highlighting the need for deeper scientific understanding. Consequently, the development of reliable and validated contrail models is critical for accurate prediction and effective mitigation of their climate impact.

This study leverages ground-based camera imagery to identify and track early-stage contrails, providing benchmark data for a high-fidelity solver that simulates initial contrail formation. The solver employs a three-dimensional large-eddy simulation (LES) framework, incorporating an Eulerian–Lagrangian approach for two-phase compressible flow, enabling the simulation of the contrail's jet and vortex regimes over short timescales (<2 minutes). Images from Reuniwatt all-sky cameras capture a 5600 km² region at 30-second intervals, enabling observation of the vortex and initial dissipation regime.

Contrails are manually identified and labeled in the images, while flight trajectories are overlaid using ADS-B information. Atmospheric conditions are derived from reanalysis datasets at flight altitude, and aircraft/engine parameters are estimated from publicly available sources. These inputs are integrated into the simulations to replicate real-world conditions for each case.

By comparing the simulation results with observational data, this study aims to evaluate the reliability and applicability of the model, as well as to shed light on contrail formation mechanisms. Particular attention is given to scenarios where other theoretical approaches and lower-fidelity models have historically been less accurate.

How to cite: Quibén Figueroa, R., Ferreira, T., Gorlé, C., and Soler Arnedo, M.: Comparing high-fidelity LES of early contrail formation with ground-based images, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17191, https://doi.org/10.5194/egusphere-egu25-17191, 2025.

EGU25-17393 | Orals | AS3.19

The Role of vPM Activation in Global Contrail Climate Assessments and Mitigation Implications 

Roger Teoh, Joel Ponsonby, Marc Shapiro, and Marc Stettler

Global aviation contrail climate forcing could match or exceed the forcing from aviation’s cumulative CO2 emissions. Aircraft engine exhaust contains various particles, including non-volatile particulate matter (nvPM), volatile particulate matter (vPM), and ambient aerosols. At cruise altitudes, these particles can activate to form water droplets if the relative humidity in the plume exceeds their activation threshold, where they subsequently freeze into contrail ice crystals. The initial number of contrail ice crystals is primarily driven by the nvPM in “soot-rich” conditions, where the nvPM number emissions index (EIn) exceeds a threshold of around 1014 kg-1; while vPM and ambient aerosols become more likely to activate to form contrail ice crystals under “soot-poor” conditions (nvPM EIn < ~1014 kg-1) (Yu et al., 2024). However, existing global contrail simulation workflows do not currently account for the potential activation of vPM, which may lead to an underestimation of the contrail climate forcing. This underestimation could likely be more significant for flights powered by: (i) cleaner lean-burn combustors, where their nvPM EIn at cruise is typically below 1012 kg-1; or (ii) sustainable aviation fuel (SAF), which can reduce the nvPM EIn by up to 70%.

An analytical model describing the microphysical pathway of contrail formation from nvPM and ambient aerosol particles was developed by Kärcher et al. (2015), which has since been extended to account for the potential activation of vPM in forming contrail ice crystals. Here, we aim to integrate this extended model into the contrail cirrus prediction model (CoCiP) to: (i) provide an updated estimate of the global annual mean contrail net radiative forcing (RF) for 2019; and (ii) quantify the simulated differences in contrail climate forcing between flights powered by conventional (rich-burn) and cleaner lean-burn combustors.

By accounting for vPM activation, our preliminary results estimates that the 2019 global contrail net RF could increase by up to 35%, depending on the assumed vPM properties (EIn and particle size distribution). On average, the contrail climate forcing from lean-burn combustors could be around 50% to 90% lower than that from conventional rich burn combustors. When compared with the simulation without vPM activation, the increase in contrail warming effects due to vPM activation in the exhaust of lean-burn combustors becomes significant only when the ambient temperature is at least 10 K below the Schmidt-Appleman criterion threshold temperature. Further work is ongoing to quantify the contrail mitigation potential from a fleetwide adoption of SAF and cleaner lean-burn engines.

References

Kärcher, B., Burkhardt, U., Bier, A., Bock, L., and Ford, I. J.: The microphysical pathway to contrail formation, Journal of Geophysical Research: Atmospheres, 120, 7893–7927, https://doi.org/10.1002/2015JD023491, 2015.

Yu, F., Kärcher, B., and Anderson, B. E.: Revisiting Contrail Ice Formation: Impact of Primary Soot Particle Sizes and Contribution of Volatile Particles, Environ Sci Technol, 58, 17650–17660, https://doi.org/10.1021/ACS.EST.4C04340, 2024.

 

How to cite: Teoh, R., Ponsonby, J., Shapiro, M., and Stettler, M.: The Role of vPM Activation in Global Contrail Climate Assessments and Mitigation Implications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17393, https://doi.org/10.5194/egusphere-egu25-17393, 2025.

EGU25-17834 | ECS | Posters on site | AS3.19

Occurrence of embedded contrails in cirrus clouds observed with the HALO research aircraft 

Mahshad Soleimanpour, Matthias Tesche, and Silke Groß

Aviation affects the Earth’s energy balance through both non-CO2 effects and exhaust gases and soot emissions. One such effect is the formation of contrails, which can alter the climate impact of cirrus clouds and their optical and microphysical properties. In this study, embedded contrails were detected during active remote sensing observations with the German research aircraft HALO. Using observations during ML-CIRRUS, it is found that embedded contrails can be identified in WALES lidar measurements through particle backscatter coefficients larger than 4 Mm−1 sr−1 and particle linear depolarization ratios (PLDR) below 30% and 43% for clouds with low and high mean PLDR, respectively. The thus identified contrail-affected lidar and lidar-radar measurements during ML-CIRRUS and other HALO campaigns will be used to assess the impact of contrails that form in already existing cirrus clouds on the optical and microphysical properties of those clouds, and in how far potential affects might also be detected in spaceborne lidar observations.

How to cite: Soleimanpour, M., Tesche, M., and Groß, S.: Occurrence of embedded contrails in cirrus clouds observed with the HALO research aircraft, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17834, https://doi.org/10.5194/egusphere-egu25-17834, 2025.

EGU25-18681 | ECS | Orals | AS3.19

Integration of mixed-fidelity aircraft/engine modelling to assess contrail mitigation strategies 

Joseph Ramsay, Indi Tristanto, Shahrokh Shahpar, and Alistair John

Aviation’s environmental impact must be addressed in a multidisciplinary manner, further targeting improvements in CO2 emissions whilst also ensuring reductions in short-term non-CO2 radiative forcing, with particular focus on the largest contributor, aircraft contrails. Considering the challenges and cost associated with experimental measurements, to begin to formulate potential strategies to mitigate the impact of contrails, increased modelling fidelity and accuracy is required. Such work allows for the processes behind a contrail’s evolution to be better understood, whilst investigating key factors which dictate initial formation, particle properties, and climatic impact. From an engineering perspective, the key regions of interest are within the early regimes, covering contrail formation and early dynamics, where choices in aircraft and engine design can impact the initial contrail evolution.

To explore such effects, high fidelity RANS CFD with in-built contrail microphysics has been conducted on a fully featured aircraft geometry and its near-field wake. This allowed for accurate assessment of air vehicle performance, contrail formation, and aerodynamic interactions at cruise flight conditions. The CFD simulations incorporated a developed parametric aircraft model with realistic engine geometry to easily allow modifications in design to be studied and assessed in a multidisciplinary manner with respect to their environmental impact. To further increase the fidelity of the work, a detailed thermodynamic engine cycle model was coupled to the CFD boundary conditions and iterated upon throughout the simulations to ensure appropriate exhaust conditions for cruise flight were attained. Particle emissions at cruise were predicted by a machine learning model dependent on engine design and thrust setting. High level engine design choices, such as bypass ratio, were parametrised, with nacelle sizing requirements linked between the output of the engine model and CAD geometry to ensure installation effects and exhaust interactions were accurately captured, in addition to the required fuel burn and particle emissions. Simulation results from the early regime are intended to assess consistency with reduced fidelity model predictions, as well as to form a parametric input for longer term, global models.

Development of such models allows for aircraft/engine design exploration to be conducted to better understand pathways to potential mitigation of aviation’s environmental impact, inclusive of both CO2 emissions and contrails.

How to cite: Ramsay, J., Tristanto, I., Shahpar, S., and John, A.: Integration of mixed-fidelity aircraft/engine modelling to assess contrail mitigation strategies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18681, https://doi.org/10.5194/egusphere-egu25-18681, 2025.

EGU25-19067 | ECS | Posters on site | AS3.19

Estimating the Climate Effect of Contrails in Mid-Latitudes Using a Lagrangian Framework in the EMAC Model 

Patrick Peter, Sigrun Matthes, Christine Frömming, Simone Dietmüller, and Volker Grewe

Optimizing flight trajectories to reduce the climate effect of non-CO2 aviation emissions - particularly by avoiding contrails and contrail cirrus - represents a promising strategy for mitigating aviation's environmental footprint. This approach depends on detailed knowledge of how localized aviation emissions affect the climate. Previous research has examined the influence of different meteorological conditions on aviation emissions and identified regions particularly sensitive to these effects. Tools like 4-dimensional climate change functions (CCFs) have been developed to assist sustainable air traffic management (ATM) in designing flight trajectories that minimize climate effects. However, these tools have so far been limited to specific regions, seasons, or weather scenarios [1,2].

In this study, we expand the geographic scope of the CCFs by conducting Lagrangian simulations across different extratropical regions of the northern hemisphere. Using the modular ECHAM5/MESSy atmospheric chemistry model (EMAC), we analyze contrail evolution along Lagrangian trajectories, offering insights into the temporal dynamics of contrail formation parameters and their radiative forcing effects. This approach allows for a detailed examination of the physical processes driving contrail-climate interactions, as well as their spatial and temporal variability.

A key advancement over previous CCFs studies is the application of an improved interpolation method, which transforms meteorological parameters from grid boxes onto Lagrangian trajectories with higher precision. Preliminary results indicate that this method enhances the accuracy of contrail property estimates, revealing regional differences in contrail persistence and radiative forcing that were previously unresolved. Our findings highlight the importance of refining modeling techniques to better assess contrail effects on climate at regional and global scales.

This study was funded by the European SESAR programme under Grant Agreement No. 101114785 (CONCERTO) and the German LuFo Project Dkult (Grant Agreement No. 20M2111A). High-performance supercomputing resources were provided by the German CARA Cluster in Dresden and the DKRZ Cluster in Hamburg.

References:  

[1] Matthes, S., Lührs, B., Dahlmann, K., Grewe, V., Linke, F., Yin, F., Klingaman, E. and Shine, K. P.: Climate-Optimized Trajectories and Robust Mitigation Potential: Flying ATM4E, Aerospace 7(11), 156, 2020.

[2]  Frömming, C., Grewe, V., Brinkop, S., Jöckel, P., Haslerud, A. S., Rosanka, S., van Manen, J., and Matthes, S.: Influence of weather situation on non-CO2 aviation climate effects: the REACT4C climate change functions, Atmos. Chem. Phys., 21, 9151–9172, https://doi.org/10.5194/acp-21-9151-2021, 2021.

How to cite: Peter, P., Matthes, S., Frömming, C., Dietmüller, S., and Grewe, V.: Estimating the Climate Effect of Contrails in Mid-Latitudes Using a Lagrangian Framework in the EMAC Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19067, https://doi.org/10.5194/egusphere-egu25-19067, 2025.

EGU25-19677 | ECS | Posters on site | AS3.19

Flying around storms: Structured supersaturation at weather systems 

Oliver Driver, Marc Stettler, and Edward Gryspeerdt

The relative humidity to ice water is crucial to determining whether or not ice crystals in contrails are able to persist. Inaccurate weather model data for this key meteorological input to contrail models is widely appreciated to be the limiting factor in current contrail models to produce accurate contrail persistence statistics. Identifying biases and constraining the inaccuracies in this weather data is needed to enable analysis of contrail models without this as a confounding factor.

Extratropical low pressure systems (storms) in the North Atlantic structure the weather in this region. These storms have a well-understood structure.  Averaging composites of many storm systems is a frequently used method to observe features in both weather model output and observations. We show that a similar method can be used to identify the structures in the contrail-sustaining ice-supersaturated regions, and the regions of flight traffic through them. In-situ humidity observations give an understanding of the accuracy of the meteorological data. Humid features are seen where models are subject to saturation adjustment but can be constrained to an accurate understanding of ice-supersaturation. Conversely, downwelling air—which is typically dry—is not as well constrained when humidity does occur. This work identifies opportunities to begin exploring contrail model validation, but also acts to steer development of more accurate weather models.

How to cite: Driver, O., Stettler, M., and Gryspeerdt, E.: Flying around storms: Structured supersaturation at weather systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19677, https://doi.org/10.5194/egusphere-egu25-19677, 2025.

EGU25-19765 | ECS | Orals | AS3.19

On the long-term propagation of contrails using a novel high-fidelity advection-diffusion model 

Amin Jafarimoghaddam, Manuel Soler, and Irene Ortiz

There is growing evidence suggesting that condensation trails (contrails) contribute to aviation-induced atmospheric warming at least as significantly as carbon dioxide emissions. Mitigating the warming effects of contrails requires the development of effective avoidance strategies, which in turn depend on accurate and computationally efficient contrail models. Contrails undergo multiple formation and evolutionary stages, beginning with their initial formation, progressing through a rapid growth phase, and culminating in their eventual dissipation or conversion into cirrus clouds. The long-term evolution of contrails—particularly their transformation into cirrus clouds—plays a critical role in defining their radiative forcing and climate impact. This stage of evolution is predominantly governed by advection-diffusion processes, coupled with particle-growth dynamics. We propose a novel contrail evolution model based on a coupled system of nonlinear advection-diffusion equations (ADE). This model integrates underexplored or previously neglected influences, including spatiotemporal wind variability, spatiotemporal and nonlinear diffusion coefficients accounting for diffusion limitation behavior, as well as significant ice-particle slip mechanisms. The proposed model is solved using an analytic discretization method, which outperforms classical numerical methods in terms of computational speed and accuracy. The model's performance is further compared against ground-based camera observations of contrails, providing an empirical basis for assessing its predictive capability. In addition, the model introduces several theoretical adjustable parameters, which can be calibrated using ground truth data to optimize its representation of advection-diffusion processes. This adaptability ensures that the model remains robust under varying atmospheric conditions and operational scenarios. By advancing our understanding of contrail dynamics and providing a computationally efficient solution framework, this work lays the foundation for more effective contrail avoidance strategies.

How to cite: Jafarimoghaddam, A., Soler, M., and Ortiz, I.: On the long-term propagation of contrails using a novel high-fidelity advection-diffusion model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19765, https://doi.org/10.5194/egusphere-egu25-19765, 2025.

EGU25-19851 | Posters on site | AS3.19

Contrail detection at nighttime combining lidar, meteorological and system  ADS-B data  

Florian Mandija, Philippe Keckhut, Dunya Alraddawi, and Abdanour Irbah

Cloud formation, especially cirrus type, is affected also by the human activities such is aviation, which emits condensation trails, called contrails. Contrails form and persist under specific environmental conditions. Their formation is conditioned by the fulfillment of the Schmidt–Appleman, and later on their persistence is guaranteed over the ice supersaturated regions. These conditions, use the air temperature and relative humidity related to water and ice as criteria for their formation and persistence. These criteria depend, not only on the meteorological conditions but also on the aircraft specification, their fuel type, engine efficiency, etc.

One interesting topic of the contrail effects is the investigation of their contribution on the formation of the cirrus clouds. The formation of the cirrus clouds requires generally significantly higher relative humidity then the contrail persistence conditions. In this way, the investigation of the persistent contrails with relative humidity lower than cirrus clouds need to be formed, enable to have insight over the contribution of the contrails on the cirrus formation.

Currently, we have a 20-year database that allows us to do statistics but at night, which requires us to develop methods for differentiating clouds and contrails. Lidar backscattering profiles are collocated with system ADS-B data of the flight overpassing the Observatory of Haute-Provence in France. Detailed information about the flight routes and meteorological conditions, associated with the contrail properties have been analyzed statistically and case by case.

Here, statistics of the contrail formation and persistence conditions over the site is presented. The events have been classified into five cases; persistent, non-persistent, potential, uncertain and no contrails. The geometrical and optical properties of the contrails, as well as related meteorological variables provided by ERA5, are grouped according to this classification. The principal factor analyses on the contrail parameters is performed and their outputs have been clustered to identify better the main features of the most important parameters.

In addition to these statistics, some special cases of the contrail events have been analysed. The information provided by system  ADS-B collocated with the lidar vertical-resolved profiles identify and follow up the evolution of the contrails over the site. Their mean altitude, geometrical thickness, spatial orientation, timespan, width, optical depth and their persistency have been analysed in thoroughly. To have adequate determination and discrimination of the contrail spots, sensitivity analyses have been performed for the backscattering ratio, and their spatial and temporal distances between their neighbors. In short, complementary analyses, using statistics and cases studies, is performed to clarify the features of the contrail main properties.

How to cite: Mandija, F., Keckhut, P., Alraddawi, D., and Irbah, A.: Contrail detection at nighttime combining lidar, meteorological and system  ADS-B data , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19851, https://doi.org/10.5194/egusphere-egu25-19851, 2025.

EGU25-19879 | ECS | Orals | AS3.19

Assessing Contrail Radiative Effects: A Comparison of MTG Satellite Detections and Physics-Based Simulations 

Irene Ortiz, Abolfazl Simorgh, Javier García-Heras, Ermioni Dimitropoulou, Pierre De Buyl, Nicolas Clerbaux, and Manuel Soler

The increasing impact of aviation on global climate change underscores the critical need for accurate quantification of its environmental effects. Among them, persistent contrails and aviation-induced cloudiness are recognized as the most significant contributors, yet the quantification of their effects remains the most uncertain [1]. During the last decades, physics-based models, which involve the simulation of contrail formation, evolution, and radiative forcing by integrating aircraft specifications and meteorological data, have been the primary tools for large-scale quantification and estimation of contrail impacts [2]. Recently, data-driven methods that leverage neural networks for satellite identification combined with radiative transfer (RT) models to estimate shortwave and longwave cloud radiative effects have emerged as reliable alternatives due to their strong foundation in observational data [3]. The alignment between these two approaches, data-driven and physics-driven, has not been thoroughly explored in the literature, despite its critical importance for ensuring consistency and reliability in studies aimed at reducing uncertainties in the assessment of contrail-related climate impacts. In this work, we perform a comparison over four full days, focusing primarily on the European domain as captured by the Flexible Combined Imager (FCI) onboard the Meteosat Third Generation (MTG)-I geostationary satellite. We compare contrail effects obtained applying an RT model on segmented contrails with a tailored neural network, with per-trajectory contrail effects simulated using the Contrail Cirrus Prediction model (CoCiP) [4] and Automatic Dependent Surveillance—Broadcast (ADS-B) flight data across multiple timeframes. This flight data accounts for time intervals extending up to two hours prior to each satellite image capture, to account for the delay in contrail visibility on the satellite. To address meteorological uncertainties, an ensemble approach uses 10 weather scenarios derived from ERA5 reanalysis data obtained from the European Centre for Medium-Range Weather Forecasts (ECMWF). Since RT simulations provide only instantaneous forcing, detected contrails in the satellite imagery are tracked over time, and the accumulated radiative forcing is calculated and compared to that of the simulated contrails. Overall, this study offers valuable insights into the agreement between observational and physics-based approaches across several key aspects: I) contrail formation, II) contrail lifetime, and III) contrail climate impacts.

[1] David S. Lee, David W. Fahey, Piers M. Forster, Peter J. Newton, Ron C. N. Wit, Ling L. Lim, Bethan Owen, and Robert
Sausen. Aviation and global climate change in the 21st century. Atmospheric Environment, 43(22):3520–3537, July 2009.
[2] Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc Stettler.
Global aviation contrail climate effects from 2019 to 2021. EGUsphere, 2023:1–32, 2023.
[3] Irene Ortiz, Ermioni Dimitropoulou, Pierre de Buyl, Nicolas Clerbaux, Javier García-Heras, Amin Jafarimoghaddam,
Hugues Brenot, Jeroen van Gent, Klaus Sievers, Evelyn Otero, Parthiban Loganathan, and Manuel Soler. Satellite-Based
Quantification of Contrail Radiative Forcing over Europe: A Two-Week Analysis of Aviation-Induced Climate Effects,
November 2024. arXiv:2409.10166 [physics].
[4] U. Schumann. A contrail cirrus prediction model. Geoscientific Model Development, 5(3):543–580, May 2012. Publisher:
Copernicus GmbH.

How to cite: Ortiz, I., Simorgh, A., García-Heras, J., Dimitropoulou, E., De Buyl, P., Clerbaux, N., and Soler, M.: Assessing Contrail Radiative Effects: A Comparison of MTG Satellite Detections and Physics-Based Simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19879, https://doi.org/10.5194/egusphere-egu25-19879, 2025.

EGU25-20111 | Posters on site | AS3.19

The Contrail OBservations And Lifecycle Tracking (COBALT) project - Observations and initial results 

Edward Gryspeerdt, Lindsay Bennett, Oliver G. A. Driver, Alex Fearn, Ryan R. Neely III, Marc E. J. Stettler, Christopher J. Walden, and Daniel Walker
Aircraft are a growing proportion of the human forcing of the climate system, with the majority of their warming effect coming from their impact on clouds. Accurate modelling of these impacts is essential for guiding climate mitigation choices, but there are limited observations available to evaluate the capability of these models.  Matching aircraft tracks to data from a cloud radar, an array of ground-based cameras and satellite observations, the Contrail OBservations And Lifecycle Tracking (COBALT) project is constructing an evaluation dataset for models of contrails and aircraft impacts on existing cloud.                                             
                                                                                                               
Here we present the design of the COBALT observations, along with initial results for data collected over the southern UK in late 2024/early 2025. Matching the ground-based observations to satellite data, we build up a composite picture of contrail evolution behind specific aircraft from the first minutes of the contrail lifecycle to several hours after formation. This provides a unique dataset for contrail model evaluation and will help guide future observational studies to further assess the non-CO2 impact of aircraft on climate.

How to cite: Gryspeerdt, E., Bennett, L., Driver, O. G. A., Fearn, A., Neely III, R. R., Stettler, M. E. J., Walden, C. J., and Walker, D.: The Contrail OBservations And Lifecycle Tracking (COBALT) project - Observations and initial results, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20111, https://doi.org/10.5194/egusphere-egu25-20111, 2025.

EGU25-20263 | Posters on site | AS3.19

A Modular, Object-Oriented Python Framework for Advanced SAF Microphysics Modelling 

Padraig Donnelly, Nicolas Bonne, and Margaux Vals

Sustainable aviation fuels (SAF) offer a promising pathway to mitigate the climate impacts of aviation by reducing contrail formation. The VOLCAN project utilises ONERA’s advanced 1D microphysical model MoMiE1, 2 (Modèle Microphysique pour Effluents) to assess SAF's effects on exhaust plumes and contrail characteristics across various fuel types and combustion modes. Written in FORTRAN, MoMiE offers exceptional computational efficiency and a robust set of libraries suitable for high-performance scientific computing. However, its rigidity can slow down development cycles and make the code less adaptable to the rapid iteration often required in research and development settings, such as in the testing of new types of sustainable aviation fuels. Currently, MoMiE supports the modelling of heterogeneous freezing on soot particles activated by sulfuric acid and organic species, homogeneous freezing of liquid sulphate and organic droplets, and the competition between these modes. Additional features include the representation of chemiionisation, Brownian coagulation, and the growth and sublimation of ice crystals. However, these processes are hardcoded into the code base, making it cumbersome to run a variety of experiments with supported species and difficult to expand to cover novel fuel scenarios.

To address these challenges, we discuss a modern, object-oriented, and modular Python-based approach tailored for emerging numerical modelling experiments of SAFs. We aim to retain the above functionality while providing a robust framework for future code development. Core components, including aerosol and molecular species distributions, scientific models (nucleation mechanisms), and thermodynamic calculations, are encapsulated within distinct Python classes, ensuring a clear separation of concerns and facilitating focused updates and development. The model objects are configured a priori with user-defined configuration files. These files specify molecular species relevant to specific fuel or burn scenarios, as well as different scientific models, nucleation schemes, experimental data sets etc., ensuring the code remains extensible without disrupting its foundational framework. In addition, all operational parameters and physical constants are externalised, making the code more flexible and encouraging maintainable, transparent coding practices. Python classes are instantiated dynamically during runtime, rather than being pre-defined at model start-up. This approach avoids unnecessary dependencies and ensures that objects are created only when needed, optimising memory usage and maintaining computational efficiency. We will explore preliminary results of quantitative scientific comparison with MoMiE in a few test cases and performance benchmarking.

The proposed development aims to replicate and extend the capabilities of 1D simulations in MoMiE, employing a design philosophy that supports scalability and adaptability. This approach aligns with the evolving scientific and operational demands of SAF research, enabling detailed and flexible modelling of complex microphysical processes.

1Vancassel X. et al., Numerical simulation of aerosols in an aircraft wake using a 3D LES solver and a detailed microphysical model, International Journal of Sustainable Aviation, 2014

2Rojo C. et al., Impact of alternative jet fuels on aircraft-induced aerosols, Fuel, 2014

How to cite: Donnelly, P., Bonne, N., and Vals, M.: A Modular, Object-Oriented Python Framework for Advanced SAF Microphysics Modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20263, https://doi.org/10.5194/egusphere-egu25-20263, 2025.

Wild (2020), and Wild and Bosilovich (2024) provide estimates of global mean energy balance components as represented in climate models and reanalyses, with reference estimates from Loeb et al. (2018), Wild et al. (2015, 2019), L’Ecuyer et al. (2015) and Kato et al. (2018). Here we add a theoretical reference estimate (TRE) based on four radiative transfer equations and geometric considerations as detailed in Zagoni (2025). The equations do not refer to the atmospheric gaseous composition or the reflective properties of the surface or clouds. The first equation is a clear-sky constraint relationship on the net radiation at the surface (RN), following from the two-stream approximation of Schwarzschild’s (1906-Eq.11) radiative transfer equation as given in standard university textbooks on atmospheric physics and radiation (Goody, Oxford, 1964_Eq.2.115; Houghton, Cambridge, 1977_Eq.2.13; Hartmann, Academic Press 1994, Eqs. 3.51-3.54;  Ambaum, RoyalMetSoc, 2021_Eq.10.56), and in university lecture notes (Stephens 2003): RN=OLR/2. The second equation is a clear-sky constraint relationship on the total radiation at the surface (RT), following from the simplest greenhouse geometry (Hartmann 1994, Fig.2.3): RT=2OLR. The third and fourth equations are all-sky versions of the first pair: RN(all-sky)= (OLR–LWCRE)/2, and RT(all-sky)=2OLR+LWCRE. Two decades of CERES observations (EBAF Ed4.1 April 2000–March 2022) give –2.33, –2.82, 2.71 and 2.44 [Wm-2] deviations for the four equations, respectively, with a mean difference of 0.00. The all-sky equations are justified by an independent estimate of GEWEX within 0.1 Wm-2 (Zagoni 2024). The solution can be given in small integer ratios relative to LWCRE as the unit flux; the best fit is 1 unit = 26.68 Wm-2, see Table1 (highres figures and other info about TRE available at TABLELINK). Some of the most remarkable precisions are in TOA SW up all-sky (=100) and clear-sky (=53). — Li, Li, Wild and Jones (2024) provide a global radiation budget from a surface perspective from 34 CMIP6 models for 2000-2022, with differences from the TRE integer positions less than 1 Wm-2 in SW down radiation, Thermal down Surface and the convective flux (Sensible heat + Latent heat); less than 2 Wm-2 in Thermal up Surface; and less than 3 Wm-2 in Reflect by surface; each within the noted ranges of uncertainty. Stackhouse et al. (2024) give Earth radiation budget at top-of-atmosphere; TRE differ from 2001-22 Climatological Mean in OLR, TSI and RSW by 0.23, 0.03 and 1.05 [Wm-2], see details in TABLELINK in References.

 

References

Li, X., Li, Q., Wild, M. and Jones, P. (2024) An intensification of surface EEI. NatureCommE&E, https://www.nature.com/articles/s43247-024-01802-z

Stackhouse, P., et al. (2024) State of the Climate 2023, Bull. Am. Met. Soc. 105:8, https://journals.ametsoc.org/view/journals/bams/105/8/2024BAMSStateoftheClimate.1.xml

Stephens, G. (2003) Colorado_State_University_AT622_Section 6_Eqs. (6.10a)-(6.10b), Example 6.3, Fig. 6.3a, https://reef.atmos.colostate.edu/~odell/AT622/stephens_notes/AT622_section06.pdf

Wild, M. (2020) The global energy balance as represented in CMIP6 climate models. Climate Dynamics 55:553–577, https://doi.org/10.1007/s00382-020-05282-7

Wild, M., Bosilovich, M. (2024) The global energy balance as represented in reanalyses. Surv Geophys, https://link.springer.com/article/10.1007/s10712-024-09861-9

Zagoni, M. (2024) Modeling and Observing Global Energy and Water Cycles by GEWEX. AGU Fall Meeting, https://agu.confex.com/agu/agu24/meetingapp.cgi/Paper/1535956

Zagoni, M. (2025) Trenberth’s Greenhouse Geometry. AMS Annual Meeting, https://ams.confex.com/ams/105ANNUAL/meetingapp.cgi/Paper/445222  see also the updated Supplementary Material video: https://www.earthenergyflows.com/Zagoni-EGU2024-Trenberths-Greenhouse-Geometry_Full-v03-480.mp4

TABLELINK: https://earthenergyflows.com/TRE20.pdf

How to cite: Zagoni, M.: Theoretical reference estimate for the components of the global energy balance, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1, https://doi.org/10.5194/egusphere-egu25-1, 2025.

EGU25-27 | Orals | CL2.1

Observational evidence of strong aerosol fingerprints on clouds and effect on radiative forcing 

Ying Chen, Jim Haywood, Yu Wang, Florent Malavelle, George Jordan, Amy Peace, Daniel Partridge, Nayeong Cho, Lazaros Oreopoulos, Daniel Grosvenor, Paul Field, Richard Allan, and Ulrike Lohmann

Aerosol-cloud-interactions (ACI) is a leading uncertainty in estimates of their radiative forcing and hence for climate projection. The aerosol radiative forcing obtained from climate models is poorly constrained by observations, because the ACI signal is frequently entangled with noise of meteorological co-variability.

       The Iceland-Holuhraun volcanic eruption in Iceland in 2014 provided an unprecedented opportunity to examine ACI of marine low-level clouds and how well they are represented in climate models. Malavelle et al. (2017) used Collection 5 data from the MODIS Aqua satellite and provided an assessment of the impact of the large release of sulfur dioxide on cloud effective radius (reff) and cloud liquid water path (LWP), finding a considerable impact on the former, but no impact on the latter. We revisit this eruption with a considerably extended satellite record which includes new Collection 6 data from the Terra and Aqua satellite and additional years of data from 2015-2020. This tripling of satellite data allows using novel data-science approach for a more rigorous assessment of ACI, including the impacts not just on cloud micro-physical properties (reff and LWP), but also on the macro property cloud coverage (Chen et al., 2022).

These results show that cloud fraction is significantly increased by 10% and appears to surpass cloud brightening and to be the dominant factor in aerosol indirect radiative cooling. The ACI cooling effect via increasing of cloud cover is even more remarkable in tropics (Fig.1, upto 50%), as demonstrated by our recent study of Hawaii volcanic natural experiments (Chen et al., 2024). Climate models are unable to replicate such strong impacts on cloud cover. These results show that the ongoing debate about the cooling impact of aerosols is far from over while climate models continue to inadequately represent the complex macro- and micro-physical impacts of ACI. These researches point towards a direction and provide new constraints for improving model representation of ACI.

Figure 1. Aerosol-induced changes in cloud cover from volcano natural experiments. Source: Chen et al., (2024)

 

 

References:

Chen, Y., Haywood, J., Wang, Y., Malavelle, F., Jordan, G., Partridge, D., Fieldsend, J., De Leeuw, J., Schmidt, A., Cho, N., Oreopoulos, L., Platnick, S., Grosvenor, D., Field, P., and Lohmann, U.: Machine learning reveals climate forcing from aerosols is dominated by increased cloud cover, Nature Geoscience, 10.1038/s41561-022-00991-6, 2022.

Chen, Y., Haywood, J., Wang, Y., Malavelle, F., Jordan, G., Peace, A., Partridge, D. G., Cho, N., Oreopoulos, L., Grosvenor, D., Field, P., Allan, R., and Lohmann, U.: Substantial cooling effect from aerosol-induced increase in tropical marine cloud cover, Nature Geoscience, https://doi.org/10.1038/s41561-024-01427-z, 2024.

Malavelle, F., Haywood, J., Jones, A. et al. Strong constraints on aerosol–cloud interactions from volcanic eruptions. Nature 546, 485–491 (2017). https://doi.org/10.1038/nature22974

 

How to cite: Chen, Y., Haywood, J., Wang, Y., Malavelle, F., Jordan, G., Peace, A., Partridge, D., Cho, N., Oreopoulos, L., Grosvenor, D., Field, P., Allan, R., and Lohmann, U.: Observational evidence of strong aerosol fingerprints on clouds and effect on radiative forcing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-27, https://doi.org/10.5194/egusphere-egu25-27, 2025.

EGU25-601 | ECS | Orals | CL2.1

Impact of Aerosol Optical Properties on Surface reaching Shortwave Radiation over Delhi in WRF-Chem 

Sumit Kumar, Gaurav Govardhan, and Sachin Ghude

The Earth's radiation budget is a fundamental determinant of climate dynamics, serving as the primary energy source for the planet and influencing its climate system's evolution. Aerosols, as a climate forcer, modify the distribution of solar radiation in the atmosphere and reduce the radiation reaching the Earth's surface. 

The Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) is actively used in operational air quality forecasting systems across the globe. Previous studies have shown that the model has limited success in predicting the air quality over the Indian national capital, New Delhi, especially when the Air Quality Index is in ‘Severe’ conditions during the winter months. It has been reported that the model depicts a mean bias of ~ 34 Wm-2 in downward shortwave radiation (SWDOWN) flux reaching the surface which may have led to overestimated near-surface temperature (~3.18 ⁰C). This warm bias in temperature might lead to a greater vertical dispersion of the near-surface pollutants, leading to an underestimation of air quality close to the surface. Such biases in the SWDOWN can be due to inadequate information of optical properties of aerosols in the model.  

This study aims to address this gap by incorporating realistic complex refractive indices of aerosol species into WRF-Chem simulations over the ambient environment of Delhi. Five sensitivity experiments (EXP) were conducted, focusing on the impact of aerosol optical properties on the radiative fluxes during the winter season of 2023-24. The results demonstrate that altering a single aerosol optical parameter leads to a reduction in surface shortwave radiation flux by 28–30 Wm⁻² during October and November, and 25 Wm⁻² during December and January, relative to control simulations. Model outputs, validated against observational data, indicate a reduction in the mean bias of SWDOWN by 12.99 Wm⁻² and 17.24 Wm⁻² in December and January, respectively. These results underscore the significant role of aerosol optical properties in modulating radiative fluxes and their implications for the surface energy budget. 

The study also examines the impacts of modified radiation parameterization on the model-simulated aerosol fields like the near-surface PM2.5 concentration using ground-based measurements and the Aerosol Optical Depth (AOD) over the region as space-based measurements from instruments like MODerate resolution and Imaging Spectroradiometer (MODIS) onboard the TERRA and AQUA satellites. Preliminary findings, revealing the impact of radiation bias on the simulation of meteorological variables and subsequent weather events, will be presented during the session of EGU 2025.

How to cite: Kumar, S., Govardhan, G., and Ghude, S.: Impact of Aerosol Optical Properties on Surface reaching Shortwave Radiation over Delhi in WRF-Chem, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-601, https://doi.org/10.5194/egusphere-egu25-601, 2025.

EGU25-633 | Orals | CL2.1

Atmospheric Radiation Laboratory (ARL) in Monsoon core zone: A unique research facility in Central India 

Burrala PadmaKumari, Anil Kumar Vasudevan, Udaya Kumar Sahoo, Jeni Victor, Yang Lian, Libin Tr, Mahesh Nikam, Sanket Kalgutkar, and Pandithurai Govindan

The Central India (CI), wherein synoptic-scale disturbances (monsoon lows and depressions) frequently pass through during the monsoon season, is identified as a monsoon core zone where detailed long-term atmospheric measurements of convection, clouds, precipitation, and radiation are overdue.

Considering the importance of observational and analytical research in this area, an Atmospheric Research Testbed in Central India (ART-CI) is established by the Ministry of Earth Sciences, Government of India. ART-CI is a huge permanent observational facility envisioned as a national research testbed with multiple laboratories (aerosol, radiation, cloud and precipitation measurements) and scientific user facilities similar to the international Atmospheric Radiation Measurement (ARM) site, USA.

Our climate system is largely determined by the Earth’s Radiation Budget, and is significantly influenced by drastic changes in clouds, aerosols, and greenhouse gases. Hence, to have long-term surface observations for monitoring the changes/trends in the Surface Radiation Budget, important for climate monitoring and prediction, Atmospheric Radiation Laboratory (ARL) is established in August 2023, as a part of the major research facility ART-CI. At ARL, a suite of radiation sensors was installed for continuous measurements of all components of solar and terrestrial radiation (such as total, direct and diffuse shortwave, long-wave, net and UV radiations) co-located with all other atmospheric data instrumentation.

Thus, this unique facility will have an extensive set of state-of-the-art observational systems that will provide continuous observations of land surface properties and surface energy budget. Site description, instrumentation and science plan of this new facility with initial results will be presented.

How to cite: PadmaKumari, B., Vasudevan, A. K., Sahoo, U. K., Victor, J., Lian, Y., Tr, L., Nikam, M., Kalgutkar, S., and Govindan, P.: Atmospheric Radiation Laboratory (ARL) in Monsoon core zone: A unique research facility in Central India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-633, https://doi.org/10.5194/egusphere-egu25-633, 2025.

EGU25-849 | ECS | Posters on site | CL2.1

Upper Tropospheric Humidity and Cloud Radiative Forcing: A Tropical Perspective 

Devika Moovidathu Vasudevan, Ajil Kottayil, and Viju O John

Earth's energy budget defines the balance between the incoming radiant solar energy reaching Earth and the energy returning to outer space. Clouds play a significant role in Earth's energy budget. Cloud Radiative Forcing (CRF) is the difference between the radiative fluxes at the top of the atmosphere in clear-sky and all-sky conditions. Clouds introduce two contrasting effects on the Earth's energy balance: the albedo effect and the longwave effect. Clouds reflect a large amount of incoming shortwave radiation and cool the Earth, known as the Albedo effect. The energy associated with the albedo effect is known as shortwave cloud radiative forcing (SWCRF). The longwave effect or longwave cloud radiative forcing (LWCRF) denotes the warming of Earth by the cloud-trapped longwave radiation that would otherwise escape to space. Understanding the variability in the amount and distribution of clouds in a warming climate is essential as they modulate the shortwave and longwave cloud radiative feedbacks (Harrison et al., 1990; Bony, S. et al., 2006) and, thereby, the Net CRF. Upper Tropospheric Humidity (UTH) is a vital climate variable that impacts the amount of outgoing longwave radiation. In the tropics, UTH is mainly driven by deep convection. The present study analyzes the influence of UTH on the longwave cloud radiative forcing in the tropics from 2000 to 2021. This study uses the satellite microwave (MW) and infrared (IR) UTH measurements. Clouds affect IR UTH measurements, while MW measurements provide UTH under all sky conditions. Clouds and the Earth's Radiant Energy System (CERES) satellite datasets are used to calculate cloud radiative forcing. This study quantifies the UTH-LWCRF relationship and shows that UTH can explain LWCRF variability in the tropics to a large extent. The joint distribution analysis shows that UTH has a significant impact on the variability of LWCRF over land, whereas over ocean regions, sea surface temperature plays a role in modulating the UTH-LWCRF relationship. Also, the UTH-LWCRF relationship is better represented with MW UTH than IR UTH, which can be attributed to the more comprehensive and accurate MW measurements even in cloudy conditions.

How to cite: Moovidathu Vasudevan, D., Kottayil, A., and O John, V.: Upper Tropospheric Humidity and Cloud Radiative Forcing: A Tropical Perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-849, https://doi.org/10.5194/egusphere-egu25-849, 2025.

EGU25-1626 | Orals | CL2.1

Investigation of Dust‐Induced Direct Radiative Forcing Over the Arabian Peninsula Based on High‐Resolution WRF‐Chem Simulations 

Rama Krishna Karumuri, Hari Prasad Dasari, Harikishan Gandham, Ravi Kumar Kunchala, Raju Attada, Ashok Karumuri, and Ibrahim Hoteit

This study investigates the impact of dust on radiation over the Arabian Peninsula (AP) during the reported high, low, and normal dust seasons (March-August) of 2012, 2014, and 2015, respectively. Simulations were performed using the Weather Research and Forecasting model coupled to a Chemistry module (WRF‐Chem). The simulated seasonal horizontal and vertical dust concentrations, and their interannual distinctions, match well with those from two ground‐based AERONET observations, and measurements from MODIS and CALIOP satellites. The maximum dust concentrations over the dust‐source regions in the southern AP reach vertically up to 700 hPa during the high dust season, but only up to 900– 950 hPa during the low/normal dust seasons. Stronger incoming low‐level winds along the southern Red Sea and those from Iraq bring in higher‐than‐normal dust during the high-dust summers. We conducted a sensitivity experiment by switching off the dust module to assess the radiative perturbations due to dust. The results suggest that active dust‐module improved the fidelity of simulated radiation fluxes distributions at the surface and top of the atmosphere vis‐à‐vis Clouds and the Earth's Radiant Energy System (CERES) measurements. Dust results in a 26 Wm− 2 short‐wave (SW) radiative forcing in the tropospheric column over the AP. The SW radiative forcing increases by another 6–8 Wm− 2 during the high dust season due to the increased number of extreme dust days, which also amplifies atmospheric heating. During extreme dust days, the heating rate exhibits a dipolar structure, with cooling over the Iraq region and warming of 40%–60% over the southern‐AP.

How to cite: Karumuri, R. K., Dasari, H. P., Gandham, H., Kunchala, R. K., Attada, R., Karumuri, A., and Hoteit, I.: Investigation of Dust‐Induced Direct Radiative Forcing Over the Arabian Peninsula Based on High‐Resolution WRF‐Chem Simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1626, https://doi.org/10.5194/egusphere-egu25-1626, 2025.

Climatic impacts of historical volcanism are principally tied to the eruption size, while observation versus model discrepancies have been commonly attributed to the uncertainties in paleo‐ reconstruction or malpresentation of volcanic aerosols in models. Here we present convergent evidence for
significant compensation effect of ocean latent heat (LH) in balancing the tropical volcanic‐induced heat loss, by introducing an effective perturbation ratio which is found to decrease with increasing eruption magnitude. Four LH compensation hot spots overlapping with the trade wind regions are identified, together with three western boundary currents regions with intensified LH loss. Comparison between the 1258 Samalas and 1452 Unidentified eruptions suggests considerable modulation of the concurring El Nino‐Southern Oscillation on LH anomaly, which is further verified by CESM large ensemble sensitivity experiments. This study depicts how the interplay between the ocean and the atmosphere could contribute to the overall resilience of the climate system in the face of volcanic disturbances.

How to cite: Gao, C. and Gao, Y.: Dwindling Effective Radiative Forcing of Large Volcanic Eruption: The Compensation Role of Ocean Latent Heat Flux, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1674, https://doi.org/10.5194/egusphere-egu25-1674, 2025.

EGU25-2516 | Posters on site | CL2.1

The Global Energy Balance as represented in Atmospheric Reanalyses 

Martin Wild and Michael Bosilovich

The representation of the global mean energy balance components in 10 atmospheric reanalyses is assessed and compared with recent reference estimates as well as the ones simulated by the latest generation of climate models from the 6th phase of the coupled model intercomparison project (CMIP6). Despite the assimilation of comprehensive observational data in reanalyses, the spread amongst the magnitudes of their global energy balance components generally remains substantial, up to more than 20 Wm-2 in some quantities, and their consistency is typically not higher than amongst the much less observationally constrained CMIP6 models. Relative spreads are particularly large in the reanalysis global mean latent heat fluxes (exceeding 20%) and associated representation of the intensity of the global water cycle, as well as in the energy imbalances at the Top-of-Atmosphere and surface. A comparison of reanalysis runs in full assimilation mode with corresponding runs constrained only by sea surface temperatures reveals marginal differences in their global mean energy balance components. This indicates that discrepancies in the global energy balance components caused by the different model formulations amongst the reanalyses are hardly alleviated by the imposed observational constraints from the assimilation process. Similar to climate models, reanalyses overestimate the global mean surface downward shortwave radiation and underestimate the surface downward longwave radiation by 3 - 7 Wm-2. While reanalyses are of tremendous value as references for many atmospheric parameters, they currently may not be suited to serve as references for the magnitudes of the global mean energy balance components.

 

Published as:

Wild, M., and  Bosilovich, M., 2024: The Global Energy Balance as Represented in Atmospheric Reanalyses, Surveys in Geophysics,  45, 1799–1825. https://doi.org/10.1007/s10712-024-09861-9

How to cite: Wild, M. and Bosilovich, M.: The Global Energy Balance as represented in Atmospheric Reanalyses, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2516, https://doi.org/10.5194/egusphere-egu25-2516, 2025.

Defined as the proportion of solar radiation transmitted through the atmosphere to the Earth's surface, the clearness index (CI) is a vital parameter widely applied in characterizing atmospheric transmittance and sky conditions. However, its application accuracy remains inadequately investigated. This study enhances the understanding and application of CI through three key advancements:

  • Establishing CI Thresholds for Sky Conditions: Standardized CI thresholds for clear-sky (>0.7) and overcast-sky (<0.2) conditions are proposed using synoptic total cloud cover, refining the previously broad ranges. Their logarithmic relationship with solar elevation angles enables accurate identification of sky conditions throughout the day.
  • Advancing Physical Threshold Testing: A CI-DF polynomial envelope, combining CI and diffuse fraction (DF), is introduced to enhance the physical threshold testing procedure. This innovation automatically and effectively filters out outliers, particularly the often-overlooked abnormally low values, thus improving the quality control of surface observations.
  • Developing a Radiation Decomposition Model: A model is established to accurately estimate direct radiation at daily and hourly scales, leveraging the logistic growth relationship between CI and the direct clearness index. This supports the growing global transition to renewable energy applications.

These findings highlight the importance of more accurate applications of CI in atmospheric radiation and energy meteorology studies.

How to cite: Wang, Y.: Enhancing the Understanding and Application of the Clearness Index, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3081, https://doi.org/10.5194/egusphere-egu25-3081, 2025.

EGU25-4221 | ECS | Orals | CL2.1

Investigating trends, variability in observed and simulated upper tropospheric humidity and outgoing longwave radiation 

Thea Stevens, Richard Allan, Michaela Hegglin, Alejandro Bodas-Salcedo, and Viju John

Upper tropospheric humidity (UTH) is a diagnostic of the atmospheric water cycle and strongly contributes to climate sensitivity. Therefore, it is important to understand UTH variability and how this is represented by global climate models. Here, infrared and microwave brightness temperature observations and satellite simulations based on ECMWF Reanalysis v5 (ERA5) and the Hadley Centre Global Environment Model version 3 (HadGEM3) Atmospheric Model Intercomparison Project (AMIP) data are used to evaluate and characterise UTH variability since 1979. UTH satellite observations have been simulated using a radiative transfer code (RTTOV) from ERA5 and HadGEM3 to provide a more direct comparison of the model and reanalysis to observations.

We present results on the sensitivities of water vapour brightness temperatures. There are competing influences of temperature and specific humidity on the brightness temperatures. The effect of these is such that fluctuations can be considered as a proxy for relative humidity. Despite this, a spurious increase in UTH of up to 1% is identified for a 1K increase in profile temperature when relative humidity remains constant.

We also investigate trends and variability of UTH. Using Principal Component Analysis, we explore the spatial and temporal impact of El Niño Southern Oscillation (ENSO) on UTH distribution and link this to changes in outgoing longwave radiation (OLR). Trends show increased UTH over the Indian Ocean and decreases over the western Pacific. This mirrors large-scale dynamic changes in the Walker Circulation, which shows a weakening of the circulation over the same period.

How to cite: Stevens, T., Allan, R., Hegglin, M., Bodas-Salcedo, A., and John, V.: Investigating trends, variability in observed and simulated upper tropospheric humidity and outgoing longwave radiation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4221, https://doi.org/10.5194/egusphere-egu25-4221, 2025.

EGU25-4577 | Orals | CL2.1

Multi-Decadal Trends of Solar Radiation Reaching the Surface Determined by Aerosol-Cloud-Radiation Interactions, Climate Change, and Anthropogenic Emissions 

Mian Chin, Huisheng Bian, Martin Wild, Donifan Barahona, Hongbin Yu, Yun Qian, Anton Darmenov, Paul Stackhouse, Norman Loeb, Rachel Pinker, and Yuanchong Zhang

Incoming solar radiation drives the Earth’s climate system. Long-term surface observations of solar radiation reaching the surface have shown decreasing or increasing trends in different regions of the world in the past several decades, indicating the change of atmospheric components that reflect and/or absorb the solar radiation. This study investigates the roles of aerosols and climate change in determining the surface radiation trends through the change of anthropogenic emission, aerosol-radiation interaction, and aerosol-cloud interactions. With a series of model simulations and analysis of ground-based observations and satellite-derived data products, we will 1) estimate the relative importance of aerosols, clouds, and other radiatively active atmospheric trace gases on the surface radiation budget, 2) compare the relative magnitudes of effects from atmospheric components (aerosols, clouds, and trace gases) and atmospheric processes (aerosol-radiation interactions and aerosol-cloud interactions) in determining the surface radiation trends, and 3) assess the consequences of climate change and anthropogenic emission trends in the change of surface radiation in different regions of the world.

How to cite: Chin, M., Bian, H., Wild, M., Barahona, D., Yu, H., Qian, Y., Darmenov, A., Stackhouse, P., Loeb, N., Pinker, R., and Zhang, Y.: Multi-Decadal Trends of Solar Radiation Reaching the Surface Determined by Aerosol-Cloud-Radiation Interactions, Climate Change, and Anthropogenic Emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4577, https://doi.org/10.5194/egusphere-egu25-4577, 2025.

EGU25-4868 | ECS | Orals | CL2.1

Investigating Bjerknes Compensation under the abrupt-4xCO2 CMIP6 experiment 

Christine Kappatou, Joseph Henry LaCasce, Camille Li, and Ada Gjermundsen
In 1964 J. Bjerknes postulated that, when an anomaly occurs in ocean heat transport (OHT), the atmosphere heat transport (AHT) exhibits an anomaly of opposite sign so that the top of the atmosphere (TOA) transport is approximately preserved. This phenomenon is now known as Bjerknes Compensation (BJC) and has been the object of many studies in the context of steady state climate simulations, on decadal and centennial time scales. Here, we examine BJC under extreme climate forcing, specifically under the quadrupling of atmospheric CO2 in the Coupled Model Intercomparison Project Phase 6 (CMIP6). The models exhibit a pronounced decline in the Atlantic Meridional Overturning Circulation (AMOC), to varying degrees, in response to melting sea ice and increased freshwater runoff. The OHT is reduced accordingly, and this can trigger an increase in AHT, particularly in the Northern Hemisphere. We examine the degree of BJC, in the context of model climate sensitivity. We also examine how changes in overturning in the Southern Hemisphere impact AHT there. The issue is significant, as increased AHT partially compensates for the cooling implied by reduced OHT. 

How to cite: Kappatou, C., LaCasce, J. H., Li, C., and Gjermundsen, A.: Investigating Bjerknes Compensation under the abrupt-4xCO2 CMIP6 experiment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4868, https://doi.org/10.5194/egusphere-egu25-4868, 2025.

Comparing with observations, the abnormally smaller cloud absorption (to solar radiation) given by climate models (namely alleged cloud absorption anomaly) ever raised widespread concerns in the mid-1990s and early 2000s but was seldom mentioned thereafter. Based on three state-of-the-art modeled products, NCEP CFSv2, ECMWF ERA5 and NASA MERRA2, and the newest collocated satellite-surface observation in the last 12 years (2012–2023), we reinvestigate this controversial issue. Our results demonstrate the observed cloud absorption of solar radiation still significantly exceeds the modeled (regardless of modeled products), but their systematic discrepancy has dropped a lot, especially for NCEP CFSv2. NCEP CFSv2 has the lowest bias with the observation, followed by ECMWF ERA5, and the bias of NASA MERRA2 is largest. This implies that cloud absorption anomaly fluctuates with not only sites (as reported by previous studies) but also models. Models’ radiation schemes that introduce the Monte Carlo Independent Column Approximation (McICA) may mitigate the systematic discrepancy between observation and modeling essentially. Additionally, it is noteworthy that there is not a perfect approach to obtaining the observed cloud absorption and particularly the water vapor difference between clear and cloudy skies often would result in its unrealistic overestimation. If the influence from the water vapor difference is neglected, NCEP CFSv2, ECMWF ERA5 and NASA MERRA2 underestimate globally-mean cloud absorption by approximately 10.07 W/m2, 16.65 W/m2 and 18.67 W/m2, respectively; and if it is corrected, the underestimations will be reduced to 7.75 W/m2, 14.33 W/m2 and 16.35 W/m2, respectively.

How to cite: Huang, G.: Is the cloud absorption of solar radiation still underestimated significantly by current climate models?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5356, https://doi.org/10.5194/egusphere-egu25-5356, 2025.

EGU25-5791 | ECS | Posters on site | CL2.1

Asian Summer Monsoon Exacerbates the transport efficiency of Stratospheric Aerosol Injection 

Ye Lu, Jianchun Bian, and Dan Li

Efficiently delivering large quantities of climate intervention material (CIM) to the stratosphere remains a technical challenge in stratospheric aerosol injection (SAI). A novel approach, solar-powered lofting (SPL), mimics the natural ascent of wildfire smoke, using small amounts of black carbon (BC) to transport SO2 from the troposphere to the stratosphere. The Asian Summer Monsoon(ASM) anticyclone over the Tibetan Plateau can also transport aerosols into the stratosphere, acting as a “chimney”. In this study, we investigate whether these two effcts, i.e.  SPL effect and ASM “chimney effect”, combined together to deploy SAI will have better effect, by using a fully coupled Earth System Model.We select the Tibetan Plateau as the injection site for the Northern Hemisphere mid-latitudes, instead of the traditional Pacific location, and compare the differences in sulfate aerosol transport efficiency, distribution, and climate impacts. From 2040 to 2047 under the SSP5-85 emission scenario, ASM’s injection results in 20% more sulfur transported to the stratosphere and a 20% reduction in radiative forcing imbalance at mid-latitudes. Additionally, they lead to a 25% increase in both global annual average surface cooling and September Arcitc sea ice recovery.

How to cite: Lu, Y., Bian, J., and Li, D.: Asian Summer Monsoon Exacerbates the transport efficiency of Stratospheric Aerosol Injection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5791, https://doi.org/10.5194/egusphere-egu25-5791, 2025.

Accurate solar irradiance measurements are critical for optimising solar energy systems, understanding atmospheric processes, and advancing climate research. Pyrheliometers, which provide Direct Normal Irradiance (DNI) measurements over a broad spectral range, are widely used due to their simplicity, cost-effectiveness, and ease of deployment. However, they cannot provide detailed spectral information, which limits their application in advanced studies requiring wavelength-specific insights. In contrast, the Bi-Tec Sensor (BTS) spectroradiometer system measures spectral solar irradiance from 300 nm to 2150 nm with high spectral resolution, covering almost ~96.5% of the solar spectrum, and is traceable to the International System of Units (SI). This detailed spectral data enables in-depth studies of solar energy distribution across different wavelengths but excludes approximately 3.5% of the total solar spectrum in the infrared region (2150–5000 nm).

To overcome this limitation and enable full-spectrum comparisons, this study utilized libradtran, an atmospheric radiative transfer model, to extend the BTS spectral range, whereas due to the requirement of computational resources and expertise, A comparatively simpler functional model was developed based on libradtran simulations, focusing on critical parameters such as solar zenith angle, water vapor, and aerosol properties. This function closely matched the results from libradtran and achieved high precision with a mean value of 96.52% and a standard deviation of  0.20% that can be used to accurately extend the BTS measurements to cover the full spectrum. The comparison between pyrheliometer and BTS spectroradiometer yields a mean ratio of 0.9897 with a standard deviation of 0.0149, achieving a good correlation with pyrheliometer data while maintaining precise spectral details.

The results confirm that BTS spectroradiometers, combined with the spectral extension model, provide an effective and detailed alternative for solar irradiance monitoring. Unlike pyrheliometers, BTS instruments deliver wavelength-specific data crucial for advanced solar energy studies and atmospheric research. Moreover, integrating the extension model into BTS systems simplifies data processing, making high-quality measurements accessible for non-expert users and resource-limited regions.

This approach bridges the gap between the spectral detail of BTS systems and the broad range of pyrheliometers, offering a reliable solution for comprehensive solar irradiance measurements. These findings mark a step forward in solar energy research and environmental monitoring, with the potential to address global data gaps in cost-effective and scalable ways.

How to cite: Jaine, D. and Gröbner, J.: Comparison of solar spectral irradiance measurements with pyrheliometer total solar irradiance data., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6703, https://doi.org/10.5194/egusphere-egu25-6703, 2025.

EGU25-8237 | Posters on site | CL2.1

Changes in global water vapor from observations and reanalysis products 

Olivier Bock, Carl Mears, Shu-Peng Ho, and Xi Shao

Understanding the long-term changes in the global water vapor content is critical for assessing natural vs. human-caused climate change. Despite the strong thermodynamical relationship between temperature and water vapor changes, substantial discrepancies still exist between observations, reanalysis products, and climate model simulations.

In this work, we assess the consistencies and discrepancies of total column water vapor (TCWV) estimates between three observational techniques and three reanalysis products. The observations include satellite-borne microwave radiometers (MWR) over the oceans, GPS–Radio Occultation (GPS-RO) observations from low-orbiting satellites over both ocean and land, and ground-based GNSS receivers over land and on islands. The three reanalyses are ERA5, MERRA-2, and JRA-55. They all assimilate radiances from the satellite microwave radiometers and bending angles produced from GPS-RO measurements. Ground-based GNSS measurements are not assimilated and serve as a fully independent validating data set.

We examine the overall agreement in global TCWV trends in the different data sets over the period from 1980 to the present. We highlight strong features of global climate variability such as the El-Niño Southern Oscillation (ENSO). We focus on the past few years which were characterized by a persistent strong La Niña period (2020-2022), followed by a strong El Niño event (2023/2024). Both ENSO phases had a tremendous impact on regional climate extremes, leading to extended heat waves and wildfires or heavy precipitation and flooding in many places around the world.

How to cite: Bock, O., Mears, C., Ho, S.-P., and Shao, X.: Changes in global water vapor from observations and reanalysis products, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8237, https://doi.org/10.5194/egusphere-egu25-8237, 2025.

Land-use change (LUC) is ranked as the second anthropogenic source of climate change after fossil fuel burning and yields negative albedo-induced radiative forcing (ARF). This cooling effect has been assessed using low spatiotemporally resolved LUC datasets derived from historical statistical data with large uncertainties. Herein, we implement a satellite remote sensing derived highly resolved LUC dataset into a compact earth system model and reassess the global and regional surface ARF by LUC from 1983 to 2010 relative to 1750. We find that the magnitude of negative ARF obtained from the present study is lower by 20% than that estimated by the Intergovernmental Panel on Climate Change, implying a weaker cooling effect. The result reveals that the global LUC-induced surface albedo change may not significantly slow down global warming as was previously anticipated. Sub-Saharan Africa made the largest net proportion to the magnitude of global ARF (39.2%), due to substantial land use conversions, typically the conversion from forest to other vegetation lands, which accompany with higher surface albedos. The most remarkable land cover changes occurred in East and Southeast Asia, which dominated the changes in global ARF in recent decades. Based on major land cover types in these two regions, we infer that vegetation lands exert a most vital effect on global ARF variation.

How to cite: Zhang, X.: Highly-resolved satellite remote sensing based land-use change inventory yields weaker surface albedo-induced global cooling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8463, https://doi.org/10.5194/egusphere-egu25-8463, 2025.

Significant uncertainties remain in the estimate of radiative forcing (RF) induced by land-use change (LUC), partially attributable to the lack of reliable LUC data with a high spatiotemporal resolution. We implemented a high spatiotemporally resolved LUC data set in an earth system model (OSCAR) to examine the response of RF to LUC from 1982 to 2010 in China. Results were compared with the RF estimated using a low spatiotemporally resolved LUC inventory employed previously. The updated LUC data set reduces negative RF by −3.8% from 2000 to 2010 due to the changes in surface albedo subject to LU transition. The simulated mean RF driven by CO2 associated with LUC from 1982 to 2010 using a high spatiotemporally resolved LUC data set reached 0.074 W m−2, considerably higher than 0.022 W m−2 of mean RF derived from the low spatiotemporally resolved LUC inventory, implying increasing net RF and more substantial LUC induced warming.

How to cite: Jian, X.: The response of radiative forcing to high spatiotemporally resolved land-use change and transition from 1982 to 2010 in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8471, https://doi.org/10.5194/egusphere-egu25-8471, 2025.

EGU25-10498 | Posters on site | CL2.1

External radiative forcing partly explains the Europe winter cooling in 1998-2012 

Lingling Suo, Ingo Bethke, Noel Keenlyside, and Francois Counillon

The Eurasia continent underwent significant winter cooling from 1998 to 2012, occurring within the context of global warming. This phenomenon has primarily been linked to internal variability, as previous research indicates; however, discussions regarding its underlying causes continue. Based on the simulations with both combined and individual external forcing, this study suggests that combined external radiative forcing accounts for approximately a quarter of the observed winter cooling in Europe from 1998 to 2012 by contributing to a negative North Atlantic oscillation. Among all individual external forcings, the influence of ozone, which includes the effects of solar cycle 23 from maximum to minimum, is most prominent.

How to cite: Suo, L., Bethke, I., Keenlyside, N., and Counillon, F.: External radiative forcing partly explains the Europe winter cooling in 1998-2012, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10498, https://doi.org/10.5194/egusphere-egu25-10498, 2025.

EGU25-10896 | Posters on site | CL2.1

Assessing the direct aerosol impact on surface irradiance using satellite-based and surface reference data 

Jörg Trentmann, Uwe Pfeifroth, and Martin Wild

The incoming surface solar radiation is an essential climate variable as defined by GCOS. Long term monitoring of this part of the earth’s energy budget is required to gain insights on the state and variability of the climate system. In addition, climate data sets of surface solar radiation have received increased attention over the recent years as an important source of information for solar energy assessments, for crop modeling, and for the validation of climate and weather models; all requiring high-quality and temporally-consistent data records.

It has been established in recent years, based on surface- and remote sensing-based data records, that surface irradiance has increased in many regions worldwide since the mid-1980, the so-called ‘global brightening’. The mechanisms behind this brightening, however, is not yet fully understood. It appears likely that changes in the atmospheric composition, mainly the aerosol loading, and possibly also atmospheric circulation have both been contributing to the global brightening.

Here we will use satellite-based data records from the CM SAF, SARAH and CLARA, which do not include an explicit treatment of the direct aerosol effect on clears-sky radiation to investigate the possible role of the aerosol on surface irradiance. Daily and monthly surface reference data (all-sky and clear-sky) are used to identify weaknesses in the satellite-based data records; aerosol information, e.g., from MERRA, are used to possibly explain these shortcomings, hence allowing to identify and to quantify the possible aerosol effect on surface irradiance.

How to cite: Trentmann, J., Pfeifroth, U., and Wild, M.: Assessing the direct aerosol impact on surface irradiance using satellite-based and surface reference data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10896, https://doi.org/10.5194/egusphere-egu25-10896, 2025.

EGU25-11349 | Orals | CL2.1

Comparing radiative forcing measures for ozone 

William Collins, Fiona O'Connor, Rachael Byrom, Øivind Hodnebrog, Patrick Jöckel, Mariano Mertens, Gunnar Myhre, Matthias Nützel, Dirk Olivié, Ragnhild Skeie, Laura Stecher, Larry Horowitz, Vaishali Naik, and Lee Murray

Ozone is the third most important greenhouse gas, contributing a forcing of 0.47 W/m2 over the historical period. All assessments of ozone forcing so far have used the stratospheric-temperature adjusted radiative forcing (SARF) calculated by offline radiative transfer models. The two most recent IPCC reports have recommended the use of effective radiative forcing (ERF) as the preferred measure of forcing, but no calculations have been available.

For the first time we calculate the future ozone online ERF from six Earth system models and compare this to the SARF calculations. The future ozone calculations are for the SSP3-7.0 scenario for the year 2050. Only the ozone changes (and any consequent impacts on meteorology) are included in the radiative forcing calculations. We find an ERF of 0.27+/- 0.09 Wm-2  and an ozone column increase of 12 DU. Approximately half of the forcing change comes from ozone recovery following the decline in halocarbons.

By decomposing the radiative forcing into instantaneous (IRF), stratospheric-temperature adjusted (SARF) and effective (ERF) radiative forcing we gain insights into the adjustment processes causing the differences between the radiative forcing measures. The ERF is typically larger than the SARF. This is mostly due to positive non-cloud adjustments through increased water vapour (particularly in the stratosphere) and decreased surface albedo. Reductions in high and mid-level cloud increase the short-wave forcing, but decrease the long-wave forcing. The adjustments to the forcing depend on the altitude of the ozone change, with adjustments to ozone changes following reductions in ozone-depleting substances being more strongly positive than those following increases in ozone precursors.

How to cite: Collins, W., O'Connor, F., Byrom, R., Hodnebrog, Ø., Jöckel, P., Mertens, M., Myhre, G., Nützel, M., Olivié, D., Skeie, R., Stecher, L., Horowitz, L., Naik, V., and Murray, L.: Comparing radiative forcing measures for ozone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11349, https://doi.org/10.5194/egusphere-egu25-11349, 2025.

EGU25-11477 | Orals | CL2.1

Understanding altitudinal temperature variations using a surface energy balance approach  

Saurabh Shukla, Axel Kleidon, Sarosh Alam Ghausi, and Tejasvi Ashish Chauhan
 

High-altitude regions are argued to react more strongly to global warming compared to low-altitude regions. However, due to a combination of feedback mechanisms, micro-climatic trends, and lack of long-term observational data, elevation-dependent warming has been difficult to understand and quantify. We address this question using a surface energy balance approach where 2m air temperature variations along altitudes are quantified following changes in surface radiation and turbulent fluxes.  The turbulent fluxes in the energy balance are constrained using the thermodynamic limit of maximum power. The downwelling longwave radiation is parameterized using the semi-emperical equation by Brutsaert (1975). We used BSRN (Baseline Surface Radiation Network) and FLUXNET dataset to test our approach and found that daily variations in 2m air temperatures reasonably well (with R2 value of 0.75) along the altitude gradient. We find that for high altitudes, the downwelling longwave radiation is lesser compared to stations at low altitudes at similar latitudes for both all sky conditions and clear sky conditions. We attribute it to less absorptive mass above the high altitudinal setting, leading to lower atmospheric emissivity and changes in lower atmospheric heat storage. On the other hand, absorbed solar radiation when normalized by potential solar radiation, shows strong seasonality, which is influenced by albedo changes and water vapor content in the atmosphere.  Future work entails extending this framework to get a physically based estimate of elevation-dependent warming using the sensitivity of temperature to components in the energy balance. This understanding is crucial for anticipating the impacts of warming on water resources and ecosystems in these regions and, consequently, for developing effective adaptation and mitigation strategies.

 

How to cite: Shukla, S., Kleidon, A., Ghausi, S. A., and Chauhan, T. A.: Understanding altitudinal temperature variations using a surface energy balance approach , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11477, https://doi.org/10.5194/egusphere-egu25-11477, 2025.

EGU25-12299 | Orals | CL2.1

Contributions of Driving Factors to Variations in Global Surface Solar Radiation 

Hejing Xiao, Yi Huang, Qiurun Yu, and Yiran Peng

Observations have recorded significant decadal changes in the global surface solar radiation (SSR) over the past, a phenomenon known as the ‘global dimming’ and ‘brightening’. Many studies suggest that changes of SSR are dominated by aerosols, clouds, and other influences at the atmosphere. However, due to the lack of suitable data and methodology, there are few global evaluations and quantitative work that reveal the relative importance of impacting factors on the SSR trends. In this study, a linear regression method is used to investigate the driving factors of global SSR and to quantify their contributions to the long-term change and distribution of SSR. Based on a reanalysis dataset, from 2000 to 2023, the distributions and trends of SSR can be well explained by the linear regression model, with crucial variables such as aerosol optical depth (AOD), cloud radiative effect and water vapor as predictors. The model performs particularly well at low and middle latitudes. We find that under all sky condition, cloud radiative effect causes approximately 70% of the variation in SSR, which has the strongest influence on SSR among the other predictors. In addition, all-sky SSR also shows very high sensitivity to water vapor and AOD.

How to cite: Xiao, H., Huang, Y., Yu, Q., and Peng, Y.: Contributions of Driving Factors to Variations in Global Surface Solar Radiation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12299, https://doi.org/10.5194/egusphere-egu25-12299, 2025.

EGU25-12571 | ECS | Orals | CL2.1

Long-Term Integrated Water Vapour (IWV) analysis in Southern Spain using remote sensing techniques and reanalysis models 

Victor Manuel Naval Hernández, Ana del Águila Pérez, Arlett Díaz Zurita, Onel Rodríguez Navarro, Jorge Muñiz Rosado, Daniel Pérez Ramírez, David Neil Whiteman, Lucas Alados Arboledas, and Francisco Navas Guzmán

Water vapour (WV) is one of the most significant greenhouse gases and plays a critical role in the majority of the thermodynamic processes that occur within the atmosphere. Thus, it significantly influences the radiative budget and cloud formation mechanisms, being of paramount importance in weather forecasting. Therefore, accurate and detailed characterisation of its spatial and temporal distribution is of undoubtedly great interest. However, measurement techniques often struggle with its variability both in space and time, making it challenging to obtain regular and reliable measurements. 

Although high resolution height-resolved profiles of water vapour mixing ratio are currently being acquired by lidar systems and providing powerful information, such instruments usually suffer from overlap issues in the lower hundred meters, precisely where greater concentrations of water vapour appear. This issue, together with the reduced global representativity due to the scarce number of operative lidar systems, hinders the use of this technique for continuous monitoring of water vapour near the ground. In contrast, other passive and active remote sensing techniques like Microwave Radiometers (MWR), Sun Photometers (SP) or Global Navigation Satellite System (GNSS) are well established and have been globally proven as a feasible and trustworthy alternative for continuous measurements of the total vertical column water vapour concentration (IWV). 

This study addresses the characterisation of IWV over Granada, a city in southern Spain, using remote sensing techniques (MWR, SP and GNSS). These techniques are first validated against in situ data collected from over 70 radiosondes (RS). The study then investigates the IWV evolution over Granada for a 14-year period. The daily, seasonal and annual cycles are described together with the statistical behaviour of the data series in search of tendency changes.

Reanalysis data from Numerical Weather Prediction (NWP) models such as MERRA-2 (Modern-Era Retrospective Analysis for Research and Applications, version 2) and ERA5 (fifth generation of European Centre for Medium-Range Weather Forecasts reanalysis) are also validated against remote sensing measurements and then considered to expand the study period to more than 40 years, allowing the climatological study of water vapour in the area. Seasonal decomposition and a Mann-Kendall statistical test discovered an increasing tendency in IWV. Analogous analysis for the temperature in the region also found a positive increase, accentuated since the beginning of the 21st century and reinforcing the results of climate change studies. The relationship between both magnitudes indicates a possible contribution of increased water vapour concentrations to the observed increased temperatures.

How to cite: Naval Hernández, V. M., del Águila Pérez, A., Díaz Zurita, A., Rodríguez Navarro, O., Muñiz Rosado, J., Pérez Ramírez, D., Neil Whiteman, D., Alados Arboledas, L., and Navas Guzmán, F.: Long-Term Integrated Water Vapour (IWV) analysis in Southern Spain using remote sensing techniques and reanalysis models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12571, https://doi.org/10.5194/egusphere-egu25-12571, 2025.

EGU25-12847 | Orals | CL2.1

The Earth Climate Observatory space mission concept for the monitoring of the Earth Energy Imbalance. 

Steven Dewitte, Thorsten Mauritsen, Benoit Meyssignac, Thomas August, Luca Schifano, Lien Smeesters, Rémy Roca, Helen Brindley, Jacqueline Russell, Nicolas Clerbaux, Rainer Hollmann, Linda Megner, Margit Haberreiter, Joerg Gumbel, Jochem Marotzke, Jérôme Riedi, Aku Riihela, Tim Trent, and Manfred Wendisch

Monitoring the Earth Energy Imbalance (EEI) is of prime importance for a predictive understanding of climate change. Furthermore, monitoring of the EEI gives an early indication on how well mankind is doing in implementing the Paris Climate Agreement. EEI is defined as the small difference between the incoming energy the Earth receives from the Sun and the outgoing energy lost by Earth to space. The EEI is cumulated in the Earth climate system, particularly in the oceans, due to their substantial heat capacity, and results in global temperature rise. Currently the best estimates of the absolute value of the EEI, and of its long term variation are obtained from in situ observations, with a dominant contribution of the time derivative of the Ocean Heat Content (OHC). These in situ EEI observations can only be made over long time periods, typically a decade or longer. In contrast, with direct observations of the EEI from space, the EEI can be measured at the annual mean time scale. However, the EEI is currently poorly measured from space, due to two fundamental challenges. The first fundamental challenge is that the EEI is the difference between two opposing terms of nearly equal amplitude. Currently, the incoming solar radiation and outgoing terrestrial radiation are measured with separate instruments, which means that their calibration errors are added and overwhelm the signal to be measured. To make significant progress in this challenge, a differential measurement using identical intercalibrated instruments to measure both the incoming solar radiation and the outgoing terrestrial radiation is needed. The second fundamental challenge is that the outgoing terrestrial radiation has a systematic diurnal cycle. Currently, the outgoing terrestrial radiation is sampled from the so-called morning and afternoon Sun-synchronous orbits, complemented by narrow band geostationary imagers. Recently the sampling from the morning orbit was abandoned. The sampling of the diurnal cycle can be improved, for example, by using two orthogonal 90° inclined orbits which give both global coverage, and a statistical sampling of the full diurnal cycle at seasonal time scale. For understanding the radiative forcing – e.g. aerosol radiative forcing - and climate feedback – e.g. ice albedo feedback - mechanisms underlying changes in the EEI, and for climate model validation, it is necessary to separate the Total Outgoing Radiation (TOR) spectrally into the two components of the Earth Radiation Budget (ERB), namely the Reflected Solar radiation (RSR) and Outgoing Longwave Radiation (OLR) and to map them at relatively high spatial resolution. The Earth Climate Observatory (ECO) mission concept was recently selected by the European Space Agency as one of the 4 candidate Earth Explorer 12 missions, that will be further studied in Phase 0 until mid 2026. The current paper provides a broad overview of the ECO mission objectives, the mission requirements, and the key elements of a baseline mission concept. During Phase 0, the ECO mission concept will be further elaborated in two parallel industrial studies, which may or may not adopt or refine the elements of the baseline concept.

How to cite: Dewitte, S., Mauritsen, T., Meyssignac, B., August, T., Schifano, L., Smeesters, L., Roca, R., Brindley, H., Russell, J., Clerbaux, N., Hollmann, R., Megner, L., Haberreiter, M., Gumbel, J., Marotzke, J., Riedi, J., Riihela, A., Trent, T., and Wendisch, M.: The Earth Climate Observatory space mission concept for the monitoring of the Earth Energy Imbalance., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12847, https://doi.org/10.5194/egusphere-egu25-12847, 2025.

EGU25-13806 | ECS | Orals | CL2.1

An insufficient subsurface depth biases the long-term surface energy balance in Land Surface Models  

Félix García-Pereira, Jesús Fidel González-Rouco, Nagore Meabe-Yanguas, Johann Jungclaus, Philipp de Vrese, and Stephan Lorenz

The land subsurface stored around a 6 % of the Earth’s energy imbalance in the last decades, being the second contributor to the partitioning after the ocean (90 %). Previous studies have shown that state-of-the-art Earth System Models (ESMs) remarkably underestimate the observational land heat uptake values. This underestimation stems from Land Surface Models (LSMs) within ESMs imposing too shallow zero-flux bottom boundary conditions to correctly represent the conductive propagation and land heat uptake with depth. However, non-significant temperature variability differences at the ground surface have been detected when these boundary conditions are prescribed deeper, so the physical process limiting land heat uptake was not yet identified. This study reveals that the underlying mechanism is the reduced incoming ground heat flux (GHF). To conclude this, GHF values coming from an ensemble of eight historical and RCP8.5 land-only simulations with different subsurface depths conducted with the LSM of the Max Planck Institute for Meteorology ESM (MPI-ESM), JSBACH, have been compared to GHF estimates yielded by a one-dimensional heat conduction forward model. Results show that GHF doubles when deepening the LSM from 10 to 25 m, saturating at a factor of 5 when the boundary condition is placed at approx. 100 m. The increase in the incoming GHF is mainly compensated by a global increase in the outgoing sensible heat flux (SHF), a small increase of the latent heat flux (LHF) in wet regions, and an increase in the surface net radiation in arid and semi-arid regions.

How to cite: García-Pereira, F., González-Rouco, J. F., Meabe-Yanguas, N., Jungclaus, J., de Vrese, P., and Lorenz, S.: An insufficient subsurface depth biases the long-term surface energy balance in Land Surface Models , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13806, https://doi.org/10.5194/egusphere-egu25-13806, 2025.

EGU25-13923 | Orals | CL2.1

Examining fast radiative feedbacks using machine-learning-based emulators of weather 

William Collins and Ankur Mahesh

The response of the Earth system to radiative perturbations is governed by a combination of fast and slow feedbacks.  Slow feedbacks are typically activated in response to changes in ocean temperatures on decadal timescales and often manifest as changes in Earth-system state with no recent analogue.  On the other hand, fast feedbacks can be activated in response to rapid atmospheric physical processes on timescales of weeks and are already operative in the present-day weather system. This distinction implies that the physics of fast radiative feedbacks is present in the historical reanalyses that have served as the training data for many of the most successful recent machine-learning-based emulators of weather.  In addition, these feedbacks are functional under the historical boundary conditions pertaining to the top-of-atmosphere radiative balance and sea-surface temperatures.    We discuss our work using historically trained weather emulators to characterize and quantify fast radiative feedbacks without the need to retrain for prospective Earth system  conditions.

How to cite: Collins, W. and Mahesh, A.: Examining fast radiative feedbacks using machine-learning-based emulators of weather, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13923, https://doi.org/10.5194/egusphere-egu25-13923, 2025.

EGU25-14211 | Orals | CL2.1

Homogenized daily sunshine duration over China from 1961 to 2022 

Yanyi He, Kaicun Wang, Kun Yang, Chunlüe Zhou, Changkun Shao, and Changjian Yin

Inhomogeneities in the sunshine duration (SSD) observational series, caused by non-climatic factors like China’s widespread transition from manual to automatic SSD recorders in 2019 or station relocations, have hindered accurate estimate of near-surface solar radiation for the analysis of global dimming and brightening as well as related applications, such as solar energy planning and agriculture management. This study compiled raw SSD observational data from 1961 to 2022 at more than 2,200 stations in China and clearly found that the improved precision from 0.1 hour to 1 minute following the instrument update in 2019 led to a sudden reduction in the frequency of zero SSD from 2019 onwards, referred to as the day0-type discontinuity. For the first time, we systematically corrected this known day0-type discontinuity at 378 stations (17%) in China, resulting in an SSD series with comparable frequencies of zero value before and after 2019. On this base, we constructed a homogenization procedure to detect and adjust discontinuities in both the variance and mean of daily SSD from 1961 to 2022. Results show that a total of 1,363 (60%) stations experienced breakpoints in SSD, of which ~65% were confirmed by station relocations and instrument replacements. Compared to the raw SSD, the homogenized SSD was more continuous to the naked eye for various periods, and presented weakened dimming across China from 1961 to 1990 but a non-significant positive trend by a reduction of 60% in the Tibetan Plateau, suggesting that the homogenized SSD tends to better capture the dimming phenomenon. The northern regions continued dimming from 1991 to 2022 but the southern regions of China brightened slightly. The implementation of the Action Plan for Air Pollution Prevention and Control since 2013 contributed to a reversal of SSD trend thereafter, which was better reflected in the homogenized SSD with a trend shift from -0.02 to 0.07 hours·day-1/decade from 2013 to 2022 in China, especially in heavily polluted regions. Besides, the relationships of cloud cover fraction and aerosol optical depth with SSD were intensified in the homogenized dataset. These results highlight the importance of the homogenized SSD in accurately understanding the dimming and brightening phenomena. The homogenized SSD dataset is publicly available for community use at https://yanyihe-rad.github.io/files/homog-daily-ssd-China-v1.0.mat.

How to cite: He, Y., Wang, K., Yang, K., Zhou, C., Shao, C., and Yin, C.: Homogenized daily sunshine duration over China from 1961 to 2022, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14211, https://doi.org/10.5194/egusphere-egu25-14211, 2025.

Almost all solar resource assessment and forecasting endeavors require gridded surface irradiance retrieved from geostationary satellites. China’s solar industry has hitherto been relying upon Himawari and Meteosat-derived surface irradiance products. Despite the maturity of those products, none provides a complete coverage of China, which implies a series of data issues, such as the inconsistency at product boundaries or limited resolution towards the edge of the field-of-view disks. However, data issues are but secondary, and the lack of autonomous capability of performing solar resourcing is what truly troubles those concerned. China’s latest geostationary weather satellite series, Fengyun-4 (FY-4), has the most advanced technology, but its service commenced only fairly recently in 2017. Hence, to meet China’s immediate needs for solar resources under its radical decarbonization target, which cannot afford to wait for FY-4 data to pile with time, soliciting information from its predecessor series, namely, FY-2, is thought to be apt. In this work, a high-resolution (1.25 km) satellite-derived surface irradiance product over a twelve-year period (2011–2022) is developed, based on the scanning radiometers onboard FY-2E, -2F, and -2G satellites. A series of analysis as to quantifying the interannual and spatial variability of solar irradiance in China, which has rarely been done before, confirm that the current product can suffice most solar resourcing applications. 

How to cite: Shi, H.: China's autonomous solar energy products with the application of Fengyun satellites, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14827, https://doi.org/10.5194/egusphere-egu25-14827, 2025.

EGU25-15920 | Orals | CL2.1 | Highlight

Recent global temperature surge intensified by record-low planetary albedo 

Helge Goessling, Thomas Rackow, and Thomas Jung

In 2023, the global mean temperature soared to almost 1.5°C above the preindustrial level, surpassing the previous record by about 0.17°C. Previous best-guess estimates of known drivers, including anthropogenic warming and the El Niño onset, fall short by about 0.2°C in explaining the temperature rise. This gap persisted in 2024, during which the stronger El Niño contribution resulted in an even higher global annual-mean temperature, exceeding the symbolic 1.5°C threshold. Using satellite and reanalysis data, we identified a record-low planetary albedo as the primary factor bridging this gap. The decline is apparently caused largely by a reduced low-cloud cover in the northern mid-latitudes and tropics, in continuation of a multiannual trend. Further exploring the low-cloud trend and understanding how much of it is due to internal variability, reduced aerosol concentrations, or a possibly emerging low-cloud feedback will be crucial for assessing the present and expected future warming.

How to cite: Goessling, H., Rackow, T., and Jung, T.: Recent global temperature surge intensified by record-low planetary albedo, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15920, https://doi.org/10.5194/egusphere-egu25-15920, 2025.

EGU25-16594 | Orals | CL2.1

Using line-by-line Monte Carlo to compute the Earth’s outgoing longwave radiation and CO2’s radiative forcing 

Dufresne Jean-Louis, Lebrun Raphaël, Nyffenegger-Pere Yaniss, Fournier Richard, and Blanco Stéphane

The Earth’s radiation budget is a crucial part of climate and its evolution. Being part of this budget, the outgoing longwave radiation (OLR) has been extensively studied, especially in the context of climate-change and anthropogenic greenhouse gases emissions modifying the Earth’s radiative equilibrium.

In this study we present a new line-by-line radiative code RadForcE, we have developed to compute the global OLR and radiative forcing over a 10-year period. Based on a backward longwave Monte Carlo method, RadForcE uses line-by-line spectroscopic data for several molecular gases (CO2, H2O, CH4 and O3) from high-resolution databases GEISA and HITRAN, as well as different continua. The clouds’ vertical distributions are taken into account with a vertical overlap subgrid parameterization that is sampled "on the fly" for each optical path along vertical atmospheric profiles. Those profiles are sampled over a 10-year period all over the globe, either from GCM outputs or from ERA5 reanalysis, to compute the unbiased global OLR at a very small computational cost (~10 minutes on a laptop).

We this new method we are also able to directly compute any greenhouse gas radiative forcing, and present estimates of the radiative forcing for a doubling of CO2. The Monte Carlo approach allows us to identify, for each outgoing optical path at the top of the atmosphere, the emitting species as well as the altitude of emission. By doing so, we can visualize the profile of altitude of emission for each species, as well as how some gases can screen other species’ emission or the surface’s emission. We can also visualize, for a doubling of CO2, the increase of stratospheric emission by CO2, and its screening of the surface’s emission and water vapor tropospheric emission.

How to cite: Jean-Louis, D., Raphaël, L., Yaniss, N.-P., Richard, F., and Stéphane, B.: Using line-by-line Monte Carlo to compute the Earth’s outgoing longwave radiation and CO2’s radiative forcing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16594, https://doi.org/10.5194/egusphere-egu25-16594, 2025.

EGU25-17123 | ECS | Orals | CL2.1

Measurements of land surface albedo at the Thule High Arctic Atmospheric Observatory (THAAO) in Pituffik, Greenland and comparison with MODIS data. 

Monica Tosco, Daniela Meloni, Filippo Calì Quaglia, Giovanni Muscari, Tatiana Di Iorio, Giandomenico Pace, Virginia Ciardini, and Alcide Giorgio di Sarra

The land surface albedo is one of the key parameters of the global radiation budget, since it regulates the shortwave radiation absorbed by the Earth’s surface. The polar regions, in particular, a decrease in snow and ice cover results in a decrease of surface albedo and in the intensification of solar heating further reducing the snow and ice areas (ice-albedo feedback). In remote areas, where in-situ instruments are absent, satellites are crucial to measure surface albedo changes.

In this work, a comparison of satellite and in-situ measurements of broadband shortwave surface albedo is conducted. The area of interest selected is around the Thule High Arctic Atmospheric Observatory (THAAO) on the North-western coast of Greenland (76.5°N, 68.8°W), where the measurements of down-welling and up-welling shortwave irradiance have been started in 2009 and 2016, respectively (https://www.thuleatmos-it.it/).

Albedo determinations based on MODIS observations from both Terra and Aqua (MODIS MCD43A3 dataset), consisting of daily values with a spatial resolution of 500 m, have been compared with the ground-based measurements.

The analysis has been conducted for all-sky and clear-sky conditions with a focus on some events to better understand the behavior of MODIS data with respect to ground-based measurements, taking advantage of the additional information (meteorological parameters, cloudiness, precipitation) available at THAAO.

The results for the period 2016-2024 show an underestimation of the albedo measurements from satellite compared to the ground-based measurements at the THAAO over a large part of the period considered. The best agreement is found in the summer when there is no snow around the Observatory, and the mean measured albedo value is 0.1633 for cloud-free conditions and 0.1903 for all-sky conditions. The mean bias during this season is around -0.0074 for cloud-free conditions and 0.0067 for all sky conditions. In spring, when the in-situ albedo values are highly variable, between 0.350 and 1, the mean bias is around -0.0645 for cloud-free conditions and -0.0159 for all sky conditions.

The fast changes in surface albedo occurring after short snow precipitation or removal events are seldom captured by satellite observations.

How to cite: Tosco, M., Meloni, D., Calì Quaglia, F., Muscari, G., Di Iorio, T., Pace, G., Ciardini, V., and di Sarra, A. G.: Measurements of land surface albedo at the Thule High Arctic Atmospheric Observatory (THAAO) in Pituffik, Greenland and comparison with MODIS data., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17123, https://doi.org/10.5194/egusphere-egu25-17123, 2025.

EGU25-17633 | ECS | Orals | CL2.1

Evaluation of surface shortwave spectral fluxes at Uccle produced by the ECMWF ecRad radiation scheme (v1.5.0) embedded in the MAR regional model (v3.14) and prediction of UV indices 

Jean-François Grailet, Robin J. Hogan, Nicolas Ghilain, David Bolsée, Xavier Fettweis, and Marilaure Grégoire

The ecRad scheme is the latest radiative transfer scheme provided by the European Centre for Medium-range Weather Forecast (ECMWF), and is notably operational in the ECMWF’s Integrated Forecasting System (IFS) since 2017. Recent developments of ecRad enable it both to run using ecCKD high resolution gas-optics models and to produce surface shortwave spectral fluxes. The combination of both features allow ecRad to produce fine surface shortwave spectral fluxes, e.g., over a 310–315 nm spectral band.

We assessed this capability after embedding ecRad (v1.5.0) in the MAR (Modèle Atmosphérique Régional) regional climate model (v3.14). For this purpose, we used ground-based spectral observations captured by the Royal Belgian Institute for Space Aeronomy at Uccle (Belgium; 50.797° N, 4.357° E) from 2017 to 2020, in the 280–500 nm range and with a precision of 0.5 nm. After carefully tuning both MAR and ecRad and configuring fine spectral bands over the 280–500 nm range, we ran a MAR simulation over Belgium for the same period as the Uccle spectral observations.

After integrating the spectral observations on the same bands as configured in our MAR/ecRad simulation, we compared both time series of spectral fluxes at Uccle. Our evaluation yielded correlation coefficients ranging from 0.9 to 0.93 for all bands above 295 nm and low biases for all bands. As our spectral fluxes cover the ultraviolet (UV) range, we tried to predict UV indices with MAR/ecRad spectral fluxes. The UV index is a metric used to inform the public about how much harmful ultraviolet radiation reaches the Earth’s surface at a given time, and consists of a weighted integral of spectral fluxes over the UV range. Our model-based and observations-based UV indices are in very good agreement, though the former falls short of finding the highest UV indices of the latter, due to the ozone mixing ratios in MAR not varying on a daily basis.

Author's note: this research work is detailed in the paper "Inclusion of the ECMWF ecRad radiation scheme (v1.5.0) in the MAR model (v3.14), regional evaluation for Belgium and assessment of surface shortwave spectral fluxes at Uccle" currently available on EGUsphere in preprint (awaiting topic editor decision after referee comments and subsequent revision).

How to cite: Grailet, J.-F., Hogan, R. J., Ghilain, N., Bolsée, D., Fettweis, X., and Grégoire, M.: Evaluation of surface shortwave spectral fluxes at Uccle produced by the ECMWF ecRad radiation scheme (v1.5.0) embedded in the MAR regional model (v3.14) and prediction of UV indices, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17633, https://doi.org/10.5194/egusphere-egu25-17633, 2025.

EGU25-18785 | Orals | CL2.1

Modification of the shortwave radiation budget of the Mediterranean Basin during intense dust episodes (2005-2018) 

Nikos Hatzianastassiou, Maria Gavrouzou, Marios-Bruno Korras-Carraca, Michalis Stamatis, Christos Lolis, Nikos Mihalopoulos, Christos Matsoukas, and Ilias Vardavas

Dust aerosols significantly affect the shortwave (SW) radiation budget from global to regional scales. This effect strengthens during intense dust outbreaks taking place with variable frequency and features over and near to the great world deserts. The greater Mediterranean Basin is such a region, frequently undergoing dust episodes originating from the nearby Sahara Desert. In the present study, a climatological assessment of the direct SW radiative effects (DREs) of intense Mediterranean dust episodes is made for the first time. Specifically, the modification of the top-of-atmosphere (TOA), atmospheric and surface SW radiative fluxes caused by 162 spatially extended intense dust episodes that took place from 2005 to 2018 is estimated using the FORTH spectral radiative transfer model (RTM). Also, the consequent modification of the regional atmospheric thermal structure and dynamics due to these DREs is computed, aiming to shed light on the role of dust aerosols on regional climate. The RTM computations are driven by a synergy of contemporary satellite (ISCCP-H) and reanalysis (MERRA-2) climatological data.

The reliability of the dust DREs (DDREs) is ensured by comparisons of the model outputs with reference fluxes at the region’s surface (BSRN stations) and TOA (CERES). The results are satisfactory indicating a nice correlation with BSRN and CERES (R values equal to 0.95 and 0.98, respectively) and a slight underestimation (5.4%) at surface and overestimation at TOA (2.7%). During the 162 intense dust episodes the surface of the Mediterranean Basin is cooled by up to -72 W/m2 on average, while the atmosphere is correspondingly heated by up to 75 W/m2. At TOA opposite effects are induced, namely a planetary heating (up to 26 W/m2) over Africa and a cooling (as much as -20 W/m2) over the Mediterranean Sea. These values are larger (up to 100 W/m2) on a seasonal basis and even stronger on a daily or hourly basis. Besides, the DDREs induce an atmospheric heating up to about 0.4 K/3-hours on average, while this heating is as strong as 2.5 K during the time interval 12:00-15:00 of the dust episode days, creating a significant positive buoyancy over the dust affected areas.

How to cite: Hatzianastassiou, N., Gavrouzou, M., Korras-Carraca, M.-B., Stamatis, M., Lolis, C., Mihalopoulos, N., Matsoukas, C., and Vardavas, I.: Modification of the shortwave radiation budget of the Mediterranean Basin during intense dust episodes (2005-2018), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18785, https://doi.org/10.5194/egusphere-egu25-18785, 2025.

EGU25-19022 | ECS | Orals | CL2.1

The important role of feedback processes for contrail cirrus climate impact 

Marius Bickel, Michael Ponater, Ulrike Burkhardt, Mattia Righi, Johannes Hendricks, and Patrick Jöckel

Contrail cirrus is regarded to be the largest contributor to aviation induced global warming based on classical radiative forcing and exceeds the corresponding climate impact of accumulated air traffic CO2 emissions. However, recent studies indicate that the leading role of contrail cirrus declines when using more advanced climate metrics, such as the effective radiative forcing, or even disappears when considering the induced surface temperature change. 

Here we present results from climate model simulations to derive a fully self-consistent set of classical radiative forcings, effective radiative forcings and corresponding surface temperature changes for a contrail cirrus and CO2 perturbation. The simulations were extensively evaluated by feedback analysis in order to determine the origin of the reduced efficacy of contrail cirrus to warm Earth’s surface. When switching from classical radiative forcing to effective radiative forcing the impact of contrail cirrus decreases by 45% relative to CO2. Feedback analysis revealed a reduced formation of natural cirrus as the major reason, as contrail cirrus formation removes large parts of available ambient humidity. When looking at surface temperature change, the efficacy of contrail cirrus turned out to be reduced, even more, by 79% relative to CO2. Again, cloud feedbacks were found to be the major reason for the different behavior between the contrail cirrus and CO2 perturbation, however, in this case mainly triggered by decreasing low- and mid-level clouds in the CO2 simulation. The efficacy reduction is also supported by a larger negative lapse rate feedback (change of the vertical temperature slope) which is the result of a temperature dipole formed by contrail cirrus, with strongest warming rates directly below the contrail cirrus cloud base and decreasing strength towards surface.

How to cite: Bickel, M., Ponater, M., Burkhardt, U., Righi, M., Hendricks, J., and Jöckel, P.: The important role of feedback processes for contrail cirrus climate impact, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19022, https://doi.org/10.5194/egusphere-egu25-19022, 2025.

EGU25-19629 | ECS | Orals | CL2.1

Phenology's Net Cooling Effect as Feedback to Global Warming 

Alexander J. Winkler and the PhenoFeedBacks Team

Recent decades have seen significant changes in land surface phenology, with earlier leaf development in northern ecosystems and diverse changes in autumn senescence, primarily attributed to climate change. These phenological changes feed back to Earth’s climate system by altering biogeochemical and biogeophysical processes at the land surface. However, little is known about the strength of these diverse effects on the Earth's energy balance, and whether their combination results in a net positive (warming) or negative (cooling) feedback to global warming.

Using a fully-coupled Earth system model (ESM) with an interactive global carbon cycle, we investigate the effects of land phenological changes on the Earth's energy balance and the subsequent biogeophysical and biogeochemical feedbacks. We prescribe transient shifts in leaf area index (LAI) in the ESM based on remote sensing estimates of phenological spring advancement (2.1 days per decade) and autumn delay (1.8 days per decade). Note these shifts are only prescribed for extratropical northern ecosystems, where robust phenological changes have been observed, however, the effect in the ESM is global including local and non-local effects. Our results provide a first quantification of the impact of these phenological changes on the processes affecting the Earth’s energy balance, namely, shortwave radiation through changes in surface albedo, surface sensible and latent heat fluxes, longwave surface emissions, ground heat flux, longwave radiation balance through greenhouse gases, and the overall radiative fluxes through cloud properties and planetary albedo.

We find that autumn LAI shifts have a stronger net effect than spring LAI shifts on the Earth's energy balance, and that these effects can compensate each other when they co-occur in the same year. Our simulations also reveal compensating effects between outgoing longwave and outgoing shortwave radiation at the top of the atmosphere, where the former points to a positive and the latter to a negative radiative forcing. Altogether, we report an average negative radiative forcing of 0.17 ± 0.1 W m-2 for a 10-day lengthening of the growing season, resulting in a global mean surface temperature cooling of 0.1 ± 0.03 °C. The effect is more pronounced in simulations when spring advancement and delay in senescence are prescribed separately in the ESM, amounting to a negative radiative forcing of 0.24 ± 0.21 W m-2 and 0.32 ± 0.25 W m-2 for a 10-day lengthening of the growing season, respectively. These simulations suggest that phenological changes triggered by global warming result in a net negative feedback to global warming. Future research is needed to confirm this first quantification and to investigate the saturation of phenological responses to global warming, which could weaken this cooling feedback effect in the future.

How to cite: Winkler, A. J. and the PhenoFeedBacks Team: Phenology's Net Cooling Effect as Feedback to Global Warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19629, https://doi.org/10.5194/egusphere-egu25-19629, 2025.

EGU25-19921 | ECS | Orals | CL2.1

Radiative forcing of anthropogenic Brown Carbon in EC-Earth3 

Akash Deshmukh, Anton Laakso, Tero Mielonen, Angelos Gkouvousis, Antti Arola, Harri Kokkola, and Tommi Bergman

Brown carbon (BrC) influences atmospheric radiative forcing through its unique light-absorption characteristics. The role of  BrC as a significant absorbing component of organic aerosols (OA) has profound implications for understanding its impact on climate systems. However, the complex processes forming BrC, along with the chemical and optical properties that determine its behavior are not yet fully understood. These challenges are compounded by the fact that BrC's sources, formation processes, and interactions with other atmospheric components remain partially unknown. 

Existing approaches to represent BrC in climate models range from intermediate schemes that explicitly account for its emission and aging to simplified methods that assume constant weak absorbing properties in OA. Furthermore, studies indicate that BrC may impose a radiative burden comparable to black carbon (BC), potentially amplifying the overall forcing exerted by carbonaceous aerosols. 

However, it is not entirely clear how brown carbon contributes to atmospheric radiation and what role it plays in climate. Previous studies have offered varying estimates of BrC  direct radiative effect (DRE), underscoring the need for refined modeling and observational data to understand BrC's role in atmospheric dynamics and its contribution to global warming.  Here, we examined the global radiative impacts of anthropogenic BrC emissions using the EC-Earth3 Earth System Model. This study aims to address the significant uncertainties in climate modeling by enhancing the representation of BrC in models. This includes incorporating additional sources to provide more accurate estimations of its radiative effects.  Furthermore, the study will assess the role of BrC in driving regional climate variations and their potential contributions to global climate forcing. For the BrC emissions, we used the ECLIPSE (Evaluating the Climate and Air Quality Impacts of Short-lived Pollutants) dataset, developed by the Finnish Environment Institute. Also, we used the Organic Carbon (OC) and BC emissions from the ECLIPSE emission dataset. EC-Earth3 simulations were conducted across different years to represent both historical and future scenarios. Each simulation was run for six years, including a one-year spin-up period.  

Our preliminary results from historical simulations for the year 2010 indicate that the global mean direct radiative forcing of anthropogenic BrC emissions is negligible. However, regional effects are significantly more pronounced, which need to be studied further. 

How to cite: Deshmukh, A., Laakso, A., Mielonen, T., Gkouvousis, A., Arola, A., Kokkola, H., and Bergman, T.: Radiative forcing of anthropogenic Brown Carbon in EC-Earth3, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19921, https://doi.org/10.5194/egusphere-egu25-19921, 2025.

The burning of solid biomass fuel in traditional cooking stoves is still a major source of air pollution in India’s rural areas. Thereby estimates of source emissions becomes extremely important considering its effect on health and environment. The present study aims to measure and characterize aerosol emissions from the use of various single and mix-solid biomass fuels (fuelwood, dung cake, crop-residue) for cooking in traditional cookstoves. A portable versatile source sampling system (VS3) having PM2.5 samplers along with aethalometer (AE33) were taken on-field in Bihar and Haryana to capture real time emission measurement during cooking activity. A total of 84 experiments were conducted during both morning and evening cooking and the data was analysed to understand the impact of various fuel types, cooking processes and emission characteristics on black carbon (BC) @880nm. The burn rates in case of single fuel use like fuelwood, dung cake, and crop residue were found 1.6 ± 0.8, 1.56 ± 0.5, and 1.83 ± 0.9 kgh-1 respectively, however, in case of mix-fuel usage like firewood with dung cake and crop-residue was 2.4 ± 1.3 kgh-1. The relationship between combustion temperature and BC was investigated using the Pearson correlation test. The results revealed a weak (R2 = 0.124) but significant association, suggesting that while combustion temperature influences BC levels, other factors also play important roles. ANOVA tests were conducted to ascertain the statistical significance of the variations in BC emissions across different fuel types and cooking techniques. The tests revealed that both fuel types and cooking processes significantly affect BC concentrations (P-value~0). To delve deeper, regression analyses were performed, revealing that these factors account for approximately 10.3% of the variability in BC. The models highlighted the influence of specific fuel types and cooking processes, underscoring the complexity of factors impacting BC emissions. This multifaceted approach not only enhances our understanding of how cooking and combustion practices influence BC emissions but also underscores the importance of considering a variety of factors when developing strategies to reduce air pollution and improve environmental health. Understanding BC emissions can guide policies to improve energy access and reduce socioeconomic disparities. The paper will focus on looking other combustion parameters like atmospheric temperature and relative humidity and the impact of single and mix-fuel use on the BC emissions.

How to cite: Kumari, J. and Habib, G.: Black Carbon Emissions and Their Relation to Emission Characteristics from Traditional Cookstoves in Rural India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20092, https://doi.org/10.5194/egusphere-egu25-20092, 2025.

EGU25-20374 | Posters on site | CL2.1

Using Decadal Variability of Surface and Satellite-based Measurements of Surface Solar Fluxes to Assess Current and Long-term Projected Changes from CMIP-6  

Paul Stackhouse, Neha Khadka, Bradley Hegyi, Stephen Cox, J. Colleen Mikovitz, and Taiping Zhang

NASA projects that provide estimates of solar irradiance in the context of meteorological conditions (i.e., clouds, aerosols and gaseous constituents, etc.) spanning from 1983 to near present (i.e., Surface Radiation Budget (GEWEX SRB), Clouds and Earth’s Radiance Energy System – CERES and Modern Era Reanalysis-assimilation for Research and Applications – MERRA2, etc.).  Those data products provide nearly 40 years of covariant information from global to regional scales.  These records provide the opportunity to assess the decadal variability of these fluxes with the capability to attribute changes to various cloud and/or aerosol processes.  Utilizing these observations, we assess the long-term projections of the surface solar fluxes from CMIP6 model runs utilizing NASA’s Earth Exchange Global Daily Downscaled Projections (NEX-GDDP) data set (Thrasher et al., 2023) for three socio-economic pathways utilized by Climate Modeling Intercomparison Project (CMIP6) that span from 1950 to 2100 and includes projections of temperature and solar irradiance with 7 other parameters.  Over the Continental United States, we find that the data products used to downscale this NEX-GDDP needs to be re-evaluated but that the long-term changes in surface solar fluxes show very little trend.  However, the 2-4 decade variability is larger by as much as a factor of 4.  This has implications in terms of surface energy flux exchange at the surface and even for assessing the solar availability for solar power resources

How to cite: Stackhouse, P., Khadka, N., Hegyi, B., Cox, S., Mikovitz, J. C., and Zhang, T.: Using Decadal Variability of Surface and Satellite-based Measurements of Surface Solar Fluxes to Assess Current and Long-term Projected Changes from CMIP-6 , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20374, https://doi.org/10.5194/egusphere-egu25-20374, 2025.

EGU25-20539 | ECS | Posters on site | CL2.1

Atmospheric process, radiation forcing, and climate effects of short-chain perfluoroketones 

Zechen Yu, Jiayu Quan, and Jianjie Fu

Perfluoroketones are recently used as a new type of fire extinguishing material which could replace halon and fluoroalkane agents to reduce the ozone depletion effects.  In this study, a combination of quantum chemical calculation and flow-tube experiments was carried out to study the photolysis reaction and degradation mechanisms of perfluorohexanone that triggered by ·OH and ozone. The results showed that the photolysis rate of perfluorohexanone molecule was about 1.72×10-5-4.48×10-5s-1. In the reaction of ·OH, the reaction rate is about 2.3×10-12 molec-1cm3s-1, and the F atom substitution reaction that occurs on the α-C atom is the main reaction pathway. The reaction rate of perfluorohexanone molecules with ozone is negligible. The degradation products were further analyzed by using a online GCMS and off-line LC-QTOF. The short-chain fluoroacetic acid, such as trifluoroacetic acid was observed. The radiation forcing of the precursor compounds as well as the degradation products were evaluated by using the radiative transfer model. The results of this study help to understand a series of reactions and conversion mechanisms of perfluorohexanone in the atmosphere, and provides the management strategy for using of volatile prefluoro compounds.

How to cite: Yu, Z., Quan, J., and Fu, J.: Atmospheric process, radiation forcing, and climate effects of short-chain perfluoroketones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20539, https://doi.org/10.5194/egusphere-egu25-20539, 2025.

EGU25-20646 | Orals | CL2.1

Updating the experimental absorption cross sections for HITRAN2024 

Robert Hargreaves, Iouli Gordon, Christian Hill, Roman Kochanov, and Laurence Rothman

Many trace gases throughout Earth’s atmosphere are known to have a large potential to impact the radiation budget. The HITRAN database provides spectroscopic parameters and supplementary data in the form of line-by-line lists, absorption cross sections, collision induced absorption, water vapor continuum, and aerosol properties that enable molecular absorption to be modeled, which allows the radiation budget and radiative forcing to be determined. For HITRAN2024, in addition to increasing the number of molecules with line-by-line lists to 61, the absorption cross sections are receiving a substantial update. The update of cross sections makes use of many newly available experimental data and results in the addition over 100 molecules to the large number of molecules already represented as absorption cross sections in HITRAN2020 (Gordon et al. 2022). The absorption cross section update will also expand the range of experimental conditions available (i.e., temperatures, pressures, broadening gases, and resolutions) for many molecules that are present in Earth’s atmosphere. The new cross-sections have been a subjected to a validation process prior to being added to the database. This talk will showcase the absorption cross sections in HITRAN, and will highlight major updates for the 2024 compilation.

Funding from NASA grant 80NSSC23K1596 is acknowledged.

Reference: Gordon, et al., JQSRT 277, 107949 (2022). https://doi.org/10.1016/j.jqsrt.2021.107949

How to cite: Hargreaves, R., Gordon, I., Hill, C., Kochanov, R., and Rothman, L.: Updating the experimental absorption cross sections for HITRAN2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20646, https://doi.org/10.5194/egusphere-egu25-20646, 2025.

EGU25-561 | ECS | Posters on site | AS3.22

Characteristic aerosol properties from ecologically sensitive high-altitude region of Western Ghats in India 

Aman Deep Gupta, Tarun Gupta, Sachin S. Gunthe, and Aishwarya Singh

The study aimed to evaluate the burden of anthropogenically emitted pollutants over an ecologically sensitive region of Munnar in Western Ghats, and quantify a baseline for aerosol measurements for comparisons with highly polluted urban clusters in India. Pre-monsoon sampling of PM₁ aerosols was carried out at the NABHA (Natural Aerosol and Bioaerosol at High Altitude) laboratory (10.09°N, 77.07°E), located ~1600 m above sea level, approximately 90 km east of the Arabian Sea. The collected PM₁ particles were analysed for metals, carbonaceous fractions, inorganic species, and polycyclic aromatic hydrocarbons (PAHs) to identify potential pollution sources and evaluate the toxicity of the sampled airmasses.

The PM₁ concentrations at this ecologically sensitive site were notably elevated, with an average of 21.7 ± 5.5 µg/m³ for the sampling duration. The physio-chemical analysis revealed the composition consisting of approximately 8% crustal dust, 7% sea salt, 20% sulphate, 7% ammonium, 42% organic mass (OM), and 4% elemental carbon (EC). Surprisingly, PM-bound nitrates were below quantifiable levels, likely due to the region's high relative humidity (>80%) and frequent precipitation, which may have scavenged nitrate salts, given their high water-solubility. However, nitrogen in the form of ammonia (1.5 ± 0.9 µg/m3) and water-soluble nitrogen (2.4 ± 0.8 µg/m3) was abundant in PM1. The concentration of PM₁-bound USEPA priority PAHs was 98.1 ± 11.2 ng/m³. This included 2–3 ring PAHs at 41.5 ± 7.5 ng/m³ and 4–6 ring PAHs at 56.7 ± 7.2 ng/m³.

Both the PM1 mass concentration and chemical characterization showed significant contribution of anthropogenically derived aerosol mass burden. The elevated OC/EC ratio (~6.6), coupled with a high water-soluble organic carbon (WSOC) fraction (~0.8), suggests a significant contribution from biomass burning emissions and active combustion sources in the region during sampling duration. Emissions from tea processing factories, coupled with the unchecked growth of tourist vehicles, are significant contributors to the regional high levels of sulphate, EC, Zn, Mn, Cu, and heavy metals in the ambient air. The influx of marine aerosols from the Arabian Sea further amplifies the regional pollutant load, particularly sulphate concentrations, formed through the atmospheric oxidation of dimethyl sulphide released by oceanic phytoplankton. These marine air masses additionally carry ship emissions, as evidenced by the significant presence of Ni and V in the aerosol composition.

The insights gained from this data at a strategically important geographic location are pioneering and have the potential to make a significant contribution to the development of pollution control policies in ecologically sensitive and high-altitude areas. Additionally, these findings could serve as a valuable resource for advancing climate change research.

How to cite: Gupta, A. D., Gupta, T., Gunthe, S. S., and Singh, A.: Characteristic aerosol properties from ecologically sensitive high-altitude region of Western Ghats in India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-561, https://doi.org/10.5194/egusphere-egu25-561, 2025.

In this study, the observation site Himalayan Cloud Observatory is located at the high-altitude location (30.34 N, 78.40 E, 1706 m above mean sea level) and established at Swami Ram Tirth Campus, Badshahithaul, Tehri Garhwal, Uttarakhand in the western Himalaya. We have identified and characterized the new particle formation events for 12-months period (January to December, 2021) of continuous monitoring of the aerosol size distribution using NanoScan Scanning Mobility Particle Sizer. Another year-long observation was carried out at the Himalayan Atmospheric and Space Physics Research Laboratory (HASPRL), Department of Physics, Hemvati Nandan Bahuguna Garhwal University (A Central University), Srinagar Garhwal, Uttarakhand, in the Alaknanda Valley (30°13'37.3"N, 78°48'14.2"E, 640 m AMSL), from January 1, 2023, to December 31, 2023.

We have observed 51 new particle formation events out of 278 days of observations having 14% frequency of new particle formation occurrence. New particle formation events were most frequent in March-April-May (pre-monsoon) and least frequent in June-July-August-September (monsoon). This trend is linked to high temperatures, strong solar radiation, and low relative humidity in pre-monsoon, which enhance the formation of low-volatility organic compounds, while in monsoon, wet scavenging reduces aerosol precursor gases. The seasonal mean of growth rate (GR11.5-27.4 nm), formation rate (J11.5), coagulation sink (CoagS11.5-27.4) and condensation sink (CSTOT, 11.5-154 nm) during the study period were 1.27±0.23 nm h-1, 0.12±0.08 cm-3 s-1, 2.92±1.65×10-5 s-1 and 9.91±3.13×10-3 s-1 respectively. Seasonal distributions show particles within 11.5–100 nm predominantly originate from secondary emissions, while particles 100–154 nm result from both direct and nucleated process, highlighting the seasonal sources of particles at Himalayan Cloud Observatory. A significant reduction (by 25%) found in incoming solar radiation on non-event days limits the oxidation of precursor gases, thereby inhibiting particle formation. Polar bivariate analysis reveals that winter airmasses, transported via mountain winds from the southwest and northeast, introduce mixed particle sizes. In contrast, the localized concentration of particles with elevated GR11.5-27.4 nm and J11.5 during pre-monsoon highlights the role of aerosol precursors, condensable vapors, and favorable meteorological conditions, emphasizing new particle formation as the dominant particle source. Comparison with prior cloud condensation nuclei study at Himalayan Cloud Observatory reveals that new particle formation significantly supplements cloud condensation nuclei production beyond primary emissions, especially in pre-monsoon. The satellite-based observation of sulfur dioxide and formaldehyde complement and support the condensable vapours during event days at Himalayan Cloud Observatory. At HASPRL, smaller-sized aerosol particles showed an increase in the morning, likely due to emissions from anthropogenic sources originating from the southwest. In the evening, larger-sized aerosol particles were observed to increase, possibly resulting from various human activities such as vehicular emissions, transportation of sand and stone, and other anthropogenic emissions from the southeast. At HCO, particle transport is likely influenced by movement from valley and forested regions, with air masses traveling from the southeast to the southwest.

In summary, this research offers fresh perspectives on the characterization of new particle formation events in the Himalayan region of Uttarakhand. These insights are crucial for comprehending secondary aerosol formation processes worldwide, particularly at the process level. 

How to cite: Gautam, D. A. S. and Singh, K.: New Particle Formation and Growth of Climate-Relevant Aerosols at Two Key Himalayan Sites in Uttarakhand, India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-635, https://doi.org/10.5194/egusphere-egu25-635, 2025.

EGU25-658 | ECS | Posters on site | AS3.22

Quantification of Chemical and Dynamical loss in Recent Antarctic Ozone depletion 

Prasanth Srinivasan, Sunilkumar Kudilil, Anand Narayana Sarma, Satheesh Sreedharan K., and Moorthy Krishnaswamy K

The Montreal Protocol which mandated the global phase-out of ozone-depleting substances, contributed to the gradual recovery of Antarctic stratospheric ozone. Current projections estimate that the Antarctic ozone level recovers to the 1980 values by 2066. However, anomalous behaviours of the Antarctic ozone hole such as increased ozone hole area and prolonged ozone depletion have been observed since 2020. During this period, extreme events such as the Australian bushfires in 2020 and the Hunga Tonga–Hunga Haʻapai volcanic eruption in 2022 injected a significant amount of aerosols into the lower stratosphere. These aerosols provided the surface for chlorine activation reactions, contributing to chemical ozone loss in the polar lower stratosphere. Concurrently, previous studies suggest that the observed ozone depletion is also attributed to dynamic changes in the polar vortex and the descent of mesospheric air to the lower stratosphere. However, the relative percentage contribution of chemical and dynamical loss contributing to total ozone loss in recent years remains unquantified. In this study, we decompose the total ozone loss into chemical and dynamical losses using the passive tracer method, where ozone is considered as a passive tracer and simulated in the Chemical Lagrangian Model of the Stratosphere (CLaMS) using reanalysis data. The difference between the observed and simulated ozone provides information about the chemical ozone loss. These findings will help in advancing our understanding of the factors leading to the recent enhanced ozone depletion and the potential implications on the long-term healing of the ozone layer.

How to cite: Srinivasan, P., Kudilil, S., Narayana Sarma, A., Sreedharan K., S., and Krishnaswamy K, M.: Quantification of Chemical and Dynamical loss in Recent Antarctic Ozone depletion, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-658, https://doi.org/10.5194/egusphere-egu25-658, 2025.

EGU25-1053 | ECS | Posters on site | AS3.22

An Investigation on Source-Specific Health Risks Associated with Metals Present in Clouds over Hilly Regions in Indian Subcontinent 

Md Abu Mushtaque, Shahina Raushan Saikh, Abhishek Biswas, Gopala Krishna Darbha, and Sanat Kumar Das

Entrance of metals in any form through any pathway causes significant damage to human health.  The present study quantifies probabilistic health risk for carcinogenic and non-carcinogenic metals entering through inhalation, ingestion, and dermal routes within the human body for different age groups (children and adults). Water soluble metals (major metals; Na, Ca, K, Al, Mg, and trace metals; Fe, Zn, Sr, Ni, Cu, Mn, Cr, Ba, and Cd,) present into clouds over hilltop sites of the Western Ghats (Mahabaleshwar) and Eastern Himalayas (Darjeeling) situated at the entrance and final destination of monsoonal clouds over Indian Subcontinents are measured using ICP-OES. pH of cloud water is found to be alkaline in nature over both measurement sites. Clouds contain two times higher total soluble metal concentration (TMC) over Mahabaleshwar than that of Darjeeling. Analysis of enrichment factor and PCA suggest road dust, contributes maximum to the loading of metals into the clouds while desert dust coming from Arabian deserts contribute more to the initial clouds found in Western Ghats and fossil fuel influences maximum to the Himalayan clouds. Heavy metal pollution index (HPI) is found to be 14.8 over Mahabaleshwar and 22.6 over Darjeeling indicating relatively higher polluted clouds over Darjeeling due to higher concentrations of toxic metals like Cd and Zn emitted from fossil fuel combustion and road dust. Inhalation of polluted clouds containing higher concentrations of toxic metals like Cd, Cr, Mn, and Ni are the most potential threat to non-carcinogenic diseases. Cd is most dominating metal in clouds over Darjeeling, mainly coming from fossil fuel combustion, and has two folds higher HQ values than the Mahabaleshwar. Cr emitted from industrial waste has the highest carcinogenic health risk factor for children and adults over Mahabaleshwar (3.2×10-7, 2.3×10-7) than that of Darjeeling (2.1×10-7, 1.5×10-7). The present study suggests that clouds contain major metals like Na, Ca, Al, etc., mainly coming from marine sources and desert dust over the Arabian Sea and nearby continental regions while entering to Indian Sub-continental region, and later contaminated with trace metals like Cd, Cr, Cu, Ni, etc. emitted from vehicular emissions, industrial waste, and road dust that have greater impact on human health via inhalation pathway responsible for non-carcinogenic and carcinogenic diseases.

How to cite: Mushtaque, M. A., Saikh, S. R., Biswas, A., Darbha, G. K., and Das, S. K.: An Investigation on Source-Specific Health Risks Associated with Metals Present in Clouds over Hilly Regions in Indian Subcontinent, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1053, https://doi.org/10.5194/egusphere-egu25-1053, 2025.

The Hindu Kush Himalayan (HKH) region holds substantial strategic significance owing to its extensive reserves of pristine water in the form of glaciers. In recent years, significant levels of particulate pollution have been documented within the high-altitude regions of the Himalayas. The influence of the albedo changes due to aerosol pollutants deposition on the glacial mass balance due to an excess and earlier snow melting, and thereby an earlier glacier runoff, is expected to impact the downstream hydrology. This is specifically of concern for the HKH region as the Himalayan glaciers are the source of major rivers in South Asia. The remote topography and severe weather conditions prevalent in the Himalayan region, however pose challenges to obtaining consistent spatial-temporal measurements of atmospheric aerosol concentration and their presence in snow. The simulated aerosol species concentration, using atmospheric chemical transport models (CTMs), which is validated by measurements, can be utilized to predict the spatial mapping of aerosol species distribution over the HKH region. In order to spatially map the estimates of atmospheric aerosol species concentration and their concentration in snow as adequately as possible, including the corresponding snow-albedo reduction over the HKH region, an integrated approach merging the relevant information from observations with a relatively consistent atmospheric chemical transport model estimates are applied in the present study.

We examine the cumulative and relative impact of aerosol species over the HKH region, including aerosol concentration in the snow, impacts on snow albedo re duction (SAR) and enhanced annual glacier snowmelt runoff identifying the hotspot locations. This is done evaluating aerosols transport simulations corresponding to dust, sulfate, and organic carbon (OC) aerosols relative to black carbon (BC) in free-running (freesimu) atmospheric general circulation model (GCM) and application of constrained (constrsimu) aerosol simulations, aerosol-snow radiative interaction model, and a novel hypsometric glacier energy mass balance model. Estimates for aerosol species concentrations from freesimu demonstrated increased accuracy at high-altitude (HA) stations compared to their performance at low-altitude (LA) stations. Conversely, estimates from constrsimu exhibited notably better performance at LA stations. The pre-monsoon aerosol species deposited in snow (> 850 µg kg−1 over Gangotri and Chorabari) were the highest among glaciers, being about 40% greater than winter with OC including BC over selected glaciers and dust across all glaciers as compared to sulphate being twice larger than winter. The annual runoff increase (ARI) from the cumulative impact due to all aerosols showed the most significant ARI for Pindari glacier (about 500 mm w.e. y−1), with five out of the nine glaciers, including Sankalpa, Milam, Gangotri, and Chorabari, had an ARI exceeding 300 mm w.e. y−1. Analysis from source- and region-tagged simulations indicates about 50 to 60% of aerosols-induced ARI can be mitigated by controlling BC aerosols over the region originating from open-biomass burning emissions mainly in the Indo Gangetic plain (IGP) and far-off region.

How to cite: Verma, S.: Simulations of cumulative and relative impact of aerosol species over the Hindu Kush Himalayan region: validation, implications on glacier runoff, and source control, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1125, https://doi.org/10.5194/egusphere-egu25-1125, 2025.

EGU25-7323 | ECS | Posters on site | AS3.22

Overview of Atmospheric Aerosol Observations during the ATWAICE Expedition in the Central Arctic 

Arun Babu Suja, Thomas Müller, Mira Pöhlker, Heike Wex, Andreas Held, Manuela van Pinxteren, Yifan Yang, Philipp Oehlke, Sabine Lüchtrath, Holger Siebert, Theresa Mathes, Maik Merkel, and Birgit Wehner

Understanding aerosol particles in the Arctic is crucial due to their impact on the region’s radiative balance and their role in modifying cloud properties. These interactions drive unique feedback mechanisms that enhance Arctic warming and influence global climate systems. Consequently, it is important to identify and quantify Arctic aerosol particle sources and sinks, including their vertical transport, and to characterize their optical properties and resulting effects on cloud formation. Despite the importance of aerosol particles in the Arctic, there is a lack of direct measurements of aerosol particles over the Arctic especially over the Arctic marine boundary layer. In this context, we have conducted aerosol measurements aboard the German research vessel Polarstern during the ATWAICE (Atlantic Water Pathways to the Ice in the Nansen Basin and Fram Strait) expedition from June to August 2022. This study included continuous measurements of physical and chemical aerosol parameters to investigate variations in aerosol properties. On-line measurements of black carbon (BC) and its mixing state were complemented by off-line analyses of seawater and fog water samples to identify transport pathways of BC particles. Additionally, seawater, aerosol filter samples, and fog water samples were analyzed to explore how ice nucleating particles are linked across these compartments. Vertical profiles of aerosol particles were measured above different surface conditions to examine the direction of vertical particle transport. Higher aerosol concentrations were recorded as the ship passed through the outer margin of the marginal ice zone, where marine sources dominate, supported by evidence of significant photochemical ageing processes. The highest values of refractory black carbon (rBC) and light scattering coefficients were measured during the transact from northern Europe to the Arctic circle (between 56°N to 70°N), with average rBC concentrations of approximately 40 ng m-3 and light scattering at 525 nm averaging ~29 Mm-1. During this period, air mass trajectories reflected a nearly equal influence from both continental and marine sources. In contrast, the lowest scattering and absorption values were observed in the central Arctic, when the ship navigated in densely packed ice regions under the influence of north-easterly air masses originating over the Arctic Ocean. A comprehensive analysis of these findings will be presented in this presentation.

How to cite: Babu Suja, A., Müller, T., Pöhlker, M., Wex, H., Held, A., van Pinxteren, M., Yang, Y., Oehlke, P., Lüchtrath, S., Siebert, H., Mathes, T., Merkel, M., and Wehner, B.: Overview of Atmospheric Aerosol Observations during the ATWAICE Expedition in the Central Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7323, https://doi.org/10.5194/egusphere-egu25-7323, 2025.

EGU25-8039 | Orals | AS3.22

What have we learned from one year of aerosol observations in the central Arctic during the MOSAiC expedition? 

Julia Schmale, Benjamin Heutte, Nora Bergner, Ivo Beck, Lubna Dada, Helene Angot, Camille Mavis, Kevin Barry, Jessica Mirrieless, Matthew Boyer, Lauriane Quelever, Tuija Jokinen, Kerri Pratt, and Jessie Creamean

The central Arctic ocean (CAO) is transforming rapidly due to climate change with wide spread consequences. Therefore, understanding the mechanisms of change, in particular related to the surface energy budget, is indispensable. Aerosols affect the surface radiation budget both directly and indirectly through interactions with clouds.

In the CAO, cloud formation and radiative processes are particularly susceptible to aerosols, because their number concentration can be very low. To date, the climatic effects of aerosols in the CAO have mostly been constrained in terms of anthropogenic emissions and direct radiation interactions, where a significant warming contribution has been found. What is missing, are effects of natural aerosols and aerosol-cloud interactions. It is hence of utmost importance to fully understand the present-day aerosol-climate interactions, constrain the most relevant processes and how they relate to Arctic change in order to anticipate future impacts.

However, the CAO is an inherently difficult place to study due to its limited physical accessibility as well as hampered satellite observations. To mitigate the observational scarcity, the ‘Multidisciplinary Observatory for the Study of Arctic Change’ (MOSAiC) expedition drifted for one year between fall 2019 and 2020 in the CAO.

In this contribution, we will present our insights from one year of aerosol observations that include variables such as cloud condensation nuclei and ice nucleating particle number concentrations, particle number size distributions, bulk and single particle chemical composition as well as optical properties. This presentation will specifically focus on unprecedented insights, for example the roles of processes like blowing snow and sea spray emissions and warm air mass intrusions, as well as the abundance of biogenic and biological aerosol components.

How to cite: Schmale, J., Heutte, B., Bergner, N., Beck, I., Dada, L., Angot, H., Mavis, C., Barry, K., Mirrieless, J., Boyer, M., Quelever, L., Jokinen, T., Pratt, K., and Creamean, J.: What have we learned from one year of aerosol observations in the central Arctic during the MOSAiC expedition?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8039, https://doi.org/10.5194/egusphere-egu25-8039, 2025.

EGU25-9716 | Posters on site | AS3.22

Expanding the Langley Calibration Method to Infrared Wavelengths: Modeling, Validation, and Applications 

Denghui Ji, Mathias Palm, Xiaoyu Sun, and Justus Notholt

Aerosol optical depth (AOD) observations are usually focused on the visible wavelength. Recent studies highlight the potential of the infrared emission waveband in providing valuable insights for aerosol compositions (Ji et al., 2023). Expanding AOD measurements into the infrared spectrum offers an approach to enhance our understanding of aerosol properties. In this study, we use solar absorption spectra measured by Fourier Transform Infrared Spectrometer (FTIR) to obtain the infrared spectrum AOD using Langley method (Barreto et al., 2020) in several stations, including Ny-Ålesund (Arctic), Bremen (mid-latitude), and Palau (tropics). Integrating FTIR and sun-photometer observations, we obtain AOD in visible and infrared spetrum regions. This work highlights the possibility of extending traditional AOD retrieval method in visible wavelengths to a broad spectrum range.

 

Reference:

Ji, D., Palm, M., Ritter, C., Richter, P., Sun, X., Buschmann, M., and Notholt, J.: Ground-based remote sensing of aerosol properties using high-resolution infrared emission and lidar observations in the High Arctic, Atmos. Meas. Tech., 16, 1865–1879, https://doi.org/10.5194/amt-16-1865-2023, 2023.

Barreto, África, Omaira Elena García, Matthias Schneider, Rosa Delia García, Frank Hase, Eliezer Sepúlveda, Antonio Fernando Almansa, Emilio Cuevas, and Thomas Blumenstock. 2020. "Spectral Aerosol Optical Depth Retrievals by Ground-Based Fourier Transform Infrared Spectrometry" Remote Sensing 12, no. 19: 3148. https://doi.org/10.3390/rs12193148

How to cite: Ji, D., Palm, M., Sun, X., and Notholt, J.: Expanding the Langley Calibration Method to Infrared Wavelengths: Modeling, Validation, and Applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9716, https://doi.org/10.5194/egusphere-egu25-9716, 2025.

EGU25-11582 | ECS | Orals | AS3.22

Seasonal characteristics in physical properties of refractory black carbon aerosols at a central European background site Melpitz 

Yifan Yang, Thomas Müller, Laurent Poulain, Baseerat Romshoo, Samira Atabakhsh, Bruna A Holanda, Jens Voigtländer, Shubhi Arora, and Mira L Pöhlker

Black carbon (BC) is the most absorbing atmospheric aerosol and, therefore, influences the Earth’s climate system. Uncertainties in BC climate forcing estimates can be attributed to a limited understanding of its size distribution, mixing state, morphology, spatiotemporal distribution, and optical properties, all of which require more representative and long-term measurements (Bond et al., 2013; Liu et al., 2020). To investigate the long-term variation of BC physical properties, continuous measurements were conducted at the central European rural background site Melpitz (Germany) from August 2021 to February 2022. Mass concentrations, size distributions, and mixing state of BC were measured by a Single Particle Soot Photometer (SP2). A thermodenuder (300⁰C) was connected upstream of the SP2 to remove the volatile coating of BC. In addition, the light absorption coefficients were measured using a multi-angle absorption photometer (MAAP).

Different air masses associated with distinct refractory black carbon (rBC) properties were identified in summer (August) and winter (December). In summer, rBC exhibited a similar mass concentration (~0.16 μg m-3) among different air masses, with the smallest mass median diameter (MMD) of rBC overserved in the long transportation from the northwest (140nm), while in winter, the highest concentration (1.23 μg m-3) and largest MMD (216 nm) were both observed in easterly air masses. Thickly coated rBC fractions increased during the daytime in summer, indicating that photochemical processes significantly influence the rBC mixing state. In winter, a higher fraction (27%) of thickly coated rBC in the cold air mass compared to the warm air masses (14%) suggests the contribution of residential heating emissions to the mixing state. Most rBC particles retained a low-volatile coating when passing the thermodenuder with a mass fraction of 58%. In summer, photochemical processes also contribute to the volatility of coating, showing a higher fraction of rBC particles containing low-volatile coatings during the daytime. In winter, low-volatile coatings showed no significant diurnal variation and were more dependent on ambient temperature. Therefore, the volatility of rBC coatings in winter is more influenced by emission sources, particularly residential heating, rather than atmospheric processes. The optical properties of rBC showed seasonal variations as well, which were caused by changes in size distribution and mixing state.

 

Bond, T. C., et al. (2013). "Bounding the role of black carbon in the climate system: A scientific assessment." Journal of Geophysical Research: Atmospheres 118(11): 5380-5552.

Liu, D., et al. (2020). "Lifecycle of light-absorbing carbonaceous aerosols in the atmosphere." npj Climate and Atmospheric Science 3(1).

              

How to cite: Yang, Y., Müller, T., Poulain, L., Romshoo, B., Atabakhsh, S., Holanda, B. A., Voigtländer, J., Arora, S., and Pöhlker, M. L.: Seasonal characteristics in physical properties of refractory black carbon aerosols at a central European background site Melpitz, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11582, https://doi.org/10.5194/egusphere-egu25-11582, 2025.

EGU25-11958 | Posters on site | AS3.22

Ships of Opportunity for Atmospheric Research: Pilot Efforts 

Jean-Francois Lamarque, Alex Wong, Samuel Kaufman, Dan Bowen, Sarah Schubert, Colm Sweeney, Betsy Andrews, and Berend van de Kraats

Processes occurring over the oceans, including greenhouse gas (GHG) fluxes and cloud-aerosol interactions, are a major source of uncertainty in the present climate state and hence in estimating near-term warming. To reduce this uncertainty, more comprehensive and specific observations over the oceans are needed. Due to the limited supply of dedicated research vessels, platforms of opportunity are essential to fill these observational gaps. We discuss here the Ships of Opportunity for Atmospheric Research (SOAR) program, a science infrastructure program built in collaboration with OceansX. SOAR’s purpose is to expand atmospheric observations in under-observed oceanic regions, providing new measurements to existing climate observation programs that provide open data to the global community.

 

We present current pilot projects under SOAR. A GHG flask sampler from NOAA Global Monitoring Lab is deployed on the Maersk Kentucky, which is taking samples as the ship transits the tropical Pacific. Sensors from NASA’s Maritime Aerosol Network (AERONET MAN), are also deployed on two other Maersk vessels and a Smyril Line vessel, where volunteer sailors are collecting aerosol optical depth measurements that are now accessible on the AERONET/MAN webpage. Finally, in collaboration with NOAA Global Monitoring Laboratory, SilverLining is developing a version of the NOAA Federated Aerosol Network (NFAN) package for deployment on ships of opportunity. This effort includes integrating instruments into a system adapted to marine environments and validating it against the NFAN technical standards. This project serves as a proof of concept for including additional higher-complexity atmospheric instrumentation packages in ships of opportunity programs

How to cite: Lamarque, J.-F., Wong, A., Kaufman, S., Bowen, D., Schubert, S., Sweeney, C., Andrews, B., and van de Kraats, B.: Ships of Opportunity for Atmospheric Research: Pilot Efforts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11958, https://doi.org/10.5194/egusphere-egu25-11958, 2025.

EGU25-12303 | ECS | Posters on site | AS3.22

Seasonal Dynamics and Radiative Impacts of Black Carbon in the Yumthang Valley in Sikkim Himalaya, India 

Aparna Gupta, Rakesh Kumar Ranjan, Abhilash Panicker, Vrinda Anand, and Rajeev Rajak

Black carbon (BC) aerosols are a major concern in changing climatic scenario due to their ability to absorb solar radiation. This study investigates the temporal variation of BC and its impact on radiative forcing in the Sikkim Himalayan region. It aimed to understand the optical properties of BC and its radiative forcing at Yumthang Valley, a high-altitude (~3800 m) remote location in North Sikkim, India. In-situ measurements were undertaken to quantify BC mass concentration, using an Aethalometer, and satellite retrieval techniques were employed to assess the optical properties of BC during May 2022 to April 2024. The monthly mean BC concentration in the valley ranged from 1.03 ± 3.07 to 9.54 ± 16.44 µgm-3, with an annual mean of 5.07 ± 16.54 µgm-3. BC concentrations decrease during monsoon months due to limited long-range transport and effective wet scavenging. Biomass burning contributes significantly to BC levels, accounting for 88% of the total, with the highest contribution in September (55%) and the lowest in February (21%). Transport models indicate inputs from the Indo-Gangetic Plain and adjacent valleys with increased biomass burning activity. Seasonal variations reflect tourism-driven emissions and local wood burning, with the lowest levels observed in the early morning hours. BC-induced direct radiative forcing (DRF) was also calculated at the surface (SFC) and top of the atmosphere (TOA) using Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) model which estimate a substantial forcing at both the surface and top of the atmosphere. The BC-induced atmospheric heating rates suggest potential regional warming, which could accelerate glacier melt in the region.

How to cite: Gupta, A., Ranjan, R. K., Panicker, A., Anand, V., and Rajak, R.: Seasonal Dynamics and Radiative Impacts of Black Carbon in the Yumthang Valley in Sikkim Himalaya, India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12303, https://doi.org/10.5194/egusphere-egu25-12303, 2025.

EGU25-12522 | ECS | Posters on site | AS3.22

When the World Stopped: Insights into Aerosol masking effect and Black Carbon Source Shifts 

Hari Ram Chandrika Rajendran Nair

Understanding the pathways through which aerosols are emitted, transformed, and removed in remote and climatically sensitive regions is essential for minimizing uncertainties in global climate modeling. This study capitalizes on the unique conditions created by the COVID-19 societal slowdown to explore anthropogenic aerosol behavior over South Asia. Observations during this period showed a marked decline in aerosol concentrations, resulting in a demasking effect comparable to nearly 75% of the radiative forcing induced by CO₂ in the region. Additionally, this reduction caused a ~7% increase in surface-reaching solar radiation and a ~0.4 K d⁻¹ decrease in atmospheric solar heating.

Black carbon (BC) aerosols were further analyzed using dual-isotope (Δ¹⁴C and δ¹³C) techniques at monitoring sites in the Maldives and Bangladesh. Findings revealed a significant decrease in fossil fuel-derived BC, dropping from 49% to 35%, while emissions from C₃ biomass burning rose from 31% to 55%. These changes reflect reduced fossil fuel usage alongside increased reliance on crop residue burning and biomass for domestic energy needs during the slowdown.

These findings highlight the complex interplay between human activities and natural processes in determining aerosol-climate interactions across South Asia. The rapid changes in emission patterns observed during societal disruptions underscore the potential for targeted policy interventions to mitigate climate impacts and reduce atmospheric pollution.

How to cite: Chandrika Rajendran Nair, H. R.: When the World Stopped: Insights into Aerosol masking effect and Black Carbon Source Shifts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12522, https://doi.org/10.5194/egusphere-egu25-12522, 2025.

EGU25-14674 | ECS | Posters on site | AS3.22

Vertical profiles of black carbon measured using high-altitude balloon experiments over an urban location in India 

Kudilil Sunilkumar, Aravindakshan Ajay, Narayana Sarma Anand, Sreedharan Krishnakumari Satheesh, and Krishnaswamy Krishna Moorthy

Aerosol Black Carbon (BC) can influence Earth’s radiation balance and climate in numerous ways. Atmospheric warming and the modification of the local thermodynamic structure of the atmosphere, cloud formation and precipitation are known to be influenced by BC aerosols. Many of these effects depend on the vertical distribution of BC. When the concentration of absorbing aerosols such as BC are significant, Aerosol Optical Depth (AOD) and chemical composition are not the only determinants of aerosol radiative effects. Under such circumstances, the altitude of the aerosol layers also plays a crucial role. Thus, high BC loading at elevated altitudes is of utmost importance to regional weather and climate. These elevated aerosols can further be lofted to the upper troposphere and lower stratospheric regions through strong tropical monsoonal updrafts. Despite the above significances of elevated BC layers, measurements of the vertical distribution of BC in the middle and upper tropical troposphere are extremely scarce due to the difficulties in devising suitable instrumentation. Hence, direct measurements of BC are virtually non-existent at altitudes around 10 km or above. Under this backdrop, we conducted a series of high-altitude balloon observations to improve the understanding of such elevated layers. Results of these experiments conducted during the winter and pre-monsoon summer seasons of the years 2023-2024 show several elevated layers of BC aerosol, reaching as high as three times that of the surface concentrations. In the mid/upper troposphere, aircraft engine exhaust is the main if not the only source for anthropogenic emissions, with a technology trade-off existing between the fuel performance of engines, and climate forcers. The role of aircraft emissions in the mid-tropospheric region in contributing to these layers has also been examined in the background of balloon experiments.

How to cite: Sunilkumar, K., Ajay, A., Anand, N. S., Satheesh, S. K., and Krishna Moorthy, K.: Vertical profiles of black carbon measured using high-altitude balloon experiments over an urban location in India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14674, https://doi.org/10.5194/egusphere-egu25-14674, 2025.

EGU25-15052 | ECS | Posters on site | AS3.22

Investigating marine driven new particle formation during the SOPHYAC-light campaign 

Lauriane L J Quéléver, Madeleine Bahr, Clémence Rose, Marie Bassez, Theresa Barthelmess, Celine Dimier, Gabriel Dulaquais, Alex Eschalier, Hendrick Fiel, William Frère, Riel Ingeniero, Baptiste Néel, Emmanuelle Raimbault, Celine Ridame, Marie Boyé, and Karine Sellegri

The Antarctic region is a large component of the global climate system.  While it is largely underrepresented in climate models due to the scarcity of in-situ data, the interactions between processes occurring mid- and high-latitude are even less investigated. Understanding the processes between the atmosphere, the ocean laying within the polar front is critical to assert the relevance of climate models and improve future climate predictions. 

The SOPHYAC-light (Responses of the Southern Ocean PHYtoplankton to climate changes, feedback to the Atmosphere -impact of Light) took place onboard of the research vessel Marion Dufresne during the Obs’Austral campaign 2025 between December 24th 2024 and February 5th 2025. Air-sea interaction process studies were performed using two Air-Sea Interface Tanks (ASIT, Sellegri et al. 2023) in the aim of quantifying realistic air-sea fluxes and their relation to seawater biochemical properties, as well as the impact of UV light on these processes.  The twotanks, one as a control and the other UV shielded, were filled with 1 m3 of seawater each at 7 different locations of the Southern Ocean, between sub-tropical and sub-Antarctic regions along the ship track.  The incubation time varied between 4 and 6 days with coordinated water sample coupled with continuous atmospheric sampling within the head space of the two ASITS, with measurements of chemical, physical & biological parameters. The atmospheric measurements were focused on the investigation of new particle formation, encompassing three mass spectrometers for the characterization of gas phase precursors of aerosols and nanoparticle size distribution. A first overview of the SOPHYAC results related to new particle formation purely driven by the marine environment and ecosystem across the tropical / polar transect will be presented at the conference.

 

How to cite: Quéléver, L. L. J., Bahr, M., Rose, C., Bassez, M., Barthelmess, T., Dimier, C., Dulaquais, G., Eschalier, A., Fiel, H., Frère, W., Ingeniero, R., Néel, B., Raimbault, E., Ridame, C., Boyé, M., and Sellegri, K.: Investigating marine driven new particle formation during the SOPHYAC-light campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15052, https://doi.org/10.5194/egusphere-egu25-15052, 2025.

EGU25-15303 | ECS | Posters on site | AS3.22

The annual cycle and sources of relevant aerosol precursor vapors in the central Arctic during the MOSAiC expedition 

Matthew Boyer, Diego Aliaga, Lauriane Quéléver, Silvia Bucci, Hélène Angot, Lubna Dada, Benjamin Heutte, Lisa Beck, Marina Duetsch, Andreas Stohl, Ivo Beck, Tiia Laurila, Nina Sarnela, Roseline Thakur, Branka Miljevic, Markku Kulmala, Tuukka Petäjä, Mikko Sipilä, Julia Schmale, and Tuija Jokinen

In this study, we present and analyze the first continuous time series of relevant aerosol precursor
vapors from the central Arctic (north of 80° N) during the Multidisciplinary drifting Observatory for the Study of
Arctic Climate (MOSAiC) expedition. These precursor vapors include sulfuric acid (SA), methanesulfonic acid
(MSA), and iodic acid (IA). We use FLEXPART simulations, inverse modeling, sulfur dioxide (SO2) mixing
ratios, and chlorophyll a (chl a) observations to interpret the seasonal variability in the vapor concentrations
and identify dominant sources. Our results show that both natural and anthropogenic sources are relevant for the
concentrations of SA in the Arctic, but anthropogenic sources associated with Arctic haze are the most prevalent.
MSA concentrations are an order of magnitude higher during polar day than during polar night due to seasonal
changes in biological activity. Peak MSA concentrations were observed in May, which corresponds with the
timing of the annual peak in chl a concentrations north of 75° N. IA concentrations exhibit two distinct peaks
during the year, namely a dominant peak in spring and a secondary peak in autumn, suggesting that seasonal IA
concentrations depend on both solar radiation and sea ice conditions. In general, the seasonal cycles of SA, MSA,
and IA in the central Arctic Ocean are related to sea ice conditions, and we expect that changes in the Arctic
environment will affect the concentrations of these vapors in the future. The magnitude of these changes and the
subsequent influence on aerosol processes remains uncertain, highlighting the need for continued observations
of these precursor vapors in the Arctic.

How to cite: Boyer, M., Aliaga, D., Quéléver, L., Bucci, S., Angot, H., Dada, L., Heutte, B., Beck, L., Duetsch, M., Stohl, A., Beck, I., Laurila, T., Sarnela, N., Thakur, R., Miljevic, B., Kulmala, M., Petäjä, T., Sipilä, M., Schmale, J., and Jokinen, T.: The annual cycle and sources of relevant aerosol precursor vapors in the central Arctic during the MOSAiC expedition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15303, https://doi.org/10.5194/egusphere-egu25-15303, 2025.

EGU25-15525 | Posters on site | AS3.22

Biogenic volatile organic compounds emissions from the coastal waters of Gulf of Finland, Baltic Sea and their role in aerosol formation 

Roseline Thakur, Maija Peltola, Kurt Spence, Heidi Hellén, Toni Tykkä, Joanna Norkko, Alf Norkko, Markku Kulmala, and Mikael Ehn

The dearth of measurements of Volatile Organic Compounds (VOCs) in the marine boundary layer have raised question on how the marine environment is impacted or can impact the overlying atmosphere. VOCs emissions in the interface between air and soil, snow or ocean plays a major role in atmospheric oxidation processes, gas-particle transfer and the formation of secondary organic aerosols. Recent studies indicate that some VOCs produce low volatility vapors through the process of autoxidation (Ehn et al., 2014). These low volatility vapors under atmospheric conditions may rapidly form highly oxygenated molecules (HOMs) which act as important precursor vapors leading to new particle formation (NPF). Extensive studies have been done for the terrestrial VOC fluxes and much less attention has been given to the marine emissions of VOCs (Yu and Li, 2021). Coastal NPF may lead to the formation of coastal/marine clouds, which affect many coastal ecosystem processes and the radiation budget globally. Some of the previous studies in coastal settings have identified biogenic emissions as the main driving factor for the NPF (O'Dowd et al., 2002). Every year extensive cyanobacterial blooms occur in the Baltic Sea region and Finnish water bodies, and these blooms could be a significant source of iodic acid, biogenic sulphuric acid and methane sulphonic acid, and possibly biogenic volatile organic compounds (BVOCs) (Thakur et al., 2022) yet no marine BVOC fluxes field studies have been reported so far from this sector.

To understand sea to air emission processes of BVOCs and their role in aerosol formation, we have set up a permanent atmospheric laboratory at the Tvärminne Zoological Station (TZS) on the Finnish coast of the Baltic Sea in 2022, under the project “CoastClim” (https://coastclim.org). The laboratory houses state of the art instrumentation to measure the gaseous composition and aerosol size distribution. The continuous measurement of Dimethyl sulphide (DMS) and monoterpenes at the coast, through proton transfer reaction-time of flight mass spectrometer (PTR-ToF-MS) suggests high emissions during the bloom period in summer (June-August 2023). A field experiment through floating glass chamber flux measurements over the algae and phytoplankton rich waters was also carried out at the coastal site of TZS station from 30th May 2022 to 8th June 2022. The samples were collected in Tenax tubes and analyzed using a thermal-desorption instrument connected to a gas chromatograph (Mäki et al., 2017) with a mass selective detector. The results showed high isoprene fluxes followed by a-pinene and other terpenes.

Further investigation on the source and processes of the biogenic VOC emission from the sea surface and oxidation chemistry happening in the air is needed to link these emissions to aerosol formation at the TZS coast. Connecting the coastal emissions to aerosol formation for understanding the impacts of climate change is one of the core aims of our multidisciplinary project “CoastClim”.

 

O’Dowd et al., 2002: doi:10.1038/nature00775

Ehn, M.et al., 2014 : https://www.nature.com/articles/nature13032

Mäki M.et al, 2017: https://doi.org/10.5194/bg-14-1055-2017.

Yu & Li., 2021: https://doi.org/10.1016/j.scitotenv.2021.145054

Thakur, R.C, et al., 2022: doi.org/10.5194/acp-22-6365-2022.

How to cite: Thakur, R., Peltola, M., Spence, K., Hellén, H., Tykkä, T., Norkko, J., Norkko, A., Kulmala, M., and Ehn, M.: Biogenic volatile organic compounds emissions from the coastal waters of Gulf of Finland, Baltic Sea and their role in aerosol formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15525, https://doi.org/10.5194/egusphere-egu25-15525, 2025.

EGU25-16516 | Orals | AS3.22

Role of ozone in enhancing the formation of aerosol precursors in the OH-initiated oxidation of naphthalene 

Avinash Kumar, Prasenjit Seal, Olga Garmash, Aliisa Ojala, Siddharth Iyer, Shawon Barua, and Matti Rissanen

The high yield of condensable vapors from OH-initiated oxidation of naphthalene raises intriguing questions about the role of ozone in this process. As the simplest polycyclic aromatic hydrocarbon (PAH), naphthalene is a significant component of anthropogenic volatile organic compounds (AVOCs) in urban atmospheres, characterized by its high reactivity and prevalence among PAHs. Emitted primarily through the incomplete combustion of fossil fuels and biomass, naphthalene plays a pivotal role in atmospheric chemistry under ambient conditions. While recent studies (Zhang et al., 2012; Garmash et al., 2020) highlight the substantial contribution of naphthalene to secondary organic aerosol (SOA) formation, these are in conflict with our current molecular level understanding of the oxidation process. In the atmosphere, naphthalene is quickly oxidized by the addition of an OH radical to the aromatic ring, forming a carbon-centered radical (Shiroudi et al., 2015, Gnanaprakasam et al., 2017). This subsequently reacts with O₂ to generate peroxy radicals, which undergo autoxidation, resulting in the formation of low-volatility products containing multiple oxygen atoms i.e., highly oxygenated organic molecules (HOM) which contribute to SOA formation. However, molecular level studies indicate autoxidation rates that are much too slow to explain the observed HOM in the oxidation of naphthalene. Also, previous experiments that measured HOM yields from OH-initiated oxidation of naphthalene (Molteni et al., 2018, Garmash et al., 2020) did not investigate the effect of ozone. We think that ozone is the missing piece in resolving the discrepancy between our current molecular level understanding of naphthalene oxidation and measurements.

In this study, laboratory experiments were conducted to investigate the oxidation of naphthalene by hydroxyl (OH) radicals using a flow reactor coupled with a nitrate-based chemical ionization mass spectrometer (NO₃⁻-CIMS). The influence of ozone on the reaction products was systematically explored. Results revealed a significant enhancement in product intensities, particularly monomers (C₁₀H₉O₅-₁₀), in the presence of ozone. The reaction time was varied from 2.1 – 0.7 seconds. At a reaction time of 0.7 seconds, the addition of ozone led to the formation of a series of monomeric products that were absent in the ozone-free environment. Complementary high-level quantum chemical calculations provided mechanistic insights into the role of ozone in product formation. To further elucidate product formation pathways, experiments were also conducted for the OH-initiated oxidation of naphthalene derivatives such as 1-naphthol and 2-naphthol. A significant effect of ozone was observed in the oxidation of 1-naphthol, whereas no prominent change was noted in the case of 2-naphthol. These findings indicate that the oxidation of naphthalene proceeds rapidly enough to compete with other bimolecular reactions such as RO2 + RO2/HO2/NO, and the presence of ozone is crucial for the formation of HOM and consequently has a pronounced effect on the SOA formation.

References:

Zhang, Z. et al (2012) Phys. Chem. Chem. Phys. 14, 2645 - 2650.

Garmash, O. et al (2020) Atmos. Chem. Phys. 20, 515-537.

Shiroudi, A. et al (2015) Phys. Chem. Chem. Phys. 17, 13719-13732.

Gnanaprakasam, M. et al (2017) Theor. Chem. Acc. 136, 131.

Molteni, U. et al (2018) Atmos. Chem. Phys. 18, 1909-1921.

How to cite: Kumar, A., Seal, P., Garmash, O., Ojala, A., Iyer, S., Barua, S., and Rissanen, M.: Role of ozone in enhancing the formation of aerosol precursors in the OH-initiated oxidation of naphthalene, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16516, https://doi.org/10.5194/egusphere-egu25-16516, 2025.

EGU25-17907 | ECS | Posters on site | AS3.22

Relating aerosol optical properties to different emission sources at a coastal site in Sweden 

Jane Tygesen Skønager, Matthew Salter, Merete Bilde, and Bernadette Rosati

Atmospheric aerosols contribute to the largest uncertainty in estimates of the Earth’s global energy balance. Their interactions with sunlight and their ability to affect cloud formation leads to both direct and indirect influence of radiative forcing. The substantial uncertainties associated with aerosol climate effects stem amongst others from the complexity of their sources, composition, and properties. Aerosols in coastal areas present a challenging mix of inorganic and organic particles from diverse sources, making measurements and characterization of their properties in these regions essential. 

This study presents measurements of the optical properties of ambient aerosols on Askö, Sweden, from October 2024 to January 2025. Askö, an island and nature reserve located approximately 80 km south of Stockholm, experiences low levels of local pollution, making it an ideal location for studying marine aerosols. Its location in the Trosa Archipelago, facing the Baltic Sea, also makes it well-suited for investigating the impact of long-range transport from Central and Eastern Europe.

Instruments were placed in a container situated on top of a floating platform near the island. Scattering coefficients, measured with a nephelometer, and absorption coefficients, measured with an aethalometer, were used to calculate Scattering and Absorption Ångström Exponents. The Ångström matrix was used to characterize aerosol types found in the area at different times. The optical data set is further complemented by local meteorological data, particle size distributions, and back trajectory analysis. This combination of data will give valuable insights into aerosol sources at this remote location, the degree of aerosol ageing, and the identification of prevailing emissions sources such as local emissions versus long-range transport of air masses.   

How to cite: Tygesen Skønager, J., Salter, M., Bilde, M., and Rosati, B.: Relating aerosol optical properties to different emission sources at a coastal site in Sweden, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17907, https://doi.org/10.5194/egusphere-egu25-17907, 2025.

EGU25-18161 | ECS | Orals | AS3.22

Aerosol volatility over High-Altitude site in Western Ghats, India: Effect of semi-volatile organics coating 

Subrata Mukherjee, Rohit Dilip Patil, Aslam Yusuf, Ghuman Singh Meena, Anil Kumar Vasudevan, Anoop Sharad Mahajan, Liselotte Tinel, Vinayak Waghmare, Sachin Suresh Patil, and Pandithurai Govindan

Sub-micron aerosols are primarily consisted of organics, sulfate, nitrate, ammonium etc. and among which organics have high complexity in its chemical and physical characteristics. In the present study, aerosol volatility of non-refractory sub-micron aerosol was extensively studied during 6th – 20th February of 2021 utilizing high-resolution Time of flight Aerosol Mass Spectrometer (HR-TOF AMS) coupled with Thermal denuder. The temperature was set to 150oC and the denuded and non-denuded ambient aerosol was then sampled utilizing a switching valve with 10 minute time interval. Nitrate and Ammonium possessed highest volatility (80% and 68%) which was followed by organics with volatility rate of 54%. Sulfate was observed to be the least volatile (26%).The volatility extent for organics was low in afternoon and night-early morning hours due to possible prevalence of oxygenated organic aerosols (secondary organic aerosol) during these time period. Further PMF was done on the denuded and non-denuded organics aerosol dataset and the analysis revealed 4 factors namely, Hydrocarbon like organic aerosol (HOA), Biomass burning organic aerosol (BBOA), semi-volatile oxygenated organic aerosol (SVOOA) and low-volatile oxygenated organic aerosol (LV-OOA). LV-OOA fractional contribution increased from 31% to 56% of total organics. SVOOA, HOA, BBOA being a primary aerosol, showed decreasing trend as they have higher volatility than LVOOA. Interestingly, of SV-OOA volatility was even higher than that of the other primary aerosols (HOA, BBOA). The possible reason may be SV-OOA is freshly formed and can be deposited on to pre-existing aerosols like inorganic aerosols, HOA, BBOA, LV-OOA etc which indicated the effect of possible coating.

How to cite: Mukherjee, S., Patil, R. D., Yusuf, A., Meena, G. S., Vasudevan, A. K., Mahajan, A. S., Tinel, L., Waghmare, V., Patil, S. S., and Govindan, P.: Aerosol volatility over High-Altitude site in Western Ghats, India: Effect of semi-volatile organics coating, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18161, https://doi.org/10.5194/egusphere-egu25-18161, 2025.

EGU25-18522 | Orals | AS3.22

Evaluation of in-situ metrics for determining the influence of the Planetary Boundary Layer at the Helmos Hellenic Atmospheric Aerosol & Climate Change (HAC)2 station  

Maria Gini, Olga Zografou, Prodromos Fetfatzis, Konstantinos Granakis, Romanos Foskinis, Christos Mitsios, Carolina Molina, Aiden Jönsson, Paul Zieger, Mika Komppula, Alexandros Papayannis, Athanasios Nenes, and Konstantinos Eleftheriadis

Understanding aerosol properties and their life cycle in regional air masses is essential for assessing their impacts on clouds, precipitation and climate. High-altitude mountain stations, often emphasized as free-tropospheric measurement sites, are ideal for cloud and climate research. However, depending on the season and time of day, high-altitude sites may be influenced by planetary boundary layer (PBL) air masses due to convective transport. The segregation between PBL-influenced and free-tropospheric (FT) air masses remains a challenging but critical issue. Being able to unravel the periods for which clouds are influenced by each air type can vastly expands the scientific value and relevance of aerosol-cloud studies at mountain tops because cloud formation and their susceptibility to aerosol and dynamic perturbations vary considerably with each air mass type; the types of droplets and ice nucleators also can vary significantly, which further expands the scope and relevance of the measurements.

The Helmos Hellenic Atmospheric Aerosol and Climate Change ((HAC)²) station in Greece (2314 m a.s.l.) is the only high-altitude station in the eastern Mediterranean, a region highly sensitive to climate change. It is located at the crossroads of different air masses; the station is well-suited for aerosol-cloud interaction studies. To enhance understanding of the processes driving the formation and evolution of warm and mixed-phase clouds, the CALISHTO (Cloud-Aerosol InteractionS in the Helmos Background TropOsphere) and CHOPIN (Cleancloud Helmos OrograPhic sIte experiment) campaigns were conducted at Mount Helmos during the autumn-winter periods of 2021–2022 and 2024–2025, respectively. During these campaigns, in-situ and remote sensing measurements at a number of sites located at the Kalavrita Ski Center and the (HAC)2 were used to study the influence of the mixing layer (PBL), and their related aerosol and gases, at (HAC)². To achieve this, both in-situ and remote sensing instruments were employed. The permanent instrumentation of the (HAC)² station (e.g., GHGs, aerosol number size distributions, aerosol optical properties, meteorological data, and liquid water content) was supplemented with additional in-situ and remote sensing instruments operated at (HAC)² and the lower-altitude sites (about 1700 m a.s.l.). During the CHOPIN campaign, radiosonde measurements were conducted to measure critical atmospheric variables and provide further details about the structure of the atmospheric layers.

A set of aerosol and gaseous species and atmospheric metrics from in-situ measurements was established to indicate the presence of PBL air at the (HAC)² based on characteristic values of the water vapor mixing ratio, the accumulation mode (particles with a diameter greater than 95 nm) number concentration, and the ratio of eBC to CO. These thresholds were established by monitoring their values when the BL-FT boundary was at the (HAC)2 altitude, determined by remote sensing of atmospheric turbulence measurements. Application of these metrics to determine the presence (or not) of BL-influenced air agreed with the classification achieved by the remote sensing observations for up to 85 % of the time. Cloudy periods were studied separately from clear-sky periods owing to the substantially different gas and particle removal mechanisms occurring in each period.

How to cite: Gini, M., Zografou, O., Fetfatzis, P., Granakis, K., Foskinis, R., Mitsios, C., Molina, C., Jönsson, A., Zieger, P., Komppula, M., Papayannis, A., Nenes, A., and Eleftheriadis, K.: Evaluation of in-situ metrics for determining the influence of the Planetary Boundary Layer at the Helmos Hellenic Atmospheric Aerosol & Climate Change (HAC)2 station , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18522, https://doi.org/10.5194/egusphere-egu25-18522, 2025.

EGU25-19905 | Orals | AS3.22

Variability in hygroscopicity parameter, CCN number concentration and chemical composition of mineral dust-dominated air masses over the Mediterranean Sea 

Agnieszka Straus (Kupc), Maximilian Dollner, Manuel Schöberl, Adrian Walser, Sudharaj Aryasree, Konrad Kandler, Anne Tipka, Petra Seibert, and Bernadett Weinzierl

Airborne mineral dust particles, next to sea salt, are the most abundant aerosol type by mass globally (Andreae, 1995). Not only these particles affect the Earth’s radiation budget, but they also modify cloud properties by serving as cloud condensation nuclei (CCN), or ice nuclei. The composition of mineral dust aerosol (i.e. pure or processed) or its origin, however, may have a different effect on cloud formation processes, and cloud characteristics, influencing not only aerosol-cloud interactions, but also global climate (Karydis et al. 2011).

In this study, we investigate whether there are any differences in the particle hygroscopicity parameter κ in mineral dust-dominated air masses. We use in situ measurements of CCN number concentration (at water vapor supersaturation (SS) up to 0.14 %), number size distributions (0.005-50 μm in diameter), and particle chemical composition made on board of DLR Falcon research aircraft during the ERC-funded A-LIFE project in the Eastern Mediterranean in April 2017.

The classification of mineral dust-dominated air masses is based on aerosol chemical composition data from the scanning electron microscope coupled with energy-dispersive X-ray spectroscopy (SEM-EDX), with the particle projected area (circle equivalent diameter) between 0.2 and 3 μm. We examine the CCN properties of mineral dust-dominated air masses (i.e. pure and polluted dust aerosol), and in particular, show that the hygroscopicity parameter κ for SS of 0.1% varies between 0.01 and 0.2, and the corresponding particle activation diameters are found to be between 0.17 and 0.5 μm. The analysis supports our hypothesis that the hygroscopicity parameter κ increases with increasing pollution. We show the composition resolved κ and CCN concentration, as well as the particle volatility measurements, and compare these observations with other parameters measured during A-LIFE, as well as with results from the SALTRACE field campaign. Further, we identify the sources of mineral dust-dominated air masses using the Lagrangian transport and dispersion model FLEXPART.

How to cite: Straus (Kupc), A., Dollner, M., Schöberl, M., Walser, A., Aryasree, S., Kandler, K., Tipka, A., Seibert, P., and Weinzierl, B.: Variability in hygroscopicity parameter, CCN number concentration and chemical composition of mineral dust-dominated air masses over the Mediterranean Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19905, https://doi.org/10.5194/egusphere-egu25-19905, 2025.

While traditional thermal infrared retrieval algorithms based on radiative transfer models (RTM) could not effectively retrieve the cloud optical thickness of thick clouds, machine learning based algorithms were found to be able to provide reasonable estimations for both daytime and nighttime. Nevertheless, stand-alone machine learning algorithms are occasionally criticized for the lack of explicit physical processes. In this study, RTM simulations and a machine learning algorithm are synergistically utilized using the optimal estimation (OE) method to retrieve cloud properties from thermal infrared radiometry measured by Moderate Resolution Imaging Spectroradiometer (MODIS). In the new algorithm, retrievals from a machine learning algorithm are used to provide a priori states for the iterative process of OE method, and an RTM is used to create radiance lookup tables that are used in the iteration processes. Compared with stand-alone OE, the cloud properties retrieved by the new algorithm show an overall better performance by using statistic a priori information obtained by machine learning algorithm. Compared with stand-alone machine-learning based algorithm, the radiances simulated based on retrievals from the new method align more closely with observations, and physical radiative processes are handled explicitly in the new algorithm. Therefore, the new method combines the advantages of RTM-based cloud retrieval methods and machine-learning models. These findings highlight the potential for machine-learning-based algorithms to enhance the efficacy of conventional remote sensing techniques.

How to cite: Huang, H., Wang, Q., Liu, C., and Zhou, C.: Optimal estimation of cloud properties from thermal infrared observations with a combination of deep learning and radiative transfer simulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1161, https://doi.org/10.5194/egusphere-egu25-1161, 2025.

EGU25-1538 | Orals | AS3.23 | Highlight

Polarimetric Remote Sensing of atmospheric aerosols: The first year of SPEXone PACE 

Otto Hasekamp, Guangliang Fu, Raul Laasner, Bastiaan van Diedenhoven, Neranga Hannadige, Zihao Yuan, Laura van der Schaaf, Richard van Hees, Martijn Smit, and Jeroen Rietjens

On February 8, 2024 the NASA Plankton, Aerosol, Cloud & ocean Ecosystem (PACE) mission has been launched with onboard the SPEXone Multi-Angle Polarimeter. SPEXone is designed to deliver unprecedented information on aerosol properties, such as size, shape, absorption (Single Scattering Albedo), and amount (Aerosol Optical Depth, number concentration), and complex refractive index. From the complex refractive index, size and shape, chemical composition can be derived in terms of volume fractions of the main aerosol components. The launch of PACE brings an end to a 10 year gap in the availability of space-based multi-angle polarimeter data, which are essential to understand and quantify the role of aerosols and clouds in climate change. In this contribution, we present the first year of aerosol data from SPEXone. As we will show, the first version of SPEXone aerosol data shows already very good agreement with ground-based AERONET observations. The presentation includes a global view on aerosol composition in terms of volume fractions of Dust, Sea Salt, Black Carbon, Organic Carbon, fine mode inorganics (Sulphate, Nitrate), and aerosol water. SPEXone shows expected patterns of high fractions of sulphates/nitrates over industrial regions and cities in Asia and (North+South) America, Black Carbon over biomass burning regions in Africa and North America, Dust over desert regions and as outflow over the ocean, and hydrated sea salt over the open ocean.  Finally, we discuss the capability of SPEXone to provide a Cloud Condensation Nuclei (CCN) product from the retrieved aerosol properties (number concentration, size distribution, water content).

How to cite: Hasekamp, O., Fu, G., Laasner, R., van Diedenhoven, B., Hannadige, N., Yuan, Z., van der Schaaf, L., van Hees, R., Smit, M., and Rietjens, J.: Polarimetric Remote Sensing of atmospheric aerosols: The first year of SPEXone PACE, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1538, https://doi.org/10.5194/egusphere-egu25-1538, 2025.

EGU25-1551 | ECS | Posters on site | AS3.23

Multilayer Retrieval of Cloud Top heights from MODIS over the Southern Ocean  

Arathy A Kurup, Caroline Poulsen, and Steven T Siems

 The Southern Ocean (SO) is one of the cloudiest places on Earth, with  distinct cloud properties including a high prevalence of multilayer clouds. Previous research has found that multilayer clouds contribute to net cloud radiative effect biases. In our previous paper,we compared and validated different LEO passive sensor retrievals (AVHRR-Patmosx, CMSAF, MODIS collection 6) over the SO against active sensor retrievals (CloudSAT- CALIOP). In the comparison of cloud top height, we found that a mean absolute bias of 0.65 km (AVHRR CMSAF), 1.03 km (MODIS), and 1.31 km (AVHRR PATMOS) was observed for single-layer cloud scenes cases. This mean bias increased to 1.86 km (AVHRR CMSAF), 3.22 km (MODIS), and 3.34 km (AVHRR PATMOS) for multilayered cloud scenes. One of the significant factors for the observed differences is the presence of  multilayer clouds.  

Given the results of the comparison and a need for more accurate cloud retrieval for multi layer clouds in particular, we developed a new multilayer retrieval algorithm for CTH from MODIS data over the SO region using an artificial neural network (NN) approach. The retrieval algorithm employs MODIS radiances and reanalysis datasets. The algorithm's performance for the topmost cloud layer demonstrates a significant improvement compared to the traditional retrieval approaches.  The MODIS CTHs mean bias error against the CloudSAT- CALIOP merged dataset was reduced to approx 0.02 km with an RMSE of 0.84 km. In multilayer scenarios,the CTHs of the top layer were retrieved with a MBE of 0.08km and RMSE of 0.98 km and the CTHs of the second layer with a MBE of 0.01km and RMSE of 1.54 km. The results were analysed to understand the influence on latitude, solar zenith angle, sensor zenith angle, cloud optical depth and surface temperature on the ANN algorithm. The research successfully demonstrated the usefulness of NN in retrieval algorithms.

How to cite: A Kurup, A., Poulsen, C., and T Siems, S.: Multilayer Retrieval of Cloud Top heights from MODIS over the Southern Ocean , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1551, https://doi.org/10.5194/egusphere-egu25-1551, 2025.

EGU25-4196 | ECS | Posters on site | AS3.23

Identifying the Role of Clouds in the Recent Decrease in Top of the Atmosphere Reflectance Over Greenland 

Alexander Mchedlishvili, Marco Vountas, and Hartmut Bösch

In the period of Arctic Amplification, with surface temperatures at high northern latitudes rising faster than those at the mid-latitudes, the Arctic is undergoing significant changes. Among these changes are the retreat of sea ice and the melting of glaciers, processes that affect the spectral reflectance of solar radiation at the surface. By detecting subtle changes in reflectance at the top of the atmosphere (RTOA) as measured by the GOME-2 scanning spectrometer, we have identified significant negative trend (at 95% confidence) over the Greenland ice sheet (GrIS) for the period 2007-2024. We analyze the causes behind this RTOA drop through a combination of the AVHRR-based CLARA-A3 CM SAF’s Cloud, Radiation and Surface Albedo data record, ECMWF Reanalysis v5 (ERA5), and ground based measurements from Summit Station, Greenland. The primary focus of this combined spatiotemporal analysis is to better understand the impact of clouds on RTOA as well as on the surface conditions over the GrIS. Moreover, we aim to deduce how the atmospheric conditions over Greenland are responding to a warming Arctic climate system and what that means for GrIS in the years to come. At EGU25, we will present our most recent findings from our multi-dataset study and share our conclusions on the role of clouds in the observed drop in RTOA above Greenland.

This research is supported by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) within the Transregional Collaborative Research Center TRR 172 “ArctiC Amplification: Climate Relevant Atmospheric and SurfaCe Processes, and Feedback Mechanisms (AC)3.

How to cite: Mchedlishvili, A., Vountas, M., and Bösch, H.: Identifying the Role of Clouds in the Recent Decrease in Top of the Atmosphere Reflectance Over Greenland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4196, https://doi.org/10.5194/egusphere-egu25-4196, 2025.

EGU25-4701 | ECS | Posters on site | AS3.23

First Retrievals of Aerosol Optical Thickness and Surface Reflectance using EnMAP Radiance Data with the XBAER Algorithm 

Simon Laffoy, Marco Vountas, Linlu Mei, and Hartmut Bösch

We present work and results of the XBAER4EnMAP project, which focuses on the adaptation and further development of the mature eXtensible Bremen Aerosol/cloud and surfacE parameters Retrieval (XBAER) algorithm for the HyperSpectral Imager (HSI) instrument on board the Environmental Mapping and Analysis Program (EnMAP) satellite mission.

The XBAER algorithm retrieves aerosol optical thickness (AOT), surface reflectance (SRF) and cloud parameters and was previously developed using radiance data from both the MEdium Resolution Imaging Spectrometer (MERIS) onboard Envisat and the Ocean and Land Colour Instrument (OLCI) onboard Sentinel 3, both of which provide radiance data at a spatial resolution of 300m to 1.2km.

We aim to update XBAER to utilize EnMAP's higher spatial resolution radiance data of 30m, and to produce equivalent spatial-resolution data products with it. We present a comparison of OLCI and EnMAP top of atmosphere reflectances (RTOA) for co-located pixels, demonstrating that EnMAP is well calibrated enough for use in the XBAER algorithm. We then present results of comparison of XBAER-derived surface reflectance (SRF) and AOT using the same co-located pixels, i.e. at OLCI spatial resolution. Furthermore, we present first results of high-spatial resolution XBAER AOT, including a preliminary comparison with AErosol RObotic NETwork (AERONET).

Finally we discuss remaining challenges, such as updating XBAER's cloud mask and surface treatment for high spatial resolution data, and how to best compare AOT retrieved for the the small EnMAP scene size to AOT retrieved from point sites.

How to cite: Laffoy, S., Vountas, M., Mei, L., and Bösch, H.: First Retrievals of Aerosol Optical Thickness and Surface Reflectance using EnMAP Radiance Data with the XBAER Algorithm, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4701, https://doi.org/10.5194/egusphere-egu25-4701, 2025.

EGU25-5535 | ECS | Posters on site | AS3.23

Impact of aerosol load on solar radiation in the northeast China region 

Xuhui Gao, Yuliia Yukhymchuk, Gennadi Milinevsky, and Xiaopeng Sun

Northeast China is influenced by a diverse range of aerosol sources, including industrial emissions, biomass burning, dust storms, and the transport of mineral dust from the Gobi and Taklamakan deserts. These varying aerosol types interact with solar radiation through scattering and absorption processes. The AERONET sun-sky-lunar CE318-T photometer was recently installed in Changchun in October 2024 to study and monitor aerosol characteristics in this region. This installation marks the beginning of systematic and accurate measurements of aerosol properties in the area, providing a valuable dataset for understanding aerosol behavior. Given the complex interactions between aerosol particles and solar radiation, it is essential to know how different aerosol types influence radiation patterns. For this study, AERONET measurements were compared with data obtained from the set of instruments installed at the SOLYS2 sun tracker. The SOLYS2 is equipped with pyranometers, pyrgeometer, pyrheliometer, and shading ball assembly. This set of sensors captures radiation from the entire hemisphere, including both direct and diffuse radiation from the sun and sky. It allows the measurement of global horizontal irradiance, direct normal irradiance, and diffuse normal irradiance to be provided, enabling a comprehensive analysis of aerosol-radiation interactions in the region. In this work, we investigate how varying aerosol loading impacts solar radiation in this region, focusing on the influence on radiation patterns and overall atmospheric conditions.

How to cite: Gao, X., Yukhymchuk, Y., Milinevsky, G., and Sun, X.: Impact of aerosol load on solar radiation in the northeast China region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5535, https://doi.org/10.5194/egusphere-egu25-5535, 2025.

Aerosol-Cloud Interactions (ACIs) remain a major uncertainty in climate predictions. While satellites provide valuable climatology to constrain ACIs and estimate their radiative forcing (e.g., Twomey effect), discrepancies among studies and measurement limitations persist. Passive sensors like the MODerate resolution Imaging Spectroradiometer (MODIS) cannot simultaneously retrieve aerosol and cloud properties, and biases arise when absorbing aerosols above clouds (AACs) affect cloud retrievals. Such biases are particularly evident during extreme events like wildfires, dust storms, or volcanic eruptions, where AACs distort measurements of Cloud Effective Radius (CER) and Cloud Optical Thickness (COT) (e.g., Haywood et al., 2004; Alfaros and Contreras, 2013; Constantino and Bréon, 2010-2013).

 

Hitherto, existing AAC studies focus on biomass burning aerosols (BBAs) over the Southeast Atlantic, limiting their scope.

Then, the objective of this work is to globalize the AAC study to several types of absorbing aerosols all over the world.  To do so, we created a new database combining aerosols and clouds properties as well as new aerosols products based on specific aerosol-cloud scenarios. We used L3 and L2 data from TROPOMI (on board the Sentinel-5P satellite) and MODIS respectively, as well as reanalysis from CAMS: ERA5 and EAC4. We covered the period from 2019 to 2023, containing noticeable events such as the Australian and Californian Wildfires (2019/2020) or regular Saharan dust storms.

In a second time, we conducted statistical analyses on COT, CER and Cloud Droplets Number Concentration (Nd), over specific regions where Nd retrievals are reliable (McCoy, 2017). The primarily results show strong responses to AAC on cloud properties during strong events. The indirect aerosol effect is not as visible as expected, but still, this work is encouraging. The next objective is to combine satellite observations with Radiative Transfer simulations (on RTTOV) to reproduce the AAC scenes and confirm our observations and better quantify the AAC biases on cloud properties as well as ACIs more generally.

How to cite: Devigne, E., Sourdeval, O., and Waquet, F.: Disentangle Aerosol-Cloud-Interactions (ACIs) using a new Aerosol-Cloud Data Base from Passive Remote Sensors and Reanalysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5636, https://doi.org/10.5194/egusphere-egu25-5636, 2025.

EGU25-5963 | Posters on site | AS3.23

Weather Radar Long-sequence Product Dataset in China 

Lei Wu

Weather radar plays a crucial role in the monitoring, forecasting, and early warning of severe convective weather. With the widespread application of artificial intelligence technology in the meteorological field, the demand for high-quality, long-sequence weather radar product is becoming increasingly urgent. To support the development of domestic independent severe convective weather models, enhance the identification and monitoring technology for severe convective weather, and promote in-depth research in numerical forecasting and mechanisms, the Meteorological Observation Center of China Meteorological Administration has applied techniques such as feature analysis and recognition, multi-source data collaborative quality control, inspection evaluation, and diagnostic error correction. Through a hierarchical processing approach involving single-station quality control, network quality control, and inspection evaluation, coarse data errors are eliminated. This process has resulted in the formation of a long-sequence, high-quality, and high spatiotemporal resolution weather radar basic product dataset (V1.0) covering the years from 2011 to 2023. This dataset incorporates post-quality control base data from nationwide weather radars, along with four types of two-dimensional mosaic products: composite reflectivity, hybrid scan reflectivity, echo top height, and vertically integrated liquid water content, as well as three-dimensional mosaic products of constant altitude plan position indicator (CAPPI). The post-quality control base data amounts to roughly 200TB, encompassing data from 247 stations with a temporal resolution of approximately 6 minutes. The two-dimensional mosaic product data totals approximately 1.2TB, featuring a temporal resolution of 6 minutes. These two-dimensional mosaic products cover a horizontal spatial range from 73.0° to 135.0°E and from 12.2° to 53.2°N, with a spatial resolution of 0.01° × 0.01°. The three-dimensional mosaic product data totals approximately 27.5TB, sharing the same temporal and horizontal resolution as the two-dimensional mosaic product data. In terms of vertical spatial coverage, it spans from 0.5 km to 16 km, consisting of 24 layers. The vertical resolution is 0.5 km for altitudes up to 8 km and 1 km for altitudes above 8 km. Currently, this dataset has played a crucial role in severe convective weather model training and the development of reanalysis data in the Chinese region.

How to cite: Wu, L.: Weather Radar Long-sequence Product Dataset in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5963, https://doi.org/10.5194/egusphere-egu25-5963, 2025.

EGU25-6443 | ECS | Posters on site | AS3.23

Retrieval and validation of aerosol and surface properties from HARP2/PACE using GRASP algorithm  

Chong Li, Oleg Dubovik, Anin Puthukkudy, Pavel Lytvynov, Anton Lopatin, David Fuertes, Alejandro García Gómez, and Juan Carlos Antuña Sánchez

NASA's Plankton, Aerosol, Clouds, and ocean Ecosystem (PACE) mission was successfully launched on February 8, 2024. A key instrument aboard the PACE platform- the Hyper-angular Rainbow Polarimeter-2 (HARP2), a state-of-the-art multi-angular polarimeter, collects data from multiple viewing angles spanning -54.5° to +54.5° across 4 channels ranging from visible to near-infrared wavelengths, with measurements of linear polarization at three directions. Thus, HARP2 has very high sensitivity to aerosol characteristics, including particle size, type, and absorption etc.

In this study, the Generalized Retrieval of Aerosol and Surface Properties (GRASP) algorithm was utilized to retrieve aerosol and surface parameters simultaneously from HARP2 measurements collected over the past half year. Validation of aerosol properties was conducted by comparing HARP2/GRASP products with ground-based AERONET observations, while surface property retrievals were evaluated against MODIS surface products. The results have demonstrated encouraging performance: spectral AOD shows a high correlation with AERONET data with correlation coefficients ~0.9and a mean bias of -0.01. The Ångström Exponent (AE) and single scattering albedo (SSA), also showed reasonable agreement, with AE and SSA achieving correlation coefficients of 0.54 and 0.9. Surface property retrievals exhibited robust correlations with MODIS data, demonstrating the effective decoupling of surface and atmospheric signals from the satellite observations.

This research highlights the potential of HARP2/GRASP products in providing accurate aerosol and surface parameters, leveraging HARP2’s polarimetric capabilities. In the future, we will also explore the synergistic potential of integrating observations from multiple PACE instruments to enhance the information content and improve retrieval coverage and accuracy

How to cite: Li, C., Dubovik, O., Puthukkudy, A., Lytvynov, P., Lopatin, A., Fuertes, D., García Gómez, A., and Antuña Sánchez, J. C.: Retrieval and validation of aerosol and surface properties from HARP2/PACE using GRASP algorithm , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6443, https://doi.org/10.5194/egusphere-egu25-6443, 2025.

EGU25-8784 | ECS | Posters on site | AS3.23

Cloudy Planet: Cirrus Detection with MODIS Data 

Żaneta Nguyen Huu, Andrzej Z. Kotarba, and Agnieszka Wypych

Clouds influence Earth's radiative budget, with high-level clouds playing a critical role in atmospheric warming. Accurate cirrus cloud characterization is crucial and can be achieved using different data sources. Active satellite sensors are presently the most accurate source for cirrus data, but their usefulness in climatological studies is limited. In contrast, passive data, available for the past 40 years, offers sufficient temporal resolution but struggles to detect cirrus clouds effectively. This study evaluates MODIS cloud masking algorithms for cirrus detection, comparing their performance to CALIOP data. Specifically, we aim to assess whether MODIS cloud detection tests used to generate MYD35 operational data can be re-used for masking of cirrus.

Using CALIOP data as the reference, we evaluated six tests for cirrus detection considered in MODIS cloud masking algorithm and their combination (ATC). Additionally we applied two ISCCP-originating tests: ISCCP3.6 and ISCCP23 tests.

Our results showed that the ATC method outperforms others, with 72.98% accuracy during the day and 59.50% at night (probability of detection: 80.87% and 25.46%, false alarm rate of 34.86% and 6.90%, and Cohen’s kappa coefficient of 0.46 and 0.19 respectively). The ATC test offers a reliable option for creating high-level cloud masks.

How to cite: Nguyen Huu, Ż., Kotarba, A. Z., and Wypych, A.: Cloudy Planet: Cirrus Detection with MODIS Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8784, https://doi.org/10.5194/egusphere-egu25-8784, 2025.

EGU25-10514 | Posters on site | AS3.23

Estimation of Cloud Condensation Nuclei (CCN) from SPEXone on PACE using a deep neural network retrieval algorithm  

Neranga K. Hannadige, Guangliang Fu, Bastiaan van Diedenhoven, Hailing Jia, and Otto Hasekamp

Proper proxies for CCN are vital to provide accurate constraints for Aerosol-Cloud Interactions (ACI) in climate models. An effective proxy for CCN is the column number of aerosol particles that surpasses a predetermined threshold radius (Nccn). This CCN proxy has been estimated from PARASOL using level 2 aerosol microphysical and/or optical property retrievals. With the launch of SPEXone on Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) satellite, further improvements on the Nccn retrievals are expected. For example, retrieved refractive index can be used to estimate the volume fraction of aerosol-water, which can help deduce the dry aerosol size distibution and subsequently dry CCN. Further, the retrieved Aerosol-Layer Height (ALH) can be used to estimate the boundary layer (BL) contribution of Nccn (Nccn (BL)) which is better suited for quantifying ACI as it is more related to CCN at cloud base than the total column.

The estimation of Nccn from physics based MAP algorithms can be challenging given its dependance on multiple retrieved aerosol parameters. We have implemented a deep neural network (NN) algorithm as an extension for the Remote sensing of Trace gas and Aerosol Products (RemoTAP)-NN algorithm to directly retrieve dry Nccn and Nccn (BL) from SPEXone measurements. The algorithm is trained on synthetic SPEXone measurements based on 3 aerosol modes which are fine mode, insoluble coarse/dust mode and soluble coarse mode. It has been validated using synthetic SPEXone measurements, simulated based on the 7 mode aerosol model from the ECHAM-HAM global aerosol-climate model. The performance of the NN algorithm was compared with RemoTAP classical algorithm.

The NN algorithm retrieved dry Nccn has a relative RMSE of 0.197 over the ocean and 0.301 over the land whereas dry Nccn estimated by RemoTAP level-2 retrievals for the same synthetic measurements has a relative RMSE of 0.382 over ocean and 0.559 over land. Nccn (BL) retrieved from the NN algorithm has a relative RMSE of 0.349 and 0.825 over the ocean and the land respectivey. The relative RMSE of Nccn (BL) derived from the RemoTAP classical algorithm is 1.039 and 1.233 over the ocean and land respectively. Our study demonstrates that the NN algorithm can accurately retrieve Nccn, outperforming the capabilities in classical algorithms.

How to cite: K. Hannadige, N., Fu, G., van Diedenhoven, B., Jia, H., and Hasekamp, O.: Estimation of Cloud Condensation Nuclei (CCN) from SPEXone on PACE using a deep neural network retrieval algorithm , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10514, https://doi.org/10.5194/egusphere-egu25-10514, 2025.

EGU25-11285 | Posters on site | AS3.23

Estimation of Global PM2.5 from Polarimetric Remote Sensing (POLDER-3/GRASP) and CAMS Reanalysis Data 

Zhen Liu, Anton Lopatin, Abhinna Behera, Milagros Herrera, Konstantin Kuznetsov, Masahiro Momoi, Marcos Giralda, Christian Matar, Siyao Zhai, Pavel Lytvynov, David Fuertes, Tatyana Lapyonok, Yevgeny Derimian, and Oleg Dubovik

Ambient fine particulate matter (PM2.5, mean aerodynamic radii less than 2.5µm) is a leading cause of millions of premature deaths annually, linked to lung cancer, pulmonary inflammation, and cardiopulmonary mortality. Therefore, accurate global measurements of PM2.5 are essential for epidemiological studies, designing air quality control strategies, and improving air quality forecasting.

The POLDER-3/GRASP multi-angular polarimetric products enable advanced retrievals of aerosol properties, such as size distribution, refractive index, particle composition, and aerosol layer height (ALH), facilitating the estimation of ground-level PM2.5. However, POLDER has limited sensitivity to ALH and relies on assumed aerosol vertical profiles, which may introduce uncertainties that propagate into PM2.5 estimations. Complementarily, the CAMS reanalysis data provides global coverage with high temporal resolution, offering detailed information on tropospheric aerosol distributions and vertical structures.

In this study, we first validate global ground-level PM2.5 estimations from POLDER/GRASP products using detailed columnar aerosol properties, such as size distribution, refractive index or chemical composition and ALH, against observational data from the US Environmental Protection Agency (EPA). Next, CAMS reanalysis aerosol products are integrated into the POLDER-3/GRASP framework to enhance the estimation accuracy. This integration combines columnar aerosol properties retrieved from POLDER/GRASP at higher spatial resolution with detailed vertical profiles from CAMS, notably ground-level aerosol fractions. Finally, we analyze the improvements achieved by comparing the integrated results with US EPA ground-based measurements. This synergistic approach investigates the potential of combining POLDER/GRASP retrievals with CAMS comprehensive vertical aerosol structures to improve global air quality assessments, paving the way for advanced monitoring capabilities from future multi-angular polarimeter missions, such as PACE/SPEX, PACE/HARPOL-2, and 3MI.

How to cite: Liu, Z., Lopatin, A., Behera, A., Herrera, M., Kuznetsov, K., Momoi, M., Giralda, M., Matar, C., Zhai, S., Lytvynov, P., Fuertes, D., Lapyonok, T., Derimian, Y., and Dubovik, O.: Estimation of Global PM2.5 from Polarimetric Remote Sensing (POLDER-3/GRASP) and CAMS Reanalysis Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11285, https://doi.org/10.5194/egusphere-egu25-11285, 2025.

EGU25-11912 | Orals | AS3.23

C3IEL, the Cluster for Cloud evolution ClImatE and Lightning Mission to Study Convective Clouds at High Spatial and Temporal Resolution 

Céline Cornet, Daniel Rosenfeld, Eric Defer, Vadim Holodovsky, Guillaume Penide, Raphaël Peroni, Colin Price, Didier Ricard, Antoine Rimboud, Yoav Schechner, Yoav Yair, Cécile Cheymol, Adrien Deschamps, Alex Frid, Laurène Gillot, Avner Kader, and Shmaryahu Aviad

The space-borne C3IEL (Cluster for Cloud evolution, ClImate and Lightning) mission, jointly developed jointly by the French and the Israeli space agency, aims at providing new insights on convective clouds, at high spatial and temporal resolutions, close to the scales of the individual convective eddies. The mission will simultaneously characterize the convective cloud dynamics, the interactions of clouds with the surrounding water vapor, and the lightning activity.

The C3IEL mission consists in a short-baseline (~150 km) train of 2 synchronized small satellites. Each satellite carries a visible camera (670 nm) for cloud imagery at a spatial resolution of ~20 meters, near-infrared water vapor imagers (1.04, 1.13 et 1.37 µm ; ~125 m at nadir) measuring in and near the water vapor absorption bands, a lightning imager (777.4 nm ; ~140 m at nadir) and at two photometers (337 and 777.4 nm).

The scientific objectives of the C3IEL mission will be first reminded. They consist in documenting the convective cloud development through their 3D evolution and their environment with the retrieval of water vapor surroundings the clouds and the use of other observations such as geostationary satellite to characterize aerosol properties. In addition, the lightning activities created by such clouds will be observed. We will introduce the satellite train configuration, the different sensors of the mission and the innovative and different observational strategy that will be applied during daytime and nighttime. We will then detail the expected observations and products. Finally we will discuss the current status of the mission and the way forward.

How to cite: Cornet, C., Rosenfeld, D., Defer, E., Holodovsky, V., Penide, G., Peroni, R., Price, C., Ricard, D., Rimboud, A., Schechner, Y., Yair, Y., Cheymol, C., Deschamps, A., Frid, A., Gillot, L., Kader, A., and Aviad, S.: C3IEL, the Cluster for Cloud evolution ClImatE and Lightning Mission to Study Convective Clouds at High Spatial and Temporal Resolution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11912, https://doi.org/10.5194/egusphere-egu25-11912, 2025.

EGU25-12956 | Posters on site | AS3.23

Optical properties of smoke particles: modeling and interpretation 

Liudmyla Berdina, Victor Tishkovets, Pavel Lytvynov, Oleg Dubovik, Tatyana Lapyonok, Qiaoyun Hu, and Philippe Goloub

Atmospheric aerosols of both natural and anthropogenic origin have a significant impact on the Earth's climate and on human health by degrading air quality. To study the influence of aerosols on climate and to monitor air pollution, it is important to know the characteristics of aerosol particles. In the case of smoke particles, their microphysical, chemical and optical properties are complex and strongly depend on the combustion sources, the aging process and the meteorological conditions.

This study is devoted to the analysis of optical properties of the particles that can be adopted as a model of smoke particles. The main attention has been paid to the analysis of the spectral dependence of the backscattering linear depolarization ratio (LDR), in particular, the strong wavelength dependence of the LDR, that is observed for some biomass burning events in lidar measurements. Among other light scattering models of smoke particles that can describe such spectral dependence and reproduce the optical properties of smoke particles, the most realistic model in the form of fractal-like clusters of carbonaceous spherules (monomers) was selected. The analysis was carried out on the basis of the created database of optical characteristics of fractal-like clusters calculated for a certain set of cluster parameters differing in their structure, size and morphological characteristics of individual monomers. Our results show that the LDR is a complex function of various factors such as particle size and shape, refractive index, fraction and composition of the core and monomer coating material, etc., and for a certain choice of morphological characteristics, a fractal-like model can reproduce the observed spectral dependence of the LDR. In the framework of such a model, the values of the LDR measured by lidars can be used to estimate the monomer size of the cluster particles, more precisely, the product of the monomer size and the real part of the refractive index of the monomer.

The integration of fractal aggregate morphology into aerosol models can improve the retrieval accuracy of microphysical and chemical properties of smoke particles. And combined analysis of Sun photometer and lidar measurements can provide complementary information for clarifying morphological characteristics of the monomers, such as size, refractive index, and cluster structure and size distribution.

How to cite: Berdina, L., Tishkovets, V., Lytvynov, P., Dubovik, O., Lapyonok, T., Hu, Q., and Goloub, P.: Optical properties of smoke particles: modeling and interpretation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12956, https://doi.org/10.5194/egusphere-egu25-12956, 2025.

EGU25-13530 | ECS | Posters on site | AS3.23

Statistics of Optical and Microphysical Properties of Ice and Mixed-Phase Clouds on the Antarctic Plateau 

Elisa Fabbri, Tiziano Maestri, Federico Donat, Michele Martinazzo, Guido Masiello, Giuliano Liuzzi, Luca Palchetti, Gianluca Di Natale, Massimo Del Guasta, and Giovanni Bianchini

The uncertainties in the cloud radiative properties are the main cause of biases in the radiative fluxes both at the top of the atmosphere and at the surface (Di Natale et al. 2022). This study aims at providing an in-depth characterisation of clouds occurrence and properties on the Antarctic Plateau by analyzing an extensive dataset of spectrally resolved downwelling radiances in the far- and mid-infrared region of the spectrum (200 − 1000 cm-1). Observations were performed by the REFIR-PAD (Radiation Explorer in the Far Infrared—Prototype for Applications and Development) spectroradiometer at the Concordia research station on the Antarctic Plateau, during the period from 2013 to 2020. An improved version of the Cloud Identification and Classification (CIC) algorithm (Maestri et al. 2019; Donat et al. 2024) is utilized for the identification of cloud layers and their classification in terms of phase (ice or mixed phase). An extended dataset, comprising about 75000 cloudy spectra, is then analysed to derive geometrical, optical, and microphysical properties of the observed layers. First, the Polar Threshold (PT) algorithm (Van Tricht et al. 2014) is applied to collocated Lidar backscatter profiles obtained from a Lidar system (INO-CNR Istituto Nazionale di Ottica 2024) to derive cloud base and top altitude. Then, the geometrical information is exploited by the Simultaneous Atmospheric and Cloud Retrieval (SACR) physical inversion algorithm (Di Natale et al. 2020), which, applied to the REFIR-PAD radiances, enables the derivation of cloud optical depth, effective dimensions, and atmospheric vertical profiles of water vapor and temperature. Statistics of clouds optical and microphysical properties for different cloud types are derived. Results show that the mean optical depth and effective diameter of ice clouds are 0.58 and 25 μm, respectively. It is found that 90% of the data indicate effective diameters smaller than 52 μm. During the austral summer, both optical depth (0.34) and effective diameter (19 μm) are at their lowest values, while maxima are found in the winter season (0.73 for optical depth and 30 μm for effective diameter). The ice clouds mean temperature is 236 K, with a seasonal cycle showing the highest temperatures in summer. Mixed-phase clouds exhibit a significantly higher mean optical depth of 2.35. Their averaged effective diameter is 8.55 μm, and the mean cloud temperature is 244 K. The base height of mixed-phase clouds is found at mean value of 0.29 km above ground level (agl) which is significantly lower than the one for ice clouds found at 0.62 km agl. Finally, a new parametrization of cloud microphysical properties based on the thermodynamic conditions of the layer is proposed for potential applications in climate and numerical weather prediction models. The effective diameter of ice crystals is parameterized as a function of the mean cloud temperature and ice water content, whereas the effective diameter of water droplets for mixed-phase clouds is expressed as a univariate function of the mean cloud temperature. A comparison with parametrizations widely used in climate and numerical weather prediction models is also provided.

How to cite: Fabbri, E., Maestri, T., Donat, F., Martinazzo, M., Masiello, G., Liuzzi, G., Palchetti, L., Di Natale, G., Del Guasta, M., and Bianchini, G.: Statistics of Optical and Microphysical Properties of Ice and Mixed-Phase Clouds on the Antarctic Plateau, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13530, https://doi.org/10.5194/egusphere-egu25-13530, 2025.

EGU25-14162 | ECS | Posters on site | AS3.23

Sensitivity and Identification of Cloud Phases in the Solar Spectrum Using Dual-View Satellite Observations 

Kameswara Sarma Vinjamuri, Marco Vountas, Vladimir Rozanov, Luca Lelli, John P. Burrows, and Hartmut Bösch

The cloud phase is expected to change in the warming world. Knowledge of the cloud phase is an initial and essential step in retrieving cloud optical parameters. Cloud optical parameters are generally retrieved by single-viewing remote sensing spectrometers. Identifying mixed-phase clouds (MPC), pure ice and liquid clouds simultaneously for cloud retrievals remains a research challenge. This study addresses this issue and uses the SCIATRAN radiative transfer model (RTM) to understand the sensitivities of the cloud phases and their varying optical and microphysical properties in the solar radiation spectrum in nadir and near-nadir viewing geometries. We use the dual-view measurements of the Surface Land and Sea Temperature Radiometer (SLSTR) to determine cloud phases. For the MPC, we introduce the parameter Ice Fraction (IF), defined as the fraction of the total extinction of solar radiation attributed to ice. To classify the cloud phases,  we use two indices: a) the  NIR  ratio of  1.64 µm to 2.25 µm backscattered intensities at the top of the atmosphere, which is sensitive to spectral absorption in the cloud,  and b) the dual-view ratio, using nadir and near-nadir intensities at 0.87 µm, which exploits the angular scattering variation of clouds. These indices form the NIR-dual view ratio (multiplication of the NIR and the dual-view ratio), enhance discrimination across the cloud phases, and especially allow MPC identification over ocean and snow surfaces. This ratio typically ranges from less than 2.75 for ice clouds and more than 3.50 for water clouds. The values in between attribute to the presence of MPC, except for MPC, having an ice contribution of > 80%. The NIR-dual view ratio is similar to water clouds for lower IF (e.g., IF < 20%). To test theoretical RTM results, we validated the NIR-dual view ratio calculated from SLSTR onboard Sentinel-3A and comparing with the CloudSat product  (2B-CLDCLASS-LIDAR).  Results demonstrate that our approach identifies all three cloud phases with more than 80% accuracy. This research highlights the potential of dual-view satellite observations to improve cloud phase classification, advancing the capabilities of cloud retrieval algorithms.

How to cite: Vinjamuri, K. S., Vountas, M., Rozanov, V., Lelli, L., Burrows, J. P., and Bösch, H.: Sensitivity and Identification of Cloud Phases in the Solar Spectrum Using Dual-View Satellite Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14162, https://doi.org/10.5194/egusphere-egu25-14162, 2025.

EGU25-14419 | ECS | Orals | AS3.23

Synergetic retrieval of aerosol and surface properties from cross-track polarimetric scanner POSP onboard GF-5(02) and DQ-1 satellites 

Cheng Chen, Xuefeng Lei, Zhenhai Liu, Pavel Litvinov, Siyao Zhai, Oleg Dubovik, Yujia Cao, Haixiao Yu, Ke Xiao, Yan Wang, Zhengqiang Li, and Jin Hong

The Particulate Observing Scanning Polarimeter (POSP) is a cross-track multispectral polarimetric scanning imager onboard both GaoFen-5(02) and DQ-1 satellites. POSP has a field of view +/- 50 degree with a nadir resolution of ~6.4 km and a swath of ~1850 km, and it measures the stokes vector (I, Q, U) at nine spectral bands from UV to SWIR, specifically 380, 410, 442, 490, 670, 865, 1610, and 2250 nm. Previous study has shown the UV-VIS-NIR-SWIR single-view polarimetric measurements from POSP/GF-5(02) could provide reliable information content for aerosol and surface characterization. In this study, we will describe the synergetic utilization of POSP measurements from GF-5(02) morning and DQ-1 afternoon satellites in order to enhance the capability to retrieve aerosol and surface properties. 

How to cite: Chen, C., Lei, X., Liu, Z., Litvinov, P., Zhai, S., Dubovik, O., Cao, Y., Yu, H., Xiao, K., Wang, Y., Li, Z., and Hong, J.: Synergetic retrieval of aerosol and surface properties from cross-track polarimetric scanner POSP onboard GF-5(02) and DQ-1 satellites, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14419, https://doi.org/10.5194/egusphere-egu25-14419, 2025.

EGU25-14494 | ECS | Orals | AS3.23

Advanced Aerosol Retrievals with RemoTAP and PARASOL: Enhancing Understanding of Aerosol-Cloud Interactions 

Piyushkumar N Patel, Bastiaan van Diedenhoven, Otto Hasekamp, and Guangliang Fu

The precise retrieval of aerosol properties from satellite data is pivotal for advancing our understanding of their impacts on climate and air quality. The RemoTAP (Remote Sensing of Trace Gas and Aerosol Products) algorithm represents a significant leap forward, leveraging data from multi-angle polarimeters (MAPs), such as the past PARASOL-POLDER instrument, the current PACE-SPEXone and the future Metop-SG-3MI and CO2M-MAP instruments. A unique ability of these instruments to measure both the intensity and polarization of sunlight across multiple wavelengths and viewing angles offers an unparalleled dataset for aerosol characterization, including number concentrations, size distributions, and refractive indices. We have substantially enhanced the RemoTAP results by integrating improved cloud fraction values derived from MAPs using a neural network approach, ensuring more accurate aerosol retrievals through better cloud filtering techniques. To further elevate data quality, advanced quality filters utilizing multiple key metrics were developed, effectively enhancing data integrity, resulting in a more refined aerosol dataset essential for precise atmospheric analysis. The validation of these enhancements involved comparisons with ground-based AERONET (Aerosol Robotic Network) observations over 284 sites, demonstrating the reliability of RemoTAP-derived aerosol properties. Furthermore, a pixel-level cross-comparison was carried out with GRASP-derived PARASOL-based aerosol data, as RemoTAP and GRASP are similar kind of algorithms for polarimetric measurements. The scientific implications of these advancements are profound, as the improved retrieval of aerosol size and composition using advanced polarimetric observations directly refines the estimation of cloud condensation nuclei (CCN) (proxy) concentrations and consequently the global CCN-Nd (cloud droplet number concentration) relationship. This refined relationship is crucial for understanding aerosol-cloud interactions, allowing for more accurate quantification of aerosol-induced cloud albedo changes, thereby reducing uncertainties in radiative forcing estimates due to aerosol-cloud interactions (RFaci). Such improvements contribute to a more precise representation of aerosol impacts in climate models, ultimately enhancing predictions of climate sensitivity and future warming scenarios. By advancing the RemoTAP algorithm, our findings underscore the transformative potential of these methodologies in delivering accurate and reliable aerosol climatology, driving forward the frontier of atmospheric science and climate research.

How to cite: N Patel, P., van Diedenhoven, B., Hasekamp, O., and Fu, G.: Advanced Aerosol Retrievals with RemoTAP and PARASOL: Enhancing Understanding of Aerosol-Cloud Interactions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14494, https://doi.org/10.5194/egusphere-egu25-14494, 2025.

EGU25-14820 | Orals | AS3.23

Aerosol Modelling & Lessons Learned from GRASP Aerosol Remote Sensing 

Oleg Dubovik, Pavel Litvinov, Tatyana Lapyonok, Benjamin Torres, Anton Lopatin, David Fuertes, Yevgeny Derimian, Cheng Chen, Lei Li, Philippe Lesueur, Masahiro Momoi, Wushao Lin, Alexander Sinyuk, and Elena Lind

The presentation discusses the approaches to model aerosol properties realized in  GRASP (Generalized Retrieval of Aerosol and Surface Properties)  algorithm (Dubovik et al., 2021). GRASP algorithm  is developed based heritage of earlier efforts on the AERONET retrieval development (Dubovik and King, 2000, Dubovik et al., 2000)  with idea to use the same algorithm for different applications. Thus, at present, GRASP is a versatile algorithm that could be applied diverse observations including laboratory, passive and active remote sensing measurements from ground and space. All those observations have different sensitivities to details of aerosol properties and, therefore, analysis of each type of observations requires adequate approach to model aerosol properties. For example, aerosol model used for interpretation of  AERONET observations includes many more paraments than aerosol model used for interpretation of satellite observations from single view satellite imager such a MODIS or OLCI. At the same time, the aerosol models used for different observations should be consistent and compatible. Following this concept,  GRASP aerosol forward model can be adequately adjusted for applications to very different observations ranging from in situ nephelometers, ground-based AERONET radiometers to satellite polarimetric and radiometric imagers, as well as, to ground-based and satellite lidar observations. The  aerosol model   describes all aerosol properties: size distribution, complex index of refraction, or composition,  particle shape, rules of for several component mixing, vertical profile description, etc.  The presentation overviews historical evolution of all details of aerosol model, the assumptions made for adaptation to different observations of different types of and  the rational used for the current  specific design od aerosol model. Finaly, the comparative analysis will be done to outline the differences and agreements with other  common approaches used in aerosol remote sensing.  

Dubovik, O., A. Smirnov, B. N. Holben, etc., “Accuracy assessments of aerosol optical properties retrieved from AERONET Sun and sky-radiance measurements”, J. Geophys. Res.,105, 9791-9806, https://doi.org/10.1029/2000JD900040, 2000.

Dubovik, O. and M. D. King, “A flexible inversion algorithm for retrieval of aerosol optical properties from Sun and sky radiance measurements”, J. Geophys. Res., 105, 20,673-20,696, https://doi.org/10.1029/2000JD900282, 2000.

Dubovik, O., D. Fuertes, P. Litvinov, et al. , “A Comprehensive Description of Multi-Term LSM for Applying Multiple a Priori Constraints in Problems of Atmospheric Remote Sensing: GRASP Algorithm, Concept, and Applications”, Front. Remote Sens. 2:706851. doi: 10.3389/frsen.2021.706851, 2021.

 

How to cite: Dubovik, O., Litvinov, P., Lapyonok, T., Torres, B., Lopatin, A., Fuertes, D., Derimian, Y., Chen, C., Li, L., Lesueur, P., Momoi, M., Lin, W., Sinyuk, A., and Lind, E.: Aerosol Modelling & Lessons Learned from GRASP Aerosol Remote Sensing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14820, https://doi.org/10.5194/egusphere-egu25-14820, 2025.

Marine aerosols are crucial for ocean-atmosphere interactions. However, there is a lack of analysis on the long-term aerosol optical characteristics and relative humidity (RH) based on large-scale ocean regions. This paper addresses this issue by analyzing the spatiotemporal variations of aerosols in China's offshore waters from 2007-2022 using Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) and European Centre of Medium-range Weather Forecasts Reanalysis v.5 (ERA5) data. The results show that in the sea area, the aerosol backscatter coefficient at 532nm and extinction coefficient at 532nm increase with increasing RH; the aerosol depolarization ratio decreases with increasing RH. The optical properties of aerosols are generally lower in summer, while they fluctuate with rising RH in other seasons. Notably, the values recorded in 2014-2019 were markedly lower than those in 2007-2013. Nevertheless, from 2020 to 2022, the proportion of aerosol types remained largely stable compared to 2014-2019, suggesting a negligible impact of the COVID-19 pandemic on emissions, but the near-shore waters' aerosol optical properties were more sensitive to minor changes than those of far-off waters. After dividing the China's offshore waters, the overall optical properties of aerosols decreased in order of the Bohai Sea and Yellow Sea, the East China Sea, and the South China Sea, due to the proportion of marine aerosols increase towards the south. After dividing the altitude layer in the sea area, within the range of 0-7 km, the higher the altitude, the less oceanic aerosols and the more terrestrial aerosols. The aerosol depolarization ratio rises, while the aerosol backscatter coefficient at 532nm and extinction coefficient at 532nm alternate downwards. We speculate this is linked to the steep decline in total aerosol content as altitude rises. Our results could provide theoretical references for further deepening the understanding of aerosol generation mechanisms in China's offshore waters.

How to cite: He, J., Li, Z., and Jiang, W.: Long-term spatiotemporal features of aerosol optical characteristics and relative humidity in China's offshore areas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15328, https://doi.org/10.5194/egusphere-egu25-15328, 2025.

EGU25-16774 | ECS | Posters on site | AS3.23

Analysis of Cloud Types and their Geometrical Properties over the Mediterranean using CloudSat Observations 

Iliana Koutsoupi, Eleni Marinou, Kalliopi Artemis Voudouri, Ioanna Tsikoudi, Peristera Paschou, Vassilis Amiridis, Alessandro Battaglia, Pavlos Kollias, and Eleni Giannakaki

Earth's climate system and weather are affected by clouds, as they regulate the global radiative budget, depending on their altitude, structure and composition. Therefore, accurate cloud information is crucial, particularly above the Mediterranean, which is considered as a climate hotspot.

In this work we utilize space-based radar products from the CloudSat mission to provide statistics on the properties of the clouds observed above the Mediterranean during the period 2007 – 2017. CloudSat’s payload, the Cloud Profiling Radar (CPR), is the first spaceborne 94-GHz (W-band) radar producing vertical cloud profiles over the globe. Three domains are selected in the Mediterranean to study the geometrical properties and the cloud types by month and altitude.

Our results reveal that low-level clouds are dominant above the Mediterranean region especially during winter and spring periods, mainly appearing at altitude up to 4 km, while high clouds prevail throughout the year at altitudes between 9 and 14 km, except in July and August above the East Mediterranean, where they are nearly absent. In the East Mediterranean, a higher frequency of low-level clouds is observed during the summer period. The majority of the deep convective clouds are observed above the West and Central Mediterranean, indicating the influence of the Atlantic systems and the mid-latitude cyclones on the Mediterranean weather conditions. Additionally, a cloud climatology is constructed in order to examine trends in each cloud type.

The results from this intercomparison will be used to derive a better understanding of the model's limitations to accurately predict cloud geometrical and microphysical properties in the region, and to improve the aerosol-cloud interaction model representation. 

How to cite: Koutsoupi, I., Marinou, E., Voudouri, K. A., Tsikoudi, I., Paschou, P., Amiridis, V., Battaglia, A., Kollias, P., and Giannakaki, E.: Analysis of Cloud Types and their Geometrical Properties over the Mediterranean using CloudSat Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16774, https://doi.org/10.5194/egusphere-egu25-16774, 2025.

Atmospheric aerosols are solid mass and liquor particles levitation in the air,

which have a significant impact on the Earth 's radiation balance of energy and world

climate, achievement of the "carbon-2 goal," and even human health..In addition,

while domestic satellites are booming, there is less satellite data available for

download and of high quality. Therefore, it is an urgent demand of the country to use

FY-3D remote sensing data to retrieve aerosol characteristics in the field of air

satellite remotely sensed.This paper describes the inverse validation of AOD before and after the epidemic in the Yangtze River Delta using the Deep Blue algorithm and the study of its spatial and temporal distribution characteristics.The inversion results show that the MOD04 DB products are significantly correlated with the resampled FY-3D/MERSI-II AOD with a correlation coefficient of 0.810. In addition, the inverted AOD have a better continuity in spatial and temporal distributions in the Yangtze River Delta region.In addition, we comprehensively analyzed the inversion AOD of FY- 3D/MERSI-II and the aerosol optical thickness of Taihu station on the ground in February-June 2018 in the Yangtze River Delta, and make out that the inversion AOD was close to the ground-based observation data and the trend was consistent, and the correlation coefficient between the two was greater than 0.75.Based on the analysis of the temporal and spatial distribution of AOD in the Yangtze River Delta region before and after the epidemic, we found that the AOD values of the entire Yangtze River Delta study area showed a decreasing trend in several cities, and the AOD of several cities decreased more significantly in 2020. From a temporal perspective, the average AOD values showed a decreasing trend from 2018 to 2020, with the largest average AOD value in 2018 and the smallest average AOD value in 2020.

How to cite: bian, X. and xiao, C.: Study on the inversion of aerosol optical parameters and their spatial and temporal distribution characteristics in Yangtze River Delta region based on FY-3D, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18028, https://doi.org/10.5194/egusphere-egu25-18028, 2025.

EGU25-18561 | ECS | Posters on site | AS3.23

Evaluation of CAMS Reanalysis Aerosol Optical Properties Against POLDER/GRASP Retrievals: Insights into Fine and Coarse Mode Aerosol Characteristics 

Milagros Herrera, Abhina K. Behera, Christian Matar, Pavel Litvinov, Oleg Dubovik, Liudmyla Berdina, Victor Tishkovets, Tatyana Lapyonok, Fabrice Ducos, and David Fuertes

Discrepancies in aerosol representation in chemistry-transport models (CTMs) arise from uncertainties in emission sources. These are exacerbated by nonlinear physico-chemical processes and transport. Assumptions about optical properties and limitations in satellite retrievals further contribute to the problem. Despite their significance, such disparities remain largely unaddressed. Under the European Commission’s CAMS Model Evolution (CAMEO) project, we conducted an intercomparison of aerosol physical properties between CAMS reanalysis and POLDER/GRASP products. POLDER, a multi-angular polarimeter onboard PARASOL, operated from 2008 to 2013. This study examines adjustments made to the GRASP retrieval algorithm to address these disparities in the CAMS CTM.

Our findings show that CAMS aerosol optical depth (AOD) at multiple wavelengths closely aligns with POLDER/GRASP data when CAMS refractive indices are incorporated into the retrieval algorithm. While CAMS assimilates MODIS 550 nm AOD data, it also produces reliable AODs across other wavelengths. Validation at AERONET stations, focusing on the year 2008, demonstrated reasonable agreement for biomass-burning aerosols, desert dust, and anthropogenic pollutants. However, uncertainties remain in estimating single scattering albedo (SSA). Furthermore, CAMS fine-mode AOD aligns well with POLDER/GRASP retrievals. In contrast, CAMS coarse-mode AOD shows a weak positive linear correlation with POLDER/GRASP. From July to September, CAMS reanalysis exhibits a non-negligible bias at sites dominated by biomass burning and anthropogenic emissions, confirmed by AERONET ground data. These results highlight persistent uncertainties in representing black carbon, brown carbon, and organic matter in both CTMs and satellite retrievals. Over dust-dominated stations, fine-mode dust exhibits light-absorbing properties, while coarse-mode dust shows minimal spectral variation. Such findings, which vary by location and season, provide crucial insights for CTM development.

This work supports future advancements in aerosol modelling and lays the groundwork for exploring the capacities of upcoming multi-angular, multi-viewing polarimetric missions, such as PACE/HARPOL-2, PACE/SPEX, and 3MI. These efforts will improve data assimilation and enhance the accuracy of CAMS reanalysis datasets.

How to cite: Herrera, M., Behera, A. K., Matar, C., Litvinov, P., Dubovik, O., Berdina, L., Tishkovets, V., Lapyonok, T., Ducos, F., and Fuertes, D.: Evaluation of CAMS Reanalysis Aerosol Optical Properties Against POLDER/GRASP Retrievals: Insights into Fine and Coarse Mode Aerosol Characteristics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18561, https://doi.org/10.5194/egusphere-egu25-18561, 2025.

EGU25-18672 | ECS | Posters on site | AS3.23

Versatile Aerosol and Cloud Obstruction Mask (ACOM) for Diverse Remote Sensing Applications 

Christian Matar, Pavel Ltivinov, Cheng Chen, Masahiro Momoi, Juan Gomez, Zhen Liu, Oleg Dubovik, and Philippe Goryl

Clouds and aerosols can obstruct the solar radiation propagating through the atmosphere before it reaches the Earth's surface due to the scattering and absorption processes. The impact of this obstruction on Earth observation is related to the degree of obstruction along the optical path, and the remote sensing application in question. Usually, such obstruction is accounted for by applying cloud and shadow masking for the observed pixels or by performing simultaneous atmosphere/surface retrieval. Estimation of the atmospheric signal (clouds and aerosol obstructions) from the top of atmosphere measurements can be used to identify clouds, cloud shadows or the presence of aerosol in the atmosphere. In ACOM this is done by extracting surface signal from atmospheric one and then separating clouds and aerosol features from each other using multi-dimensional spectral thresholds and spatial variability tests.

The concept applied in ACOM allows a quantitative estimation of the atmospheric obstruction which results in the distinction of different clouds and aerosol classes varying from low to high levels of aerosol and cloud loading in addition to cloud vicinity, cloud shadow and aerosol plumes shadow classes. ACOM shows robust results with ENVISAT/MERIS and Sentinel-3/OLCI and the algorithm can be easily extended to any other optical instruments with spectral channels in the blue and infrared ranges.

How to cite: Matar, C., Ltivinov, P., Chen, C., Momoi, M., Gomez, J., Liu, Z., Dubovik, O., and Goryl, P.: Versatile Aerosol and Cloud Obstruction Mask (ACOM) for Diverse Remote Sensing Applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18672, https://doi.org/10.5194/egusphere-egu25-18672, 2025.

EGU25-18896 | Posters on site | AS3.23

Synergy in GRASP of space multiwavelength multi-angle polarimetry and lidar measurements for vertical profiles of aerosol optical and microphysical properties 

Daniel Perez-Ramirez, Pavel Litvinov, Anton Lopatin, Onel Rodriguez-Navarro, Jorge Muñiz-Rosado, David Fuertes, Oleg Dubovik, Anin Puthukuddy, and Vanderlei Martins

During the last years there have been a great advance in the development of satellite missions for Earth Observation. Most of them rely on passive remote sensing measurements, particularly on multiwavelength multi-angular polarimetry measurements (MAP). Upcoming missions such as Sentinel-5 will also deploy MAP and there are even private initiatives to expand space MAP measurements. Although MAP measurements have been proven to be ideal for expanding our knowledge in aerosol optical and microphysical properties (Dubovik et al., 2019), they provided very limited information of the aerosol properties vertically-resolved. On the other hand, multiwavelength lidar measurements are capable of providing accurate aerosol vertical profiles but face with limitations in the retrieval of aerosol optical and microphysical properties because of the limited information content of the stand-alone lidar measurements (Perez-Ramirez et al., 2019). Here we explore the potentiality of inverting aerosol microphysical properties vertically-resolved by combining in the Generalized Retrieval of Atmosphere and Surface Properties (GRASP – Dubovik et al., 2021) space lidar and polarimetry measurements.

We present extensive simulations of aerosol optical and microphysical properties vertical-profiles retrievals combining multiwavelength MAP and lidar measurements in GRASP, with the enhanced capability of differentiating between aerosol fine and coarse mode properties. The retrieval is pushed forward by trying to obtain 22 bins size distribution, similar to those provided by AERONET. In the simulations different mixtures of fine and coarse mode were used, varying refractive indexes from low to high absorption. We have used the HARP-like polarimetry configuration that uses the heritage of POLDER space polarimetry and is deployed in the NASA PACE mission. For lidar measurements, multiwavelength configurations are tested, from single backscattering measurements to adding additional extinction measurements. Our results show full capacity of GRASP to retrieve aerosol properties vertically-resolved differentiating between fine and coarse properties, although the more accurate results are obtained when using all lidar information. However, we found out that optimized retrieval needs of constraining surface properties, particularly because of the impact of BPDF in coarse mode retrieval. Limitations in surface retrievals can be solved with the multi-pixel approach in GRASP when applied to real missions. Finally, we present case-study of synergy retrievals from airborne measurements obtained during NASA field campaigns when AirHARP + lidar flew together. The results of the simulations serve as baseline for future space mission that will combine space lidar + polarimetry or to the synergy of different satellite missions.

References

Dubovik, O., et al., 2019: Polarimetric remote sensing of atmospheric aerosols: instruments, methodologies, results, and perspectives. J. Quant. Spectrosc. Radiat. Transfer224, 474-511,

Dubovik, O, et al., 2021: A comprehensive description of multi-term LSM for applying multiple a priori constraints in problems of atmospheric remote sensing: GRASP algorithm, concept and applications. Front. Remote. Sens., 2, 706851.

Perez-Ramirez, D, et al., 2019: Retrievals of aerosol single scattering albedo by multiwavelength lidar measurements: Evaluations with NASA Langley HSRL-2 during DISCOVER-AQ field campaigns. Remote. Sens. Environ., 222, 144-164.

How to cite: Perez-Ramirez, D., Litvinov, P., Lopatin, A., Rodriguez-Navarro, O., Muñiz-Rosado, J., Fuertes, D., Dubovik, O., Puthukuddy, A., and Martins, V.: Synergy in GRASP of space multiwavelength multi-angle polarimetry and lidar measurements for vertical profiles of aerosol optical and microphysical properties, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18896, https://doi.org/10.5194/egusphere-egu25-18896, 2025.

EGU25-19194 | Orals | AS3.23

The (CLIM) Cloud Imager and the (MAP) Multi-Angle Polarimeter in the Context of Atmospheric Correction for CO2 Retrievals 

Pepe Phillips, Helmut Bauch, Martin Böttcher, Oleg Dubovik, Bertrand Fougnie, Ruediger Lang, Christian Matar, Rene Preusker, Ralf Quast, and Sruthy Sasi

The Copernicus carbon dioxide monitoring (CO2M) mission is the space component of the European integrated monitoring and verification support capacity dedicated to monitoring anthropogenic CO2 emissions. Due to the high accuracy requirements of this measurement, it is critical to measure and characterise cloud and aerosol in support of the CO2 retrieval. The Cloud Imager (CLIM) and the Multi-Angle Polarimeter (MAP) are therefore included as a payloads on the CO2M mission and the measured cloud and aerosol properties are used to correct for scattering and transmission in the downstream greenhouse gas (GHG) retrieval. The synergistic use of the cloud and aerosol products within the CO2M ground segment will be described.

 

How to cite: Phillips, P., Bauch, H., Böttcher, M., Dubovik, O., Fougnie, B., Lang, R., Matar, C., Preusker, R., Quast, R., and Sasi, S.: The (CLIM) Cloud Imager and the (MAP) Multi-Angle Polarimeter in the Context of Atmospheric Correction for CO2 Retrievals, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19194, https://doi.org/10.5194/egusphere-egu25-19194, 2025.

Global distribution of cloud properties and vertical motions are investigated by using the Japan Aerospace Exploration Agency (JAXA) level2 cloud algorithms for Earth Clouds, Aerosols and Radiation Explorer (EarthCARE), which is the JAXA and the European Space Agency (ESA) joint satellite mission. Cloud profiling radar (CPR)-only and CPR-atmospheric lidar (ATLID) synergy algorithms are based on the heritages from our algorithms for CloudSat and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) but several major improvements are made. The algorithms are evaluated using ground-based observations and statical comparisons are also conducted by CloudSat and CALIPSO and Aqua/MODIS data. Algorithms consist of cloud mask, cloud type(phase), cloud particle category (ice habit), cloud and precipitation microphysics, terminal velocity and vertical air motion schemes.

How to cite: Okamoto, H. and Sato, K.: Global characterization of cloud properties and vertical motions by using EarthCARE observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19666, https://doi.org/10.5194/egusphere-egu25-19666, 2025.

EGU25-6317 | ECS | Posters on site | AS3.24

Ghost Plumes: Artificial splitting of greenhouse gas emission plumes in passive remote sensing observations in special viewing geometries 

Sven Krautwurst, Jakob Borchardt, Sebastian Wolff, Oke Huhs, Christian Fruck, Konstantin Gerilowski, Christoph Kiemle, Mathieu Quatrevalet, Martin Wirth, John Philip Burrows, Andreas Fix, Heinrich Bovensmann, and Hartmut Boesch

Spectrally high-resolution passive remote sensing imaging spectrometers are becoming increasingly important for reliable quantification of anthropogenic greenhouse gas (GHG) emissions from a wide variety of carbon dioxide (CO2) and methane (CH4) sources. These nadir-looking air- or spaceborne instruments collect backscattered solar radiation from the Earth's surface, from which 2D atmospheric concentration maps of CO2 and CH4 are retrieved. Using, for example, mass balance approaches, emission rates can be derived from the observed GHG concentration gradients or plumes.

Depending on the atmospheric conditions, these plumes can be Gaussian-like shaped or severely distorted by the prevailing turbulence during a single overpass. In the case of a calm atmosphere and special viewing geometries, combined with an elevated emission height, such as CO2 emissions from a coal-fired power plant chimney, the observed plume appears widened, or even two plumes are detected from the same point source in the imaging data. This secondary plume is shifted in the opposite direction to the position of the sun and the effect is most pronounced close to the emission source and the higher the point of release and the solar zenith angle (sza) are. The effect is less noticeable as the gases are better mixed both horizontally and vertically down to the surface when advecting further downwind of the source.

In this work, we will analyse passive remote sensing observations from the MAMAP2D-Light imaging spectrometer collected over a coal-fired power plant near Edmonton, Canada, during the CoMet 2.0 Arctic mission in 2022. The power plant was investigated for distinct double plume structures on two different days with near-perfect conditions (moderately high sza and sun perpendicular to the prevailing wind direction). We will compare these with simultaneously acquired observations from an active lidar remote sensing instrument (CHARM-F) flown aboard the same aircraft. As the CHARM-F instrument uses its own light source in the nadir viewing geometry, no plume splitting is expected. We will also show that the plume broadening or splitting in the passive remote sensing instrument does not lead to a double counting of molecules and thus not to an increased emission rate of the power plant estimated from the observations. Furthermore, we compare the MAMAP2D-Light concentration gradients with Gaussian plume model simulations using the conditions encountered during the flight, which also show a similar plume widening or double-plume structure as observed in the real measurements. This effect can, for example, also be used in an inverse manner to retrieve the plume height of emissions. Conclusions on the conditions this plume splitting is observed by imaging spectrometer will be discussed.

How to cite: Krautwurst, S., Borchardt, J., Wolff, S., Huhs, O., Fruck, C., Gerilowski, K., Kiemle, C., Quatrevalet, M., Wirth, M., Burrows, J. P., Fix, A., Bovensmann, H., and Boesch, H.: Ghost Plumes: Artificial splitting of greenhouse gas emission plumes in passive remote sensing observations in special viewing geometries, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6317, https://doi.org/10.5194/egusphere-egu25-6317, 2025.

EGU25-6912 | Orals | AS3.24

Detection Limits of the GHGSat Constellation for Carbon Dioxide and Methane 

Mathias Strupler, Ariane Deslières, Marianne Girard, Dylan Jervis, Jean-Philippe MacLean, David Marshall, Jason McKeever, Becket Osterland, Zoya Qudsi, Antoine Ramier, Ewan Tarrant, and David Young

GHGSat launched its first satellite dedicated to carbon dioxide monitoring in October 2023, joining GHGSat’s ten satellite methane-sensing  constellation. All the satellites are designed to measure and attribute emissions at the facility level, leveraging their ~30 meter-scale spatial resolution. Understanding the detection threshold of both CO2 and CH4 satellites is crucial, not only as a fundamental performance metric, but also for interpreting observations where no emissions are detected (null observations). This understanding is especially important when combining observations from multiple sites or times. 

For methane-sensitive satellites, GHGSat has built a large dataset of controlled releases, including both self-organized and third-party single-blind studies. Analysis of this dataset shows a detection threshold of 102 kg/hr, with a 50% probability of detection (PoD) at a wind speed of 3 m/s. One shortcoming is that controlled releases repeatedly measure the same sites at varying source rates, and the number of controlled release sites is limited. These sites might not represent the full spectrum of measurement conditions encountered by the constellation around the world. To address this issue, we adapt the non-linear PoD model developed by Conrad et al.[1] with the goal of providing site- and time-specific detection thresholds.

We will also present an update on the performance of GHGSat’s first CO2-sensitive satellite. We will highlight the difference between CH4 and CO2 point source detection such as co-emission of CO2 with aerosols, multiple release points at a given facility and the high elevation of the release points. We will also present a preliminary analysis of detection threshold by comparing detection events and continuous emission monitoring data available from some power plants. 

[1] Conrad, B. M., Tyner, D. R. & Johnson, M. R. Robust probabilities of detection and quantification uncertainty for aerial methane detection: examples for three airborne technologies. Remote Sens. Environ. 288, 113499 (2023). 

How to cite: Strupler, M., Deslières, A., Girard, M., Jervis, D., MacLean, J.-P., Marshall, D., McKeever, J., Osterland, B., Qudsi, Z., Ramier, A., Tarrant, E., and Young, D.: Detection Limits of the GHGSat Constellation for Carbon Dioxide and Methane, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6912, https://doi.org/10.5194/egusphere-egu25-6912, 2025.

EGU25-8353 | Posters on site | AS3.24

End-to-end simulations for greenhouse gas monitoring from space with a spectrometer - lidar - camera sensor triplet 

Manuel Queisser, Errico Armadillo, Sergio Tomás, David Vilaseca, and Daria Stepanova

The greenhouse gases (GHG) methane (CH4) and carbon dioxide (CO2) have been emitted at an increasing rate since the Industrial Revolution, leading to amplified global warming. The Paris agreement, signed by 175 nations, represents the world’s first sound political framework to regulate GHG emissions. It entails a need to quantify GHG fluxes, ideally with global coverage. 

Since the pioneering missions able to detect and quantify trace gases in the Troposphere, green gas monitoring instrument (GMI) and scanning imaging absorption spectrometer for atmospheric cartography (SCIAMACHY) almost 30 years ago, a number of satellite missions that provide global coverage have been launched and are used to serve that need. There is, however, a significant discrepancy between bottom-up GHG emission estimates from inventories and top-down estimates using a combination of space-borne GHG concentration measurements and atmospheric dispersion modeling. Over the last 12 years or so, a new generation of satellites-borne imaging spectrometers emerged with sub-kilometre pixel resolution, able to map trace gas plumes and thus able to quantify GHG fluxes directly at the source, contributing to improved GHG inventories. Among those are the first commercial Earth observation missions to monitor GHG sources.

The commercial AIRMO mission aims to quantify GHG fluxes, notably CH4, in the planetary boundary layer using a combination of push-broom spectrometer, pulsed micro-lidar and visible camera. Raw lidar and spectrometer data (level-0 data) are processed (level-1b) to retrieve satellite images of CH4  and CO2 (level-2), from which images of column averaged enhancements are retrieved (level-3) and mass flux from point sources (level-4) are derived. This work will report on results of a sensitivity analyses aimed to identify the variables with the highest impact on level-4 error, including instrumental parameters (e.g., signal-to-noise ratio SNR, integration time, detector smile) and environmental variables (e.g., wind speed, surface albedo, aerosols). The approach used here is a combination of top-down and bottom-up analysis. The top-down analysis starts from the level-4 requirement of 100 kgCH4 /h and estimates from this the required precision and accuracy (bias). The bottom-up analysis simulates, end to end (from level-0 to level-4) or between sub-levels, the error propagation, validating the top-down approach. From the sensitivity study an error budget is established.

 

How to cite: Queisser, M., Armadillo, E., Tomás, S., Vilaseca, D., and Stepanova, D.: End-to-end simulations for greenhouse gas monitoring from space with a spectrometer - lidar - camera sensor triplet, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8353, https://doi.org/10.5194/egusphere-egu25-8353, 2025.

EGU25-9717 | ECS | Orals | AS3.24

Madrid Methane Remote Sensing: first results of a landfill field campaign 

Alberto Alvaro-Diaz, Lennart Resch, Lukas Häffner, Louisa-Marie Rüther, Marvin Knapp, Adela Collado Rodríguez, Christian Mielke, Angel del Pino-Jiménez, Leonie Scheidweiler, Noemi Taquet, Cristina Prados-Roman, and Andre Butz

Methane (CH4) is known to be one of the most potent greenhouse gases (GHGs) and it plays a key role in climate change due to its high warming potential. It is of both natural and anthropogenic origin. The main anthropogenic emissions of CH4 come from agriculture, fossil fuels (gas, oil, coal), landfills and wastewater treatment plants.


Two of the largest landfills in Europe are the Pinto and Technology Park Valdemingómez landfills in Spain. Both landfills, which are only a couple of kilometres apart, are located in the south of Madrid metropolitan area. These sorts of landfills are considered extended sources of GHGs due to their surface area, which spans a few square kilometres. Understanding the emissions from such landfills is critical to accurately assess and mitigate their impact on climate change.


In summer 2024, a ground-based remote sensing field campaign was carried out around these two landfills to evaluate the capabilities and limitations of the deployed instruments, which were two shortwave hyperspectral infrared cameras mounted on tripods scanning the horizon. Such a camera has previously been used for detecting emissions of GHGs from point sources such as a power plant (Knapp et al., 2024). The campaign in Madrid aimed at testing the cameras’ capabilities regarding extended sources of CH4 such as landfills. During the campaign, these ground-based measurements were complemented by observations from different satellites (GHGSat, EnMAP and TROPOMI-SP5).


This work will describe the field campaign and retrieval techniques as well as present first results of the observations of the campaign. Moreover, an extended study of TROPOMI’s observations of the target landfills will be presented (2019 - 2024), comparing inferred CH4 emission rates to previous studies and to values reported to PRTR-Spain (Spanish Register of Emissions and Pollutant Sources).

How to cite: Alvaro-Diaz, A., Resch, L., Häffner, L., Rüther, L.-M., Knapp, M., Collado Rodríguez, A., Mielke, C., del Pino-Jiménez, A., Scheidweiler, L., Taquet, N., Prados-Roman, C., and Butz, A.: Madrid Methane Remote Sensing: first results of a landfill field campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9717, https://doi.org/10.5194/egusphere-egu25-9717, 2025.

EGU25-9944 | Orals | AS3.24

Rewetting Driven Soil Respiration Shapes the Variability of Terrestrial CO2 Fluxes in Semi-arid Regions of the Southern Hemisphere 

Sanam Noreen Vardag, Eva-Marie Metz, Sourish Basu, Martin Jung, Lukas Artelt, and André Butz

The annual increase of atmospheric CO2 exhibits significant inter-annual variability, primarily driven by fluctuations in the terrestrial carbon cycle. These inter-annual changes in CO2 concentrations provide a unique opportunity to study the biosphere's carbon uptake and release in response to shifting precipitation patterns and temperature extremes. Semi-arid ecosystems have been identified as significantly contributing to the inter-annual global carbon sink dynamics. However, the sparse coverage of in-situ CO2 measurements on the southern hemisphere leads to uncertainties in measurement-based carbon flux estimates for the extensive semi-arid regions located there. Also, dynamic global vegetation models (DGVMs) show a large spread in their carbon flux estimates pointing to an incomplete representation of semi-arid carbon cycle processes in most of the models. We demonstrate the potential of satellite data to improve sub-continental scale carbon flux estimates on the southern hemisphere and analyse the underlying biogenic processes.

We here discuss monthly net CO2 fluxes from 2009 to 2018 derived by assimilating Greenhouse Gases Observing Satellite (GOSAT) XCO2 measurements in the global atmospheric inversion TM5-4DVar. For the three semi-arid regions in the southern hemisphere, i.e. Australia (Metz et al., 2023), South American Temperate region and South Africa (Metz et al., 2024), we find that the DGVMs are not consistent, but single models agree well with the satellite inversion fluxes and Solar Induced Fluorescence (SIF) measurements. While the satellite inversion can only provide net land-atmosphere fluxes, those selected DGVMs model the vegetation gross fluxes and allow further analyses of the carbon exchange processes. We find a net release of CO2 caused by enhanced soil respiration following soil rewetting at the beginning of the rainy season. These CO2 emissions strongly shape the seasonal cycle of carbon fluxes in all three semi-arid regions, and in Australia, dominate the interannual flux variability. Our findings suggest that rain pulses and soil rewetting events in semi-arid regions can be analysed using satellite observations. These processes play an important role in constraining the global carbon budget and should be represented more accurately in global carbon cycle models to improve the estimation of the global carbon budget.

Metz, E.-M., et al., (2023). Soil respiration–driven CO2 pulses dominate Australia’s flux variability. Science, 379(6639), 1332-1335., https://doi.org/10.1126/science.add7833

Metz, Eva-Marie, et al. "Seasonal and inter-annual variability of carbon fluxes in southern Africa seen by GOSAT." EGUsphere 2024 (2024): 1-35. https://doi.org/10.5194/egusphere-2024-1955

How to cite: Vardag, S. N., Metz, E.-M., Basu, S., Jung, M., Artelt, L., and Butz, A.: Rewetting Driven Soil Respiration Shapes the Variability of Terrestrial CO2 Fluxes in Semi-arid Regions of the Southern Hemisphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9944, https://doi.org/10.5194/egusphere-egu25-9944, 2025.

EGU25-10301 | ECS | Posters on site | AS3.24

A comprehensive analysis of regional spatiotemporal methane enhancements and trends in the Mediterranean, using ground-based FTIR measurements and CAMS observations 

Marios Mermigkas, Stergios Kartsios, Frank Hase, Chrysanthi Topaloglou, Darko Dubravica, Thomas Panou, Dimitrios Balis, and Vassilis Amiridis

Increased concentrations of greenhouse gases in the atmosphere have resulted in a rise in the Earth's average temperature in the last decades. Methane (CH4), the second most important anthropogenic greenhouse gas after carbon dioxide (CO2), is considered to be 2.6 times higher than pre-industrial levels (Jackson et al., 2024). CH4 is 28 times more efficient at trapping heat than CO2 over a 100-year period and 80 times more powerful over 20 years, even though it is present in smaller quantities in the atmosphere and has a shorter lifespan than CO2. A special interest lies in the monitoring of urban areas, because of their substantial role in global human-made emissions. Methane emissions include agriculture, particularly from livestock and rice paddies, which constitute the largest source, while fossil fuel activities contribute in the global methane budget as well. The rise in emissions from these sectors is mainly driven by increased activities in developing regions and the intensified extraction and use of fossil fuels, revealing an alarming growth rate of CH4.   

 

In this study, we present the column-averaged dry air mole fractions of methane (XCH4) over Thessaloniki, Greece (Mermigkas et al., 2021), using a portable EM27/SUN ground-based FTIR spectrometer, operating under the umbrella of COllaborative Carbon Column Observing Network (COCCON), covering the period from 2019 to 2023. To analyze methane's long-term variability and trends, we incorporate reanalysis data from the Copernicus Atmosphere Monitoring Service (CAMS) and more specifically from the EAC4 (ECMWF Atmospheric Composition Reanalysis 4) (Inness et al., 2019). This combined dataset allows us to examine the increasing methane concentrations over time, highlighting significant regional enhancements observed in Greece and Italy from 2019 to 2023.

 

To separate excess signals from background variations, filters with a characteristic duration are used depending on whether long-range or short-range enhancements are of interest. Short-range variations of greenhouse gases can potentially capture signatures of anthropogenic emission enhancements. To that end, we subtract the corresponding 3-hourly averaged XCH4 value for the same season, as the 3-hourly data point. This process is repeated for each year (2019-2023) separately to remove long-term trends. This approach allows for a more accurate assessment of CH4 concentration anomalies, ensuring that seasonal patterns are appropriately considered in the analysis.

 

 

Acknowledgement

"This project has received funding from the European Union’s Horizon Europe Research and Innovation programme under Grant Agreement No 101182007".  

 

 

References

Inness, A., Ades, M., Agustí-Panareda, A., Barré, J., Benedictow, A., Blechschmidt, A.-M., Dominguez, J. J., Engelen, R., Eskes, H., Flemming, J., Huijnen, V., Jones, L., Kipling, Z., Massart, S., Parrington, M., Peuch, V.-H., Razinger, M., Remy, S., Schulz, M., and Suttie, M.: The CAMS reanalysis of atmospheric composition, Atmos. Chem. Phys., 19, 3515–3556, https://doi.org/10.5194/acp-19-3515-2019, 2019

Mermigkas, M.; Topaloglou, C.; Balis, D.; Koukouli, M.E.; Hase, F.; Dubravica, D.; Borsdorff, T.; Lorente, A. FTIR Measurements of Greenhouse Gases over Thessaloniki, Greece in the Framework of COCCON and Comparison with S5P/TROPOMI Observations. Remote Sens. 202113, 3395 https://doi.org/10.3390/rs13173395

R B Jackson et al 2024 Environ. Res. Lett. 19 101002 https://iopscience.iop.org/article/10.1088/1748-9326/ad6463/pdf

 

 

How to cite: Mermigkas, M., Kartsios, S., Hase, F., Topaloglou, C., Dubravica, D., Panou, T., Balis, D., and Amiridis, V.: A comprehensive analysis of regional spatiotemporal methane enhancements and trends in the Mediterranean, using ground-based FTIR measurements and CAMS observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10301, https://doi.org/10.5194/egusphere-egu25-10301, 2025.

EGU25-10453 | ECS | Posters on site | AS3.24

Investigating the Impact of Modern Absorption Cross-Section Databases on CO2 Retrievals 

Lennart Thiemann, Tobias Schmitt, Manfred Birk, Christian Röske, Georg Wagner, and André Butz

Current spectrometers provide high-quality absorption spectra from both ground-based direct sun measurements and spaceborne backscatter measurements. Accurate retrievals of atmospheric CO2 concentrations from these measured spectra are fundamental for modelling large-scale atmosphere-surface exchange fluxes. When retrieving CO2 concentrations from measured spectra, high-quality spectroscopic reference data are essential to drive radiative transfer simulations and to enable accurate retrievals. Here, we investigate how various modern molecular absorption cross-section datasets affect CO2 retrievals in the 1.6 μm and 2 μm regions. This includes recent parameter sets derived from laboratory measurements at the German Aerospace Center (DLR e.V.) for line-mixing parameterizations (Birk et al., 2024) with separate continuum data, which were obtained in the frame of the ESA-funded project ISOGG (Improved Spectroscopy for satellite measurements Of Greenhouse Gases). We compare these new data to those from HITRAN 2020 (Gordon et al., 2022) with and without speed-dependent Voigt profile extension as well as to the ABSCO tables (Devi et al., 2016).

To evaluate the quality of the spectroscopic databases, we submit high-resolution direct-sun spectra collected by the TCCON (Total Carbon Column Observing Network) spectrometer at Karlsruhe to our RemoTeC retrieval algorithm under variation of the driving spectroscopic parameters. We evaluate the goodness of fit, systematic spectral residuals as well as spurious dependencies of the retrieved CO2 concentrations on slant airmass. We further use one year of GOSAT satellite measurements to assess whether and how differences in CO2 concentrations retrieved under variation of the spectroscopic parameters show dependencies on geophysical parameters such as latitude, season or surface type. Our analyses show that the new DLR cross sections and the HITRAN 2020 with speed dependence lead to noticeable improvements in spectral line modelling which in turn affects airmass dependencies as well as latitudinal and seasonal biases. Including the CO2 continuum from the DLR dataset further improves the fit quality. In contrast, using the ABSCO tables results in larger residuals and poorer fits compared to the standard HITRAN 2020 cross sections, particularly in the 2 μm region.

 

Birk, M., Röske, C., Wagner, G., & Hodges, J. T. (2024, June). New spectroscopic database of CO2 in the 1.6 and 2.0 µm spectral regions for remote sensing. The 17th International HITRAN Conference, Cambridge (MA), United States. https://elib.dlr.de/208834/

Devi, V. M., Benner, D. C., Sung, K., Brown, L. R., Crawford, T. J., Miller, C. E., Drouin, B. J., Payne, V. H., Yu, S., Smith, M. A. H., Mantz, A. W., & Gamache, R. R. (2016). Line parameters including temperature dependences of self- and air-broadened line shapes of 12C16O2: 1.6-μm region. Journal of Quantitative Spectroscopy and Radiative Transfer, 177, 117–144. https://doi.org/10.1016/j.jqsrt.2015.12.020

Gordon, I. E., Rothman, L. S., Hargreaves, R. J., Hashemi, R., Karlovets, E. V., Skinner, F. M., Conway, E. K., Hill, C., Kochanov, R. V., Tan, Y., Wcisło, P., Finenko, A. A., Nelson, K., Bernath, P. F., Birk, M., Boudon, V., Campargue, A., Chance, K. V., Coustenis, A., … Yurchenko, S. N. (2022). The HITRAN2020 molecular spectroscopic database. Journal of Quantitative Spectroscopy and Radiative Transfer, 277, 107949. https://doi.org/10.1016/j.jqsrt.2021.107949

How to cite: Thiemann, L., Schmitt, T., Birk, M., Röske, C., Wagner, G., and Butz, A.: Investigating the Impact of Modern Absorption Cross-Section Databases on CO2 Retrievals, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10453, https://doi.org/10.5194/egusphere-egu25-10453, 2025.

EGU25-10953 | ECS | Orals | AS3.24

AI-driven point source estimation for future satellite missions 

Thomas Plewa, Christian Frankenberg, André Butz, and Julia Marshall

To support the goals of the Paris Agreement, monitoring and verification support (MVS) capacities focussing on anthropogenic greenhouse gas emissions are being developed, such as the EU’s emerging Copernicus CO2 Service and Germany’s ITMS (Integriertes Treibhausgas-Monitoringsystem). Satellite concepts capable of measuring atmospheric CO2 and CH4 concentrations on small spatial scales (10s of meters) have emerged as potential contributors to such MVS systems, through their ability to image the exhaust plumes of individual facilities. To quantify emissions based on these plume images, traditional mass balance methods require an accurate knowledge of the effective speed of the wind that transports the detected CO2 or CH4 plume. Uncertainty in the wind speed is the largest source of uncertainty in the estimated emissions. It has been proposed, however, that machine learning approaches might be able to estimate emission rates directly from the turbulent plume images without the need to impose wind speeds from external sources.

Here, we present our progress on developing a deep-learning-based emission rate estimator for plume images using convolutional neural networks. Our main focus lies on the improvement of the quality and certainty of deep learning models. Therefore, we provide a model that is capable of providing estimates with, on average, little to no bias over a large scale of flux rates. We present a feasible solution to existing biases, leading to a Pearson correlation coefficient of 97.98% for true and estimated fluxes. In addition, our model provides error estimates alongside its flux predictions, making a first step towards improving the certainty of estimated predictions. Further, we present our progress on making the model more stable across different wind speed situations, and potentially extracting effective wind speed information directly from image data. Thus, we are working towards applying deep-learning-based methods in a more stable and powerful approach that is capable of efficiently analyzing large amounts of incoming data.

How to cite: Plewa, T., Frankenberg, C., Butz, A., and Marshall, J.: AI-driven point source estimation for future satellite missions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10953, https://doi.org/10.5194/egusphere-egu25-10953, 2025.

EGU25-11005 | Posters on site | AS3.24

The ITMS-FTIR network for Germany: Providing consistent XCO2, XCH4 and XCO data for satellite and model validation on the urban, regional and national scale 

Benedikt Löw, Lena Feld, Lukas Grosch, Friedrich Klappenbach, Ralph Kleinschek, Junwei Li, Andreas Luther, Moritz Makowski, Nicolas Neumann, Moritz Sindram, Josef Stauber, Jia Chen, Frank Hase, Thorsten Warneke, and André Butz

Top-down estimation of greenhouse gas emissions requires the combination of reliable measurements of their atmospheric concentrations with atmospheric inversions. The German Integrated Greenhouse Gas Monitoring System (ITMS) combines atmospheric in situ and satellite measurements, transport modelling and inverse estimation techniques aiming at an operational top-down monitoring of greenhouse gas emissions. We contribute to this effort by establishing highly consistent and accurate observations of column-average mole fractions of carbon dioxide (XCO2), methane (XCH4) and carbon monoxide (XCO) using eight FTIR instruments across Germany.

We operate spectrometers of the Collaborative Carbon Column Observing Network (COCCON, EM27/SUN) and Total Column Carbon Observing Network (TCCON) located such that the measurements cover spatial gradients on the urban, regional and national scale. Urban gradients are covered with five FTIR distributed across the Munich urban region (MCCnet). The regional scale is represented by two FTIR in Karlsruhe and Heidelberg (Rhein-Neckar region) and two FTIRs in the Bremen region in Northern Germany. All instruments together allow for measuring gradients on the national scale. These measurements provide the means to validate both satellite observations and modelling results on the spatial scales relevant for future emission inversions. To meet the stringent requirements for consistency among all stations, we operate an additional EM27/SUN as travel standard for side-by-side measurements with all instruments. As such, we tie all instruments to a common scale and, via TCCON, to the World Meteorological Organization (WMO) scale. Here, we present the ITMS-FTIR network with a special focus on our calibration efforts during the first year of operation.

How to cite: Löw, B., Feld, L., Grosch, L., Klappenbach, F., Kleinschek, R., Li, J., Luther, A., Makowski, M., Neumann, N., Sindram, M., Stauber, J., Chen, J., Hase, F., Warneke, T., and Butz, A.: The ITMS-FTIR network for Germany: Providing consistent XCO2, XCH4 and XCO data for satellite and model validation on the urban, regional and national scale, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11005, https://doi.org/10.5194/egusphere-egu25-11005, 2025.

EGU25-11171 | ECS | Posters on site | AS3.24

Analysis of Methane Emissions from the Darvaza Gas Crater 

Adriana Valverde, Itziar Irakulis-Loitxate, Javier Gorroño, and Luis Guanter

Methane (CH4), a greenhouse gas 86 times more potent than carbon dioxide (CO2) over 20 years, has become one of the main drivers of climate change, with atmospheric levels doubling since pre-industrial times. Among its various natural and anthropogenic sources, such as oil and gas systems, coal mines, or landfills, the Darvaza gas crater in Turkmenistan stands out as a unique and persistent contributor. This crater, usually known as "Door to Hell", is located in the Amu-Darya basin, a geological formation replete with large quantities of oil and natural gas, in which methane is predominant. In 1971, a drilling operation for natural gas by a soviet geologist caused the ground to collapse. The resulting crater measured approximately 70 meters in diameter and 20 meters deep. To mitigate the release of hazardous gases, authorities ignited the escaping gas, burning without interruption so far. However, since last year, the fire in the crater has been reduced by the Turkmenistan government, as we can monitor using the VIIRS Fires and Thermal Anomalies product.
Our work focuses on detecting and quantifying the Darvaza methane emissions, trying to confirm whether there is a correlation between fire reduction and emissions. At the moment, we have detected more than 20 methane emissions using the hyperspectral imaging spectrometers EnMAP, PRISMA, and EMIT spaceborne instruments. The emissions range is between 1.000-3.000 kg/h, amounting to thousands of tonnes of CH4 annually.
In addition to quantifying emissions, we examined the chronology of the crater flames. By analyzing radiance and thermal bands from Landsat 4-5, we determined the onset of the crater fire in late 1987 or early 1988, a detail previously shrouded in uncertainty. This revelation contributes to the temporal analysis of this crater and provides key information for estimating the total amount of methane released by the Darvaza crater to date.
Lastly, the unique conditions at Darvaza—continuous methane release and decades of intense fire—may have significantly altered the surrounding environment. To explore this possibility, we investigate soil composition and mineralogy changes using geological indices. This analysis aims to understand the broader environmental impact of the crater, offering insights into the long-term effects of such phenomena.

How to cite: Valverde, A., Irakulis-Loitxate, I., Gorroño, J., and Guanter, L.: Analysis of Methane Emissions from the Darvaza Gas Crater, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11171, https://doi.org/10.5194/egusphere-egu25-11171, 2025.

EGU25-11707 | ECS | Posters on site | AS3.24

High resolution Turbulence modelling to improve complicated methane emissions observed from Satellite Imagery 

Rakesh Yuvaraj, Thomas Lauvaux, Charbel Abdallah, Apisada Chulakadabba, Steven Wofsy, and Alexis Groshenry

With the growing interest to identify and quantify methane (CH4) emissions from various sources around the globe, the development and launches of satellite imagers tracking CH4 plumes have accelerated during the past decade. Thanks to high-resolution images collected by PRISMA (30-m resolution), Sentinel-2 (20-m resolution), or Tanager-1 of Carbon Mapper (30-m resolution), it is now possible to sample CH4 plumes at small scales to enable source attribution and quantification at lower detection levels. However, high-resolution images also come with limitations, due to the dominance of small-scale turbulence physics near the source. Therefore, Large Eddy Simulation (LES) modelling becomes necessary to resolve the turbulence, leading to more robust emission quantification methods. The Fire Dynamics Simulation (FDS) model offers unique capabilities by allowing to introduce infrastructures, terrain topologies, and roughness, individual trees (incl. leaves, branches, tree shapes), surface temperature gradients, velocity of the gas release, velocity of the leaked air, and to simulate the dynamics of the plume at a high resolution near the source and coarse resolution away from the source (adaptive mesh refinement). Using such high-resolution LES modelling allows us to simulate the spatial structure of the CH4 plumes, at various distances from the source, under different meteorological conditions (forced by wind measurements or re-analysis products). We aim here to (i) define more rigorously the effective wind speed used by the Integral Mass Enhancement (IME) method, (ii) to determine the sensitivity to external parameters that affect the plume dynamics, and (iii) to analyze complicated plumes (excluded in current IME analyses) thanks to our LES simulations offering additional detections to current monitoring systems (e.g., MARS).

 

More specifically, we compare and evaluate the importance of all the environmental conditions (topography, obstacles) and the characteristics of the source (temperature, velocity, height) affecting the dynamics of the turbulent CH4 plumes to determine the most favorable conditions and the uncertainties in IME estimates diagnosed from satellites and aircraft measurement campaigns. We also determine the sensitivity of the emissions to the effective wind speed simulations as a function of distance to the source and its comparison with existing wind speed calculation methods (e.g., extrapolation from 10-m wind speed measurement) used in current mass balance approaches. This study leads us to discuss the use of high-resolution LES simulations in mass balance calculations to produce more reliable estimates of facility-level sources around the globe.

How to cite: Yuvaraj, R., Lauvaux, T., Abdallah, C., Chulakadabba, A., Wofsy, S., and Groshenry, A.: High resolution Turbulence modelling to improve complicated methane emissions observed from Satellite Imagery, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11707, https://doi.org/10.5194/egusphere-egu25-11707, 2025.

EGU25-14549 | Orals | AS3.24

Carbon-I, a NASA Earth System Explorer Mission concept for Greenhouse Gas Observations 

Christian Frankenberg, Anna Michalak, Daniel Jacob, Andrew Thorpe, Yi Yin, Lori Bruhwiler, Ermias Kebreab, Alison Hoyt, Alex Turner, Paul Wennberg, Robert Green, Suniti Sanghavi, David Thompson, Philip Brodrick, and Dana Chadwick

The past two decades have seen tremendous improvements in greenhouse gas (GHG) remote sensing from space, including global area flux mappers like SCIAMACHY, GOSAT, OCO-2, GOSAT-2, TROPOMI and OCO-3 among others, with more missions planned, such as CO2M. In the past decade there has also been an increase in GHG point source imagers, a field that has grown rapidly after initial successes using AVIRIS-NG and subsequent VSWIR spectrometers (coarser spectral resolution over a broader range). While area flux mapper missions have been effective at measuring GHG with high accuracy, fundamental gaps persist in the humid tropics, where data yields are 2-3 orders of magnitude lower than elsewhere.

 

Here, we discuss the Carbon Investigation (Carbon-I), which was selected for a Phase A mission concept study within NASA’s Earth System Explorer call. Carbon-I provides a unique combination of global land coverage, high spatial resolution, and very high sensitivity required to quantify CH4, CO2, and CO emissions at both the area and point source scale. Given the importance of the tropics for global carbon budgets and in particular natural methane emissions, Carbon-I specifically targets the remaining data and knowledge gaps within the tropics, enabling a step change in our capabilities of observing the tropics with more even temporal and spatial sampling.

Carbon-I is a single-band spectrometer covering the 2040 to 2380 nm spectral range with 0.7nm spectral sampling and spatial sampling ranging from ~30m in a local target mode to ~300m for global land mapping. We will discuss the sweet spot in the tradeoff between spatial and spectral resolution, the multi-species trace gas capabilities (CH4, CO2, CO, HDO, H2O, N2O, potentially Ethane), the capabilities to measure GHG area fluxes and point sources while minimizing surface interferences and our approach to account for atmospheric scattering effects.

How to cite: Frankenberg, C., Michalak, A., Jacob, D., Thorpe, A., Yin, Y., Bruhwiler, L., Kebreab, E., Hoyt, A., Turner, A., Wennberg, P., Green, R., Sanghavi, S., Thompson, D., Brodrick, P., and Chadwick, D.: Carbon-I, a NASA Earth System Explorer Mission concept for Greenhouse Gas Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14549, https://doi.org/10.5194/egusphere-egu25-14549, 2025.

EGU25-15004 | Posters on site | AS3.24

The Potential for Future Satellite Missions to Advance the Arctic Methane Permafrost Challenge (AMPAC) 

Annett Bartsch, Bradley A. Gay, Dirk Schüttemeyer, Edward Malina, Kimberley Miner, Guido Grosse, Andreas Fix, Johanna Tamminen, Hartmut Bösch, Robert J. Parker, Kimmo Rautiainen, Josh Hashemi, and Charles E. Miller

Permafrost degradation in the Arctic is accelerating and expected to enhance greenhouse gas (GHG) emissions. The Arctic Methane and Permafrost Challenge (AMPAC) was initialized by NASA and ESA as a transatlantic networking action striving to promote scientific research and improve observational capabilities. Earth Observation technology must be harnessed, expanded and synergies exploited to accurately quantify and better understand the state of the permafrost and coincident methane emissions. AMPAC aims at improving the observation capacity over polar regions by evaluating dedicated campaign activities, by analyzing satellite data, and by identifying satellite retrieval improvements. AMPAC provides suggestions for the enhanced exploitation of the increasing Earth observation (EO) capacities of land surface, cryosphere, biosphere and atmosphere missions to enhance the scientific understanding of changes in Arctic permafrost regions and methane emissions and to bridge the gap between top-down (T-D) and bottom-up (B-U) estimates of methane fluxes in the changing Arctic.

In particular, monitoring of methane concentrations as well as landcover properties related to wetland and freeze/thaw dynamics is needed. Upcoming synthetic aperture radar missions and constellations of multiple multispectral sensors are expected to advance relevant monitoring capabilities significantly. This will allow better representation of seasonality and advance methane source attribution in general. In addition, continuity of current missions providing greenhouse gas observations, including methane, is crucial. Active optical instruments (lidar) developed for concentration retrieval are expected to substantially enhance detection capabilities across the Arctic.

We provide an overview of relevant current and approved atmosphere and land-focused satellite missions of NASA, NOAA, ESA and DLR/CNES with emphasis on advancements and remaining gaps in the context of AMPAC.

How to cite: Bartsch, A., Gay, B. A., Schüttemeyer, D., Malina, E., Miner, K., Grosse, G., Fix, A., Tamminen, J., Bösch, H., Parker, R. J., Rautiainen, K., Hashemi, J., and Miller, C. E.: The Potential for Future Satellite Missions to Advance the Arctic Methane Permafrost Challenge (AMPAC), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15004, https://doi.org/10.5194/egusphere-egu25-15004, 2025.

EGU25-15077 | Posters on site | AS3.24

Implementation of SI-traceability in the TCCON and COCCON observations: the  Metrology for Comparable and Trustworthy Greenhouse gas remote sensing datasets (24GRD06 MetCTG) project 

Dietrich G. Feist, Manfred Birk, Domenico Prudenzano, Georg Wagner, Gang Li, Alexandra Lüttschwager, Christian Monte, Rainer Stosch, Dieter Taubert, Andre Butz, Frank Hase, Jia Chen, Rigel Kivi, Jeremias Seppa, Raymond Armante, Ha Tran, Alain Campargue, Samir Kassi, Didier Mondelain, Giulio Beltramino, Francesca Durbiano, Vito Fernicola, Lucia Rosso, Sangil Lee, Maciej Chomski, Maciej Gruszczynski, Przemyslaw Glowacki, Daniel Lisak, Piotr Masłowski, Roman Ciuryło, Joachim Mohn, Paul Brewer, Marc Coleman, Tom Gardiner, Christoph Nehrbass-Ahles, Ruth Pearce, Chris Rennick, Jonathan Tennyson, Oleg Polyansky, Jeremy Harrison, Can Gozonunde, and Humbet Nasibli

Satellite remote sensing of global greenhouse gas (GHG) concentrations provides invaluable information about GHG sources and sinks, supporting efficient climate mitigation policies. Recently, the accuracy targets of upcoming GHG satellite missions have become increasingly stringent (2 ppb of CH4; 1 ppm of CO2).

Up to now, calibration and traceability of satellite GHG observations relies on two networks of ground-based remote sensing stations: the Total Carbon Column Observing Network (TCCON) and the COllaborative Carbon Column Observing Network (COCCON). Both networks are able to observe the same quantity as the satellite instruments: column-averaged dry-air mole fraction of CO2 and CH4. They also observe N2O, which will likely become another key GHG to be monitored in the future. For traceability, both networks rely on regular aircraft and balloon measurements with in-situ instruments that are traceable to the WMO scale for GHGs.

The 24GRD06 MetCTG project aims at greatly improving the accuracy of underlying spectral line parameters for the satellite GHG retrievals and validating the accuracy with in situ and ground-based observations. This will establish traceability to SI and improve data comparability and trustworthiness among GHG satellite missions. It will also improve consistency among ground-based sites and considerably reduce the need for costly aircraft calibrations.

The project joins the European metrology community with the TCCON and COCCON communities to provide the best ground-based reference for current and future GHG satellite missions.

Acknowledgments: The project (24GRD06 MetCTG) receives funding from the European Partnership on Metrology, co-financed from the European Union’s Horizon  Europe Research and Innovation Programme and by the Participating States.

How to cite: Feist, D. G., Birk, M., Prudenzano, D., Wagner, G., Li, G., Lüttschwager, A., Monte, C., Stosch, R., Taubert, D., Butz, A., Hase, F., Chen, J., Kivi, R., Seppa, J., Armante, R., Tran, H., Campargue, A., Kassi, S., Mondelain, D., Beltramino, G., Durbiano, F., Fernicola, V., Rosso, L., Lee, S., Chomski, M., Gruszczynski, M., Glowacki, P., Lisak, D., Masłowski, P., Ciuryło, R., Mohn, J., Brewer, P., Coleman, M., Gardiner, T., Nehrbass-Ahles, C., Pearce, R., Rennick, C., Tennyson, J., Polyansky, O., Harrison, J., Gozonunde, C., and Nasibli, H.: Implementation of SI-traceability in the TCCON and COCCON observations: the  Metrology for Comparable and Trustworthy Greenhouse gas remote sensing datasets (24GRD06 MetCTG) project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15077, https://doi.org/10.5194/egusphere-egu25-15077, 2025.

EGU25-16209 | Posters on site | AS3.24

First data from GEMINI-UK, the UK national network of ground-based greenhouse gas observing spectrometers 

Neil Humpage, Paul Palmer, Alex Kurganskiy, Liang Feng, Jerome Woodwark, Stamatia Doniki, and Damien Weidmann

Over the past year, the National Centre for Earth Observation have been working to establish the Greenhouse gas Emissions Monitoring network to Inform Net-zero Initiatives for the UK (GEMINI-UK), a key part of the UK Greenhouse gas Emissions Measurement Modelling Advancement (GEMMA) programme. The GEMINI-UK network comprises ten Bruker EM27/SUN shortwave infrared spectrometers, and has been designed to help quantify regional net greenhouse gas (GHG) emissions across the UK, complementary to in situ air sampling measurements collected by the existing tall tower network. Taken together with inverse modelling efforts, these data will form the backbone of a pre-operational GHG emissions monitoring framework for the UK.

The GEMINI-UK instruments observe column concentrations of carbon dioxide, methane, and carbon monoxide in cloud-free conditions, which we use in to constrain regional flux estimates of these gases by way of Bayesian inverse methods. Using a dataset of simulated measurements based on the GEOS-Chem atmospheric chemistry and transport model, we have designed the measurement network to deliver the biggest error reductions in carbon dioxide flux estimates. We are also working closely with the GEMINI-UK host partners, including UK universities, schools, and NERC facilities, with the goal of promoting the open access and transparency of the collected data. Continuous and autonomous operation of the EM27/SUNs is made possible at each site by using an automated weatherproof enclosure, based on a design developed by University of Edinburgh researchers, which previously enabled year-round measurements to be collected during the UK DARE-UK experiment in central London. In this presentation we describe the first data, current status, and longer-term goals of GEMINI-UK, including an ongoing evaluation of the GEMINI-UK EM27/SUN that operates alongside a higher specification TCCON spectrometer at the Rutherford Appleton Laboratory in Harwell, Oxfordshire.

How to cite: Humpage, N., Palmer, P., Kurganskiy, A., Feng, L., Woodwark, J., Doniki, S., and Weidmann, D.: First data from GEMINI-UK, the UK national network of ground-based greenhouse gas observing spectrometers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16209, https://doi.org/10.5194/egusphere-egu25-16209, 2025.

EGU25-16665 | Posters on site | AS3.24

Can we obtain consistent emissions in Europe from three different CH4 TROPOMI products? 

Antoine Berchet, Aurélien Sicsik-Paré, Isabelle Pison, Audrey Fortems-Cheiney, Grégoire Broquet, and Élise Potier

Satellite observations of total column methane atmospheric mixing ratios (XCH4) combined with atmospheric transport inverse modeling offer enhanced capabilities to monitor the methane (CH4) emissions at regional scale.

The TROPOspheric Monitoring Instrument (TROPOMI) onboard the Sentinel-5 Precursor (S5P) satellite provides XCH4 with global daily coverage and a relatively high (5.5×7 km²) horizontal resolution since 2017. Widely used for the hotspot detection and quantification, TROPOMI-CH4 data is also exploited in regional and global CH4 flux inversions.

Three retrieval products of XCH4are produced and routinely updated from TROPOMI: the SRON official product, the WFMD product by the University of Bremen and the BLENDED product by the University of Harvard. The official dataset (v2.04) relies on the RemoTeC full-physics algorithm, which retrieves atmospheric methane concentration alongside atmospheric scattering properties. The WFMD scientific product is based on the University of Bremen’s Weighting Function Modified Differential Optical Absorption Spectroscopy (WFM-DOAS) and a machine learning classifier for quality filtering. The BLENDED product combines S5P-TROPOMI and GOSAT-TANSO retrievals. It is a post-processed of the official TROPOMI product, correcting biases using a machine learning model trained on collocated observations from both instruments. Despite recent advances in retrieval techniques, inter-product comparisons reveal notable differences in quality filtering, observed XCH₄ values, and associated uncertainties. It leads to discrepancies in flux estimates derived from inversions, particularly at local and country scales.

We assimilate these three TROPOMI XCH4products into regional atmospheric inversions of CH₄ emissions over Europe at a 0.5°×0.5° resolution, for the year 2019. The inversions are conducted using the CHIMERE transport model within the inverse modeling platform Community Inversion Framework (CIF). In situ surface measurements are used for validation. We investigate the primary factors contributing to the inter-product differences, including albedo, aerosols and striping patterns. We also perform Observing System Simulation Experiments (OSSE) with synthetic pseudo-observations and perturbed prior fluxes to assess the sensitivity of the system to observations and isolate the causes of the differences in inversion results. We inquire into the impact of observation density, retrieval errors and inter-product biases on the posterior fluxes. The resulting methane emissions budgets are compared at pixel, country and regional scales, providing insights into the consistency of TROPOMI-based regional inversions.

How to cite: Berchet, A., Sicsik-Paré, A., Pison, I., Fortems-Cheiney, A., Broquet, G., and Potier, É.: Can we obtain consistent emissions in Europe from three different CH4 TROPOMI products?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16665, https://doi.org/10.5194/egusphere-egu25-16665, 2025.

EGU25-16982 | Orals | AS3.24

CO2 emission maps inferred from co-emitted anthropogenic NOx emissions 

Ronald van der A, Xiaojuan Lin, Jos de Laat, Jieying Ding, and Henk Eskes

Satellite observations of CO2 concentrations have limited spatial coverage, which makes it difficult to derive compete gridded maps of CO2 emissions. On the other hand, the co-emitted anthropogenic NOx emissions can be derived almost on a daily basis using the observations from the TROPOMI instrument on the Sentinel 5P satellite. We introduce an innovative approach to indirectly infer and map anthropogenic CO2 emissions using the co-emitted NOx emissions derived from TROPOMI NO2 observations using the DECSO algorithm. The satellite-derived emissions over Europe are close to the reported emissions indicating a low uncertainty of currently reported European emissions. The reported CO2 emissions over the Middle East and Africa are underestimated by about 40 % according our results, revealing significant reporting uncertainties. Our approach demonstrates the capability for fast and independent quantifying and mapping CO2 emissions on a continental scale based on global satellite observations. 
The derived annual CO2 emissions derived are compared with the CAMS CO2 emission inventory for country totals and for individual cities. The results demonstrate the potential for DECSO to quickly quantify and map anthropogenic CO2 emissions based on Sentinel 5P observations.

How to cite: van der A, R., Lin, X., de Laat, J., Ding, J., and Eskes, H.: CO2 emission maps inferred from co-emitted anthropogenic NOx emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16982, https://doi.org/10.5194/egusphere-egu25-16982, 2025.

EGU25-17010 | ECS | Orals | AS3.24

Evaluating national & urban Indian methane emissions using satellites  

Srijana Lama, Joannes D Maasakkers, Xin Zhang, Daniel J Varon, Melissa P. Sulprizio, Lucas A. Estrada, Nick Balasus, Robert J Parker, and Ilse Aben

India ranks as the third-largest methane emitter globally, with methane emissions increasing by 30% since 1990. According to India’s most recent report to the United Nations Framework Convention on Climate Change (UNFCCC), anthropogenic methane emissions are estimated at 18.7 Tg/year. However, these estimates are based on bottom-up calculations using activity data and laboratory-derived emission factors, and India lacks a dense network of ground-based measurements to validate them.

Recent advances in satellite technology, offering higher spatial and temporal resolution, have enabled the exploration of areas without ground-based measurements. We use a blended product from the TROPOspheric Monitoring Instrument (TROPOMI) and the Greenhouse Gases Observing Satellite (GOSAT) in Bayesian inversions with the Integrated Methane Inversion framework (IMI) to estimate 2021 Indian methane emissions. Prior emissions include fossil fuel exploitationsources from the Global Fuel Exploitation Inventory (GFEI v2) and other anthropogenic sources from the Emissions Database for Global Atmospheric Research (EDGAR v7). Landfill emissions from 19 solid waste disposal sites across 12 cities are assigned prior emissions using estimates based on high-resolution GHGSat observations.

Our inversion improves agreement with the blended TROPOMI data, GOSAT data, and available surface observations. We estimate Indian methane emissions for 2021 at 34 (32–39) Tg/year, 15% higher than prior estimates. The anthropogenic posterior emission is 31 (30 – 37) Tg/year, 67% higher than UNFCCC reported values, consistent with previous studies such as Janardanan et al. (2020), Zhang et al. (2021), and Belikov et al. (2024). Compared to the prior estimate, we find higher emissions from landfills and the oil & gas sector, while coal emissions are found to be lower. An analysis of 12 Indian cities reveals that emissions in 3 cities align with prior estimates, while 8 cities exhibit significantly higher emissions. In these 8 cities, waste management (solid waste and wastewater) contributes most to total emissions. Additionally, GHGSat data indicate that landfill emissions account for 10% to 50% of emissions in these cities, highlighting the critical role of solid waste management in reducing emissions.

How to cite: Lama, S., Maasakkers, J. D., Zhang, X., Varon, D. J., Sulprizio, M. P., Estrada, L. A., Balasus, N., Parker, R. J., and Aben, I.: Evaluating national & urban Indian methane emissions using satellites , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17010, https://doi.org/10.5194/egusphere-egu25-17010, 2025.

EGU25-17057 | ECS | Orals | AS3.24

Investigating Indian methane emission using TROPOMI retrievals and WRF-GHG modelling framework 

Thara Anna Mathew, Dhanyalekshmi Pillai, Monish Vijay Deshpande, Vishnu Thilakan, and Sanjid Backer Kanakkassery

Methane (CH4) has a significant global warming potential and a short atmospheric lifetime, making it a critical target for climate change mitigation. In India, the primary contributors to methane emissions are domestic ruminants, fossil fuels, waste management, rice cultivation, and wetlands. In the present study, we explore the column-averaged dry-air mixing ratio measurements of methane (XCH) from the TROPOMI (Tropospheric Monitoring Instrument) aboard the ESA Copernicus Sentinel-5 Precursor satellite and the methane simulations from Weather Research and Forecasting model coupled with Chemistry (WRF-Chem-GHG) to quantify the Indian region methane emission. The investigation focuses on the seasonal and spatial variations of the anthropogenic component of methane over India and compares them with simulations to assess the uncertainties in the current understanding. An inversion analysis utilising these satellite observations will be presented to offer critical insights into current emission trends and improvements in emission inventories over India.

How to cite: Mathew, T. A., Pillai, D., Deshpande, M. V., Thilakan, V., and Kanakkassery, S. B.: Investigating Indian methane emission using TROPOMI retrievals and WRF-GHG modelling framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17057, https://doi.org/10.5194/egusphere-egu25-17057, 2025.

EGU25-17625 | ECS | Posters on site | AS3.24

A ground-based remote sensing measurement network designed to infer net emission of CO2 and methane from the City of Edinburgh 

William Morrison, Jerome Woodwark, Douglas Finch, and Paul Palmer

Reducing emissions of greenhouse gases (GHGs) from urban areas – currently accounting for 70% of the global budget – are an integral part of the solution to meet net zero targets (IPCC, 2022). As part of the GEMINI+Edinburgh project (GHG Emissions Monitoring network to Inform Net-zero Initiatives +Edinburgh, Kurganskiy et al., 2025) we have developed an observational framework to determine long-term trends in GHG emissions from the City of Edinburgh, Scotland.

To determine these emissions, we use column concentrations of CO2 and methane retrieved from six EM27/SUN Fourier transform solar absorption spectrometers (“EM27”, Bruker GmbH, Germany) deployed in a ring around Edinburgh with 5 – 8 km separation. The spectrometers use the sun as their open-path source to measure solar radiation (4000 - 12000 cm cm-1, 0.5 cm-1 spectral resolution) from which we retrieve column abundances of CO2, methane, CO, O2 and H2O. We apply an upwind-downwind mass balance approach to the data collected from these six spectrometers to estimate city-wide net emissions. Spatial variations in near-surface wind fields are captured by eight automatic weather stations (Vaisala WXT530) and sonic anemometers (Gill WindSonic 75) co-located with each EM27 and on additional tall buildings.

We have developed methods to ensure that GEMINI+Edinburgh delivers long-term (O10 year) and reliable measurements to enable reliable CO2 and methane emission trends. As delivered, the EM27 is not weatherproof and not designed for long-term outdoor and unsupervised operation. To overcome these challenges, we have encased each instrument in a purpose-built weatherproof enclosure (Karn Scientific Ltd., Edinburgh). We demonstrate the enclosure performance by using co-located measurements from (un)enclosed EM27s during a series of intercomparisons and characterising the effect of the enclosure’s BK7 glass window. We employ a data processing workflow to enable long-term automated operation of the network, including an instrument meta data system, data transfer, processing, quick-look diagnostics plots, and archiving.

 

IPCC, 2022: Climate Change 2022: Mitigation of Climate Change. Contribution of Working Group III to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change. doi: 10.1017/9781009157926

Kurganskiy, A., Feng, L., Humpage, N., Palmer, P. I., Woodwark, A. J. P., Doniki, S., Weidmann, D., 2025. The Greenhouse gas Emission Monitoring network to Inform Net-zero Initiatives UK (GEMINI-UK): network design, theoretical performance, and initial data. Submitted to Atmospheric Measurement Techniques.

 

How to cite: Morrison, W., Woodwark, J., Finch, D., and Palmer, P.: A ground-based remote sensing measurement network designed to infer net emission of CO2 and methane from the City of Edinburgh, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17625, https://doi.org/10.5194/egusphere-egu25-17625, 2025.

EGU25-17804 | Posters on site | AS3.24

Towards Shipborne Emission Monitoring and Satellite Validation of CO2, CH4, CO, and NO2 Through Simultaneous Columnar and In Situ Observations 

Astrid Müller, Hiroshi Tanimoto, Matthias Max Frey, Vincent Enders, Prabir K. Patra, Takafumi Sugita, Ralph Kleinschek, Karolin Voss, André Butz, Isamu Morino, Shin-ichiro Nakaoka, Hideki Nara, and Toshinobu Machida

Precise observations of anthropogenic greenhouse gas (GHG) and air pollutant emissions are essential for improving emission inventories and evaluating the potential of their reduction, supporting the global stocktake. The global coverage of ship-, aircraft-, and ground-based observations by public and private networks, together with satellite observations of GHGs and other trace gases, is expanding. However, observations and reference data over ocean and coastal regions remain scarce.

We conduct continuous cargo ship-based observations with a novel semi-automatic Fourier transform infrared (FTIR) spectrometer combined with a VIS (visible spectral range) grating spectrometer to measure the column-averaged dry-air mole fractions of carbon dioxide (XCO2), methane (XCH4), carbon monoxide (XCO) and the vertical column densities of nitrogen dioxide (VCDNO2). Combined with simultaneous in situ observations (CO2, CH4, CO, NO2), we aim to constrain anthropogenic emissions and contribute to a satellite validation framework for upcoming satellite missions like the Global Observing SATellite for Greenhouse gases and Water cycle (GOSAT-GW) or the Copernicus Anthropogenic Carbon Dioxide Monitoring (CO2M) mission. These missions are designed to identify and monitor anthropogenic emissions by observing the GHG CO2 and the short-lived combustion tracer NO2 simultaneously. With our novel setup, we have the capability to validate these concurrent observations.

The cargo ship operates along major anthropogenic emission sources on Japan’s coast between the Tokyo metropolitan area and the island of Kyushu in the southwest with a weekly round-trip schedule. We present the initial analysis results of the combined columnar and in situ observations for emission plume detection and inventory validation, and provide perspectives of the setup for satellite validation and anthropogenic emission monitoring.

How to cite: Müller, A., Tanimoto, H., Frey, M. M., Enders, V., Patra, P. K., Sugita, T., Kleinschek, R., Voss, K., Butz, A., Morino, I., Nakaoka, S., Nara, H., and Machida, T.: Towards Shipborne Emission Monitoring and Satellite Validation of CO2, CH4, CO, and NO2 Through Simultaneous Columnar and In Situ Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17804, https://doi.org/10.5194/egusphere-egu25-17804, 2025.

EGU25-18300 | Orals | AS3.24

Satellite-based Detection and Quantification of Methane Emissions from Energy and Waste Sectors in Iran 

Hossein Maazallahi, Fathollah Pourfayaz, Itziar Irakulis-Loitxate, and Maryam Avishan

Methane is the second most potent anthropogenic source greenhouse gas (GHG), with a global warming potential of approximately 84 times that of carbon dioxide over a 20-year period. Methane accounts for nearly one-third of current global warming, and its emission mitigations are critical actions for slowing down global warming in the short time period. In Iran, methane emissions from the energy and waste sectors significantly contribute to the country's total GHG emissions. According on the report of the International Energy Agency (IEA) in 2024, oil and gas (O&G) production in Iran resulted in the release of approximately 6 million metric tons of methane, ranking the country among the top three global emitters. Based on limited data, it was previously estimated that 3.84 million metric of methane is released from Iran’s waste sector. However, with limited data and measurement-based campaigns, these estimates need refinements. National inventories further highlight substantial emissions from waste management practices, underscoring the need for effective mitigation strategies, which at the first step requires framing the level of emissions nationwide.

This study utilizes satellite remote sensing data, generated by UNEP's IMEO (United Nations Environment Programme International Methane Emissions Observatory) through its Methane Alert and Response System (MARS) and available via its Eye on Methane data platform, to quantify methane emissions from O&G and waste-related activities in Iran. Methane quantifications were derived by integrating data from multiple satellite platforms, including the Earth Surface Mineral Dust Source Investigation (EMIT) operated by National Aeronautics and Space Administration (NASA), Sentinel-5P and Sentinel-2 from the European Space Agency (ESA), Landsat (jointly operated by NASA and the US Geological Survey), and the Environmental Mapping and Analysis Program (EnMAP) of the German Aerospace Center (DLR). A total of 110 emission sources from O&G infrastructures were identified and visually verified through Google Earth, subsequently integrated into the MARS system for continuous monitoring. This study provides nationwide observations of methane emissions from top emitters, which can be used for reporting and emission mitigation in Iran.

How to cite: Maazallahi, H., Pourfayaz, F., Irakulis-Loitxate, I., and Avishan, M.: Satellite-based Detection and Quantification of Methane Emissions from Energy and Waste Sectors in Iran, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18300, https://doi.org/10.5194/egusphere-egu25-18300, 2025.

EGU25-18869 | Posters on site | AS3.24

Assessing the Capability of Sentinel-5P (TROPOMI) NO2 Measurements to Monitor Point Source CO2 Emissions 

Jia Chen and Vigneshkumar Balamurugan

Monitoring greenhouse gas (GHG) emissions is crucial for mitigating global warming and the associated climate change. Various satellite missions are dedicated to measuring CO2 globally, demonstrating their capability to detect GHG emission hotspots and quantify emissions effectively. However, due to the limited revisit frequency and spatial coverage of contemporary high-resolution CO2 monitoring missions such as OCO-2 and OCO-3, continuous daily monitoring of CO2 emissions from specific sources remains challenging. To overcome these limitations, combining data from different satellite missions is a promising approach. Missions such as TROPOMI provide daily monitoring of various trace gas concentrations (e.g., NO2, CO, SO2). 

CO2 is emitted from sources along with other species, such as CO and NO2. Therefore, it is possible to infer CO2 emissions from the emissions of co-emitted species. Compared to other co-emitted species, NO2 has a relatively short lifetime of a few hours to a day, which makes it easier to distinguish enhancements from background concentrations.

Individual power plant CO2 emissions are not reported in many parts of the world. Some countries, such as India, have started reporting daily coal consumption data for individual power plants since 2022. The amount of coal consumed can be used to estimate CO2 emissions due to its strong linear correlation with CO2 emissions. To overcome the limitations in reporting CO2 emissions from power plants globally, we evaluate the potential of TROPOMI NO2 measurements for monitoring CO2 emissions. This is achieved by comparing the derived daily NO2 emissions with the daily coal consumption of individual power plants in India.

A Gaussian plume (GP) model accounting for NO2 lifetime was used to estimate the daily NO2 emissions along with the NO2 lifetime. In our study, we also attempted to address a key issue found in previous literature: the presence of an additional emission source downwind of the main source can render both NO2 emission estimates and NO2 lifetime estimates unreliable. We address this issue by simultaneously modeling and fitting the NO2 emissions and NO2 lifetime of the additional source, in conjunction with the main power plant GP inversion framework.

Our findings show a moderate to good linear relationship between daily NO2 emissions and daily coal consumption of individual power plants. This suggests that TROPOMI NO2 measurements can effectively support the monitoring of CO2 emissions. Finally, this study highlights that upcoming satellite missions monitoring NO2 can be used, along with GHG satellite measurements, for regular monitoring of carbon emissions.

How to cite: Chen, J. and Balamurugan, V.: Assessing the Capability of Sentinel-5P (TROPOMI) NO2 Measurements to Monitor Point Source CO2 Emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18869, https://doi.org/10.5194/egusphere-egu25-18869, 2025.

EGU25-19252 | ECS | Posters on site | AS3.24

Global Detection and Analysis of Methane Plumes in 2024 Using TROPOMI Observations 

Ana Isabel Lopez Norena, Joannes D. Maasakkers, Berend Schuit, Solomiia Kurchaba, Matthieu Dogniaux, Shubham Sharma, and Ilse Aben

Methane (CH₄) is a potent greenhouse gas that plays a significant role in global warming, with over 60% of CH₄ emissions attributed to human activities. A substantial portion of these anthropogenic emissions originates from a small number of super-emitters, making their monitoring crucial for understanding emission patterns and implementing targeted mitigation strategies. The TROPOspheric Monitoring Instrument (TROPOMI), onboard the ESA Sentinel-5P satellite, provides daily global observations of methane mixing ratios at high spatial resolution, enabling the detection and analysis of plumes associated with these super-emitters.

To detect methane plumes globally in TROPOMI data, a two-step machine learning pipeline is employed, with weekly results now officially part of the Copernicus Atmosphere Monitoring Service (CAMS) products. The first step utilizes a convolutional neural network to identify plume-like structures in the methane data. A support vector classifier is then applied to filter out retrieval artifacts, ensuring the accurate identification of true methane emissions. Detected plumes are categorized by emission rate, and human experts conduct final verifications. In this study, we present the results for the full year 2024, during which a total of 2,311 methane plumes were identified, providing a comprehensive overview of global super-emitter activity. Preliminary analysis based on bottom-up emission inventories shows that the majority of plumes are associated with oil and gas production, landfills, and coal mining activities.

This study provides a detailed analysis of methane plume detections for 2024, highlighting temporal variations and regional hotspots. By focusing on the detected plumes rather than the detection methodology, this work delivers valuable insights into the spatial and temporal dynamics of methane emissions. The findings contribute to the growing body of knowledge required to address super-emitter mitigation and support informed policymaking for reducing global methane emissions.

How to cite: Lopez Norena, A. I., Maasakkers, J. D., Schuit, B., Kurchaba, S., Dogniaux, M., Sharma, S., and Aben, I.: Global Detection and Analysis of Methane Plumes in 2024 Using TROPOMI Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19252, https://doi.org/10.5194/egusphere-egu25-19252, 2025.

EGU25-19645 | Posters on site | AS3.24

Using satellite data and atmospheric inversion modelling to estimate CO2 budgets in nationally relevant scales: project FICOCOSS 

Tuula Aalto, Laia Amoros, Otto Lamminpää, Hannakaisa Lindqvist, Anteneh Mengistu, Antti Mikkonen, Maija Pietarila, Antti Pihlajamäki, Johanna Tamminen, Aki Tsuruta, and Rebecca Ward

Nations are accountable for their GHG emissions, and since the Paris Agreement, progress towards national emission reductions is tracked. To facilitate this, atmospheric inversion modelling is employed as the state of-the-art means to collect information from GHG observations to quantify sources and sinks. High-resolution estimation of GHG fluxes in Northern High Latitudes greatly benefits from developments in satellite data analysis and computational methods. FICOCOSS project develops these methods and assimilates OCO-2 satellite data in atmospheric inversion models (CIF-FLEXPART, CIF-TM5-MP) to estimate CO2 sources and sinks. We prepare for the high intensity CO2M satellite by developing more efficient computational methods related to e.g. large error covariance matrix operations and satellite retrieval processing. Preliminary findings indicate that more efficient methods can be developed for using satellite CO2 data in high resolution inversions.

How to cite: Aalto, T., Amoros, L., Lamminpää, O., Lindqvist, H., Mengistu, A., Mikkonen, A., Pietarila, M., Pihlajamäki, A., Tamminen, J., Tsuruta, A., and Ward, R.: Using satellite data and atmospheric inversion modelling to estimate CO2 budgets in nationally relevant scales: project FICOCOSS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19645, https://doi.org/10.5194/egusphere-egu25-19645, 2025.

EGU25-20046 | Orals | AS3.24

Simultaneous retrieval of trace gases and aerosol using RemoTAP – the global orbit ensemble study for the CO2M mission 

Sha Lu, Guangliang Fu, Jochen Landgraf, and Otto Hasekamp

In the support of the Copernicus Anthropogenic Carbon Dioxide Monitoring (CO2M) mission, SRON Netherlands Institute for Space Research developed the Remote sensing of Trace gas and Aerosol Product (RemoTAP) algorithm. RemoTAP is able to achieve simultaneous retrieval of trace gases and aerosol using measurements from the Multi-Angle Polarimeter (MAP) and CO2I Imager aboard the CO2M mission. At the same time, it has the capability to perform the retrieval of trace gas from only CO2I measurements.

This study evaluates the performance of RemoTAP for combined MAP-CO2I and CO2I-only retrievals, respectively. We base our evaluation on synthetic CO2M measurements simulated for realistic atmospheric (aerosol, cirrus), surface, geometry conditions. MAP-CO2I retrieval method can reduce the regional bias in column-averaged dry-air mole fraction of CO2 (XCO2) by a factor of 3. It shows that only by the inclusion of MAP measurements, the large aerosol-induced biases can be mitigated, resulting in the retrievals that meet the mission requirement (precision <0.7 ppm and bias <0.5 ppm).

In addition, RemoTAP has other functions to further improve the accuracy of trace-gas retrievals. It is able to retrieve cirrus at pixels with an optically thin layer of cirrus cloud. Instead of retrieving cirrus, we also provide the option to filter cirrus-contained pixels by non-scattering retrieval, which results in more accurate XCO2 retrievals but with less yield. To account for the uncertainties in surface pressure, which is related to the calculation of dry air column, RemoTAP has the option to retrieve O2 column which is proportional to dry air column from measurements of NIR band. Besides, RemoTAP retrieves Solar-Induced chlorophyll Fluorescence (SIF) over vegetation surface. The retrieval of cirrus, surface pressure/O2 column and SIF is performed simultaneously with the retrieval of other physical parameters, and the error induced by these factors in the XCO2 retrieval can be mitigated. Finally, we developed a method to perform bias correction and quality filtering using a neural network approach.

How to cite: Lu, S., Fu, G., Landgraf, J., and Hasekamp, O.: Simultaneous retrieval of trace gases and aerosol using RemoTAP – the global orbit ensemble study for the CO2M mission, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20046, https://doi.org/10.5194/egusphere-egu25-20046, 2025.

EGU25-1546 | Orals | AS3.25

Background, urban, and industrial NO2 estimated from TEMPO satellite observations 

Vitali Fioletov, Debora Griffin, Chris McLinden, Xiaoyi Zhao, Caroline Nowlan, and Gonzalo Gonzalez Abad

The hourly tropospheric NO2 vertical column density (VCD) values measured by TEMPO were used to study the NO2 diurnal andseasonal variability in 34 urban areas over North America and the Caribbean during the period from August 2023 to October 2024. A recently developed algorithm (Fioletov et al., 2024) isolated three components in tropospheric NO2 data: background NO2, NO2 from urban emissions, and from industrial point sources, and then each of these components was analyzed separately. The method is based on fitting satellite data by a statistical model with empirical plume dispersion functions driven by a meteorological reanalysis. Population density and surface elevation data as well as coordinates of major industrial sources were used in the analysis. The background component demonstrated a clear diurnal cycle with a maximum in the early morning and the minimum in the late afternoon. The urban and industrial components, expressed as total NO2 mass in urban and industrial plumes, did not show any obvious diurnal cycle in most areas. Only the Los Angeles and Mexico City urban components demonstrated a clear cycle with a maximum in the late morning and a minimum in the late afternoon. Differences between workday and weekend NO2 levels were also studied. Urban plume NO2 values on Sundays were typically 30%–60% less than workday plume values throughout the day.  The exception was Havana, where the difference between working day and Sunday values ​​was only 15%.

 

Fioletov, V., McLinden, C. A., Griffin, D., Zhao, X., and Eskes, H.: Global seasonal urban, industrial, and background NO2 estimated from TROPOMI satellite observations, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2024-1991, 2024.

How to cite: Fioletov, V., Griffin, D., McLinden, C., Zhao, X., Nowlan, C., and Gonzalez Abad, G.: Background, urban, and industrial NO2 estimated from TEMPO satellite observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1546, https://doi.org/10.5194/egusphere-egu25-1546, 2025.

EGU25-6723 | Orals | AS3.25

Complementarity of GEO, LEO, and Lagrange-1 Point Satellite Aerosol Observations  

Omar Torres, Changwoo Ahn, Hiren Jethva, and Diego Loyola

Currently deployed (GEMS, TEMPO) and soon-to-be launched (S4-UVN) sensors constitute the first GEO satellite constellation for Air Quality observations in the northern hemisphere. The simultaneous availability of similar observations from platforms at LEO and L1 orbital configurations offers a unique  opportunity for the integration of a quasi-global  Air Quality observing system. In this presentation, we will discuss specific aerosol events to show the complementary nature of GEO aerosol observations and those of LEO (S5P-TROPOMI and S5-UVNS), and Langrange1-EPIC measurements. Integrated GEO, LEO and L1 observations will be used to demonstrate inter-instrument synergy for sensor calibration transfer, and the understanding of  the nature of local events in regional and global contexts.   

How to cite: Torres, O., Ahn, C., Jethva, H., and Loyola, D.: Complementarity of GEO, LEO, and Lagrange-1 Point Satellite Aerosol Observations , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6723, https://doi.org/10.5194/egusphere-egu25-6723, 2025.

Aerosols in the atmosphere affect radiative forcing directly and indirectly. The single scattering albedo(SSA) of the aerosols describs it absorbs or scatters photons reaching the aerosol layers. Therefore, it is significant to observe SSA with the total burden (i.e., aerosol optical depth) to understand the role of aerosols in the atmosphere. Satellite-based remote sensing data provides global aerosol information. However, the accuracy of a few aerosol parameters (e.g., SSA) is not yet sufficient due to the lack of information in the measurements. Despite its limited spatial coverage, ground-based remote sensing measurements have provided reliable aerosol information as it is less affected by surface reflectance and can measure multiple angles. Previous studies developed combination retrieval techniques that use both ground and satellite measurements to complement the limitations of each method. In this study, we assessed the SSA products from ground and satellite instruments over Asia, where large amounts of aerosol persist throughout the year. We also introduce a combination technique using the EPIC and SMART-s measurements to provide reliable SSA data in the ultraviolet wavelengths.
This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)

How to cite: park, S.: Spatiotemporal variability of single-scattering albedo over Asia using ground- and satellite-based remote sensing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7802, https://doi.org/10.5194/egusphere-egu25-7802, 2025.

EGU25-8489 | Orals | AS3.25

Atmospheric composition from the Geostationary Interferometric Infrared Sounder (GIIRS) on board FengYun satellite: First two years of observations 

Zhao-Cheng Zeng, Mengya Sheng, Shangyi Liu, Shan Han, Wei Wang, Lu Lee, Chengli Qi, and Feng Lu

The Geostationary Interferometric Infrared Sounder (GIIRS) on board China’s FengYun-4 satellite series provides a unique opportunity to monitor the tropospheric composition over Asia using hyperspectral infrared observations from a geostationary orbit. In this study, we retrieve atmospheric carbon monoxide (CO), ammonia (NH3), formic acid (HCOOH) and ozone (O3) for the first two years from July 2022 to June 2024 using the FengYun Geostationary satellite Atmospheric Infrared Retrieval (FY-GeoAIR) algorithm. GIIRS measures these atmospheric compounds both day and night with a temporal resolution of 2 hours and a spatial resolution of 12km at nadir. The spatial patterns, seasonal and diurnal variations of these atmospheric compounds over Asia are analyzed using the FY-4B/GIIRS retrievals. In particular, we focus on a case study of the strong emissions from forest fires over the Indochina Peninsula (ICP) in spring due to the agricultural practice of slash-and-burn. The results show that the spatial and temporal variations of wildfire enhancements of CO, NH3 and HCOOH from Southeast Asia are well captured by the FY-4B/GIIRS. In addition, the FY-4B/GIIRS retrievals are validated with ground-based observations of CO and NH3 and compared with model simulations. Our study demonstrates the potential of GIIRS data to improve our understanding of the spatial and temporal variations of important trace gas pollutants over Asia.

How to cite: Zeng, Z.-C., Sheng, M., Liu, S., Han, S., Wang, W., Lee, L., Qi, C., and Lu, F.: Atmospheric composition from the Geostationary Interferometric Infrared Sounder (GIIRS) on board FengYun satellite: First two years of observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8489, https://doi.org/10.5194/egusphere-egu25-8489, 2025.

EGU25-9038 | ECS | Orals | AS3.25

Sensitivity of GEMS formaldehyde vertical columns to a priori profile for air mass factor during ASIA-AQ 

Gitaek Lee, Rokjin Park, Jaein Jeong, Seungun Lee, Hyeonmin Kim, and Hyeong-Ahn Kwon

Formaldehyde (HCHO), a byproduct of volatile organic compound (VOC) oxidation, is commonly used to constrain VOC emissions in chemical transport model (CTM) simulations through its vertical column density (VCD). While satellite observations provide extensive pollution maps of HCHO VCDs, they often involve significant uncertainties in vertical column retrievals, requiring continuous evaluation against ground-based observations. This study evaluates long-term GEMS HCHO products (version 3) by comparing them with Pandora HCHO VCDs from 2022 to 2024. GEMS HCHO VCDs are 10–40% lower but present good agreement (r=0.6–0.76) with Pandora observations, except for regions (Sapporo, Kobe, and Dhaka), where few samples are available due to the limited GEMS scan schedule. We examine the sensitivity of HCHO VCDs using air mass factors (AMFs) with a priori profiles from a five-CTM ensemble model with a fine spatial resolution (9 km) and updated emissions during the ASIA-AQ campaign, instead of using GEMS a priori profile. The ensemble model demonstrates improved agreement (r=0.83) with DC-8 observations compared to the GEMS a priori profile (r=-0.54), reducing overestimations of surface HCHO concentrations. Using vertical shape factors from ensemble model profiles increases AMFs by 20% in the morning at Suwon, improving agreements with MAX-DOAS observations (NMB= 86% to 33%). Our work highlights the need for continuous updates to a priori profile simulations for precise HCHO retrievals.

How to cite: Lee, G., Park, R., Jeong, J., Lee, S., Kim, H., and Kwon, H.-A.: Sensitivity of GEMS formaldehyde vertical columns to a priori profile for air mass factor during ASIA-AQ, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9038, https://doi.org/10.5194/egusphere-egu25-9038, 2025.

Accurate retrieval of tropospheric NO₂ columns relies on precise knowledge of stratospheric NO₂ columns, which can be derived from chemical transport models (CTMs) or estimated through interpolation from regions with minimal tropospheric NO₂ contributions. However, both approaches have their limitations: stratospheric NO₂ fields from CTMs and satellite retrievals often contain biases, and small-scale spatial variations in stratospheric NO₂ can diminish the accuracy of interpolated estimates. These deficiencies can result in significant errors in stratosphere-troposphere separation (STS). In this presentation, we introduce a novel STS approach that combines retrievals from both UV and visible spectra. By leveraging the differing sensitivities of UV and visible wavelengths to tropospheric NO₂, our method provides a more accurate determination of stratospheric and tropospheric NO₂ columns. We will demonstrate the effectiveness of this technique using observations from TROPOMI, GEMS, and TEMPO, showcasing its potential to enhance the accuracy of STS in satellite-based NO₂ retrievals.

How to cite: Yang, K., Wei, Z., and Flynn, L. E.: Retrievals of Stratospheric and Tropospheric Nitrogen Dioxide (NO2) Columns from Satellite Ultraviolet and Visible Spectral Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10855, https://doi.org/10.5194/egusphere-egu25-10855, 2025.

EGU25-11665 | Orals | AS3.25 | Highlight

Investigating air pollution and climate change on the African continent: a Global South perspective 

Pieternel Levelt and the MEASMA-AfricaGEO team

In the next few decades a large increase in population is expected to occur on the African continent, leading to a doubling of the current population, which will reach 2.5 billion by 2050. At the same time, Africa is experiencing substantial economic growth. As a result, air pollution and greenhouse gas emissions will increase considerably with significant health impacts to people in Africa. In the decades ahead, Africa’s contribution to climate change and air pollution will become increasingly important. The time has come to determine the evolving role of Africa in global environmental change.  

The Committee on Earth Observation Satellites (CEOS) envisions an Atmospheric Composition Virtual Constellation that includes existing polar satellites and now geostationary satellites in the Northern Hemisphere: GEMS over Asia (launch 2022); TEMPO over the USA (launch 2023) and Sentinel 4 over Europe to be launched in the 2024 timeframe. However, there are currently no geostationary satellites envisioned over the Global South, specifically Africa and South-America, where we expect the largest increase in emissions in the decades to come. Current initiatives are a combination of a Geostationary satellite over the Middle-East and Norther Africa (MEASMA) and a Geostationary satellite over Sub-Sahara Africa.

In this paper the scientific need for geostationary satellite measurements over Africa will be described, partly based on several recent research achievements related to Africa using space observations and modeling approaches, as well as first assessments using the GEMS data over Asia, and TEMPO over the USA. Our ambition is to develop an integrated community effort to better characterize air quality and climate-related processes on the African continent. 

How to cite: Levelt, P. and the MEASMA-AfricaGEO team: Investigating air pollution and climate change on the African continent: a Global South perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11665, https://doi.org/10.5194/egusphere-egu25-11665, 2025.

EGU25-13335 | ECS | Orals | AS3.25

Diurnal emission fluxes and lifetimes of nitrogen oxide estimated from GEMS observations 

Kezia Lange, Andreas Richter, John P. Burrows, Hyunkee Hong, and Hartmut Bösch

Satellite observations of nitrogen dioxide (NO2) have been widely used to estimate nitrogen oxide (NOx) emissions and lifetimes, as well as to analyze their weekday or seasonal variability. The TROPOspheric Monitoring Instrument (TROPOMI), with its high spatial resolution of 3.5 x 5.5 km2, has given new opportunities to disentangle and analyze NOx sources. However, instruments in low-earth orbits usually provide only one measurement per day and location.

The Geostationary Environmental Monitoring Spectrometer (GEMS), launched in February 2020, provides hourly daytime observations of NO2 with a spatial resolution of 3.5 x 8 km2 over a large part of Asia. This opens new opportunities to quantify the diurnal variability of NOx emissions and lifetime from space.

In this study, 4 years of GEMS IUP-UB tropospheric NO2 columns have been analyzed together with ERA5 wind, temperature, and ozone data to estimate NOx emissions and lifetime for several emission sources within the GEMS domain. The estimated emissions are compared to emission inventories and TROPOMI-based emission estimates. The high temporal resolution of GEMS with up to 10 observations per day ensures robust data availability, allowing also for the analysis of short-time variability. Using the dataset of 4 years from 2021 to 2024, hourly estimates are of good quality and are used to quantify the diurnal variability of NOx emissions and lifetime.

How to cite: Lange, K., Richter, A., Burrows, J. P., Hong, H., and Bösch, H.: Diurnal emission fluxes and lifetimes of nitrogen oxide estimated from GEMS observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13335, https://doi.org/10.5194/egusphere-egu25-13335, 2025.

EGU25-13818 | Orals | AS3.25

TEMPO Provisional Validation 

Mike Newchurch, Ron Cohen, Jim Szykman, Brad Pierce, Xiong Liu, Dave Flittner, Barron Henderson, Laura Judd, and Kelly Chance

The Tropospheric Emissions: Monitoring of Pollution (TEMPO) Instrument is a NASA Earth Venture Instrument (EV-I) project selected on November 8, 2012 in response to the second Stand Alone Mission of Opportunity Notice.  The Smithsonian Astrophysical Observatory (SAO) under the direction of the TEMPO Principal Investigator (Pl) at SAO is the lead organization for the project, responsible for TEMPO instrument development data products and science.

The Tropospheric Emissions: Monitoring of Pollution (TEMPO) Instrument [Zoogman et al., 2017] is dispersive spectrometer designed to measure solar back-scatter light in the ultraviolet (UV) and visible (VIS) spectral ranges.  The TEMPO instrument draws on several decades of heritage spectrometers (GOME, SCIAMACHY, OMI, TROPOMI, GOME-2, and OMPS; Burrows et al., 1999; Bovensmann et al., 1999; Levelt et al., 2018; Munro et al., 2016; Flynn et al., 2014) operating in low-earth-orbit (LEO), adapting and applying the technology for a geostationary satellite mission designed to monitor air quality over North America.  TEMPO takes advantage of a commercial geostationary host spacecraft to make the first North American tropospheric trace gas measurements from GEO.  Novel to TEMPO are hourly measurements (or less) during daylight hours at high spatial resolution (2 × 4.75 km2 at the center of field of regard) enabling the quantification of spatial and temporal variations of trace gases and aerosols at scales relevant for understanding urban air quality in the troposphere.

As part of the PI-led TEMPO Science Team, validation of Level 2 NO2, HCHO and O3 column data products recently achieved provisional status in the TEMPO Validation Plan (NASA, 2023).  This effort was completed under a best-efforts approach leveraging measurement and modeling assets and many scientist volunteers’ hours to produce a draft validation report currently under review.  This talk will provide an overview of the TEMPO validation effort, specifically highlighting the range of contribution from the ad-hoc TEMPO validation team and the resulting validation of the TEMPO gas products.

How to cite: Newchurch, M., Cohen, R., Szykman, J., Pierce, B., Liu, X., Flittner, D., Henderson, B., Judd, L., and Chance, K.: TEMPO Provisional Validation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13818, https://doi.org/10.5194/egusphere-egu25-13818, 2025.

EGU25-14037 | ECS | Orals | AS3.25

Aerosol Fine-Mode-Fraction Retrieval from GEO-KOMPSAT-2A/AMI using a Deep Neural Network and Spectral Deconvolution Algorithm 

Minseok Kim, Jhoon Kim, Seoyoung Lee, Hyunkwang Lim, and Yeseul Cho

Aerosol size information is important to the understanding of aerosol dynamics, which change rapidly over Asia, with size retrieval from geostationary satellite observations being vital. In this study, a deep neural network model was trained using Advanced Meteorological Imager (AMI) level 1b observations, AMI aerosol products, and observation geometries to retrieve the aerosol optical depth (AOD), Ångström exponent (AE), and spectral derivatives of AE (AE′). The fine-mode fraction (FMF) was calculated with a spectral deconvolution algorithm using retrieved AE and AE′ when AOD > 0.2. The retrieved aerosol products were validated using AERONET (AOD at 550 nm: R = 0.829, RMSE = 0.241, MBE = –0.053; AE: R = 0.723; RMSE = 0.235; MBE = 0.005; FMF: R = 0.814; RMSE = 0.083; MBE = 0.011). Case studies of dust-transport and wildfire events in Asia revealed that the retrieved aerosol size products may be used for analysis of sudden pollution events. Monthly average FMF values in Asia were consistent with previous studies, confirming that the retrieved FMF is useful for seasonal aerosol property analysis. Results of this study indicate the potential for comprehensive analysis of aerosol properties in Asia using continuous aerosol size data from geostationary Earth orbit satellite observations.

How to cite: Kim, M., Kim, J., Lee, S., Lim, H., and Cho, Y.: Aerosol Fine-Mode-Fraction Retrieval from GEO-KOMPSAT-2A/AMI using a Deep Neural Network and Spectral Deconvolution Algorithm, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14037, https://doi.org/10.5194/egusphere-egu25-14037, 2025.

EGU25-14296 | Orals | AS3.25

Tropospheric Emissions: Monitoring of Pollution (TEMPO) nitrogen dioxide and formaldehyde retrievals 

Gonzalo Gonzalez Abad, Caroline Nowlan, Kelly Chance, Xiong Liu, James Carr, Heesung Chong, John E. Davis, Jean Fitzmaurice, David E. Flittner, Jeffrey Geddes, Barron Henderson, Weizhen Hou, John Houck, Laura Judd, Hyeong-Ahn Kwon, K. Emma Knowland, Christopher Chan Miller, Ewan O'Sullivan, Junsung Park, and Brad Pierce and the TEMPO team

We present the status of the Tropospheric Emissions: Monitoring of Pollution (TEMPO) nitrogen dioxide (NO2) and formaldehyde (HCHO) retrievals one year after their public release. After multiple version updates, the TEMPO Level 2 NO2 and HCHO products have undergone significant enhancements to improve the performance and accuracy of the slant column retrievals, air mass factor calculations and post-processing corrections. Upcoming version 4 will include improved destriping for NO2 and background for HCHO corrections. We illustrate the performance of both retrievals, evaluating their fitting uncertainty and showing comparisons with independent correlative measurements and other satellite products showcasing small noise levels, good accuracy, remarkable correlation and well quantified biases. We continue by illustrating the capacity of TEMPO products focusing on different case studies showing TEMPO’s high temporal and spatial resolution. We finalize discussing aspects of the retrievals subject to improvement, our strategies to enhance their performance and the development of near real time pipelines.

How to cite: Gonzalez Abad, G., Nowlan, C., Chance, K., Liu, X., Carr, J., Chong, H., Davis, J. E., Fitzmaurice, J., Flittner, D. E., Geddes, J., Henderson, B., Hou, W., Houck, J., Judd, L., Kwon, H.-A., Knowland, K. E., Chan Miller, C., O'Sullivan, E., Park, J., and Pierce, B. and the TEMPO team: Tropospheric Emissions: Monitoring of Pollution (TEMPO) nitrogen dioxide and formaldehyde retrievals, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14296, https://doi.org/10.5194/egusphere-egu25-14296, 2025.

The Tropospheric Emissions: Monitoring of Pollution (TEMPO) is part of the global geostationary air quality monitoring constellation. It is the first satellite instrument in geostationary orbit dedicated to monitor air pollutants across North America. Its observational coverage extends from Mexico City to the Canadian oil sands and from the Atlantic Ocean to the Pacific, with hourly measurements at a resolution approaching neighborhood scale. Following its successful launch in April 2023, TEMPO began nominal operations in October 2023. TEMPO L2 data products (NO2, HCHO, Cloud and total ozone) were made publicly available in May 2024, following the release of Level 1 data in February 2024. As of December 2024, these products have been classified as the Provisional maturity level.

This presentation highlights the evaluation of the TEMPO total ozone (O3TOT) product and introduces improvements to the TEMPO ozone profile (O3PROF) product. We present a comparative analysis of total ozone columns (TOCs) from TEMPO observations against data from other satellite instruments, such as OMPS, OMI, and TROPOMI, as well as ground-based measurements from Pandora, Brewer, and Dobson instruments. Additionally, we present enhancements to the TEMPO O3PROF algorithm, particularly the empirical correction, which is scheduled for release this year. Furthermore, we compare TEMPO tropospheric ozone columns with those from EPIC, OMI, and TROPOMI satellites. Lastly, the TEMPO O3PROF product is evaluated using ground-based observations, including data from the Tropospheric Ozone Lidar Network (TOLNet) and ozonesonde observations.

How to cite: Liu, X. and Park, J. and the TEMPO ozone team: Status of the TEMPO total ozone and ozone profile data products: A comprehensive validation using various satellites and ground-based observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14533, https://doi.org/10.5194/egusphere-egu25-14533, 2025.

EGU25-15013 | ECS | Orals | AS3.25

GEMS Hourly Ozone Data: Enhancing MDA8 Estimates and Reducing Overestimated Health Risks 

Ge Song, Siwei Li, Jia Xing, Jiaxin Dong, and Jie Yang

Accurate estimation of ground-level ozone (O₃) concentration is crucial for assessing its health impacts and devising effective control strategies. Traditional methods relying on polar-orbit satellites offer limited, single-time measurements, failing to capture the significant diurnal variability of O₃. This study utilizes the Geostationary Environment Monitoring Spectrometer (GEMS), a next-generation geostationary satellite, to retrieve hourly O₃ concentrations. The GEMS data not only accurately captures hourly O₃ levels (R² = 0.94) but also significantly enhances the precision of daily maximum 8-hour average (MDA8) O₃ estimates, particularly in semi-urban regions, with an increase in R² by over 0.10 and a reduction in absolute error exceeding 7 μg/m³. Furthermore, our analysis reveals a 30% decrease in O₃-related health risks, with both short-term and long-term mortality rates lower than previous estimates based on polar-orbit satellites. This reduction particularly notable in semi-urban and rural areas, where satellite data is more critical due to the scarcity of ground measurements compared to urban areas. These findings suggest that previous assessments may have overestimated total mortalities and urban-rural spillover effects. Our study highlights the importance of employing high temporal resolution geostationary satellites like GEMS to accurately capture O₃ diurnal variability, providing a robust foundation for health risk assessments and guiding regulatory interventions to address O₃ pollution in China.

How to cite: Song, G., Li, S., Xing, J., Dong, J., and Yang, J.: GEMS Hourly Ozone Data: Enhancing MDA8 Estimates and Reducing Overestimated Health Risks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15013, https://doi.org/10.5194/egusphere-egu25-15013, 2025.

EGU25-15516 | Orals | AS3.25

An advanced aerosol optical depth retrieval algorithm based on an improved scattering angle scheme for Geostationary satellite 

Mansing Wong, Jiaqi Jin, Jing Li, Kwonho Lee, Janet Elizabeth Nichol, and Pw Chan

The Advanced Himawari Imager onboard the Himawari-8/9 geostationary satellite offers a powerful tool for aerosol monitoring at high temporal resolution, with observations available every 10 minutes. Aerosol optical depth (AOD), a key parameter for characterizing aerosols, is commonly retrieved using physics-based algorithms that depend on prior assumptions about surface reflectance and aerosol models. However, these assumptions often fail to account for the complexities of land and atmospheric conditions. This study introduces a novel AOD retrieval algorithm that enhances the accuracy of surface reflectance estimation and aerosol modeling by utilizing time-series geostationary observations and clustering aerosol properties based on precise ground-based measurements. AOD retrievals were performed for the period from 2022 to 2023 over southern China, primarily Guangdong Province, and validated using ground-based measurements from the AErosol RObotic NETwork (AERONET) and the Sun-sky radiometer Observation NETwork (SONET). The results were also compared against aerosol products from the MODerate Resolution Imaging Spectroradiometer (MODIS). The proposed algorithm demonstrated strong agreement with AERONET and SONET observations, achieving a correlation coefficient of 0.74, an RMSE of 0.18, and over 52% of retrievals falling within the expected error (EE) range of ±(0.05 + 15%). By comparison, the AOD products from the Japan Aerospace Exploration Agency (JAXA) had a lower correlation coefficient of 0.232, an RMSE of 0.330, and only about 30% of retrievals within the EE of ±(0.05 + 15%). Furthermore, the proposed algorithm outperformed MODIS in terms of accuracy over their shared retrieval regions. The algorithm’s performance benefits from a newly developed scattering scheme that significantly enhances diurnal retrieval accuracy, making it a promising approach for application to other geostationary satellites.

How to cite: Wong, M., Jin, J., Li, J., Lee, K., Nichol, J. E., and Chan, P.: An advanced aerosol optical depth retrieval algorithm based on an improved scattering angle scheme for Geostationary satellite, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15516, https://doi.org/10.5194/egusphere-egu25-15516, 2025.

EGU25-15879 | ECS | Posters on site | AS3.25

Spatiotemporal pattern analyses of AOD and NO2 VCD in Southeast Asian countries using low-Earth and geostationary orbit satellite data 

Donghee Lee, Seonggyun Na, Jeong-Ah Yoo, and Ja-Ho Koo

Based on a number of low-Earth orbit (LEO) and geostationary (GEO) satellite data, the spatiotemporal pattern of aerosol optical depth (AOD) and the vertical column density of nitrogen dioxide (NO2 VCD) was examined in Southeast Asian countries. Especially, we looked into the spatial distribution of AOD and NO2 VCD in each administrative district, which is helpful for the inter-discipline studies about health risk or environmental policy impact in a local scale. For this study, we used the AOD obtained from the Moderate Resolution Imaging Spectroradiometer (MODIS) and Geostationary Environment Monitoring Spectrometer (GEMS) measurements, and NO2 VCD from the Ozone Monitoring Instrument (OMI) measurements. First, climatological mean and diurnal variation of AOD and NO2 VCD were examined in both national and city scale. We found that there is large difference of AOD and NO2 VCD between national and city scale mean pattern in Thailand, Malaysia, and Indonesia, showing the higher developing region in Southeast Asia. Second, we found that contrast of monthly variation between mainland (e.g., Thailand, Lao PDR, etc.) and maritime (e.g., Malaysia, Indonesia, etc.) regions because the seasonal pattern and environmental properties used to be different according to the latitude. We will extend this analysis to other chemical species (SO2 and HCHO) to prepare the typical air quality information in Southeast Asian countries, where the air quality issue is getting more important as the economic development is being accelerated. We will also investigate the effect of the biomass burning to the quantity variation of AOD and columnar density of gaseous pollutants more in detail.

How to cite: Lee, D., Na, S., Yoo, J.-A., and Koo, J.-H.: Spatiotemporal pattern analyses of AOD and NO2 VCD in Southeast Asian countries using low-Earth and geostationary orbit satellite data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15879, https://doi.org/10.5194/egusphere-egu25-15879, 2025.

EGU25-16847 | Orals | AS3.25

GEMS Ozone profile retrieval: impact of version 3.0 improvements and validations during ACCLIP and ASIA-AQ campaigns.  

Juseon Bak, Jaehwan Kim, Hyunkee Hong, Won-Jin Lee, Dong-won Lee, Jhoon Kim, Xiong Liu, Arno Keppens, and Klaus-Peter Heue

In the troposphere, ozone is a powerful greenhouse gas and air pollutant, harming human health and ecosystems. In the stratosphere, ozone is essential for protecting life on Earth by absorbing harmful ultraviolet (UV) radiation from the Sun. It also plays a key role in maintaining the Earth's radiative balance and stratospheric temperature structure. Monitoring both layers supports tracking pollutant transport, climate regulation, and environmental health.The Geostationary Environmental Monitoring Spectrometer (GEMS) onboard the GEO-KOMPSAT-2B satellite provides high temporal and spatial resolution data on ozone, its precursors (NO₂ and HCHO), SO2, and aerosols over East Asia. The two primary ozone products available from GEMS are total column ozone (O3T) and ozone profile (O3P). The total column ozone is derived using the historical TOMS look-up table algorithm, while the ozone profile product, offers detailed vertical information across 24 atmospheric layers, with an optimal estimation based inversion.

This study describes improvements in the GEMS ozone profile retrieval leading to version 3.0. Compared to 2.X versions, the key updates are as follows: (1) irradiance offset correction are implemented to address the solar diffuser-induced seasonal variation and optical degradation-induced long-term variation, (2) soft calibration is applied to correct residual radiometric biases in the normalized radiances, (3) wavelength shifts are corrected for both radiance and irradiance, and (4) the instrument response function is updated from pre-flight measurements to on-orbit simulations. This has brought the tropospheric O₃ closer to the observations from OMI and TROPOMI. Furthermore, the integrated total column O₃ demonstrates better agreement with ground-based Pandora observation compared to the GEMS O3T product. We also evaluate the information content of ozone profiles in summer during the 2022 ACCLIP campaign and in winter during the 2024 ASIA-AQ campaign. We will discuss how the GEMS ozone profile product adds value in understanding the meteorological modulation of summertime ozone in the troposphere and the dynamical processes affecting wintertime ozone in the upper troposphere and stratosphere.

 

How to cite: Bak, J., Kim, J., Hong, H., Lee, W.-J., Lee, D., Kim, J., Liu, X., Keppens, A., and Heue, K.-P.: GEMS Ozone profile retrieval: impact of version 3.0 improvements and validations during ACCLIP and ASIA-AQ campaigns. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16847, https://doi.org/10.5194/egusphere-egu25-16847, 2025.

EGU25-17031 | Posters on site | AS3.25

The Path to Sentinel-4/UVN Operations: Products, Calibration and Validation, Monitoring, and Data Processing Systems 

Rasmus Lindstrot, Sebastian Gimeno Garcia, Frank Rüthrich, Vinod Kumar, Myojeong Gu, Malcolm Taberner, Alexandre Caseiro, Catherine Hayer, Nan Hao, Philipp Köhler, Christopher Diekmann, Marcel Dobber, Jochen Grandell, and Bojan Bojkov

EUMETSAT will operate the Copernicus Sentinel-4/UVN imaging spectrometer, which is hosted on the Meteosat Third Generation - Sounder (MTG-S) satellite. The first satellite in this series is scheduled to launch in the second half of 2025.

Developed by Airbus Defence and Space under an ESA contract, Sentinel-4/UVN is designed to monitor atmospheric trace gases - such as ozone, nitrogen dioxide, sulfur dioxide, formaldehyde and glyoxal - as well as aerosol and cloud properties from hyperspectral measurements in the UV, Visible and Near-Infrared (UVN). It provides high spatial resolution and hourly coverage over Europe and northern Africa, which is vital for tracking atmospheric composition and serves as a key input to the Copernicus Atmosphere Monitoring Service (CAMS). This innovative instrument will solidify the European contribution to a constellation of geostationary instruments, including the existing GEMS and TEMPO over Asia and North America, respectively. This Geo-Ring will be complemented by the fleet of Low Earth Orbit air quality missions operating in similar spectral ranges, such as GOME-2, OMI, TROPOMI, OMPS and the new Sentinel-5/UVNS mission, providing global daily coverage.

This presentation will provide an overview of the Sentinel-4/UVN instrument and its products, along with the latest updates on the status of the ground segment developments. Some insight into the analysis of the instrument's calibration key data will be part of the presentation.

We will also present the progress of EUMETSAT's data processing and monitoring facility, which is being prepared for commissioning and routine operations. This includes activities for the preparation of the calibration and validation (Cal/Val) of operational atmospheric chemistry products, performed centrally at EUMETSAT as well as with support from the scientific community.

How to cite: Lindstrot, R., Gimeno Garcia, S., Rüthrich, F., Kumar, V., Gu, M., Taberner, M., Caseiro, A., Hayer, C., Hao, N., Köhler, P., Diekmann, C., Dobber, M., Grandell, J., and Bojkov, B.: The Path to Sentinel-4/UVN Operations: Products, Calibration and Validation, Monitoring, and Data Processing Systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17031, https://doi.org/10.5194/egusphere-egu25-17031, 2025.

Aerosol and ocean remote sensing traditionally rely on top-of-atmosphere (TOA) radiance measurements to retrieve optical properties. However, there are ongoing challenges in retrieving chemical and physical parameters due to the limited information contents of the radiances. Polarization measurements, which are sensitive to several aerosol and ocean parameters, provide additional information on these parameters for more detailed characterization. The polarization measurements also give valuable insights into the interaction between aerosols and the atmosphere. Over the years, numerous efforts have been made to measure polarization, including the POLDER generations and the Glory mission. More recently, two passive multi-angular polarimeters, HARP-2 and SPEXone, were launched in February 2024 as part of the PACE mission. This study analyzed the benefit of measuring polarization for retrieving aerosols and oceans based on the optimal-estimation method (OEM). The retrieval sensitivities of two measurement types are compared: one using radiance data alone and another combining radiance with Degree of Linear Polarization (DoLP). We aim to develop an algorithm based on the optimal estimation method that can retrieve aerosols and oceans simultaneously with estimated uncertainties. The key products generated by this algorithm include Aerosol Optical Depth (AOD), the real and imaginary parts of the refractive indices, Fine Mode Fraction (FMF), particle size parameters, and ocean parameters (e.g., ocean surface roughness, chlorophyll-a concentration and CDOM). The improved retrieval capabilities may contribute to a better understanding of atmosphere-ocean interactions.

Acknowledgements

This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)

How to cite: Lee, S. and Jeong, U.: An Optimal-Estimation-based Algorithm for Simultaneously Retrieving Aerosols and Ocean Parameters using Multi-angular Polarimetric Measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17189, https://doi.org/10.5194/egusphere-egu25-17189, 2025.

EGU25-17477 | Posters on site | AS3.25

Prototype Development of Algorithms for CH4 and CO2 Observation Using Cube Satellites 

Hoejun Choi and Ukkyo Jeong

Although the total amount of methane (CH₄) is significantly lower than that of carbon dioxide (CO₂), methane is known to accelerate global warming due to its high Global Warming Potential (GWP) and recent increasing trends. As countries around the world prepare for the era of carbon neutrality, they are competitively developing systems to take a leading role in calculating emissions. While ground-based observation equipment currently provides relatively accurate data, there are limitations in quantifying greenhouse gases from various sources. These limitations are particularly evident in marine areas and regions with insufficient ground-based observation data. To overcome these challenges, this study aims to develop a CubeSat for greenhouse gas monitoring. We plan to launch the first CubeSat in 2027, followed by the launch of four additional satellites in 2028. However, CubeSats may have lower observational accuracy compared to medium and large-scale satellites, making it crucial to develop algorithms that meet data quality and user requirements. Therefore, this study focuses on developing an algorithm that optimally retrieves methane concentrations. Once developed, this greenhouse gas monitoring algorithm will serve as a foundation for more accurate assessments of emission management policies, climate change prediction resources, and both short- and long-term trends in carbon dioxide and methane emissions.

Acknowledgement

This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE).

 

How to cite: Choi, H. and Jeong, U.: Prototype Development of Algorithms for CH4 and CO2 Observation Using Cube Satellites, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17477, https://doi.org/10.5194/egusphere-egu25-17477, 2025.

Since the 21st century, the importance of fine-mode particles associated with NO2 has become increasingly prominent on a global scale, driven by reductions in SO2 emissions. NO2, sharing emission sources with aerosols, acts as a precursor for secondary aerosol formation through atmospheric chemical reactions. Ground-based remote sensing measurements provide high temporal resolution of total burden air pollutants. This study analyzed the relationship between aerosol optical depth (AOD) and total column nitrogen dioxide (NO2) from the Pandora instruments operated by the Pandonia Global Network (PGN) and Pandora Asia Network (PAN) to assess the contribution of the nitrate emissions to the aerosols. The daily coefficient of determination (DDC) between NO2 vertical column density (VCD) and AOD was analyzed across various Asian cities. By incorporating water vapor (H2O) VCD as a meteorological adjustment, a significant relationship between NO2 VCD and adjusted DDC was observed, suggesting that in sites with high NO₂ loading, NO2 is highly correlated with the AOD. Pandora’s simultaneous direct sunlight measurements of AOD, H2O VCD, and NO2 VCD provide valuable information on the relationship between atmospheric aerosols and trace gases, contributing to global air quality research.

 

Acknowledgements
This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment (MOE).

How to cite: Kim, S. and Jeong, U.: Estimations of the contribution of nitrate emissions to the total burden of aerosols in major cities of Asia from the Pandora Asia Network, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17478, https://doi.org/10.5194/egusphere-egu25-17478, 2025.

EGU25-17580 | Orals | AS3.25

The PEGASOS project for comparisons of Geo-Ring data with LEO and ground based data 

Ronny Lutz, Diego Loyola, Claus Zehner, Won-Jin Lee, Hyunkee Hong, and Jhoon Kim

The PEGASOS project (Product Evaluation of GEMS L2 via Assessment with Sentinel-5P and other Sensors) aims at the evaluation of the operational GEMS L2 data products Ozone (total, tropospheric, profile), NO2, SO2, HCHO as well as cloud-, aerosol- and surface parameters. For the evaluation of the GEMS L2 products, comparisons with space-borne instruments (including TROPOMI/S5P, OMI/Aura, GOME-2/MetOP-ABC, VIIRS/S-NPP, AMI/GK-2A, CALIOP/CALIPSO) and with ground-based measurements/networks (ozone-sondes, Dobson, Brewer, Max-DOAS, NDACC, PGN) are performed.

 In a second phase, comparisons for TEMPO with those LEO and ground-based measurements are planned to be included in the PEGASOS project.

In this contribution we provide an overview of the PEGASOS project and summarize the activities performed so far for evaluating the GEMS L2 data products mentioned above. The ESA-funded PEGASOS project is coordinated by the German Aerospace Center (DLR) and the consortium is completed by the Aristotle University of Thessaloniki (AUTH), the Royal Belgian Institute for Space Aeronomy (BIRA-IASB), and the Institute for Environmental Physics of the University of Bremen (IUP-UB).

How to cite: Lutz, R., Loyola, D., Zehner, C., Lee, W.-J., Hong, H., and Kim, J.: The PEGASOS project for comparisons of Geo-Ring data with LEO and ground based data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17580, https://doi.org/10.5194/egusphere-egu25-17580, 2025.

EGU25-17636 | ECS | Orals | AS3.25

Integrating geostationary satellite data into CAMS: Insights from the CAMEO project and GEMS data assimilation 

Zoi Paschalidi, Antje Inness, Johannes Flemming, Roberto Ribas, Kezia Lange, and Andreas Richter

The new satellite technology of the GEO-Ring constellation, offering high-quality, high-temporal-resolution observations of trace gases and aerosols, represents a transformative advance in air quality monitoring. Within the framework of the Horizone Europe CAMEO (CAMS Servive Evolution) project, efforts have focused on integrating GEMS satellite retrievals into ECMWF’s Integrated Forecast System (IFS) to enhance atmospheric composition analyses and forecasts under the Copernicus Atmosphere Monitoring Service (CAMS).

During the first phase of the project, updates to the IFS enabled the assimilation of geostationary GEMS data alongside polar-orbiting satellite observations. Initial evaluations of GEMS version 2 products provided valuable insights into their strengths and limitations, including the identification of biases and their impact on model forecasts.

The operational integration of GEMS NRT NO₂ and O₃ data into the IFS cycle CY49R1 was successfully achieved, with continuous monitoring by CAMS. The release of NRT GEMS retrieval version 3 in December 2024 demonstrated substantial improvements in data quality. Preliminary results indicate significant reductions in biases compared to version 2, particularly for NO₂. The high temporal and spatial resolution of GEMS retrievals captures diurnal patterns, such as rush hour peaks and seasonal variability, being critical for urban air pollution dynamics. For NO₂, comparisons of the NRT GEMS NO2 version 2 data with the IUP-UB alternative retrieval from the University of Bremen revealed improved agreement with TROPOMI and model outputs, reducing biases. For GEMS O₃, assimilation experiments show comparable analysis results to TROPOMI, whereas validations by independent observations show local forecast improvements, particularly over polluted regions.  

By combining geostationary and polar-orbiting satellite data, this work highlights the potential for a synergistic approach to address gaps in air quality monitoring. The findings underscore the important role of geostationary platforms in complementing polar-orbiting satellites, capturing dynamic atmospheric processes, and advancing global air quality forecasts. Future efforts to integrate TEMPO and Sentinel-4 data into the CAMS global monitoring system promise cutting-edge improvements in air quality modeling.

How to cite: Paschalidi, Z., Inness, A., Flemming, J., Ribas, R., Lange, K., and Richter, A.: Integrating geostationary satellite data into CAMS: Insights from the CAMEO project and GEMS data assimilation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17636, https://doi.org/10.5194/egusphere-egu25-17636, 2025.

EGU25-17674 | Posters on site | AS3.25

The Path to Sentinel-5/UVNS Operations: Products, Calibration and Validation, Monitoring, and Data Processing Systems 

Nan Hao, Rasmus Lindstrot, Philipp Köhler, Christopher Diekmann, Yang Wang, Myojeong Gu, Gabriele Poli, Vinod Kumar, Catherine Hayer, Frank Rüthrich, Sebastian Gimeno Garcia, Christopher Gee-Yin Lee, Rosemary Munro, and Bojan Bojkov

EUMETSAT will operate the Copernicus Sentinel-5/Ultraviolet, Visible Near-infrared Short -wave infrared (UVNS) imaging spectrometer, which is hosted on the EUMETSAT Polar System - Second Generation (EPS-SG) A satellites. The first satellite in this series is scheduled to launch in the second half of 2025.

Developed by Airbus Defence and Space under an ESA contract, Sentinel-5/UVNS is designed to monitor atmospheric trace gases - such as ozone, nitrogen dioxide, sulfur dioxide, formaldehyde, glyoxal, methane, and carbon monoxide - as well as aerosol and cloud properties. With its high spatial resolution and near-daily global coverage, it provides essential data for tracking atmospheric composition and supports the Copernicus Atmosphere Monitoring Service (CAMS). Sentinel-5/UVNS will complement and extend the existing fleet of Low Earth Orbit air quality missions operating in the UV, visible, as well as near infrared spectral ranges, such as GOME-2, OMI, TROPOMI and OMPS. Furthermore, it will play a pivotal role in the constellation of geostationary air quality missions consisting of Sentinel-4, GEMS and TEMPO, forming the Geo-Ring, by serving as a travelling standard to monitor and maintain the consistency of the geostationary mission data.  

This presentation will provide an overview of the Sentinel-5 instrument and its products, along with the latest updates on the status of the ground segment developments as well as the preparation of offline processing systems for the analysis of in-orbit calibration measurements.

We will also discuss the progress of EUMETSAT's data processing and monitoring facility, which is being prepared for commissioning and routine operations. This includes activities for the preparation of the calibration and validation (Cal/Val) of operational atmospheric chemistry products, performed centrally at EUMETSAT as well as with support from the scientific community.

How to cite: Hao, N., Lindstrot, R., Köhler, P., Diekmann, C., Wang, Y., Gu, M., Poli, G., Kumar, V., Hayer, C., Rüthrich, F., Gimeno Garcia, S., Lee, C. G.-Y., Munro, R., and Bojkov, B.: The Path to Sentinel-5/UVNS Operations: Products, Calibration and Validation, Monitoring, and Data Processing Systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17674, https://doi.org/10.5194/egusphere-egu25-17674, 2025.

EGU25-19234 | Orals | AS3.25

Event-based GEMS ozone evaluation using consecutive summertime ozonesonde measurements during ACCLIP 

Joowan Kim, Subin Oh, Juseon Bak, Ja-Ho Koo, Sang-Seo Park, and Won-Jin Lee

This study presents a case-based evaluation of Geostationary Environment Monitoring Spectrometer (GEMS) ozone products using daily ozonesonde measurements during pre-ACCLIP (2021) and ACCLIP (2022) campaigns. The analysis uses a total of 62 ozonesonde profiles along with atmospheric reanalysis to better understand daily ozone variability and circulation change related to the Asian summer monsoon. The new GEMS ozone profile (version 3) product successfully captures significant variability in tropospheric and lower stratospheric ozone, including major stratospheric ozone intrusion in 2021 and storm-induced tropospheric ozone decreases in 2022. These variations were closely related to convective activities associated with the Asian monsoon rainband and strong anticyclones in the upper troposphere and lower stratosphere. The comparison between ozonesonde data and GEMS ozone products demonstrates GEMS's capability to detect these dynamic ozone variations, highlighting its potential in monitoring chemical transport and regional-scale air quality in Asia.

How to cite: Kim, J., Oh, S., Bak, J., Koo, J.-H., Park, S.-S., and Lee, W.-J.: Event-based GEMS ozone evaluation using consecutive summertime ozonesonde measurements during ACCLIP, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19234, https://doi.org/10.5194/egusphere-egu25-19234, 2025.

EGU25-19934 | Orals | AS3.25

Current status of validation and improvement of GEMS data 

Limseok Chang, Hyunkee Hong, Jhoon Kim, Donghee Kim, and Dongwon Lee

GEMS data is constantly improved through ongoing validation and evaluation efforts. The ASIA-AQ field campaign conducted in early 2024 provided an opportunity to expand the GEMS validation area to Southeast Asia. In particular, aerial observations produced accurate vertical profile information of chemical substances, which enabled the evaluation of the uncertainty of GEMS input data. In addition, the Pandora Asia Network Project was completed in late 2024, with a total of 20 Pandoras installed in seven Southeast Asian countries. Real-time validation is now available in most GEMS scan regions, excluding South Asia. Meanwhile, the GEMS retrieval algorithm update was recently completed, and data distribution began in late 2024, and additional updates are planned for later this year. The latest results and future plans for GEMS data validation and improvement are presented in this study.

How to cite: Chang, L., Hong, H., Kim, J., Kim, D., and Lee, D.: Current status of validation and improvement of GEMS data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19934, https://doi.org/10.5194/egusphere-egu25-19934, 2025.

EGU25-19951 | Posters on site | AS3.25

Establishment of the Pandora Asia Network and validation of GEMS 

Donghee Kim, Limseok Chang, Hyunkee Hong, Dongwon Lee, Hanlim Lee, Ukkyo Jeong, and Serin Kim

The Pandora spectrometer is a valuable tool for air quality monitoring and satellite validation. From 2020 to 2024, the National Institute of Environmental Research (NIER), in collaboration with the Korea International Cooperation Agency (KOICA), the Korea Environment Corporation (KECO), and the United Nations Economic and Social Commission for Asia and the Pacific (UNESCAP), successfully established the Pandora Asia Network (PAN) by installing 20 Pandora instruments within the field of view of the Geostationary Monitoring Spectrometer (GEMS). These units were installed four in Thailand, three in Indonesia, three in Mongolia, two in Laos, four in the Philippines, three in Vietnam, and one in Cambodia. PAN could provide long-term data to validate GEMS data for Southeast Asia, along with the Pandora instruments installed in Korea, Japan, Singapore, and Malaysia. The comparison results showed a high correlation between GEMS and Pandora. NIER plans to process PAN data in near-real time and provide comparison figures with GEMS, offering greater convenience to GEMS data users. This is expected to contribute not only to GEMS validation but also to monitoring air pollution in the Asian region.

How to cite: Kim, D., Chang, L., Hong, H., Lee, D., Lee, H., Jeong, U., and Kim, S.: Establishment of the Pandora Asia Network and validation of GEMS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19951, https://doi.org/10.5194/egusphere-egu25-19951, 2025.

EGU25-666 | ECS | Posters on site | AS3.26

Unveiling Occupational Exposure: The Impact of Particulate Matter on Traffic Policemen in Industrial Zones 

Madhumita Chakraborty, Smaranika Panda, and Robin Christian

Air pollution, primarily driven by particulate matter (PM), is a major global health challenge, contributing to respiratory, cardiovascular, and neurological diseases, as well as premature mortality. Traditional ambient monitoring often fails to capture the spatial variability and individualized exposure patterns critical to understanding PM's health impacts. Personal exposure monitoring has emerged as a transformative tool, as it include diverse microenvironments. Studies reveal that personal exposure data reduce misclassification, improve exposure-health relationship modeling, and provide insights into source-specific toxicity, thereby enabling more targeted regulatory and public health interventions.

Traffic policemen, due to their constant presence in traffic-dense environments, are uniquely vulnerable to PM exposure. Despite advancements in wearable and low-cost monitoring technologies, limited research addresses occupational exposure in this high-risk group. This study aims to bridge this gap by implementing cutting-edge monitoring technologies to quantify and characterize the exposure of traffic policemen to PM. The personal exposure (PM5 & PM2.5) samples for traffic policemen standing on roads of an industrial area were collected for 15 days along with ambient air quality data for PM (PM100, PM10, PM2.5, and PM1) and gaseous pollutants (NO2, CO, and O3). The personal exposure samples were collected using an SKC personal monitor and Envirotech handy sampler, whereas the ambient air quality data was collected using a sensor-based instrument (Make: Oizom Pvt. Ltd). The collected samples were analyzed for PM concentration using gravimetric methods.PM deposits in human lungs as they enter in to the respiratory system by inhalation. The deposition of PM in different regions of the lungs was also estimated by using Multiple-Path Particle Dosimetry 3.02 model.

The findings from the study indicate that the average personal exposure concentrations for PM2.5 and PM5 were 102.96 ± 38.20 µg/m³ and 138.18 ± 30.41 µg/m³, respectively. The personal exposure level for PM2.5 was notably six times higher than the 24-hour average air quality standard set by the World Health Organization (WHO).

Analysis of ambient air quality data revealed that PM2.5 levels varied from 69.79 µg/m³ to 127.23 µg/m³, with an average concentration of 99.96 µg/m³, which, while still significantly above the WHO guidelines, was lower than the personal exposure levels. This discrepancy highlights that the population under study experienced elevated exposure to PM concentrations compared to ambient air conditions, suggesting that individual exposure conditions are influenced by specific situational and occupational factors. The identified primary sources of particulate matter include industrial fuel combustion, traffic emissions, and resuspension of road dust. Additionally, the proximity of traffic policemen to vehicle exhausts due to the low height of their standing platforms was identified as a contributing factor to the elevated personal exposure levels. This occupational setup positions individuals directly in the pathway of high concentrations of vehicular emissions, exacerbating their risk.

The study found the highest particulate matter deposition in the head region of the respiratory tract, highlighting health risks from prolonged exposure to high PM levels. These findings emphasize the need for mitigation measures, such as enhanced occupational safeguards and stricter emission controls, to protect vulnerable populations

How to cite: Chakraborty, M., Panda, S., and Christian, R.: Unveiling Occupational Exposure: The Impact of Particulate Matter on Traffic Policemen in Industrial Zones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-666, https://doi.org/10.5194/egusphere-egu25-666, 2025.

EGU25-669 | ECS | Posters on site | AS3.26

Interlinking Land Use Land Cover, Forest Biomass, and Air Quality in the Megacity Delhi, India 

Archana Rani and Manoj Kumar

The rapid urbanization and population growth of megacities like Delhi, India, have led to significant changes in land use and land cover (LULC), adversely impacting environmental conditions, including forest biomass and air quality. This study inspects the complex relationships between LULC, forest biomass, and air pollution in Delhi, a city grappling with severe environmental degradation and some of the world’s highest air pollution levels. Landsat-8 satellite imagery was used to analyze LULC changes between 2021 and 2023, focusing on urbanization and its impact on vegetation cover. Air quality data were collected from Central Pollution Control Board (CPCB) monitoring stations across four locations in the city. Two high-traffic, sparsely vegetated zones (Anand Vihar and ITO) and two densely vegetated areas (Sri Aurobindo Marg and Mandir Marg) were selected for a comparative analysis. Additionally, forest biomass was quantified through direct sampling in two major green zones: Sanjay Van near Sri Aurobindo Marg and the Ridge Forest near Mandir Marg CPCB station. LULC analysis revealed a decline in vegetative cover in urban areas due to infrastructure expansion and the conversion of green spaces into residential and commercial zones. CPCB data over six years (2018 – 2023) indicated notable differences in air quality between densely vegetated and sparsely vegetated zones. PM2.5 levels in high-traffic areas (Anand Vihar and ITO) were 24.20% and 23.19% higher than in densely vegetated areas (Sri Aurobindo Marg and Mandir Marg). Similarly, SO2 concentrations were 1.52 times greater, and NH3 levels were 1.69 times higher in regions with sparse vegetation. The biomass at Sanjay Van (112.57 tons) and the Ridge Forest (91.17 tons) significantly contributes to pollutant absorption, capturing considerable quantities of particulate matter (PM10 and PM2.5) and gaseous pollutants such as SO2, NOX, and NH3, while also mitigating the impacts of land use and land cover changes by serving as essential green lungs in an urbanized environment. These forests collectively offer an estimated pollutant absorption capacity of many tons annually, underscoring their vital role in alleviating air pollution and preserving natural equilibrium amid fast urbanization. In brief, the study highlights the essential function of forested regions in Delhi in mitigating air pollution and promoting environmental sustainability.

Keywords: Air Quality; Vegetation; LULC; Biomass; Megacity

How to cite: Rani, A. and Kumar, M.: Interlinking Land Use Land Cover, Forest Biomass, and Air Quality in the Megacity Delhi, India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-669, https://doi.org/10.5194/egusphere-egu25-669, 2025.

EGU25-787 | ECS | Orals | AS3.26

Chemical characterisation and source apportionment of PM2.5 in the cosmopolitan city of Bengaluru, India  

Kavyashree Narayana Kalkura, Mrinmoy Chakraborty, Vinod Shekar, Emil Varghese, and Subramanian Ramachandran

Over the past two decades, Bengaluru, a major city in South India, has undergone rapid urbanization and population growth, with significant increase in vehicular traffic, construction, and industrial activities. These changes can enhance local contributions from anthropogenic biomass burning and vehicular emissions, in addition to long-range transported pollutants, adversely impacting air quality, and reducing visibility. We investigated the chemical composition and sources of particulate matter (PM2.5) in Bengaluru using an Aerodyne Time-of-Flight Aerosol Chemical Speciation Monitor (ToF-ACSM) and two Aethalometers (AethLabs microAeth MA300 and Magee Scientific AE33). This study marks the first in-situ and high time resolution source apportionment of non-refractory PM2.5 (NR- PM2.5) in the city using the ToF-ACSM, commencing from post-monsoon sampling period (Aug 2024). Results thus far indicate that organic aerosols (OA) are the dominant (63%) NR-PM2.5 species, followed by sulphate (~20%) and ammonium (~9%). Positive Matrix Factorization (PMF) analysis identified two primary organic aerosol types namely hydrocarbon-like organic aerosols (HOA) and biomass-burning organic aerosols (BBOA), and two secondary organic aerosols namely less-oxidised oxygenated organic aerosols (LO-OOA) and more-oxidised oxygenated organic aerosols (MO-OOA). The air masses from the northeast (0-90°) direction were found to be associated with elevated levels of MO-OOA, which also correlated well with increased sulphate fraction. These findings highlight the role of local sources like vehicular emissions and waste burning, as well as regional sources including thermal power plant emissions, and oxidised and aged OA. Furthermore, the study includes Diwali and Kannada Rajyotsava celebrations, periods with extensive firework activity. Despite restrictions on conventional fireworks and recommended usage of green crackers, the city witnessed significant particle pollution, with hourly PM2.5 concentrations exceeding 100 µg/m³ and spikes up to 800 µg/m³. While NR-PM2.5 and black carbon (BC) increased during the firework periods, the rise in PM2.5 mass loading was much greater, resulting in incomplete mass closure (only ~16% from NR-PM2.5 + BC) in contrast to normal periods (~80% from NR-PM2.5 + BC). Further results and detailed analyses will be presented, including seasonal changes in PM2.5 composition and sources as we transition from the post-monsoon to the more polluted winter season.

How to cite: Narayana Kalkura, K., Chakraborty, M., Shekar, V., Varghese, E., and Ramachandran, S.: Chemical characterisation and source apportionment of PM2.5 in the cosmopolitan city of Bengaluru, India , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-787, https://doi.org/10.5194/egusphere-egu25-787, 2025.

EGU25-1581 | ECS | Orals | AS3.26

Mapping and Modeling CO2 traffic emissions within local climate zones in Helsinki 

Omar Al-Jaghbeer, Leena Järvi, Pak Lun Fung, and Ville-Veikko Paunu

Quantifying road traffic CO2 emissions is critical for urban climate and sustainability studies. However, detailed modeling often requires high-resolution input data that is unavailable in many regions. To address this gap, we present a simplified regression-based model that quantifies traffic-related CO2 emissions within Local Climate Zones (LCZs) using readily available data such as building surface area, asphalt surface area, population, traffic lights, and road type. This approach minimizes computational requirements and circumvents the need for traffic data, offering a practical alternative for regions with limited resources.
Our results show that road type and asphalt surface area are the most influential variables in describing CO2 emissions. Median CO2 emissions from built LCZs are 1.8 times higher than those from land cover LCZs. The generalized model can explain up to 69% of the emissions for some LCZ. Based on this model, we introduce a look-up table for LCZ-specific traffic CO2 emissions, providing a user-friendly tool to estimate emissions in data-scarce regions. This simplified methodology emphasizes accessibility and efficiency while maintaining robust results, making it an invaluable resource for urban emission studies.

How to cite: Al-Jaghbeer, O., Järvi, L., Fung, P. L., and Paunu, V.-V.: Mapping and Modeling CO2 traffic emissions within local climate zones in Helsinki, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1581, https://doi.org/10.5194/egusphere-egu25-1581, 2025.

EGU25-2269 | ECS | Posters on site | AS3.26

Analysis of Roadside PM Concentrations Using Low-Cost Air Quality Monitoring Systems in South Korea 

Misook Park, Huijeong Lim, and Hui-Young Yun

Particulate matter (PM) is a Group 1 carcinogen and a significant environmental and public health concern globally. In South Korea, concerns over the reliability of conventional air quality monitoring stations, often installed at heights above 10 meters, have led to the deployment of low-cost air quality monitoring systems positioned closer to human breathing zones (2–3 meters). This study uses data from these systems, focusing on a case study in Anyang City, to analyze PM and PM-2.5 concentrations at roadside (bus stops) and riverside/park locations.

To ensure data reliability, the top 10% and bottom 10% of extreme values were excluded, and the remaining 80% of the dataset was analyzed. The results reveal significantly higher PM and PM-2.5 concentrations at roadside locations, emphasizing the need for mitigation strategies to address public health risks. This study also proposes policy recommendations to reduce PM exposure at roadside locations, demonstrating the applicability of such approaches to urban environments in South Korea and beyond.

Acknowledgments

This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute (KEITI) funded by the Ministry of Environment (MOE).

How to cite: Park, M., Lim, H., and Yun, H.-Y.: Analysis of Roadside PM Concentrations Using Low-Cost Air Quality Monitoring Systems in South Korea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2269, https://doi.org/10.5194/egusphere-egu25-2269, 2025.

EGU25-2888 | ECS | Orals | AS3.26

Identifying Greenhouse Gas Emission Trends and Validating Hotspot Locations via Flux Measurements and Footprints in Three Pilot Cities 

Betty Molinier, Natascha Kljun, Patrick Aigner, Dominik Brunner, Jia Chen, Andreas Christen, Lionel Constantin, Hugo Denier van der Gon, Rainer Hilland, Christopher Holst, Daniel Kühbacher, Junwei Li, Robert Maiwald, Stavros Stagakis, Ingrid Super, and Sanam Vardag

Emissions of greenhouse gases (GHGs) are known drivers of climate change and related effects; however, they continue to increase every year despite current reduction efforts. Rising populations worldwide as well as changes in land use and in anthropogenic activities contribute significantly to this observed, unmitigated increase in GHG emissions. Cities are clear hotspots for anthropogenic sources of GHGs, and a regional or national emission reduction plan is not enough to effectively target their complex and unique source compositions or relative contributions. To push local or city-level action plans forward, GHG flux towers in three pilot cities (Zurich, Munich, and Paris) were established for long-term eddy-covariance measurements as part of the H2020 ICOS Cities/PAUL project (https://www.icos-cp.eu/projects/icos-cities). The cities were chosen to offer insight into how city size, topography, and source mixture affect GHG and trace gas emissions.

We present results from emission source attribution of carbon dioxide (CO2), carbon monoxide (CO), and methane (CH4) using a combination of flux measurements, footprint modelling, and local emission inventories. Turbulence measurements observed at or derived from information at each tower were implemented in the Flux Footprint Prediction (FFP) model (Kljun et al., 2015) to develop highly spatially- and temporally-resolved flux footprints for each site. These footprints were subsequently combined with (1) annual emission inventories at high spatial resolution and (2) emission sector-specific hourly temporal profiles for the aforementioned trace gases to estimate the relative contributions of emission sectors to the flux signal at each tower. We also incorporate outputs of the Vegetation Photosynthesis and Respiration Model (VPRM; Mahadevan et al., 2008) to quantify biogenic contributions to the CO2 flux signal. The presented results highlight seasonal and diurnal trends as well as spatial hotspots within the flux footprint of sector-separated CO2, CH4 and CO fluxes in cities with diverse characteristics, all of which is valuable for source attribution and for supporting localized and targeted emission reduction plans.

How to cite: Molinier, B., Kljun, N., Aigner, P., Brunner, D., Chen, J., Christen, A., Constantin, L., Denier van der Gon, H., Hilland, R., Holst, C., Kühbacher, D., Li, J., Maiwald, R., Stagakis, S., Super, I., and Vardag, S.: Identifying Greenhouse Gas Emission Trends and Validating Hotspot Locations via Flux Measurements and Footprints in Three Pilot Cities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2888, https://doi.org/10.5194/egusphere-egu25-2888, 2025.

EGU25-3011 | ECS | Posters on site | AS3.26

Evolution of Air Pollutant Emission Standards in South Korea’s Municipal Waste Incineration Facilities : A Focus on Particulate Matter 

Young-Koo Kim, Seong-Hun Kim, Yong-Kyong Park, and Hui-Young Yun

South Korea's large-scale municipal waste incineration facilities have played a vital role since their introduction in the mid-1980s, particularly amidst rapid economic growth and urbanization. Initially designed to focus on waste volume reduction, these facilities soon became a source of concern for environmental and public health due to emissions of air pollutants, including dioxins, heavy metals, and particulate matter(PM). Particulate matter, especially PM10 and PM2.5, is a critical pollutant with severe health impacts, prompting the strengthening of emission regulations for incineration facilities.

This study investigates the evolution of air pollutant emission standards in South Korea, with a specific focus on particulate matter, through a chronological comparison with those of the European Union (EU). By analyzing major policy developments from the mid-1980s to the present, the study highlights South Korea's progress in adopting international standards and identifies key areas for improvement in future air quality policies.

The findings reveal that South Korea introduced dioxin emission standards (5ng-TEQ/m3) in the 1990s and significantly strengthened regulations in the 2000s under the influence of EU directives, reducing dioxin concentrations to 0.1ng-TEQ/m3. Standards for heavy metals and particulate matter emissions were established, alongside enhanced monitoring systems. Specifically, regulations for particulate matter (PM10 and PM2.5) have been increasingly stringent, with ongoing efforts to reduce emissions in areas surrounding incineration facilities. Meanwhile, the EU has implemented stringent standards through Best Available Techniques (BAT), carbon neutrality, and greenhouse gas reduction policies. South Korea is aligning with these trends by enhancing regulations to improve air quality and adopting localized strategies for particulate matter management.

This study confirms that South Korea's emission standards for incineration facilities have reached levels comparable to those of the EU. It emphasizes the need for tailored policies that account for local characteristics and technological constraints, particularly concerning particulate matter. These findings offer practical insights for reducing air pollution and achieving carbon neutrality both nationally and globally.

 

[Acknowledgment] This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)

How to cite: Kim, Y.-K., Kim, S.-H., Park, Y.-K., and Yun, H.-Y.: Evolution of Air Pollutant Emission Standards in South Korea’s Municipal Waste Incineration Facilities : A Focus on Particulate Matter, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3011, https://doi.org/10.5194/egusphere-egu25-3011, 2025.

EGU25-3361 | Posters on site | AS3.26

Impact of Revamping on PM, NOX, and HCl Emissions in Municipal Solid Waste Incineration Facilities 

Seong-Hun Kim, Young-Koo Kim, Yong-Kyong Park, and Hui-Young Yun

Municipal solid waste incineration (MSWI) facilities play a critical role in managing increasing waste volumes driven by urbanization and population growth, serving an essential function in environmental protection. However, many existing facilities face challenges due to aging infrastructure, struggling to meet stricter air pollution regulations or process waste efficiently. In particular, discrepancies between the design specifications for waste calorific values or composition and the current heterogeneous characteristics of waste have led to reduced operational efficiency.

Building new incineration facilities is often constrained by economic and social barriers. Consequently, the revamping of existing facilities has emerged as a practical solution to enhance operational performance. Revamping typically involves the integration of advanced air pollution control technologies and process optimization, aiming to reduce air pollutant emissions while improving waste treatment efficiency.

This study examines the impact of revamping on air pollutant emissions at municipal solid waste incineration facilities in major cities across South Korea. Using data collected between 2011 and 2023, we analyzed changes in the concentrations of key air pollutants, including particulate matter (PM), nitrogen oxides (NOX), and hydrogen chloride (HCl), before and after refurbishments. Additionally, we evaluated the technological improvements implemented during the refurbishment process and their overall environmental benefits.

The analysis indicates that air pollutant concentrations decreased consistently after revamping, reflecting compliance with stricter environmental regulations and improved process efficiency. These findings provide critical insights for enhancing the operational efficiency of municipal solid waste incineration facilities and developing strategies to mitigate air pollution.

This study offers empirical evidence on the effectiveness of revamping in reducing air pollutant emissions, contributing to sustainable waste management practices and the development of informed environmental policies.

[Acknowledgement]
This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)
 
 

How to cite: Kim, S.-H., Kim, Y.-K., Park, Y.-K., and Yun, H.-Y.: Impact of Revamping on PM, NOX, and HCl Emissions in Municipal Solid Waste Incineration Facilities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3361, https://doi.org/10.5194/egusphere-egu25-3361, 2025.

Accurate NOx emission estimates are required to better understand air pollution, investigate the effectiveness of emission restrictions, and develop effective emission control strategies. This study investigates and demonstrates the ability and uncertainty of the superposition column model in combination with the TROPOspheric Monitoring Instrument (TROPOMI) tropospheric NO2 column data to estimate city-scale NOx emissions and chemical lifetimes and their variabilities. Using the recently improved TROPOMI tropospheric NO2 column product (v2.4–2.6), we derive daily NOx emissions and chemical lifetimes over the city of Wuhan for 372 full-NO2-coverage days between May 2018 and December 2023, and validate the results with bottom-up emission inventories. We find insignificant weekly cycle of NOx emissions for Wuhan. We estimate a summer-to-winter emission ratio of 0.77, which is overestimated to some extent, though it is even higher provided by the bottom-up inventories. We calculate a steady decline of NOx emissions from 2019 to 2023 (except for the valley in 2020 caused by the COVID-19 lockdown), indicating the success of the emission control strategy. The superposition model method results in ~15% lower estimation of NOx emissions when the wind direction is from distinct upwind NO2 hotspots compared to other wind directions, indicating the need to improve the approach for cities that are not relatively isolated pollution hotspots. The method tends to underestimate NOx emissions and lifetimes when the wind speed is > 5-7 m s-1, the estimation for Wuhan is ~4% for the emissions and ~8% for the chemical lifetime. The results of this work nevertheless confirm the strength of the superposition column model in estimating urban NOx emissions with reasonable accuracy.

How to cite: Zhang, Q.: Estimating the variability of NOx emissions from the city of Wuhan with TROPOMI NO2 data during 2018 to 2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3368, https://doi.org/10.5194/egusphere-egu25-3368, 2025.

EGU25-3375 | Posters on site | AS3.26

The impact of changes in Korea's electricity supply policy on air pollutants: Focusing on fine dust (PM10, PM2.5) 

Yong-Kyong Park, Seong-Hun Kim, Young-Koo Kim, and Hui-Young Yun

Air pollutant emissions originate from diverse and complex sources, making immediate reductions challenging. In South Korea, fossil fuel-based power plants are a major source of air pollution, particularly in the form of fine particulate matter (PM10, PM2.5), which significantly impacts air quality. To address this issue, the South Korean government has prioritized sustainable power supply and air quality improvement, focusing on expanding renewable energy and periodically revising the Basic Plan for Electricity Supply and Demand.

This study analyzes the changes in South Korea's power supply policies from 2014 to 2023 and examines the correlation between these policies and variations in air pollutant emissions during this period. Using government-provided data, we investigated changes in installed capacities and annual power generation by energy sources (nuclear, coal, LNG, renewables, and pumped storage), as well as regional air pollutant emissions, to assess the relationship between policy implementation and air quality improvements.

The results indicate a steady increase in renewable energy capacity and generation during the study period. This transition was accompanied by a decline in fossil fuel-based power generation and noticeable improvements in PM10 and PM2.5 concentrations in key regions.

This study highlights the potential for policy frameworks to reduce air pollutants through the expansion of renewable energy and the reduction of fossil fuel power generation. The findings serve as valuable references for future policy development aimed at improving air quality and achieving sustainable energy goals.

Keywords: Korea's electricity supply policy, fossil fuels, Renewable Energy, Air Pollutants, Fine Dust

 [Acknowledgement] 

"This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)“

How to cite: Park, Y.-K., Kim, S.-H., Kim, Y.-K., and Yun, H.-Y.: The impact of changes in Korea's electricity supply policy on air pollutants: Focusing on fine dust (PM10, PM2.5), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3375, https://doi.org/10.5194/egusphere-egu25-3375, 2025.

There are about 800 air pollution measurement networks (urban, roadside, rural and so on) in Korea, however air pollution in agricultural area are not measured. Thus it is necessary to identify air pollution in agricultural area which possess a relatively larger area than urban area. In this study, we established eight air pollution monitoring stations in agricultural area, and we conducted to comparatively analyze the air quality in agricultural and urban areas, during the periods for 1) the entire measurement data, 2) high PM episodes, and 3) non-high PM episodes. Considering the spatial distribution by region of Korea, air pollution monitoring stations were established in in agricultural area (Yeoju, Nonsan, Naju, Gimhae, Hongcheon, Danyang, Muan, and Sangju). PM-10 and PM-2.5 (ß-Ray attenuation method), SO2 (Ultraviolet fluorescent method), NOx and NH3 (Chemiluminescence method) were measured in real-time. Meteorological data such as temperature, humidity, wind direction, and wind speed were also measured. One-year measurement data from October 2023 to September 2024 were used, and high-PM episodes was defined as the period when the PM-2.5 concentration exceeds 24-hour air quality standard (35 μg/m3) of Korea and persists for 24 hours or more. The air quality data of urban area (near large cities: Suwon, Daejeon, Gwangju, Busan, Chuncheon, Cheongju, and Daegu) during the same period were used to compare to the air quality of agricultural area. During the entire period, the average concentrations in urban and agricultural areas were found to be similar for both particulate and gaseous compounds. During non- high PM episodes, agricultural and urban areas also showed similar levels. During high PM episodes (a total of 17 days), while the concentration of air pollutants in urban areas was obviously higher than those in agricultural area, but higher concentrations of particulate matter in agricultural areas were observed during certain periods (PM-10 in the morning and PM-2.5 in the afternoon). Gaseous concentrations in agricultural areas were found to be lower than those in urban area during the high PM episodes. In the future, it is necessary to analyze the characteristics of the variation of air pollution according to concentration changes by period (diurnal variation), solar intensity, and meteorological factors to clarify the differences in characteristics of air quality between agricultural and urban areas.

Acknowledgments

"This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)"

How to cite: Baek, J., Kim, J., and Joo, H.: Characteristics of air pollution of agricultural region in high PM episodes using air quality measurement data of megacity and agricultural sites from 2023 to 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3404, https://doi.org/10.5194/egusphere-egu25-3404, 2025.

EGU25-3478 | Posters on site | AS3.26

A scalable spatial decomposition of air pollution data into intercity- and neighborhood-scale components: Application to PM2.5 in South Korea 

Jihoon Seo, Ahreum Lee, Doo-Sun R. Park, Daeok Youn, Kyung Hwan Kim, Chang-Eui Park, and Jin Young Kim

Despite ongoing efforts to mitigate air pollution, the effectiveness of policies often varies across regions due to the differing spatial scales of air pollution variability, which arise from the characteristics of pollution sources as well as geographical and meteorological factors. Understanding air pollution by isolating its components at different spatial scales is crucial for designing effective mitigation strategies. In this study, we propose a simple and intuitive method for the scalable spatial decomposition of spatiotemporal air pollution data into intercity-scale (tens of kilometers) and neighborhood-scale (several kilometers) components. To separate the intercity-scale from the neighborhood-scale component, we introduce a spatially varying ‘effective range’ for intercity-scale variability, based on the distance-decaying spatial autocorrelation of background-removed components. This effective range is influenced by emissions and geographical features. We applied this method to hourly PM2.5 data from 535 air quality monitoring stations (AQMSs) across South Korea for 2021–2022. Our findings reveal that the intercity-scale component contributes most significantly to PM2.5 concentrations in urbanized and industrial regions, such as the Seoul metropolitan area. In contrast, the neighborhood-scale component is more prominent near emission hotspots, such as industrial complexes. These results suggest that in regions where intercity-scale contributions are significant, effective air pollution mitigation strategies should prioritize intercity-scale regulations, which should be managed by the central government or through inter-local agreements, rather than focusing solely on local hotspots. This study provides a robust approach for quantifying both intercity-scale and neighborhood-scale air pollution contributions using ground-based AQMS data, facilitating the development of multi-spatial-scale strategies for air quality management.

How to cite: Seo, J., Lee, A., Park, D.-S. R., Youn, D., Kim, K. H., Park, C.-E., and Kim, J. Y.: A scalable spatial decomposition of air pollution data into intercity- and neighborhood-scale components: Application to PM2.5 in South Korea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3478, https://doi.org/10.5194/egusphere-egu25-3478, 2025.

EGU25-3538 | ECS | Posters on site | AS3.26

Air Quality Challenges in a Petrochemical Urban Area: Signatures of Pollution Sources and Atmospheric Conditions 

Bianca Mihalache, Sabina Stefan, Marilena Colt, and Gabriela Iorga

Urban areas with industry focused on oil refining activities face significant challenges in air quality management due to complex interactions between local emissions, meteorology, and regional transport. The oil extraction and petrochemical industry in Ploiesti, Romania, played a pivotal role into the development of the country since 19th century. This study investigates air pollution in Ploiesti area focusing on particulate matter (PM10, PM2.5) and key gaseous pollutants (NO, NO2, SO2, CO, VOCs, O3) using hourly data sets from the city AQ Monitoring Network, local meteorological observations, and boundary layer data from the ERA5 reanalysis. For the medium term in-depth analysis of air pollutants, data were examined for a four year period (01.01.2018 - 31.12.2021), while for the long-term analysis statistical analysis was performed on a 16 year period (01.01.2007 - 31.12.2023).

The specific questions were targeted to the intra-urban variability of air pollutants versus the identification of city areas with similar pollution pattern, in relation with the meteorological observations; identification of emission sources (by source categories anthropogenic/natural); temporal patterns (daily, weekly, seasonal, annual) and trend quantifications; a check on the causes of pollution episodes (with respect to local sources or transport from medium to distant sources).

  • The anthropogenic activity in Ploiesti strongly affects atmospheric pollution levels on daily timescales (PM2.5/PM10 = 0.71). However, high-resolution measurements reveal the specificity of the surroundings of the monitoring stations.
  • The general temporal pattern of major pollutants (except O3) with lower mass concentrations during warm periods and higher levels during colder seasons follows the general annual pattern of particulate emissions and is modulated by the meteorological seasonal variations (atmospheric mixing layer height).
  • Particulate matter diurnal cycle indicates a peak during the morning rush hours (about 08:00-10:00) but no peak is clear in the afternoon/evening. This could possibly be related to the people social behavior in Ploiesti (i.e. social activities in parks and cafés, as well as various times for the job ending or shift works).
  • We identified that the temporal patterns of O3 precursors (elevated VOCs despite reduced NOx during weekends) in this mid-size city lead to the so-called O3 weekday-weekend effect.
  • From January 2018 to December 2021 a total of 36 pollution episodes were identified. It was found that local anthropogenic emissions coupled with boundary layer dynamics determined the occurrence of 42% of events, while the remaining (58%) are divided in almost equal parts between regional-scale events (27%) and events when dust advections coming from long distances (31%). The trends in the occurrence of pollution events are opposite: decreasing for local events and increasing for regional and LRT-determined events. This suggests that the large-scale air circulation patterns influenced by the higher energy in the atmosphere due to climate changes might alter the distribution and concentration of pollutants leading to fugitive air pollution events.

Acknowledgment: BM work was supported by the University of Bucharest, PhD research grant. Climate and meteorology data were extracted from https://cds.climate.copernicus.eu. Ground-level air pollution were extracted from Romanian National Air Quality Database, www.calitateaer.ro.

How to cite: Mihalache, B., Stefan, S., Colt, M., and Iorga, G.: Air Quality Challenges in a Petrochemical Urban Area: Signatures of Pollution Sources and Atmospheric Conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3538, https://doi.org/10.5194/egusphere-egu25-3538, 2025.

EGU25-3684 | ECS | Orals | AS3.26

Using airborne greenhouse gas enhancement ratios for source apportionment in Asia during ASIA-AQ 

Jason Miech, Joshua DiGangi, Glenn Diskin, Yonghoon Choi, Richard Moore, Luke Ziemba, Francesca Gallo, Carolyn Jordan, Michael Shook, Edward Winstead, Elizabeth Wiggins, Sayantee Roy, and Charles Gatebe

As Asian urban areas continue to expand, so will their contribution to global greenhouse gas (GHG) emissions, driven primarily by increases in fossil fuel combustion. Left unchecked, these emissions will negatively impact air quality and climate, therefore it is imperative that emission sources are properly identified and accounted for in emission inventories. Enhancement ratios of GHGs have been used to characterize regional emissions as either dominated by fossil fuel combustion or biomass burning. In particular, airborne assessment of short-term continuous emission ratios has proven useful to quantify relative contributions of fossil fuel and biomass burning to GHG emissions. The 2024 Airborne and Satellite Investigation of Asian Air Quality (ASIA-AQ) campaign, flying over the Philippines, Korea, Thailand, and Taiwan, sampled a variety of emissions including significant biomass burning, local urban pollution, and transport events. This work will explore the impact of GHG emissions on the distinct pollution of cities including Manila, Bangkok, Chiang Mai, Seoul, and Kaohsiung. The incorporation of missed approaches within urban areas allowed us to sample boundary layer pollution within these cities.  As airborne GHG measurements over Southeast Asia are scarce if not nonexistent, this work provides a crucial link between established ground-based measurements and state-of-the-art satellite observations such as those from South Korea’s Geostationary Environment Monitoring Spectrometer (GEMS). Analysis of GHG enhancement ratios in Asia will lead to more accurate emission inventories which can be used to implement more effective GHG control measures leading to improved air quality and minimizing the effect on climate.

How to cite: Miech, J., DiGangi, J., Diskin, G., Choi, Y., Moore, R., Ziemba, L., Gallo, F., Jordan, C., Shook, M., Winstead, E., Wiggins, E., Roy, S., and Gatebe, C.: Using airborne greenhouse gas enhancement ratios for source apportionment in Asia during ASIA-AQ, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3684, https://doi.org/10.5194/egusphere-egu25-3684, 2025.

EGU25-4060 | Orals | AS3.26

Ozone Formation and Dry Deposition in Urban Environments: Insights from WRF-Chem Modeling and Eddy Covariance Flux Measurements in Beijing 

Eran Tas, Daniel Choi, Erick Fredj, Huangfu Yibo, Bin Yuan, and Huizhil Liu

Tropospheric ozone (O3) is a major air pollutant that negatively affects human health and vegetation, while also playing a central role in atmospheric chemistry and climate change. Dry deposition, a process by which gases are deposited on a surface by air turbulence and gravity, accounts for about 20–25% of tropospheric O3 removal. However, the mechanisms controlling the O₃ dry-deposition velocity (Vd,O₃) in urban areas are poorly understood, largely due to the scarcity of measurements in such environments.

We hypothesized that: (i) Combining direct O₃ flux measurements with source apportionment of factors controlling ozone levels (e.g., NO and volatile organic compounds [VOCs]) based on comprehensive field measurements in an urban environment is essential for disentangling the simultaneous effects of emission sources and meteorological conditions on Vd,O₃. (ii) Integrating atmospheric chemistry model simulations with flux measurements can elucidate how emissions and environmental conditions influence O₃ formation and removal, providing critical insights for air-quality assessment and urban planning.

Accordingly, we conducted direct eddy covariance measurements of O₃, VOCs (via Vocus PTR-TOF-MS), and NOx ([NO] + [NO₂]) fluxes at a height of 102 m on a meteorological tower in Beijing between April 28 and June 26, 2023. Vertical profiles of meteorological parameters were measured at 15 levels along the tower. Source apportionment analysis of VOCs and NOx was conducted using the positive matrix factorization (PMF) model. Additionally, the Weather Research and Forecasting model with Chemistry (WRF-Chem) was applied to evaluate the contributions of anthropogenic and biogenic emissions to O₃ formation. WRF-Chem model simulations were validated against data from nearby air-quality monitoring stations.

Our results show that Vd,O₃ in the urban environment was primarily controlled by chemical reactions, including O₃ titration by NO and contributions from anthropogenic VOCs. Surface wetness was identified as a key factor influencing Vd,O₃, consistent with our findings from measurements in vegetated environments [1,2]. Comparing urban and vegetated settings highlighted the influence of air turbulence, relative humidity, and chemical interactions on Vd,O₃. These findings provide valuable insights for improving urban O₃ simulations and for air-quality management and urban planning strategies.

 

1. Li, Qian, et al. "Measurement-based investigation of ozone deposition to vegetation under the effects of coastal and photochemical air pollution in the Eastern Mediterranean." Science of the Total Environment 645 (2018): 1579-1597.‏

2. Li, Qian, et al. "Investigation of ozone deposition to vegetation under warm and dry conditions near the Eastern Mediterranean coast." Science of the Total Environment 658 (2019): 1316-1333.‏

How to cite: Tas, E., Choi, D., Fredj, E., Yibo, H., Yuan, B., and Liu, H.: Ozone Formation and Dry Deposition in Urban Environments: Insights from WRF-Chem Modeling and Eddy Covariance Flux Measurements in Beijing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4060, https://doi.org/10.5194/egusphere-egu25-4060, 2025.

Air pollutants (PM2.5, PM10, O3, NO2, SO2, and CO) have become a significant environmental concern, particularly in Asian metropolises. The Indian metropolis of Delhi serves as a prime example. A key challenge in addressing urban atmospheric pollution is the significant variation in pollution levels across short distances. Various factors, including nearby industries, vehicle traffic, and population density influence this heterogeneity. Thus, to accurately assess the urban pollution situation, installing multiple pollution monitoring stations that comprehensively cover an entire city, from its center to its periphery is essential. However, the number of stations monitoring entire urban areas increases gradually. For instance, the World Air Quality Historical Database currently lists only four stations in Delhi that have been operational since 2014. The number of stations in Delhi has gradually increased, and in 2024, the same database recorded 45 operational stations, providing more comprehensive coverage of the city. However, the time covered by the available pollution records varies, and, within these periods, there are numerous missing data points. The inconsistencies between stations introduce statistical artifacts when local pollution data are averaged to produce decade-long records that might be representative of the whole city area, making it difficult to assess the actual urban air quality and the effects of policies aimed at reducing urban air pollution. In this study, we propose statistical reconstructions of six daily atmospheric pollution concentrations for all 45 stations in the city of Delhi from 2014 to the present. These reconstructions aim to produce a more consistent database that could better represent the entire city area over 11 years (from January 1, 2014, to January 1, 2025). This reconstructed network is then used to evaluate an ensemble average record that could more realistically represent the daily evolution of air pollution concentration in the city of Delhi since 2014. To accomplish such network reconstruction, we apply the Regression Learner tool in MATLAB to assess 35 machine learning (ML) regression techniques. We select and use only those that perform better in modeling the available records to estimate the missing data. The ML regression models that demonstrated superior performance include: the Fine Tree (Regression Trees family), the Bagged Trees (Ensembles of Trees family), the Optimizable Ensemble (Ensembles of Trees family), the Fine Gaussian SVM (Support Vector Machine family), the Rational Quadratic (Gaussian Process Regressions family), and the Exponential (Gaussian Process Regressions family). In contrast, our analysis revealed that the commonly used multi-linear regression model underperforms compared to 20 other ML regression models. Generally, the proposed methodology can apply to all situations typically addressed in the literature using the multi-linear regression model only because its algorithm is readily available. However, the physical relationships between a given observable and its potential constructors are often nonlinear, rendering the multi-linear regression model suboptimal for such tasks. In the case of the city of Delhi, we demonstrate that the proposed analysis methodology corrects significant biases in the decadal trend for all six network pollution records, and show that from 2014 to 2024, air pollution quality has slightly improved.

How to cite: Scafetta, N. and Shafi, S.: Optimal reconstruction of incomplete urban pollution records with machine learning regression models: a case study for Delhi, India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5078, https://doi.org/10.5194/egusphere-egu25-5078, 2025.

EGU25-5706 | Posters on site | AS3.26

Continuous Monitoring of Atmospheric Halocarbons with a Dewater-Thermo Desorption Unit and GC-ECD: Insights from Industrial and Urban Environments 

Chang-Feng Ou-Yang, Jia-Lin Wang, Cheng-Yu Hsu, Chieh-Heng Wang, Chih-Chung Chang, and Neng-Huei Lin

In the face of the complex composition of atmospheric pollutants, our laboratory has developed a Thermo Desorption Unit (TD) for capturing and concentrating trace-level volatile organic compounds (VOCs) in air samples. Because of the humid climate, we added a Dewater Unit (DW) before the TD to remove excess moisture from air samples while retaining polar and non-polar species to keep sample integrity. This setup has been successfully utilized in the past by connecting the DW-TD units with gas chromatography (GC) equipped with flame ionization detection (FID) and mass spectrometry (MS). While the data quality from GC-FID was extremely stable and robust, the drift and, thus, instability in MS is significant by comparison. In this research, we attempted to use electron capture detection (ECD) to test the stability of the DW-TD units by exploiting ECD’s high sensitivity, stability, and ease of operation. Another prominent advantage of ECD is that it only needs high-purity nitrogen gas as both the carrier and make-up gas. We exploited ECD's highly sensitive and selective properties to measure trace-level atmospheric chlorofluorocarbons (CFCs) and halocarbons to demonstrate the performance of the self-built DW-TD apparatuses. Since CFCs have extremely long atmospheric lifetimes and are well-mixed in the atmosphere due to the Montreal Protocol banning them from most applications, they exhibit certain background mixing levels during a relatively short period of time, e.g., weeks, with variability smaller than most GC’s analytical precisions. We then utilized this property to assess the stability of our homemade instrument. During the one-month continuous online analysis of DW-TD/GC-ECD at an industrial park known for semiconductor and electronics manufacturing, the mole fractions of CFC-12 was found to be 485.19±0.22 ppt (parts per trillion), with RSD (Relative Standard Deviations) = 0.06%. Although CFC-11, CFC-113, and CCl4 have long been phased out, abrupt rises in signal were still detected, suggesting emissions still existed in this industrial complex. By filtering out data with relatively stable mole fractions in between events, the RSD for CFC-11, CFC-113, and CCl4 was found to be 0.12%, 0.36%, and 0.30%, respectively. To further validate the high-value events observed in the industrial park, we conducted an additional one-month continuous online analysis of DW-TD/GC-ECD at a university campus in Taipei as a contrast of environment. This comparative study yielded stable background mole fractions for CFC-12, CFC-11, CFC-113, and CCl4, with RSD of 0.05%, 0.10%, 0.32%, and 0.29%, respectively. These results will be compared with the variability from AGAGE's online data using Medusa/GC-MS and the offline data of NOAA by GC-MS. The occurrence of the high-value events during the month-long measurements can be traced back to emission sources by utilizing backward trajectories to the potential sources for further investigation.

How to cite: Ou-Yang, C.-F., Wang, J.-L., Hsu, C.-Y., Wang, C.-H., Chang, C.-C., and Lin, N.-H.: Continuous Monitoring of Atmospheric Halocarbons with a Dewater-Thermo Desorption Unit and GC-ECD: Insights from Industrial and Urban Environments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5706, https://doi.org/10.5194/egusphere-egu25-5706, 2025.

EGU25-5924 | ECS | Orals | AS3.26

Greenhouse gases total column measurements from ground-based FTIR spectrometers in the Paris' region for emission inventory optimization. 

Josselin Doc, Michel Ramonet, Morgan Lopez, François-Marie Bréon, Benoît Maquart, Maixent Cassagne, Hippolyte Leuridan, Pascal Jeseck, and Yao Té

The ICOS-Cities project aims at evaluating different observational approaches to determine CO2 emissions from large cities, such as Paris (France). A developing approach consists in building a network of three (half-)autonomous FTIR spectrometers used for CO2 total column retrieval: two EM27/SUN placed up and down the prevailing wind axis (Gonesse and Saclay) and one IFS 125 HR placed in Paris Center (Jussieu). These measurements are complementary to the surface measurements carried out in Paris for a decade in the framework of the ICOS European research infrastructure. 

When the wind blows in the instrument location axis, the spatial gradient between stations is considered to be representative of the enhancement due to the surface fluxes in the area in between. It is therefore the signal assimilated by inverse modelling for surface fluxes calculations. The columns are driven not only by the geophysical variations, but also by measurement-specific effects such as solar zenith angle) and measurement noise. Part of our work consists in characterizing these effects so as to be able to make the best use of gradients in calculating fluxes. The expected XCO2 gradients (Saclay-Gonesse) are derived from WRF-GHG modelling that accounts for prior inventory of the Paris area emissions, large scale transport of CO2 constrained by a global inversion, and atmospheric transport constrained by ECMWF meteorological parameters.  The ratio of the measured and modelled gradients is used to estimate a correction to the prior inventory leading to new estimates of the Paris area emissions.  The aim is to analyse the potential contribution of total column estimates, with respect to surface measurements, to estimate urban emissions.

How to cite: Doc, J., Ramonet, M., Lopez, M., Bréon, F.-M., Maquart, B., Cassagne, M., Leuridan, H., Jeseck, P., and Té, Y.: Greenhouse gases total column measurements from ground-based FTIR spectrometers in the Paris' region for emission inventory optimization., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5924, https://doi.org/10.5194/egusphere-egu25-5924, 2025.

EGU25-6270 | ECS | Posters on site | AS3.26

Living with VOCs: Understanding indoor emissions and their implications beyond four walls 

Ashish Kumar, Catherine O'Leary, Ruth Winkless, Matthew Thompson, Wael Dighriri, Helen Davies, David Shaw, Sari Budisulistiorini, Marvin Shaw, Nicola Carslaw, David Carslaw, and Terry Dillon

In developed countries, people spend nearly 90% of their time indoors, where activities such as cooking and cleaning are significant sources of air pollution, with consequent impacts on occupant health. Volatile organic compounds (VOCs), emitted indoors, can also escape into the urban outdoor environment and contribute to secondary pollution, e.g. via production of ozone and particulate matter formation. This comes at a time when successful regulation has led to gradual decreases in emission from some traditional emission sources such as traffic. Despite their importance, VOC from indoor sources remain understudied, with limited understanding of their emission patterns and broader environmental impacts. In this work, we used selected ion flow tube mass spectrometry (SIFT-MS) to examine VOC emissions from common indoor activities under controlled laboratory and semi-realistic domestic conditions. The speciated chemical signatures and emission rates derived from real-time measurements provide valuable insights into the sources and dynamics of these indoor emissions and help identify the tracer molecules (like nonanal, chloroform, carbon tetrachloride, nonane, etc) that can also be used to assess the contribution of indoor activities to the urban ambient air. These findings provide a valuable framework for understanding and designing comprehensive intervention strategies to address both indoor and outdoor air quality challenges.

How to cite: Kumar, A., O'Leary, C., Winkless, R., Thompson, M., Dighriri, W., Davies, H., Shaw, D., Budisulistiorini, S., Shaw, M., Carslaw, N., Carslaw, D., and Dillon, T.: Living with VOCs: Understanding indoor emissions and their implications beyond four walls, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6270, https://doi.org/10.5194/egusphere-egu25-6270, 2025.

EGU25-6714 | ECS | Posters on site | AS3.26

Natural ventilation of a room-atrium system with fluctuating opposing wind 

Teresa Di Renzo, Massimo Marro, Luca Ridoli, Pietro Salizzoni, and Riccardo Vesipa

We study the deterministic and stochastic dynamics of a naturally ventilated system composed of a room and a taller atrium. In the room, a point buoyancy source on the floor generates a turbulent plume which rises towards the ceiling. At the ceiling, the buoyant fluid accumulates, inducing a stratification. The room is connected to the atrium through an opening at the room ceiling level. Therefore, the room buoyant fluid flows through it and rises towards the ceiling of the atrium. The stack effect caused by the accumulation of buoyant fluid in both the environments drives the natural ventilation of the system. The performance of natural ventilation can be assessed by measuring the flow rate of fresh air entering the room due to the stack effect. Several external factors, such as wind, can influence this flow rate. A reduction (increment) in the flow rate is described as worsening (enhancement). We consider the occurrence of a wind opposing the stack effect. Firstly, a constant wind is considered and the corresponding deterministic dynamics is focused on. We study the steady states for different geometries of the atrium, and the transient before the steady state is reached. It is well-known that when no external wind occurs the atrium may either enhance or worsen the ventilation of the room depending on its geometry. Our main finding is that for any atrium geometry the atrium enhances the ventilation, provided that the wind velocity is large enough. However, during the transient, the atrium worsens the ventilation. Secondly, a random component is added to the wind velocity. This stochastic forcing entails a so-called ‘noise-induced transition' of the system dynamics, namely a structural change of the time-averaged behaviour: the warm-cold layers air in the room fluctuates around a mean value lower than the elevation exhibited in case of constant wind. We investigate the effects of the stochastic forcing on the system for increasing coefficient of variation of wind velocity, finding that the room-atrium system is less sensitive to stochastic forcing compared to a single room.

How to cite: Di Renzo, T., Marro, M., Ridoli, L., Salizzoni, P., and Vesipa, R.: Natural ventilation of a room-atrium system with fluctuating opposing wind, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6714, https://doi.org/10.5194/egusphere-egu25-6714, 2025.

EGU25-7547 | Posters on site | AS3.26

Physical and optical properties of black carbon observed at the 303-meter-high Tower in the urban environment.  

Saehee Lim, Yongjoo Choi, Jeonghoon Lee, Junsu Gil, I seul Cho, Ji young Kim, and Sumin Kim

Urban air pollution has consistently captured social and scientific attention due to its significant health and climatic impacts. Among the short-lived climate pollutants (SLCPs) targeted for reduction, black carbon (BC) stands out as a critical component. BC is a carbonaceous primary aerosol emitted from fossil fuel and biomass combustion, with an atmospheric lifetime of approximately five days.

This study involved a tower-based field campaign conducted in late spring in Incheon, a South Korean city adjacent to the Yellow Sea. Using a Single-Particle Soot Photometer (SP2; Droplet Measurement Technology, Boulder, CO, USA), refractory black carbon (rBC) properties, including concentrations, size distribution, and mixing state, were monitored for two weeks in May 2023 at the 303-meter-high Posco Tower-Songdo (PT).

The average ± standard deviation mass concentration of rBC was 0.2±0.1 μg m⁻³, with the mass median diameter (MMD) ranging from 133 to 227 nm. The highest mass concentration and the lowest MMD and Rshell/core (the ratio of shell-to-core diameter of rBC) were observed at 10 a.m. daily, indicating the arrival of freshly emitted local rBC particles. During pollution events characterized by elevated PM2.5 and O3 levels, Rshell/core increased to 1.4–2.0. The mass absorption cross-section (MAC) at 550 nm, estimated using the BHCOAT implementation of Mie theory with input of measured diameter and coating thickness of individual rBC particle, was enhanced by a factor of 1.7 (Eabs). Eabs was positively correlated with Ox (NO2+O3) and aerosol liquid water content (ALWC). Notably, the highest Eabs coincided with relative humidity (RH) exceeding 70% and ALWC reaching ~30 μg m⁻³. These results suggest that under high atmospheric oxidation states, coating formation on the rBC surface is enhanced, promoting the development of hygroscopic aerosols on BC particles in this urban area. More detailed analysis will be presented in the meeting.

 

This research was supported by the National Institute of Environ- mental Research (NIER) grants funded by the Korean government (NIER-2023-01-02-083) and the National Research Foun- dation of Korea (NRF) from the Ministry of Science and ICT (NRF- 2021R1C1C2011543 & RS-2023-00249553). We thank POSCO International for establishing and maintaining the site.

How to cite: Lim, S., Choi, Y., Lee, J., Gil, J., Cho, I. S., Kim, J. Y., and Kim, S.: Physical and optical properties of black carbon observed at the 303-meter-high Tower in the urban environment. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7547, https://doi.org/10.5194/egusphere-egu25-7547, 2025.

EGU25-7874 | Posters on site | AS3.26

Air Pollution Mitigation Capacity of an Urban Forest in Densely Road-Networked Area: Findings from High-Resolution Sensor Monitoring 

Jong Won Ryu, Jun Yeong Lee, Yu Kyeong Park, and Won Sik Choi

The dense roadway network leads to high emissions of air pollutants per unit area, causing adverse environmental and health impacts. Various approaches to mitigating these air pollutions have been proposed, and one of the notable strategies is the use of vegetation for air purification. Vegetation is known to remove particulate and gaseous pollutants through various processes such as stomatal uptake, physical impaction and adsorption, and blocking by surfaces. Additionally, urban forests can contribute to improving air quality by reducing the urban heat island effect, potentially leading to slower chemical reactivities for secondary pollutants. However, air pollutant removal efficiencies of urban forests can be controlled by various factors such as vegetation type, leaf density, size, location, and seasonal and meteorological conditions. Moreover, the complex urban canopy and built environments can lead to spatiotemporally heterogeneous distributions of air pollutants, adding uncertainty to the assessment of the air purification capacity of urban forests.

In this study, we conducted high-resolution measurements with an air quality sensor network to evaluate air pollution mitigation capacity of an urban forest that sits in a densely road-networked area. Air quality sensors were installed inside and outside the urban forests to monitor concentrations of both gaseous (CO, NO, NO2, O3) and particulate pollutants (PM2.5 and number density) across different seasons. Here, we present the preliminary results of our findings obtained from four intensive measurement campaigns in different seasons.

Acknowledgments

This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)

Keywords: urban forest, air pollution mitigation, sensor network, field measurements, seasonal variations

How to cite: Ryu, J. W., Lee, J. Y., Park, Y. K., and Choi, W. S.: Air Pollution Mitigation Capacity of an Urban Forest in Densely Road-Networked Area: Findings from High-Resolution Sensor Monitoring, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7874, https://doi.org/10.5194/egusphere-egu25-7874, 2025.

EGU25-7939 | Orals | AS3.26

Open waste burning leads to significantly high black carbon exposure amongst burners 

Saloni Vijay, Lennox Khonje, Mwaiwathu Laurent Chatha, and Elizabeth Tilley

Globally, about 14% of households have no option but to burn their waste.  Open waste burning is a significant source of black carbon (BC) emissions, yet the exposure of those engaged in this practice has not been interrogated. This study provides the first quantification of personal exposure to BC emissions from open waste burning, revealing critical insights into the potential health risks faced by individuals engaged in this practice. Between November–December 2023, we conducted a comprehensive field study in Blantyre, Malawi, monitoring BC exposure among 46 volunteers from 23 households over approximately 20 hours on the day waste was burned at their household. Within each household, one individual responsible for burning waste and one non-burner wore MicroAeth MA200 monitors to capture personal exposure data. To summarize exposure, the average BC concentration was calculated for each a) monitoring period, b) for burning times, and c) for non-burning times. The median of these averages was then used to characterize exposure levels. Results showed that waste burners experienced significantly higher BC exposure than non-burners during both burning periods and the overall monitoring period (Wilcoxon signed rank test, p = 0.04). During burning, the median BC exposure for burners was 12.8 μg/m³, over four times higher than the median exposure of non-burners at 2.9 μg/m³. The median BC exposure for burners during the 20-hour monitoring period was 5.1 μg/m³, compared to 3.0 μg/m³ for non-burners. Notably, BC exposure levels during non-burning periods were statistically indistinguishable between burners and non-burners (Wilcoxon signed rank test, p = 0.44), with median exposures of 3.6 μg/m³ and 2.6 μg/m³, respectively. This study highlights the extreme BC exposure faced by individuals actively burning waste, and underscores the health risks associated with this practice and the need for interventions to mitigate exposure.

How to cite: Vijay, S., Khonje, L., Chatha, M. L., and Tilley, E.: Open waste burning leads to significantly high black carbon exposure amongst burners, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7939, https://doi.org/10.5194/egusphere-egu25-7939, 2025.

EGU25-8467 | ECS | Orals | AS3.26

Estimation of carbon dioxide fluxes in the city of Paris using the ICON-ART-CTDAS model 

Nikolai Ponomarev, Pascal Rubli, Grange Stuart, Michel Ramonet, Leslie David, Lukas Emmenegger, and Dominik Brunner

Cities around the globe are aiming to reduce their carbon dioxide emissions, but monitoring and validating urban CO2 emissions is a major challenge. This motivates the ICOS cities PAUL project to use a combination of different measurement and modelling techniques to provide observation-based emission estimates in three pilot cities: Zurich, Paris, and Munich. The challenge comes due to large variations in emissions and concentration gradients, high uncertainties in prior estimates, and inherent modeling errors. Here we present the results of an inverse modeling study for the city of Paris, which builds on the insights gained from similar simulations conducted for Zurich. Our approach employs the state-of-the-art atmospheric mesoscale model ICON-ART, which we ran in conjunction with an ensemble Kalman smoother to optimize CO2 fluxes based on simulated and measured concentration differences.

Paris offers advantages for mesoscale model simulations due to its flat terrain and large size, unlike Zurich, where simulations were challenged by the city's complex topography. Furthermore, the CO2 measurements in Paris, which were collected from a network of 2 tall towers inside and 7 towers outside the city, were easier to represent by the model due to their larger spatial representativeness compared to the more locally influenced rooftops measurements in Zurich.

The ICON-ART model simulations were performed for two offline nested model domains. The outer domain covers Central Europe with a spatial resolution of 6.5 km and was chosen large enough to serve as initial and boundary conditions for the simulations over both Zurich and Paris. The inner, high-resolution domain is centered on the Île-de-France region with a spatial resolution of 1 km. According to our previous experience with Zurich simulations, the atmospheric transport is well simulated by ICON-ART in most weather situations with the exception of low wind conditions, where relative errors in wind speeds and the corresponding dilution of CO2 emitted from the city are the largest. The prior anthropogenic CO2 fluxes were based on the anthropogenic inventory data prepared by AIRPARIF for the Île-de-France area at 0.5 km spatial resolution and on TNOGHGco 2018 data (1 km) for the rest of Europe. Biogenic fluxes were computed online using the Vegetation Photosynthesis and Respiration Model (VPRM), integrated online into ICON-ART.

In this presentation, we analyze the performance of ICON-ART model against meteorological and CO₂ observations in and around Paris, and demonstrate initial results from emission inversion experiments. Furthermore, we contrast the results with those obtained for Zurich to emphasize the different challenges and modelling capabilities in the two cities.

How to cite: Ponomarev, N., Rubli, P., Stuart, G., Ramonet, M., David, L., Emmenegger, L., and Brunner, D.: Estimation of carbon dioxide fluxes in the city of Paris using the ICON-ART-CTDAS model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8467, https://doi.org/10.5194/egusphere-egu25-8467, 2025.

EGU25-8920 | Posters on site | AS3.26

Ozone Flux Measurements and Data Correction in Coastal Megacities in South Korea Busan and Ulsan, South Korea 

Yukyeong Park, Yongmi Park, Subin Han, Jongwon Ryu, and Wonsik Choi

Since the mid-1990s, ozone concentrations in the United States and Europe have steadily declined, whereas South Korea has experienced an increase to this day. Identifying the scientific causes of the ozone increase is essential, which necessitates an accurate understanding of the ozone budget equation. To quantify the ozone budget equation, it also requires measurements of dry deposition velocity. However, the dry deposition velocity is highly uncertain due to surface conditions and turbulence. Eddy covariance (EC) methods are used to measure ozone dry deposition velocities. However, the ozone flux studies using the EC method in Korea have not been conducted to our knowledge. In this study, ozone flux was directly measured using the EC method over approximately one month in the coastal megacities, Busan and Ulsan, in Korea, and here, we present the preliminary results of ozone fluxes and dry deposition velocities in the urban surface of coastal cities.

The preprocessing steps included despike, double rotation, time lag calculation, ozone concentration correction, and detrending. Diurnal variations in ozone concentrations showed a unimodal distribution in Ulsan, a typical pattern for photochemical products, whereas a bimodal distribution was observed in Busan due to a combination of local production and transport from upwind regions. The average daytime ozone flux was -3.1 nmol·m-2·s-1 in Busan and -1.3 nmol·m-2·s-1 in Ulsan. A more detailed discussion, including comparisons with previous studies, will be presented. 

 

Acknowledgments

This work was funded by the Korea Meteorological Administration Research and Development Program under Grant RS-2024-00404042.

How to cite: Park, Y., Park, Y., Han, S., Ryu, J., and Choi, W.: Ozone Flux Measurements and Data Correction in Coastal Megacities in South Korea Busan and Ulsan, South Korea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8920, https://doi.org/10.5194/egusphere-egu25-8920, 2025.

EGU25-9108 | Orals | AS3.26

Bridging the Gap in Emission Reporting: Synergistic Use of AI and Earth Observation for Real-Time Insight on Urban CO₂ Emissions. 

R. Lyana Curier, Sonja Ham, Jetse. J. Stoorvogel, and Stefano Bromuri

Accurate and timely monitoring of urban CO₂ emissions is essential for tracking progress toward climate goals and enabling effective policy interventions. In the Netherlands (NL), emissions arise from industrial, agricultural, and transportation sources. Traditionally, emission reporting in Europe has relied on annual bottom-up inventories based on activity data and emission factors, aggregating emissions from sectors such as energy, transport, industry, and agriculture. While these methods have contributed to reducing anthropogenic emissions, they lack the granularity and timeliness required for real-time decision-making or for tracking progress toward more immediate climate targets. This highlights the urgent need for enhanced spatial and temporal resolution of urban CO₂ emissions data.

This study seeks to address this gap by leveraging a novel approach: using tropospheric NO₂ columns from TROPOMI as a proxy for urban CO₂ emissions. In recent years, a general consensus has been reached that satellite-derived NO₂ from instruments like OMI and TROPOMI are indicative of surface NO₂ concentrations and can be used to estimate top-down NOx emissions. We hypothesize that combining TROPOMI tropospheric NO₂ data with advanced deep learning (DL) methods will enable near real-time estimation of urban CO₂ emissions, offering a high-resolution, dynamic approach to emission monitoring.

Our research focused on the Netherlands, covering the period from 2018 to 2023 for model training and 2024 for validation. Various DL architectures to process TROPOMI data and predict local emissions were evaluated, incorporating ground-based emission inventories and additional metadata. Our goal is to identify the most effective DL models for improving emission estimation accuracy, reducing uncertainty, and enhancing the timeliness of reporting.

Although the initial focus is on the Netherlands, with its well-established monitoring systems (the "brownfields" effect), our methodology has broader applicability for regions with limited emissions data, such as those in developing areas (the "greenfields" effect). 

A key aspect of this research is the development of trustworthy AI, ensuring the deep learning models used are transparent, reliable, and interpretable. By combining cutting-edge AI techniques with Earth observation data and validating the results against ground-based inventories, we created a robust framework for scaling emissions monitoring, especially in regions with limited infrastructure.

How to cite: Curier, R. L., Ham, S., Stoorvogel, J. J., and Bromuri, S.: Bridging the Gap in Emission Reporting: Synergistic Use of AI and Earth Observation for Real-Time Insight on Urban CO₂ Emissions., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9108, https://doi.org/10.5194/egusphere-egu25-9108, 2025.

EGU25-9568 | ECS | Orals | AS3.26

High-Resolution Urban Emission Mapping: Sensor-Driven CO2  Inverse Modeling in Glasgow 

Sandeep Kodoli, Craig Michie, Christopher Davison, Christos Tachtatzis, Naomi Asimow, and Ronald Cohen

This study presents a comprehensive analysis of CO₂ emissions in Glasgow, utilizing a dense network of Berkeley Environmental Air quality and CO2 Network (BEACON) CO2 sensors for the year 2022. The research employs a sophisticated model setup, integrating high-resolution meteorological data from the Weather Research and Forecasting (WRF) model with a Lagrangian Particle Dispersion model for footprint modeling. A Bayesian inversion framework  developed by University of California, Berkeley refines a prior emission inventory using observed CO₂ concentrations and sensitivity footprints. The analysis reveals a 23% increase in overall mean anthropogenic emission for the year 2022 compared to available prior inventory estimate with significant seasonal variations. Winter fluxes  were  70%  higher than prior estimates, driven by increased heating demands and diminished biospheric uptake. Summer showed a 29% reduction, a combined impact of less energy demand for domestic heating and CO₂ uptake . A moderate negative correlation (R² = 0.58) between winter emission episodes and minimum daily temperatures was observed, highlighting the impact of domestic heating on CO₂ emissions. The study also found a 9.8% increase in total posterior emissions on weekends compared to weekdays, a smaller gap than the 21.8% difference in prior values. Our inverse model actively adjusts the emission values based on the real time CO2 measurement from sensors and high-resolution meteorology driven transport model at finer temporal scale, which is very valuable in making adjustments and validating local authority inventory data. Spatial analysis revealed that the most substantial emission changes were concentrated in areas corresponding to the 95th percentile of the posterior-prior emission difference. These regions, consistently exhibiting higher emissions throughout the year, reflect the combined impact of transport and heating sources in the city. These results highlight the urgent necessity for both enhancing building energy efficiency and  targeted strategies to reduce street level vehicular emission. Furthermore, the results point out the importance of continuous, sensor-based measurements for achieving a more precise representation of urban emission sources. This study also examines the impact of Glasgow's Low Emission Zone (LEZ) implemented in June 2023. A comparative analysis of CO₂ emissions and concentrations before and after the LEZ implementation provides insights into its effectiveness in reducing urban emissions. The findings underscore the importance of seasonal variability in emission patterns and the need to account for both anthropogenic activities and natural processes when analysing CO₂ fluxes at finer temporal and spatial scales.

 

 

 

How to cite: Kodoli, S., Michie, C., Davison, C., Tachtatzis, C., Asimow, N., and Cohen, R.: High-Resolution Urban Emission Mapping: Sensor-Driven CO2  Inverse Modeling in Glasgow, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9568, https://doi.org/10.5194/egusphere-egu25-9568, 2025.

The influence of traffic regulations on urban air quality has been discussed for years, especially during the COVID-19 lockdowns, when significant shifts in urban air quality were observed, particularly in the concentration of nitrogen dioxide (NO₂), a key pollutant linked to vehicular emissions and industrial activities. This study provides a long-term analyzes the variation of NO₂ levels in an urban environment, and an investigation of the interplay of various influencing factors during the lockdown periods in Munich, Germany, including traffic volume, wind speed, radiation, boundary layer height, humidity, and precipitation.

Using a combination of ground-based stationary and mobile NO₂ measurements in Munich coupled with traffic flow records, we apply statistical and machine learning techniques to identify the primary drivers of NO₂ concentration variability. The analysis reveals the extent to which reductions in traffic during the lockdown contributed to NO₂ declines, while highlighting the modulating effects of meteorological conditions such as wind dispersion and atmospheric stability.

Our findings provide insights into the complex dynamics of urban air pollution and its sensitivity to human activity and weather patterns. By comparing pre-lockdown, lockdown, and post-lockdown scenarios, the study underscores the potential for targeted interventions to achieve sustained improvements in air quality and offers valuable guidance in designing evidence-based strategies to mitigate urban air pollution and its health impacts.

How to cite: Wenig, M. and Ye, S.: Long-Term analysis of the impact of traffic volume and other influencing factors on urban NO2 levels for interpreting the COVID-19 lockdown effects in Munich, Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9698, https://doi.org/10.5194/egusphere-egu25-9698, 2025.

Within the research project DE-CIST (“Developing Energy Communities with Intelligent and Sustainable Technologies”) a novel, AI-based Energy Demand Simulator has been developed by our project partners. The Energy Demand Simulator determines the energy efficiency and energy saving potential of the residential building stock in Rotterdam (The Netherlands). By adding socio-economic features to the Energy Demand Simulator, the tool will guide policy makers in developing building renovation strategies on different scales, allowing to design household-level renovation packages which consider social, financial, and physical requirements.  

From such building renovation scenarios, we calculated greenhouse gas emissions and the emission reduction potential of the renovation actions. This insight will allow policymakers to optimize the renovation strategies also for climate change mitigation. We conducted a series of high-resolution (100 m²) simulations of CO2 emissions using the Dutch Large Eddy Simulation (DALES) model for the city of Rotterdam. DALES is particularly advantageous due to its explicit simulation of boundary-layer turbulence, enhancing the accuracy of atmospheric transport and dispersion of chemical species in the urban environment. The emission inputs for DALES were refined from the Dutch national emission inventory by incorporating statistical data on household gas consumption specific to Rotterdam. This involves adjusting the emission estimates to reflect high-resolution local consumption patterns and spatial distribution, which improves the spatial accuracy of the modeled emissions. This approach will be extended to reactive gases to gain insights into the exposure of citizens to air pollution in combination with other socio-economic conditions.

How to cite: Los, A. and Doyennel, A.: Greenhouse gas emission reduction from residential building renovations in Rotterdam, The Netherlands, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10364, https://doi.org/10.5194/egusphere-egu25-10364, 2025.

In the last decades, the EU has observed an increase in the use of biomass for energy, and for space heating in particular. Climate change mitigation strategies have favoured the use of wood-based biomass for heat and power supply, to reduce dependency on fossil fuels. However, it can pose risks for ambient air quality and public health, especially when used in small-scale building heating systems in cities. To leverage synergies and avoid trade-offs between climate change mitigation and ambient air quality, policymaking should be supported by quantitative analyses and robust evidence.

This paper presents a framework to assess potential life-cycle greenhouse gas (GHG) emissions and fine particulate matter (PM2.5) impacts on health of wood-based biomass use in small-scale residential heating systems. The framework draws on a life-cycle assessment (LCA) model, and it is applied to 87 EU cities in 23 countries (i) to quantify current GHG and PM2.5 impacts associated wood-based biomass heating, and (ii) to two scenario analyses that evaluate potential trade-offs and co-benefits of climate change and air pollution mitigation actions. A complementary analysis is also performed to provide insight on the robustness of PM2.5 results, comparing health effects associated with PM2.5 using the LCA framework and city-specific emission and effect factors.

Results confirm strong correlation between GHG and PM2.5 impacts. Scenarios for GHG mitigation increased PM2.5 impacts of small-scale biomass heating per capita up to 14%, while those for PM2.5 mitigation reduced PM impacts up to 63%, with GHG mitigation co-benefits (reduction up to 50%) or trade-offs (increase up to 125%). The framework is widely applicable and provides robust results; and the scenario analyses demonstrate the importance of context-specific assessments to inform policymaking.

How to cite: Zauli Sajani, S., Bastos, J., Giuntoli, J., and Pisoni, E.: Assessing synergies and trade-offs between climate change mitigation and air quality effects of small-scale biomass heating in the residential sector, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10545, https://doi.org/10.5194/egusphere-egu25-10545, 2025.

EGU25-11082 | ECS | Posters on site | AS3.26

Air quality issues in therapeutically exposed locations 

Pavel Kalina, David-Aaron Landa, Tomáš Vylita, Eva Schořová, and Jana Walterová

The insufficient density of the air quality monitoring network is a long-standing issue that, at least in the Czech Republic, has yet to be satisfactorily resolved. In practice, greater emphasis is placed on monitoring emissions rather than immission (ambient emissions). Air quality measurements are, in most cases, conducted at the sources of polluting gases (CO, CO₂, SO₂, NOₓ). Monitoring stations are often located in areas with heavy industry. However, more detailed information on air quality is missing in places where air interacts directly with the respiratory system, such as urban agglomerations of various sizes. An illustrative example is that the Czech Hydrometeorological Institute (ČHMÚ) does not operate monitoring stations in all regional cities. This results in a critical deficiency of objective information on air pollution across the entire territory.

Insufficient information on long-term pollutant concentrations in the air is also a significant issue in locations where climatic conditions have, or could have, therapeutic benefits—specifically, in spa locations. Some areas with favorable climatic conditions (e.g., those with clinically proven benefits for cardiac patients) are certified as climatic spas under the Spa Act. However, stringent air quality standards are also required for all other spa locations. The absence of direct monitoring of tropospheric air pollution in the centres of most spa locations poses a challenge because pollution levels are estimated using mathematical models based on data collected from nearby or more distant surroundings.

To address this issue, a mobile air quality station will be procured as part of the SRC (Spa Research Centre) transformation project. The station will be capable of analyzing concentrations of various pollutants, including CO, SO₂, NOₓ, suspended particles (PM2.5, PM10), selected volatile organic compounds (e.g., benzene as a representative of VOC), selected heavy metals (e.g., Be, Cr, Cd, Ni, Pb, As, Zn), and polycyclic aromatic hydrocarbons. Moreover, the station will be equipped to transmit the collected data online in real time. The project aims to establish baseline air quality values for the most significant spa locations. These values will serve as the foundation for defining the parameters of the so-called "spa therapeutic landscape." This definition will facilitate the specification of air quality limits necessary to ensure the sustainable preservation of the favorable climate in spa locations and its associated therapeutic effects.

Initial results from measurements in the spa towns of Karlovy Vary and Lázně Kynžvart indicate that air quality in the centers of spa towns is significantly better than in areas without spa functions. This improvement can be attributed to factors such as restrictions on passenger and freight transport and other anthropogenic activities implemented to maintain the protective regime for spa clients. These findings align with observations that locations with high levels of vehicular traffic experience increased concentrations of pollutants such as NOₓ.

The primary goal of the ongoing project is to enhance detailed air quality monitoring and facilitate the establishment of air quality limits for locations where the therapeutic use of favorable climatic conditions supports the treatment of the human body.

Research within the SRC project is funded by JTF CZ 10.01.01/00/22_001/0000261.

How to cite: Kalina, P., Landa, D.-A., Vylita, T., Schořová, E., and Walterová, J.: Air quality issues in therapeutically exposed locations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11082, https://doi.org/10.5194/egusphere-egu25-11082, 2025.

EGU25-11091 | ECS | Orals | AS3.26

Particulate matter deposition on roadside trees in urban area: Evaluation of Elemental carbon and magnetic minerals. 

Laurence Delville, Jean-François Léon, Mélina Macouin, Maria Dias Alves, Océane Lenoir, and Loic Drigo

In France, 97% of cities exceed the WHO guide values for PM2.5 (2022 data). The transport sector is responsible for about 10% of PM2.5 emissions. The development of green infrastructure along roads, among other ecosystem services, could enable air pollution removal by deposition and needs to be better quantified and monitored.

We studied the chemical composition of particle deposits and the temporal evolution of the quantity of deposits on tree leaves over a 9-month period in Toulouse (~500,000 inhabitants), France. Leaf samples were taken from 9 deciduous trees and 2 evergreen trees at three roadside sites. We analyzed the deposition of elemental carbon (EC) and magnetic minerals on the leaf surface of different tree species. The EC deposit was extracted from the leaves using double-deionized water for on-surface deposition and chloroform for in-wax deposition. EC deposit was then estimated using thermo-optical techniques. Total magnetic mineral deposition was analyzed directly on total leaves by acquiring saturation isothermal remanent magnetization (SIRM) using a JR6 magnetometer.

Our results show that the average on-surface EC and total magnetic minerals deposit were respectively 4 and 12 times higher for evergreen than for deciduous trees. On-surface EC for evergreen trees was 2 times lower than in-wax EC. In contrast, on-surface EC for deciduous trees was found 11 times higher than in-wax EC. The analyses enabled the interpretation of changes in particle deposition over time as a function of meteorological conditions. Our results highlighted the potential of leaves to be used as biosensors to monitor ambient air pollution.

How to cite: Delville, L., Léon, J.-F., Macouin, M., Dias Alves, M., Lenoir, O., and Drigo, L.: Particulate matter deposition on roadside trees in urban area: Evaluation of Elemental carbon and magnetic minerals., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11091, https://doi.org/10.5194/egusphere-egu25-11091, 2025.

EGU25-11481 | Orals | AS3.26

Optimizing Air Quality Sensor Networks Using Gaussian Process Regression and Global Optimization Techniques 

Anton Sokolov, Hervé Delbarre, and Khaoula Karroum

Despite recent advancements in technology and purification techniques, industrial pollution continues to pose significant challenges in terms of human exposure and monitoring of air quality close to sources. Optimizing air quality networks and integrating them with advanced spatiotemporal statistical methods is thus essential for effective monitoring of atmospheric contamination.

This study addresses the problem of optimizing the placement of sensors for measuring air pollution at urban and regional scales. Several global optimization techniques, including the GlobalSearch Algorithm, Genetic Algorithm, and Particle Swarm Optimization, are applied to this problem.

Two interpolation methods are used to estimate contamination levels at control points: the standard triangulation-based Natural Neighbour interpolation method for scattered data and Gaussian Process Regression (GPR), which employs covariances derived from a dynamic pollution transfer model. The GPR technique is particularly suitable for simulating smoke-like, narrowly directed industrial pollution at distances of less than a few tens of kilometres from the source.

Numerical experiments were conducted using two pollution datasets: aerosol (PM10) concentrations simulated by the ADMS model for the Dunkirk region in northern France and sulphur dioxide (SO2) concentrations simulated by the CALPUFF model for the Dnipropetrovsk region in Ukraine. The first dataset involves diffuse pollution from multiple anthropogenic and natural sources, while the second involves emissions from industrial point sources.

Optimal sensor placements are identified, and estimation errors are evaluated for the interpolation methods and datasets. The described method could allow the construction of effective air quality networks for different types of atmospheric pollution and provide a means to estimate their effectiveness.

How to cite: Sokolov, A., Delbarre, H., and Karroum, K.: Optimizing Air Quality Sensor Networks Using Gaussian Process Regression and Global Optimization Techniques, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11481, https://doi.org/10.5194/egusphere-egu25-11481, 2025.

EGU25-11711 | ECS | Orals | AS3.26

High-Resolution Quantification of Biogenic CO2 Fluxes over a Metropolitan Area 

Qing Luo, Ricard Segura-Barrero, Alba Badia, Thomas Lauvaux, Junwei Li, Jia Chen, and Gara Villalba

Cities are hot spots on greenhouse gas (GHG) emissions, yet green infrastructure (GI) such as green spaces and parks provides potential solution for reducing urban carbon footprints through photosynthetic uptake and carbon sequestration. Studies have shown that the offset of urban vegetation uptake on local anthropogenic CO2 emissions varies between 2% and 100%, underscoring the complexity associated with this solution. Quantifying CO2 capture by GI is challenging due to the interplay of photosynthetic uptake and respiration, seasonal variability, the heterogeneous distribution of GI, urban climate, and soil conditions. While biosphere models have been used to quantify carbon exchange processes, they are often employed at the ecosystem level and at coarse spatial resolutions(10-100km), making them insufficient for capturing biospheric signals at the urban scale(10m-1km). Therefore, high-resolution quantification of biogenic CO2 fluxes is essential for understanding their role on urban GHG budget.

This study estimates biogenic CO2 fluxes for 2023 in the Metropolitan Area of Barcelona (AMB) at a 10 m resolution using the Vegetation Photosynthesis and Respiration Model (VPRM). Our approach integrates vegetation indices derived from Sentinel-2, a detailed vegetation land cover dataset constructed by merging local land cover and tree maps, and meteorological inputs (temperature and shortwave radiation) from the Weather Research and Forecasting (WRF) model coupled with an urban canopy scheme that better represents atmosphere exchanges inside the urban canyons. A sensitivity analysis is conducted comparing different VPRM configurations including flux parameterization, input satellite-derived vegetation indices and modifications to land cover map. To constrain the modelled biogenic CO2 emissions and determine their uncertainties, the estimated biogenic fluxes are evaluated with atmospheric CO2 mixing ratios observations from the AMB GHG monitoring network using an atmospheric transport model (WRF-Chem) in a passive tracer approach. This research presents an improved method to estimate the urban biogenic CO2 fluxes and provides guidance for improving and creating more robust ways of accounting for the contribution of urban green to aid policy and urban planners in the design and implementation of GI.

How to cite: Luo, Q., Segura-Barrero, R., Badia, A., Lauvaux, T., Li, J., Chen, J., and Villalba, G.: High-Resolution Quantification of Biogenic CO2 Fluxes over a Metropolitan Area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11711, https://doi.org/10.5194/egusphere-egu25-11711, 2025.

EGU25-12094 | Orals | AS3.26

Investigating the impact of cold-starts on the distribution of vehicle emissions in the Greater Toronto Area 

Alexandra Corapi, Jennifer Murphy, Mark Panas, Eric Ward, Debra Wunch, Sébastien Ars, and Felix Vogel

Vehicle emissions are a significant source of greenhouse gases and air quality pollutants in urban areas, yet current city-scale CO and CO2 emission inventories may not accurately reflect real-world conditions. In Toronto, Canada, traffic emissions contribute to approximately one third of the city’s total CO2 emissions. As a part of the Toronto Atmospheric Monitoring of Emissions (TAME) project, the goal of this work is to investigate the emission signatures of the vehicle fleet in the Greater Toronto Area (GTA) under different engine operating conditions and seasons. Specifically, we are interested in the role of ‘cold-start’ emissions (i.e. emissions during the engine and catalyst warm-up period) on the distribution of CO emissions in the GTA. As exhaust aftertreatment technologies improve for gasoline engines, air quality emissions that occur before the catalytic converter has warmed are expected to contribute an increasing, and possibly dominant, proportion of non-CO2 vehicle emissions. Simultaneous measurements of CO and CO2 were collected by deploying calibrated low-cost sensors in parking garages at the University of Toronto over several months. To calculate the CO and CO2 enhancements from each vehicle emission plume, a peak-finding algorithm was developed. The ΔCO/ΔCO2 ratio of the enhancements is used as an emission signature for each vehicle. The results from this study are compared to mobile and stationary measurement campaigns conducted by Environment and Climate Change Canada using a high precision analyzer (cavity ring-down spectrometer (CRDS)).  We assess the impact of choices made about data collection, peak-finding, and cold-start definitions. Using one approach, the range of ΔCO/ΔCO2 ratios observed is 0.1 to 779 ppb CO/ ppm CO2, with a median of 14 ppb CO/ ppm CO2. On average, the cold-start emission ratios are observed to be at least 2 times greater than those of warm vehicles. These results can be used to update CO and CO2 emission inventories to more accurately capture activity patterns and independently verify emission reductions as urban vehicle fleets transition to electric.

How to cite: Corapi, A., Murphy, J., Panas, M., Ward, E., Wunch, D., Ars, S., and Vogel, F.: Investigating the impact of cold-starts on the distribution of vehicle emissions in the Greater Toronto Area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12094, https://doi.org/10.5194/egusphere-egu25-12094, 2025.

EGU25-12146 | ECS | Posters on site | AS3.26

Mechanisms of Surface Ozone's Chemical Response to High Temperatures: Differences Between Urban and Rural Areas 

Chang Su, David Stevenson, and Massimo Bollasina

As climate change leads to more frequent and intense high-temperature events, elevated O3 episodes during periods of extreme heat have raised widespread concerns. This research investigates how O3's chemical response to elevated temperatures varies between urban and rural areas, particularly focusing on different emission conditions defined by ozone precursor regimes.

Simulations are carried out using the UKCA Box Model under idealised meteorological conditions. It runs chemistry-only zero-dimensional experiments in a single grid cell with chemistry relevant to the troposphere and the stratosphere. Using the UKCA Box Model, we simulated conditions typical of summer 2022 at three global hotspots (Yangtze River Delta, England and California), analysing scenarios where O3 precursors are either limited by VOCs in urban environments or by NOx in rural settings. The simulations were conducted across a temperature range of 20°C to 40°C while controlling for relevant factors such as photolysis, humidity, emissions, and initial concentrations. To determine the O3 precursors regimes, photochemical indicators such as NOy, H2O2/HNO3, H2O2/(O3+NO2) and HCHO/NO2 were employed.

The results suggest a significant diversity of O3’s chemical response to temperature in urban and rural areas. In urban areas characterised by VOC-limited conditions, O3 levels exhibited a nearly linear increase with rising temperatures. In contrast, rural areas, where O3 is typically NOx-limited, displayed a more complex relationship where negative correlations were found. Additionally, humidity emerged as a critical factor influencing these chemical dynamics. The mechanism by which O3 responds chemically to temperature changes will be examined by analysing O3 production and destruction budgets.

Our findings highlight that the O3 precursor regimes are crucial in evaluating the impact of temperature responses on ozone from a chemical perspective. This research contributes valuable insights into the mechanisms driving O3 responses to temperature changes during extreme heat events. It underscores the importance of considering urban and rural differences in ozone studies and can inform future emission control strategies aimed at mitigating ozone pollution under varying temperature conditions.

Keywords: Surface ozone; Temperature response; UKCA Box model; O3 precursor regimes; Urban and rural

How to cite: Su, C., Stevenson, D., and Bollasina, M.: Mechanisms of Surface Ozone's Chemical Response to High Temperatures: Differences Between Urban and Rural Areas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12146, https://doi.org/10.5194/egusphere-egu25-12146, 2025.

EGU25-12815 | Orals | AS3.26

Determination of equivalent Black Carbon Concentrations by MABI (Multi-Wavelength Absorption Black Carbon Instrument) and of the respective mass absorption cross section (MAC): Case study for Krakow, Poland and Athens, Greece. 

Lucyna Samek, Evangelia Diapouli, Anna Ryś, Stefanos Papagiannis, Vassiliki Vassilatou, Rakshit Jakhar, and Konstantinos Eleftheriadis

Equivalent black carbon (eBC) is generated from the partial combustion of fossil fuels and biomass. The scientific interest in eBC is large because its contribution to the PM2.5 fraction is high, especially in urban areas. It should be noted that combustion-related aerosols (including eBC) have been linked to adverse health effects and are considered more harmful than other aerosol components. In addition, eBC is considered the second most important component of global warming in terms of direct forcing. Until now. there is a lack of information on eBC concentrations in Poland, mostly due to lack of relevant instrumentation. The position of Poland in the center of Europe, as well as the presence of multiple combustion sources, make this type of measurements and data very relevant to the scientific community, both for health impact assessment and climate change studies. In the present study, the MABI (Multi-Wavelength Absorption Black Carbon Instrument), a new instrument measuring light transmission of particles collected on filters, was assessed.  MABI was developed by the Australian Nuclear Science and Technology Organization (www.ansto.gov.au). The instrument consists of an optical assembly and electronic case. The instrument optics includes, among others, the multi-wavelength light source (7 LEDs), sampler holder, and photodetector. In the instrument, opaque glass is used to scatter the scattered light back through the filter to the detector. MABI offers the advantage of off-line measurements of aerosol light transmission, at seven fixed wavelengths (from 405 nm to 1050 nm). The performance of the instrument was assessed for different types of filters (Teflon and quartz fibre) collected at two distinct atmospheric environments, an urban background site in Krakow, Poland and an urban background site in Athens, Greece. Mass absorption coefficients provided by the manufacturer were used in order to calculate eBC from light transmission data (Ryś and Samek, Atmosphere, 2022). In addition, thermo-optical analysis (Lab OC-EC Aerosol Analyzer, Sunset Laboratory Inc.) was performed on the quartz fibre samples for the determination of elemental carbon (EC) concentrations. EC data were then used in order to calculate site-specific mass absorption cross section (MAC) values for the MABI. Finally, an aethalometer (AE33, Aerosol Magee Scientific) was used in parallel to PM sampling in Athens, in order to provide a reference eBC value, against which the performance of MABI was assessed.

Acknowledgments: This research project was supported by the program “Excellence initiative—research university” for the University of Science and Technology and ATMO ACCESS TNA project

How to cite: Samek, L., Diapouli, E., Ryś, A., Papagiannis, S., Vassilatou, V., Jakhar, R., and Eleftheriadis, K.: Determination of equivalent Black Carbon Concentrations by MABI (Multi-Wavelength Absorption Black Carbon Instrument) and of the respective mass absorption cross section (MAC): Case study for Krakow, Poland and Athens, Greece., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12815, https://doi.org/10.5194/egusphere-egu25-12815, 2025.

EGU25-12873 | ECS | Posters on site | AS3.26

CHETNA-Traffic: Street level CO2 and pollutant emission analysis from road traffic in Indian cities 

Rohith Teja Mittakola, Philippe Ciais, Marc Barthelemy, Qinren Shi, Xavier Bonnemaizon, Nicolas Megel, Harish Phuleria, and Chuanlong Zhou

India, a rapidly developing economy with the world’s largest population, has set an ambitious target of achieving net-zero carbon emissions by 2070. Road transport, contributing to 12% of India’s energy-related CO2 emissions, plays a significant role in exacerbating urban air pollution. Given the country’s swift urbanization and the expansion of road transport to meet mobility demands, CO2 emissions from this sector could potentially double by 2050, risking the achievement of long-term climate objectives. Our study presents a comprehensive analysis of traffic emissions across India, leveraging high-resolution mobility data at street level, including vehicle count, types, and speeds for 100 different Indian cities. We use statistical and machine learning methods to improve data quality and extrapolate mobility data to all city traffic using city-level vehicle registration data. Here, we focus on understanding traffic and congestion patterns within and between cities, using additional data on population, urban structure, road network, public transport supply, and socio-economic variables. Finally, we simulate hourly CO2 and pollutant emissions at a street level using the COPERT model, which includes speed and vehicle-type dependent emission factors. With this study, we also aim to explore scenarios for reducing pollution, a critical issue for Indian metropolises. The findings from this study will provide valuable insights into the environmental impact of road traffic in India and inform strategies for pollution reduction. This work is part of the CHETNA project (City-wise High-resolution carbon Emissions Tracking and Nationwide Analysis), which leverages artificial intelligence and advanced datasets to deliver high-resolution, near real-time daily CO2 and air pollutant emissions data for over 100 Indian cities. 

How to cite: Mittakola, R. T., Ciais, P., Barthelemy, M., Shi, Q., Bonnemaizon, X., Megel, N., Phuleria, H., and Zhou, C.: CHETNA-Traffic: Street level CO2 and pollutant emission analysis from road traffic in Indian cities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12873, https://doi.org/10.5194/egusphere-egu25-12873, 2025.

EGU25-13038 | ECS | Posters on site | AS3.26

Comparative Analysis of Indoor Air Quality and Health Risk Assessment in Academic Workspaces in India and Australia 

Sarup Das, Gopika Indu, Shiva Nagendra SM, and Sotiris Vardoulakis

Indoor air quality (IAQ) in workplaces significantly impacts occupational health and productivity, necessitating comparative evaluations across diverse environments. This study investigates particulate matter (PM) concentrations in indoor academic workspaces in Chennai, India, and Canberra, Australia, using the GRIMM 11D aerosol spectrometer. A 12-hour monitoring campaign was done in IIT Madras, India, and ANU, Australia for 3 days during the post-winter (Spring) season. It measured the PM1, PM2.5, PM4, and PM10 levels in the indoor workspaces offering insights into PM concentrations.

The average PM concentrations in Chennai were significantly higher than in Canberra. Indian workplaces recorded PM1, PM2.5, PM4, and PM10 levels of 4.03±1.09, 8.28±2.15, 12.36±4.26, and 15.83±6.43 (µg/m³), respectively. Corresponding Australian values were notably lower, at 1.53±0.47, 2.82±1.02, 3.52±1.69, and 4.14±2.72 (µg/m³), respectively. Spikes in PM10 levels in both regions suggest occasional localized pollution events or episodic pollutant intrusions, influencing PM concentrations. Additionally, the fine PM fractions (PM1 and PM2.5) were more prominent in Canberra, indicating potential variations in pollutant sources and infiltration rates.

Health risk assessments were performed by simulating lung deposition dosages for males and females using the ‘Symmetric Lung’ configuration within the Multiple Path Dosimetry Model (MPPD). The model revealed stark contrasts in PM lung deposition doses between the two regions, with Indian workplaces presenting significantly higher health risks. In Chennai, male dosages for PM1, PM2.5, PM4, and PM10 were 4.23, 22.16, 38.98, and 56.41 µg, respectively, while females experienced slightly lower dosages of 2.79, 12.99, 23.33, and 34.70 µg. In Canberra, the respective values for males were 1.61, 5.80, 9.14, and 12.33 µg, and for females, 1.05, 3.40, 5.41, and 7.46 µg. These findings highlight a significantly higher health risk for workers in Chennai, with females in both locations receiving lower doses due to smaller lung capacities and breathing rates.

This pilot study brings out substantial regional differences in IAQ, shaped by environmental factors, building ventilation standards, and external pollutant sources and infiltration rates. Elevated PM concentrations in Chennai signal a pressing need for interventions to enhance workplace air quality, such as improved filtration and ventilation systems and awareness campaigns. Meanwhile, the finer PM fraction in Canberra warrants attention due to its deeper penetration into the respiratory tract and long-term health implications.

Further research should address long-term exposure risks, seasonal variability, and effective mitigation strategies to improve IAQ and safeguard academic workforce health in diverse geographical settings.

How to cite: Das, S., Indu, G., Nagendra SM, S., and Vardoulakis, S.: Comparative Analysis of Indoor Air Quality and Health Risk Assessment in Academic Workspaces in India and Australia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13038, https://doi.org/10.5194/egusphere-egu25-13038, 2025.

EGU25-13794 | Posters on site | AS3.26

Coop'Air : a participatory research initiative to monitor classrooms indoor air quality in classrooms through combined measurements of active devices and biosensors (France, Ivory Coast and Brazil). 

Sonia Rousse, Aude Calas, Volia Belleville, Hélène Gauthier, Astrid Avellan, Sylvain Gnamien, Regina de Miranda, Loic Drigo, Valentin Labelle, Adama Bakayoko, Fatima de Andrade, and Laure Laffont

Ensuring good air quality in children's environments is recognized as a critical public health issue, which raises the question of monitoring indoor air quality (IAQ) in classrooms as poor air quality affects children's health and academic performance. To better understand the dynamics that affect classroom air quality in urban environments, we examined some physical characteristics of the classroom, including ventilation and occupancy in contrasting contexts. A combined set of low-cost optical devices, CO2, humidity and temperature sensors as well as passive biosensors (Tillandsia usneoides, tree barks) was implemented in 5 classrooms in the urban context of the medium-sized Toulouse city (France), 3 classrooms in the West African capital city of Abidjan (Ivory Coast) and 2 classrooms in the megacity of Sao Paulo (Brazil). Concentrations of particulate matter (PM), CO2 and comfort data (humidity and temperature) were monitored every 2 minutes over more than 6 months in 2024.  Processing the data according to whether the class is occupied or not allows to assess the impact of the presence of children and their activities on IAQ. Besides, the elemental composition of PM deposited on biocaptors exposed in the classroom, analyzed by ICP-MS for Toulouse and Abidjan, allows the identification of PM sources within classrooms. The results are part of the Coop’Air participatory research experiment designed by an interdisciplinary team to co-construct with the children appropriate measures to improve indoor air quality in their classroom.

How to cite: Rousse, S., Calas, A., Belleville, V., Gauthier, H., Avellan, A., Gnamien, S., de Miranda, R., Drigo, L., Labelle, V., Bakayoko, A., de Andrade, F., and Laffont, L.: Coop'Air : a participatory research initiative to monitor classrooms indoor air quality in classrooms through combined measurements of active devices and biosensors (France, Ivory Coast and Brazil)., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13794, https://doi.org/10.5194/egusphere-egu25-13794, 2025.

EGU25-14270 | ECS | Posters on site | AS3.26

Advanced Oxidation-Based System for Odor and Cooking Fume Reduction in Korean Barbecue Restaurants: Long-Term Evaluation and Impact Analysis 

Hyeokjin Oh, Seung-Yol Yoo, Kyung-Suk Cho, and Hee-Wook Ryu

In typical Korean-style barbecue restaurants, either customers or employees grill meat directly at the table using charcoal or natural gas as fuel. During the direct grilling process, significant amounts of odor and cooking fumes, including particulate matter (PMs) and volatile organic compounds (VOCs), are generated, resulting in numerous complaints from neighboring residents. To address this issue, this study developed an abatement system that can simultaneously remove PMs, odors, and VOCs using a filtration device and an advanced oxidation agent. A 50 m³/min capacity abatement device, capable of treating polluted air emitted from approximately 20 barbecue tables, was installed in a restaurant, and its performance was evaluated over 18 months.

The abatement system comprises (1) a dry advanced composite oxidation and adsorption layer, (2) a membrane filter utilizing advanced oxidants and adsorbent powders as filter aids, and (3) a real-time monitoring system for odor, VOCs, and PMs at the inlet and outlet.

During the entire operation period, the average concentration of complex odor in the exhaust gas, expressed as air dilution ratio, was 606±811. After treatment by the abatement system, the complex odor concentration was reduced to 50±96, meeting the odor management standards stipulated by the Korean Odor Prevention Act. Additionally, the system demonstrated stable reduction efficiencies of 86.6±15.0% for PM10 and 86.2±14.5% for VOCs.

Seasonal variations in emission characteristics were observed. The highest complex odor concentration occurred in winter (865±962 OU), followed by autumn (689±811 OU), summer (456±715 OU), and spring (444±757 OU). PM10 concentration peaked in autumn (2,060±8,957 μg/m³), followed by summer (1,335±7,736 μg/m³), spring (638±5,228 μg/m³), and winter (462±3,328 μg/m³). The VOC concentration was highest in autumn (0.35±1.13 ppm) and similar in summer (0.25±0.72 ppm) and winter (0.25±0.90 ppm).

Despite significant seasonal fluctuations in pollutant emissions, the abatement system provided stable operation and reduction performance. Regardless of the season, the average complex odor concentration at the outlet was maintained at 50±95, PM10 concentration was reduced by over 90% to an average of 215±621 μg/m³, and VOC removal efficiency was stably maintained at 88.0±15.7%.

The impact of installing the abatement system on air quality improvement around the restaurant was analyzed using the CALPUFF modeling system. The results confirmed that the system effectively reduced the diffusion of odors and cooking fumes, significantly improving the air quality in the surrounding area. In conclusion, this study suggests that a dry advanced oxidation-based system offers a practical and scalable solution for stable performance under various operating conditions and seasonal factors, contributing to air quality improvement and the protection of public health.

 

Acknowledgements

This research was supported by Basic Science Research Program through the National Research Foundation of Korea(NRF) funded by the Ministry of Education (2020R1A6A1A03044977)

How to cite: Oh, H., Yoo, S.-Y., Cho, K.-S., and Ryu, H.-W.: Advanced Oxidation-Based System for Odor and Cooking Fume Reduction in Korean Barbecue Restaurants: Long-Term Evaluation and Impact Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14270, https://doi.org/10.5194/egusphere-egu25-14270, 2025.

EGU25-14289 | Orals | AS3.26

Urban Air Quality and Greenhouse Gases from Recent Airborne Field Campaigns in the United States 

Steven Brown, Wyndom Chace, Caroline Woamck, Nell Schafer, and Jeff Peischl and the The AEROMMA and AiRMAPS Teams

The NOAA Chemical Sciences Laboratory has led a series of recent airborne campaigns in the U.S. to investigate urban air quality, emissions and greenhouse gases.  The Atmospheric Emissions and Reactivity Observed from Megacities to Marine Areas (AEROMMA) flew the three largest U.S. cities (New York, Chicago and Los Angeles) in 2023 on the NASA DC-8 with a comprehensive suite of trace gases, aerosols, radiation and meteorology.  The Airborne and Remote Sensing Methane and Air Pollutant Surveys (AiRMAPS) is a series of campaigns sampling urban areas and oil and gas basins over 3 years.  Airborne measurements during AEROMMA probed nonlinear O3 photochemistry in New York, Chicago and Los Angeles. The mean ozone production efficiency (OPE), the ratio of Ox (O3 + NO2) to NOx oxidation product enhancements, were 9 ± 4 (1 s), 6 ± 3 and 6 ± 3 ppbv ppbv-1, respectively. OPE exhibited a nonlinear, inverse dependence on total reactive nitrogen (NOy, a proxy for initial NOx) and a positive correlation with ∆VOC/∆NOy. A zero-dimensional photochemical model supports these observed OPE dependences on NOx and VOCs and shows that OPE is a distinct metric from total O3 production that may be informative to the development of O3 pollution control strategies.  AEROMMA flights also quantified the magnitude and sources of urban methane (CH4) emission from in-situ measurements of CH4, CO­­2, CO, and C2-C5 alkanes in Los Angeles. Using the CA Air Resources Board CO emissions inventory alongside CH4/CO enhancement ratios, the analysis determines summertime CH4 and C2–C5 alkanes emissions.  Roughly half of Los Angeles CH4emissions are from natural gas sources and half from sources such as landfills and dairies.   Comparison to historical aircraft campaigns from 2010-2023 shows declining CH4 but increasing ethane emissions, with the latter due to changes in pipeline natural gas ethane content.

How to cite: Brown, S., Chace, W., Woamck, C., Schafer, N., and Peischl, J. and the The AEROMMA and AiRMAPS Teams: Urban Air Quality and Greenhouse Gases from Recent Airborne Field Campaigns in the United States, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14289, https://doi.org/10.5194/egusphere-egu25-14289, 2025.

EGU25-14294 | Orals | AS3.26

In situ measurements of emissions from Kwabia Ghana 

Wade McGillis, Charles Apraku, Steve Chillrud, and Patricia Culligan

Continuous measurements of carbon dioxide and black carbon emissions in Kwabia Ghana are presented.  The community is discrete and dominated by wood burning.  Here a mass balance array is deployed to measure upstream and downstream concentrations of black carbon, PM2.5, and carbon dioxide.  A report on the 2022 deployment demonstrates that top-down flux measurements using a plume superposition modeling technique is innovative and comprehensive. Accurate measurements of carbon dioxide and black carbon provides a combined quantification of the dynamics of green house gas emissions, particle/air-quality emissions, and the devastating impact of deforestation.  Results show that morning and evening cooking time introduce dangerous levels on air-quality and the subsequent emission of carbon dioxide to the atmosphere. 

How to cite: McGillis, W., Apraku, C., Chillrud, S., and Culligan, P.: In situ measurements of emissions from Kwabia Ghana, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14294, https://doi.org/10.5194/egusphere-egu25-14294, 2025.

EGU25-14619 | Orals | AS3.26

Capturing urban methane emissions with commercial aircraft profiles 

Colm Sweeney and Vanda Grubisic
For decades, our understanding of the carbon cycle has relied on a limited network of direct and remote sensing systems to measure atmospheric greenhouse gases (GHGs). This has allowed for a broad understanding of both natural and human-caused sources and sinks of GHGs. However, this network is inadequate to monitor the subtle emission changes resulting from climate change, mitigation efforts, and interventions. Moving forward, new technologies, combined with existing ones, will need to be enhanced through public-private partnerships to build a network capable of verifying GHG emissions and uptake from global to local scales.

 

The recent collaboration between NOAA and United Airlines exemplifies the growing partnerships with the private sector to enhance GHG observation. By leveraging commercial aircraft flights, United Airlines is providing a platform that enables up to eight atmospheric profiles daily at a fraction (1%) of the cost of similar research aircraft. 

The low cost and increased frequency of these observations are further enhanced by the opportunity to sample large metropolitan areas frequently visited by mid-size aircraft like the Boeing 737. These profiles bridge the gap between ground-based direct measurements and satellite-based remote measurements, essential for monitoring GHG emissions across all scales. Enhancement ratios of methane to CO2 and CO captured by these profiles also enables a unique look at methane emissions for urban environments that have proven to be under estimated based on bottom up inventory estimate of emissons.

This talk provides an overview and update of NOAA's effort to leverage commercial aircraft for GHG observation.

How to cite: Sweeney, C. and Grubisic, V.: Capturing urban methane emissions with commercial aircraft profiles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14619, https://doi.org/10.5194/egusphere-egu25-14619, 2025.

EGU25-14898 | Orals | AS3.26

The impact of metropolitan's Air Quality Policies on air pollution improvement in Taiwan 

Hsin-Ling Chang, Hsin-Chih Lai, Min-Chuan Hsiao, and Li-Wei Lai

In recent years, the impact of air quality on health has drawn significant attention. The World Health Organization has highlighted that prolonged exposure to high concentrations of PM2.5 can increase the incidence and mortality rates of cardiovascular and respiratory diseases, as well as elevate the risk of premature death, particularly among highly sensitive populations. Therefore, reducing air pollution levels and developing air quality policies require collaborative efforts from both the government and the public.

This study uses the WRF-CMAQ model to evaluate the inter-regional interactions of PM2.5 and to assess the emission reduction benefits of the State Implementation Plan (SIP) implemented by Taiwan's six major cities. Taipei City, New Taipei City, Taoyuan City, Taichung City, Tainan City, and Kaohsiung City are Taiwan's primary urban centers, and their air pollution control efforts are essential for improving environmental quality nationwide.

The SIP measures in the six metropolitan focus on three major sources of pollution. For stationary sources, the policies include stricter standards for large emitters such as factories and coal-fired power plants, along with the promotion of low-pollution technologies. For mobile sources, the measures involve phasing out high-polluting vehicles, increasing the adoption of electric vehicles, and improving public transportation systems. For non-stationary sources, efforts are directed at strengthening the monitoring and control of construction dust and agricultural burning.

The policy's effectiveness is reflected in significant emission reductions: Taipei reduced PM2.5 emissions by 283 tons; New Taipei, by 72 tons; Taoyuan, by 599.4 tons; Taichung, by 73.3 tons; Tainan, by 2,150 tons; and Kaohsiung, by 2,043 tons. For instance, in Taichung, the latest SIP measures are expected to reduce PM2.5 concentrations from 16.8 μg/m³ to 15.7 μg/m³, a 7% improvement.

Despite these achievements, inter-regional pollutant transport continues to affect the six metropolitan, particularly in southern Taiwan. Future policies must balance regional pollutant transport, climate change, and economic development needs. Moreover, collaboration with neighboring countries will be essential to reduce transboundary pollution.

Overall, the SIP policies implemented in Taiwan's six metropolitan areas have successfully improved air quality and offer valuable insights for reducing air pollution. However, continuous adjustments and strategic refinements will be necessary to address emerging challenges and ensure the long-term effectiveness of these policies.

How to cite: Chang, H.-L., Lai, H.-C., Hsiao, M.-C., and Lai, L.-W.: The impact of metropolitan's Air Quality Policies on air pollution improvement in Taiwan, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14898, https://doi.org/10.5194/egusphere-egu25-14898, 2025.

EGU25-14947 | ECS | Orals | AS3.26

Carbon Sequestration across Urban Vegetation Types in Changing Climate in Finnish Cities 

Aarni Koiso-Kanttila, Leif Backman, and Liisa Kulmala

Urbanisation and climate change are global megatrends. Currently, more than half of the world's population lives in urban areas and this number is expected to increase in the future. Urban areas are vulnerable to climate change-induced extreme weather events due to urban characteristics such as the urban heat island (UHI), but are also large sources of anthropogenic greenhouse gas emissions. Urban green spaces are increasingly being explored as a solution to offset these emissions and adapt to climate change in cities. Our knowledge of urban carbon sequestration is mainly derived from research in natural ecosystems and is lacking in the urban context. Urban environments are characterized by a high degree of complexity due to their fragmented and heterogeneous nature and intensive anthropogenic management and modification. More knowledge on carbon sequestration in different urban vegetation types and the influence of management is needed to guide the planning of resilient and climate-smart urban green spaces.

Here, the JSBACH, a process-based land surface model, was used to understand how carbon sequestration in different Nordic urban vegetation types responds to possible future climates in Finnish cities. JSBACH, previously tested for urban conditions in Helsinki, was used to simulate seven urban vegetation types in 20 Finnish cities between the years 2006 and 2100. The urban vegetation types used were urban lawn, park site with Tilia cordata, urban birch-dominated forest, mesic meadow and dry meadow. In addition, irrigated versions of urban lawn and park with Tilia cordata were also simulated. JSBACH was driven by daily EURO-CORDEX data from global models CanESM2, MIROC5 and CNMR-CM5 using  RCP4.5 and RCP8.5 emission pathways downscaled to the EUR-44 domain.

Based on these simulations, urban ecosystems with trees were more consistent carbon sinks and less sensitive to future weather conditions than vegetation types dominated by grasses. Drought decreased primary production in some vegetation types during summertime, but on an annual scale, productivity was mainly driven by the length of the growing season.  In these simulations irrigation caused a decrease in Net Ecosystem Production (NEP) compared to their non-irrigated counterparts, highlighting the role of moisture as a driver of respiration.

How to cite: Koiso-Kanttila, A., Backman, L., and Kulmala, L.: Carbon Sequestration across Urban Vegetation Types in Changing Climate in Finnish Cities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14947, https://doi.org/10.5194/egusphere-egu25-14947, 2025.

EGU25-15353 | Posters on site | AS3.26

Understanding GHG Emission Trends in Romania: Sectoral and Regional Perspectives 

Alin Scarlat, Alexandru Tudor, and Gabriel Iorga

The influence of greenhouse gas (GHG) emissions on climate change represents a critical global issue. This study investigates the dynamics of three key greenhouse gases-carbon dioxide (CO2), methane (CH4), and nitrous oxide (N2O)-from 1990 to 2021 across Romania's development regions, including a focused analysis of emissions in the urban area of Bucharest and the surrounding Ilfov region. Data for the analysis were sourced from the EDGAR database (Emissions Database for Global Atmospheric Research), with emissions categorized by major activity sectors, including transport, waste management, biomass burning, manufacturing and construction, fossil fuel usage, and agricultural practices such as rice cultivation and livestock. This categorization allows for a comprehensive examination of sectoral contributions to overall GHG emissions.

To capture the evolution of GHG emissions, the study applies advanced statistical tools. Temporal variations in the GHG time series were analyzed using Change Point Analysis, identifying both major and minor change points, all statistically significant at the 99% confidence level. Monotonic annual trends in emissions were further assessed using the non-parametric Mann-Kendall test in combination with Sen’s method, providing a nuanced understanding of long-term emission patterns.

The findings reveal substantial regional disparities in CO2, CH4, and N2O emissions, with distinct periods of increase or reduction. These variations correlate with factors such as industrial development, shifts in agricultural practices, and the implementation of environmental regulations. By analyzing both national and regional trends, the study sheds light on the sectoral drivers of emissions and their long-term behavior.

This research enhances understanding of Romania's GHG emission trends over the past three decades, emphasizing the influence of regional variations and sectoral contributions to shaping the country's overall emissions profile.

How to cite: Scarlat, A., Tudor, A., and Iorga, G.: Understanding GHG Emission Trends in Romania: Sectoral and Regional Perspectives, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15353, https://doi.org/10.5194/egusphere-egu25-15353, 2025.

EGU25-15602 | ECS | Posters on site | AS3.26

CHETNA-Power Sector: High-Resolution Mapping of Power Sector Emissions in Indian Cities: Bridging Data Gaps for Effective GHG Mitigation and Urban Energy Planning 

Abhinav Sharma, Chuanlong Zhou, Philippe Ciais, Ahana Sarkar, Arnab Jana, and Harish Phuleria

India's power sector plays a pivotal role in the country's greenhouse gas (GHG) mitigation efforts, contributing 45% of national CO2 emissions, with coal-fired power plants responsible for 72% of CO2 emissions from fuel combustion in 2022. The sector's dependence on coal and rising electricity demand pose significant challenges to achieving India's targets of reducing GDP emission intensity by 45% and transitioning to 50% non-fossil fuel installed capacity by 2030. Monitoring emissions at the city level is especially critical, as urban areas concentrate electricity demand, with the residential and industrial sectors accounting for 25.77% and 41.16% of total consumption, respectively. High-resolution, city-specific data is essential for identifying emission hotspots, optimizing renewable energy deployment, and prioritizing energy efficiency improvements.

To address the current dataset gaps in India, we conducted a high spatial-temporal resolution analysis of CO2 and air pollutant emissions for 100 Indian cities. This analysis integrates diverse open-source datasets, including power plant locations, capacities, and fuel types from the Global Energy Monitor (GEM) and OpenStreetMap (OSM); transmission grid data from OSM; industrial factory data from Indian statistical databases and OSM; emission factors from the Central Electricity Authority (CEA) of India; power generation and outage data from the Indian National Power Portal (NPP); and gridded population and land-use data from the Global Human Settlement Layer and Copernicus Global Land Cover Layers.

The power generation time series was first completed using a machine learning model to address missing data. Then, we developed a grid gravity-based power distribution model to analyze power consumption and emissions. This model evaluates the relative "attractiveness" of power consumption for each grid by incorporating large industrial factories, grid population, and cropland areas. An optimization algorithm was employed to allocate power generation, constrained by transmission grid capacity and minimizing the losses. Parameters were fine-tuned using regional monthly electricity consumption data, establishing a robust framework for spatial emission mapping while excluding electricity imports and exports. Using this gridded power distribution model, we generated high-resolution maps of both CO2 and air pollutant emissions for each city, offering valuable insights into their spatial distribution across urban areas.

This work, part of the CHETNA project (City-wise High-resolution Carbon Emissions Tracking and Nationwide Analysis), leverages artificial intelligence and advanced datasets to deliver near real-time, high-resolution emissions data for over 100 Indian cities. 

How to cite: Sharma, A., Zhou, C., Ciais, P., Sarkar, A., Jana, A., and Phuleria, H.: CHETNA-Power Sector: High-Resolution Mapping of Power Sector Emissions in Indian Cities: Bridging Data Gaps for Effective GHG Mitigation and Urban Energy Planning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15602, https://doi.org/10.5194/egusphere-egu25-15602, 2025.

EGU25-15751 | Orals | AS3.26

Constraining Anthropogenic CO2 Emissions using XCO2 Observations from OCO-3 over Xiamen-Zhangzhou-Quanzhou Metropolitan Area 

Xinxin Ye, Weijiao Li, Thomas Lauvaux, Shuifa Lin, Ziwei Zhang, Yunxiao Lin, Jingfen Hua, and Jianyi Lin

Accurate quantification and monitoring of urban fossil-fuel CO2 (FFCO2) emissions at improved spatial granularity are critical to emission control and climate change mitigation policies. In this work, we use a top-down Bayesian inversion method and Eulerian transport modeling to constrain FFCO2 emissions from the Xiamen-Zhangzhou-Quanzhou metropolitan area, China, based on high-resolution areal snapshots of total column CO2 (XCO2) from OCO-3 Snapshot Area Maps (SAMs) during September 2019 to July 2023. The emissions from point sources and different areas are constrianed simultaneously, including the area sources Xiamen, local power plants in Xiamen, and other adjacent urban areas. Observed XCO2 enhancements range from 0.70±0.53 ppm to 2.29±1.16 ppm, indicating potential capability of OCO-3 SAMs on detecting emission signatures.  We show the mean posterior emission from Xiamen of about 7.79 ± 0.92 MtC/yr, being within the spread of different inventories and 34 % higher than their average. Several challenges hampering the inversion performance are revealed, including the spatial displacements of the modeled and observed enhancements, the limited representation of local power plants, and data availability. The results provide insights on inversely disentangling imprints of emission sources based on dense space-borne observations, facilitating applications of future missions with improved XCO2 mapping coverage and frequency. 

How to cite: Ye, X., Li, W., Lauvaux, T., Lin, S., Zhang, Z., Lin, Y., Hua, J., and Lin, J.: Constraining Anthropogenic CO2 Emissions using XCO2 Observations from OCO-3 over Xiamen-Zhangzhou-Quanzhou Metropolitan Area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15751, https://doi.org/10.5194/egusphere-egu25-15751, 2025.

EGU25-15891 | Posters on site | AS3.26

Measurement of Methane Concentrations at Ground Level in Bucharest during August 2024 Using a Mobile Laboratory 

Alexandru Tudor, Alin Scarlat, and Gabriela Iorga

Methane (CH₄) is a significant greenhouse gas, playing a critical role in air quality and climate change. In situ measurements of CH4 in Romania are very scarce. This study presents results from a ground-level measurement campaign of atmospheric methane concentrations in Bucharest, Romania. One of the main objectives was to map the spatial distribution of methane concentrations. The campaign was performed using a mobile laboratory, between August 6 and 27, 2024 and covered over 1500 km throughout Bucharest. Methane concentrations were measured using a Sniffer4D TDLAS analyzer with a resolution of 1 ppm. Bucharest was divided into three zones: northwest, northeast, and south. A designated route was established for each zone and crossed a total of 4 times: once at night and during the daytime over 3 different days. This data collection approach ensured statistical consistency and captured temporal and spatial variations in methane concentrations.

The results are presented as grid maps to highlight significant diurnal and spatial variations more clearly, indicating anthropogenic contributions from traffic and industrial activities during the day. At night, concentrations exhibited a more uniform distribution, suggesting relatively constant background emissions and a reduced influence of local activities.

This study contributes to understanding methane levels and sources in the urban environment of Bucharest and provides a critical reference for future monitoring efforts. The findings emphasize the importance of continuous methane concentration surveillance to support air quality management strategies and climate change mitigation.

How to cite: Tudor, A., Scarlat, A., and Iorga, G.: Measurement of Methane Concentrations at Ground Level in Bucharest during August 2024 Using a Mobile Laboratory, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15891, https://doi.org/10.5194/egusphere-egu25-15891, 2025.

EGU25-15945 | Orals | AS3.26

Field Applications with Air Quality Monitoring: From Social Equity to CO2 Infrastructure 

Morten Stoltenberg, Thor-Bjørn Ottosen, Stig Koust, Francesco Cappelluti, Søren Møller, Søren Jørgensen, Sara Cox, Naja Villadsen, Lars Overgaard, Gintaras Simaitis, Christoffer Karoff, Angel Vara-Vela, Anna Eikeland, Jon Knudsen, Rafaela Alberti, and Anne Sofie Engedal

Urban air quality monitoring presents unique challenges due to complex emission patterns and operational difficulties. Our work and research combine multiple approaches to address these challenges, focusing particularly on three areas: improving quality of life for vulnerable population groups in cities, managing a sensor network on a construction-site, and leakage monitoring of fugitive greenhouse gas emissions.

Through the DivAirCity project, implemented across five European cities, we developed an integrated monitoring framework that combines quantitative air quality measurements with social equity considerations, specifically addressing the disproportionate impact of pollution on vulnerable communities. Our monitoring framework combines quantitative air quality measurements with social equity considerations, requiring careful attention to sensor placement, data quality assurance, and long-term reliability.

As part of the Green Construction Site of the Future project, we gained valuable experience in deploying and maintaining sensor networks in challenging and dynamic construction environments. Over a two-year period, we successfully operated a continuous monitoring system, investigating dust mitigation strategies and PM2.5 dispersion patterns from source points. This implementation provided valuable insights into the practical challenges of maintaining long-term sensor networks in harsh urban environments.

For our environmental monitoring project MONICO, we demonstrate and evaluate the integration of low-cost sensors, satellite observations, inverse modelling, and drone measurements for quantifying fugitive emissions in the CO2 infrastructure. Through controlled release experiments, we validated and tested methodologies for selecting and deploying sensor networks around point sources, while addressing challenges in weather influence and data reliability.

Together, these projects contribute to the practical aspects of operating sensor networks across different contexts, contributing to environmentally conscious cities and establishing best practices for effective monitoring strategies.

How to cite: Stoltenberg, M., Ottosen, T.-B., Koust, S., Cappelluti, F., Møller, S., Jørgensen, S., Cox, S., Villadsen, N., Overgaard, L., Simaitis, G., Karoff, C., Vara-Vela, A., Eikeland, A., Knudsen, J., Alberti, R., and Engedal, A. S.: Field Applications with Air Quality Monitoring: From Social Equity to CO2 Infrastructure, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15945, https://doi.org/10.5194/egusphere-egu25-15945, 2025.

EGU25-16129 | ECS | Posters on site | AS3.26

Determining Key Factors Influencing Ozone Formation in Taichung City, Taiwan Using Machine Learning Models 

Jonalyn Madriaga and Charles Chou

Ozone pollution remains a significant environmental challenge in urban areas, with elevated ground-level ozone posing risks to public health, ecosystems, and climate stability. In Taichung City, Taiwan, rapid urbanization and industrial activities have contributed to deteriorating air quality, making it crucial to identify the key factors driving ozone formation for effective mitigation strategies. This study employs machine learning (ML) models, including Random Forest (RF) and eXtreme Gradient Boosting (XGBoost), to analyze ozone pollution in Taichung. Moreover, feature importance analysis is used to identify the key factors driving ozone variability, including volatile organic compounds (VOCs), nitrogen oxides (NO and NO₂), and meteorological variables such as temperature, humidity, wind speed, and solar radiation. The models were trained and tested on the hourly observational data collected from the Urban Air Pollution Research Station (UAPRS) in Taichung City from January to December 2023. To enhance the models’ accuracy, GridSearchCV is utilized to select optimal parameters and reduce the risk of overfitting. Preliminary results indicated that the number of predictors impacts ML performance—RF outperforms XGBoost when fewer predictors are used. However, with a more comprehensive set of predictors, XGBoost demonstrated superior performance, achieving determination coefficients of 0.945 and 0.886 for the training and test datasets, respectively. Feature importance analysis revealed that the top three contributors to ozone variability in 2023 were NO (44%), humidity (19%), and NO₂ (12%). For high ozone episodes, NO, humidity, and solar radiation were identified as the key drivers. By combining the predictive power of ensemble ML techniques with feature importance analysis, this study provides valuable insights into the interactions between chemical and meteorological factors driving ozone formation. The results highlight the relative significance of these factors in influencing ozone levels and provide actionable insights for air quality management in Taichung. Additionally, the study demonstrates the potential of ML models as powerful tools for advancing urban air quality research, with implications for policy interventions and future environmental studies. Future work will focus on refining the models to predict ozone episodes in real time and exploring their applicability to other rapidly urbanizing cities facing similar air quality challenges.

How to cite: Madriaga, J. and Chou, C.: Determining Key Factors Influencing Ozone Formation in Taichung City, Taiwan Using Machine Learning Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16129, https://doi.org/10.5194/egusphere-egu25-16129, 2025.

EGU25-16731 | ECS | Orals | AS3.26

High-Resolution LES-Based Air Quality Modeling Over Munich: Evaluation of Model Performance, and Pollution Drivers 

Vigneshkumar Balamurugan, Jia Chen, Harald Saathoff, Christopher Claus Holst, Adrian Wenzel, Ayah Abu-Hani, Yanxia Li, Yaowei Li, Sophie Abou-Rizk, and Frank N Keutsch

Air pollution is a critical issue, particularly in urban areas, making the monitoring and understanding of the  air pollutant’s sources essential. Urban regions are often very heterogeneous due to the complexity of buildings, roadways, vegetation, and various emission sources. Governments prioritize these areas to implement intervention measures aimed at addressing air pollution, as urban regions are both major sources of pollution and densely populated. Therefore, simulating the dispersion of air pollutants at high spatial and temporal resolution is crucial for understanding pollution sources and evaluating different intervention measures.

In this context, we have set up the Large-Eddy Simulation (LES)-based air quality model, PALM-4U (Parallelized Large-Eddy Simulation Model for Urban), over Munich, Germany. The goal is to simulate meteorology and concentrations of air quality relevant species at high spatial (10 meters) and temporal (10 minutes) resolution across the city. The model uses high-resolution static parameters (e.g., building height, vegetation height), dynamic meteorological variables from the WRF model (with a 400-meter resolution) for boundary conditions, and a high-resolution emission inventory (100 meters). The boundary conditions for air quality species were obtained from CAMS model ensemble outputs. 

We compared the simulated meteorology and air pollutant concentrations with data from an extensive measurement campaign conducted in August 2023 for selected days. The results showed good agreement for wind speed (Mean Bias (MB) = 0.23 m/s, Pearson correlation coefficient (R) = 0.86) and wind direction (MB = 35°, R = 0.83). The PALM-4U model overestimated NO2 concentrations by 0.82 ppb (+15.5 %), underestimated O3 concentrations by 4.5 ppb (-13.7 %) and overestimated PM10 concentrations by 1.4 µg m-3 (+11.7 %), although it accurately captured the diurnal variations. Sensitivity analysis revealed that the boundary conditions from the mesoscale model have a significant impact on the modeled air quality concentrations.

This model setup will be further utilized to evaluate the effectiveness of various measures, such as low-speed zones, low-emission zones, and the extent of electric vehicle adoption required to achieve safe air pollution levels within Munich.

How to cite: Balamurugan, V., Chen, J., Saathoff, H., Claus Holst, C., Wenzel, A., Abu-Hani, A., Li, Y., Li, Y., Abou-Rizk, S., and N Keutsch, F.: High-Resolution LES-Based Air Quality Modeling Over Munich: Evaluation of Model Performance, and Pollution Drivers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16731, https://doi.org/10.5194/egusphere-egu25-16731, 2025.

EGU25-16784 | ECS | Orals | AS3.26 | Highlight

Towards high-resolution air pollutants sensing through dense low-cost sensor networks – a case study in Munich 

Adrian Wenzel, Jia Chen, Tobias Klama, Felix Böhm, Moritz Angleitner, and Reinhard Lobmaier

Being Germany’s 3rd largest city, Munich has the nation’s highest number of daily commuters leading to high traffic volumes and adding up to the urban air pollution through emissions from combustion and tire and brake wear. Although urban air quality is generally improving over the past years, all measurement stations by the Bavarian State Office for Environment (LfU) in Munich still exceed the critical NO2 level of 10 µg/m3 as suggested in the updated WHO guidelines 2021.

For quantifying air quality at high spatiotemporal resolution in the city, we developed a self-sufficient low-cost sensor system equipped with electrochemical cells (ECs) for measuring NO2, NO, CO and O3 as well as an optical particle counter.

In summer 2023, we started setting up a dense sensor network of 25 sites in the inner city and since then, we have gathered 22 million data points. Prior to installation at their final locations, we mounted each sensor system for several weeks at an automated measurement station operated by the LfU in order to acquire high-accuracy reference data for calibrating our system. During operation of the sensor network, several nodes are occasionally returned to the reference site and three sensor nodes have been mounted there continuously ever since. In total, 8 million data points have been gathered during these co-location measurements. The combination of frequent rotation of sensor nodes between network locations and reference site as well as long-term co-location nodes yields a unique dataset for a novel calibration approach. Here, we analyze the calibration performance of NO2; other pollutants will follow.

Firstly, we analyzed the correlation of the EC’s raw hourly signal to the reference station by assessing their coefficient of determination (R2). Remarkably, highest R2 values occurred in fall and winter time with temperatures in the range of -5 to +15 °C. Lowest and even negative R2 values occurred during summer and during long-term co-locations facing seasonal changes.

Secondly, for assessing a real-world scenario, we analyzed the performance of one node with long-term co-location at the reference station. The raw EC data yields an R2 of 0.35 over 27 weeks. By applying a Random Forest Regressor using the first 30 % of the data points for training and including temperature, humidity and NO as features, R2 could be increased to 0.7. Currently, we are developing a novel calibration strategy that leverages this extensive co-location data set with advanced machine learning methods to increase the calibration performance and to map air quality within our sensor network at high resolution and accuracy.

How to cite: Wenzel, A., Chen, J., Klama, T., Böhm, F., Angleitner, M., and Lobmaier, R.: Towards high-resolution air pollutants sensing through dense low-cost sensor networks – a case study in Munich, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16784, https://doi.org/10.5194/egusphere-egu25-16784, 2025.

EGU25-17440 | Orals | AS3.26

Advanced Mobile Monitoring of Greenhouse Gases and Air Pollutants Using a Compact Spectrometer 

Morten Hundt, Jonas Bruckhuisen, and Oleg Aseev

Urban air pollution and greenhouse gas (GHG) emissions stem from diverse sources, including transportation, heating, buildings, waste management, industrial and agricultural activities, and natural events like forest fires. Simultaneous monitoring of air pollutants and GHGs with high selectivity and sensitivity is crucial for identifying and evaluating their sources and sinks, as well as understanding their interactions. Accurate measurements across various spatial and temporal scales are essential for modeling and validating emission inventories or satellite observations.

Traditionally, solutions for monitoring air pollutants or GHGs with high precision and temporal resolution have been "one-gas-one-instrument," resulting in large, stationary setups with high energy consumption. MIRO Analytical’s compact laser absorption spectrometer that integrates multiple mid-IR lasers enables simultaneous high-precision measurements of greenhouse gases (CO2, N2O, H2O, CH4), pollutants (CO, NO, NO2, O3, SO2, NH3), and trace gases (OCS, HONO, CH2O) within a single instrument. With a time-resolution of up to 10Hz, it is well-suited for detecting the relationships between co-emitted pollutants and GHGs as well as eddy-covariance flux studies.

In our presentation, we will showcase examples of our instrument's applications for mobile monitoring of 10 GHGs and air pollutants in urban areas, as well as airborne measurements using airships or planes. Additionally, we will present results from parallel monitoring with our instrument and conventional gas analyzers used for GHG and air pollutant measurements. This demonstrates our instrument's capability to serve as an all-in-one solution, replacing up to seven standard gas analyzers and enabling a wide range of new mobile multi-compound gas monitoring applications, such as in airplanes or cars.

How to cite: Hundt, M., Bruckhuisen, J., and Aseev, O.: Advanced Mobile Monitoring of Greenhouse Gases and Air Pollutants Using a Compact Spectrometer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17440, https://doi.org/10.5194/egusphere-egu25-17440, 2025.

EGU25-17841 | ECS | Orals | AS3.26

Assessment of Munich’s CO2 emissions via Bayesian inversion using MUCCnet data from 2020-2025 

Josef Stauber, Jia Chen, Friedrich Klappenbach, Junwei Li, Andreas Luther, Moritz Makowski, Haoyue Tang, Nikolai Ponomarev, and Dominik Brunner

The Munich Urban Carbon Column network (MUCCnet) consists of five solar-tracking Fourier Transform spectrometers (EM27/SUN) measuring column-averaged mole fractions of carbon dioxide (XCO2), methane (XCH4), and carbon monoxide (XCO). They are strategically placed in the center of Munich and in every cardinal direction. Starting with one instrument in 2015, MUCCnet has been collecting data continuously with five instruments since 2020, allowing a detailed analysis of Munich's urban greenhouse gas emissions based on inverse methods. To this end, we use the Bayesian inversion approach: We compute the observed enhancements in dependence of the wind direction using one network site as background (observed background) and derive spatially resolved emissions. The forward model uses a Munich-specific inventory (100×100 m2 resolution) for anthropogenic fluxes and the Vegetation Photosynthesis and Respiration Model (VPRM) for biogenic fluxes. The transport is modeled with the Lagrangian particle dispersion model STILT.

A critical aspect of our analysis is the estimation of uncertainties within the inversion framework. Balancing the confidence in transport and measurements against prior information (inventories) is of great importance. Furthermore, we investigate the number and spatial distribution of state vector parameters based on the available degrees of freedom for signal. The choice of an appropriate background is crucial, since the urban enhancements for Munich are typically below 1 ppm, which is small (< 1%) compared to the background XCO2 concentrations (> 400 ppm). In addition to the observed background approach, we investigate background approaches derived from models (e.g. ICON-ART), and fitted, a posteriori backgrounds from the inversion approach.

Our inversion results represent spatially resolved, long-term, top-down CO2 emission estimates for Munich. Over a comprehensive measurement period of five years, we highlight seasonal and annual trends, providing valuable insights into Munich's CO2 emissions.

How to cite: Stauber, J., Chen, J., Klappenbach, F., Li, J., Luther, A., Makowski, M., Tang, H., Ponomarev, N., and Brunner, D.: Assessment of Munich’s CO2 emissions via Bayesian inversion using MUCCnet data from 2020-2025, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17841, https://doi.org/10.5194/egusphere-egu25-17841, 2025.

EGU25-17963 | Orals | AS3.26

Urban CO2 and CH4 atmospheric measurements in the Milan city area (northern Italy) 

Paolo Cristofanelli, Nora Zannoni, Francesco Apadula, Francesca Barnaba, Alessandro Bracci, Annachiara Bellini, Francescescopiero Calzolari, Luca Diliberto, Giovanni Manca, Valeria Mardonez, Cecilia Magnani, Simonetta Montaguti, Laura Renzi, Giulia Zazzeri, and Angela Marinoni

Northern Italy is one of the most polluted and densely populated areas in Europe. The diversity of land use in the Po basin makes this region an important contributor to greenhouse gas emissions from different sources. Medium and large cities, as well as industrialised areas, contribute significantly to emissions from industrial processes, combustion, waste management and natural gas distribution.

As part of the H2020 RI-URBANS project (https://riurbans.eu/) and in synergy with PNRR “ITINERIS” Project, a pilot study has been carried out in the Milan urban area with the aim of supporting the local authorities to evaluate the effectiveness of air quality policies and the effects of pollutants on human health. A one-year long measurement campaign was carried out using a mobile platform in the premises of the CNR facility (AdRMi1, 45°28’47"N 9°13’54"E; 120 m a.s.l.), located in in the urban area of Milan, in the University district. The mobile platform has been equipped with a suite of instruments (ACSM, Vocus Chemical Ionization TOF-MS, Aethalometer, NOx CLD) to provide near real time (NRT) information on aerosol source partitioning and to characterise nanoparticle contributions from urban hot spots. From July 2023 to March 2024, the mobile platform has been equipped with a Cavity Ring Down Analyser for continuous observations of carbon dioxide (CO2) and methane (CH4).

In this work we will provide a first characterization of the diel cycles and seasonal variations (from late summer to early spring) of atmospheric CO2 and CH4 in the urban area of Milan. Thanks to the combined analysis of other atmospheric tracers, first insights about the influence by atmospheric processes (i.e. PBL dynamics) and emission sources (fossil fuel and biomass burning combustion, biogenic, waste management) will be discussed. Finally, we provided a preliminary “top-down” estimate of CH4 emission for the Milan urban area by using the interspecies correlation approach: the obtained values were higher (but still within the range of uncertainties) than emissions provided by statistical “bottom-up” inventories (e.g. INEMAR).

Acknowledgments:  RI-URBANS t has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement No 101036245. This reserach was partially supported by the European Unione- Next Generation EU, Missione 4 Componente 2 - CUP B53C22002150006 -  IR0000032 – ITINERIS, Italian Integrated Environmental Research Infrastructures System

How to cite: Cristofanelli, P., Zannoni, N., Apadula, F., Barnaba, F., Bracci, A., Bellini, A., Calzolari, F., Diliberto, L., Manca, G., Mardonez, V., Magnani, C., Montaguti, S., Renzi, L., Zazzeri, G., and Marinoni, A.: Urban CO2 and CH4 atmospheric measurements in the Milan city area (northern Italy), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17963, https://doi.org/10.5194/egusphere-egu25-17963, 2025.

EGU25-18076 | ECS | Orals | AS3.26

Eddy covariance measurements of CO2 fluxes along an urban-to-rural gradient in the Paris area 

Bignotti Laura, Jérémie Depuydt, Pedro-Henrique Herig-Coimbra, Alain Fortineau, Anais Feron, Patrick Stella, Pauline Buysse, Carmen Kalalian, Guillaume Nief, Michel Ramonet, and Benjamin Loubet

Cities are one of the main sources of greenhouse gases, accounting for over 70% of global CO2 emissions. Accurate quantification of these emissions through direct observations is crucial for developing and assessing the effectiveness of adopted mitigation strategies.

As part of the European project ICOS Cities (https://www.icos-cp.eu/projects/icos-cities), three eddy covariance towers were installed in the Paris area to capture the variability of surface-atmosphere CO2 fluxes as a function of an urbanization gradient. Specifically, the selected sites were chosen to be representative of a highly urbanised and densely built-up area (Jussieu), an urban forest (Vincennes), and a heterogeneous area combining highly urbanised areas with areas of vegetation (Romainville). The observations from the urban sites were also integrated with the EC flux measurements conducted on the ICOS atmosphere tower of Saclay and the observations from the ecosystem sites of Fontainebleau (FR-FON, forest) and Grignon (FR-GRI, crop).

Long-term measurements of CO2 fluxes (2 years for the sites of Romainville and Jussieu and 1 year for the site of Vincennes) showed seasonal dynamics that reflected their respective degrees of urbanisation. The Jussieu site, in the city center, was constantly dominated by anthropogenic CO2 emissions, with maximum emission (up to  15 µmol m-2 s-1) during the winter months (November-February) and low absorptions (up to  -2.5 µmol m-2 s-1) during the summer (July-August) in the central hours of the day. On the other hand, the mixed urban forest of Vincennes showed a strong biogenic signature, characterized by a predominant CO2 absorption in the central hours of the day (up to -10 µmol m-2 s-1 in the months of May, June and July). The 100 m-tall tower of Romainville  showed instead the coexistence of anthropogenic and biogenic fluxes, each contributing its own seasonal and daily variations to the measured flux. A comparison between our observations and the emissions of the City of Paris will be included in the presentation.

How to cite: Laura, B., Depuydt, J., Herig-Coimbra, P.-H., Fortineau, A., Feron, A., Stella, P., Buysse, P., Kalalian, C., Nief, G., Ramonet, M., and Loubet, B.: Eddy covariance measurements of CO2 fluxes along an urban-to-rural gradient in the Paris area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18076, https://doi.org/10.5194/egusphere-egu25-18076, 2025.

EGU25-18113 | ECS | Orals | AS3.26

 Spatial-temporal analysis of recent trends in nitrogen dioxide (NO2) and volatile organic compounds (VOCs) in the Mediterranean metropolitan area of Valencia city 

Daeun Jung, Enrique Mantilla, Esther Borrás, Teresa Vera, Tatiana Gómez, and Amalia Muñoz

Nitrogen dioxide (NO2) and volatile organic compounds (VOCs) are of concern in urban environments as primary pollutants and as main precursors of tropospheric O3, which has adverse effects on both human health and vegetation. Furthermore, as a secondary pollutant, its complex nature due to its non-linear chemistry makes it difficult to reduce with the reduction in the precursors.

This study is carried out to spatially characterise the urban air pollution, using NO2 and VOCs, and to evaluate the recent temporal trends of these compounds, which are closely related to the O3 formation in the metropolitan area of Valencia. Being the third largest Spanish city, with one of the Mediterranean's largest ports, the complex emission sources contribute to high ozone levels in the surrounding areas.

A total of 97 passive samplers for NO2 were used in the study area, covering an area of 11 km x 10 km including the urban centre with a resolution of about 1 km x 1 km. The temporal resolution of the measurement covers the winter and summer seasons (one exposure week every February and July, respectively) for the last 8 years, from 2017 to 2024. Meanwhile, the passive samplers for VOCs were installed at 10 selected points through the urban centre among the 97 points, following the main wind direction of the region. The measurement period is two years shorter than those for NO2 from 2019 to 2024 but covers the same seasons. The measured NO2 levels were determined using ultraviolet-visible (UV-VIS) spectroscopy, while the VOCs levels were analysed through gas chromatography-mass spectrometry (GC-MS) and liquid chromatography-mass spectrometry (LC-MS).

To characterise the spatial patterns of the city, the k-mean clustering is used to group all points where NO2 levels are measured. As a result, the city is divided into overall two clusters. Cluster 1 is close to road traffic emissions and follows the prevailing wind direction, resulting in relatively high levels of NO2. Cluster 2 represents the rest of the points, which have lower levels. As for VOCs, the analysis is performed at two specific points, where NO2 has the highest and the lowest among the given 10 points, in the city centre and in the harbour area, representing Cluster 1 and Cluster 2, respectively. In the city centre, the aromatic hydrocarbons are more abundant, while in the harbour area, the contribution of the aldehydes is greater.

The Theil-Sen method is used for the temporal analysis of each cluster. NO2 shows a decreasing trend in both clusters. The reduction is more pronounced in Cluster 1 where the levels tend to be greater than the other cluster, especially in winter. However, total VOCs levels seem to be increasing overall. In particular, there is a tendency to increase in winter, while VOCs decrease slightly in summer.

This result shows that the ozone formation regime of this area has been changing as NO2 levels are decreasing while VOCs are generally increasing. Therefore, ozone levels may be locally increasing.

How to cite: Jung, D., Mantilla, E., Borrás, E., Vera, T., Gómez, T., and Muñoz, A.:  Spatial-temporal analysis of recent trends in nitrogen dioxide (NO2) and volatile organic compounds (VOCs) in the Mediterranean metropolitan area of Valencia city, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18113, https://doi.org/10.5194/egusphere-egu25-18113, 2025.

EGU25-19635 | Orals | AS3.26

Volatile organic compounds at two urban areas in the Italian Po Valley: Milan and Bologna 

Angela Marinoni, Nora Zannoni, Paolo Cristofanelli, Marco Paglione, Marco Rapuano, Camilla Perfetti, Alessandro Bracci, Annachiara Bellini, Francesca Barnaba, Cristina Colombi, and Matteo Rinaldi

Volatile organic compounds (VOCs) released into the atmosphere by natural and anthropogenic sources play a key role in atmospheric processes. They can react with atmospheric oxidants leading to secondary organic aerosols and tropospheric ozone, with effects on air pollution, human health and climate.

In Europe, the improvement of air quality policies in the last decades has caused some pollutants’ concentrations to decrease. This is the case for nitrogen dioxide and particulate matter concentrations that decreased between 30-50% during 2000-2010, leading to a decreasing trend of the associated health effects on people exposed to them. Yet, 70% of EU citizens lives in urban areas, and 99-97% of this population is exposed to concentrations of ozone and fine particulate matter above the guidelines recommended by WHO in 2021 for protecting public health (EEA, 2021). The Po Valley, located in the North of Italy is one of the areas in Europe suffering the worst air pollution, with several air quality threshold exceedances throughout the years. A recent example was recorded in the city of Milan in winter 2024, when, during several days of high atmospheric pressure conditions, PM 2.5 concentration was above 100 μg/m3, while the WHO recommended threshold is 15 μg/m3 on a 24-hour averaging time.

Within the EU-funded H2020 project RI-URBANS and ACTRIS, we conducted two field campaigns at two urban areas of different size, 200 km apart in the Italian Po Valley: Milano and Bologna. In both cases, VOCs were measured with a Vocus CI-ToF (chemical ionization time of flight) 2R mass spectrometer (Tofwerk, Switzerland) that was deployed first in Milan from January 2023 during one year, then in Bologna in September 2024 for one month. The analysis of our study focuses on sixteen VOCs common to both measuring sites, identified and quantified with a certified VOC mixture and covering the measured mass range 42-371 amu. The absolute concentration, the diel and seasonal variability of the VOC measured in Milan and Bologna are discussed and compared. In particular, we determined the effect of atmospheric dilution and atmospheric reactivity on the measured concentrations. We also discuss the results in terms of potential formation of ozone and secondary organic aerosols.   

How to cite: Marinoni, A., Zannoni, N., Cristofanelli, P., Paglione, M., Rapuano, M., Perfetti, C., Bracci, A., Bellini, A., Barnaba, F., Colombi, C., and Rinaldi, M.: Volatile organic compounds at two urban areas in the Italian Po Valley: Milan and Bologna, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19635, https://doi.org/10.5194/egusphere-egu25-19635, 2025.

EGU25-19788 | ECS | Posters on site | AS3.26

Short-term energy and carbon balance calculation and footprint-based land cover classification at an urban site 

Francesco Piroddu and Costantino Sirca

The research takes place within the EU Horizon 2020 program, and the ICOS Cities project, that aims to support cities in formulating climate action plans, through the delivery of data on fossil fuel emissions from urban areas. The EC station is located on the roof of a building in Sassari (Sardinia, Italy N 40° 43' 0.4836 E 8° 34' 32.88, 254 m asl). Measurement height is fixed at 23 m from ground. Instruments include a Gill HS-50 sonic anemometer and a closed-path LI-7200 gas analyzer, for H2O and CO2 fluxes. The Eddy Covariance approach for environmental studies is a powerful technique that is used in many applications in the study of urban ecosystems and fluxes. The post-processing phase of data consisted in energy and carbon budgets calculations, together with the flux footprint land mapping, at the ICOS urban EC site ‘ITSas’, which were realized using the software ‘Tovi’ (from LI-COR®). The daily variation of the energy components revealed that the heat storage reaches high values in the morning, while drops out later in the evening. The correction of the regression model revealed the action of GHGs in delaying the daily heat flux peak. The seasonal variations of energy terms revealed that the latent heat flux, the evapotranspiration and the water vapor flux varied at the same rate and correlated positively with high air temperatures and strong radiation values. The energy balance residuals seemed to correlate well with energy availability and heat storage, while they kept a fairly constant variation, with only little deviations falling along the main wind directions (NW and SW winds). The daily C cycle was made up of two main daily maximum peaks, associated with traffic peaks and urban emissions. The footprint-based land mapping of flux contributions demonstrated the urban typology of the flux data since most of the contributions (about 60%) to footprint climatology came from urban areas, while a minor input was delegated to vegetated surfaces.

How to cite: Piroddu, F. and Sirca, C.: Short-term energy and carbon balance calculation and footprint-based land cover classification at an urban site, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19788, https://doi.org/10.5194/egusphere-egu25-19788, 2025.

EGU25-19806 | ECS | Posters on site | AS3.26

Oxidative Potential of Indoor Particulate Matter Collected During Campaigns in the UK, Slovenia, and Sweden 

Alexander Zherebker, Matthew Williams, and Chiara Giorio

The health effects of particulate matter (PM) are well-documented, with long-term exposure to elevated concentrations of respirable PM linked to increased risks of respiratory conditions such as allergic reactions, lung inflammation, and asthma. A key contributor to these health effects is the oxidative stress induced by PM, stemming from heavy metals and the generation of reactive oxygen species (ROS).

In this study, we measured the oxidative potential (OP) of respirable dust and inhalable PM collected from households in Slovenia, Sweden, and the UK as part of the international INQUIRE project on air quality. Samples were collected using active samplers, and OP was assessed using a simulated epithelial lung fluid (SELF) model, following established protocols. Quantitative mass spectrometry was employed to determine the depletion rates of key lung antioxidants, including glutathione, cysteine, and ascorbic acid, alongside the accumulation of glutathione dimer.

Our results revealed statistically significant higher antioxidant depletion rates in experiments with PM compared to control samples. To elucidate the underlying mechanisms, we measured the concentrations of soluble heavy metals and analyzed water-soluble organic matter (WSOM) from both coarse and fine PM fractions using high-resolution mass spectrometry. Correlations between the relative abundance of organic constituents and antioxidant depletion rates highlighted the role of specific organic compounds in driving oxidative potential.

These findings underscore the need for targeted intervention strategies to mitigate the health risks associated with PM-induced oxidative stress in indoor environments.

How to cite: Zherebker, A., Williams, M., and Giorio, C.: Oxidative Potential of Indoor Particulate Matter Collected During Campaigns in the UK, Slovenia, and Sweden, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19806, https://doi.org/10.5194/egusphere-egu25-19806, 2025.

Exposure to air pollution contributes to chronic cardiovascular and respiratory diseases as well as mortality, particularly in urban areas. For assessing the health impacts of air pollution, integrated mobility – emissions – air quality – exposure modelling chains have been developed in recent years (Gurram, Stuart, et Pinjari 2019). Numerous studies have highlighted the importance of considering daily mobility when assessing air pollution exposure (Dias et Tchepel 2018). However, the question of uncertainties associated with these modelling chains remains little studied, in particular uncertainties related to models’ spatiotemporal resolution. This work aims to perform a sensitivity analysis of individual exposure to ambient air pollution with an agent-based mobility model coupled with emission, air quality and exposure models.

This study is based on a modelling chain to assess individuals’ exposure with an agent-based approach. Individuals’ daily mobility and car traffic within the region are simulated with MATSim. As urban air quality is both affected by long-range pollution transport and local pollution sources within the urban canyon layer, spatial resolution of air quality was addressed. To this end, we developed novel methodology to generate a disaggregated car fleet attributing car types (i.e. fuel and Euro norm) to households depending on their socioeconomic characteristics, instead of the state-of-the-art average emitting car. This car fleet model aims to better represent spatial heterogeneities in car traffic emissions. Moreover, air quality is simulated at the street scale with the MUNICH street-network model (Kim et al. 2022) while urban background concentrations are simulated with the Polair3D Eulerian chemical transport model (CTM). The exposure model, at last, combines individual travel patterns and street-level pollution concentrations to assess individuals’ exposure, taking into account ambient air pollution infiltration and exposure in transportation.

To study the modelling chain sensitivity, three scenarios comparisons will be performed to assess the impact of the spatiotemporal resolution of car emissions, air quality and individual activities. First, we compare individuals’ exposure when implementing emissions based on a disaggregated car fleet versus a homogenous car fleet composed of an average emitting car. Secondly, we explore the impact of air quality spatial representation on exposure by comparing the use of the background CTM model alone (Polair3D) and the combined CTM and street air quality model. The third test will compare an exposure model incorporating mobility with a traditional static approach, where individuals stay at home.

 

References

Dias, Daniela, et Oxana Tchepel. 2018. « Spatial and Temporal Dynamics in Air Pollution Exposure Assessment ». International Journal of Environmental Research and Public Health 15 (3): 558. https://doi.org/10.3390/ijerph15030558.

Gurram, Sashikanth, Amy Lynette Stuart, et Abdul Rawoof Pinjari. 2019. « Agent-Based Modeling to Estimate Exposures to Urban Air Pollution from Transportation: Exposure Disparities and Impacts of High-Resolution Data ». Computers, Environment and Urban Systems 75 (mai):22‑34. https://doi.org/10.1016/j.compenvurbsys.2019.01.002.

Kim, Youngseob, Lya Lugon, Alice Maison, Thibaud Sarica, Yelva Roustan, Myrto Valari, Yang Zhang, Michel André, et Karine Sartelet. 2022. « MUNICH v2.0: A Street-Network Model Coupled with SSH-Aerosol (v1.2) for Multi-Pollutant Modelling ». Geoscientific Model Development 15 (19): 7371‑96. https://doi.org/10.5194/gmd-15-7371-2022.

 

How to cite: Lannes, M., Roustan, Y., and Coulombel, N.: Sensitivity analysis of a mobility – emissions – air quality – exposure modelling chain to assess individuals’ exposure in metropolitan areas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20635, https://doi.org/10.5194/egusphere-egu25-20635, 2025.

EGU25-1282 | ECS | Posters on site | AS3.27

Novel Insights into Atmospheric Methane Variability and Climatic Drivers in Eastern Saudi Arabia Using TROPOMI/Sentinel 5P Observations 

Md Masudur Rahman, Roman Shults, Sankaran Rajendran, Arfan Arshad, and Hatem Keshk

Methane (CH4​) is a critical atmospheric trace gas and a potent greenhouse gas contributing to global warming, yet its relationship with climate variables remains underexplored, particularly in eastern Saudi Arabia, which hosts over 70% of the country’s oil fields. This study presents the first comprehensive evaluation of the spatiotemporal variability of CH4​ and its climatic drivers in eastern Saudi Arabia, using novel TROPOMI (Tropospheric Monitoring Instrument)/Sentinel-5P data and innovative approaches applied over the period from 2019 to 2024. Google Earth Engine (GEE)-based analysis shows significant annual and seasonal changes, with CH4​ concentrations increasing from 1892 ppb to 1927 ppb. Seasonal patterns show maximum concentrations in summer and autumn and minimum concentrations in winter and spring. ArcGIS-based spatial trend analysis indicates an area-averaged increase of 5.61 ppb per year across the majority of the examined regions. These spatiotemporal variabilities are driven by anthropogenic factors (e.g., oil and gas activities, urbanization, and agriculture) and natural climatic factors (e.g., wetlands, soil activity, and changing climate variables). Emission sources are validated using the Global Fuel Exploitation Inventory (GFEIv2) dataset. Geographically Weighted Regression (GWR) modelling is adopted to understand the spatial-scale connections between CH4 and climate variables. The results, with a model fit R² of 0.85, reveal that CH4​ is negatively correlated with temperature, solar radiation, and precipitation, but positively correlated with humidity and wind speed. For instance, in 2023, the mean correlation coefficient between CH4​ and temperature was -3.89, indicating that CH4 concentrations decreased by 3.89 ppb across most of the studied areas per year for each unit increase in temperature. This decrease may be attributed to accelerated oxidative processes at higher temperatures, as the eastern region of Saudi Arabia is known for its consistently high temperatures. To assess the degree of importance of these connections, the Random Forest model is employed, outperforming statistical models with an R2 of 0.75 and an RMSE of 2.79 ppb. The findings highlight that temperature and incoming solar radiation have the highest importance, followed by humidity, wind speed, and precipitation, in driving CH4 variability. These results provide valuable insights to guide future research efforts across the Middle East and support policymakers in developing effective strategies for monitoring and managing atmospheric methane.

How to cite: Rahman, M. M., Shults, R., Rajendran, S., Arshad, A., and Keshk, H.: Novel Insights into Atmospheric Methane Variability and Climatic Drivers in Eastern Saudi Arabia Using TROPOMI/Sentinel 5P Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1282, https://doi.org/10.5194/egusphere-egu25-1282, 2025.

EGU25-1754 | ECS | Orals | AS3.27

Declining opportunity and enhanced targeting of short-term emission controls for major events in China 

Hanying Wang, Yu Zhao, Qin He, Kong Hao, Kai Qin, Bo Zheng, and Jintai Lin

Short-term air quality measures have been commonly conducted for major events held in China, while their effectiveness on emission reduction was insufficiently analyzed due to deficient capability of tracking the fast-changing emissions of cities. Here we combined a machine learning algorithm, multiple satellite measurements, and an air quality model, and deduced 7-day moving averages of NOX emissions for host and neighboring cities of 11 events held from 2010 to 2023 in Yangtze River Delta (YRD). We find the benefits of short-term controls on emissions for these events have been weakened over time, due to gradually tightened long-term controls and to a more cautious strategy of air quality improvement for recent events. The main sector of emission abatement for events shifted from power to industry and transportation, reflecting the diverse progresses of regular controls for different sectors. As a legacy, short-term controls supported better design of long-term air quality policies.

How to cite: Wang, H., Zhao, Y., He, Q., Hao, K., Qin, K., Zheng, B., and Lin, J.: Declining opportunity and enhanced targeting of short-term emission controls for major events in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1754, https://doi.org/10.5194/egusphere-egu25-1754, 2025.

EGU25-1814 | Orals | AS3.27

Observing volcanic SO2 from a constellation of FengYun hyperspectral infrared sounders 

Zhao-Cheng Zeng, Lieven Clarisse, Bruno Franco, Chengli Qi, Lu Lee, and Xiuqing Hu

Sulfur dioxide (SO2) from volcanic eruptions can have a significant impact on atmospheric chemistry and climate, and pose a threat to aviation. Satellite observations provide a unique opportunity to track the spatial distribution, vertical structure and temporal evolution of volcanic SO2 plumes. In this study, we use observations from the FengYun-3 (FY-3) series of meteorological satellites, which have formed a Hyperspectral Infrared Atmospheric Sounder (HIRAS) constellation in dawn-dusk, mid-morning and afternoon sun-synchronous orbits. The constellation provides six global observations in one day in the thermal infrared with equatorial overpass times of 5:30 am/pm (FY-3E), 10:00 am/pm (FY-3F) and 2:00 am/pm (FY-3D). SO2 layer height and total column are obtained from HIRAS spectra observations for two volcanic eruptions in 2024 in the tropics and high latitudes, respectively. The retrieval results from the three sounders are generally consistent. Intercomparisons with existing data from IASI satellites, model simulations and Microwave Limb Sounder are performed to assess the robustness of the retrieved data products. Our results show that the global FengYun-3 HIRAS constellation captures well the spatial and vertical evolution of lofted volcanic SO2 plumes after eruptions. This study represents an important application of a global constellation of FengYun hyperspectral infrared sounders for monitoring global variations in atmospheric composition.

How to cite: Zeng, Z.-C., Clarisse, L., Franco, B., Qi, C., Lee, L., and Hu, X.: Observing volcanic SO2 from a constellation of FengYun hyperspectral infrared sounders, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1814, https://doi.org/10.5194/egusphere-egu25-1814, 2025.

EGU25-2882 | ECS | Orals | AS3.27

Intercomparison of lower-tropospheric NO2 profiles from the CINDI-3 measurement campaign, the CAMS regional model, and the NitroNet neural network 

Leon Kuhn, Steffen Beirle, Steffen Ziegler, Andrea Pozzer, and Thomas Wagner

Nitrogen dioxide (NO2) plays a key role in the formation of urban smog and its adverse impact on human health. However, the routinely deployed measurements of NO2 are essentially limited to:

  • tropospheric NO2 columns with global daily coverage, measured by the TROPOMI satellite instrument with a horizontal resolution of up to 3.5 x 5.5 km2
  • near-surface NO2 concentrations, measured by in situ instruments at typically 0-8 m above ground with sparse spatial coverage
  • NO2 profiles from MAX-DOAS measurements, with extremely sparse coverage and significant retrieval uncertainties 

Regional chemistry and transport models (CTMs) facilitate the prediction of air pollutants with dense spatial coverage at urban-scale resolutions (e.g. 10 x 10 km2 or better), thereby yielding a valuable extension to the available observational data. Furthermore, significant progress has recently been made in developing neural network surrogate models with the ability to partially replace the computationally expensive CTM simulations. The NitroNet model, for example, can predict tropospheric NO2 profiles based on TROPOMI satellite observations and other ancillary variables, such as emission data and meteorological information.

A particular challenge is the validation of such models at altitudes within the boundary layer due to the lack of suitable observations, but data from measurement campaigns can partially fill these gaps. The CINDI-3 measurement campaign took place in May 2024 and comprised diverse spectroscopic measurements of NO2 concentrations in the lowest few hundred meters above ground. Moreover, CINDI-3 is the first CINDI campaign since the launch of the TROPOMI instrument, whose measurements are the main input to the NitroNet model.

We present an intercomparison of lower-tropospheric NO2 profiles from CINDI-3 long-path DOAS measurements, the CAMS CTM, and the NitroNet neural network. We provide a comprehensive overview of the near-surface NO2 profile shapes, as well as the level of agreement between measurements and simulation results obtained with different modelling approaches (here: a classic CTM simulation and a neural network based surrogate model).

How to cite: Kuhn, L., Beirle, S., Ziegler, S., Pozzer, A., and Wagner, T.: Intercomparison of lower-tropospheric NO2 profiles from the CINDI-3 measurement campaign, the CAMS regional model, and the NitroNet neural network, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2882, https://doi.org/10.5194/egusphere-egu25-2882, 2025.

Monitoring the spatiotemporal distribution of formaldehyde (HCHO) is crucial for reducing volatile organic compounds (VOCs) emissions, and the long-term evolution of socio-natural sources contributions to tropospheric HCHO over China is still unclear. We propose an oversampling algorithm for quantitatively tracking the evolution of uncertainty, which lowers the uncertainty of the original Level 2 OMI HCHO data (50% -105%) to 0-50%, and then we examine the evolution of contributions from various emissions sources applying multi-scale correlation. We found that the high formaldehyde emissions caused by human activities in eastern China are crossing the Hu Huanyong Line, which was formerly used to demarcate the population distribution. National-scale analysis indicate that HCHO emissions are significantly correlated with per capita Gross Domestic Product (per capita GDP) (r = 0.948) and Normalized Difference Vegetation Index (r = 0.864), while no substantial correlation with land surface temperature (LST) (r = 0.233). Diagnosis at pixel scale reveals that anthropogenic emissions continue to weaken the contributions of HCHO emissions caused by the increase in vegetation proportion. Our research identifies the evolutionary process and characteristics of the spatiotemporal distribution and socio-nature sources contributions of tropospheric formaldehyde of China from 2005 to 2022. 

How to cite: Xia, H.: Revealing the characteristics of long-term Chinese tropospheric formaldehyde under the influence of socio-natural sources, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3172, https://doi.org/10.5194/egusphere-egu25-3172, 2025.

EGU25-3426 | Posters on site | AS3.27

Top-down NOx estimation from TROPOMI observation over East Asia 

Kyung M. Han

Atmospheric nitrogen oxides play a crucial role as a precursor of nitrate and ozone formations. East Asia is still one of the significant contributors to the global NOx budget. Therefore, we evaluated the accuracy of bottom-up and top-down NOx emissions by comparing tropospheric NO2 columns simulated from the CMAQ with those from the TROPOMI over East Asia for four months. The CMAQ simulation using the UNIMIX inventory illustrates an overestimation of NO2 columns by approximately 28-53% in Central East China (CEC) compared to the TROPOMI observation. In contrast, the South Korean (SK) region shows an underestimation of 8-28% for the same period, except for an overestimation of 18% in April. To improve the accuracy of NOx emissions in East Asia, we estimated top-down NOx emissions using an algorithm based on the Finite Difference Mass Balance (FDMB) method with TROPOMI observation data. The top-down approach indicated a decrease of 4-32% in emissions for the CEC region and an increase of 9-24% for the SK region compared to bottom-up estimates. Utilizing the top-down NOx emission in the CMAQ simulation demonstrated enhanced spatial and temporal consistency with the TROPOMI-observed NO2 columns. Additionally, we evaluated the accuracy of the top-down NOx emission from a comparison between the simulation and independent in-situ observations of the AirKorea network.  

How to cite: Han, K. M.: Top-down NOx estimation from TROPOMI observation over East Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3426, https://doi.org/10.5194/egusphere-egu25-3426, 2025.

EGU25-3688 | Posters on site | AS3.27

Impact of wind fluctuations on the performance of the divergence method: How steady is the state? 

Steffen Beirle, Leon Kuhn, and Thomas Wagner

The divergence, i.e. the spatial derivative of the horizontal flux, allows to identify point sources due to the strong local gradients, and to quantify emissions from satellite measurements of atmospheric pollutants or greenhouse gases such as NO2 or CH4.
A central assumption made in this approach is that steady state is fulfilled. I.e., spatio-temporal changes of emissions, chemical conditions, or wind fields are not accounted for. Thus it has to be expected that the emission estimate is affected and probably biased in case of deviations from steady state.

Here we investigate quantitatively how far deviations from steady state affect the results of the divergence method. In particular, we quantify the spatial and temporal variability of wind fields and relate them to NOx emission estimates for selected power plants based on individual TROPOMI orbits as well as on WRF-Chem simulations.
The goal is to provide a measure for "steadiness" that could be used to identify and mask out unfavourable conditions. With this filter, it is expected that the remaining emission estimates have lower uncertainties. Other methods for emission estimates that are based on steady state assumption as well, like the calculation of cross-sectional fluxes, will probably also benefit from this.

How to cite: Beirle, S., Kuhn, L., and Wagner, T.: Impact of wind fluctuations on the performance of the divergence method: How steady is the state?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3688, https://doi.org/10.5194/egusphere-egu25-3688, 2025.

EGU25-4718 | ECS | Posters on site | AS3.27

Atmospheric pollution in Ukraine (2022-2023): role of fires in CO, NO2, and aerosol emissions during two years of military conflict  

Liudmyla Malytska, Evgenia Galytska, Annette Ladstätter-Weißenmayer, Mykhailo Savenets, and Stanislav Moskalenko

More than two years of hostilities, which began on the 24th of February 2022 with the invasion by Russian armed forces into Ukraine, have altered the emission patterns by destructing industrial facilities and the emerging new local pollution sources from military actions and missile strikes. In this respect, we discuss the changes in air quality across Ukraine during the first two years of the conflict (2022–2023), with a specific focus on fires as a key contributor to pollution. To facilitate spatial and temporal analysis, we distinguish eight regions within the territory of  Ukraine, which makes it possible to map the extent and magnitude of fire-related emissions and track their evolution in response to the changes in the front-line location. We utilized data from the European Forest Fire Information System (EFFIS), specifically the MODIS/SENTINEL-2 Burnt Areas product, to identify the extent of burnt areas, analyze fire activity, categorize affected land cover types, and assess the resulting influence on atmospheric pollution levels. To link fire episodes with pollution, we used Sentinel-5 Precursor (S5P) TROPOMI Level 2 data for tropospheric NO2, CO, and the Absorbing Aerosol Index (AAI). Additionally, we incorporated ground-based observations from the Ukrainian National Air Quality Network (NAQN), a system of about 100 monitoring stations in 39 cities across Ukraine that measure atmospheric chemicals, which has not been done before. 

It was found that in Ukraine in 2022, the war was a major driver of fire activity, with 66% of the total burned area located within a 30-km zone along the front line. In 2023, this proportion increased to nearly 80% within the same 30-km zone. The retrieved satellite emissions showed that peak fire activity was accompanied by increases in NO2, CO, and aerosol concentrations, which exceeded the historical daily maxima for 2018-2021. Ground-based observations showed mixed tendencies, with concentrations decreasing in 16 cities and significantly rising in others (9 cities). The proximity of monitoring stations to industrial sources complicates the ability to isolate air quality changes that were not directly caused by industry or industrial destruction. Only Sloviansk (Donetsk region, located 20-30 km from the front line) showed reliable increases in NO2, CO, and dust concentrations, which could be directly attributed to military activities. To demonstrate the contribution of increased fire activity to atmospheric pollution, we compared biomass burning emissions, based on fire radiative power, with anthropogenic emission inventories from periods before and during the hostilities. During severe fire seasons (2020, 2022, and 2023), both the Copernicus Atmosphere Monitoring Service (CAMS) and Global Fire Assimilation System (GFAS) inventories reported comparable NOx emission levels, while CO emissions increased by up to 11-fold. In contrast, during a milder fire season (2021), NOx emissions were 2.5 times lower than industrial emissions, whereas CO levels were similar to or slightly exceeded those from industrial sources. This evidence suggests that in Ukraine, pollution from fires, also caused by war, can be as significant as emissions from industrial sources, depending on the intensity of the fire season.

How to cite: Malytska, L., Galytska, E., Ladstätter-Weißenmayer, A., Savenets, M., and Moskalenko, S.: Atmospheric pollution in Ukraine (2022-2023): role of fires in CO, NO2, and aerosol emissions during two years of military conflict , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4718, https://doi.org/10.5194/egusphere-egu25-4718, 2025.

EGU25-4902 | ECS | Posters on site | AS3.27

Four-decade Trends and Latitudinal Variations of Satellite-derived Aerosol in Global Oceanic Regions  

Linxuan Li, Xiaohui Bi, and Yinchang Feng

Air pollution over the oceans has received less attention compared to densely populated urban areas of continents. Over the past four decades, satellite-derived Aerosol Optical Depth (AOD) data reveal significant spatial and temporal variations across global oceans. The global mean AOD is approximately 0.112, with higher levels in the Central Atlantic (~0.206), North Indian Ocean (~0.201), and Western North Pacific (~0.197). Latitudinal analysis shows that the highest AOD values are concentrated in the Northern Hemisphere, particularly between latitudes 0° and 70° N. except for the Gulf of California and Hudson Bay, AOD values in the other fourteen surveyed inland seas surpass the mean levels found at similar latitudes in oceanic regions. Over the last four decades, AOD trends have revealed a significant decrease across about 89.5% of global oceanic grids, while an increase in AOD is observed in low-latitude oceanic areas (30° S-30° N). The turning-points of the AOD in each inland sea confirm the success of regional emission control policies initiated on the adjacent continents. Our findings suggest that regional emission control policies have been successful in many areas, but further adjustments, such as relocating heavy industries away from coastal areas, are needed to reduce pollution in regions like the Bohai Sea.

How to cite: Li, L., Bi, X., and Feng, Y.: Four-decade Trends and Latitudinal Variations of Satellite-derived Aerosol in Global Oceanic Regions , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4902, https://doi.org/10.5194/egusphere-egu25-4902, 2025.

EGU25-5690 | ECS | Posters on site | AS3.27

Quantifying Sulfur Dioxide Emissions from Industrial Activities by a Helicopter-borne System and TROPOMI in the Southern Arabian Peninsula 

Niclas Maier, Eric Förster, Heidi Huntrieser, Benjamin Witschas, Falk Pätzold, Lutz Bretschneider, Astrid Lampert, Mark Lunt, and Anke Roiger

Sulfur dioxide (SO2) is an air pollutant that is toxic to humans and, as a precursor to sulfuric acid, has far-reaching consequences for the environment and climate. Anthropogenic emissions are responsible for two-thirds of total SO2 emissions into the atmosphere. Stricter regulations and technical developments, such as the installation of desulfurization systems in coal-fired power plants, are reducing emissions in parts of the world such as Europe. However, inventories show a stagnation in emissions in the Middle East region in recent years. In the global SO2 catalogue provided by NASA, satellite instruments such as TROPOMI (onboard Sentinel-5P) assign many point sources in this region to the production of oil and gas. Two of these hotspots are detected in the southern Sultanate of Oman.

 As part of the METHANE-To-Go-Oman campaign in 2023, for the first time the helicopter-borne probe HELiPOD (weight 325kg, length 5m) was used to determine SO2 emissions from selected oil and gas facilities in Oman. The HELiPOD was equipped with a UV fluorescence instrument (Envea AF22e) to measure SO2 in-situ with high precision (1ppb), as well as with a precise wind measurement system. The entire SO2 plume from selected facilities was sampled at different altitudes (50 m to 2000 m) at variable distances (1 km to 4 km) downwind from the source. Flight pattern were designed on a day-to-day basis based on actual wind speed and wind direction measured with a ground-based Doppler wind lidar (Streamline XR, Halo Photonics).

In this study, top-down derived SO2 mass flux estimates based on HELiPOD data are presented for six selected point sources from the oil and gas industry in northern and southern Oman. Subsequently, these top-down estimates are compared to bottom-up emission inventories available for the region.  In addition, TROPOMI data from the years 2018 to 2023 are analyzed to investigate the temporal development of SO2 point sources in the whole Middle East area. The satellite data show a very good temporal coverage and we were able to identify a new emission source in the northern part of Oman in 2023. In the present global SO2 catalogue provided by NASA this source is not yet included. The signal strength of this northern source is similar to the southern hotspots in the years before. The HELiPOD mass flux estimates also confirm the significant decrease in emissions between 2021 and 2023 from one of the two hotspots in the southern Oman based on TROPOMI data. In general, our study indicates low SO2 emissions from the oil and gas industry in Oman compared to other countries in the Middle East. 

How to cite: Maier, N., Förster, E., Huntrieser, H., Witschas, B., Pätzold, F., Bretschneider, L., Lampert, A., Lunt, M., and Roiger, A.: Quantifying Sulfur Dioxide Emissions from Industrial Activities by a Helicopter-borne System and TROPOMI in the Southern Arabian Peninsula, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5690, https://doi.org/10.5194/egusphere-egu25-5690, 2025.

EGU25-5821 | ECS | Posters on site | AS3.27

Estimation of Long-Term Ozone Variability in East Asia (2005–2024): Integration of OMI, TROPOMI, and GEMS Satellite Data 

Ha Jeong Jeon, Jae Hwan Kim, Jeong-Ah Yu, Sang-Min Kim, and Sang Seo Park

East Asia is a region with particularly high emissions of ozone precursors due to the effects of industrialization and urbanization, making continuous monitoring of air pollution and environmental changes crucial. To address this need, the GEMS sensor onboard the GK-2B satellite, launched in 2020, serves as an important tool for real-time observation of the East Asian region from a geostationary orbit. While GEMS offers the advantage of continuous monitoring of air quality in East Asia, its relatively short observation period limits its use for long-term analysis. To overcome this limitation, this study integrates GEMS, OMI and TROPOMI satellite data to construct a 20-year record (2005–2024) and analyze the seasonal and spatial characteristics of ozone variability. Level 2 data from each satellite were processed using a consistent algorithm to generate Level 3 data, and the discrepancies during overlapping observation periods between the satellites were corrected to reduce inconsistencies. The corrected data were validated through cross-verification between the satellites. The validation results showed a slope ranging from 0.95 to 1, an R-squared value above 0.9, and an RMSE of less than 5 DU. To further assess the accuracy of the long-term data generated in this study, validation with ground-based observations is also necessary.

 

This work was supported by the National Research Foundation of Korea(NRF) grant funded by the Korea government(MSIT) (NRF-RS-2023-00219830) and a grant from the National Institute of Environment Research (NIER), funded by the Ministry of Environment (MOE) of the Republic of Korea (NIER-2024-01-02-042).

How to cite: Jeon, H. J., Kim, J. H., Yu, J.-A., Kim, S.-M., and Park, S. S.: Estimation of Long-Term Ozone Variability in East Asia (2005–2024): Integration of OMI, TROPOMI, and GEMS Satellite Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5821, https://doi.org/10.5194/egusphere-egu25-5821, 2025.

EGU25-6271 | ECS | Orals | AS3.27

Integration of satellites and low-cost sensors for high-resolution air quality mapping in East African megacities 

Samuel Chua, Otienoh Oguge, Richard Sserunjogi, Deo Okure, Asinta Manyele, Katrianne Lehtipalo, Martha A. Zaidan, and Tuukka Petäjä

In East Africa, scarcity of air quality data in rapidly expanding cities has hindered planners’ ability to mitigate air pollution effectively. We explored how low-cost air quality sensors, reference monitors, and satellite-derived products from Sentinel-5p and MODIS can be integrated to generate ground-truthed, high-resolution (1 km × 1 km) daily maps of PM2.5 concentrations over the megacities of Kampala, Nairobi, and Dar es Salaam. These maps and accompanying codes, which in principle can be applied to other data-scarce cities, would be made available during the session. The findings reveal that average PM2.5 concentrations sometimes exceed recommended air quality thresholds, with significant seasonal and spatial variability. Challenging existing preconceptions, the study found that PM2.5 levels could be higher in suburban zones than in city centres, due to seasonal vegetation shifts and combustion-related activities. This work further demonstrates the feasibility of combining low-cost sensors with satellite data to improve air quality monitoring especially in data-scarce regions.

How to cite: Chua, S., Oguge, O., Sserunjogi, R., Okure, D., Manyele, A., Lehtipalo, K., Zaidan, M. A., and Petäjä, T.: Integration of satellites and low-cost sensors for high-resolution air quality mapping in East African megacities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6271, https://doi.org/10.5194/egusphere-egu25-6271, 2025.

EGU25-8135 | Orals | AS3.27

 Detection of hotspot areas using Sentinel-5P and GEMS imagery for evaluating bottom-up emission inventorie 

Thierno Doumbia, Claire Granier, Hugo Merly, Gerrit Kuhlmann, Oscar Collado, and Marc Guevara

Emissions from power plants contribute significantly to the overall greenhouse gas and air pollutant levels. Satellite observations of compounds such as NO2 and CO can help improve CO2 emission estimates, as proposed in the CORSO (CO2 Monitoring and Verification Support Research on Supplementary Observations) project. One of the key objectives of CORSO is to improve global and local capabilities in using observations of co-emitted species (NO2 and CO) to better estimate anthropogenic CO2 emissions. In this presentation, we will discuss a methodology developed to detect hotspots associated with power plants using NO2 data from the TROPOMI instrument on the Copernicus Sentinel-5P satellite, as well as observations from the Geostationary Environment Monitoring Spectrometer (GEMS) over Eastern and Southeast Asia. The final goal is to improve the accurate detection of hotspot locations to identify missing sources in emission inventories and refine their geolocation. It is important to note that the detectability of the anthropogenic signal from co-emitted species is generally much higher than that of CO2. Various statistical methods have been tested to identify high-probability hotspots in the NO2 tropospheric column densityfrom TROPOMI and GEMS. This includes an exploratory spatial data analysis for cluster detection (Getis-Ord Gi*), which evaluates each spatial variable’s neighborhood to determinewhether its values are significantly higher or lower than those in the surrounding area. The results indicate agreement between the hotspots identified through the Gi* method and the locations of power plants from the literature. These identified hotspot coordinates can be used to enhance the quanification of emissions and address mislocation in power plant emissions withinemission inventories.

How to cite: Doumbia, T., Granier, C., Merly, H., Kuhlmann, G., Collado, O., and Guevara, M.:  Detection of hotspot areas using Sentinel-5P and GEMS imagery for evaluating bottom-up emission inventorie, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8135, https://doi.org/10.5194/egusphere-egu25-8135, 2025.

EGU25-9106 | Orals | AS3.27

Surface albedo fitting in the optimal estimation routine of the TROPOMI oxygen A-band aerosol layer height product. 

Martin de Graaf, Maarten Sneep, Mark ter Linden, L. Gijsbert Tilstra, and J. Pepijn Veefkind

The Sentinel-5P/TROPOMI  Aerosol Layer Height (ALH) is based on an optimal estimation (OE) approach, fitting cloud-free measurements to synthetic reflectances in the strongest oxygen absorption (O2-A) band, provided by a neural network trained with high resolution simulated reflectances. The ALH has been continuously improved since its release in 2019, focusing especially on (bright) land surfaces, over which the ALH product showed underestimated aerosol layer heights (biased towards the surface). In this presentation the latest updates of the ALH product will be discussed, including the introduction of the Directional Lambertian-Equivalent Reflectance (DLER) climatology to improve the surface albedo characterisation over land. Secondly, by adding the surface albedo in the feature vector of the OE inversion, using the DLER as prior information, retrievals improved considerably over land, especially in the case of bright surfaces. New retrievals over land now largely match the retrievals over ocean, which have shown a good comparison with validation data since its release, most notably with CALIOP weighted extinction heights. The albedo is fitted for both land and ocean surfaces, but the implementation is different over land and ocean because of the large range of land surface albedos. Over ocean, the retrievals are optimised by tuning the a priori error settings, while over land the a priori surface albedo values are relaxed so the fitting procedure can incorporate the albedo effects in the retrieval.  About 1.5 times more converged results were obtained with the current implementation, with low land-ocean contrasts in the aerosol layer height retrievals. The average difference with CALIOP weighted extinction height decreased for selected cases from about −1.9 km to −0.9 km over land and from around −0.8 km to +0.1 km over ocean.

We will show the latest results of the TROPOMI ALH products, by comparisons with CALIOP and GEMS Aerosol layer height retrievals, and show some preliminary results with EarthCARE data. Implementing of this algorithm for Sentinel-3/OLCI O2-A band measurements and the algorithm developments for the upcoming Sentinel-4 and Sentinel-5 mission will also be highlighted.

How to cite: de Graaf, M., Sneep, M., ter Linden, M., Tilstra, L. G., and Veefkind, J. P.: Surface albedo fitting in the optimal estimation routine of the TROPOMI oxygen A-band aerosol layer height product., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9106, https://doi.org/10.5194/egusphere-egu25-9106, 2025.

This study focuses on TROPOMI based observations and retrieval uncertainties of tropospheric CO and HCHO in Central Asia, an area experiencing rapid development. The data is applied within the Model Free Inversion Estimation Framework (MFIEF), to calculate daily, grid-by-grid CO emissions and uncertainty range from 2019 to 2023.

The framework herein has been expanded by integrating the data with explicit observational uncertainties, and applying a new and unbiased analytical system to perform comprehensive uncertainty analysis. Results show that the observational uncertainties have a significant impact on the calculated emissions, with approximately 55% of the data deemed unreliable. After filtration, the remaining data reveals more distinct high-value areas, while excluding the small number of extremely high values which were as likely to be due to observational noise as the large number of very low emissions pixels. Remaining pixels generally conform to know industrial, power, coal, steel, mining, and urban areas, enhancing the reliability of emission estimates. A few interesting exceptions, as discussed herein include large underground coal fires.

The CO emissions exhibit distinct temporal and spatial patterns. In urban and industrial areas of China from 2019 to 2022, emissions show a downward trend, followed by a slight increase in 2023, while in underground coal fire areas and in non-Chinese areas of Central Asia there are different trends observed. Emissions are highest during the months with the least UV radiation and coldest temperatures, such as December and January. Spatially, high emissions are concentrated in urban and industrial areas, while natural areas have relatively lower emissions, with the notable exception of underground burning coal fields which are found to be roughly as significant as large steel, power, and industrial sites.

Comparisons with EDGAR indicate our results have both different spatial distribution and temporal variation. Our results show a greater likelihood of decreasing over time and more variability (daily to weekly scale). This provides a scientific basis for understanding CO emissions in Central Asia while also contributing to the improvement of emission inventories, air quality models, as a basis dataset for CO and CH4 retrievals, and even for attribution studies to be performed.

How to cite: Feng, Y., Cohen, J. B., Li, X., and Qin, K.: CO emissions inversion using satellite CO observations and uncertainty in tandem identify and Attribute New and Unknown Sources over Central Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9171, https://doi.org/10.5194/egusphere-egu25-9171, 2025.

EGU25-9209 | ECS | Posters on site | AS3.27

Dynamic lightning NOx production rates obtained with space-based low-Earth orbiting and geostationary lightning imagers 

Rebekah Horner, Eloise Marais, and Lee Murray

Lightning is a crucial driver of nitrogen oxides (NOx) in the free troposphere where tropospheric ozone formation is limited by the availability of NOx. NOx production per lightning flash in models is typically represented with a single temporally and spatially static value, likely affecting the accuracy in simulating past, present, and future lightning NOx and consequent changes in tropospheric ozone (O3) and other oxidants. We determine spatially (0.5° × 0.625°) varying hourly NOx production rates (mol N fl⁻¹) using literature reported relationships between NOx yields and lightning flash radiant energies from Lightning Imaging Sensors (LIS) aboard the Tropical Rainfall Measuring Mission (TRMM) and the International Space Station (ISS). The diurnal and spatial variability of the radiant energies from the LIS instruments are assessed to be overall consistent with optical energies from the Geostationary Lightning Mapper (GLM) instrument, which monitors the Americas every 5 minutes. The diurnal variability between the two datasets differs by < 15%. Our lighting NOx production rates are added to GEOS-Chem, yielding global emissions of 6.5 Tg N yr-1 for 2015-2019, closely aligning with 5.8 Tg N yr-1 in the original parameterised representation, but with large differences in the spatial distribution of lightning NOx. Our updated parameterisation causes increases of > 50 pptv in NO2 across the troposphere, particularly in the tropics coincident with deep convection. The resultant changes in tropospheric composition improve agreement with satellite-derived vertical profiles of NO2 obtained via cloud-slicing TROPOMI by decreasing the model underestimate in free tropospheric NO2. Assessment against cloud-sliced O3 is underway.

How to cite: Horner, R., Marais, E., and Murray, L.: Dynamic lightning NOx production rates obtained with space-based low-Earth orbiting and geostationary lightning imagers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9209, https://doi.org/10.5194/egusphere-egu25-9209, 2025.

EGU25-9438 | ECS | Posters on site | AS3.27

Retrieval and Comparison of Multi−Satellite Atmospheric composition concentration Data from the EMI Series Instruments 

Wu kaili, Luo yuhan, Si fuqi, and Zhou haijin

The Environmental Trace Gases Monitoring Instruments (EMI) are the second generation of spectrometers on-aboard the Gaofen-5 (GF-5) and Daqi-1 (DQ-1) satellites in China, which can be used to analyze trace gases such as O3 , NO2 and BrO. EMI enables continuous daily global trace gas observations at a spatial resolution of 7×13 km2. In this study, the differential optical absorption spectroscopy (DOAS) algorithm was used to invert EMI spectral data to obtain the total column concentrations of O3 , NO2 and BrO of the three satellite loads. Due to the different overpass times of different loads, the daily variation trend of trace gases is obtained through comparative analysis, and the overall quality and reliability of EMI series data sets are verified by cross-comparison. The daily EMI total ozone column (TOC) was compared with the vertical column density (VCD) collected by the TROPOspheric Monitoring Instrument (TROPOMI). The results showed that the spatial distribution of daily EMI series TOC and TROPOMI TOC from September to December 2023 had a good correlation (R≥0.95), and the relative differences were less than 5% when verified with data from ground-based stations. In addition, the EMI series TOC data fusion results were highly correlated with TROPOMI TOCs (R = 0.99), weighted fusion assigns weighting factors to each instrument by inverting RMS of different loads. The consistency of NO2 between EMI loads was high (R ≥ 0.90), and the correlation between the total column concentration of NO2 and TROPOMI was also high (R ≥ 0.80). Retrieval results of BrO products from March to May 2024 in Arctic region also revealed significant increases in BrO concentrations caused by bromine explosion events in the spring. The results of these products highlight the potential of EMI instruments for long-term continuous monitoring of global trace gas distribution and changes, helping to build high-quality atmospheric component concentration data sets.

 

How to cite: kaili, W., yuhan, L., fuqi, S., and haijin, Z.: Retrieval and Comparison of Multi−Satellite Atmospheric composition concentration Data from the EMI Series Instruments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9438, https://doi.org/10.5194/egusphere-egu25-9438, 2025.

Retrievals of column average methane mixing ratio (XCH4) from satellites can provide a wealth of information on the fluxes of CH4. The TROPOMI instrument onboard the satellite Sentinel-5P is particularly interesting for flux estimation using atmospheric inversions as it provides global coverage with relatively high-resolution ground pixels of 5.5 × 7.5 km2 (at nadir). Furthermore, there are several different retrieval products available for TROPOMI XCH4, making it possible to compare these and quantify the effect that differences between them have on CH4 fluxes from atmospheric inversions.

In this study, we have compared XCH4 from three retrieval products: i) the official ESA product provided by SRON, ii) the Weighting Function Modified Differential (WFMD) product from the University of Bremen, and iii) the blended TROPOMI-GOSAT product (S5P-BLND) from Harvard University, in atmospheric inversions over Europe for the year 2020. In addition, we compare fluxes from each of these with those derived with an inversion using ground-based observations from the ICOS atmospheric network. For flux estimation, we use the Bayesian inversion framework, FLEXINVERT, and the Lagrangian atmospheric transport model, FLEXPART, driven by ECMWF ERA5 meteorological reanalysis data.

We find that the fluxes derived using WFMD and S5P-BLND products agree better with those derived using ICOS data. The difference in performance of the official ESA product versus the WFMD and S5P-BLND products appears to be related to the albedo bias correction used in the ESA product, which may result in an overcorrection giving too high values of XCH4 in regions of low albedo and too low values over regions of high albedo. Moreover, this study emphasizes the need to compare different retrieval products and, if available, ground-based observations, in atmospheric inversions to identify any biases and address these.

How to cite: Thompson, R., Schneider, P., and Stebel, K.: Using different TROPOMI XCH4 retrieval products in atmospheric inversions of CH4: a comparison and reconciliation over Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9567, https://doi.org/10.5194/egusphere-egu25-9567, 2025.

EGU25-9700 | ECS | Orals | AS3.27

Enhancing Satellite-Based NO2 Monitoring with Machine Learning: From Near Surface Concentration Estimation to A-Priori Profile Development 

Wenfu Sun, Frederik Tack, Lieven Clarisse, and Michel Van Roozendael

Satellite observation plays an important role in air quality monitoring. Nitrogen dioxide (NO2) is an important atmospheric trace gas that significantly impacts air quality, public health, and ecosystems. While satellite NO2 observations have been widely used in the application of machine learning (ML) to estimate surface NO2 distributions, this surface NO2 modeling deserves further investigation, including examining satellite’s contributions to the estimation of NO2 at different concentration levels. In addition, as satellite data evolve towards higher spatiotemporal resolution, the demand for high-resolution a-priori NO2 profiles is increasing. Generating such profiles using traditional numerical models is computationally expensive, but ML offers an efficient solution to address this challenge. This presentation illustrates two developments based on ML technology: one focusing on the application of satellite observations to estimate surface NO2 distributions, and the other on the development of high-resolution a-priori NO2 profiles for satellite retrievals. Western Europe is used as the study area.

The first part addresses estimating high-resolution surface NO2 concentrations (1 km, daily) using the Boosting Ensemble Conformal Quantile Estimator (BEnCQE). This model integrates diverse datasets, including TROPOMI NO2 tropospheric vertical column densities (TVCDs), and demonstrates reliable performance validated against European Environmental Agency (EEA) surface observations (r = 0.80, R² = 0.64, RMSE = 8.08 µg/m³). Quantile regression in BEnCQE provides uncertainty estimates and feature importance analysis across different NO2 levels. Results show that satellite observations significantly contribute to background NO2 predictions but have less influence on high-concentration estimates, likely due to the relatively coarse spatial resolution of current satellite data. These findings highlight the need for higher-resolution satellite missions, such as CO2M (2 km resolution), to better capture localized pollution.

The second part focuses on generating high spatial resolution a-priori NO2 profiles for satellite retrievals. We developed Deep Atmospheric Chemistry NO2 (DACNO₂), a convolutional neural network framework, to produce 3D NO2 distributions (8 levels from the surface to 5,000 m, 2 km spatial resolution, daily). Using a multi-constraint training approach that combines coarse-resolution CAMS-EU synthetic NO2 data (10 km) and fine-scale EEA surface observations (2 km), DACNO2 captures detailed spatial gradients near emission hotspots while maintaining broad physical consistency. The evaluation shows good performance aligned with EEA observations (r = 0.81, R² = 0.64, RMSE = 5.10 µg/m³) and CAMS-EU synthetic NO2 (r = 0.94, R² = 0.89, RMSE = 1.11 µg/m³). The implementation of DACNO2 is efficient, taking only minutes to compute one day's result using GPU acceleration.

Overall, this presentation introduces ML-based works on application and development aspects for satellite NO2 observations to advance the coupling of ML technology and satellite observations of pollution.

How to cite: Sun, W., Tack, F., Clarisse, L., and Van Roozendael, M.: Enhancing Satellite-Based NO2 Monitoring with Machine Learning: From Near Surface Concentration Estimation to A-Priori Profile Development, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9700, https://doi.org/10.5194/egusphere-egu25-9700, 2025.

Atmospheric ammonia (NH3) is a reactive nitrogen compound that affects air quality and threatens public health. Real-time monitoring of atmospheric NH3 variations using satellite measurements will provide a reliable scientific basis for evaluating emission management strategies for anthropogenic sources. As the world's first geostationary hyperspectral infrared sounder, the Geostationary Interferometric Infrared Sounder (GIIRS) on board the FengYun-4 series of satellites provides an important advance to monitor NH3 total columns with day/night measurements at a 2-hour temporal resolution and a spatial resolution of 12 km at nadir. Using GIIRS NH3 retrievals, this study focused on the analysis of industrial and agricultural NH3 point sources over East Asia and in particular the diurnal cycle of these point sources. The identified point sources are first compared with estimates from the Emissions Database for Global Atmospheric Research (EDGAR) and similar hyperspectral infrared satellites, such as IASI and CrIS. The diurnal variations of NH3 point sources are further compared with simulations from chemical transport model such as GEOS-Chem. The findings demonstrate the unique capability of FY-4B/GIIRS in identifying NH3 point sources and capturing their temporal changes over East Asia, offering critical insights beyond the capabilities of current low-Earth orbit (LEO) instruments.

How to cite: Sheng, M., Zeng, Z.-C., and Hua, J.: Monitoring ammonia point sources over East Asia from the Geostationary Interferometric Infrared Sounder (GIIRS) on board China's FengYun-4 satellite, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10058, https://doi.org/10.5194/egusphere-egu25-10058, 2025.

EGU25-10148 | Orals | AS3.27

Global carbon monoxide emissions constrained by TROPOMI 

Mihalis Vrekoussis, Johann Rasmus Nüß, Nikos Daskalakis, Fabian Günther Piwowarczyk, Angelos Gkouvousis, Oliver Schneising, Michael Buchwitz, Maria Kanakidou, and Maarten C. Krol

Since carbon monoxide (CO) in the atmosphere adversely affects air quality and climate, knowledge about its sources is crucial. However, current global bottom-up emission estimates retain significant uncertainties. In this study, we attempt to reduce these uncertainties by optimizing emission estimates for the second half of the year 2018 on a global scale with a focus on the northern hemisphere through the top-down approach of inverse modeling. Specifically, we introduce data from the TROPOspheric Monitoring Instrument (TROPOMI) into the TM5-4DVAR model. For this purpose, we developed novel methods to handle the unprecedented amount of data provided by TROPOMI. We compare the results from three inversion experiments that optimize CO emissions based on different observational data. In one experiment we only assimilate TROPOMI data, in a second experiment we only assimilate NOAA surface flask measurements, and in a third experiment we assimilate both datasets. We show that the inversion that assimilates only satellite observations reproduces flask measurements south of 55° N almost as well as the inversions that assimilated these measurements. These results show that the assimilation of TROPOMI data alone may provide reliable CO source estimates globally.

How to cite: Vrekoussis, M., Nüß, J. R., Daskalakis, N., Piwowarczyk, F. G., Gkouvousis, A., Schneising, O., Buchwitz, M., Kanakidou, M., and Krol, M. C.: Global carbon monoxide emissions constrained by TROPOMI, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10148, https://doi.org/10.5194/egusphere-egu25-10148, 2025.

EGU25-10824 | ECS | Orals | AS3.27

Geographic and Temporal Variability of atmospheric surface Ammonia (NH3) in France, Belgium, and the Netherlands (2015 – 2023) across different land-use types: Insights from Ground-Based and combined Satellite Observations. 

Varun Katoch, Anna Font, Aude Bourin, Esperanza Perdrix, Mark Shephard, Lieven Clarisse, Jeroen Staelens, Hans Berkhout, Martin Van Damme, and Véronique Riffault

This research study analyzes atmospheric ammonia (NH₃) surface concentrations in France, Belgium (Flanders region), and the Netherlands, highlighting their geographic, temporal, and diel variability from 2015 to 2023 using ground-based measurements (31 sites) and combined satellite data (IASI and CrIS). NH3 is the major alkaline gas in the atmosphere, affects air quality and aerosol formation, and degrades ecosystems, making its monitoring essential. The highest annual average NH₃ levels were observed in the Netherlands (7.4 ± 4.1 µg/m³), followed by Belgium (4.5±3.4 µg/m³) and France (3.7±2.1 µg/m³) as per in-situ observations. Rural areas characterized by agricultural practices showed higher levels than other land-use types, peaking in spring and summer due to fertilizer application and manure volatilization. Rural sites reached 8.5 ± 4.0 µg/m³ and 5.4 ± 3.9 µg/m³, in the Netherlands and Belgium (Flanders region) respectively. Urban areas recorded noticeable NH₃ concentrations either across Belgium (Flanders region) (3.5±2.0 µg/m³) and France (4.4 ± 2.0 µg/m³) which may be attributable to vehicular traffic, wastewater management, industrial operations, and the geographical dispersion of agricultural emissions. Seasonal variations observed notable NH₃ peaks in spring and summer, due to agricultural intensification and increased temperatures, while winter had the lowest concentrations due to decreased emissions. Diel patterns showed midday peaks in rural areas due to increased volatilization, while urban areas showed morning peaks related to traffic emissions. Satellite-derived NH₃ data from combined IASI and CrIS sensing showed moderate to strong correlations with ground-based measurements (R = 0.32–0.8), while satellites tended to underestimate local concentrations. Unlike surface measurements, satellite data revealed NH₃ concentrations across land-use types were little different, with means and standard deviations as follows: Crops (2.35 ± 2.08 µg/m³), High-Density Urban (2.39 ± 2.20 µg/m³), Low-Density Urban (2.35 ± 2.14 µg/m³), and Rural (2.26 ± 2.00 µg/m³). Comparable trends were noted in entire Belgium (+0.023 µg/m³ per year) and the Netherlands (+0.043 µg/m³ per year), where NH₃ concentrations were higher in 2020 and decreased in the following years possibly due to improved air dispersion and increased precipitation. The results highlight the key role of agriculture, which is the dominant source of NH₃ emissions, but urban regions also contribute significantly through vehicular and industrial activities. Effective mitigation techniques are crucial, including optimal fertilizer application, sophisticated manure management, and stringent urban emission regulations. These plans are in line with regional and national regulations, such as France’s PREPA plan, which aims to reduce NH₃ emissions by 13% by 2030 (Chatain et al., 2022). The integration of satellite and ground-based data offers a thorough understanding of NH₃ dynamics, facilitating the formulation of specific regulatory frameworks to reduce emissions, protect ecosystems, and improve air quality in these areas.

References

Chatain, M., Chretien, E., Crunaire, S., & Jantzem, E. (2022). Road Traffic and Its Influence on Urban Ammonia Concentrations (France). Atmosphere, 13(7), Article 7. https://doi.org/10.3390/atmos13071032

 

How to cite: Katoch, V., Font, A., Bourin, A., Perdrix, E., Shephard, M., Clarisse, L., Staelens, J., Berkhout, H., Damme, M. V., and Riffault, V.: Geographic and Temporal Variability of atmospheric surface Ammonia (NH3) in France, Belgium, and the Netherlands (2015 – 2023) across different land-use types: Insights from Ground-Based and combined Satellite Observations., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10824, https://doi.org/10.5194/egusphere-egu25-10824, 2025.

EGU25-11070 | ECS | Orals | AS3.27

From ground to orbit: Improving global methane emission inversions with adaptive weighting of TROPOMI and NOAA data 

Santiago Parraguez Cerda, Johann Rasmus Nüß, Nikos Daskalakis, Arjo Segers, Oliver Schneising, Michael Buchwitz, Mihalis Vrekoussis, and Maria Kanakidou

Methane (CH₄) has a relatively short, compared to other greenhouse gases, atmospheric lifetime (~9 years) and a highly effective radiative forcing, contributing ~31% (1.19 W m-2) of the additional radiative forcing from anthropogenic emissions during the industrial era. Therefore, reducing CH₄ emissions is a necessary target for limiting near-term climate change. Despite progress in understanding processes and improving estimates, uncertainties in CH₄ sources and sinks create discrepancies between bottom-up and top-down estimates. Recent satellites carrying high-resolution, accurate instruments have provided better information on the concentrations and distributions of atmospheric trace gases. High-confidence observations and in-situ measurement networks are essential to reduce discrepancies and increase confidence in the results of data-driven methods.

This study evaluates the feasibility and efficiency of performing inversions integrating satellite-based remote observations, weighted according to their temporal and spatial distribution with in-situ measurements. The inversions assimilate retrieved data from the high-resolution TROPOMI WFMD methane product and background stations from the NOAA network. Compared to the operational ESA product, the TROPOMI WFMD product provides enhanced global daily coverage, especially at higher latitudes, and more realistic uncertainty estimates, offering better insight into the distribution of methane concentrations. Results compare different inversions of global methane emissions for 2019 at 1° × 1° resolution, with and without an adaptive per-pixel weighting factor, performed utilising the TMVar (TM5-MP/4DVar) system. The adaptive inflation factor is applied to the satellite term of the cost function, balancing its contribution relative to the smaller data volume of station measurements. Data from the ground-based TCCON network validate the simulations. This network operates as a standard reference for atmospheric chemistry-transport models and satellite retrievals due to its precision and low uncertainty in total column values.

Preliminary results show no significant differences when including satellite data with the in-situ ones without applying a weighting factor, mainly due to the overwhelming volume of satellite data compared to station measurements. However, introducing a constant weighting factor for satellite observations improves inversion accuracy. Adding an adaptive weighting factor, adjusted based on the observations' temporal and spatial distribution, further enhances the results. This approach outperforms unweighted and constant-weighting methods by addressing the underuse of station data and neglect of satellite information in regions with lower coverage due to lower point density. Therefore, incorporating appropriately weighted sources of information on the total atmospheric state helps to optimise the inversion results and ultimately reduce the error in the constrained surface fluxes.

How to cite: Parraguez Cerda, S., Nüß, J. R., Daskalakis, N., Segers, A., Schneising, O., Buchwitz, M., Vrekoussis, M., and Kanakidou, M.: From ground to orbit: Improving global methane emission inversions with adaptive weighting of TROPOMI and NOAA data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11070, https://doi.org/10.5194/egusphere-egu25-11070, 2025.

EGU25-11419 | Orals | AS3.27

Burning season emissions of reactive nitrogen from fires in subtropical southern Africa determined with TROPOMI and IASI 

Eloise Marais, Lieven Clarisse, Martin Van Damme, Christine Wiedinmyer, and Killian Murphy

Widespread and intense dry season burning in subtropical southern Africa (2-20°S), peaking in June to September, results from ignition by humans for agricultural practices and is propagated by a continuous dry savanna landscape. These fires produce large quantities of the reactive nitrogen compounds nitrogen oxides (NOx≡NO+NO2) and ammonia (NH3), influencing tropospheric ozone and aerosol budgets and so affecting climate. Here we use observations of NO2 from the TROPOspheric Monitoring Instrument (TROPOMI) and NH3 from the Infrared Atmospheric Sounding Interferometer (IASI) to evaluate NO2 and NH3 simulated by the GEOS-Chem model driven with 3 distinct biomass burning inventories. These inventories differ in their use of satellite data products to constrain the timing, extent, severity and longevity of fires. The Global Fire Emissions Database version 4 with small fires inventory (GFEDv4s) uses burned area, Fire INventory from NCAR version 2.5 (FINNv2.5) uses fire counts detected as thermal anomalies, and the Global Fire Assimilation System version 1.2 (GFASv1.2) uses fire radiative power. All use similar landcover-specific, temporally static emission factors. The emissions from these inventories for the 2019 burning season are the same for NOx from GFEDv4s and FINNv2.5 (4.3 Tg as NO), peaking in July for GFEDv4s and August for FINNv2.5, and much less for GFASv1.2 (1.5 Tg), peaking in August. For NH3, emissions from GFEDv4s (0.68 Tg) and GFASv1.2 (0.52 Tg) are about half that from FINNv2.5 (1.3 Tg) and peak emission months are the same as NOx for GFEDv4s and FINNv2.5, but a month earlier (July) for GFASv1.2. Averaging kernels from the satellite products are used to mitigate influence of the vertical sensitivity of the instrument and a priori assumption of the vertical profile of NH3 when comparing to GEOS-Chem. We apply TROPOMI NO2 averaging kernels to GEOS-Chem for comparison to TROPOMI and re-retrieve IASI NH3 columns using GEOS-Chem as a priori. In our comparison to TROPOMI, GEOS-Chem monthly mean NO2 driven with GFASv1.2 and GFEDv4s is more spatially consistent (R ≥ 0.9) than FINNv2.5 (R = 0.4-0.6) and is typically just 12-27% less than TROPOMI using GFASv1.2, compared to up to 80% more for GFEDv4s and 55% more for FINNv2.5. The much greater NOx emissions from GFEDv4s and FINNv2.5 contribute to tropospheric ozone chemical production that totals 38-49 Tg in June-September compared to 29 Tg for GFASv1.2, though differences in volatile organic compound emissions will also influence these production rates. Assessment against IASI NH3 is underway.

How to cite: Marais, E., Clarisse, L., Van Damme, M., Wiedinmyer, C., and Murphy, K.: Burning season emissions of reactive nitrogen from fires in subtropical southern Africa determined with TROPOMI and IASI, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11419, https://doi.org/10.5194/egusphere-egu25-11419, 2025.

EGU25-12938 | ECS | Posters on site | AS3.27

Enhancing the flux divergence approach for accurate NOx emission estimation: An evaluation using high-resolution synthetic satellite data 

Felipe Cifuentes, Henk Eskes, Enrico Dammers, Charlotte Bryan, and Folkert Boersma

The Flux Divergence Approach (FDA) is a technique for deriving NOx emissions from satellite data. Here we will focus on NOx emissions derived from NO2 measured by the Sentinel-5P TROPOMI instrument. The FDA simplifies the complex three-dimensional transport and chemical processes in the atmosphere into a two-dimensional continuity equation for the column-integrated concentration. Emissions are thus calculated by combining spatial distribution patterns from satellite imagery with horizontal wind components that transport the column. Despite its widespread application, the accuracy of this method remains underexplored, primarily because of the limited availability of direct stack emission measurements. Additionally, comparisons with traditional bottom-up inventories provide only a general indication of its performance. In this study, we performed an end-to-end evaluation to assess the capability of the FDA to accurately reproduce known NOx emissions. A high-resolution model (LOTOS-EUROS) was used to generate synthetic, idealized satellite observations for the Netherlands. The FDA method was then applied to these observations, and the resulting emissions were compared with the input emissions used in the model. The results showed that the FDA reproduces the magnitude and spatial distribution of NOx emissions in the Netherlands with high accuracy (absolute bias <9 %). But such a good accuracy is only obtained if high-resolution model information is used as input in the FDA to account for critical factors, including the spatial variability of NO2 lifetime along pollution plumes (linked to OH concentration), the NOx:NO2 ratio, and the NO2 profile shape used for correcting satellite retrievals. These factors exhibit strong spatial and temporal variability on the kilometer scale. Interestingly, the FDA shows limited sensitivity to the specific wind field used, provided it accurately represents the flow within the planetary boundary layer (PBL). Moreover, restricting the analysis to observations within the PBL improves the accuracy of the estimated emissions. In its original form, the FDA generated detailed emission location maps, but it frequently led to notable biases in quantitative emission estimates. To improve accuracy, we therefore propose extending the FDA for NOx emissions from TROPOMI by incorporating additional information from a high-resolution CTM (2 km or better), which provides the necessary spatially and temporally varying inputs, including the replacement of the a-priori profile in the retrieval. Our results indicate that this enhanced FDA approach yields more reliable emission estimates. Although integrating a single high-resolution CTM run increases computational costs, it remains significantly faster than alternative methods, such as ensemble data assimilation or 4D-Var emission inversion systems, which require numerous model runs.

How to cite: Cifuentes, F., Eskes, H., Dammers, E., Bryan, C., and Boersma, F.: Enhancing the flux divergence approach for accurate NOx emission estimation: An evaluation using high-resolution synthetic satellite data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12938, https://doi.org/10.5194/egusphere-egu25-12938, 2025.

EGU25-13358 | ECS | Posters on site | AS3.27

Five years of satellite-based HCHO and NO2 monitoring over the Metropolitan Area of São Paulo, Brazil: insights from the BIOMASP+ project 

Arthur Freitas, Daniel Zacharias, Agnès Borbon, and Adalgiza Fornaro

Formaldehyde (HCHO) and nitrogen dioxide (NO2) are important precursors of tropospheric ozone through photochemical reactions. HCHO also acts as a marker for the oxidation of volatile organic compounds (VOCs). In the Metropolitan Area of São Paulo (MASP), these precursors are directly emitted by over 7 million vehicles, which burn a complex blend of ethanol and gasoline [1, 2, 3]. The present work analyzed vertical columns of HCHO and NO2 over MASP, using data retrieved from the TROPOMI sensor onboard the Sentinel-5P satellite. The analysis covered a five-year period from 2019 to 2023. A study region spanning ~6,500 km2 within the MASP was divided into 50 areas, each measuring 0.1° x 0.1° in latitude and longitude. This approach enabled the classification of the areas into distinct land-use types: 18 representing urban regions, 15 corresponding to green regions, and 17 covering transitional zones [4].

The three areas with the lowest and highest HCHO columns were two transition regions and one green region (minimum = 10.6 x 1015 molecules/cm2, extreme southwest), and three densely urbanized areas (maximum = 13.9 x 1015 molecules/cm2, central region), respectively. The three areas with the lowest and highest of NO2 columns were green regions (minimum = 2.5 x 1015 molecules/cm2, extreme southwest) and urban areas (maximum = 9.4 x 1015 molecules/cm2, central region), respectively. Both atmospheric constituents displayed higher column densities during the southern hemisphere winter (dry season).

The formaldehyde to nitrogen dioxide ratio (FNR) was calculated for each of the 50 areas, highlighting the São Paulo city center — particularly Marginal Tietê and Marginal Pinheiros — as a hotspot for ozone formation [5]. Despite its proximity to the urban center, the important Atlantic Forest (Reserve of Morro Grande) showed significantly lower concentrations of HCHO and NO2 compared to those recorded in the central areas. TROPOMI HCHO and NO2 data are proving essential for a better characterization of atmospheric chemical processes in the MASP, contributing to describe the formation of secondary pollutants, supporting the objectives of the BIOMASP+ project.

Keywords: Formaldehyde, Nitrogen Dioxide, Ozone, São Paulo megacity, TROPOMI

Acknowledgments: This work is funded and supported by BIOMASP+ Project (FAPESP 2020/07141-2) and Postgraduate Program in Meteorology (IAG-USP).

References

[1] Nogueira, T. et al., Atmosphere, 8(8), 144, 2017, https://doi.org/10.3390/atmos8080144

[2] Chiquetto, J. B. et al., Science of the Total Environment, 945, 2024, https://doi.org/10.1016/j.scitotenv.2024.173968

[3] CETESB, 2024, https://cetesb.sp.gov.br/ar/wp-content/uploads/sites/28/2024/08/Relatorio-de-Qualidade-do-Ar-no-Estado-de-Sao-Paulo-2023.pdf

[4] Pellegatti-Franco, D. M. et al., Urban Climate, 27, 293–313, 2019, https://doi.org/10.1016/j.uclim.2018.12.007

[5] Acdan, J. J. M. et al., Atmospheric Chemistry and Physics, 23(14), 7867–7885, 2023, https://doi.org/10.5194/acp-23-7867-2023

How to cite: Freitas, A., Zacharias, D., Borbon, A., and Fornaro, A.: Five years of satellite-based HCHO and NO2 monitoring over the Metropolitan Area of São Paulo, Brazil: insights from the BIOMASP+ project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13358, https://doi.org/10.5194/egusphere-egu25-13358, 2025.

Accurate, timely, and high-resolution NOx emissions are essential for formulating pollution control strategies and improving the accuracy of air quality modelling at fine scales. Since late 2018, the Tropospheric Monitoring Instrument (TROPOMI) aboard the Sentinel-5 Precursor (S5P) satellite has provided daily monitoring of NO2 column concentrations with global coverage and a small footprint of 5.5 km × 3.5 km, offering great potential for tracking daily high-resolution NOx emissions. In this study, we develop a data assimilation and emission inversion framework that couples an Ensemble Kalman Filter with the Community Multiscale Air Quality model (CMAQ), to estimate daily NOx emissions at 3-km scales in Beijing and surrounding areas in 2020. By assimilating the TROPOMI NO2 tropospheric vertical column densities (TVCDs) and taking the bottom-up inventory as prior emissions, we produce a posterior NOx emission dataset with a reasonable spatial distribution and daily variations at the 3-km scale. The proxy-based bottom-up emission mapping method at fine scales overestimates NOx emissions in densely populated urban areas, whereas our posterior emissions improve this mapping by reducing the overestimation of urban emissions and increasing emissions in rural areas. The posterior NOx emissions show considerable seasonal variations and provide more timely insight into NOx emission fluctuations, such as those caused by the COVID-19 lockdown measures. Evaluations using the TROPOMI NO2 column retrievals and ground-based observations demonstrate that the posterior emissions substantially improved the accuracy of 3-km CMAQ simulations of the NO2 TVCDs, as well as the daily surface NO2 and O3 concentrations in 2020. However, during the summer, despite notable improvements in surface NO2 and O3 simulations, positive biases in the posterior model simulations persist, indicating weaker constraints on surface emissions from satellite NO2 column retrievals in summer. The posterior daily emissions on the 3-km scale estimated by our inversion system not only provide insights into the fine-scale emission dynamic patterns but also improve air quality modelling on the kilometer scale.

How to cite: Kong, Y., Zheng, B., and Liu, Y.: Tracking daily NOx emissions from an urban agglomeration based on TROPOMI NO2 and a local ensemble transform Kalman filter, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14326, https://doi.org/10.5194/egusphere-egu25-14326, 2025.

EGU25-14388 | Orals | AS3.27

A New Era of Air Quality Monitoring from Space over North America with TEMPO: Early Years in Orbit 

Xiong Liu, Kelly Chance, Heesung Chong, John Davis, Jean Fitzmaurice, Gonzalo Gonzalez Abad, John Houck, Weizhen Hou, Caroline Nowlan, Junsung Park, Raid Suleiman, and Huiqun Wang and the TEMPO team

We present a status overview of the TEMPO mission including its operation, validation and status of baseline data products and upcoming algorithm improvements, implementation of Near-Real-Time (NRT) and other data products.

TEMPO is NASA’s first Earth Venture Instrument (EVI) selected in 2012, and the North America component of the geostationary air quality constellation along with GEMS (launched in Feb. 2020) over Asia and Sentinel-4 (to launch in 2025) over Europe. It is the first spaceborne instrument providing revolutionary hourly daytime air pollution over North America from Mexico City to the Canadian oil sands, and from the Atlantic to the Pacific, at neighborhood scale (~10 km2 at boresight). It uses UV/visible spectroscopy (293-493 nm, 538-741 nm) to measure key elements of tropospheric air pollution chemistry including O3, NO2, HCHO and aerosols, and capture the inherent high variability in the diurnal cycle of emissions and chemistry. TEMPO was successfully launched on board IS-40E into the geostationary orbit at 91°W in April 2023. It conducted its first light Earth observations in early August 2023, kicking off a new era of air quality monitoring from space over North America. It started its nominal operation in October 2023 for a 20-month of baseline Phase E. The baseline mission has been recently extended to September 2026, with further extension via NASA senior reviews. At night, TEMPO can observe city lights, gas flaring, maritime lights from fishing and offshore oil platforms, clouds and snow in the moonlight, lightning, aurorae, and nightglow without interfering with its primary daytime air quality/chemistry mission. Baseline V3 data products were released to the public in May 2024 from NASA’s Atmospheric Science Data Center (ASDC). These data products were upgraded from beta to provisional level in December 2024 after the validation team approval. TEMPO near-real-time (NRT) and other science quality data products were funded by NASA Satellite Needs Working Group (SNWG) to assist in air quality forecasting and modeling efforts and develop better pollution control strategies.

How to cite: Liu, X., Chance, K., Chong, H., Davis, J., Fitzmaurice, J., Gonzalez Abad, G., Houck, J., Hou, W., Nowlan, C., Park, J., Suleiman, R., and Wang, H. and the TEMPO team: A New Era of Air Quality Monitoring from Space over North America with TEMPO: Early Years in Orbit, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14388, https://doi.org/10.5194/egusphere-egu25-14388, 2025.

EGU25-15056 | Orals | AS3.27

Intercomparison of Geostationary Environment Monitoring Spectrometer (GEMS) observations during the ASIA-AQ Field Campaign 

Jhoon Kim, Rokjin Park, Ukkyo Jeong, Hanlim Lee, Jae-Hwan Kim, Sangseo Park, Myoung-Hwan Ahn, Limseok Chang, Won-Jin Lee, Hyunkee Hong, Yeon Jin Jung, Juseon Bak, Minseok Kim, Wook Kang, Yujin Chae, Yejun Seo, James Crawford, Scott Janz, Laura Judd, and Johnathan W. Hair

The Airborne and Satellite Investigation of Asian Air Quality (ASIA-AQ) campaign took place in February and March 2024 as part of a global initiative to collect detailed atmospheric data across various locations in Asia. This campaign utilized aircraft, satellites, and ground-based instruments to improve the understanding of winter air quality in the region. Since 2020, the Geostationary Environment Monitoring Spectrometer (GEMS) has been providing hourly observations of air quality in Asia for the first time.

During the ASIA-AQ campaign, GEMS data offered comprehensive observations of aerosols, ozone, NO₂, SO₂, HCHO, CHOCHO, and other pollutants over a wide area. These observations were compared with independent measurements from aircraft and ground-based instruments, including high spectral resolution lidar (HSRL), GEO-CAPE Airborne Simulator(GCAS), PANDORA, AERONET etc. This study highlights the intercomparison and evaluation of the GEMS dataset for various scenarios, such as urban pollution, biomass burning, emissions from power plants, and volcanic eruptions observed during the campaign.

How to cite: Kim, J., Park, R., Jeong, U., Lee, H., Kim, J.-H., Park, S., Ahn, M.-H., Chang, L., Lee, W.-J., Hong, H., Jung, Y. J., Bak, J., Kim, M., Kang, W., Chae, Y., Seo, Y., Crawford, J., Janz, S., Judd, L., and Hair, J. W.: Intercomparison of Geostationary Environment Monitoring Spectrometer (GEMS) observations during the ASIA-AQ Field Campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15056, https://doi.org/10.5194/egusphere-egu25-15056, 2025.

EGU25-16544 | ECS | Orals | AS3.27

Towards MTG-IRS retrieval of CO using IASI from the interferogram domain 

Nejla Eco, Sébastien Payan, and Laurence Croizé

Onboard of MetOp satellite series, Infrared Atmospheric Sounding Interferometer (IASI) is a Fourier Transform spectrometer based on the Michelson interferometer. IASI acquires interferograms from which high-resolution atmospheric emission spectra are provided, enabling the derivation of temperature and humidity profiles (among other parameters) with exceptional spectral resolution. In this study, we will use the IASI archive to evaluate a retrieval approach in the interferogram domain, which we anticipate will be well-suited for near-real-time (NRT) analysis of extensive spectral datasets expected from next-generation tropospheric sounders like MTG-IRS. The Partially Scanned Interferograms (PSI) method, applied to the retrieval of trace gases from IASI, has only rarely been studied. However, existing studies suggest its potential for specific gases, including CO, CO₂, CH₄, and N₂O, which could enable highly accurate trace gas column density retrievals at the resolution of a single IASI footprint.

We will present the interferogram retrieval approach of CO from IASI simulations. These results are based on the set of simulations of IASI interferograms for which the identified regions (optical path differences), sensitive to the carbon monoxide species, are noised and then used for retrievals. Furthermore, the study which aims to compare the performance of the interferogram retrieval approach compared to the conventional (i.e. from the spectral domain) will also be presented. The expected advantage compared to the usual methods is an efficient use of the information contained in all IASI channels that are available in the absorption bands of a specific gas species. Finally, using interferogram points sensitive to parameters of interest, we will also present a proof of concept of a neural network algorithm for classification of the interferograms predicting the surface temperature and the abundance of H2O and CO.

The simulation of IASI spectra was conducted using the LATMOS Atmospheric Retrieval Algorithm (LARA), a robust and validated radiative transfer model based on Least Squares estimation [Segonne et al., 2021]. The climatological library TIGR [Chédin et al., 1985; Chevallier et al., 1998] was used to generate IASI interferograms with LARA. TIGR comprises 2311 atmospheric scenarios, each characterized by temperature, water vapor, and ozone concentration values across a specified pressure grid from the surface to the top of the atmosphere. The study focuses on carbon monoxide, a key trace gas for understanding air quality and climate forcing. Carbon monoxide exhibits a characteristic “comb” absorption pattern within the 2050–2350 cm⁻¹ wavenumber range [Serio et al., 2012]. Simulations were performed for surface temperatures ranging from -15 to +15 K, in 5 K increments from the base temperature, to assess the impact of thermal contrast [Baudin et al., 2016]. Additionally, the study explores the potential of correlating interferogram characteristics with surface temperature and H₂O content, aiming to enhance the accuracy of CO column retrievals.

How to cite: Eco, N., Payan, S., and Croizé, L.: Towards MTG-IRS retrieval of CO using IASI from the interferogram domain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16544, https://doi.org/10.5194/egusphere-egu25-16544, 2025.

EGU25-16722 | Posters on site | AS3.27

Assimilation of SO2, CO, HCHO and O3 satellite data with Optimal Interpolation implemented in Atmospheric Modelling System MINNI 

Andrea Bolignano, Mario Adani, Gino Briganti, Felicita Russo, and Mihaela Mircea

SO2, CO, HCHO, NO2 and O3 satellite data measured by the TROPOspheric Monitoring Instrument (TROPOMI) instrument on board the Copernicus Sentinel-5 Precursor satellite launched in October 2017 provides a comprehensive atmospheric composition dataset at high horizontal resolution (5.5 km -7 km). Here, we used total column SO2, CO, HCHO and tropospheric O3 L2 products for testing Optimal Interpolation (OI) algorithm implemented in the atmospheric modelling system MINNI. The three-dimensional hourly concentrations fields produced with the chemical transport model FARM at European scale were adjusted with satellite retrievals of pollutants simultaneous and, separately, for O3. The three-dimensional optimal interpolation (OI) scheme developed for satellite data assimilation consider the spatial and temporal error structures of the background field through the background error covariance matrix (B). This matrix was estimated in the same way for all five pollutants and, for simplicity, was assumed diagonal considering thus that the retrievals at different points do not influence each other. Besides, model data were corrected only where the observations were available.

This simple OI scheme is computationally feasible but not effective in the same way for all pollutants. There are also differences in assimilating a single species or all together for those formed in the atmosphere such as O3. The differences in the three-dimensional modelled concentrations without and with assimilation for all pollutants and single species are discussed as well as their performances in comparison with ground observations for evaluating the impact of assimilation.

To understand the limitations of the implemented OI algorithm, several experiments were run to investigate the effects of using different definitions of B in different states of atmospheric composition. The comparisons and quantitative evaluations were performed both horizontally and vertically, analysing 2D fields and point time series.

The preliminary results show that the assimilation can improve modelled NO2 and capture SO2 volcano eruptions which are not present in anthropogenic emission inventories. However, the assimilation of the short-lived species like NO2, HCHO and O3 poses many problems, in particular due to their interdependencies, therefore more research is needed.

How to cite: Bolignano, A., Adani, M., Briganti, G., Russo, F., and Mircea, M.: Assimilation of SO2, CO, HCHO and O3 satellite data with Optimal Interpolation implemented in Atmospheric Modelling System MINNI, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16722, https://doi.org/10.5194/egusphere-egu25-16722, 2025.

EGU25-17035 | ECS | Orals | AS3.27

Contribution of Geostationary Satellites to the Observation of Atmospheric NH3 

Nadir Guendouz, Camille Viatte, Zhao-Cheng Zeng, Anne Boynard, Sarah Safieddine, Carsten Standfuss, Solène Turquety, Martin Van Damme, Lieven Clarisse, Pierre Coheur, Raymond Armante, Pascal Prunet, and Cathy Clerbaux

Ammonia (NH3) is an atmospheric pollutant mainly emitted by the agricultural sector, which has an effect on public health since it is a precursor of fine particles (PM2.5). The diurnal variability of NH3 in the atmosphere and its transformation into particles are poorly constrained and strongly depend on meteorological parameters, in particular temperature. Polar orbit satellite observations, such as the Infrared Atmospheric Sounder Instrument (IASI), are keys to assess spatio-temporal variabilities of NH3 with observations twice a day. Geostationary instruments offer a comprehensive assessment of NH3 diurnal variability and its dependence on atmospheric temperature.

 

This study analyses the contribution of geostationary instruments to observe ammonia variabilities and their link to atmospheric temperature. We use IASI observations, as well as the Geostationary Interferometric Infrared Sounder (GIIRS) on board China’s FengYun-4B satellite launched in June 2021 that measure atmospheric ammonia over East Asia and parts of South Asia and Southeast Asia every 2 hours at 12 km at nadir. We also evaluate the InfraRed Sounder (IRS) instrument that will be launched onboard the Meteosat Third Generation (MTG) satellite into geostationary orbit over Europe and Africa in late 2025. IRS will offer the ability to assess NH3 diurnal variabilities with frequent measurements (every 30-45 minutes) and better spatially resolved observations than IASI (4 km x 4 km at the Equator and Greenwich meridian).

 

In this work, GIIRS NH3 total columns are validated with IASI observations between July 2022 and June 2024. Then, the link between NH3 variabilities and atmospheric temperature are analyzed over Asia using GIIRS observations. Finally, a NH3 sensitivity analysis considering measurement noises is made for the future IRS-MTG mission and is discussed with respect to IASI. 

How to cite: Guendouz, N., Viatte, C., Zeng, Z.-C., Boynard, A., Safieddine, S., Standfuss, C., Turquety, S., Van Damme, M., Clarisse, L., Coheur, P., Armante, R., Prunet, P., and Clerbaux, C.: Contribution of Geostationary Satellites to the Observation of Atmospheric NH3, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17035, https://doi.org/10.5194/egusphere-egu25-17035, 2025.

EGU25-18728 | Posters on site | AS3.27

Temporal variability of NH3 in European hot spots based on satellite and in-situ observations 

Karol Przeździecki, Dipson Bhandari, Ainur Nagmarova, Jacek Kamiński, Aleksandra Starzomska, and Joanna Strużewska

Ammonia (NH₃) is primarily emitted from agricultural sources, including livestock farming and fertilizer application. Animal farms are significant contributors to ammonia emissions, particularly under low rainfall, as rainfall typically leads to nitrogen leaching and ammonia removal from the soil. In addition to agricultural activities, combustion-related NH₃ emissions, primarily from fossil fuel burning and biomass combustion, also contribute to atmospheric ammonia; however, these sources remain poorly understood. Ammonia emissions mainly arise from the volatilization of NH₃ from NH₄⁺-containing substrates, such as fertilized soils, animal waste, and nitrogen-polluted water, as well as from combustion-related processes, including coal combustion, vehicle exhaust, and biomass burning.

Ammonia significantly impacts air quality as a precursor to fine particulate matter (PM2.5), which has considerable health implications. A study by Vieno et al. (2016) (https://acp.copernicus.org/articles/23/15253/2023/)  demonstrated that reducing NH₃ emissions in the United Kingdom could lower PM2.5 levels. Despite this recognized impact, NH₃ monitoring networks are inconsistently implemented across Europe, with only a few countries, such as the Netherlands, the UK, and Belgium, maintaining dedicated NH₃ monitoring systems. Projections indicate that NH₃ emissions are likely to increase due to rising global temperatures and the growing demand for animal products, emphasizing the need for accurate, traceable, and routine NH₃ monitoring to better understand the complexities of ammonia in the atmosphere.

This study aims to identify NH₃ hot-spot regions in Europe based on satellite data from METOP IASI for 2019 to 2022 and compare these findings while accounting for surface variability and reported emission sources. Furthermore, we explore NH₃ CAMS profile analysis and NH₃ observations from the EBAS database of atmospheric measurements.

How to cite: Przeździecki, K., Bhandari, D., Nagmarova, A., Kamiński, J., Starzomska, A., and Strużewska, J.: Temporal variability of NH3 in European hot spots based on satellite and in-situ observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18728, https://doi.org/10.5194/egusphere-egu25-18728, 2025.

EGU25-19924 | ECS | Posters on site | AS3.27

Presenting a Concise OMI and TROPOMI NO2 Afternoon Data Record.  

Isidora Anglou, Folkert Boersma, Isolde Glissenaar, Pieter Rijsdijk, Tijl Verhoelst, Steven Compernolle, Herizo Narivelo, and Henk Eskes

Satellite instruments like OMI (2004) and TROPOMI (2018) have transformed global monitoring of tropospheric nitrogen dioxide (NO₂). Here we present a new Level 3 (L3) dataset produced within ESA’s CCI ECV project, created by averaging OMI and TROPOMI NO₂ columns spatially and temporally. This compact, user-friendly dataset is suitable for trend analysis, emission estimation, and climate modeling validation. It includes OMI (2004-2021) and TROPOMI (2018-2021) NO₂ data, uncertainty estimates, and additional variables like the averaging kernel, which informs vertical sensitivity to NO₂. The data set can be found at : https://www.temis.nl/airpollution/no2col/cci-no2-omi.php & https://www.temis.nl/airpollution/no2col/cci-no2-tropomi.php

The L3 dataset consists of OMI and TROPOMI NO2 measurements spatially and temporally averaged in a consistent manner and includes full L3 uncertainty estimates. The uncertainty propagation includes measurement related uncertainties (from L2) as well as a spatial and a temporal representativity component. The data include additional spatiotemporally averaged variables, such as the averaging kernel, which provides relevant information on the vertical sensitivity to NO2. The L3 data have been produced in different resolutions ranging from 0.2 to 2 degrees and have been used for GEOS-Chem model evaluation. We show that the relative L3 uncertainties fall within the 15-20% range in polluted regions, lower than uncertainties in separate level 2 orbit retrievals, and brings tropospheric NO2 columns to within the GCOS ‘goal’ and ‘breakthrough’ requirements. Validation of the L3 against independent MAX-DOAS and PANDORA NO2 columns shows consistency up to 20%.

Our aim is to make the L3 dataset as consistent as possible, by minimizing sensor-related differences to obtain a clearer view of NO2 changes over time. While OMI and TROPOMI have similar retrieval algorithms, there is a 15-minute difference in overpass time, the algorithms use different cloud algorithms, and OMI suffers from the ‘row anomaly’ phenomenon that causes a decrease in spatial coverage and hence sampling differences with TROPOMI. We show that by co-sampling (in space and time) OMI and TROPOMI NO2 columns, the consistency between the datasets improves. For example, for Beijing the relative absolute difference of OMI and TROPOMI for winter months in 2019 and 2020 is 14% and 22% drops to 8% and 11% when co-sampling. Furthermore, the row anomaly phenomenon causes reduced coverage in OMI from 2007 onward. We show how long-term trends in tropospheric NO2 columns are affected by the row anomaly and present a recipe to avoid such spurious trends.

How to cite: Anglou, I., Boersma, F., Glissenaar, I., Rijsdijk, P., Verhoelst, T., Compernolle, S., Narivelo, H., and Eskes, H.: Presenting a Concise OMI and TROPOMI NO2 Afternoon Data Record. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19924, https://doi.org/10.5194/egusphere-egu25-19924, 2025.

EGU25-20332 | Orals | AS3.27 | Highlight

Air Quality on the Neighborhood Scale: All Means Necessary 

Russell Dickerson, Tad Aburn, Matthew Aubourg, Joel Dressen, Timothy Canty, Hao He, Zhanqing Li, Tiberius Okanga, Xinrong Ren, Akanskha Singh, Phillip Stratton, and Jing Wei

Effective measures to improve air quality and optimize health benefits require teamwork to scale from satellite observations with broad coverage and surface-based measurements with research-grade instruments and local arrays of low-cost sensors.  Results must be evaluated with models and communicated to regulatory agencies for corrective action.  The bulk of the most vulnerable communities lack monitors and satellites can help fill in the gaps.  Historically these efforts have been carried out by scientists but historically the worst air quality has been in disadvantaged communities with inadequate monitoring and justifiably distrustful of government agencies.  Communities must be encouraged to express their concerns and empowered to seek mitigation action.  A neighborhood in Baltimore has long complained of coal dust but suffers from myriad air pollution problems – a legacy of residential communities surrounded by industry and heavy traffic.  A community in suburban Washington has formed an effective environmental justice action team to measure, display, and report AQ problems.  Success includes improved enforcement of regulations on pollution sources and a $147M grant to replace diesel with electric vehicles around the Port of Baltimore.  Unfortunately, these are just two of dozens of afflicted communities in the area.  We report on successes and challenges and how these efforts might be generalized and scaled up. 

How to cite: Dickerson, R., Aburn, T., Aubourg, M., Dressen, J., Canty, T., He, H., Li, Z., Okanga, T., Ren, X., Singh, A., Stratton, P., and Wei, J.: Air Quality on the Neighborhood Scale: All Means Necessary, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20332, https://doi.org/10.5194/egusphere-egu25-20332, 2025.

EGU25-20500 | Posters on site | AS3.27

Validation of all S5P ozone products (total columns, tropospheric columns and profiles) with a single reference network.  

Corinne Vigouroux, Bavo Langerock, and Martine De Mazière and the FTIR observation Team

Ground-based Fourier Transform Infrared (FTIR) instruments from the Network for the Detection of Atmospheric Composition Change (NDACC) provide long-term and continuous measurements of many atmospheric trace gases at more that 20 stations. This network is already used in the S5P validation of CO and CH4 (Sha et al., 2021) as well as HCHO (Vigouroux et al., 2020), and NO2 (validation reports https://mpc-vdaf.tropomi.eu/).

Ozone is one of the major FTIR NDACC target gas and its retrieval strategy is harmonized within the network (Vigouroux et al. 2015). Nonetheless, while ozone data from FTIR measurements are contributing to many ozone trend studies (e.g. Vigouroux et al., 2015, Godin-Beekman, et al., 2022, Van Malderen et al. ,2025), they have been poorly used for satellite validation. The reasons are partly historical (Brewen/Dobson are traditionally used for total column validation) and partly scientific (FTIR has low vertical resolution so the ozone sondes and lidars are preferred for profile validation of Limb satellites).

However, the ground-based FTIR ozone products are well suited for the validation of Nadir sounding satellites such as S5P: FTIR retrievals provide both ozone total column with a high precision better than 2% and ozone profiles with low vertical resolution (approximately 4 degrees of freedom for signal - DOFS), which is similar to the S5P ozone profile products (about 5 DOFS). The strength of FTIR data compared to ozone sondes measurements is that they have sensitivity up to about 45 km, allowing the validation of S5P profiles above the 30 km limit reached by the sondes. These higher altitudes can be reached by Lidar data, but the stations equipped with such instruments are sparse and therefore provide lower representativeness of the validation. In addition, FTIR has also a good sensitivity in the troposphere (1 DOFS) which allows for the validation of the specific S5P tropospheric column product as well, although only 3 FTIR stations are located within the 20°S – 20°N band for which the S5P ozone tropospheric product is provided.

We will show validation results for the three different S5P products: total columns,  tropospheric columns, and profiles. The profile validation will be made by comparing ozone from both instruments in 4 vertical layers following the FTIR averaging kernels and DOFS. The effect of the different a priori information and vertical sensitivities of both S5P and FTIR will be investigated. Our results (accuracy and precision of the S5P ozone products) will be put in perspective with the past S5P ozone validation studies (Garane et al., 2019; Hubert et al., 2021, Keppens et al., 2024).

This validation exercise is the first step towards the future use of FTIR for the validation of geostationary satellites such as S4/S5 (ESA project CHEOPS S4/5) or TEMPO. One of the major advantage of this reference network is to enable the evaluation of the ozone diurnal cycle, as FTIR acquisitions are made throughout the day in clear sky conditions.

 

How to cite: Vigouroux, C., Langerock, B., and De Mazière, M. and the FTIR observation Team: Validation of all S5P ozone products (total columns, tropospheric columns and profiles) with a single reference network. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20500, https://doi.org/10.5194/egusphere-egu25-20500, 2025.

In this work we are aiming at unification of information about spatial behavior of long-term average concentration of selected air pollutants coming from both measurement and numerical modeling on a large spatial scale. Statistical model that we develop is of inherently Bayesian nature and reflects both detailed spatial features (background and urban increment Markov random fields) and calibration of numerical model outputs (CAMx and Symos model outputs coming as covariates in the comprehensive model). We fit the model in a computationally highly effective way based on INLA (Integrated Nested Laplace Approximation). While such a model is of independent interest for spatial interpolation allowing for both details (such as effects of major highways) and good calibration against empirical data, we will focus on its use for design problems related to the measurement network. Statistical design principle that we develop is derived from the model consequences in a fully formalized, probabilistic way. Namely, our design approach is of mini-max type (minimizing maximum interpolation standard error over a grid covering area of interest with respect to placement of measurement points). Due to the construction of our Bayesian model, the design accounts for both regression (non-empirical, related to numerical modeling) and spatial interpolation (empirical, measurement related spatially autocorrelated field) parts and reflects various types of uncertainties that are typically overlooked. Since we have access to the posterior distribution of the comprehensive statistical model structural parameters, we can reflect uncertainty in their estimates and assess the effects it has upon the selection of measurement design points. Using our stepwise design point selection algorithm, we will illustrate several tasks of different complexity related to the network design: reduction (omitting pre-specified number of stations), improvement (moving existing stations to improve overall network performance) and expansion (adding more stations to the network). At the same time, we will discuss the role of various logistically and theoretically motivated measurement location placement restrictions and show how they influence the resulting network performance. Deployment of our statistical model and measurement network design selection algorithm will be illustrated on country-wide scale in the Czech Republic. The work has been done in cooperation with the Czech Hydrometeorological Institute and is related to the Technology Agency Czech Republic project ARAMIS, SS02030031). 

How to cite: Brabec, M.: Spatial air pollution modeling generating design of measurement network, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-142, https://doi.org/10.5194/egusphere-egu25-142, 2025.

Benzo[α] pyrene (BaP), a polycyclic aromatic hydrocarbon (PAHs), is a ubiquitous environmental contaminant. Since 1998, PAHs have been listed in the Convention on Long-Range Transboundary Air Pollution (CLRTAP) Protocol on Persistent Organic Pollutants. This pollutant is of great public concern because of its toxicity and potential carcinogenicity. Emissions of BaP occurred as early in 1970s, increased till 1990, then decreased before spiking again from 2000 onwards. This shift in emissions from developed to developing countries is largely attributed due to shifting of BaP emitting industries, with China and India being the largest emitters of PAHs. In light of environmental significance, it is important to know the emission scenario of BaP. Results indicated that Asia has the highest regional emissions (1.73 х 108 kg), while Australia (1.03 х 106 kg) has the lowest. In the present study, have used the BETR-Global model to understand the BaP scenario at global scale. Here, we will highlight the long-term trends (1970 – 2018) of BaP transboundary seasonal depositions and seasonal inflows across Asia, Europe, Africa, North America, South America, Australia, Arctic and, Antarctica. This research underscores the importance of understanding the shifting dynamics of BaP emissions for effective environmental management and policy development.

How to cite: Yadav, P. and Qureshi, A.: Source attribution of seasonal continental deposition and trans-continental fluxes of benzo [α] pyrene, 1970-2018, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-998, https://doi.org/10.5194/egusphere-egu25-998, 2025.

EGU25-2279 | Posters on site | AS3.28

100-Meter High-Resolution Modeling and Validation of PM and NO2 Concentrations in Urban Areas of South Korea 

Hui-Young Yun, Kyung-Hui Wang, Min-Woo Jung, Seung-Hee Han, Ju-Yong Lee, Kwon Jang, and Dae-Ryun Choi

  Fine particulate matter (PM) and nitrogen dioxide (NO2) are major air pollutants that significantly contribute to health risks, including cardiovascular and respiratory diseases. This study develops and validates 100-meter resolution air pollution data for South Korean cities, focusing on PM and NO2 concentrations. A hybrid modeling approach combining the Chemical Transport Model (CMAQ) and the Dispersion Model (CALPUFF) was employed to estimate the spatiotemporal distribution of these pollutants in major metropolitan areas, including Seoul, Busan, and Incheon.

  The CMAQ model generated baseline data at typical resolutions of 9 km and 1 km grids, which were further refined using the CALPUFF model to produce high-resolution 100 m datasets. The hybrid modeling approach integrated primary pollutant concentrations from CMAQ with CALPUFF's precise dispersion modeling to accurately reflect localized pollutant variations critical for urban health assessments. The resulting 100 m resolution data were validated by comparing them with roadside air quality monitoring measurements, demonstrating high correlation and ensuring temporal and spatial reliability.

  This study overcomes the limitations of traditional 1 km and 9 km resolution datasets and presents a novel approach for analyzing fine-scale pollutant distributions in urban environments. The methodology is applicable to other regions globally, particularly those facing severe air pollution challenges, and serves as a foundational tool for urban air quality improvement efforts. The generated data will facilitate research on the relationship between air pollution exposure and health outcomes and support the development of targeted air quality management policies. Future work will focus on integrating real-time air quality monitoring data to improve model accuracy and support the implementation of evidence-based air quality management policies.

 

Acknowledgement

  This research was supported by the Korea National Institute of Health (KNIH) research project (Project No. 2024-ER0606-00) and the Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute (KEITI), funded by the Ministry of Environment (MOE).

 

How to cite: Yun, H.-Y., Wang, K.-H., Jung, M.-W., Han, S.-H., Lee, J.-Y., Jang, K., and Choi, D.-R.: 100-Meter High-Resolution Modeling and Validation of PM and NO2 Concentrations in Urban Areas of South Korea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2279, https://doi.org/10.5194/egusphere-egu25-2279, 2025.

EGU25-2307 | ECS | Posters on site | AS3.28

Application of a Super-Resolution Algorithm to Improve the Spatial Resolution of Air Pollutant Concentrations in the Seoul Area 

Kyung-Hui Wang, Min-Woo Jung, Seung-Hee Han, Ju-Yong Lee, Kwon Jang, Dae-Ryun Choi, and Hui-Young Yun

Air pollution not only poses harmful effects on human health but also causes various diseases, leading to severe issues such as increased premature mortality. To accurately assess the health impacts and exposure levels of air pollution, high-resolution spatiotemporal concentration data is essential.

In previous studies, Hybrid Modeling combining CMAQ and CALPUFF was applied to estimate air pollutant concentrations at a spatial resolution of 100m. However, the Hybrid Model has limitations in that each modeling process must be conducted independently, requiring significant time and computational resources.

This study aims to improve computational efficiency and simplify the modeling process by applying a Super-Resolution Convolutional Neural Network  (SRCNN) algorithm. SRCNN uses low-resolution (9km) CMAQ data as input to produce spatial distributions similar to those generated by the Hybrid Model at a high resolution of 100m. The target pollutant is PM2.5 and NO2 in Seoul, with a training period from 2015 to 2021 and a test period in 2022. 

Model evaluation results show that SRCNN outperformed CMAQ in terms of PSNR, SSIM, and Spatial RMSE metrics. This demonstrates the potential of  SRCNN to efficiently generate high-resolution air pollution concentration data, contributing to more precise exposure assessments and health impact analyses.

  

Acknowledgement

This research was supported by the Korea National Institute of Health (KNIH) research project (Project No.2024-ER0606-00) and Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute (KEITI) funded by the Ministry of Environment (MOE) 

How to cite: Wang, K.-H., Jung, M.-W., Han, S.-H., Lee, J.-Y., Jang, K., Choi, D.-R., and Yun, H.-Y.: Application of a Super-Resolution Algorithm to Improve the Spatial Resolution of Air Pollutant Concentrations in the Seoul Area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2307, https://doi.org/10.5194/egusphere-egu25-2307, 2025.

Air pollution in Eastern and Southern Africa (E&SA) presents a severe public health concern, contributing to over 23,000 premature deaths annually and exacerbating respiratory ailments for millions. Despite this, air quality forecasting remains challenging due to sparse observational infrastructure. To address these challenges, we are developing an advanced air quality forecasting framework using the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) and its associated data assimilation system (WRF-DA). Our approach incorporates VIIRS aerosol optical depth (AOD) assimilation, with background error statistics derived through the community Gridpoint Statistical Interpolation (GSI). Meteorological inputs are sourced from the Global Forecast System (GFS), while monthly anthropogenic emissions from CAMS and real-time fire emissions from the Fire Inventory from NCAR (FINN) enhance our 48-hour forecasts at 15 km resolution. The forecasts are demonstrated for a case study in June 2022, capturing wildfires, dust storms, and local anthropogenic emissions. We used an updated AOD error estimate using AERONET stations and evaluate the forecast capabilities by comparing the base and assimilation runs against AirNow PM2.5 observations and AERONET observations. Additionally, we assess the impact of observation covariance and background error on the assimilated forecasts and provide insights into pollution source attribution. This work discusses the improvements for operational air quality forecast in data-sparse regions like E&SA.

How to cite: Bahramvash Shams, S., Kumar, R., and Weeks, V.: Error Assessment of Air Quality Forecasting through Chemical Data Assimilation over Southern and Eastern Africa: Characterizing Background and Observation Covariance Errors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2617, https://doi.org/10.5194/egusphere-egu25-2617, 2025.

EGU25-2692 | ECS | Posters on site | AS3.28

The application study of the revised IMPROVE atmospheric extinction algorithm in atmospheric chemistry model focusing on improving low visibility prediction in eastern China 

Chen Han, Hong Wang, Yue Peng, Zhaodong Liu, Wenjie Zhang, Yang Zhao, Huiqiong Ning, Ping Wang, and Huizheng Che

Abstract. Low visibility event, as a disastrous weather, has great impacts on traffic and transportation, aircraft, and people’s daily life, etc. Timely and accurate forecasts of low visibility events are urgently needed and meaningful. The reasonable algorithm of atmospheric extinction in atmospheric chemistry models is the basis for quantitatively predicting low visibility. The revised IMPROVE algorithm (RIMP) of atmospheric extinction is incorporated into the chemistry-weather interacted model GRAPES_Meso5.1/CUACE CW V1 to improve the prediction of low visibility events (LVEs) in the urban agglomerations in eastern China, which is compared with the original IMPROVE algorithm (OIMP) used in this model. The study results show that the RIMP effectively reduces the overestimation of low visibility prediction by OIMP in general, leading to a decrease of root-mean-square errors (RMSEs) and an increase of Threat Score (TS) of visibility less than 3 km, 5 km, and 10 km overall both at regional and city scales in varying degrees due to its more detailed processing of aerosols’ size, optical feature and hygroscopic growth; The improvements of visibility prediction of LVEs by RIMP depends on the combined contribution of high relative humidity (RH)  and PM2.5 instead of single high RH or PM2.5. The relative contributions of RH and PM2.5 concentration on different levels of low visibility are different in Beijing-Tianjin-Hebei (BTH) and Yangtze River Delta (YRD) regions due to their different RH and PM2.5, which leads to the different improvement of RIMP in the two regions. The larger improvements by RIMP occur for visibility less than 5 km in BTH, while in YRD, the larger improvements by RIMP occur for visibility less than 10 km and greater than 5 km. Moreover, the improvements by RIMP were more evident with higher RH conditions in both regions. The uncertainty created by the extinction algorithm is one important factor of the multiple factors affecting LVEs prediction; accurate modeling of high RH near saturation is also very important for LVEs prediction.

How to cite: Han, C., Wang, H., Peng, Y., Liu, Z., Zhang, W., Zhao, Y., Ning, H., Wang, P., and Che, H.: The application study of the revised IMPROVE atmospheric extinction algorithm in atmospheric chemistry model focusing on improving low visibility prediction in eastern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2692, https://doi.org/10.5194/egusphere-egu25-2692, 2025.

A coupled film-intraparticle pore diffusion model was derived to explain the deviations between measured apparent bulk particle/gas distribution coefficients (Log𝐾𝑝𝑔,𝑏,𝑎) and equilibrium values (Log𝐾𝑝𝑔,𝑏) predicted either from octanol-air distribution coefficients (𝐾𝑜𝑎) or subcooled liquid vapor pressures (PLo) of PAHs. The coupled model accounts for both external mass transfer resistance in the bulk air and internal resistance within the intraparticle pore space. For low molecular weight compounds (with small Log𝐾𝑝𝑔,𝑏), mass transfer is dominated by intraparticle pore diffusion, following the square root of time law and the apparent distribution coefficients increase or decrease with the square root of 𝐾𝑜𝑎 or PLo. In contrast, for high molecular weight compounds, external film diffusion becomes the limiting factor, resulting in observed distribution coefficients that appear independent of 𝐾𝑜𝑎 or PLo (slope = 0). Moderate molecular weight compounds fall in between, with the slope transitioning from 1/2 to 0, requiring consideration of both external and internal resistances. The coupled model is strongly influenced by parameters such as intraparticle porosity, airborne particle concentration, grain size, and the contact time between airborne particles and ambient air. High Log𝐾𝑝𝑔,𝑏,𝑎 values are associated with fast kinetics, which are enhanced by increased intraparticle porosity, higher airborne particle concentration, smaller particle size, or prolonged contact time (aged particles). The model was validated using three datasets with varying contact times from recent publications. Results for Log𝐾𝑝𝑔,𝑏,𝑎 derived from local sources, such as oil combustion tests in the lab and urban data, were well explained by the sorption model. However, data from polar regions required a desorption model with unexpectedly slow solid diffusion rates (𝐷𝑠 = 10−18.5 m2 s−1). This finding suggests that the properties of aged particles, such as viscosity, change during long-distance transport, leading to more complex mass transfer processes in the remote areas.

How to cite: Liu, B., Finkel, M., and Grathwohl, P.: Modeling of particle/gas distribution kinetics of polycyclic aromatic hydrocarbons(PAHs) in the atmosphere: Relevance of mass transfer resistance shifts , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2776, https://doi.org/10.5194/egusphere-egu25-2776, 2025.

EGU25-3013 | ECS | Posters on site | AS3.28

An Application of Deep Learning in the Zhuoshui River Basin for Multi-Station PM10 Forecast  

Pu Yun Kow, Fi-John Chang, Chia-Yu Hsu, Wei Sun, and Yun-Ting Wang

Air pollution, particularly particulate matter (PM10), presents a critical environmental and public health challenge, with the Zhuoshui River Basin in Taiwan being a severely affected region. One-day-ahead multi-station PM10 forecasting is essential for effective air pollution management. In this study, we propose a deep learning architecture that integrates 3D image datasets and time series data, enabling the extraction of key information from heterogeneous inputs. The model significantly enhances forecasting accuracy compared to benchmarks, achieving R² improvements of 15–70% and RMSE reductions of 6–25%.

Regional PM10 forecasting is crucial for protecting public health, as PM10 exposure is linked to severe respiratory and cardiovascular risks and exacerbation of pre-existing conditions. Accurate forecasts enable authorities to issue timely warnings, implement mitigation measures, and allocate resources efficiently. Seasonal PM10 forecasting is equally important, as air quality exhibits significant seasonal variations driven by meteorological and environmental factors. Our analysis reveals that the proposed model performs best during summer, achieving the smallest R² and largest RMSE improvements, while performance decreases in winter due to adverse conditions like temperature inversions and stagnant air masses.

These seasonal insights are critical for developing targeted strategies, such as stricter emission controls and public health advisories during winter months when PM10 levels are highest. Moreover, accurate seasonal forecasts provide essential guidance for long-term urban and regional planning, including green infrastructure placement, enhancement of public transportation policies, and development of resilient air quality management systems. By integrating advanced deep learning models into air quality management frameworks, this research contributes to protecting public health and fostering sustainable development in the Zhuoshui River Basin.

How to cite: Kow, P. Y., Chang, F.-J., Hsu, C.-Y., Sun, W., and Wang, Y.-T.: An Application of Deep Learning in the Zhuoshui River Basin for Multi-Station PM10 Forecast , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3013, https://doi.org/10.5194/egusphere-egu25-3013, 2025.

The rapid decline in air quality across Southeast and Western Pacific Asia is occurring at an accelerated pace due to population growth and industrial development. The region’s Meteorological factors, including the monsoon seasonality, exert a significant influence on air pollution levels, particularly PM2.5 concentrations. In this study, we employ a statistical modeling approach to derive daily PM2.5 levels from meteorological parameters in five major polluted cities: Lahore (Pakistan), Delhi (India), Dhaka (Bangladesh), Hanoi (Vietnam), and Shanghai (China). The incorporated meteorological parameters are wind speed, barometric pressure, temperature, and rainfall, which are known to affect air pollution levels from 2020 to 2022. The statistical modeling was based on the comparative analysis of 35 different machine learning (ML) regression techniques with the purpose of selecting the algorithms most efficient for reconstructing and predicting PM2.5 levels from meteorological variables alone. Specifically, each ML regression model was trained to reconstruct daily PM2.5 levels in 2020–2021, and then used to reconstruct both missing daily PM2.5 levels in 2020–2021 and forecast the whole of 2022 using only the 2022 meteorological records. The results indicated that most of the daily and seasonal variability in daily PM2.5 levels could be reconstructed from meteorological conditions. However, the performance of the various ML models (as assessed by Root Mean Square Error tests) exhibited considerable variability. Among the tested models, the Ensembles Boosted Tree ML method demonstrated optimal efficiency during the training period (the first 2 years, 2020 and 2021) and it also was highly efficient in predicting the third year (2022) using only meteorological data. Additionaly, the Trilayer Neural Network ML method was found the most effective at reconstructing the data after 3 years of training and may therefore be preferred to fill in short periods of missing PM2.5 data. In contrast, our comparative analyses showed that the traditional multi-linear regression models under-performed in both constructing and predicting PM2.5 data. This study demonstrates the necessity and usefulness of assessing multiple ML regression methodologies for selecting which ones better perform for reconstructing the data of interest (in our case PM2.5 records) from their hypothesized constructors (in our case meteorological parameters). In particular, this study has highlighted the utility of using ML regression techniques for forecasting air quality and reconstructing missing pollution data, which is crucial for policy-making across South-East and Western-Pacific Asia regions, where only limited pollution monitoring infrastructure are available.

How to cite: Shafi, S. and Scafetta, N.: Optimal machine learning techniques for meteorological modeling of PM2.5 concentration in five major polluted cities of South-East Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3240, https://doi.org/10.5194/egusphere-egu25-3240, 2025.

Secondary air pollution, especially ozone (O3) and secondary aerosols, are emerging air quality challenges confronting China. Nitrous acid (HONO), as the predominant source of hydroxyl radicals (OH), are acknowledged to be essential for secondary pollution. However, HONO concentrations are usually underestimated by current air quality models due to the inadequate representations of its sources. In the present study, we revised the Weather Research and Forecasting & Chemistry (WRF-Chem) model by incorporating additional HONO sources, including primary emissions, photo-/dark oxidation of NOx, heterogeneous uptake of NO2 on surfaces, and nitrate photolysis. By combining in-situ measurements in the Yangtze River Delta (YRD) region, we found the improved model show much better performance on HONO simulation and is capable of reproducing observed high concentrations. The source-oriented method is employed to quantitatively understand the relative importance of various processes, which showed that heterogeneous NO2 uptake on the ground surface was the major contributor to HONO formation in urban areas. Comparatively, photo-oxidation of NOx is a main contributor in rural areas. The introduction of multiple sources of HONO led to an apparent increase in OH and hydroperoxyl (HO2) radicals. The promoted HO2 levels further increased diurnal O3 concentration by 4.5–12.9 ppb, while secondary inorganic and organic concentrations were also increased by 14–32% during a typical secondary pollution event. The improved description of HONO emission and formation in the model substantially narrowed the gaps between simulations and observations, highlighting the great importance in understanding and numerical representations of HONO in secondary pollution study.

How to cite: Zhang, H. and Huang, X.: Improving HONO Simulations and Evaluating its Impacts on Secondary Pollution in the Yangtze River Delta Region, China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3372, https://doi.org/10.5194/egusphere-egu25-3372, 2025.

EGU25-5155 | Posters on site | AS3.28

A modeling study for assessment of air quality across European countries 

Efthimios Tagaris, Nektaria Traka, Ioannis Stergiou, Dimitris G Kaskaoutis, and Rafaella Eleni P Sotiropoulou

Air pollution remains a significant environmental challenge, with adverse effects on human health, ecosystems, and climate. Accurate modeling of pollutant concentrations is essential for developing effective mitigation strategies and informing policy decisions. As such, the aim of the study is to simulate the concentrations of gaseous and particulate pollutants across Europe assessing the discrepancies between observed and predicted values for various countries. The Community Multiscale Air Quality (CMAQ) v.5.3 Modeling System is used to estimate air quality for 2019, employing a 20 km × 20 km grid resolution for the whole Europe. Anthropogenic emission data from the European Monitoring and Evaluation Programme (EMEP) for 2019 at a resolution of 0.1 × 0.1 degrees have been used. The available data include emissions for CO, NH3, NMVOC, NOx, PM10, PM2.5 and SOx classified into 13 categories, depending on the source of origin. These emissions were processed using the Sparse Matrix Operator Kernel Emissions (SMOKE) system to align with the air quality model’s requirements. Biogenic emissions were integrated using the Biogenic Emission Inventory System (BEIS), supported by land use data at 1 km resolution from the United States Geological Survey (USGS). In addition, the meteorological fields are derived using The Weather Research and Forecasting (WRF) Model. The simulation results show satisfactory predictions for O3, PM2.5, NO2 and SO2 concentrations, while identifying regions with the most pronounced deviations from observed values.

How to cite: Tagaris, E., Traka, N., Stergiou, I., Kaskaoutis, D. G., and Sotiropoulou, R. E. P.: A modeling study for assessment of air quality across European countries, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5155, https://doi.org/10.5194/egusphere-egu25-5155, 2025.

EGU25-5628 | ECS | Orals | AS3.28

Emulating tropospheric chemistry with physics-informed machine learning 

Alessio Melli, Camille Mouchel-Vallon, Hervé Petetin, and Oriol Jorba Casellas

Massive computing resources are nowadays required by current chemical transport models (CTMs) operating at global and/or regional scale to solve the system of ordinary differential equations associated with chemical kinetics. The sheer complexity of our atmosphere (in terms of the number of different constituents and reactions) together with the orders of magnitude differing between the chemical and the transport time scales, hinder the use of comprehensive mechanisms in large-scale 3D models. The rapid advancements in the field of machine learning (ML), alongside with the latest improvements in parallel computing, supplied new and powerful tools to the equipment of present-day atmospheric modelers. A notable example is given by physics-informed ML, where specialized network architectures are designed to satisfy the physical constraints of the system under investigation, leading to promising results in the emulation of physical processes. Indeed, physics may be introduced in the ML architecture at different stages, therefore determining the type of constraint (hard vs soft) embedded into the model. 

In this work, the baseline performance is defined on a fully-connected multilayer perceptron (fc-MLP) trained to predict the concentration change using the composition vector at a given time as input. The dataset is generated using Sobol sampling of different initial conditions within a specified concentration range to ensure comprehensive and efficient coverage of the input space. As a first attempt of including physics in the model architecture, we introduce the mech-MLP model, obtained by exploiting an array of MLPs—one per each chemical reaction present in the mechanism—whose outputs (i.e., the change in composition) are aggregated together to determine the total change to each chemical species. Furthermore, chemical and physical soft constraints are introduced also via the use of custom loss functions by imposing penalty terms for un-physical predictions (e.g., negative concentration or divergence from stoichiometry). The trade-off between dataset size, creation cost, and training efficiency, the inductive biases arising from the architecture choice, and the reliability of the model when tested on unseen conditions will be presented for two study cases: an explanatory mechanism involving 3 species and 2 reactions, and a simple, stiff air pollution mechanism (POLLU, doi.org/10.1137/0915076) composed by 20 species and 25 reactions.

How to cite: Melli, A., Mouchel-Vallon, C., Petetin, H., and Jorba Casellas, O.: Emulating tropospheric chemistry with physics-informed machine learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5628, https://doi.org/10.5194/egusphere-egu25-5628, 2025.

EGU25-6582 | ECS | Orals | AS3.28

Gaseous Pollutants Driven Ozone Variability 

Samrat Santra

Ground-level ozone (O3) is a secondary air pollutant and one of the major air pollutants that shape the atmospheric chemistry and influence many chemical reactions in the atmosphere. O3 is the second most significant air pollutant after particulate matter contributing mortality world-wide. To explore the O3 (a criteria pollutant) concentration variability influenced by primary air pollutants, especially criteria air pollutants such as volatile organic compounds (VOC), carbon monoxide (CO), nitrogen dioxide (NO2), and sulfur dioxide (SO2), we conducted a field campaign at Kharagpur city in India on April 2024. Sample air was measured by the USEPA approved Serinus 10 ozone analyser, Serinus 40 NOx analyser, Serius 500 Portable Air Quality Monitor (with swappable sensor heads) to get O3, NOx (NO+NO2), total VOC (TVOC), CO, and SO2 concentrations, respectively. The measurement was carried out on National Highway 49 (NH-49) (22.379128°N, 87.361647°E) in Kharagpur. Results showed a strong negative correlation between O3 and NO (r = -0.82), a weak positive correlation with NO2 (r = 0.19), moderate negative correlations with TVOC (r = -0.54) and CO (r = -0.49), and a very weak positive correlation with SO2 (r = 0.11). All correlations are statistically significant at the p < 0.01 level. We applied Quantile Regression Model (QRM) to explore a robust framework for analyzing the relationships between dependent (O3) and independent variables (NO, NO2, TVOC, CO, SO2) across different points of the data distribution by capturing conditional quantiles. Analysis revealed nonlinear distribution of O3 concentration across all the quantiles (τ) with a strong performance at the median quantile (τ = 0.5) that explained 76.06% of variability in O3 concentration (R1(τ)0.5) = 0.7606) with high accuracy and low predicting errors (MAE = 14.19, RMSE = 17.86). The local measure of goodness of fit, R1(τ) were diminished at lower (below τ = 0.1) and higher quantiles (above τ = 0.95) and the Quantile Loss of 7.10 confirms effective handling of O3 variability. The standardized coefficients for NO were negative across all quantiles and became less negative at higher quantiles (0.8-1.0) that indicated a weaker adverse effect as O3 increased. NO2 showed positive coefficients that peaked at the 0.4 quantile and declined at higher quantiles and suggesting a stronger influence at moderate O3 levels. TVOC consistently exhibited negative coefficients with a stronger effect at lower quantiles (0.1-0.2) that stabilizes at higher quantiles. CO and SO2 coefficients fluctuate around zero and shows minimal and inconsistent influence. Monte Carlo simulation of health risk assessment showed that O3 could significantly pose the development of non-carcinogenic health risks (Hazard Quotient (HQ) > 1). Sensitivity analysis revealed the variance in the O3 Hazard Index (HI) where NO significantly contributed the most (60.4%), followed by NO2 (23.3%), TVOC (12.1%), SO2 (4.0%), and CO (0.2%). The Air Quality Index (AQI) analysis categorized Kharagpur as a ‘Moderately Polluted’ region. Overall, NOx and TVOC are the two types of major gaseous pollutants that contributed majorly in O3 concentration variability, thus O3 pollution levels. Targeted policies to reduce VOC and NOx emissions are essential.

How to cite: Santra, S.: Gaseous Pollutants Driven Ozone Variability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6582, https://doi.org/10.5194/egusphere-egu25-6582, 2025.

EGU25-7253 | Orals | AS3.28

Scenario Simulations for Estimating Environmental Impacts of Canadian Oil Sands Emissions 

Paul Makar, Sepehr Fathi, Stefan Miller, Colin Lee, Craig Stroud, Mahtab Majdzadeh, Junhua Zhang, Ali Katal, Mohammad Koushafar, Wanmin Gong, Oumarou Nikiema, Veronique Brousseau-Couture, Ivana Popadic, Hazel Cathcart, Greg Wentworth, Stephanie Connor, Yayne-abeba Aklilu, Amanda Cole, and Mathieu Rouleau

Ten one-year simulations were conducted using a nested high-resolution air-quality model (Global Environmental Multiscale-Modelling Air-quality and CHemistry; GEM-MACH).  The model nesting is from a 10km grid cell size North American domain, to a 2.5km grid cell size domain covering the Canadian provinces of Alberta and Saskatchewan (1350 x 1345 km).  The simulation period was from October 1, 2017 through September 30, 2018.  In addition to a base case simulation (see Fathi et al., 2025, this session, for the evaluation of this base case), nine additional scenario simulations were carried out.  These included six “Zero-Out” scenarios, in which specific contributions to the base case emissions were removed – comparisons to the base case thus provide the relative impact of these emissions sources.  Specific Zero-Out scenarios included the removal of all emissions associated with Oil Sands activities, all anthropogenic emissions, emissions associated with the Oil Sands off-road mining vehicle fleet, emissions associated with large stack sources, emissions associated with tailings ponds, and emissions associated with Oil Sands fugitive dust.  Three additional scenarios examined the impact of converting mine fleet vehicles from the 2018 fleet to Tier 4 level emissions control vehicles, the impact of revised land use fields for deposition to wetlands, and the impact of co-deposition of base cations and SO2 on the latter’s deposition flux.


Comparisons between the base case and the scenarios allow us to estimate the relative impact of the different emissions sources on air concentrations and deposition of pollutants of interest.  The zero-out scenarios thus give estimates of the relative impact of emissions from all Oil Sands sources, all anthropogenic sources, the Oil Sands off-road fleet, Oil Sands large stack sources, Oil Sands tailings ponds and Oil Sands fugitive dust on concentrations and deposition in the simulation area.  We also present the impact of a potential change in mine fleet emissions from the 2018 vehicle fleet composition to Tier 4 level vehicle emissions, of the land use data used as model input, and of co-deposition.   Two approaches will be used to investigate impacts:  in the first approach, the raw model output will be used for impact estimation; in the second approach, a simple form of model-measurement fusion will be applied to the gridded fields prior to impact estimation.   Ecosystem impacts will be assessed through applying model and model-measurement fusion deposition fields towards calculating exceedances of critical loads for forest, aquatic and bog ecosystems.  Human health impacts of the base case and scenarios will also be assessed using using a health impact function for fatal and non-fatal effects using the Air Quality Benefits Assessment Tool (AQBAT).

How to cite: Makar, P., Fathi, S., Miller, S., Lee, C., Stroud, C., Majdzadeh, M., Zhang, J., Katal, A., Koushafar, M., Gong, W., Nikiema, O., Brousseau-Couture, V., Popadic, I., Cathcart, H., Wentworth, G., Connor, S., Aklilu, Y., Cole, A., and Rouleau, M.: Scenario Simulations for Estimating Environmental Impacts of Canadian Oil Sands Emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7253, https://doi.org/10.5194/egusphere-egu25-7253, 2025.

EGU25-7297 | Posters on site | AS3.28

Key Atmospheric Processes in The Canadian Oil Sands Identified through Model Evaluation 

Sepehr Fathi, Paul Makar, Colin Lee, Alexandru Lupu, Craig Stroud, Stefan Miller, Mahtab Majdzadeh, Junhua Zhang, Ali Katal, Eric Edgerton, Matt Landis, Emily White, Oumarou Nikiema, Véronique Brousseau-Couture, Ivana Popadic, Helen Burgess, Calin Zaganescu, Andrea Darlington, and Greg Wentworth

We describe the current status of the ongoing model improvement and evaluation of the Oil Sands version of the Global Environmental Multiscale – Modelling Air-quality and CHemistry (GEM-MACH-OS) model.  GEM-MACH-OS was designed to provide 2.5km horizontal grid cell size model predictions for the chemical processing of gases and particulate matter emitted from industrial activities in the Canadian Oil Sands and other sources in the Canadian provinces of Alberta, Saskatchewan and neighboring regions.  Starting in 2022, a successive series of model updates and evaluations were carried out for the model simulation year October 1, 2017 through September 30, 2018.  We report here on several of these simulations how the comprehensive dataset from different monitoring networks was used to improve GEM-MACH-OS predictions, and identify key processes for Oil Sands chemistry.  The monitoring networks included the Wood Buffalo Environmental Association (WBEA, which provided hourly air concentration data for NO2, SO2, PM2.5, O3, NO and CO, daily intermittent total and speciated PM2.5 and PM10, and passive monthly to bimonthly SO2, NO2, HNO3, NH3 and O3), the National Trends Network (NTN, providing weekly precipitation totals and ions in precipitation for SO42-, NO3-, NH4+, Ca2+, Mg2+, K+, Na+ and Cl-), the National Air Pollution Surveillance program (NAPS, providing continuous hourly samples of NO2, SO2, PM2.5, O3, NO and CO, as well as daily intermittent samples of HNO3, SO2 speciated PM2.5, speciated total PM at CAPMoN stations), and the Canadian Air and Precipitation Monitoring Network (CAPMoN, providing daily intermittent samples of precipitation and ions in precipitation for the same species as NTN).

Examples of evaluation over 5 consecutive model versions will be shown, demonstrating both the improvement in model performance over time, and identifying chemical species for which further improvement is desired.  The evaluation also identified key processes governing chemical transformation in the region.  These included: (1) O3:  relatively little photochemical production from local emissions takes place, but down-mixing from the upper atmosphere creates a substantial seasonal signal; (2) SO2:  mostly emitted from large stacks, with the plume heights depending on a parameterization including latent heat release from combustion water (Fathi et al., 2024), and co-deposition potentially has a significant influence on SO2 deposition; (3) NO2:  a key reaction governing concentrations in the region is the reaction of NO2 on particle surfaces to form HONO and HNO3; (4) Forest fires in the region emit much lower levels of SO2 and NOx than standard inventory emission factors would suggest, and have a different particle speciation; (5) Particulate matter from Oil Sands fugitive dust sources is influenced both by vehicle-induced turbulence and meteorological modulation (with coarse mode emissions dropping off as temperatures drop below a fixed temperature when the ground is frozen, during rainfall and snowfall events, and as the surface soil water increases).  Planned next steps in model improvement will also be discussed.

How to cite: Fathi, S., Makar, P., Lee, C., Lupu, A., Stroud, C., Miller, S., Majdzadeh, M., Zhang, J., Katal, A., Edgerton, E., Landis, M., White, E., Nikiema, O., Brousseau-Couture, V., Popadic, I., Burgess, H., Zaganescu, C., Darlington, A., and Wentworth, G.: Key Atmospheric Processes in The Canadian Oil Sands Identified through Model Evaluation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7297, https://doi.org/10.5194/egusphere-egu25-7297, 2025.

EGU25-8756 | ECS | Orals | AS3.28

Importance of Anthropogenic Sources for Seasonal and Spatial Variability of Primary and Secondary Particulate Matter in Central Europe 

Hanna Wiedenhaus, Roland Schroedner, Ralf Wolke, Shubhi Arora, Laurent Poulain, and Radek Lhotka

In this study, the chemical transport model COSMO-MUSCAT (Wolke et al., 2012) is used to investigate the sources of particulate matter (PM). Model results are compared with observational data from winter and summer campaigns conducted at one site in Germany and two sites in the Czech Republic. These sites are located in a central European transition zone with a gradient from highly polluted to less polluted regions.

A non-reactive tagging approach was used to track primary organic matter (OM) and black carbon (BC) emissions by sector and country of origin at a high spatial resolution of about 2 km. In addition, sensitivity analyses were performed to assess the impact of volatile organic compound (VOC) emissions and associated secondary organic aerosol (SOA) formation.

Source attribution showed that residential heating is a major contributor to primary particulate matter (PM2.5) in winter. Sensitivity tests indicated that the model likely underestimates SOA production from AVOCs emitted during wood and coal combustion. By adjusting the SOA yields and emission rates for these combustion sources, modeled OM concentrations increased by up to 40% on average at the monitoring sites.

The findings underscore the significant role of AVOC precursors in the SOA budget, which is currently underrepresented in the model. Comparison with summer campaign data provides further insights into model performance and highlights seasonal variations in PM composition and sources across this critical region of Central Europe.

How to cite: Wiedenhaus, H., Schroedner, R., Wolke, R., Arora, S., Poulain, L., and Lhotka, R.: Importance of Anthropogenic Sources for Seasonal and Spatial Variability of Primary and Secondary Particulate Matter in Central Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8756, https://doi.org/10.5194/egusphere-egu25-8756, 2025.

High-resolution modelling of air pollutants such as NO2 and PM2.5 is an essential step in the quantification of the impacts on human health, especially in urban areas. Often, such modelling uses relatively coarse-resolution chemistry transport models (CTMs), which exhibit biases when compared to measurements and cannot consider the heterogenity of urban pollutant concentrations.

This study develops a machine learning (ML) framework to downscale CAMS regional air quality reanalyses for PM2.5 and NO2 from approximately 10×10 km² (0.1 degrees) to 1×1 km² resolution, enabling more detailed urban air quality assessments across Europe.

The downscaling methodology integrates meteorological, land-use, and spatial predictors to bridge the resolution gap. Key steps include: (1) interpolating CAMS outputs to a 1×1 km² grid, (2) constructing a training dataset by pairing interpolated CAMS data with ground-based measurements, (3) applying XGBoost (a gradient-boosted decision tree algorithm) and Gaussian Processes to model pollutant concentrations at 1×1 km² resolution, and (4) validating model performance using independent measurement data and FAIRMODE evaluation principles (e.g. Model Quality Objective, MQO). Predictor variables encompass meteorological inputs (e.g., daily temperature extremes, surface pressure, boundary layer height), geographical features (e.g., terrain height, proximity to roads, and coastlines), temporal indicators (e.g., year, month, date), and land-use data (e.g., Corine Land Cover and urban bounding boxes).

Preliminary results demonstrate the ability of the downscaling approach to capture fine-scale spatial patterns in urban air quality for a range of cities in Europe, with improved alignment to ground-based measurements compared to CAMS reanalyses. The high-resolution (1×1 km²) predictions reveal urban-level detail, enabling better inference on pollutant distribution in urban environments. Adherence to FAIRMODE principles ensures transparency and quality of results.

Future work will refine the ML framework, extend its application to other pollutants, and explore spatial and temporal scalability, ultimately aiming to deliver a transferable tool for high-resolution air quality modeling in any urban area across Europe.

How to cite: Ramacher, M. O. P. and Keil, P.: Machine Learning Downscaling of CAMS Regional Air Quality Reanalyses: High-Resolution Urban Concentrations of PM2.5 and NO2 Across Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9157, https://doi.org/10.5194/egusphere-egu25-9157, 2025.

EGU25-9571 | ECS | Orals | AS3.28

Decadal trends and drivers of global aerosol acidity: insights from model simulations and observational data 

Xurong Wang, Alexandra P. Tsimpidi, and Vlassis A. Karydis

Aerosol acidity is an essential property of atmospheric particles that affects not only atmospheric processes such as cloud formation, oxidation capacity, climate, and gas-particle phase partitioning, but also the Earth system, such as nutrient availability in terrestrial and marine ecosystems, and human health. The global distribution of aerosol acidity exhibits distinct spatial and temporal patterns, driven by variability in aerosol chemical composition, aerosol abundance, and local meteorological parameters. Due to the implementation of related clean air policies, a substantial reduction in aerosol abundance and a significant shift in chemical composition have been observed in recent times (Tsimpidi et al., 2024). However, the response of aerosol acidity remains modest and depends on the combined effect of aerosol changes and meteorology (Karydis et al., 2021). The contribution of each driving factor is debated, and the decadal trend of aerosol acidity is not well understood. In this study, we present a decadal simulation of global aerosol acidity using the EMAC atmospheric chemistry-climate model. The simulation is evaluated with results derived from field measurements over the continents of North America, Europe, and Asia. A one-at-a-time approach is employed to quantify the contributions of key driving factors, including temperature, relative humidity, and the availability of sulfate, total (gas and aerosol) nitrate, ammonium, and chloride, and nonvolatile cations  (sum of Na+, Ca2+, K+, and Mg2+) to annual and seasonal trends in aerosol acidity. Compared to field measurements, our simulation accurately reproduces temperature and relative humidity and shows good agreement of aerosol acidity with field measurements in Europe and the Pearl River Delta. We find that the underestimation of acidic ions, particularly sulfate, is the main reason for the low bias in simulated aerosol acidity in North America, and the underestimation of alkaline nonvolatile cations leads to high bias in aerosol acidity in the North China Plain. These findings highlight the nuanced interplay between chemical composition and meteorological factors in shaping global aerosol acidity trends and emphasize the importance of regional analyses in understanding long-term changes.

 

References

Karydis, V.A., Tsimpidi, A.P., Pozzer, A., Lelieveld, J., 2021. How alkaline compounds control atmospheric aerosol particle acidity. Atmospheric Chemistry and Physics 21, 14983-15001.

Tsimpidi, A.P., Scholz, S.M.C., Milousis, A., Mihalopoulos, N., Karydis, V.A., 2024. Aerosol Composition Trends during 2000-2020: In depth insights from model predictions and multiple worldwide observation datasets. EGUsphere 2024, 1-66.

How to cite: Wang, X., Tsimpidi, A. P., and Karydis, V. A.: Decadal trends and drivers of global aerosol acidity: insights from model simulations and observational data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9571, https://doi.org/10.5194/egusphere-egu25-9571, 2025.

EGU25-10060 | ECS | Orals | AS3.28

Ambient volatile organic compounds and their impact on ozone pollution regulation: insights from multi-platform observations and model representations from the 2021-2022 HKEPD-HKUST field campaign in Hong Kong 

Xueying Liu, Yeqi Huang, Zhe Wang, Yao Chen, Xin Feng, Yang Xu, Yi Chen, Dasa Gu, Hao Sun, Zhi Ning, Jianzhen Yu, Beryl Chow, Changqin Lin, Yan Xiang, Tianshu Zhang, and Jimmy Fung

Volatile organic compounds (VOCs) are crucial for atmospheric radical recycling and ozone formation. Despite significant reductions in other air pollutants in China since 2013, ozone and VOC levels remain persistently high, shifting air quality management toward VOC control. However, limited and short-term speciated VOC measurements hinder our understanding of regional VOC characteristics and effective emission reduction strategies for ozone mitigation in many Chinese cities. Therefore, in this study, we leveraged year-round routine VOC measurements in Hong Kong, together with field campaign and spaceborne TROPOMI data, to explore regional VOC characteristics and their relationships with ozone in the CMAQ chemical transport model. Results show that non-methane hydrocarbons (NMHCs) had higher concentrations in colder months and lower levels in warmer months, while oxygenated VOCs (OVOCs) peaked in September, coinciding with the annual ozone maximum and indicating strong photochemical activity in late summer. Notably, HCHO demonstrated a strong temporal correlation with total measured VOCs (R = 0.72–0.85) and ozone (R = 0.7). Among all measured VOC species, many are unaccounted for in the model, resulting in the model capturing only 30% of the total observed concentrations for NMHCs and 26% for OVOCs, as well as 14% of the ozone formation potential for NMHCs and 25% for OVOCs. This underrepresentation led to an overestimation of VOC sensitivity in ozone formation, classifying more areas as VOC-limited in the model. The findings provide valuable insights into regional VOC characteristics, aiding VOC-related model development and informing ozone air quality management strategies in VOC-limited urban environments.

How to cite: Liu, X., Huang, Y., Wang, Z., Chen, Y., Feng, X., Xu, Y., Chen, Y., Gu, D., Sun, H., Ning, Z., Yu, J., Chow, B., Lin, C., Xiang, Y., Zhang, T., and Fung, J.: Ambient volatile organic compounds and their impact on ozone pollution regulation: insights from multi-platform observations and model representations from the 2021-2022 HKEPD-HKUST field campaign in Hong Kong, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10060, https://doi.org/10.5194/egusphere-egu25-10060, 2025.

EGU25-11407 | Orals | AS3.28

On the applicability of the deposition velocity concept for ambient aerosols 

Rostislav Kouznetsov, Mikhail Sofiev, Andreas Uppstu, and Risto Hänninnen

Dry deposition is an important process of removal of various airborne substances from the atmospheric boundary layer. In many applications it is convenient to assume that the deposition flux of a substance is proportional to the near-surface concentration, and that the proportionality coefficient does not depend on particle concentration. This assumption is based on the idea of a constant-flux layer between the reference height and the surface, and holds for substances that have no sources/sinks in the layer. The deposition velocity concept is a core part of dry deposition schemes of atmospheric transport models.

We address large discrepancies between field and wind-tunnel measurements of deposition velocities of aerosols with aerodynamic diameter between approximately 0.1µm and 2µm. In seemingly similar conditions, deposition velocities derived from field measurements are in range of 1-10 cm/s, while wind-tunnel measurements show a fraction of a millimeter per second. This difference translates to the discrepancy in dry deposition parametrizations.

 

SILAM chemistry transport model features a dry deposition scheme for particles by Kouznetsov and Sofiev (2012, https://doi.org/10.1029/2011JD016366) that predicts 'low' deposition velocities. With such a scheme, simulations that explicitly account for aerosol transformations are able to reproduce the ambient observed fluxes and agree well with the 'high' apparent deposition velocity. A regional simulation covering the period of the Gallagher (2007, https://doi.org/10.1016/S1352-2310(96)00057-X) field campaign was capable of reproducing both magnitude and temporal evolution of aerosol fluxes measured over a forest.

 

We demonstrate that the conservation of aerosol mass in the immediate vicinity of the surface is not fulfilled for ambient aerosols when the aerosols include a fraction of ammonium nitrate. For such a mixture the fluxes of ambient aerosols are not controlled by particle deposition but rather by gas-particle partitioning in the vicinity of the surface and by the deposition flux of nitric acid. The particle flux does not depend on particle concentrations in quite a wide concentration range. For such a mixture the entire concept of deposition velocity is inapplicable.

 

Simulations of atmospheric aerosol composition show that the presence of ammonium nitrate as a part of aerosol is rather common in many places of the world. Moreover, we are not aware of any publication that demonstrates a linear dependency between the flux and concentration for ambient accumulation-mode aerosols. Based on our findings and the results of wind tunnel measurements we suggest that field campaigns could observe detectable fluxes of aerosol only if the fluxes were caused by aerosol processes in air. Therefore, such measurements cannot be used to directly infer particle deposition velocities, and the measurements with known conservative particles should be used instead. Parametrizations of deposition velocities that are based on the field-measured fluxes do not predict flux-concentration relation for particles if ammonium nitrate is present, and strongly over-deposit conservative aerosols. Therefore, the parametrizations based on wind-tunnel measurements with calibrated particles should be used instead, despite high-vegetation cases are not covered by such experiments.

How to cite: Kouznetsov, R., Sofiev, M., Uppstu, A., and Hänninnen, R.: On the applicability of the deposition velocity concept for ambient aerosols, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11407, https://doi.org/10.5194/egusphere-egu25-11407, 2025.

EGU25-13421 | Posters on site | AS3.28

Anthropogenic and natural emissions data for 2000-2023 at the global and regional scales for air quality forecasts and reanalyses  

Hugo Denier van der Gon, Santiago Arellano, Paula Camps, Stijn Dellaert, Michael Gauss, Claire Granier, Marc Guevara, Jukka-Pekka Jalkanen, Jeroen Kuenen, Cathy Li, Elisa Majamaki, Katerina Sindelarova, Emma Schoenmakers, David Simpson, and Nicolas Zilbermann

Emission inventories are the key starting point for understanding the causes and possible mitigation of air pollution. They provide information about the sources of air pollution, which can be used in air quality models to make air-quality forecasts and historical reanalyses. Therefore, the Copernicus Atmosphere Monitoring Service (CAMS) has a dedicated service to provide global and European anthropogenic and natural emissions data at high resolution to support consistent and quality-controlled information related to air pollution and health, solar energy, greenhouse gases and climate forcing, everywhere in the world. CAMS, including its emission service, has been fully operational since 1 July 2015 with its first phase ending in 2021. During the first emissions service contract under the 2nd phase of CAMS, ending in 2025, many new datasets are developed. Here we will give an overview of the CAMS emission products to inform modellers on the current state-of-the-art data. Anthropogenic emissions by source sector considering greenhouse gases and air pollutants are available for the global scale at 0.1x0.1 degree resolution for 2000-2025 (CAMS-GLOB-ANT) and European regional scale for 2005-2023 (CAMS-REG) at 0.1x0.05 degree resolution. These emissions come with auxiliary data such as emission height end emission timing following the sector-, country- and pollutant-dependent temporal profiles given by the CAMS-TEMPO dataset to provide monthly, daily or hourly emissions. For the European scale we now provide provisional recent years estimates to reduce the latency of emission data. Natural emissions are available from the CAMS emissions dataset, for biogenic, oceanic, soil, and volcanic emissions. The monthly emissions of 25 biogenic volatile organic compounds are given by the CAMS-GLOB-BIO dataset, for the 2000-2023 period at a 0.25x0.25 degree resolution. The recent years of CAMS-GLOB-BIO illustrate the dramatic growth of biogenic emissions due to the warming climate. CAMS-GLOB-SOIL provides NOx emissions from soils, for the 2000 -2023 period, for four categories. The new CAMS-GLOB-OCE dataset provides oceanic emissions of DMS and halogenated species for the 2000-2023 period at 0.5x0.5 degrees spatial resolution calculated with an Earth System model using ERA5 meteorological data and oceanic observations. The volcanic SO2 emissions from continuously degassing volcanoes for 2005-2023 are given in the CAMS-GLOB-VOLC, based on observations from the NOVAC (Network for Observation of Volcanic and Atmospheric Change) network and from a combination of satellite sensors, and show that 90% of sources have SO2 emissions below 1 kt/d and within the troposphere. In this presentation we discuss the latest developments, various trends and how to access the datasets.

How to cite: Denier van der Gon, H., Arellano, S., Camps, P., Dellaert, S., Gauss, M., Granier, C., Guevara, M., Jalkanen, J.-P., Kuenen, J., Li, C., Majamaki, E., Sindelarova, K., Schoenmakers, E., Simpson, D., and Zilbermann, N.: Anthropogenic and natural emissions data for 2000-2023 at the global and regional scales for air quality forecasts and reanalyses , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13421, https://doi.org/10.5194/egusphere-egu25-13421, 2025.

EGU25-13481 | ECS | Posters on site | AS3.28

Evaluating machine learning models for ozone pollution forecasting 

Joshua Miller and Oliver Wild

As global average temperatures rise, so too are wildfires projected to grow in size and frequency. This will cause an increase in wildfire-induced pollution, including ozone, a combustion byproduct, which is detrimental to human health. Accurate forecasts of air pollution are critical to provide early warnings to vulnerable communities, and in recent years different types of machine learning (ML) models have been created to predict the movement of pollutants in the atmosphere. However, there is little consensus about which type of model performs best, and very few studies consider the relationship between wildfires and ozone. We created several ML models to forecast tropospheric ozone concentrations over Africa between 2018 and 2022. Based on ML pollution forecasting literature, we chose to evaluate the Gradient Boosting Machine, Random Forest (RF), dense neural network (NN), convolutional NN, long-short term memory (LSTM) NN and Transformer NN models. Their inputs were daily wildfire activity, previous ozone concentration, wind speed/direction, and temperature; their output was the daily tropospheric ozone concentration. We evaluated the models’ forecasts using three metrics: mean-squared-error (MSE), ability to match the spatial heterogeneity of ozone concentrations in the target data, and correctly identifying ozone hotspots—concentrations above the 99th percentile. A convolutional NN coupled with a Transformer performed best overall, the RF was second-best, and the LSTM performed worst overall according to our metrics. To quantify how useful information about wildfires is to the accuracy of the forecasts, we removed fire from the training data and retrained and reevaluated all models. The results were inconsistent, and averaged across all models they were negligible: -0.955% MSE, +0.671% spatial variability mismatch, and +0.168% hotspot accuracy. We found a positive correlation (0.286) between daily wildfire activity and ozone concentrations and evidence that wildfire-produced ozone is consistently transported from East-to-West by wind. Our results show that convolutional-based models and the RF can and do accurately forecast ozone concentrations, and they outperform many other commonly used ML models used in similar domains.

How to cite: Miller, J. and Wild, O.: Evaluating machine learning models for ozone pollution forecasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13481, https://doi.org/10.5194/egusphere-egu25-13481, 2025.

EGU25-14560 | Orals | AS3.28

A dynamical ensemble approach to characterizing uncertainties in the prediction of air quality downstream of massive Western US wildfires in 2020 

Stefano Alessandrini, Rajesh Kumar, Christopher Rozoff, Jared A. Lee, Paddy McCarthy, and Wenfu Tang

To help guide advisories and various societal decision processes aimed at reducing humanity’s detrimental exposure and risks tied to poor air quality, NOAA predicts ozone (O3), fine particulate matter (PM2.5), and other harmful pollutants daily. Unfortunately, air quality forecasts still suffer from errors emanating from the driving datasets, inaccurate emissions, and an incomplete understanding of air quality processes. With increasingly intense western North American wildfires producing expansive and harmful smoke plumes that impact millions of people downstream, it is important to improve predictions. This work aims to design a dynamical ensemble based on the NOAA’s Online Community Multiscale Air Quality (Online CMAQ) embedded within the UFS. The ensemble is based on perturbations of (a) meteorological and chemical initial and lateral boundary conditions, (b) anthropogenic, biogenic, and biomass burning emissions, (c) secondary organic aerosol response to temperature changes and solubility of semi-volatile organic compounds (SVOCs), and (d) removal processes including the hygroscopicity of aerosols and dry deposition velocities of O3, precursors, and SVOCs. Such a perturbation strategy leads to >50 ensemble members. In this presentation, the ensemble is evaluated against AirNOW observations of O3 and PM2.5 in the summer of 2020 when historic western US wildfires generated extensive smoke plumes. The ensemble validation and analysis of the uncertainty will be the central focus of this presentation. The project's ultimate goal is to develop down-selection techniques with calibration to reduce the ensemble size to ~10 members such that the majority of skill and ensemble quality is retained. This will provide a cost-effective air quality ensemble for NOAA’s operational air quality forecasting.

How to cite: Alessandrini, S., Kumar, R., Rozoff, C., Lee, J. A., McCarthy, P., and Tang, W.: A dynamical ensemble approach to characterizing uncertainties in the prediction of air quality downstream of massive Western US wildfires in 2020, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14560, https://doi.org/10.5194/egusphere-egu25-14560, 2025.

EGU25-16433 | ECS | Orals | AS3.28

Machine learning for high-resolution mapping of air pollutants over Italy (2021–2023) 

Karam Mansour, Matteo Rinaldi, Stefano Decesari, Marco Paglione, and Tony Christian Landi

Air pollution poses significant risks to human health and the environment. Nitrogen dioxide (NO2) is a key air pollutant with well-documented adverse health effects and a precursor to ozone (O3). Generally, particulate matter (PM) is a major global cause of mortality, with both short-term and long-term exposure linked to severe health outcomes (WHO, 2021). High-resolution maps of near-surface air pollutant concentrations are essential to assess these impacts effectively.

We will present daily gridded maps of near-surface NO2 and O3, as well as PM2.5 and PM10 (particles with an aerodynamic diameter equal to or less 2.5 and 10 µm respectively) concentrations across the Italian territory, generated for 2021–2023 at a spatial resolution of 0.01° × 0.01° (~1 km). Machine learning (ML) models are trained using a combination of spatial and spatiotemporal predictors, informed by in-situ ground measurements from over 300 monitoring stations sourced from the European Air Quality Portal (AQP), managed by the European Environmental Agency (EEA) (EEA, 2024). Key spatial predictors include CORINE Land Cover, which provides 44 thematic classes at 100 m resolution; the Global Human Settlement Layer, reflecting human presence; NASA’s Digital Elevation Model, offering topographical information; and the ESA Plant Functional Type dataset (Harper et al., 2023). Spatiotemporal predictors integrate meteorological fields from ERA5-Land and aerosol optical depth (AOD) data from the Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2).

We will evaluate various supervised ML models (Mansour et al., 2024b), including neural networks, regression ensembles, and regression trees across various landscapes (urban, suburban, and rural) to identify the optimal approach for each context. Additionally, explainable AI techniques (e.g., partial dependence analysis and Shapley additive exPlanations) and statistical analysis (e.g., clustering and empirical orthogonal functions) will be employed to elucidate the relationships between predictors and aerosol spatiotemporal distributions (Mansour et al., 2023; Mansour et al., 2024a), providing novel insights into the dynamics of air quality across regions. These advancements contribute to a more refined understanding of air pollution patterns and their underlying drivers.

Funding:

Project funded under the National Recovery and Resilience Plan (NRRP), Mission 04 Component 2 Investment 1.5 – NextGenerationEU, Call for tender n. 3277 dated 30/12/2021. Award Number: 0001052 dated 23/06/2022 (ECS_00000033_ECOSISTER).

References:

EEA: Europe’s air quality status (2024), https://www.eea.europa.eu//publications/europes-air-quality-status-2024.

Harper, et al. (2023), Earth System Science Data, 15, 1465-1499, 10.5194/essd-15-1465-2023.

Mansour, et al. (2023), Science of The Total Environment, 871, 10.1016/j.scitotenv.2023.162123.

Mansour, et al. (2024a), npj Climate and Atmospheric Science, 7, 10.1038/s41612-024-00830-y.

Mansour, et al. (2024b), Earth System Science Data, 16, 2717–2740, 10.5194/essd-16-2717-2024.

WHO (2021), World Health Organization, https://iris.who.int/handle/10665/345329.

How to cite: Mansour, K., Rinaldi, M., Decesari, S., Paglione, M., and Landi, T. C.: Machine learning for high-resolution mapping of air pollutants over Italy (2021–2023), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16433, https://doi.org/10.5194/egusphere-egu25-16433, 2025.

EGU25-16770 | Posters on site | AS3.28

Street-scale Air Pollution Modelling in İstanbul – The Case of Beşiktaş District 

Huseyin Ozdemir, Enes Birinci, Jibran Khan, and Ali Deniz

Air pollution has become one of the most critical global challenges, exacerbated by climate change and the growing human population. It poses a significant threat to public health, particularly in urban areas where high population density and increased vehicle numbers contribute to poor air quality. The primary motivation of this study is to estimate street-scale air pollution in Beşiktaş, İstanbul, Türkiye, with the Operational Street Pollution Model (OSPM®). Beşiktaş district is a hotspot for traffic density with approximately 170,000 residents, and it hosts critical roadways connecting the European and Asian sides of the city. Understanding air pollution at this scale in Beşiktaş is crucial due to the area’s high population density and traffic volume, significantly impacting public health and urban air quality. The road connecting the Beşiktaş district to the İstanbul Bosphorus was selected as a Case Study and our Area of ​​interest (AOI). This study provides an overview of the data collected, including air quality measurements (PM10, PM2.5, NO2) from a nearby Air Quality Monitoring Station (AQMS), meteorological data from Turkish State Meteorological Service (TSMS), and geographic and traffic data from İstanbul Metropolitan Municipality. A representative 800-meter-long road segment was selected for modeling, focusing on traffic-related air pollution using hourly vehicle data. In this study, air pollution measurement data such as PM10, PM2.5, and NOX are evaluated on the street in the Beşiktaş region with AirGIS and OSPM® modeling to be subsequently analyzed. Air quality data (PM10, PM2.5, NO2) were obtained from a nearby AQMS, while meteorological data were obtained from the TSMS, 3.5 km from the street. Geographic data and traffic data were obtained from İstanbul Metropolitan Municipality.  According to the World Health Organization (WHO), PM2.5 and NO2 concentration values ​​exceeded the limit value every day, while PM10 exceeded it for 13 days during the study period. The highest traffic density occurred at 10:00 a.m, and the average number of vehicles was found to be 1,942. In terms of traffic emissions, gasoline vehicles in total 31,829, which has a much larger share compared to diesel vehicles (7,234). The temporal changes (hourly and daily) in air pollution will be analyzed by this model. At the same time, a correlation analysis will be made between the model's concentration values and those measured by AQMS. This model enables both short- and long-term assessments of air pollution exposure, contributing to studies on human health impact.

How to cite: Ozdemir, H., Birinci, E., Khan, J., and Deniz, A.: Street-scale Air Pollution Modelling in İstanbul – The Case of Beşiktaş District, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16770, https://doi.org/10.5194/egusphere-egu25-16770, 2025.

EGU25-16806 | Posters on site | AS3.28

Improvements and challenges of modeling air pollutants by assimilating Sentinel-5p TROPOMI observations 

Zhuyun Ye, Kaj M. Hansen, Jesper H. Christensen, Lise M. Frohn, and Camilla Geels

Within the framework of the CAMS Evolution (CAMEO) project, we implement a three-dimensional variational (3D-Var) data assimilation system in the Danish Eulerian Hemispheric Model (DEHM) to improve simulations of key atmospheric pollutants in Europe including sulfur dioxide (SO2), ozone (O3), carbon monoxide (CO), and formaldehyde (HCHO). The data assimilation framework integrates Sentinel-5p (S5p) TROPOMI satellite observations with model predictions to provide more accurate estimates of these species. The 2023 Mount Etna eruptions, captured in S5p observations, provide an opportunity to evaluate the performance of the modeling system under extreme emission scenarios. Of particular interest is the ability of the system to capture not only the substantial SO2 plumes from volcanic eruptions, but also their cascading effects on other pollutants – including the formation of CO through magmatic processes, and perturbations in O3 concentrations due to complex gas and heterogeneous chemical processes. Our approach confronts several key challenges, including the representation of highly localized and dynamic pollutant distributions, interactions of different chemical species, and the refinement of error covariance structures for both regular and extreme episodes. Evaluations with both satellite and ground observations show enhancements of SO2 concentrations especially at upper layers (e.g. 2-4 km) but also show challenges to improve ground-level concentrations compared to observations. Sensitivity analyses are conducted to assess the impact of assimilation frequency, observation error specifications, and the inclusion of supplementary ground-based data. Results demonstrate improvements in the capability of DEHM to simulate atmospheric transport and chemical processes across various temporal and spatial scales, from regional background conditions to intense emission events. The study highlights the potential of near-real-time satellite data assimilation in enhancing vertical distribution and provides insights into optimizing model performance during dynamic emission events. The findings also provide insights into optimizing model performance for varying spatial and temporal scales of atmospheric phenomena.

How to cite: Ye, Z., Hansen, K. M., Christensen, J. H., Frohn, L. M., and Geels, C.: Improvements and challenges of modeling air pollutants by assimilating Sentinel-5p TROPOMI observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16806, https://doi.org/10.5194/egusphere-egu25-16806, 2025.

EGU25-17162 | Posters on site | AS3.28

Tracing Wildfire-Derived Carbon Monoxide: Insights into Global Transport and Atmospheric Impacts Using a Chemistry-Transport Model 

Nikos Daskalakis, Maria Kanakidou, Laura Gallardo, and Mihalis Vrekoussis

Carbon monoxide (CO) is a key atmospheric trace gas generated from both natural sources, such as biomass burning and volcanic activity, and human-related activities, including vehicle emissions, agricultural practices, and industrial operations. CO plays a key role in atmospheric chemistry as a precursor for tropospheric ozone (O3) in the background atmosphere, thereby influencing the oxidative capacity of the global atmosphere. Elevated CO concentrations are linked to adverse effects on air quality, human health, and also climate, particularly through O3 and CO2 formation.

A growing concern is the contribution of wildfires to CO emissions, as their frequency and severity have risen in response to climate change. CO released from wildfires has immediate effects on air quality and long-term implications for atmospheric composition, making it critical to evaluate its role in air quality, climate dynamics, and public health.

In this study, we use the TM4-ECPL global chemistry and transport model, a highly validated and widely used tool, to examine the pathways and impacts of wildfire-related CO. Our analysis incorporates historical emissions data from the advanced Climate Model Intercomparison Project 6 (CMIP6) database. To achieve regional specificity, we use 13 tracers aligned with the 13 source regions identified by the Hemispheric Transport of Air Pollution version 2 (HTAPv2) framework. Model simulations are driven by ERA-interim meteorology and cover a 20-year period (1995–2015), allowing the analysis of climatological trends and prominent biomass burning events. The contributions of regional CO emissions and their transport across the global ocean are calculated, shedding light on their influence on atmospheric composition and global air quality.

We find that ENSO has a significant impact only on the CO emitted from South East Asia, where from all other source regions we see minimal deviation from the average climatological data. Furthermore, we find that Southern African emitted pollution has the greatest potential impact on the global ocean, with South East Asia being a major contributor in the North and South Pacific and Indian Ocean, and South America a major contributor in the South Pacific.

How to cite: Daskalakis, N., Kanakidou, M., Gallardo, L., and Vrekoussis, M.: Tracing Wildfire-Derived Carbon Monoxide: Insights into Global Transport and Atmospheric Impacts Using a Chemistry-Transport Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17162, https://doi.org/10.5194/egusphere-egu25-17162, 2025.

EGU25-17198 | ECS | Orals | AS3.28

Implementation of a particle resuspension model in a Large Eddy Simulation code 

Victor Bourgin, Mohamed Sellam, and Amir Feiz

In urban areas, pollutant deposition leads to the accumulation of particles on surfaces. These particles include emissions from traffic, heavy metals, micro-plastics and other debris. In the right meteorological conditions, these pollutants can be detached from the surface and resuspended, adversely affecting air quality near the ground and directly exposing city inhabitants. Soil resuspension was found to be a lingering cause of lead exposure for children in several US cities [1]. With the advent of electrical vehicles, indirect sources such as resuspension will become greater contributors to air pollution.

However, quantifying the contribution of resuspension to pollutant exposure remains challenging. Field studies often rely on indirect measurement methods, and wind tunnel experiments use simplified topologies. Computational fluid dynamics tools (CFD) have been employed in only a few studies, with even fewer utilizing the Large Eddy Simulation (LES) framework.

Here we present the coupling of a particle resuspension model to PALM, an open-source LES code. Resuspension is simulated according to the Rock’n’Roll model [2], a probability based approach estimating the resuspension rate from macroscopic properties. The originality of the coupling is that the distribution of adhesion forces is discretized. This allows resuspension to interact with deposition, which is crucial to apply the Rock’n’Roll model to urban air quality studies.

The coupling has been validated against experimental data from [2]. Further validation is planned against more recent datasets, paving the way for the expansion of the Rock’n’Roll model to include effects such as surface roughness [3], flow acceleration [4] and non-spherical particles. We will discuss preliminary results obtained in the case of a street canyon, offering insights into resuspension dynamics in urban environments. Our work aims to provide guidelines to create healthier urban environments and understand how evolving transportation technologies will shape pollutant exposure patterns.

 

[1] M. Laidlaw, G. Filippelli, Resuspension of urban soils as a persistent source of lead poisoning in children: A review and new directions, Applied Geochemistry, Volume 23, Issue 8,  2021-2039, (2008).

[2] M.W. Reeks, D. Hall, Kinetic models for particle resuspension in turbulent flows: theory and measurement, Journal of Aerosol Science, Volume 32, Issue 1, 1-31, (2001).

[3] S. Peillon et al., Adhesion forces of radioactive particles measured by the Aerodynamic Method–Validation with Atomic Force Microscopy and comparison with adhesion models, Journal of Aerosol Science, Volume 165, (2022).

[4] C. Cazes, Resuspension of microparticles in the air induced by transient events in the flow, experimental approach, Ecole nationale supérieure Mines-Telecom Atlantique, (2023)

 

 

How to cite: Bourgin, V., Sellam, M., and Feiz, A.: Implementation of a particle resuspension model in a Large Eddy Simulation code, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17198, https://doi.org/10.5194/egusphere-egu25-17198, 2025.

EGU25-18159 | Posters on site | AS3.28

A physics-based and orientation-aware method for the direct calculation of  the settling speed of prolate spheroidal particles in the atmosphere : theoretical basis and comparison to laboratory and CFL data 

Sylvain Mailler, Sotirios Mallios, Arineh Cholakian, Vassilis Amiridis, Laurent Menut, and Romain Pennel

We have developed a new method to calculate the settling speed of non-spherical aerosols in the atmosphere, beginning with prolate spheroidal aerosol even though the method could be generalized to other shapes such as oblate spheroids or fibers. Most existing formulations of the settling speed are empirical numerical fits designed to match the results of either laboratory measurements or CFD simulations. On the contrary, the method we expose is based essentially on theoretical results on the drag and orientation of settling particles, with a minimal use of empirical numerical fits. As a result, the present method is more simple than existing methods and (with less empirical coefficients), and permits to calculate the settling speed of a prolate particle settling in the atmosphere as a function of the characteristics of the particle and of the atmospheric conditions, with no additional information. The varying distribution of particle orientation is accounted for using the results of Mallios et al. (2021), and the force-to speed relationships are based on Mailler et al. (2024), which we have extended to intermediate orientations and systematized to reach the present results.

The method presented here has been implemented in Fortran in the AerSett module, and the corresponding implementation is distributed under the free GPL-3.0 license . We hope that this novelty will permit to take into account more frequently particle elongation in chemistry-transport models, which may prove important in the case of, e.g., giant dusts, or microplastic particles with elongated shapes.

How to cite: Mailler, S., Mallios, S., Cholakian, A., Amiridis, V., Menut, L., and Pennel, R.: A physics-based and orientation-aware method for the direct calculation of  the settling speed of prolate spheroidal particles in the atmosphere : theoretical basis and comparison to laboratory and CFL data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18159, https://doi.org/10.5194/egusphere-egu25-18159, 2025.

EGU25-18163 | ECS | Orals | AS3.28

LUVR: An interpretable Land Use and Visual Regression model embedding Street View images in air pollution modeling with mobile monitoring 

Zhendong Yuan, Jules Kerckhoffs, Gerard Hoek, and Roel Vermeulen

Mobile monitoring campaigns using Land Use Regression (LUR) models effectively capture fine-scale spatial variations in urban air pollution. While traditional LUR models rely on land-use and demographic features, integrating micro-environmental information from Google Street View (GSV) images offers the potential to further enhance the model performance.

We developed LUVR, a framework that integrates vision-transformer-based (ViT) object detection and semantic segmentation features derived from GSV images into LUR models. Using 5.7 million mobile air pollution measurements and 0.37 million GSV images collected in Amsterdam, we modeled nitrogen dioxide (NO₂), black carbon (BC), and ultrafine particles (UFP) in 50m road segments. Three temporal image selection strategies—specific year, most nearby year, and season-weighted—were tested with stepwise linear regression and random forest models.

We found that adding GSV-derived features improved model performance, increasing R² by 0.01–0.05 and reducing errors by 0.7%–10.3%. The most-nearby-year strategy performed the best for NO2, while BC and UFP benefited slightly more from the season-weighted strategy. This result suggests that for air pollution modeling, GSV-derived built environment features remain relatively stable across years. Using an open-vocabulary object detection module, we detected customized objects described in natural language in a zero-shot fashion, revealing previously unrecognized predictors such as chimneys, traffic lights, and shops. Combined with segmentation-derived features like walls, roads, and grass, visual features contributed 8%–18% to the overall model prediction.

This study demonstrates the potential of integrating visual features into LUR models to enhance hyperlocal air pollution monitoring and exposure assessment. Future research should optimize feature selection and expand applications to broader urban and environmental health studies.

How to cite: Yuan, Z., Kerckhoffs, J., Hoek, G., and Vermeulen, R.: LUVR: An interpretable Land Use and Visual Regression model embedding Street View images in air pollution modeling with mobile monitoring, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18163, https://doi.org/10.5194/egusphere-egu25-18163, 2025.

EGU25-18306 | ECS | Posters on site | AS3.28

A super-simplified OH chemistry scheme for ICON-ART 

Philipp Dietz, Roland Ruhnke, and Peter Braesicke

Monitoring greenhouse gas (GHG) emissions is essential to face global warming and climate change. The ITMS project (“Integriertes Treibhausgas Monitoringsystem”, in English “integrated GHG monitoring system”)[1], is designed to establish an operational GHG data assimilation service at the German Meteorological Service (DWD) based on the model system ICON-ART[2] to enable Germany to operationally monitor the sources and sinks of three important GHGs: carbon dioxide (CO2), methane (CH4) and nitrous oxide (N2O).

In the first phase of the ITMS project DWD together with the Karlsruhe Institute of Technology (KIT) and other partners are focusing on the emission, distribution and depletion of methane. In the troposphere, methane is mainly depleted by the chemical reaction with the OH radical. Tropospheric OH is created mostly by the photolytic destruction of ozone (O3) and thus its abundance depends mainly on the available solar UV radiation and the ozone concentration. The calculation of this chemical system is computationally expensive. Therefore, a simplified calculation of the OH chemistry has to be included in the ICON-ART forward model.

Here, we present first results of a super-simplified OH-chemistry scheme for ICON-ART, a data-driven approach based on Minschwaner et al., 2011[3]. The OH concentration is hereby estimated based on the solar zenith angle (SZA) at the respective grid cell. The required parameters are pre-trained on SZA information and OH concentration from the CAMS global reanalysis (EAC4)[4].

[1] www.itms-germany.de

[2] Schröter, J., Rieger, D., Stassen, C., Vogel, H., Weimer, M., Werchner, S., Förstner, J., Prill, F., Reinert, D., Zängl, G., Giorgetta, M., Ruhnke, R., Vogel, B., and Braesicke, P.: ICON-ART 2.1: a flexible tracer framework and its application for composition studies in numerical weather forecasting and climate simulations, Geosci. Model Dev., 11, 4043–4068, https://doi.org/10.5194/gmd-11-4043-2018, 2018.

[3] Minschwaner, K., Manney, G. L., Wang, S. H., and Harwood, R. S.: Hydroxyl in the stratosphere and mesosphere – Part 1: Diurnal variability, Atmos. Chem. Phys., 11, 955–962, https://doi.org/10.5194/acp-11-955-2011, 2011.

[4] Inness et al. (2019), http://www.atmos-chem-phys.net/19/3515/2019/

How to cite: Dietz, P., Ruhnke, R., and Braesicke, P.: A super-simplified OH chemistry scheme for ICON-ART, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18306, https://doi.org/10.5194/egusphere-egu25-18306, 2025.

The HAM-M7 aerosol scheme within OpenIFS 48r1: developing EC-Earth4

 

Lianghai Wu*, Eemeli Holopainen,Tommi Bergman, Twan van Noije, Philippe Le Sager, Ramiro Checa-Garcia, Xuemei Wang, Adrian Hill, Marcus Koehler, Harri Kokkola, Anton Laakso, Vincent Huijnen

 

*Royal Netherlands Meteorological Institute, 3730 AE De Bilt, the Netherlands

 

We implemented a new interactive aerosol module as part of the OpenIFS 48r1. The module is based on the Hamburg Aerosol Module (HAM) version 2.3 with at its core the M7 microphysics scheme. By representing aerosol in multiple modes, the M7 scheme enables a detailed description of aerosol particle characteristics, optical properties, and aerosol-cloud interactions. The new module will be used in the Earth system model EC-Earth 4 to improve the modelling of the life cycle of anthropogenic and natural aerosols, their direct and indirect radiative effects, and to deepen our understanding of their influence on climate change and weather patterns.

 

The implementation presented several challenges including a significant jump of five IFS cycles from the initial implementation in OpenIFS 43r3 to the presented implementation in 48r1, the coupling between other key modules such as the radiative transfer kernel (ecRad), cloud scheme and existing chemistry modules, and missing parallelization and restartability functionality. Additionally, the lack of a prior reference implementation to evaluate the performance of the implemented scheme added to the complexity. To address these challenges, we reviewed the entire model workflow, including emissions, removal processes (sedimentation, wet and dry deposition), optical properties, and diagnostics, to identify and resolve performance issues.

 

In this presentation, we will share our progress and the latest global aerosol simulation results driven by the emissions from the Copernicus Atmosphere Monitoring Service (CAMS). We will highlight the global distribution of aerosol properties, including mass concentrations, aerosol removal fluxes, and aerosol optical depth, along with preliminary evaluation against independent observations. We identify missing elements which require further improvements.

How to cite: Wu, L.: The HAM-M7 aerosol scheme within OpenIFS 48r1: developing EC-Earth4, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18376, https://doi.org/10.5194/egusphere-egu25-18376, 2025.

EGU25-18517 | Posters on site | AS3.28

Plume dispersion, mixing and chemistry simulation using the Lagrangian Volumetric Particle Approach with realistic atmospheric chemical kinetics mechanisms 

Massimo Cassiani, Armin Wisthaler, Tove Svendby, Gabriela Sousa Santos, and Sverre Solberg

The Lagrangian Volumetric Particle Approach (VPA), introduced by Cassiani (2013), has been implemented within an operational Lagrangian Stochastic Particle Dispersion Model, which now includes a set of chemical kinetics equations for atmospheric chemistry. The model is coupled on-line with a grid-based Eulerian Chemistry Transport Model (CTM), which solves the same set of atmospheric chemical kinetics equations.

By employing the Lagrangian VPA, the high-order covariances arising from the averaging operator applied to the nonlinear chemical kinetics mechanisms are represented in closed form. This capability enables the VPA to model, with high accuracy, both the near-source turbulent dispersion and mixing as well as the impacts of atmospheric turbulence on highly nonlinear plume chemistry.

The integration with the Eulerian CTM allows the separation of background and plume chemistry using a plume-in-grid scheme. This advanced modeling system has been developed as part of the FuNitr project (Future Drinking Water Levels of Nitrosamines and Nitramines near a CO2 Capture Plant), which aims to investigate potential chemical transformations within plumes emitted by Carbon Capture and Storage (CCS) facilities.

Here, we present the modeling system alongside simulations of reactive plumes, incorporating a reduced but realistic atmospheric chemical kinetic mechanism.  Reference: Cassiani, M. (2013). The volumetric particle approach for concentration fluctuations and chemical reactions in Lagrangian particle and particle-grid models. Boundary-Layer Meteorology, 146(2), 207–233.

How to cite: Cassiani, M., Wisthaler, A., Svendby, T., Sousa Santos, G., and Solberg, S.: Plume dispersion, mixing and chemistry simulation using the Lagrangian Volumetric Particle Approach with realistic atmospheric chemical kinetics mechanisms, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18517, https://doi.org/10.5194/egusphere-egu25-18517, 2025.

EGU25-18837 | Posters on site | AS3.28

PM10 Spatiotemporal Patterns in Portugal: Functional Data Analysis from 2017 to 2018 

Rita Durao, Manuel Ribeiro, Madalena Simões, André Brito, Célia Gouveia, and Ana Russo

Air pollution significantly and severely affects human health, environment, materials, and economy, emerging as a key microclimate and air quality regulation issue. Hence, the spatial and temporal characterization of air pollutants and their relationship with meteorological constraining factors is critical, particularly from a climate change perspective.

Within this context, we present an exploratory statistical assessment combining functional data analysis (FDA) with unsupervised learning algorithms and spatial statistics to extract meaningful information about the main spatiotemporal patterns underlying air pollutant exceedances in mainland Portugal. Air pollutants’ spatial and temporal characterization over Portugal was performed, focusing particularly on the emissions of Particulate Matter (PM) during the major wildfire events in 2017-2018 and based on the Copernicus Atmosphere Monitoring (CAMS) data. Firstly, the temporal evolution of PM concentrations on each CAMS grid node was described as a function of time and outline the main temporal patterns of variability using a functional principal component analysis. Afterwards, CAMS grid nodes are classified according to their spatiotemporal similarities through hierarchical clustering adapted to spatially correlated functional data. Preliminary results show the main spatial patterns of AQ variability and indicate the regions presenting higher PM levels, especially during wildfire events. The present approach shows the potential of existing exploratory tools for spatiotemporal analysis of PM10 data, over regions less covered by the national air quality monitoring network.

Acknowledgements: This work is supported by the Portuguese Fundação para a Ciência e Tecnologia, FCT, I.P./MCTES through national funds (PIDDAC): UID/50019/2025 and LA/P/0068/2020 https://doi.org/10.54499/LA/P/0068/2020); and also on behalf of DHEFEUS -2022.09185.PTDC and the project FAIR- 2022.01660.PTDC).

How to cite: Durao, R., Ribeiro, M., Simões, M., Brito, A., Gouveia, C., and Russo, A.: PM10 Spatiotemporal Patterns in Portugal: Functional Data Analysis from 2017 to 2018, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18837, https://doi.org/10.5194/egusphere-egu25-18837, 2025.

EGU25-19339 | ECS | Orals | AS3.28

 Reconstruction, Regionalization, and Prediction of Tropospheric Pollution in the Mediterranean Basin: A Machine Learning Approach 

Francisco Sánchez-Jiménez, Eloisa Raluy-López, Leandro Cristian Segado-Moreno, Ester García-Fernández, Pedro Jiménez-Guerrero, and Juan Pedro Montávez
Atmospheric pollution at the tropospheric level is a critical concern, particularly in the Mediterranean basin, which experiences significant air quality challenges. This study focuses on key pollutants: ozone (O₃), particulate matter (PM₁₀ and PM₂₅), nitrogen monoxide (NO), and nitrogen dioxide (NO₂). Hourly measurements from 3323, 4727, 2317, 3446, and 4933 monitoring stations, respectively, spanning the period 2000–2022, were analyzed. These data, sourced from the AirBase database provided by the European Environmental Agency (EEA), exhibit challenges typical of long-term monitoring, such as missing data, inconsistencies, outliers, and station reassignments due to relocations.
To address these challenges, a robust and reliable database was constructed, applying advanced data-cleaning techniques to ensure data quality while maximizing valid entries. Subsequently, a backward-reconstruction algorithm for time series was developed, leveraging the higher data density available from 2013 onwards. This algorithm, based on Bayesian Ridge Regression and interpolation methods, successfully reconstructed historical records station by station, incorporating crucial temporal trends and spatial coherence. The methodology enabled complete reconstruction for stations with sufficient data quality post-2013.
The reconstructed dataset facilitated a regional clustering analysis, grouping stations by similar spatiotemporal pollution patterns. This regionalization revealed distinct areas with shared trends in tropospheric pollution evolution. Integrating meteorological variables such as solar radiation, temperature, cloud cover, precipitation, and pollution persistence further enriched the analysis. Advanced machine learning techniques, including Principal Component Analysis (PCA) and Random Forest models, were employed to develop predictive models for each pollutant, enabling accurate contamination forecasts.
This research highlights the potential of combining statistical reconstruction techniques, spatiotemporal clustering, and machine learning to enhance our understanding and prediction of atmospheric pollution trends. By addressing long-standing data issues and leveraging modern computational tools, the study contributes a robust framework for long-term air quality analysis in the Mediterranean region, offering insights applicable to other regions facing similar challenges.

How to cite: Sánchez-Jiménez, F., Raluy-López, E., Segado-Moreno, L. C., García-Fernández, E., Jiménez-Guerrero, P., and Montávez, J. P.:  Reconstruction, Regionalization, and Prediction of Tropospheric Pollution in the Mediterranean Basin: A Machine Learning Approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19339, https://doi.org/10.5194/egusphere-egu25-19339, 2025.

EGU25-19789 | Orals | AS3.28

Impact of Biogenic Emissions on Ozone Episode Evolution During the July 2022 Heatwave: A TFMM Modelling Exercise 

Joanna Struzewska, Tomasz Przybyła, Aleksander Norowski, Jacek Kaminski, and Grzegorz Jeleniewicz

Despite mitigation efforts, ozone pollution in Europe remains a significant issue. As part of the EMEP program, the Task Force on Measurement and Modelling (TFMM) conducted a measurement campaign from 12-19 July 2022 to evaluate the impact of various VOC species on ozone concentration levels and variability. This campaign coincided with adverse thermal conditions – a strong heatwave moving from west to east across Europe, enhancing biogenic VOC emissions and ozone production.
To interpret the campaign results, TFMM launched an air quality modelling exercise involving 11 models that reproduced the variability of chemical tracer concentrations in July 2022. Apart from the experiments to reproduce the evolution of concentrations, additional scenarios aimed at assessing the contribution of anthropogenic vs. biogenic VOC emissions were undertaken. The importance of the dry deposition of ozone was also evaluated. We will show preliminary results from the study focusing on model performance during the peak of the episode and the spread between individual models based on measurements taken at EMEP stations and during the campaign. The average contribution of biogenic emissions to ozone and its precursors will also be assessed.

How to cite: Struzewska, J., Przybyła, T., Norowski, A., Kaminski, J., and Jeleniewicz, G.: Impact of Biogenic Emissions on Ozone Episode Evolution During the July 2022 Heatwave: A TFMM Modelling Exercise, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19789, https://doi.org/10.5194/egusphere-egu25-19789, 2025.

EGU25-20076 | ECS | Orals | AS3.28

A Deep-Pollutant-Spatial-Operator-Network (DPSON) for spatial estimation of PM2.5, PM10, O3 and NO2, case study at Delhi, India 

Subhojit Mandal, Mainak Thakur, Vigneshkumar Balamurugan, Jia Chen, and Arijit Roy

Atmospheric pollutants affect human health, disrupt ecosystems, and impact the economy. Spatial prediction of atmospheric pollutants using data from ground monitoring stations (GMS) is vital for informed decision-making and sustainable ecosystem management. To estimate atmospheric pollutants, this study introduces the Deep-Pollutant-Spatial-Operator-Network (DPSON) framework that combines GMS data with multi-source spatial covariates in order to produce precise predictions at a 1 km × 1 km grid across Delhi (Indian capital city). Pollutant data from 40  Central Pollution Control Board, India (CPCB) monitored GMS locations (January 2021–December 2022) were used for this purpose. The PM2.5 and PM10 datasets are available at a 3-hour resolution, while O3 and NO2 at a 1-hour resolution.

Normalized static spatial covariates, such as population density, waterbody concentration, road-length concentration, green cover, and Land Use Land Cover (LULC), were included to improve the DPSON model’s accuracy. To improve the dataset's generalization in relation to spatial covariate variations, additional samples were generated using the Sequential Gaussian Simulation (SGS) algorithm, randomly simulating pollutant observations at 100 grid locations on a 1 km² spatial grid for each timestamp and pollutant species, based on the pollutant concentrations observed at 40 GMS locations. These SGS-generated and GMS-observed datasets were combined for developing the DPSON model.

A specially crafted reference Distance-Assisted Location Embedding (DALE) approach was utilized to provide accurate spatial scaling and embedding of the locations within the DPSON network. The approach utilizes cosine and sine transformations of latitude and longitude, combined with a sine transformation of the distance from a reference point, to create suitable spatial embeddings for the network. The model architecture comprises two parameterized networks: (1) the Branch Network and (2) the Trunk Network. The Branch Network is responsible for embedding the pollutant data observed by GMS along with the static spatial covariates of the corresponding locations and their DALE. The Trunk network uses the DALE of unsampled locations, their static spatial covariates to estimate the pollutant concentration at those locations. The DPSON network’s reconstruction error (i.e.: Trunk network output) on the CPCB locations were considered for checking the model capability. The DPSON model was eventually compared with other baseline models. The proposed DPSON model achieved the following performance metrics: for PM2.5, RMSE of 31.91 µg/m³, MAE of 18.35 µg/m³, and R² of 0.88; for PM10, RMSE of 49.95 µg/m³, MAE of 32.02 µg/m³, and R² of 0.87; for O3, RMSE of 11.75 µg/m³, MAE of 7.27 µg/m³, and R² of 0.85; and for NO2, RMSE of 12.05 µg/m³, MAE of 7.67 µg/m³, and R² of 0.88. The proposed DPSON model outperforms all the baseline models for each of the pollutants and is adept at managing various types of spatial covariates, accommodating complex GMS observation distributions, while also providing a computationally efficient framework for the spatial estimation of pollutants.

How to cite: Mandal, S., Thakur, M., Balamurugan, V., Chen, J., and Roy, A.: A Deep-Pollutant-Spatial-Operator-Network (DPSON) for spatial estimation of PM2.5, PM10, O3 and NO2, case study at Delhi, India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20076, https://doi.org/10.5194/egusphere-egu25-20076, 2025.

EGU25-20377 | Orals | AS3.28

Changes in air pollutant emissions in China during two clean-air action periods derived from the newly developed Inversed Emission Inventory for Chinese Air Quality (CAQIEI)  

Xiao Tang, Lei Kong, Zifa Wang, Jiang Zhu, Jianjun Li, Huangjian Wu, Qizhong Wu, Huansheng Chen, Lili Zhu, Wei Wang, Bing Liu, Qian Wang, Duohong Chen, Yuepeng Pan, Jie Li, Lin Wu, and Gregory Carmichael

A new long-term emission inventory called the Inversed Emission Inventory for Chinese Air Quality (CAQIEI) was developed in this study by assimilating surface observations from the China National Environmental Monitoring Centre (CNEMC) using an ensemble Kalman filter (EnKF) and the Nested Air Quality Prediction Modeling System. This inventory contains the constrained monthly emissions of NOx , SO2 , CO, primary PM2.5, primary PM10, and non-methane volatile organic compounds (NMVOCs) in China from 2013 to 2020, with a horizontal resolution of 15 km × 15 km. This paper documents detailed descriptions of the assimilation system and the evaluation results for the emission inventory. The results suggest that CAQIEI can effectively reduce the biases in the a priori emission inventory, with the normalized mean biases ranging from −9.1 % to 9.5 % in the a posteriori simulation, which are significantly reduced from the biases in the a priori simulations (−45.6 % to 93.8 %). The calculated root-mean-square errors (RMSEs) and correlation coefficients were also improved from the a priori simulations, demonstrating good performance of the data assimilation system. Based on CAQIEI, the total emissions from 2015 to 2020  decreased by 54.1 % for SO2, 44.4 % for PM2.5, 33.6 % for PM10, 35.7 % for CO, and 15.1 % for NOx but increased by 21.0 % for NMVOCs. It is also estimated that the emission reductions were larger during 2018–2020 (from −26.6 % to −4.5 %) than during 2015–2017  (from −23.8 % to 27.6 %) for most of the species. In particular, the total Chinese NOx and NMVOC emissions were shown to increase during 2015–2017, especially over the Fenwei Plain area (FW), where the emissions of particulate matter (PM) also increased. The situation changed during 2018–2020, when the upward trends were contained and reversed to downward trends for the total emissions of both NOx and NMVOCs and the PM emissions over FW. This suggests that the emission control policies may be improved in the 2018–2020 action plan. We also compared CAQIEI with other air pollutant emission inventories in China. CAQIEI suggested higher CO emissions in China, with CO emissions estimated by CAQIEI (426.8 Tg) being more than twice the amounts in previous inventories (120.7–237.7 Tg). CAQIEI suggested higher NMVOC emissions than previous emission inventories by about 30.4 %–81.4 % over the North China Plain (NCP) but suggested lower NMVOC emissions by about 27.6 %–0.0 % over southeastern China (SE). CAQIEI suggested lower emission reduction rates during 2015–2018 than previous emission inventories for most species, except for CO. In particular, China’s NMVOC emissions were shown to have increased by 26.6 % from 2015 to 2018, especially over NCP (by 38.0 %), northeastern China (by 38.3 %), and central China (60.0 %). These results provide us with new insights into the complex variations in air pollutant emissions in China during two recent clean-air actions. All of the datasets are available at https://doi.org/10.57760/sciencedb.13151.

How to cite: Tang, X., Kong, L., Wang, Z., Zhu, J., Li, J., Wu, H., Wu, Q., Chen, H., Zhu, L., Wang, W., Liu, B., Wang, Q., Chen, D., Pan, Y., Li, J., Wu, L., and Carmichael, G.: Changes in air pollutant emissions in China during two clean-air action periods derived from the newly developed Inversed Emission Inventory for Chinese Air Quality (CAQIEI) , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20377, https://doi.org/10.5194/egusphere-egu25-20377, 2025.

Various air pollution problems ultimately have a serious negative impact on human health and welfare, damage to property, and adversely affect animals and plants. For this reason, people's interest in air pollution problems has increased, and researchers' study to solve air pollution problems has become more diverse and increased. In order to efficiently manage PM2.5 and prepare effective control measures, qualitative and quantitative analysis of pollutants emitting PM2.5 must be conducted first, and PM2.5 must be collected from the receptor and its characteristics analysed. Receptor methods that estimate and evaluate the contribution of pollutants are continuously implemented. The receptor model is a mathematical and statistical methodology that analyses the physical and chemical characteristics of air pollutants at the receptor, identifies sources that affect air quality, and quantitatively estimates the contribution of each source (source apportionment).

Since the release of PMF2 and ME, these programs have been successfully applied to assess ambient PM source contributions in many locations of virous countries. However, PMF and ME models are somewhat difficult to use because these models are DOS-base programs that require understanding of a special script language. Therefore, in order to provide a widely applicable PMF with a user-friendly and graphic user interface (GUI)-based program, the US Environmental Protection Agency (EPA) developed an EPA version of PMF. The US EPA continued to upgrade to the EPA-PMF model including the factor rotation functions. Therefore, the current version 5.0 model has been developed and widely used to source apportionment.

Pohang, the study area of this study, is where Korea's representative steel industry and steel-related industries are gathered, and a steel-related industrial complex is located there. In addition, it is one of the areas with severe air pollution that emits large amounts of particulate matter such as PM2.5 and various gaseous pollutants due to the frequent operation of heavy trucks to transport produced steel products. Therefore, in this study, we performed EPA-PMF modeling using data from the PM2.5 Pohang monitoring site, identified the PM2.5 sources, and then estimated the contribution of each source.

The PM2.5 samples were collected at Pohang air pollution monitoring site from January 2018 to August 2022 and 27 species (OC, EC, SO42-, NO3-, Cl-, Na+, NH4+, K+, Mg2+, Ca2+, As, Br, Ca, Cd, Cr, Cu, Fe, K, Mn, Ni, Pb, S, Se, Si, Ti, V, and Zn) were analyzed by XRF (X-ray fluorescence spectroscopy; Xact-series 620, USA), IC (ion chromatography; URG-9000D, USA), and TOT (thermal optical transmittance; 4F-semi continuous field analyzer, USA) methods. The EPA-PMF model was used to identify sources and estimate source apportionment in Pohang site. The source apportionment data for this study area, which is characterized by the location of a large-scale steel plant and related industrial complexes, can be said to be of great importance, unlike the results of source contribution studies for the study area that have been widely conducted in general. More detailed results of source apportionment for PM2.5 samples in Pohang site will be presented.

How to cite: Hwang, I. and Park, J.: Source Apportionment of Ambient PM2.5 Data using the EPA-PMF Model at Monitoring site near the steel mill, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-39, https://doi.org/10.5194/egusphere-egu25-39, 2025.

EGU25-1087 | ECS | Orals | AS3.29

Advancing PM2.5 Source Apportionment through Dispersion Normalized PMF: A Comprehensive Study across India 

Delwin Pullokaran, Ankur Bhardwaj, Diksha Haswani, Ramya Sunder Raman, Deeksha Shukla, Abisheg Dhandapani, Jawed Iqbal, Naresh Kumar R, Sadashiva Murthy BM, and Laxmi Prasad

The recent IPCC report highlights PM2.5 as one of the most important contributors to air pollution and its health impacts. Determining the sources of air pollution, quantifying their contributions to ambient pollutant levels, and characterizing their spatial and temporal patterns are all important steps in developing effective mitigation strategies (Hopke, 2016). Source apportionment studies, especially those using receptor models, are critical for this purpose. Of these, Positive Matrix Factorization (PMF) is a widely applied methodology. The current work evolves standard PMF (S-PMF) by Tapper and Paatero, 1994 based on the implementation of dispersion-normalized PMF (DN-PMF) suggested by Dai et al., 2020 that includes meteorologically-influenced enhancement towards increasing local source emissions resolution. DN-PMF preserves source information otherwise obscured by variable atmospheric conditions, yielding refined and distinct source profiles.
            This research investigates the spatial and seasonal variability of PM2.5 sources across three Indian cities—Bhopal (MSL: 486 m), Mesra (MSL: 517 m), and Mysuru (MSL: 759 m)—as part of the COALESCE network in 2019. A Multiple Seasonal-Trend Decomposition using LOESS (MSTL) was applied to mixed layer height time series to decompose into their daily, weekly, and trend components. Stationarity tests were performed using the Augmented Dickey-Fuller with a p-value <0.05. Reconstructed mass (RCM) from PM2.5 chemical constituent was validated against measured PM2.5 gravimetric mass as suggested by Pullokaran et al., 2024. DN-PMF analysis was performed on chemically speciated datasets comprising organic and elemental carbon fractions (OC1, OC2 OC3,OC4, OP, EC1, EC2, EC3), water-soluble inorganic ions F-, Cl-, NO3, SO4-2, Na+, NH4+, K+), elements (Al, Mg, Ca, Si, P, K, V, Ti, Co, Ni, Cu, Cd, Fe, Ni, Zn, Se, Ba, Hg, Pb), and non-water-soluble potassium (Knws).

A total of nine factors were resolved in Bhopal, the residential heating factor (23.1%) showed the highest contribution. A smelter source was also identified, due to the high explained variance in EC3 (40%), Zn (71%), Pb, Cu, and EC2. At Mysuru, seven factors were identified, with secondary sulfate (26.2%) identified as the dominant factor. Based on the high explained variance of F- (57%), SO4-2 (39%), and minor loadings of NO3-, Mn, Fe, and Si a brick kiln source was identified in Mysuru. Mesra revealed eight factors, with secondary sulfate (22.8%) and secondary nitrate (19.1%) as major contributors. The biomass burning emissions peaked during India’s stubble burning period (pre-monsoon and post-monsoon) at all three sites. Potential regional and local sources of PM2.5 sources were identified using the Potential Source Contribution Function (PSCF) analysis. The findings provide robust chemically speciated PM2.5 data and improved source apportionment through DN-PMF. These results offer actionable insights for policymakers and environmental agencies, facilitating effective air quality management and targeted mitigation strategies.

How to cite: Pullokaran, D., Bhardwaj, A., Haswani, D., Sunder Raman, R., Shukla, D., Dhandapani, A., Iqbal, J., Kumar R, N., Murthy BM, S., and Prasad, L.: Advancing PM2.5 Source Apportionment through Dispersion Normalized PMF: A Comprehensive Study across India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1087, https://doi.org/10.5194/egusphere-egu25-1087, 2025.

EGU25-2700 | ECS | Posters on site | AS3.29

Methods and issues of reducing reactive loss impacts in ambient VOC source apportionments 

Baoshuang Liu, Yao Gu, Yutong Wu, Qili Dai, Shaojie Song, Yinchang Feng, and Philip K. Hopke

With the increase in ozone (O3) concentrations in multiple cities or regions worldwide in recent years, accurate source apportionment methods of its key precursor VOCs have been acquired increasing attention. Chemical reactive losses of ambient VOCs have been a long-term issue yet to be resolved in the VOC source analyses research. Thus, we systematically assessed the common methods and existing issues in ways to reduce losses and loss impacts in source apportionment studies by reviewing relevant publications and suggests research directions for improved VOC source apportionments. Compared to any other mathematical models, positive matrix factorization (PMF) is now a main VOC source apportionment approach. The issue in using any apportionment tool is the processing of the data to be analyzed to reduce the impacts of reactive losses. Calculating the initial concentrations of VOC species based on photochemical age has become a major method to reduce reactive loss effects in PMF, except for selecting low-reactivity species or nighttime data into the analysis. The initial concentration method only considers daytime reactions with hydroxyl (•OH) radicals at present. However, the •OH rate constants vary with temperature, and that has not been considered. Losses from reactions with O3 and NO3 radicals remain to be included. Therefore, the accuracy of the currently photochemical age estimation is uncertain. Beyond developing accurate quantitative methods for chemical losses, source apportionment methods of the consumed VOCs and the accurate quantification of source contributions to O3 and secondary organic aerosol (SOA) are important directions for future studies.

How to cite: Liu, B., Gu, Y., Wu, Y., Dai, Q., Song, S., Feng, Y., and Hopke, P. K.: Methods and issues of reducing reactive loss impacts in ambient VOC source apportionments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2700, https://doi.org/10.5194/egusphere-egu25-2700, 2025.

EGU25-3840 | Posters on site | AS3.29

Effect of dispersion normalisation on PM10 elemental sources at a rural background site in Central Europe  

Petra Pokorná, Laurence Windell, Adéla Holubová Šmejkalová, Ondřej Vlček, Naděžda Zíková, Radek Lhotka, Jaroslav Schwarz, Jakub Ondráček, and Vladimír Ždímal

Rural background sites, representative of a wider area, are important for investigating the influence of regional and long-range transport as well as long-term trends in PM concentrations (Putaud et al., 2010). Dispersion normalisation using the ventilation coefficient has recently been shown to be an effective approach that provides improved source apportionment results with clearer diel and seasonal patterns for speciated PM datasets (Dai et al., 2020). The focus of this study was to assess the influence of dispersion conditions represented by ventilation coefficient on speciated PM10 concentrations and their origins at the National Atmospheric Observatory Košetice (NAOK, 49°35'N, 15°05'E), a rural background site in Central Europe (LRI ACTRIS ERIC, https://www.actris.eu/).

PM10 elemental composition was measured every 4-h for three years (2021 – 2023) by the Xact625i (Cooper Environmental Services, USA), an online ED-XRF ambient multi-metals monitor. Ventilation coefficient was calculated with 1-h resolution by the numerical weather prediction model ALADIN for subsequent dispersion normalisation of highly time-resolved and speciated PM10 data. Advanced receptor modelling (US EPA PMF 5.0) was applied to both non-dispersion and dispersion normalised highly time-resolved PM10 elemental datasets.

PMF resolved five factors of PM10 (secondary sulphate, residential heating – biomass and coal, soil/re-suspended dust, sea/road salt, industry) for both datasets with almost identical chemical profiles. The factor contributions were positively (lower contributions – secondary sulphate, residential heating, and salt) and negatively (higher contributions – soil/re-suspended dust and industry) influenced by dispersion conditions. Dispersion normalisation provided improved source apportionment results with clearer diel and seasonal patterns, primarily for secondary sulphate and residential heating, the main sources of elemental PM10.

This conference contribution was supported by the Ministry of Education, Youth and Sports of the Czech Republic under grant ACTRIS-CZ (LM2023030).

 

Putaud, J.P., et al., 2010. A European aerosol phenomenology — 3: physical and chemical characteristics of particulate matter from 60 rural, urban, and kerbside sites across Europe. Atmos. Environ. 44, 1308–1320.

Dai, Q. at al., 2020. Dispersion Normalized PMF Provides Insights into the Significant Changes in Source Contributions to PM2.5 after the COVID-19 Outbreak. Environ. Sci. Tech. 54, 16, 9917–9927.

How to cite: Pokorná, P., Windell, L., Holubová Šmejkalová, A., Vlček, O., Zíková, N., Lhotka, R., Schwarz, J., Ondráček, J., and Ždímal, V.: Effect of dispersion normalisation on PM10 elemental sources at a rural background site in Central Europe , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3840, https://doi.org/10.5194/egusphere-egu25-3840, 2025.

EGU25-4111 | Orals | AS3.29

RI-URBANS: Source apportionment of different pollutants in urban Europe 

Xavier Querol, Fulvio Amato, Thérèse Salameh, Gaëlle Uzu, Kaspar Daellenbach, Marta Via, Marjan Savadkooh, Meritxell Garcia-Marlès, Tuukka Petäjä, Hilkka Timonen, Marco Pandolfi, Andrés Alastuey, Jesús de la Rosa, Xiansheng Liu, and Philip Hopke

RI-URBANS (Research Infrastructures Services Reinforcing Air Quality (AQ) Monitoring Capacities in European Urban & Industrial AreaS) is a research project supported by the European Commission under the Horizon 2020 – Research and Innovation Framework Programme, H2020-GD-2020 (grant 10103624) that connects the atmospheric observation expertise from Aerosols, Clouds and Trace gases Research InfraStructure (ACTRIS), with the urban air quality observation capacities of the regulatory air quality monitoring networks. It is specifically connected to the new European AQ Directive (NAQD) 2024/2881/CE published on 20 November 2024.

RI-URBANS focuses on the infrastructures to measure emerging pollutants for AQ and the well-being of the citizens. Particularly, service tools (STs) for novel pollutants, such as ultrafine particles (UFP), UFP-number size distribution (PNSD), black carbon (BC), as well as ammonia (NH3) and numerous volatile organic compounds (VOCs), and measurements of tracers of potential toxicity of PM (oxidative potential (OP) of particulate matter PM), are provided for urban supersites in order to support scientific understanding of their effects on health and the environment. The NAQD has been introduced in Art. 10 the measurements of these new pollutants in a new network of AQ supersites.

In essence, these STs are guidance documents that RI-URBANS have reviewed, in some cases developed, tested, and recommended for advanced AQ assessment in urban areas. Two of these STs focus on the source apportionment of PM based on receptor modelling with offline and online PM speciation (ST10) and on UFP-PNSD, BC, VOCs and OP of PM. The electronic files of the guidance documents of ST10 and ST11 can be downloaded at https://riurbans.eu/project/#service-tools

PMF is used in most cases (PM, VOCs, UFP-PNSD), and it is coupled with multi-linear regression for (OP), and aethalometer source apportionment for BC.

Here we present the results from the application of these source apportionment tools to datasets of PM speciation, UFP-PNSD, VOCs, BC and OP data available in urban Europe. The results have a high interest for AQ policy (identifying major sources contributing to air quality impairment, but also identifying measures needed and evaluating the impact of policy actions), evaluation of the health outcomes, and identifying the source contributions with higher toxicity potential.

The creation of the European network of AQ supersites by the European NAQD will provide very valuable datasets for source apportionment receptor modelling of a number of pollutants, however the required PM speciation in the NAQD is quite limited for obtaining detailed source apportionment results. It is important to intensify the source apportionment studies to support the need of more tracers of PM to be included in the supersites in the next review of the Directive, which will take place in five years.

How to cite: Querol, X., Amato, F., Salameh, T., Uzu, G., Daellenbach, K., Via, M., Savadkooh, M., Garcia-Marlès, M., Petäjä, T., Timonen, H., Pandolfi, M., Alastuey, A., de la Rosa, J., Liu, X., and Hopke, P.: RI-URBANS: Source apportionment of different pollutants in urban Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4111, https://doi.org/10.5194/egusphere-egu25-4111, 2025.

EGU25-4263 | Orals | AS3.29

Source apportionment of aerosol particle number in background Stockholm: impact of aviation and shipping 

Fulvio Amato, Michael Norman, Sanna Silvergren, Daniel Schlesinger, Lina Broman, Ellen Bergseth, and Ulf Olofsson

Ultrafine particles (UFP) have gained increased attention during recent years due to their adverse health effects (WHO, 2021). Both the WHO and the EU have therefore recommended systematic measurements of particle number concentration (PNC) and particle number size distributions (PNSD) in cities.

The nPETS project (nanoparticles Emissions from the Transport Sector) aimed to study the lifecycle of sub-100 nm particles from different sources. The nPETS project in Stockholm included measurements of PNSD and PNC in urban background air on a rooftop. PNSDs were measured during two years with 16 channels between 10 and 410 nm and Positive Matrix Factorization (PMF) source apportionment was used to analyse these data.

 

Four different emission source profiles were attributed by the PMF analysis:

 

  • The most important factor with on average 38 % of the PNC had a peak between 25 – 45 nm. It was most dominant during periods with high PNC, high NOx and low wind speed. It also followed the local rush hours and was identified as traffic with a typical diesel contribution.

 

  • The second most important factor with 36 % of the PNC had at peak 60- 150 nm. It was dominating with northeasterly and higher wind speeds with strongest signal late afternoons and evening. The size distribution showed similarity with ship emissions from other nPETS measurements. Trajectories also showed influence from the Baltic Sea.

 

  • The third factor was associated with a peak below 20 nm in size. It showed similarity to aircraft particles from other nPETS measurements and had also strongest impact during moderate northwesterly winds which corresponds to the direction of the local Bromma airport. This factor was contributing to 17 % of the PNC.

 

  • The fourth factor had a peak in particles larger than 200 nm. It showed strong correlation with PM1 mass and air mass trajectories from easterly Europe. This factor was thought to be long-range transport and was contributing to 8 % of the PNC.

 

The PMF analysis was compared with dispersion modelling of PNC in the Stockholm region. The emission database (EDB) used was from Eastern Sweden Air Quality Association with inputs from the nPETS project. Based on the dispersion modelling the traffic is the largest source, while shipping is a minor source and aviation negligible. Long range transport was not included in the modelling. The magnitude of UFP emissions from aviation in Stockholm is still largely unknown with low emissions in the EDB. Shipping in central Stockholm is limited to passenger ships in port only during some hours per day which explains the relatively small emissions in the EDB.

The discrepancy between the PMF analysis and the dispersion modelling for shipping and aviation demands further investigations.

 

Reference.

WHO (2021). WHO global air quality guidelines

How to cite: Amato, F., Norman, M., Silvergren, S., Schlesinger, D., Broman, L., Bergseth, E., and Olofsson, U.: Source apportionment of aerosol particle number in background Stockholm: impact of aviation and shipping, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4263, https://doi.org/10.5194/egusphere-egu25-4263, 2025.

EGU25-4394 | ECS | Orals | AS3.29

PM10 source apportionment in two sites of southern Spain by Positive Matrix Factorization. Evaluation of the relevance of sampling site altitude to the PM10 fingerprint. 

Alessandro Zappi, Erika Brattich, Pietro Morozzi, Mariassunta Biondi, Mauro Masiol, José Antonio Orza, and Laura Tositti

The evaluation of the sources of particulate matter (PM) is one of the most important topics in environmental science. Both natural and anthropogenic sources are involved in the overall PM pollution in both urban and rural areas. Mathematical methods, as Positive Matrix Factorization (PMF), applied to chemical data are the most powerful tools for the discrimination of PM sources.

In the present work, the results obtained from a three-year sampling campaign (between 2017 and 2019) are presented. 700 PM10 filters were collected in the framework of FRESA Project (Impact of dust-laden African air masses and of stratospheric air masses in the Iberian Peninsula. Role of the Atlas Mountains) from two sites in Andalusia, southern Spain: the first one is in the city of Granada, while the second one is in Sierra Nevada. Filters were analyzed by ion chromatography and Particle-Induced X-ray Emission (PIXE) for elemental analysis.

The two stations are relatively close to each other (around 20 km). However, the Sierra Nevada station is located at an altitude of 2550 m a.s.l, while the Granada station is at 738 m a.s.l. This altitude difference of almost 2000 m makes the two sites very different from a PM-sources point of view, as highlighted by the two parallel PMF models applied to chemical data. Indeed, Sierra Nevada samples showed the impact of frequent mineral dust intrusions from Sahara Desert, that greatly affected the overall PM composition; in Granada site, instead, samples showed the typical urban fingerprint, with lower evidences of Saharan dust intrusions, due to the different circulation as a function of height.

How to cite: Zappi, A., Brattich, E., Morozzi, P., Biondi, M., Masiol, M., Orza, J. A., and Tositti, L.: PM10 source apportionment in two sites of southern Spain by Positive Matrix Factorization. Evaluation of the relevance of sampling site altitude to the PM10 fingerprint., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4394, https://doi.org/10.5194/egusphere-egu25-4394, 2025.

EGU25-4796 | Posters on site | AS3.29

PMF-Bayesian Modeling for Spatial Source Apportionment of Airborne Particulate Matter 

Qili Dai, Tianjiao Dai, Jingchen Yin, Jiajia Chen, Baoshuang Liu, Xiaohui Bi, Jianhui Wu, Yufen Zhang, and Yingchang Feng

Mass concentrations of ambient particulate matter (PM) have been extensively monitored in urban areas worldwide. Despite the widespread availability of such data, it has rarely been utilized in receptor-based source apportionment studies, which predominantly rely on PM chemical speciation data. In this study, we used over one million data points of PM concentrations from more than 100 monitoring sites within a Chinese megacity to perform spatial source apportionment of coarse particles (PM2.5-10). These particles are believed to primarily originate from local emissions and are often characterized by significant spatial heterogeneity. We employed an enhanced positive matrix factorization (PMF) approach, designed to handle large datasets, in combination with a Bayesian multivariate receptor model to determine spatial source impacts. Four primary sources were successfully identified: residential burning, industrial processes, road dust, and meteorologically-related sources. The combined methodology demonstrates substantial potential for broader application in other regions.

How to cite: Dai, Q., Dai, T., Yin, J., Chen, J., Liu, B., Bi, X., Wu, J., Zhang, Y., and Feng, Y.: PMF-Bayesian Modeling for Spatial Source Apportionment of Airborne Particulate Matter, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4796, https://doi.org/10.5194/egusphere-egu25-4796, 2025.

EGU25-4799 | ECS | Posters on site | AS3.29

Substantial Differences in Source Contributions to Carbon Emissions and Health Damage Revealed by Adjoint Modeling 

Yilin Chen, Huizhong Shen, Guofeng Shen, Jianmin Ma, Yafang Chen, Armistead Russell, Shunliu Zhao, Amir Hakami, Shu Tao, Jiao Du, and Jing Meng

China's dual strategy to mitigate climate change and air pollution is constrained by insufficient data on the distinct sources of carbon emissions and associated health damages. This study utilizes adjoint emission sensitivity modeling with the CMAQ Adjoint model, alongside an exposure-response model and a multiregional input-output model, to perform high-resolution source attribution across 53 production sectors and fuel/process combinations, as well as 42 consumption economic sectors. Our analysis uncovers significant discrepancies between sources of CO2 emissions and PM2.5-related premature mortality, with monetized health damages surpassing climate impacts in over half of the subsectors examined. Additionally, more than one third of the CO2 emissions and health damages are outsourced from well-developed coastal provinces to less-developed inland provinces, though the regions absorbing these burdens differ geographically. CO2 emissions are primarily shifted to the northwestern region, which relies heavily on coal as an energy source, while PM2.5-related deaths are concentrated in the central region, the heavy industrial hub of China with high population densities. These findings demonstrate that high population densities and lower adoption of control technologies exacerbate health damages, particularly in downstream provinces that bear the majority of emission leakages. The CMAQ Adjoint model’s capability to evaluate the marginal benefits of emission reductions at a granular level enabled precise source attribution by incorporating emission profiles, population density, and atmospheric conditions. This research underscores the critical advantage of adjoint modeling in integrating health and climate impacts, advocating for tailored mitigation strategies that address emissions from both production and consumption sides to achieve balanced decarbonization and effective health risk mitigation in China.

How to cite: Chen, Y., Shen, H., Shen, G., Ma, J., Chen, Y., Russell, A., Zhao, S., Hakami, A., Tao, S., Du, J., and Meng, J.: Substantial Differences in Source Contributions to Carbon Emissions and Health Damage Revealed by Adjoint Modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4799, https://doi.org/10.5194/egusphere-egu25-4799, 2025.

Air quality is significantly influenced by weather patterns, such as wind direction, wind speed, and atmospheric dispersion, which play a direct role in driving fine particulate matter (PM2.5) concentrations. This study employed three online monitoring instruments to conduct assessments of the chemical species in PM2.5 during the winter season of 2020–2021. By applying the positive matrix factorization (PMF) model, pollution sources and their contributions were identified within Taipei City. To further explore the relationship between meteorological conditions and pollution, clustering techniques were employed to classify weather patterns associated with PM2.5 levels exceeding 25 µg/m³.

The analysis revealed three distinct high-concentration weather patterns, each linked to specific pollution sources: (1) Low wind speed and poor dispersion conditions were associated with elevated traffic-related emissions, peaking at 7.4 µg/m³; (2) Strong northeast monsoon patterns resulted in relatively lower PM2.5 levels due to reduced pollutant accumulation in the basin; and (3) Northwest wind patterns were characterized by significant contributions from coal and fuel combustion, industrial sources, and secondary aerosols, with PM2.5 concentrations reaching up to 56 µg/m³.

This study is the first to combine source apportionment results from individual receptor sites with nonparametric trajectory analysis (NTA). Under weak wind conditions, traffic-related pollutants were observed to accumulate predominantly south of the receptor site, with maximum concentrations of 14 µg/m³. In contrast, northwest wind patterns showed notable accumulation of pollutants from civil construction and metalwork northwest of the receptor site, with concentrations reaching 8 µg/m³.

These findings highlight the critical role of weather pattern classification in understanding PM2.5 pollution sources, offering valuable guidance for policymakers to implement effective air quality controls. Building on this foundation, future research will adapt these methodologies to explore the pollution sources of ozone and its precursors. Specifically, the new approach will integrate data from multiple monitoring stations with NTA to achieve spatial mapping of pollution source contributions. This advancement aims to provide a more comprehensive understanding of the distribution and impact of ozone and its precursors, deepening insights into the complex interactions between meteorology, atmospheric chemistry, and air quality management.

How to cite: Hsieh, P.-Y. and Wu, C.-F.: Integrating Weather Patterns with PMF Modeling: Insights into PM2.5 Pollution Sources and Future Applications to Ozone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4893, https://doi.org/10.5194/egusphere-egu25-4893, 2025.

EGU25-6097 | Posters on site | AS3.29

Formation sensitivity and source analysis of tropospheric ozone in a typical industrial city in China based on the observation data coupled with chemical mechanism 

Yulong Yan, Yueyuan Niu, Ke Yue, Jiaqi Dong, Jing Wu, Yuhang Wang, and Lin Peng

Tropospheric ozone (O3) is a typical secondary pollutant and produced by a series of chemical reactions of precursors such as nitrogen oxides (NOx) and volatile organic compounds (VOCs) under light conditions. The emission of precursors in industrial cities is large and complex, and the relationship between O3 and its precursors is not clear, making it is challenged to identify the key factors and source influencing O3 formation. This study used observation-based-model (OBM), based on the precursors’ observation data and chemical mechanism, to analyze O3 sensitivities to VOCs and NOx during summer in a typical industrial city in China. In our research, higher concentrations of O3 precursors were observed during O3 polluted periods in summertime indicating that precursor accumulation contributed to the higher max net (O3) (16.6 ppbv∙h-1) and HOx· concentrations. The important reactions in ROx· recycling was mainly dominated by the precursors of NO, NO2 and alkene, which were mainly discharged from sources caused by the developed industry. Analyses of relative incremental reactivity (RIR) indicated that O3 production during polluted period is in a chemical transition regime and was sensitive to both VOCs (RIR=0.39) and NOx (RIR=0.56), particularly emphasizing the crucial of phased control of O3 precursors. Results from PMF analysis indicated that gasoline vehicle emissions were the major contributor to VOCs (27.0%), followed by coal combustion (20.3%), diesel vehicle emissions (15.9%), industrial processes (15.1%). For NOx, coal combustion (44.0%) and diesel vehicle emissions (35.2%) had the largest contribution, followed by industrial processes (12.5%) and gasoline vehicle emissions (8.3%). Based on PMF results and OBM, O3 source was analyzed used RIR method in this study, and industrial process (36.7%) and biogenic source (24.6%) were the major sources of O3. The sensitivities of O3 formation to these sources depend on if both VOC and NOx sensitivities are considered. Previous studies only considered the influence of VOCs on O3 formation when analyzing the source of O3, but this study indicated that the influence of NOx in industrial cities on O3 formation should not be ignored. Meanwhile, considering only VOCs but not NOx in the analysis of O3 sources will underestimate the emission proportion of anthropogenic sources and overestimate the proportion of biogenic sources, resulting in inaccurate results. Industrial cities are typical cities in transition areas, and the sensitivity of O3 to both VOCs and NOx should also be taken into account when analyzing the source of O3 in transition areas, which can ensure the accuracy of source analysis results. In addition, emission reduction of VOCs and NOx simultaneously should be considered in the control of O3 in transition areas. This study provides an improved direction for the source analysis of O3 in industrial cities and even cities in transition areas.

How to cite: Yan, Y., Niu, Y., Yue, K., Dong, J., Wu, J., Wang, Y., and Peng, L.: Formation sensitivity and source analysis of tropospheric ozone in a typical industrial city in China based on the observation data coupled with chemical mechanism, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6097, https://doi.org/10.5194/egusphere-egu25-6097, 2025.

EGU25-6691 | Posters on site | AS3.29 | Highlight

Alpha Release of the US Environmental Protection Agency’s Environmental Source Apportionment Toolkit (ESAT) 

Philip Hopke, Deron Smith, Michael Cyterski, John Johnston, Kurt Wolfe, and Rajbir Parmar

In environmental data analysis, source apportionment can be an important approach to extract useful information that might otherwise be hidden within the data. The United States Environmental Protection Agency (EPA) has developed an open-source python package, the Environmental Source Apportionment Toolkit (ESAT), which enables source apportionment modeling and error estimation workflows. ESAT is intended to replace Positive Matrix Factorization v5 (PMF5) that has substantial data size limitations. ESAT is currently in alpha testing with development plans for enhanced functionality and support of large datasets, High-performance Computing (HPC) execution through a command line interface (CLI), and a standalone desktop graphical user interface (GUI). The alpha product of ESAT is publicly available and offers a complete application programming interface (API) to replicate the workflows and functionality of PMF5, with examples provided through Jupyter Notebooks. The ESAT computing module currently contains two non-negative matrix factorization (NMF) algorithms for model training, with the module designed for other algorithms to be easily added. The two algorithms currently available are the least-squares NMF (LS-NMF) and weighted-semi NMF (WS-NMF). Each algorithm offers different benefits depending on project or data requirements. The ESAT python codebase has been optimized to run in a highly parallelized manner, with most of the numerical computations implemented in Rust, a low-level language comparable in performance to C. ESAT replicates the model error estimation methods of PMF5, namely bootstrap, displacement, and a hybrid method. To facilitate experimentation and testing, ESAT contains a synthetic dataset generator and model simulator that can evaluate how well ESAT can recreate synthetic factors and contributions. Continuous development of new features are tested and added to the python package on a regular basis. One such feature is the addition of an uncertainty perturbation workflow, which will run a collection of models while slightly perturbing the uncertainty matrix, and then evaluating the impact on the solution profiles and contributions. The alpha version of the ESAT python package is available for installation from pypi at https://pypi.org/project/esat/. Further testing and development of the alpha version will proceed to a full release in late 2025. The development of a GUI desktop application is currently planned to begin after the ESAT full release.

How to cite: Hopke, P., Smith, D., Cyterski, M., Johnston, J., Wolfe, K., and Parmar, R.: Alpha Release of the US Environmental Protection Agency’s Environmental Source Apportionment Toolkit (ESAT), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6691, https://doi.org/10.5194/egusphere-egu25-6691, 2025.

EGU25-7229 | ECS | Orals | AS3.29

Connecting Urban Black Carbon Emissions and Measured Concentrations: A Fusion of Hyperlocal Monitoring and Bayesian Techniques 

Chirag Manchanda, Robert Harley, Ronald Cohen, Ramon Alvarez, Tammy Thompson, Maria Harris, Julian Marshall, Alexander Turner, and Joshua Apte

Understanding urban air pollution at fine scales is essential for pinpointing emission sources that disproportionately impact vulnerable communities. Traditional emission inventories often suffer from insufficient spatial granularity and lack observational grounding, thus hampering effective source-specific interventions.

Here, we introduce a novel application of receptor-oriented models (RMs) for the hyperlocal source apportionment of black carbon (BC). By integrating a rich dataset from both dense mobile monitoring and temporally detailed fixed-site measurements into a Bayesian inversion framework using the WRF-STILT model, we quantify BC contributions in the community of West Oakland, CA, USA from diverse urban sources including on-road vehicles (notably diesel trucks), locomotives, port cargo-handling equipment, and maritime vessels, with a high spatial resolution of 150 meters (~0.02 km2). We reveal a wide variety of uninventoried neighborhood-scale emissions sources that substantially impact this overburdened community.

Our method employs a data-driven spatiotemporal model that combines both mobile and fixed-site data within a factor analysis framework, providing robust observational constraints for Bayesian inference. The robustness of our method is particularly notable given the uncertainties in prior emissions inventories. Moreover, we demonstrate that with only 10 strategically placed stationary sensors within a 15 km2 area, supplemented by time-averaged mobile measurements, reliable source apportionment can be achieved.

This study advances the methodology of RMs by providing a scalable and adaptable approach for incorporating hyperlocal measurements, providing critical insights into the effectiveness of these models in real-world urban scenarios. Future applications of the method would support observationally constrained strategies for fine-scale urban emissions tracking and community-centered air quality improvements.

How to cite: Manchanda, C., Harley, R., Cohen, R., Alvarez, R., Thompson, T., Harris, M., Marshall, J., Turner, A., and Apte, J.: Connecting Urban Black Carbon Emissions and Measured Concentrations: A Fusion of Hyperlocal Monitoring and Bayesian Techniques, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7229, https://doi.org/10.5194/egusphere-egu25-7229, 2025.

EGU25-7495 | ECS | Posters on site | AS3.29

Source Apportionment of Optical Properties of Carbonaceous Aerosols between Urban and Rural areas in Republic of Korea, spring 2022 

Seung Mee Oh, Junghee Kwon, Seung Ha Lee, Yong Pyo Kim, Chang Hoon Jung, and Ji Yi Lee

Light-absorbing carbonaceous aerosols (LACs) are key contributors to climate change due to their ability to absorb solar radiation and reduce surface albedo. These aerosols primarily comprise black carbon (BC) and brown carbon (BrC). The optical properties of LACs are influenced by a complex interplay of factors, including emission sources, atmospheric conditions, and secondary formation processes. However, clearly distinguishing the light-absorption characteristics of various sources remains a significant challenge. Instruments such as the Aethalometer, for example, can differentiate between BC from fossil fuel combustion and biomass burning based on the frequency dependency of absorption strength. Yet, the reliance on empirical values for the Absorption Ångström Exponent (AAE) introduces uncertainties in these estimates. Source apportionment models, such as Positive Matrix Factorization (PMF) and the Multilinear Engine (ME-2), help address these uncertainties by directly attributing sources through the integration of optical and chemical composition data (Wang et al., ACP, 2020). In this study, we applied the PMF model to quantify and compare the source-specific optical properties of carbonaceous aerosols in Chuncheon, a rural area surrounded by forests, and Seoul, a representative urban area in Republic of Korea, during the spring of 2022. The input data included ionic, carbonaceous, and elemental components, as well as light absorption coefficients measured using an Aethalometer (model AE33, Magee Scientific, United States) from March 14 to April 13, 2022. The PMF analysis identified four major sources; mineral dust, biomass burning, industrial emissions, and traffic emissions. Biomass burning was the largest contributor to light absorption in Chuncheon, whereas traffic emissions were the dominant contributor in Seoul. This trend was consistently reflected in the AAE and Mass Absorption Cross-section (MAC) values calculated for each source. This study provides new insights into the quantification of source-specific optical properties of aerosols using PMF, offering a robust approach to understanding their impacts on atmospheric radiative forcing.

How to cite: Oh, S. M., Kwon, J., Lee, S. H., Kim, Y. P., Jung, C. H., and Lee, J. Y.: Source Apportionment of Optical Properties of Carbonaceous Aerosols between Urban and Rural areas in Republic of Korea, spring 2022, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7495, https://doi.org/10.5194/egusphere-egu25-7495, 2025.

Ultrafine dust research is being conducted using the Positive Matrix Factorization (PMF) model to identify receptor-centered pollutants. Among the various chemical components used in the PMF model, trace elements such as heavy metals serve as indicators of pollutants emitted by industries. ICP-MS and XRF are used to analyze these trace elements. ICP-MS is the most widely used method for analyzing heavy metals and has a low detection limit, allowing it to analyze even trace concentrations. However, there are limits to reanalysis because it requires a complex sample pretreatment process and consumes samples. On the other hand, XRF has the advantage of being able to analyze samples without pretreatment and that reanalysis is possible at any time because the samples are not consumed. However, compared to ICP-MS, the detection limit is relatively high and the uncertainty increases when the amount is small. In this study, we sought to determine whether these differences in analysis methods affect the identification of industrial pollutants. The PMF model was performed by analyzing 107 PM2.5 filters collected at 4-day intervals from November 2021 to December 2022. The same analysis method was used for carbon and ion components, excluding trace elements. Through this study, we will be able to find out what differences the model results obtained through different analysis methods have in deriving industrial pollution sources. Additionally, it is expected that more reliable results will be obtained in accurate pollutant source estimation and weight determination.

Acknowledgement

This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute (KEITI) funded by the Ministry of Environment (MOE).

 

How to cite: Kim, M., Shin, H., and Lee, S.-M.: A comparative study of PM2.5 source apportionment and toxicological effects based on differences in heavy metal analysis methods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7532, https://doi.org/10.5194/egusphere-egu25-7532, 2025.

EGU25-7712 | ECS | Posters on site | AS3.29

Comparative Evaluation of Secondary Organic Aerosols in PM2.5 in Shenzhen Using Multiple Methodologies 

Xing Peng, Feng-Hua Wei, and Xiao-Feng Huang

Accurate quantification secondary organic aerosols (SOA) in ambient PM2.5 is crucial for addressing the current challenges in visibility improvement and further exploring the climate impacts of SOA. In this study, we conducted synchronous measurements of PM2.5 components in Shenzhen from November 1 to December 15, 2022, utilizing a suite of multiple online instruments, including high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS), semi-continuous OC/EC carbon aerosol analyzer, a monitor for aerosols and gases (MARGA), and a continuous multi-metals monitor (Xact-625). Three methods were employed for SOA in PM2.5 quantification, including AMS-PMF, Online-PMF, and the EC (elemental carbon) tracer method. The three methods yielded generally consistent SOA mass concentrations of 4.2 ± 3.2 μg m-3, 3.6 ± 2.6 μg m-3 and 3.5 ± 2.4 μg m-3, respectively. A strong correlation (r = 0.95) was found between AMS-PMF and Online-PMF results. While the EC tracer method showed lower consistency with AMS-PMF and Online-PMF, with correlation coefficients r of only 0.82 and 0.79, respectively. The AMS-PMF method determined that SOA accounted for 61.3 % of the organic mass (33.7% for more oxygenated organic aerosols, MO-OOA, and 27.6% for less oxygenated organic aerosols, LO-OOA), and the Online-PMF method estimated 57.0 %. However, the EC tracer method estimated only 50.5 %, primarily due to the higher uncertainty associated with SOA quantification in this method. The daily SOA variations from all three methods showed consistent peaks in the afternoon (14:00 ~ 15:00), and a significant rise at night. These patterns were attributed to increased photochemical activity in the afternoon and changes in boundary layer height at night. These analyses further support the reliability of the SOA quantification results in this study, encompassing both MO-OOA and LO-OOA.

How to cite: Peng, X., Wei, F.-H., and Huang, X.-F.: Comparative Evaluation of Secondary Organic Aerosols in PM2.5 in Shenzhen Using Multiple Methodologies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7712, https://doi.org/10.5194/egusphere-egu25-7712, 2025.

Volatile Organic Compounds (VOCs) could contribute to the formation of secondary organic aerosols and ozone, both of which are detrimental to human health and the environment. There has been growing interest in developing more precise methods for analyzing VOC sources, and Positive Matrix Factorization (PMF) is widely used. However, overlapping chemical compositions of the retrieved factor profiles often pose challenges in accurately distinguishing sources, even with high-resolution VOC data. While the role of organic compounds (OC) in enhancing PMF-based source apportionment of PM2.5 has been well-documented, studies integrating VOCs with organic molecular tracers remain limited. This study aims to integrate VOCs and organic molecular tracers into PMF analysis to improve the accuracy of source identification and quantification.

Hourly VOC monitoring and 12-hour integrated filter sampling were conducted during a 21-day period in summer at an industrial complex in southern Taiwan. A two-stage PMF modeling approach was applied, with the first stage focusing on VOC analysis and the second stage incorporating both VOC and OC markers. In Stage 1, seven factors were identified, with the three highest contributors attributed to Vehicle Gasoline Combustion (18%), Industrial Emissions (17%), and Synthetic Resin and Paints (16%). In Stage 2, after incorporating OC data, additional sources were identified, including biogenic emissions, cooking sources and  biomass burning, offering a more comprehensive source apportionment. These findings demonstrate that incorporating organic species can bridge gaps in VOC source apportionment, enhancing the resolution and accuracy of pollution source identification.

How to cite: Liu, Y.-H., Lai, K.-L., Chen, C.-Y., and Wu, C.-F.: Source Apportionment of Volatile Organic Compounds with Continuous Speciation Monitoring Data and Time-integrated measurements of Organic Markers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7769, https://doi.org/10.5194/egusphere-egu25-7769, 2025.

EGU25-9207 | ECS | Orals | AS3.29

Sparsity introduction in Bayesian Autocorrelation Matrix factorization for organic aerosol source apportionment 

Marta Via, Jure Demšar, Yufang Hao, Griša Močnik, and Kaspar R. Daellenbach

The Positive Matrix Factorisation (PMF) algorithm (Paatero and Tapper, 1994) has been the most widely used receptor model for a long time and has only recently been challenged with new methodologies. The novel Bayesian auto-correlated matrix factorisation method (BAMF, Rusanen et al. 2024) integrates an auto-correlation term emulating real-world pollutant sources time evolution has produced higher accuracy compared to PMF. However, both PMF and BAMF struggle to provide well-separated profiles manifested as mixed time series contributions.

 A sparsity-handling algorithm named horseshoe (HS) regularisation has beenapplied to BAMF in order to improve profile determination. The horseshoe application pushes some parameters to be close to zero and others to have large values (Piironen and Vehtari, 2017). The BAMF+HS method reduces the dimensionality of the problem by suppressing the non-significant species for each profile. The resulting profiles are expected to be less noisy and better representing the nature of the atmospheric pollution sources. Figure 1 shows the effect of BAMF+HS (in orange) compared to the regular BAMF (in blue) and the PMF (in green) on a toy dataset, consisting on an oversimplified dataset with very sparse profiles. The BAMF+HS results show contributions pushed to zero, making the profiles closer to the truth (in black) with respect to the less sparse results of BAMF and PMF. This same comparison has been carried out on realistic synthetic datasets to show the effectiveness of sparsity introduction into source apportionment.

Figure 1. Comparison to truth of source apportionment profiles resulting from three different receptor models for a toy dataset.

Acknowledgement: This work is supported by the European Union's Horizon Europe research and innovation programme under the Marie Skłodowska-Curie Postdoctoral Fellowship Programme, SMASH co-funded under the grant agreement No. 101081355. The SMASH project is co-funded by the Republic of Slovenia and the European Union from the European Regional Development Fund. K.R.D. acknowledges support by SNSF Ambizione grant PZPGP2_201992.

References

Piironen, J., & Vehtari, A. (2017). Sparsity information and regularization in the horseshoe and other shrinkage priors.

Rusanen, A., Björklund, A., Manousakas, M., Jiang, J., Kulmala, M. T., Puolamäki, K., & Daellenbach, K. R. (2023). Atmospheric Measurement Techniques Discussions2023, 1-28.

Paatero, P., & Tapper, U. (1994). Environmetrics5(2), 111-126.

How to cite: Via, M., Demšar, J., Hao, Y., Močnik, G., and Daellenbach, K. R.: Sparsity introduction in Bayesian Autocorrelation Matrix factorization for organic aerosol source apportionment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9207, https://doi.org/10.5194/egusphere-egu25-9207, 2025.

EGU25-9466 | ECS | Orals | AS3.29

Chemical Characterization and Source Apportionment of airborne PM2.5 at an urban site in Astana, Kazakhstan 

Gulden Ormanova, Philip Hopke, Dhawal Shah, and Mehdi Amouei Torkmahalleh

Atmospheric fine particulate matter (PM2.5), a complex mixture of various chemical species, has emerged as a significant air quality issue in urban areas. PM2.5 is a key factor in harmful health effects, significantly contributes to the disease burden, plays a significant role in atmospheric visibility and climate change. These tiny particles can scatter and absorb sunlight, leading to haze and reduced visibility, especially in urban areas. Additionally, some components of PM2.5, like Black Carbon (BC), can contribute to global warming by absorbing heat in the atmosphere.

Central Asia is home to several republics that have been striving for independent development over the past 25 years. Kazakhstan is probably the most advanced of these countries as well as the largest in area. It is rich in mineral resources, particularly fossil fuels and thus, has relied primarily on coal for its heating, electricity generation, and industrial base operations. Its air quality is not well characterized to the rest of the world since governmental monitoring data are not publicly available and few prior studies of the amounts or sources of particulate matter have been published.

Currently, the capital Astana has become one of the most polluted cities. Thus, this work that provides almost two years of compositional data and source contributions provides an initial assessment of particulate air quality in Astana. This initial study thoroughly investigates the chemical compositions and source apportionment of PM2.5 based on elements, ions, BC, and estimated UMM, due to the lack of organic carbon data from the samples. Source apportionment was obtained by the U.S. EPA’s Positive Matrix Factorization (PMF) (v5.0) receptor model and Conditional Bivariate Probability Function (CBPF) analyses. Identified source types and average contribution to PM2.5 were ‘Spark Ignition’, ‘Coal Flyash’, ‘Secondary Nitrate’, ‘Primary Sulfate-Fuel Combustion’, ‘Secondary Sulfate-Coal Combustion’, ‘Soil/Road Dust’, ‘Diesel’, and ‘Local Power Plant(s)’. Carbonaceous matter, sulfates, and nitrates account for a significant PM2.5 fraction since power plants burn high-ash coal and fuel oil year-round in Astana city. The major contributions are heating power plants (CHPP-1 and CHPP-2), private residential chimney heating systems, autonomous boilers, vehicles, and local construction activities.

Kazakhstan recently declared its intent to decarbonize by 2030 and achieve carbon neutrality by 2060 that should substantially improve air quality. This study will thus provide baseline data against which future apportionment studies can be compared.

 

 

How to cite: Ormanova, G., Hopke, P., Shah, D., and Torkmahalleh, M. A.: Chemical Characterization and Source Apportionment of airborne PM2.5 at an urban site in Astana, Kazakhstan, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9466, https://doi.org/10.5194/egusphere-egu25-9466, 2025.

EGU25-10883 | ECS | Posters on site | AS3.29

Source attribution of fine particulate matter in European cities for different meteorological years 

Anthony Rey-Pommier, Enrico Pisoni, Philippe Thunis, Stefano Zauli-Sajani, and Alexander de Meij

Ambient fine particulate matter (PM2.5) poses a significant risk to health in Europe, where many cities are exposed to levels above World Health Organization guidelines. To support the implementation of optimal PM2.5 reduction policies, air quality models are necessary. In such context, source-receptor relationships (SRRs) are models that can be used to replace fully-fledged Chemical Transport models, and save significant computation time when simulating various emission reduction scenarios. They allow calculating the relative potential of a given source at a receptor, i.e. the share of PM2.5 concentration at a given receptor that results from the complete removal of the emissions from that source. Here, we use the SRR model SHERPA, based on the EMEP Chemical Transport Model for four different meteorological years (2015, 2017, 2019 and 2021), to evaluate relative potentials for 150 European cities. These potentials are evaluated for five different emission precursors, twelve emission sectors, and four reduction scopes (city core, commuting zone, remaining national territory and rest of Europe). Results show that relative potentials vary little between meteorological years for most cities. The industry, transport and residential sectors generally bear the highest values of relative potential for most cities through emissions of primary particulate matter. Cities near important ports where the shipping sector exhibits high values through sulfur oxides. High potentials are observed for agriculture at the national and international scales. Cities in Southern Europe have low reduction potentials due to high PM2.5 levels originating from natural sources. Smaller cities have a higher relative potential for national and international emissions, while larger cities have high relative potentials for city core emissions. Relative potentials are generally low for commuting zones. These results underline the reliability of SRRs in guiding targeted air quality interventions, thereby helping to reduce PM2.5 exposure effectively across diverse urban settings in Europe.

How to cite: Rey-Pommier, A., Pisoni, E., Thunis, P., Zauli-Sajani, S., and de Meij, A.: Source attribution of fine particulate matter in European cities for different meteorological years, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10883, https://doi.org/10.5194/egusphere-egu25-10883, 2025.

EGU25-11663 | Posters on site | AS3.29

The inclusion of photochemical initial concentrations in the combined-phase source apportionment of PM2.5, PAHs and VOCs from an industrialized environment 

Uwayemi Sofowote, Ewa Dabek-Zlotorzynska, Mahmoud Yassine, Dennis Mooibroek, May Siu, Valbona Celo, and Philip Hopke

PM2.5 species, PAHs and VOCs were sampled between 2013 and 2019 once every three or six days for a period of 24 hours in an industrialized city in Ontario, Canada, and analyzed to apportion their common sources. The consequences of using these species jointly for receptor modelling were assessed via combined-phase source apportionment that used the data as is, and in an approach that considered the potential for photochemical losses of gas-phase species. Thus, initial concentrations corrected for photochemistry, called PIC were calculated. The data were then analyzed either with positive matrix factorization or its dispersion-normalized variant (DN-PMF). Comparisons of applying PMF to the originally observed input data (BASE) and DN-PMF on data with PIC corrections were made. When the combined phase input data were analyzed, nine factors were resolved for both BASE and DN-PIC PMF. These factors were: particulate sulphate, secondary organic aerosol (SOA), particulate nitrate (pNO3), biomass burning with natural gas, crustal matter, winter blend of gasoline, coking/coal combustion, steelmaking, and summer blend/light duty vehicular emissions. On comparison of the BASE and DN-PIC PMF results, the average PM mass contribution of the summer gasoline fuel factor increased from 2% in BASE case to 5%, suggesting severe underestimation of this source’s initial contributions without DN-PIC. Also, substantial increases of reactive VOCs in the SOA factor, and PAHs with ≥four rings in the pNO3 and steelmaking factors were observed with DN-PIC PMF compared to the BASE PMF case, indicating that for the SOA factor, reactive VOCs at the location of study contributed to its sources.

How to cite: Sofowote, U., Dabek-Zlotorzynska, E., Yassine, M., Mooibroek, D., Siu, M., Celo, V., and Hopke, P.: The inclusion of photochemical initial concentrations in the combined-phase source apportionment of PM2.5, PAHs and VOCs from an industrialized environment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11663, https://doi.org/10.5194/egusphere-egu25-11663, 2025.

EGU25-13996 | ECS | Posters on site | AS3.29

Hourly chemical composition and source apportionment of PM in industrial and mining areas of SW Europe using a near real-time technique 

Pablo Pérez-Vizcaíno, Ana M. Sánchez de la Campa, Daniel Sánchez-Rodas, Jesús D. de la Rosa, Andrés Alastuey, and Xavier Querol

Industrial and mining activities are important anthropogenic sources of metals and metalloids in the air. Traditionally, 24-h offline sampling of particulate matter (PM) is considered and chemical composition is determined by ICP-MS and ICP-OES analysis. In recent years, near real-time techniques have been developed that allow high time resolution (1-h) studies to be carried out. An example is the Xact 625i Ambient Metals Monitor, based on reel-to-reel filter tape sampling followed by nondestructive X-ray fluorescence analysis.

Our study presents the results of metals and metalloids sampling and analysis with Xact 625i over three years at three stations in a southwestern region of Europe with urban-industrial (Campus, Pérez-Vizcaíno et al., 2025), industrial (La Rabida) and mining (La Dehesa de Riotinto) influence. The high concentrations were associated with channeled and fugitive emissions from different sources: copper smelter, Port of Huelva, oil refinery, and/or open-pit mining. At the three stations, the daily, weekly and annual variation patterns of each element were obtained. Hourly As peaks in PM10 of up to 311 ng m-3 in the city of Huelva, 292 ng m-3 in La Dehesa de Riotinto and in PM2.5 of up to 578 ng m-3 in La Rabida were measured. The application of the Positive Matrix Factorization (PMF v5.0 EPA) model made it possible to identify sources and the contribution of each of them, showing the relevance of industrial and mining activities throughout the day.

This work highlights the need to conduct high time resolution studies to understand the hourly behavior of different pollutants and their correlation with meteorological parameters, complement air quality models, and better understand the impacts of atmospheric pollution on public health.

 

References

Pérez-Vizcaíno, P., Sánchez de la Campa, A.M., Sánchez-Rodas, D., de la Rosa, J.D., 2025. Application of a near real-time technique for the assessment of atmospheric arsenic and metals emissions from a copper smelter in an urban area of SW Europe. Environmental Pollution 367, 125602. https://doi.org/10.1016/j.envpol.2024.125602.

How to cite: Pérez-Vizcaíno, P., Sánchez de la Campa, A. M., Sánchez-Rodas, D., de la Rosa, J. D., Alastuey, A., and Querol, X.: Hourly chemical composition and source apportionment of PM in industrial and mining areas of SW Europe using a near real-time technique, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13996, https://doi.org/10.5194/egusphere-egu25-13996, 2025.

Assessing the site-to-site variability of source contributions to the ambient PM2.5 concentrations plays an important role in estimation of exposure misclassification in epidemiological studies. Exposure misclassification error may be substantially lowered when accounting for the heterogeneity of source contributions resulting in a lower relative risk evaluation.

The aims of this study were to identify the common pollution sources and their contributions from the PM2.5 compositional data collected during the two sampling campaigns (2012/13 and 2018/19) of the Multiple Air Toxics Study (MATES) at ten sites across the South Coast Air Basin using positive matrix factorization and to characterize the spatial variations among the source contributions by coefficients of determination and divergence.

The results of the study showed that the major common contributor to the PM2.5 mass at all sampling sites was the “gasoline vehicle” source followed by “aged sea salt”, “biomass burning”, “secondary nitrate”, “secondary sulfate”, “diesel vehicles”, “soil/road dust” and “OP-rich”. The contribution patterns of all eight sources were highly heterogeneous over time. Among them, the highest spatial variability was found for the contributions from “OP-rich” source in both MATES campaigns suggesting the different wildfire contributions that occurred in the region. Alternatively, the smallest spatial site diversities were observed for the highly correlated contributions of the “secondary sulfate” and “aged sea salt” sources obtained from the MATES data collected in 2012/13 and for the “soil/road dust” sources from 2018/19 campaign. Overall, the source contributions obtained for Inland Valley and Rubidoux were the most different in comparison to the other sites likely due to their distant location from the Pacific Ocean and the major industrial region in Los Angeles.

How to cite: Stanimirova, I. and Hopke, P. K.: Assessment of spatial variability in PM2.5 source contributions during two sampling campaigns (2012/13 and 2018/19) across ten sites in the South Coast Air Basin, California, the USA., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14163, https://doi.org/10.5194/egusphere-egu25-14163, 2025.

EGU25-15427 | ECS | Posters on site | AS3.29

BTEX in Urban Air: Source Apportionment, Seasonal Trends, and Health Risk Assessment Across Three Western Indian Metropolitan Cities  

Vrinda Anand, Anoop P Sreevalsam, Bhagyashri Katre, Abhilash S Panicker, and Sachin D Ghude

The air pollutant compounds BTEX (Benzene, Toluene, Ethylbenzene, and Xylenes) have emerged as significant urban air pollutants, raising increasing environmental and health concerns. This study presents a comparative analysis of BTEX concentrations across three major metropolitan cities in Western India; Pune, Mumbai, and Ahmedabad. A clear seasonal pattern has been observed in BTEX concentrations across all three cities, with peak levels observed during winter and post-monsoon seasons. The spatial distribution revealed that Mumbai and Pune exhibited the highest concentrations of Benzene, Ethylbenzene, and Xylenes, while Toluene was highest in Ahmedabad. Source apportionment using interspecies ratios identified vehicular emissions as the primary contributor of BTEX at all locations. Notably, Mumbai's higher Benzene/Toluene ratios (>0.5) suggested long-range transport of these pollutants. Further analysis using interspecies correlations showed strong relationships (correlation coefficient >0.7) between all BTEX parameters in Pune and Mumbai, supporting common emission sources. The health risk assessment quantified through Lifetime Cancer Risk (LCR) calculations indicated that BTEX exposure levels were below both the prescribed cancer risk threshold of 10⁻⁴ and the US-EPA recommended limit of 10⁻⁶ across all study locations. These findings provide valuable insights into the distribution patterns, potential sources, and health implications of BTEX pollutants in Western Indian urban environments.

How to cite: Anand, V., P Sreevalsam, A., Katre, B., Panicker, A. S., and Ghude, S. D.: BTEX in Urban Air: Source Apportionment, Seasonal Trends, and Health Risk Assessment Across Three Western Indian Metropolitan Cities , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15427, https://doi.org/10.5194/egusphere-egu25-15427, 2025.

This study focuses on PM2.5 pollution in the Taichung Metropolitan Area, Taiwan, with an emphasis on the application of an advanced PMFxPMF method for detailed source identification. Initial Positive Matrix Factorization (PMF) analysis identified six major pollution sources, including regional secondary pollution (41%), carbonaceous aerosols (24%), and Heavy metal-rich industrial processes (8%). To refine the attribution of industrial sources, a second-phase PMFxPMF analysis was employed, specifically targeting heavy metals within the industry factor. By integrating source fingerprints from chimney samples of coal combustion and sintering furnaces, the analysis revealed that these sources contributed 18.4% and 4.9%, respectively, to the total heavy metals in the industry factor. When excluding Fe, the contributions increased to 35.5% and 8.4% for non-Fe heavy metals. The application of the PMFxPMF method was crucial in accurately linking specific industrial activities to heavy metal emissions, offering a more precise understanding of pollution sources. These insights are essential for developing targeted strategies to reduce PM2.5 levels and mitigate the associated health risks in the Taichung region, particularly through stricter control of emissions from coal combustion and metal processing industries.

How to cite: Sun, S. S.-E. and Chou, C. C.-K.: Observation-based investigation unveils major local sources of heavy metals associated to fine particulate matters (PM2.5) in an urban area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15558, https://doi.org/10.5194/egusphere-egu25-15558, 2025.

EGU25-15834 | ECS | Orals | AS3.29

Traditional and new Approaches in Source Apportionment: A Critical Evaluation of Bias and Limitations 

Mohamed Gherras, Jean-Eudes Petit, Alicia Gressent, Caroline Marchand, Augustin Colette, Valerie Gros, and Olivier Favez

Source apportionment is a cornerstone in environmental sciences, providing essential insights into the contributions of diverse pollution sources to ambient air quality. Understanding these contributions is vital for designing effective regulatory and mitigation strategies. Among the most commonly employed techniques for source apportionment, Positive Matrix Factorization (PMF) has proven to be a powerful receptor model. PMF decomposes complex environmental datasets into source profiles and their corresponding contributions while accommodating measurement uncertainties Hopke [2016], Paatero and Tapper [1994]. Despite its advantages, PMF is not without limitations, such as rotational ambiguity, reliance on accurate input uncertainties, and potential biases in source attribution Reff et al. [2007].

In recent years, the emergence of artificial intelligence (AI)-based methodologies has opened new horizons for source apportionment. These approaches often build upon classical methods like PMF, aiming to enhance the interpretability and performance of source apportionment models Geng et al. [2020]. Machine learning techniques, including deep learning, leverage large datasets to identify patterns and relationships that may elude traditional approaches. Additionally, hybrid methods integrating classical models with AI frameworks have demonstrated potential for improved accuracy and robustness Wang et al. [2021].

A critical question remains unanswered: do the intrinsic limitations of PMF, such as biases and errors, propagate into these AI-driven alternatives? For instance,  AI methods are theoretically capable of overcoming such challenges, their reliance on data-driven training may introduce new sources of bias or amplify existing uncertainties if the underlying data or assumptions are flawed.
Moreover, how do these biases compare to those in other receptor models, such as the Chemical Mass Balance (CMB) model ?

This work aims to look on the extent to which the errors and biases inherent to PMF are inherited by alternative methods, including AI-based approaches and other receptor models. By critically assessing these methods, we seek to provide a comprehensive understanding of the strengths and limitations of emerging tools for source apportionment and their potential to overcome traditional challenges.

 

Xiaoyu Geng, Lin Zhang, and Yu Wang. Ai-based approaches for source apportionment in atmospheric science: A review and perspective. Atmospheric Environment, 223: 117276, 2020. doi: 10.1016/j.atmosenv.2020.117276.

 

Philip K. Hopke. Review of receptor modeling methods for source apportionment. Journal of the Air Waste Management Association, 66(3):237–259, 2016. doi: 10.1080/10962247.2016.1140693.

Pentti Paatero and Unto Tapper. Positive matrix factorization: A non-negative factor model with optimal utilization of error estimates of data values. Environmetrics, 5(2): 111–126, 1994. doi: 10.1002/env.3170050203.

 

Adam Reff, Sierra I. Eberly, and Prakash V. Bhave. Receptor modeling of ambient particulate matter data using positive matrix factorization: Review of existing meth- ods. Journal of the Air Waste Management Association, 57(2):146–154, 2007. doi: 10.1080/10473289.2007.10465319.

Feifei Wang, Hui Zhang, and Xiaodong Li. Hybrid receptor models and machine learning for air pollution source apportionment: Advances and future directions. Environmental Research, 195:110827, 2021. doi: 10.1016/j.envres.2021.110827.

 

John G. Watson. Chemical mass balance receptor model methodology for assessing the sources of fine and coarse particulate matter. Environmental Software, 5(2):38–49, 1990. doi: 10.1016/0266-9838(90)90008-

 

How to cite: Gherras, M., Petit, J.-E., Gressent, A., Marchand, C., Colette, A., Gros, V., and Favez, O.: Traditional and new Approaches in Source Apportionment: A Critical Evaluation of Bias and Limitations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15834, https://doi.org/10.5194/egusphere-egu25-15834, 2025.

PM2.5 consists of  various chemical constituents originating from multiple sources and is associated with adverse health effects, including cardiovascular and respiratory diseases. Effective source specific management strategies are essential for mitigating these impacts. Positive Matrix Factorization (PMF) has been widely used as a receptor model to identify sources and quantify their contributions. However, conventional PMF (C-PMF) often overestimates or underestimates source contributions due to meteorological influences. To address this limitation, the Dispersion-Normalized PMF (DN-PMF) model has been introduced. This advanced approach accounts for meteorological conditions, providing more accurate source contributions.

In this study, hourly data for 28 chemical constituents of PM2.5, measured from 2019 to 2022 at National Intensive Monitoring Stations (NIMS) in Daejeon and Gwangju, South Korea, were used as input data for both C-PMF and DN-PMF. The study aimed to identify sources whose contributions are significantly influenced by meteorological factors and to compare regional variations.  Ten sources were resolved by both models in each city, and differences in source contributions between the two approaches were calculated. Seasonal and temporal variations were also examined to determine meteorologically influenced sources and regional differences.

In Daejeon, a significant difference in secondary nitrate contributions was observed between the models, particularly during winter, when the atmospheric conditions favor its formation. In contrast, contributions of secondary sulfate showed minimal differences, suggesting it is primarily affected by long-range transport and less sensitive to local meteorological conditions.  In Gwangju, secondary nitrate and sulfate contributions showed relatively small differences, indicating lower sensitivity to local meteorological factors. Additionally, differences in contributions were observed for sources influenced by local emissions, highlighting variations between the two regions, for the same sources. These regional differences are likely attributable to the specific emission characteristics, meteorological conditions, and sources locations of each city. Supporting data, including emission inventories, meteorological parameters, and the Conditional bivariate probability function (CBPF) were used to explain the observed variations. This study underscores the influence of local meteorological conditions on source contributions and provide valuable insights for developing region-specific PM2.5 management strategies.

Acknowledgement

This research was supported by “Study on the analysis of medium- and long-term factors affecting PM2.5 emission changes” funded by National Air Emission Inventory and Research Center of the Ministry of Environment under grant, South Korea. This work was supported by the National Institute of Environmental Research (NIER) of the Ministry of Environment under grant, South Korea No. NIER-2021-03-03-001. This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute (KEITI) funded by the Ministry of Environment (MOE).

How to cite: Kim, T., Han, S., Ryoo, I., Rim, D., Kim, M., and Yi, S.-M.: Influence of local meteorological conditions on source contributions of PM2.5: A comparison of Conventional Positive Matrix Factorization (C-PMF) and Dispersion Normalized PMF (DN-PMF) models in Daejeon and Gwangju, South Korea. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16131, https://doi.org/10.5194/egusphere-egu25-16131, 2025.

EGU25-16605 | Posters on site | AS3.29

Trend Analysis of PM2.5 Source Contributions in Seoul and Ulsan, South Korea (2016-2022) 

Seung-Muk Yi, Taeyeon Kim, Sujung Han, Ilhan Ryoo, and Moonkyung Kim

PM2.5, identified as a health-hazardous substance and classified as a Group 1 carcinogen by the International Agency for Research on Cancer in 2013, poses significant risks to public health.  To combat these risks, the South Korean government established the ambient air quality standard for PM2.5 mass concentration through the Air Quality Preservation Act in 2013, initially implemented in Seoul and expanded nationwide in 2015. Since December 2019, the Seasonal Management Program has targeted major PM2.5 sources during winter (December–March), a period of frequent high concentration events. While these measures initially achieved notable reductions, the downward trend in PM2.5 mass concentration has slowed in recent years. In 2022, South Korea recorded an annual average PM2.5 mass concentration of 18.3 μg/m³, exceeding the national air quality standard of 15 μg/m³.

This study aimed to analyze long-term trends in PM2.5 source contributions using the meteorologically adjusted Dispersion-Normalized Positive Matrix Factorization (DN-PMF) model. Hourly monitoring data from 2016 to 2022, provided by the National Institute of Environmental Research (NIER), were analyzed for two sites: Seoul, the capital city, and Ulsan, an industrial hub. The dataset included PM2.5 mass concentrations, carbonaceous components (OC, EC), ionic species (NO3-, SO42-, Cl-, NH4+, Na+, K+), and trace elements (S, K, Si, Al, Ca, Ti, V, Cr, Mn, Fe, Ni, Cu, Zn, As, Se, Br, Ba, Pb). The Conditional Bivariate Probability Function (CBPF) model was utilized to identify the direction of local sources. Comprehensive trend analyses, including Theil-Sen regression, Seasonal Trend Decomposition based on LOESS (STL), and Piecewise Regression, were conducted to assess variations in source contributions over time.

This study resolved 10 sources through PMF modeling at each site: secondary sulfate, secondary nitrate, motor vehicles, biomass burning, incineration, oil combustion, coal combustion, soil, industry, and sea salt. Temporal variations revealed differing trends between the two sites. In Seoul, PM2.5 mass concentrations consistently decreased, with significant reductions in contributions from incineration, oil combustion, and industry sources. In contrast, Ulsan exhibited a more rapid decline in PM2.5 mass concentrations particularly for biomass burning and oil combustion sources. Addressing secondary sulfate and mobile sources remains critical for further air quality improvements.

This study provided essential receptor-based evidence to support the development of future air quality management strategies, addressing both local and transboundary PM₂.₅ sources effectively.

Acknowledgment

This research was supported by “Study on the analysis of medium- and long-term factors affecting PM2.5 emission changes” funded by the National Air Emission Inventory and Research Center of the Ministry of Environment under grant, South Korea. This work was supported by the National Institute of Environmental Research (NIER) of the Ministry of Environment under grant, South Korea No. NIER-2021-03-03-001. This research was supported by the Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute (KEITI) funded by the Ministry of Environment (MOE).

How to cite: Yi, S.-M., Kim, T., Han, S., Ryoo, I., and Kim, M.: Trend Analysis of PM2.5 Source Contributions in Seoul and Ulsan, South Korea (2016-2022), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16605, https://doi.org/10.5194/egusphere-egu25-16605, 2025.

EGU25-16932 | Posters on site | AS3.29

Source Apportionment of PM2.5 in Southeast Asia: Bangkok, Thailand, and Jakarta, Indonesia 

Sujung Han, Taeyeon Kim, Minsoo Kang, Jaewook Hwang, Yein Kim, Kraichat Tantrakarnapa, Santoso Muhayatun, Donghyun Rim, Moonkyung Kim, and Seung-Muk Yi

Air pollution was responsible for 8.1 million deaths globally in 2021, making it the second leading risk factor for mortality (5th edition of the SoGA report, 2021). Among air pollutants, PM2.5, airborne particles with an aerodynamic diameter of 2.5 μm or less, is particularly harmful, as it penetrates deeply into the alveoli and can reach the respiratory and cardiovascular system, exacerbating diseases such as asthma, lung cancer, and heart arrhythmia. In Southeast Asia, PM2.5 mass concentrations have risen over the decades due to rapid urbanization, industrial activities, and biomass burning.  This study aims to identify the sources of PM2.5 and quantify their contributions in Bangkok, Thailand, and Jakarta, Indonesia.

PM₂.₅ samples were collected from rooftop sites in both cities over 24-hour intervals every third day from September 2023 to December 2024, using three types of filters (Teflon, Quartz, Nylon). PM2.5 mass concentrations were measured using Teflon filters with an automatic weighing system. Trace elements, including Cl, Al, Ca, Cr, Cu, Fe, K, Mg, Mn, Pb, Si, Ti, V, Zn, Ni, As, S, Se, Ba, and Br, were analyzed using Energy Dispersive X-ray Fluorescence (ED-XRF). Carbonaceous components (OC, EC) were measured with an OC/EC analyzer on Quartz filters, while ionic species (NO3-, SO42-, Cl-, NH4+, Na+, and K+) were analyzed using Ion Chromatography on Nylon filters.

The Positive Matrix Factorization (PMF) model was applied to identify and quantify PM2.5 sources and the Conditional Bivariate Probability Function (CBPF) model was used for the directional analysis of PM2.5 sources.  Seasonal variations in PM2.5 mass concentrations were examined by comparing wet and dry seasons, providing insights into seasonal differences. Additionally, chemical constituent concentrations and proportions were analyzed at each site to identify site-specific characteristics. The contributions of sources were quantified, and the study further explored the directions of local sources and geographical influences. The findings of this study provide critical scientific evidence for the development of policies to manage ambient PM2.5, aiming to improve air quality while balancing economic and social considerations.

Acknowledgment

This research was supported by “Clean Air for Sustainable ASEAN (CASA)” funded by the ASEAN Korea Cooperation Fund (AKCF). This research was supported by the Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute (KEITI) funded by the Ministry of Environment (MOE). 

How to cite: Han, S., Kim, T., Kang, M., Hwang, J., Kim, Y., Tantrakarnapa, K., Muhayatun, S., Rim, D., Kim, M., and Yi, S.-M.: Source Apportionment of PM2.5 in Southeast Asia: Bangkok, Thailand, and Jakarta, Indonesia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16932, https://doi.org/10.5194/egusphere-egu25-16932, 2025.

EGU25-17471 | ECS | Orals | AS3.29

New approach to real-time analysis of multi-site Volatile Organic Compound (VOC) observation data from an industrial zone in the South of France 

Zahra Benmouhoub, Liselotte Tinel, Grégory Gille, Céline Cancedda, Stéphane Sauvage, and Nadine Locoge

Volatile Organic Compounds (VOCs), from anthropogenic or biogenic sources, participate in the formation of ozone and particulate matter (PM), impacting health, climate, and ecosystems. They can also be directly harmful, in particular anthropogenic VOCs such as vinyl chloride monomer (chloroethene), benzene or 1-3-butadiene, that are carcinogenic.1 In the southern region of France, the French thresholds for ozone (240 µg m³ hourly) and for PM2.5 (10 µg m³ annual) are regularly exceeded. A 2018-study showed an exceedance for O3 on 144 days and for PM on 28 days during a 14 month period.2 These exceedances contributed to over 1,800 hospitalizations in the region from 2010 to 2019.3

To better understand the drivers behind these exceedances and anticipate the population’s exposure, a detailed study in an impacted industrial area is conducted. The study area is located in the south of France, around a brackish lake called the Étang de Berre. This area includes three major industrial complexes (Berre l'Étang, Martigues Lavéra and Port-de-Bouc), where major metallurgical and petrochemical industries are located, known to be high emitters of VOCs. Notably, the region has a high industrial density, with 56 SEVESO high-threshold sites and the Fos/Berre zone presenting the second largest site concentration in France. Further, a petrochemical plant in Lavéra is particularly noteworthy, as it produces 25% of France's chlorine and 40% of its vinyl chloride monomer (VCM).4 The region's VOC dynamics are influenced by the orography and specific meteorological conditions, particularly a regime of land and sea breezes, that advects relatively clean marine air during the nighttime. In this complex region, three observation stations, run by the local air quality organization AtmoSud are monitoring continuously the concentrations of 68 VOCs since January 2022. The stations are installed in strategic locations close to the industrial complexes and in a residential area in proximity of school.

The observations reveal distinct behaviors for specific VOCs, that show a transient variability with very high intensity peaks. For example, at the Berre l’Etang station, cyclohexane exhibits baseline concentrations below 50 µg m-³, punctuated by peaks reaching up to 218 µg m-³. Similarly, VCM concentrations are typically below 20 µg m-³, with occasional spikes up to 600 µg m-³. For other VOCs, such as ethane and acetylene, more stable levels are observed following regional dynamics. We use a source-receptor approach to better characterize the sources of VOCs in this challenging area and developed an online uncertainty tool to ensure quality-controlled entry data for the Positive Matrix Factorization (PMF).  Preliminary results reveal notable chemical signatures, including a pronounced cyclohexane profile and an aromatic profile, we attributed to emissions from the industrial platform northeast of the monitoring station. Further source apportionment results, including seasonal trends, will be discussed.

References:

(1) Report: 1,3-Butadiene, Ethylene Oxide and Vinyl Halides, (IARC, Lyon, 2008).

(2) Chazeau, B. et al.. Atmospheric Chem. Phys. 21, 7293–7319 (2021).

(3) Khaniabadi, Y. O. & Sicard, P. A Chemosphere 278, 130502 (2021).

(4) KEM ONE - Site KEM ONE de Lavéra. https://www.kemone.com/A-propos/Implantations/Lavera.

How to cite: Benmouhoub, Z., Tinel, L., Gille, G., Cancedda, C., Sauvage, S., and Locoge, N.: New approach to real-time analysis of multi-site Volatile Organic Compound (VOC) observation data from an industrial zone in the South of France, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17471, https://doi.org/10.5194/egusphere-egu25-17471, 2025.

EGU25-19384 | Posters on site | AS3.29

Aerosol source apportionment in two contrasting Italian sites: a comparison between physical and chemical PMF in Aosta and Lecce  

Caterina Mapelli, Daniele Contini, Henri Diémoz, Adelaide Dinoi, Daniela Cesari, and Francesca Barnaba

Positive Matrix Factorization (PMF) is a powerful method for the apportionment of aerosol sources. Traditionally applied to chemical datasets, it has more recently been extended to physical datasets, focusing predominantly on size distributions of ultra-fine particles (Hopke et al., 2022). In this study, aerosol physical properties (particle size distributions, from ultrafine to coarse mode, and spectral aerosol absorption) were used as input to PMF (EPA 5.0) for identifying emission sources of two distinct sites, and results compared with those from chemical PMF. 

Located at the two extremes of the Italian territory, the sites of Aosta and Lecce represent two markedly different environments. The first lies in the mountainous area of the northwestern Alps, the second in a flat area at the southeastern edge of the peninsula, in a typical Mediterranean context. In previous studies, PMF of aerosol chemical composition was performed using chemical speciation of PM over the period 2019-2021 (Aosta, e.g. Diemoz et al., 2019) and 2017 (Lecce, Giannossa et al., 2022).  

The PMF input dataset at the urban-background site in Aosta included aerosol size distributions measured by an Optical Particle Counter (OPC) across the 0.18–18 µm range and wavelength-dependent aerosol absorption from an AE33-aethalometer. At the urban-background observatory in Lecce, an aerosol size distribution range (0.02–10 µm) was available using both a Scanning Mobility Particle Sizer (SMPS) and an OPC, complemented by single-wavelength aerosol absorption (Multi-Angle Absorption Photometer, MAAP) providing eBC concentrations. Ancillary data included meteorological parameters and trace-gases concentration. Although with differences in the physical properties used, at both sites the physical PMF allowed the identification of 6 aerosol sources. In Aosta, the aerosol sources included fossil fuel combustion, biomass burning, secondary droplet mode, secondary condensation, dust, and coarse particles. In Lecce, the sources were nucleation (thanks to the additional use of the SMPS), traffic emissions, secondary nitrate, secondary sulfate, regional transport (sea spray and dust), and local resuspension (coarse particles). 

The work will present a comparison of the two PMF approaches (Chemistry- and Physics-based PMF) and advantages and limits of the different physical input datasets used at the two sites. For example, at the Lecce site, the information on ultrafine and fine particle distribution well captured features of the nucleation and traffic factors, while the absence of wavelength-dependent absorption coefficients limited the ability to distinguish biomass burning from fossil fuel sources, which was key for Aosta. Overall, the use of physical aerosol data as input to PMF proved to be an effective method for source apportionment and could usefully complement the chemical-PMF analysis. In fact, this approach offers significant advantages, such as the capability for quasi real-time monitoring and the relative ease of instruments use and data analysis compared to the ‘traditional’ chemical analysis of PM. 

The authors acknowledge the MUR for funding the research through the CIR01_00015-PER-ACTRIS-IT. 

 

Diémoz, H.et al., https://doi.org/10.5194/acp-19-10129-2019, 2019.  

Giannossa, L. et al., http://doi.10.1016/j.jenvman.2022.115752, 2022. 

Hopke, P. K. et al., https://doi.org/10.1016/j.scitotenv.2022.153104, 2022. 

How to cite: Mapelli, C., Contini, D., Diémoz, H., Dinoi, A., Cesari, D., and Barnaba, F.: Aerosol source apportionment in two contrasting Italian sites: a comparison between physical and chemical PMF in Aosta and Lecce , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19384, https://doi.org/10.5194/egusphere-egu25-19384, 2025.

The air quality in the Indian subcontinent has been a growing concern in recent years, with particulate matter (PM) being one of the major pollutants. PM2.5, in particular, has a significant impact on human health and the environment as it can penetrate deep into the respiratory system. PM2.5 has been linked to several health issues including respiratory and cardiovascular disease, while Water-Soluble inorganic Ions (WSII) contribute to the acidity and salinity of the air. In this study, we aim to investigate the seasonal variation and contributing sources of PM2.5 and 9 associated WSII (Na+, NH4+, K+, Mg2+, Ca2+, F-, Cl, NO3 and SO42−) in two non-attainment Indian cities, Alwar and Amritsar in the states of Rajasthan and Punjab respectively. The study regions are selected owing to the unique meteorological conditions, population density and industrial activities. The study employs a combination of field measurements and comparative analysis to understand the sources and seasonal patterns of PM2.5 and WSII in these cities. Initial analysis of PM2.5 winter samples shows Nitrate (22.078 μg/m3) and Sulphate (17.408 μg/m3) to be the dominant anionic species and Ammonium (13.046 μg/m3) and Sodium (5.452 μg/m3) to be dominant cationic species for both day and night respectively in Alwar city. The total average day anionic concentrations for the same period were observed to be 31.37 μg/m3 and night concentrations to be 52.52 μg/m3 with total observed average day cationic concentrations to be 15.23 μg/m3 and night concentrations to be 23.29μg/m3.

This study provides valuable insights into the seasonal patterns of PM2.5 and WSII and help understand the contributing factors and sources. This information can be used by policymakers to develop strategies for mitigating air pollution and improving the air quality in the region.

 

How to cite: Jain, Y., Kota, S. H., and Kumar, V.: Seasonal Variation and Source Apportionment of PM2.5 bound Water-Soluble Inorganic Ions (WSII) in Tier 2 and 3 Non-Attainment cities of India using PMF 5.0, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20150, https://doi.org/10.5194/egusphere-egu25-20150, 2025.

EGU25-258 | Posters on site | AS3.30

Granulometric Insights into PAH Concentrations and Health Risks: A Study of Urban Street Dust in Warsaw, Poland 

Sylwia Klaudia Dytłow, Jakub Karasiński, and Julio Cesar Torres-Elguera

The study investigated the total concentrations, toxicity, and health risks of 16 carcinogenic priority polycyclic aromatic hydrocarbons (PAHs) in street dust collected from urban areas in Warsaw, Poland. Samples were analyzed across six granulometric fractions. Dust was collected from 149 sampling points divided between Area 1 (central Warsaw districts, left bank of the Vistula River, dominated by traffic-related pollution) and Areas 2 and 3 (suburban residential areas, right bank of the river).

Street dust was assessed both as a whole (“all”) and after separation into five size fractions: (1–0.8 mm, “0.8”), (0.8–0.6 mm, “0.6”), (0.6–0.4 mm, “0.4”), (0.4–0.2 mm, “0.2”), and (below 0.2 mm, “<0.2”). The average ΣPAH concentration was 3.21 mg/kg in Area 1 and 0.89 mg/kg in Areas 2 and 3. Collectively for all areas, the ΣBaPTPE values were 318.3, 83.5, 131.1, 81.4, 164.3, and 339.7 ng/g for “all”, “0.8”, “0.6”, “0.4”, “0.2”, and “<0.2”, respectively. Notable differences in ΣBaPTPE values were observed among the fractions and areas, with the “<0.2” fraction showing the highest values: 339.7 ng/g across all areas, 318.9 ng/g in Area 1, and 531.6 ng/g in Areas 2 and 3. Coarser fractions (“0.8”, “0.6”, and “0.4”) consistently had the lowest average ΣBaPTPE values.

Cancer risk levels for children and adults were comparable for dermal contact and ingestion, ranging from 10⁻⁵ to 10⁻⁴, while risks from inhalation were significantly lower, ranging from 10⁻¹⁰ to 10⁻⁸. Thus, inhalation of resuspended street dust poses negligible risk compared to other exposure pathways.

These findings suggest a pressing need for both scientific and governmental interventions to mitigate the health risks posed by PAHs in urban street dust. Specifically, the spatial analysis of PAH concentrations revealed that areas with high-density development and traffic exhibit the greatest pollution, further emphasizing the need for targeted strategies to reduce emissions in such locations.

Future research should extend this investigation across different seasons to capture potential temporal variations in PAH concentrations due to seasonal activities and environmental conditions. Additionally, refining health risk assessments through the incorporation of locally specific exposure scenarios could provide more precise estimates of the carcinogenic and non-carcinogenic risks to Warsaw's residents. Such efforts will not only deepen our understanding of urban pollution but also inform policies aimed at safeguarding public health from the adverse effects of PAHs in street dust.

Acknowledgments

This research was funded in whole by the National Science Centre (Poland), grant number 2021/43/D/ST10/00996. This work was supported by a subsidy from the Polish Ministry of Education and Science for the Institute of Geophysics, Polish Academy of Sciences. The authors would like to thank Dominika Kwiecień, a student who participated in the field and laboratory and Klaudia Tetfejer for contributing her technical expertise and for assisting with data collection.

How to cite: Dytłow, S. K., Karasiński, J., and Torres-Elguera, J. C.: Granulometric Insights into PAH Concentrations and Health Risks: A Study of Urban Street Dust in Warsaw, Poland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-258, https://doi.org/10.5194/egusphere-egu25-258, 2025.

EGU25-355 | ECS | Posters on site | AS3.30

Long-term Assessment of Black Carbon Variation and Mechanisms Driving Extreme Events in Major Global Source Regions 

Yurong Zhang, Yong Han, Yan Liu, Ximing Deng, Tianwei Lu, Qicheng Zhou, and Li Dong

Black carbon (BC), primarily emitted from the incomplete combustion of fossil fuels and biomass, is a significant short-lived climate forcer that increasingly contributes to global climate change and environmental pollution. The BC properties in regions such as Eastern China (EC), Indian Subcontinent (IS), Sub-Saharan Africa (SSA), and Central South America (CSA) play a crucial role in global emissions due to intensive human activities and biomass burning, affecting air quality, climate change, and human health. Utilizing MERRA-2 reanalysis data and emission inventories, we quantified the long-term spatiotemporal variations and vertical distributions of atmospheric BC, along with anthropogenic emissions across various sectors (2000–2023). Additionally, we comprehensively explored the formation mechanisms of extreme cases in representative cities (Beijing, Delhi, Luanda, and Sucre) in these four regions, integrating meteorological conditions, potential source contribution function and concentration-weighted trajectory analysis. The results indicate consistent annual trends in BC surface concentration (BCSurface) and column density (BCColumn). BC concentrations in IS, SSA, and CSA exhibit an increasing trend, while EC shows a decreasing trend. In EC and IS, BC is primarily from anthropogenic emissions, whereas in SSA and CSA, biomass combustion predominates. Notable variations in anthropogenic BC emissions exist across different regions, with all sectors in SSA exhibiting a marked upward trend. Seasonal patterns are influenced by local meteorological conditions and emissions from both anthropogenic and biomass burning sources. In EC and IS, BC concentrations decline rapidly from 1000 to 850 hPa, while in SSA and CSA, the decline is slower in the lower atmosphere, with a rapid decrease around 700 hPa. High-concentration BC events in representative cities are linked to the interaction of local emissions, adverse meteorological conditions, and regional atmospheric circulation. Our study quantifies the long-term characteristics of BC in major global source regions from multiple perspectives, providing valuable scientific insights for both regional and global atmospheric environmental research and management.

How to cite: Zhang, Y., Han, Y., Liu, Y., Deng, X., Lu, T., Zhou, Q., and Dong, L.: Long-term Assessment of Black Carbon Variation and Mechanisms Driving Extreme Events in Major Global Source Regions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-355, https://doi.org/10.5194/egusphere-egu25-355, 2025.

EGU25-1780 | ECS | Orals | AS3.30

Advancing Collaborative Solutions to Transport-Related Air Pollution: Insights from the MI-TRAP Project 

Giorgos Chatzinakos, Georgia Tseva, Argiris Balatsoukas, Ioanna Tyligada, Amaryllis Zachariadou, Giannis Adamos, and Chrysi Laspidou

Transport-related emissions are a leading contributor to urban air pollution, posing significant challenges to public health, environmental sustainability, and quality of life. This presentation discusses the MItigating TRansport-related Air Pollution in Europe (MI-TRAP) project, a HORIZON EUROPE Innovation Action, that seeks to address these  challenges through advanced monitoring technologies, citizen science methodologies, stakeholder engagement, and evidence-based policymaking. Implemented across ten European City Pilots, MI-TRAP establishes a robust framework for reducing transport-related air pollution in diverse urban settings.

A cornerstone of MI-TRAP is the International Living Lab (ILL), a collaborative platform designed to engage stakeholders in co-creating and validating solutions for transport-related air pollution. The ILL comprises three sequential workshops, each targeting to drive stakeholder-led innovation. The first workshop establishes the ILL's objectives, gathers insights into local air quality challenges, and documents stakeholder concerns and community needs, ensuring the diverse contexts of each City Pilot are well-represented. This process lays a strong foundation for international collaboration. The second workshop focuses on validating solutions developed across MI-TRAP’s work packages, including technical innovations, epidemiological findings, and nature-based strategies, ensuring their feasibility in real-world urban environments. The third workshop translates these validated solutions into actionable, evidence-based policy recommendations for stakeholders and policymakers. 

This presentation analyses the outcomes of the first ILL workshop (19 February 2024), underscoring the critical role of stakeholder engagement in fostering collaboration among policymakers, researchers, and civil society. By integrating localised data and innovative approaches, the workshop addressed air quality challenges tailored to the unique urban contexts of the City Pilots. MI-TRAP’s stakeholder-driven methodology aligns with broader EU objectives, such as the Zero Pollution Action Plan, illustrating how participatory processes bridge the gap between emissions data and effective policy interventions. By highlighting the insights and strategies derived from the ILL, this presentation emphasises the transformative potential of stakeholder collaboration in addressing transport-related air pollution. The outcomes showcase how co-created solutions can lead to cleaner, healthier, and more sustainable urban environments across Europe, advancing the integration of science, policy, and community action.

How to cite: Chatzinakos, G., Tseva, G., Balatsoukas, A., Tyligada, I., Zachariadou, A., Adamos, G., and Laspidou, C.: Advancing Collaborative Solutions to Transport-Related Air Pollution: Insights from the MI-TRAP Project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1780, https://doi.org/10.5194/egusphere-egu25-1780, 2025.

The high-resolution ship emission inventory plays a critical role across multiple disciplines, including atmospheric and marine sciences as well as environmental management. In this study, we present a global high spatiotemporal resolution ship emission inventory developed using the Shipping Emission Inventory Model (SEIMv2.2) at a resolution of 0.1° × 0.1° for the years 2013, 2016–2021. Leveraging 30 billion Automatic Identification System (AIS) signals, SEIMv2.2 integrates real-time vessel positions, speeds, and technical parameters to model ship emissions from the bottom-up for key species, including CO2, NOx, SO2, PM2.5, CO, HC, N2O, CH4, and BC. According to our inventory results, which are freely accessible online (https://zenodo.org/records/11069531), temporally, global ship emissions exhibited minimal daily fluctuations. Spatially, high-resolution datasets revealed varying patterns of ship emission contributions by different vessel types across maritime regions. Research on the high spatiotemporal resolution ship emission inventory model SEIMv2.2 has been accepted by Earth System Science Data (https://essd.copernicus.org/preprints/essd-2024-258/).

 

Using our inventory, it is possible to reveal the variability of ship emissions across different regions and temporal scales. Taking 2020 as an example, we found that overall ship emissions of NOx, CO, HC, CO2, and N2O declined by 7.4%–13.8%, primarily due to the impacts of the COVID-19 pandemic. In the meanwhile, ship emissions of SO2, PM2.5, and BC dropped significantly by 40.9%–81.9% in 2020 compared to 2019, mainly driven by the implementation of low-sulfur fuel regulations. Focusing on the pandemic's influence, temporally, the largest drop in global ship emissions occurred in February 2020, followed by a gradual recovery in September as trade demand rebounded. Spatially, the shock originated in Asia and gradually extended to Europe and North America. Our analysis of the spatiotemporal variability of global ship emissions during the pandemic highlights the resilience of global maritime emissions, evidenced by the relatively small impact of the pandemic and the rapid pace of recovery. This resilience can be attributed partly to robust trade demand, and partly to the connectivity of maritime trade across continents, stemming from the fact that the trade in one region begins to recover, it often stimulates recovery in its trading partners. Research on the spatiotemporal variability of global ship emissions during the pandemic has been published online (https://www.sciencedirect.com/science/article/pii/S0048969724067895).

 

We further examined the characteristics of ship emissions in the Arctic region (defined as the area north of 60°N), which has been attracting research interests in recent years. Between 2016 and 2021, Arctic ship BC emissions increased by 6%, accounting for 1.5% of global ship emissions in 2021. Seasonally, BC emissions from ships during the Arctic summer (July–September) were 1.3 times higher than those in winter (January–March). In terms of vessel type contributions, cargo ships (including general cargo ships, bulk carriers, and container ships) accounted for 44.8% of BC emissions, followed by fishing vessels at 34.8% and oil tankers at 15.0%, in 2021. In the future, distinguishing between ship emissions driven by different transportation demands, such as transit cargo transport and energy transport is crucial for scientifically predicting future Arctic ship emissions and developing effective Arctic ship emission reduction strategies.

How to cite: Yi, W. and Liu, H.: High-resolution global shipping emission inventory by Shipping Emission Inventory Model (SEIM): Insights into multiyear spatiotemporal variability, pandemic impacts, and emerging Arctic shipping emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1997, https://doi.org/10.5194/egusphere-egu25-1997, 2025.

EGU25-2502 | ECS | Posters on site | AS3.30

Study and update on the characteristic composition of urban emission sources of ozone precursor VOCs in Taiwan 

Yen-Chen Chen, Chih-Yuan Chang, Wen-he Kao, Chian-Yi Liu, and Chih-Chung Chang

Over the past three decades, the daily maximum eight-hour and annual average concentrations of ozone in Taiwan have not significantly improved with the reduction of its precursors, volatile organic compounds (VOCs) and nitrogen oxides (NOx). High ozone in the lower troposphere may be attributed to a variety of factors, mainly from localized photochemical formation and regional transport as well as minor stratospheric intrusions. Even though the total emissions of precursor VOCs have been significantly reduced in recent years, the reaction potential of different VOCs to ozone formation can vary by dozens of times, as well as their potential to generate SOA and their toxicity to organisms. The composition and quantity of many emission data are old and no longer meet the current conditions under today's new industrial equipment, process methods, new vehicles, engines, catalytic technologies, new lifestyle products and new emission regulations, showing the necessity of updating the emission composition of each major VOCs emission source. The long-term goal of this study is to gradually increase and update the VOC emission characteristics of various major types of emission sources (point sources, line sources, area sources, and biological sources) in the city. The first phase will focus on "mobile source" traffic emissions in urban areas. The composition analysis would be conducted based on vehicle exhaust, indoor parking lots, tunnel vehicle arrays and other sources. Furthermore, the traffic emission indicator, methyl tertiary butyl ether (MTBE), and complete combustion product, CO2, would be exploited to evaluate the VOC composition characteristics and emission factors of various emission sources.

How to cite: Chen, Y.-C., Chang, C.-Y., Kao, W., Liu, C.-Y., and Chang, C.-C.: Study and update on the characteristic composition of urban emission sources of ozone precursor VOCs in Taiwan, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2502, https://doi.org/10.5194/egusphere-egu25-2502, 2025.

This study investigates the impact of Road Transport Emission Reduction Policies (RTERPs) on air pollutant and greenhouse gas (GHG) emissions in Vijayawada, a non-attainment city in India. Utilising the Activity-Structure-Emission Factor (ASF) modeling technique, we developed an on-road transportation sector emission inventory for the base year 2021, encompassing both vehicle exhaust and non-exhaust emissions. The study found that vehicle exhaust emissions of PM10, NO2, CO, and HC in 2021 were 4.7 Gg, 5.6 Gg, 17.3 Gg, and 2.4 Gg, respectively.

The study evaluated the effectiveness of RTERPs under different scenarios for 2030. Alternative Scenario I (ALT-I-2030), incorporating national-level policies such as vehicle scrappage, cleaner fuels, and electric vehicle promotion, is projected to reduce pollutant emissions by 22-45%. For instance, PM10 emissions are expected to decrease by 22%, while NO2 emissions could see a reduction of up to 45%. ALT-II-2030, due to local-level strategies like low-emission zones in addition to national policies, demonstrates a more significant reduction in vehicle exhaust emissions, ranging from 42% to 68%. Under this scenario, PM10 emissions are projected to decrease by 42%, and NO2 emissions could potentially decline by 68%.

While ALT-II-2030 reduces CO2 emissions from vehicle exhaust by 29% (from 550 Gg in 2021 to 390 Gg in 2030), the study highlights the potential for indirect CO2 emissions from coal-based electricity generation to power the growing electric vehicle fleet, potentially offsetting the positive effects of RTERPs.

Non-exhaust emissions were also quantified, with resuspended road dust constituting the primary source, contributing approximately 94% of PM emissions (nearly 2.4 Gg) in 2021. Meanwhile, tyre, brake, and road wear contributed to 1%, 3%, and 2% respectively.  The spatial distribution of both vehicle exhaust and non-exhaust emissions exhibits significant heterogeneity, emphasising the need for localised control strategies in urbanising regions. This study underscores the importance of adopting balanced strategies that simultaneously address air quality concerns and promote sustainable transportation systems, aligning with Sustainable Development Goals 11.2 and 11.6.2.

Keywords: Road transport emissions, Emission inventory, Urban air quality, Scenario analysis, Exhaust and non-exhaust emissions 

How to cite: Sharma, M., Jain, S., and Badavath, B.: Assessing the Effectiveness of Emission Reduction Policies in Mitigating Road Transport-Induced Air Pollution and GHG Emissions in a Non-Attainment City in India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2809, https://doi.org/10.5194/egusphere-egu25-2809, 2025.

EGU25-3097 | Orals | AS3.30

Vehicle emissions under real driving conditions: investigating the impact of semi-volatile compounds on air quality 

Amira Jabbari-Hichri, Yassine Azizi, Bernard Guiot, Antoinette Boreave, and Christian George

Keywords: Air quality, vehicle emissions, semi-volatile organic compounds, chemical composition.

Vehicle emissions significantly affect air quality, particularly through the release of particulate matter (PM), which pose severe health risks such as respiratory and cardiovascular diseases1. The world health organization (WHO) has updated guidelines to restrict exposure to these pollutants2. Traditional emission models often overlook semi-volatile organic compounds (SVOCs) and intermediate-volatility organic compounds (IVOCs), which play crucial roles in forming secondary organic aerosols (SOAs)3. These compounds contribute to the formation of fine particulate matter (PM) and can have significant health implications due to their ability to penetrate deep into the respiratory system4.

This study investigates the impact of the emissions coming from various automotive vehicles on air quality, with a specific focus on semi-volatile organic compounds (SVOCs) measured across different real driving conditions, including urban, rural, and highway. A number of advanced on-line analytical instruments were used to gain a detailed understanding on the emitted compounds. The particle concentration and its distribution size, using a TSI EEPS 3090 and the Horiba OBS ONE SPN23 and SPN10, meanwhile the gas phase analysis was carried out using a Horiba FTX. In addition to real-time measurements, a novel collection system was developed to capture tailpipe emissions as a function of vehicle speed. Those various speed conditions dependent emissions, condensed in liquid phase through a cooling process, were subsequently analyzed offline using an UPLC-Orbitrap-MS. The compounds identified were then classified according to their volatility using the Volatility Basis Set (VBS)5.

The relationship between the molecular mass of the emitted compounds and their volatility, based on the engine speed during various test drives was established, providing deeper insights into car emissions of SVOCs and IVOCs.

These findings are important for enhancing the accuracy of air quality models and developing targeted strategies to reduce pollution.

References

1 Hussain M, Madl P, Khan A (2011), Part-I. Health 2(2):51–59.

2 World Health Organization (2021), Geneva, World Health Organization.

3 Robinson AL, Donahue NM, Shrivastava MK, Weitkamp EA, Sage AM, Grieshop AP, Lane TE, Pierce JR, Pandis SN (2007), Science 315(5816):1259–1262.

4 Sun J, Shen ZX, Zhang T, Kong SF, Zhang HA, Zhang Q, Niu XY, Huang SS, Xu HM, Ho KF, Cao JJ (2022), Environmental International 165:107344.

5 Li Y, Pöschl U, Shiraiwa M (2016), Atmospheric Chemistry and Physics 16(6):3327-3344.

How to cite: Jabbari-Hichri, A., Azizi, Y., Guiot, B., Boreave, A., and George, C.: Vehicle emissions under real driving conditions: investigating the impact of semi-volatile compounds on air quality, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3097, https://doi.org/10.5194/egusphere-egu25-3097, 2025.

EGU25-4132 | ECS | Orals | AS3.30

Health impact of non-exhaust particles from road transports 

Alice Mirailler, André Schröder, Adina Lazar, Thierry Granjon, Salah Khardi, and Ana-Maria Trunfio-Sfarghiu

Air pollution causes around 4.2 million premature deaths worldwide every year [1]. Several studies have demonstrated the harmful effects of poor air quality on health: onset of respiratory diseases [2], cardiovascular problems [3] and neurological disorders [4]. For traffic-related pollution, exhaust emissions are widely studied and their level is actually in decrease, thanks to relevant policies. Still, this is not the case for non-exhaust emissions (brakes, tires, pavement, vehicle components and re-suspension phenomena), which account for the majority of particulate emissions [5]. In order to characterize the non-exhaust emissions and to evaluate their potential toxicity, two industrial partnerships have been set up. Indeed, braking tests were carried out in the laboratory as part of the INSA - VOLVO Chair collaborative project and additional tests were performed with a system directly integrated into the vehicle to analyze particles from tire-road contact within the framework of the INSA - MICHELIN Chair.

For each test, we used an innovative collection system developed in the laboratory, allowing us to capture particles from the brakes or tires directly into a culture medium or a biomimetic surfactant (a new device developed under the Pulsalys DPPA project). This setup also includes a particle counter, with particle size range from 10 nm up to 10 µm, enabling particle size distribution analysis during the tests, along with a carbon tab for particle collection, which is subsequently examined using SEM-EDX to determine the particles’ composition. In order to identify the health impacts of the collected non-exhaust particles, the effect of the collection media on cellular viability was evaluated using RAW264 macrophages cell line. Changes in the physicochemical properties of pulmonary surfactant, as well as the biophysical properties of cells, upon contact with non-exhaust particles were also evaluated.

The collected non-exhaust particles did not show a significant impact on cell viability. However, using a fluidity marker (DIOLL), we detected changes in cell biophysical properties and surfactant structure: indeed, cells in the presence of particles became more rigid, while pulmonary surfactant in the presence of particles became more fluid.

This study underlines thus a significant disturbance in cell metabolism and cellular homeostasis, despite an apparently unaffected cell viability. The observed biophysical changes seem to represent an early marker of chronic pathologies such as cancer or pulmonary fibrosis.

 

[1] Fuller et al, “Pollution and health: a progress update,” Lancet Planet Health, vol. 6, pp. 535–547, 2022.

[2] Caillaud et al, “Outdoor pollution and its effects on lung health in France,’’ Revue des Maladies Respiratoires, vol. 36, p. 1150—1183, 2019.

[3] Lelieveld et al, “Cardio- vascular disease burden from ambient air pollution in europe reassessed using novel hazard ratio functions.,” European Heart Journa, vol. 40, p. 1590–1596, 2019.

[4] Piguet, “Neurosciences grand public pollution environnementale maladies du cerveau : Les pistes actuelles,” NeuroCampus, vol. Brochure 1, 2018.

[5] Martini, “Scientific evidence on vehicle’s emissions,” The European Commission’s science and knowledge service, 2018.

 

How to cite: Mirailler, A., Schröder, A., Lazar, A., Granjon, T., Khardi, S., and Trunfio-Sfarghiu, A.-M.: Health impact of non-exhaust particles from road transports, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4132, https://doi.org/10.5194/egusphere-egu25-4132, 2025.

EGU25-4529 | ECS | Orals | AS3.30

SIMROUTE: A Tool for Assessing the Emissions Mitigation Potential of Weather Routing in Short Sea Shipping  

Clara Borén, Manel Grifoll, and Marcella Castells-Sanabra

Ocean-going vessels contribute substantially to global carbon dioxide emissions, compelling effective mitigation strategies. This research investigates the potential of weather ship routing (WSR) for emissions reduction, focusing on Short Sea Shipping (SSS) in the Mediterranean Sea, bridging the gap between shipping pollutant estimation and weather routing optimization, two areas often studied independently.

The study utilizes SIMROUTE, an open-source software tool employing the A* pathfinding algorithm to optimize routes based on wave action derived from Copernicus Marine Environment Monitoring Service (CMEMS) data. SIMROUTE calculates both minimum distance and optimized routes, minimizing sailing time by considering weather conditions. This research builds upon SIMROUTE’s core functionalities by specifically quantifying the emissions reductions achievable through WSR.

WSR is formulated as an optimization problem incorporating various parameters, including vessel type, propulsion machinery, fuel type, and wave effects on navigation. Fuel consumption and ship emissions calculations are performed using a methodology inspired by the STEAM2 bottom-up approach, further incorporating the increased power required to overcome speed reductions caused by waves. Wave effects are primarily parameterized using the Bowditch methodology, recognized for its simplicity, with sensitivity analyses conducted using Aertssen’s and Khokhlov’s formulations.

Despite the limited fetch and relatively small significant wave heights typical of the Mediterranean, substantial reductions in fuel consumption and emissions are achieved through SIMROUTE simulations. This implies even greater benefits in open ocean conditions with larger wave heights, as supported by a case study of a large Pacific Ocean route demonstrating a 13.25% emission reduction. This aligns with existing literature advocating for sector-specific emissions analysis due to variations in influencing factors.

Derived from the SIMROUTE simulations’ results, it is concluded that, while emissions reductions on very short routes are modest, their cumulative effect over time, considering storm frequency and service schedules, warrants further investigation. Notably, significant emissions reductions, up to 30%, were observed for SSS routes up to 600 nautical miles. Consequently, SIMROUTE software stands out as a tool for demonstrating that there is an emissions mitigation potential in SSS routes, providing vessel-specific data demonstrating meaningful results regardless of distance covered, highlighting the value of WSR as a practical emissions reduction strategy.

How to cite: Borén, C., Grifoll, M., and Castells-Sanabra, M.: SIMROUTE: A Tool for Assessing the Emissions Mitigation Potential of Weather Routing in Short Sea Shipping , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4529, https://doi.org/10.5194/egusphere-egu25-4529, 2025.

EGU25-4876 | ECS | Posters on site | AS3.30

Seasonal Trends, Sources, and Health Impacts of PAH-Bound PM10 in Krakow Amidst the COVID-19 Pandemic 

Rakshit Jakhar, Przemysław Furman, Alicja Skiba, Dariusz Widel, Mirosław Zimnoch, Lucyna Samek, and Katarzyna Styszko

The main objective of this research was to evaluate the seasonal variability of PM10-bonded polycyclic aromatic hydrocarbons (PAH) and their sources and analyse their health impacts during the COVID-19 pandemic period.  PM10samples were collected in Krakow in 2020-2021. The chemical composition of PM10 in terms of the content of polycyclic aromatic hydrocarbons (PAHs) was carried out using the gas chromatography-mass spectrometry (GC-MS) technique. A total of 92 samples of particulate matter (PM10 fraction) were analysed. The analyses contained 16 basic PAHs identified by the US EPA as the most harmful. Acenaphtene (Acn), Acenaphthylene (Acy), Anthracene (Ant), Benzo[b]fluoranthene (B[b]F), Benzo[a]anthracene (B[a]A), Benzo[a]pyrene (B[a]P), Benzo[ghi]perylene (B[ghi]P), Benzo[k]fluoranthene (B[k]F), Chrysene (Chry), Dibenzo[ah]anthracene (D[ah]A), Fluoranthene (Flt), Fluorene (Flu), Indeno[1,2,3-cd]pyrene (IP), Naphthalene (Nap), and Phenanthrene (Phen) and Pyrene (Pyr). The information obtained on the concentrations of PAHs was used to determine the profiles of pollution sources, exposure profiles, and the values of toxic equivalency factors recommended by the EPA: mutagenic equivalent to B [a] P (ang. mutagenic equivalent, MEQ), toxic equivalent to B[a]P (ang. toxic equivalent, TEQ) and carcinogenic equivalent to 2,3,7,8-tetrachlorodienzo-p-dioxin (ang. carcinogenic equivalent, CEQ). In addition, the air trajectory frequency analysis were performed to obtain information on the possibility of transporting pollutants from selected areas in the vicinity of the studied site. The analyses were performed using the NOAA Air Resources Laboratory's HYSPLIT model (Hybrid Single-Particle Lagrangian Integrated Trajectory Model) developed by the NOAA Air Resources Laboratory (National Oceanic and Atmospheric Administration). Interpreting the trajectory results provided information on the nature of air pollution sources.

Acknowledgement: This research project was supported by the programme "Excellence Initiative – Research University" for the AGH University of Krakow, Poland [project no. 501.696.7996 L34,D.4,V ed.,wn. 10457

 

How to cite: Jakhar, R., Furman, P., Skiba, A., Widel, D., Zimnoch, M., Samek, L., and Styszko, K.: Seasonal Trends, Sources, and Health Impacts of PAH-Bound PM10 in Krakow Amidst the COVID-19 Pandemic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4876, https://doi.org/10.5194/egusphere-egu25-4876, 2025.

EGU25-5879 | ECS | Orals | AS3.30

Atmospheric aerosol from on-road transport in Europe: The role of different vehicle types 

Stella-Eftychia Manavi, Ksakousti Skyllakou, Evangelia Siouti, and Spyros Pandis

On-road vehicles are an important source of atmospheric particulate matter (PM), producing both primary aerosol and gas-phase precursors, which react in the atmosphere and lead to the formation of secondary aerosol. Over the past 50 years, the emissions from the exhaust of passenger cars have been thoroughly studied, on the contrary, other on-road vehicles, like mopeds, buses, and heavy-duty vehicles, have received less attention. Moreover, as regulatory measures reduce the concentrations of primary aerosol emitted from on-road vehicles, the significance of the gas-phase precursors increases. The aim of this study is to assess both the overall effect of different on-road vehicle types on particle mass concentrations over Europe, as well as the specific role of volatile and intermediate volatility organic compounds to the formation of secondary organic aerosol (SOA). To achieve this, the results of the EASVOLEE (Effects on Air Quality of Semi-VOLatile Engine Emissions) emission characterization campaigns were used to update PMCAMx inputs and parameterizations. The three-dimensional chemical transport model was used to simulate a summer month (July 2019) in Europe. The contribution of different vehicle types to the total PM2.5 and to the concentrations of primary and secondary OA. The model simulations provide insights about the significance of specific volatile and intermediated volatility compounds emitted from on-road vehicles over Europe.

How to cite: Manavi, S.-E., Skyllakou, K., Siouti, E., and Pandis, S.: Atmospheric aerosol from on-road transport in Europe: The role of different vehicle types, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5879, https://doi.org/10.5194/egusphere-egu25-5879, 2025.

EGU25-6117 | Orals | AS3.30

Plug-In Hybrid Light-Duty vehicle emission measurements over custom RDE test cycle on the road and in the various laboratory conditions 

Wojciech Honkisz, Piotr Bielaczyc, Andrzej Szczotka, Dariusz Klimkiewicz, Päivi Aakko-Saksa, Anssi Järvinen, Topi Rönkkö, Katariina Kylämäki, Milja Jäppi, Laura Salo, Teemu Lepisto, Rabbia Asgher, Hilkka Timonen, Matti Rissanen, Luis Barreira, Minna Aurela, Tereza Červená, Michal Vojtisek, and Jan Topinka

INTRODUCTION

Real Driving Emissions (RDE) methods are essential for assessing the environmental performance of Plug-In Hybrid Electric Vehicles (PHEVs), which differ significantly from Internal Combustion Engine (ICE) vehicles due to their dual powertrain systems. These systems have different operating modes, either prioritizing electric power (in this case Automatic mode) or balancing ICE use to maintain battery state of charge (SOCH; here Hybrid mode), which influence emission profiles. Such distinctions necessitate tailored RDE testing to capture emissions under real-world conditions accurately.

This study focuses on two PHEVs: one equipped with a gasoline engine (PHEVG) and the other with a diesel engine (PHEVD).

Gaseous and particulate emissions were quantified to assess the effects of temperature, powertrain type, and driving mode.

METHODS

Emissions of gaseous compounds—carbon dioxide (CO2), carbon monoxide (CO), nitrogen oxides (NOx), total hydrocarbons (THC), and particle number (PN)—were measured in both on-road RDE and laboratory conditions. Tests were conducted at -9°C, 23°C, and 35°C to simulate varying driving environments. To ensure comparable testing, a "golden" on-road RDE test was used to develop the laboratory-based RDEsim cycle. This custom cycle was executed on a chassis dynamometer. The study investigated PHEVG and PHEVD, capturing emissions in both AUTOMATIC and HYBRID driving modes for PHEVG and COMFORT mode for PHEVD under consistent SOCH levels.

RESULTS

Emission patterns varied significantly between the two PHEVs under different temperatures and driving modes. CO2 emissions increased at -9°C, with PHEVD consistently achieving lower levels due to the efficiency of the diesel technology. AUTOMATIC mode for PHEVG emphasized electric power, reducing fuel consumption but increasing energy use, while HYBRID mode prioritized SOCH stability with more frequent internal combustion engine usage. NOx emissions were minimal for PHEVG but rose for PHEVD in colder conditions. Both vehicles showed elevated THC and PN emissions at -9°C, with diesel-powered PHEVD maintaining lower PN levels overall due to advanced filtration systems. These results underscore the impact of driving modes and environmental conditions on emission behaviours.

CONCLUSIONS

This study demonstrates the distinct emission characteristics of PHEVG and PHEVD across varying conditions. AUTOMATIC mode favored electric power utilization, leading to reduced tailpipe emissions but increased electric energy consumption. HYBRID mode offered consistent SOCH management, relying more on the internal combustion engine, which increased emissions.

Colder temperatures (-9°C) had the most pronounced effect, significantly elevating CO2, NOx, and THC emissions for both vehicles. Diesel-powered PHEVD consistently outperformed PHEVG in CO2 and PN emissions, showcasing the advantages of diesel technology under diverse conditions.

The findings underscore the need for tailored RDE testing methods to reflect the unique operational behaviours of PHEVs. By accounting for driving mode, temperature, and powertrain type, this study contributes to improving emission standards and ensuring accurate assessment of plug-in hybrid vehicles in real-world scenarios.

ACKNOWLEDGEMENTS

This work was supported by the European Union’s Horizon Europe research and innovation programme under grant agreement No 101096133 (PAREMPI: Particle emission prevention and impact: from real-world emissions of traffic to secondary PM of urban air).

How to cite: Honkisz, W., Bielaczyc, P., Szczotka, A., Klimkiewicz, D., Aakko-Saksa, P., Järvinen, A., Rönkkö, T., Kylämäki, K., Jäppi, M., Salo, L., Lepisto, T., Asgher, R., Timonen, H., Rissanen, M., Barreira, L., Aurela, M., Červená, T., Vojtisek, M., and Topinka, J.: Plug-In Hybrid Light-Duty vehicle emission measurements over custom RDE test cycle on the road and in the various laboratory conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6117, https://doi.org/10.5194/egusphere-egu25-6117, 2025.

EGU25-6146 | Orals | AS3.30

Secondary organic aerosol formation from transportation emissions 

Christos Kaltsonoudis, Damianos Pavlidis, Christina N. Vasilakopoulou, Silas Androulakis, Christina Christopoulou, Georgia Argyropoulou, Katerina Seitanide, Yanfang Chen, Andre S.H. Prevot, and Spyros N. Pandis

Transportation emissions can be a significant source of secondary organic aerosol (SOA) both in urban areas and regionally. Aromatic hydrocarbons and large alkanes are expected to be the major SOA precursors. However, there are still major uncertainties in understanding SOA from vehicle exhaust in different timescales.

To address these uncertainties, this study focuses on measuring SOA formation from vehicle emissions in a real-world environment. The SOA formation from vehicle emissions in a large underground parking structure was investigated using an oxidation flow reactor (OFR). The organic vapors in the study were dominated by cold start emissions. The air in the parking structure was continuously fed to the OFR. The OH exposure was controlled by varying combinations of the OFR’s UV lamps. Α scanning mobility particle sizer (SMPS) was used to continuously measure the SOA formation inside the OFR. A high-resolution aerosol mass spectrometer and a high-resolution proton-transfer-reaction time-of-flight mass spectrometer coupled to a CHARON inlet were used to characterize the particulate phase alternating sampling between the parking garage and the OFR every 20 minutes. The PTR-MS also monitored the gas phase, while quartz filters were collected for offline analysis. Trace gases (NO, NO2, CO, CO2, O3, and SO2) and black carbon were quantified using dedicated instruments that continuously sampled air from the parking garage.

Significant SOA formation was observed increasing the organic aerosol levels several times. The SOA increased with the intensity of UV lamp exposure in the OFR. The results of the measurements can be used for the parameterization of SOA formation from the vehicle emissions at both intermediate and longer timescales.

How to cite: Kaltsonoudis, C., Pavlidis, D., Vasilakopoulou, C. N., Androulakis, S., Christopoulou, C., Argyropoulou, G., Seitanide, K., Chen, Y., Prevot, A. S. H., and Pandis, S. N.: Secondary organic aerosol formation from transportation emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6146, https://doi.org/10.5194/egusphere-egu25-6146, 2025.

EGU25-6147 | ECS | Posters on site | AS3.30 | Highlight

Real world cold-start emissions measurements in a parking garage 

Damianos Pavlidis, Christos Kaltsonoudis, Silas Androulakis, Christina Vasilakopoulou, Georgia Argyropoulou, Christina Christopoulou, Katerina Seitanide, and Spyros Pandis

Despite progress in emission reductions, motor vehicles are a significant contributor to urban air pollution, releasing emissions containing various compounds in both particulate and gas phases. Studies have shown that the highest emissions are exhibited during the cold start due to the inefficient operation of the catalyst and engine at low temperature (Kontses et al. 2020; Hu et al. 2023).

This study aims to enhance our understanding of cold-start emissions from passenger cars, which dominate urban traffic. To achieve this, emissions of a vehicle fleet were measured under realistic conditions within a parking garage. The measurements were conducted from November 27 to December 24, 2024, in  an undergraduate parking garage with  250 parking  spaces, located in a shopping mall in Patras, Greece. The particle phase was measured by a scanning mobility particle sizer (SMPS), a high-resolution aerosol mass spectrometer (HR-ToF-AMS) and a high-resolution proton-transfer-reaction time-of-flight mass spectrometer (PTR-ToF-MS) coupled to a CHARON inlet (Ionicon Analytik Inc.). Black carbon was quantified by an Aethalometer (AE33) and a Single Soot Photometer (SP2-XR). An Electrical Low-Pressure Impactor (ELPI, Dekati) was also operated on site. The gas-phase composition was characterized by the PTR-MS while trace gases such as NO, NO2, CO, CO2, O3 and SO2 were continuously monitored. For offline analysis, samples were collected using quartz filters and Tenax tubes.  Additionally, the traffic flow was recorded at both the entrance and exit of the garage. Measurements of CO2 were conducted at six different locations in the garage and indicated that the measurements were representative of most of the volume of the structure.

The measured concentrations varied significantly during the day with peaks in the morning and the evening. The measurements of the traffic and the concentrations were combined to derive average emissions of gas and particulate phase pollutants per cold start and per kilogram of fuel.

 

References

Kontses, A., Triantafyllopoulos, G., Ntziachristos, L., and Samaras, Z. 2020. Particle number (PN) emissions from gasoline, diesel, LPG, CNG and hybrid-electric light-duty vehicles under real-world driving conditions, Atmos. Environ., 222, 117126.

Hu, J., Frey, H. C., and Boroujeni, B. Y. (2023). Contribution of cold starts to real-world trip emissions for light-duty gasoline vehicles. Atmosphere, 14, 35.

How to cite: Pavlidis, D., Kaltsonoudis, C., Androulakis, S., Vasilakopoulou, C., Argyropoulou, G., Christopoulou, C., Seitanide, K., and Pandis, S.: Real world cold-start emissions measurements in a parking garage, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6147, https://doi.org/10.5194/egusphere-egu25-6147, 2025.

Indoor ventilation optimization is important for air quality, thermal comfort, and airborne transmissions of infectious droplets, but research on cruise ships is scarce, especially across whole year seasons. How to weigh air quality and human comfort is an essential and practical issue. We utilize numerical simulations verified by field experiments to examine the thermal comfort and infection risk under natural ventilation and air-conditioning ventilation in various seasons. The scientific problem of this study is the proper utilization of natural and mechanical ventilation at the inter-annual scale to provide a good environment for passengers in the transportation environment. The effect of window opening configurations and ambient wind directions on natural ventilation has been explored. Varying filtration efficiencies are considered for air conditioners. The Monte Carlo method and dose-response model are adopted to quantify infection risk (IR). 
Results reveal that surrounding turbulent airflows create positive pressure on the windward side ship's surface and negative pressure on the leeward side. Compared to driving following wind and against the wind, the best ventilation in the cabin occurs during side wind, due to the large windward area with an air change rate per hour (ACH) above 61.78 h-1. In spring and fall, opening all side windows provides good thermal comfort (-1<PMV<+1) and maintains low IR (median below 0.61%, 95% CI: 0.27% to 2.00%). However, thermal comfort decreases and mechanical ventilation is required in summer and winter. When using mechanical ventilation, comfort is improved (PMV=-0.21). However, the median IR reaches 6.14% (95% CI: 5.71% to 7.87%) under recirculating air conditioners. With filtration efficiency increasing to 30%, the median IR decreases to 0.79% (95% CI: 0.82% to 1.02%). Threshold analysis indicates that a filtration efficiency of 14.06% is the threshold to decrease IR effectively. To ensure human thermal comfort and infection risk, windows can be opened for natural ventilation when the temperature is suitable. However, if mechanical ventilation is required, an air conditioner system with a filtering and sterilization function must be adopted.

How to cite: luo, Q. and Hang, J.: Inter-annual optimization of ventilation strategies in cruise ships: Integrating thermal comfort and infection risk mitigation across seasonal variations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6520, https://doi.org/10.5194/egusphere-egu25-6520, 2025.

EGU25-7152 | ECS | Posters on site | AS3.30

Source apportionment and biomonitoring approaches to quantify the contribution and spatial spread of particulate matter from shipping in a major UK port city 

Nat Easton, Adeline Sivyer, Matthew Cooper, Lareb Dean, James Parkin, Agnieszka Michalik, Sargent Bray, Donna Davies, Damon Teagle, Gavin Foster, and Matthew Loxham

Shipping emissions are an important source of Particulate Matter (PM) associated with an estimated 400,000 premature deaths per year globally. These negative effects on air quality disproportionately impact port and coastal communities, which include many of the world’s largest cities. Despite the English Channel being the busiest shipping lane in the world, and in close proximity to many major cities, the physicochemical characterisation of shipping emissions and their contribution to air quality in the UK remains understudied.

Coarse (PM10-2.5) and fine (PM2.5-0.1) PM samples were collected between 2017 and 2020 at the UK port of Southampton. This port is Europe’s leading turnaround cruise port, handling 86% of all UK cruise passenger traffic in 2023.  In addition, Southampton is one of the UK's major gateway container ports, being the UK’s leading vehicle import/export and deep-sea trade port, attracting some of the world's largest ships. Importantly, as Southampton is located centrally on the south coast of England, this falls within the North Sea Emission Control Area and therefore, ships in this area are subject to the most stringent fuel restrictions of 0.1% S, or equivalent exhaust cleaning.

To determine the contribution of shipping emissions to air quality, a positive matrix factorisation source apportionment model was generated using PM elemental concentrations measured by inductively coupled plasma mass spectrometry. The shipping fuel combustion factor was characterised by the traditional tracers of V and Ni within the expected ratio (V/Ni = 2.6) indicative of Heavy Fuel Oil (HFO) associated shipping. However, Co was identified as a novel tracer species, which may be an artefact from the catalysis of fuel desulfurisation. The final five-factor model found that shipping fuel contributed almost exclusively to fine PM, rather than coarse PM, with an average contribution of 15% fine PM at the Port. This contribution was significantly elevated between April and September, representing the peak cruise shipping season.

To study the spatial spread of PM emissions, samples of tree bark were used, as airborne particles can become trapped in the bark structure. This biomonitoring approach represents a cost- and time-effective alternative to the use of multiple PM-sampling sites.  Here, samples of bark from lime (Tilia spp.), oak (Quercus spp.) and aspen (Populus tremula) trees were collected at locations across the city of Southampton. The elemental concentration of the identified shipping tracers Ni and Co in the bark samples were investigated (V was unsuitable as a tracer due to uptake by bark lichens). This showed that concentrations of Ni and Co in tree bark displayed an exponential increase with increasing proximity to the port. Our data suggest deposited concentrations 300 m from the port are 2.5x higher than 2.2 km away and 4x greater than 6 km away.

Collectively the contribution of shipping emissions to port city PM, and the spread of these emissions identified in this study underline the importance of including shipping in strategies to improve air quality. These strategies would be aided by a better understanding of the key aspects of port and shipping activity which drive these emissions.

How to cite: Easton, N., Sivyer, A., Cooper, M., Dean, L., Parkin, J., Michalik, A., Bray, S., Davies, D., Teagle, D., Foster, G., and Loxham, M.: Source apportionment and biomonitoring approaches to quantify the contribution and spatial spread of particulate matter from shipping in a major UK port city, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7152, https://doi.org/10.5194/egusphere-egu25-7152, 2025.

EGU25-7575 | Orals | AS3.30

Future Spatial Patterns and Environmental Impacts of Aviation Emissions in China by 2035 

Junheng Yan, Ruoxi Wu, Jingran Zhang, Shaojun Zhang, and Ye Wu

China's civil aviation transportation is expected to become the world’s largest aviation market soon. However, synergistically reducing CO2 and pollutants in aviation presents significant challenges, making it one of the most difficult sectors for future emission reductions. To assess the environmental impacts of the growing aviation market in China, this study aims to outline the future spatial patterns of aviation pollutant emissions in China by 2035 based on a localized bottom-up analysis, incorporating planned airport infrastructure, projected demand growth in city pairs, fleet expansion, and technological composition. Two methodologies are used, a random-forest regression model to predict air route passenger flow by 2035, and a spatial pollutant emission approach performed bottom-up that considers improving aircraft and engine technology, optimizing operations and using sustainable aviation fuel (SAF). Then, the Community Multiscale Air Quality (CMAQ) Integrated Source Apportionment Method (ISAM) modeling system (v5.3.2) is utilized to stimulate the physical and chemical processes aviation-derived air pollutants of the expected scenario in 2030. Our findings highlight the increasing impact of aviation in China, particularly in cities with dual airports, and reveal the challenges of accelerating coordinated reductions in CO2 and air pollutants within the aviation sector. Despite most new airports being constructed in Southwest China, the disparity in spatial pollutant distribution will continue to grow due to increased aviation activities at central hubs in Eastern China. The proportion of aviation-attributed near ground PM2.5 and O3 in total concentrations would have increased from 2.9% and 9.4% to 6.7% and 14.2% in developed regions from 2017 to 2030 as other sectors progress towards decarbonization and pollutant emissions reduction. Stricter and more diversified control measures are needed to help the aviation industry reduce pollutant emissions while achieving decarbonization.

How to cite: Yan, J., Wu, R., Zhang, J., Zhang, S., and Wu, Y.: Future Spatial Patterns and Environmental Impacts of Aviation Emissions in China by 2035, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7575, https://doi.org/10.5194/egusphere-egu25-7575, 2025.

EGU25-8370 | ECS | Orals | AS3.30

Performance evaluation of CEN-SMPS with a novel fast scan mode for better identification of UFPs in MI-TRAP 

Arpit Malik, Andreas Nowak, Johannes Rosahl, Kostas Eleftheriadis, and Maria Gini

Introduction: Precise measurement and characterization of ultrafine particles (UFPs) is one of the key objectives of the MI-TRAP (Mitigating Transport Related Air Pollution in Europe) project. The scanning mobility particle sizers (SMPS) have been conventionally used worldwide for measuring the particle number size distributions (PNSD) from transport emissions as well as in ambient air. Consequently, they are an integral part of the air quality monitoring network under the MI-TRAP consortia and the measurements are harmonized with the standard protocol (CEN/TS 17434:2020) by the European Committee for Standardization (CEN). This standard specifies the diameter range for a SMPS scan from 10 nm up to 800 nm, consequently leading to large scan time over 5 minutes. However, the size distribution of UFPs monitored by SMPS at several European sites have been found to be predominately centered around geometric mean diameter (GMD) < 100 nm [1]. Moreover, the introduction of new European emission standards like Euro 6 have led to decrease the GMDs of transport emissions as well (GMD = 50-60 nm observed for Euro 6 gasoline and port fuel injected engines) [2]. Therefore, this wide scan range is less efficient and time consuming for monitoring UFPs from transport emissions. All these factors necessitate the introduction of a fast-scanning mode with a narrower scan range without compromising the accuracy and tailored for the specific needs of UFP measurements.

Methodology: Our study presents the performance evaluation of the novel fast-scanning mode (1-minute) of a CEN-SMPS and investigates its suitability/applicability to measure UFPs in its scan range (10-237 nm). The reference SMPS (TSI-3938, CPC-TSI-3755) system was compared against a reference CPC (TSI-3750) measuring the total particle number (TPN). Another reference CPC (TSI-3750) was used in combination with catalytic stripper (CS) to simulate the solid particle number (SPN). Therefore, soot particles with varying parameters like particle number (PN), PNSD, fuels to gas ratio in soot generator (λ), and organic load (OL), were generated using a Mini-CAST (5303C) and aerosol conditioning facility of PTB, Germany. Furthermore, the impact of varying λ and PNSD on organic fractions of soot particles was evaluated through SPN / TPN, and finally a shrinking ratio was estimated based on ratio of GMD (Solid particles) to GMD (Total Particles) i.e., SGMD/TGMD.

Results & Discussion: The figure below presents our first findings for described metric, only λ = 0.9 (lean conditions) is shown here. Similar analyses were performed for λ = 1.3 (moderate), and 1.8 (fat), respectively. The TPN, SPN measured by reference CPCs and simultaneous cumulative particle number measured by reference SMPS (CS-, CS+) were in good agreement (within ±10%). Additionally, the SPN/TPN and SGMD/TGMD ratios decreased with decrease in the GMD, suggesting either a higher organic fraction or higher diffusion losses in CS at lower GMD.

References: 

[1]  https://doi.org/10.1016/j.envint.2023.107744 

[2]  https://dx.doi.org/10.3390/catal9070586

How to cite: Malik, A., Nowak, A., Rosahl, J., Eleftheriadis, K., and Gini, M.: Performance evaluation of CEN-SMPS with a novel fast scan mode for better identification of UFPs in MI-TRAP, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8370, https://doi.org/10.5194/egusphere-egu25-8370, 2025.

Several global and regional inventories have been developed in recent years, but none of them provide information on the uncertainties of the emissions. As part of the CAMS EvOlution project (CAMEO), we have developed a tool to evaluate the uncertainties of emissions from transportation in different countries around the world. This tool, the Copernicus Online Computation of Anthropogenic Emission Uncertainties (COCAU), is a web-based platform for exploring greenhouse gas (GHG) emissions and their uncertainties, with a focus on the transportation sector. Built with modern online technologies, COCAU enables users to filter and visualize emissions data interactively. The emissions are calculated based on emission factors and activity data collected through the CO2MVS Research on Supplementary Observations European project (CORSO) ensuring scientific rigor and reliability. This tool allows users to display emissions at various scales, from country-level to regional-level. We will discuss the COCAU tool and the data used to calculate the uncertainties, and present its features, such as customizable charts, interactive maps, and downloadable datasets in JSON and CSV formats, offering a comprehensive and interactive view of emissions data.

How to cite: Merly, H., Doumbia, T., Liousse, C., Guevara, M., and Granier, C.: A web-based tool for exploring and visualizing GHG emissions from transportation and their uncertainties: the Copernicus Online Computation of Anthropogenic emission Uncertainties (COCAU)., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8613, https://doi.org/10.5194/egusphere-egu25-8613, 2025.

EGU25-8748 | Orals | AS3.30

Real-Time Source Apportionment with ACSM-Xact-Aethalometer (AXA) and SoFi RT 

Manousos Manousakas, Olga Zografou, Francesco Canonaco, Evangelia Diapouli, Stefanos Papagiannis, Maria Gini, Vasiliki Vassilatou, Anna Tobler, Stergios Vratolis, Kaspar Daelenbach, Jay Slowik, Andre Prevot, and Konstantinos Eleftheriadis

Particulate matter (PM) air pollution poses a significant threat to public health and the environment, particularly in urban areas. To mitigate these impacts, understanding the sources of PM through accurate source apportionment (SA) is essential for informed air quality management. Traditional SA methods rely on offline data collection, which delays responses to pollution events. However, advancements in monitoring technology have made real-time SA possible, providing continuous and detailed insights into pollution contributors. This study introduces the first deployment of the ACSM-Xact-Aethalometer (AXA) system combined with SoFi RT software for real-time PM source apportionment (RT-SA) in Athens, Greece.

The AXA system integrates chemical, elemental, and black carbon data, offering a holistic view of PM sources in an urban context. The analysis identified traffic emissions as the largest PM contributors, while secondary components, such as organic aerosols, sulfate, nitrate, and ammonium, accounted for for over 50% of the total PM mass. Primary emissions from sources like biomass burning and cooking contributed around 10% each, while natural sources such as sea salt and dust made up the remainder. By capturing organic, elemental, and black carbon fractions, the AXA setup provides a comprehensive profile of PM composition.

The use of SoFi RT software enables continuous, near-instant SA with automated data analysis, enhancing the identification of pollution sources in real time. The findings demonstrate the system’s capability to accurately detect key PM contributors and highlight its potential to revolutionize urban air quality monitoring, paving the way for targeted interventions to reduce PM pollution.

How to cite: Manousakas, M., Zografou, O., Canonaco, F., Diapouli, E., Papagiannis, S., Gini, M., Vassilatou, V., Tobler, A., Vratolis, S., Daelenbach, K., Slowik, J., Prevot, A., and Eleftheriadis, K.: Real-Time Source Apportionment with ACSM-Xact-Aethalometer (AXA) and SoFi RT, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8748, https://doi.org/10.5194/egusphere-egu25-8748, 2025.

EGU25-8815 | Orals | AS3.30

Analysing High Resolution Ultrafine Particle Count Data to Differentiate Local Road Traffic from Background Contributions to Personal Exposure 

Roy M. Harrison, Seny Damayanti, Dimitrios Bousiotis, Arunik Baruah, and Francis D. Pope

During personal exposure monitoring, short-term peaks, or “spikes”, in pollutant concentration, were observed frequently in proximity to the local pollution sources, especially road traffic. This phenomenon may influence the overall exposure. The current study examined spikes in particle number concentration (PNC) to differentiate local from background contributions by eliminating spikes from the personal exposure dataset.

Personal exposures were measured on 33 walking trips alongside major and minor roads between 20th May and 26th June 2024, in a heavily populated residential area close to the University of Birmingham. A portable miniature particle counter (Testo DiSCmini) was carried in a backpack, measuring particle number concentration with a high temporal resolution of 1 second. Particle Number Count data (10-100nm) were also collected with a reference-grade instrument (Scanning Mobility Particle Sizer (SMPS)) at a local urban background air quality monitoring station.

The time series of PNC contained short-term excursions (spikes) to higher concentrations.  There were several steps involved in removing the spikes from the dataset including baseline calculation, spike identification and removal, and background data interpolation. The first step was done using a moving median with 10 minutes average before and after all data points. Secondly, a threshold i.e., 10% of the baseline was chosen which can capture spikes optimally based on visual observation. Data above the threshold was subsequently identified as spikes and excluded from the data set. Finally, the edited background data was interpolated using a linear method.

The results show that roughly 25% (by time) of the walking data was categorized as short-term peaks. Removal resulted in a reduction of the overall average PNC by nearly 19%. Temporal variation according to weekday/weekend and period of the day revealed a decline in average PNC ranges of 12-34%, with the most significant fall of 34% occurring during weekday mornings (MWD), due to a substantial number of PNC spikes observed during this period.  PNC measured during walking was scaled to SMPS-equivalent values using data from an instrument intercomparison and was compared to urban background SMPS data during measurement. It was shown that the average of corrected de-peaked PNC from walking (11801±8357 #/cm³) was 9% higher than that recorded in the urban background (10816±6711 #/cm³). Local diffuse sources are probably responsible for this higher concentration, while the spikes appear to be due to road traffic emissions and locally operating sources such as off-road mobile machinery.

By separating short-term peak concentrations from personal exposure monitoring data, the data indicate that limiting pollutant hotspots, especially in areas with high population density, may reduce exposure to pollutants, particularly those with significant geographical and temporal variability such as ultrafine particles (UFP).

How to cite: Harrison, R. M., Damayanti, S., Bousiotis, D., Baruah, A., and Pope, F. D.: Analysing High Resolution Ultrafine Particle Count Data to Differentiate Local Road Traffic from Background Contributions to Personal Exposure, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8815, https://doi.org/10.5194/egusphere-egu25-8815, 2025.

EGU25-8854 | ECS | Orals | AS3.30

NOx emissions from inland shipping using plume cross-sections obtained from MAX-DOAS measurements 

Simona Ripperger-Lukošiūnaitė, Steffen Ziegler, Philipp Eger, Sebastian Donner, Steffen Beirle, Peter Hoor, and Thomas Wagner

Nitrogen Oxides (NO­x, i.e., NO and NO2) are major contributors to local air pollution. They negatively affect human health and play an essential role in tropospheric chemistry. While air quality concerns are often focusing on heavy road traffic and seagoing ships, long-lasting diesel engines of inland waterway vessels can also be strong NOx emitters and might represent a significant local pollution source. The Rhine River, Europe’s most important and busiest inland waterway, connects key seaports, industrial hubs, and densely populated cities, highlighting its importance for emission monitoring. Emissions from inland ships are concentrated near waterways, making their effect on air quality particularly relevant in residential areas located along intensively used waterways. Understanding and quantifying these emissions is important to assess inland shipping’s impact on local air quality.

 

In this work, we analyse NOx emissions from inland ship exhaust plumes based on measurements performed in cooperation with the Federal Institute of Hydrology at the Rhine River in Koblenz, Germany. Over the course of more than one year, NO2 measurements were taken using two MAX-DOAS (Multi-AXis Differential Optical Absorption Spectroscopy) instruments, providing high temporal resolution (6-8 seconds) and a large dataset for good statistical analysis. This remote sensing technique captures ship exhaust plumes from a riverbank while the ships pass by the line of sight of the instrument, making the detection of ship emissions less dependent on wind direction compared to using in-situ measurements. By measuring NO2 column densities at different elevation angles, MAX-DOAS provides not just a single average value for the entire plume, but information about vertical NO2 distribution within the plume. Here, we estimate the emission flux through the cross-section of the plume (in grams per second) based on measured column densities, ship position information, and wind data. Retrieved emission rates then can be converted to units in grams per kilowatt-hour, allowing for a direct comparison with European emission standards.

How to cite: Ripperger-Lukošiūnaitė, S., Ziegler, S., Eger, P., Donner, S., Beirle, S., Hoor, P., and Wagner, T.: NOx emissions from inland shipping using plume cross-sections obtained from MAX-DOAS measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8854, https://doi.org/10.5194/egusphere-egu25-8854, 2025.

EGU25-8939 | Posters on site | AS3.30

Secondary aerosol formation potential of vehicles representing different transport sectors 

Hilkka Timonen, Päivi Aakko-Saksa, Luis Barreira, Petteri Marjanen, Leila Simon, Anssi Järvinen, Hannu Kuutti, Wojciech Honkisz, Katariina Kylämäki, Milja Jäppi, Laura Salo, Matti Rissanen, Tereza Červená, Michal Vojtisek-Lom, Jan Topinka, Piotr Bielaczyc, Topi Rönkkö, and Sanna Saarikoski

The exhaust emissions from transport sector as well as their air quality impacts have been steadily decreasing in urban areas due to the more stringent emission limits. The secondary aerosol formation process from inorganic and organic gaseous precursors emitted by traffic remains poorly characterized and is likely very different for different vehicles. The aim of this study is to explore the influence of fuel, engine technology and aftertreatment systems on the secondary aerosol formation potential from exhaust emissions by different traffic sectors.  

The measurement data utilized in this abstract originates both scientific literature and from various national and international projects spanning the period from 2014 to 2024, including both laboratory and field studies. In studies, secondary aerosol formation was investigated employing an oxidation flow reactor (OFR). In addition, in most studies a comprehensive characterization of the physical (e.g. particle number, size distribution, PM, volatility) and chemical properties (e.g. BC, organics, inorganics) of fresh (before OFR) and aged exhaust (after OFR) was conducted. The secondary aerosol formation potential is compared between transportation sectors as well as for different fuels, engine and aftertreatment technologies. The results from the conducted campaigns show a large variation in secondary aerosol formation potential for different vehicles and vessels. While conducted studies contribute to the analysis of factors influencing secondary aerosol formation, they also indicated significant gaps in our understanding regarding the secondary aerosol formation.

This work was supported by the European Union’s horizon Europe research and innovation programme under grant agreement No 101096133 (PAREMPI: particle emission prevention and impact: from real-world emissions of traffic to secondary PM of urban air).

How to cite: Timonen, H., Aakko-Saksa, P., Barreira, L., Marjanen, P., Simon, L., Järvinen, A., Kuutti, H., Honkisz, W., Kylämäki, K., Jäppi, M., Salo, L., Rissanen, M., Červená, T., Vojtisek-Lom, M., Topinka, J., Bielaczyc, P., Rönkkö, T., and Saarikoski, S.: Secondary aerosol formation potential of vehicles representing different transport sectors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8939, https://doi.org/10.5194/egusphere-egu25-8939, 2025.

To reduce the primary emissions of traffic and therefore the harm caused to humans and the environment, alternative fuels, for example Compressed Natural Gas (CNG), have been developed. However, the amount of secondary particles, that are formed in the atmosphere from gaseous precursors such as Volatile Organic Compounds (VOC), can even exceed primary particle emissions. Their emissions and formation mechanisms remain poorly understood.

As a part of a larger project, the primary and secondary emissions of seven passenger cars were measured. In this study, three cars are compared: a Euro 6d-TEMP CNG (model year 2020, gasoline as a backup fuel), a Euro 6b gasoline (2015) and a Euro 4 diesel (2006) vehicle. All the vehicles had an oxidation catalyst, but no particulate filter. The measurements were done on a chassis dynamometer, which was in a temperature-controlled test cell with test temperatures of -9, 23, and 35 ˚C. The test cycle simulated Real Driving Emissions (RDE) and was 72 min and 47 km long.

The raw exhaust was diluted with a porous tube diluter (PTD) and an ejector diluter (ED), and then characterized physically and chemically. For example, the VOC spectra of the fresh exhaust was measured with a Proton Transfer Reaction Time of Flight mass spectrometer PTR-ToF-CIMS (VOCUS, Aerodyne Research, US). This instrument allows high time and mass resolution analysis of the spectra.

Based on the preliminary results, the VOC composition in the CNG and the diesel car exhaust was similar, with emphasis on oxygenated VOCs. In contrast, the gasoline car emitted more aromatic, polyaromatic and aliphatic hydrocarbons. The VOC concentrations from the CNG car were on average lower than from the diesel car, but the CNG car emitted higher concentrations at cold start and at highway. The VOC concentrations from the gasoline vehicle were also highest at cold start and at highway during the cycle.

In summary, the CNG vehicle seems to emit low VOC concentrations, and the emitted compounds have low secondary aerosol formation potential. However, at cold start and during high engine load, the concentrations increase greatly, potentially due to gasoline usage. This study provided new information about the VOC composition in a CNG car exhaust and supported previous studies in terms of diesel and gasoline cars.

 

ACKNOWLEDGEMENTS: This work was supported by the European Union’s Horizon Europe research and innovation programme under grant agreement No 101096133 (PAREMPI: Particle emission prevention and impact: from real world emissions of traffic to secondary PM of urban air).

How to cite: Kylämäki, K. and the PAREMPI project team: Volatile Organic Compound concentrations in the exhaust of a natural gas, a gasoline, and a diesel passenger car under various driving conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9086, https://doi.org/10.5194/egusphere-egu25-9086, 2025.

The summer of 2023 has seen an anomalous increase in temperatures even when considering the ongoing greenhouse-gases driven warming trend. Here we demonstrate that regulatory changes to sulfate emissions from international shipping routes, which resulted in a significant reduction in sulfate particulate released during international shipping starting on January 1 2020, might have been a major contributing factor to the monthly surface temperature anomalies during the last year. We do this by including in Community Earth System Model (CESM2) simulations the appropriate changes to emission databases developed for the Climate Model Intercomparison Project version 6 (CMIP6). The aerosol termination effect simulated by the updated CESM2 simulations of +0.14 ± 0.07 W/m2 and 0.08K ± 0.03K is consistent with observations of both radiative forcing and surface temperature, manifesting a similar delay as the one observed in observational datasets between the implementation of the emission changes and the anomalous increase in warming. Our findings highlight the importance of considering realistic near-future changes in short-lived climate forcers for future climate projections, such as for CMIP7, for an improved understanding and communication of short-term climatic changes.

How to cite: Visioni, D. and Quaglia, I.: Modeling 2020 regulatory changes in international shipping emissions helps explain 2023 anomalous warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10668, https://doi.org/10.5194/egusphere-egu25-10668, 2025.

EGU25-11307 | Orals | AS3.30

Warming effects of reduced sulfur emissionsfrom shipping 

Masaru Yoshioka, Daniel Grosvenor, Ben Booth, Colin Morice, and Ken Carslaw

The regulation introduced in 2020 that limits the sulfur content in shipping fuel has reduced sulfur emissions over global open oceans by about 80 %. This is expected to have reduced aerosols that both reflect solar radiation directly and affect cloud properties, with the latter also changing the solar radiation balance. Here we investigate the impacts of this regulation on aerosols and climate in the HadGEM3-GC3.1-LL climate model. The global aerosol effective radiative forcing caused by reduced shipping emissions is estimated to be 0.13 W m−2, which is equivalent to an additional ∼50 % to the net positive forcing resulting from the reduction in all anthropogenic aerosols from the late-20th century to the pre-2020 era. Ensembles of global coupled simulations from 2020–2049 predict a global mean warming of 0.04 K averaged over this period. Our simulations are not clear on whether the global impact is yet to emerge or has already emerged because the present-day impact is masked by variability. Nevertheless, the impact of shipping emission reductions either will have already committed us to warming above the 1.5 K Paris target or will represent an important contribution that may help explain part of the rapid jump in global temperatures over the last 12 months. Consistent with previous aerosol perturbation simulations, the warming is greatest in the Arctic, reaching a mean of 0.15 K Arctic-wide and 0.3 K in the Atlantic sector of the Arctic (which represents a greater than 10 % increase in the total anthropogenic warming since pre-industrial times).

How to cite: Yoshioka, M., Grosvenor, D., Booth, B., Morice, C., and Carslaw, K.: Warming effects of reduced sulfur emissionsfrom shipping, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11307, https://doi.org/10.5194/egusphere-egu25-11307, 2025.

EGU25-11614 | ECS | Orals | AS3.30

A Dedicated European Emission Inventory for Road Transport with special focus on Ultrafine Particles and Semi- and Intermediate-Volatile Organic Compounds 

Marya el Malki, Antoon Visschedijk, Tilman Hohenberger, and Jeroen Kuenen

Despite significant reductions in emissions from road transport driven by air quality regulations, this sector continues to rank among the largest contributors to air pollution globally and within Europe, with profound implications for human health. For certain pollutants, including ultrafine particles (UFP) and semi- and intermediate-volatility organic compounds (S/IVOCs), emission control regulations are lagging behind. In the case of particle number, solid particles are regulated by the Euro standards but the contribution to volatile particle formation is not. This is partly due to insufficient understanding of their emission levels and health impacts. S/IVOCs, which occupy a volatility spectrum between non-methane volatile organic compounds (NMVOCs) and particulate matter (PM), are particularly concerning as they are efficient precursors to secondary organic aerosols (SOAs).

In this study, we present the development and refinement of a high-resolution (6×6 km) road transport emission inventory for Europe, undertaken as part of the EASVOLEE and RI-Urbans projects, by combining information on vehicle mileages by country and emission factors for all major air pollutants, including newly derived factors for total particle number (TPN) and S/IVOCs.

Through a comprehensive literature review, we derived updated and more detailed TPN emission factors that consider fuel injection technologies and particle filters for petrol vehicles and the effect of regeneration for diesel particle filters. To improve the robustness of these factors, they will be further refined using results from measurement campaigns conducted under the EASVOLEE project, including real-world driving and lab measurements. Cold starts and non-exhaust emissions were explicitly modelled for all pollutants. For S/IVOCs, emission profiles were introduced to specify the total SVOC and IVOC mass fractions as a proportion of NMVOC emissions. Furthermore, the spatial distribution of emissions was refined to achieve a more representative allocation of road transport emissions.

Our initial findings highlight that, while PM2.5 emissions from exhaust road transport are less significant compared to other sources, TPN emissions remain a substantial contributor, second only to shipping. Another notable distinction is the strong contribution of non-exhaust sources to PM mass compared to their marginal influence on TPN. This trend aligns with existing research, as non-exhaust emissions predominantly consist of larger particles. Furthermore, cold starts, while varying by pollutant, were found to contribute to roughly 10% of total emissions, emerging as a key consideration for emission inventories, considering that these emissions predominantly occur in urban areas. For the S/IVOC profiles, IVOCs account for approximately 50% of NMVOC emissions from diesel vehicles and 5% from petrol vehicles, while SVOCs contribute 9% and 1.5%, respectively.

These advancements directly support the efforts of modellers to improve the quantification of particulate number concentrations and SOA formation. By enhancing the accuracy of emission data, this work underpins the development of robust policies in line with the EU’s new Ambient Air Quality Directive, which tightens pollutant limit values and drives progress toward cleaner air and improved public health.

How to cite: el Malki, M., Visschedijk, A., Hohenberger, T., and Kuenen, J.: A Dedicated European Emission Inventory for Road Transport with special focus on Ultrafine Particles and Semi- and Intermediate-Volatile Organic Compounds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11614, https://doi.org/10.5194/egusphere-egu25-11614, 2025.

EGU25-11826 | ECS | Posters on site | AS3.30

Transport and Ultrafine Particles: Source Apportionment Across Europe 

Elena Poulikidi, David Patoulias, and Spyros N. Pandis

Ultrafine particles (UFPs) are a critical component of urban air pollution, with potentially significant implications for public health due to their ability to translocate to different organs in the human body. Transportation remains a dominant source of  UFPs. This study investigates the contribution of various emission sources, with a particular focus on transportation, to UFP concentrations across Europe. The results provide insight into spatial and seasonal variability of UFP sources, with detailed analyses for Barcelona, Paris, and Athens.

PMCAMx-UF simulates both the number and mass distributions of atmospheric aerosols (Fountoukis et al., 2012). It incorporates processes such as horizontal and vertical advection, dispersion, wet and dry deposition, nucleation, coagulation, and gas-phase chemistry. The Posner and Pandis (2015) zero-out source apportionment methodology was applied using PMCAMx-UF for January and July 2019, with a 36 x 36 km grid resolution for Europe and 1 x 1 km for each city studied.

Our simulations highlight the significant contribution of transportation to UFP concentrations, with notable seasonal and spatial variations.  The PMCAMx-UF model’s predictions were compared with air quality monitoring data, demonstrating an overall good performance with some notable underprediction of N10 concentrations in certain urban areas.

 

Fountoukis, C., Riipinen, I., Van Der Gon, H. D., Charalampidis, P. E., Pilinis, C., Wiedensohler, A., O’Dowd, C., Putaud, J. P., Moerman, M., & Pandis, S. N. (2012). Simulating ultrafine particle formation in Europe using a regional CTM: contribution of primary emissions versus secondary formation to aerosol number concentrations. Atmospheric Chemistry and Physics, 12(18), 8663–8677.

Posner, L. N., & Pandis, S. N. (2015b). Sources of ultrafine particles in the Eastern United States. Atmospheric Environment, 111, 103–112. https://doi.org/10.1016/j.atmosenv.2015.03.033

How to cite: Poulikidi, E., Patoulias, D., and Pandis, S. N.: Transport and Ultrafine Particles: Source Apportionment Across Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11826, https://doi.org/10.5194/egusphere-egu25-11826, 2025.

EGU25-13035 | Orals | AS3.30

Mineral characterization of a major source of the traffic-related non-exhaust emissions 

Beatrix Jancsek-Turóczi, András Hoffer, János Osán, and András Gelencsér

Nowadays the relative contribution of non-exhaust emissions (NEEs) to the total traffic-related PM10 has increased to 60–90% (Piscitello et al., 2021) due to engine developments, tightening emission standards and the growing share of electric vehicles. Among the major sources of NEEs, urban road dust is a complex mixture of particles from different primary sources, such as resuspension from soil, construction and demolition works and traffic-related sources. The respirable fraction of urban road dust may contain potentially hazardous pollutants which may cause adverse health effects.

A special mobile sampling unit (Jancsek-Turóczi et al., 2013) was successfully deployed to collect resuspended and respirable urban road dust (PM1−10) samples for source apportionment studies. The availability of bulk PM1−10 fraction of the collected road dust without a filter matrix facilitated the application of XRD method for the determination of the mineralogical composition. The identified main crystalline phases (calcite, quartz, dolomite, chlorite, plagioclase, alkali feldspar, mica and gypsum) in the PM1−10 fraction of resuspended road dust can be attributed to two major sources, namely construction/demolition works and soil resuspension, with a significant degree of overlap.

In order to further differentiate between the two major sources, resuspended road dust samples were collected on construction and demolition sites and from their vicinity in order to determine specific mineralogical tracer of construction works by XRD analysis. In three of the six urban road dust samples, we have successfully identified pseudowollastonite, a mineral phase of CaSiO3 that is exclusively formed in high temperature processes of cement production (Santos et al., 2019). It can occur in relatively abundant in slags and cement, but is virtually absent in native rocks since its formation requires a complex interplay of specific factors that barely happens in nature (Seryotkin et al., 2012). In our study we prove that this crystalline phase can be an excellent tracer for assessing the contribution of the construction and demolition works to common mineral particles found in ambient PM10 and resuspended road dust.

 

This work was supported by the Sustainable Development and Technologies National Programme of the Hungarian Academy of Sciences (FFT NP FTA) and the János Bolyai Research Scholarship of the Hungarian Academy of Sciences.

 

Piscitello, A., Bianco, C., Casasso, A., Sethi, R. (2021) Sci. Total Environ. 766, 144440.

Jancsek-Turóczi, B., Hoffer, A., Nyírő-Kósa, I., Gelencsér, A. (2013) J. Aerosol Sci. 65, 69-76.

Seryotkin, Y.V., Sokol, E.V., Kokh, S.N. (2012) Lithos 134-135, 75-90.

Santos, D., Santos, R.L., Pereira, J., Horta, R.B., Colaco, R., Paradiso, P. (2019) Materials 12, 3457.

How to cite: Jancsek-Turóczi, B., Hoffer, A., Osán, J., and Gelencsér, A.: Mineral characterization of a major source of the traffic-related non-exhaust emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13035, https://doi.org/10.5194/egusphere-egu25-13035, 2025.

EGU25-14936 | Posters on site | AS3.30

Understanding the impacts of climatic background on winter PM2.5 over East Asia 

Sunmin Park and Jae-Seung Yoon

Previous studies have explored the exchange effect between atmospheric condition and PM2.5 variation to understand their relationship. However, most works pay attention to a specific date or month when a severe pollution event happened. East Asia has experienced rapid economic development, well known for extreme PM2.5 concentration events, particularly in winter. In this study, we applied EOF analysis to classify high and low PM2.5 years from 1982-2022. We use three reanalysis data such as NOAA OISST, MERRA2, and ERA5 for sea surface temperature, PM2.5, and climate factors including temperature, precipitation, and winds. The first mode EOF explains winter PM2.5 variation with 55.85% (2nd mode: 18.4% and 3rd mode: 5.6%). The first mode of EOF timeseries indicates eleven high years from 2002 to 2013 and nine low years from 1991 to 1999 (over ±0.5σ). The high PM2.5 events are related to sea surface temperature (PDO-like pattern) and wind over the eastern Pacific. Vertical velocity is not a key factor during the winter but has a weak impact on vertical dispersion.

How to cite: Park, S. and Yoon, J.-S.: Understanding the impacts of climatic background on winter PM2.5 over East Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14936, https://doi.org/10.5194/egusphere-egu25-14936, 2025.

EGU25-14959 | ECS | Orals | AS3.30

Fresh and Secondary Exhaust Emission Outcomes of Lubricating Oil Blended into Marine Fuel 

Petteri Marjanen, Katariina Kylämäki, Milja Jäppi, Lassi Markkula, Teemu Lepistö, Rabbia Asgher, Sana Farhoudian, Hannu Kuutti, Luis Barreira, Tereza Červená, Michal Vojtisek-Lom, Wojciech Honkisz, Hilkka Timonen, Päivi Aakko-Saksa, and Topi Rönkkö

Pollutants emitted by internal combustion engines harm human health and contribute to climate change. Diesel engines, commonly used to power ships, are a significant source of these emissions. Eichler et al. (2017) identified lubricating oil as a major contributor to ship exhaust particles. As the shipping industry transitions to decarbonized fuels, the combustion of lubricating oil may remain a source of organic aerosol emissions. This study highlights the role of minimizing lubricating oil combustion in reducing exhaust emissions from ships.

In this study we used a small diesel generator to produce aerosol emissions from marine fuels. Lubricating oil was blended into marine distillate fuel (DMB) to investigate its impact on exhaust emissions. Our results revealed that the addition of lubricating oil led to increased particle number emissions, a marked rise in nucleation-mode particle formation and a reduction in black carbon emissions. We also examined the effects on volatile organic compound emissions (with a PTR-MS), secondary aerosol formation potential (with an OFR), particle chemical composition (with a SP-AMS), and toxicity (with an air-liquid interface). These results, currently under analysis, will be presented in due course.

How to cite: Marjanen, P., Kylämäki, K., Jäppi, M., Markkula, L., Lepistö, T., Asgher, R., Farhoudian, S., Kuutti, H., Barreira, L., Červená, T., Vojtisek-Lom, M., Honkisz, W., Timonen, H., Aakko-Saksa, P., and Rönkkö, T.: Fresh and Secondary Exhaust Emission Outcomes of Lubricating Oil Blended into Marine Fuel, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14959, https://doi.org/10.5194/egusphere-egu25-14959, 2025.

EGU25-15145 | Orals | AS3.30

Comprehensive characterization of organic aerosol in a traffic environment 

Sanna Saarikoski, Minna Aurela, Jarkko V Niemi, Luis Barreira, Hanna E Manninen, Topi Rönkkö, and HIlkka Timonen

A substantial fraction of submicron particulate matter in urban areas consists of organic aerosol (OA). This study aimed to elucidate the chemical characteristics and sources of OA at a traffic location in Helsinki, Finland, using four datasets collected from 2018 to 2024. The measurement site was located at the curbside of Mäkelänkatu (Helsinki Supersite), maintained by the Helsinki Region Environmental Services (HSY). OA composition and mass size distribution were measured using a Soot Particle Aerosol Mass Spectrometer, while Positive Matrix Factorization was used to separate OA into different types.

The results showed that traffic predominantly produces two types of OA: hydrocarbon-like OA (HOA) and traffic-related oxygenated OA (Tr-OOA), each contributing 10–18% to the total OA. HOA, consisting mostly of hydrocarbon ions, peaked typically during the morning rush hour between 7 and 9 am. Tr-OOA peaked later in the morning, and was more oxygenated than HOA. Tr-OOA showed significant signals for C2H4O2+ (at m/z 60) and C3H5O2+ (at m/z 73), which are typically associated with biomass burning OA (BBOA). Additionally, Tr-OOA had a notable signal for C2H5O2+ (m/z 61), especially high during the winter 2022 campaign. Besides HOA and Tr-OOA, semi-volatile oxygenated OA (SV-OOA) also appeared somewhat related to traffic emissions, though its secondary nature suggested a stronger link to regional pollution than local traffic emissions.

The specific origin of Tr-OOA remained unclear. However, it could be somewhat atmospherically processed, as its concentration stayed elevated a few hours longer than HOA in the morning, and its mass size distribution peaked at a larger size than HOA. The hydrocarbon ratios in the mass spectra of Tr-OOA suggested a connection to modern vehicles with efficient exhaust after-treatment systems, which operate later in the morning than heavy-duty vehicles or diesel buses.

This study provides a comprehensive view of OA in an urban environment. The novel information on sources and size distributions will enhance the understanding of urban OA and support air quality authorities and decision-makers in finding effective measures to reduce the harmful effects of urban particulate matter.

This work was supported by the European Union’s Horizon Europe research and innovation programme under grant agreement No 101096133 (PAREMPI) and No 101036245 (RI-URBANS).

How to cite: Saarikoski, S., Aurela, M., Niemi, J. V., Barreira, L., Manninen, H. E., Rönkkö, T., and Timonen, H.: Comprehensive characterization of organic aerosol in a traffic environment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15145, https://doi.org/10.5194/egusphere-egu25-15145, 2025.

EGU25-15203 | ECS | Orals | AS3.30

Towards real-world TRWP quantification: Combining a novel enclosed collection system with optical sensors to mitigate particle loss in tire emission measurements 

Miriam Chacón-Mateos, Manuel Löber, Nina Reijrink, Sven Reiland, Michael Eßl, Fabius Epple, Nina Gaiser, Franz Phillipps, and Markus Köhler

The significant impacts of tire and road wear particles (TRWP) on human health and the environment are increasingly being recognized. As a major source of microplastics, tire abrasion presents a pressing challenge, especially with the introduction of the Euro 7 standard, which will regulate brake and tire wear emissions for the first time. However, the absence of standardized methods for airborne TRWP measurements remains a critical barrier. Accurate quantification of airborne TRWP emissions requires complex measurement systems, which are often susceptible to particle loss during sampling.

As part of the “Models and Data for Future Mobility_Supporting Services (MoDa)” project, we aim to develop customer-oriented solutions to support the transformation of the transport sector. One such solution is AirQualityLive (AQL), designed to generate actionable insights from air quality data and enable evidence-based decision-making for cleaner and more sustainable mobility.

This study aimed to enhance measurement precision and mitigate particle loss during tire emission assessments conducted on a chassis dynamometer test bench during Worldwide Harmonized Light Vehicles Test Cycles (WLTCs) applied to a electric car. To achieve this, we designed an enclosed tire system (patent pending) and tested the integration of low-cost optical particle counters (OPCs) to measure airborne tire emissions. Two isokinetic particle collection systems were compared: (1) a closed collection system encapsulating the tire, isolating it from brake and environmental interferences, and (2) an open collection system. For that purpose, two parallel set-ups were mounted behind the back tires including for each system gravimetric measurements of PM10 and PM2.5, a cascade impactor with four particle size stages (>PM10, PM2.5–10, PM2.5, and <PM1), continuous particle number measurements using a mixing condensation particle counter (Brechtel Model 1720; 7 nm–2 µm), and an optical particle sizer (TSI Model 3330; 0.3–10 µm). The background concentration was monitored using an additional optical particle sizer. Furthermore, four low-cost optical particle counters (Alphasense Model OPC-N3; 0.35 - 40 µm) were deployed: one in each of the sampling set-ups, one for background monitoring, and one for optimal measurement placement studies.

The enclosed collection system demonstrated superior performance for UPF and PM measurements, collecting up to 10 times more particles in the 7 nm–2 µm size range and up to 3 times more particles in the 0.3–10 µm size range compared to the open system. Moreover, preliminary results indicate that calibrated sensors can effectively measure highly time-resolved PM coarse concentrations if placed in close proximity to the tire, being a cost-effective complement to the gravimetric and PM measurements.The results underscore the importance of the measurement system and how the combination of a closed collection system with direct PM sensor measurements can enhance the quantification of real-world tire emissions.  

How to cite: Chacón-Mateos, M., Löber, M., Reijrink, N., Reiland, S., Eßl, M., Epple, F., Gaiser, N., Phillipps, F., and Köhler, M.: Towards real-world TRWP quantification: Combining a novel enclosed collection system with optical sensors to mitigate particle loss in tire emission measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15203, https://doi.org/10.5194/egusphere-egu25-15203, 2025.

EGU25-15287 | Orals | AS3.30

Extremely low black carbon emissions from modern passenger cars and heavy-duty vehicles 

Topi Rönkkö, Milja Jäppi, Katariina Kylämäki, Petteri Marjanen, Wojciech Honkisz, Lassi Markkula, Laura Salo, Henna Lintusaari, Teemu Lepistö, Sanna Saarikoski, Anssi Järvinen, Kimmo Teinilä, Tereza Cervena, Michal Vojtisek, Matti Rissanen, Piotr Bielaczyc, Jan Topinka, Päivi Aakko-Saksa, and Hilkka Timonen

Black carbon (BC) emissions deteriorate air quality in cities and affect human population health. They are important also from climate point of view since atmospheric BC can absorb the solar radiation, affect cloud formation, and decrease ground albedo when deposited to snow or ice. BC is emitted to atmosphere from large variety of different anthropogenic sources. In respect of human exposure to the BC emissions, especially the on-road traffic emissions have had important role, which has led to tightening emission regulations and advanced emission mitigation actions.

In this study, we fulfil the data gaps found in recent literature review by new BC emission measurements. Measurements were done for passenger cars, including diesel, diesel-hybrid, gasoline, gasoline-hybrid, and CNG passenger cars, and for two heavy-duty diesel trucks. The measurements with passenger cars were conducted at BOSMAL, Poland, in the laboratory at a chassis dynamometer in a temperature-controlled test cell, where the used driving cycle simulated real driving emissions (RDE). Temperatures in the test cell were -9 °C, 23 °C and 35 °C. The experiments with heavy-duty trucks were conducted on road in Finland in winter-time conditions. In both measurements the exhaust gas was sampled partially and diluted before the characterization with an aethalometer (AE33, Magee). BC measurements were done parallel with large number of other measurements for trace gases and particles.

Our preliminary results indicate that the BC emissions of cars varied significantly depending on exhaust aftertreatment systems and driving situations. Very low BC emissions were measured for the cars and heavy-duty trucks with exhaust filtration, and ambient temperature variations had only minor effects on BC emission levels of the studied vehicles.

ACKNOWLEDGEMENTS: This work was supported by the European Union’s Horizon Europe research and innovation programme under grant agreement No 101096133 (PAREMPI: Particle emission prevention and impact: from real world emissions of traffic to secondary PM of urban air).

How to cite: Rönkkö, T., Jäppi, M., Kylämäki, K., Marjanen, P., Honkisz, W., Markkula, L., Salo, L., Lintusaari, H., Lepistö, T., Saarikoski, S., Järvinen, A., Teinilä, K., Cervena, T., Vojtisek, M., Rissanen, M., Bielaczyc, P., Topinka, J., Aakko-Saksa, P., and Timonen, H.: Extremely low black carbon emissions from modern passenger cars and heavy-duty vehicles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15287, https://doi.org/10.5194/egusphere-egu25-15287, 2025.

EGU25-15321 | Orals | AS3.30

Multi-model effective radiative forcing of the 2020 sulfur cap for shipping 

Ragnhild Bieltvedt Skeie, Rachael Byrom, Øivind Hodnebrog, Caroline Jouan, and Gunnar Myhre

Strict regulations on sulfur emissions from shipping, introduced in 2020, have drastically reduced SO2 emissions from international shipping. As SO2 is an aerosol precursor, this decline in anthropogenic emissions over the ocean will weaken the total aerosol effective radiative forcing (ERF) that historically has masked an uncertain fraction of the greenhouse gas induced warming.

Here, we use four global climate models and a chemical transport model to calculate the ERF resulting from an 80% reduction in SO2 emissions from international shipping relative to 2019 emission estimates. The individual model means range from 0.06 to 0.09 W m-2, corresponding to the ERF resulting from the increase in CO2 concentration over the last 2 to 3 years. The impact of this one-year drop in shipping emissions in 2020 is overshadowed by the long-term effects of reduced anthropogenic SO₂ emissions over the past decades, also in oceanic regions.

Using a single model, we investigate sensitivities due to Dimethyl sulfide (DMS) emissions and calculate the forcing from the emission reduction in 2020 as represented by the most recent emission inventories.

As for aerosol ERF in general, the ERF due to the new shipping sulfur regulations has a large uncertainty range. Although not fully quantified here, this will very likely be high considering the contribution of uncertainties in shipping SO2 emissions, the sulfur cycle, the modelling of cloud adjustments and the impact of interannual variability on the method for calculating radiative forcing.

How to cite: Skeie, R. B., Byrom, R., Hodnebrog, Ø., Jouan, C., and Myhre, G.: Multi-model effective radiative forcing of the 2020 sulfur cap for shipping, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15321, https://doi.org/10.5194/egusphere-egu25-15321, 2025.

EGU25-15514 | Orals | AS3.30

Measuring VOCs under real driving emission conditions by means of PTR-MS with active countermeasures for the humidity dependence 

Andreas Mauracher, Klaus Winkler, Rene Gutmann, and Philipp Sulzer

In this contribution, we present a dedicated instrument for monitoring volatile organic compounds (VOCs) under real driving emissions (RDE) conditions in line with the objectives of the EU and UKRI funded AEROSOLS project. This instrument fulfils the necessary criteria to be installed and operated in an SUV passenger car and to measure the emitted VOCs in a time-resolved manner. The VOCs are ionised and analysed using the proton transfer reaction (PTR) in combination with a time-of-flight (TOF) mass spectrometer. PTR mass-spectrometry (PTR-MS) has proven for many years to be a versatile ionisation technique for the quantification of VOCs, provided that the ion chemistry within the drift tube is well defined. However, for a number of compounds, the ion yield of the detected VOCs is dependent on humidity, making quantification difficult. There have been several attempts to solve this problem. One strategy is a labour- and time-intensive calibration at different humidity levels prior to the actual measurement and correction of the derived concentration after the measurement. Another strategy is to flood the drift tube with large amounts of water vapour, which contradicts the well-defined ion chemistry. Here we present the results of a study using a novel method that eliminates any influence of changing sample humidity on the measurements and has virtually no drawbacks. By introducing a controlled flow of water vapour directly into the PTR reaction region, the humidity is always kept constant. We present both laboratory-based studies on compounds of known humidity dependence and a long-time measurement of the outside air. In the former, we found a signal variation of about a factor of five between dry and 23 g m-3 absolute sample humidity for hydrogen sulphide, for example. By automatically injecting between 0.4 and 1.2 sccm of water vapour, the ion yield intensities for all compounds were decoupled from the sample humidity. In the latter study, we present a measurement during summertime, and despite the change from dry to humid conditions, the humidity in the PTR reaction region remained constant. Therefore, all changes in ion yield intensities represent true concentration changes and not artefacts due to varying water concentration in the air.

Acknowledgement: This research was co-funded by the European Union’s Horizon Europe research and innovation programme within the AEROSOLS project under grant agreement No. 101096912 and UK Research and Innovation (UKRI) under the UK government’s Horizon Europe funding guarantee [grant numbers 10092043 and 10100997].

How to cite: Mauracher, A., Winkler, K., Gutmann, R., and Sulzer, P.: Measuring VOCs under real driving emission conditions by means of PTR-MS with active countermeasures for the humidity dependence, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15514, https://doi.org/10.5194/egusphere-egu25-15514, 2025.

EGU25-15650 | ECS | Posters on site | AS3.30

Modelling the source contribution in the urban background of major air pollutants for 10 European cities in near-real time with LOTOS-EUROS 

Markus Thürkow, Richard Kranenburg, Sabine Banzhaf, Ilona Jäckel, and Martijn Schaap

Air quality is a key aspect of present environmental discussions. Due to the global networking of individual mobility and goods traffic as well as the long-distance transport of pollutants, air pollution now has not only a regional but also continental, European, and intercontinental dimensions. Today, millions of people currently living in polluted regions and are exposed to concentration levels of particulate matter and nitrogen oxides, leading to increased mortality rates. To protect human health, limit values have been set throughout Europe. The newly proposed limit values by the European commission for nitrogen dioxide and particulate matter are currently exceeded in most cities in Europe.

Substantial health benefits may be achieved through political mitigation strategies. This requires a strategy for monitoring cross-border air pollution and quantifying the contributions by source groups and regions of origin. For area-wide analyses and statements detailed, temporally and spatially high-resolution approaches based on chemistry transport models (CTMs) are typically carried out. CTMs aim to reproduce observed pollution variability as good as possible and can be used to forecast air pollution. CTMs can further be used to perform source attribution studies. However, near real-time (NRT) information on the contribution to air pollutants for different emission sources is so far limited.

Within the MI-TRAP project, we are setting up a NRT transport-oriented source apportionment service by provision of a daily analyses of hourly averaged concentrations of the priority pollutants (PM2.5, PM10, NO and NO2) in the urban background. By avoiding the use of city-specific proprietary data we will create a highly scalable solution for NRT mapping for cities in Europe. Through a nesting procedure we will provide the information of the background concentration in 10 cities on a ~1x1 km² horizontal grid resolution. The LOTOS EUROS model is used in a NRT operational configuration with meteorological input data from the German Weather Service (DWD) and with emissions as provided through CAMS-REG. Local emissions will be incorporated after a separate NRT emission modelling.

We will calculate the contribution of the different transport modes at the urban background scale using the source apportionment functionality of the LOTOS-EUROS model. The model contains a labelling approach for particulate matter and nitrogen oxides, allowing to flexibly track the contributions of predefined source categories for regions, sectors or combinations thereof. The contributions are calculated and tracked for each process description in the model and are valid for current atmospheric conditions, since all chemical transformations occur at the same concentrations of oxidants.

First results show that combustion processes from traffic, industry & energy production and residential heating are the most important domestic sources. The contributions from residential combustion, energy & industry, shipping and agriculture vary significantly from region to region and between the seasons. The largest variation from day to day and between night and day were observed for road transport. The contribution from non-road transport is most important along the main shipping routes.

We aim to present the results of the first model simulations and its evaluation against observations at the conference.

How to cite: Thürkow, M., Kranenburg, R., Banzhaf, S., Jäckel, I., and Schaap, M.: Modelling the source contribution in the urban background of major air pollutants for 10 European cities in near-real time with LOTOS-EUROS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15650, https://doi.org/10.5194/egusphere-egu25-15650, 2025.

EGU25-15808 | ECS | Posters on site | AS3.30

Model Study of Water Vapor and VOCs Adsorption on Bulk Jet Engine Soot Particles: Thermodynamic and Kinetic Aspects 

Yiheng Liang, Jon Bell, Luca Artiglia, Markus Ammann, and Jacinta Edebeli

Understanding the interactions between jet engine soot and exhaust plume vapor components, such as water vapour and benzene, is crucial for assessing post-combustion soot modification and the resulting impact on the environment and human health. This study focuses on the adsorption and desorption of single component exhaust plume species, namely, water vapor and volatile organic compounds (VOCs) with varying physicochemical properties, on soot particles derived from different combustion conditions, thus providing fundamental insights into the vapor-solid partitioning process and, therefore, the thermodynamic and kinetic mechanisms governing soot aging in jet exhaust plumes.

Model jet soot particles were synthesized by two methods: (1) enclosed spray combustion using Jet-Al fuel, which contains surface-adsorbed organic compounds, and (2) controlled oxidation of carbon black to mimic the physicochemical properties of jet soot without any adsorbed organic compounds to separate the role of soot core-shell structure, porosity, and surface chemistry on the solid-vapour partitioning process. Water vapor and VOCs adsorption isotherms, including components relevant to jet exhaust (e.g., toluene and benzene), were measured on soot powders using gravimetric dynamic vapor sorption under precisely controlled temperature and partial pressure conditions. Preliminary results indicated Type II isotherms for VOCs, driven by soot’s functional groups and particle surface area. Thermodynamic analysis of adsorption isotherms showed a moderate enthalpy of adsorption (31.8–45.4 kJ/mol) at low surface coverage and ambient temperature, consistent with a physisorption mechanism. Kinetic modeling using the linear driving force (LDF) and stretched exponential (SE) diffusion models showed that single aromatic species followed the LDF mechanism, displaying rapid adsorption kinetics (average k=0.016 s-1), indicative of interparticle void filling. In contrast, water vapor adsorption mainly followed the Fickian diffusion mechanism and was much slower (average k=0.001 s-1), possibly due to intraparticle diffusion of water vapor to oxygen functional groups on the edges of graphitic planes.

This study highlights how soot's physicochemical properties, such as pore size distribution, surface area, and surface chemistry, govern adsorption characteristics that control solid-vapor partitioning. By investigating the fundamental sorption mechanisms, these findings could advance our understanding of atmospheric jet soot aging and provide a foundation for modeling multicomponent vapor interactions in complex, real-world environments. The results could also inform strategies for mitigating the environmental and health impacts of aviation emissions through modifications to the combustion process.

How to cite: Liang, Y., Bell, J., Artiglia, L., Ammann, M., and Edebeli, J.: Model Study of Water Vapor and VOCs Adsorption on Bulk Jet Engine Soot Particles: Thermodynamic and Kinetic Aspects, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15808, https://doi.org/10.5194/egusphere-egu25-15808, 2025.

EGU25-15887 | Orals | AS3.30 | Highlight

Determining Volatile Organic Compounds (VOC) and Particulate Matter (PM1) shipping Emission Factors from land-based, high time resolution observations in an Emission Control Area of northern France 

Liselotte Tinel, Erwan Volent, Quentin Gunti, Barbara D'Anna, Joel F. De Brito, Marina Jamar, Brice Temime-Roussel, Jana Moldanova, Hilkka Timonen, Heidi Hellen, Grazia Lanzafame, Miikka Dal Maso, Véronique Riffault, and Stéphane Sauvage

Exhaust gases and particles from ships are a significant and growing contributor to the total emissions from transport. Globally, the sector is a significant contributor to global emissions of NOx and SO2.1,2 Recently, the International Maritime Organisation (IMO) has reduced the sulphur content of marine fuels globally through Annex VI of MARPOL, and sulphur emissions are further restricted in specific Sulphur Emission Control Areas (SECA), such as the English Channel between France and the UK. Similarly, NOx emission limits have been set for ships built after 2016 in NOx Emission Control Areas (NECA).

However, other pollutants such as Volatile Organic Compounds (VOCs) or Particulate Matter (PM), are not regulated in relation to ship emissions. Here, we present new emission factors (EFs) for regulated and non-regulated pollutants from ship emissions derived from a land-based measurement campaign in the port of Dunkirk, France in the framework of the PIRATE and SHIPAIR projects. A comprehensive suite of gas-phase and particulate-phase pollutants was investigated with a focus on VOCs, based on PTR-MS measurements, and PM1 composition, based on AMS measurements. About 150 plumes were detected from three similar ferries, and EFs were calculated for 84 pollutants.

Despite being located in an Emission Control Area (ECA) for SOx and NOx, we show that SO2 remains a reliable tracer of ship emissions for land-based measurements in the port area. A sensitivity test of the EF with respect to background considerations was performed, showing significant discrepancies depending on the method of background calculation. This underlines the importance of explicit background considerations in EF calculations.

The EF of the particulate phase is dominated by the organic fraction (OA), between 0.05 and 15.88 g/kg fuel, two to three orders of magnitude higher than nitrate and sulphate. Particle Number (PN) EFs vary between 1.08·1014 and 1.60·1017 part./kgfuel, with a unimodal mode centred at 90 nm. The VOC EFs are dominated by oxygenated species, such as acetaldehyde (30.7 - 404.8 mg/kg fuel). The second most emitted group of VOCs are C5 cyclic compounds, of which cyclopentane has the highest EF (12.8 - 439.6 mg/kg fuel). Aromatic VOCs, such as benzene, toluene and xylenes, are also detected, with EFs below 80 mg/kg fuel. We also present the emissions as a function of the navigation phases, suggesting that certain pollutants are emitted more during the arrival of the ferries than during their departure. In particular, the speciated VOC EFs are expected to improve current emission inventories.

References :

(1) Aakko-Saksa, P. T. et al. Reduction in greenhouse gas and other emissions from ship engines: Current trends and future options. Progress in Energy and Combustion Science 94, 101055 (2023). (2) Lehtoranta, K. et al. Particulate Mass and Nonvolatile Particle Number Emissions from Marine Engines Using Low-Sulfur Fuels, Natural Gas, or Scrubbers. Environmental Science and Technology 53, 3315–3322 (2019).

How to cite: Tinel, L., Volent, E., Gunti, Q., D'Anna, B., F. De Brito, J., Jamar, M., Temime-Roussel, B., Moldanova, J., Timonen, H., Hellen, H., Lanzafame, G., Dal Maso, M., Riffault, V., and Sauvage, S.: Determining Volatile Organic Compounds (VOC) and Particulate Matter (PM1) shipping Emission Factors from land-based, high time resolution observations in an Emission Control Area of northern France, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15887, https://doi.org/10.5194/egusphere-egu25-15887, 2025.

EGU25-15913 | Posters on site | AS3.30

Modelling of road contributions to PM2.5 and particle number concentrations with the LOTOS-EUROS model 

Astrid Manders, Ruud Janssen, Quinten Bohte, Tilman Hohenberger, Marya El Malki, Martijn Schaap, and Jeroen Kuenen

Road traffic is a major contributor to ultrafine particles and to PM2.5. The contribution of volatile organic compounds (VOCs), in particular of intermediate (IVOC) and low (SVOC) volatility is still uncertain. One reason is that species are not in emission inventories, another reason is that their pathways to form secondary organic aerosol (SOA) are strongly simplified in chemistry-transport models (CTM). In the framework of the EASVOLEE project, the CTM LOTOS-EUROS is being updated to better account for SOA formation and to better describe particle size and number from road traffic.

To this end, the LOTOS-EUROS model has recently been extended with the CB7 chemistry scheme. This scheme includes more VOC species and more detailed organic chemistry than the operational CBM4 chemistry scheme. This update also allows for the uptake of the developments of Manavi and Pandis (2022, 2024) to efficiently include SOA formation from road transport S/I/VOCs. In addition, the Volatility Basis Set (VBS) scheme was updated to make the model for SOA more accurate and faster. LOTOS-EUROS has adopted the SALSA2 module to model particle size distributions and particle number concentrations. In the near future, the organic vapors from the VBS calculations will be coupled to SALSA2 to investigate the impact of condensable organic vapors to ultrafine particle concentrations and size distributions. The model will then use new road emissions from the EASVOLEE project to represent the contribution of road transport to particle number concentrations and PM2.5. The envisaged model approach and preliminary results will be presented.

How to cite: Manders, A., Janssen, R., Bohte, Q., Hohenberger, T., El Malki, M., Schaap, M., and Kuenen, J.: Modelling of road contributions to PM2.5 and particle number concentrations with the LOTOS-EUROS model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15913, https://doi.org/10.5194/egusphere-egu25-15913, 2025.

EGU25-16555 | ECS | Orals | AS3.30

Emission Factors of Primary Pollutants from a Real-world Tunnel Measurement 

Yuantao Wang, Yanfang Chen, Michael Bauer, Damianos Pavlidis, Carolina Molina, Christian George, Athanasios Nenes, Spyros N. Pandis, David M. Bell, Imad El Haddad, and Andre S. H. Prevot

With over 1.6 billion vehicles worldwide, the combustion of fossil fuels is a major source of particulate matter (PM) and trace gases, which significantly contribute to air pollution, climate change and cause health burden. Heavy-duty vehicles (HDVs) constitute a small fraction of the global vehicle population but account for a disproportionately large share of total emissions when compared with light-duty vehicles (LDVs). However, uncertainty remains about which vehicle type contribute most to the emission factors (EFs) of various pollutants, particularly in Europe, where diesel technology has historically been favored for LDVs.

Because traditional engine emission tests may not accurately reflect the real-world emissions, there is a need for on-road, real-world emission assessments. In this study, we conducted a three-week measurement campaign in the Fréjus Road Tunnel using MIRO MGA-10, aethalometer and SMPS. We developed a practical method to determine the EFs of primary pollutants, including trace gases (NOx, CO2, CO, N2O, NH3, CH4), black carbon (BC), and ultrafine particles (UFP). The calculated EFs will be reported, and selected pollutant species will be compared with previously published data from Asia and America in equivalent units.

Figure 1 shows the results for the species mentioned, where HDV* indicates the proportion of HDVs to the total number of vehicles, taking into account the CO2 emissions from a single HDV and LDV. The results indicated that for most pollutant species, LDVs exhibited higher EFs than HDVs. However, HDVs emitted a higher fraction of N2O compared to LDVs. The EFs of NOx, CO, BC, and NH3 were consistent with previous studies conducted in Europe but lower than data reported from Asia and America. This study’s findings will raise public awareness and provide valuable insights for policymakers to develop strategies to mitigate emissions. 

Figure 1. Emission Factors (g/kg fuel)

How to cite: Wang, Y., Chen, Y., Bauer, M., Pavlidis, D., Molina, C., George, C., Nenes, A., N. Pandis, S., M. Bell, D., El Haddad, I., and S. H. Prevot, A.: Emission Factors of Primary Pollutants from a Real-world Tunnel Measurement, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16555, https://doi.org/10.5194/egusphere-egu25-16555, 2025.

EGU25-16715 | ECS | Orals | AS3.30

Evaluation of modeled versus observed road traffic source apportionment and aerosol oxidation potential using the EMEP MSC-W model 

Willem van Caspel, David Simpson, Gaëlle Uzu, Jean-Luc Jaffrezo, and Olivier Favez

The ability to induce oxidative stress has been suggested as a potential driver of the toxicity of
particulate matter (PM) exposure, being driven by aerosol composition and its relation to emission sources and chemical aging processes. PM originating from road traffic emissions has been especially implicated as being an important driver of aerosol oxidation potential (OP). In this work, road traffic PM simulated by the European Monitoring and Evaluation Programme (EMEP) Meteorological Synthesizing Centre – West (MSC-W) model is evaluated against source apportionment data across 19 sites in Europe. The source apportionment data includes information on both aerosol mass and source-specific OP of vehicular wear metals and primary and secondary vehicle exhaust organic aerosol, building upon the studies of Weber et al. (2021) and Daellenbach et al. (2020). Using the source-specific OP factors determined by the latter studies, the modeled contributions to OP are evaluated through comparisons with (OP) measurements for both the DTT and AA assays. We also briefly discuss the impact of model methodology, focusing on the choice of emission inventory, secondary organic aerosol formation scheme, and model resolution.

How to cite: van Caspel, W., Simpson, D., Uzu, G., Jaffrezo, J.-L., and Favez, O.: Evaluation of modeled versus observed road traffic source apportionment and aerosol oxidation potential using the EMEP MSC-W model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16715, https://doi.org/10.5194/egusphere-egu25-16715, 2025.

EGU25-17030 | Orals | AS3.30

How does aerosol grow in a real atmosphere? Measurement of aerosol precursor gases during a highly complex urban air simulation campaign SAPHIR-CHANEL 

Matti Rissanen, Rabbia Asgher, Shawon Barua, Sana Farhoudian, Siddharth Iyer, Avinash Kumar, Fariba Partovi, Netta Vinkvist, Georgios Gkatzelis, and Saphir-Chanel Team

Atmospheric secondary organic aerosol (SOA) formation is a tremendously complex phenomena which details keep eluding the researchers. The overwhelming combinatorics in gas-phase organic oxidation demands that in any real atmosphere the aerosol formation and growth occur by a network of interactions likely involving at least thousands of chemical compounds, making development of molecular level description a formidable task. By extension, any single component study will not be able to describe the inherent complexity of ambient gas-phase, necessitating the usage or evermore complex gas mixtures in order to bridge the gap to the real world processes.

In the present work we have performed investigations on probably the most complete gas mixture representing ambient urban conditions. The experiments were performed during the CHANEL measurement campaign during Summer 2024 in the large atmospheric simulation chamber SAPHIR in Forschungszentrum Jülich. The evolving gas mixture and aerosol formation were followed with an unusually large suite of instruments with around 10 chemical ionization mass spectrometers equipped with state-of-the-science detection techniques, including practically all the latest nanoparticle thermal desorption sampling instrumentation, and several nanoparticle sizing methods. The  data presented here were mainly obtained with a high-resolution orbitrap nitrate (NO3-) chemical ionization mass spectrometry (CIMS) with up to 120 000 mass resolution. The nitrate ionization is highly selective towards very polar and highly functionalized gas-phase compounds and thereby the data includes most oxygenated reaction products that are expected to play an important role in the generation of secondary aerosol. The experiment philosophy was to investigate very complex gas mixtures by including or excluding select mixture components to determine their individual impacts. Significant differences in the measured aerosol precursors were observed as a function of the complexity of the oxidized hydrocarbon pool.

How to cite: Rissanen, M., Asgher, R., Barua, S., Farhoudian, S., Iyer, S., Kumar, A., Partovi, F., Vinkvist, N., Gkatzelis, G., and Team, S.-C.: How does aerosol grow in a real atmosphere? Measurement of aerosol precursor gases during a highly complex urban air simulation campaign SAPHIR-CHANEL, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17030, https://doi.org/10.5194/egusphere-egu25-17030, 2025.

EGU25-17347 | Orals | AS3.30

Assessing Exhaust Gas Exposure in Real Driving Conditions with a Portable Air-Liquid Interface Chamber 

Michal Vojtisek-Lom, Lubos Dittrich, Tereza Cervena, Katerina Honkova, Tana Zavodna, Pavel Rössner, Anssi Järvinen, Hannu Kuutti, Wojciech Honkisz, Petteri Marjanen, Teemu Lepistö, Laura Salo, Katarina Kylämäki, Milja Jäppi, Kimmo Teinilä, Delun Li, Hilkka Timonen, Jan Topinka, Topi Rönkkö, and Päivi Aakko-Saksa and the PAREMPI project team

Responding to the outdoor air pollution being one of the gravest environmental and health hazards, mobile source emissions have been subject to scrutiny and emissions reduction efforts through increased efficiency, improved fuels, engine design, combustion control, exhaust aftertreatment, and traffic management. Assessment of the effects of various improvements on human health has been extended from basic laboratory measurements to testing under real-world (real-driving) conditions and to more health relevant metrics than, for example, total particulate mass.

Exposure of cell cultures at air-liquid interface (ALI), mimicking i.e. human lung surface, is believed to be one of the most realistic means to model toxicity of complex mixtures of pollutants on human health. While a number of ALI exposure systems have been developed, the complexity of the close cooperation of “emissions source” and toxicology groups and of the instrumentation are among the limiting factors of ALI use. This work combines these two approaches into portable, on-board ALI exposure chamber, capable of operating in a moving vehicle, delivering its exhaust to living cell cultures.

Cell cultures grown on commercially available 6 mm Transwell inserts are positioned in a compact, airtight exposure box, where the sample is evenly distributed across eight wells of a standard 24-well plate at 25 cm³/min per insert. In a 40x35x45 cm inner dimensions incubator, sample and control air, conditioned to 5% CO2, 37°C and >85% humidity, are drawn through 2-4 exposure boxes. Characterization with silver nanoparticles revealed 50% particle losses at 15 nm and deposition rate of approximately 1.5% at both 10 and 21 nm mean diameter. The system has undergone an extensive field validation, including 4 h of exposure and 2 h transport in a vehicle each day for 5 days, 5-day operation outside in vans and tents at -7 to +32°C.

In the PAREMPI project, the ALI exposure chamber has been mounted on an instrumented trailer used to measure emissions from two heavy-duty diesel trucks. Diluted exhaust produced during operation of the truck on public road in Finland in winter conditions was supplied to an advanced in vitro human airway epithelium MucilAir™ (Epithelix), a reconstituted, fully differentiated, and functional human respiratory tissue derived from primary cells, capable of long-term culture at the air-liquid interface, recognised as one of the closest representations of human lung tissue available for in vitro studies.

This is the first known use of ALI exposure chamber as a portable on-board system (PEMS). In other experiments within the project, the exposure chamber was sampling exhaust from light-duty vehicles of different types and emissions standards, operating on different fuels.

The portable exposure chamber, along with a field-deployable auxiliary mobile base including a small laminar flow box, additional incubator and freezer, can be easily used to study the toxicity of various emissions, effluents and polluted air, aiming for a more relevant toxicity measure than chemical composition alone.

The presentation will focus on the ALI exposure chamber design, with results of toxicological assays being presented at a later time.

ACKNOWLEDGEMENTS: EU Horizon Europe project 101096133 PAREMPI (tests), Czech Science Foundation grant 22-10279S (exposure chamber development)

How to cite: Vojtisek-Lom, M., Dittrich, L., Cervena, T., Honkova, K., Zavodna, T., Rössner, P., Järvinen, A., Kuutti, H., Honkisz, W., Marjanen, P., Lepistö, T., Salo, L., Kylämäki, K., Jäppi, M., Teinilä, K., Li, D., Timonen, H., Topinka, J., Rönkkö, T., and Aakko-Saksa, P. and the PAREMPI project team: Assessing Exhaust Gas Exposure in Real Driving Conditions with a Portable Air-Liquid Interface Chamber, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17347, https://doi.org/10.5194/egusphere-egu25-17347, 2025.

EGU25-17428 | ECS | Orals | AS3.30

Emissions of Volatile Methyl Siloxanes (VMSs) from Vehicles 

Yanfang Chen, Yuantao Wang, Siyao Yue, Michael Bauer, Damianos Pavlidis, Georgia Argyropoulou, Andreas Aktypis, Christos Kaltsonoudis, Philippe Wili, Pierre Comte, Danilo Engelmann, Imad El Haddad, Jay G. Slowik, Spyros N. Pandis, Andre S. H. Prevot, and David M. Bell

Volatile Methyl Siloxanes (VMSs) are anthropogenic molecules emitted from personal care products and industrial chemical products. Recent studies have found that concentrations of VMSs tend to be higher in densely populated urban areas, although research in large urban centers remains limited. Toxicity of such molecules remain uncertain with often conflicting reports. Previous literature has also reported the presence of long chain siloxanes in the particle phase from traffic emissions, and represented the first identification and quantification of siloxanes mostly likely emitted from vehicles.

In this study, the chassis dynamometer measurements were conducted to characterize the gaseous components from a variety of vehicles, including gasoline passenger cars, diesel passenger cars, and scooters. Time-resolved volatile organic compound (VOC) emissions during the cold start through a full driving cycle from different vehicles were chemically characterized by the Vocus proton-transfer-reaction time-of-flight mass spectrometer (VOCUS PTR-TOF-MS). The emission factors (EFs) of Hexamethylcyclotrisiloxane (D3), Octamethylcyclotrisiloxane (D4) and Decamethylcyclotrisiloxane (D5) were determined, and will be discussed with only specific types of vehicles emitting significant quantities of VMSs. Our results will also be compared to recent tunnel measurements, which demonstrated elevated concentrations of VMSs. Additionally, our results offer new insights into characterization and source appointment siloxanes in the atmosphere.

Figure 1. Real-time concentrations of D3, D4, D5, acetone, benzene, toluene, and driving cycle for a) a gasoline engine and b) a diesel engine.

 

How to cite: Chen, Y., Wang, Y., Yue, S., Bauer, M., Pavlidis, D., Argyropoulou, G., Aktypis, A., Kaltsonoudis, C., Wili, P., Comte, P., Engelmann, D., El Haddad, I., G. Slowik, J., N. Pandis, S., S. H. Prevot, A., and M. Bell, D.: Emissions of Volatile Methyl Siloxanes (VMSs) from Vehicles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17428, https://doi.org/10.5194/egusphere-egu25-17428, 2025.

EGU25-18158 | ECS | Posters on site | AS3.30

Exploring the oxidative potential of vehicles emissions from bench dynamometer to underground tunnels and parking lots  

Carolina Molina, Damianos Pavlidis, Giorgia Argyropoulou, Andrea Aktypis, Christina Christopoulou, Christos Kaltsonoudis, Yanfang Chen, Yuantao Wang, David M. Bell, Andre S. H. Prevot, Spyros Pandis, Christian George, Pierre Comte, and Athanasios Nenes

Health effects associated with aerosol exposure have been widely studied, demonstrating a positive association with mortality and poor health from a diversity of ailments. Emissions from vehicular traffic have been a major source of air pollutants, especially in urban and highly-populated environments, and emissions controls have considerably reduced the amount of aerosol from these sources. Nevertheless, policy based on mass concentration alone overlooks the possibility that certain aerosol sources may be more toxic than others. To address this, oxidative potential (OP) has been used as a metric that incorporates these properties, and ties in together mass and toxicity into a single metric that is a proxy of oxidative stress – thought to be a mechanism associated with adverse health effects from particulate matter exposure.

In this work, we focus on evaluating the oxidative potential of vehicular emissions using the dithiothreitol assay (DTT) during various field observations conducted as part of the EASOLEE project. Emissions from controlled environmental and driving conditions were characterized to compare diverse types of vehicles. Real driving conditions for large vehicle fleets inside a 12 km underground tunnel connecting France with Italy, as well as emissions from an underground parking lot were characterized. Our results showed a lower OP mass normalized (OPm) for fresh particles compared to aged particles. Diesel vehicles (47±67 pmol DTT min-1 μg-1) also exhibited a lower OPm when compared to scooters and gasoline vehicles (142±193 pmol DTT min-1 μg-1 and 130±75 pmol DTT min-1 μg-1 respectively). Measurements in the tunnel also revealed a lower OPm on average than previous studies (below 6 pmol DTT min-1 μg-1), possibly from the usage of a more modern ventilation system; in all cases, aging of the primary emissions led to more OP-active aerosol, with an enhancement of up to a factor of 10 in some cases. The implications therefore are that health impacts of particles away from their sources, especially certain types of vehicles, may be affected by increases of their toxicity from atmospheric aging.

How to cite: Molina, C., Pavlidis, D., Argyropoulou, G., Aktypis, A., Christopoulou, C., Kaltsonoudis, C., Chen, Y., Wang, Y., Bell, D. M., Prevot, A. S. H., Pandis, S., George, C., Comte, P., and Nenes, A.: Exploring the oxidative potential of vehicles emissions from bench dynamometer to underground tunnels and parking lots , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18158, https://doi.org/10.5194/egusphere-egu25-18158, 2025.

EGU25-18349 | Orals | AS3.30

Polyaromatic hydrocarbons from modern cars and trucks in real-driving at cold ambient temperatures: contributions in particulate matter and semi-volatile compounds  

Päivi Aakko-Saksa, Anssi Järvinen, Hannu Kuutti, Wojciech Honkisz, Katariina Kylämäki, Milja Jäppi, Petteri Marjanen, Matti Rissanen, Tereza Cervena, Michal Vojtisek, Luis Barreira, Sanna Saarikoski, Bo Strandberg, Taina Ohra-aho, Jan Topinka, Piotr Bielaczyc, Topi Rönkkö, and Hilkka Timonen

Vehicular particulate matter (PM) emissions have been studied widely in view of their composition and health effects, while less is known of the composition of the semi-volatile compounds (SVC) fraction. Furthermore, tightening exhaust emission standards in road-transport sector do not cover semi-volatiles or harmful polyaromatic hydrocarbons (PAHs) and their derivatives dibenzothiophenes (DBTs), nitrated (nitro-PAHs) and oxygenated (oxy-PAHs) PAHs present in vehicular exhaust. We studied PAH and their derivatives emissions from PM and SVC fractions collected from the exhaust from modern cars and trucks during real-driving at cold ambient temperatures.

PAHs were found in higher concentrations from the SVC fraction than from the PM. Carcinogenic heavy PAHs were present mainly in the PM, while lighter PAHs dominated the SVC fraction. Oxy-PAHs were found in samples and in some cases, nitro-PAHs and DBTs were also detected. PAH emissions originate mainly from incomplete combustion of fuel and lubricating oil.

Even for the most modern cars and trucks, PAH species were found in the exhaust. Many PAH groups detected are not included in the air quality monitoring. The potential of PAH found in the exhaust of modern cars and trucks to pose harmful health effects emphasizes the need for further development of fuels, lubricating oils, engines and aftertreatment technologies to mitigate these emissions

This work was supported by the European Union’s horizon Europe research and innovation programme under grant agreement No 101096133 (PAREMPI: particle emission prevention and impact: from real-world emissions of traffic to secondary PM of urban air).

How to cite: Aakko-Saksa, P., Järvinen, A., Kuutti, H., Honkisz, W., Kylämäki, K., Jäppi, M., Marjanen, P., Rissanen, M., Cervena, T., Vojtisek, M., Barreira, L., Saarikoski, S., Strandberg, B., Ohra-aho, T., Topinka, J., Bielaczyc, P., Rönkkö, T., and Timonen, H.: Polyaromatic hydrocarbons from modern cars and trucks in real-driving at cold ambient temperatures: contributions in particulate matter and semi-volatile compounds , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18349, https://doi.org/10.5194/egusphere-egu25-18349, 2025.

Emissions from the on-road transport sector are widely recognised as one of the major sources of air pollution in urban areas, especially in developing countries like India. The congested traffic flow pattern and plying of obsolete vehicle technology may result in the heterogeneous spatial distribution of vehicular exhaust emissions, with a high concentration gradient near traffic junctions. Comprehensive information on the spatial and temporal pattern of vehicular fleet emissions is essential to formulating road transport emission reduction policies for effective air quality management. However, computing such detailed emissions is a very complex task as it requires detailed and accurate traffic activity data such as vehicle volume, type, speed, age, fuel and technology share, etc. 
The present study adopted the globally recognised vehicle emission COPERT model to quantify the road transport-related spatial and diurnal emission patterns at 0.01° gridded resolution. The study is novel in its application of deep learning techniques, i.e., the Yolo model for vehicle detection,  achieving greater precision and reducing uncertainty in the activity data for heterogeneous traffic flow patterns. The emission estimate of overall PM is highest at the peak morning, i.e., 8-10 AM time, showcasing approximately 48.5 kg/hr, whereas NOx emissions resulted in being highest in 6-8 PM duration, emitting maximum load from buses, i.e., 106 kg/hr. The hourly emission variations exhibit a distinct bimodal pattern, characterised by prominent peaks in the morning and dominant peaks in the evening, largely associated with traffic congestion and peak travel times. The emissions estimates are observed to be highest for two-wheelers (scooters and motorbikes) and cars at the main traffic junctions inside the city area. Emissions from heavy commercial vehicles are observed to be concentrated on the highways during the nighttime. The developed methodology offers a framework for future real-time emission models in Indian urban regions, using real-time traffic activity data in tier II cities.

Keywords: Road transport emissions, deep learning, urban air quality, YOLO

How to cite: Badavath, B., Sharma, M., Sengar, V., and Jain, S.: Predicting road-specific emissions of the active vehicular fleet over the tier-II city in India: Integrating deep learning and speed information, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18968, https://doi.org/10.5194/egusphere-egu25-18968, 2025.

EGU25-19197 | Posters on site | AS3.30

Agentic AI for ship routing 

Fearghal O'Donncha, Abigail Langbridge, Alexander Timms, Antonis Antonopoulos, Antonis Mygiakis, and Eleni Voulgari

The complexity of the shipping industry, with its dynamic operational drivers and diverse data sources, presents significant scalability challenges for digital twins. Agentic Large Language Models (LLMs), augmented with external tools, offer a promising solution to streamline operations and improve decision-making. By leveraging pre-trained knowledge and reasoning capabilities, these LLMs can autonomously select the most relevant tools and data streams, facilitating real-time decision-making that optimizes ship routes, fuel consumption, and operational efficiency.

In this demonstration, we explore how agentic LLMs can enhance the scalability, flexibility, and efficiency of digital twins in shipping by optimising route planning with consideration for weather conditions, fuel consumption, and speed. By integrating weather data and analysing trade-offs between fuel consumption, speed, and routing choices, the system enables more effective decision-making to balance operational goals with environmental considerations. This approach facilitates a deeper understanding of how shipping operations can be adjusted for reduced emissions and improved fuel efficiency while considering the complexities of real-world constraints.

We showcase how this agentic digital twin solution supports more efficient route optimisation, ultimately contributing to the shipping industry’s transition to low-carbon fuels and reduced environmental impacts. This interactive system demonstrates the potential of agentic LLMs to reduce operational complexity and improve the practical application of digital twins in real-world settings.

How to cite: O'Donncha, F., Langbridge, A., Timms, A., Antonopoulos, A., Mygiakis, A., and Voulgari, E.: Agentic AI for ship routing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19197, https://doi.org/10.5194/egusphere-egu25-19197, 2025.

Previous emission inventories have reported fast growing on-road transport sector as one of the major contributors to emissions of aerosol and its carbonaceous fraction in India. The diesel-powered heavy-duty vehicles (HDVs Trucks and tractor/trailers) dominate emissions of light absorbing black carbon at national level. These emission inventories relied on emission factors generated from dynamometer studies which are known to be unrepresentative of real-world driving cycle. Therefore, data generated from dynamometers studies can be considered illusionary. This study will present the emission factors and climate relevant properties of aerosol emitted from on-road operation diesel powered trucks and tractors. The aerosol emissions were measured during on-road operation of heavy-duty vehicles using Versatile Source Sampling System (VS3). The VS3 was designed to iso-kinetically to withdraw a fraction of emission directly from tailpipe and abruptly mix with particle free dilution air for complete aerosol quenching. Before on-road experiments the VS3 was evaluated for homogenous mixing inside dilution tunnel, particle loss and formation. The emission factors of PM2.5 and BC were estimated as 1.2 – 2.4 and 0.5 – 1.3 gkg-1 respectively. The mass absorption cross section for heavy duty trucks were observed as 0.9 – 6.5 m2/gPM2.5. Emission factors of heavy-duty trucks in different emission norms along with the emission factor of organic carbon (OC) will be presented in the paper. The study will also discuss the chemical and optical properties of emissions from HDVs in detail including mass scattering coefficients (MSC), Absorption Angstrom exponent (AAE) and single scattering albedo (SSA). The finding from this study has implications in climate assessment through climate models and framing the policies for on-road vehicles for improving local air quality.

How to cite: Khan, M. S., Habib, G., Imran, M., and Un Nabi, M.: Optical and chemical properties of aerosol from on-road experiments of heavy-duty vehicles in India: Key inputs for climate assessment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19298, https://doi.org/10.5194/egusphere-egu25-19298, 2025.

EGU25-19470 | Posters on site | AS3.30

Climate Relevant Properties of Aerosol Emissions from Iron & Steel and Thermal Power Plant Emissions in India 

Karigowda Gowda, Mohd Shahar Khan, Gazala Habib, Rahul Kumar, and Swarndeep Roy Chaudhary

Industrial and power plant emissions are among the major contributors to air pollution in India, accounting for 37% of atmospheric PM2.5 emissions, with significant implications for climate change and human health. These emissions, primarily resulting from combustion processes, include carbonaceous aerosols such as particulate matter and light-absorbing carbon. The type of fuel used, the air pollution control technology implemented, and the industrial processes adopted heavily influence emissions from industrial sources. Aerosol optical properties, such as the mass absorption cross-section (MAC) and mass scattering coefficients (MSC), are critical for regional climate assessments. This study presents real-world measurements of MACs and MSCs from iron & steel, and thermal power plant emissions under Indian conditions. Stack emission measurements were conducted in real-world settings at iron and steel plants and thermal power plants, using the Versatile Source Sampling System (VS3). The VS3 system allowed a fraction of stack emissions to pass through an isokinetic particle sampling probe into a dilution tunnel, ensuring homogeneous mixing, negligible wall losses, and complete aerosol quenching. Dilution ratios of 20–60 with zero air simulated atmospheric dilution conditions. PM2.5 mass was collected on various filter substrates for gravimetric and chemical analyses. Particle absorption and scattering were measured using an Aethalometer (AE33) and a Nephelometer (IN102), respectively, while the light-absorbing carbonaceous fraction of PM2.5 was analysed on quartz filters using a thermal-optical reflectance analyser. PM2.5 emission factors from iron & steel (sponge iron) and thermal power plants are 0.11 – 0.16 and 0.07 – 0.44 g/kg of fuel used respectively. MAC values (m²/g PM2.5) were determined to range from 0.01 – 0.14 m²/g PM2.5 for iron and steel plants and 0.03 – 0.29 m²/g PM2.5 for thermal power plants. The EC, and OC emission factors and other optical properties including MSCs, AAE, and SSA will be discussed for these industries in the paper. Findings from this study have significant implications for climate assessments and the development of policies aimed at improving air quality, particularly for the major sources in the industrial sector.

How to cite: Gowda, K., Khan, M. S., Habib, G., Kumar, R., and Chaudhary, S. R.: Climate Relevant Properties of Aerosol Emissions from Iron & Steel and Thermal Power Plant Emissions in India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19470, https://doi.org/10.5194/egusphere-egu25-19470, 2025.

EGU25-19731 | ECS | Orals | AS3.30

Volatility of ultrafine and solid particles at a traffic site in Athens, Greece. 

Christina Spitieri, Maria Gini, Martin Gysel-Beer, Andreas Nowak, and Konstantinos Eleftheriadis

Atmospheric aerosols significantly impact the Earth’s climate and human health. The fraction of ultrafine particles (UFPs) present significant health risks because of their high surface area-to-mass ratio and their ability to penetrate deep into the lungs. Urban areas are hot spots for human exposure to UFPs, because they are strongly influenced by traffic exhaust emissions. Those emissions can be emitted directly as primary particles (soot, carbonaceous aggregates) or as so called secondary particles formed in the tailpipe after cooling of the exhaust gases or even in ambient air by further oxidation process induced by sunlight (volatile nucleation mode particles).

Once they are released into the atmosphere, soot particles undergo aging processes, during which they become internally or externally mixed with secondary organic and inorganic species, resulting in a core-shell structure. The solid core mainly consists of black carbon, while the shell is primarily composed of volatile and semi-volatile organic compounds. To identify the link between traffic exhaust emission in the tailpipe with “real-word” emission, also solid particle number (SPN) measurements have to be performed in ambient conditions. Thermodenuders, catalytic strippers, and Volatility Tandem Differential Mobility Analyzers (VTDMA) are state of the art techniques for SPN measurements. Thermodenuders and catalytic strippers are designed for the rapid removal of volatile components from solid particles, while VTDMA offers more detailed insights into the mixing state of size-selected aerosol particles.

This study aims to characterize UFPs at a traffic site in Athens by analyzing particle number concentrations, size distributions and volatility. Those measurements were compared to the Demokritos Athens suburban research station. Volatility measurements of size-selected particles (30 nm, 50 nm, 80 nm, and 120 nm) were performed using a custom-made VTDMA, operated at temperatures of 25°C, 110°C, 200°C, and 300°C. Data processing was carried out using the TDMAinv algorithm (Gysel et al., 2009). Additionally, a comparison of the VTDMA and catalytic stripping techniques was conducted under controlled conditions during lab experiment with miniCAST test aerosol at the PTB facility for exhaust emission tester.

Volatility was expressed in terms of aerosol particle number fraction (NFR) and volume fraction (VFR) remaining, shrink factor (SF) and mixing state. The aerosol particles at the traffic site appear to be closely linked to road traffic, as their solid particle number concentration peaks during traffic rush hours.  These particles are externally mixed and consist of volatile, semi-volatile, and refractory components. The NFR at 300°C was 8 % for nuclei mode particles, while for Aitken mode the  NFR was higher (>50%), indicating that a significant fraction of Aitken mode particles is composed of a solid particle fraction consist of black carbon particles. The SF was 70% for nuclei mode particles and around 50% for Aitken particle.

Gysel, M., McFiggans, G.B., Coe, H., Inversion of tandem differential mobility analyser (TDMA) measurements, J. Aerosol Sci., 40, 2009, https://doi.org/10.1016/j.jaerosci.2008.07.013, 2009.

How to cite: Spitieri, C., Gini, M., Gysel-Beer, M., Nowak, A., and Eleftheriadis, K.: Volatility of ultrafine and solid particles at a traffic site in Athens, Greece., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19731, https://doi.org/10.5194/egusphere-egu25-19731, 2025.

EGU25-19744 | ECS | Orals | AS3.30

Renewable Fuel: Assessing VOC and Particle Emission Reduction in a Hybrid Diesel Engine 

Andrea C. Wagner, Jussi Hoivala, Petteri Marjanen, and Miikka Dal Maso

Transportation remains a major contributor to global CO2 emissions, with road transport being the largest source. While electrification advances, additional mitigation strategies are needed to meet emission reduction targets. This study investigates how particle and trace gas emissions change when using renewable diesel fuel compared to fossil diesel in a hybrid engine. Measurements were conducted at Tampere University's Hybrid Engine Research Platform (HERPA), utilizing a comprehensive instrument fleet including FTIR spectroscopy, particle sizing, and Vocus PTR mass spectrometry for volatile organic compound (VOC) analysis. The renewable biodiesel, produced from waste fats and oils, demonstrated significant emission reductions compared to conventional diesel. During standardized RMC-C1 test cycles, the renewable fuel achieved approximately 30% lower particle emissions and showed reduced trace gas levels, including a threefold reduction in SO2 emissions due to lower sulfur content in the fuel. While both fuels exhibited similar qualitative emission patterns during engine operation, the renewable fuel consistently produced lower emissions across multiple pollutant categories. These findings demonstrate that renewable diesel offers substantial emission reduction benefits beyond CO2, presenting a viable pathway for cleaner transportation solutions. 

How to cite: Wagner, A. C., Hoivala, J., Marjanen, P., and Dal Maso, M.: Renewable Fuel: Assessing VOC and Particle Emission Reduction in a Hybrid Diesel Engine, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19744, https://doi.org/10.5194/egusphere-egu25-19744, 2025.

EGU25-20134 | Posters on site | AS3.30

In vitro assessment of biological impact of volatile/semi-volatile primary and secondary emissions derived from vehicles 

Zili Sideratou, Barbara Mavroidi, Fotios Katsaros, and Soheil Zeraati-Rezaei

Primary particle emissions, and the formation of secondary aerosols through atmospheric processing, are believed to be the pollutant with the greatest public health impact. In general, it is known that exposure to emissions leads to increased pulmonary inflammation and respiratory symptoms aggravation due to oxidative stress and direct toxic injury. Within the AEROSOLS project, the biological impact of volatile/semi-volatile (V/S-V) primary and secondary compounds derived from the engine and exhaust systems of vehicles will be assessed. In particular, in vitro tests based on traditional cell cultures (i.e. submerged monolayer cultures) as well as human air-liquid-interface (ALI) organotypic airway tissue models derived from primary tracheobronchial epithelial cells will be performed to predict the effects of these compounds on animals and humans without ethical concerns. The ALI model is an alternative airway model in which differentiating primary airway cells cultured on microporous membrane scaffolds can be directly exposed to gases and aerosols at the air-liquid interface. Compared to submerged monolayer cultures, primary cells that undergo cellular differentiation can reproduce an in vivo–like transcriptional profile similar to that of human airway epithelium. Therefore, organotypic ALI airway models have a more realistic in vivo–like structure, as well as barrier properties and metabolic functions, similar to those found in vivo. In addition, ALI models can be dosed in a more human-relevant manner than that in submerged cultures. Within the AEROSOLS project, human alveolar adenocarcinoma A549 epithelial cells are initially used for the safety evaluation of the key V/S-V compounds on traditional cell cultures or on VITROCELL® Essentials ALI exposure system (VITROCELL SYSTEMS GmbH, Waldkirch, Germany). In vitro cytotoxicity of V/S-V compounds is assessed following standard protocols, while further studies on genotoxicity, mutagenicity/carcinogenicity and immunotoxicity are performed. Additionally, the potential of these compounds to induce oxidation stress and inflammation is studied as it is known that these parameters are strongly related to the development of respiratory diseases. These results will be helpful to categorize and prioritize the V/S-V compounds based on their health impact.

Acknowledgement: This research was funded by the European Union’s Horizon Europe research and innovation programme within the AEROSOLS project under grant agreement No. 101096912 and UK Research and Innovation (UKRI) under the UK government’s Horizon Europe funding guarantee [grant numbers 10092043 and 10100997].

How to cite: Sideratou, Z., Mavroidi, B., Katsaros, F., and Zeraati-Rezaei, S.: In vitro assessment of biological impact of volatile/semi-volatile primary and secondary emissions derived from vehicles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20134, https://doi.org/10.5194/egusphere-egu25-20134, 2025.

EGU25-20159 | Orals | AS3.30

Evaluation of primary and secondary emissions from two Euro 6 SUV in laboratory and under real driving conditions 

Mickaël Leblanc, Armin Wisthaler, Joonas Vanhanen, Andreas Mauracher, Mohammed Salim Alam, Philipp Eichler, Soheil Zeraati-Rezaei, and Fotis Katsaros

The AEROSOLS project aims to define robust and transparent measurement and modelling methodologies to quantify the currently disregarded volatile/semi-volatile (V/S-V) primary and secondary emissions, assess their associated risks, and propose technological and legislative monitoring and abating mechanisms to help improve air quality and public health. This work will present the overall methodology utilized to extensively assess the regulated and unregulated, gaseous and particulate, emissions from the vehicles.

The project includes two comprehensive vehicle-level experimental campaigns during which the primary and secondary emissions of two state-of-the-art Euro 6 sport utility vehicles (SUV) will be assessed, both on a chassis dynamometer under controlled conditions and on open roads under winter and summer conditions.

During the Real Driving Emissions (RDE) experiments on roads, the vehicles will be equipped with a Proton-Transfer-Reaction Time-of-Flight Mass Spectrometer (PTR-ToF-MS) in addition to the standard Portable Emission Measurement System (PEMS). This allows extended characterization of the emitted gaseous compounds beyond the current Euro 6 protocol, with a particular focus on Volatile Organic Compounds (VOC). In the laboratory, the emissions from the vehicles will be evaluated under standard driving conditions using the Worldwide harmonized Light vehicles Test Cycle (WLTC) and under more realistic conditions reproducing the RDE trips previously characterized on roads. In addition to the standard devices used for the Euro 6 testing, the experimental protocol will include additional instruments to comprehensively assess the emissions of unregulated organic and inorganic gaseous compounds, and aerosols characteristics, e.g., particle number (PN) down to 1 nm.

Thanks to these complementary evaluations and extensive protocols, the AEROSOLS project will achieve a better understanding of vehicles’ primary emissions compared to the current Euro 6 and upcoming Euro 7 standards, and of Secondary Organic Aerosols (SOA) and their potential precursors. Furthermore, three different atmospheric ageing devices (a simulation chamber and two oxidation flow reactors) will be employed for the laboratory tests to also allow enhanced understanding of the ageing conditions’ effects on SOA formation.

Acknowledgments:

This research was funded by the European Union’s Horizon Europe research and innovation programme within the AEROSOLS project under grant agreement No. 101096912 and UK Research and Innovation (UKRI) under the UK government’s Horizon Europe funding guarantee [grant numbers 10092043 and 10100997].

How to cite: Leblanc, M., Wisthaler, A., Vanhanen, J., Mauracher, A., Alam, M. S., Eichler, P., Zeraati-Rezaei, S., and Katsaros, F.: Evaluation of primary and secondary emissions from two Euro 6 SUV in laboratory and under real driving conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20159, https://doi.org/10.5194/egusphere-egu25-20159, 2025.

The radiative impact of ship emissions, mostly through iteracting with marine low clouds, is uncertain. Survey of literature shows an almost 1000-fold difference in its magnitude. Here we use detected ship-tracks, bottom-up, and top-down geospatial krigging, top-down, to constrain its magnitude in the Southeast Atlantic. We show that physics derived based on bottom-up approach provides similar estimate of the forcing estimate as the top-down approach. With the derived physics, we further estimate the forcing of the total ship emissions. In particular, the forcing due to the recent IMO 2020 is estimated to play a significant role in driving short-term additional warming. We discuss the policy implications of our estimate in terms of regulations and geoengineering.

How to cite: Yuan, T.: Understanding the radiative impact of ship emissions through both bottom-up and top-down approaches, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20730, https://doi.org/10.5194/egusphere-egu25-20730, 2025.

EGU25-21415 | Posters on site | AS3.30

Methane emissions from LNG-powered vessels 

Kati Lehtoranta, Niina Kuittinen, Hannu Vesala, and Päivi Aakko-Saksa

The use of liquefied natural gas (LNG) as shipping fuel has increased in recent years with the most popular way to use LNG in low-pressure dual-fuel (LPDF) engines together with diesel fuel for ignition. Lower sulphur and nitrogen oxides, together with lower particulate emissions are reported with LNG use compared to diesel use. Moreover, CO2 emissions are lower as well but there is an issue with the methane slip with the LNG used in low-pressure dual fuel engines. The methane being a strong greenhouse gas and regulations introduced to consider methane emissions from ships, have made the engine manufacturers to take further development steps in preventing the methane slip. By today, there are still only few studies presenting emissions of methane from LNG-powered vessels with engines built in 2020 or after. The present study provides the results of the emission studies conducted onboard two LNG-powered vessels built in 2021 and 2022. The first campaign took place on-board a Ro-Pax ferry (built in 2021) operating in the Baltic Sea and the second was conducted on-board a cruise ship (built in 2022) operating in the Mediterranean.

The results indicate that the current state-of-the-art LPDF engines show lower methane levels compared to previous studies, which is good news when thinking of the climate effects. Air pollution levels from LNG use are again proven to be lower than from diesel use, contributing to better air quality. Overall, LNG is considered to be a transition fuel and the technologies developed today should be capable of utilizing biobased gas or a renewable synthetic in origin. Methane slip minimization and avoiding other pollutants produced are not only important today but also for future fuels, even though such fuels could be produced sustainably.

Acknowledgements: This research was funded by European Union, grant number 101056642.

How to cite: Lehtoranta, K., Kuittinen, N., Vesala, H., and Aakko-Saksa, P.: Methane emissions from LNG-powered vessels, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21415, https://doi.org/10.5194/egusphere-egu25-21415, 2025.

EGU25-21788 | Orals | AS3.30

Quantification of the Impact of Rail Traffic to Air Pollution at an Aboveground Train Station and its Surroundings 

Daniel Obando, Ulrich Vogt, Ingo Düring, and Sabrina Michael

In Germany, rail traffic is crucial when it comes to land transport of passengers and goods, according to the last report of the Deutsche Bahn AG, in 2023 more than 5 million passengers and 540 kt per day were transported [1]. Although this type of transport has been at the forefront in terms of sustainability and environmental friendliness, it is not exempted from generating effects on the environment.
According to the national emission inventory, the estimation of particulate matter (PM) emissions from train fuel combustion have decreased over the last 25 years (from ~ 2 kt/year to ~0.1 kt/year), however in the case of non-exhaust-emissions they have remained relatively constant at about 8 kt/year. Similarly, nitrogen oxide (NOX) emissions have considerably fallen from > 45 kt/year in 1995 to < 10 kt/year in 2022 [2].
Despite these data, which are by the way estimates, are not that detailed aggregated, that they could show e.g. the distribution of the air pollutants within the vicinity of the rails.
This study addresses this gap by measuring air quality in different structures of the German railway network: plain line, freight station, underground- and aboveground station, and tunnel.
Methodology
Air pollutant measurements were carried out at Augsburg central train station (handling about 234,000 trains annually) from February to May 2023. Using a windward-leeward approach, four measurement stations were installed, two for measuring the urban background concentrations and two directly on train platforms.
PM was measured by gravimetry (24 – 72 h averages) and continuous light scattering spectrometers and NOx with a chemiluminescence monitor (continuously) at one station and with passive samplers (2 – 4 weeks averages) at all stations.
Some filters from the gravimetric measurements were analyzed in the laboratory for a broad spectrum of trace elements (e.g., Fe, Cu, Mg, etc.). Ultrafine particles and black carbon were also measured at one station.
A motion sensor camera recorded train passages to differentiate impacts from passenger/freight trains and diesel/electric locomotives.
Results
The results show a relatively low additional load of PM at around 2 μg/m³, while in the case of NOx the value was between 17 and 20 μg/m3. On the other hand, when the short-term influence was assessed, following train passages showed significant peaks, the concentrations of PM rose to almost 100 μg/m³ and NOx even up to 600 μg/m³ for several minutes.
As it was not the case that all trains generated the same increase in pollutant concentration, a statistical analysis was carried out in which more than 10,000 events (train passages) were evaluated. The events were categorized by train type (S-Bahn, IC/ICE, regional, freight) and locomotive (diesel/electric). By this means means, probabilities of additional pollutant concentrations were also calculated.
The results showed that one in 20 trains produced an additional PM load exceeding 10 μg/m3 for all train types and in the cases of diesel trains, one in five trains caused an increase in NOX concentration of at least 50 μg/m3.

How to cite: Obando, D., Vogt, U., Düring, I., and Michael, S.: Quantification of the Impact of Rail Traffic to Air Pollution at an Aboveground Train Station and its Surroundings, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21788, https://doi.org/10.5194/egusphere-egu25-21788, 2025.

EGU25-644 | ECS | Orals | AS3.31

Assessing the Impact of Emission Reductions on Surface O3 and PM2.5 in India 

Arshitha Anand K A, Dilip Ganguly, and Sagnik Dey

The rapid industrialization and urbanization across South Asia in recent years have driven significant increases in surface ozone (O₃) and fine particulate matter (PM₂.₅) concentrations, posing serious environmental and public health challenges. This study investigates the potential of precursor emission reductions in mitigating surface O₃ and PM₂.₅ levels over the Indian subcontinent, with a focus on the pre-monsoon season. Using the WRF-Chem model, we applied two chemical mechanisms: MOZCART, representing a simpler approach, and MOZART-MOSAIC, incorporating more complex gas-phase and aerosol interactions.

Through a series of sensitivity experiments, we analysed the effects of a 50% reduction in key precursors—nitrogen oxides (NOₓ), volatile organic compounds (VOCs), carbon monoxide (CO), methane (CH₄), and their combined reductions. The results revealed distinct responses to emission reductions. For surface O₃, MOZCART mechanism showed substantial reductions (~ 8 ppbv) in northern India under curtailed NOₓ emission, highlighting dominant role of NOx in O₃ production in this region. In contrast, VOC and CO reductions had limited impacts on O₃ levels (~5 ppbv), suggesting a VOC-limited regime in certain areas. The MOZART-MOSAIC mechanism provided deeper insights, revealing substantial PM₂.₅ reductions (~3 ug/m3) under combined precursor reductions, emphasizing the intricate coupling between gas-phase and particulate chemistry.

Further analysis of diurnal and nocturnal variations highlighted differences in chemical dynamics between the two mechanisms. MOZCART indicated an increase in daytime O₃ levels (~ 8 ppbv) under combined precursor reductions, likely due to shifts in photochemical regimes, whereas MOZART-MOSAIC exhibited nighttime O₃ reductions (~ 4 ppbv) driven by changes in nocturnal chemical pathways.

This study underscores the critical importance of multi-pollutant emission reductions to achieve meaningful improvements in surface O₃ and PM₂.₅ levels. It also highlights the complex and region-specific interactions between atmospheric precursors, emphasizing the need for integrated and holistic approaches to air quality management in South Asia.

How to cite: Anand K A, A., Ganguly, D., and Dey, S.: Assessing the Impact of Emission Reductions on Surface O3 and PM2.5 in India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-644, https://doi.org/10.5194/egusphere-egu25-644, 2025.

Near-surface ozone pollution is one of the biggest challenges for Chinese air quality improvement, while its future spatiotemporal evolution and driving factors have not been fully investigated. Here, we developed a two-stage model combining a machine learning technique (XGBoost) and a chemical transport model (WRF-CMAQ) to assess the ozone change till 2060 in China under three scenarios with various trajectories of climate change, energy transition and pollution controls. The new model effectively corrected overestimation and underestimation of ozone levels by CMAQ and global climate models, respectively. Anthropogenic efforts will overcome the adverse effect of climate and reduce future ozone concentration, especially in eastern China and warm season with greater ozone pollution. From a long-term perspective, energy structure transition was estimated to play a more important role than end-of-pipe emission controls, with a former to latter ratio of ozone reduction during 2017-2060 at 2.7. With observational information incorporated, our model was demonstrated to better capture the ozone response to precursor emission change than WRF-CMAQ, and corrected the underestimation of ozone reduction for developed urban areas.

How to cite: Wang, Y. and Zhao, Y.: Future evolution of Chinese near-surface ozone concentrations: the insight from a new two-stage model combining machine learning and chemical transport modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1498, https://doi.org/10.5194/egusphere-egu25-1498, 2025.

EGU25-2578 | ECS | Orals | AS3.31

Assessing the Air Quality Impacts of Net-Zero GHG Emissions in Europe and Switzerland with ICON-ART 

Corina Keller, Lukas Emmenegger, and Dominik Brunner

The European Union and the Swiss Federal Council have both set the ambitious goal of achieving net-zero greenhouse gas (GHG) emissions by 2050. While reducing fossil fuel use is widely assumed to improve air quality due to the co-emission of air pollutants during fossil fuel combustion, specific choices regarding alternative energy sources and changes in the building, industrial, and agricultural sectors may have very different and potentially detrimental impacts on air quality.

In this context, we study the air quality implications of transitioning to a net-zero GHG society in Europe and Switzerland by comparing two distinct scenarios for the year 2050: a net-zero pathway and a business-as-usual (BAU) scenario. The BAU scenario reflects the continuation of current energy policies without additional measures to achieve net-zero emissions. Comparing the BAU and net-zero scenarios allows us to assess how transformations in energy systems and associated changes in anthropogenic emissions shape the levels, composition, and dynamics of air pollutants.

Our analysis is based on simulations conducted with the state-of-the-art atmospheric chemistry and transport model ICON-ART. We have incorporated the latest MOZART tropospheric chemistry scheme to accurately represent key oxidation processes involving ozone, nitrogen oxides, and volatile organic compounds. ICON-ART also features advanced modules for aerosol dynamics, gas-aerosol interactions, and emissions from biogenic and natural sources. Emission inventories for the year 2050 are developed in alignment with Switzerland's energy strategy and European projections. Anthropogenic emissions of gas-phase species and particulate matter are integrated into ICON-ART using its online emission module.

Based on air quality simulations with ICON-ART, we will discuss the effects of reducing primary air pollutants on the formation of secondary air pollutants and the removal of air pollutants from the atmosphere, and show how Swiss and European air quality levels change as we move towards a net-zero society.

How to cite: Keller, C., Emmenegger, L., and Brunner, D.: Assessing the Air Quality Impacts of Net-Zero GHG Emissions in Europe and Switzerland with ICON-ART, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2578, https://doi.org/10.5194/egusphere-egu25-2578, 2025.

Introduction

Given its atmospheric lifetime of days to a week, fine particulate matter (PM2.5) – an air pollutant responsible for adverse health effects – can be advected far beyond its sources and across political borders. This uncomfortable exchange leads to inequality, in which a country may bear air pollution-related health impacts associated with anthropogenic emission activity beyond its borders. Climate action is irrevocably linked to this inequality. Anthropogenic sources of greenhouse gases often co-emit air pollutants and their chemical precursors; thus, action targeting greenhouse gases can result in air pollution-related co-benefits that are realized through improvements in air quality.

 

Methods

Despite this close linkage, much of the research on co-benefits has focused on quantifying benefits in terms of magnitude or absolute number. This ignores how atmospheric composition source-receptor dynamics could be affected by climate action. In this study, we quantify how air pollution exchanges within and between regions (e.g., Africa and Europe) could vary across different shared socioeconomic pathways (SSPs) and representative concentration pathways (RCPs). We perform thousands of GEOS-Chem adjoint simulations to calculate the sensitivities of country-scale PM2.5 exposures to their precursor emissions. We then combine these simulated sensitivities with gridded emission projections for the SSPs and RCPs to determine how source-receptor relationships between specific countries and regions may differ across different climate futures. Lastly, we leverage methods from the Global Burden of Disease study to assess the impacts of transboundary air pollution exchange on human health.

 

Results and Discussion

We find that reductions in anthropogenic emissions from climate action in more sustainable futures (SSP1-19) results in more co-benefits (480 thousand deaths avoided) than worst-case scenario fragmentation futures (SSP3-60) (140 thousand deaths avoided). In sustainable futures (SSP1), African countries have more influence on climate co-benefits; they contribute between 2.3-2.8 times as many benefits to European countries than vice-versa. However, in fragmented futures (SSP3), this dynamic flips and African countries become more dependent on European climate action as they contribute between 1.7-0.4 times as many benefits. Ultimately, this suggests that changes in anthropogenic emissions associated with climate action have the capacity to not only affect atmospheric composition through improved air quality but also to modify exchange relationships between individual countries and regions.

How to cite: Nawaz, M. O. and Henze, D.: Exploring the role of climate action in transboundary air pollution inequality using GEOS-Chem adjoint sensitivities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3624, https://doi.org/10.5194/egusphere-egu25-3624, 2025.

Glyoxal (CHOCHO) is a short-lived oxidative volatile organic compound (OVOC) in the atmosphere, which is an intermediate product of the oxidation of most VOCs in the atmosphere. Glyoxal is a weak trace gas, but it has a significant impact on air quality. Glyoxal is a short-term chemical indicator of non methane volatile organic compound (NMVOC) emissions from biological activities, biomass burning, and human activities, and it contributes significantly to the formation of secondary organic aerosols. This study used data from 2019 to 2021 from the TROPOMI CHOCHO Level 2 product published by Sentinel-5p+Innovation, and increased the spatial resolution to the order of 0.05 º using oversampling algorithm to discuss the spatial-temporal distribution changes of glyoxal caused by the changes in human activities on a national scale caused by the COVID-19, and reveal the influencing factors and potential contributions of the increase in glyoxal emissions in China. Currently, there is relatively little research among domestic scholars on using satellite remote sensing to monitor atmospheric glyoxal. It is hoped that through this study, we can understand the spatiotemporal variation characteristics of glyoxal in China and improve scientific decision-making.

How to cite: zhaolong, S.: Temporal and spatial distribution of tropospheric glyoxal in China before and after the COVID-19 and its influencing factors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3710, https://doi.org/10.5194/egusphere-egu25-3710, 2025.

EGU25-6389 | ECS | Posters on site | AS3.31

Modelling emission-driven air-quality changes over Central Europe 

Alvaro Patricio Prieto Perez and Peter Huszar

In this study, we explore how changes in emissions affect future air quality in the Central European region while assuming that climate changes are minimal. For this, we used two future scenarios (RCP4.5 and RCP8.5) for the periods 2026-2035 and 2046-2055. With advanced modelling tools, we simulated the current and future air pollution levels.

Five simulations have been conducted so far: one with present-day conditions (2010-2019) and four with future emission scenarios. The present-day conditions were validated by comparing the simulated results for pollutants like oxides of nitrogen, ozone and particulate matter with observed data. The validation revealed that the models generally underestimated pollutant levels (except for ozone).

The analysis of future projections indicate a general decrease in most pollutants’ concentrations. Some exceptions occur, however, such as with ozone during the winter months. Despite the uncertainties intrinsic to the modelling process, this study helps understand how reductions in emissions can lead to improved air-quality.

How to cite: Prieto Perez, A. P. and Huszar, P.: Modelling emission-driven air-quality changes over Central Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6389, https://doi.org/10.5194/egusphere-egu25-6389, 2025.

EGU25-7386 | Orals | AS3.31

Trends in emissions of atmospheric constituents at the global scale: evaluation and improvements using regional inventories 

Claire Granier, Cathy W. Y. Li, Stijn Dellaert, Hugo Denier van der Gon, Thierno Doumbia, Marc Guevara, Jukka-Pekka Jalkanen, Jeroen Kuenen, Cathy Liousse, Elisa Majamaki, Hugo Merly, Emma Schoenmakers, and Nicolas Zilbermann

Different emissions inventories have been developed in recent years, which provide emissions of gaseous and particulate atmospheric species for the past decades at both global and regional scales. As part of the Copernicus Atmosphere Monitoring Service, we have developed the CAMS-GLOB-ANT inventory (version 6.2), which provides monthly emissions of 36 chemical compounds at a spatial resolution of 0.1x0.1 degree. The evaluation of the emissions has revealed issues in some regions, particularly for the emissions of nitrogen oxides and sulfur dioxide. To evaluate the dataset in more detail, we have gathered data provided by several inventories for the 2000-2024 period developed for the global as well as for the regional scale. The changes in the emissions provided by these global and regional inventories have been intercompared, and we will discuss the comparisons of the emissions of carbon monoxide, nitrogen oxides, sulfur dioxide and black and organic carbon. We have used different sets of regional emissions for Europe, the USA and China to improve the CAMS-GLOB-ANT dataset. The methodology to build the CAMS mosaic of emissions (CAMS-GLOB-ANT-M1) will be discussed, and comparisons between the improved and the original CAMS global emissions will be presented.

How to cite: Granier, C., Li, C. W. Y., Dellaert, S., Denier van der Gon, H., Doumbia, T., Guevara, M., Jalkanen, J.-P., Kuenen, J., Liousse, C., Majamaki, E., Merly, H., Schoenmakers, E., and Zilbermann, N.: Trends in emissions of atmospheric constituents at the global scale: evaluation and improvements using regional inventories, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7386, https://doi.org/10.5194/egusphere-egu25-7386, 2025.

EGU25-7639 | Posters on site | AS3.31

Day and night variations in aerosol properties and particulate matter in Changchun, China 

Xuanyi Wei, Yuliia Yukhymchuk, Gennadi Milinevsky, Xuhui Gao, and Yu Shi

Changchun is a city in Northeast China influenced by diverse aerosol sources and particulate matter (PM), including emissions from industrial activities, traffic, biomass burning, and mineral dust transport from deserts in the West. The aerosol property data are now accessible through the newly installed sun-sky-lunar CE318-T photometer. We are monitoring the PM1, PM2.5, and PM10 levels in two city regions in situ using the AirVisual sensors. This study analyses day and night observations from AERONET and AirVisual sensors. Key aerosol properties, such as aerosol optical depth (for total, coarse, and fine modes), Angstrom Exponent, and particle size distribution, are analyzed for different times of the day. Additionally, the concentrations of PM1, PM2.5, and PM10 during daytime and nighttime are evaluated to identify daily patterns in aerosol behavior. The findings reveal temporal variations in aerosol composition that reflect changes in atmospheric conditions, differences between outdoor-indoor concentrations, and shifts in their sources. These results provide insights into the dynamics of atmospheric aerosols, highlighting their impact on air quality and regional climate during both day and night. This comprehensive analysis contributes to a deeper understanding of aerosol behavior and its environmental implications.

 

How to cite: Wei, X., Yukhymchuk, Y., Milinevsky, G., Gao, X., and Shi, Y.: Day and night variations in aerosol properties and particulate matter in Changchun, China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7639, https://doi.org/10.5194/egusphere-egu25-7639, 2025.

EGU25-8170 | Orals | AS3.31

Access to Emissions Distributions and Related Ancillary Data through the ECCAD database  

Nicolas Zilbermann, Claire Granier, and Cathy Leal Liousse

The Emissions of atmospheric Compounds & Compilation of Ancillary Data (ECCAD) database provides a user-friendly access to surface emissions and ancillary data, i.e. data on land use, active fires, burned areas, population, etc. These data can be directly viewed or downloaded. ECCAD is the emissions database of the GEIA (Global Emissions InitiAtive) project and a sub-project of AERIS the French Data and Services Cluster for Atmosphere (CNES and CNRS, https://www.aeris-data.fr/). ECCAD distributes also the emissions dataset developed as part of the Copernicus Atmosphere Monitoring Service (https://atmosphere.copernicus.eu/)

The ECCAD database includes more than 100 datasets with a large diversity of sources, which provide global and regional surface emissions for a large set of chemical compounds, at several resolutions (0.25x025, 0,1x0,1, 1x1 degree etc) and several sectors. The database has currently more than 2500 users originating from more than 80 countries on 836 institutes. The project benefits from this large international community of users to expand the number of emission datasets made available.

ECCAD provides detailed metadata for each of the datasets, including information on references, how to cite the datasets when used, the methodology, and links to the original inventories. It can also provides DOIs. Several tools are provided for the visualization of the data, for computing global and regional totals and for an interactive spatial and temporal analysis. The data can be downloaded as interoperable NetCDF CF-compliant files, i.e. the data are compatible with many other client interfaces.

The ECCAD database and web interface are under constant development to enhance the user experience: better download granularity, new tools to improve the analysis and comparison of emissions and ancillary data. They include geographical masking, arithmetic expressions to combine different maps, new tools for temporal profiles analysis, and comparisons of data at different scales.

The presentation will provide information on all the datasets available within ECCAD, as well as examples of the analysis work that can be done online through the website: https://eccad.sedoo.fr

How to cite: Zilbermann, N., Granier, C., and Leal Liousse, C.: Access to Emissions Distributions and Related Ancillary Data through the ECCAD database , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8170, https://doi.org/10.5194/egusphere-egu25-8170, 2025.

EGU25-10011 | ECS | Posters on site | AS3.31

Long-Term Trends in Surface Ozone Over Ireland: Insights from long-term measurement dataset and advanced model contributions. 

Nikhil Korhale, Liz Coleman, Tabish Ansari, and Tim Butler

This study extends previous research analysing the long-term measurement records of surface ozone (O3) across Ireland, focusing on the Mace Head atmospheric research station. Due to its proximity to the Atlantic, Ireland plays a vital role in O3 monitoring, influenced by local and long-range pollutant transport. Using innovative trajectory analysis techniques, exceedances of O3 concentrations linked to different pollution sectors were identified, revealing distinct seasonal patterns. The findings show a significant rising trend in surface O3 at urban sites over the past two decades but without a similar trend at coastal sites. The highest O3 levels and exceedances at coastal sites, less influenced by local emissions, are heavily influenced by meteorological processes, including transboundary pollution and stratospheric intrusion. Observations at coastal sites reveal seasonal cycles with a springtime maximum. At Mace Head, a declining trend is observed in springtime O3 levels, contrasted with a rising trend during the winter months. When examining data from the clean-air sector, similar springtime declines are observed; however, a rise in winter is not seen, implying that the rising wintertime trends are a response to decreasing European emissions and the weekend effect. It is found that during the spring season, exceedances correlate with high maxima. To complement these observations, advanced modelling is used to quantify O3 contributions from various sources, elucidating key drivers behind the observed changes. The analysis indicates that European emissions play a significant role during the summer months, while North American emissions are comparable during other seasons. The elevated springtime O3 levels are primarily attributed to stratospheric transport, influences from westerly transboundary air pollution, and nitrogen oxides from lightning activity. Trend analysis reveals that reductions in baseline O3 levels and early-spring exceedances require targeted methane mitigation, while overall emission reductions are essential to curb exceedances across seasons. Late-spring and summer exceedances can be effectively reduced by addressing European and local pollution sources. This research highlights the importance of seasonal factors in air quality management across Ireland, emphasizing the need for a multi-faceted approach to control O3 levels and reduce exceedances through global and regional emission reductions.

How to cite: Korhale, N., Coleman, L., Ansari, T., and Butler, T.: Long-Term Trends in Surface Ozone Over Ireland: Insights from long-term measurement dataset and advanced model contributions., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10011, https://doi.org/10.5194/egusphere-egu25-10011, 2025.

EGU25-10177 | ECS | Posters on site | AS3.31

Short-term human intervention did not significantly improve urban air quality 

Wenping Li and Chengkai Qu

Short-term interventions may create a false sense of progress in addressing air quality issues. We find that despite the implementation of several short-term strategies during the coronavirus disease 2019 (COVID-19) pandemic, such as traffic restrictions, the anticipated improvements in air quality were not realized. On the contrary, the regional transportation of pollutants and the formation of secondary aerosols may still influence the air quality. Through a comprehensive analysis of air quality data collected before, during, and after the interventions in COVID-19, employing nonlinear statistical methods to assess changes in key pollutants, it can be inferred that the long-term memory mechanisms, nonlinear dynamic mechanisms of the atmospheric system play a crucial role in the evolution of air pollutants. Thus, the short-term human intervention did not significantly improve urban air quality. Besides, when pollution processes occur, the reason may not be unique, we must comprehensively interpret it. Policymakers are encouraged to consider more comprehensive and long-term strategies that integrate continuous monitoring and evaluation of air quality interventions.

How to cite: Li, W. and Qu, C.: Short-term human intervention did not significantly improve urban air quality, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10177, https://doi.org/10.5194/egusphere-egu25-10177, 2025.

EGU25-11543 | ECS | Posters on site | AS3.31

Understanding the Changes in Future Air Quality and its Drivers in India  

Mukul Kumar, Dilip Ganguly, and Sagnik Dey

The composition of PM2.5 plays a critical role in determining the health impacts of acute and chronic air pollution exposure. Exposure to PM2.5 and O3, the two most essential criteria pollutants, depends not only on primary emissions but also on the atmospheric processes that lead to secondary PM2.5 and O3 via chemistry. Climate change is expected to modulate ambient PM2.5 exposure. Thus, understanding the changes in both primary and secondary pollutants separately due to meteorological and emission changes in the future is crucial for mitigation strategies.
This study utilizes the WRF-Chem chemical transport model to investigate the concentration of PM2.5 and its components. A hybrid emission inventory was developed by integrating the local SMOG-India and global EDGAR (Version-8.1) inventories for the base year 2019. Sensitivity simulations were conducted to identify optimal chemical schemes for representing air pollution chemistry and dynamics. The simulated concentration of PM2.5 and its components (BC, OC, SO4) successfully captured the spatial distribution and diurnal variation, including significant hotspots compared to MERRA-2 reanalysis data. Magnitude-wise, the CBMZ-MOZAIC chemical scheme overestimated PM2.5 concentrations in coastal and oceanic regions, while the MOZART-MOZAIC scheme underestimated them in northwestern India. Next, we will work on the simulations for the future 2040, isolating the effects of evolving emissions and meteorological conditions to assess their contributions to PM2.5 concentrations under the most likely scenario (SSP370).

How to cite: Kumar, M., Ganguly, D., and Dey, S.: Understanding the Changes in Future Air Quality and its Drivers in India , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11543, https://doi.org/10.5194/egusphere-egu25-11543, 2025.

This study investigates the speciation of the total oxides of nitrogen (NOy) in Taichung, Taiwan, which is a highly developed urban area. Positive correlation between the daily mean of PM2.5 and the daytime (8-hr) mean of O3 shows that photochemical reactions are the major mechanisms underlying the observed air pollution phenomena. Furthermore, a strong linear correlation between the ambient levels of PM2.5 and NOz (NOy-NOx) found during the high PM episodes evidences that the atmospheric oxidation of NOx is the key processes leading to the air quality deterioration in the urban area. An in-depth analysis on the variations in the NOy composition as well as in the ozone precursors (VOCs and NOx) will be presented, and the significance of atmospheric oxidation capacity in the urban air quality is highlighted.

How to cite: Chou, C. and Lin, C.-Y.: A study on the speciation of NOy and its implications for the atmospheric oxidation capacity in Taichung, Taiwan, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14428, https://doi.org/10.5194/egusphere-egu25-14428, 2025.

India experiences some of the highest ambient PM2.5 pollution concentrations in the world, which led to an estimated 1.67 million premature deaths in 2019. The power sector alone accounts for 20% of PM2.5-related deaths in the country, making it the highest contributor to PM2.5-related mortality per unit of generating capacity globally. In addition, a transition from coal power to renewable energy in India is critical for meeting global climate targets, while currently India’s CO2 emissions are rapidly rising. With India's electricity demand projected to quadruple between 2022 and 2047, understanding the environmental trade-offs between various power sector expansion pathways, particularly the effects of continuing to operate coal power plants without pollution controls, implementing pollution controls on them, or increasingly implementing renewable energy (RE) is critical for weighing the impact of the future power sector on air pollution, public health and climate.

We have developed an integrated assessment framework to investigate the current and future air quality, public health, and carbon emission implications of India’s power sector operation. In addition, our analysis also considers the climate effects associated with aerosols from power sector, which can influence regional radiative forcing and temperature patterns. We have constructed a detailed, plant-level emission inventory for India’s coal-fired power plants, which had a total installed capacity of 212 GW in 2022. We then implemented our plant-level coal power emission inventory in the WRF-Chem 4.6.1 air quality model to simulate the impact of various possible power sector expansion pathways on regional air pollution and radiative forcing resulting from various aerosol distributions.

We also developed a new tagging scheme in WRF-Chem that attributes simulated PM2.5 concentrations to individual power plant emissions and evaluates the location-specific impacts of these emissions on air quality and public health. This approach allows us to identify those power plants with the largest adverse impacts on public health. This information can then be used by policy makers in determining power generation and public health priorities.

How to cite: Zhou, M., Mauzerall, D., Velamuri, V., and Kota, H.: Implementing pollution controls in India’s coal power plants and utilizing renewable energy: Synergies and trade-offs for air quality, public health and climate., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14625, https://doi.org/10.5194/egusphere-egu25-14625, 2025.

EGU25-17230 | ECS | Orals | AS3.31 | Highlight

Quantifying the Climate Penalty on Air Quality in Europe – Insights from INSPEnCaT Project 

Patricia Tarín-Carrasco, Hervé Petetin, María Gonçalves Ageitos, Marc Guevara, Francesco Marangio, Carlos Pérez García-Pando, Joan Ballester, Xavier Querol, and Oriol Jorba

The European Commission’s Zero Pollution Action Plan sets ambitious goals to reduce air, water, and soil pollution by 2050, including a 55% reduction in premature deaths from air pollution by 2030. In 2022, fine particulate matter (PM₂.₅), nitrogen dioxide (NO₂), and ozone (O₃) caused 239,000, 48,000, and 70,000 premature deaths, respectively. The interaction between climate change and air pollution presents significant challenges for achieving these ambitious goals. Rising temperatures, frequent heatwaves, and drought conditions enhance the production of O₃ and the formation of secondary organic aerosols (SOA), increasing PM₂.₅ levels by up to 5% in some regions. These compounded effects heighten health and environmental risks. 

The Mediterranean Basin, a recognized climate change hotspot, faces particularly severe challenges. Under high-warming scenarios (+4°C), intensify emissions of O₃ precursors and wildfire activity in southern Europe. The “climate penalty” — the additional burden of air pollution under changing climate conditions— could at least partly offset the benefits of current mitigation measures. For example, projections indicate a 15% increase in O₃-related premature mortality and respiratory hospitalizations in southern Europe by mid-century. However, uncertainties remain regarding the isolated contribution of climate change to these trends.

The INSPEnCaT project addresses these critical challenges by quantifying the air pollution climate penalty across Europe, focusing on the influence of climate change under present-day and future emission scenarios.The study outlines three key objectives: (1) to develop a regional climate-chemistry modeling system for Europe, (2) to assess the air pollution climate penalty under different abatement scenarios, and (3) to quantify impacts on policy-relevant metrics, including human and vegetation exposure and associated health effects. More specifically, we are developing a modeling chain coupling global chemistry-climate simulations with the EC-Earth3-AerChem model with regional weather-chemistry simulations with the MONARCH model. Simulations will focus on two 10-year periods (2005–2014 for present-day and 2045–2054 for future conditions). These simulations will isolate the effect of climate change on air quality under present-day and future emission scenarios for that, two scenarios will be performed: (1) present-day emissions with present-day climate (2005–2014) and (2) present-day emissions with future climate under SSP2-4.5 scenario (2045–2054). MONARCH model will downscale these simulations to a 20x20 km² resolution, providing detailed air quality projections across Europe based on different air pollution abatement scenarios. Regarding anthropogenic emissions, EC-Earth3-AerChem relies on CMIP6 historical and projected emissions under the SSP245 for present-day and future, respectively. MONARCH relies on the CAMS-REG-APv4.2 for present day while different policy emission scenarios will be used for the future (i.e. Current legislation, maximum feasible reduction). In this contribution, we will present and discuss the preliminary results of atmospheric composition obtained under these different long-term emission scenarios.

The results of this study will offer valuable insights into the climate penalty’s effects on air pollution in key hotspot regions across Europe. INSPEnCaT results will support policymakers to design more effective strategies to mitigate air pollution and its associated health risks, ensuring alignment with ambitious European objectives such as the Zero Pollution target by 2050.

How to cite: Tarín-Carrasco, P., Petetin, H., Gonçalves Ageitos, M., Guevara, M., Marangio, F., Pérez García-Pando, C., Ballester, J., Querol, X., and Jorba, O.: Quantifying the Climate Penalty on Air Quality in Europe – Insights from INSPEnCaT Project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17230, https://doi.org/10.5194/egusphere-egu25-17230, 2025.

EGU25-17382 | ECS | Posters on site | AS3.31

Assessment the effect of emission reductions on long-term trend in carbonaceous aerosols from 2014 to 2021 in eastern China 

Chang Zhou, Wei Nie, Xuguang Chi, Caijun Zhu, and Aijun Ding

As a key fraction of fine particulate matter (PM2.5), carbonaceous aerosol has a significant impact on climate and human health. This study investigates the long-term variations in carbonaceous aerosols from 2014 to 2021 in Nanjing, China. We observed substantial decreasing trends in organic carbon (OC) (-8.0% yr-1) and elemental carbon (EC) (-8.3% yr-1), mainly driven by reductions in primary carbonaceous components. Notably, secondary organic carbon (SOC) did not exhibit a significant decreasing trend (-2.0% yr-1), while its contribution to OC increased substantially (16.4% yr-1), indicating its growing importance in organic aerosol. Compared to changes in meteorological factors, emission reduction played a dominant role in the decrease of carbonaceous aerosols. Moreover, considering two key clean air actions and the COVID-19 pandemic, we thoroughly assessed the effect of emission reduction on different carbonaceous components throughout three phases: Phase I (2014-2017), Phase II (2017-2019), and Phase III (2019-2021). The varying trends of primary carbonaceous components over the three phases highlight their dynamic response to various emission control measures implemented over distinct phases. Given the relatively stable atmospheric oxidation and the limited decrease in volatile organic compounds (VOCs) in Phase III, the unexpected significant reduction trend observed in SOC (-12.7% yr-1) during that phase may be significantly attributed to the notably higher reduction rate in primary carbonaceous components, as secondary organic aerosol (SOA) formation can be enhanced in the presence of primary organic aerosol (POA). Our findings provide a new insight into assessing the effectiveness of emission control measures on SOC trend.

How to cite: Zhou, C., Nie, W., Chi, X., Zhu, C., and Ding, A.: Assessment the effect of emission reductions on long-term trend in carbonaceous aerosols from 2014 to 2021 in eastern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17382, https://doi.org/10.5194/egusphere-egu25-17382, 2025.

EGU25-857 | ECS | PICO | AS3.32

Decadal Shifts in Surface Ozone Trends at a Central Himalayan Site: Revealing Contrasting Phases from 2007 to 2022. 

Vikrant Tomar, Manish Naja, Rajesh Kumar, Prajjwal Rawat, and Upendra Kumar

Understanding long-term changes in surface ozone pollution across South Asia, particularly remote region, remains a critical challenge due to the scarcity of surface-based observations. Tropospheric ozone is secondary pollutant and a greenhouse gas whose higher levels pose a serious hazard to human health, crop yield, environment, and climate. In view of this, continuous surface ozone observations was initiated in October 2006 at a high-altitude site Nainital (29.25°N, 79.45°E, 1948 m amsl) in the central Himalayas. This study examines the long-term trends of surface ozone (2007–2022) at this site using ground observations, WRF-Chem model simulation, and reanalysis datasets. The long term trend analysis is done using statistical method adopted by TOAR II  which revealed a negative trend in surface ozone during 2007–2022. However, a negative trend ( about -0.5 ppbv/year) was observed from 2007-2015, and a positive trend (1.2 ppbv/year) from 2016-2022. Investigating different percentiles for such trend highlights that some specific percentiles play a pivotal role in shaping the trend rather than a uniform distribution around the mean or median. Daily peak-to-peak ozone amplitude shows positive trend, with spring exhibiting the steepest rise and autumn the least. While the annual MDA8 ozone exceedance (>50 ppbv) suggests a slight negative trend over the study period with 2022 recorded the highest exceedance. The ERA5 reanalysis ozone shows a negative trend during 2007-2015 and positive trend during 2016-2022 for the nearest pressure levels which is similar tendency as in observed surface ozone. While trend from MERRA-2, CAMS, and AIRS data showed different tendencies. Tropospheric column ozone trends from OMI/MLS indicate a modest positive trend (about 0.2 DU/year) during 2007–2020. WRF-Chem model simulation is able to produce the diurnal and seasonal variation of ozone with some overestimation. Notably, long-term trends diverge, with WRF-Chem model simulations showing positive trend while observations indicate a negative trend. An investigation into meteorological parameters provided no definitive explanation for the shift in trends across the two periods. The trend observed during 2016–2022 over the central Himalayan region underscores the need for a well-defined action plan to mitigate emissions of ozone precursor gases.

How to cite: Tomar, V., Naja, M., Kumar, R., Rawat, P., and Kumar, U.: Decadal Shifts in Surface Ozone Trends at a Central Himalayan Site: Revealing Contrasting Phases from 2007 to 2022., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-857, https://doi.org/10.5194/egusphere-egu25-857, 2025.

EGU25-975 | ECS | PICO | AS3.32

Tropospheric NO2 over South and East Asia measured by OMI and modelled by UKCA 

Alok K. Pandey, David Stevenson, Alcide Zhao, Richard Pope, Ryan Hossaini, and Krishan Kumar

South and East Asia (S/E Asia), home to nearly half the world's population, are major contributors to global nitrogen oxide (NOx = NO + NO2) emissions due to recent rapid industrialization, urbanization, and growth in energy consumption. We compare tropospheric column NO2 in the United Kingdom Chemistry and Aerosol (UKCA) model v11.0 with satellite measurements from NASA’s Earth Observing System (EOS) Aura satellite Ozone Monitoring Instrument (OMI) to investigate the seasonality and trends of tropospheric NO2 over S/E Asia. UKCA is the atmospheric composition component of the UK Earth System Model (UKESM). UKCA was run with nudged meteorology, producing hourly output over S/E Asia for 2005–2015. OMI averaging kernels have been applied to the model hourly data sampled at Aura’s local overpass time of 13:45 ± 15 to allow consistent model-data comparison. Background UKCA and OMI tropospheric column NO2 typically ranges between 0 – 2 × 1015 molecules/cm2. Diurnal cycles and vertical profiles of the tropospheric NO2 column in UKCA show that the daily minimum tropospheric column NO2 occurs around the satellite overpass time. UKCA captures the seasonality but overestimates NO2, by a factor of ~2.5, especially during winter over E China and N India, at times and locations with high aerosol loadings. Heterogeneous chemistry is represented in the version of UKCA used here as uptake of N2O5 on internally generated sulfate aerosol. However, aerosol surface area may be underestimated in polluted locations, contributing to overestimation of NO2. In addition, the model may underestimate emissions of volatile organic compounds and associated peroxy acetyl nitrate (PAN) formation, leading to insufficient long-range transport of oxidised nitrogen, also contributing to overestimation of NO2 over polluted regions and underestimation over remote regions. Quantifying and understanding discrepancies in modelled NO2 warrant further investigation as they propagate into modelling of multiple environmental issues.

Keywords: Tropospheric NO2; UKCA Model; Air Quality; Satellite Data; Climate Modelling

How to cite: Pandey, A. K., Stevenson, D., Zhao, A., Pope, R., Hossaini, R., and Kumar, K.: Tropospheric NO2 over South and East Asia measured by OMI and modelled by UKCA, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-975, https://doi.org/10.5194/egusphere-egu25-975, 2025.

EGU25-2137 | PICO | AS3.32

A Study on the seasonal correlation between O3 and PM2.5 in Seoul 

Huijeong Lim, Misook Park, and Hui-Young Yun

Tropospheric ozone (O3) and fine particulate matter (PM2.5) are key air pollutants that significantly impact air quality, human health, and the environment. O3, a secondary pollutant, is primarily formed through photochemical reactions involving nitrogen oxides (NOx) and volatile organic compounds (VOCs) under sunlight, with its levels peaking in summer. In contrast, PM2.5 comprises both primary emissions and secondary aerosols, often showing higher concentrations in winter due to heating-related emissions and reduced atmospheric dispersion. In Korea, PM2.5 monitoring officially began in 2015, enabling more detailed analyses of its seasonal trends and correlations with other pollutants.

This study analyzed the seasonal correlation between O3 and PM2.5 using data from 25 air quality monitoring stations in Seoul from 2015 to 2024. Seasonal correlations were evaluated using Pearson correlation coefficients, and the relative contributions of NOx and PM2.5 to O3 levels were quantified through multiple linear regression models. A strong positive correlation was observed during summer (June, July, and August), attributed to the simultaneous formation of these pollutants driven by enhanced atmospheric oxidation capacity under strong sunlight and high temperatures. In contrast, winter (January, February, and December) exhibited a weak negative correlation, influenced by aerosol-radiation interactions and the O3 titration effect, where O3 is depleted through reactions with NOx.

Unlike previous studies that primarily focused on either O3 or PM2.5 trends independently, this study integrates seasonal correlation analyses with a quantitative assessment of the interplay between NOx and PM2.5 in O3 suppression. The findings indicate that NOx plays a more dominant role than PM2.5 in reducing O3 levels, especially under low O3 conditions. Seoul, as a megacity with complex emission sources and distinct seasonal dynamics, provides valuable insights that can inform air quality management strategies in other urban areas worldwide.

These findings provide a foundation for optimizing seasonal air quality management policies, particularly in regions with similar emission patterns and meteorological conditions. Future studies could extend this analysis by incorporating real-time meteorological data or applying chemical transport models to better capture the mechanisms driving seasonal variations in O3 and PM2.5.

 

Acknowledgments:

This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute (KEITI) funded by the Ministry of Environment (MOE)

How to cite: Lim, H., Park, M., and Yun, H.-Y.: A Study on the seasonal correlation between O3 and PM2.5 in Seoul, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2137, https://doi.org/10.5194/egusphere-egu25-2137, 2025.

EGU25-4456 | PICO | AS3.32

Trends of stratospheric BrO (1995 to 2025) derived from ground-based DOAS observations at Kiruna, Northern Sweden 

Thomas Wagner, Myojeong Gu, Carl-Fredrik Enell, Bianca Lauster, Kornelia Mies, Cornelius Otten, Ulrich Platt, Janis Pukite, Uwe Raffalski, and Steffen Ziegler

Stratospheric bromine originates partly from natural and partly from anthropogenic sources. After the Montreal protocol and following amendments, anthropogenic emissions (halons and methyl bromide) were largely reduced. This reduction was not only seen in tropospheric in situ measurements, but also in a reduction of stratospheric bromine levels (estimated from BrO measurements) after about 2002.

Here, we report on ground-based observations of stratospheric BrO carried out between 1995 and present in Kiruna (northern Sweden). The (slant) column density of BrO is analysed from UV spectra of zenith scattered sun light at solar zenith angles of 80° and 90°. Our measurements are in agreement with predictions predictions and existing observational data sets for the period before about 2019 for which a steady decline of the BrO levels is found. However, after 2019 the stratospheric BrO levels increased again, in contrast to the expected trend. The reason for this discrepancy is not yet known. Possible explanations might be increasing natural emissions of methyl bromide and/or very short lived bromine containing compounds, perhaps related to climate change (e.g. a warmer sea surface). Also recently again increasing anthropogenic emissions of methyl bromide might contribute. The variation of stratospheric aerosols is unlikely to explain the changed trend after 2019.

How to cite: Wagner, T., Gu, M., Enell, C.-F., Lauster, B., Mies, K., Otten, C., Platt, U., Pukite, J., Raffalski, U., and Ziegler, S.: Trends of stratospheric BrO (1995 to 2025) derived from ground-based DOAS observations at Kiruna, Northern Sweden, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4456, https://doi.org/10.5194/egusphere-egu25-4456, 2025.

EGU25-5926 | ECS | PICO | AS3.32

Past and future evolution of large-scale ozone episodes in Europe: results from reanalysis and Earth system models 

Rodrigo Crespo-Miguel, Carlos Ordóñez, Ricardo García-Herrera, Jordan L. Schnell, and Steven T. Turnock

Extreme near-surface ozone concentrations often cluster into large episodes that last several days. They strongly depend on meteorology, precursor emissions, and ambient photochemical conditions. A new pseudo-Lagrangian algorithm has been employed to identify the spatiotemporal patterns of episodes, allowing for a good characterization of their areal extent and an assessment of their drivers. The algorithm has been used to track ozone episodes in Europe from April to September over twenty years (2003–2022) of the Copernicus Atmosphere Monitoring Service (CAMS) reanalysis as well as in the historical simulation (1950–2014) and four Shared Socio-economic Pathways (SSPs, spanning 2015–2100) of three Earth system models (UKESM1-0-LL, EC-Earth3-AerChem and GFDL-ESM4). The algorithm has also been applied to detect ozone episodes in variations of the reference scenario ssp370 of UKESM1-0-LL, either with reduced precursor emissions or with the same emissions but present-day climate.

The results from CAMS show that, despite the overall increase in the number of episodes in recent years, the frequency of large episodes has decreased following European precursor emission reductions. The 100 largest episodes mainly occurred in northern Europe during spring and in the center and south of the continent from June onwards, whereas the top 10 episodes occurred in the first years of the century associated with high temperatures and anticyclonic conditions.

Despite the decrease in large episodes in recent years, there is uncertainty regarding future episodes. Episodes of reduced size are found for SSPs with weak greenhouse forcing and low precursor emissions. In contrast, episode sizes increase in scenarios with high methane concentrations and enhanced radiative forcing, even exceeding the maximum historical size. Furthermore, the comparison of episodes in variations of the reference scenario in UKESM1-0-LL enables the exploration of the separate contributions of climate change and precursor emissions. This analysis reveals that regional precursor reductions and global methane reductions are efficient strategies to significantly decrease the size of ozone episodes across the entire continent. On the other hand, global warming has contrasting effects which are, in any case, weaker than those of precursor emissions. 

This work is distributed under the Creative Commons Attribution 4.0 License. This licence does not affect the Crown copyright work, which is re-usable under the Open Government Licence (OGL). The Creative Commons Attribution 4.0 License and the OGL are interoperable and do not conflict with, reduce or limit each other.

How to cite: Crespo-Miguel, R., Ordóñez, C., García-Herrera, R., Schnell, J. L., and Turnock, S. T.: Past and future evolution of large-scale ozone episodes in Europe: results from reanalysis and Earth system models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5926, https://doi.org/10.5194/egusphere-egu25-5926, 2025.

EGU25-6871 | ECS | PICO | AS3.32

Comparison of reference upper-air GRUAN and homogenized RHARM data with GNSS-RO 

Fabrizio Marra, Emanuele Tramutola, Ilaria Gandolfi, Gessica Cosimato, Marco Rosoldi, and Fabio Madonna

The study of thermodynamical variables, such as temperature and relative humidity in the upper troposphere/lower stratosphere (UT/LS), is one of the key elements for the study of climate change. Several studies estimated trends both regionally and globally in the UT/LS, using both satellite and ground-based data and different measurement techniques. However, the measurement quality and coverage, in time and space, may significantly affect the estimated trends. In this work the temperature and relative humidity in the UT/LS from upper-air reference and homogenized datasets are compared with satellite GNSS-RO (Global Navigation Satellite System - Radio Occultation) and, in particular, the dataset RHARM (Radiosounding HARMonization), and the GNSS-RO with respect to GRUAN (Global Climate Observing System (GCOS) Reference Upper-Air Network) are investigated. Bias from these datasets have been estimated and compared at the GRUAN stations, used as the reference. Same quantities are also intercompared since 2001 at all the stations available in RHARM.

The comparison with GRUAN includes ascents since 2008 to 2024 and covers only mandatory levels from 850 hPa to 10 hPa on data provided by five stations (Sodankyla, Lindenberg, Ny Alesund, Lamont and Barrow), selected because of their long and dense data records. The RHARM data are matched to the GRUAN data applying an interpolation in a range of 40 Pa around mandatory levels between 850 hPa and 300 hPa and of 5 Pa below 300 hPa pressure. Then, a linear interpolation is applied between the minimum and the maximum pressures selected according to these criteria, Madonna (2022), Haimberger (2014).

Instead, the GNSS-RO data are matched to the GRUAN stations:

  • selecting all the profiles provided within a space-time mismatch of 200km - 3h, interpolating the samples at the mandatory pressure levels;
  • analyzing the profiles in function of the bending angle provided by GNSS-RO data.

The results of the comparison will be discussed: preliminary analysis, in terms of bias, shows a good agreement between RHARM and GRUAN, and a closer agreement of GNSS-RO with RHARM.

 

REFERENCES

 

Haimberger, L., 2012: Homogenization of the Global Radiosonde Temperature Dataset through Combined Comparison with Reanalysis Background Series and Neighboring Stations. J. Climate, 25, 8108–8131.

Madonna, F., 2022: The new Radiosounding HARMonization (RHARM) data set of homogenized radiosounding temperature, humidity, and wind profiles with uncertainties. Journal of Geophysical Research: Atmospheres, 127, e2021JD035220. 

How to cite: Marra, F., Tramutola, E., Gandolfi, I., Cosimato, G., Rosoldi, M., and Madonna, F.: Comparison of reference upper-air GRUAN and homogenized RHARM data with GNSS-RO, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6871, https://doi.org/10.5194/egusphere-egu25-6871, 2025.

EGU25-7654 | ECS | PICO | AS3.32

Long-Term Trends of Atmospheric Black Carbon Deposition across China 

Yourong Fan, Abdallah Shaheen, Fang Wang, Robabeh Yousefi, and Quansheng Ge

Background ozone is highlighted as a factor that reflects the impact of intercontinental transport and international emissions of precursors as well as regional photochemical pollution. In this study, we used daily mean, MDA8 (max. daily 8-hour average), and MinDA8 (min. daily 8-hour average) ozone concentrations obtained from three national background air pollution monitoring stations—Jeju, Ulleung, and Baengnyeong—to investigate the long-term trends of Korea's background ozone concentrations. Ensemble Empirical Mode Decomposition (EEMD) was applied to decompose ozone time series of these concentrations into long-term, medium-termeasonal, and short-term variability for 2001 – 2022. Here, we define the background ozone variations as the long-term component extracted from the daily mean time series to compare them with those estimated in the west coast of the United States and Europe in the previous study.

The results showed that Jeju's background ozone concentration has steadily increased at the rate of 0.26 ppb per year since 2001 similar to those observed in urban monitoring stations, whereas both Ulleung and Baengnyeong stations initially showed increasing trends but shifted to declining trends after 2015, with annual rates of -0.37 and -0.25 ppb per year, respectively. To explore these differences, we defined daily ozone production (DOP) as the difference between MDA8 and MinDA8. The long-term components of DOP in urban stations, extracted using EEMD, was approximately 10 ppb higher than at background stations due to precursor emissions from anthropogenic sources, with little variation over time. In contrast, background DOP has steadily decreased since 2015, with decreasing rates of 0.26 and 0.25 ppb per year in Jeju and Ulleung, respectively.

In California, the contribution of background ozone to the ozone design value (ODV) has steadily increased, reaching approximately 70% in 2022 due to exponential decrease in anthropogenic ozone production. By comparison, the contribution of background ozone in background regions began to increase, starting in 2016, and reached about 50% in 2022. These findings underscore the importance of addressing background ozone in national air quality management strategies and offer a scientific basis for establishing effective mitigation policies.

Acknowledgments

This work was funded by the Korea Meteorological Administration Research and Development Program under Grant RS-2024-00404042.

How to cite: Lee, J. and Choi, W.: Long-Term Trends and Regional Differences in Background Ozone Concentrations in Korea: Insights from EEMD Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7984, https://doi.org/10.5194/egusphere-egu25-7984, 2025.

EGU25-8446 | PICO | AS3.32

The atmospheric station at Plateau Rosa: use of methane mole fractions and modelling to detect methane source areas in Europe 

Giulia Zazzeri, Francesco Apadula, Stephan Henne, and Andrea Lanza

The atmospheric monitoring station at Plateau Rosa, situated in the Central European Alps and part of the ICOS (Integrated Carbon Observation System) framework since 2021, is measuring methane mole fractions since 2018 with a cavity ring down spectrometer (Picarro G2301). Concentration measurements at this site, 3480 meter AMSL, are particularly valuable for tracking the atmospheric background and global trend of methane, but are also impacted by various source areas in Europe.

In this study, we analyzed the continuous record of methane mole fractions at the station, and we identified prolonged periods (more than 6 hours) of enhanced methane levels over the background that are associated with pollution events at regional scale. From 2020 until 2024, we detected 15 very pronounced pollution events, when air masses were coming mainly from central Europe and the UK. We used the FLEXPART atmospheric transport model coupled to the high-resolution (1 km x 1 km) output of the numerical weather prediction model COSMO to produce concentration footprints and simulate regional methane contributions. We assessed how well this transport model, coupled with different bottom-up inventories (EDGAR, TNO), can capture the selected pollution events. Finally, we compared the source areas identified with the TROPOMI satellite emission plumes measured in Europe.

We demonstrate how methane mole fraction data measured continuously at the station at Plateau Rosa can be used to attribute pollution events to specific regional source areas that might not be accounted by the inventories and are not detectable by satellite data.

How to cite: Zazzeri, G., Apadula, F., Henne, S., and Lanza, A.: The atmospheric station at Plateau Rosa: use of methane mole fractions and modelling to detect methane source areas in Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8446, https://doi.org/10.5194/egusphere-egu25-8446, 2025.

EGU25-8610 | PICO | AS3.32

The state of greenhouse gases in the atmosphere using global observations through 2023 

Oksana Tarasova, Alex Vermeulen, Xin Lan, and Kazuhiro Tsuboi

This paper highlights the main findings of the twentieth annual Greenhouse Gas Bulletin (https://library.wmo.int/records/item/69057-no-20-28-october-2024) of the World Meteorological Organization (WMO). The results are based on research and observations performed by laboratories contributing to the WMO Global Atmosphere Watch (GAW) Programme (https://community.wmo.int/activity-areas/gaw).

The Bulletin presents global analyses of observational data collected according to GAW recommended practices and submitted to the World Data Center for Greenhouse Gases (WDCGG). Bulletins are prepared by the WMO/GAW Scientific Advisory Group on Greenhouse Gases in collaboration with WDCGG.

Observations used for the global analysis are from 146 marine and terrestrial sites for CO2, 153 for CH4 and 112 for N2O. The globally averaged surface mole fractions calculated on the basis of these observations reached new highs in 2023, with CO2 at 420.0±0.1 ppm, CH4 at 1934±2 ppb and N2O at 336.9±0.1 ppb. These values constitute, respectively, increases of 151%, 265% and 125% relative to pre-industrial (before 1750) levels. The increase in CO2 from 2022 to 2023 (2.3 ppm) was slightly higher than the increase observed from 2021 to 2022 and slightly lower than the average annual growth rate over the last decade, which was most likely partly caused by natural variability, as fossil fuel CO2 emissions have continued to increase. This increase marked the twelfth consecutive year with an increase greater than 2 ppm.

The Bulletin reports that within-year variability of CO2 was 2.8 ppm in 2023, the fourth largest within-year annual increase since modern CO2 measurements started in the 1950s. Such increase may be a result of enhanced fire emissions and reduced net terrestrial carbon sinks. The CO2 growth rate varies from year to year (between 2.1 and 3.2 ppm during 2014-2023), with the variability mostly driven by the terrestrial biosphere exchange of CO2, as confirmed by measurements of the stable carbon isotopes ratio, 13C:12C in atmospheric CO2. Coincidental with the large CO2 increase during 2023 was the largest increase in atmospheric carbon monoxide (CO) in the past two decades, suggesting enhanced CO2 emissions from fires.

The increase of CH4 mole fraction from 2022 to 2023 (11 ppb) was lower than that observed from 2021 to 2022 but still slightly higher than the average annual growth rate over the last decade. The record rise in atmospheric CH4 from 2020 to 2022 was accompanied by a significant drop in atmospheric δ13CCH4. The unexpected change in the amount of atmospheric δ13CCH4 is best explained by a transition from fossil fuels to microbial emissions as the dominant driver of increasing CH4. Moreover, the geographic distribution of CH4 growth from 2020 to 2022 suggest strong increases in isotopically light emissions from tropical and boreal wetland areas, which is indicative of positive climate feedback on CH4 emissions in response to climate transition to an El Niño phase in 2023.

In the near future, climate change itself could cause ecosystems to become larger sources or sinks of GHGs. Identifying and tracking the potential climate feedbacks require continued high accuracy observations also at currently undersampled regions.

How to cite: Tarasova, O., Vermeulen, A., Lan, X., and Tsuboi, K.: The state of greenhouse gases in the atmosphere using global observations through 2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8610, https://doi.org/10.5194/egusphere-egu25-8610, 2025.

Recent successes in reducing PM2.5 concentrations in the atmosphere have led to significant shifts in the concentrations of various compounds. Sustaining the efficacy of control measures requires continuous monitoring of these changes. This study examined the decadal variations from 2012 to 2022 of concentrations of PM2.5 and its inorganic components—sulfate, nitrate, ammonium, chloride, and non-volatile cations (NVC)—assessed via offline filters at an urban site (Yuen Long, YL) and a suburban site (HKUST, UST) in Hong Kong. We also cross-referenced the offline filter data with online MARGA results at both sites over a portion of the ten-year period for data validation. Our analysis indicates a consistent decline in PM2.5 concentrations, registering an average reduction of 1.55 ± 0.16 μg/m³ (p < 0.01) per year in YL and 1.37 ± 0.17 μg/m³ (p < 0.01) per year in UST during the ten-year period. Inorganic compounds constituted 47.4 ± 10.1% and 51.5 ± 10.0% of PM2.5 by mass in YL and UST, respectively, with sulfate accounting for over half of PM2.5 at both sites. The decline in inorganic compounds over the years was primarily attributed to sulfate, which decreased at rates of 0.63 ± 0.04 μg/m³ (p < 0.01) per year in YL and 0.67 ± 0.05 μg/m³ (p < 0.01) per year in UST. While nitrate remained relatively steady in its concentrations, it constituted a larger mass fraction of both inorganic compounds and PM2.5 at both sites. Seasonal variations were explored by comparing summer and winter trends. The rate of sulfate reduction in winter was approximately twice that in summer at both sites, contributing to ~40% of PM2.5 reduction, as sulfate and PM2.5 concentrations were significantly higher in winter. In contrast, nitrate concentrations exhibited an upward trend during winter, with notable increases from 1.87 μg/m³ to 7.63 μg/m³ in YL and from 0.75 μg/m³ to 3.47 μg/m³ in UST between 2020 and 2021, elevating its mass fraction in PM2.5. In comparison, summer nitrate concentrations averaged below 1 μg/m³.

Our data validation indicated that offline filter-based nitrate measurements were underestimated under high-temperature conditions, casting high uncertainty on summer filter measurements. MARGA data revealed nitrate mass fractions as high as 28% in suburban UST in 2021, significantly greater than the 13% estimated from filter data due to this underestimation. This study highlights the escalating significance of nitrate alongside successful sulfate reductions in the PM2.5 composition of both urban and suburban areas of Hong Kong, particularly during winter. Future air quality improvement policies should prioritize addressing nitrate. Furthermore, caution is warranted when interpreting nitrate concentrations measured by filters under high-temperature conditions due to the associated measurement uncertainty.

How to cite: Zhang, Z. and Yu, J.: Ten-year trend of PM2.5 sulfate, nitrate, and other inorganic constituents from 2012 to 2021 in urban and suburban sites of Hong Kong, China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9750, https://doi.org/10.5194/egusphere-egu25-9750, 2025.

EGU25-9901 | PICO | AS3.32

A 45-year chemistry and aerosol simulation with IFS-COMPO: trend analysis and first evaluation 

Vincent Huijnen, Ramiro Checa-Garcia, Samuel Rémy, Retish Senan, Swen Metzger, Simon Chabrillat, and Johannes Flemming

Within the Copernicus Atmosphere Monitoring Service (CAMS), ECMWF operates the Integrated Forecasting System with atmospheric composition extension (IFS-COMPO) to provide global forecasts and reanalyses of aerosols and trace gases. In support of ongoing preparations for a new CAMS reanalysis, which will cover the years 2003-present, multi-decadal model simulations with a fixed IFS-COMPO model configuration, but excluding composition data assimilation, have been produced for the same period. Recently these simulations have been extended into the past, back to 1978, with the aim to produce a consistent assessment of trends in atmospheric composition-related aspects. This includes an analysis of model trends in tropospheric and stratospheric ozone, aerosol optical depth, and nitrogen and sulfur deposition, and methane lifetime.  For this purpose we apply a version of CMIP emissions for years prior to 2003, when no CAMS-GLOB emissions are available, along with appropriate surface nudging of CFC’s, nitrous oxide and methane. We run multiple batches of multi-year simulations in parallel, driven by ERA5 meteorology. We take care of a reasonable hand-shake procedure for the different emission estimates as they cross for the year 2003.

In this contribution we report on the design and first assessment of global atmospheric composition trends for the period 1978-2024 in these model simulations, and discuss evaluation results with emphasis for the 2003-2020 period, focusing on trends in simulated methane loss rate, and factors which drive these results.

How to cite: Huijnen, V., Checa-Garcia, R., Rémy, S., Senan, R., Metzger, S., Chabrillat, S., and Flemming, J.: A 45-year chemistry and aerosol simulation with IFS-COMPO: trend analysis and first evaluation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9901, https://doi.org/10.5194/egusphere-egu25-9901, 2025.

EGU25-10421 | PICO | AS3.32

The GAW-QC App: Improving Quality Control through Data Science and Numerical Forecasts 

Yuri Brugnara, Simone Baffelli, Martin Steinbacher, Christoph Zellweger, and Lukas Emmenegger

The Global Atmosphere Watch (GAW) Programme of the World Meteorological Organization coordinates a worldwide network of hundreds of ground-based in-situ monitoring stations that provide reliable scientific data on the chemical composition of the atmosphere. Within the framework of the GAW Programme, the Quality Assurance/Scientific Activity Centre Switzerland has developed a web app (GAW-QC, available at www.empa.ch/gaw, see also Brugnara et al., 2024) to support station operators in timely detecting issues in their in-situ measurements of various trace gases.

GAW-QC consists of a dashboard that highlights anomalous values using a mixture of purely data-driven and hybrid anomaly detection techniques. It exploits historical measurements made at the target station as well as the archive of gridded numerical forecasts by the Copernicus Atmosphere Monitoring Service (CAMS). The accuracy of the latter for the specific site is improved through machine learning using multiple predictors, including meteorological parameters and aerosol concentrations.

The app allows station operators to upload their latest measurements, visualize the data with different temporal aggregations, and detect anomalous values using just their internet browser. By combining the information gathered from the dashboard with logbook entries and local expertise, they can effectively flag problematic measurements and even detect instrumental issues that would remain unnoticed otherwise. First case studies indicate that this process can indeed facilitate the detection of malfunctions in the analytical setup and reduce the ingestion of erroneous data into international data repositories. Moreover, it has the potential to shorten data gaps if applied timely.

GAW-QC is publicly available and can be used to analyze historical time series of carbon dioxide, carbon monoxide, methane, and ozone made at 98 GAW stations worldwide. The applicability to a given station depends on whether historical data have been submitted to the GAW world data centers by the station operator. Additional gas species may be added in the future depending on user feedback.

 

Brugnara, Y., Steinbacher, M., Baffelli, S., and Emmenegger, L.: Technical note: An interactive dashboard to facilitate quality control of in-situ atmospheric composition measurements, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2024-3556, 2024.

How to cite: Brugnara, Y., Baffelli, S., Steinbacher, M., Zellweger, C., and Emmenegger, L.: The GAW-QC App: Improving Quality Control through Data Science and Numerical Forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10421, https://doi.org/10.5194/egusphere-egu25-10421, 2025.

EGU25-10935 | PICO | AS3.32

Do rural background sites capture changes in primary PM2.5 emissions at the national scale? Recent trends in PM2.5 and its main components in metropolitan France. 

Anna Font, Joel F. de Brito, Véronique Riffault, Sébastien Conil, Jean-Luc Jaffrezo, and Aude Bourin

Trends in daily PM2.5 mass concentrations were assessed at 5 rural background sites in France over the period 2014-2021, together with major particulate components associated with (i) anthropogenic emissions including fossil fuels (FF) and biomass burning (BB) from primary emissions; and (ii) non-sea-salt sulphate, nitrate and ammonium, i.e., secondary particulate constituents from gaseous precursors sulphur dioxide, nitrogen oxides and ammonia, respectively. To disentangle the influence of weather, long-range transport, and the oxidative capacity of the atmosphere, boosted regression tree (BRT) models were built at each site; and normalised time series were calculated by randomising the value of the explanatory variables at a given time. Different BRT models were formulated and two types of normalised PM2.5 time series were calculated: de-weathered time series (without the influence of the meteorological and long-range transport) and de-weathered & de-oxidised time series (randomisation of meteorology, transport and OX (NO2 + O3) levels). Over the studied period, PM2.5 concentrations decreased at approximatively -5% year-1, almost 1.5 times faster than changes in primary emissions in France. Overall trends in de-weathered, and de-weathered and de-oxidised PM2.5 concentrations were lower than trends in PM2.5 observations for the same period, at -3.9% year-1 and -3.2 % year-1, respectively. Trends in de-weathered & de-oxidised PM2.5 were close to those in emissions, demonstrating the importance of including variables capturing the oxidative capacity of the atmosphere in the normalising techniques to compare trends in PM2.5 with trends in primary emissions. Trends in observations of PM2.5 were consistent with trends in nitrate particles from reduced NOX emissions, and to trends in ammonium particles and biomass burning.

How to cite: Font, A., F. de Brito, J., Riffault, V., Conil, S., Jaffrezo, J.-L., and Bourin, A.: Do rural background sites capture changes in primary PM2.5 emissions at the national scale? Recent trends in PM2.5 and its main components in metropolitan France., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10935, https://doi.org/10.5194/egusphere-egu25-10935, 2025.

EGU25-11261 | PICO | AS3.32

Prognostic Ozone For ICON: Enabling UV Forecasts 

Valentin Hanft, Roland Ruhnke, Axel Seifert, and Peter Braesicke

Stratospheric Ozone (O3) absorbs biologically harmful solar ultraviolet radiation, mainly in the UV-B and UV-C spectral range. When reaching the surface, such UV radiation poses a well documented hazard to human health. In order to quantify this amount of UV radiation and to make it generally understandable, the World Health Organization (WHO) has defined an UV Index [1]. It is calculated by weighting the incoming solar irradiance at surface level between 250 and 400 nanometers with their ”harmfulness” to the skin and scaling the results to values that normally range between 1 and 10, surpassing 10 for excessive UV exposure.

In our project we extend the capability of ICON (ICOsahedral Nonhydrostatic Model,[2]), the operational forecast model used by the German Meteorological Service, to provide a configuration of self-consistent UV Index forecasts that do not require external data. For this, we use ICON-ART [3],[4] with a linearized prognostic ozone scheme (LINOZ,[5]) and couple the prognostic ozone to the atmospheric radiation scheme Solar-J [6].

With this setup, we define a global test run from March to July 2022. This time frame contains distinct ozone features above Europe due to the polar vortex as well as its breakup and the transition to the summer circulation. We use the results to validate the UV Index forecast with respect to  parameters that influence it, e.g. aerosol optical depth, surface albedo, or cloud cover. For the comparison we use other model data (CAMS,[7]) as well as ground-based and satellite measurements (e.g. CERES,[8]).

References:

[1] World Health Organization and World Meteorological Organization and United Nations Environment Programme and International Commission on
Non-Ionizing Radiation Protection. Global solar UV Index : a practical guide, 2002.
[2] G. Zängl, et al. The ICON (icosahedral non-hydrostatic) modelling framework of dwd and mpi-m: Description of the non-hydrostatic dynamical core. Quarterly Journal of the Royal Meteorological Society, 141(687):563–579, 2015.
[3] J. Schröter, et al. ICON-ART 2.1: a flexible tracer framework and its application for composition studies in numerical weather forecasting and
climate simulations. Geoscientific Model Development, 11(10):4043–4068,2018.
[4] D. Rieger, et al. ICON–ART 1.0 – a new online-coupled model system from the global to regional scale. Geoscientific Model Development, 8(6):1659–1676, 2015.
[5] C. A. McLinden, et al. Stratospheric ozone in 3-d models: A simple chemistry and the cross-tropopause flux. Journal of Geophysical Research: Atmospheres,105(D11):14653–14665, 2000.
[6] J. Hsu, et al. Aradiative transfer module for calculating photolysis rates and solar heating in climate models: Solar-j v7.5. Geoscientific Model Development, 10(7):2525–2545, 2017.
[7] CAMS Global Atmospheric Composition Forecasts, https://ads.atmosphere.copernicus.eu/datasets/cams-global-atmospheric-
composition-forecasts?tab=overview, 01 2025.
[8] NASA/LARC/SD/ASDC. CERES and GEO-Enhanced TOA, Within-Atmosphere and Surface Fluxes, Clouds and Aerosols 1-Hourly Terra-Aqua
Edition4A, 09 2017.

How to cite: Hanft, V., Ruhnke, R., Seifert, A., and Braesicke, P.: Prognostic Ozone For ICON: Enabling UV Forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11261, https://doi.org/10.5194/egusphere-egu25-11261, 2025.

EGU25-11279 | ECS | PICO | AS3.32

ENSO impact on mid-tropospheric composition above the Tropical Western Pacific via air mass transport 

Katrin Müller, Tim Röpke, Xiaoyu Sun, Ingo Wohltmann, and Markus Rex

The Tropical West Pacific (TWP) is the key entry point of air into the stratosphere during Northern Hemispheric winter. Thus, the local air composition can influence global atmospheric chemistry and dynamics. Its interannual variability is itself affected by the El Niño Southern Oscillation (ENSO). The transport history of tropospheric air masses above the TWP is in particular reflected by the local ozone (O3) and relative humidity (RH) characteristics (Müller et al., 2024b).

We use regular balloon-borne profile measurements of these quantities from the Palau Atmospheric Observatory (PAO) to assess the (interannual) variability of TWP air masses and controlling processes (Müller et al., 2024a). Located in the centre of the tropical warm pool (7°N, 134°E) in Koror, Palau, the PAO has been filling a previous observational gap in this region since 2016 and has recently become a member of the SHADOZ (Southern Hemisphere Additional Ozonesondes) network. Our latest analysis of the PAO ozonesonde record showed how transport to the TWP mid-troposphere (5-10 km altitude) is modulated by the movement of the Intertropical Convergence Zone, allowing transport of polluted air masses from tropical Asia mainly between February and April into the otherwise clean air column (Müller et al. 2024b, Sun et al. 2023).

Here, we present an extended view on air mass transport to the region with a focus on the impact of ENSO on its interannual variability using an updated PAO time series (2016-2024), interhemispheric transport modelling using GEOS-Chem (Sun et al. 2023) and trajectory calculations from the Lagrangian Chemistry and transport model ATLAS (Wohltmann and Rex 2009). We found that very humid and ozone-poor air masses are suppressed in the free troposphere during El Niño. For La Niña conditions, the O3/RH distribution is shifted towards higher RH indicating enhanced convection compared to neutral conditions, but seasonal observations of dry ozone-rich air masses and long-range transport from Asia still occur.

The high convective activity in the TWP induces and maintains an ozone-poor humid tropospheric background. Its modulation by ENSO via sea-surface temperature and dynamical changes consequently either suppresses (El Niño) or strengthens (La Niña) the background composition. However, for the given time series the seasonal transport patterns prevail, which relate to a background composition of low O3 and high RH between July and October and dynamic disturbances of this background in form of dry ozone-rich layers between November and April.

How to cite: Müller, K., Röpke, T., Sun, X., Wohltmann, I., and Rex, M.: ENSO impact on mid-tropospheric composition above the Tropical Western Pacific via air mass transport, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11279, https://doi.org/10.5194/egusphere-egu25-11279, 2025.

EGU25-11621 | PICO | AS3.32

Global Inversion of a Black Carbon Emissions based on FLEXPART modelling and a Bayesian inversion algorithm 

Sabine Eckhardt, Rona L. Thompson, Nikolaos Evangeliou, Ignacio Pisso, Karl-Espen Yttri, Christine Groot Zwaaftink, and Stephen M. Platt

Black carbon (BC) is a significant climate forcer and a major health hazard especially close to its sources. BC has both natural (e.g., wildfires) and anthropogenic sources (e.g., industry, traffic, oil and gas industries). Its distribution in the atmosphere is highly inhomogeneous. Understanding both the spatial distribution and the magnitude of BC emissions is critical for accurate climate modeling. However, emission inventories for BC are fraught with uncertainties, largely stemming from uncertainties in emission factors, which complicate global scale modeling efforts. Observational data, especially when obtained by different measurement techniques, which is essential for constraining emission estimates, carry their own uncertainties.

In this study, we present a global inversion of BC emissions over a 5-year period, using a combination of global observations, atmospheric modeling with FLEXPART, and a Bayesian inversion algorithm (FLEXINVERT). Our approach aims to reconcile uncertainties in both emissions and observations, providing a more robust estimate of BC distribution and sources. Even though presenting a global picture, we focus on Europe, an area with a high density of observation sites, enabling more precise emission estimates. The tropics and southern hemisphere have only sparse observations. Moreover, we highlight the significant role of wildfires as a source of BC, with implications for both local and global climate impacts.

Our findings contribute to improving the accuracy of BC inventories which can be used both for climate modelling and air quality assessments.

How to cite: Eckhardt, S., Thompson, R. L., Evangeliou, N., Pisso, I., Yttri, K.-E., Groot Zwaaftink, C., and Platt, S. M.: Global Inversion of a Black Carbon Emissions based on FLEXPART modelling and a Bayesian inversion algorithm, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11621, https://doi.org/10.5194/egusphere-egu25-11621, 2025.

EGU25-12166 | PICO | AS3.32

Chlorine activation as seen by TROPOMI OClO 2017 – 2025 measurements 

Janis Pukite, Steffen Ziegler, and Thomas Wagner

Chlorine dioxide (OClO) is a by-product of the ozone depleting halogen chemistry in the stratosphere. Although being rapidly photolysed during daytime, it plays an important role as an indicator of the chlorine activation in polar regions during polar winter and spring under twilight conditions because of the nearly linear dependence of its formation on chlorine oxide (ClO).

The TROPOspheric Monitoring Instrument (TROPOMI) is an UV-VIS-NIR-SWIR instrument on board the Sentinel-5P satellite developed for monitoring the composition of the Earth’s atmosphere. Launched on 13 October 2017 in a near polar orbit, it provides    continuous monitoring possibilities for many constituents including the observations of OClO at an unprecedented spatial resolution.

We analyze the time series (2017 – 2025) of slant column densities (SCDs) of chlorine dioxide (OClO) at polar regions. Especially we focus on the higly variable conditions in the NH polar region by comparing the OClO timeseries with meteorological data. This allows us to investigate the conditions under which the chlorine activation starts and ends.

 

How to cite: Pukite, J., Ziegler, S., and Wagner, T.: Chlorine activation as seen by TROPOMI OClO 2017 – 2025 measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12166, https://doi.org/10.5194/egusphere-egu25-12166, 2025.

EGU25-12725 | PICO | AS3.32

IAGOS in situ observations of NOx in the upper troposphere over the tropical Atlantic 

Christoph Mahnke, Ulrich Bundke, Norbert Houben, Chris Schleiermacher, Torben Galle, Philippe Nédélec, Bastien Sauvage, Valérie Thouret, Hannah Clark, and Andreas Petzold

Nitrogen oxides (NOx), ozone (O3), and carbon monoxide (CO) are important air quality indicators, while NOx is also one of the main precursors of O3. These trace gases have anthropogenic and natural sources at ground level and in the troposphere. At ground level, the main sources are transport emissions, industry, agriculture, and biomass burning. In the troposphere, additional sources include lighting and aircraft emissions and in the upper troposphere, downmixing from the stratosphere also makes a significant contribution to the ozone budget. Furthermore, the abundances of NOx and O3 in the troposphere are controlled by photochemistry.

The European Research Infrastructure IAGOS (www.iagos.org) uses in-service passenger aircraft as observation platforms, equipped with instruments to measure gaseous species, aerosols, and cloud particles. Since 2023 an IAGOS-CORE NOx instrument (Package 2b) is installed aboard an IBERIA Airbus A330-200. Based in Madrid (Spain), this IAGOS-CORE aircraft covers routes to North, but mainly Central and South America. On the routes from Europe to Central and South America, the atmospheric abundances of the climate and air quality relevant trace gases CO, O3, NO, NO2, and NOx were observed in the photochemically active region over the tropical Atlantic over the course of one year. From this unique dataset, we characterize the variability and the horizontal distribution of these trace gases across the Intertropical Convergence Zone and discuss the origin of the observed air masses.   

Acknowledgments: We thank all members of IAGOS-CORE, in particular IBERIA for enabling these IAGOS-CORE observations. The German Federal Ministry of Education and Research (BMBF) is acknowledged for financing the instruments operation and data analysis as part of the joint project IAGOS-D under grant 01LK1301A.

How to cite: Mahnke, C., Bundke, U., Houben, N., Schleiermacher, C., Galle, T., Nédélec, P., Sauvage, B., Thouret, V., Clark, H., and Petzold, A.: IAGOS in situ observations of NOx in the upper troposphere over the tropical Atlantic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12725, https://doi.org/10.5194/egusphere-egu25-12725, 2025.

EGU25-15590 | PICO | AS3.32

The Evolution of Surface Ozone Data Quality over the Past 3 Decades 

Christoph Zellweger, Martin Steinbacher, and Lukas Emmenegger

For nearly 30 years, Empa has operated the World Calibration Centre for Carbon Monoxide, Methane, Carbon Dioxide and Surface Ozone (WCC-Empa) as a Swiss contribution to the Global Atmosphere Watch (GAW) programme. In this capacity, WCC-Empa has played a central role in sustaining and improving the data quality and availability required for climate and environmental research.

A core activity of WCC-Empa is the quality control of GAW stations through on-site system- and performance audits. We have conducted more than 120 audits as an independent verification of the traceability of measurements to the accepted standards of the WMO/GAW programme, which are hosted and distributed by Central Calibration Laboratories (CCLs). These audits also include operator training and capacity building to improve data availability and quality, especially in less developed regions.

Our presentation will focus on the evolution of surface ozone data quality over the past three decades. We have assessed the stability of the traceability chain from the primary reference standard (the NIST Standard Reference Photometer family) to the transfer standards and the analysers used in the field. Unlike other parameters, the technique for measuring ozone has not changed in the last 30 years, and most surface ozone measurements are made using the UV absorption technique. About two-thirds of the comparisons met the data quality objectives (maximum bias of 1 nmol mol-1) of the GAW programme.

Looking ahead, a new ozone absorption cross-section will be implemented in 2025 (bipm.org/en/ozone). This will improve the accuracy of ozone measurements but will have an impact on exceedances of air quality standards by increasing ozone values by 1.29%. We will discuss the implications of the new cross-section value and provide guidance on how to make the transition.

How to cite: Zellweger, C., Steinbacher, M., and Emmenegger, L.: The Evolution of Surface Ozone Data Quality over the Past 3 Decades, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15590, https://doi.org/10.5194/egusphere-egu25-15590, 2025.

EGU25-15792 | ECS | PICO | AS3.32

Multi-year evolution of tropospheric ozone pollution and its main drivers over East Asia during spring analyzed from multispectral satellite observations and in situ measurements 

Beatrice Biagi, Juan Cuesta, Hiroshi Tanimoto, Yugo Kanaya, Gaëlle Dufour, Matthias Beekmann, and Maxim Eremenko

Air quality is a major societal concern in East Asia, contributing to (approximately) two million premature deaths annually. Rapid economic growth in regions such as the North China Plain and Punjab, combined with extensive urbanization of megacities, has led to a significant rise in air pollutant emissions. Ozone precursors emitted from this region are transported across long distances, undergoing chemical transformations and affecting downwind regions, including Japan and even North America. This long-range transport highlights the need to better understand the processes driving ozone eastward dispersion across the Pacific Ocean.

The primary objective of this study is to provide a robust, multi-year quantification of tropospheric ozone transport from East Asia, particularly from air pollution hotspots and its transport to downwind regions. We aim to characterize key conditions influencing eastward ozone transport:  meteorological patterns, stratosphere-troposphere exchange (STE), surface emissions of ozone precursors including biomass burning, etc. For our study, we use long-term satellite observations from the IASI+GOME2 multispectral satellite product offering particularly enhanced sensitivity in the lowermost troposphere (below 3 km of altitude) and ground-based in situ measurements from surface stations and ship. Meteorological models are used to analyze atmospheric transport and atmospheric conditions.

Preliminary analyses indicate that eastward transport events occur during the spring, specifically in March, mainly influenced by meteorological condition (the rising of temperature and insolation) that leads to an increase of photochemistry and the active presence of sources, such as agricultural biomass burning. Moreover, the study allows us to highlight several transport pathways of tropospheric ozone reaching the Pacific Ocean.

How to cite: Biagi, B., Cuesta, J., Tanimoto, H., Kanaya, Y., Dufour, G., Beekmann, M., and Eremenko, M.: Multi-year evolution of tropospheric ozone pollution and its main drivers over East Asia during spring analyzed from multispectral satellite observations and in situ measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15792, https://doi.org/10.5194/egusphere-egu25-15792, 2025.

EGU25-15915 | PICO | AS3.32

Air Quality Challenges in Gangtok, Sikkim Himalaya: A Study of Aerosol Variability and Impacts 

Rakesh Kumar Ranjan, Aparna Gupta, Rajeev Rajak, Bidyutjyoti Baruah, Ankita Roy, Shruti Dutta, and Amit Prakash

The study investigates the spatial and altitudinal variability of aerosol components, including Black Carbon (BC), PM1, PM2.5, PM10, Total Suspended Particles (TSPM), respirable, thoracic, and inhalable particulate matter, across different sites in Gangtok, Sikkim Himalaya. The monitoring locations - Residential (Site 1, 900 m), Commercial (Site 2, 1800 m), and Control (Site 3, 2200 m) demonstrate distinct altitudinal gradients in ambient aerosol concentrations. The measurements were conducted during the winter of 2024 using an Aethalometer AE-33 to measure BC and an EDM 264 to analyse various size of aerosols in the ambient atmosphere. BC associated with PM2.5 decrease from 4.94 µg/m³ at Site 1 to 2.62 µg/m³ at Site 2 and 1.49 µg/m³ at Site 3, while PM2.5 concentrations follow a similar pattern, declining from 84.88 µg/m³ to 18.62 µg/m³. Comparable trends are observed for PM1, PM10, and TSPM, with higher concentrations at lower altitudes indicating the dominance of anthropogenic activities and population density. These components also exhibited strong diurnal variability, with daytime levels consistently higher than night-time levels across all sites. For instance, at Site 1, the mean daytime BC concentration is 5.59 µg/m³, compared to 3.63 µg/m³ at night. This variation is attributed to increased vehicular emissions and other human activities during the day. Additionally, a strong correlation is observed between BC and PM2.5 levels indicating common sources such as combustion-related activities. Lower temperatures and higher RH at each site, enhanced aerosol condensation and particle deposition, resulting in reduced pollutant concentrations. Components like respirable, thoracic, and inhalable particulates, critical for assessing health impacts, also show decreasing trends with altitude but remain concerning in residential areas at lower altitudes due to their ability to penetrate the respiratory system. BC's role as a short-lived climate pollutant with high radiative forcing potential further emphasizes its environmental significance in the ecologically sensitive Himalayan region. Addressing the sources of aerosols, particularly in densely populated lower-altitude areas, is vital for improving air quality and mitigating health and climate impacts in the Sikkim Himalaya.

How to cite: Ranjan, R. K., Gupta, A., Rajak, R., Baruah, B., Roy, A., Dutta, S., and Prakash, A.: Air Quality Challenges in Gangtok, Sikkim Himalaya: A Study of Aerosol Variability and Impacts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15915, https://doi.org/10.5194/egusphere-egu25-15915, 2025.

EGU25-16483 | ECS | PICO | AS3.32 | Highlight

The contribution of natural emissions to tropospheric composition above the Amazon 

Flossie Brown and Colette Heald

Natural emissions, such as BVOCs and soil NOx, from tropical forests can affect tropospheric composition, reliant on the magnitude of emission and on what escapes from the canopy. In-canopy processes are not typically resolved in 3D regional or global models. Here, we investigate the diurnal variability of emissions, deposition and chemistry occurring at the ATTO site in the Amazon using the FORCAsT column model, which resolves the canopy space in 17 levels and extends above the boundary layer. Comparison to observations of meteorology and chemical species made at 8 heights confirms satisfactory performance of the model for the ATTO site. We explore the contribution of soil NOx to the atmospheric oxidative capacity above the canopy including its role in O3 formation. In combination with canopy level deposition, we identify substantial deposition of NOx at the soil surface due to slow mixing at this height. In addition, at this dark level within the forest, NO reaction with O3 is an important driver of chemistry. Finally, our model suggests buildup and net removal of NOx within the canopy overnight as mixing decreases, followed by release of NO in the morning. These findings reveal the role of in-canopy chemistry and deposition on above-canopy composition under pristine conditions, providing a baseline for comparison to polluted conditions and to global models without a resolved canopy.   

How to cite: Brown, F. and Heald, C.: The contribution of natural emissions to tropospheric composition above the Amazon, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16483, https://doi.org/10.5194/egusphere-egu25-16483, 2025.

Trifluoroacetic acid (TFA), a short chain perfluorocarboxylic acid (scPFCA), is a contaminant of emerging concern because its emissions are projected to rapidly increase, it is highly persistent, and remediation is challenging. Recent studies based on ice core records report large increases (up to a factor of ~10) in Arctic TFA deposition since the 1970s. The ice core temporal trends suggest that CFC replacement gases introduced following the Montreal Protocol could be an important source. However, TFA is a “substance from multiple sources” and their relative importance remains poorly quantified; a challenge which needs to be addressed for the emission trend to be reversed through regulation. Here we use a chemical transport model (FRSGC/UCI-CTM) to examine the global TFA budget from the production of long-lived source gases, namely, hydrochlorofluorocarbons (HCFCs), hydrofluorocarbons (HFCs), and inhalation anaesthetics. A detailed degradation scheme describing TFA production from each precursor was added to the model and simulations performed using time-varying loadings of its major emitted precursors. Model results showed that TFA production from CFC-replacements increased by a factor of four from 2000 (6.3 Gg/yr) to 2016 (25.4 Gg/yr), with cumulative deposition over this period reaching 226 Gg/yr. HCFC-123, HCFC-124, and HFC-134a account for the majority of this production. TFA deposition shows a latitudinal dependence with the majority occurring in extrapolar regions. Model results are compared to measurements from ice core data and precipitation concentrations. While demonstrating the increasing contribution of CFC replacements to TFA, we highlight the challenges in elucidating their significance against other sources from sparse TFA measurements records, particularly in regions where TFA deposition is highest.

How to cite: Hart, L., Hossaini, R., and Wild, O.: Rising Trifluoroacetic Acid Levels: Evaluating Contributions from long-lived CFC replacements and anaesthetics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17312, https://doi.org/10.5194/egusphere-egu25-17312, 2025.

EGU25-17517 | ECS | PICO | AS3.32

High-resolution modeling of organic aerosol and its components over Europe 

Abhishek Upadhyay, Imad El Haddad, and AURORA project collaborators

Aerosol components have distinct health and climate impacts, hence considering them is essential to reduce uncertainty in estimating the health impacts attributed to aerosol. Organic aerosols (OAs) are one of the significant components of aerosol having a substantial share in total aerosol mass in Europe with significant seasonal and spatial variations. OAs are majorly emitted from fossil fuel combustion and generated through secondary aerosol formation too and based on the origin OA components can be categorized into biomass-burning organic aerosol (BBOA), hydrocarbon-like aerosol (HOA), and oxygenated organic aerosol (OOA).  OA measurements are limited, and measurements of its components are even more sparse due to the need for highly sophisticated instruments and advanced technical expertise. Additionally, OA and its components are not mandated for monitoring at all sites under government regulations, they are measured only at spatially sparse supersites. Chemical transport modeling provides spatially and temporally continuous OA and OA components with some vested uncertainty, but they are generally done at coarser resolution because of computational constraints. Whereas epidemiologist requires data at a finer resolution to link them with the local scale health data. Hence we are modeling total OA and OA components (BBOA, HOA, and OOA) at a fine resolution over Europe. Here, we use an integrated modeling approach combining a chemical transport model and machine learning algorithms. We simulated OA and its components using a comprehensive air quality model with extensions (CAMx) at around 10 km resolution over Europe for 10 years. In the subsequent step, a random forest (RF) model was trained using CAMx outputs, meteorological parameters, and land use variables as predictors to estimate observed aerosol component concentrations as the target to improve the predictions and enable downscaling of the outcome. Here we used an unparallel large OA and OA components observation inventory made with measurements from various research and operational groups across the world, consisting of 50,000 daily observations for OA and 15,000 daily observations for OA components from 140 and 40 locations respectively. This approach improves predictions with an increase in r2 to 0.43 from 0.31 for total OA and reduces the RMSE from  1.5, 0.8, 3.1 µg/m³ to 0.3, 0.2 and 0.45 µg/m³ for BBOA, HOA, and OOA respectively, while also enabling downscaling. This provided us with OA and OA components at a higher resolution of 200m across Europe for 10 years. The high-resolution modeled map illustrates the regional to local spatial distribution of OA and its components. Such high-resolution aerosol component modeling is instrumental for epidemiological studies when combined with local health datasets. Local-scale analysis with such datasets helps identify dominant aerosol components and their sources.

How to cite: Upadhyay, A., El Haddad, I., and collaborators, A. P.: High-resolution modeling of organic aerosol and its components over Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17517, https://doi.org/10.5194/egusphere-egu25-17517, 2025.

EGU25-18197 | ECS | PICO | AS3.32

Looking for ozone recovery in the Arctic 

Caroline Jonas, Robin Björklund, Corinne Vigouroux, Martine De Mazière, Bavo Langerock, Anne Boynard, James W. Hannigan, Nis Jepsen, Rigel Kivi, Norrie Lyall, Johan Mellqvist, Mathias Palm, Viktoria Sofieva, Kimberly Strong, David Tarasick, and Yana Virolainen

Polar regions are strategic in the study of stratospheric long-term ozone trends: since these regions are highly impacted by the effective-chlorine levels, the ozone recovery expected from the reduced emission of ozone depleting substances (Montreal Protocol) should be observed most easily there. However, contrary to the Antarctic, positive ozone trends have not yet been observed in the Arctic (WMO 2022) due to the higher natural variability of ozone in that region. Studying tropospheric ozone trends in the Arctic is also crucial because it can help in reconciling total and stratospheric ozone trends, additionally to the intrinsic interest in ground-level ozone as one of the main greenhouse gases.

The Network for the Detection of Atmospheric Composition Change (NDACC) provides amongst others long-term ozone data from Fourier Transform Infrared (FTIR) spectrometers as well as ozone sonde instruments. We present long-term trends (2000-2022) for total, stratospheric and tropospheric ozone from seven FTIR ground-based stations and from seven ozone sonde stations in the Arctic. The FTIR stratospheric trends are provided in three different layers, covering the lower stratosphere up to 45 km, according to the FTIR vertical resolution.  Based on a previous representativeness study, we also obtain regional trends with reduced uncertainties by combining different instruments and stations. Annual and seasonal trends are calculated using a multiple linear regression technique involving a set of proxies that represent physical processes influencing the natural ozone variability. Using this network of ground-based measurements, we further validate tropospheric and stratospheric ozone trends in the Arctic as derived from satellite observations (MEGRIDOP, SUNLIT, IASI).

How to cite: Jonas, C., Björklund, R., Vigouroux, C., De Mazière, M., Langerock, B., Boynard, A., Hannigan, J. W., Jepsen, N., Kivi, R., Lyall, N., Mellqvist, J., Palm, M., Sofieva, V., Strong, K., Tarasick, D., and Virolainen, Y.: Looking for ozone recovery in the Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18197, https://doi.org/10.5194/egusphere-egu25-18197, 2025.

EGU25-18852 | ECS | PICO | AS3.32

Regional dynamics and trends of N2O and O3 in the lower stratosphere 

Silver Põlgaste, Margit Aun, and Ülo Mander

In the troposphere, N2O is among the most important anthropogenic greenhouse gases, with its long lifetime and a global warming potential in the order of 300 times higher than the same mass of CO2. Furthermore, in the stratosphere, it is the primary ozone(O3)-depleting gas not regulated by the Montréal protocol. As N2O’s anthropogenic emissions grow, its impact on the Earth’s climate also increases. This paper investigates the dynamics of both N2O and O3 in the lower stratosphere using data from the Aura satellite’s MLS (Microwave Limb Sounder) instrument which has been gathering data for both gases since 2004. The study focuses on the lower stratosphere (pressures between 68-22 hPa, corresponding to ~18-26 km at the equator), at 30 selected locations above equatorial and temperate land regions. Both long-term increase and positive correlations between simultaneous N2O and O3 concentrations were examined. The results showed weak increase for O3 and more noticeable ones for N2O, with the latter also including some negative trends, though that is likely related to the MLS instrument’s age. Regarding the relationship between N2O and O3, it was found that the correlation between the gases changes with altitude differently depending on the latitude of the study region. Near the equator, almost no correlation between the gases at 68 hPa level was found but as altitude increases, a negative correlation was observed; it increased up to at least 22 hPa level. At higher latitudes, an inverted version of this phenomenon was observed – negative correlations at lower altitudes first weakened and were afterwards replaced by positive correlations as altitudes increased.

How to cite: Põlgaste, S., Aun, M., and Mander, Ü.: Regional dynamics and trends of N2O and O3 in the lower stratosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18852, https://doi.org/10.5194/egusphere-egu25-18852, 2025.

EGU25-19881 | PICO | AS3.32

A study of the ozone effective temperature temporal and spatial features 

John Christodoulakis, Georgios kouremadas, and konstantinos Goudas

The primary objective of this work is to analyze the temporal and spatial characteristics of the Ozone Effective Temperature (Teff). This study utilized Teff data derived from the Tropospheric Emission Monitoring Internet Service (TEMIS; https://www.temis.nl/climate/efftemp/overpass.php). The dataset includes daily values spanning the period from 1961 to 2023, providing an extensive temporal coverage. To ensure a comprehensive and representative analysis, the study examined data from 358 sites. These sites were carefully selected to achieve uniform coverage across all latitudinal and longitudinal zones.

To explore the spatiotemporal distribution of Teff, detailed spatial analyses were conducted. The results include essential statistical measures for each site, such as the mean Teff values and their standard deviations. Additionally, a thorough spatiotemporal analysis of the time series was performed, highlighting variations and differences across distinct geographical zones. The study also examines trends in Teff over time, providing insights into the evolution of Ozone Effective Temperature across various latitudinal zones.

This multifaceted approach not only reveals significant patterns and trends in Teff but also underscores its variability and differences between regions, contributing to a deeper understanding of its global behavior. The inclusion of statistical and trend analyses further enhances the robustness and relevance of the findings.

How to cite: Christodoulakis, J., kouremadas, G., and Goudas, K.: A study of the ozone effective temperature temporal and spatial features, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19881, https://doi.org/10.5194/egusphere-egu25-19881, 2025.

EGU25-20042 | ECS | PICO | AS3.32

Occurrence and risk of atmospheric pesticides in Northern China 

Mingyu Zhao, Dawei Chen, Junxue Wu, Daniel Figueiredo, Mahrooz Rezaei, Coen Ritsema, Li Li, Qifan Liu, Fanrong Zhao, Jiajun Han, Xuejun Liu, and Kai Wang

The widespread distribution of pesticides in the global atmosphere has been well-documented, posing significant threats to ecosystems and human health, particularly from highly hazardous pesticides (HHPs) characterized by elevated toxicity and/or persistence. Recent studies suggest that certain environmental transformation products of pesticides may be even more hazardous than their precursors. However, related knowledge remains limited currently, hindering our comprehensive assessment and effective response.
Here, we developed a pseudo-targeted analysis strategy designed for rapid-response scenarios, enabling the identification of thousands of pesticide-related compounds in air samples using high-resolution mass spectrometry. Applying this framework to the North China Plain, a key agricultural and densely populated region, we conducted monthly sampling over one year and identified 127 pesticides and transformation products in the local atmosphere. Distinct seasonal variations (monthly fluctuations) and spatial distributions (urbanization gradients) were observed, highlighting agricultural activities as the primary drivers of atmospheric pesticide levels.
Risk assessments for humans and animals were conducted based on environmental concentrations and toxicological data. By comparing concentrations in the organisms with internal effect concentrations, we quantified risk values and found that atmospheric pesticide risks in the North China Plain are unacceptable under some specific situation. Notably, the nonlinear relationship between total concentration and risk values underscores the dominant role of HHPs.
The HYSPLIT model was employed to identify the transport pathways and potential sources of atmospheric pesticides. The results indicate that the North China Plain experiences both external inputs and intercity migration within the region, with Eurasia and the Pacific Ocean potentially serving as sources of atmospheric pesticides.

How to cite: Zhao, M., Chen, D., Wu, J., Figueiredo, D., Rezaei, M., Ritsema, C., Li, L., Liu, Q., Zhao, F., Han, J., Liu, X., and Wang, K.: Occurrence and risk of atmospheric pesticides in Northern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20042, https://doi.org/10.5194/egusphere-egu25-20042, 2025.

EGU25-1166 | Posters on site | AS3.33

Traitement IASI-NG L1C : développement, validation et produits 

Béatrice Petrucci, Julien Nosovan, Sandrine Bijac, Quentin Cebe, Clemence Le Fevre, and François Bermudo

Within the EUMETSAT program EPS-SG, CNES is responsible of purchasing the IASI-NG system, consisting in three instruments on-board of METOP-SG satellites, the L1C products processors, the Mission Performances Expertise Centre and all the simulators needed for these developments.

IASI-NG mission will produce data for the meteorological, atmospheric chemistry and climatology user's community. L1C products are the first level of products that will be distributed to end-users.

IASI-NG space segment transmits the measurements to ground where they are organized in raw L0 products. L0 products are the main input of the L1C processor that calibrates the spectra and images radiometrically and spectrally, and enriches these data with geolocation and additional information for further spectra exploitation.

CNES has developed several L1C processors in order to generate this L1C product:

  • L1CPOP (L1C Product Operation Processor) for the global and regional mission, that will be integrated in EUMETSAT PDAP (Payload Data Acquisition and Processing) Ground Segment to support the routine phase
  • L1CLOP (L1C Local Operation Processor) for the local mission, that will be integrated in SAF (Satellite Application Facilities) ground stations
  • L1CTOP (L1C Temporary Operational Processor) extending the L1CLOP to the global mission, that will be integrated in the EUMETSAT T-GPS (Temporary Ground Processing System) Ground segment to support the commissioning of METOP-SGA-1 satellite.

This presentation:

  • Présentation de la mission IASI-NG et présentation des produits L1C qui seront distribués par EUMETSAT aux utilisateurs finaux
  • présente les traitements et algorithmes de base de L1C et leur processus de vérification basé sur l’utilisation des outils de simulation du CNES et des données IASI-NG réelles issues d’essais d’instruments
  • L’intégration du traitement L1C dans L1CPOP dans l’infrastructure PDAP complexe basée sur une solution Big Data in-memory
  • L’intégration des traitements L1C dans L1CLOP et L1CTOP dans l’infrastructure simplifiée basée sur une solution d’échange de fichiers.

 

How to cite: Petrucci, B., Nosovan, J., Bijac, S., Cebe, Q., Le Fevre, C., and Bermudo, F.: Traitement IASI-NG L1C : développement, validation et produits, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1166, https://doi.org/10.5194/egusphere-egu25-1166, 2025.

EGU25-1595 | ECS | Orals | AS3.33

Influence of the parameterised transport in ICON-ART on the simulated methane concentrations over Europe 

Diego Jiménez de la Cuesta Otero, Beatrice Ellerhoff, Buhalqem Mamtimin, Thomas Rösch, Valentin Bruch, and Andrea Kaiser-Weiss

Targeted climate change mitigation strategies to reduce greenhouse gas emissions benefit from robust and reliable emission quantification. During the first phase of the Integrated Greenhouse Gas Monitoring System for Germany (ITMS), we aim to obtain top-down estimates of German methane emissions with the help of numerical weather prediction models. Accurately representing the effects of convection and turbulent eddies in a numerical weather prediction model is fundamental for simulating the transport of trace gases with emissions located near the surface, as in our case. In the current configuration of our numerical weather prediction model, ICON-ART, convection and turbulence are parameterised. Using a parameterised transport denial approach and obtaining model equivalents for the ICOS European Obspack dataset, we develop a qualitative picture of the parameterised transport errors at each Obspack station. These insights help to identify the potential sources of error in the simulation and thus improve the accuracy of methane emission estimates, which is crucial for concentration data assimilation and top-down observation-based emission estimation, the so-called "inversions".

How to cite: Jiménez de la Cuesta Otero, D., Ellerhoff, B., Mamtimin, B., Rösch, T., Bruch, V., and Kaiser-Weiss, A.: Influence of the parameterised transport in ICON-ART on the simulated methane concentrations over Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1595, https://doi.org/10.5194/egusphere-egu25-1595, 2025.

EGU25-2805 | ECS | Posters on site | AS3.33

Heterogeneous Observation-Based Threshold Velocity Dataset for Wind Erosion and Its Implementation in the iDust Prediction System 

Mei Chong, Xi Chen, Shengkai Wang, Yuan Liang, Shian-Jiann Lin, and Zhi Liang

Wind speed is one of the most sensitive meteorological factors influencing dust storm simulations. The dust emission threshold wind speed (ut) represents the critical point, beyond which dust emission increases notably as wind speed intensifies. However, ut exhibits spatial and temporal variability, lacks direct measurement compared to conventional meteorological parameters, and is challenging to estimate. This study integrates in-situ observations, satellite data, and reanalysis datasets to develop a global dust emission threshold wind speed dataset. Site-specific ut values are determined using in-situ observations by defining and optimizing a dust emission threshold score (DuTS). Based on these site-level ut values, along with satellite dust optical depth (DOD) and wind speed reanalysis data, a global ut distribution dataset is created. This dataset is implemented and validated in a NWP-grade global dust-weather integrated model, iDust. Evaluating iDust against particulate matter (PM)  concentration and DOD observations demonstrates that incorporating this dataset significantly improves the seasonal variation of dust simulations and enhances PM concentration simulations across multiple regions.

How to cite: Chong, M., Chen, X., Wang, S., Liang, Y., Lin, S.-J., and Liang, Z.: Heterogeneous Observation-Based Threshold Velocity Dataset for Wind Erosion and Its Implementation in the iDust Prediction System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2805, https://doi.org/10.5194/egusphere-egu25-2805, 2025.

EGU25-2859 | ECS | Orals | AS3.33

The evaluation of model simulations and analysis of error sources for typical spring dust events in China. 

Yang Zhao, Hong Wang, Wenjie Zhang, Yue Peng, Huiqiong Ning, Chen Han, and Jikang Wang

Dust weather is a type of hazardous weather phenomenon predominantly occurring in arid and semi-arid regions. It arises from the interaction between specific desert ecological environments and meteorological conditions, significantly affecting climate change, ecological systems, human health, and transportation. Over the past decade, the frequency of blowing dust and dust storms in China has exhibited an upward trend, particularly with multiple occurrences of severe dust storms during the spring in the last four years. This study employs the CMA_Meso/CUACE_SDS model to analyze 15 typical dust events that transpired in China from 2021, 2023, and 2024, systematically assessing the model's forecasting performance concerning key characteristics of dust, such as transmission paths, distribution ranges, and durations. Furthermore, based on the different systems that trigger dust weather (Mongolian cyclones and cold fronts or only cold fronts), we selected four representative dust cases with varying process types (blowing dust or dust storms), focusing on analyzing the model's forecast accuracy in relation to weather systems (Mongolian cyclone intensity and cold front intensity) and local meteorological factors (temperature, wind speed, etc.). The results demonstrate that the CMA_Meso/CUACE_SDS model can accurately simulate the transmission paths, distribution ranges, and durations of dust events; however, it tends to overestimate the intensity of both Mongolian cyclones and cold fronts, as well as wind speeds near dust source areas. This overestimation further exacerbates dust emissions from these areas, ultimately diminishing the model's forecasting accuracy for dust events. This study offers valuable insights for enhancing the model's capability to simulate transboundary dust events in the future.

How to cite: Zhao, Y., Wang, H., Zhang, W., Peng, Y., Ning, H., Han, C., and Wang, J.: The evaluation of model simulations and analysis of error sources for typical spring dust events in China., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2859, https://doi.org/10.5194/egusphere-egu25-2859, 2025.

Compared with climate models, the role of aerosol-cloud interaction (ACI) in mesoscale numerical weather prediction (NWP) models still needs to be better understood, especially in haze regions with relatively high aerosol concentration. Here, we perform two sensitivity experiments with and without ACI (ACI and NO-ACI) in the atmospheric chemistry model CMA_Meso/CUACE to investigate the impact of ACI on mesoscale NWP during the low-cloud period in winter 2016 over varying haze regions (severe polluted Jing-Jin-Ji (JJJ), polluted Yangtze River Delta (YRD), and weak polluted Pearl River Delta (PRD)) in China. The study results show that the real-time ACI improves underestimated cloud optical thickness (COT) and cloud water liquid path (CLWP) in haze regions, with the mean bias of simulated COT (CLWP) decreased by 27% (3%), 60% (14%), and 55% (3%) in JJJ, YRD, and PRD, respectively. The increased COT and CLWP lead to a decrease of 6.8, 21, and 13 W m-2 in daytime surface downward shortwave radiation (SDSR) in JJJ, YRD, and PRD, helping to reduce the mean bias of daytime SDSR by 6%, 13%, and 9%. In addition, ACI mitigates the warm bias of temperature at 2 m and dry bias of relative humidity (RH) at 2 m to a certain extent in haze regions, particularly in YRD with the mean absolute bias improved by 13% and 6%. The simulated vertical structure of temperature and RH in the ACI experiment is more consistent with observations than in the NO-ACI experiment. Further investigations find that the ACI effects on mesoscale NWP strongly depend on COT and CLWP magnitude over varying haze regions. Higher COT and CLWP, hence more significant meteorology changes due to ACI, occur in YRD, followed by PRD and JJJ. This study demonstrates the importance and complexity of ACI in modifying mesoscale NWP over varying haze regions of China, which promotes the further understanding of ACI in operational NWP models and bridges the gap with climate models.

How to cite: Zhang, W., Wang, H., Zhang, X., and Peng, Y.: The impact of aerosol-cloud interaction on mesoscale numerical weather prediction in winter over major polluted regions of China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5017, https://doi.org/10.5194/egusphere-egu25-5017, 2025.

EGU25-5670 | ECS | Posters on site | AS3.33

Impacts of chemical and meteorological data assimilation on air-quality and meteorological predictions in the Korean Peninsula 

Yunjae Cho, Hyun Mee Kim, Min-Gyung Seo, and Dae-Hui Kim

In the Korean Peninsula, intricate meteorological conditions influence fine particulate matter (PM) concentrations, making the improvement of both air-quality and meteorological forecasts crucial for better PM predictions. Data assimilation (DA) can help enhancing air-quality forecasts by reducing initial condition uncertainties of air-quality and meteorology. This study investigates the impacts of chemical and meteorological DA on air-quality and meteorological forecasts during a high PM event in the Korean Peninsula. Observational verification showed that the combined application of chemical and meteorological DA yielded the greatest improvements in air-quality and meteorological forecasts. While chemical DA primarily enhanced air-quality predictions, meteorological DA was essential for improving meteorological forecasts. 

The study also assessed the effects of chemical and meteorological DA on air-quality and meteorological forecasts in both DA cycling and non-cycling processes, with respect to the forecasts without DA. Based on the root-mean-square differences between forecasts with and without DA, the impacts of chemical and meteorological DA on air-quality forecasts were found to be similar in cycling and non-cycling processes. In the simultaneous chemical–meteorological DA experiment, the effects of the chemical DA and meteorological DA complemented each other. In the cycling DA process, chemical DA influenced meteorological forecasts, and meteorological DA affected air-quality forecasts due to cumulative DA effects. Chemical DA improved the absolute levels of PM in forecasts, while meteorological DA enhanced the spatiotemporal accuracy of PM distribution by refining transport processes. 

Consequently, simultaneous chemical–meteorological DA proved to be the most effective approach for changing air-quality and meteorological forecasts, and could offer substantial improvements in air-quality and meteorological forecasts in the Korean Peninsula. 

 

Acknowledgements

This study was supported by the National Research Foundation of Korea (2021R1A2C1012572) funded by the South Korean government (Ministry of Science and ICT) and the Yonsei Signature Research Cluster Program of 2024 (2024-22-0162).

How to cite: Cho, Y., Kim, H. M., Seo, M.-G., and Kim, D.-H.: Impacts of chemical and meteorological data assimilation on air-quality and meteorological predictions in the Korean Peninsula, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5670, https://doi.org/10.5194/egusphere-egu25-5670, 2025.

EGU25-6940 | Orals | AS3.33

On the Impact of Satellite Data Assimilation on Mineral Dust Predictions 

Emanuele Emili, Jeronimo Escribano, Eleni Karnezi, Miriam Olid, Calum Meikle, Oriol Jorba, and Carlos Péréz Garcia-Pando

Mineral dust plays a significant role in climate systems, air quality, and human health, making its accurate prediction essential. This study explores the impact of satellite data assimilation (DA) on mineral dust forecasts, with a focus on the first pre-operational DA system at the Barcelona Supercomputing Center (BSC) using VIIRS aerosol optical depth (AOD) observations.

Results from the DA system which employs the MONARCH (Multiscale Online Non-hydrostatic AtmospheRe Chemistry) model for VIIRS AOD assimilation will be presented. MONARCH contributes to the Barcelona Sand and Dust Storm Warning Advisory System (SDS-WAS) and has previously been used to produce a decadal dust reanalysis based on MODIS, showcasing its reliability in modeling and assimilating mineral dust related observations. The new NRT MONARCH DA system produces daily dust analyses and DA initialized forecasts with a 3 days range since October 2024. The presentation will discuss key methodological choices, including ensemble perturbations, with a particular emphasis on meteorological perturbations and their influence on dust assimilation. Evaluation against the operational control simulation, AERONET ground-based observations and other leading dust forecasting systems will provide a comprehensive assessment of forecast accuracy as a function of forecast range and insights about the impact of different DA setups for mineral dust predictions.

Additionally, the impact of offline satellite-estimated dust emissions on forecast quality will be analyzed with MONARCH. These emissions are derived using an ensemble Kalman Smoother applied to multi-year MONARCH simulations and VIIRS observations, providing a robust estimate of dust sources. This work underscores the importance of integrating diverse data sources to enhance dust modeling and prediction capabilities. The findings contribute to the development of more robust operational dust forecasting systems, with implications for climate research, air quality management, and health risk mitigation.

How to cite: Emili, E., Escribano, J., Karnezi, E., Olid, M., Meikle, C., Jorba, O., and Péréz Garcia-Pando, C.: On the Impact of Satellite Data Assimilation on Mineral Dust Predictions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6940, https://doi.org/10.5194/egusphere-egu25-6940, 2025.

EGU25-12348 | Posters on site | AS3.33 | Highlight

Towards the next CAMS reanalysis of atmospheric composition 

Johannes Flemming, Antje Inness, Melanie Ades, Enza Di Tomaso, Flora Kluge, Zoi Paschalidi, Roberto Robas, Christopher Kelly, Samuel Remy, and Vincent Huijnen

Global reanalyses of atmospheric composition (AC) have become a valuable data source to study trends of aerosols, reactive gases, and greenhouse gases. These reanalyses are produced by data assimilation of satellite retrievals of atmospheric composition with atmospheric composition models. The AC reanalysis data are consistent gridded data sets at high temporal resolution (“maps without gaps”) covering decades. Reanalyses are well suited for the study of trends as the users do not have to deal with spatial and temporal gaps in the assimilated observations and their inter-instrument biases. However, the trends and variability of the atmospheric composition fields in AC reanalysis are also influenced by the trends of the model input data such as emissions from anthropogenic sources and wildfires as well as from the meteorological conditions and changes in the availability of the assimilated satellite data.

The Copernicus Atmosphere Monitoring Service (CAMS, atmosphere.copernicus.eu) has produced several AC reanalyses for the period starting in 2003 by assimilating satellite retrievals of atmospheric composition with the ECMWF model. The latest version is the CAMS Reanalysis (EAC4, Inness et al 2019) which is continued in near-real-time with a delay of a few weeks. It has been used for a wide range of applications such as the monitoring of the ozone hole, trends of surface PM2.5 and AOD, tropospheric ozone, and carbon monoxide.

CAMS currently prepares the production of a new AC reanalysis (EAC5). EAC5 has a more advanced modelling approach that also includes stratospheric chemistry and a wider range of secondary aerosols than EAC4. Further, more satellite retrievals in particular from the TropOMI instrument will be assimilated. In this presentation we will give a status update of the preparations for EAC5 and present the efforts on modelling and data assimilation to ensure the production of a consistent data set. Results of scouting analysis and model simulations will be shown to indicate the expected improvements of EAC5 with respect to EAC4.

How to cite: Flemming, J., Inness, A., Ades, M., Di Tomaso, E., Kluge, F., Paschalidi, Z., Robas, R., Kelly, C., Remy, S., and Huijnen, V.: Towards the next CAMS reanalysis of atmospheric composition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12348, https://doi.org/10.5194/egusphere-egu25-12348, 2025.

EGU25-12599 | Orals | AS3.33

A Deep Learning Method for Model-Measurement Fusion of Atmospheric Concentrations with Physical Constraints 

Jia Xing, Bok H Baek, Siwei Li, Chi-Tsan Wang, Ge Song, Siqi Ma, Daniel Tong, and Joshua Fu

Accurate and efficient retrieval of atmospheric chemical concentrations across space and time is crucial for weather prediction and health assessments. However, existing model-measurement fusion methods suffer from limitations due to imbalanced samples from ground measurements or less effective assimilation of satellite data along with numerical modeling. To address these limitations, this study introduces a novel Deep-learning Measurement-Model Fusion method (DeepMMF) constrained by physical and chemical laws inferred from numerical chemical transport models (CTM). This method is applied to NO₂ species over the Continental United States (CONUS) domain for the years 2019 and 2020. By pre-training with abundant CTM simulations, fine-tuning with satellite and ground measurements, and employing a novel optimization strategy for selecting weighting loss and prior emissions, the retrieved spatiotemporally continuous surface NO₂ concentrations present consistent values and daily variations with observations (NMB reduced from -0.3 to -0.1 compared to original CTM simulation). Importantly, the corresponding emissions have been simultaneously adjusted, showing good agreement with changes reported in the national emission inventory (NEI) between 2019 and 2020. Interpretation analysis suggests that the DeepMMF model effectively identifies the importance of satellite data at the regional level and ground measurements at the city level, which is scientifically sound. It exhibits consistent prediction of ground measurements while successfully avoiding the sample imbalance problem that leads to overestimation (up to +100%) of downwind/rural concentrations compared to other existing methods. These results demonstrate the great potential of DeepMMF in data assimilation and retrieval studies for other pollutants and regions, to better support weather forecasting and heatlh studies.

How to cite: Xing, J., Baek, B. H., Li, S., Wang, C.-T., Song, G., Ma, S., Tong, D., and Fu, J.: A Deep Learning Method for Model-Measurement Fusion of Atmospheric Concentrations with Physical Constraints, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12599, https://doi.org/10.5194/egusphere-egu25-12599, 2025.

EGU25-12830 | Posters on site | AS3.33

Enhancing Volcanic Eruption Simulations with the WRF-Chem Model 

Alexander Ukhov and Ibrahim Hoteit

Volcanic eruptions are one of the major natural hazards, exerting profound effects on the environment, economy, and infrastructure. The emissions associated with such eruptions pose substantial risks to terrestrial systems and public health, particularly through the induction of acid rain and air pollution. Additionally, these emissions impact the climate by releasing sulfur dioxide (SO2), which subsequently undergoes conversion into sulfate aerosols due to oxidation by hydroxyl radicals (OH) and hydrogen peroxide (H2O2). Sulfate aerosols, SO2, and volcanic ash influence extensive populations at distances reaching several thousand kilometers from the erupted volcano. In addition, information on ash concentration and the location of the volcanic cloud is crucial for air traffic control. Considering these aspects, accurate modeling of the transport and deposition of volcanic debris is essential. Among the available forecasting tools, the online WRF-Chem Eulerian model is distinguished for its capability to simulate the transport and deposition of volcanic debris.

Here, we enhance the existing and add new functionalities to the WRF-Chem code. In particular, we account for major sinks (wet and dry deposition of ash, sulfate, and chemical transformation of SO2). We identified and rectified a bug in the subroutine for gravitational deposition of the ash. Due to this bug, the ash mass balance was violated. Furthermore, we established a mass balance for sulfate, SO2, and ash by incorporating diagnostic variables into the model's output. Additionally, we corrected the deposition velocity of the coarse (>60 microns in diameter) ash particles and integrated gravitational settling for sulfate aerosols.

Emissions of sulfate along with water vapor, which are other (along with ash and SO2) constituents of a typical volcanic eruption, were also added to the model code. Water vapor is an important greenhouse gas. The recent underwater eruption of the Hunga-Tonga volcano released approximately 150 Mt of water vapor, which affected the dynamics of the debris cloud as a result of the radiative cooling of the water vapor cloud.

The WRF-Chem code has been further enhanced to incorporate the direct radiative effects of ash and sulfate aerosols, acknowledging the substantial radiative forcing exerted by volcanic eruptions on the climate system. In particular, the ash released into the upper atmosphere can inhibit sunlight from reaching the Earth's surface for an extended period, cooling the surface and causing disruptions in ecosystems and agriculture. The stratospheric sulfate aerosol clouds can persist from a few months to a couple of years, reflecting solar radiation into space and causing global cooling.

In addition, we developed an open-source emission preprocessor written in Python. In comparison with the existing PREP-CHEM-SRC utility, our tool facilitates the workflow and adds flexibility in prescribing the volcanic eruption process given the eruption source parameters.

We demonstrate the effect of changes and additions implemented into the WRF-Chem code. The capabilities added to the code allow for significant advancement in volcanic debris forecasting and studies of the effects of volcanic eruptions on climate.

How to cite: Ukhov, A. and Hoteit, I.: Enhancing Volcanic Eruption Simulations with the WRF-Chem Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12830, https://doi.org/10.5194/egusphere-egu25-12830, 2025.

EGU25-12848 | Orals | AS3.33

Towards a representation of fungal spores in IFS-COMPO 

Samuel Remy, Gunnar Felix Lange, Hilde Fagerli, Vincent Huijnen, Jean-Luc Jaffrezzo, Gaëlle Uzu, Thierry Elias, and Johannes Flemming

Fungal spores have been recognized as a significant source of particulate matter as PM10. They also represent a public health and air quality topic, as high concentrations of fungal spores can cause respiratory issues. Within the Copernicus Atmosphere Monitoring Service (CAMS), ECMWF operates the Integrated Forecasting System with atmospheric composition extension (IFS-COMPO) to provide global forecasts and reanalyses of aerosols and trace gases. In the context of the Horizon Europe CAMAERA (CAMS Aerosol Advancement) project, a first attempt has been made to include a simple representation of fungal spores in IFS-COMPO. Several emission schemes from the literature have been tested, using a variety of meteorological and land use variables as precursors. Evaluation is carried out against: 1) a growing database of fungal spores related observations composed of surface concentration of polyols (arabitol and mannitol) over Europe, which are a good proxy for fungal spores, fungal spores counts over the U.S. from the American Academy of Allergy, Asthma and Immunology (AAAI) and fungal spores DNA abundance as collected worldwide by the Global Spore Sampling Project (GSSP); and 2)  against PM10 observations worldwide. In this contribution, we compare the skill of different fungal spores emission schemes and discuss the opportunity of adding fungal spores to the portfolio of CAMS products.

How to cite: Remy, S., Lange, G. F., Fagerli, H., Huijnen, V., Jaffrezzo, J.-L., Uzu, G., Elias, T., and Flemming, J.: Towards a representation of fungal spores in IFS-COMPO, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12848, https://doi.org/10.5194/egusphere-egu25-12848, 2025.

Online-coupled meteorology atmospheric composition models (CCMM) have greatly evolved in recent at least three decades. Although mainly developed by the air quality modeling community, these integrated models are also of interest for numerical weather prediction and climate modeling as they can consider both the effects of meteorology on air quality, and the potentially important effects of atmospheric composition on weather. Migration from offline to online integrated modeling and seamless environmental prediction systems are recommended for consistent treatment of processes and allowance of two-way interactions of physical and chemical components, particularly for AQ and numerical weather prediction (NWP) communities.

Regarding AQF and atmospheric composition modelling, the CCMM approach will certainly improve forecast capabilities as it allows a correct way of jointly and consistently describing meteorological and chemical processes within the same model time steps and grid cells. Applications that may benefit from CCMM are numerous and include: chemical weather forecasting (CWF), numerical weather prediction for precipitation, visibility, thunderstorms, etc., integrated urban meteorology, environment and climate services, sand and dust storm modeling and warning systems, wildfire atmospheric pollution and effects, volcano ash forecasting, warning and effects, high impact weather and disaster risk, effects of short-lived climate forcers, earth system modelling and projections, data assimilation for CWF and NWP, and weather modification and geo-engineering. Online integrated models, however, need harmonized formulations of all processes influencing meteorology and chemistry.

This presentation provides an overview and analysis of integrated meteorology & chemistry model developments during the last 30 year focusing on the main achievements, main trends in developments and applications, as well as the challenges and future research priorities. A special focus will be done on new requirements for further development and applications of CCMM for:

  • Multi-hazard early warning systems,
  • Integrated urban weather, climate and environmental systems,
  • Adaptation and mitigation strategy for climate-smart cities,
  • Earth System Prediction on different scales.

How to cite: Baklanov, A.: Three Decades of Integrated Atmospheric Composition & Meteorology Model Developments: Current Status and New Requirements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13348, https://doi.org/10.5194/egusphere-egu25-13348, 2025.

EGU25-13618 | Posters on site | AS3.33

 Current and Future Advances in NOAA’s Air Quality Predictions from a regional to global perspective 

Barry Baker, Fanglin Yang, Jianping Huang, Patrick Campbell, Youhua Tang, Wei Li, Kai Wang, Raffaele Montuoro, Partha Bhattacharjee, Li Pan, Neil Barton, Cory Martin, Andrew Tangborn, Brian Curtis, Li Zhang, Shobha Kondragunta, and Bing Fu

The U.S. National Oceanic and Atmospheric Administration (NOAA) provides operational air quality (AQ) predictions over the United States and global aerosol forecasts.  The current operational model, the National Air Quality Forecast Capability (NAQFC) at NOAA, has undergone a fundamental paradigm shift through its integration into the Earth system modeling Unified Forecast System (UFS) as a coupled component, the Air Quality Modeling component (AQMv7). AQMv7 embeds the U.S. EPA Community Multiscale Air Quality Model (CMAQ) and it  has been operational at the National Weather Service (NWS) since May 2024. The model was also updated with a larger domain size and new emissions, including the development of the NOAA Emission and eXchange Unified System (NEXUS) along with dynamic processes such as using Model of Emissions of Gases and Aerosols from Nature (MEGAN) v2.1 and the FENGSHA dust scheme, and the Regional Advanced Baseline Imager (ABI)-Visible Infrared Imaging Radiometer Suite (VIIRS) Emissions (RAVE) biomass burning algorithm. 

Operational global aerosol modeling is performed through the NOAA Global Ensemble Forecast System with Aerosols and has been operational in this manner since 2020. Planned future advances include upgrading to a fully coupled atmosphere/land/ocean/sea-ice/wave/aerosols systems developed within the Unified Forecast System (UFS) framework. In its final configuration, the coupled UFS system will consist of: (1)  FV3 dynamical core and CCPP atmospheric physics package using the Noah-MP land model, (2) MOM6 ocean model, (3) CICE6 sea ice model, (4) WAVEWATCH III wave model, and (5) the UFS-Aerosol component, based on NASA’s 2nd generation GOCART aerosol model. GOCART is a simplified chemistry and aerosol component that predicts the major aerosol species including dust, organic and black carbon, sea salt, and sulfate aerosols.  

In this presentation we will discuss NOAA’s current and future AQ and air composition forecasting capabilities and the performance of each system. 



How to cite: Baker, B., Yang, F., Huang, J., Campbell, P., Tang, Y., Li, W., Wang, K., Montuoro, R., Bhattacharjee, P., Pan, L., Barton, N., Martin, C., Tangborn, A., Curtis, B., Zhang, L., Kondragunta, S., and Fu, B.:  Current and Future Advances in NOAA’s Air Quality Predictions from a regional to global perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13618, https://doi.org/10.5194/egusphere-egu25-13618, 2025.

EGU25-16042 | ECS | Orals | AS3.33

Assessing the impacts of assimilating SO2 TROPOMI retrievals with MINNI and DART at the European scale: a case study of the Mount Etna eruption 

Alessandro D'Ausilio, Giorgia De Moliner, Camillo Silibello, Andrea Bolignano, Gino Briganti, Felicita Russo, and Mihaela Mircea

The Mount Etna eruptions are not included in the anthropogenic emission inventories used to simulate air quality in Europe. This study examines the potential of using satellite data assimilation techniques for “adding” the volcanic contribution to atmospheric concentrations. Sulfur dioxide (SO₂) column data from the Sentinel-5p L2 COBRA retrievals (5.5 km x 3.5 km resolution and 2660 km swath) is incorporating through Data Assimilation in 3D SO2 concentrations (0.15° x 0.1°, 14 vertical levels) simulated with MINNI, an atmospheric modelling system member of the CAMS regional air quality ensemble (https://atmosphere.copernicus.eu/charts/packages/cams_air_quality/products/europe-air-quality-forecast-regulated?base_time=202501140000&layer_name=composition_europe_o3_forecast_surface&level=key_0&originating_centre=85_205&projection=opencharts_europe&valid_time=202501140000) which is based on the Chemical Transport Model FARM. The work is part of the CAMs EvOlution (CAMEO, https://ww.cameo.project.eu/) project.

The Data Assimilation framework based on the Ensemble Adjustment Kalman Filter (EnAKF) is for the first time designed and implemented to couple FARM with the Data Assimilation Research Testbed (DART) tool (http://doi.org/10.5065/D6WQ0202). The system runs a 20-member ensemble over an hourly assimilation window. The model perturbations are achieved by varying anthropogenic emissions and boundary conditions to estimate model uncertainties. A specific forward operator based on the Copernicus Satellite Operator (CSO, CAMS / CSO · GitLab) is implemented in DART to obtain the simulation of retrieval products from the model state using averaging kernels. Vertical localization was performed using the 5th-order Gaspari-Cohn (GC) rational function, while prior inflation was applied to minimize filter divergence due to insufficient variance. The Quantile Conserving Ensemble Filter Framework Method was applied to preserve the positivity of the trace gas concentrations. Furthermore, it is assumed that the impact of increments due to SO2 observations only influences the model SO2states.

The DA experiment has been conducted for August 2023. The comparison of the time series, illustrated in Figure 1, shows the vertical column TROPOMI SO2, the prior ensemble mean and the posterior ensemble mean averaged on a subdomain including Sicily, Malta and part of the Mediterranean Sea. Both the prior and the posterior exhibit a negative bias, highlighting the necessity of incorporating volcanic emissions to address this discrepancy. During the period influenced by volcanic activity (08/13 – 08/17), the modelled concentrations after assimilation are enhanced in correspondence of the volcanic plume across the Mediterranean Sea, as depicted in Figure 2.

Figure1. Time series of sulphur dioxide (SO₂) retrieval over a selected region (inset map) during August 2023. black: S5P_PAL_L2_SO2CBR observations, orange:  prior ensemble mean, blue: posterior ensemble mean.

Figure 2. Comparison of S5P (left), prior ensemble mean (centre) and posterior ensemble mean (right) on 2023-08-14 13:00.

How to cite: D'Ausilio, A., De Moliner, G., Silibello, C., Bolignano, A., Briganti, G., Russo, F., and Mircea, M.: Assessing the impacts of assimilating SO2 TROPOMI retrievals with MINNI and DART at the European scale: a case study of the Mount Etna eruption, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16042, https://doi.org/10.5194/egusphere-egu25-16042, 2025.

EGU25-16136 | Posters on site | AS3.33

Integrating Low-cost Sensor Systems and Networks to Enhance Air Quality Forecasting and Reanalysis Applications  

Sara Basart, Carl Malings, Nicolás Huneeus, and Johannes Flemming

Air quality forecasting is essential for protecting public health and the environment. The World Meteorological Organization (WMO) has developed initiatives like the Global Air Quality Forecasting and Information System (GAFIS), the Sand and Dust Storms Warning Advisory and Assessment System (SDS-WAS) and the Vegetation Fire and Smoke Pollution Warning Advisory and Assessment System (VFSP-WAS) to enhance forecasting capabilities.  

In this context, low-cost air quality sensor systems (LCS) are transformative tools in modern air quality management, offering new opportunities to complement traditional monitoring methods. By integrating LCS data with established systems, such as satellite observations and reference-grade instrumentation, the reliability and applicability of air quality data for forecasting can be significantly enhanced. 

A key strength of LCS is their ability to expand the spatial and temporal reach of monitoring networks. However, their use must address inherent limitations in accuracy and precision. Co-locating LCS with reference-grade monitors is essential to quantify uncertainties and ensure data quality. This calibration step enables the deployment of LCS in advanced applications like air quality forecasting. Successfully implementing LCS networks for global, regional, or urban forecasting requires careful planning to ensure adequate spatial coverage, data quality, and timely updates, as well as seamless integration with other systems for actionable insights.  

The World Meteorological Organization (WMO) has been instrumental in coordinating global efforts to optimize LCS deployment. Through guidelines, best practices, and integration frameworks, the WMO supports national and regional initiatives to enhance air quality management. A recent WMO report (WMO, 2024) underscores the importance of incorporating LCS into comprehensive monitoring frameworks for supporting air quality forecasting and reanalysis applications. 

Ongoing advancements in LCS technology and standardization—led by organizations like WMO —are vital to unlocking their full potential. These efforts promise a more equitable and effective approach to air quality management, ensuring that LCS contribute meaningfully to global strategies for monitoring and forecasting. The present contribution will overview the main outcomes of the WMO’s 2024 report on the use of LCS for air quality forecasting and reanalysis applications. 

References:  

WMO, UNEP and IGAC; Integrating Low-cost Sensor Systems and Networks to Enhance Air Quality Applications, 2024, https://library.wmo.int/idurl/4/68924 

How to cite: Basart, S., Malings, C., Huneeus, N., and Flemming, J.: Integrating Low-cost Sensor Systems and Networks to Enhance Air Quality Forecasting and Reanalysis Applications , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16136, https://doi.org/10.5194/egusphere-egu25-16136, 2025.

EGU25-17295 | Posters on site | AS3.33

Implementation of the Aerosol Module HAM-M7 within OpenIFS: Evaluation of Surface Concentrations 

Tommi Bergman, Eemeli Holopainen, Lianghai Wu, Harri Kokkola, Anton Laakso, Hermanni Halonen, Kasper Juurikkala, Philippe Le Sager, Vincent Huijnen, Twan van Noije, Ramiro Checa-Garcia, Adrian Hill, and Marcus Köhler

Aerosols are an important component of the Earth’s atmosphere, where they influence radiative forcing, cloud microphysics, and air quality. Accurate modelling of their spatiotemporal evolution is needed for producing reliable simulations of climate and air quality impacts. Thus far the aerosol description of the ECMWF IFS (Integrated Forecasting System) has relied on a bulk-bin scheme, which provides limited information on the aerosol size distributions. For more accurate calculation of the climate effects and air quality detailed simulations of both mass and number concentrations of aerosols are required. For this work we have utilised OpenIFS-AC, which is a portable and easy-to-use version of the IFS which was recently extended with online chemistry calculation. In the OpenIFS model we replaced the bulk-bin description with the HAM-M7 (Hamburg Aerosol Model M7) modal aerosol scheme. The HAM-M7 module describes aerosol processes such as emissions, transport, deposition, and microphysical interactions across seven log-normal modes, including both mass and number concentrations as size-resolved properties for key aerosol species, including sulfate, black carbon, organic matter, sea salt, and dust. Furthermore, the current implementation within OpenIFS Cy48r1 includes aerosol interactions with radiation and cloud microphysics.

We used the model to simulate the global evolution of the different aerosol components and evaluate the performance against observational data. The model is run for one year for 2010 with CMIP6 emissions and 2024 with CAMS emissions with one year of spinup. The simulated aerosol fields are compared with observed number and mass concentrations of aerosols for the observational sites in the ACTRIS network, Furthermore, the simulated surface concentrations are compared with those provided by the aerosol models within the AeroCom project. Moreover, as the modal aerosol module is computationally more expensive than the bulk-bin module we will discuss the computational cost of running the new aerosol module.

This work was supported by the European Union’s Horizon Europe projects CAMAERA - CAMS AERosol Advancement (number 101134927) and FOCI, Non-CO2 Forcers and Their Climate, Weather, Air Quality and Health Impacts (number 101056783).

How to cite: Bergman, T., Holopainen, E., Wu, L., Kokkola, H., Laakso, A., Halonen, H., Juurikkala, K., Le Sager, P., Huijnen, V., van Noije, T., Checa-Garcia, R., Hill, A., and Köhler, M.: Implementation of the Aerosol Module HAM-M7 within OpenIFS: Evaluation of Surface Concentrations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17295, https://doi.org/10.5194/egusphere-egu25-17295, 2025.

EGU25-17696 | Posters on site | AS3.33

Harnessing machine learning and deep learning methods to forecast whitecap fraction and sea-salt aerosol emissions in the ECMWF Integrated Forecast System (IFS-COMPO) 

Nathan Capon, Rose-Cloé Meyer, Samuel Remy, Magdalena Anguelova, Jean Bidlot, Josh Kousal, Thierry Elias, and Antonino Bonanni

Within the Copernicus Atmosphere Monitoring Service (CAMS), ECMWF operates the Integrated Forecasting System with atmospheric composition extension (IFS-COMPO) to provide global forecasts and reanalysis of aerosols and trace gases. Emissions of sea-salt aerosols in IFS-COMPO are estimated by first computing the whitecap fraction, using a polynomial fit between a dataset of retrieved whitecap fraction from remote sensing and wind speed and sea-surface temperature (SST), and applying a shape function on the whitecap fraction to derive sea-salt aerosol emissions.

In the context of the Horizon Europe CAMAERA (CAMS AERosol Advancement) project, we apply a range of deep learning and machine learning algorithms to estimate whitecap fraction offline, using a two-year long dataset of whitecap fraction derived from remote sensing observations. Meteorological and oceanic predictors are used, including wind speed and direction, sea-surface temperature, significant wave height from wind- and total-sea, as well as the turbulent energy of breaking waves. The latter two parameters are provided by the wave model (WAM) that is included in IFS-COMPO. For some of the deep-learning and machine learning methods, the correlation and error of the estimated whitecap fraction are much improved as compared to the usual physical models used in the atmospheric composition and remote sensing communities. 

This work can be seen as a benchmark of machine learning/deep learning methods for the simulation of atmospheric composition processes. This expertise will be used for other processes such as desert dust emissions, in the CAMAERA project.

How to cite: Capon, N., Meyer, R.-C., Remy, S., Anguelova, M., Bidlot, J., Kousal, J., Elias, T., and Bonanni, A.: Harnessing machine learning and deep learning methods to forecast whitecap fraction and sea-salt aerosol emissions in the ECMWF Integrated Forecast System (IFS-COMPO), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17696, https://doi.org/10.5194/egusphere-egu25-17696, 2025.

EGU25-18231 | Orals | AS3.33

Modelling stratospheric composition for the Copernicus Atmosphere Monitoring Service Cy49R1: polar ozone depletion and sulfate aerosols 

Simon Chabrillat, Samuel Rémy, Vincent Huijnen, Christine Bingen, Jonas Debosscher, Quentin Errera, Swen Metzger, Daniele Minganti, Marc Opdebeek, Jason Williams, Henk Eskes, and Johannes Flemming

The daily analyses and forecasts of atmospheric composition delivered by the Copernicus Atmosphere Monitoring Service (CAMS) are produced by the  ECMWF Integrated Forecasting System configured for COMPOsition (IFS-COMPO). On 27 June 2023, this system was upgraded to Cy48R1 which solves explicitly for stratospheric chemistry through a module extracted from the  Belgian Assimilation System for Chemical ObsErvations (BASCOE). On 12 November 2024, the system was further upgraded to Cy49R1 which improves the representation of stratospheric composition with an adjusted parameterization of Polar Stratospheric Clouds (PSC), updated chemical rates for heterogeneous chemistry, and the implementation of missing processes to model the distribution of sulfate aerosols in the stratosphere.

We report on these improvements and evaluate the resulting stratospheric composition in forecast mode, i.e. with no assimilation of composition observations. These evaluations focus on aerosol extinction in the global stratosphere and on ozone depletion processes in the polar lower stratosphere. For ozone depletion events we compare forecasts of ozone, water vapor, N2O, HNO3, HCl and ClO with a reanalysis of observations by the Aura Microwave Limb Sounder (MLS) for three Antarctic events (2008, 2009, 2020) and four Arctic events (ending in 2009, 2011, 2012 and 2020). We show that the model configuration currently used by CAMS (IFS-COMPO Cy49R1) simulates successfully these processes and events. This enables the assimilation of multiple satellite observations of stratospheric composition in an operational Data Assimilation System developed primarily for Numerical Weather Forecasting and provides a useful tool for further studies of the couplings between stratospheric aerosols and gas-phase chemistry.

How to cite: Chabrillat, S., Rémy, S., Huijnen, V., Bingen, C., Debosscher, J., Errera, Q., Metzger, S., Minganti, D., Opdebeek, M., Williams, J., Eskes, H., and Flemming, J.: Modelling stratospheric composition for the Copernicus Atmosphere Monitoring Service Cy49R1: polar ozone depletion and sulfate aerosols, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18231, https://doi.org/10.5194/egusphere-egu25-18231, 2025.

EGU25-19585 | Orals | AS3.33

Harmonization of the aerosol models in remote sensing and global transport models for data assimilation from new generation of polarimetric measurements 

Pavel Litvinov, Oleg Dubovik, Abhinna Behera, Milagros Herrera, Soheila Jafariserajehlou, Bertrand Fougnie, Julien Chimot, Samuel Remy, and Johannes Flemming

New generation of the multi-angular polarimeters (3MI, PACE/SPEX and HARP2) will essentially improve the aerosol characterization from remote sensing measurements, providing extended set of the advanced optical and microphysical properties. This will open new possibility for aerosol composition assimilation.

Significant differences exist at present time between aerosol modelling methodologies employed in various remote sensing algorithms and global climate models. This complicates the aerosol data assimilations in reanalysis.  This gap also impacts remote sensing approaches, as global climate models provide global information about aerosol masses emissions, accounting for atmospheric states, aerosol sources, and sinks. Consequently, the aerosol information predicted or derived climatologically from global climate models, such as aerosol type and vertical profile, serves as valuable a priori information to constrain remote sensing measurements.

Directly applying the CAMS aerosol modelling approach to remote sensing introduces complexities in the forward model and significantly increases the number of retrieved parameters. However, achieving harmonization between aerosol approaches in global climate modelling and remote sensing holds the potential to enhance the accuracy of aerosol retrieval, as well provide new possibility for aerosol parameters assimilations.

Here we discuss feasibility studies on harmonization of aerosol model approaches in remote sensing and transport models. Different retrieval approaches harmonized with CAMS aerosol model representation are tested on synthetic and real PARASOL measurements as a proxy for future 3MI instrument. The retrieved optical properties are compared with CAMD reanalysis data collocated to PARASOL measurements and will be discussed.

How to cite: Litvinov, P., Dubovik, O., Behera, A., Herrera, M., Jafariserajehlou, S., Fougnie, B., Chimot, J., Remy, S., and Flemming, J.: Harmonization of the aerosol models in remote sensing and global transport models for data assimilation from new generation of polarimetric measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19585, https://doi.org/10.5194/egusphere-egu25-19585, 2025.

EGU25-20379 | Posters on site | AS3.33

Initial steps towards an inversion system for biogenic isoprene emissions in CAMS: Evaluation of IFS-COMPO formaldehyde simulations 

Flora Kluge, Johannes Flemming, Vincent Huijnen, Antje Inness, Christopher Kelly, Jean-Francois Müller, Glenn-Michael Oomen, Klaus Pfeilsticker, Roberto Ribas, Trissevgeni Stavrakou, Ben Weyland, and Miró van der Worp

We report on the analysis of formaldehyde (HCHO) simulations performed by the CAMS (Copernicus Atmosphere Monitoring Service) atmospheric composition forecasting system (IFS-COMPO) in different tropospheric regions, seasons, altitudes and air masses using a comprehensive data set of airborne measured HCHO vertical column densities and mixing ratios. The observations are derived from measurements of the HALO mini-DOAS instrument operated from aboard the German research aircraft DLR HALO during six international research missions in the years 2017 to 2019 and TROPOMI S5P satellite observations. In addition, measurements over the South American tropical rain forest in 2014 are included, as this region is of particular interest in the analysis of global biogenic emissions. In particular, the presented analysis evaluates HCHO in biogenic air masses and the impact of recent advances of biogenic emission estimation in IFS-COMPO on simulated biogenic VOCs. For this purpose, we evaluate operational IFS-COMPO HCHO simulations, which apply a climatology of monthly averaged biogenic emissions (Cams-Glob-BioV3.1), and HCHO simulations based on a recently developed online biogenic emission estimation module.

The above findings are part of the ongoing research carried out in the Horizon Europe CAMEO (CAMS EvOlution) project, which aims to develop an inversion of biogenic emissions within ECMWF’s Integrated Forecasting System. As a first step towards a successful implementation of HCHO assimilation and inversion capability within the IFS, a tangent linear and adjoint have been derived based on a simplified, linearized HCHO chemistry scheme. The impact of the assimilation of HCHO in IFS-COMPO is currently analyzed using TROPOMI S5P formaldehyde observations, with a particular focus on its impact on other atmospheric reactive trace gases, such as isoprene and ozone, and on aerosols.

How to cite: Kluge, F., Flemming, J., Huijnen, V., Inness, A., Kelly, C., Müller, J.-F., Oomen, G.-M., Pfeilsticker, K., Ribas, R., Stavrakou, T., Weyland, B., and van der Worp, M.: Initial steps towards an inversion system for biogenic isoprene emissions in CAMS: Evaluation of IFS-COMPO formaldehyde simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20379, https://doi.org/10.5194/egusphere-egu25-20379, 2025.

EGU25-21242 | Orals | AS3.33

An interoperable fire behavior model for coupling with atmospheric models: The Community Fire Behavior model 

Pedro Jimenez, Maria Frediani, Masih Eghdami, Daniel Rosen, Michael Kavulich, and Katherine Katherine

This presentation will provide an overview of the Community Fire Behavior model (CFBM, Jimenez y Munoz et al, 2024). Fire behavior models allow for an explicit representation of the fire progression accounting for feedback between the atmosphere and fires. The CFBM has been designed to facilitate coupling with different atmospheric models. To this end, we rely on modern software engineering standards and the Earth System Modeling Framework (ESMF) libraries (https://github.com/NCAR/fire_behavior). In its current version (v0.2.0), CFBM closely follows the methods of the Weather Research and Forecasting (WRF) model with fire extensions (WRF-Fire). This allowed us to ensure the adequacy of our implementations. The CFBM has been implemented in the National Oceanic and Atmospheric Administration (NOAA) Unified Forecast System (UFS) and we are in the process of coupling the model to WRF. The results from idealized fire simulations, and the consistency shown between UFS-CFBM and WRF-Fire, as well as WRF-CFBM and WRF-Fire, were the starting point for our ongoing extensions. This includes accounting for the impact of the fuel moisture content on smoke emissions from wildland fires. Our strategy to enhance the evolution of fire emissions for air quality systems will be also outlined. The results obtained so far and the interoperability of the model, that allows for coupling to other atmospheric models, should facilitate its adoption; which would foster collaborative developments to improve fundamental understanding of fire-atmosphere processes including wildland fire impacts on atmospheric composition.

 

Jimenez y Munoz, P.A., M. Frediani, M. Eghdami, D. Rosen, M. Kavulich, and T.W. Juliano, 2024: The Community Fire Behavior model for coupled fire-atmosphere modeling: Implementation in the Unified Forecast System. Geosci. Model Dev. Discuss. Preprint.

How to cite: Jimenez, P., Frediani, M., Eghdami, M., Rosen, D., Kavulich, M., and Katherine, K.: An interoperable fire behavior model for coupling with atmospheric models: The Community Fire Behavior model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21242, https://doi.org/10.5194/egusphere-egu25-21242, 2025.

EGU25-21823 | Orals | AS3.33

The progression and global dispersion of the Hunga aerosol cloud, and influence from co-emitted water vapour, aligned to the APARC Hunga impacts report 

Graham Mann, Yunqian Zhu, Bill Randel, Margot Clyne, Sandip Dhomse, Ghassan Taha, Mathieu Colombier, and Paul Newman

The January 2022 Hunga eruption generated the strongest stratospheric aerosol optical depth for 30 years (e.g. Khaykin et al., 2022; Taha et al., 2022; Bourassa et al., 2023), but the eruption emitted only a modest 0.4-0.5Tg of SO2 to the stratosphere (Carn et al., 2022).

The most explosive eruption in the satellite era (Wright et al., 2022), an upper portion of the Hunga plume was initially at ~35-40km altitude (Taha et al., 2022), but the main detrainment occurred lower at ~27-30km, with a highly unusual initial steep descent of the plume seeing the layer of Hunga-enhanced aerosol form at ~22-26km (e.g. Kloss et al., 2022; Legras et al., 2022; Baron et al., 2023).

The shallow underwater explosion also detrained ~150Tg of water vapour deep into the stratosphere (e.g. Millan et al., 2022), shown by Zhu et al. (2022) and Asher et al. (2023) to have accelerated SO2 oxidation and enhanced the growth of volcanic sulphate aerosol to optically-active sizes. The total water vapour present within the Hunga plume was greater, with also an estimated 23 Tg of SO2 present (Colombier et al., 2023), the vast majority of emitted sulphur removed via ice sedimentation in the initial days.

The potential for such an explosive eruption to influence climate and the ozone layer, and the effects from the strong enhancement to stratospheric water vapour, motivated APARC to begin a special “Hunga impacts” cross-activity project. The activity’s main role is to co-ordinate community activity to write a special “Hunga impacts report”, and author teams were convened in early 2024, each chapter 1st draft peer-reviewed in autumn 2024, ahead of publication in summer 2025.

This presentation will focus on the Hunga aerosol, and the initial months after the eruption, aligned to the 2025 report. We will present findings from the interactive stratospheric aerosol HTHH-MOC experiment 3, a co-ordinate multi-model analysis of the Hunga aerosol progression, the protocols to identify how the model predictions of the co-emitted water vapour effects vary.

The Hunga aerosol progression has commonalities with the 1883 Krakatau eruption, both eruptions injecting very large amounts of vaporised seawater deep into the stratosphere. Krakatau is estimated to have emitted 500Tg water vapour (Joshi and Jones, 2009), i.e. 4 times greater than Hunga. Krakatau’s highest plume-altitude explosions are thought to have occurred after caldera collapse, from pyroclastic density currents entering the sea (see Self and Rampino, 1981; Self 1992),

Purple twilight duration observations in the Royal Society Krakatoa committee report  (Russell & Archibald, 1888) show the Krakatau cloud descended between August 1883 and January 1884 (see Nature Feb 1888 summary of the report). The observations presented in Pernter (1889) indicate an initial descent from 32km to 24km in the first few weeks.  a similar altitude for the subsequent 2-3 months (September to November 1883), then a descent resuming to 19km in December 1883 and 17km in January 1884.

How to cite: Mann, G., Zhu, Y., Randel, B., Clyne, M., Dhomse, S., Taha, G., Colombier, M., and Newman, P.: The progression and global dispersion of the Hunga aerosol cloud, and influence from co-emitted water vapour, aligned to the APARC Hunga impacts report, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21823, https://doi.org/10.5194/egusphere-egu25-21823, 2025.

EGU25-452 | ECS | Orals | AS3.34 | Highlight

Improving nitrous oxide (N₂O) emissions accounting in Kenya: Insights and measurement results relating to fertilizer practices, environmental drivers, and N isotopic composition  

Turry Ouma, Phillip Agredazywczuk, Matti Barthel, Abigael Otinga, Ruth Njoroge, Sonja Leitner, Yuhao Zhu, Collins Oduor, Kevin Churchil Oluoch, Guillaume Obozinski, Johan Six, and Eliza Harris

The use of mineral fertilizers in Sub-Saharan Africa (SSA) is crucial for enhancing agricultural productivity but also raises concerns about emissions of nitrous oxide (N₂O), a potent greenhouse gas. Despite their importance for agriculture, N₂O emissions remain poorly understood in SSA, limiting the development of accurate emissions inventories and the adoption of climate-smart agricultural practices.

In the N2O-SSA project, we quantified N₂O emissions from maize and potato cropping systems under nitrogen application rates of 50 kg N/ha and 100 kg N/ha, compared to control plots, using automated static chamber methods. Fertilizer treatments included urea and triple superphosphate (TSP), and control plots received no nitrogen. Preliminary results showed significant temporal and treatment-specific variability in N₂O emissions, with peaks following fertilizer applications and rainfall events, highlighting the interaction between nitrogen availability and soil moisture. Cumulative annual N₂O emissions were found to vary widely depending on nitrogen application rates and crop types, with fertilizer treatments driving the majority of emissions. Emission factors (EFs) were within ranges consistent with previous studies, highlighting differences between crops such as maize and potatoes. Control plots consistently showed negligible emissions, underlining the critical role of nitrogen inputs in driving N₂O fluxes.

These findings underline the importance of crop-specific nitrogen dynamics in shaping N₂O emissions, and the need for tailored nitrogen management strategies to balance agricultural productivity with environmental sustainability. In the next phase of the project, we will analyze soil samples for N₂O isotopic composition, measuring δ¹⁵N-NH₄ and δ¹⁵N-NO₃, in addition to analyzing gas samples to provide further insights into the sources of N₂O emissions. This will inform more efficient nitrogen management practices for sustainable agricultural systems in Sub-Saharan Africa.

How to cite: Ouma, T., Agredazywczuk, P., Barthel, M., Otinga, A., Njoroge, R., Leitner, S., Zhu, Y., Oduor, C., Oluoch, K. C., Obozinski, G., Six, J., and Harris, E.: Improving nitrous oxide (N₂O) emissions accounting in Kenya: Insights and measurement results relating to fertilizer practices, environmental drivers, and N isotopic composition , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-452, https://doi.org/10.5194/egusphere-egu25-452, 2025.

EGU25-1203 | Posters on site | AS3.34

Top-down estimation of ammonia emissions from pig farm area using Backward Lagrangian Stochastic model 

Yeonhoo Kim, Joonhyeok Choi, Jinsik Kim, Hyungdo Song, Chul Yoo, and Mijung Song

Ammonia (NH3) emitted into the atmosphere contributes to increase in fine particulate matter concentrations through secondary formation and affects human comfort through unpleasant odors. Pig farms are a significant source of ammonia, but the actual emissions are highly variable depending on facility types, meteorological conditions, and operational practices, causing high uncertainty in estimating emissions. In this study, hourly atmospheric ammonia concentrations were measured in Yongji, Gimje, South Korea, a region well known for its large-scale old pig farming, over all four seasons from September 2023 to July 2024. Using the data, seasonal ammonia emissions from pig farms were simulated with the WindTrax Backward Lagrangian Stochastic model. Our findings will be presented. This can provide a foundation for validating bottom-up estimates of ammonia emissions and valuable insights on reducing uncertainties associated with ammonia emissions from pig farms.

How to cite: Kim, Y., Choi, J., Kim, J., Song, H., Yoo, C., and Song, M.: Top-down estimation of ammonia emissions from pig farm area using Backward Lagrangian Stochastic model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1203, https://doi.org/10.5194/egusphere-egu25-1203, 2025.

EGU25-1240 | ECS | Posters on site | AS3.34

Seasonality and health risk assessment of anthropogenic volatile organic compounds (VOCs) in a rural Seosan, South Korea 

Avinash Shastri, Jayant Nirmalkar, Seunggi Kim, Sangmin Oh, Kwangyul Lee, and Mijung Song

Atmospheric volatile organic compounds (VOCs) were measured in this study during four seasons (winter, summer, spring, and autumn) between 2020 to 2022, using gas chromatography equipped with a photoionization detector (PID), at Seosan, South Korea. The mean concentration of ∑34VOCs was 21.2 ± 26.6 µg/m3, with the highest levels measured in autumn (33.6 ± 40.4 µg/m3). The toluene/benzene ratio indicated industrial activities dominated in winter and spring, while solvent use and agriculture were key in autumn, with biomass burning common in both seasons. The secondary organic aerosol formation potential (SOAFP) was highest during autumn and summer, significantly contributing to PM2.5 levels. The Monte Carlo simulation revealed benzene concentrations frequently exceeded the permissible carcinogenic risk threshold (1 × 10-6), suggesting potential health hazards. Meanwhile, the non-carcinogenic risks of seven selected VOCs remained within acceptable limits (hazard quotient [HQ] < 1). The outcomes of the study emphasized the importance of understanding VOC characteristics, sources, and implications for public health.

How to cite: Shastri, A., Nirmalkar, J., Kim, S., Oh, S., Lee, K., and Song, M.: Seasonality and health risk assessment of anthropogenic volatile organic compounds (VOCs) in a rural Seosan, South Korea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1240, https://doi.org/10.5194/egusphere-egu25-1240, 2025.

EGU25-2618 | ECS | Orals | AS3.34

Global ammonia emission could be halved with cost-effective measures 

Xiuming Zhang, Baojing Gu, Wilfried Winiwarter, Hans van Grinsven, Mark Sutton, and Shaohui Zhang

Excess ammonia (NH3) emissions from human activities pose critical risks to global ecosystems and human health. Despite the urgent need for NH3 emission controls, a comprehensive evaluation of the cost-effectiveness of mitigation strategies remains underdeveloped. In this study, we adopt a multi-model framework to assess the cost and impact of 32 mitigation measures across seven key sectors in 185 countries. Our results indicate that targeted implementation of these measures, particularly in the agricultural sector, could reduce global NH3 emissions by 49% (36–57%). The estimated implementation cost of $279±69 billion outweighs the projected environmental, health, and resource benefits of $568±182 billion. China and India emerge as critical regions for prioritizing NH3 mitigation, offering the highest societal returns, while Sub-Saharan Africa shows limited economic viability. Future scenario analysis reveals that sustainable policy pathways could reduce NH3 emissions by 55% by 2050. Conversely, weak climate action and inadequate nitrogen regulations may result in a 19% increase in emissions, exacerbating environmental degradation and hindering progress toward sustainable development goals. Our findings underscore the urgent need for coordinated global efforts and region-specific policies to establish and achieve effective NH3 mitigation targets.

How to cite: Zhang, X., Gu, B., Winiwarter, W., van Grinsven, H., Sutton, M., and Zhang, S.: Global ammonia emission could be halved with cost-effective measures, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2618, https://doi.org/10.5194/egusphere-egu25-2618, 2025.

EGU25-3228 | ECS | Posters on site | AS3.34

The effect of post-harvest cover crop management on N2O emissions 

Harika Bommisetty, Lars Elsgaard, and Lars Juhl Munkholm

Agricultural soils are the primary source of nitrous oxide (N2O) emissions into the atmosphere, contributing 78% of total N2O emissions. These emissions are influenced by different tillage practices and types of plant cover that are left after harvest. Cover crops (CC) are widely used in agriculture to take up excess nitrogen from the fields, thereby reducing nitrate leaching and increasing soil carbon accrual. However, despite these benefits, agricultural soils containing cover crops have often resulted in high N2O emissions.

A two-year field study with measurement of N2O emissions was conducted in Denmark using a long-term conservation agriculture experiment, including cover cropping, no tillage and crop rotation. The study focused on the influence of soil tillage and cover cropping on soil physical properties and N2O emissions. The tillage systems included no tillage (direct seeding) and conventional ploughing; CC management included paired subplots with oil-seed radish (Raphanus sativus L.), where (i) the cover crop residues were terminated and removed in autumn (CC-rem), and (ii) the cover crop residues were killed by the frost and left in the field (CC-left). Bare soil treatment (i.e., without CC) is included as a reference. Spring oats (Avena sativa L.) grew as the main crop during the first year followed by spring barley (Hordeum vulgare L.) in the second year.

The first-year results for N2O fluxes showed that there were no significant differences in N2O emissions between the tillage practices. However, emissions varied significantly among CC treatments. Compared to the reference without CC, peak emissions (up to 74 µg N2O-N m-2 h-1) were observed for both cover crop treatments. During the cropping season, most of the emissions occurred after fertilization. Especially, +CC-left emitted more N2O than CC-rem during the main cropping season. Before establishing the main crop, CC-rem emitted more N2O than CC-left. Volume-effective porosity, air permeability, bulk density and gas diffusivity are critical soil physical properties that influenced N2O emissions among the cover crop treatments.

How to cite: Bommisetty, H., Elsgaard, L., and Juhl Munkholm, L.: The effect of post-harvest cover crop management on N2O emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3228, https://doi.org/10.5194/egusphere-egu25-3228, 2025.

EGU25-4260 | ECS | Posters on site | AS3.34

Decadal analysis of ammonia emission levels in the lowlands of eastern Germany using remote sensing data 

Christian Saravia and Katja Trachte

Ammonia (NH3) emissions play a significant role in air quality degradation, biodiversity loss, and human health risks by forming secondary pollutants such as fine particulate matter (PM2.5). This study presents a decadal (2013–2022) spatiotemporal analysis of NH3 emissions in the lowlands of eastern Germany, using data from the Infrared Atmospheric Sounding Interferometer (IASI-B) onboard the MetOp-B satellite. The region, characterized by predominantly agricultural land use (54.71%), offers a valuable case for understanding NH3 emission dynamics across diverse landscapes. Integrating satellite remote sensing, machine learning, and atmospheric modeling, this analysis reveals pronounced seasonal and spatial variations, with agricultural activities identified as the primary source of emissions. K-means clustering highlights the influence of cropland, grassland, and urban areas on NH3 emission patterns, identifying significant agricultural hotspots. Additionally, advanced geospatial analysis establishes significant correlations between NH3 concentrations and meteorological variables. NH3 emissions were positively associated with surface solar radiation, temperature, atmospheric boundary layer height, and convective available potential energy, while precipitation, moisture flux, and wind speed exhibited negative correlations. Backward trajectory dispersion modeling employing the HYSPLIT model provided insights into NH3 transport pathways. The results confirmed the influence of both, local sources and non-local contributions. These findings show the major role of meteorological conditions in NH3 dispersion and underscore the importance of sustainable agricultural practices in mitigating emissions.

How to cite: Saravia, C. and Trachte, K.: Decadal analysis of ammonia emission levels in the lowlands of eastern Germany using remote sensing data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4260, https://doi.org/10.5194/egusphere-egu25-4260, 2025.

Crop production is a major source of agricultural carbon emissions, yet the life cycle carbon footprints (LCCFs) of key global staple crops remain underexplored. This study quantifies the LCCFs of three major grain crops—maize, rice, and wheat—using a hybrid approach that integrates machine learning (ML) models and life cycle assessment (LCA) for the period from 2006 to 2019. We systematically calculated the cradle-to-farm-gate carbon footprint (CF), accounting for emissions from upstream inputs, transportation, and field operations. Emission factors (EFs) and CF compositions were assessed over different time periods. Additionally, we developed a novel Supply-Demand Balanced Carbon Allocation Model (SD-CAM) to trace the sources and flows of upstream CF. Our results reveal a steady increase in the CF of these crops over time, with significant regional variations in both EFs and CF composition. The primary carbon footprint of global rice production is mainly attributed to field carbon emissions, with nitrogen fertilizers as the secondary carbon source. In contrast, nitrogen fertilizers are the dominant carbon source for maize and wheat. Interestingly, while maize's total field emissions are a net carbon source, wheat production acts as a carbon sink. The majority of the CF is concentrated in a few key grain-producing countries, such as China, India, and the United States. Regarding the upstream carbon footprint (IUCCF), major producing countries like China and Canada have consistently been the primary sources of upstream carbon inputs throughout the study period. However, with the rise of global economic initiatives like the Belt and Road, emerging upstream contributors such as Morocco and Vietnam have increasingly become significant contributors in upstream carbon emissions. This study provides valuable insights into the environmental impacts of agricultural production over time, offering guidance for sustainable agricultural policies, carbon responsibility allocation, and international low-carbon cooperation.

How to cite: Liu, S., He, Y., Liu, Y., and Jiang, Q.: Tracing the life cycle carbon footprint of global staple crops: an integrated approach combining machine learning and life cycle assessment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4965, https://doi.org/10.5194/egusphere-egu25-4965, 2025.

EGU25-6101 | Orals | AS3.34

Ammonia emission estimates using CrIS satellite observations over Europe 

Jieying Ding, Ronald van der A, Henk Eskes, Enrico Dammers, Mark Shephard, Roy Wichink Kruit, Marc Guevara, and Leonor Tarrason

Over the past century, ammonia (NH3) emissions have increased with the growth of livestock and fertilizer usage. The abundant NH3 emissions lead to secondary fine particulate matter (PM2.5) pollution, climate change, and a reduction in biodiversity, and they affect human health. Up-to-date and spatially and temporally resolved information on NH3 emissions is essential to better quantify their impact. In this study we applied the existing Daily Emissions Constrained by Satellite Observations (DECSO) algorithm to NH3 observations from the Cross-track Infrared Sounder (CrIS) to estimate NH3 emissions. Because NH3 in the atmosphere is influenced by nitrogen oxides (NOx), we implemented DECSO to estimate NOx and NH3 emissions simultaneously. The emissions are derived over Europe for 2020 on a spatial resolution of 0.2°×0.2° using daily observations from both CrIS and the TROPOspheric Monitoring Instrument (TROPOMI; on the Sentinel-5 Precursor (S5P) satellite). Due to the limited number of daily satellite observations of NH3, monthly emissions of NH3 are reported. The total NH3 emissions derived from observations are about 8 Tg yr−1, with a precision of about 5 %–17 % per grid cell per year over the European domain (35–55° N, 10° W–30° E). The comparison of the satellite-derived NH3 emissions from DECSO with independent bottom-up inventories and in situ observations indicates a consistency in terms of magnitude on the country totals, with the results also being comparable regarding the temporal and spatial distributions. The validation of DECSO over Europe implies that we can use DECSO to quickly derive fairly accurate monthly emissions of NH3 over regions with limited local information on NH3 emissions

How to cite: Ding, J., van der A, R., Eskes, H., Dammers, E., Shephard, M., Wichink Kruit, R., Guevara, M., and Tarrason, L.: Ammonia emission estimates using CrIS satellite observations over Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6101, https://doi.org/10.5194/egusphere-egu25-6101, 2025.

EGU25-8327 | Posters on site | AS3.34

Predicting Enteric Methane Emissions in Dairy Cows Using Deep Learning Models 

Amir Sahraei, Deise Knob, Christian Lambertz, Andreas Gattinger, and Lutz Breuer

This study evaluates the potential of deep learning (DL) models to predict enteric methane (CH₄) emissions in dairy cows using data from automated milking and feeding systems, behavioral sensors, and public weather databases. Methane emissions were recorded for 52 cows from October 2022 to December 2023 using the sniffer technology at Gladbacherhof, an organic research farm run by the Justus Liebig University Giessen, Germany. Among the tested models, Long Short-Term Memory (LSTM) networks outperformed Convolutional Neural Networks (CNNs) and hybrid CNN-LSTM models given that data from all sources were available (Scenario S1), achieving an R² of 0.88 and a mean bias error (MBE) of 13.55 ppm CH₄. To assess model applicability under varying data scenarios, features were categorized as "rare," "moderate," or "public" based on their ease of acquisition. Using only public weather data (Scenario S2) resulted in poor predictions, while incorporating moderate-effort farm data (Scenario S3) improved accuracy (R² = 0.45, MBE = 17.60). Adding three rarely available feed-related features, namely feed efficiency, concentrate intake, and total dry matter intake considerably enhanced performance (Scenario S4: R² = 0.74, MBE = 14.36). Random forest analysis highlighted feed-related data as critical for improving prediction performance. These findings demonstrate the capability of DL models to accurately predict CH₄ emissions using readily accessible farm data integrated with a small set of high-impact feed-related features. This approach provides a valuable tool for developing targeted strategies to mitigate methane emissions in dairy farming.

How to cite: Sahraei, A., Knob, D., Lambertz, C., Gattinger, A., and Breuer, L.: Predicting Enteric Methane Emissions in Dairy Cows Using Deep Learning Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8327, https://doi.org/10.5194/egusphere-egu25-8327, 2025.

EGU25-8992 | ECS | Orals | AS3.34

FERTIPAS: Emissions of organic FERTIlizers as Secondary Organic Aerosol Precursors 

Mostafa khazma, Henri Wortham, Julien Kammer, and Brice Temime-roussel

Agriculture is a major source of volatile organic compounds (VOCs), key precursors of secondary air pollutants such as ozone and aerosols. These VOCs react with atmospheric oxidants (e.g., hydroxyl radicals, ozone, nitrate radicals) to form more oxidized compounds with a low volatility that can condense to the particulate phase, driving the formation of secondary organic aerosols (SOA). SOA, a major component of atmospheric aerosols, significantly impacts air quality, climate, and human health. However, estimating SOA production remains highly uncertain due to the complexity of these processes and the diversity of precursors. The shift toward sustainable agriculture has increased the use of organic fertilizers, such as sewage sludge, compost, and animal waste. Given the vast agricultural land area, the spreading of organic fertilizers represents a potentially significant source of VOC emissions. However, their impact on the atmosphere remains poorly understood, mainly due to a lack of studies. The general aim of this work is to improve our knowledge on the impact of spreading these organic fertilizers on air quality, as a source of VOCs. Laboratory study was carried out to analyze VOC emissions from organic fertilizers (sewage sludge, compost and methanization digestate) and to assess the impact of temperature on these emissions. An experimental set-up combining a proton transfer reaction time-of-flight mass spectrometer (PTR-ToF-MS), an emission chamber and a multi-valve system was employed to assess VOC emission from three different organic fertilizers, at three temperatures (10°C, 20°C and 30°C).The analysis revealed a total emission of 118 VOCs from digestate, 99 from sewage sludge and 200 from compost. One notable observation is the perceptible diversity in the chemical composition of these three organic fertilizers. Specifically, each fertilizer presents hydrocarbon, oxygenated and nitrogenated compounds, with hydrocarbons and oxygenated compounds dominating in all three fertilizers. On the other hand, sulfur compounds are only present in sludge and compost, while digestate had a significantly higher prevalence of nitrogenated compounds. Acetone (C3H6O) is the most emitted compound from digestate and sewage sludge, while methanol (CH4O) predominates in compost emissions.  In addition, compounds such as monoterpenes (C10H16), cresols (C7H8O) and phenols (C6H6O), known SOA precursors, were among the most emitted compounds. Secondly, most compounds showed a positive response to temperature, with some increasing linearly and others exhibiting exponential response. Conversely, very few VOCs, such as acetic acid, unexpectedly decreased with rising temperatures. The impact of temperature variations on VOC emissions and the mechanisms driving these patterns will be discussed. Lastly, the potential of organic fertilizers to form ozone through VOC emissions has been estimated for each emitted molecule. Compost had the highest ozone-forming potential followed by sewage sludge and digestate. For digestates and composts, the primary species responsible for ozone formation were hydrocarbons (63% and 60%, respectively), even though oxygenated compounds dominated their emissions. In contrast, for sewage sludge, 56% of the ozone were produced by oxygenates. The results suggested that, from the perspective of air quality, digestate may be a preferable organic fertilizer compared to compost and sewage sludge.

How to cite: khazma, M., Wortham, H., Kammer, J., and Temime-roussel, B.: FERTIPAS: Emissions of organic FERTIlizers as Secondary Organic Aerosol Precursors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8992, https://doi.org/10.5194/egusphere-egu25-8992, 2025.

EGU25-9186 | ECS | Posters on site | AS3.34

Development of a Satellite-Based Algorithm for Detecting Methane Emission Changes from Rice Paddies  

Seongmun Sim, Ye-Seul Yun, Subin Cho, SeongWook Park, Boram Seong, Yeongho Kim, Myungseok Lee, and Keunhoo Cho

With the acceleration of climate change, there is an increasing focus on the management of greenhouse gases. Although carbon dioxide is a primary concern, methane and nitrous oxide significantly contribute to the overall greenhouse gas concentration in the atmosphere, necessitating research on their monitoring and quantification. More than 50% of methane emissions originate from sources including natural gas and oil processing, enteric fermentation, and landfills, making those industries the focus of intensive monitoring attempts, encompassing satellite-based observations for extensive and periodic assessment. Further, methane plumes can be detected and emission rates assessed using wind field data for high-concentration sources.

 

In agriculture, rice paddies are a major source of methane emissions. Nonetheless, a low emission rate per unit area frequently produces undetectable plumes, resulting in dependence on inventory-based simulations instead of measurement-based monitoring. Despite the low emission rate, the extensive expanse of rice fields implies that alterations in fertilizer application or agricultural methodologies can result in substantial changes in overall emissions, thereby requiring prompt monitoring. Moreover, rice cultivation is predominantly concentrated in Asia, which could significantly affect emissions if disrupted by climatic and meteorological changes in the region.

 

This research develops an algorithm to identify changes in methane emissions utilizing satellite-derived methane concentration data from TROPOspheric Monitoring Instrument (TROPOMI) onboard Sentinel-5p, TANSO-FTS-2 (Thermal And Near infrared Sensor for carbon Observation – Fourier Transform Spectrometer-2) onboard GOSAT (Greenhous gases Observing SATellite), and AIRS (Atmospheric Infrared Sounder) onboard Aqua. Through the analysis of over three years of aggregated data and its comparison with crop calendars, reference datasets named baseline data specifically designed for the growth and agricultural cycles of rice were developed with the valid value ranges. These were employed to identify increases or decreases in greenhouse gas emissions or alterations in emission timing by contrasting current observations with baseline data. The algorithm was implemented in principal rice cultivation regions of South Korea, effectively detecting substantial methane emissions during the irrigation phase causing anaerobic fermentations to soil under the water. This method illustrates the capability of satellite data to improve the comprehension and regulation of agricultural methane emissions. Additionally, guidelines for sustainable agricultural practices and the management of greenhouse gas emissions in agriculture will be feasible.

How to cite: Sim, S., Yun, Y.-S., Cho, S., Park, S., Seong, B., Kim, Y., Lee, M., and Cho, K.: Development of a Satellite-Based Algorithm for Detecting Methane Emission Changes from Rice Paddies , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9186, https://doi.org/10.5194/egusphere-egu25-9186, 2025.

EGU25-9903 | ECS | Posters on site | AS3.34

Modeling the impacts of ozone deposition on wheat yields 

Manuela Harrel Njiki, Ronny Lauerwald, Jean-François Castell, and Raia-Silvia Massad

 In recent years, there has been a growing concern about the impacts of ozone pollution on crop
production, particularly in peri-urban cropping areas. As an oxidant, ozone affects plant
biochemical and physiological processes, which in turn disrupt crop development and result in
yield losses. Wheat, a staple crop that sustains billions of people worldwide, is particularly
susceptible to ozone pollution. Quantifying the effects of ozone on wheat yields is crucial for
shaping agronomic and environmental policies at both national and European levels, not only
for the present but also for future scenarios involving climate change, air quality, and
agricultural land management. Another key element to consider is the effect of ozone on soil
organic carbon sequestration in croplands. Crop models play a vital role in quantifying the
combined effects of ozone and management practices on crop growth, yield, biomass
accumulation, and soil carbon dynamics.
The CERES-O3 model developed in 2005 which extends from the CERES-EGC crop model
by integrating Farquhar’s photosynthesis model, efficiently fulfills these requirements.
CERES-O3 simulates the effects of elevated ozone concentrations on photosynthetic rates,
including Rubisco carboxylation efficiency, and consequently on biomass production and
yields.
We use new sets of experimental data obtained at the Grignon ICOS (Integrated Carbon
Observation System) site under varying pedoclimatic conditions against experimental data from
the literature to evaluate the model’s performance. Model simulations reveal that elevated
ozone concentrations reduce photosynthetic rates, stomatal conductance, and Rubisco
carboxylation efficiency, culminating in diminished biomass and grain yield. Furthermore,
parameterizations for two wheat cultivars (Premio and Soissons) show similar ozone effects on
both cultivars.
Although developed more than 20 years ago, CERES-O3 remains a promising tool to quantify
current and predict future ozone impacts at local and global scales. It has strong potential to
enable the exploration of mitigation strategies, including cultivar development, improved
agronomic practices, and policy interventions to curb ozone pollution. It can be used to better
understand the combined effects of ozone pollution and climate stress, which are essential for
ensuring food security in changing global environments. Future steps regarding the model
involve assessing the potential impacts of ozone on soil carbon sequestration in croplands,
which remains a little-known factor in nature-based solutions to mitigate climate change.
Keywords: Ozone, wheat, crop yield, photosynthesis, modeling, stomatal conductance,
CERES-O3

How to cite: Njiki, M. H., Lauerwald, R., Castell, J.-F., and Massad, R.-S.: Modeling the impacts of ozone deposition on wheat yields, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9903, https://doi.org/10.5194/egusphere-egu25-9903, 2025.

EGU25-10491 | ECS | Posters on site | AS3.34

Surfatm-PM: a model of bi-directional particulate matter exchanges over a grassland 

Aubin Courty, Patrick Stella, Rachna Bhoonah, Didier Hébert, Philippe Laguionie, Denis Maro, Pierre Rouspard, Eric Lamaud, Denis Quelo, Erwan Personne, and Sébastien Saint-Jean

According to the Global Burden of Diseases, PM2.5 (particles with a diameter under 2.5 µm) is the leading cause of diseases and deaths in 2021 (Brauer et al., 2024). Along with decreased emissions, removal through deposition is used to reduce exposure to particulate matter (PM). With a leaf area index (m² of leaf per m² of land) usually higher than 1, plants allow for a higher deposition surface, hence more particle removal from ambient air. Thus, understanding and estimating PM deposition on vegetation is necessary to assess the impact of vegetation on air quality. In situ measurements above vegetation have shown that PM (vertical) deposition velocity can be positive and negative (Pellerin et al., 2017). No 1-dimensional PM deposition model can predict such values. The objective of this study is to implement a working bi-directional PM exchange scheme in the Surfatm exchange model (Personne et al., 2024), a 1-dimensional SVAT model, using a resistive scheme. The bi-directional fluxes are introduced using a compensation point approach, which can be interpreted as the PM surface concentration. This allows the concentration gradient to change signs depending on the difference of concentration between ambient air and the surface. Two PM exchange datasets above a grassland in Lusignan (France) are used to calibrate and validate the model respectively (Pellerin et al., 2017). The Surfatm-PM model can predict positive and negative deposition velocities, with notable differences attributable to the formation mechanism of the particles, such as the process of coagulation or nucleation or condensation between ambient air and (vegetated) interfaces.

How to cite: Courty, A., Stella, P., Bhoonah, R., Hébert, D., Laguionie, P., Maro, D., Rouspard, P., Lamaud, E., Quelo, D., Personne, E., and Saint-Jean, S.: Surfatm-PM: a model of bi-directional particulate matter exchanges over a grassland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10491, https://doi.org/10.5194/egusphere-egu25-10491, 2025.

EGU25-11422 | Orals | AS3.34

Nitrosat, a satellite mission concept for mapping reactive nitrogen at the landscape scale 

Pieternel Levelt and Pierre Coheur and the Nitrosat Team

Two key forms of reactive nitrogen (Nr) in the atmosphere are nitrogen oxides (NO+NO2) and ammonia (NH3). Both species are abundantly emitted from anthropogenic sources (fossil fuel combustion, agriculture) with devastating consequences on the environment, human health and climate. Complementing sparse ground-based measurements, current satellite sounders provide daily coverage of their global distribution. However, the spatial resolution of these instruments (>20 km² for NO2 and >100km² for NH3) is orders of magnitudes greater than the typical size of the main Nr sources (industries, farms, roads), which makes identification of the emitters, and corresponding quantification of their emission strengths particularly challenging.

 

To understand and address the impacts of a perturbed nitrogen cycle, and in response to the current observational gap, a dedicated satellite for the monitoring of NO2 and NH3 at high spatial resolution has been conceptualised, called Nitrosat. Its main objective is to quantify simultaneously the emission sources of NH3 and NOx at the landscape scale (<0.25 km²) and to characterize seasonal patterns (<1 month) in their emissions. The two imaging spectrometers onboard Nitrosat will operate respectively in the infrared for NH3 and the visible for NO2, offering gapless coverage in a single swath.

 

Starting from representative examples of measurement techniques that are presently used to derive emission fluxes from NH3 and NO2 satellite observations, we discuss the limitations of current sounders. We introduce the Nitrosat measurement concept and, exploiting both model simulations and aircraft campaign data, provide examples from the EE11 Phase 0 studies of how Nitrosat will enable retrieval of emission fluxes from local and diffuse sources in a way that will not be possible with other current or planned missions.

How to cite: Levelt, P. and Coheur, P. and the Nitrosat Team: Nitrosat, a satellite mission concept for mapping reactive nitrogen at the landscape scale, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11422, https://doi.org/10.5194/egusphere-egu25-11422, 2025.

EGU25-13536 | ECS | Orals | AS3.34

Leveraging In Situ and Satellite Data to understand Changing Ammonia above an Agricultural Hotspot 

Lillian Naimie, Da Pan, Amy P. Sullivan, Kimberley A. Corwin, Katherine Benedict, Lena Low, and Jeffrey L. Collett

The Colorado Front Range urban corridor and the plains to the east are important source regions of ammonia (NH3), an unregulated pollutant primarily emitted from agricultural activities. Upslope flows driven by the mountain-plains circulation and synoptic scale storm circulations periodically transport these emissions into Rocky Mountain National Park located 50 km west, where excess reactive nitrogen (N) deposition is a historical problem with well documented impacts on the ecosystem. A combination of low-cost Radiello passive sampler NH3 measurements and NH3 total column retrievals from the Infrared Atmospheric Sounding Interferometer (IASI) are used to assess temporal and spatial variability in NH3 across three distinct land use categories in the region: agricultural, urban, and rural. The NH3 mixing ratio from passive measurements was strongly correlated with the number of confined animal feedlot operations (CAFOs) within a 12 km radius, confirming the importance of that emission source category. Ground-level passive NH3 measurements have a strong correlation with monthly gridded IASI satellite retrievals. Using satellite retrievals, we find an increasing NH3 trend of approximately 3% per year in agricultural and urban sub-regions. We attribute less than 0.2% of the increasing NH3 trend to reductions in particle sulfate. The absolute trend follows the spatial distribution of CAFOs. In the agricultural sub-region, the absolute NH3 trend is on average greater than 2 times larger than that observed in the urban sub-region. The ground-based observations do not have a trend. The lack of ground-based trend is attributed to increasing boundary layer height and dilution of concentrations, through analysis of ERA5 reanalysis data. Lofting NH3 higher into the atmosphere can increase atmospheric lifetime, associated with transport and deposition further from source regions and increased particle formation. Elevated NH3 from wildfire smoke was observed in August 2020, a period of active wildfire activity in northern Colorado, from IASI satellite retrievals. This elevation was less apparent in surface measurements, likely also due to the lofting of the smoke plume. Modeled smoke plumes from the Hazard Mapping System were used to assess the potential impacts of wildfires on observed NH3 trends.

How to cite: Naimie, L., Pan, D., Sullivan, A. P., Corwin, K. A., Benedict, K., Low, L., and Collett, J. L.: Leveraging In Situ and Satellite Data to understand Changing Ammonia above an Agricultural Hotspot, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13536, https://doi.org/10.5194/egusphere-egu25-13536, 2025.

EGU25-15997 | ECS | Posters on site | AS3.34

Assessing the ammonia mitigation potential from the Indian agriculture sector for improving air quality in India 

Rakhi Chaudhary, Sagnik Dey, Gazala Habib, and Pallav Purohit

As an agrarian country, India heavily depends on fertilizers for food production to meet consumption demands, which contributes to a significant portion of global ammonia emissions. Ammonia is an essential precursor gas to form secondary PM2.5 by reacting with SO2 and NO2 and degrades air quality significantly. Thus, it is imperative to implement mitigation strategies to reduce ammonia emissions from the agricultural sector for air quality improvement. In this study, we have updated the sub-sectoral agriculture activity data for each state of India, using 2022 as the base year. Ammonia emissions from each sub-sectoral activity for each state were estimated in the GAINS model for baseline and future scenarios under the current policy framework. We estimated the mitigation potential for ammonia emissions in agriculture by applying different alternate control scenarios. Under the current baseline scenario, the ammonia emissions (in Kilotons) from urea application are the highest among all the states, followed by other livestock such as sheep and horses, other cattle (Beef), dairy cattle, poultry, nitrogenous fertilizer use and production, and agricultural waste burning. The major contributor states to annual ammonia emissions (in Kt/yr) from urea application are Uttar Pradesh (625 ), followed by Andhra Pradesh (290.67) and Madhya Pradesh (271.32). The major contributor states to NH3 emissions from livestock sectoral activities (other cattle, dairy cattle, sheep and horses, poultry, etc.) are Uttar Pradesh (827.73) followed by Andhra Pradesh (478.65) and Rajasthan (491.13). The NH3 emissions (kt/y) from nitrogenous fertilizer production and consumption was highest from Uttar Pradesh (23.28), followed by Gujarat (10.86) and Maharashtra (10.44), while the contribution from agriculture waste burning was estimated largely from Uttar Pradesh (61.10), followed by Andhra Pradesh (32.91) and Tamil Nadu (30.04).  We consider several strategies, such as deep manure placement, low nitrogen feed, scrubber for livestock housing, urea substitution, neem-coated urea, and biochar additives to reduce NH3 emissions and estimate their mitigation potentials in this work. To date, there are no specific regulations in India targeting agricultural ammonia emissions at the same level as those of other sector pollutants. Therefore, our results will be useful for policymakers for developing state-specific sub-sectoral mitigation strategies to address this critical issue.

Keywords: Ammonia, fertilizer, livestock, emissions, control scenarios

How to cite: Chaudhary, R., Dey, S., Habib, G., and Purohit, P.: Assessing the ammonia mitigation potential from the Indian agriculture sector for improving air quality in India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15997, https://doi.org/10.5194/egusphere-egu25-15997, 2025.

EGU25-17390 | Orals | AS3.34

Online fluxes of pesticides over bare soil in France with a PTRMS: results from French the Online-PTR4-Pest study 

Benjamin Loubet, Florence Lafouge, Céline Decuq, Raluca Ciuraru, Pauline Buysse, baptiste Esnault, and Valérie Gros

In agriculture, plant protection products (i.e. pesticides) protect crops from pests, weeds and diseases. However, pesticides introduced into our environment can also contaminate the air, partly due to volatilisation after pesticide application. Measuring volatilisation in field crops requires trapping techniques, which are costly and time-consuming. There is therefore a strong need for metrological developments to implement (1) analysers that can measure pesticide concentrations continuously over a short period of time, (2) the monitoring of pesticide emissions over a sufficiently long period to capture the entire volatilisation period and (3) the acquisition of data sets in little-explored situations, particularly in wine-growing practices.

The aim of the Online-PTR4-Pest project was to develop the measurement of concentration and volatilisation for three pesticides using proton transfer mass spectrometry (PTR-MS). This technique should eventually enable real-time measurement of pesticide concentrations in the air, as well as field measurement of pesticide volatilisation (using inverse modelling or possibly turbulent covariance methods).

Three pesticides were selected: Prosulfocarb, Pendimethalin (two herbicides used in field crops) and Cyflufenamide (a vine fungicide). Several analysers were used: gas chromatography with thermodesorption mass spectrometry (TD-GC-MS) and PTR-MS. Measurement of the two herbicides was validated using the highly sensitive PTR-Qi-TOF-MS (a time-of-flight mass spectrometer with a proton transfer ionisation source and quad used as an ion guide). Gas-phase calibration is a key stage in the metrological development of PTR-MS measurements. A permeation calibration system was developed and successfully tested, enabling the PTR-MS to be calibrated over a concentration range of 3 ppt to 10 ppb for prosulfocarb and 1 ppt to 3 ppb for pendimethalin.

A three-week field campaign was carried out at the ‘BioEcoAgro’ cross-border joint research unit of INRAE in Mons, with measurements on wheat plots. Air concentrations of Proculfocarb and Pendimethalin were quantified (using both analytical chains and a time step of 5 minutes). These air concentrations varied between 0 and 15 µg m 3 for Prosulfocarb and 0 to 3 µg m 3 for Pendimethalin. Volatilisation fluxes for these two herbicides were estimated using two different methods (aerodynamic gradient and inverse modelling). Over the first few days of field measurements, volatilization of Prosulfocarb was around ten times higher than that of Pendimethalin, regardless of the method used. However, the two methods gave different volatilisation values, as the inverse modelling method was made more uncertain by the applications of these pesticides in the surrounding fields. Finally, the Volt'air-Veg model of pesticide volatilisation was tested on the two datasets. The feasibility of measuring gaseous pesticides in the air in real time using a PTR-MS has been demonstrated.

How to cite: Loubet, B., Lafouge, F., Decuq, C., Ciuraru, R., Buysse, P., Esnault, B., and Gros, V.: Online fluxes of pesticides over bare soil in France with a PTRMS: results from French the Online-PTR4-Pest study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17390, https://doi.org/10.5194/egusphere-egu25-17390, 2025.

EGU25-17465 | ECS | Posters on site | AS3.34

Agricultural sources impact on NH3 and PM levels in the South-Central Anatolia  

Aykut Mehmet Alban, Seda Tokgoz, Serra Saracoglu, and Burcak Kaynak

Atmospheric ammonia (NH3) is a significant pollutant that rapidly reacts with atmospheric acids like sulfuric acid (H2SO4) and nitric acid (HNO3) to form fine particulate matter (PM2.5), which has negative effects on both the environment and public health. NH3 has several kinds of sources but main emitter is agriculture, which originates from crop production and livestock managements. Besides conventional emissions from agriculture, agricultural waste burning is also significant in some regions although prohibited.

Türkiye is an agricultural producing country, and the largest agricultural areas and livestock farms are located in South-Central Anatolia. This study aims to investigate the possible causes of high NH3 and PM levels in this region, focusing on agricultural activities such as crop production, livestock farming, and agricultural residue burning. Using IASI Level-2 NH3 retrievals, the spatio-temporal changes in NH3 levels was investigated over the region. Annual and seasonal changes in NH3 levels were evaluated together with meteorological parameters and ground-based PM10 and PM2.5 measurements. In order to understand the effect of agricultural burning on high NH3 and PM levels in fall season, biomass burning regions were determined with VIIRS S-NPP Fire Radiative Power (FRP) product and aerosol types were examined with CALIOP Level-1 and Level-2 VFM product. High NH3 levels were detected in the study area which has the highest agricultural activity in Türkiye. Seasonal distributions of the region showed that significant levels in fall season, unlike all other regions in Türkiye indicating highest summer NH3 levels. These findings indicated a different source causing high NH3 levels in the fall season other than the agricultural activities usually having highest impact in spring and summer seasons. In the fall seasons (2019-2023), the highest FRP values were observed with values three times or higher than of other seasons. Especially, the highest number of fires occurred in fall of 2020 and 2023, when higher NH3 levels were also observed. Additional to regional high values, hotspots of NH3 were identified in Konya–Eregli, Nigde–Bor, and Aksaray–Merkez. NH3 levels were also observed higher during winter seasons in these hotspots where livestock farms are frequently located. Therefore, effects of livestock farming and residual burning as a NH3 source stood out in this region rather than conventional fertilizer applications. It is important that these lesser known and investigated emission sources of NH3 need to be evaluated to understand their role in secondary particulate matter formation and their impact on public health in the region.

Keywords: Ammonia, Agricultural residue burning, Livestock management

Acknowledgements: IASI is a joint mission of EUMETSAT and the Centre National d'Etudes Spatiales (CNES, France). The authors acknowledge the AERIS data infrastructure for providing access to the IASI data in this study and ULB-LATMOS for the development of the retrieval algorithms. This study was supported by the Scientific and Technological Research Council of Türkiye under the grant number 123Y364.

How to cite: Alban, A. M., Tokgoz, S., Saracoglu, S., and Kaynak, B.: Agricultural sources impact on NH3 and PM levels in the South-Central Anatolia , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17465, https://doi.org/10.5194/egusphere-egu25-17465, 2025.

EGU25-17924 | ECS | Orals | AS3.34

Long-Term NH3 Assesment with Meteorological Parameters to Obtain Temporal Profiles in Agricultural Regions 

Seda Tokgoz, Aykut Mehmet Alban, Serra Saracoglu, and Burcak Kaynak

The impact of climate change on agricultural emissions becomes important, and strongly affects pollutant levels such as NH3 in the atmosphere. Atmospheric NH3 levels and emission rates are very sensitive to meteorology factors such as temperature and precipitation. Being one of the major pollutants emitted from agriculture, NH3 becoming increasingly important, both because it is a pollutant itself and it contributes to the formation of secondary particulate matter. Long-term assessment of IASI NH3 retrievals showed localized consistent hotspots in some regions of Türkiye, often associated with agricultural activities. Although, the reported emission levels do not chance, there was significant temporal variation observed in the NH3 retrievals in those regions.

In this study, twelve years of NH3 retrievals were spatially processed to obtain annual, seasonal and monthly NH3 distribution maps with a 1x1 km2 gridded domain covering whole Türkiye. The results indicated significant temporal variability which also changes according to different regions. The temporal changes of NH3 for three localized hotspots with significant agricultural activity among the highest NH3 levels in Türkiye were selected and evaluated as; Igdir (Cold semi-arid), Izmir (Hot summer Mediterranean) and Samsun (Humid sub-tropical). The selection was performed to identify the different climatic conditions, crop and fertilizer types. Level-2 IASI NH3 retrievals, yearly agricultural statistics, and meteorological measurements were utilized for understanding the changes in NH3 levels. Among these hotspots, Igdir has the highest seasonal variation with maximum late spring to summer, and Samsun is with least seasonal variation. Within the years investigated, 2015, 2018-2019 and 2022-2023 showed highest number of extreme NH3 retrievals. This study aims to provide a new approach to the assessment of agricultural NH3 variability by the long-term assessment to obtain region-specific temporal profiles which the regional air quality models strongly depend on.

Keywords: ammonia, meteorological factors, temporal variation

Acknowledgements: IASI is a joint mission of EUMETSAT and the Centre National d'Etudes Spatiales (CNES, France). The authors acknowledge the AERIS data infrastructure for providing access to the IASI data in this study and ULB-LATMOS for the development of the retrieval algorithms. This study was supported by the Scientific and Technological Research Council of Türkiye under the grant number 123Y364.

How to cite: Tokgoz, S., Alban, A. M., Saracoglu, S., and Kaynak, B.: Long-Term NH3 Assesment with Meteorological Parameters to Obtain Temporal Profiles in Agricultural Regions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17924, https://doi.org/10.5194/egusphere-egu25-17924, 2025.

EGU25-20286 | ECS | Orals | AS3.34

 The use of open-path FTIR techniques to measure nitrous oxide, ammonia, and methane emissions from a sugarcane farm in Australia 

Pongsathorn Sukdanont, Mei Bai, Shu Kee Lam, Helen Suter, and Deli Chen

Intensive agricultural systems are a main source of greenhouse gas (GHG) emissions. The nitrogen (N) fertilizers that are applied to crops to increase crop productions during growing season can lose approximately half of the applied N to the atmosphere as nitrous oxide (N2O) and ammonia (NH3).This results in growers’ financial losses and can cause environmental pollutions. Quantification of gas emissions not only helps to develop inventories of regional and national emissions but also to improve management practices to mitigate the emissions. However, accurate quantification of the gas emissions at farm scale is challenging as the natural reactive ammonia gas is a “sticky” gas, and N2O has spatialand temporal variability. There is a need of proper techniques to continually measure a suite of gases including N2O and NH3simultaneously to reduce the complexity of using multiple gas sensors for measurements.

A trial was conducted in July 2024 to measure N2O, NH3, and CH4emissions following the fertilizer and fertilizer inhibitor applications at a commercial sugarcane farm in Queensland, Australia. Two separate plots were chosen, one plot was for a control plot with urea fertilizer and the second one was for the treatment plot applying urea and urea inhibitor. At each plot, a slant-path Fourier transform infrared spectrometer (slant-path FTIR) was deployed to measure a suite of gas concentrations for three weeks, including N2O, NH3, and CH4, simultaneously.Thirty-min averaged wind statistics and the coordinates of locations of equipment and experimental plots were collected. These measurements of gas concentration and wind statistics were used to calculate gas fluxes using a micrometeorological technique. The fluxes of N2O, NH3, and CH4from control and treatment plots showed that the effects of inhibitor on reduction of N2O and CH4 emissions were significant over the measurement period but NH3 flux reduction was only triggered by the irrigation event.

How to cite: Sukdanont, P., Bai, M., Kee Lam, S., Suter, H., and Chen, D.:  The use of open-path FTIR techniques to measure nitrous oxide, ammonia, and methane emissions from a sugarcane farm in Australia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20286, https://doi.org/10.5194/egusphere-egu25-20286, 2025.

EGU25-3074 | ECS | PICO | AS3.35

The impact of chlorocarbons on tropospheric composition: a global model study 

Kathryn Vest, Ryan Hossaini, Oliver Wild, Andrea Mazzeo, Xuewei Hou, and Fiona O'Connor

Tropospheric chlorine has the potential to perturb atmospheric oxidation capacity, which plays an important role in climate change and air quality. Although sea-salt is the predominant source of tropospheric chlorine, oxidation of chlorocarbons could prove to be a more important source of tropospheric chlorine than previously thought due to their increasing abundances over the last 2 decades. The most abundant chlorocarbon, methyl chloride (CH3Cl) is predominantly emitted from natural sources and has stayed relatively stable over the last 20 years. However, the concentrations of a range of chlorine-containing very short-lived substances (Cl-VSLS) have varied substantially over the same time period, particularly anthropogenically emitted Cl-VSLS: dichloromethane (CH2Cl2), 1,2-dichloroethane (C2H4Cl2), perchloroethylene (C2Cl4), trichloromethane (CHCl3) and trichloroethylene (C2HCl3). Additionally, there are a number of bromine and iodine containing Cl-VSLS (e.g. CH2BrCl) that are released from natural sources.

Here, the Frontier Research System for Global Change version of the University of California Irvine Chemical Transport Model is used to explore the impact of Cl-VSLS in the troposphere. A tropospheric chlorine chemistry scheme including appropriate sources, reactions and sinks of chlorine species was incorporated into the model and multi-year simulations were used to assess the spatio-temporal trends in Cl-VSLS. Two approaches were compared to assess the impact of Cl-VSLS. The first method involves constraining the chlorocarbons using latitude- and time-varying surface concentrations generated from measurement data, whilst the second method used fully geographically varying emissions. We consider a more comprehensive set of chlorocarbons than previous studies and explore how their abundances have changed over time. We find that the contribution of chlorocarbons to tropospheric inorganic chlorine has increased; from ~4100 Gg/year in 2000 to ~4600 Gg/year in 2022. The impact of chlorocarbons on tropospheric composition will also be presented.

How to cite: Vest, K., Hossaini, R., Wild, O., Mazzeo, A., Hou, X., and O'Connor, F.: The impact of chlorocarbons on tropospheric composition: a global model study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3074, https://doi.org/10.5194/egusphere-egu25-3074, 2025.

EGU25-3966 | PICO | AS3.35

Concentration characteristics and emission estimates ofmajor HCFCs and HFCs at three typical fluorochemical plants in China based on a Gaussian diffusion model 

Jing Wu, Zehua Liu, Tengfei Ma, Minde An, Tong Ye, Xingchen Zhao, Mingzhu Li, Fan Wang, Mao Yuan, Dongmei Hu, Yueling Zhang, and Lin Peng

Estimating the emissions of hydrochlorofluorocarbons (HCFCs) and hydrofluorocarbons (HFCs) is of great significance for assessing global ozone depletion and climate change, where the emissions from fluorochemical plants play an important role. However, no research has been conducted on the HCFC and HFC emissions from fluorochemical plants based on observation data and diffusion model. This study observed the concentration of two HCFCs and six HFCs around three typical fluorochemical plants in China. It used the Gaussian plume diffusion model to explore their emissions. The results showed that the concentration difference between the downwind and upwind sites (from now on referred to as down-up difference) of each substance is ranked. Only in plant A, the substance with the largest down-up difference is HCFC. The total HFC down-up differences of the three plants were higher than that of HCFCs, and the total emissions of six HFCs accounted for 46% of three plant’s emission, suggesting that the HFC production of the three typical fluorochemical plants in China had reached a large scale with the phase-out of ODSs (ozone-depleting substances). The total emissions of HCFCs and HFCs from the three plants are 56.62 Mt (million ton) CO2-equiv yr−1. The emissions from the three plants are approximately 20–76% of the bottom-up national emissions estimated using IPCC 2019 emission factors. On the contrary, the emissions of the three plants are 2–6 times higher than the national emissions (contained 20 fluorochemical plants) based on the IPCC 2006 emission factor. This revealed that using the default emission factors for fluorochemical production recommended by IPCC 2006 to estimate the emissions of HCFCs and HFCs from fluorochemical plants in China may lead to underestimation.

How to cite: Wu, J., Liu, Z., Ma, T., An, M., Ye, T., Zhao, X., Li, M., Wang, F., Yuan, M., Hu, D., Zhang, Y., and Peng, L.: Concentration characteristics and emission estimates ofmajor HCFCs and HFCs at three typical fluorochemical plants in China based on a Gaussian diffusion model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3966, https://doi.org/10.5194/egusphere-egu25-3966, 2025.

EGU25-4239 | ECS | PICO | AS3.35

Long-path DOAS observations of halogen oxides at Utqiagvik, Alaska 

Bianca Lauster, Sebastian Donner, Udo Frieß, Ulrich Platt, Lucas Reischmann, William Simpson, Steffen Ziegler, and Thomas Wagner

Halogen chemistry is a central element of tropospheric ozone depletion events (ODEs) during polar spring. Key processes such as source mechanisms that produce reactive halogen species, their transport, and interhalogen interactions as well as the influence of the quickly changing climate, however, remain in the centre of Arctic research.

We deployed a Long-Path Differential Optical Absorption Spectroscopy (LP-DOAS) instrument in Utqiagvik (formerly Barrow), Alaska, in December 2023. First results from measurements performed between March and May 2024 show that this period exhibits active halogen chemistry with many episodes of enhanced bromine monoxide coinciding with strongly reduced ozone concentrations. Further, analysis results of chlorine monoxide are presented. Additional Multi-AXis (MAX-) DOAS observations have been conducted since the beginning of April 2024.

Comparison to data from the instrument’s previous deployment at the German research station Neumayer, Antarctica (Nasse, 2019), indicates differences in the prevailing atmospheric conditions and trace gas amounts between both hemispheres which will be discussed in detail.

How to cite: Lauster, B., Donner, S., Frieß, U., Platt, U., Reischmann, L., Simpson, W., Ziegler, S., and Wagner, T.: Long-path DOAS observations of halogen oxides at Utqiagvik, Alaska, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4239, https://doi.org/10.5194/egusphere-egu25-4239, 2025.

EGU25-6802 | ECS | PICO | AS3.35

Quantifying the role of bromine in the atmospheric oxidation of mercury (Hg) 

Aryeh Feinberg, Jeroen Sonke, and Alfonso Saiz-Lopez

The cycles of the toxic element mercury (Hg) and bromine (Br) are inextricably linked, since Br radicals are a major oxidant for elemental mercury, Hg(0). Global dispersion of Hg occurs through transport of Hg(0), due to its atmospheric lifetime of 6 months. Upon oxidation of Hg(0) to soluble divalent mercury, Hg(II), deposition will occur on timescales of approximately 1 week. There are many uncertainties associated with atmospheric Hg chemistry, leading to uncertain predictions of its fate and impacts on ecosystems. Here we assess the role of Br in the oxidation of Hg(0) using a chemistry-climate model WACCM and quantify sources of uncertainty due to different factors. Oxidation of Hg(0) by Br is found to dominate near the surface in the Southern Hemisphere midlatitudes, as well as throughout the upper troposphere and lower stratosphere. Elsewhere in the troposphere, the reaction of Hg(0) by hydroxyl (OH) radicals is the primary oxidation pathway. However, these results are highly dependent on the model’s lower troposphere bromine concentrations. Comparing different model versions of GEOS-Chem and WACCM, the chemical lifetime of Hg(0) can vary by a factor of more than 20 in the Southern Hemisphere midlatitudes due to differences in simulated Br concentrations. The models show much closer agreement in their simulated OH concentrations, highlighting the higher uncertainties in Br chemistry. We also explored the uncertainty in Hg reaction rates using global sensitivity analysis in a box model representing WACCM chemistry. Uncertainties in the OH-driven oxidation reactions of Hg(0) dominate uncertainties in the Hg(0) lifetime in the Northern Hemisphere, while the reaction rate of Br with Hg(0) is the key uncertainty over much of the Southern Ocean. We identify ~10 reactions out of the full chemical mechanism of 72 Hg-related reactions that contribute almost all of the variability in outputs, indicating the potential for constructing a simplified mechanism for Hg chemistry. Overall, our results emphasize that predictions of Hg deposition are highly impacted by uncertainties in lower troposphere Br radical concentrations, suggesting that more observational constraints on Br are necessary to improve the accuracy of Hg models.

How to cite: Feinberg, A., Sonke, J., and Saiz-Lopez, A.: Quantifying the role of bromine in the atmospheric oxidation of mercury (Hg), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6802, https://doi.org/10.5194/egusphere-egu25-6802, 2025.

EGU25-7049 | PICO | AS3.35

Modelling Arctic springtime ozone depletion events: role of snow sourced bromine chemistry and its impact on Arctic tropospheric ozone budget 

Wanmin Gong, Stephen Beagley, Kenjiro Toyota, Henrik Skov, Jesper Christensen, Alexandru Lupu, Diane Pendlebury, Junhua Zhang, Ulas Im, Yugo Kanaya, Alfonso Saiz-Lopez, Roberto Sommariva, Peter Effertz, John Halfacre, Nis Jepsen, Rigel Kivi, Theodore Koenig, Katrin Müller, Claus Nordstrøm, and Irina Petropavlovski and the TOAR-II Ozone Over the Oceans Focus Working Group - Arctic

A large portion of the Arctic is covered by ocean and sea ice, from which reactive halogen species can be emitted to the atmosphere. Springtime ozone depletion events (ODEs) have been primarily attributed to catalytic destruction of ozone by reactive bromine released from snowpacks and blowing snow over sea ice and cycled through heterogeneous reactions on aerosol surfaces. Mechanisms to represent polar springtime bromine explosions and ODEs have been developed and tested in various atmospheric models, by considering both blowing snow and snowpacks, with varying degrees of success when compared with observations of reactive bromine and ozone in polar regions. In this study, two independent chemical transport models (CTMs), DEHM (Danish Eulerian Hemispheric Model) and GEM-MACH (Global Environmental Multi-scale – Modelling Air quality and Chemistry), were used to simulate Arctic lower tropospheric ozone for the year 2015. Both models include bromine chemistry and a representation of snow-sourced bromine mechanism: a blowing-snow bromine source mechanism in DEHM and a snowpack bromine source mechanism in GEM-MACH.

The comparison of model simulation results with available observations in the Arctic showed that the model with the snowpack bromine source mechanism (GEM-MACH) was able to capture most of the observed springtime ODEs in the Arctic, while the model considering blowing-snow sourced bromine alone (DEHM) simulated much fewer ODEs. The snowpack-sourced mechanism is seen to be essential in sustaining the continued bromine production under a variety of meteorological conditions, while the blowing-snow bromine source mechanism triggered by high wind conditions tends to be more episodic. This is consistent with observational evidence that the ODEs observed in the Arctic tend to occur during calm wind conditions favouring the snowpack bromine source mechanism to take effect in the surface air with ODEs at high wind speed conditions to occur sporadically. The study demonstrated that the springtime ozone depletion process plays a central role in driving the surface ozone seasonal cycle in the Central Arctic, and that the bromine-mediated ODEs, while occurring most notably within the lowest few hundred metres of air above the Arctic Ocean, can induce a 5-7% of loss in the total pan-Arctic tropospheric ozone burden during springtime. The study also demonstrated that atmospheric aerosols play an integral role in the Arctic springtime bromine explosions and ODEs through heterogeneous cycling of reactive bromine, particularly over a deeper vertical layer and at distance from the snowpack bromine source area, which has implications for the potential role of Arctic haze aerosols that may play in the springtime ODEs. The uncertainty in parameterising the Arctic bromine source mechanism will also be discussed.

How to cite: Gong, W., Beagley, S., Toyota, K., Skov, H., Christensen, J., Lupu, A., Pendlebury, D., Zhang, J., Im, U., Kanaya, Y., Saiz-Lopez, A., Sommariva, R., Effertz, P., Halfacre, J., Jepsen, N., Kivi, R., Koenig, T., Müller, K., Nordstrøm, C., and Petropavlovski, I. and the TOAR-II Ozone Over the Oceans Focus Working Group - Arctic: Modelling Arctic springtime ozone depletion events: role of snow sourced bromine chemistry and its impact on Arctic tropospheric ozone budget, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7049, https://doi.org/10.5194/egusphere-egu25-7049, 2025.

EGU25-8956 | PICO | AS3.35

Arctic halogens reduce ozone in the northern mid-­latitudes 

Carlos A. Cuevas, Rafael P. Fernandez, Lucas Berná, Orlando G. Tomazzeli, Anoop S. Mahajan, Qinyi Li, Douglas E. Kinnison, Siyuan Wang, Jean-François Lamarque, Simone Tilmes, Henrik Skov, and Alfonso Saiz-Lopez

While the dominant role of halogens in Arctic ozone loss during spring has been widely studied in the last decades, the impact of sea-­ice halogens on surface ozone abundance over the northern hemisphere (NH) mid-­latitudes remains unquantified. Here, we use a state-­of-­the-­art global chemistry-­climate model including polar halogens (Cl, Br, and I), which reproduces Arctic ozone seasonality, to show that Arctic sea-­ice halo- gens reduce surface ozone in the NH mid-­latitudes (47°N to 60°N) by ~11% during spring. This background ozone reduction follows the southward export of ozone-­poor and halogen-­rich air masses from the Arctic through polar front intrusions toward lower latitudes, reducing the springtime tropospheric ozone column within the NH mid-­latitudes by ~4%. Our results also show that the present-­day influence of Arctic halogens on surface ozone destruction is comparatively smaller than in preindustrial times driven by changes in the chemical interplay between anthropogenic pollution and natural halogens. We conclude that the impact of Arctic sea-­ice halogens on NH mid-­latitude ozone abundance should be incorporated into global models to improve the representation of ozone seasonality.

How to cite: Cuevas, C. A., Fernandez, R. P., Berná, L., Tomazzeli, O. G., Mahajan, A. S., Li, Q., Kinnison, D. E., Wang, S., Lamarque, J.-F., Tilmes, S., Skov, H., and Saiz-Lopez, A.: Arctic halogens reduce ozone in the northern mid-­latitudes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8956, https://doi.org/10.5194/egusphere-egu25-8956, 2025.

EGU25-9344 | PICO | AS3.35

Enhanced inorganic iodine in the upper troposphere potentially driven by elevated emission and/or fast vertical transport by tropical cyclone 

Karolin Voss, Benjamin Weyland, André Butz, Valentin Lauther, C.Michael Volk, Bärbel Vogel, Andreas Engel, Tanja Schuck, Timo Keber, Meike Rotermund, and Klaus Pfeilsticker

Halogens are known to deplete ozone both in the troposphere and stratosphere. As the source distribution and thus the local contribution of chlorine and bromine containing species to atmospheric ozone depletion is reasonably well known, the respective role of iodine containing species is subject of current research. In contrast to the major sources of chlorine in the stratosphere which derive from man-made chlorinated hydrocarbons, about half of stratospheric bromine stems from bromocarbons of natural origin while iodine predominantly originates from inorganic species (I2, and HOI) emitted from the oceans. It has been indicated previously that tropical cyclones emit elevated amounts of brominated species (e.g. CHBr3 and CH2Br2) which are efficiently transported into the extratropical upper troposphere and eventually into the lower stratosphere. Here we provide evidence that also significant amounts of inorganic iodine emitted from the ocean surface and/or through sea-spray are transported to the extratropical upper troposphere through tropical cyclone driven fast vertical transport.

Our finding is based on the simultaneous detection of elevated amounts of brominated very short-lived substances (VSLS) and iodine oxide (IO, ~0.3 pptv) while simultaneously relatively low mixing ratios of the anthropogenically emitted CH2Cl2 were measured in the upper troposphere (~13 km, θ~360 K) of the mid-Atlantic on October 1st,2017. CLaMS back-trajectory calculations driven by ECMWF ERA-Interim reanalysis suggest that these iodine-rich air masses originate from marine surface air masses being uplifted by the category 5 hurricane Maria.

The measurements were performed from aboard HALO (High Altitude and LOng range Aircraft) during the WISE (Wave-driven ISentropic Exchange) campaign over the mid-Atlantic in September and October 2017. IO was detected in limb scattered skylight using the miniDOAS instrument, while the organic chlorinated and brominated species were detected by the HAGAR-V and GhOST GC/MS instruments.

Our findings suggest that tropical storms lead to elevated emissions of inorganic iodine rapidly transported from the tropical marine boundary layer into the upper troposphere. This mechanism implies a potentially significant role of iodine in ozone destruction in the remnant air of tropical storms and a possible pathway for iodine to enter the lower stratosphere in significant amounts.

How to cite: Voss, K., Weyland, B., Butz, A., Lauther, V., Volk, C. M., Vogel, B., Engel, A., Schuck, T., Keber, T., Rotermund, M., and Pfeilsticker, K.: Enhanced inorganic iodine in the upper troposphere potentially driven by elevated emission and/or fast vertical transport by tropical cyclone, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9344, https://doi.org/10.5194/egusphere-egu25-9344, 2025.

EGU25-9442 | ECS | PICO | AS3.35

Source mechanisms of tropospheric bromine monoxide in Ny-Ålesund between 2017 and 2023 

Qidi Li, Yuhan Luo, Xin Yang, Bianca Zilker, and Andreas Richter

Arctic tropospheric bromine monoxide (BrO) plays a critical role in atmospheric chemistry, particularly during ozone depletion events and the oxidation of gaseous elemental mercury in spring. The contributions of various potential sources, such as sea ice, open ocean, and aerosols, to the production of reactive bromine remain unclear. In this study, we present long-term observations of BrO and aerosol profiles retrieved from Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) measurements in Ny-Ålesund, Svalbard (78.92°N, 11.93°E), covering the periods from March to May between 2017 and 2023. Retrieved tropospheric BrO partial columns are then compared with BrO observations from the GOME-2 satellite instrument and model results from a global chemistry transport model, p-TOMCAT, respectively. Aerosol extinction exhibits the strongest correlation with BrO (R=0.67 in March, 0.54 in April, 0.47 in May), indicating that airborne particles are associated with the enhancement of reactive bromine.

Five days of backward trajectories in an altitude range of 0–3 km (at 200 m intervals) were used to calculate the contact time of air masses with various surface types (sea ice, open ocean, land, and the free troposphere). Along the trajectories, whenever the air mass meets open ocean or sea ice surface (e.g. < 500 m), the corresponding bromine emission flux from sea salt aerosols generated from open ocean (Gong et al., 2003) and blowing snow (Yang et al., 2008) is calculated and accumulated. Results show that, in March, MAX-DOAS BrO is in a positive correlation with sea ice contact time (R=0.29) and bromine emission flux from blowing snow on sea ice (R=0.33), suggesting that sea-ice-sourced sea salt aerosols generated by blowing snow could represent a significant source of reactive bromine. Throughout the entire spring (March-May), the contact time with sea ice accounts for 52.41% of all bromine explosion events (BEEs) observed in Ny-Ålesund, whereas the contact time with open ocean accounts for only 2.85%. This indicates that, in comparison to sea ice, the contribution of open ocean is less significant in Ny-Ålesund. These results confirm the critical role of sea ice-related processes in the production of reactive bromine during spring.

How to cite: Li, Q., Luo, Y., Yang, X., Zilker, B., and Richter, A.: Source mechanisms of tropospheric bromine monoxide in Ny-Ålesund between 2017 and 2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9442, https://doi.org/10.5194/egusphere-egu25-9442, 2025.

EGU25-16206 | ECS | PICO | AS3.35

Validation of TROPOMI tropospheric BrO columns employing CHACHA airborne campaign measurements 

Bianca Zilker, Andreas Richter, Nathaniel Brockway, Peter Peterson, Katja Bigge, William R. Simpson, Heesung Chong, Nicolas Theys, Sora Seo, Hartmut Bösch, and John P. Burrows

The observation of bromine monoxide (BrO) in the polar regions, in particular the study of tropospheric bromine explosion events (BEEs) during the polar spring, has been an ongoing task since the late 1980s. Since the mid-1990s, BrO has also been monitored from satellites, allowing global observation of BrO and the large-scale tropospheric BrO plumes resulting from BEEs in polar regions. With the launch of the TROPOspheric Monitoring Instrument (TROPOMI) in October 2017, there is an instrument that enables daily high-resolution measurements of BrO. From the satellite measurements, total BrO columns are obtained. However, the total column consists mainly of stratospheric BrO and usually only a small amount of BrO is located in the lower troposphere. In order to investigate the tropospheric BEEs, a stratospheric separation method must be applied to subtract the stratospheric contribution from the total BrO column and thereby estimate the amount of tropospheric BrO.

In this study, five different stratospheric separation methods are applied to the TROPOMI BrO dataset to calculate the amount of tropospheric BrO: (1) a constant stratospheric BrO value, (2) a high pass filtering method applied in near real time processing, (3) an empirical multiple linear regression model, (4) a climatology-based method developed by Theys et al. (2011), and (5) a recently developed method for the OMPS satellite by Chong et al. (2024). The different separation methods are compared to each other and the results of all five methods are validated using airborne tropospheric BrO measurements from the Heidelberg Airborne Imaging DOAS Instrument (HAIDI) during the CHemistry in the Arctic: Clouds, Halogens, and Aerosols (CHACHA) campaign, which took place in Alaska in spring 2022.

 

This work was supported by the DFG funded Transregio-project TR 172 “Arctic Amplification (AC)³in subproject C03.

How to cite: Zilker, B., Richter, A., Brockway, N., Peterson, P., Bigge, K., Simpson, W. R., Chong, H., Theys, N., Seo, S., Bösch, H., and Burrows, J. P.: Validation of TROPOMI tropospheric BrO columns employing CHACHA airborne campaign measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16206, https://doi.org/10.5194/egusphere-egu25-16206, 2025.

EGU25-16865 | ECS | PICO | AS3.35

Assessing the Impact of Bromine and Iodine Chemistry on Tropospheric Composition 

Jessica Randell, Ryan Hossaini, Oliver Wild, Andrea Mazzeo, and Xuewei Hou

Halogens (chlorine, bromine and iodine) have been studied extensively in the stratosphere, where they catalytically destroy ozone, but more recently there has been growing interest in their effect on tropospheric composition and oxidative capacity. Of particular interest is how they affect ozone, a powerful greenhouse gas and air pollutant at the Earth’s surface. Reactive halogen species such as  BrO and IO can impact ozone concentrations directly through catalytic cycles and indirectly via affecting the partitioning of HOX and NOX, resulting in important effects on tropospheric composition that are not yet fully understood.

Here, we explore how bromine and iodine chemistry can impact tropospheric ozone concentrations. Using the FRSGC/UCI CTM, we expand the existing tropospheric chemistry scheme (that includes a comprehensive description of iodine chemistry) by including a detailed bromine chemistry scheme. This encompasses major gas-phase and heterogeneous reactions, including reactions occurring on ice particles, alongside physical processes like wet and dry deposition. Sources of bromine include (1) CH3Br and emissions of five short-lived bromocarbons (CHBr3, CH2Br2, CH2BrCl, CHBr2Cl and CHBrCl2), (2) debromination of sea-salt aerosol from the open ocean and from blowing snow in polar regions, and (3) transport from the stratosphere. We explore different approaches to representing open ocean sea-salt debromination, comparing a ‘depletion factor’ based parameterisation with sea-salt debromination arising from a series of heterogeneous reactions. The impact of these different parameterisations on the resulting bromine budget is shown.

A detailed evaluation of the model performance is presented using ground-based, aircraft and satellite observations of key radicals (e.g. halogen oxides) with the results comparing reasonably well with observations. We also explore the spatial and temporal variation of natural halogens in the troposphere and the importance of different sources, and further quantify the impact of reactive halogens on present-day ozone concentrations and tropospheric oxidising capacity.

How to cite: Randell, J., Hossaini, R., Wild, O., Mazzeo, A., and Hou, X.: Assessing the Impact of Bromine and Iodine Chemistry on Tropospheric Composition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16865, https://doi.org/10.5194/egusphere-egu25-16865, 2025.

EGU25-17490 | PICO | AS3.35

Comparison of seasonal differences in hydrogen chloride observations from an inland urban site 

John W. Halfacre, Jordan Stewart, Matthew Rowlinson, Emily Matthews, Thomas Bannan, Jaime R. Green, William Vizuete, Mat J. Evans, Scott C. Herndon, Joseph R. Roscioli, Christoph Dyroff, Tara I. Yacovitch, James Allan, Hugh Coe, Stephen J. Andrews, Steven S. Brown, and Pete M. Edwards

Reactive chlorine radicals are known to efficiently react with ambient hydrocarbons, thereby affecting boundary layer oxidation capacity and pollutant lifetimes. HCl is the most abundant and long-lived inorganic chlorine reservoir species in the troposphere, yet high frequency, in situ observations are limited due to sampling challenges. In this work, we report HCl field observations using a Tunable Infrared Laser Direct Absorption Spectrometer (TILDAS), deployed in Manchester, England, during the 2021-2022 Integrated Research Observation System for Clean Air campaign. Instrument precision was estimated as 1.1 pptv (Allan Werle minimum of 1.4 minute), with 3σ limits of detection of 3.3 pptv. 

Observations obtained during June and July 2021 generally exhibited a diurnal profile on clear days, peaking at midafternoon (mean daily mixing ratios ranging between 15 – 89 pptv). Conversely, observations from February 2022 displayed no obvious profile with mixing ratios remaining muted throughout the observation period (mean daily mixing ratios ranging between 7-13 pptv), suggesting suppression of Cl-liberation mechanisms. Despite observations occurring in an inland polluted urban environment, particle dispersion analysis for both seasons shows air masses spend most of their time passing over the ocean in the 72-hours preceding arrival at the observation site. The thermodynamic equilibrium model ISORROPIA II will be used to explore the role of partitioning between particulate phase Cl- and gas phase HCl, with model inputs supplied from observed non-refactory, submicron particulate SO42-, NO3-, NH4+, and Cl- ions, as well as gas phase observations of HCl, HNO3 and NH3.  Data will be further interpreted using gas phase box modelling, further incorporating co-located CIMS observations of other inorganic Cl-species, including ClNO2 andCl2, to gain a greater understanding of seasonal chlorine chemistry mechanisms at an inland, urban measurement site. 

How to cite: Halfacre, J. W., Stewart, J., Rowlinson, M., Matthews, E., Bannan, T., Green, J. R., Vizuete, W., Evans, M. J., Herndon, S. C., Roscioli, J. R., Dyroff, C., Yacovitch, T. I., Allan, J., Coe, H., Andrews, S. J., Brown, S. S., and Edwards, P. M.: Comparison of seasonal differences in hydrogen chloride observations from an inland urban site, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17490, https://doi.org/10.5194/egusphere-egu25-17490, 2025.

EGU25-1237 | Orals | AS3.36

The Speciated Detection of Gas-phase Organic Peroxy Radicals and Related Intermediates by Proton Transfer Mass Spectrometry 

Barbara Noziere, Olivier Durif, Felix Piel, and Armin Wisthaler

In spite of the importance of organic peroxy radicals in the oxidizing capacity of the atmosphere few techniques exist to monitor them individually, leaving large uncertainties in the understanding of the atmospheric oxidation cycles. This presentation will give an overview of the on-going ERC-advanced project EPHEMERAL focusing on the detection of these radicals using proton transfer mass spectrometry and aiming at monitoring them in ambient air. Current advances in their detection and in that of related intermediates will be presented. The main advantages and limits of the technique will be discussed, in particular the challenges and various strategies for determining the radical absolute concentration (calibrations). While the technique is still being improved, the performances already obtained allow to study new reactions, such as the interactions of the gas-phase radicals with surfaces, which will be also rapidly presented. 

How to cite: Noziere, B., Durif, O., Piel, F., and Wisthaler, A.: The Speciated Detection of Gas-phase Organic Peroxy Radicals and Related Intermediates by Proton Transfer Mass Spectrometry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1237, https://doi.org/10.5194/egusphere-egu25-1237, 2025.

EGU25-3493 | ECS | Posters on site | AS3.36

Enhanced nocturnal oxidation chemistry in the upper mixing layer of megacities 

Yujie Qin, Haichao Wang, Shaojia Fan, Steven Brown, and Keding Lu

The troposphere is considered an oxidizing atmospheric environment with radical chemical reactions. During the day, hydroxyl radicals (OH) are the primary oxidants, while at night, nitrate radicals (NO3) take on this role. NO3 radicals can react with volatile organic compounds (VOCs), especially alkenes, to form organic aerosols. In addition, NO3 radicals can also generate nitrate aerosols through the heterogeneous reaction of N2O5, leading to severe air pollution issues. Nighttime atmospheric oxidizing capacity refers to the ability of oxidants to convert primary pollutants into secondary pollutants. Since NO3 radicals are the main oxidants at night, the nitrate radical production rate (PNO3) is often used as an indicator of nighttime atmospheric oxidizing capacity. However, unlike the well mixed during the day, nighttime air exhibits strong vertical stratification due to the cooling of the ground. As a result, there are significant differences in the concentration of pollutants and chemical reaction processes at different heights, leading to substantial variations in atmospheric oxidizing capacity with altitude. Therefore, ground-based observations cannot fully represent the entire nighttime boundary layer. To accurately describe the oxidative characteristics of the nighttime atmosphere, we combined vertical tower observation data to analyze the distribution characteristics of PNO3 with altitude and classified the distribution patterns of PNO3 under different environmental conditions.

How to cite: Qin, Y., Wang, H., Fan, S., Brown, S., and Lu, K.: Enhanced nocturnal oxidation chemistry in the upper mixing layer of megacities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3493, https://doi.org/10.5194/egusphere-egu25-3493, 2025.

EGU25-3673 | ECS | Posters on site | AS3.36

Accurately Predicting Spatiotemporal Variations of Near-Surface Nitrous Acid (HONO) Based on a Deep Learning Approach 

Xuan Li, Can Ye, Keding Lu, Chenghao Wang, and Yuanhang Zhang

Gaseous nitrous acid (HONO), a critical precursor of hydroxyl radicals (OH), plays a key role in the atmosphere’s oxidizing capacity, driving the production of secondary pollutants. However, large uncertainties in its formation and removal mechanisms impede accurate simulation of HONO levels using chemical transport models (CTMs). In this study, a deep neural network (DNN) model was established based on routine air quality data (NO2, CO, O3, PM2.5) and meteorological parameters (temperature, relative humidity, solar zenith angle and season) collected from four typical megacity clusters in China. The DNN model exhibited robust performance on both train sets (slope = 1.0, r2 = 0.94, RMSE = 0.29 ppbv) and two independent test sets (slope = 1.0, r2 = 0.79, RMSE = 0.39 ppbv). It demonstrated excellent capability in reproducing the spatial temporal variations of HONO and outperformed an observation-constrained box model incorporated with newly proposed HONO formation mechanisms. Nitrogen dioxide (NO2) was identified as the most impactful features for HONO prediction using the SHapely Additive exPlanation (SHAP) approach, highlighting the contribution of NO2 conversion in HONO formation. The DNN model was applied to predict future change of HONO levels under different NOx mitigation scenarios, which is expected to decrease 27-44% under 30-50% NOx reduction, consistent with the box model outputs. These results suggest a dual effect brought by NOx abatement, leading to not only reduction of O3 and nitrate precursors but also decrease in HONO levels and hence primary radical production rates. The model was further employed to construct an hourly-resolved nationwide HONO dataset for China spanning 2015-2023, offering a valuable tool for constraining ozone production in the CTMs.

The construction and application of the DNN model has been published on Environ. Sci. & Tech. (Environ. Sci. Technol. 2024, 58, 29, 13035–13046).

How to cite: Li, X., Ye, C., Lu, K., Wang, C., and Zhang, Y.: Accurately Predicting Spatiotemporal Variations of Near-Surface Nitrous Acid (HONO) Based on a Deep Learning Approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3673, https://doi.org/10.5194/egusphere-egu25-3673, 2025.

EGU25-3713 | ECS | Posters on site | AS3.36

Photolysis of atmospherically important carbonyls: Quantum yield measurements using an NO radical tracer method 

Ruth Winkless, Andrew Rickard, and Terry Dillon

Carbonyls are an important class of volatile organic compounds (VOC) in the atmosphere, being both directly emitted and produced by the oxidation of other VOCs. UV-B carbonyl photolysis produces radicals and so is an important driver of atmospheric radical cycles, that are a key route for the breakdown of primary pollutants and formation of secondary pollutants such as ozone and organic aerosol.

However, photochemical data concerning atmospheric photolysis of carbonyl compounds (i.e. photolysis cross-sections and quantum yields) are limited, and air quality research tools such as the Master Chemical Mechanism (MCM; mcm.york.ac.uk) must rely on using parameters from a small number of surrogate compounds to estimate photolysis rates for a larger suite of photo-labile VOCs.

To address this, we have developed a new laboratory flow reactor that utilises UV-LED technology to study photolysis quantum yields. This uses nitric oxide as a tracer for the peroxy radical photoproducts, assisted by a zero-dimensional chemical box model of the reactor system. Preliminary results for acetaldehyde and butanone show reasonable agreement with literature values, and the technique is fast and relatively easy to apply to a range of previously understudied compounds such as longer chain and branched ketones.

A wider understanding of the structure-reactivity trends of carbonyl quantum yields will improve atmospheric modelling capabilities, including better predictions of atmospheric impacts on air quality and human health.

How to cite: Winkless, R., Rickard, A., and Dillon, T.: Photolysis of atmospherically important carbonyls: Quantum yield measurements using an NO radical tracer method, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3713, https://doi.org/10.5194/egusphere-egu25-3713, 2025.

EGU25-5603 | Posters on site | AS3.36

Global southward shift in anthropogenic emisisons enhance tropospheric hydroxyl radicals during 1999-2019 

Yu Zhu, Lu Shen, Gang Liu, and Shushi Peng

The hydroxyl radical (OH), the main atmospheric oxidant, removes most pollutants including potent greenhouse gas methane. However, its short lifetime precludes direct observational quantification, so its temporal variability is poorly understood. Here, we used a three-dimensional chemical transport model GEOS-Chem, to investigate global tropospheric OH concentrations changes (ΔOH) from 1999 to 2019, driven by nitrogen oxides and carbon monoxide. We showed that ΔOH relative to 1999 increased rapidly from 2000 to 2008, dropped until 2010 and then continued to grow from 2011 to 2019, culminating in a 4.7% increase by 2019. The increase in ΔOH is primarily attributed to emissions from land (63%), followed by emissions from aircraft (24%) and shipping (13%). Notably, the tropics, particularly East Asia, Southeast Asia, South Asia, and Central America, contributed 74% of the global ΔOH burden in 2019. We also performed fractional simulations to separate the influence of land emissions influence from changes in the spatial distribution (LandS) and magnitude of emissions (LandM). We found that as land NOx emissions shifted equatorward from middle and high latitudes to low latitudes, the influence of landS increased persistently, exceeding LandM by 2014, and the relative contribution of LandS to ΔOH due to land emissions reached 58% in 2019. Looking forward, with the continued global southward shift in anthropogenic emissions, the role of LandS in global OH levels should not be overlooked. These insights underscore the need to consider anthropogenic emission patterns in projecting future OH concentrations and developing climate mitigation strategies.

How to cite: Zhu, Y., Shen, L., Liu, G., and Peng, S.: Global southward shift in anthropogenic emisisons enhance tropospheric hydroxyl radicals during 1999-2019, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5603, https://doi.org/10.5194/egusphere-egu25-5603, 2025.

EGU25-5762 | ECS | Posters on site | AS3.36

The development of Open path cavity-enhanced absorption spectroscopy for detecting ambient nitrate radicals 

Yiming Wang, Haichao Wang, Xiaorui Chen, and Shaojia Fan

Nocturnal oxidation driven by nitrate radicals is an important process in atmospheric chemistry, regulating the fate of volatile organic compounds and nitrogen oxide, and affecting the particulate pollution levels. While detecting NO3 is challenging due to its extremely low concentration. Currently, techniques such as Cavity Ring-Down Spectroscopy (CRDS) and Cavity-enhanced absorption Spectroscopy (CEAS) are widely used in NO3 measurement but suffer from the sampling loss due to its high reactivity. Here, we try to develop an open CEAS system to detect the ambient NO3, which eliminates the sampling loss. However, this method has its technical challenges, including the interferences of water absorptions during the NO3 absorption window near 662 nm and the effects of particle extinction and relative humidity and temperature during the field observation. We applied a small cavity cage (~40 cm high reflectivity mirror distance) during the hardware design, which features great stability. In addition, we calculated the real-time water vapor cross-section by measuring the ambient temperature and relative humidity to retrieve the water vapor concentration with high accuracy. And we proposed an I0-database method to eliminate the effects of particle extinction and variations in environmental meteorological conditions. Finally, we will present the instrumental performance in the laboratory tests and field applications.

How to cite: Wang, Y., Wang, H., Chen, X., and Fan, S.: The development of Open path cavity-enhanced absorption spectroscopy for detecting ambient nitrate radicals, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5762, https://doi.org/10.5194/egusphere-egu25-5762, 2025.

EGU25-7156 | ECS | Orals | AS3.36 | Highlight

Biogenic Emissions Modulate the Tropospheric Hydroxyl Radical (OH) Response to Climate Warming 

Qindan Zhu, Nicole Neumann, Arlene Fiore, Robert Pincus, Jian Guan, George Milly, Clare Singer, Brian Medeiros, and Paolo Giani

The hydroxyl radical (OH) sets the oxidative capacity of the atmosphere and determines the lifetime of reactive greenhouse gases such as methane (CH4). The response of OH to climate warming is influenced by uncertain and compensating processes involving weather-sensitive chemistry and emissions. In this study, we extend the idealized aquaplanet configuration of the Community Earth System Model (CESM) Community Atmosphere Model version 6 (CAM6) to include atmospheric chemistry (“AquaChem”).  Beyond the aquaplanet’s zonally symmetric sea surface temperatures (SSTs) and lack of seasonality, we further simplify the spatial variability of trace gas and aerosol emissions. We show that the AquaChem configuration generates a robust OH chemical budget, including both production and loss pathways, with relatively short simulations. Thus, the AquaChem model serves as an effective tool for rapidly assessing the sensitivity of OH chemistry, including both production and loss pathways. Rapid convergence allows us to assess the sensitivity of OH chemistry to surface warming.  The strongest direct response in OH to increased surface temperatures is an increase in “primary” OH production due to higher water vapor concentrations. We then test the sensitivity of OH sources and sinks to different assumptions regarding the response of emissions to rising temperatures.  AquaChem simulations indicate that biogenic emissions are a dominant factor influencing the OH response to climate warming. In tropical regions, climate warming enhances biogenic emissions and increases the OH loss rate, outweighing the increase in OH production resulting from rising water vapor and resulting in a decrease in OH abundance.

How to cite: Zhu, Q., Neumann, N., Fiore, A., Pincus, R., Guan, J., Milly, G., Singer, C., Medeiros, B., and Giani, P.: Biogenic Emissions Modulate the Tropospheric Hydroxyl Radical (OH) Response to Climate Warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7156, https://doi.org/10.5194/egusphere-egu25-7156, 2025.

Nitryl chloride (ClNO₂), an important precursor of chlorine radicals (Cl•), significantly enhances atmospheric oxidative capacity (AOC) during early morning hours. Previous studies have shown that ClNO₂ exhibits distinct vertical characteristics, with concentrations typically higher in coastal areas, raising concerns about chlorine-induced pollution. This study investigates the vertical formation of ClNO₂ in the Pearl River Delta (PRD), focusing on the contribution of sea spray aerosols (SSA). Using field observations and WRF-CMAQ model simulations, we assess the impact of SSA on nocturnal heterogeneous reactions driving ClNO₂ formation. The observations show that ClNO₂ mixing ratios are significantly higher in the upper boundary layer (200 m) compared to surface measurements, with peak mixing ratios occurring in the early morning. Air mass trajectory analysis shows that the marine air masses are primarily responsible for elevated ClNO₂ levels aloft. The maximum contribution of SSA to ClNO₂ yield is found to be more than 97% of the total yield. Process analysis identifies the upper boundary layer as the critical region for ClNO₂ formation, with SSA playing a dominant role. Moreover, SSA not only enhances ClNO₂ production but also increases the mixing ratios of chlorine and hydroxyl radicals at higher altitudes the following day (400 m), significantly boosting AOC, with an increase in AOC of up to 10%. These findings highlight the pivotal role of SSA in modulating vertical ClNO₂ formation and its broader impacts on regional air quality, particularly in coastal areas.

How to cite: Zhu, Y. and Liu, Y.: Significant contributions of sea spray aerosol to vertical ClNO2 formation over coastal South China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7933, https://doi.org/10.5194/egusphere-egu25-7933, 2025.

EGU25-9998 | ECS | Posters on site | AS3.36

Exploring the influence of OH fields and secondary CO production on CO emission estimates 

Johann Rasmus Nüß, Nikos Daskalakis, Angelos Gkouvousis, Maria Kanakidou, Maarten C. Krol, and Mihalis Vrekoussis

Inverse modeling can provide valuable insights into the sources of atmospheric tracers based on observations and a set of boundary conditions. However, biases in these boundary conditions can lead to biases in the optimized emissions. In this study, we present a series of global inversion experiments of carbon monoxide (CO) emissions using the TM5-4dvar inverse modeling suit constrained by satellite data from the TROPOspheric Monitoring Instrument (TROPOMI) and surface flask measurements from NOAA. These experiments are designed to systematically assess the impact of different boundary conditions, with a particular focus on hydroxyl radical (OH) distributions, a key determinant of both the sources and sinks of CO.

Methyl chloroform (MCF) measurements are commonly used to constrain global atmospheric OH climatological fields. We find that our OH fields that are modeled with global atmospheric chemistry calculations are biased high. Despite this bias, these OH fields often provide more realistic lateral distributions than climatological OH fields, particularly in the tropical boundary layer. Another critical boundary condition for inverse modeling of CO is its secondary production from Volatile Organic Compounds (VOCs) and methane. Due to the challenges of directly measuring secondary CO production, model-based estimates are used instead.

Our results show that combining modeled secondary CO production estimates with modeled OH fields leads to a closed budget, reducing aliasing across emission categories and enhancing confidence in the optimized anthropogenic and biomass burning emissions. Although the individual budget terms of both the secondary production and the chemical loss of CO may be overestimated, their combined effect yields realistic steady-state CO mixing ratios, as validated by TROPOMI CO observations. This study emphasizes the critical need for improved OH fields to accurately estimate CO emissions, and advances the understanding of potential biases in future inversions.

How to cite: Nüß, J. R., Daskalakis, N., Gkouvousis, A., Kanakidou, M., Krol, M. C., and Vrekoussis, M.: Exploring the influence of OH fields and secondary CO production on CO emission estimates, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9998, https://doi.org/10.5194/egusphere-egu25-9998, 2025.

EGU25-10283 | ECS | Posters on site | AS3.36

Accurate Elucidation of Oxidation Under Heavy Ozone Pollution: A Full Suite of Radical Measurement In the Chemical-complex Atmosphere 

Guoxian Zhang, Renzhi Hu, Pinhua Xie, Changjin Hu, and Wenqing Liu

A full suite of radical measurements (OH, HO2, RO2, and kOH) was established in Yangze River Delta (YRD) region to accurately elucidate the limitations of oxidation processes in the chemical-complex atmosphere. The diurnal peaks of radicals exhibited considerable variations in 3.6 to 27.1×106 cm-3 for OH, 2.1 to 33.2×108 cm-3 for HO2, and 4.9 to 30.5×108 cm-3 for RO2. The simulated results provided by the RACM2-LIM1 mechanism failed to adequately match the observed data both in radical concentration and experimental budget at a heavy ozone pollution episode. Sensitivity tests utilizing a comprehensive set of radical measurements revealed that the reactive aldehyde chemistry effectively complements the regeneration of OH radicals with 4.4% - 6.0% compared to the base scenario, while the concentrations of HO2 and RO2 radicals have shown increments of about 7.4% and 12.5%, respectively. The incorporation of larger alkoxy radicals stemming from monoterpenes has refined the consistency between measurements and modeling in the context of ozone production under elevated NO levels, diminishing the disparity from 4.17 to 2.33. Moving forward, by implementing a comprehensive radical detection approach, further investigations should concentrate on a broader range of OVOCs to rectify the imbalance associated with RO2 radicals, thereby providing a more precise understanding of oxidation processes during severe ozone pollution episodes.

How to cite: Zhang, G., Hu, R., Xie, P., Hu, C., and Liu, W.: Accurate Elucidation of Oxidation Under Heavy Ozone Pollution: A Full Suite of Radical Measurement In the Chemical-complex Atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10283, https://doi.org/10.5194/egusphere-egu25-10283, 2025.

EGU25-10586 | ECS | Posters on site | AS3.36

Long-term field measurements of OH reactivity using laser flash photolysis coupled with time-resolved broadband UV absorption spectroscopy 

Thomas Luke, Midhun George, Ambili Vallipparambil Babu, Siqi Hou, Thomas Wynn, William Bloss, Lisa Whalley, Dwayne Heard, and Daniel Stone

Air quality is an important issue to human health and the climate. Poor air quality has been proven to be a risk factor in a wide range of cardiovascular and respiratory diseases, and it contributes to 6.9 million premature deaths worldwide [1]. Air quality also has complex links to climate change, with primary and secondary pollutants affecting the radiative forcing on Earth [2]. Therefore, accurate measurements of air pollutants, alongside understanding of their emissions and atmospheric sinks, is crucial information for informing policy on air quality.

Volatile organic compounds (VOCs), emitted from both anthropogenic and biogenic sources, impact air quality, as they are involved in processes that produce secondary pollutants like ozone and secondary organic aerosol. There is an estimated >100,000 VOCs found in ambient air [3], and they cannot all be measured using traditional direct techniques such as gas chromatography and mass spectrometry. As an alternative to measuring the total quantities of each individual VOC, techniques used to measure OH reactivity have been developed over the last 25 years. OH reactivity (kOH), the inverse of the chemical lifetime of OH, provides a quantitative measure of the total reactive pollutant loading in an air mass. This information can be used to determine the extent to which measured OH sinks contribute to the OH loss rate and can be used to determine the total impact of VOCs. The measured OH reactivity can be compared to modelled OH reactivity to assess the completeness of models used to assess and predict air quality. Current instruments designed for measurements of OH reactivity are precise and accurate but are often technically challenging and expensive, which limits current OH reactivity measurements to short intensive field campaigns.

We have recently developed an instrument designed to make continuous long-term measurements of OH reactivity based on laser flash photolysis coupled with time-resolved broadband UV absorption spectroscopy. We will present measurements of OH reactivity made in Leeds, UK, using the UV absorption instrument, as well as results obtained using an instrument based on laser-induced fluorescence (LIF) spectroscopy [4] during an intercomparison exercise. The instruments both sampled ambient air from an urban site at the University of Leeds during February and March 2024. Results from the intercomparison will be presented, which indicated that OH reactivity varied between 0.5 and 45.5 s-1, with a mean reactivity of 9.7 s-1. It was found that the agreement between instruments was good and that the new instrument can successfully measure OH reactivity over a range of environmental conditions.

The instrument has been successfully deployed in the Birmingham Air Quality Supersite at the University of Birmingham, UK since November 2024. Initial measurements from this long-term campaign will be presented, alongside detailed chemical modelling using the Master Chemical Mechanism.

References:

[1]   World Health Organisation, https://www.who.int/news-room/fact-sheets/detail/ambient-(outdoor)-air-quality-and-health [Accessed 20/07/2024] (2022).

[2]   Intergovernmental Panel on Climate Change, Camb. Uni. Press, 923–1054 (2023).

[3]   A. H. Goldstein & I. E. Galbally, Env. Sci. & Tech. 41(5), 1514-1521 (2007)

[4]   D. Stone et al., Atmos. Meas. Tech, 9 2827–2844 (2016).

How to cite: Luke, T., George, M., Vallipparambil Babu, A., Hou, S., Wynn, T., Bloss, W., Whalley, L., Heard, D., and Stone, D.: Long-term field measurements of OH reactivity using laser flash photolysis coupled with time-resolved broadband UV absorption spectroscopy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10586, https://doi.org/10.5194/egusphere-egu25-10586, 2025.

Both sulfuric acid (H2SO4) (SA) and hydroxyl radical (OH) play critical roles in the atmospheric chemistry processes. In most environments, from the pristine Tibet plateau to highly populated megacities, SA is the decisive nucleation precursor. OH, on the other hand, dominates the atmospheric oxidation capacity under most circumstances. Therefore, accurate measurements of SA and OH are important for atmospheric chemistry studies. This study developed an instrument based on chemical ionization mass spectrometry (CIMS) to measure SA and OH in the air simultaneously. The working principle was based on the nitrate (NO3-) CIMS. SA was ionized by NO3- directly to form bisulfate anion (HSO4-), which was then detected with a high-resolution time-of-flight mass spectrometer (HR-ToF-MS). OH was first converted into SA by excess sulfur dioxide (SO2) and then detected as SA total, which is the sum of ambient SA, OH-converted SA, and background signals due to the high concentration of SO2 (~1ppmv). In order to minimize wall losses, a 3-cm ID, 50-cm long sample inlet was used, and a blower was employed to suck in ambient air at ~100 L min-1. Two 1/16 in gas injectors were installed at the front end of the inlet and 30 cm downstream of the front injector. The instrument was operated in three sequential modes, i.e., the ambient SA mode, OH mode, and background (BG) mode. No reagent gases were injected in the SA mode, and ambient SA was detected directly. During the OH mode, SO2 was injected into the sample flow through the first injector. For the BG mode, both SO2 and pure propane (C3H8) were injected into the sample flow through the first injector. Since C3H8 concentration was about a few hundred ppmv, nearly two orders of magnitude higher than SO2, OH was completely scavenged during the BG mode, and only ambient SA and SO2 BG were detected. A constant stream of propane was injected into the inlet through the second injector to prevent further free radical cycling. Therefore, the difference between the OH mode and the BG mode was the ambient OH signal. Each mode was operated for about 3-min, and the 9-min detection limits of SA and OH were ~2×105 molecules cm-3 and 4×105 molecules cm-3 (3σ), respectively. The instrument was calibrated by known concentrations of SA standards generated by a low-pressure Hg-lamp, the intensity of which was determined by the N2O-actinometry. The instrument was field tested in a mountain site located in Longquan Mountain, Chengdu, China. Both SA and OH showed clear diurnal patterns following the solar radiation, ranging from less than the detection limit to a few 106 molecules cm-3. Further intercomparison between the measurements and model simulations was also conducted to verify the measurement results.

How to cite: Zheng, J. and Ma, Y.: A versatile instrument for simultaneous detection of atmospheric H2SO4 and OH radicals, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10634, https://doi.org/10.5194/egusphere-egu25-10634, 2025.

Inlet-pre-injectors (IPIs) are now increasingly used by the HOx measurement community (e.g. Mao et al., 2012; Novelli et al., 2014; Woodward-Massey et al., 2020; Cho et al., 2021) when measuring ambient OH by laser-induced fluorescence (LIF) to provide an interference-free measurement.

Traditionally, OH is detected by LIF in a low-pressure detection cell by tuning the laser wavelength on and off an OH transition to distinguish the OH fluorescence signal from the instrument background signal which is comprised of laser and solar scatter and any detector dark counts. However, this method of OH detection, which is often known as OHWAVE, does not allow the signal contribution from any OH generated within the detection cell to be differentiated from the ambient OH signal. The injection of propane (C3H8) or perfluoropropene (C3F6) scavenger via an IPI before the OH sampling nozzle leads to rapid removal of ambient OH and provides a measure of the instrument background signal whilst tuned to the OH transition. By this method, which is often known as OHCHEM, any signal from OH generated internally within the detection cell contributes to the background signal and so is distinguished from the ambient OH signal.

The concentration of OH scavenger injected via the IPI before sampling by the LIF instrument must be high enough to rapidly remove ambient OH, but not too high such that there is also removal of any internally-generated OH. A point-source of OH, generated by a Hg lamp in a humidified zero air flow, can be used to optimise the concentration of scavenger required. Here we will show, however, that higher concentrations of scavenger are often required to fully remove ambient OH as the scavenger must out-compete the reactions occurring under ambient conditions (e.g. HO2+NO) that are continually producing OH within the IPI.

Taking examples from previous OH measurement campaigns in two contrasting environments (forested and urban), the efficiency of an IPI to remove ambient OH is investigated using a detailed chemistry box-model based on the Master Chemical Mechanism (MCMv3.3.1) and constrained to measurements made during the campaigns. Taking typical residence times between scavenger injection and sampling by the low-pressure LIF detection cell, and varying the concentration of scavenger added, we show that under certain scenarios, >25 % of ambient OH could remain and may be erroneously considered as an OH interference.

Cho et al., Atmospheric Measurement Techniques, 14, 1851 – 1877, 2021

Mao et al., Atmospheric Chemistry and Physics, 12, 8009 – 8020, 2012

Novelli et al., Atmospheric Measurement Techniques, 7, 3413 – 3430, 2014

Woodward-Massey et al., Atmospheric Measurement Techniques, 13, 3119 – 3146, 2020

How to cite: Whalley, L. and Heard, D.: A modelling study investigating the efficiency of inlet-pre-injectors in removing ambient OH under different atmospheric conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10751, https://doi.org/10.5194/egusphere-egu25-10751, 2025.

EGU25-11702 | ECS | Posters on site | AS3.36

Atmospheric Nitrous Acid (HONO) in Contrasting Environments 

xuelian zhong, hengqing shen, and likun xue

Nitrous acid (HONO) is a crucial precursor to hydroxyl radical (OH) in the atmosphere and significantly influences atmospheric photochemical processes. Despite extensive field observations, the quantitative understanding of HONO formation processes in varying environments remains elusive, particularly due to the divergent parameters used in different studies that have led to contradictory conclusions. This study measured HONO at four sites characterized by contrasting environments: an urban site in the Yellow River Delta, a mountain site in the North China Plain, and two coastal sites at varying distances from the sea in Qingdao. The HONO concentration at the urban site is the highest, with peaks occurring at night, consistent with previous observations in other urban areas, yet markedly different from the daytime HONO peaks observed at other three clean sites. Using an observation-based model incorporated with unified parametrizations, we identify the dominant HONO formation pathways in these sites. Results show that the model effectively reproduces HONO concentrations and diurnal variations at both urban and mountainous sites. In urban areas, HONO formation is primarily driven by the heterogeneous conversion of NO2 and the photolysis of particulate nitrate, while in the polluted mountainous region, the photolysis of nitrate plays a more significant role, with vertical transport potentially contributing to morning HONO increases. However, the model could not replicate daytime HONO peaks at the two coastal sites, suggesting the presence of an unidentified or underestimated marine HONO source. At all four sites, HONO contributes significantly to atmospheric OH radicals and ozone production, and the missing marine source may affect evaluations of its influence in coastal regions. In summary, this study provides a comprehensive analysis of HONO sources in contrasting environments, underscoring the need for further observations, especially in clean marine/coastal atmospheres.

How to cite: zhong, X., shen, H., and xue, L.: Atmospheric Nitrous Acid (HONO) in Contrasting Environments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11702, https://doi.org/10.5194/egusphere-egu25-11702, 2025.

EGU25-12714 | ECS | Posters on site | AS3.36

Investigating HO2 uptake onto the surface of secondary organic  

Abigail McConnell, Daniel Stone, and Dwayne Heard

The concentrations of HO2, a critical radical in the atmosphere, are often overestimated in atmospheric models (1). These discrepancies have sometimes been attributed to the heterogeneous uptake to atmospheric aerosols.

However, the correct treatment of heterogeneous chemistry in models is a significant source of uncertainty, partly due to the complexity of atmospheric aerosols and the need for laboratory experiments to formulate a robust parameterisation of HO2 uptake. There is a significant lack of experimental data for the uptake coefficient γ(HO2) of HO2 onto secondary organic aerosols (SOAs), even though they represent a high proportion of atmospheric aerosols and a significant fraction of particulate matter below 2.5 μm (PM2.5).

We report the first γ(HO2) measurements onto SOAs over a range of relative humidities (30 - 85 %). Atmospherically relevant SOA has been produced in a Potential Aerosol Mass Chamber (PAM) from the oxidation, by OH and ozone, of the volatile organic compounds α-pinene, ∆-limonene, 1,3,5 – trimethyl benzene (TMB) and toluene.  An aerosol flow tube coupled to a Fluorescence Assay Gas Expansion (FAGE) detection cell, which utilises laser-induced fluorescence (LIF) spectroscopy, is used to measure the uptake of gas-phase HO2 onto the aerosols, with a limit of detection of γ(HO2) = 0.003.

Results show that the aerosol liquid water (ALW) content plays an important role in heterogeneous reactions by enhancing HO2 uptake onto aerosols. The measured γ(HO2) was low (γ ≤ 0.004) for TMB and toluene SOA and undetectable for both α-pinene and ∆-limonene, and no correlation was observed between RH and γ(HO2). The aerosol size distribution of the SOA remained constant over the range of relative humidities, suggesting the RH had little effect on the ALW of purely organic aerosols. Whereas, when ammonium sulfate seed aerosols are added to enhance SOA formation, the measured γ(HO2) for toluene-derived SOA increases from 0.006 to 0.03 with an increase in RH from 38 – 84 %. The increase in the geometric mean of the toluene-derived SOA at higher RH suggests that the ALW increases. Thus, the presence of seed particles results in a more significant γ(HO2), which increases with RH and potentially impacts the atmospheric abundance of HOx.

 

 

1. Dyson, Joanna E., et al. "Impact of HO2 aerosol uptake on radical levels and O3 production during summertime in Beijing." Atmospheric Chemistry and Physics Discussions(2022): 1-43.

How to cite: McConnell, A., Stone, D., and Heard, D.: Investigating HO2 uptake onto the surface of secondary organic , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12714, https://doi.org/10.5194/egusphere-egu25-12714, 2025.

Nitrate radicals (NO3) in the nocturnal boundary layer are key oxidants that influence nighttime atmospheric oxidation capacity and the nitrogen cycle. However, their low concentrations, short lifetimes, and complex nighttime chemistry pose challenges for large-scale spatiotemporal observations. In this study, we couple a machine learning model with the CMAQ model and historical observation data to predict NO3 over the long term. This approach combines an exact physical-chemical framework with observational data support to better capture the spatial and temporal characteristics of NO3. Our results show that: (1) CMAQ accurately simulates NO2 and O3 concentrations and also performs well for N2O5, indicating that the nighttime NO3 reaction framework in CMAQ is correct. (2) Combined with the CMAQ result, the stacking model improves the R of NO3 predictions by an average of 0.17 compared with single models, and its SHAP results align with current atmospheric chemistry. (3) After predicting NO3 levels and comparing summer and winter conditions in Shanghai and Beijing, our results reveal a notable decrease in NO3 in Shanghai during summer, likely due to declining nighttime O3. However, reduced heterogeneous hydrolysis during Shanghai’s winter nights may lead to a slight rise in NO3 concentrations. Additionally, NO3 in Beijing do not show a strong decrease and even increases slightly.

How to cite: Fu, W., Qin, M., and Hu, J.: Prediction of NO3 Radical Concentrations from 2015 to 2020 in Beijing and Shanghai Based on Air Quality Models and Machine Learning Methods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12750, https://doi.org/10.5194/egusphere-egu25-12750, 2025.

EGU25-12780 | Orals | AS3.36

Ozone Formation under high NOx conditions: Insights from the AEROMMA NYC-METS field campaign 

Ezra Wood, Khaled Joy, Andrew Lindsay, Lee Feinman, Rob Roscioli, Conner Daube, Megan Claflin, Manjula Canagaratna, Brian Lerner, Daniel Blomdahl, and Drew Gentner

Despite well over a half century of research, gaps remain in our understanding of ozone formation chemistry. Net ozone formation results from the oxidation of NO to NO2 by peroxy radicals (HO2 and RO2) followed by photolysis of NO2. Measurements of peroxy radicals made by several analytical methods over the past decade in numerous locations across the world have revealed discrepancies under high NOx conditions ([NO] > 1 ppb), with zero-dimensional models apparently underestimating peroxy radical concentrations and ozone production rates (P(O3)) by up to a factor of eight. These findings suggest that models may misidentify when ozone formation is NOx-limited vs. NOx-saturated (VOC-limited) and that our knowledge of the relevant reactions is incomplete. To investigate these anomalously high P(O3) values at high NOx, we used the Drexel University Ethane Chemical AMPlifier (ECHAMP) instrument to measure total peroxy radicals at a roof-top site in Manhattan (NYC) as part of the NOAA AEROMMA/NYC-METS project.  A wide assortment of other measurements were made by spectroscopic and mass spectrometric methods. We will present results from this field project with special emphasis on our measurements during a few “high-NOx” periods (roughly defined as daytime periods with NO mixing ratios greater than 1 ppb).

How to cite: Wood, E., Joy, K., Lindsay, A., Feinman, L., Roscioli, R., Daube, C., Claflin, M., Canagaratna, M., Lerner, B., Blomdahl, D., and Gentner, D.: Ozone Formation under high NOx conditions: Insights from the AEROMMA NYC-METS field campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12780, https://doi.org/10.5194/egusphere-egu25-12780, 2025.

EGU25-14586 | Orals | AS3.36

Vertical changes in volatile organic compounds (VOCs) and impacts on ozone formation 

Bin Yuan, Xiaobing Li, Xin Song, and Yibo Huangfu

Volatile organic compounds (VOCs) play crucial roles in regulating the photochemical formation of ozone. However, limited knowledge on the interactions between vertical VOCs change and ozone formation in the planetary boundary layer (PBL) has hindered effective ozone control strategies, particularly in large cities. To address concern, we investigated the vertical changes in concentrations, compositions, and key drivers of a large suite of VOCs using online gradient measurements taken from a 325 m tall tower in urban Beijing, China. The impacts of these vertical VOC variations on ozone formation were also analyzed using box model simulations. We find that VOCs exhibited differentiated vertical gradients due to their differences in both sources and chemical reactivities, along with the diurnal PBL evolution. In daytime, reactive VOCs (e.g., hydrocarbons) are rapidly oxidized and their concentrations generally decreased with height, accompanied by the formation and accumulation of oxygenated VOCs (OVOCs) in the middle and upper layers. We also find that the formation of ozone responds positively to changes in both NOx and VOCs. As a result, the production rate of ozone declines with height due to the simultaneous decreases in concentrations of reactive VOCs and NOx, but remains high in the middle and upper layers due to the presence of high OVOCs concentrations. Therefore, careful consideration should be given to the vertical variations in both ozone production rates and formation regimes in the whole PBL when developing regional ozone control strategies.

How to cite: Yuan, B., Li, X., Song, X., and Huangfu, Y.: Vertical changes in volatile organic compounds (VOCs) and impacts on ozone formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14586, https://doi.org/10.5194/egusphere-egu25-14586, 2025.

EGU25-14854 | ECS | Posters on site | AS3.36

Contributions of Anthropogenic Chlorine Emissions to secondary pollutions in China 

Ao Shen, Yiming Liu, and Qi Fan

Chlorine species play a crucial role as precursors to Cl radicals, which can significantly impact the atmospheric oxidation capacity and influence the levels of trace gases related to climate and air quality. We developed The Anthropogenic Chlorine Emission Inventory for China (ACEIC), which was the first chlorine emission inventory for China based on local data, and explored the impact of chlorine species emissions on secondary pollutants in 2019 in China using the CMAQ model. Considering chlorine emissions, the concentration of chlorine radicals (Cl·) in China increased by about 1000 molecules/cm3 on average, with a maximum increase of more than 6000 molecules/cm3 in major cities. Cl2 and HOCl emissions were the most important contributors to the increase of Cl·, with both Cl2 and HOCl emissions originating mainly from the residential sector. Regarding monthly variation, the increase in Cl· was most significant in summer due to intensified human activities. Regarding daily variation, the increase in Cl· peaked around 9 am and decreased to zero at night. Process analyses showed that the main reactions affecting the change in Cl· were the photolysis reactions of Cl2 and HOCl and the consumption reactions of Cl· and VOCs. As an important precursor of Cl·, the concentration of Nitryl chloride (ClNO2) in China increased by about 50 ppt on average, with a maximum increase of more than 150 ppt in major cities. HCl and fine particulate Cl- emissions were the most important contributors to the increase of ClNO2. The increase in ClNO2 was most significant in winter, peaked around 6 am and decreased to zero at daytime. Process analysis identified the upper boundary layer as the critical region for ClNO2 formation. Chlorine emissions caused some increase in O3 concentration. Maximum Daily 8-hour Average O3 (MDA8 O3) concentration increased by about 1 ppb, with O3 increasing much higher in winter than in summer. In the daily variation, the ozone increase was most significant at 12 am, with a maximum increase of more than 1.5 ppb. These findings highlight the significant contribution of chlorine emissions to secondary pollutants and can aid in the formulation of emission control strategies to mitigate secondary pollution in China.

How to cite: Shen, A., Liu, Y., and Fan, Q.: Contributions of Anthropogenic Chlorine Emissions to secondary pollutions in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14854, https://doi.org/10.5194/egusphere-egu25-14854, 2025.

EGU25-15619 | ECS | Orals | AS3.36

Towards automated inclusion of representative autoxidation chemistry in explicit models 

Lauri Franzon, Richard Valorso, Bernard Aumont, Marie Camredon, Julia Lee-Taylor, John Orlando, Anni Savolainen, Siddharth Iyer, Matti Rissanen, and Theo Kurtén

RO2 autoxidation is the most important class of chemical reactions for modelling instantaneous formation of low-volatility organics in the atmosphere. However, systematic inclusion of these reactions in atmospheric chemistry models is tricky for reasons both fundamental (huge environmental variability in the importance of individual reactions) and technical (reaction rate data relies on experiments on complex radicals with complex reaction branching). This being the case, automatic mechanism generation based on structure-activity relationships (SAR) are crucial for the development of autoxidation-including atmospheric chemistry models. We thus aim to update the mechanism generator GECKO-A (Aumont et al, ACP, 2005) with an autoxidation module based on up-to-date SARs for RO2 H-shift (Vereecken & Nozière, ACP, 2020), ring-closure (Vereecken et al, PCCP, 2021), as well as linear RC(O)O2 H-shift reactions (Seal et al, PCCP, 2023).

At the meeting we will briefly present our strategy for adapting autoxidation mechanisms for different environments and discuss the impact of H-scrambling isomerisations on RO2 chemistry, as these are the largest challenges in developing the autoxidation module. In addition, we present our computational efforts to expand the above SARs in order to more accurately represent the most rapid reactions. Our calcualtions include H-shifts from aldehyde groups in RC(O)O2, ring-closures and allylic H-shifts in unsaturated RC(O)O2, and H-shifts from enol groups in RO2, which have all been found to be exceptionally rapid in previous studies (Rissanen et al, JPCA, 2015; Ojala et al, In Preparation; Peeters & Nguyen, JPCA, 2012). Out of these, we especially highlight the RC(O)O2 ring-closures, as this appears to be the main fate of unsaturated RC(O)O2 in most environments.

In summary, we are aiming to develop the most complete and chemically explicit autoxidation mechanism generator that can be achieved with our current knowledge, and we hope that the modelling community will make great use of it when more specialized truncated models are developed.

How to cite: Franzon, L., Valorso, R., Aumont, B., Camredon, M., Lee-Taylor, J., Orlando, J., Savolainen, A., Iyer, S., Rissanen, M., and Kurtén, T.: Towards automated inclusion of representative autoxidation chemistry in explicit models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15619, https://doi.org/10.5194/egusphere-egu25-15619, 2025.

EGU25-16213 | Posters on site | AS3.36

Volcanic vents – OH mixing ratios as in a Bunsen burner flame? 

Nicole Bobrowski, Gianluigi Ortenzi, Lucie Boucher, Johannes Degen, Andreas Engel, Bastien Geil, Giovanni Giuffrida, Melisende Metais-Bossard, Tanja Schuck, and Thorsten Hoffmann

Volcanic gas emissions influence the composition of the atmosphere and therefore also our climate. For some gas species, volcanoes represent even the most important natural source. In atmospheric research, however, volcanoes are often neglected as an important source of many gas species and are still little studied, partly also because of the challenges in terms of the necessary technology and logistics.

In volcanic gas mixtures near the source, very high OH mixing ratios (ppb-ppm) are often assumed, usually based on thermodynamic equilibrium calculations (e.g. Gerlach, 2004). However, no OH measurements have been successfully performed in such environments.

Here we report on CO/CO2 measurements in the downwind volcanic gas plume of Mount Etna, which were obtained by taking air core samples with an UAV and analysed immediately afterwards with Cavity Ring-Down Spectroscopy in July 2024 (T. Schuck et al., 2025). We relate these results to previous near-source CO/CO2 emission measurements and to calculated CO/CO2 emission ratios from petrological studies. The observed change of more than two orders of magnitude in the CO/CO2 ratio can only be explained by the oxidation of CO and therefore allows us to estimate the amount of OH necessary to explain the high proportion of CO oxidation. Our estimate based on kinetic chemistry, happening after the first seconds of the gas release, leads indeed to results of unusual high amounts of OH in the source region.

Gerlach, T. M. (2004). Volcanic sources of tropospheric ozone‐depleting trace gases. Geochemistry, Geophysics, Geosystems, 5(9).

Schuck, T., Degen J., Bobrowski, N., Metais-Bossard M., Boucher L., Chen, H., Geil, B.H., Giuffrida, G.B. van Heuven, S.,  Hoffmann, T., Ortenzi G., and Engel A. (2025). First deployment of a drone-borne active AirCore in a volcanic plume at Mount Etna, submitted to EGU

How to cite: Bobrowski, N., Ortenzi, G., Boucher, L., Degen, J., Engel, A., Geil, B., Giuffrida, G., Metais-Bossard, M., Schuck, T., and Hoffmann, T.: Volcanic vents – OH mixing ratios as in a Bunsen burner flame?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16213, https://doi.org/10.5194/egusphere-egu25-16213, 2025.

EGU25-16408 | Orals | AS3.36

Portable laser-flash photolysis Faraday rotation spectrometer for real-time in-situ measurement of total OH reactivity 

Bo Fang, Weixiong Zhao, Nana Wei, Weijun Zhang, and Weidong Chen

The total OH reactivity (kOH′), which is equal to the reciprocal of the lifetime (τOH) of the hydroxyl (OH) radical in the atmosphere, is an important parameter for quantitatively assessing the atmospheric oxidation capacity. Although kOH′ was first measured in the laboratory more than 20 years ago, the required instrumentation is costly and complex, and only a few research groups can perform such measurements. Long-term observation of kOH′ remains challenging and difficult to achieve. In this presentation, we report the development of a portable laser-flash photolysis Faraday rotation spectroscopy (LP-FRS) instrument for real-time and in-situ measurement of kOH′. OH decay is directly measured using a time-resolved FRS spectrometer at 2.8 μm. Since FRS relies on the detection of the rotation of the polarization state of the probe light induced by paramagnetic molecules in a longitudinal magnetic field, the laser noise and molecule interferences are significantly reduced, which enables the FRS system to directly and highly sensitive monitor OH concentration without chemical interferences. The LP-FRS instrument has a kOH detection precision of 1.0 s-1 with an averaging time of 300 s. The instrument’s optical box measures 130 cm × 40 cm × 35 cm, making its convenient for field applications.

How to cite: Fang, B., Zhao, W., Wei, N., Zhang, W., and Chen, W.: Portable laser-flash photolysis Faraday rotation spectrometer for real-time in-situ measurement of total OH reactivity, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16408, https://doi.org/10.5194/egusphere-egu25-16408, 2025.

EGU25-17088 | ECS | Posters on site | AS3.36

Investigating Isoprene Oxidation in the Upper Troposphere: Insights from Cold-Temperature Chamber Experiments 

Felix Kunkler, Philip Holzbeck, Douglas Russell, Jiali Shen, Bernhard Mentler, Armin Hansel, Jasper Kirkby, Xu-Cheng He, Joachim Curtius, Jos Lelieveld, and Hartwig Harder

Isoprene, the most abundantly volatile organic compound (VOC), plays a significant role in atmospheric chemistry, particularly in the upper troposphere. In the tropics, it is emitted in large quantities by rainforests. Driven by prevailing high solar radiation, temperature, and humidity, Isoprene rich air is transported from the boundary layer to the upper troposphere by deep convective systems. Without nighttime photo-oxidation, isoprene can accumulate in this region, where it reacts with hydroxyl radicals during the day, contributing to aerosol formation (Shen et al, 2024, Curtius et al., 2024). This study explores the oxidation processes of isoprene at low temperatures (-50°C), typical of the upper troposphere, with a focus on the effects of varying NOx concentrations (low and high NOx) on these mechanisms. Experiments were conducted in the CLOUD chamber at CERN, simulating these atmospheric processes under controlled conditions.

While previous research has largely focused on isoprene oxidation at relatively high near-surface temperatures, the chemistry at low temperatures, particularly radical recycling, has not been sufficiently studied. Our study's cold-temperature measurements are particularly relevant for understanding upper tropospheric processes. We aim to elucidate the oxidation mechanisms of isoprene by analyzing radical production, concentration, and recycling under various chemical conditions at low temperatures. The findings will enhance our understanding of atmospheric chemistry in the upper troposphere and improve the accuracy of climate and air quality models.

 

References:

Shen, J., et al. New particle formation from isoprene under upper-tropospheric conditions. Nature 636, 115–123 (2024).

Curtius, J., et al. Isoprene nitrates drive new particle formation in Amazon’s upper troposphere. Nature 636, 124–130 (2024).

How to cite: Kunkler, F., Holzbeck, P., Russell, D., Shen, J., Mentler, B., Hansel, A., Kirkby, J., He, X.-C., Curtius, J., Lelieveld, J., and Harder, H.: Investigating Isoprene Oxidation in the Upper Troposphere: Insights from Cold-Temperature Chamber Experiments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17088, https://doi.org/10.5194/egusphere-egu25-17088, 2025.

EGU25-17264 | ECS | Orals | AS3.36

Elucidating Tropospheric Radical Chemistry and Atmospheric Oxidation Capacity: Insights from the EXACT Campaign in China 

Xuefei Ma, Zhaofeng Tan, Keding Lu, Renzhi Hu, and Shengrong Lou

Atmospheric radicals are central to the oxidation capacity and self-cleansing ability of the troposphere, driving the formation of secondary air pollution and the removal of short-lived climate forcers such as methane (CH4) and hydrofluorocarbons (HFCs). Understanding radical chemistry is thus critical for air quality improvement and climate change mitigation. While tropospheric radical chemistry has been extensively studied since the 1990s, significant gaps remain, particularly in the underestimation of hydroxyl (OH) and hydroperoxyl (HO2) radicals under low- and high-NO concentration regimes, respectively. These gaps hinder the development of effective pollution control and climate mitigation strategies.

In this study, we introduce the Ensembled eXperiment of Atmospheric oxidation Capacity in the Troposphere (EXACT) campaign conducted in China. This comprehensive initiative employs state-of-the-art instrumentation to measure key radicals (OH, HO2, RO2, NO3) and their precursors, covering diverse chemical and environmental conditions across urban, regional, and background settings in the North China Plain. Seasonal campaigns conducted in autumn, winter, spring, and summer aim to unravel the molecular-level sources and transformation mechanisms of atmospheric radicals. The research further seeks to elucidate the evolution patterns and driving mechanisms of atmospheric oxidation in critical regions of China.

This presentation will provide an overview of the EXACT campaign design and methodology, alongside preliminary results and discussions from the completed autumn and winter campaigns. These findings offer new insights into diurnal radical sources, transformation pathways, and the broader implications for atmospheric oxidation dynamics in China.

How to cite: Ma, X., Tan, Z., Lu, K., Hu, R., and Lou, S.: Elucidating Tropospheric Radical Chemistry and Atmospheric Oxidation Capacity: Insights from the EXACT Campaign in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17264, https://doi.org/10.5194/egusphere-egu25-17264, 2025.

EGU25-17736 | ECS | Posters on site | AS3.36

Chemical budgets of OH, HO2+RO2 and H2SO4 in a sub-urban temperate forest near Paris 

Yang Jiao and Alexandre Kukui and the ACROSS Rambouillet Measurements Team

Understanding the OH and peroxy radical chemistry in different environments is essential to predict atmospheric lifetimes and chemical transformations of compounds emitted to the atmosphere of both biogenic and anthropogenic origin.  The extent to which insight into radical chemistry can be gained by comparing simulated and measured radical concentrations has been found to depend on the environment. In particular, significant discrepancies between modeled and measured OH and peroxy radical concentrations have been observed in forested regions characterized by relatively high VOCs and low NO concentrations. The objective of this study was to assess the importance of different radical production and loss processes as well as the role of OH in the production of sulfuric acid, a major precursor of newly formed atmospheric particles, in a sub-urban temperate forest.
Measurements were performed as part of the ACROSS project (Atmospheric ChemistRy Of the Suburban foreSt) during June-July of 2022 at a forested site in Rambouillet located along the path of pollution plumes from Paris. OH radicals were measured in a forest clearing at ground-level (about 6 m). Co-located measurements of HO2+RO2 (i.e. the sum of hydroperoxy and organic peroxy radicals) and gas-phase H2SO4 were also made on top of a 40 m tower (~20 m above the forest canopy).  A budget analysis was performed using steady-state calculations for OH and H2SO4 using other available measurements on the ground and on the tower (photolysis rates, NOx, O3, VOCs, OH reactivity, aerosol particle size distribution, etc.). A detailed budget analysis for OH and peroxy radicals was performed with a box-model using a MCM derived mechanism. 
Calculated daytime and nighttime OH concentrations on the ground, using measured OH reactivity, showed good correlation with the measurements and reproduced the observed daytime maximum and nighttime levels of about 4×106 molecule cm-3 and (2-6)×105 molecule cm-3, respectively. The production of OH radicals in the clearing and above the canopy during the day was found to be dominated by its regeneration in reactions of HO2 and RO2 with nitric oxide. During the night, the ozonolysis of monoterpenes was a significant OH production pathway with its contribution depending on the nighttime NO concentrations. The box-model resulted in significant underestimation, up to a factor of two in daytime OH and an overestimation of OH reactivity. At the same time, the model sum of peroxy radicals was larger than measurements, especially during the night with lowest observed NO concentration. However, most of the time the model reproduced the observed peroxy radical temporal behavior on the ground and above the canopy, as well as their slightly lower concentrations over the canopy during the day.
The formation of H2SO4 was observed every day during the measurement period, with the median maximum H2SO4 concentration of 2.5×106 molecule cm-3 similar to that observed at some other forested sites. The calculated and measured daytime H2SO4 concentrations were highly correlated with formation of sulfuric acid via SO2+OH reaction accounting for (90±20)% of the observed H2SO4.

How to cite: Jiao, Y. and Kukui, A. and the ACROSS Rambouillet Measurements Team: Chemical budgets of OH, HO2+RO2 and H2SO4 in a sub-urban temperate forest near Paris, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17736, https://doi.org/10.5194/egusphere-egu25-17736, 2025.

Urban ozone (O3) pollution correlates with temperature, and higher O3 often occurs during heat waves, threatening public health. However, limited data on how anthropogenic volatile organic compound (AVOC) precursor emissions vary with temperature hinders understanding their impact on O3. Here, we show that the increase in non-combustion AVOC emissions (e.g., from volatile chemical products) during a heat wave in Shanghai contributes significantly to increased O3, based on ambient measurements, emission testing, and air quality modelling. AVOC concentrations increase ~2  when the temperature increases from 25 °C to 35 °C due to air stagnation and increased emissions. During the heat wave, higher concentrations result in an 82% increase in VOC OH reactivity. Air quality simulations reveal that temperature-driven AVOC emission increases account for 8% (1.6 s-1) of this reactivity increase and enhance O3 by 4.6 ppb. Moreover, we predict a more profound (2 ) increase in OH reactivity of oxygenated VOCs, facilitating radical production and O3 formation. Enhanced AVOC emissions trigger O3 enhancements in large cities in East China during the heat wave, and similar effects may also happen in other AVOC-sensitive megacities globally. Reducing AVOC emissions, particularly non-combustion sources, which are currently less understood and regulated, could mitigate potential O3 pollution in urban environments during heat waves.

How to cite: Qin, M.: Increased Urban Ozone in Heat Waves due to Temperature-Induced Emissions of Anthropogenic Volatile Organic Compounds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18072, https://doi.org/10.5194/egusphere-egu25-18072, 2025.

EGU25-18818 | ECS | Orals | AS3.36

Development of a novel instrument for long-term measurements of OH reactivity  

Midhun George, Thomas Luke, Ambili Babu, Lisa Whalley, Dwayne Heard, Mark Blitz, and Daniel Stone

Improving air quality is one of the main challenges in achieving a sustainable future. The mitigation strategies for air quality and climate change require accurate knowledge of both the amount of trace gases present in the atmosphere and chemical processes involving these trace gases. The primary removal mechanism of trace species such as methane (CH4), volatile organic compounds (VOCs), and NOx (NOx = NO + NO2) in the atmosphere is the reaction with hydroxyl radical (OH), which leads to the formation of secondary pollutants such as ozone (O3) and secondary organic aerosol (SOA). Thus, understanding the behavior of OH in the atmosphere is critical to understanding the lifetimes of many trace species and the reaction pathways leading to the production of secondary pollutants. Although it is not possible to quantify all species in the atmosphere that react with OH, it is possible to quantify their impacts on air quality and climate through measurements of OH reactivity (kOH) (Kovacs and Brune, 2001). OH reactivity is the total pseudo-first-order coefficient describing the loss of OH, which is the inverse of the OH chemical lifetime, and defined as , where is the rate coefficient for reaction of OH with species Xi.
Measurements of kOH have been made successfully in the field using several techniques (Sadanaga et al., 2004; Sinha et al., 2008; Stone et al., 2016), but long-term continuous measurements have proved challenging, particularly in high NOx environments (Fuchs et al., 2017). In this work we describe the development of a novel instrument based on laser flash photolysis coupled with time-resolved broadband UV absorption spectroscopy to make long-term measurements in a wide range of environments. In the field configuration, the instrument has a limit of detection (LOD) of kOH around 1.5 s-1 and LOD of [OH] around 5 × 1010 molecules cm-3.  We will present details about the instrument development, characterisation and the field intercomparison with a laser-induced fluorescence (LIF) instrument. 

How to cite: George, M., Luke, T., Babu, A., Whalley, L., Heard, D., Blitz, M., and Stone, D.: Development of a novel instrument for long-term measurements of OH reactivity , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18818, https://doi.org/10.5194/egusphere-egu25-18818, 2025.

EGU25-19714 | Orals | AS3.36

Improved Simulation of Atmospheric Oxidation Capacity Using the MAX1 Chemical Mechanism in North China Plain, China 

Yanhui Liu, Chunmei Geng, Wenyu Bai, Nan Zhang, Wen Yang, Houhua Zhou, Wenyu Wei, Xueshun Chen, Ming Zhou, Xuefei Ma, Xinping Yang, Huan Song, Xiaorui Chen, Haichao Wang, Zhaofeng Tan, Zifa Wang, Yuanhang Zhang, and Keding Lu

Atmospheric Oxidation Capacity (AOC) quantifies the ability of atmosphere to oxidize primary species. It plays a crucial role in initiating atmospheric chemical processes and impacts the formation of secondary pollutants, such as ozone (O₃) and secondary aerosols. AOC is fundamentally determined by the concentrations and reactivity of atmospheric oxidants, including O₃, hydroxyl radicals (OH), and nitrate radicals (NO₃). Due to the inherent challenges in direct measurement, AOC is typically inferred through numerical modeling. However, the chemical mechanisms implemented in commonly used 3-D chemical transport models (CTMs) often simplify organic species, leading to underestimations of radical concentrations and AOC.

The Mechanism for Air pollution compleX version 1.0 (MAX1) describing detailed tropospheric chemical processes has been therefore developed to improve the simulation of radicals. MAX1 contains 940 reactions including photolysis, gaseous reactions and heterogeneous reactions of 300 species, which is adequate for both box model and CTM applications. Detailed chemical processes of chlorine chemistry, chemistry of Criegee radicals and heterogeneous uptake of HO2 and N2O5 have been implemented and updated. With this level of explicitness, MAX1 can support investigations on the quantification of secondary pollutant productions and the chemical behavior of the crucial intermedia such as organic peroxy radicals. MAX1 has been validated in box model and regional models. Simulations of MAX1 well captured the variation of O₃ in all cases tested. Meanwhile, significant improvement was made on predictions of radicals compared to other mechanisms, especially under the low NOx environment. 

How to cite: Liu, Y., Geng, C., Bai, W., Zhang, N., Yang, W., Zhou, H., Wei, W., Chen, X., Zhou, M., Ma, X., Yang, X., Song, H., Chen, X., Wang, H., Tan, Z., Wang, Z., Zhang, Y., and Lu, K.: Improved Simulation of Atmospheric Oxidation Capacity Using the MAX1 Chemical Mechanism in North China Plain, China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19714, https://doi.org/10.5194/egusphere-egu25-19714, 2025.

EGU25-1800 | ECS | Posters on site | AS3.37

New particle formation induced byanthropogenic–biogenic interactions on the southeastern Tibetan Plateau 

Shiyi Lai, Ximeng Qi, Xin Huang, Sijia Lou, Xuguang Chi, Liangduo Chen, Chong Liu, Yuliang Liu, Chao Yan, Tengyu Liu, Mengmeng Li, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding

New particle formation (NPF) plays a crucial role in the atmospheric aerosol population and has significant implications on climate dynamics, particularly in climate-sensitive zones such as the Tibetan Plateau (TP). However, our understanding of NPF on the TP is still limited due to a lack of comprehensive measurements and verified model simulations. To fill this knowledge gap, we conducted an integrated study combining comprehensive field measurements and chemical transport modeling to investigate NPF events on the southeastern TP during the pre-monsoon season. NPF was observed to occur frequently on clear-sky days on the southeastern TP, contributing significantly to the cloud condensation nuclei (CCN) budget in this region. The observational evidence suggests that highly oxygenated organic molecules (HOMs) from monoterpene oxidation participate in the nucleation on the southeastern TP. After updating the monoterpene oxidation chemistry and nucleation schemes in the meteorology–chemistry model, the model well reproduces observed NPF and reveals an extensive occurrence of NPF across the southeastern TP. The dominant nucleation mechanism is the synergistic nucleation of sulfuric acid, ammonia, and HOMs, driven by the transport of anthropogenic precursors from South Asia and the presence of abundant biogenic gases. By investigating the vertical distribution of NPF, we find a significant influence of vertical transport on the southeastern TP. More specifically, strong nucleation near the surface leads to an intense formation of small particles, which are subsequently transported upward. These particles experience enhanced growth to larger sizes in the upper planetary boundary layer (PBL) due to favorable conditions such as lower temperatures and a reduced condensation sink. As the PBL evolves, the particles in larger sizes are brought back to the ground, resulting in a pronounced increase in near-surface particle concentrations. This study highlights the important roles of anthropogenic–biogenic interactions and meteorological dynamics in NPF on the southeastern TP.

How to cite: Lai, S., Qi, X., Huang, X., Lou, S., Chi, X., Chen, L., Liu, C., Liu, Y., Yan, C., Liu, T., Li, M., Nie, W., Kerminen, V.-M., Petäjä, T., Kulmala, M., and Ding, A.: New particle formation induced byanthropogenic–biogenic interactions on the southeastern Tibetan Plateau, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1800, https://doi.org/10.5194/egusphere-egu25-1800, 2025.

EGU25-2512 | ECS | Orals | AS3.37

Shielding effect of brown organic coating on black carbon aerosols 

Zexuan Zhang, Yuanyuan Wang, Xiyao Chen, Liang Xu, Zhonghua Zheng, Joseph Ching, Shupeng Zhu, Dantong Liu, and Weijun Li

The light absorption of black carbon (BC) particles is influenced by their mixing structures and coating compositions. Liquid-liquid phase separation (LLPS) is an important microscopic phenomenon which can separate organic and inorganic phases and redistribute BC from the inorganic core (Icore) to organic coating (Ocoating). This study combines transmission electron microscopy and a 3D modeling method—Electron-Microscope-To-BC-Simulation (EMBS) to investigate how microphysical properties, such as coating compositions, Ocoating thickness, and BC position, influence the light absorption of BC particles. We found that the position of BC significantly influences its light absorption. The light absorption of BC centering in Icore is stronger below 600 nm than BC in the Ocoating. When Ocoating is considered as BrC, it reduces the light absorption of BC within Icore and Ocoating by 1.8% and 49.8%, respectively, at 350 nm due to the shielding effect, which blocks more photons from reaching the BC core. However, when accounting for the intrinsic light absorption of BrC and BC, the contribution of BrC shielding effect to individual BC particle is merely –3.0%±1.6%. The result indicates that the primary role of BrC coating still keeps light absorption rather than shielding effect in the LLPS particles. This study highlights that brown organic coating and mixing structure of BC should be comprehensively considered pertaining to optical absorption of BC-containing particles in atmospheric models.

How to cite: Zhang, Z., Wang, Y., Chen, X., Xu, L., Zheng, Z., Ching, J., Zhu, S., Liu, D., and Li, W.: Shielding effect of brown organic coating on black carbon aerosols, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2512, https://doi.org/10.5194/egusphere-egu25-2512, 2025.

EGU25-3922 | ECS | Orals | AS3.37

Size-Dependent Sigmoidal Reaction Kinetics for Pyruvic Acid Condensation in Single Aqueous Microdroplets 

Meng Li, Shu Yang, Satish Kumar, Cari Dutcher, Robert Continetti, and Vicki Grassian

Although aqueous microdroplets have been shown to exhibit enhanced chemical reactivity compared to bulk solutions, mechanisms for these enhancements are not completely understood. Pyruvic acid (PA) is an abundant α-keto acid in aerosols, fogs, and clouds in the atmosphere, and its conjugate base, pyruvate, is an important intermediate in several metabolic pathways. Utilizing in situ micro-Raman spectroscopy as a probe, we investigated the chemistry of PA within aqueous microdroplets in a relative humidity (RH)- and temperature-controlled environmental cell. We found that PA undergoes a condensation reaction to yield mostly zymonic acid (ZA). Interestingly, the reaction follows a size-, RH- and temperature-dependent sigmoidal kinetic profile. We developed a diffusion–reaction–partitioning model to simulate the complex kinetics observed in the microdroplets. Combined experimental measurements and kinetic modeling showed that the condensation reaction of PA in microdroplets is driven by coupled surface reactions and gas-phase partitioning. Importantly, the kinetic model best fits the data when an autocatalytic step is included in the mechanism, i.e. a reaction step where the product, ZA, catalyzes the interfacial condensation reaction. Overall, the dynamic nature of aqueous microdroplet chemistry and the coupling of interfacial chemistry with gas-phase partitioning are demonstrated. Furthermore, autocatalysis of small organic molecules at the air–water interface for aqueous microdroplets, shown here for the first time, has implications for several fields including prebiotic chemistry, atmospheric chemistry and chemical synthesis.

How to cite: Li, M., Yang, S., Kumar, S., Dutcher, C., Continetti, R., and Grassian, V.: Size-Dependent Sigmoidal Reaction Kinetics for Pyruvic Acid Condensation in Single Aqueous Microdroplets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3922, https://doi.org/10.5194/egusphere-egu25-3922, 2025.

Pulsed laser photolysis/laser-induced fluorescence (LP/LIF) was used to study the rate coefficients of the  OH reaction with CO, NO, NO2 and of the HO2 reaction with NO2 in synthetic air at different water vapour concentrations (partial pressure up to 22 hPa) and at room temperature and at atmospheric pressure. The decay of the radicals was monitored by LIF, which allowed the calculation of the bimolecular rate coefficients. The rate coefficients for the reaction of OH with NO and NO2 agree very well with current NASA/JPL and IUPAC recommendations and have a high accuracy (< 5%). These rate coefficients were found to be independent of the presence of water vapour at 1 atm of total pressure. At high pressures and low water vapour mixing ratios, as in the experiments in this work, only a small effect of the collisional stabilisation by water molecules is expected. The measured rate constant of HO2 with NO2 was found to be significantly dependent on the water vapour concentration. The water dependence can be explained by an approximately two times higher rate coefficient of the reaction of NO2 with the HO2 complex with water.

How to cite: Fuchs, H., Rolletter, M., Hofzumahaus, A., and Novelli, A.: Kinetics of the termolecular reaction of OH with NO, NO2, and of HO2 with NO2 in 1 atm air at 298K and tropospheric water vapour concentrations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4738, https://doi.org/10.5194/egusphere-egu25-4738, 2025.

EGU25-6000 | Posters on site | AS3.37

Analysis of Hygroscopic Cloud Seeding Materials Using K-CPEC facility 

Bu-Yo Kim, Miloslav Belorid, Joo Wan Cha, Youngmi Kim, and Seungbum Kim

This study presents the methodology and results of the chamber experiments conducted using the Korea Cloud Physics Experiment Chamber (K-CPEC) established by the Korea Meteorological Administration (KMA)/National Institute of Meteorological Sciences (NIMS) in South Korea. The research focused on warm clouds in South Korea, utilizing NaCl and CaCl2, powder-type hygroscopic materials commonly used for cloud seeding experiments. The characteristics of these particles were measured, and their effects on cloud droplet growth were observed. Detailed descriptions of the aerosol and cloud chambers at K-CPEC, along with the experimental setup and measurement instruments, are provided. The methods outlined in this study can aid in the development and evaluation of new cloud-seeding materials, enhancing the effectiveness of cloud seeding techniques.

 

Acknowledgments: This work was funded by the Korea Meteorological Administration Research and Development Program “Research on Weather Modification and Cloud Physics” under Grant (KMA2018-00224).

How to cite: Kim, B.-Y., Belorid, M., Cha, J. W., Kim, Y., and Kim, S.: Analysis of Hygroscopic Cloud Seeding Materials Using K-CPEC facility, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6000, https://doi.org/10.5194/egusphere-egu25-6000, 2025.

EGU25-7329 | Orals | AS3.37 | Highlight

Deposition ice nucleation via homogeneous freezing of adsorbed water 

Ari Laaksonen, Golnaz Roudsari, Ana Piedehierro, and André Welti

Deposition ice nucleation (DIN) occurs when water insoluble particles (that are not immersed in water or aqueous solution droplets) initiate the growth of ice crystals in water vapor supersaturated with respect to ice. The classical view (Fletcher, 1959) of DIN is similar to that of the heterogeneous nucleation of liquid droplets: a sufficient number of water molecules originating from the vapor phase come together at a surface within a sufficiently short period of time, forming a critical cluster that is large enough so that it does not decay but starts collecting more vapor molecules and growing. In addition to being large enough, the ice cluster must also organize into a crystalline configuration, which obviously drastically decreases the probability of a nucleation event. It therefore seems likely that an intermediate liquid phase (Ostwald, 1897) is involved in the DIN process. During the past decade, the pore condensation and freezing mechanism (Marcolli, 2014), in which liquid water condenses in the pores of insoluble aerosols and subsequently freezes, has been considered a candidate for the mechanism of atmospheric DIN events. However, it is known from laboratory studies that DIN can also occur on nonporous aerosols. In this work, we have developed a theoretical framework for describing DIN as homogeneous freezing in multilayer adsorbed water. We compare the predictions of the theory to laboratory data of critical supersaturations for DIN on nonporous silica particles at temperatures down to 208 K and find very good agreement.     

Fletcher, N. H. (1959). On ice-crystal production by aerosol particles, J. Atmos. Sci., 16, 173–180.

Marcolli, C. (2014) Deposition nucleation viewed as homogeneous or immersion freezing in pores and cavities, Atmos. Chem. Phys., 14, 2071–2104,

Ostwald, W. (1897). Studien über die Bildung und Umwandlung fester Körper. 1. Abhandlung: Übersättigung und Überkaltung. Z. Phys. Chem., 22, 289-330.

 

How to cite: Laaksonen, A., Roudsari, G., Piedehierro, A., and Welti, A.: Deposition ice nucleation via homogeneous freezing of adsorbed water, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7329, https://doi.org/10.5194/egusphere-egu25-7329, 2025.

The formation and breakup of non-covalently-bound nitrate ion-analyte clusters is an important process in newly developed nitrate ion CIMS (Chemical Ionization Mass Spectrometry) instruments designed to detect trace molecules implicated in atmospheric aerosol and new-particle formation.  Here, we show some results from using mainly classical molecular dynamics methods with empirical force fields to model these systems. These cheap methods allow us to approach the problem as a statistical one, by easily running 100s-1000s of separate simulations.

We study three different scenarios: 1) Cluster decomposition in vacuo, 2) Cluster decomposition in presence of N2, 3) Acceleration of the charged cluster by an electric field, leading to collisions with N2 and eventual decomposition. For scenarios 1 and 2, we find that the distribution of survival times has a very long tail, and can be effectively modelled as a stretched exponential, or a sum of two of them. Analysis of the survival time distribution at different initial temperatures can be used to predict the mean lifetime of the clusters at 300 K. We aim to use these data to aid the interpretation of CIMS experiments in our group[1].

Under the influence of electric field, average lifetimes vary with gas pressure and field strength [see figure]. As in similar studies of small water-ion clusters, we note that collisions between the cluster and gas can be energetic enough to cause decomposition directly in high field and low pressure[2].  However, at low field and atmospheric pressure (similar to conditions in the CIMS inlet) our results show that cluster decomposition is unlikely to occur.

[1] N. Hyttinen et al., J. Phys. Chem. A, 122, 269 (2018); S. Iyer et al., JPCA, 120, 576 (2016); A. Kumar et al., JACS 146, 15562 (2024); O. Garmash et al., Environ. Sci.: Atmos., DOI: 10.1039/d4ea00087k (2024)
[2] C.D. Daub and N.M. Cann, Anal. Chem., 83, 22393 (2011).

How to cite: Daub, C. D., Kurtén, T., and Rissanen, M.: Molecular dynamics simulations as probes of the decomposition kinetics of atmospheric molecular complexes: A case study of nitrate chemical ionization, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8620, https://doi.org/10.5194/egusphere-egu25-8620, 2025.

In the initial stages of atmospheric aerosol particle formation, molecules collide and stick together, forming dimers and small clusters. This is an inherently dynamic process. Molecular dynamics (MD) simulations allow us to model the dynamic behavior of these collision systems. In MD simulations, the trajectory of a system is divided into discrete timesteps, with forces on the nuclei computed at each step to propagate the system. Traditionally, these forces are calculated using classical force fields, which are highly efficient and allow for simulations of large systems over long time scales. However, classical force fields either neglect or only crudely approximate important features like chemical reactions. Atmospheric particle formation depends on proton transfers and cluster reactions to form stable aggregates, making it essential to capture these processes accurately.

Ab initio molecular dynamics (AIMD) use quantum chemistry (QC) calculations to determine the forces on nuclei at each time step. While AIMD can accurately model chemical reactions and other quantum effects, it is computationally unfeasible for anything beyond short simulations of small systems. Recently, machine learning (ML) methods have been applied to create ML potentials for MD simulations. These potentials can replicate high-level QC data while maintaining the efficiency of classical force fields. However, many ML methods rely on a local atomic environment approximation, where the potential is constructed from interactions within a user-defined cutoff radius around each nucleus. This approach fails to capture long-range interactions, which are particularly significant for polar atmospheric molecules like sulfuric acid, as these interactions typically extend well beyond the cutoff radius.

We are training ML potentials for MD simulations of collisions between atmospheric particle-forming molecules, with a focus on accurately capturing long-range interactions. A training set was generated by performing MD simulations of collisions between two sulfuric acid molecules using the semi-empirical GFN1-xTB method, followed by gradient calculations on structures along the collision trajectory. This approach ensures that the free molecules, dimers, and structures along the collision trajectory are well-represented. We then use this dataset to train ML potentials with the paiNN and PhysNet architectures. Both methods rely on the local atomic environment approximation, but PhysNet additionally incorporates long-range electrostatic interactions through learned partial charges and dispersion interactions via Grimme’s D3BJ dispersion correction. By exploring various training sets and model parameters, such as the cutoff radius for the local environment, we aim to develop ML potentials that accurately capture long-range interactions. This project serves as an initial step toward enabling large-scale MD simulations of atmospheric particle formation.

How to cite: Neefjes, I., Kubečka, J., and Elm, J.: Training machine learning potentials with accurate long-range interactions for atmospheric molecular dynamics collision simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9100, https://doi.org/10.5194/egusphere-egu25-9100, 2025.

EGU25-9215 | ECS | Posters on site | AS3.37

 Computational methods for generating clusters of oxygenated organic molecules  

Jaakko Kähärä, Lauri Franzon, Theo Kurten, and Hanna Vehkamäki

The contribution of oxygenated organic molecules (OOM) in new particle formation is well known yet weakly understood. In this work, we present methods for generating optimized OOM cluster configurations. The framework for configurational sampling, optimizing, and analysing of molecular clusters is provided by JKCS program (Kubečka, Besel, et. al., 2023). Initial sampling of cluster configurations is done at semi-empirical level of theory. Local and global minimum energy configurations are found through successive rounds of filtering a subset of results and re-optimization at higher DFT levels of theory. Finally, we select the lowest energy structures to calculate the binding free energies for each cluster type. 

Experimental research suggests that OOMs with more than 10 carbon atoms contribute to aerosol cluster formation. The size and complexity of OOM clusters significantly limits the number of DFT calculations we can perform, and even very large samplings of cluster configuration space do not guarantee that the global minimum is found. To improve upon existing methods, we introduce constraints to initial sampling which force hydrogen formation between molecules. We also use metadynamics simulations to search for additional local minima. OOMs are observed to cluster in configurations which maximise the number of hydrogen bonds. Thus, the binding free energies are highly dependent on the structure of each molecule and on their ability to form internal hydrogen bonds. OOMs used in this work were obtained using Gecko-AP (Franzon et. al, 2024), a RO2 + RO2 accretion product generator based on the Gecko-A software.

Machine learning force fields have the potential to predict DFT level energies with a fraction of the computational cost. However, most ML force fields do not scale well to larger molecules and fail to correctly model long-range interactions. It is also necessary to sample a dataset which covers the relevant region of the potential energy surface.  We trained a neural network model to predict electronic energies for 2-OOM clusters containing 130-150 atoms. In future work we wish to train a machine learning force field which generalizes to atmospheric molecules and to decrease the prediction error close to chemical accuracy.

References

Kubečka, J., Besel, V., Neefjes, I., Knattrup, Y., Kurtén, T., Vehkamäki, H. and Elm, J. (2023) ACS Omega, 8, 45115. 

Franzon, L., Camredon, M., Valorso, R., Aumont, B. and Kurten T. (2024) Atmos. Chem. Phys., 24, 11679–11699.

How to cite: Kähärä, J., Franzon, L., Kurten, T., and Vehkamäki, H.:  Computational methods for generating clusters of oxygenated organic molecules , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9215, https://doi.org/10.5194/egusphere-egu25-9215, 2025.

EGU25-9607 | ECS | Orals | AS3.37

Hydration layer structure and ice nucleation ability of K-feldspar surfaces investigated using molecular dynamics and machine learning 

Rasmus Nilsson, Patrick Rinke, Hanna Vehkamäki, and Bernhard Reischl

K-feldspar mineral dust particles have been observed to nucleate ice heterogeneously at higher supercooling compared to other atmospheric minerals. There is experimental and computational evidence pointing to the importance of high energy (100) crystallographic planes, mostly exposed in surface cracks, but the exact atomistic ice nucleation mechanism remains unknown (Kiselev et al., 2017). Recent atomistic molecular dynamics simulations did not exhibit spontaneous ice nucleation on flat (100) K-feldspar microcline surfaces (Soni and Patey, 2019). This could have been caused by inaccurate force fields, insufficient sampling time, or considering too simple surfaces that do not present active sites for ice nucleation. We try to shed new light on the phenomenon by combining molecular dynamic simulations with machine learning models. To validate the force field used in our simulations, we compare the calculated hydration layer structures with recent 3D AFM experiments at the feldspar-water interface and find good agreement between the two (Dickbreder et al., 2024). Using non-equilibrium molecular dynamics, we determine the onset freezing temperature on a large sample of K-feldspar (100) surfaces with different termination and topographical features, such as step edges, defects, and strained lattices, by looking for a potential energy jump as the simulation temperature is decreased. Machine learning models are then trained on this data set to predict the onset freezing temperature based on the characteristics of the surface, and by using feature analysis we will determine which surface characteristics enable higher onset freezing temperatures (Fitzner et al., 2020).  

 

Dickbreder, T., Sabath, F., Reischl, B., Nilsson, R. V. E., Foster, A. S., Bechstein, R., and Kühnle, A.: Atomic structure and water arrangement on K-feldspar microcline (001), Nanoscale, 16, 3462-3473, 2024. 

Fitzner, M., Pedevilla, P., and Michaelides, A.: Predicting heterogeneous ice nucleation with a data-driven approach, Nat. Commun., 1-9, 2020. 

Kiselev, A., Bachmann, F., Pedevilla, P., Cox, S. J., Michaelides, A., Gerthsen, D., and Leisner, T.: Active sites in heterogeneous ice nucleation-the example of K-rich feldspars, Science, 355, 367-371, 2017. 

Soni, A. and Patey, G. N.: Simulations of water structure and the possibility of ice nucleation on selected crystal planes of K-feldspar, J. Chem. Phys., 150, 214501, 2019. 

How to cite: Nilsson, R., Rinke, P., Vehkamäki, H., and Reischl, B.: Hydration layer structure and ice nucleation ability of K-feldspar surfaces investigated using molecular dynamics and machine learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9607, https://doi.org/10.5194/egusphere-egu25-9607, 2025.

Organic peroxy radicals (RO2) are key species in the troposphere as their chemistry leads to the formation of secondary organic aerosols and ozone. RO2 radicals mainly react with nitric oxide (NO) in the lower troposphere, leading to either (i) radical propagation, which sustains the atmospheric oxidation capacity, or (ii) the formation of organic nitrates (RONO2), where both RO2 and NO2 are sequestered, thus reducing radical propagation rates and the formation of secondary pollutants. The latter pathway exhibits RONO2 yields ranging from negligible up to 35%, depending on the RO2 molecular structure.

We propose a new approach to quantify RONO2 yields from RO2+NO reactions, taking advantage of the measurement principle of chemical amplifiers (CA), initially developed for measuring ambient concentrations of ROx radicals (OH, HO2 and RO2). We will show that the CA can be used as a  kinetic apparatus to quantify an “integrated” RONO2 yield for chemical systems where a specific volatile organic compound (VOC) is oxidized by OH. In this presentation, we will discuss applications for the following chemical systems: ethane+OH, cyclohexane+OH and isoprene+OH, emphazing how the determinations contrast to published data. Both advantages and drawbacks will be highlighted for this new approach.

 

How to cite: Strunz, C., Tomas, A., Noziere, B., and Dusanter, S.: Development of a new approach to quantify organic nitrate yields from RO2+NO reactions – Application to ethane-, cyclohexane- and isoprene-derived RO2 radicals, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9743, https://doi.org/10.5194/egusphere-egu25-9743, 2025.

EGU25-9874 | ECS | Orals | AS3.37

Simulation chamber study of the spectral optical properties of flame soot and their link to composition 

Johannes Heuser, Claudia Di Biagio, and Jean-Francois Doussin and the B2C team

Carbonaceous soot aerosol formed during the incomplete combustion of fossil fuels, biofuels, and biomasses is an important light-absorbing species containing both Black and Brown Carbon (BC, BrC). Despite being key climate forcers, soot and its BC and BrC components are still difficult to represent in models due to persisting uncertainties of its spectral optical properties, such as the complex refractive index, mass absorption/scattering/extinction cross-sections (MAC/MSC/MEC, in m2g–1) and the single scattering albedo (SSA). In particular, the dependence of optical properties on the variable composition, morphologies, and mixing state of the atmospheric soot remains poorly understood.

In order to advance on this topic, a set of experiments was performed using the 4.2 m3 CESAM simulation chamber on soot aerosol generated from a propane diffusion flame. Experiments were conceived to mechanistically investigate the dependence of soot spectral optical properties on 1/ combustion conditions and varying particle composition, and 2/ different aging processes. To investigate point 1/ the soot aerosols were generated under different combustion conditions covering both fuel–lean and fuel-rich conditions, resulting in particles with varying sizes and elemental/organic carbon (EC, OC) content. For investigating point 2/, the EC-richer soot was subjected to simulated atmospheric aging including exposure to humidity, radiation, and additional gaseous phases (O3, SO2), also inducing the formation of a coating by a second scattering aerosol phase produced via the photo-oxidation of SO2 or the ozonolysis of α-pinene.

The datasets retrieved from the chamber experiments permitted to analyse the dependence of the soot spectral absorption on their BC and BrC particle’s content, resulting in predictive relationships to use in models. Systematic simulation chamber experiments showed that the MAC has a variability associated with the EC/TC ratio in soot. The MAC at 550 nm increases for increasing EC/TC, with values of 1.0 m2g-1 for EC/TC=0.0 (BrC-dominated soot) and 4.6 m2g-1 for EC/TC=0.79 (BC-dominated soot). The Absorbing Angstrom Exponent (AAE) and the SSA at 550 nm decrease from 3.79 and 0.29 (EC/TC=0.0) to 1.27 and 0.10 (EC/TC=0.79). A combination of our results for propane soot with literature data for laboratory flame soot from diverse fuels supports a generalized exponential relationship between particle EC/TC and its MAC and AAE values, representing the spectral absorption of soot with varying maturity to lie in an optical continuum. From this, we extrapolate a MAC of 7.9 and 1.3 m2g-1 (550 nm) and an AAE (375–870 nm) of 1.05 and 4.02 for pure EC (BC-like) and OC (BrC-like) propane soot. The established relationship can provide a useful parameterization for models to estimate the absorption from combustion aerosols and their BC and BrC contributions. Results from this analysis are presented in the Heuser et al. paper available at https://egusphere.copernicus.org/preprints/2024/egusphere-2024-2381/.

How to cite: Heuser, J., Di Biagio, C., and Doussin, J.-F. and the B2C team: Simulation chamber study of the spectral optical properties of flame soot and their link to composition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9874, https://doi.org/10.5194/egusphere-egu25-9874, 2025.

EGU25-10681 | ECS | Orals | AS3.37

Measurements of photocatalytic chloride to chlorine conversion by iron-salt aerosols at the European Photoreactor (EUPHORE) 

Luisa Pennacchio, Marie K. Mikkelsen, Chloe Brashear, Rubén Soler, Ezra Woods, Mila Ródenas, Amalia Muñoz, Maarten van Herpen, Thomas Röckmann, and Matthew S. Johnson

Recent studies have shown that when iron-containing mineral dust mixes with aerosols containing chloride, iron(III)chloride salts are formed enabling the photocatalytic production of Cl2 [1-3]. Work has shown that the iron salt aerosol mechanism is the largest source of chlorine radicals over the North Atlantic. The mechanism is catalytic both in iron and chlorine. Despite clear evidence from field studies, laboratory studies and modelling [2-5], significant questions remain (effect of RH, iron activity, pH limited behavior, etc.). The goal of this study is to answer these questions through experiments performed in the European Photoreactor (EUPHORE) in Valencia, Spain. The reactor is 200 m3 and utilizes natural sunlight and is therefore ideal for simulating atmospheric behavior. Measurements were collected with long-path FTIR, CIMS, OPS, SMPS, PTR-MS, ACSM, LIF-FAGE, Picarro G2108 and G2201-i as well as monitors for O3, CO, NO, NO2, NOx and HCHO. Furthermore, flask samples were collected for analysis of [CO], δ13C-CO, [CH4], δ13C-CH4 and VOCs at Utrecht University. Two sets of experiments were carried out, one to investigate the effect of the iron and chloride in the aerosols and one to investigate the mechanism using real dust samples. In the first set of experiments, solutions of FeCl3+NaCl, NaCl or FeSO4 were aerosolized to evaluate the effect of iron and chlorine separately and together. In the second set of experiments, acidic NaCl aerosols were introduced to the reactor along with aerosolized dust injections, for more realistic simulations. We will report our results concerning the rate of Cl2 production in the dark via the Fenton mechanism and by ISA.

[1] Chen et al. (2024) Environ. Sci. Technol., 58(28), 12585-12597

[2] van Herpen et al. (2023) PNAS, 120, 31

[3] Mikkelsen et al. (2024) Aerosol Research, 2, 31-47

[4] Wittmer et al. (2015) Environmental Chemistry, 12(4), 461-475

[5] Wittmer et al (2017) Journal of Atmospheric Chemistry, 74, 187-204

How to cite: Pennacchio, L., K. Mikkelsen, M., Brashear, C., Soler, R., Woods, E., Ródenas, M., Muñoz, A., van Herpen, M., Röckmann, T., and S. Johnson, M.: Measurements of photocatalytic chloride to chlorine conversion by iron-salt aerosols at the European Photoreactor (EUPHORE), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10681, https://doi.org/10.5194/egusphere-egu25-10681, 2025.

EGU25-11081 | Orals | AS3.37

Air quality and health hazard of domestic Biomass Burning heating appliances: the experiment at the EUPHORE Chamber 

Ettore Petralia, Maurizio Gualtieri, Mila Ródenas, Ilaria D'Elia, Laura Caiazzo, Teresa M.G. La Torretta, Giandomenico Pace, Antonio Piersanti, Milena Stracquadanio, Rossella Bengalli, Sara Marchetti, Giulia Motta, Teresa Vera, Rubén Soler, Esther Borrás, Beatríz Domínguez, and Amalia Muñoz

Biomass burning (BB) represents a global concern due to its impact on air pollution, health and climate change, resulting in 2.3 million premature deaths yearly. BB in the residential sector is one of the main sources of primary Particulate Matter emissions. BB emits a significant amount of black and brown carbon, Polycyclic Aromatic Hydrocarbons, and contributes to secondary formation of ozone by photochemical reaction of volatile organic compounds and nitrogen oxides. On the other side, BB is a green and renewable alternative source to fossil fuels reducing carbon dioxide emissions with lower costs, whose use is even expanded due to the last energy crisis and natural gas cost, increasing its impact on both rural and urban areas.

Significantly, BB emission factors (EFs) are affected by a wide range of uncertainties, in terms of primary and secondary air pollutants contribution and in term of health impact estimates. Comprehensive chemical characterization of primary and secondary emissions, combined with the understanding of its potential health effects, requires dedicated experiments to assess a proper offset of BB.

During the MIND-BB campaign primary gaseous and particulate BB emissions from domestic heating devices were sampled and measured within the outdoor EUPHORE chamber, monitoring chemical and physical properties. EUPHORE, sited at CEAM (Valencia-ES), is highly instrumentalized and adapted to introduce fumes from domestic stoves. Given its large size and thanks to its Teflon® FEP cover and to the possibility of opening and closing its sun barrier, the facility can simulate near-real conditions, under both sunlight and night situations. EUPHORE allowed the analysis as well as the aging of the primary emissions. In parallel, we exposed A549 lung epithelial cells cultured at the air-liquid-interface (ALI) to the primary and secondary emissions to evaluate their toxicological hazard mimicking human exposure conditions. Two types of stoves, fuelled with pellet or wood-logs, were tested, and the latter with two different types of wood: Pine and Oak. Measures were performed on primary emissions and aged compounds for each type of fuel (certified pellet, pine, oak), under different conditions (daylight and night) and operation phases (flaming, smouldering). Moreover, for the first time in an outdoor simulation chamber, we performed the direct ALI exposure of human lung cells to primary and aged emissions to define their toxicological hazard providing new and unavailable data.

The results of this integrated innovative methodology will produce a trans-disciplinary improvement in understanding the impacts of BB primary vs secondary emissions on air pollution and its toxicological hazard. These findings will allow to enhance the estimates of emission inventories and scenarios, and to offset the pros and cons of using woody biomass as energy source and its effects on air quality, climate change and health.

Acknowledgments:

This work is part of a project supported by the EC under the Horizon 2020–R&I FP through the ATMO-ACCESS Integrating Activity under GA N.101008004, and by the R+D project ATMOBE (PID2022-142366OB-I00), funded by MCIN/AEI/10.13039/501100011033/ and the "ERDF A way of making Europe” and EVER project CIPROM/20200/37.

We also thank Tatiana Gómez and M.Luisa Martinez for their work on the experiments

How to cite: Petralia, E., Gualtieri, M., Ródenas, M., D'Elia, I., Caiazzo, L., La Torretta, T. M. G., Pace, G., Piersanti, A., Stracquadanio, M., Bengalli, R., Marchetti, S., Motta, G., Vera, T., Soler, R., Borrás, E., Domínguez, B., and Muñoz, A.: Air quality and health hazard of domestic Biomass Burning heating appliances: the experiment at the EUPHORE Chamber, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11081, https://doi.org/10.5194/egusphere-egu25-11081, 2025.

Organic peroxy radicals (ROO) are critical intermediates in atmospheric chemistry, yet their interactions with solid surfaces remain poorly understood due to challenges in monitoring these reactive species. We present a new experimental flow tube setup designed to overcome these limitations, enabling direct measurement of the uptake of ROO on solid surfaces.

In our approach, ROO (specifically CH3OO and 1-C3H7OO) are generated photolytically and introduced into reaction tubes composed of, or filled with, various materials. The system is coupled with a Proton-Transfer-Reaction Time-of-Flight Mass Spectrometer (PTR-TOF-MS), allowing direct detection of ROO. Reaction kinetics are determined by varying the residence time in the reactor tube, achieved either by adjusting the tube length or changing the gas flow rate.

Using this method, we successfully monitored the uptake of CH3OO and 1-C3H7OO on solid surfaces and identified reaction products. Results shown that the ROO uptake is highly dependent on the surface material. Non-conductive materials such as borosilicate glass and perfluoroalkoxy alkane (PFA) showed negligible uptake, whereas metallic surfaces exhibited significant reactivity. A second study examined atmospherically relevant inorganic salts. 

Our findings highlight the pivotal role of material redox properties in driving the surface reactivity of organic peroxy radicals, providing new insights into their fundamental behavior and raising new questions about their role in atmospheric environments.

How to cite: Durif, O. and Nozière, B.: A Novel Flow Tube Method for Measuring Gas-Phase Reactions Kinetics and Uptake on Solid Surfaces: Application to Organic Peroxy Radical, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11187, https://doi.org/10.5194/egusphere-egu25-11187, 2025.

EGU25-12982 | ECS | Orals | AS3.37

Investigations on the fate of selected peroxy radicals using synthetized precursors and isomeric speciation 

Niklas Illmann, Imad Zgheib, Fabienne Fache, Iulia Patroescu-Klotz, Felipe Lopez, Stephan Graf, Sebastian Gerber, Michael Kamrath, and Matthieu Riva

Peroxy radicals (RO2) play a central role in the atmospheric degradation of volatile organic compounds (VOC) whose atmospheric lifetime and further reactions depend strongly on the prevailing conditions. In air masses influenced by anthropogenic activities the fate of a peroxy radical is typically dominated by its reaction with NO which finally results in the formation of tropospheric ozone. Once NO no longer dominates, peroxy radical chemistry becomes more complex and includes reactions with HO2, other peroxy radicals or unimolecular isomerization (H shift). The last can occur multiple times, each shift being followed by progressive addition of O2. The resultant highly oxidized peroxy radicals either decompose or undergo bimolecular reactions. This process causes rapid formation of low-volatility vapours that contribute to new particle formation.

Apart from the progress made over the last decade in understanding peroxy radical chemistry and the formation of highly oxidized species in particular, the formation mechanisms and the influence of the peroxy radical structure on the reactivity are still not well-established. The detection of highly oxygenated organic molecules (HOM) was achieved by chemical ionisation mass spectrometry which provides only information on the chemical formula. Further, oxidation experiments on biogenic VOC (terpenes etc.) result in a complex mixture of peroxy radicals impeding to gain detailed information on formation mechanisms.

To address existing analytical and experimental shortcomings in characterizing the formation and fate of peroxy radicals, three iodo-carbonyl precursors (i.e., C7H13OI) were synthesized to produce specific peroxy radicals via photolysis. The experiments were performed in the QUAREC atmospheric simulation chamber (University of Wuppertal). The model reaction systems were monitored by Fourier-Transform infrared (FTIR) spectroscopy and molecular characterization of the resulting oxidation products was retrieved using the low pressure IMS-Tof-CIMS. The experimental set-up was carefully adjusted to differentiate between autoxidation processes, permutation reactions, and the reaction of peroxy radicals with HO2. The influence of the peroxy radical structure on the reactivity will be discussed.

How to cite: Illmann, N., Zgheib, I., Fache, F., Patroescu-Klotz, I., Lopez, F., Graf, S., Gerber, S., Kamrath, M., and Riva, M.: Investigations on the fate of selected peroxy radicals using synthetized precursors and isomeric speciation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12982, https://doi.org/10.5194/egusphere-egu25-12982, 2025.

Collisions of neutral molecules and clusters is the most prevalent pathway in atmospheric new particle formation (NPF), and therefore such collisions have direct implications on air quality and climate. Until recently, these collisions have been modeled mainly using non-interacting hard-sphere (NHS) models, which systematically underestimate collision and particle formation rates, due to omission of long-range interactions. Lately, atomistic simulations have been used to study neutral molecule-molecule and molecule-cluster collisions (Halonen et al., 2019; Yang et al., 2023), but studies on cluster-cluster collisions are still lacking despite the relevant role they can play e.g. in haze formation in polluted urban areas (Guo et al., 2014). To calculate more realistic collision rates between clusters of acid-base pairs, we have studied collisions between neutral clusters of N bisulphate and N dimethylammonium ions at T = 300 K up to N = 32 using atomistic molecular dynamics (MD) simulations. Direct simulation results are then compared against both the traditional NHS model and the newly proposed interacting hard-sphere (IHS) variant (Yang et al., 2023), respectively. We find the collision rates in the atomistic MD simulations to be enhanced by factors of 2.2 - 5.6 over the NHS results, with enhancement slowly decreasing with increasing cluster size. In contrast, the IHS model yields a constant enhancement factor of 3.4 for all collisions between same-sized clusters, which decreases with increasing cluster size ratio. Our results demonstrate how even collisions between clusters of tens of acid-base pairs at a relatively high temperature cannot be accurately modeled when long-range interactions are neglected, as convergence towards the non-interacting limit is slow when cluster radius grows. Nor can the results be explained by simple point-particle models, highlighting the importance of atomistic details of intermolecular interactions.

Guo, S., Hu, M., Zamora, M. L., Peng, J., Shang, D., Zheng, J., Du, Z., Wu, Z., Shao, M., Zeng, L., et al.: Elucidating severe urban haze formation in China, Proc. Nat. Acad. Sci. USA, 111, 17373-17378, 2014.

Halonen, R., Zapadinsky, E., Kurtén, T., Vehkamäki, H., and Reischl, B.: Rate enhancement in collisions of sulfuric acid molecules due to long-range intermolecular forces, Atmos. Chem. Phys., 19, 13355-13366, 2019.

Yang, H., Neefjes, I., Tikkanen, V., Kubečka, J., Kurtén, T., Vehkamäki, H., and Reischl, B.: Collision-sticking rates of acid–base clusters in the gas phase determined from atomistic simulation and a novel analytical interacting hard-sphere model, Atmos. Chem. Phys., 23, 5993-6009, 2023.

How to cite: Reischl, B., Tikkanen, V., Yang, H., and Vehkamäki, H.: Gas-phase collision rate enhancement factors for acid-base clusters up to 2 nm in diameter from atomistic simulation and the interacting hard sphere model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14930, https://doi.org/10.5194/egusphere-egu25-14930, 2025.

EGU25-15627 | Orals | AS3.37

Simulation chamber studies on the atmospheric oxidation of skatole 

Emma Galloway, Mixtli Campos-Pineda, Andy Ruth, and John Wenger

Skatole (C9H9N) is an odour-producing member of the indole family and is known to be emitted from animal excreta. It is a common emission from animal husbandry due to the practice of spreading slurry and manure as an organic fertiliser. Little is known about the atmospheric reactivity of skatole with ozone (O3), the hydroxyl radical (OH) and the nitrate radical (NO3), or the potential impacts of the oxidation products on air quality and climate. 

A series of atmospheric simulation chamber experiments were performed at the Irish Atmospheric Simulation Chamber (IASC) to study the atmospheric reactivity of the gas-phase reaction of skatole with O3, OH and NO3 to determine the kinetics, products and the potential for SOA formation. The rate coefficients were determined using the relative rate method.

A time-of-flight chemical ionisation mass spectrometer (ToF-CIMS) was operated with benzene and iodide as the reagent ions. Benzene allows for the detection of hydrocarbons, aromatic compounds and nitrogen heterocycles, so it was used to detect skatole and the initial oxidation products formed. Iodide is more suited to detecting highly oxygenated compounds and was used to identify higher generation oxidation products formed in the latter stages of the reactions. A scanning mobility particle sizer (SMPS) was used to monitor the formation of secondary organic aerosols (SOA), which were also chemically analysed by ToF-CIMS fitted with a Filter Inlet for Gases and AEROsols (FIGAERO).

The results from this series of experiments provide new information regarding the atmospheric reactivity of skatole, providing a greater understanding of the impact of emissions from the practice of using slurry and manure as organic fertilisers on air quality and climate.

How to cite: Galloway, E., Campos-Pineda, M., Ruth, A., and Wenger, J.: Simulation chamber studies on the atmospheric oxidation of skatole, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15627, https://doi.org/10.5194/egusphere-egu25-15627, 2025.

EGU25-15787 | ECS | Posters on site | AS3.37

Machine Learning Interatomic Potential for Atmospheric Chemistry 

Lucas Bandeira, Hilda Sandström, and Patrick Rinke

Aerosols consist of solid or liquid particulate matter suspended in the atmosphere, varying in chemical composition and dimension. They play crucial roles in Earth’s climate system by affecting radiative forcing, cloud formation, and air quality, for instance, thus impacting both the environment and human health. Organic compounds, in particular, can largely contribute to the initial stage of particle aggregation[1, 2]. Computational chemistry methods have been fundamental to elucidating the reactions and processes involving aerosol particles in Earth’s atmosphere[3]. Nevertheless, these tools are limited by the size of the systems under investigation due to computational expenses, demanding faster and cheaper alternatives for large-scale modeling. Here, we present a scheme for a machine learning interatomic potential (MLIP) trained on the atmospherically relevant organic molecules derived from the GeckoQ dataset[1]. This model can be utilized for molecular dynamics simulations, providing results at the same level of accuracy as DFT, besides being capable of expediting the exploration of conformational chemical space. In addition, our MLIP will be trained to predict the saturation vapor pressure (a measure of a molecule’s volatility) of atmospheric molecules instead of only energies and forces. This particular property is central in atmospheric chemistry since organic molecules with low saturation vapor pressure tend to participate in particle formation processes. We anticipate the devised interatomic potential can supplant conventional quantum chemistry methods in further studies in aerosol chemistry. One of the most promising applications is the investigation of larger systems, such as accretion products (a class of large, low-volatility organic compounds resulting from chemical reactions) and clusters. Understanding the role of these products is essential in atmospheric chemistry as they are considered paramount to particle formation.

This work was supported by the VILMA (Virtual Laboratory for Molecular-Level Atmospheric Transformations) Center of Excellence, funded by the Academy of Finland under grant 13346377.

[1] Vitus Besel et al. “Atomic structures, conformers and thermodynamic properties of 32k atmospheric molecules”. In: Scientific Data 10.1 (July 2023). issn: 2052-4463. doi: 10.1038/s41597-023-02366-x. url: http://dx.doi.org/10.1038/s41597-023-02366-x.

[2] Veli-Matti Kerminen et al. “Atmospheric new particle formation and growth: review of field observations”. In: Environmental Research Letters 13.10 (Sept. 2018), p. 103003. issn: 1748-9326. doi: 10.1088/1748-9326/aadf3c. url: http://dx.doi.org/10.1088/1748-9326/aadf3c.

[3] Jonas Elm et al. “Quantum chemical modeling of organic enhanced atmospheric nucleation: A critical review”. In: WIREs Computational Molecular Science 13.5 (May 2023). issn: 1759-0884. doi: 10.1002/wcms.1662. url: http://dx.doi.org/10.1002/wcms.1662.

How to cite: Bandeira, L., Sandström, H., and Rinke, P.: Machine Learning Interatomic Potential for Atmospheric Chemistry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15787, https://doi.org/10.5194/egusphere-egu25-15787, 2025.

The atmospheric oxidation of aromatic hydrocarbons contributes to the formation of secondary organic aerosol (SOA). Phenolic compounds are aromatic products from the OH oxidation of primary aromatics such as benzene, toluene, xylenes and others. They are an important class of atmospheric trace gases as they are efficient SOA precursors, even more efficient than the parent aromatics (Nakao et al. 2011). As compounds oxidize, they accumulate oxygen-containing functional groups. This lowers the volatility of the compounds, and condensation to the particle phase is possible. Explicit oxidation mechanisms are needed in order to understand this process and to better model SOA formation in the atmosphere.

Current molecular scale understanding of how phenolics oxidize cannot explain the high SOA potentials of these compounds. To address this, we use quantum chemical methods to study the early steps of OH oxidation of phenol, cresol, catechol and methylcatechol, and show that the largely neglected geminal diol pathway is key to the rapid formation of highly oxygenated low-volatility products. OH addition to the OH-substituted carbon in the phenolic precursor leads to a geminal diol alkyl radical that can add O2 and, over two rapid steps, lead to a geminal diol bicyclic peroxy radical (BPR). It has previously been shown that certain BPRs from primary aromatics such as toluene and xylene undergo molecular rearrangement reactions that break both structural rings at rate coefficients close to 1 s-1. These ring broken peroxy radicals oxidize more efficiently, and the fast rate of the molecular rearrangement reaction makes the formation of SOA precursors competitive even under polluted conditions (Iyer et al. 2023). Remarkably, geminal diol BPRs undergo molecular rearrangement reactions that are about 3 orders of magnitude faster, directly producing less volatile peroxy radicals with carboxylic acid functionalities that are also efficient at oxidizing further. The fraction of the initial geminal diol alkyl radical goes from minor for phenol to the dominant fate for catechol, explaining the increasing SOA potential trend, benzene < phenol < catechol, observed in measurements. (Borrás et al. 2012)

Primary aromatics in the atmosphere are constantly oxidized and either directly lead to SOA or produce phenolic products with SOA potentials of their own. It has been known for some time that the SOA potentials of phenolics outcompete those of the parent aromatics, and this work provides the first molecular scale mechanisms that explain why. These mechanisms are crucial blueprints needed to model SOA yields at different stages of aromatic oxidation and help to characterize the multigenerational nature of SOA production from aromatic oxidation.

References:
Nakao, S. et al. (2011) Secondary organic aerosol formation from phenolic compounds in the absence of NOx. Atmos. Chem. Phys. 11, 10649–10660.

Iyer, S. et al. (2023) Molecular rearrangement of bicyclic peroxy radicals is a key route to aerosol from aromatics. Nat Commun 14, 4984.
Borrás, E. Et al. (2012) L. A. Secondary organic aerosol formation from the photo-oxidation of benzene. Atmos. Environ. 47, 154–163.

How to cite: Ojala, A. and Iyer, S.: Role of the geminal diol pathway in organic aerosol formation from multigenerational aromatic oxidation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16753, https://doi.org/10.5194/egusphere-egu25-16753, 2025.

EGU25-17320 | Orals | AS3.37

Photodegradation of 1-nitronaphthalene, 2-nitronaphthalene, and 2-methyl-1-nitronaphthalene in the atmosphere 

Sergio Blázquez, Rubén Soler, Mila Ródenas, Teresa Vera, Esther Borrás, Christina Quaassdorff, Alberto Notario, and Amalia Muñoz

Polycyclic aromatic hydrocarbons (PAHs) are ubiquitous compounds in the atmosphere. These compounds cover a wide range of structures and chemical properties. Among them, nitro derivatives of PAHs (nitro-PAHs) are of particular interest. Nitro-PAHs are formed both by direct emissions, such as from diesel combustion engines, and by secondary reactions, such as nitration of parent PAHs. Furthermore, nitro-PAHs are recognized as toxic pollutants with adverse effects on human health [1], requiring detailed studies of their atmospheric behavior, transformations and effects.

This work focuses on three nitro-PAHs: 1-nitronaphthalene (1NN), 2-nitronaphthalene (2NN) (being these two the most abundant nitro-PAHs in the gas phase [2]), and 2-methyl-1-nitronaphthalene (2M1NN) (frequently detected in diesel exhaust [3]). The photolysis of these compounds was studied in order to understand their degradation pathways and to identify their main reaction products.

Experiments were carried out under sunlight conditions at the outdoor EUropean PHOtoREactor (EUPHORE) in Valencia, Spain.

A comprehensive suite of analytical techniques was employed, including chemical ionization mass spectrometry (CIMS), proton transfer-time of flight-mass spectrometry (PTR-ToF-MS), Fourier transform infrared (FTIR) spectroscopy, scanning mobility particle sizer (SMPS), among others. The main reaction products detected have been certain common acids such as nitrous, formic, acetic, nitric, or lactic acids. These methods provided detailed insights into the chemical transformations and effects of nitro-PAHs under atmospheric conditions, contributing to a better understanding of their environmental and health impacts. In addition, other compounds have been detected, albeit in smaller quantities, due to the partial decomposition of these nitronaphthalenes, such as 1- and 2-napthol, 2-carboxybenzaldehyde, or nitrobenzoic acid. This study sheds light on the nature of these nitronaphthalenes and their reaction mechanism in the atmosphere.

This work is part of a project that is supported by CAPOX RTI2018-097768-B-C21 funded by MCIN and co-funded by ERDF, by ATMOBE PID2022-142366OB-I00 funded by MCIN/AEI/10.13039/501100011033, by “ERDF A way of making Europe”, and by PROMETEO (EVER project) CIPROM/2022/37.

 

References:

[1] Benbrahim-Tallaa, L. et al., Lancet Oncol. 2012, 13, 663.

[2] Albinet, A. et al. Sci. Total Environ. 2007, 384, 280.

[3] Paputa-Peck, M.C. et al. Anal. Chem. 1983, 55, 1946.

How to cite: Blázquez, S., Soler, R., Ródenas, M., Vera, T., Borrás, E., Quaassdorff, C., Notario, A., and Muñoz, A.: Photodegradation of 1-nitronaphthalene, 2-nitronaphthalene, and 2-methyl-1-nitronaphthalene in the atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17320, https://doi.org/10.5194/egusphere-egu25-17320, 2025.

EGU25-17557 | Orals | AS3.37

Comparison of ROx radicals measurements in the atmospheric simulation chamber SAPHIR 

Anna Novelli, Weidong Chen, Sebastian Dusanter, Christa Fittschen, Maria Dolores Andrés Hernández, Kubistin Dagmar, Coralie Schoemaecker, Lisa Whalley, Weixiong Zhao, and Hendrik Fuchs and the ROxCOMP team

Accurate measurements of organic peroxy radicals (RO₂) are critical to understanding the formation of secondary pollutants, as the loss rate of RO2 radicals determines the rate and fraction of ozone (O3) and particulate matter formed. Due to their large structural variability and low concentrations in the troposphere, the measurement of RO2 radicals in ambient air is challenging, with most techniques relying on conversion to other species before detection.

In the summer of 2022, a series of experiments covering a wide range of chemical conditions were carried out in the SAPHIR atmospheric simulation chamber at Forschungszentrum Jülich. The experiments focused on the oxidation of biogenic and anthropogenic precursors at current and future nitrogen oxides levels (from a few ppb to a few ppt of nitric oxide), using different oxidants such as hydroxyl radical (OH), O3, and nitrate radicals (NO3), covering daytime and nighttime conditions. One experiment was conducted by flushing the chamber with ambient air. Three different techniques were compared: PEroxy Radical Chemical Amplification (PERCA, three research groups), Laser Induced Fluorescence (LIF, three research groups) and Chemical Ionization Mass Spectrometry (CIMS, one research group).

Overall, good agreement (within the stated accuracy of each instrument) was found for most of the conditions investigated, with deviations observed for one PERCA instruments for high temperatures and acyl peroxyl nitrates (APNs) concentrations. The results highlight the strengths and limitations of each measurement method in terms of sensitivity, accuracy, temporal resolution and potential interferences from other species.

How to cite: Novelli, A., Chen, W., Dusanter, S., Fittschen, C., Andrés Hernández, M. D., Dagmar, K., Schoemaecker, C., Whalley, L., Zhao, W., and Fuchs, H. and the ROxCOMP team: Comparison of ROx radicals measurements in the atmospheric simulation chamber SAPHIR, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17557, https://doi.org/10.5194/egusphere-egu25-17557, 2025.

EGU25-18142 | ECS | Posters on site | AS3.37

Investigation of APNs Chemistry from the Oxidation of Volatile Organic Compounds in the Atmospheric Simulation Chamber SAPHIR 

Yichen Gu, Franz Rohrer, Robert Wegener, Eva Y. Pfannerstill, Michelle Färber, Birger Bohn, Hendrik Fuchs, and Anna Novelli

Acyl peroxy nitrates (APNs) are important secondary pollutants in the troposphere, acting as reservoir for NOx (=NO2+NO). The relatively long lifetime of APNs (around 40 min at 298K) allows them to be transported from highly polluted areas to remote areas, causing an increase in both NOx and ozone concentrations on site. Various techniques are used to measure APNs in both field and laboratory experiments. These include direct methods such as Gas Chromatography (GC), and Chemical Ionization Mass Spectrometry (CIMS), as well as indirect methods such as Thermal Decomposition (TD) where APNs are decomposed and NO2 is detected.

In this contribution, the chemistry of APNs generated by the oxidation of different BVOCs (Biogenic Volatile Organic Compounds) is investigated at different levels of NOx. A series of experiments was conducted in the atmospheric simulation chamber SAPHIR, Forschungszentrum Jülich, Germany using a newly developed TD instrument which measures NO2 by Iterative Cavity enhanced DOAS (ICAD). To investigate formation of APNs from species emitted by the chamber foil (e.g., acetaldehyde) experiments injecting only methane and/or CO were conducted to obtain a baseline value for the experiments with BVOCs. These were followed by experiments with isoprene, α-pinene, and β-pinene for NO ranging between 0.3 and 9 ppbv using hydroxyl (OH) and nitrate (NO3) radicals as oxidants. Measured APNs as well as precursors and radicals were compared with results from zero-dimensional box model calculations using the Master Chemical Mechanism (MCM v 3.3.1).

How to cite: Gu, Y., Rohrer, F., Wegener, R., Pfannerstill, E. Y., Färber, M., Bohn, B., Fuchs, H., and Novelli, A.: Investigation of APNs Chemistry from the Oxidation of Volatile Organic Compounds in the Atmospheric Simulation Chamber SAPHIR, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18142, https://doi.org/10.5194/egusphere-egu25-18142, 2025.

EGU25-18730 | Posters on site | AS3.37

Characterization of APi-ToF-CIMS Sensitivity to Multifunctional Organic Molecules at EUPHORE Chambers 

Rubén Soler, Ezra Wood, Teresa Vera, Mila Ródenas, Esther Borrás, and Amalia Muñoz

We conducted a series of tests using the FIGAERO-HR-ToF-CIMS to assess its sensitivity to a diverse array of multifunctional organic molecules. These experiments were conducted under dark conditions in the 200 m³ outdoor chambers at EUPHORE, ensuring nearly stable concentrations of the studied compounds within a controlled environment.

 

The goal of these tests was to characterize the state-of-the-art instruments I-HR-ToF-CIMS coupled with the FIGAERO inlet, which allows both gas and particle phase analysis. It aimed at exploring the limits of the instruments, optimizing their performance, and ensuring the quality of their data. A series of compounds at nearly stable concentrations were measured under a range of declustering conditions, determined by the voltage settings in the transfer stages between the ion molecule reactor (IMR) and the ToF region. The concentration of the compounds was quantified using the FTIR and PTR-TOF-MS techniques.

 

These tests comprised two types: one involving the introduction of compounds into the chamber and another derived from biomass burning experiments. The relationship between the “dV50” and the sensitivity has been explored. Overall, higher dV50 values were observed compared to the consulted literature (Lopez-Hilkfiker et al. 2016), demonstrating the importance of characterizing each individual instrument. These results are connected to a series of compounds, among which formic acid, nitric acid, and propionic acid are included, that we aim to expand on to better understand the instrument's sensitivity. This instrumental characterization is contributing to a molecular characterization of gas- and particulate phase biomass burning compounds studied in the EUPHORE chamber.

 

This work is part of a project supported by the European Commission under the Horizon 2020 – Research and Innovation Framework Programme through the ATMO-ACCESS Integrating Activity (H2020-INFRAIA-2020-1) and by the R+D project ATMOBE (PID2022-142366OB-I00), funded by MCIN/AEI/10.13039/501100011033/, the "ERDF A way of making Europe”, the Valencian Regional Government (GVA) and the EVER project (CIPROM/2022/37). EUPHORE is part of the ACTRIS (Aerosol, Clouds and Trace Gases Research Infrastructure) network. Acknowledgements to the staff members Tatiana Gómez, Maria L. Martínez, and the PhD student Beatriz Domínguez for their collaboration in performing the experiments.

 

References:

Lopez-Hilfiker, F. D., Iyer, S., Mohr, C., Lee, B. H., D'Ambro, E. L., Kurtén, T., and Thornton, J. A.: Constraining the sensitivity of iodide adduct chemical ionization mass spectrometry to multifunctional organic molecules using the collision limit and thermodynamic stability of iodide ion adducts, Atmos. Meas. Tech., 9, 1505–1512, https://doi.org/10.5194/amt-9-1505-2016, 2016.

How to cite: Soler, R., Wood, E., Vera, T., Ródenas, M., Borrás, E., and Muñoz, A.: Characterization of APi-ToF-CIMS Sensitivity to Multifunctional Organic Molecules at EUPHORE Chambers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18730, https://doi.org/10.5194/egusphere-egu25-18730, 2025.

EGU25-19209 | ECS | Orals | AS3.37

Binding free energy from umbrella sampling at ML-enhanced Born-Oppenheimer MD simulations 

Jakub Kubecka, Georg Baadsgaard Trolle, Yosef Knattrup, Jonas Elm, and Ivo Neefjes
Molecular dynamics (MD) simulations of systems with many atoms are often constrained by computational limitations, requiring either short simulation times or the use of force-field methods. Recently, we demonstrated that machine-learning (ML) potentials can be trained on small molecular systems, such as molecular clusters, that are computationally explorable via accurate quantum chemistry methods. These ML potentials can subsequently be used to model larger molecular systems while maintaining the same energy-per-atom and force-per-atom accuracy. This allows us to perform Born-Oppenheimer MD (BOMD) simulations using Hamiltonians derived from ML-modeled quantum chemistry calculations.
 
In this work, we calculate the binding free energies of molecular clusters using umbrella sampling (US) combined with the aforementioned ML-enhanced BOMD simulations. We validated this approach on small molecular dimers, such as water and sulfuric acid dimers, where the use of a low level of theory (e.g., GFN1-xTB) allowed us to perform and compare quantum chemistry calculations, BOMD, and ML-enhanced BOMD simulations. Furthermore, we extended the methodology to compute the binding free energies of larger molecular clusters.
 
Our approach highlights the advantage of US in accounting for free energy contributions arising from multiple energy minima (i.e., conformers) and vibrational anharmonicity. These entropic effects, often neglected in traditional statistical thermodynamics applied to quantum chemistry calculations, are crucial for an accurate understanding of binding free energies in complex molecular systems.

How to cite: Kubecka, J., Trolle, G. B., Knattrup, Y., Elm, J., and Neefjes, I.: Binding free energy from umbrella sampling at ML-enhanced Born-Oppenheimer MD simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19209, https://doi.org/10.5194/egusphere-egu25-19209, 2025.

EGU25-19459 | Orals | AS3.37

Investigation of the light absorption properties of wood combustion particles using the extended wavelength range of the new AE36s Aethalometer 

Bálint Alföldy, Asta Gregorič, Irena Ježek-Brecelj, Matic Ivančič, Mila Ródenas, Rubén Soler, Amalia Muñoz Cintas, Teresa Vera Espallardó, Esther Borras, Eduardo Yubero, Jaime Javier Crespo Mira, and Martin Rigler

Particulate matter from wood combustion has a significant impact on climate and human health. Black carbon (BC) and brown carbon (BrC) are strong light absorbers that reduce the transparency of the atmosphere in the long and short wavelength range. As the aerosol ages, some of the molecular chromophores break down and the particles become less absorbent (photobleaching). On the other hand, photochemical ageing can modify organic molecules, which become light-absorbing even though they were colorless after emission. In addition, the secondary formed particles increase the light absorption and scattering of the pollution emitted by wood burning. To better estimate the contribution of particles emitted from wood combustion to the global radiation balance, it is therefore necessary to understand the optical properties of secondary particles and the changes in optical properties with ageing of primary aerosols. Limited information is available, in particular on the light absorption in the deep UV region where BrC is expected to have significant absorption. To extend the spectral information on the aerosol light absorption, the aerosol sample from wood combustion was measured with the new Aethalometer model (AE36s, Aerosol Magee Scientific), which has a spectral resolution of nine wavelengths in the 340-950 nm interval. The measurements were performed in the 200 m3 simulation chamber of the CEAM-EUPHORE research center in Valencia, Spain. Flaming and smoldering burning conditions were separately investigated and compared to diesel emission. After emission, the combustion products were introduced into the chamber, where the particles were subjected to different types of ageing (photooxidation, dark ageing). In addition to the light absorption, light scattering of the particles was measured by a nephelometer (Aurora 3000, ACOEM). The OC/BC ratio was also measured using the real-time Carbonaceous Aerosol Speciation System (CASS, Aerosol Magee Scientific). Particle formation and growth dynamics were monitored by SMPS (TSI) measurement. The optical properties of the primary emitted particles can be related to the combustion mode. Diesel emission resulted in the most absorbing aerosol over the whole wavelength range, while particles emitted from smoldering wood burning were the least absorbing, except in the UV range where BrC has high absorbance. During the photooxidation period, significant changes in the optical properties of the aerosol were observed. The absorbance of particles from smoldering emission increased significantly after the light exposure in the 470-660 nm wavelength interval. Later the absorbance decreased due to the photobleaching effect. During the photooxidation period, secondary organic aerosol formation was observed. The increase in absorbance was found to be lower than the increase in mass of the newly formed particles, while the increase in light scattering exceeded the increase in particle mass. These results suggest that the secondary aerosol was mostly transparent or had lower mass absorption efficiency but a higher scattering cross section compared to the primary emission. Therefore, the consideration of secondary formation and aging is crucial for a better understanding of the climate impact of wood combustion aerosol.

How to cite: Alföldy, B., Gregorič, A., Ježek-Brecelj, I., Ivančič, M., Ródenas, M., Soler, R., Muñoz Cintas, A., Espallardó, T. V., Borras, E., Yubero, E., Crespo Mira, J. J., and Rigler, M.: Investigation of the light absorption properties of wood combustion particles using the extended wavelength range of the new AE36s Aethalometer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19459, https://doi.org/10.5194/egusphere-egu25-19459, 2025.

EGU25-19764 | Orals | AS3.37

A novel chemical ionization source for proton-transfer-reaction mass spectrometry and other chemical ionization schemes  

Vasyl Yatsyna, Imad Zgheib, Matthieu Riva, Michael Kamrath, Urs Rohner, Hariprasad Alwe, and Felipe Lopez-Hilfiker

We present the development and characterization of a novel chemical ionization source useful for sensitive detection and analysis of atmospherically-relevant species in real time. The source can be used for proton-transfer-reaction mass spectrometry (PTR-MS) as well as other chemical ionization schemes generating both positive and negative analyte ions. It features fast reagent ion switching on the timescale of seconds or better, and can be operated in a broad range of ion-molecule reactor pressures (0.1 - 10 mbar) and sample flows. We couple the novel source with the high-resolution time-of-flight mass spectrometer and demonstrate sub pptv detection limits (<<1 pptv) along with a high dynamic range. We also present two weeks of ambient measurements in Thun, Switzerland using the novel ionization source switching between H3O+ and O2+ reagent ions as well as flow tube experiments which demonstrate the utility of multiple reagent ion switching between positive and negative ion modes.   

How to cite: Yatsyna, V., Zgheib, I., Riva, M., Kamrath, M., Rohner, U., Alwe, H., and Lopez-Hilfiker, F.: A novel chemical ionization source for proton-transfer-reaction mass spectrometry and other chemical ionization schemes , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19764, https://doi.org/10.5194/egusphere-egu25-19764, 2025.

EGU25-21308 | ECS | Posters on site | AS3.37

Secondary Organic Aerosol Formation from the Photooxidation of Naphthalene and Benzene Mixtures under Different Reaction Conditions 

Amir Ben Brik, Merve Polat, Niall O'Sullivan, Mixtli Campos-Pineda, Marteen Kieft, Jakob Klenø Nøjgaard, Matthew Stanley Johnson, Albert Andy Ruth, and John Wenger
The atmospheric oxidation of aromatic hydrocarbons is a major source of secondary organic aerosol (SOA). This study investigates the OH-initiated oxidation of naphthalene (Nap) and benzene (Bz) mixtures under a variety of reaction conditions. Nap and Bz are common air pollutants produced from fuel combustion and are also simultaneously present at high concentrations in asphalt pavement emissions.
Experiments were conducted in the Irish Atmospheric Simulation Chamber, a 27 m³ Teflon reactor, where Nap and Bz were exposed to OH radicals generated via H₂O₂ photolysis. The photooxidation of Nap and Bz was investigated individually and in combination under varying NOx, SO2 and relative humidity (RH) conditions. Gas phase products were monitored using a Time-of-Flight Chemical Ionization Mass Spectrometer (ToF-CIMS) coupled to a Filter Inlet for Gases and AEROsol (FIGAERO) for particle composition analysis using both toluene and iodide as reagent ions. Aerosol number and mass evolution were measured using a Scanning Mobility Particle Sizer (SMPS), while NOx, SO2 and O3 concentrations were monitored with automated gas analysers and a custom-designed cavity enhanced absorption setup.
Analysis of experiments under high and low NOx conditions have so far shown that Nap + OH and Bz + OH reactions yielded C10H8O+ (m/z 144) and C6H6O⁺ (m/z 94) as the main primary products, respectively, corresponding to the addition of a hydroxyl group. Intense signals at m/z 160 and m/z 110 were subsequently observed, i.e. the addition of a second OH group. Experiments on Nap/Bz mixtures resulted in the same products, even in the presence of NO, which also produced nitroaromatic compounds like C10H7NO3+ (m/z 189) and C6H5NO3+ (m/z 139). A range of C12, C16 and C20 compounds were also identified and assigned to dimers produced from self- and cross-reactions of C6 and C10 radicals produced during the photooxidation process. The photooxidation of Bz alone (up to 120 ppbv) did not produce SOA. In contrast, SOA formation from Nap (30 ppbv) was rapid and affected by the reaction conditions. RH strongly influenced SOA formation, with lower RH delaying particle growth and reducing total mass. Introducing NO (55–144 ppbv) to the Nap + OH system enhanced SOA formation, while adding Bz suppressed SOA formation.
First results of SO2 experiments show that the addition of SO2 (17 ppbv) to the Nap + Bz + OH mixture significantly accelerated SOA formation, nearly doubling the SOA mass, particularly in the presence of NO. Future work will focus on completing the experimental matrix to deepen our understanding of chemical mechanisms leading to the formation of the detected products.

How to cite: Ben Brik, A., Polat, M., O'Sullivan, N., Campos-Pineda, M., Kieft, M., Nøjgaard, J. K., Johnson, M. S., Ruth, A. A., and Wenger, J.: Secondary Organic Aerosol Formation from the Photooxidation of Naphthalene and Benzene Mixtures under Different Reaction Conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21308, https://doi.org/10.5194/egusphere-egu25-21308, 2025.

EGU25-21431 | ECS | Orals | AS3.37

Coalescence of Two Carbonaceous Nanoparticles: A Steered Molecular Dynamics Study of the First Steps of the Soot Aggregate Formation 

Nicolas Brosseau-Habert, Maria Lbadaoui-Darvas, Michel Devel, and Sylvain Picaud

Soot nanoparticles, resulting from incomplete combustion processes of fossil fuel or biomass, play a central role in many environmental and industrial phenomena, while posing major challenges for public health and global warming estimate. A better quantification of all the soot impact is thus strongly needed, which requires a better understanding of their formation and ageing processes. Experiments carried out on the structure of soot nanoparticles highlighted that their morphology is characterized by aggregation of spherical primary soot grains (carbonaceous spherules of a few to tens of nanometers in size), the resulting aggregates being of submicrometer size [1,2]. 

In the present work, we have used the steered molecular dynamics (MD) method [3] to investigate, at the atomic level, the coalescence of two carbonaceous spherules, aiming at modeling thus the very first steps of the aggregation process. Computations have been performed with the molecular dynamics software LAMMPS, and the AIREBO interaction potential model has been used to calculate the carbon-carbon interactions in the corresponding systems. Because it is the first time (as far as we know) that such an approach is used in this context, a thorough investigation of the influence of the intrinsic parameters of the steered MD on the results has been performed, by varying the temperature, the duration of the simulations, the spring constant values, and the thermostat. This work, which can thus be viewed as a mandatory stage for our studies on spherule aggregation, emphasizes that using steered MD is a promising approach for accurately modeling, at the atomic scale, structural changes resulting from soot aging.

[1] H. Michelsen, Probing soot formation, chemical and physical evolution, and oxidation: A review of in situ diagnostic techniques and needs, Proceedings of the Combustion Institute, 36 (2017) 717–735

[2] P. Parent et al., Nanoscale characterization of aircraft soot: A high-resolution transmission electron microscopy, raman spectroscopy, X-ray photoelectron and near-edge X-ray absorption spectroscopy study, Carbon, 101 (2016) 86–100.

[3] M. Lbadaoui-Darvas et al., Molecular-scale description of interfacial mass transfer in phase-separated aqueous secondary organic aerosol, Atmos. Chem. Phys., 21 (2021) 17687-17714 

How to cite: Brosseau-Habert, N., Lbadaoui-Darvas, M., Devel, M., and Picaud, S.: Coalescence of Two Carbonaceous Nanoparticles: A Steered Molecular Dynamics Study of the First Steps of the Soot Aggregate Formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21431, https://doi.org/10.5194/egusphere-egu25-21431, 2025.

EGU25-267 | ECS | Orals | BG1.2

Uncertainties in carbon emissions from land use and land cover change in Indonesia 

Ida Bagus Mandhara Brasika, Pierre Friedlingstein, Stephen Sitch, Michael O'Sullivan, Maria Carolina Duran-Rojas, Thais Michele Rosan, Kees Klein Goldewijk, Julia Pongratz, Clemens Schwingshackl, Louise Chini, and George Hurtt

Indonesia is currently one of the three largest contributors of carbon emissions from land use and land cover change (LULCC) globally, together with Brazil and the Democratic Republic of the Congo. However, until recently, there was only limited reliable data available on LULCC across Indonesia, leading to a lack of agreement on drivers, magnitude, and trends in carbon emissions between different estimates. Accurate LULCC should improve robustness and reduce the uncertainties of carbon dioxide (CO2) emissions from Land Use Change (ELUC) estimation. Here, we assess several cropland datasets that are used to estimate ELUC in Dynamic Global Vegetation Models (DGVMs) and Bookkeeping models (BKMs). Available cropland datasets are generally categorized as either census-based such as the Food and Agricultural Organization (FAO) annual statistical dataset, or satellite-based such as the Mapbiomas dataset, which is derived from Landsat Satellite images. Our results show that census-based and satellite-based estimates have little agreement on temporal variability and cropland area changes. In some islands, they show spatial similarity, but differences appear in the main islands such as Kalimantan, Sumatra and Java. These differences lead to spatio-temporal uncertainty in carbon emissions. The different land cover forcings (census-based vs satellite-based) in a single model (JULES-ES) result in ELUC uncertainties of about 0.08 [0.06 to 0.11]  PgC/yr. Furthermore, we found that uncertainties in ELUC estimates are also due to differences in the carbon cycle models in DGVMs, as DGVMs driven by the same land cover dataset show differences in ELUC estimates of 0.12 ± 0.02 PgC/yr with 95% confidence level and range [-0.04 to 0.35] PgC/yr. This is consistent with other product such as BKMs that estimates 0.14 [0.12 to 0.15] PgC/yr with both steady trend. We also compare emissions with those from the National Greenhouse Gas Inventory (NGHGI) product. The NGHGI estimates (based on BUR3; periodic official government report on Greenhouses Gas to UNFCCC) have much lower carbon emissions (0.06 ± 0.06 PgC/yr), though with an increasing trend. These numbers double when we include emissions from peat fire and peat drainage: the DGVM ensemble indicates emissions of 0.23 ± 0.05 PgC/yr and BKMs indicate emissions of 0.24 [0.22-0.25] PgC/yr. In contrast, emissions based on the Indonesian NGHGI remain much lower (BUR2: 0.18±0.07 PgC/yr BUR3: 0.13 ± 0.10 PgC/yr). Furthermore, emission peaks occur in year of moderate-to-strong El Nino events. Several improvements might reduce uncertainties in carbon emissions from LULCC in Indonesia, such as: combination of satellite-based dataset with census-based dataset, inclusion of peat-related emissions in DGVMs and potentially explicit inclusion of palm oil in the models as this is a major crop in Indonesia. Overall, the analysis shows that carbon emissions have no decreasing trend in Indonesia, Therefore, deforestation and forest fire prevention remain vital for Indonesia. 

How to cite: Brasika, I. B. M., Friedlingstein, P., Sitch, S., O'Sullivan, M., Duran-Rojas, M. C., Rosan, T. M., Goldewijk, K. K., Pongratz, J., Schwingshackl, C., Chini, L., and Hurtt, G.: Uncertainties in carbon emissions from land use and land cover change in Indonesia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-267, https://doi.org/10.5194/egusphere-egu25-267, 2025.

EGU25-1596 | ECS | Posters on site | BG1.2

Hurricanes trigger ocean CO2 uptake and phytoplankton bloom in a high-resolution Earth system model simulation 

David M. Nielsen, Fatemeh Chegini, Nuno Serra, Arjun U. Kumar, Nils Brueggemann, Cathy Hohenegger, and Tatiana Ilyina

North Atlantic tropical cyclones (i.e. hurricanes) are observed to drive intense air-sea CO2 exchange and trigger primary production by phytoplankton. However, Earth system models (ESMs) with coarse spatial resolution are not able to capture such effects. Here, we address this limitation and resolve the impacts of hurricanes on the ocean carbon cycle in an ESM for the first time. We present the first 1-year global, coupled, high-resolution (5 km ocean, 5 km atmosphere) ESM simulation including ocean biogeochemistry with the ICON (ICOsahedral Non-hydrostatic) model framework. Our simulation realistically reproduces the effects of hurricanes at: 1) instantaneously increasing air-sea CO2 fluxes by a factor of 10-30 due to strong surface winds (>58 m/s, hurricane category 4); 2) promoting longer-lasting surface ocean cooling by 2-4°C, and thus decreasing surface ocean partial pressure of CO2 (pCO2); and 3) triggering large-scale phytoplankton blooms, spatially modulated by mesoscale ocean eddies. We show that the hurricane-driven sea-surface cooling is mainly caused by extreme latent heat loss (>1200 W/m2), whose impact on decreasing pCO2 outweighs the mixing and upwelling of dissolved inorganic carbon. Our simulated hurricanes contribute to inverting the direction of the local air-sea pCO2 imbalance, thus promoting ocean CO2 uptake. Intense wind speeds also trigger vertical diffusion of nutrients, as well as near-inertial oscillations, which become the dominant mode of subsurface ocean variability in the wake of the cyclones. While the proportion of intense tropical cyclones is projected to increase with climate change, their future role in the ocean carbon cycle remains unclear. Resolving tropical cyclones in ESMs will allow us to better understand their response and impact to ongoing climate change at regional and global scales.

How to cite: Nielsen, D. M., Chegini, F., Serra, N., U. Kumar, A., Brueggemann, N., Hohenegger, C., and Ilyina, T.: Hurricanes trigger ocean CO2 uptake and phytoplankton bloom in a high-resolution Earth system model simulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1596, https://doi.org/10.5194/egusphere-egu25-1596, 2025.

EGU25-2043 | ECS | Posters on site | BG1.2

Increasing Methane Summer Diurnal Amplitude in Siberia: A 2010–2021 Analysis from the ZOtino Tall Tower Observatory (ZOTTO) 

Dieu Anh Tran, Jordi Vilà-Guerau de Arellano, Ingrid Luijkx, Santiago Botía, Kim Faassen, Christoph Gerbig, and Sönke Zaehle

Siberia’s extensive wetlands, permafrost, and boreal forests are significant sources of methane, positioning this region as crucial for global methane (CH4) monitoring. However, Siberia remains sparsely monitored by atmospheric and ecosystem observatories, highlighting the need to leverage existing datasets to refine CH4 budgets with better spatial and temporal precision. Utilising the ZOtino Tall Tower Observatory (ZOTTO; 60°48' N, 89°21' E) dataset, which provides continuous, high-resolution CH4 mole fraction and meteorological measurements from six heights up to 301 meters, combined with ERA5 meteorological data at 60°75' N, 89°25' E, we conducted a comprehensive analysis of long-term trends and variations in atmospheric CH4 at ZOTTO, examining its diurnal and seasonal patterns from 2010 to 2021. Our analysis reveals a significant increase in the summer diurnal amplitude of CH4, which could be driven by both forest and meteorological dynamics, through the effects of daytime mixing and nighttime stability on the CH4 mole fraction, and ecosystem CH4 flux. We found that while atmospheric dynamics showed no significant trends contributing to this diurnal amplitude increase, there was an increasing trend in nighttime CH4 ecosystem flux in summer (predominantly August) over the 11-year period, with high emissions predominantly originating from the west and southwest of the station. Additionally, episodic high methane CH4 was observed in 2012 and 2019, linked to wildfires, and in 2016, attributed to enhanced wetland activity. Lastly, there were significant positive correlations between the calculated CH4 surface flux and soil temperature and moisture at ZOTTO.

How to cite: Tran, D. A., Vilà-Guerau de Arellano, J., Luijkx, I., Botía, S., Faassen, K., Gerbig, C., and Zaehle, S.: Increasing Methane Summer Diurnal Amplitude in Siberia: A 2010–2021 Analysis from the ZOtino Tall Tower Observatory (ZOTTO), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2043, https://doi.org/10.5194/egusphere-egu25-2043, 2025.

EGU25-2215 | ECS | Orals | BG1.2

Global trends in ocean fronts: impacts on air-sea CO2 flux and chlorophyll concentrations 

Kai Yang, Amelie Meyer, Peter G. Strutton, and Andrew M. Fischer

Ocean fronts are dynamic features that play a critical role in regulating marine ecosystems and influencing global carbon cycles. These regions, characterized by strong horizontal gradients in temperature, salinity, and other properties, enhance vertical mixing and advection, driving increased nutrient supply that supports elevated primary production. Despite their importance, the impacts of changing ocean fronts on the budget and trends of ocean CO2 uptake remain insufficiently understood. In this study, we perform a comprehensive global analysis of ocean fronts using 20 years of satellite observations (2003–2023), identifying key regions of intense frontal activity and areas undergoing rapid changes in frontal dynamics. Our results show that nearly 50% of global ocean CO2 uptake occurs in these key frontal areas, underscoring their disproportionate role in the ocean’s carbon sink. Furthermore, we observe that trends in sea surface chlorophyll concentration—a proxy for primary production—and ocean CO2 uptake are strongly correlated with local changes in frontal activity. Our findings provide critical insights into the role of ocean fronts as modulators of global biogeochemical processes and air-sea CO2 exchanges. By linking ocean fronts to changes in primary production and air-sea CO2 exchange, this study contributes to a more detailed understanding of how changing ocean dynamics may influence carbon cycles under future climate scenarios.

How to cite: Yang, K., Meyer, A., Strutton, P. G., and Fischer, A. M.: Global trends in ocean fronts: impacts on air-sea CO2 flux and chlorophyll concentrations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2215, https://doi.org/10.5194/egusphere-egu25-2215, 2025.

EGU25-2466 | ECS | Posters on site | BG1.2

Underestimation of Methane Emissions From the Sudd Wetland: Unraveling the Impact of Wetland Extent Dynamics 

Bogang Dong, Shushi Peng, Gang Liu, Tianjiao Pu, Cynthia Gerlein‐Safdi, Catherine Prigent, and Xin Lin

Tropical wetlands account for ∼20% of the global total methane (CH4) emissions, but uncertainties remain in emission estimation due to the inaccurate representation of wetland spatiotemporal variations. Based on the latest satellite observational inundation data, we constructed a model to map the long-term time series of wetland extents over the Sudd floodplain, which has recently been identified as an important source of wetland CH4 emissions. Our analysis reveals an annual, total wetland extent of 5.73 ± 2.05 × 104 km2  for 2003–2022, with a notable accelerated expansion rate of 1.19 × 104 km2 yr−1 during 2019–2022 driven by anomalous upstream precipitation patterns. We found that current wetland products generally report smaller wetland areas, resulting in a systematic underestimation of wetland CH4 emissions from the Sudd wetland. Our study highlights the pivotal role of comprehensively characterizing the seasonal and interannual dynamics of wetland extent to accurately estimate CH4 emissions from tropical floodplains.

How to cite: Dong, B., Peng, S., Liu, G., Pu, T., Gerlein‐Safdi, C., Prigent, C., and Lin, X.: Underestimation of Methane Emissions From the Sudd Wetland: Unraveling the Impact of Wetland Extent Dynamics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2466, https://doi.org/10.5194/egusphere-egu25-2466, 2025.

EGU25-6054 | ECS | Posters on site | BG1.2

Four decades of full-scale nitrous oxide emission inventory in China 

Minqi Liang, Zheyan Zhou, Peiyang Ren, Han Xiao, Ri Xu, Zhongmin Hu, Shilong Piao, Hanqin Tian, Qing Tong, Feng Zhou, Jing Wei, and Wenping Yuan

China is among the top nitrous oxide (N2O)-emitting countries, but existing national inventories do not provide full-scale emissions including both natural and anthropogenic sources. We conducted a four-decade (19802020) of comprehensive quantification of Chinese N2O inventory using empirical emission factor method for anthropogenic sources and two up-to-date process-based models for natural sources. Total N2O emissions peaked at 2287.4 (1774.82799.9) Gg N2O yr-1 in 2018, and agriculture-developed regions, like the East, Northeast, and Central, were the top N2O-emitting regions. Agricultural N2O emissions have started to decrease after 2016 due to the decline of nitrogen fertilization applications, while, industrial and energetic sources have been dramatically increasing after 2005. N2O emissions from agriculture, industry, energy, and waste represented 49.3%, 26.4%, 17.5%, and 6.7% of the anthropogenic emissions in 2020, respectively, which revealed that it is imperative to prioritize N2O emission mitigation in agriculture, industry, and energy. Natural N2O sources, dominated by forests, have been steadily growing from 317.3 (290.3344.1) Gg N2O yr-1 in 1980 to 376.2 (335.5407.2) Gg N2O yr-1 in 2020. Our study produces a Full-scale Annual N2O dataset in China (FAN2020), providing emergent counting to refine the current national N2O inventories.

How to cite: Liang, M., Zhou, Z., Ren, P., Xiao, H., Xu, R., Hu, Z., Piao, S., Tian, H., Tong, Q., Zhou, F., Wei, J., and Yuan, W.: Four decades of full-scale nitrous oxide emission inventory in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6054, https://doi.org/10.5194/egusphere-egu25-6054, 2025.

EGU25-6416 | ECS | Posters on site | BG1.2

Analysis of ground-based column and in situ surface concentrations of CO2 at Xianghe, China, using WRF-Chem simulations 

Sieglinde Callewaert, Martine De Mazière, Minqiang Zhou, Ting Wang, Bavo Langerock, Pucai Wang, and Emmanuel Mahieu

Since June 2018, ground-based remote sensing measurements are performed at the suburban Xianghe site in China, situated in the heart of the densely populated Beijing-Tianjin-Hebei megalopolis. These observations are performed with Fourier Transform Infrared (FTIR) spectrometers and provide  column-averaged dry-air concentrations of gases such as CO2, CH4 and CO. They are affiliated to the international Total Column Carbon Observing Network (TCCON). Co-located with these measurements is a PICARRO cavity ring-down spectroscopy (CRDS) analyser observing in situ concentrations of CO2 and CH4 at an altitude of 60 m.

To gain a better understanding of the causes of the observed temporal variabilities at this site, we employed the Weather Research and Forecasting model coupled with Chemistry in its greenhouse gas configuration (WRF-GHG). Our study analyses both column-averaged (XCO2) and surface in situ CO2 concentrations and simultaneously evaluates the model’s performance at Xianghe.  The CO2 exchange with the biosphere is simulated with the integrated Vegetation Photosynthesis and Respiration Model (VPRM), while the anthropogenic emissions are taken from the global CAMS-GLOB-ANT inventory and transported in separate tracers according to their source sector. 

The model shows good performance, achieving correlation coefficients of 0.70 for XCO2 and 0.75 for afternoon in situ concentrations. For XCO2, a mean bias of -1.43 ppm relative to TCCON is found, primarily attributed to biases in the CAMS reanalysis used as initial and lateral boundary conditions. Anthropogenic emissions from the industry and energy sectors emerged as dominant contributors to CO2 concentrations, alongside the biosphere, which acts as a sink for XCO2 from April to September and becomes a source for the rest of the year. Synoptic weather patterns were shown to strongly determine the variation in CO2 levels, with enhanced impacts during summer due to the large spatial and temporal heterogeneity of biogenic fluxes in the region. Near the surface, the observed large diurnal variation associated to the evolution of the planetary boundary layer is  relatively well simulated by WRF-GHG.

Our analysis demonstrates the utility of WRF-GHG in simulating both column and surface CO2 concentrations, offering insights into the sectoral and meteorological drivers of variability at Xianghe and its surrounding region.

 

How to cite: Callewaert, S., De Mazière, M., Zhou, M., Wang, T., Langerock, B., Wang, P., and Mahieu, E.: Analysis of ground-based column and in situ surface concentrations of CO2 at Xianghe, China, using WRF-Chem simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6416, https://doi.org/10.5194/egusphere-egu25-6416, 2025.

EGU25-6427 | ECS | Orals | BG1.2

Improved air-sea CO2 flux estimates by adding sailboat measurements  

Jacqueline Behncke, Peter Landschützer, Fatemeh Chegini, and Tatiana Ilyina

Sailboats expand the observational network of sea surface partial pressure of CO2 (pCO2), particularly in the undersampled Southern Ocean through regularly repeating circumnavigations, however, their added value to the fCO2-product based ocean sink estimate (Socean) has thus far not been quantified. Here, we show through an observing system simulation study with different sampling schemes how integrating sailboat data from different race tracks improves air-sea CO2 flux estimates.
We find that neural network reconstruction of the air-sea CO2 flux used within the Global Carbon Budget, when reconstructing a model that mimics present-day real-world sampling, underestimates the ocean carbon sink. This is consistent with recent studies on the interior accumulation of carbon. Increased and continuous sampling by sailboats reveals a stronger carbon sink and improves present-day estimates from 0.06 to -0.02 mol C m⁻² yr⁻¹ (0.99 μatm to -0.32 μatm for the fCO2 estimate), particularly in the Southern Ocean between 40°S and 60°S. The improvement in reconstructions persists even when data from three circumnavigation tracks contain artificial measurement biases. However, the additional data remains insufficient to correct the overestimated air-sea CO2 flux trend. While sailboat data has the potential to improve air-sea CO2 flux reconstructions, expanding the observational network and maintaining long-term time series is crucial to minimize discrepancies between fCO2-products and Global Ocean Biogeochemical Models.

How to cite: Behncke, J., Landschützer, P., Chegini, F., and Ilyina, T.: Improved air-sea CO2 flux estimates by adding sailboat measurements , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6427, https://doi.org/10.5194/egusphere-egu25-6427, 2025.

EGU25-6908 | ECS | Orals | BG1.2

Upscaling near-real-time biospheric CO2 fluxes over Europe with a modified Vegetation Photosynthesis Respiration Model (VPRM) 

Otto Briner, Hassan Bazzi, Philippe Ciais, and Diego Santaren

Monitoring ecosystem carbon dioxide (CO2) exchange is crucial for assessing the impacts of climate extremes and constructing carbon budgets to inform land management and enforce international climate treaties. To this end, we present here gridded hourly ecosystem CO2 fluxes upscaled from eddy covariance observations at 0.1° × 0.1° resolution and updated at low latency. Sentinel-2 indices are used to drive a modified Vegetation Photosynthesis Respiration Model (VPRM) following Bazzi et al. (2024) with a restructured Ecosystem Respiration equation and explicit soil moisture stress functions. VPRM parameters are optimized to half-hourly eddy covariance Net Ecosystem Exchange (NEE) and Gross Primary Production (GPP) datasets for each of 36 FLUXNET sites. Additionally we modify the temperature dependence of GPP by optimizing minimum and maximum temperatures as parameters and estimating optimum temperatures from mean annual temperature. We find these temperature modifications reduce RMSE for NEE and GPP respectively by 11% and 12% overall, 16% and 18% at evergreen needleleaf forests, 14% and 12% at grasslands, and 12% and 16% at mixed forests. Using site data on meteorology and vegetation, we train a random forest to produce mapped VPRM parameters representing the spatial heterogeneity in ecosystem characteristics. Gridded VPRM NEE estimates are presented based on both modeled parameter maps and multi-site optimizations by plant functional type, and upscaled products can be produced within hours of satellite data availability.

 

[1] Bazzi, H. et al. "Assimilating Sentinel-2 data in a modified vegetation photosynthesis and respiration model (VPRM) to improve the simulation of croplands CO2 fluxes in Europe." International Journal of Applied Earth Observation and Geoinformation 127 (2024): 103666.

How to cite: Briner, O., Bazzi, H., Ciais, P., and Santaren, D.: Upscaling near-real-time biospheric CO2 fluxes over Europe with a modified Vegetation Photosynthesis Respiration Model (VPRM), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6908, https://doi.org/10.5194/egusphere-egu25-6908, 2025.

EGU25-7573 | Posters on site | BG1.2

Coupled Simultion of Atmospheric CO2 in CAS-ESM 

Jiawen Zhu, Juanxiong He, Duoying Ji, Yangchun Li, He Zhang, Minghua Zhang, Xiaodong Zeng, Kece Fei, and Jiangbo Jin

The atmospheric carbon dioxide (CO2) concentration has been increasing rapidly since the Industrial Revolution, which has led to unequivocal global warming and crucial environmental change. It is extremely important to investigate the interactions among atmospheric CO2, the physical climate  system, and the carbon cycle of the underlying surface for a better understanding of the Earth system. Earth system models are widely used to investigate these interactions via coupled carbon–climate simulations. The Chinese Academy of Sciences Earth System Model version 2 (CAS-ESM2.0) has successfully fixed a two-way coupling of atmospheric CO2 with the climate and carbon cycle on land and in the ocean. Using CAS-ESM2.0, we  conducted a coupled carbon–climate simulation by following the CMIP6 proposal of a historical emissions-driven experiment. This paper examines the modeled CO2 by comparison with observed CO2 at the sites of Mauna Loa and Barrow, and the Greenhouse Gases Observing Satellite (GOSAT) CO2 product. The results showed that CAS-ESM2.0 agrees very well with observations in reproducing the increasing trend of annual CO2 during the period 1850–2014, and in capturing the seasonal cycle of CO2 at the two baseline sites, as well as over northern high latitudes. These agreements illustrate a good ability of CAS-ESM2.0 in simulating carbon–climate interactions, even though uncertainties remain in the processes involved. This paper reports an important stage of the development of CAS-ESM with the coupling of carbon and climate, which will provide significant scientific support for climate research and China’s goal of carbon neutrality.

How to cite: Zhu, J., He, J., Ji, D., Li, Y., Zhang, H., Zhang, M., Zeng, X., Fei, K., and Jin, J.: Coupled Simultion of Atmospheric CO2 in CAS-ESM, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7573, https://doi.org/10.5194/egusphere-egu25-7573, 2025.

EGU25-7650 | Posters on site | BG1.2

Characteristics of carbon sink and the influence factors in Ngoring Lake, Qinghai-Tibet Plateau 

Mengxiao Wang, Lijuan Wen, Zhaoguo Li, Xianhong Meng, and Dongsheng Su

Lakes, as a fundamental component of the Earth's surface system, play a crucial role in the carbon cycle, closely linked to climate change. However, understanding carbon flux in Qinghai-Tibet Plateau (QTP) lakes is restricted by environmental factors and limited observations, hindering insights into regional and global climate change. Continuous annual carbon dioxide (CO2) flux, encompassing ice-covered periods, has been monitored in the largest freshwater lake on the QTP. Utilizing continuous eddy system data, the characteristics and mechanisms influencing carbon flux at various temporal scales in this lake were investigated. Findings revealed Ngoring Lake as predominantly a carbon sink year-round, with two CO2 absorption peaks in spring and autumn, respectively. These peaks were associated with mixing state triggered by cooling processes. In spring, as temperatures rose above the lake water's maximum density temperature (3.98 ℃ for freshwater lake), subsequent rapid cooling and mixing occurred upon ice melt. In autumn, cooling and mixing were induced by decreasing air and water temperatures alongside strong winds. These cooling processes facilitated significant CO2 absorption. As the lake transitioned from stratification to mixing, lake mixing played a dominant role. Biochemical reactions driven by water temperature play a dominant role during stable stratification and complete mixing phases.

How to cite: Wang, M., Wen, L., Li, Z., Meng, X., and Su, D.: Characteristics of carbon sink and the influence factors in Ngoring Lake, Qinghai-Tibet Plateau, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7650, https://doi.org/10.5194/egusphere-egu25-7650, 2025.

Freeze-thaw periods contribute disproportionately to annual N₂O emissionsrepresenting a critical yet understudied component of its global budget. Understanding drivers of these hot moments and their sensitivity to climate change is essential, but their episodic nature and great spatiotemporal variability pose substantial challenges. Combining cross-ecoregion soil core incubations with in-situ automated measurements, we explored snow regime shift effects on N2O emissions. Our findings revealed ~50-day pulse emissions during freeze-thaw periods, accounting for over 50% of annual fluxes, increasing nonlinearly with snow depth. Emissions were regulated by water-filled pore space (WFPS) thresholds: below 43%, soil moisture dominated; at 43%–66%, moisture and microbial attributes jointly triggered emissions; above 66%, microbial attributes, particularly N enzyme kinetics, prevailed. Hotspots of freeze-thaw-induced emissions were linked to high root production and microbial activity in cold, humid grasslands. This hierarchical control of WFPS and microbial processes provides a framework for predicting the location and magnitude of freeze-thaw-induced N₂O pulses, improving N₂O accounting and informing mitigation strategies.

How to cite: Liu, L. and Luo, J.: Moisture-microbial interaction amplifies N2O emission hot moments under deepened snow in grasslands, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7905, https://doi.org/10.5194/egusphere-egu25-7905, 2025.

EGU25-7918 | Orals | BG1.2

New advances and new questions for atmospheric methane 

Martin Manning, Xin (Lindsay) Lan, Sylvia Michel, and Euan Nisbet

Scenarios to keep global warming below 2°C include significant decreases in short lived atmospheric methane to allow time for the much longer-lived atmospheric CO2 to decrease more slowly. A methane decrease during the 2020s decade has been built into SSP scenarios and the need for this is reinforced by recent studies [Reisinger, 2024; Shindell et al., 2024]. In reality, the atmospheric methane burden has been growing very rapidly since 2006.

Atmospheric methane destruction is predominantly through oxidation by hydroxyl (OH). There is now evidence that since 1997, OH has been increasing in the Southern Hemisphere [Morgenstern et al., 2025]. This is based on 30 years of data for cosmic-ray produced 14C in atmospheric carbon monoxide (CO). Although most atmospheric chemistry models expect an increase in OH, the observed Southern Hemisphere increase of about +5% per decade is significantly greater than expected. Unfortunately, 14CO data in the Northern Hemisphere are insufficient to compare with models there.

The increase in methane removal rate inferred from the 14CO data means that methane sources are larger than prior estimates based on an almost-constant removal rate. If so, this new finding reduces a long standing discrepancy between “top-down” estimates of methane emissions from wetlands and consistently larger “bottom-up” estimates [Saunois et al., 2024].

While the increasing availability of satellite data is leading to better determination of methane’s source distribution, it is also necessary to differentiate between fossil fuel and biogenic sources. The positive trend of atmospheric δ13CCH4 for two centuries prior to 2006 reflected methane emissions from fossil fuel sources, but the strongly negative trend in δ13CCH4 since 2006 is primarily driven by biogenic sources such as wetlands and agriculture [Michel et al., 2024]. The magnitude of the source increase, particularly when the OH increase is taken into account, implies strong growth in wetland emissions, especially from northern tropical Africa.

More recent δ13CCH4 data for 2023 have shown flattening of its post-2006 trend at many Northern Hemisphere sites. While something similar was seen in 2012 this apparent shift in methane sources now appears more pronounced.

Given the urgency of reducing atmospheric methane to keep to the 2°C target, the recent changes in δ13CCH4 show atmospheric methane is in a very dynamic period of change. Future changes in the global methane budget may be less predictable than is currently assumed.

 

References:

Michel, S.E., Lan, X., Miller, J., et al, 2024: Rapid shift in methane carbon isotopes suggests microbial emissions drove record high atmospheric methane growth in 2020–2022. Proceedings of the National Academy of Sciences - PNAS, 121(44), e2411212121.

Morgenstern, O., Moss, R., Manning, M., et al, 2025: Radiocarbon monoxide indicates increasing atmospheric oxidizing capacity. Nature Communications, 16, 249.

Reisinger, A., 2024: Why addressing methane emissions is a non-negotiable part of effective climate policy. Frontiers in Science, 2, 5.

Saunois, M., et al., 2024: Global Methane Budget 2000-2020. Earth System Science Data, https://doi.org/10.5194/essd-2024-115 Discussion started: 6 June 2024, 147.

Shindell, D., Sadavarte, P., Aben, I., et al , 2024: The methane imperative. Frontiers in Science, 2, 1349770.

How to cite: Manning, M., Lan, X. (., Michel, S., and Nisbet, E.: New advances and new questions for atmospheric methane, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7918, https://doi.org/10.5194/egusphere-egu25-7918, 2025.

EGU25-8281 | Orals | BG1.2

Evolution of atmospheric methane under the global methane pledge: insights from an Earth system model 

Ulas Im, Kostas Tsigaridis, Susanne Bauer, Drew Shindell, Dirk Olivié, Simon Wilson, Lise Lotte Sørensen, Peter Langen, Sabine Eckhardt, Lena Hoglund Isaksson, Zig Klimont, and Lori Bruhwiler

The global methane pledge (GMP) aims to cut methane (CH4) emissions across all sectors by at least 30 percent below 2020 levels by 2030, which can thereby provide benefits in air quality and health, as well as in climate, relative to not cutting the emissions. We have used a fully coupled Earth system model (ESM) with interactive CH4 sources and sinks to study the future levels and trends of global atmospheric CH4 concentrations under different emission scenarios. Fully coupled simulations have been performed from 1995 to 2050, using multispecies emissions from the ECLIPSE V6b emissions database supplemented by new anthropogenic methane emissions estimates for Current Legislation (CLE), Maximum Feasible Reduction (MFR) and Global Methane Pledge (GMP) from IIASA/GAINS to simulate the future evolution of CH4 levels. In the baseline CLE scenario, global anthropogenic CH4 emissions increase from 298 Tg in year 2000 to 335 Tg in 2015, then continues to increase to 430 Tg in 2050 under CLE. Under MFR, anthropogenic CH4emissions first drop to 240 Tg in 2030, then slightly decrease to 220 Tg in 2050, while under the GMP scenario, they first drop to 300 Tg in 2030, then slightly increase to 320 Tg in 2050.

Preliminary results show that the interactive simulation slightly underestimates the observations on average by 2% between 1995-2022. All scenarios show an increase in the global CH4 concentrations, from 1.8 ppm in the present-day CH4 to 1.9 ppm (6%) in 2050 in the MFR scenario, 2.2 ppm (22%) in the CLE scenario, and 2.1 ppm (17%) in the GMP scenario. In addition, while anthropogenic CH4 emissions decrease, all simulations predict increasing wetland CH4emissions, by up to 10% in 2050 compared to 2020. Corresponding atmospheric CH4 lifetimes also increase in all simulations from 8.4 years in 2020 to lowest 8.5 years in CLE, 9.2 years in MFR, and 9.4 years in GMP. The increasing CH4 lifetime and concentrations in all scenarios despite reductions in emissions highlights that the response of concentrations are not necessarily linear with the changes in emissions as the chemistry is non-linear, and dependent on the oxidative capacity of the atmosphere due to other species such as CO and VOCs. In addition, missing sinks in ESMs such as halogens chlorine can lead to less chemical removal and longer lifetime compared to the box model.

We will further present the impact of these scenarios on the global surface temperatures and evaluate if the GMP will achieve its goal by 2050. However, preliminary results, compared with the recent 2021 AMAP SLCF assessment, suggest that despite the reduction in emissions, the atmospheric global CH4 levels simulated in the present study may not fulfil the larger goals of the GMP such as decreasing global CH4 concentrations and avoiding a 0.2°C warming by 2050 relative to 2020. However, reductions in emissions can still be achieved, which can lead to benefits in air quality and health. This work was accomplished through the Reduc(h4)e project funded by the Nordic Council of Ministers-and contributes to ongoing AMAP assessment work.

How to cite: Im, U., Tsigaridis, K., Bauer, S., Shindell, D., Olivié, D., Wilson, S., Sørensen, L. L., Langen, P., Eckhardt, S., Isaksson, L. H., Klimont, Z., and Bruhwiler, L.: Evolution of atmospheric methane under the global methane pledge: insights from an Earth system model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8281, https://doi.org/10.5194/egusphere-egu25-8281, 2025.

EGU25-9043 | Orals | BG1.2

Quantifying greenhouse gas emissions from landscape fires due to the Russo–Ukrainian War and the impact on the carbon sequestration capacity of forests 

Roman Vasylyshyn, Rostyslav Bun, Viktor Myroniuk, Lennard de Klerk, Oleksandr Soshenskyi, Sergiy Zibtsev, Svitlana Krakovska, Linda See, Mykola Shlapak, Volodymyr Blyshchyk, Lidiia Kryshtop, Zoriana Romanchuk, Orysia Yashchun, Eugene Kalchuk, and Yuriy Rymarenko

Vegetation acts as an essential land-based carbon sink, which can be affected by military conflicts and wars through landscape fires that can cover large territories and will lead to additional greenhouse gas (GHG) emissions into the atmosphere. To investigate this impact, we spatially analyzed the effect of the ongoing Russo–Ukrainian War on the GHG emissions from landscape fires and determined the change to the carbon sequestration capacity of the forests. Using remotely sensed data from 2022–2023, we first identified the fire perimeters in the territory of Ukraine. We then classified the burned areas into coniferous and deciduous forests, croplands, and other landscapes, and evaluated the distribution of the fires according to their intensity based on the differenced normalized burn ratio. We used several fire weather condition indices and calculated the attribution factor to identify the share of fires that were war related and were thus not caused by natural factors or human activity that would be typical in times of peace. We estimated the war-related biomass losses during the first two years of the war, considering the landcover type, the species and the age structure of the forest stands, the fire intensity, and the biomass content. The corresponding GHG emissions in the immediate term were estimated to be 9.08 Mt carbon dioxide equivalent (CO2e), with a relative uncertainty of ±46% (95% confidence interval). The estimated future (long-term) biomass losses due to current forest fires and their corresponding GHG emissions were calculated to be 16.86 Mt CO2e (±21%). Finally, losses in the carbon sequestration capacity of the burned forests during the first five years following the landscape fires were estimated to be 2.9 Mt CO2e.

 

How to cite: Vasylyshyn, R., Bun, R., Myroniuk, V., de Klerk, L., Soshenskyi, O., Zibtsev, S., Krakovska, S., See, L., Shlapak, M., Blyshchyk, V., Kryshtop, L., Romanchuk, Z., Yashchun, O., Kalchuk, E., and Rymarenko, Y.: Quantifying greenhouse gas emissions from landscape fires due to the Russo–Ukrainian War and the impact on the carbon sequestration capacity of forests, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9043, https://doi.org/10.5194/egusphere-egu25-9043, 2025.

EGU25-9368 | ECS | Posters on site | BG1.2

Assessing the optimal drivers for flux data gap-filling using random forest networks 

Nicola Lieff, Daniel Metzen, Cacilia Ewenz, Peter Isaac, Ian McHugh, and Anne Griebel

The Terrestrial Ecosystem Research Network (TERN) OzFlux group operates a network of eddy covariance stations that collect long-term atmospheric and soil measurements for monitoring and understanding changes in climate and the environment. Ideally, all data collected would be gap-free, however, all real data has gaps where instruments have not recorded measurements or data has been discarded due to low turbulence. To allow this data to be used as a continuous time-series in further analysis, the missing data is gap-filled using PyFluxPro. The standard community approach uses a predefined set of variables (drivers) for gap-filling, which are the same variables for all stations irrespective of location. However, the stations are located in a large range of climate zones, hence the standard gap-filling drivers might not be ideal for all sites. This is because the drivers were chosen for a small set of initial sites and might not be representative for a heating and drying climate.

To identify which drivers were best suited for each station, we developed a random forest model to objectively assess the relative importance of input variables used to gap-fill ustar, carbon, and energy fluxes. We trained this model on the published TERN OzFlux data for all available Australian sites using a large range of input variables. This model then determined the relative importance of variables, mean absolute errors, and R2 for the accuracy of the model prediction for a target variable at each site. Next, we grouped the variables into atmospheric, energy, turbulence and soil categories of drivers, which highlighted a distinct variation in the contribution of each category of driver across sites. To assess the ecological significance of these trends, the model importances were sorted by the aridity index and grouped by the Köppen-Geiger classification of each site. There is a notable shift in the importance of energy, turbulence, and soil groups with decreasing aridity, and driver contributions were generally consistent within Köppen-Geiger classifications. Reprocessing the gap-filling of a representative subsample of sites demonstrated a marked improvement in predicting the gap-filled target variables, highlighting that this approach can inform driver selection at new and established sites and will improve the understanding of the ecological significance of different drivers in various climate regions.

 

How to cite: Lieff, N., Metzen, D., Ewenz, C., Isaac, P., McHugh, I., and Griebel, A.: Assessing the optimal drivers for flux data gap-filling using random forest networks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9368, https://doi.org/10.5194/egusphere-egu25-9368, 2025.

Methane (CH₄) emissions from the Tibetan Plateau, often referred to as the "Third Pole," are critical to understanding global methane dynamics due to the region's extensive wetland ecosystems and unique environmental characteristics. However, quantifying CH₄ fluxes in this region is challenging due to sparse observational data, complex topography, and highly variable climatic and hydrological conditions. This study introduces a high-resolution machine learning framework tailored for the Tibetan Plateau by integrating satellite-based observations, ground measurements, and modeled data. The framework incorporates a diverse set of environmental drivers, including temperature, soil moisture, vegetation indices, and hydrological factors. This approach aims to address spatial and temporal gaps in methane flux estimates while capturing the complex interactions governing CH₄ emissions in high-altitude mountainous ecosystems.

How to cite: Zhang, Z.: High-Resolution Wetland Methane Flux Modeling for the Tibetan Plateau Using Machine Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10099, https://doi.org/10.5194/egusphere-egu25-10099, 2025.

EGU25-10326 | ECS | Orals | BG1.2 | Highlight

Declining coral calcification to enhance twenty-first century ocean carbon uptake by gigatons 

Alban Planchat, Lester Kwiatkowski, Marc Pyolle, Charlotte Laufkötter, and Laurent Bopp

As the oceans warm and acidify, the calcification of coral reefs declines, with net calcium carbonate dissolution projected even under moderate emissions scenarios. The impact of this on the global carbon cycle is however yet to be accounted for. We use a synthesis of the sensitivity of coral reef calcification to climate change, alongside reef distribution products to estimate alkalinity and dissolved inorganic carbon fluxes resulting from reductions in reef calcification. Using the global ocean biogeochemical model NEMO-PISCES, we simulate the impact of these fluxes on ocean carbon uptake under different emissions scenarios, accounting for uncertainty in present-day calcification rates.

Reductions in global coral reef carbonate production could enhance the ocean anthropogenic carbon sink by 0.34 PgC yr-1by mid-century (0.13 PgC yr-1 median estimate) with cumulative ocean carbon uptake up to 110 PgC greater by 2300 (46 PgC median estimate). Under medium to high emissions scenarios, two critical aspects emerge: (i) the full potential for coral reef degradation to affect carbon fluxes is reached within decades, and (ii) air-sea carbon fluxes remain substantial for centuries, due to the imbalance between carbon and alkalinity sinks/sources for the global ocean.

Accounting for the coral reef feedback into Earth system models could revise upward remaining carbon budget estimates, increasing the likelihood of achieving net-zero emissions without relying on negative emissions. The coral reef feedback could have a 21st-century impact comparable in magnitude to boreal forest dieback, though opposite in sign. This underscores a critical paradox: conserving calcifying organisms, such as coral reefs, may counteract a natural mechanism for mitigating climate change, but at the cost of protecting vital biodiversity. This challenges the "all-carbon" framework often used to address environmental issues, highlighting the complex trade-offs between carbon cycle regulation and biodiversity conservation.

How to cite: Planchat, A., Kwiatkowski, L., Pyolle, M., Laufkötter, C., and Bopp, L.: Declining coral calcification to enhance twenty-first century ocean carbon uptake by gigatons, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10326, https://doi.org/10.5194/egusphere-egu25-10326, 2025.

EGU25-10374 | Posters on site | BG1.2

Methane budget, seasonality and interannual variability of the three major river basins in Tropical South America 

Shrutika Wagh, Luana Basso, Ayan Fleischmann, Joao Amaral, John Melack, Hella Asperen, Stijin Hantson, Thorsten Schäfer, and Santiago Botia

Tropical wetlands are one of the largest natural methane sources but lack of in-situ observations and uncertainty in wetland extent leads to large uncertainly. In this study we analyze the methane budget from three major river basins in South America: the Orinoco, the Amazon, and the Pantanal basins using two atmospheric inversions:  the CAMS-CH4inversion, which assimilates satellite and in-situ data and the CarboScope methane inversion system constrained by in-situ data only. We make a comparative analysis focusing on the seasonal cycle, interannual variability, and the total methane budget from 2000 to 2019.

The budget difference in posterior estimates between CAMS-CH4 and CarboScope for these basins are as follows: Amazon Basin: -18.03 TgCH4/yr, Pantanal Basin: -11.65 TgCH4/yr, Orinoco Basin: -0.96 TgCH4/yr.  All together the total flux difference is -30.56 TgCH4/yr, indicating that CarboScope estimates larger total methane fluxes than the CAMS-CH4 inversion. Note that a similar difference (30.98 TgCH4/year) is also seen in the prior fluxes, suggesting that the optimization does not reduce the prior difference in the regions of interest.  While the Amazon Basin emits largest amount of methane, the Orinoco Basin exhibits the highest emissions per unit area, with 21.2 mgCH4/m²/day. In comparison, Amazon and Pantanal basins have emission of 19.26 mgCH4/m²/day and 13.36 mgCH4/m²/day. This shows the significant contribution of the smallest basin, in terms of methane flux density. Not surprisingly, both models indicate that wetlands are the primary methane source in the Amazon and Orinoco basins (~80%). In the Pantanal, CAMS-CH4 shows equal contributions from wetlands and anthropogenic sources, whereas CarboScope attributes dominance to anthropogenic emissions. Interestingly, seasonal patterns differ between the two models. In CAMS-CH4 there is a strong seasonality, with maximum methane emissions occurring during the wet season across all basins, in CarboScope, there is a double-peak in the Amazon Basin during March (wet) and August (dry). Finally, we investigate the inundation patterns and their relationship to methane emissions trends in these basins, as well as the factors influencing interannual variability to enhance our understanding of the processes driving these emissions.

How to cite: Wagh, S., Basso, L., Fleischmann, A., Amaral, J., Melack, J., Asperen, H., Hantson, S., Schäfer, T., and Botia, S.: Methane budget, seasonality and interannual variability of the three major river basins in Tropical South America, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10374, https://doi.org/10.5194/egusphere-egu25-10374, 2025.

EGU25-11802 | ECS | Orals | BG1.2

Tracking methane across South America: an inversion of TROPOMI satellite observations to quantify emissions and sectoral contributions 

Aurélien Sicsik-Paré, Isabelle Pison, Audrey Fortems-Cheiney, Grégoire Broquet, Elise Potier, Adrien Martinez, Florencio Utreras-Diaz, and Antoine Berchet

Methane (CH4) emissions from South America have been estimated to account for approximately 15% of global emissions over the past decade. While natural emissions are predominantly driven by wetlands, anthropogenic emissions include contributions from livestock and landfills. However, bottom-up estimates remain highly uncertain, particularly for wetland contributions. The top-down approach, based on atmospheric transport inverse modeling, offers a critical tool for enhancing the monitoring of regional CH4 emissions. Given the sparse network of in-situ measurements and limited aircraft campaigns in the region, satellite observations of total column methane mixing ratios (XCH4) provide a valuable source of observations for inverse modeling.

The TROPOspheric Monitoring Instrument (TROPOMI) aboard the Sentinel-5 Precursor (S5P) satellite, launched in 2017, provides XCH4 with global daily coverage and a relatively high (5.5×7 km²) horizontal resolution. Three different products are derived from the raw spectra measurements and are used in this study: the official product by SRON, the WFMD product by the University of Bremen and the BLENDED product by the University of Harvard. While widely used for detecting localized methane plumes linked to super-emitters, TROPOMI CH4 data also support regional and global flux inversions, enabling improved mapping of CH4 emissions. In 2019, TROPOMI provided over 4 million observations across South America, though with uneven spatial coverage, particularly limited over the tropical region due to cloud cover.

We assimilate the TROPOMI XCH4observations into regional atmospheric inversions of CH4 emissions over South America at a 0.2°×0.2° resolution, for 2019. The inversions are performed with the CHIMERE transport model coupled with the inverse modeling platform Community Inversion Framework (CIF). We first compare prior emission dataset, evaluating sector-specific uncertainties and spatial-temporal correlations within the background error covariance (B). The study then assesses system sensitivity to key input datasets and parametrization, including deep convection modeling, prior datasets and TROPOMI product selection, and optimization parameters. Additionally, the response of simulated XCH4 to sectoral contributions is analyzed. Particular focus is given over the tropical region and especially the Amazon basin, where extensive wetland emissions and low satellite observation coverage pose significant challenges. Finally, posterior CH4 emission budgets are presented at local, country, and regional scale, with detailed analysis of sectoral contributions from livestock, landfills, and wetlands, offering insights into the drivers of South America’s methane emissions.

How to cite: Sicsik-Paré, A., Pison, I., Fortems-Cheiney, A., Broquet, G., Potier, E., Martinez, A., Utreras-Diaz, F., and Berchet, A.: Tracking methane across South America: an inversion of TROPOMI satellite observations to quantify emissions and sectoral contributions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11802, https://doi.org/10.5194/egusphere-egu25-11802, 2025.

EGU25-12730 | ECS | Posters on site | BG1.2

Refining methane emission estimates in the Amazon basin: Addressing spatiotemporal variability and habitat diversity 

Santiago Botía, Ayan Santos Fleischmann, Luana Santamaria Basso, Shrutika Wagh, Jost Lavric, Ahmad Al Bitar, and John Melack

Recent studies highlight the critical role of methane emissions from tropical wetlands in driving the accelerated atmospheric CH4 growth rate observed in the last decade. The Amazon lowland region, where up to 30% of the area can be seasonally flooded, is one of the largest natural methane sources. The total methane flux estimates for the Amazon basin from top-down and bottom-up approaches converge at 31–46 TgCH₄/year. However, understanding methane emission trends and interannual variability—such as inundation extent and seasonality—requires improved attribution of emissions to specific wetland types and habitats. In this study, we present a refined bottom-up estimate of methane fluxes for the lowland Amazon that addresses key challenges to regionalizing fluxes in the basin: i) the large seasonal variation in inundated areas and habitats, ii) the diversity of aquatic ecosystems across the Amazon, and iii) the spatiotemporal variability of methane fluxes. 

We link local methane flux measurements collected during more than 20 years of field campaigns to specific river and wetland types and incorporate seasonal variability in inundation extent using dynamic remote sensing products (i.e. open water data from the Global Surface Water for lakes, Global River Width from Landsat (GRWL) for rivers, and wetland inundation extent from the High-Resolution Surface WAterFraction (SWAF-HR, based on SMOS L-band imagery) for the Amazon basin, and (4) GIEMS-D15 (merge of multiple satellites) for the remaining portions of South America). Wetland types (herbaceous and woody vegetation) were obtained from the JERS-1 L-band based classification of Hess et al. (2015) for the Amazon Basin and ESA-CCI land cover for the rest of South America. The magnitude and seasonal variability of our bottom-up fluxes are evaluated against fluxes derived from atmospheric CH4 mole fraction measurements at two Amazonian sites, whose footprints go beyond the Amazon Basin. While our product successfully captures the seasonal variability at both sites, it underestimates the overall magnitude of emissions compared to other estimates, even when accounting for emissions from flooded forest tree stems. Our findings represent an important improvement of bottom-up estimates representing the diversity of wetland habitats and processes driving methane emissions, but further work is needed to understand the mismatch with other methane emissions products.

How to cite: Botía, S., Santos Fleischmann, A., Santamaria Basso, L., Wagh, S., Lavric, J., Al Bitar, A., and Melack, J.: Refining methane emission estimates in the Amazon basin: Addressing spatiotemporal variability and habitat diversity, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12730, https://doi.org/10.5194/egusphere-egu25-12730, 2025.

EGU25-13556 | Posters on site | BG1.2

Let’s Investigate Methane for Climate Action 

Sander Houweling, Roxana Petrescu, Mekky Zaidi, Thomas Roeckmann, Jean-Daniel Paris, Torsten Sachs, Tuula Aalto, Manuel Gloor, Hartmut Boesch, Andreas Stohl, Hugo Denier van der Gon, Marielle Saunois, Rona Thompson, Sergey Gromov, Lena Höglund-Isakkson, and Ernest Koffi

2025 started with the launch of the H-Europe project IM4CA to enhance the quantification and understanding of methane emissions and sinks. A consortium of 25 partners joins forces to investigate pressing questions about the evolution atmospheric methane levels in recent decades, to reduce the uncertainty in future projections and design efficient solutions for monitoring and mitigating emissions in and outside of Europe. It will build new measurement and modelling infrastructure for improved monitoring of the progress toward short- and long-term emission reduction targets, with a prominent role for existing and upcoming satellite missions for measuring atmospheric composition and land surface properties.

The changing European methane emissions are an important focus of the project, which we keep track of with help of eastward extensions of the ICOS monitoring network in Poland and Romania. Intensive measurement campaigns in Rumania are conducted combining surface, aircraft, and total column measurements to improve the accuracy of emission quantification techniques using satellite data. The world-wide applicability of these techniques will extend the impact of our campaigns far beyond European borders.

Besides changing anthropogenic emissions, climate impacts on natural sources and sinks of methane are an important focus of IM4CA also. The four-year research program will initiate new measurement infrastructure in Congo to help characterize emissions from tropical wetlands in Africa. Campaigns will be conducted in Northern Scandinavia along a transect of disappearing permafrost to investigate impacts on vegetation and methane emissions using techniques that can be applied to high-resolution satellite instruments for circumpolar emission mapping.

This presentation will provide an overview of the planned activities and goals of IM4CA. The project offers a great opportunity to learn about methane in a cooperative spirit and to reach out and provide support to those who can turn knowledge about methane into climate action.    

How to cite: Houweling, S., Petrescu, R., Zaidi, M., Roeckmann, T., Paris, J.-D., Sachs, T., Aalto, T., Gloor, M., Boesch, H., Stohl, A., Denier van der Gon, H., Saunois, M., Thompson, R., Gromov, S., Höglund-Isakkson, L., and Koffi, E.: Let’s Investigate Methane for Climate Action, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13556, https://doi.org/10.5194/egusphere-egu25-13556, 2025.

EGU25-14051 | ECS | Posters on site | BG1.2

Temporal variability in dissolved inorganic carbon, δ13CDIC, and anthropogenic CO2 in the North Indian Ocean from 1995 to 2016: assessing the influence of anthropogenic CO2 

Pasindi Kaluthotage, Amavi Silva, Maheshi Dheerasinghe, and Hashan Kokuhennadige

The dynamics of dissolved inorganic carbon (DIC), stable carbon isotopes of DIC (δ13CDIC), and anthropogenic CO2 (CO2ant) in the upper 500 m of the water column were examined in two upwelling-favourable regions: the Sri Lankan Dome (SLD) and the central Bay of Bengal (BOB) in the Northern Indian Ocean over the period 1995 to 2016. This study aimed to investigate the spatiotemporal variability of these carbon parameters and assess the influence of CO2ant in these oceanic environments. Data from the GLODAPv2.2022 database, including cruise-based biogeochemical bottle measurements, were utilized to examine temporal trends in DIC and δ13CDIC. The TrOCA (Tracer combining Oxygen, Carbon, and Alkalinity) approach was employed to calculate CO2ant. Although DIC concentrations showed minimal variability across the water column in both the SLD and central BOB, significant fluctuations in CO2ant and δ13CDIC were observed in the upper 50 m in both regions between 1995 and 2016. Specifically, δ13CDIC values in the upper 50 m decreased by 0.45 ‰ (at a rate of 0.021 ‰ yr-1) in the SLD and by 0.41 ‰ (at a rate of 0.02 ‰ yr-1) in the central BOB over the study period. This decline is likely attributable to the combined effects of upwelling of remineralized DIC and increased CO2ant invasion in the upper 50 m of these oceanic regions, occurring at rates of 0.93 µmol kg-1 yr-1 in the SLD and 1.97 µmol kg-1 yr-1 in the central BOB. Additionally, a weaker correlation between δ13CDIC and CO2ant was observed in the central BOB, whereas a stronger correlation in the SLDsuggests that the invasion of isotopically lighter CO2ant contributed significantly to the observed depletion of δ¹³CDIC in both regions from 1995 to 2016. These findings underscore the significant role of anthropogenic CO2 in influencing carbon dynamics in the upper ocean of these upwelling-prone regions.

How to cite: Kaluthotage, P., Silva, A., Dheerasinghe, M., and Kokuhennadige, H.: Temporal variability in dissolved inorganic carbon, δ13CDIC, and anthropogenic CO2 in the North Indian Ocean from 1995 to 2016: assessing the influence of anthropogenic CO2, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14051, https://doi.org/10.5194/egusphere-egu25-14051, 2025.

EGU25-14074 | ECS | Orals | BG1.2

Net carbon exchange in the Amazon, Cerrado, and Caatinga: Challenges and Insights from the 2023/2024 Drought 

Santiago Botía and the Amazon drought 2023 team

Tropical South America plays a critical role in the global carbon cycle. On one hand, the Amazon stores large stocks of carbon (150-200 PgC), representing 50% of the tropical rainforest biomass.  On the other hand, the semiarid biomes of the neighbouring Cerrado and the Caatinga contribute largely to the inter-annual variability of the global land carbon sink. Both biomes are experiencing large threats due to deforestation, forest degradation, agricultural expansion and climate variability. While these threats in the Amazon have been largely studied, vegetation loss and associated carbon emissions from the Cerrado and Caatinga biomes have been somewhat overlooked. As a result, the mean and long-term trend in net carbon exchange in both biomes remains largely unknown. In this talk, I will give an overview of recent estimates in net carbon exchange and their uncertainty range for the Amazon and the Cerrado and Caatinga biomes. I will particularly focus on the development of the 2023/2024 drought and the carbon cycle response in the region. For this we leverage multiple data streams, from bottom-up models and top-down inversion systems, to remotely-sensed vegetation dynamics and in-situ flux and atmospheric measurements. I finalize highlighting the spatial heterogeneity of carbon fluxes across the region and emphasize on the remaining challenges to reduce the uncertainty in carbon cycle estimates and the need for enhanced atmospheric monitoring networks to improve our understanding of biome-specific drivers of net carbon exchange.

How to cite: Botía, S. and the Amazon drought 2023 team: Net carbon exchange in the Amazon, Cerrado, and Caatinga: Challenges and Insights from the 2023/2024 Drought, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14074, https://doi.org/10.5194/egusphere-egu25-14074, 2025.

EGU25-14801 | Orals | BG1.2

Challenges and opportunities in atmospheric methane mitigation from freshwater and marine environments 

Lu Shen, Minghao Zhuang, Shushi Peng, Vincent Gauci, Wei Wei, Lidong Wu, and Michael MacLeod

Methane emissions from the aquatic environment exhibit distinct characteristics: while oceans, covering 70% of Earth’s surface, emit 9 Tg of methane annually, freshwater wetlands, which occupy only 2% of Earth’s surface, emit 150-200 Tg per year. This significant contrast raises important questions about the underlying mechanisms and potential strategies to mitigate methane emissions in these water systems. In this work, we explore the challenges and opportunities of methane mitigation in both freshwater and marine environments. 

For freshwater wetlands, existing projections of future methane emissions usually neglect feedbacks associated with global biogeochemical cycles. Here, we employ data-driven approaches to estimate both current and future wetland emissions, considering the effects of changing meteorology and biogeochemical feedbacks arising from atmospheric sulfate deposition and CO2 fertilization. We show that, under low-CO2 scenarios (1.5 and 2°C warming pathways), the suppressive effect of sulfate deposition on wetland methane emissions largely diminishes by 2100 due to clean air policies, resulting in an additional emission increase of 7 ± 2 Tg a-1. This increase account for 35% and 22% of total wetland emission changes under 1.5 and 2°C warming pathways, a factor not yet considered by current Integrated Assessment Models.

For marine waters, we assess the methane emissions from mariculture’s aquatic environment at 10-km resolution globally, using measurements from research cruises and satellite-observed net primary productivity. Mariculture’s aquatic emission intensity is estimated to be 1–6 gCH4 per kg of carcass weight (CW), >95% lower than freshwater systems, due to suppressed microbial production in marine waters and inefficient ventilation to the atmosphere. The life-cycle assessment shows that mariculture’s carbon footprints are ~40% lower than those of freshwater aquaculture, suggesting considerable climate benefits of mariculture expansion to meet future protein needs.

How to cite: Shen, L., Zhuang, M., Peng, S., Gauci, V., Wei, W., Wu, L., and MacLeod, M.: Challenges and opportunities in atmospheric methane mitigation from freshwater and marine environments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14801, https://doi.org/10.5194/egusphere-egu25-14801, 2025.

EGU25-14803 | ECS | Posters on site | BG1.2

Regional method to quantify coastal anthropogenic carbon changes 

Xinyu Li and Brendan Carter

The global ocean plays a critical role in mitigating climate change by sequestering atmospheric CO2, removing approximately 26% of anthropogenic carbon emissions since the Industrial Revolution. While significant progress has been made in estimating open-ocean anthropogenic carbon (Canthro), the coastal ocean remains less understood due to its dynamic nature and complex processes and shortage of long-term high-quality datasets. Hence it is challenging to quantify the coastal anthropogenic carbon from the observation data. In this study, we propose a regional empirical regression-based anthropogenic carbon estimation approach (RECA) tailored for coastal regions. Using synthetic data from six different global ocean biogeochemical models, we evaluate the uncertainties in Canthro estimation and assess the contributions of non-steady-state natural and anthropogenic components to estimation biases in the four North American coast oceans. We also compare RECA with established regression-based methods (CAREER and eMLR(C*)) that are widely used in open-ocean regions to determine their applicability in coastal settings. Our results demonstrate that RECA effectively captures overall Canthro with minimal large-scale biases. However, subregional analyses reveal challenges in separating anthropogenic and natural CO2 signals, emphasizing the influence of natural variability. This study provides a unified framework for high-resolution Canthro estimation in coastal waters, evaluates its uncertainties, and paves the way for improved coastal carbon monitoring and climate action.

How to cite: Li, X. and Carter, B.: Regional method to quantify coastal anthropogenic carbon changes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14803, https://doi.org/10.5194/egusphere-egu25-14803, 2025.

EGU25-15075 | ECS | Posters on site | BG1.2

Assessing Bottom-Up and Top-Down Methane Emission Estimates in Northern High Latitude Regions (2018–2021)  

Rebecca Ward, Maria Tenkanen, Aki Tsuruta, Sara Hyvärinen, Anteneh Mengistu, Hannakaisa Lindqvist, Johanna Tamminen, Tiina Markkanen, Maarit Raivonen, Antti Leppänen, and Tuula Aalto

The northern high latitudes (NHLs) are undergoing rapid environmental changes with global warming, which may trigger feedback mechanisms that amplify natural methane emissions from wetlands and increase contributions from wildfires. Studying year-to-year variations in these emissions can provide understanding of the key factors driving natural methane fluxes. In addition, the NHLs produce substantial methane emissions from fossil fuel production. However, the spatial heterogeneity and overlap of methane sources in the region complicates the attribution of emissions to specific sources. 

This study presents an intercomparison of methane emissions estimates across four NHL regions—Russia, Canada, Alaska, and Norway-Sweden-Finland—between 2018 and 2021, focusing on the magnitude and seasonality of emissions. Emissions are compared using a combination of bottom-up and top-down estimates. Bottom-up estimates for key sectors, including anthropogenic activities, biomass burning, and wetlands, are produced by inventories and process models. Top-down estimates are derived from an ensemble of atmospheric inversions that separately optimise anthropogenic and biospheric emissions. The inversions, derived from the CarbonTracker Europe-CH4 model, incorporate a range of prior estimates, uncertainties, and atmospheric methane measurements from in-situ surface stations and satellite observations from TROPOMI and GOSAT.  

Preliminary findings indicate that for all four regions, posterior natural emissions are strongly influenced by the choice of prior emissions in shaping both their seasonality and magnitude. The CarbonTracker Europe-CH4 ensemble produces posterior emissions estimates consistent with the Global Carbon Project ensemble, which utilised different inversion models.  

By integrating a wide range of emissions estimates, this study aims to improve our understanding of the NHL methane budget. The findings contribute to ongoing methane emission assessments under the Eye-CLIMA, IM4CA (Investigating Methane for Climate Action), ESA SMART-CH4 (Satellite Monitoring of Atmospheric Methane) projects and ESA-AMPAC (Arctic Methane and Permafrost Challenge). 

How to cite: Ward, R., Tenkanen, M., Tsuruta, A., Hyvärinen, S., Mengistu, A., Lindqvist, H., Tamminen, J., Markkanen, T., Raivonen, M., Leppänen, A., and Aalto, T.: Assessing Bottom-Up and Top-Down Methane Emission Estimates in Northern High Latitude Regions (2018–2021) , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15075, https://doi.org/10.5194/egusphere-egu25-15075, 2025.

EGU25-15314 | ECS | Orals | BG1.2

The contribution of storm-induced outgassing to the CO2 air-sea flux in the Southern Ocean in a high-resolution, atmosphere-ocean simulation with ICON 

Arjun Kumar, David Nielsen, Nuno Serra, Fatemeh Chegini, Johann Jungclaus, and Tatiana Ilyina

The global ocean uptake of anthropogenic CO2 is sensitive to the uptake in the Southern Ocean, which accounts for 40-50% of the total uptake. At the same time, the Southern Ocean is the windiest region on the planet and experiences storms all year round. These storms, in turn, play an important role for the CO2 uptake in the Southern Ocean, because they can trigger outgassing of CO2 to the atmosphere. Storms induce outgassing by stirring the mixed layer via wind forcing, which leads to entrainment of waters rich in dissolved inorganic carbon into the mixed layer and elevates ocean pCO2 at the air-sea interface. However, since storms occur on synoptic time scales, such outgassing events are highly localised and short lived. Recent work based on in-situ measurements suggests that the magnitude of storm-induced outgassing and its contribution to the total Southern Ocean CO2 air-sea flux may have been severely underestimated by previous modelling studies, which do not sufficiently resolve storms and outgassing events. In this study, we take advantage of a cutting-edge simulation conducted with a fully-coupled, global, atmosphere-ocean model (ICON) with ocean biogeochemistry. Running on the assumption that the smaller grid spacing of 5 km better resolves storms and variability in wind forcing, we analyse the simulated contribution of storm-induced outgassing to the Southern Ocean uptake of CO2. 

How to cite: Kumar, A., Nielsen, D., Serra, N., Chegini, F., Jungclaus, J., and Ilyina, T.: The contribution of storm-induced outgassing to the CO2 air-sea flux in the Southern Ocean in a high-resolution, atmosphere-ocean simulation with ICON, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15314, https://doi.org/10.5194/egusphere-egu25-15314, 2025.

EGU25-15370 | Orals | BG1.2

SOCOMv2: On the strengths and limits of pCO2 interpolations products to estimate the ocean carbon sink 

Alizée Roobaert, Daniel J. Ford, Christian Rödenbeck, Nicolas Gruber, Judith Hauck, Amanda R. Fay, Thea Hatlen Heimdal, Jacqueline Behncke, Abby Shaum, Gregor Luke, Andrew Watson, Laique M. Djeutchouang, Sreeush Mohanan, Marion Gehlen, Annika Jersild, Jiye Zeng, Yosuke Iida, Frederic Chevallier, Galen A. McKinley, and Jamie D. Shutler and the SOCOMv2 team

The ocean is an important sink for anthropogenic carbon dioxide (CO2), but recent data from the Global Carbon Budget (GCB) highlight discrepancies in ocean carbon uptake estimates. Since the early 2000s, reconstructions of in-water CO2 fugacity (fCO2) using advanced interpolation techniques (data-products) have shown a growing divergence from estimates derived from global hindcast model simulations. This offsets in the mean flux amounts to approximately 0.49 GtC per year in the decade 2014-2023. The reasons for this discrepancy are not fully understood but may stem from a combination of factors including insufficient data coverage, uncertainties in scaling measurement-based estimates, and errors in model simulations. Previous studies suggests that biases in the fCO2 data-products from the under-sampled Southern Hemisphere, may contribute significantly to this gap.

To address these concerns, the Surface Ocean CO2 Mapping project has launched its second phase (SOCOMv2). This initiative aims to identify and quantify the accuracy and uncertainties related to data availability, changing observational networks, and input data. SOCOMv2 includes four key experiments: 1) a comprehensive geospatial uncertainty analysis, and three subsampling studies employing: 2) GCB hindcast simulations to capture true climate variability, 3) large ensemble simulations representing multiple climate states, and 4) idealized carbon uptake scenarios without climate variation. These efforts aim to provide a clearer understanding of the underlying factors contributing to the observed discrepancies in ocean carbon uptake estimates.

Results from the GCB subsampling hindcast simulation experiments reveal that individual fCO2 data-product reconstructions can significantly overestimate or underestimate both the annual mean and the trend of the ocean carbon sink relative to the models ‘truth’. Nonetheless, the ensemble mean of the fCO2 data-products tends to exhibit only a small overestimation of the model ‘truth’ ocean carbon sink. These discrepancies highlight the impact of limited data coverage and the inherent challenges of extrapolating from sparse measurements but cannot fully explain the observed divergence between models and fCO2 reconstructions in the GCB.

SOCOMv2 aims to improve the accuracy and precision of ocean carbon flux estimates, contributing to improved observational approaches and guiding policy development for climate mitigation. SOCOMv2 efforts have been driven by the community, with supporting funding within a larger European Space Agency ocean carbon study (Ocean Carbon for Climate).

How to cite: Roobaert, A., Ford, D. J., Rödenbeck, C., Gruber, N., Hauck, J., Fay, A. R., Heimdal, T. H., Behncke, J., Shaum, A., Luke, G., Watson, A., Djeutchouang, L. M., Mohanan, S., Gehlen, M., Jersild, A., Zeng, J., Iida, Y., Chevallier, F., McKinley, G. A., and Shutler, J. D. and the SOCOMv2 team: SOCOMv2: On the strengths and limits of pCO2 interpolations products to estimate the ocean carbon sink, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15370, https://doi.org/10.5194/egusphere-egu25-15370, 2025.

EGU25-15454 | Posters on site | BG1.2

Inverse modelling of global CH4 emissions using surface based measurements and GOSAT satellites retrievals. 

Francesco Graziosi, Giovanni Manca, Delia Segato, Srdan Dobricic, and Nicola Arriga

Atmospheric methane (CH₄) is a significant greenhouse gas with a warming potential 84 times greater than that of CO₂ over a 20-year time horizon. Given its relatively short atmospheric lifetime of approximately 10 years and its high warming potential, reducing anthropogenic methane emissions is crucial for limiting near-term increases in global temperatures. Methane is emitted from both natural and anthropogenic sources and is primarily consumed through reactions with hydroxyl (OH) radicals in the atmosphere. To a lesser extent, it is also removed through soil interactions. The limited understanding of the interplay between sources and sinks leads to an unclear explanation of the interannual variability in atmospheric methane concentrations over the past decades. Moreover, there are growing concerns about the possibility that climate change could amplify natural CH₄ fluxes. Here we present an inverse model-based reanalysis of global CH₄ emissions (2018-2021). To achieve this, we employ the TM5-4DVAR inverse model system, which is driven by ECMWF-ERA5 meteorological data at a resolution of 1° x 1° for both latitude and longitude, and encompasses 137 vertical levels. This four-dimensional inverse system generates monthly global fields of CH₄ fluxes across four source categories: wetlands, rice fields, biomass burning, and anthropogenic activities. The methane fluxes are optimized using high-resolution surface-based measurements from the NOAA Earth System Research Laboratory (ESRL) global cooperative air sampling network, as well as column-averaged dry mixing ratio XCH₄ data from the GOSAT satellite. The primary aim of this work is to identify the major geographical areas and source categories driving the interannual variability and trends of global CH₄ fluxes during the study period. Moreover, the temporal variability of natural methane fluxes is analysed in relation to physical parameters to investigate how natural CH4 emissions respond to climate factors (e.g. temperature).

How to cite: Graziosi, F., Manca, G., Segato, D., Dobricic, S., and Arriga, N.: Inverse modelling of global CH4 emissions using surface based measurements and GOSAT satellites retrievals., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15454, https://doi.org/10.5194/egusphere-egu25-15454, 2025.

EGU25-15780 | ECS | Orals | BG1.2

Mitigation and implications of methane emissions from dairy cow barns 

Jonathan Buzan, Jens Terhaar, Fortunat Joos, Niels Iversen, and Peter Roslev

Reaching the Paris Agreement temperature goals of no higher than +1.5°C or +2.0°C of global mean temperature change is quickly becoming difficult to reach by the end of the century. Not making the Paris Agreement temperature targets will impact all aspects of human society.

 

Around 1/3rd of global mean surface temperature changes, is estimated to be caused by methane making it the second most powerful greenhouse gas released anthropogenically.  Anthropogenic sources emit 349 Tg of methane per year and are responsible for more than 50% of global methane emissions. The main emitters are the energy sector (>36% of emissions) and agriculture (40%). Fortunately, methane is a short-lived greenhouse gas, and removal of anthropogenic emissions sources may dramatically change the global concentrations on decadal timescales.

 

In response to the unlikelihood that methane emissions will be attenuated sufficiently in the coming decade by production reductions, methane emission mitigation technologies are under development. However, these technologies are yet to be rolled out on an industrial scale. New methane mitigation technologies can reduce a 50 ppm emissions source at ~60% efficiency and require an air volume rate of 4.36e13 m3/yr to remove 1 Tg CH4 per year. The volume of air required to process low concentrations to make a substantive impact on total emissions is major roadblock to their implementation. For example, for CO2 capture—a related carbon mitigation method—many test technologies are constructing large independent ventilation facilities. However, novel methane emission mitigation technologies are currently being tested and evaluated in several countries. These new technologies may capture CH4 and/or convert CH4 to molecules with less radiative forcing potential.

 

Here, we propose using dairy cow barns as a viable pathway for methane emission mitigation by utilizing existing infrastructure while targeting a major source of agricultural methane. Currently, there are ~264 M dairy cows worldwide. In Europe, there are 23 M dairy cows, and ~33% are housed in barns annually. For example, 70% of Denmark’s and 90% of Italy’s dairy cows are housed annually. For the health and welfare of the animals, barns are ventilated to maintain comfortable temperature and humidities, as well as ventilate abhorrent gases, such as methane. Standards for ventilation require 400 m3/hr/cow (high heat situations require 2500 m3/hr/cow), which is 3.5e6 m3/cow annually. A dairy cow emits between 55-100 kg CH4 per year. Which translates to 0.4-0.9 Tg CH4 per year for the ~7.59 M housed dairy cows in the European Union. The amount of air estimated to move through the EU dairy barns is 2.66e13 m3/yr and is within the estimated amount of air required to remove 1 Tg of CH4 from emerging technologies (4.36e13 m3/yr).  Implementation of this type of methane mitigation is feasible and with additional air recycling, potentially capture methane emissions from dairy cow barns.

How to cite: Buzan, J., Terhaar, J., Joos, F., Iversen, N., and Roslev, P.: Mitigation and implications of methane emissions from dairy cow barns, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15780, https://doi.org/10.5194/egusphere-egu25-15780, 2025.

Accurate simulation of regional carbon dioxide (CO2) concentrations is essential for understanding carbon flux dynamics, refining emission inventories, and supporting climate mitigation policies. Using the WRF-Chem-VPRM model at 3 km resolution, this study simulated CO2 concentrations in Jiangsu Province, China, with hourly outputs. Model verification against nine ground-based CO2 monitoring stations confirmed its reliability.
Before integrating emission inventories into the model, we conducted a comprehensive analysis of six widely used emission inventories (ODIAC, EDGAR, MEIC, CHRED, GID, GRACED), revealing significant discrepancies in total emissions and spatial patterns in China. Provincial-scale annual carbon emissions discrepancies reached 52%, whereas urban-scale discrepancies averaged 137%, attributed to differences in emission proxies and spatial resolution. 
Sensitivity experiments for July and December 2022, representing summer and winter, assessed the impacts of spatial, temporal, and vertical allocation processes. Vertical allocation coefficients emerged as a critical factor, particularly under stable nighttime boundary layer conditions, where deviations exceeded 50 ppm. Their influence equaled or even surpassed that of emission inventory selection, underscoring the necessity of precise vertical parameterization.
Spatial allocation discrepancies primarily affected urban concentrations, where dense and diverse sources contributed to higher variability. Winter simulations exhibited increased uncertainties due to heightened heating emissions and limited vertical mixing.
These findings highlight the importance of refining vertical and spatial allocation in emission inventories to improve regional CO2 modeling. The study provides insights for advancing carbon inversion methodologies and supporting robust Monitoring, Reporting, and Verification (MRV) systems in urbanizing regions.
Emission inventories analyzed include:
•    ODIAC: Open-source Data Inventory for Anthropogenic CO2,
•    EDGAR: The Emissions Database for Global Atmospheric Research,
•    MEIC: The Multi-resolution Emission Inventory for China,
•    CHRED: China High-resolution Emission Database,
•    GID: Global Infrastructure emissions Detector,
•    GRACED: Global Gridded Daily CO2 Emissions Dataset.

How to cite: Feng, W., Tang, X., Zhu, J., and Zhou, X.: High-Resolution simulation of  CO2 Concentrations Over Jiangsu Province in China Based on WRF-Chem-VPRM and Six Emission Inventories, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16464, https://doi.org/10.5194/egusphere-egu25-16464, 2025.

EGU25-16559 | ECS | Orals | BG1.2

Using atmospheric O2 to disentangle the natural and anthropogenic CO2 signals  

Kim Faassen, Joram Hooghiem, Auke van der Woude, Anne-Wil van den Berg, Boaz Hilman, Lucas Hulsman, Aleya Kaushik, Remco de Kok, Marnix van de Sande, Wouter Peters, and Ingrid Luijkx

Atmospheric oxygen (O2) allows to separate the natural and anthropogenic components in the atmospheric CO2 signal, thereby providing additional constraints on these processes in the global carbon cycle. This is enabled through the ratio of O2 and CO2 in carbon cycle processes: the Exchange Ratio (ER). This ER signal has distinct values for combustion of different fossil fuel types, as well as between photosynthesis and respiration processes. Using these ER signals, we aim to further explore the potential of using atmospheric O2 observations in CO2 emission verification. For that, we are developing a global scale data assimilation system that can, next to CO2, assimilate O2 observations. This is our new multi-tracer implementation, specifically aimed at decadal and annual timescales: the CarbonTracker Europe Long Window system. Additionally, we implemented O2 and the O2/CO2 exchange ratios into the Simple Biosphere model (SiB4) to further understand the influence of biosphere exchange on using Atmospheric Potential Oxygen (APO) as a tracer for fossil fuel emissions. We will present the results from this biosphere O2 and CO2 modelling to get a first theoretical assessment of the variability of the biosphere O2 and CO2 ER signals, both over space (related to the plant functional types) and time (related to seasonal patterns). These biosphere model results, are subsequently used in our first attempt of atmospheric inverse estimates of CO2 fluxes using O2 as a tracer. Finally, we will show our progress towards understanding the implications of the variability in the ERs for photosynthesis and respiration on APO calculations, as well as their influence on fossil fuel estimates using atmospheric O2.

How to cite: Faassen, K., Hooghiem, J., van der Woude, A., van den Berg, A.-W., Hilman, B., Hulsman, L., Kaushik, A., de Kok, R., van de Sande, M., Peters, W., and Luijkx, I.: Using atmospheric O2 to disentangle the natural and anthropogenic CO2 signals , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16559, https://doi.org/10.5194/egusphere-egu25-16559, 2025.

EGU25-17087 | ECS | Posters on site | BG1.2

Assessment of Forest Carbon Management Using Net Primary Productivity on the Korean Peninsula 

Whijin Kim, Cholho Song, and Woo-Kyun Lee

The functions of terrestrial ecosystems are various, and recent study suggests the major three functions which are carbon, water, and energy cycling. They are all originated from land, the fundamental components of terrestrial ecosystems. Land consists of major five land cover: cropland, grassland, built-up area, wetland, and forest land. Forest land is described as high potential to remove Greenhouse gases under climate change era and thus the forest carbon management has been raised for effective land management in terms of carbon removal. Korean peninsula, South Korea and North Korea, has undergone the severe war between them and it damaged the whole territory, which consists of more than 60% of forest land. Therefore, two countries tried to revegetate and implemented forestation plans for recover the forest land over 50 years. Therefore, this study assessed the forest carbon management on the Korean Peninsula using Net Primary Productivity(NPP) from the 1980s to 2010s. To estimate NPP, Carnegie-Ames-Stanford Approach(CASA) model was applied. The study adopted the carbon demand and supply method for assessment. We defined carbon demand as amount of carbon loss from forest land in previous year due to forest land changes, and carbon supply as amount of newly updated carbon sink from forest land due to afforestation. According to research findings, even though South Korea achieved successful forest expansion, it only focused on the amount of forest area rather the quality of carbon management. However, the situation in North Korea described not only the failure of increasing forest area but also forest carbon management. Further research would be analyzed the outcomes with forest plans in South Korea and North Korea.

How to cite: Kim, W., Song, C., and Lee, W.-K.: Assessment of Forest Carbon Management Using Net Primary Productivity on the Korean Peninsula, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17087, https://doi.org/10.5194/egusphere-egu25-17087, 2025.

EGU25-18709 | ECS | Posters on site | BG1.2

Emissions of climate-altering species from open vegetation fires in the Mediterranean region - A review on methods and data 

Rabia Ali Hundal, Saurabh Annadate, Rita Cesari, Alessio Collalti, Michela Maione, and Paolo Cristofanelli

The climate change over the Mediterranean region poses serious concerns about the role of open vegetation fires in the emissions of climate-altering species. The aim of this work is to review the current methodologies for quantifying the emissions of greenhouse gases and black carbon from open vegetation fires, as well as the data provided by four state-of-the-art inventories of emissions of carbon dioxide (CO2), methane (CH4), nitrous oxide (N2O) and black carbon (BC) in the Mediterranean region for the period 2003–2020.

A limited number of studies specifically addressed the quantification of emissions from open fires in the Mediterranean region. Our data review of fire emissions in the Mediterranean region, where “top-down” methods have not yet implemented, reveals discrepancies across the four inventories examined (GFED v4.1s, GFAS v1.2, FINN v2.5, and EDGAR v8.0). Among these, FINN v2.5 consistently reported the highest emissions, while GFED v4.1s reported the lowest. We observed that the relative ranking of total emissions between the inventories varied for the species considered (e.g. CO2 vs. CH4) and that different proportions of emissions were attributed to the individual countries included in the Mediterranean domain. We argued that these differences were related to the different spatial resolutions of the input data used to detect the occurrence of fires, the different approaches to calculating the amount of fuel available, and the emission factors used.

The three inventories reporting wildfire emissions were consistent in identifying the occurrence of peaks in the emissions for the years 2007, 2012 and 2017. We hypothesized that La Niña events could partially contribute to triggering the occurrence of these emission peaks.To increase the accuracy and consistency of climate-altering emission data related to open vegetation fires in the Mediterranean region, we recommend to integrate bottom-up approaches with top-down inversion methods based on satellite and in-situ atmospheric observations.

How to cite: Hundal, R. A., Annadate, S., Cesari, R., Collalti, A., Maione, M., and Cristofanelli, P.: Emissions of climate-altering species from open vegetation fires in the Mediterranean region - A review on methods and data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18709, https://doi.org/10.5194/egusphere-egu25-18709, 2025.

EGU25-18920 | ECS | Posters on site | BG1.2

Net community production in the Greenland Sea: a comparative case study using Argo data of nitrate, oxygen, and DIC 

Ingrid Sælemyr, Are Olsen, Meike Becker, Siv K. Lauvset, Kjell Arne Mork, Ailin Brakstad, and Filippa Fransner

In this case study, we derive and compare estimates of annual net community production (NCP) in the Greenland Sea from Argo float data of nitrate, oxygen, and dissolved inorganic carbon (DIC). We added tracers of the inorganic carbon system, nitrate, dissolved oxygen, and air-sea gas exchange to the 1-D Price-Weller-Pinkel mixing model (Price et al., 1986) tuned to the Greenland Sea (Moore et al., 2015; Brakstad et al., 2019). By reinitializing the model with every Argo profile, we were able to estimate NCP as the difference between the abiotic model output and the Argo profiles. This method has previously been employed in various other regions (Plant et al. 2016;  Briggs et al. 2017, Mork et al. 2024). While we here compare NCP estimates from both nitrate, oxygen, and DIC, previous work has considered maximum two of these concurrently. Through our comparison, we discovered quantitative discrepancies in the NCP and annual NCP (ANCP) estimates. These results were sensitive to trends in the raw data and artefacts deriving from processes that were unresolved in the model, such as internal waves. Effects from internal waves were challenging to remove without introducing new artefacts. Qualitatively, the NCP seasonal cycle was well resolved: the summer of 2019, NCP fluctuated between periods of weak net biological production and periods of weak net heterotrophy. NCP was close to zero through winter, before two strong blooms were observed in late April and May 2020. However, the amplitude of the NCP signal from DIC was somewhat larger than from nitrate and oxygen. DIC derived NCP also exhibited stronger signs of remineralization from November 2019 to January 2020 compared to the two other estimates. Thus, this work shows the importance of careful consideration when utilizing biogeochemical Argo data in the Greenland Sea.

How to cite: Sælemyr, I., Olsen, A., Becker, M., Lauvset, S. K., Mork, K. A., Brakstad, A., and Fransner, F.: Net community production in the Greenland Sea: a comparative case study using Argo data of nitrate, oxygen, and DIC, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18920, https://doi.org/10.5194/egusphere-egu25-18920, 2025.

EGU25-19322 | ECS | Orals | BG1.2

Assessing the recent ocean carbon sink with data assimilation into a global ocean biogeochemistry model 

Frauke Bunsen, Lars Nerger, and Judith Hauck

Global ocean biogeochemistry models are a key tool for estimating the global ocean carbon uptake. These models are designed to represent the most important processes of the ocean carbon cycle, but the idealized process representation, uncertainties in the initialization of model variables and in the atmospheric forcing lead to errors in their estimates. To improve the agreement with observations, we use ensemble-based data assimilation into the ocean biogeochemistry model FESOM2.1-REcoM3. In addition to the recently implemented assimilation of temperature and salinity observations, which improves the physical model state and indirectly influences biogeochemical variables, we extend the set-up further. Here, we explicitly include the assimilation of biogeochemical observations. Specifically, in-situ sea surface pCO2 measurements, remotely sensed chlorophyll-a, and in-situ measurements of dissolved inorganic carbon, alkalinity, oxygen, and nitrate, are assimilated to reduce the uncertainty stemming from the ecosystem model. This directly affects the modelled air-sea CO2 flux. Here, we present an updated estimate of the ocean carbon uptake for the period 2010–2020 and compare it to prior estimates.

How to cite: Bunsen, F., Nerger, L., and Hauck, J.: Assessing the recent ocean carbon sink with data assimilation into a global ocean biogeochemistry model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19322, https://doi.org/10.5194/egusphere-egu25-19322, 2025.

EGU25-21437 | Orals | BG1.2

The ocean carbon sink under record-high sea surfacetemperatures in 2023/24 

Jens Daniel Müller, Nicolas Gruber, Aline Schneuwly, Dorothee C.E. Bakker, Marion Gehlen, Luke Gregor, Judith Hauck, Peter Landschützer, and Galen A. McKinley

In 2023, sea-surface temperatures (SST) reached record highs. Historically, the years with highest global mean SST anomalies were associated with a slight increase in oceanic CO₂ uptake, primarily due to reduced CO2 outgassing from the tropics during El Niño. In contrast, our observation-based estimates reveal that the global non-polar ocean absorbed about 10% less carbon in 2023 than expected (+0.16±0.28 PgC yr-1).


This weakening of the ocean carbon sink occurred although the CO2 outgassing in the tropics was indeed as low as expected. Instead, the decline in CO2 uptake was concentrated entirely in the extratropics, driven largely by elevated SSTs in the Northern Hemisphere. While thermally induced reductions in CO2 uptake are well-documented in the extratropics, our analysis using two ocean biogeochemical models highlights a mitigating process in the subtropical North Atlantic: the depletion of dissolved inorganic carbon in the surface mixed layer. Such negative feedbacks caused an overall muted response of the ocean carbon sink to the record high SSTs, but this resilience may not persist under long-term warming or more severe SST extremes.


By the time of this presentation, we anticipate confirming – or refining – our expectation that the ocean carbon sink in 2024 remained unusually weak, because the CO2 outgassing from the tropics revived, whereas remaining high SSTs in the extratropics continued to suppress the CO2 uptake.

How to cite: Müller, J. D., Gruber, N., Schneuwly, A., Bakker, D. C. E., Gehlen, M., Gregor, L., Hauck, J., Landschützer, P., and McKinley, G. A.: The ocean carbon sink under record-high sea surfacetemperatures in 2023/24, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21437, https://doi.org/10.5194/egusphere-egu25-21437, 2025.

EGU25-428 | Posters on site | AS3.41

Advancements in Methane in Air Standards for ground-based concentration measurement and emissions quantification 

Edgar Flores, Joële Viallon, Tiphaine Choteau, Philippe Moussay, and Robert Wielgosz

Methane (CH4) emission quantification that is based on ground level measurements of enhancements in CH4 in air concentrations requires instruments that are accurately calibrated with fit for purpose gas standards. Developments in the availability, accuracy and internal consistency of CH4 in air gas standards will be described, with standards now available with standard uncertainties below 1 nmol/mol over the range of below ambient background concentrations to over 3000 nmol/mol. When greater levels of precision are required for the measurement of enhancements in CH4 concentrations, the scale approach for standards can be adopted, as is done for WMO mole fraction scale standards for CH4 in air, with recent comparative measurements demonstrating that internal consistencies between standards of 0.1 nmol/mol can be reached.

According to WMO, the annual increase in atmospheric CH4 was 16 nmol/mol in 2022 and 11 nmol/mol in 2023, both of which exceed the average growth rate observed over the past decade. In addition, enhancements in atmospheric CH4 concentrations at short temporal scales due to localized emissions can be measured at ground-level. When selecting gas calibration standards to be used for such measurements, the achievable uncertainty and internal consistency of the standards used needs to be considered. The aim is to ensure that measured changes can be undoubtedly attributed to atmospheric concentration enhancements, and not to differences in standards used at different sites. Additionally, a consistent system in which all measurement results are traceable to the same references allows different datasets to be combined without the introduction of biases.

To enhance the accuracy, reliability, and robustness of global CH4 measurements over the past two decades, the BIPM, National Metrology Institutes (NMIs) and the WMO’s Central Calibration Laboratory have worked on improving the system of CH4 standards traceable to the International System of Units (SI), and demonstrating equivalence with standards developed for the WMO scale, the latter used principally for background CH4 trend measurements .

Improvements in the compatibility of CH4 in air standards from 2003 to 2023 will be described. Current standards now have accuracies of better than 1 nmol/mol, and pairwise comparisons of standards have demonstrated internal consistencies of 0.1 nmol/mol in sets of standards from National Metrology Institutes and the WMO’s CCL. This builds upon  preliminary comparisons of primary CH4-in-air gas standards conducted in 2003 (CCQM-P41), showing a standard deviation of approximately 30 nmol/mol and 10 nmol/mol for a more limited set of standards. Whereas in 2013, the CCQM-K82 comparison studied CH4-in-air primary reference mixtures in the range of 1800 nmol/mol to 2200 nmol/mol, with a demonstrated tenfold improvement in compatibility, with uncertainties of reference values for standards ranging from 0.68 nmol/mol to 0.71 nmol/mol and a standard deviation of 1.70 nmol/mol across the standards. In 2023, a new comparison (CCQM-K82.2023) was conducted to further monitor the compatibility of CH4-in-air primary reference mixtures within the 1800–2200 nmol/mol range. Preliminary  results will be discussed, as well as progress in extending the availability of  CH4 in air scale standards, when the very highest levels of internal consistency between standards is required.

How to cite: Flores, E., Viallon, J., Choteau, T., Moussay, P., and Wielgosz, R.: Advancements in Methane in Air Standards for ground-based concentration measurement and emissions quantification, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-428, https://doi.org/10.5194/egusphere-egu25-428, 2025.

The mitigation of anthropogenic climate forcing necessitates substantial reductions in methane emissions, given methane's elevated radiative forcing potential. While the Global Methane Pledge establishes a framework for 30% emissions reduction by 2030, precise quantification of fugitive emissions remains challenging due to their stochastic spatiotemporal characteristics.

This investigation presents the application of trailer-mounted Quantum Gas Lidar instrumentation for the detection, visualisation, and quantification of methane flux rates from holes drilled for coal exploration in Queensland, Australia. The methodology leverages high-resolution spatial and temporal sampling capabilities to enable flux quantification of traditionally challenging emission sources. Extended temporal measurement campaigns reveal significant variability in emission rates, highlighting the necessity of continuous monitoring protocols for accurate flux determination.

The results demonstrate the effectiveness of Quantum Gas Lidar technology in fugitive methane quantification, offering uninterrupted accurate measurements through a range of weather conditions.  Real-time visualisation and temporal quantification capabilities enhance understanding of emission dynamics. This work illustrates the significance of advanced sensing methodologies in achieving Global Methane Pledge objectives and emphasising the role of innovative monitoring approaches for targeting abatement strategies.

How to cite: Hayes, P. and Hoerning, S.: Quantifying Fugitive Methane from Coal Exploration Boreholes Using A Trailer-Mounted Quantum Gas Lidar System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1364, https://doi.org/10.5194/egusphere-egu25-1364, 2025.

Introduction

Methane emissions from oil and gas sector have high spatial and temporal variability. Previous studies with limited sample size and very few (if any) numbers of repeated measurements have often been used to estimate basin and national scale emissions, leading to high uncertainties to the inventory estimation. This study investigates methane emission data on point sources collected in repeated surveys of Permian Basinover 2019–20231, focusing on the spatiotemporal variability of emissions and the sampling strategy for developing a relatively accurate annual emission inventory for large oil gas regions with limited number of surveys that capture the temporal variation and a fraction of the facilities that can cover the spatial variability.

Methodology

We have developed a multi-faceted approach reorganizing repeated flight overpass data into surveys to estimate source persistence and construct emission events characterized by unique combinations of rates, duration (in terms of number of surveys), and frequency (number of repeated events). Using multiple time series construction approaches including discrete event simulations, we model the annual variability of point source emissions at multiple scales: sub-basin (25, 100, 400 km2) and basin (4000 km2), and use random sub-sampling to determine minimum coverage criteria to capture annual emission variability accurately. Our criteria are based on two parameters—the number of surveys conducted and % facilities covered in the basin.

 

Results and Discussion

 Our findings highlight that considerable temporal variability in methane emissions can occur, especially for areas of sub-basin scale (≈100–400 km2). The emission rates of detected facility-scale sources vary significantly across years (average Coefficient of Variation, COV ≈ 2.3). Our results also reveal that emission events are short-lived (≥75% events lasting ≤ 2 surveys), occur infrequently (average persistence ≤ 33%), yet significantly contribute to total detected emissions (~70%). Nevertheless, these intermittent facility-scale emissions translate to significantly lower variability across sub-basin scale surveys (COV ≈ [0.2–1.3]) and basin-scale surveys (COV ≈ 0.5).

We also study the spatial and temporal variability of emission estimates for sub-basin and basin-scale surveys. At the basin scale, even a single survey sufficiently captures the annual emission variability (bias ≤ 10%) and the emission distribution across different sub-basins (cosine similarity of 0.8–1.0). However, at a sub-basin scale, even estimates based on 25 surveys can be biased (bias ≈ 20%). We find low correlations (Spearman R < 0.5) of time series patterns of sub-basin-sub-basin and sub-basin-basin-scale areal emissions, pointing to the diverse emission patterns within the basin.

 

Concluding Remarks

Our findings on spatial (areal coverage) and temporal (number of surveys) considerations can help build annual emission measurement strategies for oil and gas production regions.

Reference

  • Cusworth, et al., 2022. Strong methane point sources contribute a disproportionate fraction of total emissions across multiple basins in the United States, PNAS, 119 (38) e2202338119, https://doi.org/10.1073/pnas.2202338119

 

 

How to cite: Xie, D., Bhandari, S., and Albertson, J.: Spatiotemporal Variation of Point Source Emissions in Permian Basin and its Implication on Basin Level Inventory Building and Mitigation , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1675, https://doi.org/10.5194/egusphere-egu25-1675, 2025.

EGU25-2167 | ECS | Orals | AS3.41

Quantifying U.S. methane emission trends (2019-2024) through high resolution inversion of satellite observations 

Lucas Estrada, Daniel Jacob, Daniel Varon, Megan He, James East, Melissa Sulprizio, Nicholas Balasus, Sarah Hancock, and Kevin Bowman

The United States is the world’s largest emitter of methane from oil and gas and the second-largest methane emitter overall. Inversions of atmospheric observations provide an empirical method for evaluating progress on emission goals. Here, we present U.S. annual methane emission trends from 2019 to 2024 at up to ~25 km resolution inferred from analytical inversion of blended TROPOMI+GOSAT satellite observations. For each year, we use the U.S. Greenhouse Gas Inventory as the prior estimate, then generate an ensemble of posterior emission estimates by applying the Integrated Methane Inversion (IMI 2.0) inverse modeling framework. Our results include closed-form error characterization through analytical minimization of the Bayesian cost function and uncertainties derived from the ensemble of inversion estimates. The high resolution of our posterior estimate allows us to generate sector-resolved emissions at the national, state, and basin level. Our results comprehensively assess U.S. progress on methane mitigation and demonstrate the capability of advanced modeling tools for rapid generation of top-down emission estimates to inform climate policy.

How to cite: Estrada, L., Jacob, D., Varon, D., He, M., East, J., Sulprizio, M., Balasus, N., Hancock, S., and Bowman, K.: Quantifying U.S. methane emission trends (2019-2024) through high resolution inversion of satellite observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2167, https://doi.org/10.5194/egusphere-egu25-2167, 2025.

Global gas flaring from the oil and gas industry was estimated to be 148 billion cubic meters in 2023, based on satellite observations from the Visible Infrared Imaging Radiometer Suite (VIIRS; World Bank, 2024). Both lit and unlit flares are sources of potent greenhouse gases and health hazards, making it a source requiring accurate global monitoring. The VIIRS instrument often forms the basis for gas flaring volumes, but our study reveals that these estimates are underestimated in Canada, and potentially elsewhere.

Comparing VIIRS flaring observations with industry reporting across Western Canada for 2012-2023, we found that industry reports ~2.3-times more gas flaring than estimated by satellite. This appears to be primarily the result of small/medium-sized flares going undetected (generally less than 350 m3/h, or 220 kg/h, assuming 90% methane content), but we also estimate that ~17% of industry-reported flaring was missed because of enclosed combustors, which do not have a flame visible to VIIRS. For flares that are detected by VIIRS, aggregate volume estimates agree within ~8% of industry reporting, although individual flares can be +/- an order of magnitude from industry reporting, similar to offshore findings from Brandt (2020).

If this issue of underestimated flaring volumes from VIIRS is limited to Canada, global gas flaring estimates would increase by only 1%, but Canada would be the 10th most flaring country (up from 23rd). However, if undetected flares are more widespread, global flaring could be much more deeply underestimated. VIIRS’s theoretical detection limits imply that smaller flares should be detected, implying other factors are impacting detection/quantification, such as VIIRS data filtering, flaring practices (e.g., daytime-only blowdown flaring), or persistent cloud cover.

 

References

Brandt AR. 2020. Accuracy of satellite-derived estimates of flaring volume for offshore oil and gas operations in nine countries. Environmental Research Communications 2(5). IOP Publishing. doi: 10.1088/2515-7620/ab8e17

World Bank. 2024. Global Gas Flaring Tracker Report. (June). Washington, DC. Available at https://www.worldbank.org/en/programs/gasflaringreduction/global-flaring-data. Accessed 2024 Jul 2.

How to cite: Seymour, S., Xie, D., and Kang, M.: Global gas flaring volumes may be underestimated: comparisons with over a decade of industry reporting in Canada, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3295, https://doi.org/10.5194/egusphere-egu25-3295, 2025.

EGU25-3528 | ECS | Orals | AS3.41 | Highlight

MethaneSAT: Quantifying Discrete and Dispersed Methane Sources on Basin-Scales 

Marvin Knapp, Joshua Benmergui, Ethan Kyzivat, Zhan Zhang, Maryann Sargent, Sébastien Roche, Christopher Chan Miller, Sasha Ayvazov, Marcus Russi, and Steven C. Wofsy

MethaneSAT is a satellite that observes the total column dry-air mole fraction of methane (XCH4) at high spatial resolution (100 m x 400 m) and precision (20 - 40 ppb) over target areas of 200 km x 200 km. Its observations uniquely enable the simultaneous quantification of discrete point and dispersed area methane sources within a single scene, addressing a critical gap in space-based methane monitoring. The mission focuses on characterizing methane emissions from the oil and gas industry, targeting over 80% of the sector’s global emissions.

We present methane observations from MethaneSAT and showcase a methodology to quantify sources within the target area. Emissions of discrete point sources causing distinct methane plumes are quantified using the Divergence Integral algorithm1. Additionally, an inverse modeling approach, informed by atmospheric transport simulated with the Stochastic Time Inverted Lagrangian Transport (STILT)2 model, is employed to constrain the magnitude and location of dispersed sources.

1Chulakadabba et al., 2023: Methane point source quantification using MethaneAIR: a new airborne imaging spectrometer
2Lin et al., 2003: A near-field tool for simulating the upstream influence of atmospheric observations: The Stochastic Time-Inverted Lagrangian Transport (STILT) model

How to cite: Knapp, M., Benmergui, J., Kyzivat, E., Zhang, Z., Sargent, M., Roche, S., Miller, C. C., Ayvazov, S., Russi, M., and Wofsy, S. C.: MethaneSAT: Quantifying Discrete and Dispersed Methane Sources on Basin-Scales, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3528, https://doi.org/10.5194/egusphere-egu25-3528, 2025.

EGU25-4622 | ECS | Orals | AS3.41

Evaluating the Utility of Satellite Observations for Improving Bottom-Up National Emission Inventories: Application to Colombia 

Sarah Hancock, Lucas Estrada, Nicholas Balasus, James East, Melissa Sulprizio, Xiaolin Wang, Zichong Chen, Daniel Varon, Rodrigo Jiménez, Andrés Ardila, Luis Morales-Rincon, Nestor Rojas, Christian Frankenberg, and Daniel Jacob

Methane is a potent greenhouse gas, and detailed understanding of its contributions from different countries and source sectors is necessary for climate action. Livestock is the dominant anthropogenic methane source, but bottom-up estimates of its emissions have high uncertainties. Inversions of satellite observations of atmospheric methane can offer valuable top-down information, but the related uncertainties need to be carefully characterized. Colombia has a large proportion of methane from livestock, and past work over the region has identified discrepancies between bottom-up and top-down emissions estimates, particularly for the livestock sector. Here, we explore this discrepancy in detail by quantifying 2023 methane emissions in Colombia and the contributions from different sectors at up to ~12 km × 12 km resolution including error characterization using an analytical inversion ensemble of TROPOMI and GOSAT satellite observations of atmospheric methane. We also assess the potential of future Carbon-I satellite observations to further reduce uncertainties in emissions. We show that choices in the inversion setup, including the number of state vector elements and the prior emission inventories, have a significant impact on emission estimates. The high resolution of our inversion results allows us to relate our emission estimates to bottom-up processes. Results demonstrate the ability of satellite observations of methane to improve our process-based understanding of methane emissions in Colombia.

How to cite: Hancock, S., Estrada, L., Balasus, N., East, J., Sulprizio, M., Wang, X., Chen, Z., Varon, D., Jiménez, R., Ardila, A., Morales-Rincon, L., Rojas, N., Frankenberg, C., and Jacob, D.: Evaluating the Utility of Satellite Observations for Improving Bottom-Up National Emission Inventories: Application to Colombia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4622, https://doi.org/10.5194/egusphere-egu25-4622, 2025.

EGU25-4728 | ECS | Orals | AS3.41

Airborne Measurements and Modelling of Methane Emissions from Oil and Gas Industry During the ROMEO Campaign 2019 

Hossein Maazallahi and the Airborne In Situ Measurements and Modeling Team of the ROMEO Campaign

Romania’s oil and gas infrastructures belong to the strongest CH4 emitters in Europe. Despite this, quantification of emissions in the region has been limited. During the large multi-scale ROMEO (ROmanian Methane Emissions from Oil and gas) campaign in 2019, top-down methane emission estimates were derived using in-situ measurements from two aircraft, supported by two atmospheric model simulations.

Annual emissions from the Southern Romanian Oil and Gas (O&G) infrastructure were estimated at 227 ± 86 kt CH4 yr⁻¹ resulting in a per-site Emission Factor of 5.3 ± 2.0  kg CH4 h-1 site-1. This is consistent with previously published ground-based site-level measurements conducted during the same period. Low wind conditions during the campaign complicated direct comparisons of individual plumes between measurements and the model simulations. Nevertheless, correlations of CH4 plumes observed during large-scale raster flights and mass balance flights with modelled plumes suggest that the emission factors derived for a limited number of production clusters and regions are representative for the larger southern Romanian production basin.

Our results show agreement between aerial and ground-based estimates and corroborate significant underreporting of methane emissions from Romania's O&G industry to the United Nations Framework Convention on Climate Change (UNFCCC) in 2019. Furthermore, the study highlights substantial underestimation of O&G emissions in the Emissions Database for Global Atmospheric Research (EDGAR) v7.0 for the study domain.

How to cite: Maazallahi, H. and the Airborne In Situ Measurements and Modeling Team of the ROMEO Campaign: Airborne Measurements and Modelling of Methane Emissions from Oil and Gas Industry During the ROMEO Campaign 2019, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4728, https://doi.org/10.5194/egusphere-egu25-4728, 2025.

EGU25-5106 | Posters on site | AS3.41

Direct measurements of methane emissions from natural gas end use in Germany 

Mary Kang, Rainer Hilland, Tamara Weghorst, Timo Sanzol Rieth, Jia Chen, Stefan Schloemer, Martin Blumenberg, and Andreas Christen

Natural gas appliances and piping in buildings, or post-meter sources, are estimated to represent 15% of U.S. natural gas distribution sector emissions of methane. However, recent atmospheric methane measurement studies in urban areas indicate that end use emissions may be several times higher than currently estimated in national inventories. National inventories use bottom-up methods to estimate post-meter methane emissions, but due to the relatively small set of direct measurements, if available, many inventory estimates are likely to be highly uncertain. Moreover, there are systematic differences in building heating systems and natural gas appliance usage across countries and regions. For example, North American households mainly use forced air systems that rely on ducts and vents; while in Germany, it is common to distribute heat from a central heating unit through radiators. Therefore, although there have been several publications of direct measurement studies conducted in the U.S., it is difficult to extrapolate these findings to other countries and regions, including Germany, the largest natural gas user in Europe.

To better understand and quantify emissions from natural gas end use in Germany, we analyze spatially-integrated tall-tower eddy covariance surface fluxes of methane and conduct direct measurements of methane emissions from natural gas appliances and piping in homes and other buildings. The measurement data includes gas composition analysis and are analyzed in conjunction with natural gas appliances and building attributes. Our results can inform effective methane emission mitigation strategy development and energy transition policies in Germany and elsewhere.

How to cite: Kang, M., Hilland, R., Weghorst, T., Sanzol Rieth, T., Chen, J., Schloemer, S., Blumenberg, M., and Christen, A.: Direct measurements of methane emissions from natural gas end use in Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5106, https://doi.org/10.5194/egusphere-egu25-5106, 2025.

Non-producing oil and gas wells emit methane, a greenhouse gas with approximately 80 times the warming potential of carbon dioxide over a 20-year period. Reducing methane emissions from the oil and gas industry is crucial in assuring Canada reaches its pledge of cutting greenhouse gas emissions by 40% below 2005 levels by 2030. Currently, British Columbia (BC) hosts approximately 20,000 non-producing oil and gas wells. The British Columbia Energy Regulator (BCER) has been conducting annual LiDAR-based helicopter surveys of methane emissions, with 1,334 non-producing oil and gas wells surveyed from 2017 to 2024. To estimate methane emissions rates using BCER's helicopter survey data, we performed a controlled release test of the Lasen Airborne LiDAR Pipeline Inspection System to evaluate the detection range. The controlled-release testing involved multiple helicopter flyovers over a single site, during which various methane flow rates, ranging from 0.05 to 1.8 kg/hr, were released. We used our test results to combine available BCER aerial survey data and ground-based measurements and estimate total methane emissions from non-producing oil and gas wells across BC.

How to cite: Woolley, L. and Kang, M.: Estimating Methane Emissions from Non-Producing Oil and Gas Wells in British Columbia Using a Helicopter-Based Methane Detection System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5125, https://doi.org/10.5194/egusphere-egu25-5125, 2025.

EGU25-5202 | Posters on site | AS3.41

Longterm urban eddy covariance observations of methane and other trace gases reveal characteristic anthropogenic emission hotspots 

Thomas Karl, Michael Stichaner, Werner Jud, Christian Lamprecht, Niels Jensen, Giovanni Manca, Arianna Peron, Martin Graus, and Shahid Naqui

Eddy covariance observations are particularly well suited to study emission processes at the ecosystem scale. Here we combine longterm observations of methane, carbon dioxide and nitrogen oxides, with campaign-based observations of NMVOC fluxes in an urban area. The complex dataset allows unravelling the fate of urban methane emissions for the city of Innsbruck. Our analysis shows that most of the methane in the urban area is emitted via pre-flush operation and partially burned methane from poorly maintained gas furnaces. Methane fluxes show a negative temperature dependence and are highly correlated with ethane fluxes. An average ethane to methane flux ratio of 5% is observed, consistent with the gas composition supplied to Western Austria/Southern Germany. The 20y GWP of the emitted methane in the residential, commercial and public sector can be as high as 20-30% relative to CO2. This study shows that the conversion of gas furnaces to heat pumps can have an additional immediate benefit through the reduction unburned methane.

How to cite: Karl, T., Stichaner, M., Jud, W., Lamprecht, C., Jensen, N., Manca, G., Peron, A., Graus, M., and Naqui, S.: Longterm urban eddy covariance observations of methane and other trace gases reveal characteristic anthropogenic emission hotspots, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5202, https://doi.org/10.5194/egusphere-egu25-5202, 2025.

EGU25-5538 | Posters on site | AS3.41

Aircraft- and ground-based quantification of coal mine methane emissions in the Hunter Coalfields, Australia 

Bryce F.J. Kelly, Nicholas M. Deutscher, Stephen J. Harris, Hannah Beaton, Tarra Brain, Andrew McGrath, Jorg Hacker, Adrain Murphy, Wolfgang Junkermann, Clare Paton-Walsh, Nicholas B. Jones, and Hasan Nawaz

In recent years, credible atmospheric observations of methane emissions suggest that annual methane emission estimates in inventories for some Australian coal mining regions or facilities may be underestimated. A lack of well-constrained, mine-scale studies for open-cut (pit) coal mines continues to hinder discussions on emission estimates and the refinement of estimation methods for Australian open-cut coal mining facilities. Here, we present preliminary results from aircraft- and ground-based atmospheric measurements recorded in November 2024 in the Hunter Coalfield, NSW, Australia.

Australia employs higher-Tier IPCC methodologies – Tier 2 (basin-specific) and Tier 3 (mine-specific, Methods 2 and 3 ) – under its National Greenhouse and Energy Reporting (NGER) Scheme to estimate open-cut coal mine emissions. These methods rely on the use of coal core gas content to estimate methane emissions from open-cut mine complexes. However, Methods 2 and 3 have never been validated using airborne or ground-based time series observations.

While coarse-resolution satellites like TROPOMI can quantify coal mine emissions at regional scales (Sadavarte et al., 2021; Palmer et al., 2021), their limited spatial resolution reduces their effectiveness for verifying annual inventory reported emissions at the scale of individual mines. Additionally, the ability of point-source imaging satellites to quantify emissions from individual open-cut coal mines remains uncertain. Coal seam blasting prior to extraction can be considered a point source; however, open-cut coal mines have various continuous diffuse methane sources that also need to be quantified. The diffuse sources include, among others, emissions from beneath the pit floor, lateral diffusion along coal seams and other rock strata in the mine walls, rock waste piles, and areas of in situ biological production, such as water management ponds. Aircraft- and ground-based technologies have the potential to measure both point and diffuse sources of methane, thus providing a potential pathway for verifying greenhouse gas inventories determined using approved IPCC methodologies.

During this measurement campaign in the Hunter Coalfield, a research aircraft flew instruments to collect in-situ atmospheric measurements of methane and carbon dioxide mole fractions, along with GPS and meteorological data. These data were used to make rate of methane emission estimates downwind of individual coal mine complexes. Aerosol size and particle number concentration measurements and high-resolution airborne  LiDAR imagery were also acquired to aid in source attribution. These measurements were complemented by ground-based EM27/SUN solar absorption spectrometer instruments positioned upwind and downwind of the same coal mining complexes. Comparisons between emissions derived from the aircraft-base, ground station EM27/SUN observations, and operator-reported coal mine methane emissions will be presented.

Palmer, P. I., Feng, L., Lunt, M. F., Parker, R. J., Bösch, H., Lan, X., Lorente, A., and Borsdorff, T.: The added value of satellite observations of methane for understanding the contemporary methane budget, Phil. Trans. R. Soc. A., 379, 20210106, https://doi.org/10.1098/rsta.2021.0106, 2021.

Sadavarte, P., Pandey, S., Maasakkers, J. D., Lorente, A., Borsdorff, T., van der Gon, H. D., Houweling, S., and Aben, I.: Methane emissions from superemitting coal mines in Australia quantified using TROPOMI satellite observations, Environmental Science & Technology, 55, 16573–16580, https://doi.org/10.1021/acs.est.1c03976, 2021.

How to cite: Kelly, B. F. J., Deutscher, N. M., Harris, S. J., Beaton, H., Brain, T., McGrath, A., Hacker, J., Murphy, A., Junkermann, W., Paton-Walsh, C., Jones, N. B., and Nawaz, H.: Aircraft- and ground-based quantification of coal mine methane emissions in the Hunter Coalfields, Australia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5538, https://doi.org/10.5194/egusphere-egu25-5538, 2025.

EGU25-5668 | Orals | AS3.41

Methane Emissions from Offshore Shuttle Tanker Loader Installations in the North Sea 

Ruth Purvis, Ralph Burton, James Lee, James Hopkins, Will Drysdale, Tom Moore, Grant Allen, and Kyle Dawson

The full range of emissions from oil and gas production, especially offshore, is still not fully understood due to the vast number of sources and lack of observational data. Emissions from shuttle tanker loading are not well characterised, with research limited and mainly non methane volatile organics (NMVOCS) rather than methane (CH4). There is also a grey area on where they should be included in inventories and the latest National Atmospheric Emissions Inventory United Kingdom Green House Gas (NAEI_UK_GHG) Inventory Improvement Report (July 2022) cited evidence for emissions factors from methane (CH4) and non methane volatile organics (NMVOCS) compounds from oil loading as a future priority research area. 

This work shows CH4 emissions results from a campaign in October 2023 designed to investigate CH4 and NMVOC emissions from oil loading to shuttle tankers over the whole loading cycle.  The project used aircraft measurements from a research aircraft and unmanned aerial vehicle along with different modelling techniques to evaluate emissions from the complete tanker loading process. Increases in CH4 emissions were observed when the shuttle tanker was present when compared to the standard platform operating conditions. 

How to cite: Purvis, R., Burton, R., Lee, J., Hopkins, J., Drysdale, W., Moore, T., Allen, G., and Dawson, K.: Methane Emissions from Offshore Shuttle Tanker Loader Installations in the North Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5668, https://doi.org/10.5194/egusphere-egu25-5668, 2025.

EGU25-7528 | Orals | AS3.41

Measurement-based insights into methane emissions from LNG export terminals in Australia 

Mark Lunt, Jorg Hacker, Stephen Harris, and Wolfgang Junkermann

Global liquefied natural gas (LNG) exports were around 400 Mt in 2023, with 20% of this production from Australia. The industry-wide extent of methane (CH4) emissions from LNG export terminals are not well characterized in the literature through measurement-based methods, leading to a range of values being used in life cycle analyses.  As part of UNEP’s International Methane Emissions Observatory Methane Science Studies, a series of scientific flights were conducted around eight LNG liquefaction terminals in Australia between 2021 and 2024, covering 95% of Australian LNG nameplate capacity. In-situ mole fractions of CH4 and carbon dioxide (CO2) were measured on the research aircraft, in addition to meteorological data, GPS data and measurements of ultrafine particles. The measurements resulted in over 100 CH4 mass balance quantifications and an extensive dataset to explore tracer correlations between CH4 and CO2 which aid emissions quantification and understanding. Here, we present the most extensive measurement-based analysis of site-level emissions to date from LNG export terminals, enabling us to examine industry-wide methane emissions and emission intensities. We explore factors that impact derived emission intensities from different LNG sites and the implications for methane emissions from the wider LNG supply chain. 

How to cite: Lunt, M., Hacker, J., Harris, S., and Junkermann, W.: Measurement-based insights into methane emissions from LNG export terminals in Australia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7528, https://doi.org/10.5194/egusphere-egu25-7528, 2025.

Atmospheric methane (CH4), the second most important greenhouse gas, poses substantial uncertainties with its global emission inventory. We use inverse modeling analyses with Greenhouse Gases Observing Satellite (GOSAT) XCH4 data to reduce those uncertainties and obtain improved quantitative estimates of sectoral monthly methane emissions from January 2010 to December 2019. We first conducted GEOS-Chem simulations with global emission inventories, including GFEIv2, EDGARv8, and WetCHARTs. The model with the global emission inventories showed a cumulative negative bias of approximately -1% per year compared to the GOSAT data, primarily due to the underestimation of tropical wetland emissions. Simulated monthly mean methane concentrations with the Kalman filter were used to optimize monthly variations of different sectoral CH4 emissions over the decade, focusing on anthropogenic sources often assumed to be aseasonal in previous studies. Our inverse analyses resulted in increases of the global CH4 emission trend of 3.86 Tg yr-1 from 2.55 Tg year-1, driven mainly by increases of agricultural and waste management sources. The seasonality of global methane emissions is more prominent in our top-down emission estimates than bottom-up emission, mainly driven by increased agricultural emissions in the Northern Hemisphere and tropical regions during June, July, and August. Furthermore, the top-down estimates of waste management emissions exhibited a significant summer peak in the Northern Hemisphere, indicating its temperature sensitivity, which was previously not recognized. The inverse analysis of methane emissions significantly reduced the spatiotemporal biases of the GEOS-Chem model compared to TCCON XCH4, demonstrating the robustness of the inversion.

How to cite: Oh, S.-I. and Park, R. J.: Constraining the Seasonal and Interannual Variability of Global Sectoral Methane Emissions in the 2010s using GOSAT XCH4 data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8399, https://doi.org/10.5194/egusphere-egu25-8399, 2025.

EGU25-8421 | ECS | Orals | AS3.41

Toward a robust quantification of methane emissions in a medium-sized city: initial results from mobile and stationary measurements 

Kaiwen Liu, Martin Goxe, Grégoire Broquet, Adrien Mignot, Chloé Menant, Olivier Laurent, Elise Potier, Philippe Bousquet, and Jean-Daniel Paris

Quantifying methane (CH₄) emissions at the scale of medium-sized European cities remains a significant challenge due to the relatively low annual levels, the spatial and temporal heterogeneity of these emissions. We aim to develop a framework for quantifying urban CH4 emission including nature gas and waste emissions, following a protocol compatible with the reporting framework of the Oil & Gas Methane Partnership (OGMP) 2.0 for natural gas distribution operators.

Le Mans, a medium-sized city in the Pays de la Loire region of France with a population of approximately 150,000 is selected as a pilot case. The approach combines mobile measurements and fixed monitoring stations to quantify CH₄ emissions and identify natural gas leaks and other potential emission hotspots in the city.

Here, we report on the tests of five Aeris mid infra-red analysers MIRA LDS intended for fixed deployment in the city to monitor CH₄ concentration variations due to the urban emissions. The resulting system demonstrated sufficient precision, with methane and ethane measurement accuracies better than 5 ppb and a few ppt, respectively. We modified the analysers and implemented a two-level calibration strategy with daily injections to achieve sensor stability.

Additionally, mobile surveys were conducted, covering approximately 36% of the streets of the city Le Mans and parts of the roads in the suburbs. These campaigns aimed to: (1) detect and quantify fugitive point source emissions, (2) characterize large-scale CH₄ variations, (3) evaluate the effect of air inlet location, and (4) quantify emissions from major emitting sites. We identified CH₄ point sources linked to natural gas infrastructure and non-natural gas sources. We distinguish between large plumes presumably from large emitters and fugitive spikes indicative of possible local gas leaks. Over 15 transects have been led across the plume from the wastewater treatment plant (WWTP) in Le Mans and allow to estimate the site’s contribution to the city’s emission. Additionally, the analysis of air inlet positions revealed that higher air inlet locations are more suitable for analyzing the plume transects, whereas lower air inlet positions are better suited for detecting peaks associated to near ground or subsurface fugitive emissions.

Finally, exploiting these results, we discuss the capability of a network of fixed stations to measure small variations of CH4 (of the order of tens of ppb) across the city. These results will lead to the implementation of the fixed network over the next 2 years in the city (at the end of 2026), complemented by continued mobile campaigns to analyze emission trends, variability, and sector-specific contributions.

How to cite: Liu, K., Goxe, M., Broquet, G., Mignot, A., Menant, C., Laurent, O., Potier, E., Bousquet, P., and Paris, J.-D.: Toward a robust quantification of methane emissions in a medium-sized city: initial results from mobile and stationary measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8421, https://doi.org/10.5194/egusphere-egu25-8421, 2025.

EGU25-8493 | Orals | AS3.41

Observing Chinese Coal Mine Methane Emissions Smoothly Across Scales: Powering Future Mitigation 

Jason Cohen, Wei Hu, Yanqiu Liu, Fan Lu, Shuo Wang, Bo Zheng, Lingxiao Lu, Pravash Tiwari, Qin He, and Kai Qin

This work describes observations made over the past three years at high gas coal mines in Shanxi and Xinjiang observed from underground; surface concentrations and fluxes; horizontal and upward looking FTIR; high spatial resolution remote sensing using moderate spectral resolution (GF5 and PRISMA); and lower spatial resolution remote sensing using high spectral resolution (TROPOMI). Systematic analysis is made using flexible, mass-conserving, and computationally fast inversion tools. High resolution emissions are computed and analyzed considering spatial variation, wind, three-dimensional spread, and observational uncertainty. These emissions are observed to contain fat tail distributions and uncertainties. When applied in attribution forward-backward mode, a probabilistic attribution is computable, with results consistent between different observations tyles when and where they were made. Attribution is sometimes possible both for the known sources and other second source (i.e., adjacent mines, additional fissures or ventilation shafts, or long-range transport from outside the domain). Advantages, weaknesses, and ranges of uncertainties of each observation type is explored.

These results are then used to train mesoscale mass conservation systems that govern the transport, diffusion, and interactions, allowing for emissions estimation, uncertainty, and attribution. These trained models are applied to TROPOMI and other observations at the kilometer to 10-kilometer scale, and demonstrate day-by-day and grid-by-grid emissions which are quantifiable and reasonable when compared with independent surface observations. Furthermore, the results are shown to be smooth and consistent across some other coal mining areas, when and where observational uncertainties were initially strictly considered in the model fitting and after unbiased analysis is applied.

Issues of when the errors are large or emissions estimations are not reliable are discussed including: different coal fields, underground coal fires, high absorbing aerosol conditions, and variable topography. When emissions can be computed under these conditions, reasons are given, and future work options are discussed. New measurements and campaigns and modeling enhancements will be discussed. In specific, limitations on the current generation of surface and remotely sensed measurements will be made in terms of ever tightening emissions rules. Steps to rectify the identified gaps are proposed.

General results reflect current understanding: high gas mines are significant sources of methane emissions which require active mitigation or yield emissions larger than current bottom-up estimates. Treating emissions as normally distributed leads to results not being sufficiently robust to extrapolate to annual or longer datasets. Some scientific points raised include: active consideration of observational error frequently leads to emissions inversions not being reliable; applying unbiased filters to observational uncertainty removes both high and low emissions inversions, allowing more confidence in unfiltered low emissions sources; attribution of multiple sources on a single TROPOMI grid may be easier when applied over a common coal field, allowing field wide emissions predictions under lower-gas or higher mitigation conditions.

How to cite: Cohen, J., Hu, W., Liu, Y., Lu, F., Wang, S., Zheng, B., Lu, L., Tiwari, P., He, Q., and Qin, K.: Observing Chinese Coal Mine Methane Emissions Smoothly Across Scales: Powering Future Mitigation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8493, https://doi.org/10.5194/egusphere-egu25-8493, 2025.

Methane (CH4), due to its strong global warming potential and roughly decade lifetime, plays a pivotal role in near-term climate mitigation strategies. Coal mine methane (CMM) is a major source of CH4 globally, and particularly so in coal-producing regions. Effective control of CMM emissions is crucial for mitigating climate change impacts. This study integrates multi-scale observational datasets including in-situ observations, column FTIR observations, and daily satellite remote sensing together with high-resolution atmospheric modeling to investigate CH4 transport and source contributions. The steps are hoped to lead to future development of a quantitative inverse modeling system flexible enough to provide for spatially-targeted, high-frequency mitigation strategies and interventions.

The Weather Research and Forecasting model is configured with its greenhouse gas tracer option (WRF-GHG) to separate sources of CH4 on a grid-by-grid basis. This work employs a nested three-domain structure with the central region covering China’s major coal-producing regions, including the Qinshui Coalfield and 139 coal mines at 3km resolution. Ground-based in situ measurements from eddy covariance flux tower, mobile measurements using portable LGR analyzers, and upward looking EM27 FTIR previously deployed by the AERSC team at around 950 m elevation in Changzhi in Shanxi Province, provide high-frequency a priori emissions to drive the model, as well as in situ data to refine the simulations. Observations from TROPOMI, TCCON (in the 9km region) and the GAW WLG station (in the 27km region), provide additional datapoints for comparison and quantification of the spatial, temporal, and goodness of representation of fit. This study resolves CH₄ concentration dynamics across scales, from regional to individual coal mines. It is hoped that the results can offer a quantitative means to identify and attribute emissions from these major emitting regions at high spatial and temporal frequency.

A few interesting scientific points are explained in detail. (1) The WRF-GHG model shows improved agreement with observational datasets, especially so in terms of capturing more extreme events, when the AERSC team’s emissions datasets are used. Quantitative differences between WRF-GHG and TROPOMI_L3 demonstrate that while some areas are robust, other areas have significant differences, explained in part by the improved emissions inventories used herein. (2) Existing inventories lead to average values of XCH4 simulated across 139 individual coal mines being lower than the observations made by the AERSC group, while at the same time leading to average values of XCH4 in a subset of other regions not measured as being much higher than available observations. These regions and differences are detailed, and rationales for these differences are proposed. (3) Near-surface CH4 concentrations show that anthropogenic CH4 emissions contributes only 17.1% of total CH4 within a 12 km radius of coal mining sites which is far too low, although the diurnal variations are closely linked to coal production activities, highlighting the model's robustness in capturing these dynamics but the problems with the spatial and magnitude aspects of current emission inventories.

How to cite: Liu, Y., Qin, K., and Cohen, J. B.: High Spatial and Temporal Resolution Assessment of Methane Emissions in Major Coal-Producing Regions of China Driving In Situ and Column Observations by WRF-GHG, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9311, https://doi.org/10.5194/egusphere-egu25-9311, 2025.

EGU25-10622 | Posters on site | AS3.41

Methane Emissions from Industrial Activities: Quantification of Selected Polish and Middle East Sources by a Unique Helicopter Probe 

Heidi Huntrieser, Eric Förster, Falk Pätzold, Lutz Bretschneider, Niclas Maier, Jaroslaw Necki, Jakub Bartyzel, Pawel Jagoda, Benjamin Witschas, Anke Roiger, Astrid Lampert, Oman Environmental Services Holding Company (be´ah), and Mark Lunt

Global warming is proceeding rapidly and quick actions are required to suspend the increasing temperatures globally. Here we give an overview of a series of measurement studies, supported and funded by UNEP´s International Methane Emissions Observatory (IMEO) in 2022-2023. Methane (CH4) is the primary focus of all these studies, since it is one of the most potent greenhouse gases, which at the same time has a relative short lifetime. Due to these specific characteristics, CH4 is presently the prime target for mitigating emissions from industrial activities.

Our approach focused on a variety of CH4 emissions from the coal, oil and gas (O&G), and waste industry in Poland and in the Middle East within the framework of METHANE-To-Go-Poland and METHANE-To-Go-Oman. A unique helicopter-towed probe, HELiPOD, was equipped with in situ CH4 instrumentation complemented by mobile ground-based CH4 measurements. The well-known mass balance approach was applied to quantify the CH4 emissions from the targeted sources. Final comparisons of our top-down estimates with bottom-up industry or inventory data have been carried out to assist the involved companies and related governments in prioritizing their CH4 emission mitigation actions and policies for future endeavours. Several non-captured CH4 source strengths, compared to the available bottom-up data, were discovered in the course of these top-down studies. For a number of reasons evaluated during our operations, the novel HELiPOD set-up is proposed to be a suitable platform for upcoming satellite evaluation studies focusing on CH4. In particular, the HELiPOD measurements (CH4 mixing ratio plus 3D wind) can capture the whole vertical and horizontal extension of targeted CH4 plumes, which is necessary for the CH4 mass flux quantification, a number that can be directly comparable to available satellite-based flux rates in UNEP´s Methane Alert and Response System (MARS).  

How to cite: Huntrieser, H., Förster, E., Pätzold, F., Bretschneider, L., Maier, N., Necki, J., Bartyzel, J., Jagoda, P., Witschas, B., Roiger, A., Lampert, A., (be´ah), O. E. S. H. C., and Lunt, M.: Methane Emissions from Industrial Activities: Quantification of Selected Polish and Middle East Sources by a Unique Helicopter Probe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10622, https://doi.org/10.5194/egusphere-egu25-10622, 2025.

EGU25-10770 | ECS | Posters on site | AS3.41

Development of a Mobile Measurement Unit to Identify and Map Local Methane Sources 

Christoph Asam, Daniel Kühbacher, Andreas Luther, Josef Stauber, and Jia Chen

Methane is a significant contributor to global warming, with its radiative forcing being approx. 32 times greater than that of CO2 over a hundred-year time frame. To advance the understanding of the earth's climate and mitigate global warming, collecting precise and reliable CH4 concentration data is essential. 

We present a mobile measurement unit to identify and map local methane sources. The unit is mounted on a cargo bike, enabling flexible use in urban areas such as parks, pedestrian zones, or event spaces. It incorporates a high-precision CRDS trace gas analyzer (Picarro G2401) to measure CH4 concentrations and a wind sensor to capture wind speed and direction. A shock-absorbing frame ensures suspension during the transporting of the analyzer and supporting equipment. The mobile unit’s power distribution system allows dynamic switching between mains and battery power and hot-swapping of batteries during operation. A modular software stores the collected data and displays the mapped concentrations in real-time to the cargo bike driver via smartphone.

We conducted 13 measurement trips across Munich, covering a total distance of 170km, to map areas with potential methane emissions, including two wastewater treatment plants, a former landfill, a combined heat and power plant, and the Oktoberfest grounds. Fluctuations up to +2% above the baseline were observed across the city. The baseline was defined as the 5th percentile of all measurements of the corresponding trip. Additionally, significant enhancements of up to 204.9 ppm were detected, which were attributed to an unidentified methane leak near Munich's central station, with an estimated emission rate of 20.5 l/min. 

We further integrated an OF-CEAS trace gas analyzer (LI-COR LI7810) into the setup for three side-by-side trips, allowing for a preliminary comparison and assessment of analyzer performance. 

With this setup being easily transferable to other cities or, e.g., industrial parks, a versatile tool is present to detect and analyze methane sources and advance methane emission mitigation.

How to cite: Asam, C., Kühbacher, D., Luther, A., Stauber, J., and Chen, J.: Development of a Mobile Measurement Unit to Identify and Map Local Methane Sources, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10770, https://doi.org/10.5194/egusphere-egu25-10770, 2025.

EGU25-11837 | Orals | AS3.41

Challenges with Developing Comprehensive Oil and Natural Gas Operator-Level Measurement-Based Methane Emissions Inventories in the U.S.  

Bailey Fosdick, Chris Moore, Hon Xing Wong, Zachary Weller, Abigail Corbett, Yannik Roell, Ella Martinez, Amanda Berry, and Natalia Gielczowski

Measurement-based methane emissions inventories are essential for U.S. oil and natural gas operators to track their progress toward emissions targets and demonstrate the impact of improved operational and monitoring practices. However, translating raw emission measurement data, whether from continuous monitoring systems, aerial flyovers, or operational cause analyses, into emissions inventories is nontrivial. In this talk, we discuss findings from a United States Department of Energy funded project where we investigated how to combine a bottom-up inventory required by regulatory agencies, data from continuous monitoring systems, data from aerial flyovers, and follow-up operator cause analysis data to develop an operator-level emissions inventory. We introduce the concept of a comprehensive measurement-based emissions inventory, which represents all emissions across the entire time frame, across all spatial assets, and of all emissions sizes. We carefully characterize the extrapolation efforts necessary to create a comprehensive emissions inventory estimate with data from each type of technology. Understanding these methods is essential for operators preparing defensible emissions inventory reports that adhere to reporting frameworks such as Veritas and OGMP 2.0. In many cases, there are several possible extrapolation approaches of varying complexity and with various underlying assumptions. We provide simple examples to illustrate the sensitivity of annual emissions estimates to the various extrapolation approaches and highlight the challenges, strengths, and limitations when working with data from each of the technologies. 

How to cite: Fosdick, B., Moore, C., Wong, H. X., Weller, Z., Corbett, A., Roell, Y., Martinez, E., Berry, A., and Gielczowski, N.: Challenges with Developing Comprehensive Oil and Natural Gas Operator-Level Measurement-Based Methane Emissions Inventories in the U.S. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11837, https://doi.org/10.5194/egusphere-egu25-11837, 2025.

EGU25-11860 | Posters on site | AS3.41

Methane retrievals and emission estimates of localized sources from EnMAP and EMIT space-borne data 

Maximilian Reuter, Michael Hilker, Stefan Noël, Jonas Hachmeister, Michael Buchwitz, Oliver Schneising-Weigel, Heinrich Bovensmann, John P. Burrows, and Hartmut Bösch

Anthropogenic emissions of methane (CH4) are the second-largest anthropogenic source of greenhouse gases after carbon dioxide (CO2) and are a major driver of climate change. Rapid reductions in emissions would help reduce near-term warming. Analysis of satellite data provides information on methane emissions from important localized methane sources such as landfills and fossil fuel extraction sites. This information is used to identify emission sources, quantify their emissions, and monitor progress in reducing emissions. However, this application requires careful analysis of the satellite data because extracting reliable information on atmospheric methane concentration variations and emission estimates from the measured radiance is not trivial, as the measured radiance is affected not only by methane but also by many other interfering effects, including clouds and surface features. Several ESA (GHG-CCI, MEDUSA, SMART-CH4) and EU (EYE-CLIMA) projects focus on the further development of the algorithms needed for reliable emission detection and quantification. This includes the application of the algorithms to several important methane sources and intercomparisons with results from other groups using independently developed methods. In this context, we are developing the HighResolutionFit (HiFI) package, which implements several methods to retrieve atmospheric methane information from high-resolution satellite sensors such as EnMAP and EMIT. The corresponding atmospheric data products are used to obtain emission information using a Cross-Sectional Flux (CSF) method. Here we present the latest status of these activities, including comparisons with corresponding results from other groups.

How to cite: Reuter, M., Hilker, M., Noël, S., Hachmeister, J., Buchwitz, M., Schneising-Weigel, O., Bovensmann, H., Burrows, J. P., and Bösch, H.: Methane retrievals and emission estimates of localized sources from EnMAP and EMIT space-borne data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11860, https://doi.org/10.5194/egusphere-egu25-11860, 2025.

EGU25-11938 | ECS | Orals | AS3.41

A Demonstrated Reconciliation of Top-Down and Bottom-Up Methane Measurements to Derive Verified Emission Intensities 

Shona Wilde, David Tyner, Bradley Conrad, and Matthew Johnson

Oil and gas companies striving to attain the OGMP2.0 “Gold Standard” for methane Measurement, Reporting, and Verification (MRV) are required to find and measure individual methane sources across all their operating assets, and in particular, to verify total emissions using an independent "top-down" measurement.  The process of comparing source-level and top-down measurements is termed “reconciliation” and is an essential part of meeting the “Gold Standard”.  However, to date, there is no prescriptive OGMP 2.0 protocol on how to reconcile site and source-level measurements, and there are key knowledge gaps regarding calculation methods, required sample sizes, and uncertainty protocols.

This study demonstrates a novel framework for reconciling on site source measurements with independent source-resolved aerial survey data to derive corporate methane emissions and intensity data sufficient to meet or exceed the OGMP 2.0 Gold Standard certification requirements. Critically, the protocol allows for direct analysis of measurement uncertainties.  In partnership with an oil and gas producer operating in Canada, a source-level inventory is first created based on extensive ground measurements and company-specific emission factors.  Independent source-resolved measurements, covering 100% of the company’s operating assets, are then conducted using Bridger Photonics Inc.’s Gas-Mapping LiDAR (GML).  Multi-pass aerial data are analyzed using detailed probability of detection models, which consider the conditions of each pass, and integrated with the bottom-up data to account for unmeasured sources.  The result is a comprehensive, verified inventory of total methane emissions for the company.  As part of this demonstration, the analysis is repeated using up to four independent aerial surveys, providing real-world insights to the importance of temporal variability in emissions and its influence on required sample sizes for accurate reconciliation.  The results have important implications for creating MRV protocols that ensure reported emissions adequately represent the variable nature of emissions, particularly when sample sizes are small because measurements are limited to assets from a single operator as is the case under OGMP2.0 reporting.

How to cite: Wilde, S., Tyner, D., Conrad, B., and Johnson, M.: A Demonstrated Reconciliation of Top-Down and Bottom-Up Methane Measurements to Derive Verified Emission Intensities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11938, https://doi.org/10.5194/egusphere-egu25-11938, 2025.

EGU25-11972 | ECS | Posters on site | AS3.41

Characterization and methane emissions potential of non-producing oil and gas wells in Colombia and Argentina 

Manuela González Sánchez, Jade Boutot, Florencia Carreras, Andreea Calcan, James Lawrence France, and Mary Kang

Non-producing oil and gas wells can pose a significant risk to the environment and human health, and contribute to climate change by emitting methane, a potent greenhouse gas. However, the characterization, distribution, and methane emission profile of non-producing wells remain highly uncertain across the world. Here, we present a database analysis of non-producing oil and gas wells across Colombia and Argentina, which are countries with a long history of oil and gas development. By comparing well data from governmental and proprietary databases, we find more than 26,000 oil and gas wells in Colombia, of which about 6,000 (23%) are non-producing and more than 84,000 oil and gas wells in Argentina, of which approximately 51,000 (61%) are non-producing. Using these numbers, we estimate methane emissions from non-producing wells in Colombia and Argentina. In addition, we analyze well attributes such as well depth, well type (e.g., oil and gas), location, and well age and perform a spatial analysis to identify the regions/wells in Colombia and Argentina for field measurements. We find that the provinces of Santa Cruz, Chubut and Neuquén in Argentina, and the departments of Meta, Santander and Casanare in Colombia have the highest number of non-producing wells. Overall, these findings can be used to improve the characterization of existing oil and gas wells and to select representative samples of non-producing wells for methane emission monitoring in Colombia and Argentina.

How to cite: González Sánchez, M., Boutot, J., Carreras, F., Calcan, A., Lawrence France, J., and Kang, M.: Characterization and methane emissions potential of non-producing oil and gas wells in Colombia and Argentina, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11972, https://doi.org/10.5194/egusphere-egu25-11972, 2025.

EGU25-12148 | ECS | Posters on site | AS3.41

Drone-based methane emissions monitoring from orphaned oil and gas wells in Pennsylvania, US 

Jade Boutot, James L. France, Margaret Coleman, Adam S. Peltz, Valerie Fox-Coughlin, Neil Keown, Hari Viswanathan, and Mary Kang

More than a hundred thousand documented orphaned oil and gas wells are known to exist in the United States, with potentially millions remaining undocumented. Due to funding shortfalls, many orphaned wells remain unplugged and continue to emit methane, a potent greenhouse gas. Drone-based methane emission measurements can help prioritize mitigation efforts for orphaned wells and aid in locating undocumented orphaned wells, which are wells with unknown locations and conditions. In collaboration with the Pennsylvania Department of Environmental Protection (PA DEP) and the US Department of Energy’s (DOE) Orphan Well Program, we will present the results of drone-based methane emission measurements across four regions in Pennsylvania with a high likelihood of containing undocumented orphaned wells. We will share our insights on the potential for detecting methane emissions using drone-based tunable diode laser absorption spectroscopy (TDLAS), an emerging technology for methane monitoring in the oil and gas sector. Additionally, this work explores the foundation of a screening method for providing first-order estimates of methane emission rates at orphaned well sites. We will compare the methane measurements with potential well locations identified using drone-based magnetometry data, historical maps, LiDAR, and atmospheric data. Our results will be helpful for prioritizing plugging and remediation for the hundreds of thousands, and potentially millions, orphaned wells across the US and the world.

How to cite: Boutot, J., France, J. L., Coleman, M., Peltz, A. S., Fox-Coughlin, V., Keown, N., Viswanathan, H., and Kang, M.: Drone-based methane emissions monitoring from orphaned oil and gas wells in Pennsylvania, US, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12148, https://doi.org/10.5194/egusphere-egu25-12148, 2025.

EGU25-12569 | Orals | AS3.41

Using Repeated Aerial Methane Measurements to Assess Inventory Protocols and Track Year-over-year Trends in Emissions 

Matthew R. Johnson, Shona E. Wilde, David R. Tyner, and Bradley M. Conrad

Measurement-based inventories combining source-resolved aerial LiDAR measurements with bottom-up emission and activity data have provided unprecedented insight into the origins and magnitudes of oil and gas sector methane emissions and, in Canada, are now being used to inform methane estimates used in official national greenhouse gas inventory reporting.  However, the protocols for creating measurement-based inventories are new and continue to be refined as both measurement technology and scientific understanding of the oil and gas sector improve.  In this study, we examine independent, measurement-based inventory estimates derived from aerial survey data collected during 2020, 2021, 2023, and 2024 in the Canadian province of Saskatchewan; 2021, 2023, and 2024 in the province of British Columbia; and 2021 and 2023 in the province of Alberta.  Data for each province are used to quantify region-specific sample size requirements, providing important insights into how prescribed sample sizes may need to vary depending on the characteristics of the production basin.  Year-over-year emission trends are also examined in detail, which reveal varying degrees of success in reducing emissions in regions with distinct regulatory frameworks while highlighting key remaining sources to target for mitigation.

How to cite: Johnson, M. R., Wilde, S. E., Tyner, D. R., and Conrad, B. M.: Using Repeated Aerial Methane Measurements to Assess Inventory Protocols and Track Year-over-year Trends in Emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12569, https://doi.org/10.5194/egusphere-egu25-12569, 2025.

EGU25-12688 | ECS | Orals | AS3.41

Comparison of Three Different Landfill Surface Methane Mapping Techniques: Lessons Learned and Policy Implications 

Simon Festa-Bianchet, Isabella Cerquozzi, Cole Van de Ven, and Matthew Johnson

Three different landfill methane surface emissions monitoring (SEM) techniques were compared at active and inactive landfills and in separate controlled release tests.  The deployed SEM techniques included traditional walking surveys with a human operator equipped with a portable methane concentration analyzer with a sampling pump, the drone-based equivalent of this traditional survey where the methane analyzer is instead mounted to a drone and a long sampling tube drags on the landfill surface, as well as a recently introduced laser-based sensor that mounts beneath a drone and measures path-integrated methane concentration between the drone and the ground.  Both drone-based solutions have received commercial interest as they address safety concerns with humans traversing challenging terrain on foot, and can increase the area covered by the survey, especially with the path-integrated sensor which can probe landfill areas with active machinery.  

 

Testing at landfill sites showed that while the drone-mounted, downward-facing laser was the easiest solution to implement in the field, it was also the least effective at identifying hotspots.  Although the walking survey and drone-based equivalent produced generally comparable hotspot mappings, the latter was faster to implement and also gave the cleanest and most repeatable indication of hotspots.  However, critically, results of the controlled release tests revealed poor correlation between methane surface concentration and emission rate for all techniques.  Additionally, parameters such as drone flight speed and the response time of the gas analyzer will affect the absolute magnitude of collected methane concentrations.  This is problematic for the likely success and efficiency of current and proposed regulations that require mitigation action based on specific volume fraction (concentration) thresholds such as 500 ppm.  Based on these results we recommend that site-total emission quantification techniques should be prioritised in both research and regulations, such that problematic landfills can properly be prioritise for action, which can then be supported by SEM data to identify where on the landfill the emissions are occurring.  

How to cite: Festa-Bianchet, S., Cerquozzi, I., Van de Ven, C., and Johnson, M.: Comparison of Three Different Landfill Surface Methane Mapping Techniques: Lessons Learned and Policy Implications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12688, https://doi.org/10.5194/egusphere-egu25-12688, 2025.

EGU25-12842 | ECS | Posters on site | AS3.41

Gas Flaring Efficiencies of Selective Oil and Gas Facilities in the Sultanate of Oman 

Halima Al-Hinaai, Heidi Huntrieser, Eric Förster, Niclas Maier, Falk Pätzold, Lutz Bretschneider, Astrid Lampert, Mark Lunt, Anke Roiger, and Jia Chen

Flaring is the controlled burning of natural gas, a common practice in the oil and natural gas (O&G) industry. Ideally, the combustion process is supposed to convert the potent methane (CH4) completely into carbon dioxide (CO2), yet in real-world situations this is not the case. According to the International Energy Agency (IEA), flaring is responsible for about 10 % of the total methane emission of the O&G sector.  Therefore, it is important to understand and quantify how efficiently the carbon in the flared fuel is converted to CO2, to support the mitigation of flaring emissions. This is especially the case for countries with high reliance on the O&G industry, and a clear commitment to achieve net zero emissions by 2050, such as the Sultanate of Oman.

This study presents the first thorough examination of flaring emissions in Oman using a novel airborne platform. The measurements were performed during the METHANE-To-Go-Oman field experiment funded by UNEP's International Methane Emissions Observatory (IMEO), which was conducted from November to December 2023. It used a unique helicopter-towed probe called HELiPOD. The experiment covered six pre-selected O&G facilities within three concession areas in northern and southern Oman, during ~70 flight hours. 

In this study, VIIRS Nightfire data were used to identify the flaring plume positions and measured in situ data from the HELiPOD were used to capture the plume composition. The airborne in-situ instruments include: Picarro G2401-m to measure CH4 and CO2 with a high precision (1 ppb), Licor-7700 for high CH4 temporal resolution measurements up to 40 Hz, and Licor-7500A for CO2. Also, a variety of data related to combustion products and by-products were collected such as aerosols, water vapor, and temperature, which can be used to verify and understand the chemical and physical characteristics of the flaring plumes. Furthermore, various meteorological data were collected during the experiment, such as the 3D wind vector, which was crucial for the flaring plume identification.

The lowest flaring efficiency observed in this study was related to a gas facility.  Providing valuable insights into the flaring emissions is the aim of this study, which could be translated into mitigation opportunities for policymakers and the industry.






How to cite: Al-Hinaai, H., Huntrieser, H., Förster, E., Maier, N., Pätzold, F., Bretschneider, L., Lampert, A., Lunt, M., Roiger, A., and Chen, J.: Gas Flaring Efficiencies of Selective Oil and Gas Facilities in the Sultanate of Oman, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12842, https://doi.org/10.5194/egusphere-egu25-12842, 2025.

EGU25-13054 | ECS | Orals | AS3.41

Estimating methane emissions from surface coal mines using satellite observations 

Shubham Sharma, Joannes D. Maasakkers, Matthieu Dogniaux, Jason McKeever, Dylan Jervis, Marianne Girard, Berend J. Schuit, Tobias A. de Jong, Itziar Irakulis-Loitxate, Nicholas Balasus, Daniel J. Varon, and Ilse Aben

Monitoring and mitigating methane emissions from super-emitting sources is critical for addressing climate change. The TROPOMI instrument onboard Sentinel-5P provides daily global coverage of methane concentrations at 5.5 × 7 km² resolution, enabling the detection of methane super-emitters (>~8 t hr⁻¹). These data are instrumental in identifying hotspots that can be further investigated using high-resolution (~25 m) satellite instruments to pinpoint facility-level emissions. In support of the UNEP-IMEO Methane Alert and Response System (MARS), we have identified over 250 super-emitter hotspots. These hotspots include oil and gas production sites and urban landfills, while a third are associated with coal mining operations, including unexpected sources like surface coal mines. Given the crucial role of coal in the global energy landscape and steel production, it is essential to monitor and accurately estimate the associated methane emissions.

This work highlights the synergy between TROPOMI and high-resolution instruments through an analysis of surface coal mine clusters in Kazakhstan, Russia, and India. We estimate 2021-2023 annual methane emissions from these three clusters using TROPOMI data in a Bayesian inversion approach. Our results align with emissions calculated using UNFCCC emission factors and mine-level production data, except in India, where significantly lower emissions are observed. Comparisons with bottom-up gridded emission inventories EDGAR v7 & GFEI v2 reveal notable discrepancies, primarily due to inaccuracies in spatial disaggregation. In Kazakhstan, methane emissions increase substantially between 2021 and 2023 despite stable coal production, suggesting that coal seam characteristics and other factors influence emission dynamics. Our emission estimates align closely with GHGSat-based estimates across all mines and years where a sufficient number of GHGSat observations are available. Moreover, spatial correlations are identified between GHGSat-detected methane enhancements and mining activities within the mine. Additionally, atmospheric temperature inversions are found to significantly contribute to the accumulation of methane within the mine pit, complicating emission quantifications based on high-resolution observations. The findings of this study underscore the importance of combining TROPOMI data with high-resolution satellite data to refine methane emission estimates from complex sources like surface coal mines.

How to cite: Sharma, S., Maasakkers, J. D., Dogniaux, M., McKeever, J., Jervis, D., Girard, M., Schuit, B. J., Jong, T. A. D., Irakulis-Loitxate, I., Balasus, N., Varon, D. J., and Aben, I.: Estimating methane emissions from surface coal mines using satellite observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13054, https://doi.org/10.5194/egusphere-egu25-13054, 2025.

EGU25-13193 | ECS | Posters on site | AS3.41

Progress Toward a First Measurement-Based Oil and Gas Sector Methane Inventory for Colombia 

Nikolai Calderon-Cangrejo, Simon A. Festa-Bianchet, Bradley M. Conrad, David R. Tyner, Shona E. Wilde, and Matthew R. Johnson

Methane is a critical focus of international efforts to achieve short-term reductions in greenhouse gas emissions.  Oil and gas and waste sector methane sources are understood to be the easiest and fastest to mitigate, but require robust measurement-based emissions inventory protocols to identify sources, to prioritize mitigation actions, and to track success or failure in reducing emissions.  In particular, the complexity and variability of oil and gas sector sources necessitates combining measurements and data at different scales to accurately define the full distribution of emissions.  This presentation describes the use of a hybrid, top-down / bottom-up inventory protocol to inform Colombia’s national methane inventories.  The top-down campaign conducted between March and May 2024, comprised aerial LiDAR measurements at 3,826 oil and gas sector sites across 6 different production regions as well as measurements at three landfills.  A separate bottom-up campaign is currently scheduled for the first quarter of 2025 and will include OGI surveys at approximately 320 sites, along with targeted measurements of select tanks, compressor engines and flares at a subset of 20 sites.  Preliminary results from the top-down approach for both oil and gas and waste sectors will be discussed during the presentation, along with progress toward completing Colombia’s first-ever measurement-based methane inventory for the oil and gas upstream sector.  This study, funded by UNEP - International Methane Emissions Observatory (IMEO) is intended to support MMRV development and verified reporting under the International Oil and Gas Methane Partnership (OGMP 2.0).

How to cite: Calderon-Cangrejo, N., Festa-Bianchet, S. A., Conrad, B. M., Tyner, D. R., Wilde, S. E., and Johnson, M. R.: Progress Toward a First Measurement-Based Oil and Gas Sector Methane Inventory for Colombia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13193, https://doi.org/10.5194/egusphere-egu25-13193, 2025.

EGU25-13298 | Orals | AS3.41

Characterization of methane emissions from coal mining in Australia 

Stephen Harris, Jakob Borchardt, Jorg Hacker, Nicholas Deutscher, Bryce Kelly, Mark Lunt, Sven Krautwurst, Andrew Mcgrath, Adrian Murphy, Heinrich Bovensmann, Robert Field, Wolfgang Junkermann, Clare Paton-Walsh, Nicholas Jones, and Hasan Nawaz

In 2022, Australia produced over 450 million tonnes of coal, accounting for approximately 7% of global production. About 75% of this output came from coal mines located in the Bowen Basin (Queensland) and the Hunter Coalfields (New South Wales). According to Australia’s 2022 UNFCCC submissions, open-cut and underground coal mining contributes around one-fifth of the nation’s methane emissions, positioning it as a key focus for methane mitigation efforts. These emissions are calculated using a combination of IPCC Tier 2 methodologies, which rely on average basin-specific coal gas contents, and IPCC Tier 3 methodologies, which involve mine-specific coal core gas distribution modelling. Despite employing higher Tier IPCC reporting methods, top-down studies using the TROpospheric MONitoring Instrument (TROPOMI) have suggested that fugitive methane emissions may be underestimated at some Australian coal mining facilities (Sadavarte et al., 2021; Palmer et al., 2021). However, the spatial resolution of TROPOMI (~7 km by 5.5 km) limits its capability for identifying emissions from individual facilities within an observation footprint cell, which constrains its effectiveness for bottom-up emission verification for individual mines.

Here, we present an overview of findings from a series of mine-scale atmospheric surveys conducted across coal mines in the Bowen Basin between 2022 and 2023, and in the Hunter Coalfields in 2024. These studies utilized aircraft-based in-situ and remote sensing instruments, along with ground-based EM27/SUN Solar Absorption Spectrometers, all capable of isolating methane emission rates from individual coal mine facilities. We discuss the broader implications of these results within the context of Australia’s national and international greenhouse gas reporting framework.

References:

Palmer, P. I., Feng, L., Lunt, M. F., Parker, R. J., Bösch, H., Lan, X., Lorente, A., and Borsdorff, T.: The added value of satellite observations of methane for understanding the contemporary methane budget, Phil. Trans. R. Soc. A., 379, 20210106, https://doi.org/10.1098/rsta.2021.0106, 2021.
 
Sadavarte, P., Pandey, S., Maasakkers, J. D., Lorente, A., Borsdorff, T., van der Gon, H. D., Houweling, S., and Aben, I.: Methane emissions from superemitting coal mines in Australia quantified using TROPOMI satellite observations, Environmental Science & Technology, 55, 16573–16580, https://doi.org/10.1021/acs.est.1c03976, 2021.

How to cite: Harris, S., Borchardt, J., Hacker, J., Deutscher, N., Kelly, B., Lunt, M., Krautwurst, S., Mcgrath, A., Murphy, A., Bovensmann, H., Field, R., Junkermann, W., Paton-Walsh, C., Jones, N., and Nawaz, H.: Characterization of methane emissions from coal mining in Australia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13298, https://doi.org/10.5194/egusphere-egu25-13298, 2025.

EGU25-14322 | Orals | AS3.41

Measurement of Methane Emissions from a sewage treatment lagoon in Victoria Australia 

Mei Bai, Pieter De Jong, Peter Wardrop, Clayton Butterly, and Deli Chen

Wastewater treatment facilities are a significant source of greenhouse gas (GHG) emissions released to the atmosphere (Czepiel et al., 1993). Greenhouse gas emission environmental impact has become one aspect of assessing the performance of waste water treatment plants (WWTPs)  (Mohsenpour et al., 2021). A better understanding of current GHG emission rates from these facilities will help to improve national GHG inventories and to develop mitigation strategies. At present there are large uncertainties associated with these emissions, as WWTPs use generalised default emission factors that may have limited applicability to Australian conditions and the specific sewage treatment infrastructure and operations.

Two methane (CH4) emission measurement campaigns were conducted at a sewage treatment plant in Victoria using inverse-dispersion modelling (IDM) coupled with open-path spectroscopic techniques. The first campaign was from February to March 2024 (summer campaign) and the second one was from August to October 2024 (winter campaign). Three open-path lasers (1x Boreal Laser GasFinder 2.0 and 2 x Unisearch Associates Inc.) measured line-averaged gas concentrations at upwind and downwind locations of a sewage treatment lagoon. Real-time CH4 concentrations (ppm over 100 m path-length, one way) were continually measured for over one month during each campaign. Climatic conditions including wind statistics were also recorded with a 3-dimentional sonic anemometer (CSAT3, Campbell Scientific) at a frequency of 10 Hz. These measurements of gas concentration and wind statistics were used as the IDM inputs to calculate CH4 fluxes. During the same periods, effluent samples were also collected and analysed. In this study, we present the CH4 fluxes (μg/m2/s) from the treatment lagoon in summer and winter seasons. The effects of other factors on the emissions including the chemical and physical properties of effluents, aerators operation status, and effluent flow rates were also investigated. We found that measured CH4 emissions were higher than those estimated by national GHG reporting guidelines and seasonal and spatial variations were significant.

How to cite: Bai, M., De Jong, P., Wardrop, P., Butterly, C., and Chen, D.: Measurement of Methane Emissions from a sewage treatment lagoon in Victoria Australia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14322, https://doi.org/10.5194/egusphere-egu25-14322, 2025.

EGU25-14476 | ECS | Orals | AS3.41

High-resolution estimates of national methane emissions for all countries of the world using TROPOMI observations 

James D. East, Daniel J. Jacob, Dylan Jervis, Lucas A. Estrada, Nicholas Balasus, Zichong Chen, Sarah E. Hancock, Melissa P. Sulprizio, Daniel J. Varon, and John R. Worden

Observational constraints on national scale methane emissions are needed to assist progress towards the goals of the Paris Agreements and the Global Methane Pledge. Here, we use 2023 blended TROPOMI+GOSAT observations of atmospheric methane in multiple analytical inversions to estimate emissions for all countries of the world at up to 25 km resolution. Prior emissions estimates are spatially distributed according to state-of-the-science bottom-up inventories, and country-level prior totals are adjusted by sector to match the emissions most recently reported to the UNFCCC. We enhance each inversion’s ability to capture point-source emissions not included in bottom-up inventories by redistributing oil-gas and coal emissions based on a gridded inventory constructed from GHGSat plume and null detections, and by enforcing native resolution emissions optimization at locations where plumes were observed by point source imagers including PRISMA, Sentinel-2, Landsat, EnMAP, GOES, and EMIT, and where large plumes were detected by TROPOMI. Our global total posterior emission of 562 Tg for 2023 is in line with previous coarse-scale global inversion studies. The inversions’ high resolution allows source separation and independent optimization of individual countries, confirmed by small posterior error correlations between countries. China (52.7 Tg), the U.S. (32.2 Tg), India (25.7 Tg), Brazil (18.5 Tg), and Indonesia (10.7 Tg) have the highest anthropogenic emissions, representing 14%, 9%, 7%, 5%, and 3% of the global total anthropogenic source, respectively. Uncertainty estimates come from an inversion ensemble with varied inversion parameters. Results provide an estimate of emissions from all countries in a globally consistent inverse modeling framework, serve as a direct comparison and aid of countries’ UNFCCC reporting, and provide up-to-date observational constraints on emissions from countries where reporting is unfeasible or out of date.

How to cite: East, J. D., Jacob, D. J., Jervis, D., Estrada, L. A., Balasus, N., Chen, Z., Hancock, S. E., Sulprizio, M. P., Varon, D. J., and Worden, J. R.: High-resolution estimates of national methane emissions for all countries of the world using TROPOMI observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14476, https://doi.org/10.5194/egusphere-egu25-14476, 2025.

EGU25-14581 | Posters on site | AS3.41

Methane emission reduction potential in the Chinese oil and gas industry 

Ming Xue, Yuxi Wang, Fan Nie, and Deping Jiang

Methane is the second largest greenhouse gas after carbon dioxide, and the oil and gas industry is a significant anthropogenic methane emission source. In this study, methane emission was estimated in two scenarios from 2000 to 2060. Combined with the emission sources and the cost-effectiveness of current emission reduction technologies, the marginal abatement costs of those technologies in 2030 and 2060 were estimated. The results showed that: methane emissions from petroleum system decreases slightly, while methane emissions from natural gas system will grow slowly in 2020 to 2060. The reduction potential from technology application with negative benefits in 2030 and 2060 was 22.0% and 44.4%, respectively. From 2021 to 2023, the Chinese oil and gas industry have applied remote sensing, vehicle-based or drone-based site level measurements, and leak detection and repair during the national carbon monitoring trial project. The applicability of various measurement methods were tested in diverse oil and gas basins, a measurement-based methodology for the generation of emission factors were raised. In the mid- and long-term, the oil and gas industry of China needs to accelerate the construction of a robust measurement, reporting and verification system (MRV) , moving towards a measurement-based inventory, while providing guidance on methane abatement for local oil and gas operators. The next generation of leak detection and repair technology, and the co-treatment of methane/volatile organic carbon are the future directions for technology development. The incorporation of green economy, China certified emission reduction (CCER) would further foster the application of methane emission measurement and reduction in the industry.

How to cite: Xue, M., Wang, Y., Nie, F., and Jiang, D.: Methane emission reduction potential in the Chinese oil and gas industry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14581, https://doi.org/10.5194/egusphere-egu25-14581, 2025.

EGU25-14858 | ECS | Posters on site | AS3.41

Advancing methane emission quantification: a robust methodology for site-level measurements 

Gerrit Jan de Bruin, Ilona Velzeboer, Daniëlle van Dinter, Pim van den Bulk, Harmen van Mansom, Baye Thera, and Arjan Hensen

The Oil and Gas Methane Partnership 2.0 (OGMP 2.0), led by the United Nations Environment Programme (UNEP) and supported by the European Commission, is currently the only measurement-based international reporting framework for the oil and gas sector. OGMP 2.0 aims to standardize and enhance the accuracy of methane emission reporting, enabling the industry to systematically quantify and reduce emissions.

This study introduces a robust methodology to meet OGMP Level 5 requirements, which call for site-level methane measurements integrated with specific Emission Factors (EF) and Activity Factors (AF) for individual sources. Previously, emissions reporting relied solely on inventory data, but independent site-level measurements now reconcile source-level inventories (Level 4) and thus enhance confidence in reported emissions.

The Dutch oil and gas sector serves as a case study. In 2023, the Dutch Emission Registration reported 639 kton of methane emissions nationally, which 17 kton (2.7%) attributed to the oil & gas sector. As part of this study, we measured emissions at over hundred oil and gas production and distribution sites.

We demonstrate the application of the Tracer Dispersion Method (TDM) to quantify methane emissions at the site level. This approach involves releasing a tracer gas with a known emission rate and measuring its concentration, along with methane, downwind of the facility with a specially equipped measurement truck. We determine the concentration of various gaseous components, allowing us to differentiate the emissions to the various types of sources that may be present. We drive by at multiple occasions along a predetermined route downwind of the site, enabling us to capture data under various meteorological and operational conditions. This ensures robust data collection and facilitates the automatic determination of the site-level emission factor, significantly reducing associated uncertainties.

This methodology not only complements source-level measurements but also improves the detection of previously unidentified emission sources, enhancing the overall reliability of emission inventories. We will discuss the requirements, advantages, and limitations of the TDM approach and outline next steps for further refinement.

By providing a scalable and accurate methodology for site-level methane quantification, this work contributes to the global effort to achieve transparent and actionable emission reduction strategies in the oil and gas sector.

How to cite: de Bruin, G. J., Velzeboer, I., van Dinter, D., van den Bulk, P., van Mansom, H., Thera, B., and Hensen, A.: Advancing methane emission quantification: a robust methodology for site-level measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14858, https://doi.org/10.5194/egusphere-egu25-14858, 2025.

EGU25-15400 | Orals | AS3.41

Methane emission to the atmosphere from the first gas-producing well in Transylvania 

Calin Baciu, Eduard Ghiorghiu, Iulia Ajtai, Ildiko Martonos, Mustafa Hmoudah, Alexandra Orban, Alexandru Lupulescu, Liana Spulber, Alexandra Cozma, Stefan Sfabu, Roxana Moga, and Giuseppe Etiope

Historically, the Transylvanian basin is one of the most important natural gas-producing areas in Europe. The existence of commercial gas reserves was incidentally discovered in the early 1900's while drilling for potassium salts in the Miocene deposits that fill the basin. Well #2 Sarmasel, that was positioned close to an area with natural gas emissions, has intercepted very shallow strata containing gas. Drilling had to be stopped on 22 April 1909, after 5 months of work, at a depth of 300 m, due to overwhelming technical difficulties related to the high pressure of gas. Thus, this date marks the beginning of the gas extraction in Transylvania. The well has been left open until 23 June 1910, when a first attempt at closure was made. Twenty hours after closure, gas was observed escaping in a neighbouring field, which required the reopening of the well. A second closure attempt occurred on 31 July 1911, subsequent to the external encasement of the well for the initial 120 meters of depth. No gas leak was detected, and the closure seemed to be effective at this stage. On 29 October 1911, a powerful gas eruption occurred in the fields east of the well, accompanied by considerable gas emissions in the surrounding area, local seismic activity, saline water leakage, and the appearance of several craters located between 100 and 400 meters from the well. The well was reopened once again, until the end of 1913, when it was connected to the pipeline conveying gas to consumers. More than 1.3×109 m3 of gas has been released to the atmosphere during a span of four years. An additional 556×106 m3 of gas was supplied to consumers from 1913 to 1935, when the well was capped. The total volume is around 2 billion cubic meters of gas from a single, 300-meter-deep well! The main crater generated by the 1911 outburst, despite being filled with soil post-explosion, persists in emitting gas that sustains a perpetual fire. 

Our research demonstrated that Sarmasel is a case of ongoing, prolonged gas leakage caused by manmade activities (drilling and gas extraction) conducted over a century ago, functioning in conjunction with, and likely intensified by, a natural seepage process. Sarmasel can thus be regarded as a hybrid leakage-seepage system. This study exemplifies the risk of generating fugitive emissions when drilling occurs within a natural seepage system.
Acknowledgments: This work was supported by the Project DTIE21-EN3485 funded by UNEP and by the Project 14/11.11.2023—ENGAGE, PNRR-III-C9-2022—I8, supported by the EU through the Romanian Govt.

How to cite: Baciu, C., Ghiorghiu, E., Ajtai, I., Martonos, I., Hmoudah, M., Orban, A., Lupulescu, A., Spulber, L., Cozma, A., Sfabu, S., Moga, R., and Etiope, G.: Methane emission to the atmosphere from the first gas-producing well in Transylvania, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15400, https://doi.org/10.5194/egusphere-egu25-15400, 2025.

EGU25-16113 | Orals | AS3.41

Evaluation of inverse models to estimate methane emissions from European countries 

Alexandre Danjou, Peter Andrews, Daniela Brito Melo, Alice Ramsden, Hélène De Longueville, Alison Redington, Brendan Murphy, Joseph Pitt, Matthew Rigby, Alistair Manning, Stephan Henne, and Anita Ganesan

Methane is a powerful greenhouse gas that is a major contributor to climate change. Quantifying emissions by process is therefore important, especially as many countries (including most European countries) have pledged to drastically reduce their emissions through the Global Methane Pledge and regional regulations. These countries report their emissions annually to the UNFCCC through National Inventory Documents (NIDs).

While reported emissions are estimated using established methods based on bottom-up activity data, the UK and Switzerland additionally include in their NIRs an assessment using atmospheric observations. This independent assessment is derived using atmospheric inverse modelling or “top-down” methods. The Horizon Europe project Process Attribution of Regional emISsions (PARIS) extends “top-down” comparisons with inventories to several additional European countries.

In this work, we carry out a sensitivity analysis of methane inversions over Europe from 2018 to 2023. This enables us to first assess the influence of different inversion parameters, such as the number of sites, the transport model, estimation of boundary conditions, and the role of data filtering and model uncertainty. We thus evaluate our confidence in European methane inversions and identify the main parameters that lead to discrepancies between inversions.  Two transport models: NAME and FLEXPART; and three inversion models: ELRIS from Empa, InTEM from MetOffice and RHIME from the University of Bristol are used.

We then focus on a 35 year assessment of methane emissions over the UK over the period (1989-2023) using RHIME and InTEM, thus re-evaluating the emissions reported by the UK over the last few decades using two different inversion models. The RHIME and InTEM estimates are broadly in agreement, however, both estimate significantly lower emissions than those reported in the latest UK NIR for the 1990s and early 2000s. Although fewer sites were available on the 1989-2000 period than in the years covered in the PARIS project, the use of two inversion methods provides additional confidence that a large disagreement between atmospheric measurements and the UK inventory exists until the early 2000s.

How to cite: Danjou, A., Andrews, P., Brito Melo, D., Ramsden, A., De Longueville, H., Redington, A., Murphy, B., Pitt, J., Rigby, M., Manning, A., Henne, S., and Ganesan, A.: Evaluation of inverse models to estimate methane emissions from European countries, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16113, https://doi.org/10.5194/egusphere-egu25-16113, 2025.

EGU25-16153 | ECS | Posters on site | AS3.41

Methane emissions estimated from airborne measurements from open-pit and underground coal mines in the Bowen Basin, Australia 

Jakob Borchardt, Stephen J. Harris, Jorg M. Hacker, Mark Lunt, Sven Krautwurst, Hartmut Bösch, Heinrich Bovensmann, John P. Burrows, Shakti Chakravarty, Robert A. Field, Konstantin Gerilowski, Oke Huhs, Wolfgang Junkermann, Bryce F. J. Kelly, Martin Kumm, Andrew McGrath, and Josua Schindewolf and the Campaign Support Team

Methane (CH4) is the second most important greenhouse gas (GHG) whose atmospheric abundance is modified by anthropogenic activity. The reduction of CH4 emissions has been identified as an essential mitigation target for slowing man-made climate change. According to inventories, coal mining accounts for roughly 33% of fossil fuel and 11% of all anthropogenic CH4 emissions. Accurate identification of coal mining-related CH4 sources and quantification of their annual emission rate is needed for corporate reporting requirements, national inventory verification, and the development of CH4 mitigation strategies. In Australia, coal mining accounts for approximately 20% of reported CH4 emissions.

In the Bowen Basin in Queensland, Australia, over 40 active mines are distributed over 60,000 km2, with both open-pit and underground coal mines. A study using TROPOMI satellite measurements to estimate CH4 emissions from 3 clusters of coal mines in this region showed discrepancies with reported emissions during 2018 and 2019.

In September-October 2023, the Bowen Basin CH4 Mapping (BBCMap) Campaign was carried out. It was funded by and performed in collaboration with UNEP’s International Methane Emissions Observatory as part of its Methane Science Studies. Two identical HK36 TTC Eco-Dimona research aircraft specifically designed as sensor platforms were deployed to conduct the measurements. One of these aircraft carried the MAMAP2D-Light (Methane Airborne MAPper 2D – Light) imaging spectrometer to estimate atmospheric CH4 and CO2 column anomalies, as well as a LIDAR to provide up-to-date topography scans. The second aircraft was fitted with an LGR UGGA gas analyzer and a suite of meteorological instrumentation to measure atmospheric CH4, CO2, and water vapor concentrations, as well as accurate winds and other basic meteorological parameters. It also carried a bag sampler to capture air samples for later isotopic analysis.

The campaign investigated emissions from approximately 33 mines in the Bowen Basin. In this contribution, we discuss CH4 emission estimates for both open-pit and underground coal mines using both in-situ and remote sensing measurements.

How to cite: Borchardt, J., Harris, S. J., Hacker, J. M., Lunt, M., Krautwurst, S., Bösch, H., Bovensmann, H., Burrows, J. P., Chakravarty, S., Field, R. A., Gerilowski, K., Huhs, O., Junkermann, W., Kelly, B. F. J., Kumm, M., McGrath, A., and Schindewolf, J. and the Campaign Support Team: Methane emissions estimated from airborne measurements from open-pit and underground coal mines in the Bowen Basin, Australia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16153, https://doi.org/10.5194/egusphere-egu25-16153, 2025.

EGU25-16833 | Posters on site | AS3.41

Improved estimations of waste-related methane emissions using satellite observations: a case study on a US landfill 

Malika Menoud, Tarek Abichou, Itziar Irakulis Loitxate, James L. France, and Andreea Calcan

Reducing methane (CH4) emissions offers the opportunity to slow down global temperature rise in the near term. More than 10 % of anthropogenic CH4 is emitted by the degradation of solid waste, when accumulated in open dumps or managed landfills. Methane production at solid waste sites depends upon various parameters, influenced by waste composition and amounts, landfill operation, as well as climate and meteorological variables. Therefore, landfill emissions are spatially and temporally heterogeneous, which challenges global mitigation efforts. 

Atmospheric measurements from ground and aerial vehicles can be used to quantify and monitor emissions on a facility level. Large facilities located nearby densely populated areas are emission hotspots that can be detected with satellite instruments. We present a case study of the use of CH4 satellite data to derive emission estimates of the Miramar landfill in California, United States. We used observations from UNEP’s International Methane Emissions Observatory (IMEO), through its Methane Alert and Response System (MARS) to detect and quantify four CH4 plumes measured with EMIT satellite between August 2023 and August 2024. We characterized the landfill in terms of amounts and composition of waste, population served and development index, landfill management and gas capture infrastructure, as well as temperature and precipitations.  

Estimated fluxes were 1.69 ± 0.85, 2.74 ± 1.38, 4.79 ± 2.41 t/h and 38.7 ± 19.4 t CH4/h. The exceptionally high maximum likely occurred while the gas collection system was down. The landfill operator declares a total amount of 20,790 t CH4 collected over the year 2023 and reports total emissions equivalent to 1.56 and 0.526 t CH4/h, based on the two US-EPA standards methods. The reported emissions and our observed estimate reveal substantial methane losses, despite apparent gas recovery efforts. 

These inconsistencies, combined with the variability in satellite-derived fluxes, underscore the difficulty of aligning measurement methodologies. They highlight the need to integrate satellite observations, landfill operations data, and inventory models to refine methane emission estimates to support more effective mitigation strategies. 

Our case further shows that atmospheric measurements and the analysis of landfill characteristics can be used in a global classification of facilities and to derive appropriate emission factors. We therefore identified opportunities brought by this measurement-based approach, going from small scale to larger scale: (1) to target efficient methane mitigation action at large-emitting facilities, (2) to quantify the efficiency of waste management policies, (3) to improve country-reported contributions.

This research has been funded in the framework of UNEP’s IMEO. 

How to cite: Menoud, M., Abichou, T., Irakulis Loitxate, I., France, J. L., and Calcan, A.: Improved estimations of waste-related methane emissions using satellite observations: a case study on a US landfill, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16833, https://doi.org/10.5194/egusphere-egu25-16833, 2025.

EGU25-17051 | Posters on site | AS3.41

IMEO’s Baseline Science Studies improves country-level methane quantification 

Xuefei Li, Marci Baranski, James Lawrence France, Nataly Velandia Salinas, Andreea Calcan, Paul Balcome, Rodrigo Jimenez, Guus Velders, Daniel J. Jacob, and Manfredi Caltagirone

UNEP’s International Methane Emissions Observatory (IMEO) is a data-driven, action-focused initiative. IMEO exists to provide open, reliable, integrated methane emissions data to facilitate actions to reduce methane emissions. The Baseline Science Studies are a subset of IMEO’s science studies, which aim to estimate the current total and sectoral methane emissions (with uncertainties) at country-level through multi-scale measurement studies and integration with existing data. It will assist governments, civil society, industry, and other stakeholders to prioritize actions to reduce methane emissions.

IMEO’s Baseline Studies couple multi-scale top-down approaches with more granular analysis of bottom-up data to improve the understanding of key methane emission sources relevant to selected countries. The focused sectors for methane emission are oil and gas, agriculture and waste. Currently, there are two Baseline Studies at the design phase for Colombia and Nigeria. We will conduct an initial assessment per country through literature and reports, feed the existing prior to satellite inversion model and apportion the emission by sector. Using the literature review and satellite information, we identify the major methane sources and those with large uncertainties in each country, and design small studies to provide measurement data where little to no data in-country is available. By combining activity data and geospatial mapping, the ultimate aim is creating a gridded methane inventory at the country level. This information will be used to update the country level methane budget and build local capacity to enable future estimations and refinement of sectoral emissions. The presentation here will demonstrate the concept and generalised progress of the IMEO baseline studies

How to cite: Li, X., Baranski, M., France, J. L., Velandia Salinas, N., Calcan, A., Balcome, P., Jimenez, R., Velders, G., Jacob, D. J., and Caltagirone, M.: IMEO’s Baseline Science Studies improves country-level methane quantification, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17051, https://doi.org/10.5194/egusphere-egu25-17051, 2025.

EGU25-17584 | ECS | Posters on site | AS3.41

Estimation of methane emissions from gas excavation activities in the Transylvanian Basin, Romania. 

Paweł Jagoda, Jarosław Nęcki, Jakub Bartyzel, Aleksandra Figura-Jagoda, Andrei Radovici, Alexandru Mereuta, Calin Baciu, and Thomas Roeckmann

The vast gas reservoirs in the Transylvanian Basin have been exploited for over a century, primarily managed by the state-owned company ROMGAZ. With over 100 gas fields scattered throughout the region, it remains the foremost gas producer among Central and South-Eastern European countries.  The International Energy Agency estimates that 45% of emissions reductions from the energy sector can be achieved at no net monetary cost and could even result in economic savings, considering methane's commercial value as the main component of natural gas.

 

Five teams with participants from Poland and Romania were deploying various techniques (GPM, OTM-33A, High Flow Sampler, Tracer release, large-scale flux chamber and screenings) for quantifications of the methane emission rates. Additional instruments from other participants of the ROMEO project were shipped to Romania and used for mobile measurements. A total of 520 individual sites from the O&G operator inventory were at least screened for a source of emissions attribution. 160 quantifications with 5 techniques were performed. The study focuses on combining all measurement methods as complementary tools for emission quantifications. We attempt to upscale the emission for the Transylvanian basin based on 18% of the operator’s active inventory in the region.

 

The findings presented were made possible through equipment funded by the "Excellence Initiative - Research University" program at AGH University of Science and Technology. The authors express their gratitude to all participants and supporters of the ROMEO campaign. Work on this study is supported by UNEP’s IMEO. Future research focused on quantifying emissions from oil and gas is planned as part of the IM4CA “Investigating Methane for Climate Action” project.

How to cite: Jagoda, P., Nęcki, J., Bartyzel, J., Figura-Jagoda, A., Radovici, A., Mereuta, A., Baciu, C., and Roeckmann, T.: Estimation of methane emissions from gas excavation activities in the Transylvanian Basin, Romania., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17584, https://doi.org/10.5194/egusphere-egu25-17584, 2025.

EGU25-18230 | Posters on site | AS3.41

Source and Site Level Reconciliation of Methane Emissions at the Midstream Sector 

Violeta Bescos Roy, Hossein Maazallahi, Robert Ziegler, and Mures Zarea

Efficient methane reduction efforts require reliable, measurement-based and transparent inventories. Site-level technologies serve as essential tools for gathering data on emissions at operational sites. However, significant knowledge gaps persist regarding the performance of these technologies in real-world conditions and their effective utilization to enhance the accuracy of reported data by operators. This study evaluates the snapshot reconciliation - an instantaneous comparison- of site and source level quantification methods to provide midstream operators with general recommendations when the relevant quantification methods and reconciliation practices are applied at their sites.

Prior to this campaign, which took place at a compressor station in Zelzate, data from a previous phase of the project conducted in Spain -where controlled releases were carried out in real-world conditions- were analysed to understand the uncertainties associated with site-level technologies. This analysis was used for the selection of technologies with the best performance, i.e. closeness of the technology providers’ emission quantifications to the controlled and blind release rates. In Zelzate, a two-day campaign was designed, consisting of two distinct phases based on the operational status of one of the site’s compressors. During the campaign, site-level quantification methods were deployed in parallel with source-level quantification techniques.

The reconciliation process was assessed to understand how it can be implemented for verifying bottom-up data. Following the results of this test, detailed recommendations for implementing snapshot reconciliation were provided in alignment with OGMP 2.0 (Oil and Gas Methane Partnership 2.0) guideline. These recommendations prioritize identifying and addressing areas of improvement in emission quantification (e.g. bottom-up sampling and measurement strategy) to achieve consolidated Level 5 inventories. Furthermore, reconciliation process should not primarily focus on the potential overlap between site-level and source-level measurements, owing to limited understanding of the uncertainty ranges required for such analyses.

The outcomes of this study offer deep and valuable insights into several key aspects:

  • Performance of Site-Level Methods: Understanding the capabilities and limitations of site-level quantification technologies in real-world field conditions.
  • Reconciliation Recommendations: Providing practical guidance for implementing effective reconciliation procedures, with a focus on achieving robust and transparent methane inventories.

 

How to cite: Bescos Roy, V., Maazallahi, H., Ziegler, R., and Zarea, M.: Source and Site Level Reconciliation of Methane Emissions at the Midstream Sector, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18230, https://doi.org/10.5194/egusphere-egu25-18230, 2025.

EGU25-18683 | Orals | AS3.41

Contrasting Methane Emissions from Solid Waste Landfills: Side by Side Assessment of Ground, Drone, and Satellite Based Technologies 

Tarek Abichou, Itziar Irakulis-Loitxate, Malika Menoud, James France, and Andreea Calcan

Tracer Correlation Method (TCM) testing was conducted at a U.S. landfill to quantify fugitive methane emissions, with flux values ranging from 1,353 to 4,996 kg/hr. SEM2Flux, another ground-based method, reported lower fluxes ranging from 430 to 1,177 kg/hr with standard deviations of 24 to 164 kg/hr in the same landfill. The lower flux estimates from SEM2Flux may be due to the limited number of data points, inadequate coverage of the waste footprint, or emissions originating from gas collection infrastructure above ground rather than directly from the landfill surface.

Satellite platforms, including EnMAP, EMIT, and PRISMA, provided broader flux ranges, with values spanning from 2,430 to 9,840 kg/hr. EMIT reported the highest fluxes but also the largest uncertainties, averaging 4,931 kg/hr. EnMAP and PRISMA reported more moderate fluxes with uncertainties of 892 kg/hr and 1,824 kg/hr, respectively. The higher estimates from satellite detections may be related to their detection limit, as it is only possible to detect methane plumes when emissions are large enough, although there may be other factors that have yet to be explored. Satellite data offers broader spatial coverage, high data frequency if the data is requested, and independent measurements based on open data. However, the variability and higher uncertainties underscore the need for validation against reliable ground-based measurements like TCM.

Reported emissions for the site, calculated using the USEPA-recommended methods, equate to hourly fluxes of approximately 754 kg/hr and 740 kg/hr. These values significantly underestimate emissions when compared to TCM, SEM2Flux, and satellite data. The discrepancies between the different technologies/techniques emphasize the need for more comprehensive validation experiments integrating ground-based and satellite measurements to improve emissions inventories and enhance monitoring systems across varying site conditions and methodologies.

 

This research has been partially funded in the framework of UNEP’s International Methane Emissions Observatory (IMEO).

How to cite: Abichou, T., Irakulis-Loitxate, I., Menoud, M., France, J., and Calcan, A.: Contrasting Methane Emissions from Solid Waste Landfills: Side by Side Assessment of Ground, Drone, and Satellite Based Technologies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18683, https://doi.org/10.5194/egusphere-egu25-18683, 2025.

EGU25-18856 | Orals | AS3.41

Reconciling Regional Mass Balance and Point Source Measurements for Understanding Methane Emissions in the Appalachian Basin 

Shannon Stokes, Shuting Yang, David Allen, and Arvind Ravikumar

Anthropogenic sources of methane, especially those from the oil and gas industry, are significant. Increasingly, global measurement campaigns have been conducted to capture regional emissions intensity using satellite and mass balance technologies. However, these technologies often lack the fine-scale resolution needed for detailed source attribution, making them difficult to use for mitigation prioritization. Meanwhile, individual operators are employing aerial technologies to measure their assets and assist in leak detection and repair initiatives, but this fine-scale data is not used to inform the regional estimates. This study focuses on reconciling aircraft-based regional mass balance data with aircraft-based point source measurements in identical regions of the Appalachian Basin of the United States in 2024. Aerial LIDAR measurements were used to measure approximately 6000 sites, including all major oil and gas and non-oil and gas sources. Regional mass balance flights were conducted on subdivided polygons encompassing the sites surveyed by the aerial LIDAR measurements. Some emission sources have been deliberately excluded due to cost, such as pipelines, distribution systems and non-producing wells. Comparing the sum of the point sources measured and the mass balance approaches will allow us to examine the relevance of the sources that were not measured. Additionally, while the mass balance measurements and point source measurements occur in the same quarter, the flights are not contemporaneous. It is well documented that emissions from oil and gas sources vary in their size and duration, with large emission events that may be short in duration. This can lead to considerable disagreement between the point source measurements and the regional mass balance estimates. This work will address the short duration, large emission events and their effect on the uncertainty in the regional methane emission estimates.

How to cite: Stokes, S., Yang, S., Allen, D., and Ravikumar, A.: Reconciling Regional Mass Balance and Point Source Measurements for Understanding Methane Emissions in the Appalachian Basin, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18856, https://doi.org/10.5194/egusphere-egu25-18856, 2025.

EGU25-19062 | ECS | Posters on site | AS3.41

Synthesis of the ROMEO Project Findings: Assessing Romania’s O&G Methane Emissions and Advancing Accurate Methane Emission Inventories 

Foteini Stavropoulou, Hugo Denier van der Gon, Calin Baciu, Magdalena Ardelean, Andreea Calcan, Stefan Schwietzke, Daniel Zavala-Araiza, and Thomas Röckmann

Romania is one of Europe’s oldest oil and gas (O&G) producers with a history dating back to 1857 and remains one of the major producers within the EU. The country’s O&G sector continues to play a significant role in the regional energy supply, and recent discoveries of large natural gas reserves in the Black Sea highlight Romania’s interest in even further development. However, the recent EU regulation on methane (CH4) emissions requires member states to mitigate and to improve accuracy of measurement, reporting, and verification of emissions. Uncertainty in current CH₄ emission estimates and the lack of empirical data until now presents significant challenges in meeting climate objectives.

The ROMEO (ROmanian Methane Emissions from Oil and Gas) project aimed to provide independent, scientific estimates of CH₄ emissions from Romania’s onshore O&G sector. Using a range of measurement techniques including ground-based, drone-based, and airborne-based platforms, the project focused on the upstream O&G sector during three intensive campaigns in 2019 and 2021. Phase I targeted the oil production region of southern Romania, Phase II focused on gas production sites in Transylvania, and Phase III involved a follow-up survey in southern Romania. Results from the studies reveal a significant underestimation of CH4 emissions in the national inventory from Romania’s O&G industry in 2019 and 2021, highlighting the substantial mitigation potential within the country’s O&G production infrastructure.

This synthesis consolidates findings from the ROMEO project’s multi-scale measurement campaigns and offers a comprehensive assessment of CH₄ emissions across facility types and regions in Romania. The implications of these findings are also discussed for both mitigation strategies and inventory reporting. One of the challenges is that activity data used for the measurements (e.g. oil production sites and other infrastructure locations) are not the same as the ones used in the reporting in countries using the Tier 1 approach (e.g. oil or gas production rates). This simple difference fundamentally complicates the direct incorporation of research findings into the reporting.  We explore how field measurements can more effectively inform and improve inventory methodologies and support the development of more accurate emissions inventories.

How to cite: Stavropoulou, F., van der Gon, H. D., Baciu, C., Ardelean, M., Calcan, A., Schwietzke, S., Zavala-Araiza, D., and Röckmann, T.: Synthesis of the ROMEO Project Findings: Assessing Romania’s O&G Methane Emissions and Advancing Accurate Methane Emission Inventories, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19062, https://doi.org/10.5194/egusphere-egu25-19062, 2025.

EGU25-19083 | ECS | Orals | AS3.41 | Highlight

UNEP's IMEO Methane Alert and Response System to drive the mitigation of anthropogenic methane emissions 

Itziar Irakulis-Loitxate, Manuel Montesino-SanMartin, Gonzalo Mateo-García, Meghan Demeter, Giulia Bonazzi, Anna Vaughan, Vit Ruzicka, Tobias A. de Jong, Shubham Sharma, Joannes D. Maasakkers, Ilse Aben, Adriana Valverde, Robert A. Field, Małgorzata Kasprzak, Malika Menoud, Tarek Abichou, Kushal Tibrewal, Luis Guanter, and Andreea Calcan

UNEP's International Methane Emissions Observatory (IMEO) launched the Methane Alert and Response System (MARS) in 2023 to provide open, reliable, and actionable data to those individuals with the agency to act on them and ultimately reduce methane emissions. MARS uses satellite observations to detect and monitor large methane emissions and then notifies governments and companies worldwide. With the development of MARS, IMEO opened a new level of transparency that reveals dozens of large methane emissions around the world every week. Thanks to the synergistic use of more than a dozen different open-access satellite missions, combined with the development of Machine Learning models that support and optimize the work of the MARS analysis group, IMEO provides the largest open-access database of point source methane emissions detected with different satellites. At the same time, since its launch in January 2023, MARS has directly notified stakeholders of more than 1900 methane plumes linked to the oil and gas (O&G) sector in about 30 countries.  As a result of these notifications, IMEO has confirmed a number of mitigated emission sources following stakeholder action. Throughout the MARS process, we also learn new information and lessons about the accuracy of our measurements, the root causes behind the observed emissions, and the real feasibility of mitigating emission sources under different scenarios and geographic areas, among others.

While MARS notifications are currently on sent for recent O&G point source emissions, it also has the capability to detect and monitor emissions from other sectors, such as coal and waste. Additionally, we have the ability to explore satellite archive data to conduct more in-depth analyses of the historical behaviour of the emitters. As a result, IMEO is currently expanding MARS’ capacity to further support IMEO's scientific studies and its efforts towards increasing transparency in the metallurgical coal and waste sectors to drive emissions reduction.

In this contribution, we will show case studies we have recently dealt with, lessons learned, improvements, and new data and methodologies integrated into MARS based on scientific research. We will also give an overview of IMEO’s efforts in the metallurgical coal sector and in the waste sector through scientific studies and with the support of remote sensing data generated through MARS. 

How to cite: Irakulis-Loitxate, I., Montesino-SanMartin, M., Mateo-García, G., Demeter, M., Bonazzi, G., Vaughan, A., Ruzicka, V., de Jong, T. A., Sharma, S., Maasakkers, J. D., Aben, I., Valverde, A., Field, R. A., Kasprzak, M., Menoud, M., Abichou, T., Tibrewal, K., Guanter, L., and Calcan, A.: UNEP's IMEO Methane Alert and Response System to drive the mitigation of anthropogenic methane emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19083, https://doi.org/10.5194/egusphere-egu25-19083, 2025.

EGU25-19193 | ECS | Posters on site | AS3.41

Validation of a methodology for methane flux quantification from an aircraft using a controlled release experiment 

Patryk Łakomiec, Stéphane Bauguitte, Irene Monreal Campos, Matthew Baker, Dave Sproson, Audrey McManemin, Adam Brandt, Catherine Juéry, Vincent Blandin, and Jordi Jourde

The oil and gas industry is responsible for 22% of global methane emissions (Saunois et al. 2020), yet accurately quantifying them remains a significant challenge. Oil and gas facilities often underreport methane emissions due to reliance on bottom-up estimation methods based on theoretical calculations and their susceptibility to systematic errors. Accurate top-down quantification tools for methane emission fluxes from this sector are crucial.

We evaluate a novel methodology to quantify methane emission fluxes using the commercially available dispersion model ADMS6 and airborne measurements. The model takes into consideration many parameters such as meteorology, source characteristics, and the dispersion domain topography. This complexity doesn’t implicate high demands on the computing time and the simulation time is short, up to a few minutes.

In September 2024, FAAM flew one mission during a single-blind controlled release experiment organised by Stanford University and TotalEnergies.  The International Methane Emissions Observatory sponsored this experiment conducted at the TotalEnergies Anomalies Detection Initiatives (TADI) site in Lacq, southwest France. FAAM targeted three separate releases with controlled methane rates up to 60 g/s. Over 40 orbits were flown at distances at  3.5 and 9 km around the TADI site over 3 hours, at altitudes between 180 and 500 m above ground. 

We present fast CO, CO2, CH4, SO2, NOx and 0.1–3 µm aerosol number concentrations and interpret the sampled emission sources.  We discuss the meteorological conditions encountered during the mission and their impact on the release atmospheric dispersion modelling.  We evaluate the accuracy of our quantification methodology against the known release rates and identify shortcomings and how they can be circumvented. Despite the challenging sampling conditions, we successfully detected emissions and confirmed the extent of our method validity.

How to cite: Łakomiec, P., Bauguitte, S., Monreal Campos, I., Baker, M., Sproson, D., McManemin, A., Brandt, A., Juéry, C., Blandin, V., and Jourde, J.: Validation of a methodology for methane flux quantification from an aircraft using a controlled release experiment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19193, https://doi.org/10.5194/egusphere-egu25-19193, 2025.

EGU25-20141 | Orals | AS3.41

Bridging inventory reporting and atmospheric inversion estimates of anthropogenic greenhouse gas emissions in Europe: The PARIS project 

Thomas Röckmann, Anita Ganesan, Alistair Manning, and Stephan Henne and the The PARIS Team

National greenhouse gas emission reporting in Europe is facilitated by national agencies based on activity data and emission factors, and in some cases, more sophisticated process modeling approaches, for many different activities and emission sectors. These “bottom-up” emission estimates are essential for providing guidance for emission mitigation measures relevant for international treaties and negotiation, for monitoring national progress towards targets, and for separating emissions processes and sector level breakdowns of sources and sinks.

Emissions of gases to the atmosphere result in atmospheric concentrations that are locally enhanced compared to background levels. These enhancements can be measured with precise instrumentation and used to quantify the emissions. When these measurements are evaluated with inverse atmospheric transport models, they can deliver independent “top-down” emission estimates, i.e., emission estimates that are consistent with the measured concentration enhancements. Due to the complexity of atmospheric transport, such estimates are difficult, but they have now reached a level where they can provide independent information on emissions and can support the bottom-up approach.

Switzerland and the UK are two countries that already provide top-down emission estimates as annexes to their annual national emission reports to the UNFCCC. Within the PARIS project we have extended the top-down approach for national scale emission estimates to 6 further countries (Germany, the Netherlands, Italy, Norway, Hungary, Ireland), and produced consistent drafts for annexes to the National Inventory reports for all 8 countries.    

A weakness of top-down approaches is that they can not always distinguish between emissions from different source sectors, which makes comparison to the National Inventories difficult. As a second focus of PARIS, we aim at developing measurable signatures to facilitate a more detailed attribution of the derived emissions to specific source sectors. These signatures include measurements of isotopic composition for CH4 and N2O, atmospheric O2 for CO2, other co-emitted species, as well as detailed composition measurements for organic and black carbon aerosols.

This presentation will include some interesting aspects from the draft annexes to the National Inventory Reports, innovative new measurements for source sector attribution and new tools for evaluation and comparison of emission estimates.

How to cite: Röckmann, T., Ganesan, A., Manning, A., and Henne, S. and the The PARIS Team: Bridging inventory reporting and atmospheric inversion estimates of anthropogenic greenhouse gas emissions in Europe: The PARIS project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20141, https://doi.org/10.5194/egusphere-egu25-20141, 2025.

EGU25-20392 | Posters on site | AS3.41

Detection and quantification of anthropogenic methane emissions in Germany using mobile measurements 

Martina Schmidt, Julia Wietzel, Till Gonser, Ilka Sauer, and Maren Zeleny

The detection and quantification of anthropogenic CH4 emissions is still a challenge due to the complex and heterogeneous distribution of the emitters and the large variability, e.g. leakages in the natural gas network, biogas plants, agriculture, waste and wastewater treatment.  Mobile measurements at street level, using cars or bicycles, are a good way to detect methane emission sources. The measured CH4 peaks can be converted to emission rates using a Gaussian plume model.

The emission factors for the waste and wastewater sector as well as for biogas plants are still subject to large uncertainties. In this study, mobile measurements for several CH4 source categories in Germany are presented. The main focus is on CH4 emission rates from the waste and wastewater sector and from biogas plants. We performed mobile methane measurements to detect emission plumes from more than 30 different biogas plants in Germany, focusing on one biogas plant for long-term monitoring since 2016.  Methane emission rates ranged from 0.1 to 46 kgCH4/h. This corresponds to a loss relative to the biogas production rates of 2 to 13 % l. Measurements at several wastewater treatment plants show CH4 emission factors between 0.04 and 1.9 kg CH4/a per capita.

The determined emission rates are statistically analysed and compared with the emission factor used in regional and national inventories.

How to cite: Schmidt, M., Wietzel, J., Gonser, T., Sauer, I., and Zeleny, M.: Detection and quantification of anthropogenic methane emissions in Germany using mobile measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20392, https://doi.org/10.5194/egusphere-egu25-20392, 2025.

EGU25-21353 | ECS | Posters on site | AS3.41

A dual-platform approach for quantifying methane emissions at site level 

Roubina Papaconstantinou, Jean-Daniel Paris, Pierre-Yves Quehe, Maria Kezoudi, George Biskos, and Jean Sciare

The increasing atmospheric concentrations of carbon dioxide (CO2) and methane (CH4) from anthropogenic activities pose a major challenge for climate change mitigation. Methane, with a global warming potential 28 times greater than CO2 over a 100-year period, is the second most impactful greenhouse gas (GHG) and requires urgent attention. Effective CH4 reduction hinges on addressing emissions at the level of industrial facilities (natural gas), landfills, and farms. Consequently, the development of reliable tools for site-specific emission detection and quantification is critical for implementing targeted mitigation strategies.

Recent advancements in CH4 atmospheric measurement techniques have enabled in situ mobile technologies deployed on aircraft, cars and now unmanned aerial vehicles (UAVs). UAVs can sample dispersion plumes at both point and facility scales, particularly in challenging locations where traditional methods may fall short (Liu et al., Atmospheric Measurement Techniques, 2024). Here we describe a dual-ground/air approach combining simultaneous CH4 measurements from mobile (car mounted) and aerial (drone-based) systems. This integrated method provides complementary data, offering improved coverage into methane plume dynamics and spatial distribution.

The UAV system employs an ABB LGR GLA131 sensor and 3D wind measurements on a high endurance octocopter with advanced autopilot capabilities, enabling precise detection and quantification of methane sources. The mobile platform features the MIRA Ultra Mobile LDS, delivering high resolution, ground-level emission mapping. Together, these platforms enhance the accuracy and scope of CH4 monitoring efforts.

We present measurements at sites revisited from earlier work that relied only on mobile measurements (Liu et al., Science of The Total Environment, 2023). This earlier work revealed that top-down estimates of methane emissions from waste and livestock in Cyprus exceeded bottom-up national inventory values by 160% and 40%, respectively. Integrating car- and drone-based mapping enables three-dimensional plume characterization providing an enhanced plume sampling and hence more precise quantification estimates. It sheds light on plume development, dispersion, and variability. This framework is particularly advantageous for tackling emissions from diverse and mixed sources such as agricultural operations, industrial facilities, and landfills, where complex environmental and topographical factors influence methane behaviour.

How to cite: Papaconstantinou, R., Paris, J.-D., Quehe, P.-Y., Kezoudi, M., Biskos, G., and Sciare, J.: A dual-platform approach for quantifying methane emissions at site level, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21353, https://doi.org/10.5194/egusphere-egu25-21353, 2025.

EGU25-21355 | Orals | AS3.41

New Insights for Estimating Diurnal Methane Emissions from Landfills 

Maryam Golbazi, Madjid Delkash, and Paul Imhoff

Methane is a short-lived yet extremely potent greenhouse gas in the atmosphere. Methane currently accounts for about one-third of global warming attributed to all greenhouse gases. Landfills, which are the third-largest source of methane emissions, are estimated to emit about 50% more methane than reported by the U.S. Environmental Protection Agency (U.S. EPA) inventory. While some landfills estimate emissions based on waste volume and other specific data, others rely on methane capture and operational information. A previous study on 70 high-emitting landfills in the U.S. revealed that their actual emissions were 77% higher than reported to the EPA. Among the 38 facilities that captured gas, their emissions were, on average, 200% greater than reported. Thus, a more accurate landfill methane emission estimate will have significant impact on our understanding on total atmospheric methane concentrations.

Recent advancements in quantifying landfill emissions reveal that traditional waste decay models are inaccurate for emission estimations due to spatial and temporal variability. Consequently, short-term measurements often fail to represent diurnal average emissions, especially in landfills without gas collection systems. Analyzing the 2020 U.S. EPA Landfill Database, we found that almost 41% of landfills lack gas collection systems. Using the Weather Research and Forecasting model, we simulated barometric pressure over 2267 unique landfills for April 2020. We found that changes in barometric pressure impact methane emissions, with 99% of landfills having more days with higher emissions between 10 AM and 4 PM than other times of the day. This suggests that short-term measurements during these hours, commonly used in field measurements, may overestimate diurnal average emissions, particularly in the absence of gas collection systems. Utilizing an unsaturated soil model, we estimated emission overestimation / underestimation under extreme barometric pressure conditions. Our soil model indicates that emissions measured between 10 AM and 4 PM could be overestimated by up to 25% of their average values. These findings underscore the need for continuous measurements or corrections in short-term emissions to accurately represent diurnal averages for annual greenhouse gas inventories.

For future direction, we aim to fill critical gaps in understanding open waste landfill methane emissions, globally, and improve the accuracy of the atmospheric chemistry models by improving the emission estimations. By providing more accurate estimates of methane emissions from landfills, we will support climate policy development, improve public health outcomes, and advance scientific research.

How to cite: Golbazi, M., Delkash, M., and Imhoff, P.: New Insights for Estimating Diurnal Methane Emissions from Landfills, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21355, https://doi.org/10.5194/egusphere-egu25-21355, 2025.

EGU25-1108 | ECS | Orals | AS3.43

Field based greenhouse gas emission measurement from onsite containments in Nepal. 

Prativa Poudel, Sarana Tuladhar, Anish Ghimire, Guy Howard, Miller Alonso Camargo-Valero Camargo-Valero, Barbara Evans, Olivia Reddy, and Subodh Sharma

On-site sanitation systems (OSS) generate greenhouse gases (GHGs) during the decomposition of fecal matter. The reported measurements of these emissions are confined to a restricted number of research examining septic tanks in high-income nations. We conducted field measurements of onsite containments to generate emissions data for Nepal. This represents the first empirical investigation of greenhouse gas emissions from onsite containments in low- and middle-income countries. Emissions were recorded from a panel of pit latrines (n=18), holding tanks (n=6), septic tanks (n=3), between December 2021 and December 2022. A calibrated static flux chamber was designed was and deployed to collect gases samples at each containment site. Portable gas analyzers were employed to quantify methane (CH4), carbon dioxide (CO2), and nitrous oxide (N2O). Results will be provided in detail. Preliminary investigation showed a substantial range in emissions rates notably CH4 across different types of onsite sanitation containments. Statistical test indicated methane emission rates varied considerably within containment types (P value<0.05). N2O was not discovered in any of the sample containments. Our preliminary findings indicate that onsite containment emissions are greater than anticipated and may be a key area for improvement in order to get net zero emissions.

How to cite: Poudel, P., Tuladhar, S., Ghimire, A., Howard, G., Camargo-Valero, M. A. C.-V., Evans, B., Reddy, O., and Sharma, S.: Field based greenhouse gas emission measurement from onsite containments in Nepal., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1108, https://doi.org/10.5194/egusphere-egu25-1108, 2025.

EGU25-1198 | Posters on site | AS3.43

Capturing and translating the dynamics of traffic emissions using a congestion-based framework 

Pak Lun Fung, Daniel Kühbacher, Tilman Hohenberger, Jia Chen, and Leena Järvi

Traffic congestion remains one of the biggest environmental and social issues in urban cities. Insights from traffic reports, modelling results, and real-world measurements show that traffic congestion would exacerbate vehicular emissions of up to 55%, compared to optimal driving conditions in highly congested urban areas.

To capture the dynamics of traffic patterns, we built our geospatial framework by utilising multiple sources of traffic data: traffic counts and speeds by local in-situ traffic counters, open-access aggregated floating car data (TomTom and Google Traffic), and a standardised functional road classification. The framework also incorporates meteorological parameters that affect the traffic capacity of urban road network to calculate the traffic density. Together with a projected fleet composition and its corresponding speed-dependent traffic emission factors, we computed the resulting dynamic traffic emissions of greenhouse gases (e.g. carbon dioxide CO2) and air pollutants (e.g. carbon monoxide CO and nitrogen oxides NOx) in gridded format. These can then be deployed in existing urban climate models to quantify climatic effects and air pollutant exposure induced by road transportation, and in particular congestion.

We applied the framework in two cities in Europe with distinct traffic behaviour: Helsinki and Munich. The preliminary results show relatively good performance in capturing the dynamics of traffic density in both cities (R2 = 0.78–0.88). The framework was further evaluated against their local emission inventory. However, this gave varying results for different emittants for different road classes in both cities. Beyond local applicability, we also explored the scalabilty of the framework. Applying the calibration coefficients trained in one city and testing in another, we found that road classes such as local connecting roads behaved similarly in both places (r = 0.70–0.96 ) while some others did not.

This initiative sheds light on the feasibility of translating the framework to a larger scale beyond a few cities in Europe. Our future step is to improve the scalability of the framework by including existing large-scale multi-city traffic datasets on urban roads worldwide to better model the heterogeneity of the traffic patterns and emissions in the world.

How to cite: Fung, P. L., Kühbacher, D., Hohenberger, T., Chen, J., and Järvi, L.: Capturing and translating the dynamics of traffic emissions using a congestion-based framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1198, https://doi.org/10.5194/egusphere-egu25-1198, 2025.

EGU25-1263 | ECS | Orals | AS3.43

Drivers of CO2 emissions from road transport in U.S. urban areas 

Xavier Bonnemaizon, Philippe Ciais, Chuanlong Zhou, Simon Ben Arous, Nicolas Megel, Gunnar Berghaüser, and Steven J. Davis

Road transportation in U.S. urban areas accounts for roughly two-thirds of on-road CO2 emissions. Yet the drivers of those transportation emissions and differences among cities are not well-understood owing to limited availability of detailed data until recently. Here, we use high-resolution Floating Car Data to analyze street-level transportation emissions in 457 U.S. urban areas (hereinafter referred to as cities) in 2022, and decompose the key drivers of differences among them. Our study reveals that cities with greater population densities tend to have lower per capita road transportation emissions due to lower travel demand (R2 = 0.36) without significant increases in traffic congestion that represent only a fraction of the total (2-10%). Furthermore, we find that variations in vehicle fleets (e.g., electrification) are still a secondary driver of city-scale transportation emissions. These findings underscore the importance of tailored interventions to mitigate cities’ transportation emissions and may be used to support more sustainable urban transportation systems.

How to cite: Bonnemaizon, X., Ciais, P., Zhou, C., Ben Arous, S., Megel, N., Berghaüser, G., and J. Davis, S.: Drivers of CO2 emissions from road transport in U.S. urban areas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1263, https://doi.org/10.5194/egusphere-egu25-1263, 2025.

Detecting, reporting, and mitigating fugitive methane leaks has been identified as one way of  lowering national methane emissions in the United States.  To that effect, the United States Environmental Protection Agency has launched a new super emitter program that relies on technologies that can detect and report methane leaks for mitigation.  NOAA is exploring the option of utilizing its fleet of geostationary and polar-orbiting satellite sensors to operationalize the short wave infrared Multi Band Multi Pass methane detection algorithm developed by Harvard University.  Prior to transitioning the technology to NOAA operations, a careful evaluation of retrievals from the two sensors, Advanced Baseline Imager on GOES-R series and Visible Infrared Imaging Radiometer Suite on JPSS series is needed.  NOAA satellites can detect only large methane plumes (tons per hour) and benchmarking the capability is critical to work with stakeholders such as the EPA.  To do that, NOAA is partnering with facility operators that conduct timed large methane releases during pipeline blowdown events to validate satellite methane detections and quantification of emissions. NOAA, in partnership with the Pipeline Research Council International, conducted its first pipeline blowdown experiment on October 8, 2024, deploying methane-monitoring technologies across ground, air, and space to track a controlled methane release. Three NOAA geostationary satellites viewing the plume from different geometries detected the plume along with various ground and airborne instruments - all systems reported methane flux estimates that are closer to the values reported by the pipeline operator.  Results of this controlled release experiment will be presented along with plans to conduct additional experiments, jointly with NASA, to validate methane plumes from civilian satellite data as well as those detected by commercial plume mappers such as GHGSat, CarbonMapper, and MethaneSat.

How to cite: Kondragunta, S., Varon, D., and He, T.: Assessing Methane Detection Capabilities of Operational Satellite Sensors using Controlled Release Experiments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3293, https://doi.org/10.5194/egusphere-egu25-3293, 2025.

EGU25-4446 | Posters on site | AS3.43

Improving GHG emissions estimates and multidisciplinary climate research using nuclear observations: the NuClim project 

Susana Barbosa and Scott Chambers and the NuClim Team

Radon (Rn-222) is a unique atmospheric tracer, since it is an inert gaseous radionuclide with a predominantly terrestrial source and a short half-life (3.8232 (8) d), enabling quantification of the relative degree of recent (< 21 d) terrestrial influences on marine air masses. High quality measurements of atmospheric radon activity concentration in remote oceanic locations enable the most accurate identification of baseline conditions. Observations of GHGs under baseline conditions, representative of hemispheric background values, are essential to characterise long-term changes in hemispheric-mean GHG concentrations, differentiate between natural and anthropogenic GHG sources, and improve understanding of the global carbon budget.

The EU-funded project NuClim (Nuclear observations to improve Climate research and GHG emission estimates) will establish world-leading high-quality atmospheric measurements of radon activity concentration and of selected GHG concentrations (CO2, and CH4) at a remote oceanic location, the Eastern North Atlantic (ENA) facility, managed by the Atmospheric Radiation Measurement (ARM) programme (Office of Science from the U.S. Department of Energy), located on Graciosa Island (Azores archipelago), near the middle of the north Atlantic Ocean. These observations will provide an accurate, time-varying atmospheric baseline reference for European greenhouse gas (GHG) levels, enabling a clearer distinction between anthropogenic emissions and slowly changing background levels. NuClim will also enhance measurement of atmospheric radon activity concentration at the Mace Head Station, allowing the identification of latitudinal gradients in baseline atmospheric composition, and supporting the evaluation of the performance of GHG mitigation measures for countries in the northern hemisphere.

The high-quality nuclear and GHG observations from NuClim, and the resulting classification of terrestrial influences on marine air masses, will assist diverse climate and environmental studies, including the study of pollution events, characterisation of marine boundary layer clouds and aerosols, and exploration of the impact of natural planktonic communities on GHG emissions. This poster presents an overview of NuClim, outlines the project objectives and methodologies, and summarises the relevant data products that will be made available to the climate community.

Project NuClim received funding from the EURATOM research and training program 2023-2025 under Grant Agreement No 101166515.

How to cite: Barbosa, S. and Chambers, S. and the NuClim Team: Improving GHG emissions estimates and multidisciplinary climate research using nuclear observations: the NuClim project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4446, https://doi.org/10.5194/egusphere-egu25-4446, 2025.

 Thermoelectric coolers (TECs) differ from conventional cooling devices that use refrigerants in that they utilize the Peltier effect to convert electrical energy into thermal energy, generating a cooling effect [1]. Therefore, unlike conventional cooling devices that use refrigerants such as CFCs, which have a high global warming potential and emit greenhouse gases, thermoelectric coolers have a different environmental impact. Particularly during the usage phase, since electrical energy is converted into thermal energy during operation, it is important to assess the emissions during electrical energy generation. Particularly, the COP of thermoelectric coolers is currently much lower compared to conventional coolers [2], meaning that a greater amount of electrical power is required to achieve the same cooling amount.

 Additionally, during the production phase, the manufacturing of alumina plates generates 90.7% of greenhouse gas emissions, and the sintering process involved in the production of alumina plates contributes 87.3% of the emissions. The primary cause of greenhouse gas emissions during the sintering process is the high temperature and pressure, and the large amount of power used to compact the powder. Therefore, methods to reduce energy consumption should be considered to address the hotspots of the sintering process and reduce the greenhouse gases associated with alumina plates production phase.

 Consequently, possible methods and quantities of greenhouse gas reduction were aimed to be identified by improving the process to reduce energy consumption in the sintering process. In addition, since the main input material is electricity, there is a way for the grid mix to become more eco-friendly. For this purpose, a method of adding sintering aids and applying eco-friendly grid mix is considered. Sintering aids can reduce energy consumption by up to 1.4 times [3], resulting in 28.6% reduction in emissions during the sintering process, from 466.1 kg CO2-eq to 333.0 kg CO2-eq. Additionally, producing with the 2030 power grid mix, which reduces fossil fuel use and increases renewable energy, results in a reduction of 80.0kg CO2-eq, leading to a 38.6% decrease in emissions during sintering process.

 

Reference

[1] Newby, S., Mirihanage, W., Fernando, A., 2025. Body heat energy deriven knitted thermoelectric garments with personal cooling. Applied Thermal Engineering, 258 (A)., pp. 124546.

[2] Tian, M., Aldawi, F., Anqi, A.E., Moria, H., Dizaji, H.S., Wae-hayee, M., 2021. Cost-effective and performance analysis of thermoelectricity as a building cooling system; experimental case study based on a single TEC-12706 commercial module. Case Studies in Thermal Engineering, 27, pp. 101366.

[3] Heidary, D. S. B., Lanagan, M., and Randall, C. A., 2018. Contrasting energy efficiency in various ceramic sintering processes. Journal of the European Ceramic Society 38(4), 1018-1029.

How to cite: Kim, H. Y. and Wee, D.: Analysis on greenhouse gas reduction strategies for thermoelectric coolers using cradle-to-gate life cycle assessment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4694, https://doi.org/10.5194/egusphere-egu25-4694, 2025.

EGU25-4839 | Orals | AS3.43

Monitoring urban CO2 emissions from space: current status and future potential 

Abhishek Chatterjee, Doyeon Ahn, Dustin Roten, Matthaus Kiel, Robert Nelson, Thomas Kurosu, Dien Wu, John Lin, and Kevin Gurney

Cities with their large, dense populations are concentrated sources of CO2 emissions to the atmosphere. Although more than 60% of global fossil fuel CO2 emissions are from cities, yet we lack high-quality city-level emissions inventories and/or independent verification datasets across the majority of global cities. Several cities have also adopted ambitious goals of reaching net-zero emissions by 2030 or 2050. In fact, most recently at COP28, several cities, including those in non-Annex I countries, signed up to be part of the Coalition for High Ambition Multilevel Partnerships for Climate Action (CHAMP ; UNFCCC COP28), thereby obligating themselves to report emissions on a timely basis. So, how can we assist city-scale and local policy and decision-making entities to utilize information from space-based observations to monitor and track GHG emissions? In this presentation, I will show the application of OCO-2 and OCO-3 data across a suite of global cities worldwide. I will show that well-defined and robust mathematical frameworks can exploit the information content in dense, fine-scale, space-based CO2 data to deliver not only whole-city or total emission estimates but also attribute them to individual sectors, such as large point sources, on-road emissions, etc. I will also show some examples from recent studies that illustrate the value of exploiting co-located emissions of other species (such as CO, NO2, CH4) to obtain novel insights into sectoral emission characteristics. Examples from OCO-3, TROPOMI and EMIT data will be shown to demonstrate the value of assimilating information from disparate tracers for reliable source attributions. Even though there are methodological challenges in setting up a multi-species framework, the problem is not insurmountable. Development and refinement of such multi-species frameworks need to start now in order to unlock the true potential of space-based datasets. This is also crucial to optimally utilizing the information from future space-based CO2 emission monitoring sensors, such as Carbon Mapper, ESA’s CO2M, JAXA’s GOSAT-GW and other planned missions. The presentation will conclude with a discussion of implications of space-based datasets for tracking city- and country-level progress towards meeting proposed CO2 emission reduction goals and its value and benefit for advancing bottom-up emission inventories.

How to cite: Chatterjee, A., Ahn, D., Roten, D., Kiel, M., Nelson, R., Kurosu, T., Wu, D., Lin, J., and Gurney, K.: Monitoring urban CO2 emissions from space: current status and future potential, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4839, https://doi.org/10.5194/egusphere-egu25-4839, 2025.

EGU25-5294 | ECS | Posters on site | AS3.43

Leveraging wide area XCO2 deep learning in estimating urban CO2 emissions from space 

Zeyu Wang and Feng Zhang

Urban areas account for more than 70% of fossil fuel carbon dioxide (CO2) emissions worldwide. Recent (OCO-3 released in 2019) and forthcoming (CO2M, TANSAT-2, and GOSAT-GW) greenhouse gas satellites can observe wide area column average dry air mole fraction of carbon dioxide (XCO2) of entire urban areas. Although top-down urban emission monitoring has improved in terms of spatial coverage and frequency, the challenge remains in how to utilize space-based observations to perform accurate inversion of source area’s emission. The high uncertainty mainly arises from XCO2 observations’ low signal-to-noise ratio due to non-anthropogenic fluxes and missing data due to sophisticated atmospheric conditions. 

To achieve accurate urban emission estimation from space, we propose a deep learning (DL) framework which can intelligently capture XCO2 patterns from wide area XCO2 observations. The synthetic CO2M dataset serves as model pre-training materials for its ideal XCO2 observations given by chemical transport model. Transformer is selected as the architecture of DL model for its ability to model global dependency across wide area observations. The proposed model has been validated on the Berlin city’s synthetic CO2M dataset and OCO-3 snapshot area map (SAM) mode observations. In both cases, the pre-trained DL model effectively interpolated missing XCO2 values throughout the XCO2 snapshot, and showed outperformance on urban plume signal identification compared to conventional algorithms. Furthermore, by incorporating DL model’s prediction results with inversion methods, we performed emission estimates for Berlin city on synthetic CO2M data and multiple cities globally on OCO-3 SAMs. Our top-down emission estimation results showed high consistency with prior bottom-up inventories. This study provides valuable insights into advancing intelligent methodologies for urban emission inversion from wide area satellite observations.

How to cite: Wang, Z. and Zhang, F.: Leveraging wide area XCO2 deep learning in estimating urban CO2 emissions from space, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5294, https://doi.org/10.5194/egusphere-egu25-5294, 2025.

EGU25-5388 | ECS | Posters on site | AS3.43

The nitrous oxide budget in China 

Ziyuan Sun, Zimeng Li, and Songbai Hong

Nitrous oxide (N2O) is a kind of long-lived greenhouse gas. Since the Industrial Revolution, increasing atmospheric N2O concentrations have contributed to the depletion of the stratospheric ozone layer and climate change. China has been a hot spot for global N2O emissions, with a rapid growth. However, estimates of N2O emissions from China’s ecosystem remain largely uncertain. Therefore, here we provide a multi-method estimates (inventory, process-based model and atmospheric inversion) of terrestrial ecosystem N2O emissions in China. The process-based models were further modified based on observational datasets. Finally, we provide a comprehensive quantification of China's N2O emissions caused by natural and anthropogenic ecosystems from 1980 to 2023.

How to cite: Sun, Z., Li, Z., and Hong, S.: The nitrous oxide budget in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5388, https://doi.org/10.5194/egusphere-egu25-5388, 2025.

EGU25-5425 | Orals | AS3.43

Quantify natural gas methane emissions from a city cluster in East China 

Yuzhong Zhang, Yujia Zhao, Xinlu Wang, Rui Wang, Botian Qiu, Shuang Zhao, Yanli Zhang, Zhengning Xu, Xiangyu Pei, Zhibin Wang, Youwen Sun, Cheng Huang, and Ying Zhou

The consumption of natural gas in China, predominantly in cities, has nearly tripled over the past decade. However, there is an absence of measurement-based assessment of methane emissions from natural gas consumption in Chinese cities. Moreover, it is challenging to separate the contribution of natural gas relative to other major urban methane sources (e.g., wastewater, landfills) using only methane observations. Here, we use in-situ and total-column ethane observations across the Yangtze River Delta, one of China’s most important metropolitan areas, between 2012 and 2021, to quantify methane emissions from the natural gas sector. Ethane is co-emitted with methane in natural gas and has no significant biogenic sources, and therefore serves as a tracer to separate the contribution of natural gas from other methane sources. To interpret ethane observations, we apply atmospheric chemical transport simulations with the GEOS-Chem model to account for transport, mixing, and chemical decay. Our analysis reveals that surface ethane concentrations have increased by 0.25–0.3 ppb a-1 at city-cluster sites, in contrast to a stable global background concentration and a slightly negative trend in regional total-column measurements. The simulation indicates that a substantial natural gas leakage rate (2.5–4.1%) is required to replicate the observed trend. This leakage rate implies that natural gas consumption emits 0.55–0.9 Tg methane emissions annually in the Yangtze River Delta, accounting for about 5.1–8.4% of the regional total emissions. Our findings indicate that natural gas usage is a substantial contributor to methane emissions and their growth in East China.

How to cite: Zhang, Y., Zhao, Y., Wang, X., Wang, R., Qiu, B., Zhao, S., Zhang, Y., Xu, Z., Pei, X., Wang, Z., Sun, Y., Huang, C., and Zhou, Y.: Quantify natural gas methane emissions from a city cluster in East China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5425, https://doi.org/10.5194/egusphere-egu25-5425, 2025.

EGU25-5703 | Orals | AS3.43

Inverse Modeling of High Global Warming Potential Perfluorinated Greenhouse Gases in Southeastern China 

Yuyang Chen, Bo Yao, Minde An, Ao Ding, Song Liu, Xicheng Li, Yali Li, Simon O'Doherty, Paul Krummel, and Lei Zhu

Sulfur hexafluoride (SF6), nitrogen trifluoride (NF3), and three types of perfluorocarbons (PFCs; PFC-14, PFC-116, and PFC-318) are perfluorinated greenhouse gases (PF-GHGs). PF-GHGs have long atmospheric lifetimes and global warming potentials thousands of times greater than carbon dioxide (CO2). Using high-frequency continuous in situ observations from the Xichong Monitoring station at Shenzhen, China and a Bayesian inversion framework, we assess the 2021-2023 PF-GHG emissions in southeastern China, a region featuring substantial growth in population and industries. We find a continued increase in emissions of all PF-GHGs. During 2021-2023, NF3 emissions show the highest annual growth rate of 40.38% yr-1, likely linked with the increasing demand in semiconductor industries in this region, while PFC-14 has the lowest of 5.87% yr-1. Regarding CO2-equivalent emissions, SF6 contributes the most to total PF-GHG growth (51.75%), followed by NF3 (30.86%). As for the seasonality in PF-GHG emissions in southeastern China, SF6 and PFC-116 emissions show significant seasonal variation. The seasonal variabilities in SF6 are likely associated with the high winter electricity demand, while the winter peaks in PFC-116 emissions may tie with semiconductor manufacturing. PFC-318 exhibits the largest seasonal variation, with a winter-to-spring and autumn emissions ratio of 5.10. The increased PFC-318 emissions in winter might be due to heightened HCFC-22 feedstock uses. The findings provide guidance for targeted mitigation strategies to address the rising emissions.

How to cite: Chen, Y., Yao, B., An, M., Ding, A., Liu, S., Li, X., Li, Y., O'Doherty, S., Krummel, P., and Zhu, L.: Inverse Modeling of High Global Warming Potential Perfluorinated Greenhouse Gases in Southeastern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5703, https://doi.org/10.5194/egusphere-egu25-5703, 2025.

EGU25-6791 | ECS | Posters on site | AS3.43

Global Emissions of Tetrafluoromethane (CF4) Hexafluoroethane (C2F6) Determined by Inverse Modeling 

Benjamin Püschel, Luise Kandler, Martin Vojta, and Andreas Stohl

We determined global emissions of the perfluorocarbons (PFC) tetrafluoromethane (CF4) and hexafluoroethane (C2F6) from 2004 to 2023 using an inverse modeling approach. These PFCs are characterised by their exceptionally long atmospheric lifetimes (~50.000y for CF4 and ~10.000y for C2F6) and strong infrared absorption, making them some of the most potent greenhouse gases. Emissions of these gases are almost entirely anthropogenic, originating primarily from aluminium smelting and semiconductor manufacturing. Previous studies have highlighted significant discrepancies between bottom-up inventories, based on activity and industry data, and top-down estimates derived from atmospheric measurements. In this study, we use continuous and flask measurements combined the Bayesian inversion algorithm FLEXINVERT+ and the Lagrangian particle dispersion model FLEXPART to estimate global emissions of CF4 and C2F6 and their regional distribution. Our findings indicate a decline in emissions until approximately 2009, followed by an increase in subsequent years, contrasting with bottom-up inventories, which show a steady decrease over the study period. The largest emissions are located primarily in East Asia, with substantial potential emissions in South and Southeast Asia, followed by North America and Europe. India and Malaysia, with their growing aluminium (India) and semiconductor (Malaysia) industries, emerge as significant sources of uncertainty in our emission estimates due to limited observational coverage in these regions. While emission reduction measures in the aluminium industry appear to be effective, the impact of mitigation efforts by semiconductor manufacturers are likely overestimated.

How to cite: Püschel, B., Kandler, L., Vojta, M., and Stohl, A.: Global Emissions of Tetrafluoromethane (CF4) Hexafluoroethane (C2F6) Determined by Inverse Modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6791, https://doi.org/10.5194/egusphere-egu25-6791, 2025.

EGU25-6956 | ECS | Orals | AS3.43

Emissions of the powerful greenhouse gas HFC-23 suggest significant under-reporting since the implementation of the Kigali Amendment 

Ben Adam, Luke Western, Jens Muhle, Haklim Choi, Paul Krummel, Simon O'Doherty, Dickon Young, Kieran Stanley, Paul Fraser, Christina Harth, Peter Salameh, Ray Weiss, Ronald Prinn, Jooil Kim, Hyeri Park, Sunyoung Park, Alistair Manning, Anwar Khan, Dudley Shallcross, and Matt Rigby

HFC-23 (trifluoromethane) is a potent greenhouse gas, believed to be emitted to the atmosphere primarily as a by-product during the production of the refrigerant and feedstock HCFC-22 (chlorodifluoromethane). Due to the high global warming potential of HFC-23 (GWP100 ~ 14,700), the Kigali Amendment to the Montreal Protocol requires countries to limit their emissions of HFC-23 as much as possible and report these emissions to the United Nations Environment Programme. Global reported emissions have been in the range 2-3 Gg yr-1 since 2019 and reflect the near-total destruction of emissions from HCFC-22 production reported by the countries with major HCFC-22 manufacturers, such as China and India. However, atmospheric observations show that, whilst emissions fell from their maximum in 2019 of 17.3 ± 0.8 Gg yr-1 to 14.0 ± 0.9 Gg yr-1 in 2023, they remain many times higher than reported. In addition, regional inverse modelling was performed based on measurements from the AGAGE site at Gosan, South Korea, using three different Bayesian inverse models (FLEXINVERT+, InTEM and RHIME) to estimate emissions from eastern China. These inversions use the same observational data, but different transport models, baselines, priors and uncertainties. Results are compared to better quantify regional emissions and their uncertainties. The results suggest that emissions from eastern China are four to six times higher than reported for the whole of China.  

In addition, we examine the emission of HFC-23 as a by-product during the production of other hydrofluorocarbons and fluorochemicals. In-atmosphere HFC-23 production (from the breakdown of certain hydrofluoroolefins used as replacements for HFCs) is also investigated further using a 3D chemical transport model incorporating photolysis and ozonolysis reactions. Our results indicate that, based on currently available information, these potential alternative sources contribute less than 2.0 Gg yr-1 to global emissions. This suggests that HFC-23 emissions from HCFC-22 production have been consistently under-reported since the implementation of the Kigali Amendment. It therefore appears likely that abatement of HFC-23 emissions has not occurred to the extent reported in this period. Improved monitoring and verification of HFC-23 emissions from industrial sources is essential to the continued success and efficacy of the Kigali Amendment.

How to cite: Adam, B., Western, L., Muhle, J., Choi, H., Krummel, P., O'Doherty, S., Young, D., Stanley, K., Fraser, P., Harth, C., Salameh, P., Weiss, R., Prinn, R., Kim, J., Park, H., Park, S., Manning, A., Khan, A., Shallcross, D., and Rigby, M.: Emissions of the powerful greenhouse gas HFC-23 suggest significant under-reporting since the implementation of the Kigali Amendment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6956, https://doi.org/10.5194/egusphere-egu25-6956, 2025.

EGU25-8355 | ECS | Orals | AS3.43

Bridging the Fleet Distribution Data Gap with Satellite Imagery and Deep Learning for GHG Estimation 

Bilal Aslam, Toby Hocking, Pawlok Dass, Anna Kato, and Kevin Gurney

Precise quantification of greenhouse gas (GHG) emissions is important for better urban sustainability. Transportation is one of the primary contributing sources of greenhouse gas emissions. To quantify better on-road GHG emissions, it is essential to decode fleet distribution. However, globally, many cities do not have the infrastructure to calculate a fleet distribution. Therefore, there will always be an uncertain error in the on-road GHG emissions estimation. However, very high-resolution satellite data can be helpful to overcome this gap due to its global temporal coverage. Hence, this study proposes a deep learning method, Faster Region-based Convolutional Neural Network (Faster R-CNN), and You Look Only Once (YOLO) based vehicle detection to identify the vehicles and vehicle categories from the very high-resolution satellite data and estimate the fleet distribution. The results show that our model can identify, Passenger Cars, Buses, Trucks, and Large Passenger Cars with the precision of 93.30%, 79.50%, 78.90%, and 81.15%, respectively. We applied this model to temporally available satellite images of Phoenix and calculated the fleet distribution and calculated the FFCO2 based on that fleet distribution and compared it with FFCO2 estimated using CURB dataset fleet distribution. Results show that CURB data-based FFOC2 is over-predicting by 22%, while using fleet distribution estimated by this method, FFCO2 over-predicting by 17% w.r.t VULCAN. These findings demonstrate the effectiveness of satellite-based fleet distribution estimation for improving FFCO₂ quantification in cities lacking robust data infrastructure. This approach provides a scalable and data-driven pathway to more accurate urban emissions modeling, enabling better-informed urban planning and sustainability efforts.

How to cite: Aslam, B., Hocking, T., Dass, P., Kato, A., and Gurney, K.: Bridging the Fleet Distribution Data Gap with Satellite Imagery and Deep Learning for GHG Estimation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8355, https://doi.org/10.5194/egusphere-egu25-8355, 2025.

EGU25-8609 | Posters on site | AS3.43

Enhancing top-down HFC-134a emission estimates through parameter space exploration 

Seyed omid Nabavi, Martin Vojta, Anjumol Raju, Sophie Wittig, and Andreas Stohl

Bayesian inverse modeling is a widely used approach for estimating greenhouse gas (GHG) emissions from atmospheric measurements. However, this method is subject to various uncertainties, including errors in the transport model, inaccuracies in baseline mole fractions, and uncertainties associated with the parameters of the Bayesian inversion framework.

In this study, we investigated the impact of these uncertainties on the Bayesian inversion of a key hydrofluorocarbon contributing to climate change, HFC-134a. We first conducted a grid search to refine the nudging parameters for simulating three-dimensional initial HFC fields using the FLEXible PARTicle-Linear Chemistry Module (FLEXPART-LCM). Subsequently, we employed Latin Hypercube Sampling (LHS) to explore inversion uncertainties by sampling a broad parameter space within the Bayesian inverse modeling framework FLEXINVERT.

Through over 250 ensemble simulations for initial fields and 15,000 ensemble inversion runs, we identified the most influential parameters and optimized configurations for the inverse modeling of HFC-134a. These findings improve the reliability of HFC-134a emission estimates and provide insights into the role of inversion parameters, applicable to the inversion of other greenhouse gases.

How to cite: Nabavi, S. O., Vojta, M., Raju, A., Wittig, S., and Stohl, A.: Enhancing top-down HFC-134a emission estimates through parameter space exploration, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8609, https://doi.org/10.5194/egusphere-egu25-8609, 2025.

EGU25-10046 | Orals | AS3.43

Measurement and modelling of Eddy-covariance fluxes of CO2 in the city of Zurich 

Dominik Brunner, Leonie Bernet, Lionel Constantin, Betty Molinier, Natascha Kljun, Rainer Hilland, Andreas Christen, Ingrid Super, Junwei Li, Jia Chen, Stavros Stagakis, and Lukas Emmenegger

The city of Zurich, Switzerland, aims to achieve net-zero greenhouse gas emissions by the year 2040. To support the city in monitoring its path towards this ambitious goal, an emission monitoring program has been established with two complementary approaches. The first involves a network of CO2 mid- and low-cost sensors in combination with atmospheric transport inverse modelling. The second, presented here, combines CO2 flux measurements from an Eddy-covariance system installed on a 17 m mast on top of a 95 m tall building in the city center with flux footprint modeling and a high-resolution emission inventory.

Here we present a detailed comparison between hourly simulated and observed CO2 fluxes for a period of two years (August 2022 – August 2024) to evaluate the inventory and its partitioning into source sectors. The simulated fluxes were obtained by multiplying the footprints with the sectorially resolved emissions from the inventory, all available on a 10 m x 10 m grid. The sectorial emissions were scaled by temporal factors describing diurnal, day-of-week and seasonal variability. Traffic emissions, for example, were scaled using actual traffic counts from 182 counters and heating emissions were scaled with a heating-degree-day factor based on outdoor temperatures. In addition to anthropogenic emissions, biospheric CO2 fluxes from trees, lawns and cropland were simulated at 10 m x 10 m resolution with the Vegetation Photosynthesis and Respiration Model (VPRM), driven by local temperature and radiation measurements and Sentinel-2 satellite observations.

The simulated hourly fluxes, which change in time due to the varying footprints and temporal scaling factors, were found to be strongly correlated with the observed fluxes but were, on average, higher, suggesting that the inventory overestimates the actual emissions from the city. The comparison also allowed us to improve the temporal scaling factors of certain sectors, for example, to better represent the reduced emissions during holidays or the heating demand during the transition periods between winter and summer. Accurately representing the temporal variability is important, as it allows disentangling source sectors that follow different temporal profiles. The results demonstrate the capability of tracking the CO2 emissions of a central part of Zurich with a single, well-placed flux tower with an accuracy that is suitable for evaluating the expected emission reductions in the coming decades.

How to cite: Brunner, D., Bernet, L., Constantin, L., Molinier, B., Kljun, N., Hilland, R., Christen, A., Super, I., Li, J., Chen, J., Stagakis, S., and Emmenegger, L.: Measurement and modelling of Eddy-covariance fluxes of CO2 in the city of Zurich, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10046, https://doi.org/10.5194/egusphere-egu25-10046, 2025.

EGU25-10322 | ECS | Posters on site | AS3.43

 Utilizing tropospheric CO isotope observations from a low-latitude Atlantic sampling network to constrain the oxidative chlorine sink  

Chloe Brashear, Maarten van Herpen, Berend van de Kraats, Matthew Johnson, Luisa Pennacchio, Marie Mikkelsen, Alfonso Saiz-Lopez, Daphne Meidan, and Thomas Röckmann

The isotopic composition of CO can be used to detect enhanced oxidation of methane by atomic chlorine due to the strong kinetic isotope effect related to this reaction (KIECH4+Cl = 66 per mil). Importantly, this detection method has demonstrated the presence of a large ground-level North Atlantic chlorine source for the years 1996-1997, linked to the geographic distribution of iron-rich Sahara dust within the marine boundary layer (Mak et al., 2003; van Herpen et al., 2023). Here, we present 2023-2024 d13CCO and d18OCO data from an air sampling network established across the low-latitude Atlantic Ocean, including bi-weekly measurements from Tenerife (IEO and IZO), Cape Verde (CVAO), Barbados (RPB), and northern Brazil (ATTO). In addition, the network includes intermittent flask samples taken aboard commercial shipping vessels as they complete trans-Atlantic routes. Our analysis supports the existence of a large chlorine sink of methane in dust-associated regions, which varies seasonally. Underestimates in the occurrence of chlorine oxidation propagate to isotope-constrained top-down global methane models, shifting predicted contributions away from fossil fuels and towards biological sources. Ultimately, our results provide an opportunity to reconcile missing chlorine sources, which may have significant implications for global methane source estimations.

How to cite: Brashear, C., van Herpen, M., van de Kraats, B., Johnson, M., Pennacchio, L., Mikkelsen, M., Saiz-Lopez, A., Meidan, D., and Röckmann, T.:  Utilizing tropospheric CO isotope observations from a low-latitude Atlantic sampling network to constrain the oxidative chlorine sink , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10322, https://doi.org/10.5194/egusphere-egu25-10322, 2025.

EGU25-10345 | ECS | Orals | AS3.43

Using NO2 satellite observations to constrain ffCO2 

Chlöe Schooling, Paul Palmer, and Liang Feng

Success of the Paris Agreement relies on rapid reductions in fossil fuel CO2 (ffCO2) emissions, which can be independently verified using atmospheric data. However, estimating changes in ffCO2 from atmospheric CO2 is challenging due to large and variable contributions from natural fluxes and background concentrations. Nitrogen oxides (NOx = NO + NO2), which are a major contributor to surface air pollution that have adverse effects on human health, are co-emitted with CO2 during incomplete fossil fuel combustion. Because atmospheric NOx has a relatively short lifetime (hours to days), low background concentrations, and limited natural sources, it is possible to link elevated NO2 satellite columns to their parent emissions.

We present results from an Ensemble Kalman Filter (EnKF) based model inversion using the GEOS-Chem atmospheric chemistry and transport model, along with NO2 TROPOMI observations, to estimate NOx emissions across mainland Europe. Leveraging sector-specific CO2:NOx emission ratios, we then convert the NOx posterior dataset to ffCO2. Additionally, we present preliminary findings for an alternative methodology that relies less on prior knowledge of emission ratios. This approach uses a combined CO2:NOx inversion, integrating TROPOMI NO2 and OCO-2 CO2 measurements to directly constrain ffCO2.

Our results describe a more accurate and direct approach for estimating fossil fuel CO2 emissions, which we anticipate will offer valuable insights for verifying national emission reductions and informing global climate mitigation strategies.

 

How to cite: Schooling, C., Palmer, P., and Feng, L.: Using NO2 satellite observations to constrain ffCO2, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10345, https://doi.org/10.5194/egusphere-egu25-10345, 2025.

EGU25-10382 | ECS | Orals | AS3.43

Designing CO2 sensor networks for German cities: Insights from synthetic studies in Berlin and Munich  

Christopher Lüken-Winkels, Lukas Pilz, Simon Cello, and Sanam N. Vardag

Cities are major contributors to global anthropogenic CO2 emissions and their share relative to national emissions is increasing in many countries. This makes urban areas critical targets for effective CO2 mitigation strategies. To monitor and verify mitigation efforts, measurement-based emission estimates of anthropogenic CO2 emissions can be used. Many cities, however, lack the infrastructure to precisely constrain these emissions. 

To support the development of urban sensor networks within the Integrated Greenhouse Gas Monitoring System (ITMS) for Germany, we use Observing System Simulation Experiments (OSSEs). In these experiments, we evaluate synthetic in-situ sensor networks in Berlin and Munich with regards to their potential to constrain anthropogenic CO2 emissions. 

Our OSSEs use a Bayesian inversion framework, with atmospheric transport simulated by the Lagrangian Particle Dispersion Model FLEXPART-WRF and meteorology computed by the Weather Research and Forecasting (WRF) model at a 1 km resolution for urban areas over an entire year. 

We analyze the effect of number, location and precision of CO2 sensors, as well as of co-located CO concentration measurements.  We suggest favorable city-specific sensor network configurations and identify key factors for efficient network designs across the two cities. Our results support the deployment of efficient and effective sensor networks for measurement-based CO2 emission monitoring and verification in Berlin, Munich and similar cities and will be the basis for future planned sensor network installations in Germany. 

How to cite: Lüken-Winkels, C., Pilz, L., Cello, S., and Vardag, S. N.: Designing CO2 sensor networks for German cities: Insights from synthetic studies in Berlin and Munich , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10382, https://doi.org/10.5194/egusphere-egu25-10382, 2025.

EGU25-10688 | Posters on site | AS3.43

Diversity and uncertainty in the assessment of GHG emissions in national inventories: a sectoral analysis of Northeastern European countries 

Iveta Steinberga, Ivo Vinogradovs, Agrita Briede, Zanda Peneze, and Kristine Ketrina Putnina

The correlation between estimated national GHG emissions and uncertainty is generally known. The causes and sources of the uncertainties are diverse and relate to source activity (field studies and research, census data), methodologies, variations in emission factors, and scientific studies/publications. Uncertainty has occurred due to a lack of knowledge of true values, in which uncertainty is assessed by the probability density function. Uncertainty analysis helps identify and prioritize activities (monitoring, inventory, evaluation methods, etc.) to improve the evaluation and reduce uncertainty. A quantitative uncertainty analysis is often performed for a 95% confidence interval. 
Different calculation methodologies are used in each sector (waste, energy, LULUCF, industry, transport, and agriculture); the mechanisms for producing emissions of emitted substances are complex and variable and require scientifically based research to update them. Regional differences are also essential, as climate, access to technologies, the possibility of introducing them, and other physio-geographic conditions have a significant impact. One of the challenging issues in the GHG emissions assessment relates to future emission projections related to future unpredictability due to climate change; changes in economic growth plans also create a lot of uncertainty. For example, in the forest management and land use sectors, the intensity of CO2 sequestration in the ecosystem must be assessed. Recent studies, including those informing Latvia's LULUCF emission factors, reveal significant uncertainties in estimating GHG emissions from organic-rich soils due to short-term measurements, limited sampling, and neglect of long-term soil carbon dynamics.  Another relatively more straightforward source of data uncertainty is identified in the waste management sector. In this sector, the analysis of methane emissions from landfills from disposed solid municipal waste requires a precise morphological composition of the waste, as the result of the calculation depends not only on the amount of waste but also on the content of organic matter and the intensity of aerobic or anaerobic degradation. It is self-evident that the composition of waste can be variable and monitored effectively today. Still, different waste fractions are characterized by different degradation intensities, and according to the assessment method, degradation should be assessed over a period of 100 years, which means that the historical morphological composition of waste is required. The lack of such data often leads to up to 150 % uncertainty. 
When analyzing the national reports of the Northeastern Region of Europe (Latvia, Finland, Estonia, and Lithuania), the most considerable uncertainties can be found in the LULUCF sector, which, in view of these countries' economic activities, is very substantial in the overall assessment. Reducing uncertainty in this area is of the utmost importance as it is closely linked to national climate plans and the measures taken to achieve climate neutrality. 

How to cite: Steinberga, I., Vinogradovs, I., Briede, A., Peneze, Z., and Putnina, K. K.: Diversity and uncertainty in the assessment of GHG emissions in national inventories: a sectoral analysis of Northeastern European countries, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10688, https://doi.org/10.5194/egusphere-egu25-10688, 2025.

EGU25-10769 | Orals | AS3.43

EYE-CLIMA: A Horizon Europe project using atmospheric inversions to improve national estimates of greenhouse gas emissions 

Wilfried Winiwarter, Rona Thompson, Andreas Stohl, Philippe Peylin, Philippe Ciais, Hartmut Boesch, Tuula Aalto, Antoine Berchet, Maria Kanakidou, Glen Peters, Dmitry Shchepashchenko, Jean-Pierre Chang, Roland Fuß, Ignacio Pisso, Richard Engelen, Almut Arneth, Nina Buchmann, Stefan Reimann, Stephen Platt, and Nalini Krishnankutty

EYE-CLIMA is a Horizon Europe project that aims to improve estimates of emissions of climate forcers (CO2, CH4, N2O, SF6, HFCs, and black carbon aerosols) by using atmospheric observations. Atmospheric observations can be used, with the help of an atmospheric transport model, in a statistical optimization framework to estimate surface-to-atmosphere fluxes – a method known as atmospheric inversion. These fluxes can be used to estimate national and sub-national emissions (and removals) and can help support national monitoring and reporting and ultimately the Global Stocktake process.

One of the main goals of EYE-CLIMA is to develop atmospheric inversions into a useful tool for improving national greenhouse gas inventories (NGHGIs). This entails establishing good practice guidelines for atmospheric inversions (with a particular focus on the national scale) including a full assessment of the uncertainties, as well as developing the methodology to prepare sectorial emission estimates from atmospheric inversions and make these comparable to what is reported in national greenhouse gas inventories (NGHGIs). EYE-CLIMA collaborates with NGHGI agencies on pilot projects comparing and reconciling inventory and atmospheric inversion-based emission estimates, as well as on establishing a good practice for atmospheric observation-based verification of NGHGIs.

This presentation will present an overview of the EYE-CLIMA methodology and the pilot projects with NGHGI agencies. In particular, the pilot projects cover: i) land use, land use change and forestry (LULUCF) emissions and removals of CO2 in France, ii) N2O emissions from agriculture in Germany, and iii) CH4 emissions from agriculture and waste in France and Germany.

How to cite: Winiwarter, W., Thompson, R., Stohl, A., Peylin, P., Ciais, P., Boesch, H., Aalto, T., Berchet, A., Kanakidou, M., Peters, G., Shchepashchenko, D., Chang, J.-P., Fuß, R., Pisso, I., Engelen, R., Arneth, A., Buchmann, N., Reimann, S., Platt, S., and Krishnankutty, N.: EYE-CLIMA: A Horizon Europe project using atmospheric inversions to improve national estimates of greenhouse gas emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10769, https://doi.org/10.5194/egusphere-egu25-10769, 2025.

EGU25-10965 | ECS | Posters on site | AS3.43

Towards an urban CO2 and air pollution network in Heidelberg-Mannheim 

Kenneth Murai von Buenau, Pia Haas, Robert Maiwald, Veit Ulrich, Sebastian Block, André Butz, and Sanam N. Vardag

Cities have a great responsibility to mitigate CO2 emissions, as they contribute substantially to global anthropogenic CO2. To assist cities in efficient mitigation planning an independent data-driven approach to monitor emissions within urban areas is required. 

The Rhine-Neckar area comprises the cities of Mannheim and Heidelberg and is characterized by large emissions due to significant energy production and industry on the one hand, and by ambitious climate goals on the other hand. To monitor and support mitigation efforts of these cities, we are developing an urban monitoring network using mid-cost CO2 and air quality sensors for Heidelberg and Mannheim. The network will consist of 18 sensor nodes provided by the University of California, Berkeley. Each node is identical in construction to the sensors in the Berkeley Air Quality and CO2 Network (BEACO2N) (Shusterman et al., 2016) and measures CO2, CO, PM2.5 and NO2.

In conjunction with the measurement network, we use GRAMM/GRAL to model atmospheric transport in the domain on high resolution. GRAMM/GRAL is run following a catalog approach, in which hourly steady-state wind conditions are assumed. This way the computational costs can be reduced enabling the simulation of longer time scales on street canyon resolving spatial resolution (Berchet et al., 2017, May et al., 2024). We feed the model with high-resolution inventories of fossil fuel and biogenic emissions and compare the simulated enhancements to the measurements of the first deployed nodes.  We discuss the capability of the conjunction of high-resolution modeling and mid-cost observations to detect emission patterns within the Rhine-Neckar area.

Shusterman, A. A., et al., (2016). The BErkeley Atmospheric CO2 Observation Network: initial evaluation. Atmos. Chem. Phys., 16, 13449–13463., https://doi.org/10.5194/acp-16-13449-2016

Berchet, A., et al., (2017). A cost-effective method for simulating city-wide air flow and pollutant dispersion at building resolving scale. Atmospheric Environment, 158, 181-196., https://doi.org/10.1016/j.atmosenv.2017.03.030

May, M., et al., (2024). Evaluation of the GRAMM/GRAL Model for High-Resolution Wind Fields in Heidelberg, Germany. Atmospheric Research, 300, 107207., https://doi.org/10.1016/j.atmosres.2023.107207

How to cite: Murai von Buenau, K., Haas, P., Maiwald, R., Ulrich, V., Block, S., Butz, A., and Vardag, S. N.: Towards an urban CO2 and air pollution network in Heidelberg-Mannheim, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10965, https://doi.org/10.5194/egusphere-egu25-10965, 2025.

EGU25-11020 | ECS | Orals | AS3.43

CHETNA-Brick Sector: Estimating GHG and Pollutant Emissions from Brick Kilns in India Using Sentinel-2 Imagery and Deep Learning 

Clément Goldmann, Sugandha Arora, Chuanlong Zhou, Philippe Ciais, Fabian Gieseke, Kushal Tibrewal, and Harish Phuleria

India, the world’s second-largest brick producer, operates over 100,000 kilns. These kilns emit 170 kt of PM2.5 (15% of the national total) and 120 Mt of CO2 (6% of the national total) annually, along with substantial SOx and NOx emissions. Transitioning from traditional Fixed Chimney Bull’s Trench Kilns (FCBTKs) to cleaner technologies, such as Zigzag Kilns (ZZKs), has the potential to reduce coal consumption by 20% and particulate matter emissions by 70%. However, comprehensive datasets for kiln locations across India remain scarce. This study contributes to the CHETNA project (City-wise High-resolution carbon Emissions Tracking and Nationwide Analysis), which leverages artificial intelligence and advanced datasets to deliver high-resolution, near real-time daily CO2 and air pollutant emissions data for over 100 Indian cities. 

To address this gap, we leveraged Sentinel-2 imagery, with a spatial resolution of 10–20 m, to develop a cost-effective and scalable approach. Most existing studies focus on specific geographic areas, such as northern India, and rely on expensive, high-resolution satellite imagery that is often not readily available, limiting their broader applicability. In contrast, our study represents the first nationwide mapping of brick kilns in India, using openly accessible satellite data and advanced machine learning models.

Using a curated dataset of 9,600 geo-tagged labels covering 18,000 km², we developed a method combining Sentinel-2 imagery with convolutional neural networks (CNN) to detect brick kilns and classify their operational technologies (e.g., FCBTK, Zigzag). Labels were annotated using Google Earth layers on QGIS and validated based on distinct visual features, such as oval or rectangular ochre-colored shapes. The model leverages RGB bands to detect active kilns, while the addition of NIR, SWIR, and NDVI metrics enhances its ability to identify abandoned kilns, often concealed by vegetation, and reduces false positives.

The model achieved a precision of 0.90, a recall of 0.89, and an accuracy of 0.91 on the test set. Detected kiln centroids were highly accurate, with precise GPS coordinates matching their actual locations. Nationwide, the model identified 44,000 brick kilns in India for 2022. We benchmarked multiple models to optimize false positive reduction and improve technology classification. Building on these results, we applied the model to neighboring countries in the Indo-Gangetic Plain (IGP), spanning Pakistan, Bangladesh, and parts of Nepal, which also contribute significantly to the brick kiln industry, identifying approximately 20,000 kilns in 2022.

Beyond location mapping, we are generating annual gridded emission maps for CO2 and pollutants such as PM2.5, black carbon, and NOx. These maps provide time-series insights into emission trends, reduce uncertainties in carbon and pollutant emissions, quantify reductions achieved through cleaner technologies, and identify regional hotspots. By focusing on underregulated, high-emission sectors like brick kilns, this study offers critical insights for targeted mitigation strategies and sustainable urban planning. It equips policymakers with tools to evaluate regulations and demonstrates the feasibility of using Sentinel-2 imagery for cost-efficient, large-scale monitoring. 

How to cite: Goldmann, C., Arora, S., Zhou, C., Ciais, P., Gieseke, F., Tibrewal, K., and Phuleria, H.: CHETNA-Brick Sector: Estimating GHG and Pollutant Emissions from Brick Kilns in India Using Sentinel-2 Imagery and Deep Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11020, https://doi.org/10.5194/egusphere-egu25-11020, 2025.

EGU25-11062 | Posters on site | AS3.43

Green4Clim: Making the University of Zurich a real-world laboratory for climate change mitigation 

Raleigh Grysko, Maria Santos, and Eugenie Paul-Limoges

Universities and other institutions are currently faced with the goal of utilizing responsible practices regarding carbon dioxide (CO2) emissions. At the University of Zurich, the initiative to start real-world laboratories inspired innovations and science-based studies to explore additional options for mitigating CO2 emissions from operations through both direct and indirect vegetation processes, i.e. direct sequestration and reduction in emissions from reduced energy consumption of buildings due to the shading and cooling effect of trees, respectively. As of now, it is unknown how much CO2 is sequestered by the vegetation on the University of Zurich Irchel campus and also which vegetated areas are possibly emitting CO2 (through soil respiration, decomposition, etc.). Within this initiative, the Green4Clim project monitors and quantifies the current CO2 sources and sinks on the Irchel campus and, in close collaboration with campus gardeners,determines options to optimize CO2 sequestration and cooling on campus. In this presentation, we present the preliminary results on (i) establishing a protocol for measuring direct and indirect effects of trees and other vegetation carbon sequestration, shading and cooling effects, and (ii) the measurements obtained on CO2 sources and sinks of natural areas on Irchel campus. Our measurements were taken at the leaf and soil level with a portable photosynthesis system and soil chamber systems to create an inventory of measurements, focusing on the four dominant tree species, green roofs, and the three dominant land cover types on campus (shrubs/bushes, short grass, and tall grass). Through this experiment we will identify the most suitable places and the most efficient plant species and communities to sequester CO2 on Irchel campus and suggest a management strategy that maximizes the CO2 reduction of the University of Zurich Irchel campus.

How to cite: Grysko, R., Santos, M., and Paul-Limoges, E.: Green4Clim: Making the University of Zurich a real-world laboratory for climate change mitigation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11062, https://doi.org/10.5194/egusphere-egu25-11062, 2025.

EGU25-11561 | Orals | AS3.43

Steps towards improved inverse modelling of GHG fluxes: recent work within ITMS 

Christoph Gerbig, Rachael Akinyede, Ðanilo Custódio, Michał Gałkowski, David Ho, Fabian Maier, Saqr Munassar, Yang Xu, and Thomas Koch

Within the Integrated Greenhouse Gas Monitoring System for Germany (ITMS), the main aim is to provide regular, accurate, observation-based emission estimates that will enhance the transparency in GHG emission reporting needed to build the necessary trust on the path to net zero emissions. Reliable inverse atmospheric transport modelling using atmospheric GHG observations is one of the main ingredients for this. However, multiple studies have shown rather large differences in GHG flux estimates from regional inverse modelling, related to differences in implementation of atmospheric transport processes such as vertical mixing and convective transport. Within the ITMS-M (modelling) project, a number of approaches are taken towards either improving atmospheric transport and mixing, or to reduce the impact of related uncertainties in atmospheric transport. These approaches include the utilization of vertical profiles from ICOS tall towers (using stable layer tracer enhancements during night time, expressed as partial columns as input to the inversion), profile information from IAGOS and mixing height information from ceilometer networks (diagnosing/correcting for uncertainties in daytime vertical mixing), but also multi-tracer inversions using correlated model-data-mismatch errors (utilizing independent knowledge on e.g. Radon surface fluxes in a Rn-CH4 inversion). We will give an overview of these approaches and current status of their developments within ITMS.

How to cite: Gerbig, C., Akinyede, R., Custódio, Ð., Gałkowski, M., Ho, D., Maier, F., Munassar, S., Xu, Y., and Koch, T.: Steps towards improved inverse modelling of GHG fluxes: recent work within ITMS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11561, https://doi.org/10.5194/egusphere-egu25-11561, 2025.

EGU25-11782 | ECS | Posters on site | AS3.43

Near-real-time CO2 traffic emission maps of 10 European cities based on high-resolution GPS-based data 

Qinren Shi, Philippe Ciais, Xavier Bonnemazion, Rohith Teja Mittakola, Nicolas Megal, and Chuanlong Zhou

On-road transportation is one of the major contributors to energy consumption and CO2 emissions in global megacities, and high-resolution CO2 traffic emission maps are needed to analyze emission patterns. In this study, commercial GPS-based data provides hourly, road-specific information on vehicle speed and traffic volume, and machine learning models are employed to address data gaps and transform sample counts into real traffic flux. Combined with COPERT, we developed on-road transportation CO2 emission maps for 10 selected cities in France, Germany, and the Netherlands. Our analysis offered insights into annual, per capita, and area-specific emissions for each city. Spatial emission patterns reflect urban structures and commuting behaviors, with cities such as Paris exhibiting concentrated hotspots along its ring road, whereas Berlin demonstrates a more uniform spatial distribution. Temporal variations reveal distinct weekly and seasonal trends, with more significant reductions during holidays and summer in French cities compared to German and Dutch cities. This approach enhances the spatial and temporal characterization of CO2 emissions in on-road transportation compared to the previous method used in Carbon Monitor, indicating the potential of GPS-based data for supporting future efforts in emission monitoring and developing emission reduction policies.

How to cite: Shi, Q., Ciais, P., Bonnemazion, X., Mittakola, R. T., Megal, N., and Zhou, C.: Near-real-time CO2 traffic emission maps of 10 European cities based on high-resolution GPS-based data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11782, https://doi.org/10.5194/egusphere-egu25-11782, 2025.

EGU25-12856 | ECS | Orals | AS3.43

Inverse modelling of N2O fluxes over Europe: An EYE-CLIMA initiative 

Nalini Krishnankutty, Rona Thompson, Antoine Berchet, Wilfried Winiwarter, Stephan Henne, and Ute Karstens

Nitrous Oxide (N₂O) is a long-lived and highly potent greenhouse gas, recognized as the third most significant contributor to radiative forcing, with a substantial proportion of its emissions originating from a large area source, agricultural soils, due to the application of mineral fertilizer and livestock manure. As part of the Horizon Europe project EYE-CLIMA, we performed atmospheric inversions to improve the estimates of N2O fluxes across Europe at two spatial resolution scales. The first inversion, spanning the period from 2005 to 2023, was performed at a resolution of 0.5° × 0.5°. The second inversion, covering the period from 2018 to 2023, was carried out at a higher resolution of 0.2° × 0.2°. The method integrates the Community Inversion Framework (CIF) with the Lagrangian particle dispersion model, FLEXPART v11 (CIF-FLEXPART), to estimate N2O emissions using ground-based measurements of atmospheric N2O concentrations. Comprehensive prior N2O flux estimates were generated by incorporating monthly data from key source categories, including agriculture, other anthropogenic activities such as combustion, industry or waste treatment, biomass burning, natural soils, and ocean fluxes. For consistency, observed atmospheric concentrations of N2O were sourced from a newly harmonized dataset for Europe, compiled collaboratively by EYE-CLIMA and the Horizon Europe projects AVENGERS and PARIS.

Following the inversion, the modelled concentrations showed improved agreement with observations, capturing the seasonal cycle and increasing trend from 2005 onward. Statistical analyses revealed high correlations between modelled and observed concentrations at most stations. The N2O emissions from the inversion differ from the prior estimates in intensity and spatial distribution with increased emissions in regions of specifically high agricultural activity and reductions in other areas. Monthly flux variations exhibited a consistent seasonal cycle, with peak emissions occurring in early summer (May–June) and lower emissions during winter months. Across all years, total posterior emissions were lower than the prior estimates. While the phase of the seasonal cycle remained consistent from year to year, interannual variability in the amplitude was observed.

How to cite: Krishnankutty, N., Thompson, R., Berchet, A., Winiwarter, W., Henne, S., and Karstens, U.: Inverse modelling of N2O fluxes over Europe: An EYE-CLIMA initiative, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12856, https://doi.org/10.5194/egusphere-egu25-12856, 2025.

EGU25-13030 | ECS | Posters on site | AS3.43

 Evaluating ICON-ART’s Performance in Simulating Methane: A Benchmark Against aircraft observations, CAMS, and WRF Models 

Danilo Custódio, David Ho, Michał Gałkowski, and Christoph Gerbig

Methane (CH₄), a potent greenhouse gas, is a key player in atmospheric chemistry and climate forcing. Its spatial and temporal variability is driven by emissions, atmospheric transport, and chemical loss processes. Accurate modelling of CH₄ is essential for understanding its sources, sinks, and role in Earth’s energy budget. In this study, we evaluate the skill of forward methane simulations of ICON-ART (ICOsahedral Nonhydrostatic - Aerosols and Reactive Trace gases) implementation established at Max Planck Institute for Biogeochemistry in Jena. The ICON-ART model represents a cutting-edge atmospheric modelling system jointly developed by the consortium of German and Swiss institutes. Its proven capability to realistically simulate trace gases, aerosols, and chemical interactions makes it a versatile tool for regional-to-global atmospheric studies focusing on improving flux estimates of a variety of atmospheric compounds, including methane. This work was conducted within the framework of the ITMS project (Integrated Greenhouse Gas Monitoring System for Germany), designed to enable Germany to operationally monitor the source and sinks of the most import long-lived greenhouse gases.

In the study, we evaluate the performance of the ICON-ART simulations set over the ICON-EU domain at 7 km horizontal resolution and compare their results other, more established modelling systems, including CAMS (Copernicus Atmosphere Monitoring Service) inversion optimized product (v21r1), CAMS reanalysis (EGG4) and the WRF-GHG (Weather Research and Forecasting with GHG module) model run at 5 km horizontal resolution. Both ICON-ART and other models include realistic realizations of anthropogenic emissions, natural fluxes, and boundary conditions that allow for realistic representation of atmospheric methane. We further compare all model results to in-situ airborne observations performed with HALO (High Altitude and LOng Range) during CoMet Campaign in May-June 2018, providing high-resolution CH₄ measurements, including vertical profiles spanning from the planetary boundary layer (PBL) to the low stratosphere (LS). The comparability of the models was ensured through collocated data analysis and performance metrics. These methodological frameworks minimize biases arising from resolution differences, enabling a fair assessment of the models’ capabilities.

The results reveal that ICON-ART is able to capture uplift transport and strong vertical mixing processes with remarkable fidelity. Displaying only 1.8 ppb mean bias error (MBE) for CH4, it outperforms both WRF and global CAMS products, across the used metrics. In the PBL, ICON-ART resolves small-scale CH₄ variability better than CAMS and WRF. Similarly, in the free troposphere, ICON-ART successfully simulates CH₄ transport and mixing, aligning closely with aircraft observations. Notably, ICON-ART shows better agreement in the LS, which is linked to improved stratosphere-troposphere exchange processes, but also underlines the importance of realistic lateral boundary conditions.

How to cite: Custódio, D., Ho, D., Gałkowski, M., and Gerbig, C.:  Evaluating ICON-ART’s Performance in Simulating Methane: A Benchmark Against aircraft observations, CAMS, and WRF Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13030, https://doi.org/10.5194/egusphere-egu25-13030, 2025.

EGU25-13577 | ECS | Orals | AS3.43 | Highlight

CHETNA-Overview: City-wise High-resolution Carbon Emissions Tracking and Nationwide Analysis 

Chuanlong Zhou, Philippe Ciais, Arnab Jana, Ahana Sarkar, Rohith-Teja Mittakola, Kushal Tibrewal, Kounik De Sarkar, Abhinav Sharma, Vipul Parmar, Fouzi Benkhelifa, Biqing Zhu, Clément Goldmann, and Harish Phuleria

We present the CHETNA (City-wise High-resolution Carbon Emissions Tracking and Nationwide Analysis) project, an innovative framework designed to generate near real-time high-resolution carbon emissions data for 100 Indian cities across five major sectors: power, traffic, residential, industrial, and aviation. Utilizing advanced technologies including artificial intelligence, large-scale open data scraping, satellite imagery, sophisticated energy models, and field surveys, CHETNA will address critical gaps in emissions tracking and modeling at the city level. CHETNA’s methodologies focus on regions with limited official datasets and inadequate high-resolution data, providing essential insights to support urban planning, climate mitigation, and sustainable urbanization efforts both in India and globally.

India, the world’s third-largest emitter of greenhouse gases (GHGs), plays a pivotal role in global climate mitigation efforts. Its rapidly urbanizing population, expanding economy, and coal-dominated energy structure present both challenges and opportunities for sustainable development. To meet its Paris Agreement commitments, India has pledged to reduce its GHG emissions intensity—emissions per unit of GDP—by 33%–35% by 2030, relative to 2005 levels. However, critical data gaps persist, particularly at the city level, hindering effective city-specific climate action and data-driven decision-making in India’s urban decarbonization. 

To ensure a robust and scalable system for sectoral high-resolution CO₂ emission tracking, CHETNA employs an integrated workflow that combines GHG emission inventories and high-resolution sectoral activity modeling. For sectors such as power, large industrial, and aviation, where reliable national or regional emission inventories are available from open data sources, we developed sophisticated downscaling models to generate gridded emission maps based on those open-source datasets. For sectors lacking comprehensive emission inventories, such as traffic and residential, we adopted a bottom-up approach. Activity models were developed for each sector using machine learning, field-collected data (e.g., traffic sensor and field survey data), and satellite imagery. These activity models were then coupled with advanced emission models. For instance, a fleet-speed-emission model was developed for the traffic sector, while a building-climate-energy model was implemented for the residential sector. In addition to CO₂ emissions, CHETNA provides air pollutant co-emissions by integrating detailed activity data with pollutant-specific emission factors. This approach allows for the assessment of air quality benefits resulting from GHG mitigation efforts, highlighting the co-benefits of reduced air pollutants. 

The dataset generated with the CHETNA project enables policymakers to develop city- and sector-specific strategies, contributing to India's sustainable urban development. Its sectoral high-resolution data would provide insights for guiding urban planning, air pollutant reduction, optimizing transportation systems, enhancing energy efficiency, and implementing effective industrial regulations. Representing a significant advancement in urban GHG emissions monitoring, CHETNA also offers a scalable and replicable framework for other counties or cities facing similar challenges. 

This presentation provides an overview of the CHETNA project, outlining its scope, general concept, workflow design, and simplified methodologies for each sector. At EGU25, we will also present detailed sectoral methodologies and results, including traffic, residential, power, and small industrial sectors.

How to cite: Zhou, C., Ciais, P., Jana, A., Sarkar, A., Mittakola, R.-T., Tibrewal, K., De Sarkar, K., Sharma, A., Parmar, V., Benkhelifa, F., Zhu, B., Goldmann, C., and Phuleria, H.: CHETNA-Overview: City-wise High-resolution Carbon Emissions Tracking and Nationwide Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13577, https://doi.org/10.5194/egusphere-egu25-13577, 2025.

EGU25-14671 | Posters on site | AS3.43

Prospects of scientific monitoring ,verification and reporting to support national and subnational GHG inventories 

Andreas Ibrom, Konstantin Kissas, Anastasia Gorlenko, Ziqiong Wamg, Susanne Wiesner, and Charlotte Scheutz

Scientific monitoring, verification and reporting (MRV) is necessary to independently examine the quality of national greenhouse gas (GHG) inventories as assessment methods are inherently uncertain including systematic effects from biased input information and lack of knowledge. The atmospheric research community develops observation systems to monitor the large-scale net GHG exchange with remote sensing and tall tower based concentration field measurements and atmospheric transport model inversion techniques. Because the spatial and temporal scales of these approaches are too coarse for small nations and even more so for local government districts, we used an alternative direct method to estimate the GHG budget of an agricultural landscape in Denmark, the tall tower eddy covariance method. In the presentation, we will use this case study to illustrate the strengths and limitations of net GHG flux measurements to test against GHG inventories.

We compared our one year’s data set of continuous GHG (CO2, N2O and CH4) flux measurements  with the estimates from IPCC based emission methods that were refined for the Danish agricultural landscape. We calculated GHG emissions and their uncertainties using the IPCC methods and propagated those to annual estimates. Likewise, we estimated the uncertainty for annual budgets from turbulent flux measurements including a number of factors that are deemed most important for the quality of net flux estimates.

While the emission estimates for the non-CO2 GHG were at least similar, the IPCC inventory characterized the area as a net GHG source, whereas the measured fluxes determined a large GHG sink, owing to an overwhelming CO2 uptake.

In our presentation, we will resolve this apparent contradiction and conclude on the strengths and limitation of MRV from scientific net GHG exchange approaches.

Acknowledgement:

We acknowledge funding by the Free Danish Research Council (DFF, grant number 1127-00308B) and the contribution of MSc. Victoria Abelenda and MSc. Isabel Lopez in their MSc. Project “Comprehensive Assessment of Greenhouse Gas Emissions  (N2O, CO2, CH4) in Agricultural Practices: A Case Study from a Rural Area in Denmark”, Inst. of Resouce and Environmental Engineering, Technical University of Denmark (DTU) Kgs. Lyngby, Denmark (2024).

How to cite: Ibrom, A., Kissas, K., Gorlenko, A., Wamg, Z., Wiesner, S., and Scheutz, C.: Prospects of scientific monitoring ,verification and reporting to support national and subnational GHG inventories, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14671, https://doi.org/10.5194/egusphere-egu25-14671, 2025.

EGU25-14965 | Orals | AS3.43

Public-Private Partnerships in Climate System Observations  

Vanda Grubišić and Colm Sweeney

Systematic – regular and routine – observations are vital for understanding and monitoring the Earth climate system. Systematic observation networks, traditionally built and operated by the public sector, provide relevant data that inform climate models and respective pathways, forecasts, products and services. Critical in that regard, in particular, are high precision, accurate, and comprehensive greenhouse gas measurements. Initiatives for enhancing such networks and observations for scaling up climate data collection and monitoring are important, as is doing this in a sustainable manner by leveraging opportunities and advancing cooperation though public-private partnerships. This presentation highlights recent NOAA initiatives in that regard, including recent partnerships with United Airlines and with Maersk for data collection from commercial aircraft and commercial shipping vessels. 

How to cite: Grubišić, V. and Sweeney, C.: Public-Private Partnerships in Climate System Observations , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14965, https://doi.org/10.5194/egusphere-egu25-14965, 2025.

EGU25-15002 | ECS | Posters on site | AS3.43

Study on the influence of the origin region on the relationship between carbon dioxide and methane concentrations in South Korea 

Jaemin Kim, Yun Gon Lee, Sunju Park, and Ho-Yeon Shin

Greenhouse gases (GHGs) are the main cause of climate change, and their concentrations are steadily increasing due to continuous emissions from anthropogenic activities. To establish effective carbon emission reduction policies and mitigate climate change, monitoring changes in atmospheric GHG concentrations and identifying their origin regions is essential. In this study, we analyzed the regional characteristics of carbon dioxide (CO2) and methane (CH4) at the Global Atmospheric Watch (GAW) stations (AMY, GSN, and ULD) in South Korea and investigated regional differences in the relationship between the two substances. We also explored the relationship between the regional differences and the source regions of greenhouse gases. The STILT mode (a Lagrangian dispersion model) and the EDGAR (an anthropogenic emission dataset) were used to identify the source regions of GHGs. The relationships (correlation coefficient and ratio) between CO2 and CH4 at three stations showed regional differences (GSN > ULD > AMY). It was investigated that these differences were caused by differences in the characteristics of major airflow patterns and emission sources that affect CO2 and CH4 concentration changes in the corresponding regions. The results of this study can help identify the causes of regional greenhouse gas concentration changes.

How to cite: Kim, J., Lee, Y. G., Park, S., and Shin, H.-Y.: Study on the influence of the origin region on the relationship between carbon dioxide and methane concentrations in South Korea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15002, https://doi.org/10.5194/egusphere-egu25-15002, 2025.

EGU25-15020 | Posters on site | AS3.43

Toward Monitoring Greenhouse Gas Emissions from National to Regional and Urban Scales 

Hengmao Wang, Fei Jiang, and Shuzhuang Feng

Monitoring and verifying anthropogenic greenhouse gases (GHG) Emissions at high spatiotemporal resolution with observation-based evidence is desirable for climate policymakers. A multiple-scale nested GHG assimilation system, named GCASv3, was developed for quantifying anthropogenic GHG emissions at high spatiotemporal resolution. GCASv3 uses a four level nested scheme and consists of one global module and one regional module. The global model is capable of assimilating XCO2 and XCH4 data to infer global CO2 flux and CH4 emissions at 10x10 resolution, while the regional module is able to assimilate ground and satellite GHG observations to quantify anthropogenic GHG emissions on national, regional and urban scales at 27km, 9km and 1km resolution respectively. This presentation describes briefly the framework and the major components of GCASv3. Anthropogenic CO2 emissions and CH4 emissions inferred by GCASv3 at different scales are presented and discussed.

How to cite: Wang, H., Jiang, F., and Feng, S.: Toward Monitoring Greenhouse Gas Emissions from National to Regional and Urban Scales, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15020, https://doi.org/10.5194/egusphere-egu25-15020, 2025.

EGU25-15759 | ECS | Orals | AS3.43

Assessing European HFC Emissions Using Inverse Modelling Systems 

Helene De Longueville, Daniela Brito Melo, Alice Ramsden, Alison Redington, Alexandre Danjou, Peter Andrews, Joseph Pitt, Brendan Murphy, Matthew Rigby, Stephan Henne, Alistair Manning, and Anita Ganesan and the other members of the PARIS team

Hydrofluorocarbons (HFCs) are potent greenhouse gases that contribute substantially to climate change. Their emissions are rapidly evolving due to changes in production and use that are driven by the Kigali Amendment to the Montreal Protocol and regional regulations. Atmospheric data and inverse modelling systems can be valuable for evaluating the effectiveness of these controls and the emissions reported to the United Nations Framework Convention on Climate Change (UNFCCC). Currently in Europe, the United Kingdom and Switzerland include atmospheric top-down emission estimates as part of their National Inventory Reports to the UNFCCC, and now the Horizon Europe project Process Attribution of Regional emISsions (PARIS) aims to expand similar inventory evaluation to several additional European countries. 

In this PARIS study, we derived HFC emissions for north-western Europe from 2012 to 2023 using the NAME transport model and three Bayesian inversion systems (InTEM, ELRIS, RHIME), focusing on HFC-134a, HFC-143a, HFC-32, HFC-125, HFC-23, HFC-152a, HFC-227ea, HFC-236fa, HFC-245fa, HFC-365mfc, and HFC-4310mee. Our results indicate an overall decline in HFC emissions in north-western Europe, broadly consistent with European F-gas regulations. Derived emissions trends are compared with National Inventory Reports, highlighting discrepancies. Moreover, we explore the driving factors behind these trends. These findings contribute to understanding emissions trends and improving inventory evaluations in Europe.

How to cite: De Longueville, H., Brito Melo, D., Ramsden, A., Redington, A., Danjou, A., Andrews, P., Pitt, J., Murphy, B., Rigby, M., Henne, S., Manning, A., and Ganesan, A. and the other members of the PARIS team: Assessing European HFC Emissions Using Inverse Modelling Systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15759, https://doi.org/10.5194/egusphere-egu25-15759, 2025.

EGU25-16572 | ECS | Posters on site | AS3.43

Significant Overestimation in Anthropogenic Methane Emissions in China 

Shuzhuang Feng, Fei Jiang, Hengmao Wang, and Yongguang Zhang

China, as the largest contributor to global anthropogenic methane (CH4) emissions, has pledged to reduce its global CH4 emissions by 30% in 2030 compared to 2022 levels. Accurate estimation of CH4 emissions is crucial for climate prediction and mitigation policies but poses a significant challenge for methods relying solely on economic statistics and emission factors. In this study, we developed a regional carbon assimilation system (RegGCAS) to integrate TROPOMI XCH4 observations for inferring daily CH4 emissions across China. Our estimated national total CH4 emission for 2022 was 45 Tg·yr⁻¹, approximately 35% lower than the widely used EDGARv8 inventory (prior estimate). Notable reductions were primarily observed in Northern China, with only sporadic increases in Shanxi Province, which contributes one-third of China's coal production. Increases were primarily concentrated in the Sichuan Basin, the southeast coastal provinces, and Heilongjiang Province in Northeast China. The optimized CH4 emission estimate exhibited more pronounced seasonal variations, with a significant decrease in emissions during winter. However, constraints on emissions in summer were limited due to the lack of observational data. Posterior simulations demonstrated better consistency with both TROPOMI XCH4 observations and ground-based observations. These findings enhance our understanding of the spatiotemporal patterns of CH4 emissions in China.

How to cite: Feng, S., Jiang, F., Wang, H., and Zhang, Y.: Significant Overestimation in Anthropogenic Methane Emissions in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16572, https://doi.org/10.5194/egusphere-egu25-16572, 2025.

The presence of CO2 in the atmosphere facilitates the maintenance of adequate levels of heat, which is essential for the establishment and sustenance of life on Earth. Although its concentration has varied dramatically throughout the planet's history, recent levels of atmospheric CO₂ are the result from a delicate balance among processes such as volcanism, weathering, photosynthesis, respiration and combustion. However, extensive use of fossil fuels has altered this balance causing atmospheric CO2 concentrations to rise, thereby intensifying global warming and accelerating climate change

While relatively few countries in the intertropical region release substantial amounts of CO2, nations in the northern hemisphere have been the primary contributors to CO₂ emissions over the past centuries, largely due to industrialization. Since the Industrial Revolution, urban development has concentrated several people around heavily industrialized cities, which have become central drivers of climate change. Global atmospheric circulation facilitates the rapid dispersion of CO₂ emissions originating from tropical latitudes throughout the troposphere. In contrast, emissions from mid- to high-latitude regions persist longer on a regional scale. Consequently, the latitude of CO₂ emissions significantly influences their climatic effects, with high-latitude emissions remaining in the atmosphere for longer time.  On the other hand, growing urban areas in the transitional mid-latitude regions are particularly vulnerable to the impacts of climate change, with Mediterranean cities being especially susceptible to extreme events. These include more frequent heatwaves, rising sea levels, droughts, and intense rainfall, all of which pose significant threats to infrastructure, public health, and urban ecosystems. Moreover, rising temperatures enhance social and economic inequalities, underscoring the urgent need for resilient and sustainable adaptation strategies. 

This study addresses the rationale for and development of a research infrastructure aimed at monitoring atmospheric CO₂ and its latitudinal variation within the Mediterranean region. The objective is to assess the impacts of actions taken to reduce anthropogenic CO₂ emissions as outlined in the European Green Deal. 

The proposed infrastructure is designed to collect and disseminate data for a comprehensive examination of the causes of latitudinal and temporal variations in atmospheric CO₂ across a north-south transect from the Alpine glaciers in Valle d’Aosta to the island of Lampedusa, both located in Italy. This system includes 12 automatic monitoring stations equipped to measure the concentration and isotopic composition of carbon and oxygen in atmospheric CO₂. Extensive research highlights the importance of monitoring carbon isotopes (e.g., ¹³C, ¹²C) to identify emission sources, as well as triple oxygen isotope ratios (¹⁶O, ¹⁸O, and ¹⁷O) to trace the fate of CO₂ within the interconnected carbon and water biogeochemical cycles.

The network’s high-frequency acquisition capability (minute intervals) enables near real-time evaluation, facilitating the identification and characterization of diverse CO₂ sources and the apportionment of their emissions. 

How to cite: Di Martino, R. M. R. and Gurrieri, S.: Monitoring Atmospheric CO₂ in the Mediterranean: A Strategic Infrastructure for Climate Action and Latitudinal Impact Assessment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16829, https://doi.org/10.5194/egusphere-egu25-16829, 2025.

EGU25-16892 | ECS | Orals | AS3.43

A Hybrid Approach to Carbon Monitoring in India by combining Satellite-based NO2 and CO2 mixing ratios 

Jithin Sukumaran, Dhanyalekshmi Pillai, Abhinav Dhiman, and Vishnu Thilakan

Quantifying carbon emissions in the Indian region is fraught with uncertainties, largely due to the limited availability of atmospheric trace gas observations and robust techniques. Atmospheric inverse modeling approaches, though highly potential, are often constrained by sparse observational datasets over India. To address these challenges, this study investigates a novel data-driven methodology that leverages satellite-based NO2 and CO2 concentrations for plume detection and associated emission quantification. Specifically, we utilize highly accurate and precise NO2 measurements from the TROPOMI instrument onboard Sentinel-5P to identify and trace emission hotspots, such as thermal power plants and densely populated urban centers, which significantly contribute to regional emissions. Using this NO2-driven plume detection as a proxy, we explore the potential of atmospheric dry-air column CO2 concentrations to quantify hotspot emissions. The present study utilises the modeled dry-air column CO2 concentrations, which observations can later replace. The focus is given to illustrate a methodology that can combine both  NO2 and CO2 concentrations derived from satellite instruments to infer the spatial distribution of  CO2 emission over a region that is rapidly evolving and industrialized, like India. The above task is particularly in preparation for upcoming satellite missions like CO2M, which will offer co-located NO2 and CO2 observations that can be utilized for cost-effective solutions for carbon monitoring. Hence, the study outcome will not only improve our understanding of regional emissions but also establish a framework for leveraging future satellite missions to assist in establishing carbon emission reduction policies.

How to cite: Sukumaran, J., Pillai, D., Dhiman, A., and Thilakan, V.: A Hybrid Approach to Carbon Monitoring in India by combining Satellite-based NO2 and CO2 mixing ratios, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16892, https://doi.org/10.5194/egusphere-egu25-16892, 2025.

EGU25-17019 | ECS | Posters on site | AS3.43

A scalable approach to high-resolution, bottom-up GHG emission inventories using open data 

Sebastian Block, Veit Ulrich, Maria Martin, Kirsten von Elverfeldt, Kenneth Murai von Buenau, Pia Haas, Robert Maiwald, André Butz, and Sanam N. Vardag

Targeting and tracking climate change mitigation efforts requires accurate bottom-up inventories of GHG emissions, verified by independent atmospheric measurements. So far, most policy decisions have been based on annual emission inventories at national and city scales. Inventories with higher resolution in both space (sub-city) and time (daily to hourly), while generally more uncertain, have major advantages. First, they are a key input to inverse modelling of emission sources from atmospheric measurements, which offers a semi-independent approach to verify bottom-up estimates. Second, they can serve as simulation tools to assess the impact of specific interventions (from policy to industrial standards and household behavior) on GHG emissions and measured atmospheric concentrations. Third, by offering more localized emission estimates almost in real time, they may act as more powerful motivators of behavioral and policy change when used to communicate and track climate action. 

Here we present a simple approach to develop bottom-up inventories of carbon dioxide emissions from road traffic (at street level) and residential space heating (in a 100-m grid) using crowd-sourced data from OpenStreetMap and other publicly available data sources. Our approach can be easily scaled to all of Germany and, with some modifications, can be tailored to a wide range of contexts and applications. We demonstrate the approach for the cities of Mannheim and Heidelberg, in the Rhine-Neckar Metropolitan Area in Germany. 

Emissions from road traffic are derived from multiplying estimates of average daily traffic volume – based on road type information, number of lanes, and population density – by speed- and fuel-dependent emission factors and data about the national vehicle fleet composition. Space heating emissions rely primarily on gridded data from the 2022 German census on population density, living space per capita, heating energy carriers, and building age.

We validate our traffic volume estimates with independent traffic count data and compare our emission estimates to available inventories. Road traffic emissions in the Rhine-Neckar region were 1.6% higher than TNO estimates for the region (Super et al. 2021), a widely used inventory of disaggregated emission in Europe. Our residential space heating emissions estimates were slightly lower than estimates from emissions inventories for the cities of Mannheim and Heidelberg (12% and 8%, respectively), largely attributable to the type of emission factors used in the calculations. 

How to cite: Block, S., Ulrich, V., Martin, M., von Elverfeldt, K., Murai von Buenau, K., Haas, P., Maiwald, R., Butz, A., and Vardag, S. N.: A scalable approach to high-resolution, bottom-up GHG emission inventories using open data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17019, https://doi.org/10.5194/egusphere-egu25-17019, 2025.

EGU25-17412 | Orals | AS3.43

Beyond Bias: Radon-Based Technique for Reducing Uncertainty in Greenhouse Gas Verification Frameworks 

Dafina Kikaj, Craig Lils, Scott D. Chambers, Grant Forster, and Arnoud Frumau

The accuracy of greenhouse gas (GHG) emission estimates is significantly limited by uncertainties in atmospheric transport models (ATMs). These uncertainties largely arise from difficulties in accurately representing sub-grid turbulence and mixing processes. Furthermore, the use of modelled meteorological data to filter observations before inversion frameworks results in the exclusion of 40–75% of continuous GHG measurements, thereby reducing the reliability of emission estimates.

To overcome these challenges, we propose the use of radon measurements - a naturally occurring radioactive noble gas with well-characterised sources and sinks. Radon will be used as a metric to define atmospheric mixing classes, providing a novel approach to validate ATM performance and address its inherent uncertainties. These mixing classes, which reflect varying atmospheric stability conditions, offer a valuable benchmark for evaluating model parameterisations and meteorological inputs.

Our study utilises radon measurements from the Weybourne Atmospheric Observatory (UK) and Cabauw Tower (Netherlands) to assess the reliability of meteorological inputs and parameterisation in ATMs. Preliminary results demonstrate that radon-derived mixing classes can reduce biases in data filtering while improving the representation of atmospheric transport dynamics. This innovative method helps to bridge gaps in current inversion frameworks, enabling more accurate GHG emission estimates and supporting the development of evidence-based climate policies.

How to cite: Kikaj, D., Lils, C., Chambers, S. D., Forster, G., and Frumau, A.: Beyond Bias: Radon-Based Technique for Reducing Uncertainty in Greenhouse Gas Verification Frameworks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17412, https://doi.org/10.5194/egusphere-egu25-17412, 2025.

EGU25-17986 | ECS | Posters on site | AS3.43

Addressing uncertainties in top-down estimates of national-scale greenhouse gas emissions across different inversion systems 

Daniela Brito Melo, Alice Ramsden, Hélène De Longueville, Alison Redington, Alexandre Danjou, Peter Andrews, Brendan Murphy, Joseph Pitt, Eric Saboya, Matthew Rigby, Lukas Emmenegger, Alistair Manning, Stephan Henne, and Anita Ganesan

As part of the current international effort to limit global warming, signatories to the Paris Agreement are required to quantify their greenhouse gas (GHG) emissions. Former Kyoto Annex I countries thus report their emissions  annually to the United Nations Framework Convention on Climate Change (UNFCCC) . This assessment allows countries to evaluate their progress in reducing GHG emissions and their compliance with existing agreements.
The general approach to quantifying GHG emissions at the national level is to use activity data and emission factors  (bottom-up method). An independent  quantification can be achieved with inverse modelling, which makes use of an a priori estimate, atmospheric transport models (ATM), and atmospheric measurements of GHG concentrations (top-down method). However, the accuracy and uncertainty of inverse estimates are highly dependent on several parameters and modelling choices. Consequently, inter-model variability can be significant, potentially limiting the use of this technique in policy-relevant discussions.
A representative quantification of GHG emissions based on inverse modelling requires an in-depth understanding of different inverse model estimates, their uncertainties and model limitations.  An intercomparison of three inverse methods and a suite of sensitivity tests were performed. This exercise considered two fluorinated gases (HFC-143a and PFC-218), which are potent GHGs with very different emission characteristics (diffuse versus point source). Both are covered under the European F-gas regulation. Additionally, HFC-143a is expected to be phased-down under the Kigali Amendment to the Montreal Protocol.
We found that top-down estimates for Central and Western European countries are most sensitive to the ATM used. For gases with localised emission sources, such as PFC-218, the choice of a priori emissions and assigned model-data mismatch uncertainty are particularly relevant. For gases with widely distributed emission sources, such as HFC-143a, the emission estimates are more consistent and less sensitive to modelling choices. This detailed understanding of uncertainties in top-down estimates is then used to inform how inverse modelling can be used to support the reporting of halogenated GHG emissions at the national and European level.

How to cite: Brito Melo, D., Ramsden, A., De Longueville, H., Redington, A., Danjou, A., Andrews, P., Murphy, B., Pitt, J., Saboya, E., Rigby, M., Emmenegger, L., Manning, A., Henne, S., and Ganesan, A.: Addressing uncertainties in top-down estimates of national-scale greenhouse gas emissions across different inversion systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17986, https://doi.org/10.5194/egusphere-egu25-17986, 2025.

EGU25-18706 | ECS | Posters on site | AS3.43

A Standardised Procedure for Estimating Greenhouse Gas Baselines Using Radon-222 

Craig Lils, Dafina Kikaj, Edward Chung, Scott Chambers, Alan Griffiths, Franz Conen, Paul Fukumura-Sawada, and Paul Krummel

Top-down verification methods are crucial for ensuring confidence in the bottom-up approaches used to report greenhouse gas emissions. These methods are reliant on robust baseline estimates, which can be calculated via several methods using a combination of meteorological data, transport models, and tracers such as CO and radon-222. In particular, high-quality radon measurements have been shown to reliably and consistently identify baseline airmasses across the globe, due to radon’s unique properties as a terrestrial tracer. However, the methodology used in this process differs between studies, as a result of variations in the location (e.g. remote, coastal, terrestrial), altitude, and atmospheric features of each observation site, as well as the sensitivity of the instruments available at the time/location.

This study aims to provide a universal procedure with which to calculate baseline estimates of greenhouse gases using radon, accounting for differences between stations. To evaluate and adjust this procedure, data from the Kennaook/Cape Grim (Tasmania), Mauna Loa (Hawaii), Jungfraujoch (Switzerland), Mace Head (Ireland) and Monte Cimone (Italy) observatories will be assessed, encompassing a range of locations and altitudes. This will include analysis of a variety of greenhouse gases, to understand whether alterations in the technique are required when estimating baselines of different gases and highlight how features such as low pollution spikes of N2O or sudden pollution events of SF6 influence our ability to estimate their baseline levels. Furthermore, using back trajectories obtained from the FLEXPART atmospheric dispersion model and high-frequency trace gas observations at each site, modelled baseline estimates will be derived to provide a direct comparison to the radon methodology. In doing so, this research will provide an unambiguous procedure for future baseline estimates, increasing the accessibility of this technique and improving comparability between studies.

How to cite: Lils, C., Kikaj, D., Chung, E., Chambers, S., Griffiths, A., Conen, F., Fukumura-Sawada, P., and Krummel, P.: A Standardised Procedure for Estimating Greenhouse Gas Baselines Using Radon-222, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18706, https://doi.org/10.5194/egusphere-egu25-18706, 2025.

EGU25-19189 | ECS | Posters on site | AS3.43

High-resolution CO2 flux modelling on the building-scale using GRAMM/GRAL and in-situ measurements for the Paris metropolitan area 

Robert Maiwald, Hervé Utard, Michel Ramonet, Olivier Laurent, Theo Glauch, Hugo Denier van der Gon, Thomas Lauvaux, and Sanam N. Vardag

The city of Paris aims to reach net zero emissions by 2050, an ambitious target whose achievement will need to be verified. Atmospheric measurements of CO2 can provide independent information on the city emissions and therefore, play an important role in monitoring the effectiveness of emission reduction plans.   

To derive emissions from measured concentrations, an atmospheric transport model is needed. This model should cover long time periods to detect trends and emission patterns, and run at high-resolution to simulate the air flow around urban structures. We use GRAMM/GRAL to model CO2 transport over Paris at 10m resolution with a catalogue approach. The hourly occurring meteorological situation and its respective concentration field is selected from a catalogue of around 1000 precomputed meteorological conditions, which are representative of wind situations over Paris. The selection of the appropriate catalogue entry is based on minimizing differences to wind measurements in the modelling domain. Thus, long time series of concentration enhancement maps can be calculated with low computational costs. Our setup for Paris includes anthropogenic fluxes, biogenic fluxes from Sentinel-2-based VPRM, and boundary conditions derived from in-situ measurements to allow a direct comparison to the observed concentrations in the city. 

We compare the simulated CO2 concentrations to measurements for 2023 from the ICOS Cities project. The modelled signals generally capture the diurnal dynamics and agree with the measured CO2. There are certain meteorological conditions where GRAMM/GRAL fails to capture the measured signal. GRAMM/GRAL does not accurately capture meteorological situations with lower boundary layer heights which most often occur during nighttime and in winter. However, we present a method of estimating a time-dependent uncertainty using concentration distribution from multiple catalogue entries. This uncertainty can be used in an inversion.  

We determine the underlying emission patterns and analyse the importance of the resolution of the emission inventory for emission quantification and emission sector disaggregation. Such detailed sector-specific information can help to inform policymakers about progress towards reduction goals and the effectiveness of specific reduction measures. 

How to cite: Maiwald, R., Utard, H., Ramonet, M., Laurent, O., Glauch, T., Denier van der Gon, H., Lauvaux, T., and Vardag, S. N.: High-resolution CO2 flux modelling on the building-scale using GRAMM/GRAL and in-situ measurements for the Paris metropolitan area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19189, https://doi.org/10.5194/egusphere-egu25-19189, 2025.

EGU25-21706 | Posters on site | AS3.43

Enhancing Urban GHG Monitoring: Progress of the NIST test-bed system 

Israel Lopez-Coto, Tyler Boyle, Julia Marrs, Anna Karion, Kimberly Mueller, Annmarie Eldering, Hratch Semerjian, and James Whetstone

As the U.S. Metrology Institute, the National Institute of Standards and Technology (NIST) has responded to the measurements and standards challenge of monitoring, reporting, and verifying greenhouse gas (GHG) emissions from a broad range of sources, with an emphasis on urban environments, to: a) improve U.S. capabilities to measure GHG emissions accurately; b) demonstrate the capabilities of atmospheric urban monitoring networks (top-down or atmospheric measurement approaches) to determine quantitatively GHG fluxes from industrial, residential, transportation, power generation and other activities; c) complement such measurements with spatially explicit emissions modeling (bottom-up or emissions modeling) approaches based on socio-economic data; and d) demonstrate that the combination improves confidence in emission estimates while identifying areas of improvement. 

As part of these efforts, NIST established its first Urban Test Bed in Indianapolis, Indiana (the INFLUX Project) in 2010 with Purdue University, NOAA, and Penn State University collaborators. Additional testbeds were established in Los Angeles (2012) and the Northeast Corridor (2014) to test applicability of methodologies over a range of meteorological conditions and emissions profiles. In this talk, we summarize some of the results obtained where we demonstrated methodologies for biogenic emission and uptake processes estimation, network design and emissions quantification from dense tower-networks and aircraft measurements. In addition, we highlight current efforts to transfer the research to operations, facilitate the adoption of the techniques by developing lower cost monitoring stations, and promote transparency by consolidating the methods in open-source computational tools.

How to cite: Lopez-Coto, I., Boyle, T., Marrs, J., Karion, A., Mueller, K., Eldering, A., Semerjian, H., and Whetstone, J.: Enhancing Urban GHG Monitoring: Progress of the NIST test-bed system, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21706, https://doi.org/10.5194/egusphere-egu25-21706, 2025.

EGU25-1822 | ECS | Posters on site | AS3.44

Global CO2 flux estimation using NISMON-CO2 and GOSAT for carbon cycle analysis improvement 

Suman Maity, Yosouke Niwa, Tazu Saeki, Yu Someya, and Yukio Yoshida

Accurate estimation of carbon dioxide (CO2) flux is essential for better understanding of the global carbon budget and its impact on climate changes, which would further suggest strategies for emission reduction. Bottom-up approaches, while fundamental, often face challenges in capturing the complexities of CO2 fluxes due to uncertainties in emission inventories and limitations in representing spatio-temporal variability of CO2 flux across diverse regions. In contrast, top-down methods, which combine simulations and observations with inverse modeling approach, offer powerful tools for dynamically constraining CO2 flux estimates. In comaparison to limited in-situ observations, satellite provides broader spatial coverage and therefore it is expected to enhance the flux estimation. In this study, we apply an integrated flux inversion framework NISMON-CO2 to a CO2 inversion with column-averaged dry air mole fraction of CO2 (XCO2), stored in NIES Level 2 product from the Greenhouse gases Observing SATellite (GOSAT) measurements and assess general features of the inversion results by comparing with an already established surface in-situ data inversion. NISMON-CO2 incorporates NICAM-TM (Nonhydrostatic ICosahedral Atmospheric Model-based Transport Model) for forward simulation, coupled with a 4DVar (four dimensional variational) data assimilation system for inverse computations. The 4DVar leverages the adjoint of NICAM-TM alongside the quasi-Newtonian optimization scheme. GOSAT, a Japanese satellite launched in 2009 by Japan Aerospace Exploration Agency (JAXA) in collaboration with the Ministry of the Environment (MOE) and the National Institute for Environmental Studies (NIES), provides high quality greenhouse gas mesurements from space to study their global distribution.

The prior flux data include four fluxes: fossil fuel emissions from GridFED (Gridded Fossil Emission Dataset), biomass burning emissions from Global Fire Emission Database (GFED), biospheric fluxes (gross primary production, respiration and land use change) from the Vegetation Integrative SImulator for Trace gases (VISIT) and air-sea exchange flux data from Japan Meteorological Agency (JMA). In this study, meteorological data that drive NICAM-TM is updated to the Japanese Reanalysis for Three Quarters of a Century (JRA-3Q) from JRA-55. Several numerical experiments are conducted for the period since April, 2009 till date to understand the performance of the inversion by analyzing the consistency of the resultant flux and concentration. This study illustrates the power of integrating satellite-derived products to provide comprehensive CO2 flux estimates, significantly enhancing our understanding of CO2 dynamics at global and regional scales.

Keywords: CO2 flux estimation, GOSAT, XCO2, 4DVar, NICAM, transport model, satellite data assimilation.

How to cite: Maity, S., Niwa, Y., Saeki, T., Someya, Y., and Yoshida, Y.: Global CO2 flux estimation using NISMON-CO2 and GOSAT for carbon cycle analysis improvement, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1822, https://doi.org/10.5194/egusphere-egu25-1822, 2025.

EGU25-2991 | ECS | Posters on site | AS3.44

Impact of Global Climatic Phenomena on the Carbon Exchange Dynamics of the Indian Terrestrial Biosphere 

Emili Singha Roy, Sajeev Philip, and Matthew S. Johnson

A better understanding of the country-scale terrestrial biospheric carbon dioxide (CO2) budget is crucial for formulating national climate policies aimed at limiting carbon emissions. The scarcity of continuous and dense regional CO2 measurements in India poses a significant challenge to accurately quantifying its carbon budget. Moreover, there are no observation-based studies investigating the regional carbon-climate interactions and carbon cycle response due to large-scale climatic events currently exist. In this study, we use the OCO-2 satellite atmospheric CO2 column (XCO2) retrievals, Solar Induced Fluorescence (SIF) and various observational data to study the Indian terrestrial biosphere’s response to large-scale climatic events such as El Niño-Southern Oscillation and Indian Ocean Dipole (IOD). The XCO2 data was assimilated in an ensemble of eight global top-down CO2 flux inverse models as part of the OCO-2 v10-Ext multi-model intercomparison project. We found a decrease in Indian terrestrial biosphere carbon uptake during El Niño and an increase during La Niña and positive IOD events. The increase in carbon uptake, driven by pIOD and La Niña events (~150 TgC) accounts for approximately one-quarter of India's annual fossil fuel carbon emissions. Studies indicate that the frequency of pIOD and La Niña events may rise under future global warming scenarios. This can potentially enhance the capacity of the Indian terrestrial biosphere to sequester more atmospheric carbon. Satellite-derived carbon-climate constraints over India as found in this study provide critical insights for developing effective strategies to achieve net-zero emissions in the future.

Acknowledgements: OCO-2 v10-Ext MIP modelers.

How to cite: Singha Roy, E., Philip, S., and S. Johnson, M.: Impact of Global Climatic Phenomena on the Carbon Exchange Dynamics of the Indian Terrestrial Biosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2991, https://doi.org/10.5194/egusphere-egu25-2991, 2025.

EGU25-3937 | ECS | Posters on site | AS3.44

Improved estimates of net ecosystem exchanges in mega-countries using GOSAT and OCO-2 observations 

Lingyu Zhang, Fei Jiang, Wei He, Mousong Wu, Jun Wang, Weimin Ju, Hengmao Wang, Yongguang Zhang, Stephen Sitch, and Jing M. Chen

Accurate national terrestrial net ecosystem exchange estimates are crucial for the global stocktake. Net ecosystem exchange estimates from different inversion models vary greatly at national scale, and the relative impacts of prior fluxes and observations on these inversions remain unclear. Here we estimate the net ecosystem exchange of 51 land regions for the 2017-2019 period, focusing on the 10 largest countries, using prior fluxes from 12 terrestrial biosphere models and XCO2 retrievals from GOSAT and OCO-2 satellites as constraints. The average uncertainty reduction for the 10 countries increases from 37% with GOSAT and 45% with OCO-2 to 50% with combined observations, indicating a trend towards robust estimates. At finer spatial scales, even with combined observations, the uncertainty reduction is only 33%, i.e., the prior flux dominates the estimates. This finding underscores the critical importance of integrating multi-source observations and refining prior fluxes to improve the accuracy of carbon flux estimates.

This study provides valuable insights for improving atmospheric inversions in the future, and offers a deeper understanding of the inversion results for the carbon cycle community. Additionally, the improved estimates of carbon fluxes for the 10 largest countries presented here can inform policy makers in making more informed decisions regarding climate and carbon management strategies.

How to cite: Zhang, L., Jiang, F., He, W., Wu, M., Wang, J., Ju, W., Wang, H., Zhang, Y., Sitch, S., and Chen, J. M.: Improved estimates of net ecosystem exchanges in mega-countries using GOSAT and OCO-2 observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3937, https://doi.org/10.5194/egusphere-egu25-3937, 2025.

EGU25-4002 | ECS | Orals | AS3.44

Can radon-222 help to improve methane emission estimates? Results from a dual-tracer inversion 

Fabian Maier, Christian Rödenbeck, Ute Karstens, Frank-Thomas Koch, Maksym Gachkivskyi, and Christoph Gerbig

Atmospheric transport models cause a large part of the uncertainty in top-down estimates of greenhouse gas fluxes derived by atmospheric inversions. In particular, deficits in transport models, such as inadequate description of vertical mixing in the planetary boundary layer (PBL), can lead to systematic biases in the flux estimates. While their quantification is critical for reliable flux estimation, such model biases and uncertainties are difficult to assess. One way of evaluating the performance of atmospheric transport models is to compare the modelled with the measured activity concentration of the radioactive noble gas radon-222 (Rn), provided that the Rn fluxes are sufficiently well known. Rn is produced by the decay of radium-226 in the soil and diffuses through the soil pores into the atmosphere. As the Rn lifetime (3.8 days) is comparable to the ventilation time scale of the PBL, atmospheric measurements of Rn activity concentrations provide sensitive information on vertical mixing.

By comparing the mismatch between the modelled (using the Stochastic Time-Inverted Lagrangian Transport model, STILT, and posterior flux estimates) and measured concentrations of methane (CH4) with that of Rn, we found significant correlations for many sites in Europe (the median correlation coefficient of all sites is r=0.6), indicating that a large part of the variability in the CH4 and Rn model-data mismatch can be explained by transport model errors. To exploit this information, we set up a joint inversion for (the targeted tracer) CH4 and Rn, taking into account realistic prior uncertainties and making use of the fact that the transport model error is correlated between the two gases. By comparing the results of the CH4-Rn inversion with those of a single-tracer CH4-only inversion, we assess the potential of Rn to improve CH4 emission estimates and highlight the importance of having accurate Rn flux maps. 

How to cite: Maier, F., Rödenbeck, C., Karstens, U., Koch, F.-T., Gachkivskyi, M., and Gerbig, C.: Can radon-222 help to improve methane emission estimates? Results from a dual-tracer inversion, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4002, https://doi.org/10.5194/egusphere-egu25-4002, 2025.

EGU25-4375 | ECS | Posters on site | AS3.44

Reconstruction and downscaling of historical land surface boundary conditions with Machine Learning 

Amirpasha Mozaffari, Stefano Materia, Vinayak Huggannavar, Lina Teckentrup, Iria Ayan, Etienne Tourigny, and Markus Donat

Understanding the role of land surface physics and biogeochemistry is crucial for improving climate models and weather prediction, particularly in the context of long-term variability, local feedbacks, and extreme events. Accurate boundary conditions—such as land cover (LC) and land use (LU)—are key to enhancing the realism of climate simulations by better representing land-atmosphere interactions that influence surface energy balance, and ecosystem processes. Moreover, they provide the substratum for a realistic representation of the terrestrial carbon cycle components, such as vegetation and soil biogeochemistry.

The CERISE project aims to produce high-resolution (1 km) LC and Leaf Area Index (LAI) datasets covering the period 1925–2020, contributing to novel reanalysis datasets (e.g., ERA6-Land), and seasonal forecasts (e.g., SEAS6). In the first phase, we reconstructed historical LU and LAI by leveraging machine learning (ML) models to downscale coarse-resolution LU datasets (LUH2f, HILDA+). Our workflow integrates multiple ML techniques, such as Random Forest and XGBoost, to train models over high-resolution LC and LAI satellite observations, while actively exploring methods to enhance both performance and interpretability. To capture monthly LAI variations from annual LU inputs, we developed an auxiliary network to model intra-annual variability. Initial results show promising performance in reconstructing LC and LAI across various test years and regions, demonstrating the feasibility and robustness of this ML-based approach for historical reconstructions.

Future phases, including the CONCERTO and TerraDT projects, will extend this work to generate consistent high-resolution LU datasets for the historical (1850-present) and future scenarios (present–2100), supporting CMIP7 climate simulations and scenario-based studies. These efforts will incorporate additional auxiliary data (e.g., elevation, soil types, climate indices) to improve feature representation and develop autoregressive models that account for long-term temporal dependencies and dynamic changes. Ultimately, our goal is to build a robust ML-based emulator for generating scalable, high-resolution land surface boundary conditions to support digital twin applications, thereby enhancing climate simulation and prediction capabilities.

How to cite: Mozaffari, A., Materia, S., Huggannavar, V., Teckentrup, L., Ayan, I., Tourigny, E., and Donat, M.: Reconstruction and downscaling of historical land surface boundary conditions with Machine Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4375, https://doi.org/10.5194/egusphere-egu25-4375, 2025.

EGU25-4834 | Orals | AS3.44 | Highlight

A decade of progress in carbon cycle science from NASA’s Orbiting Carbon Observatory (OCO-2 and OCO-3) missions 

Abhishek Chatterjee, Vivienne Payne, and Junjie Liu and the OCO-2 and OCO-3 Science and Project Team

As pathfinder missions, NASA’s Orbiting Carbon Observatory-2 (OCO-2) and its sister mission Orbiting Carbon Observatory-3 (OCO-3) have significantly expanded global CO2 observation coverage, providing high-quality atmospheric CO2 data at unprecedented spatial and temporal resolutions. Additionally, both missions retrieve solar-induced chlorophyll fluorescence (SIF), an indicator of photosynthetic activity. The OCO-2/3 team have achieved the extraordinary accuracy and precision requirement of delivering single-column CO2 retrievals with errors less than 1.0 ppm (less than 0.25%), making this data the "gold-standard" of remotely sensed atmospheric CO2. Both missions are now operating well beyond their designed lifetimes, showcasing technological excellence and demonstrating the value of space-based atmospheric CO2 measurements for improving our understanding of the carbon cycle at a variety of spatiotemporal scales, ie., from global carbon budgets to monitoring regional carbon cycle response to extreme events and tracking local emissions from urban areas and power plants. Our extended operations have allowed the project and science team to continuously improve all aspects of the missions, thus enabling the scientific community to investigate long-term trends in the carbon cycle and pursue policy-level applications that would not have been possible with only two-three years of data.

In this talk, we will synthesize the major scientific achievements and breakthroughs in applications from the scientific community using the OCO-2/3 data, emphasizing how the science achievements and requirements on the data accuracy have evolved during the last decade. We will also address current challenges and limitations of the data as well as discuss new scientific and application areas that this growing data record can advance. In the end, we will briefly touch on the synergistic scientific questions that can be addressed by combining the OCO-2/3 data record with the growing constellation of CO2 satellites, such as ESA's CO2M, JAXA's GOSAT-GW and others. 

How to cite: Chatterjee, A., Payne, V., and Liu, J. and the OCO-2 and OCO-3 Science and Project Team: A decade of progress in carbon cycle science from NASA’s Orbiting Carbon Observatory (OCO-2 and OCO-3) missions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4834, https://doi.org/10.5194/egusphere-egu25-4834, 2025.

The extensively distributed grasslands of the Qinghai-Tibet Plateau (QTP) play a vital role in the global carbon cycle and climate regulation. Gross primary productivity (GPP), a crucial indicator of ecosystem carbon sequestration capacity, remains highly uncertain partly due to neglecting the memory effects of environmental conditions (i.e., the influence of past states on current GPP). Moreover, existing models have difficulty in simultaneously handle multidimensional spatio-temporal data and dynamic climate responses, leading to simulation deviations and exacerbating uncertainties. Here, we integrated climate and vegetation data with time series characteristics and spatial characteristics to simulate the GPP of alpine grassland on the QTP, by developing a deep learning model CNN-LSTM that combined Convolutional Neural Networks (CNNs) and Long Short-Term Memory networks (LSTM). The conclusions were as follows: (a) The CNN-LSTM model effectively captured spatial patterns using CNNs and temporal dependencies with LSTMs, incorporating memory effects to consider the impact of past environmental conditions. This integration enhanced GPP simulation accuracy and improved the model's ability to capture interannual variability. (b) The training and optimization of the CNN-LSTM models revealed that the comprehensive memory effect length of GPP on historical climate and vegetation dynamics operates in a 4-month timescale, with the memory effects of GPP varied across environmental variables in both duration and intensity. (c) During 2001–2021, The mean annual GPP of the alpine grassland in QTP was 332.29 g C m-2 a-1, with a growth rate of 1.84 g C m-2 a-2. (d) Precipitation exhibited relatively longer durations and higher intensities compared to other factors, and the interannual variability of GPP was mainly influenced by water conditions. This study highlights the importance of integrating environmental memory into GPP modeling, which would enhance our comprehension of the mechanisms driving GPP and the impacts of climate change on carbon cycling in terrestrial ecosystems.

How to cite: Zhang, Q. and Zhou, T.: Deep learning-based identification of environmental memory effects on gross primary productivity of alpine grasslands in Qinghai-Tibetan Plateau, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5574, https://doi.org/10.5194/egusphere-egu25-5574, 2025.

In this study, a high-resolution CO2 data assimilation (DA)-forecast system was developed to improve atmospheric CO2 concentration simulations in East Asia. The Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) was used for simulating regional CO2 concentrations and the ensemble adjusted Kalman filter (EAKF) in modified Data Assimilation Research Testbed (DART) was used for assimilating CO2 concentration observations. To evaluate the performance of the developed DA-forecast system, observing system simulation experiment (OSSE) was performed in January and July 2019. Four experiments, which assimilated pseudo surface CO2 observations from four observation site networks, were conducted to avoid the influence of observation site distributions. In January and July 2019, the ratios of the root mean square error (RMSE) to the ensemble total spread for surface CO2 concentrations were 1.00 and 0.97, respectively. By assimilating surface CO2 concentrations, the bias and RMSE of simulated CO2 concentrations reduced by 1.23 ppm and 1.24 ppm in January and 1.41 ppm and 1.84 ppm in July, implying the stability of the developed DA-forecast system. Among four experiments, the experiment with an evenly distributed observation site network showed the smallest RMSE for surface CO2 concentration. The RMSE of the experiment with the existing CO2 observation network was greater than that with the evenly distributed observation network, but was smaller than that without DA. While the DA using the evenly distributed observation network showed the best performance for simulating CO2 concentrations in East Asia, the DA using the existing surface CO2 observation network also improved CO2 simulation performance compared to the experiment without DA.

Acknowledgments

This study was supported by a National Research Foundation of Korea (NRF) grant funded by the South Korean government (Ministry of Science and ICT) (Grant 2021R1A2C1012572) and the Yonsei Signature Research Cluster Program of 2024 (2024-22-0162).

How to cite: Seo, M.-G. and Kim, H. M.: Development and evaluation of high-resolution regional CO2 data assimilation-forecast system in East Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5697, https://doi.org/10.5194/egusphere-egu25-5697, 2025.

EGU25-6531 | ECS | Posters on site | AS3.44

Using explainable machine learning to study restored peatland CH4 flux heterogeneity 

Ilona Tamm, Kadir Yildiz, Evelyn Uuemaa, Mihkel Pindus, Ain Kull, and Kuno Kasak

Eddy Covariance (EC) method provides a valuable opportunity to monitor greenhouse gases, enabling informed decisions on climate change mitigation. Despite the abundance of EC data, explainable machine learning (ML) methods have not been effectively utilized to study the complex nature of methane (CH4) fluxes, especially heterogeneity of emissions within ecosystems. This study explores the application of random forest ML model to analyse CH4 flux spatiotemporal heterogeneity using flux data from the Ess-soo restored peatland in Estonia. This site, 30 years ago abandoned peat extraction area, was restored in 2021. To study CO2 and CH4 fluxes, open path EC analysers (LI-7500 and LI-7700, LICOR Biosciences) were installed in 2023. Additionally, CO2 and CH4 fluxes were measured biweekly using chamber method with the LI-7810 trace gas analyser (LICOR Biosciences) from 12 sampling spots in the EC footprint area. Other parameters such as water pH, electrical conductivity, dissolved oxygen concentration, temperature, oxidation reduction potenital, pH, and water level were conducted.

Chamber measurements revealed significant spatial CH4 heterogeneity within EC flux footprint. The mean CH4 flux from chamber measurement points during the summer months was 0.052 ± 0.013 µmol m-2 s-1 with a range of -0.001 to 0.555 µmol m-2 s-1. Looking into whole year EC dataset, main driver for CH4 flux was water temperature. Day and nighttime fluxes responded differently to environmental changes, with air temperature and wind speed being significant drivers for day and night, respectively. The random forest model predicted CH4 heterogeneity considerably better than general linear models performed (R² = 0.31 and 0.10, respectively). Besides identifying the main drivers, ML models can also combine EC and chamber measurements to detect hotspots and moments that are overlooked by EC alone. In that case, high spatial or temporal resolution  remote sensing data (e.g. LiDAR, Sentinel-1, Sentinel-2) was used. For instance, topographic wetness index calculated from LiDAR data in all points within EC flux footprint, was combined with water level—an important driver of both EC and chamber CH4 fluxes. This information, together with chamber data was used to train ML models to estimate CH4 fluxes spatially and temporally.

This work brings out the advantages in using ML and high spatial and temporal resolution remote sensing data to study CH4 flux heterogeneity in wetlands. However, more testing is needed to see if these methods give similar results in other wetland sites.

How to cite: Tamm, I., Yildiz, K., Uuemaa, E., Pindus, M., Kull, A., and Kasak, K.: Using explainable machine learning to study restored peatland CH4 flux heterogeneity, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6531, https://doi.org/10.5194/egusphere-egu25-6531, 2025.

EGU25-8137 | ECS | Posters on site | AS3.44

Coupling large-eddy simulations with UAV measurement through inversion technique to estimate patch-level fluxes from heterogeneous tundra landscapes 

Theresia Yazbeck, Mark Schlutow, Abdullah Bolek, Nathalie Ylenia Triches, Elias Wahl, Martin Heimann, and Mathias Göckede

Land cover change has direct implications on natural greenhouse gas emissions, as land-atmosphere interactions are function of the changing heterogeneity of the surface. Rapidly changing ecosystems, such as the Arctic, where permafrost wetting and draining is taking place in different regions in the northern latitudes, underlines the necessity of assessing patch-level emissions of greenhouse gases to better estimate net total fluxes. In this study, we combine high-resolution modelling of the atmospheric boundary layer with inverse modelling concepts to constrain land-atmosphere exchange fluxes at local to landscape scales, and explore relationships between different land cover types within heterogeneous landscapes and the net exchange processes between surface and atmosphere. We use EULAG (EUlerian LAGrangian), an established Large-Eddy Simulation model, to simulate high-resolution flow patterns induced by heterogeneous permafrost surfaces, and apply inversion techniques to infer the fluxes of the corresponding patch type forming the mixed land cover. Uncrewed Aerial Vehicles (UAV)-based grid surveys of gas concentrations are used to benchmark the spatial variability of modeled concentrations using EULAG, where we optimize for surface fluxes associated with each patch. We present a case study at Stordalen Mire in subarctic Sweden, where we use UAV measurements of methane and carbon dioxide mole fractions, and implement this inversion method to differentiate the flux rate signatures from different patch types, namely palsa, bog, and lakes. The inferred fluxes were validated with patch-level chamber measurements of methane and carbon dioxide. Our model evaluation shows a good match between modeled and observed concentrations while the resulting patch-level fluxes agree with the observed fluxes from chamber measurements. Our novel technique shows promising results in inferring patch type flux heterogeneity while facilitating the application of inversion methods to high resolution atmospheric models.

How to cite: Yazbeck, T., Schlutow, M., Bolek, A., Triches, N. Y., Wahl, E., Heimann, M., and Göckede, M.: Coupling large-eddy simulations with UAV measurement through inversion technique to estimate patch-level fluxes from heterogeneous tundra landscapes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8137, https://doi.org/10.5194/egusphere-egu25-8137, 2025.

EGU25-9204 | ECS | Posters on site | AS3.44

Modelling atmospheric CO2 and CH4 mixing ratios over mixed natural-agricultural wetlands in the Ebre River Delta  

Ricard Segura-Barrero, Alba Badia, Gara Villalba, and Ariane Arias-Ortiz

Terrestrial ecosystems play a crucial role in mitigating climate change by reducing greenhouse gas (GHG) emissions and sequestering significant amounts of atmospheric carbon dioxide (CO2). Wetlands, particularly coastal wetlands, are highly efficient carbon sinks but can also be large sources of methane (CH4). Natural and agricultural wetlands, such as rice paddies, contribute to 37 % of global CH4 emissions. Monitoring wetland-atmosphere carbon exchange is essential to evaluate the effectiveness of natural climate solutions (NCS), such as wetlands restoration and sustainable agricultural practices, in reducing GHG emissions and increasing soil carbon storage. Traditional methods for quantifying GHG emissions from wetlands include chamber flux measurements and eddy-covariance flux towers. These techniques provide valuable insights into carbon dynamics at the plot and ecosystem scale levels but fail to capture carbon fluxes at a regional scale, where policy decisions are often made. Recently, atmospheric composition observations have been used at regional scales and over urban areas to constrain the spatial and temporal distribution of GHG fluxes derived from land surface models. Applying similar methodologies to wetland regions, provided sufficient atmospheric observations are available, could enhance understanding of atmospheric carbon dynamics in these areas. The Ebre River Delta, a mixed natural-agricultural wetland system of international importance in terms of sustaining economic activities and biodiversity, offers a unique opportunity to investigate carbon sequestration and GHG emissions. This potential is enhanced by the availability of atmospheric GHG observations from in situ site tower and vehicle transects conducted across the regions.

Here, we integrate advanced modelling techniques and observational data to refine our understanding of GHG fluxes in the Ebre Delta. Biogenic GHG emissions over the Delta are estimated using a high-resolution Vegetation Photosynthesis and Respiration Model (VPRM) adapted for wetland ecosystems for CO2, and the Kaplan model embedded in the Weather Research and Forecasting (WRF) Greenhouse Gas (WRF-GHG) model to estimate CH4 emissions.  A sensitivity analysis is performed to compare VPRM CO2 emissions from different model configurations, entailing a default and a wetland-adapted model versions, and two sources of input satellite-vegetation indices, MODIS and Sentinel-2, with contrasting  spatial resolutions. Then, modelled atmospheric CO2 and CH4 mixing ratios with WRF-GHG during growing season are compared with in situ observations from the site tower and vehicle transects to assess their accuracy. The framework developed in this study will provide the basis for investigating sequestration and emission hotspots over a mosaic of wetland land-uses and evaluate the region's potential for climate change mitigation and adaptation. 

How to cite: Segura-Barrero, R., Badia, A., Villalba, G., and Arias-Ortiz, A.: Modelling atmospheric CO2 and CH4 mixing ratios over mixed natural-agricultural wetlands in the Ebre River Delta , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9204, https://doi.org/10.5194/egusphere-egu25-9204, 2025.

EGU25-10249 | ECS | Posters on site | AS3.44

Uncertainty in Land Carbon Fluxes Simulated by CMIP6 Models from Treatment of Crop Distributions and Photosynthetic Pathways 

Joseph Ovwemuvwose, Heather Graven, and Colin Prentice

A reliable representation of the diversity and variability of terrestrial ecosystems, both natural and managed, is crucial to the accurate simulation of their present and future roles in biogeochemical cycles and global climate. In this study we compare the treatment of vegetation distributions and of photosynthetic pathways (C3 versus C4) of both natural vegetation and crops across Earth System Models (ESMs) in the 6th Coupled Model Intercomparison Project (CMIP6). Of the 11 CMIP6 models reporting variables on crop and C3 versus C4 distribution use, 10 models use the crop distributions of the Land Use Harmonization v2 (LUH2) dataset, which has an increase of ~188 and ~254% in C3 and C4cropland, respectively, from 1850 to 2014. The models simulate a 10% decrease in the area coverage of natural vegetation with the C3 photosynthetic pathway but disagree on the trend of C4. The impact on carbon isotopic discrimination from simulated C3 and C4 GPP trends only, not accounting for physiological effects, is generally to drive a decreasing trend in discrimination, especially in models with increasing C4 vegetation cover, opposite to the trend derived from atmospheric data. Our findings suggest that implementation of C3 and C4 vegetation area abundance and GP of C3 and C4 vegetation contribute to uncertainty in land carbon fluxes and need further constraints and improvement in ESMs.

 

How to cite: Ovwemuvwose, J., Graven, H., and Prentice, C.: Uncertainty in Land Carbon Fluxes Simulated by CMIP6 Models from Treatment of Crop Distributions and Photosynthetic Pathways, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10249, https://doi.org/10.5194/egusphere-egu25-10249, 2025.

EGU25-10599 | ECS | Posters on site | AS3.44

Investigating ecosystem respiration CO2 signals using night-time ICOS tower observations 

Yang Xu, Michal Galkowski, Saqr Munassar, David (Tzu-Hsin) Ho, Frank-Thomas Koch, and Christoph Gerbig

The biosphere-atmosphere CO2 exchange is the largest carbon flux in the global carbon cycle, yet substantial uncertainties remain in quantifying gross primary production (GPP) and ecosystem respiration (Re). Top-down atmospheric inversion modeling provides a powerful approach to reduce the uncertainties in surface fluxes through a combination of atmospheric observations and transport modeling. However, as during nighttime mixing process of the atmosphere is weakly developed and hard to simulate in atmospheric transport models, atmospheric inversions typically rely on afternoon observations when both GPP and Re occur simultaneously, making it challenging to isolate their individual contributions.  In order to disentangle the respiration signals and simultaneously utilize previously unused observational data, we established a novel algorithm for the identification of night-time mixing height, based on the temporal variation of virtual potential temperature from ICOS tower measurements. The method is validated using profile information on greenhouse gases. We then integrated CO2 signals below the diagnosed mixing height and incorporated these partial column increment as observational operators in CarboScope-Regional (CSR), a Bayesian inverse modeling framework. This enhanced inversion scheme enables improved quantification of ecosystem respiration (and, by extension, GPP), bringing about a better understanding and constrains on the the role of biological fluxes in European carbon budgets.

How to cite: Xu, Y., Galkowski, M., Munassar, S., Ho, D. (.-H., Koch, F.-T., and Gerbig, C.: Investigating ecosystem respiration CO2 signals using night-time ICOS tower observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10599, https://doi.org/10.5194/egusphere-egu25-10599, 2025.

EGU25-12471 | Orals | AS3.44

BenchFlux: Advancing Nature-Based Climate Solutions through Scale-Aware CO2 Flux Benchmarks 

Emma Izquierdo-Verdiguier, Álvaro Moreno-Martínez, Paul Stoy, Oliver Sonnentag, Christopher Pal, Yanghui Kang, Trevor Keenan, Ankur R Desai, Stefan Metzger, Jingfeng Xiao, Matthew Fortier, Maoya Bassiouni, Sadegh Ranjbar, Samuel Bower, Sophie Hoffman, Danielle Losos, and Nicholas Clinton

Addressing the escalating climate crisis necessitates precise tools for evaluating nature-based climate solutions (NbCS). The BenchFlux project represents a significant advancement by developing scale-aware benchmarks for carbon dioxide (CO₂) fluxes, leveraging flux tower measurements and Earth Observation (EO) data. Unlike existing scale-agnostic approaches, BenchFlux introduces a methodology that explicitly accounts for the emergent, nonlinear behaviors inherent in carbon flux dynamics across spatial and temporal scales.

The objective of this project is to harmonize bottom-up CO2 inventories with top-down atmospheric inversions, thereby providing substantial tools for precise carbon accounting on global-to-local scales. By integrating flux tower ground-truth data and multi-source EO datasets, BenchFlux employs machine learning (ML) and cloud computing tools to develop ML-ready benchmarks with enhanced precision and uncertainty quantification. By transitioning from scale-agnostic to scale-aware data joins, the project optimizes the statistical power of flux tower measurements while maintaining consistency across various scales.

BenchFlux is built on three pillars:

  • Observational Inputs: Nested integration of flux tower ground-truth and EO predictors to produce a harmonized, ML-ready dataset. This includes multi-resolution, spatialized CO₂ flux data with uncertainties across spatial-temporal scales, enabled by Google Earth Engine and cloud-optimized workflows.
  • Models: Development of advanced ML models, such as Bayesian and knowledge-guided approaches, to improve predictive accuracy and functional consistency for carbon flux estimation.
  • Benchmark Outputs: Comprehensive datasets, baseline models, and uncertainty-aware evaluation metrics to foster collaboration and inform NbCS policies from local to global scales.

BenchFlux is a collaborative project across six international research teams, integrating expertise in flux tower data processing, remote sensing, and ML. By fostering open science practices, the project will provide accessible tools, tutorials, and datasets to empower the global scientific community. The project outcomes will catalyze the adoption of NbCS, ensuring accountability in net-zero pledges and advancing climate solutions grounded in scientific rigor.

How to cite: Izquierdo-Verdiguier, E., Moreno-Martínez, Á., Stoy, P., Sonnentag, O., Pal, C., Kang, Y., Keenan, T., Desai, A. R., Metzger, S., Xiao, J., Fortier, M., Bassiouni, M., Ranjbar, S., Bower, S., Hoffman, S., Losos, D., and Clinton, N.: BenchFlux: Advancing Nature-Based Climate Solutions through Scale-Aware CO2 Flux Benchmarks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12471, https://doi.org/10.5194/egusphere-egu25-12471, 2025.

EGU25-13541 | ECS | Orals | AS3.44

Constraining interannual variability of terrestrial carbon fluxes using proxy data in the CarbonTracker long-window data assimilation system 

Xiaoting Huang, Joram Hooghiem, Auke Van Der Woude, Remco De Kok, Peiyi Peng, Zhu Liu, and Wouter Peters

Interannual variability (IAV) represents a critical aspect of understanding changes in the terrestrial carbon cycle. Climate drivers such as temperature and water availability mainly influence the IAV of terrestrial carbon fluxes. Their contributions vary spatiotemporally across different regions and seasons and are simulated with various bottom-up and AI-based terrestrial ecosystem models. However, significant uncertainties remain in simulating terrestrial carbon flux IAV using such models, particularly in the tropics where correlations between temperature and/or water anomalies and atmospheric CO₂ observations were shown to be large. This study demonstrates a data assimilation system that decomposes net ecosystem exchange (NEE) into components across different timescales, with a specific focus on optimizing the poorly constrained IAV. Instead of directly optimizing NEE fluxes, this framework replaces the IAV component with a regression that links NEE IAV to proxy data, such as temperature and water-related variables, as well as light interception by the canopy. This approach allows the system to optimize the sensitivity of NEE IAV to these proxies, providing a robust method to simulate IAV in NEE also for locations and times where the IAV is not directly observed from atmospheric CO₂, or properly simulated by terrestrial biosphere models. This presentation will demonstrate the selection of proxy data and assess their robustness for use in CTE long-window system. The first results from the data assimilation system will be presented and compared to outputs from the regular Carbon Tracker Europe approach (CTE2024). The comparison will focus on quantifying the IAV of NEE and evaluating ecosystem responses to representative extreme events (e.g., heatwaves and droughts), highlighting differences in the system's ability to capture the impacts of such extreme events.

How to cite: Huang, X., Hooghiem, J., Van Der Woude, A., De Kok, R., Peng, P., Liu, Z., and Peters, W.: Constraining interannual variability of terrestrial carbon fluxes using proxy data in the CarbonTracker long-window data assimilation system, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13541, https://doi.org/10.5194/egusphere-egu25-13541, 2025.

EGU25-13589 | ECS | Posters on site | AS3.44

Towards a high-resolution inversion system over France using in-situ observations  

Carla D'angeli, Thomas Lauvaux, David Matajira Rueda, Ke Che, Charbel Abdallah, Hassan Bazi, Philippe Ciais, Michel Ramonet, Morgan Lopez, and Leonard Rivier

The global Stocktake, a fundamental component of the Paris Agreement tracking progress on national mitigation actions, collects the Nationally Determined Contributions (NDCs) generated through the means of annual national inventories. Carbon capture through the natural ecosystem is essential to reach the Paris Agreements and thus it is crucial to understand the interaction of the atmosphere/biosphere and its changes with global warming. We present the model performances of our regional inversion system over France for the year 2022, with a special focus on an extreme drought event that impacted southern Europe during the summer. Our inversion system optimizes CO2 fluxes from fossil fuel and biogenic fluxes at higher spatiotemporal resolutions over France (3km, hourly). The Lagrangian Particle Dispersion Model (LPDM) developed running in a backward-in-time model, driven by meteorological inputs from a 3-km run of the Weather Research Forecast Model (WRF-Chem), establishes the transport of CO2 molecules. Employing a Bayesian inversion technique, we optimize prior CO2 flux estimates by integrating tower footprints and ICOS atmospheric measurements into a newly developed inversion framework, combining block matrix decomposition and adaptive mesh refinement. We infer the prior flux estimates using the TNO high-resolution fossil fuel inventory and biogenic CO2 fluxes produced by the Vegetation Photosynthesis Respiration Model (VPRM). We start by evaluating the WRF-chem model performances at high resolution compared to low resolution simulations. Then we assess the meteorology and CO2 exchanges over continental France throughout the year 2022. With the Lagrangian Model, we can explore the actual ICOS network constraints by determining the share of biogenic and fossil fuel sources at each tower of the ICOS network. We discuss here how our inversion system could help constrain the regional distribution of CO2 fluxes, including sub-annual variations at seasonal and monthly timescales to track current climate change impacts (forest fires, droughts), and the effects of emission mitigation policies. Finally, we determine potential networks of surface stations (extension of the current ICOS network) to enable the monitoring of CO2 fluxes and emissions at policy-relevant scales over continental France.

How to cite: D'angeli, C., Lauvaux, T., Matajira Rueda, D., Che, K., Abdallah, C., Bazi, H., Ciais, P., Ramonet, M., Lopez, M., and Rivier, L.: Towards a high-resolution inversion system over France using in-situ observations , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13589, https://doi.org/10.5194/egusphere-egu25-13589, 2025.

EGU25-13739 | ECS | Orals | AS3.44

Optimizing CO2 emission estimates in Paris through enhanced urban atmospheric monitoring 

Ke Che, Thomas Lauvaux, Ingrid Chanca, William Morrison, Laura Bignotti, Theo Glauch, Pedro Coimbra, Benjamin Loubet, Samuel Hammer, Andreas Christen, Simone Kotthaus, Olivier Perrussel, Philippe Ciais, Leonard Rivier, Michel Ramonet, and Olivier Laurent

As part of the EU-funded PAUL project (ICOS Cities), the metropolitan area of Paris, in parallel with Munich and Zurich, has been instrumented with various observing systems to define the most-suitable approaches for CO2 emissions monitoring. This effort is underpinned by an extensive urban atmospheric monitoring network, comprising nine towers equipped with high-accuracy and mid-cost sensors designed to capture  variations in atmospheric concentrations. Driven by 1-km meteorological fields (from WRF), the Stochastic Time-Inverted Lagrangian Transport (STILT) model has been employed for backward simulations of CO2 enhancements based on state-of-the-art high-resolution inventories for 2023. Transport errors have been significantly reduced ( from about 4-5 m/s to  1~2 m/s) through the assimilation of three-dimensional wind profiles obtained from multiple Lidar data over Paris (Urbisphere project), using 3DVar data cycling assimilation. Fossil fuel emissions (TNO, AirParif) and biogenic emissions (using offline VPRM MODIS and Sentinel-2) serve as prior inventories in our inverse modeling framework. This framework employs a Bayesian inversion technique producing hourly fluxes with time-varied adaptive mesh grids (1 km in the downtown area, gradually aggregated to 100 km across the region), balancing computational efficiency with inversion accuracy near monitoring sites. However, direct comparisons revealed systematic discrepancies in the inversion results, particularly in the adjustments between anthropogenic and biogenic emissions. To address this, radiocarbon (14C) observations from two Parisian sites were incorporated as additional constraints, improving the partitioning of fossil fuel and biogenic contributions in the inversion.

How to cite: Che, K., Lauvaux, T., Chanca, I., Morrison, W., Bignotti, L., Glauch, T., Coimbra, P., Loubet, B., Hammer, S., Christen, A., Kotthaus, S., Perrussel, O., Ciais, P., Rivier, L., Ramonet, M., and Laurent, O.: Optimizing CO2 emission estimates in Paris through enhanced urban atmospheric monitoring, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13739, https://doi.org/10.5194/egusphere-egu25-13739, 2025.

Terrestrial ecosystems gain carbon through photosynthesis and lose it through respiration in autotrophs and heterotrophs. Continuously measured values of carbon fluxes of a forest ecosystem, particularly net ecosystem exchange (NEE) could be used as a general indicator of forest ecosystem functioning. Subsequently, quantification of the ecosystem functioning as a response to changes in the microclimate and environmental variables is necessary to frame sustainable adaptive measures and conservation policies. The Himalayan Chir- Pine (Pinus roxburghii Sarg.) is a gregarious, fire-resistant, indigenous tree species, often form pure forests and having the characteristics of high regeneration potential.  The Chir-Pine is widely distributed across the western and central part of the Indian Himalayan Region and thereby acts as a major control of land-atmosphere processes. In the recent years, studies have provided insights on sub-daily to annual scale interactions of Chir-Pine ecosystem with microclimatic and environmental variables, and it was reported that Chir-Pine ecosystem is a heat dominating ecosystem with high carbon sequestration potential. However, almost no information is available on environmental drivers resulting carbon sequestration of Himalayan Chir-Pine ecosystem. In this context, it is widely reported that the data driven models are well suited for identifying and prioritizing drivers for ecosystem carbon exchange. Therefore, this study is aimed at developing a data-driven model for predicting day-time net ecosystem exchange of a Chir-Pine forest of central Himalaya, Uttarakhand, India. And further aims to quantify driver-response relationship between net ecosystem exchange (NEE) and micro-climatic variables using machine learning classifiers. In order to address the objectives, high frequency (30-min) day-time observations of NEE and micrometeorological parameters during March, 2020 to December, 2022 are collected and compiled from a 30 m eddy covariance tower situated at Kosi-Katarmal, Almora, Uttarakhand, India (29º38'22"N, 79º37'2"E). Subsequently, four machine learning algorithms such as K-nearest neighbor, Naïve Bayes, support vector machine and decision trees are used to predict the day-time NEE using individual and combinations of predictors such as rainfall, net radiation, air temperature, soil moisture and soil temperature. To obtain a robust model, 100 times bootstrapping has been performed in each simulation where 2/3rd of the dataset is used for training the model and rest is used for testing.  The model performance during training and testing has been assessed using receiver operator characteristics and the prioritization of the driver impacting NEE is carried out by identifying highest area under curve (AUC) value during model testing. The initial results indicate that the decision tree classifier is the best model amongst the four selected model for predicting day-time NEE of Chir-Pine ecosystem, and the best predictors having high AUCs are air-temperature, net-radiation and soil moisture. The prediction of the NEE through data-driven models of Chir-Pine ecosystem is expected to be beneficial for quantifying the regional scale extent of change in carbon fluxes under warmer scenarios.

How to cite: Lohani, P., Mukherjee, S., and Pundir, S.: Investigation of eco-hydrogical processes influencing Himalayan Chir-Pine net ecosystem exchange using machine learning classifiers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14709, https://doi.org/10.5194/egusphere-egu25-14709, 2025.

Achieving sustainable urban development necessitates a significant reduction in carbon dioxide (CO2) emissions from transportation. Urban road traffic CO2 concentrations display intricate spatial patterns influenced by street layouts, mobile sources, and human activities. However, a comprehensive grasp of these patterns, which entail complex interactions, remains elusive due to the omission of human perspectives on road interface characteristics.

Our research team has developed an innovative integrated AI carbon emission monitoring technology through vehicle-based surveys. This technology utilizes panoramic visual sensors and various greenhouse gas (GHG) analyzers for spatiotemporal collaborative observations, data processing, and modeling. It provides insights into the dynamic connections between the physical urban space and road traffic emissions, offering a precise and refined carbon and pollutant emission source tracing system. This method automatically extracts attributes of objects and landscapes in urban scenes, aiding in evaluating the relative importance of built environments and road traffic to emission intensities in real scenarios. Based on a thorough understanding of in-situ conditions, this approach aims to identify coordinated development paths for buildings and transportation to enhance emission reduction effects.

In this study, a mobile travel platform was constructed to collect on-road navigation Street View Panoramas (OSVPs) and corresponding CO2 concentrations, obtaining over 100,000 sample pairs covering 675.8 km of roads in Shenzhen, China. Four ensemble learning (EL) models were used to establish nonlinear connections between the semantic and object features of streetscapes and CO2 concentrations. After EL fusion modeling, the predictive R2 in the test set exceeded 90%, and the mean absolute error (MAE) was <3.2 ppm. The model was applied to Baidu Street View Panoramas (BSVPs) in Shenzhen to generate a 100 m resolution map of average on-road CO2, and the Local Indicator of Spatial Association (LISA) was used to identify high CO2 intensity spatial clusters. Light Gradient Boost-SHapley Additive exPlanation (LGB-SHAP) analysis revealed that vertically planted trees can reduce on-road CO2 emissions. Moreover, factors affecting on-road CO2 exhibit interaction and threshold effects. Street View Panoramas (SVPs) and Artificial Intelligence (AI) were used to enhance the spatial measurement of on-road CO2 concentrations and the understanding of driving factors. This approach facilitates the assessment and design of low-emission transportation in urban areas, which is critical for promoting sustainable traffic development.

How to cite: Wang, L. and Zhang, Y.: Vehicle-based monitoring and AI unravel patterns of on-road carbon and pollutant emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14732, https://doi.org/10.5194/egusphere-egu25-14732, 2025.

EGU25-16220 | ECS | Posters on site | AS3.44

X-BASE: terrestrial carbon and water flux products from FLUXCOM-X 

Jacob A. Nelson, Sophia Walther, Basil Kraft, Fabian Gans, Gregory Duveiller, Ulrich Weber, Zayd Hamdi, Weijie Zhang, and Martin Jung and the FLUXCOM-X Team

Mapping in-situ eddy covariance measurements (EC) of terrestrial carbon and water fluxes to the globe is a key method for diagnosing terrestrial fluxes from a data-driven perspective. We describe the first global products (called X-BASE) from a newly implemented up-scaling framework, FLUXCOM-X. The X-BASE products cover the globe at 0.05° spatial resolution for every hour and include estimates of CO2 net ecosystem exchange (NEE) and gross primary productivity (GPP).

Compared to previous FLUXCOM products, the new X-BASE NEE better reconciles the bottom-up EC-based NEE and estimates from top-down atmospheric inversions (global X-BASE NEE is -5.75±0.33 PgC yr-1). The improvement of global NEE was likely only possible thanks to the international effort to improve the precision and consistency of eddy covariance collection and processing pipelines, as well as to the extension of the measurements to more site-years resulting in a wider coverage of bio-climatic conditions. However, X-BASE NEE shows low inter-annual variability, which is common to state-of-the-art data-driven flux products and remains a scientific challenge. With 124.7±2.1 PgC yr-1, X-BASE GPP is slightly higher than previous FLUXCOM estimates, mostly in temperate and boreal areas, and temporal patterns agree well with TROPOMI-based SIF.

Many further opportunities for development exist. We will outline how the new FLUXCOM-X framework provides the necessary flexibility to experiment, diagnose, and converge to more accurate global flux estimates. Pathways of exploration include methodological choices in the selection and processing of eddy-covariance and satellite observations, their ingestion into the framework, and the configuration of machine learning methods.

How to cite: Nelson, J. A., Walther, S., Kraft, B., Gans, F., Duveiller, G., Weber, U., Hamdi, Z., Zhang, W., and Jung, M. and the FLUXCOM-X Team: X-BASE: terrestrial carbon and water flux products from FLUXCOM-X, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16220, https://doi.org/10.5194/egusphere-egu25-16220, 2025.

EGU25-16327 | Orals | AS3.44

Towards reconciliation of top-down and bottom-up national-scale N2O emission estimates in Europe 

Stephan Henne, Hélène De Longueville, Alison Redington, Shauna-kay Rainford, Clemens Weber, Peter Andrews, Eric Saboya, Daniela Brito Melo, Alice Ramsden, Brendan Murphy, Joseph Pitt, Alexandre Danjou, Matthew Rigby, Lukas Emmenegger, Sonja G. Keel, Benjamin Wolf, Alistair Manning, and Anita Ganesan

Nitrous oxide (N2O) is the third most important anthropogenic greenhouse gas (GHG). In Europe, N2O contributes about 6 % to total GHG emissions and about 75 % of these emissions are from the agricultural sector. More than half of agricultural emissions arise from microbial production in managed soils with the amount of added fertilizer nitrogen, soil properties, and soil environmental conditions controlling the emissions. These drivers lead to large spatio-temporal variability in N2O fluxes, which is only poorly accounted for by simple bottom-up methods relying on emission factor approaches (IPCC Tier 1 and Tier 2 methods), and which are commonly used in national GHG inventory estimates.

The Horizon Europe project Process Attribution of Regional emISsions (PARIS) strives to improve national-scale flux estimates by employing regional-scale inverse modelling to atmospheric observations of N2O (top-down) and biogeochemical soil models. In recent years (2018 onwards), the density and quality of atmospheric observations in Western and Central Europe have improved to the point where inverse modelling at the temporal and spatial scales required for the comparison to nationally reported emissions (UNFCCC) and biogeochemical model output becomes feasible. Here, we report inverse modelling results for the period 2018-2023 for Western and Central Europe derived from three inverse modelling systemsnTEM, UK MetOffice; RHIME, University of Bristol; ELRIS, Empa. These were operated with two different atmospheric transport models: NAME-UM and FLEXPART-ECMWF. Overall, the total N2O fluxes agreed well, but were larger than in the national reporting to UNFCCC for several countries in Western and Central Europe. Results confirmed strong seasonality in N2O fluxes for the UK, Benelux, and Germany. In comparison, fluxes from France exhibited less pronounced seasonality. The variability in N2O fluxes was analysed with respect to environmental drivers, corroborating the important role of soil temperature and soil water content. Finally, the results allow a first comparison of the inversely obtained N2O fluxes and fluxes simulated by two biogeochemistry models for agricultural soils in Switzerland (DayCent, Agroscope) and Germany (LandscapeDNDC, KIT).

How to cite: Henne, S., De Longueville, H., Redington, A., Rainford, S., Weber, C., Andrews, P., Saboya, E., Brito Melo, D., Ramsden, A., Murphy, B., Pitt, J., Danjou, A., Rigby, M., Emmenegger, L., Keel, S. G., Wolf, B., Manning, A., and Ganesan, A.: Towards reconciliation of top-down and bottom-up national-scale N2O emission estimates in Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16327, https://doi.org/10.5194/egusphere-egu25-16327, 2025.

EGU25-17063 | Posters on site | AS3.44

Machine Learning and the Carbon Cycle: Chasing the Holy Grail 

Markus Reichstein

Over the past two decades, machine learning (ML) has become a key tool in carbon cycle research, offering new methods to quantify fluxes, map carbon stocks and turnover, and disentangle processes like photosynthesis and respiration. Early efforts with classical ML models enabled scalable integration of remote sensing and ground-based observations, significantly reducing uncertainties. More recent advancements in deep learning and hybrid modeling approaches now support multi-scale analyses, integrating diverse datasets across terrestrial, oceanic, and atmospheric domains.

However, the quest for a comprehensive ML framework faces persistent challenges. Confounding factors in observational data complicate the identification of key drivers of carbon fluxes, while causal modeling remains underexploited. Extrapolation in space and time, integrating heterogeneous data sources, ensuring robust uncertainty quantification, and balancing predictive power with interpretability are further challenges.

This talk reviews major milestones and explores whether an all-encompassing ML solution is within reach—or if tailored approaches addressing specific challenges are the more realistic path forward.

How to cite: Reichstein, M.: Machine Learning and the Carbon Cycle: Chasing the Holy Grail, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17063, https://doi.org/10.5194/egusphere-egu25-17063, 2025.

EGU25-17324 | ECS | Orals | AS3.44

Using machine learning to enable national methane emissions inference from large satellite datasets 

Elena Fillola, Raul Santos-Rodriguez, Rachel Tunnicliffe, Jeff Clark, Nawid Keshtmand, Anita Ganesan, and Matthew Rigby

The growing volume of methane measurements from space provides new opportunities for evaluating and improving countries' self-reported emissions. Surface emissions can be estimated from atmospheric observations using inverse modelling systems, which often rely on Lagrangian Particle Dispersion Models (LPDMs) to simulate how methane is transported through the atmosphere. Ensembles of particles are transported backwards in time from the measurement point, to define source-receptor relationships (“footprints”), which reflect the sensitivity of a measurement to all potential upwind sources within the domain. However, LPDM-based techniques are computationally costly, struggling to scale to the size of modern satellite datasets and limiting the amount of data that can be used for emissions inference. Previously, we presented a machine learning-driven LPDM emulator that can approximate satellite footprints using only meteorology and topography, and demonstrated its use over the South American continent, achieving speed-ups of over three orders of magnitude compared to the LPDM. We integrated the emulator into an emissions inference pipeline to estimate Brazil’s methane emissions from GOSAT observations in 2016 and 2018, and found that the emulator-based estimates were consistent with those obtained using the more expensive physics-based LPDM. Here, we show preliminary results of applying the emulator to other regions with high natural methane emissions, like North Africa and India. We compare the emulator’s performance across the selected time periods and geographical domains as well as the estimated emissions. Furthermore, we discuss solutions to improve performance and reduce the training data needed, like transfer learning across domains.

How to cite: Fillola, E., Santos-Rodriguez, R., Tunnicliffe, R., Clark, J., Keshtmand, N., Ganesan, A., and Rigby, M.: Using machine learning to enable national methane emissions inference from large satellite datasets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17324, https://doi.org/10.5194/egusphere-egu25-17324, 2025.

EGU25-17329 | ECS | Posters on site | AS3.44

Recalibrating neural network estimates of net ecosystem exchange in a Bayesian synthesis inversion 

Vitus Benson, Martin Jung, Theo Glauch, Yuming Jin, Basil Kraft, Julia Marshall, Christian Reimers, Alexander J. Winkler, and Markus Reichstein

Using neural networks to upscale eddy covariance measurements is a common approach to obtain global estimates of net ecosystem exchange (NEE) and thereby the land carbon sink. Unfortunately, this approach suffers from a limited representativeness of eddy covariance sites of the global picture, resulting in discrepancies between such data-driven bottom-up estimates of the land-atmosphere fluxes in comparison to independent top-down products from atmospheric inversions. Here, we introduce a novel method to bridge both approaches: recalibrating the last neural network layer in a Bayesian synthesis inversion. In other words, we find the least squares estimate of the last neural network layer weights, by first transporting the deep features and then inverting the covariance matrix of transported features to obtain a least squares estimator against atmospheric observations. This approach is possible because atmospheric tracer transport of CO₂ is a linear operator with respect to the surface fluxes. It is also computationally tractable due to a small number of degrees of freedom, namely just the regression coefficients for the approximately 50 deep features. For comparison, modern CO₂ inversions typically model the land surface flux with over 1000 parameters, which requires them to leverage variational or ensemble approaches for optimization.

 

The NEE estimates recalibrated using atmospheric data differ significantly from those obtained through pure eddy covariance training within the FLUXCOM-X framework. Namely, the recalibrated estimates show increased agreement with observational data from atmospheric measurement stations, when transported with the atmospheric transport model TM3. Surprisingly, this agreement does not necessarily arise from a greater agreement of global flux maps with results from the Jena CarboScope inversion. Here, the approach may suffer from low robustness of deep features or from regridding fluxes to a lower resolution before transporting them. We discuss ways to alleviate these limitations and outline what our results mean for improving neural network estimates of NEE.

 

How to cite: Benson, V., Jung, M., Glauch, T., Jin, Y., Kraft, B., Marshall, J., Reimers, C., Winkler, A. J., and Reichstein, M.: Recalibrating neural network estimates of net ecosystem exchange in a Bayesian synthesis inversion, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17329, https://doi.org/10.5194/egusphere-egu25-17329, 2025.

EGU25-17604 | ECS | Posters on site | AS3.44

Hybrid modelling for crop carbon cycle 

Yunan Lin, Maximilian Gelbrecht, Maha Badri, Philipp Hess, Sebastian Bathiany, and Niklas Boers

Given the ongoing climate change and the increasing frequency of extreme weather events, accurately assessing their impacts on crop productivity is crucial for developing adaptation strategies to mitigate negative impacts and ensure sustainable food security in the future. Process-based crop models are the preferred tools to simulate and predict crop yields under climate change. However, due to the simplified representations of complex biophysical processes, these models generally introduce uncertainty when used to account for crop yield losses. Integrating process-based crop models with data-driven machine learning methods shows great promise. In our study, we are developing a hybrid crop model, particularly the carbon cycle components (photosynthesis, carbon allocation, soil carbon decomposition, etc.), based on the state-of-the-art process-based vegetation model LPJmL (Lund-Potsdam-Jena managed Land). The empirical processes and parameters in the carbon cycle of LPJmL are replaced or augmented with neural networks. The resulting hybrid crop model can leverage information from observational data to simulate previously unresolved processes while maintaining the process-based understanding. We showcase how the hybrid crop model generalizes from the LPJmL to capture the carbon cycle under unseen climate conditions.

How to cite: Lin, Y., Gelbrecht, M., Badri, M., Hess, P., Bathiany, S., and Boers, N.: Hybrid modelling for crop carbon cycle, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17604, https://doi.org/10.5194/egusphere-egu25-17604, 2025.

EGU25-18007 | ECS | Posters on site | AS3.44

Towards a greenhouse gas emission monitoring and Verification system for Belgium (VERBE): Evaluation of WRF-GHG simulations with observational data 

Jiaxin Wang, Sieglinde Callewaert, Filip Desmet, Minqiang Zhou, and Martine De Mazière

Belgium’s national greenhouse gas (GHG) inventory currently relies on a bottom-up approach, but incorporating top-down methods using atmospheric observations and inverse modeling offers significant potential to improve the understanding of CO2 and CH4 emissions. The VERBE project aims to develop such a system tailored for Belgium by combining satellite, ground-based remote sensing, and in situ observations from the Integrated Carbon Observation System (ICOS) network with inverse modeling techniques. As part of this effort, we start by assessing the ability of the atmospheric transport model to accurately reproduce the spatiotemporal distribution of GHGs in this region.  

We employed the Weather Research and Forecast model coupled with chemistry in its Greenhouse Gas configuration (WRF-GHG) to simulate the Western Europe region, with a focus over Belgium, from June to August 2018. Simulations were conducted at horizontal resolutions of 9 km and 3 km over two domains. In comparison with meteorological data from Automatic Weather Stations in Belgium and ICOS sites, our results indicate that the WRF-GHG simulation is capable to capture the variations of the near surface meteorological fields (temperature, wind speed and wind direction) very well, especially for temperature.

The simulated CO2 and CH4 are compared with near-surface concentrations at different heights from four ICOS sites around Belgium and with column-averaged dry-air concentrations from the Total Carbon Column Observing Network (TCCON) site in Orléans, France. While WRF-GHG successfully reproduces most observed variations, discrepancies were identified. These include an overestimation of the CO2 peak values at most ICOS sites and an overall underestimation of near-surface CH4 concentrations by 20-30 ppb at three of the four ICOS sites. Additionally, the TCCON comparison revealed a significant deviation in XCO2 in early June, likely due to inaccuracies in biogenic fluxes which are calculated based on the Vegetation Photosynthesis and Respiration Model (VPRM). For XCH4, we find an increasing bias towards the end of summer, possibly related to the background signal.

We will present the latest results of our analysis, including additional observational data and updates to the model configuration aimed at improving model-data agreement such as the integration of the TNO high-resolution fossil fuel inventory and refinements to the VPRM fluxes.

How to cite: Wang, J., Callewaert, S., Desmet, F., Zhou, M., and De Mazière, M.: Towards a greenhouse gas emission monitoring and Verification system for Belgium (VERBE): Evaluation of WRF-GHG simulations with observational data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18007, https://doi.org/10.5194/egusphere-egu25-18007, 2025.

EGU25-18221 | ECS | Posters on site | AS3.44

Investigating the Benefits of Large-Eddy Simulation for Simulating Urban CO2 Emissions Using WRF-LES Over the Paris Area 

Alohotsy Rafalimanana, Thomas Lauvaux, Charbel Abdallah, Ke Che, Michel Ramonet, Josselin Doc, Olivier Laurent, Morgan Lopez, Anja Raznjevic, Maarten Krol, Leena Järvi, Leslie David, Olivier Sanchez, Andreas Christen, Sue Grimmond, and Will Morrison

Urban areas are significant contributors to global CO2 emissions, and simulating CO2 dispersion in these regions, especially near emission hotspots, presents considerable challenges due to the complex dynamics at small scales. High-resolution simulations are crucial for accurately capturing the dispersion of CO2 in urban environments. As part of the Carbon Atmospheric Tracer Research to Improve Numerics and Evaluation (CATRINE) project, this study employs the Weather Research and Forecasting model with the Large-Eddy Simulation mode (WRF-LES) to simulate CO2 concentrations over the Paris area, aiming to improve plume simulation accuracy. The study evaluates the model's performance in urban environments and investigates the added value of LES by comparing simulation results with those from mesoscale configurations. A series of simulations using five nested domains, with resolutions ranging from 8.1 km to 100 m, were performed to examine the sensitivity of plume structures to model resolution. The study also investigates the propagation of errors when running a pseudo-data CO2 inversion using high-resolution 100-m resolution WRF outputs to generate data, but inverting using lower resolution simulations (300-m and 900-m resolutions). The focus is on understanding how resolution influences inversion model results and quantifying aggregation errors introduced when aggregating higher-resolution outputs to coarser resolutions. 

Preliminary findings emphasize the advantages of LES in capturing complex plume features, reducing numerical diffusion, and producing more concentrated, well-defined CO2 plumes. Resolution intercomparisons highlight that higher resolutions better capture sharp concentration gradients, localized dispersion patterns, significantly outperforming traditional mesoscale models. Additionally, WRF model outputs were validated against observations from various sources, including the Paris Mid-cost CO2 sensor network, total column of CO2 measurements from EM27 and Total Carbon Column Observing Network (TCCON), and wind LIDAR data from six stations across Paris and Île-de-France, collected during the URBISPHERE project. Future studies will extend this research to other urban cities, utilizing different LES models such as WRF-LES, Micro-HH, and Parallelized Large-Eddy Simulation Model (PALM). Intercomparing these models will provide performance metrics on model resolution when assimilating complex urban plumes combining multiple diffuse sources and point sources, thereby further refining the accuracy of CO2 dispersion models for urban emissions monitoring and climate mitigation strategies.

How to cite: Rafalimanana, A., Lauvaux, T., Abdallah, C., Che, K., Ramonet, M., Doc, J., Laurent, O., Lopez, M., Raznjevic, A., Krol, M., Järvi, L., David, L., Sanchez, O., Christen, A., Grimmond, S., and Morrison, W.: Investigating the Benefits of Large-Eddy Simulation for Simulating Urban CO2 Emissions Using WRF-LES Over the Paris Area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18221, https://doi.org/10.5194/egusphere-egu25-18221, 2025.

EGU25-18419 | ECS | Orals | AS3.44

Predictive models of ecosystem productivity in water-limited conditions 

Samantha Biegel, Konrad Schindler, and Benjamin Stocker

Accurate predictions of environmental controls on ecosystem photosynthesis are essential for understanding the impacts of climate change and extreme events on the carbon cycle and the provisioning of ecosystem services. Widely used machine learning models for simulating ecosystem photosynthesis do not consider temporal dependencies in the data, even though process-understanding suggests these should exist through effects such as soil moisture stress. Here, we investigate the impact of accounting for temporal structure in modelling ecosystem photosynthesis.

Using time-series measurements of ecosystem fluxes paired with measurements of meteorological variables from a network of globally distributed sites and remotely sensed vegetation indices, we train three different models to predict ecosystem gross primary production (GPP): a mechanistic, theory-based photosynthesis model, a straightforward multilayer perceptron (MLP) and a recurrent neural network (Long-Short-Term Memory, LSTM). Through comparisons of patterns in model error, we assess the ability of these models to account for temporal dependencies that arise through effects such as soil moisture stress and cold acclimation. We further investigate the influence of different environmental factors on the generalisability across space.

We find that both deep learning models outperform the mechanistic model, and that the LSTM performs best with an R2 of 0.74. In particular, model skill is consistently good across moist sites with strong seasonality. Model error tends to increase with increasing potential cumulative water deficit, in particular in ecosystems with evergreen vegetation. Generalisation patterns reveal that the LSTM tends to be more successful than the MLP in adapting to arid environments and to ecosystems with seasonal dryness, suggesting an advantage of recurrent models for GPP modelling in those conditions. However, there remains a large variability in model skill across arid sites.

Our findings reveal the impacts on model error due to unknown effects of water limitation when predicting fluxes across different ecosystems. Due to climate change, temporal dependencies such as water limitation are becoming more prevalent, making an accurate representation of such processes increasingly important for modelling ecosystem function.

How to cite: Biegel, S., Schindler, K., and Stocker, B.: Predictive models of ecosystem productivity in water-limited conditions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18419, https://doi.org/10.5194/egusphere-egu25-18419, 2025.

EGU25-20406 | ECS | Posters on site | AS3.44

An uncertainty quantification framework for data-driven carbon flux upscaling 

Qi Yang, Sophia Walther, Jacob Nelson, Gregory Duveiller, Zayd Hamdi, and Martin Jung

Data-driven upscaling of biogenic fluxes from eddy covariance (EC) sites to the global scale is a powerful complementary approach to process-based models for the derivation of global flux estimates. Nevertheless, significant uncertainties arise due to specific methodological choices such as data availability, data source differences, machine learning model differences, and feature selection. Accurately quantifying these uncertainties from diverse sources is essential for providing error estimates of the simulated fluxes. These uncertainties not only improve our general understanding of carbon cycle processes but also directly inform atmospheric inversions, which can use the upscaled net ecosystem exchange (NEE) as a prior. However, most existing data-driven global carbon flux products focus solely on flux estimates or provide incomplete uncertainty assessments limited to a few sources.

In this study, we introduce a comprehensive framework for quantifying the uncertainties associated with carbon flux upscaling across potential sources. The framework involves three key steps: (1) pre-ensemble generation, (2) screening, and (3) uncertainty attribution. First, we construct ensemble members by training machine learning models with varying configurations, which include climate forcing datasets, feature combinations, subsets of EC sites, machine learning algorithms, and their hyperparameters. The experiments are supported by the recently developed data-driven modeling framework FLUXCOM-X, which enables a wide range of experiments with diverse methodological choices. We crafted a feature set that includes about 300 features to capture both current and historical state information. To capture the site representativeness uncertainty, we sample subsets from global EC sites based on geolocation and feature space. Additionally, we will also investigate different machine learning models and the variation of hyperparameters to generate the ensemble. Second, ensemble members that have a low contribution to the ensemble variance will be eliminated while we retain the most representative ones. We employ a feature selection algorithm, HybridGA, to screen important subfeature sets from near-infinite combinations. Moreover, we screen other ensemble members by assessing the distribution and spread of members. Finally, we will attribute uncertainties to various categories from the perspectives of machine learning and process-based modeling, and potential strategies to reduce these uncertainties are discussed. The framework is initially used to evaluate spatiotemporal NEE uncertain patterns in Europe, and will subsequently expand globally. Additionally, the estimated biogenic carbon flux uncertainty will be assessed with independent products. This work not only advances our understanding of the sources and patterns of upscaled flux uncertainties but also enhances the robustness of posterior estimates in atmospheric inversion models.

How to cite: Yang, Q., Walther, S., Nelson, J., Duveiller, G., Hamdi, Z., and Jung, M.: An uncertainty quantification framework for data-driven carbon flux upscaling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20406, https://doi.org/10.5194/egusphere-egu25-20406, 2025.

EGU25-1429 | ECS | Orals | AS3.47

Assessment of Hydrogen’s Climate Impact Is Affected by Model OH Biases 

Laura Yang, Daniel Jacob, Haipeng Lin, Ruijun Dang, Kelvin Bates, James East, Katherine Travis, Drew Pendergrass, and Lee Murray

Hydrogen fuel can help decarbonize the economy, but hydrogen leakage has indirect climate consequences. Atmospheric oxidation of hydrogen by hydroxyl radicals (OH) increases methane, ozone, and stratospheric water vapor concentrations. Current global 3-D atmospheric chemistry models estimate a global warming potential for hydrogen of 12 ± 3 over a 100-year horizon (GWP-100), but the models overestimate global OH concentrations and underestimate OH reactivity (OHR). These OH biases cause overestimates of the responses of methane and ozone to hydrogen. Here, we compare the hydrogen GWP-100 calculated from the standard GEOS-Chem model and a modified GEOS-Chem model where OH and OHR biases are corrected with missing organic emissions and a terminal OH sink over continents. The hydrogen GWP-100 from the standard GEOS-Chem model agrees with previous studies, but the modified GEOS-Chem model is 20% lower. Better understanding of the factors controlling global OH concentrations and OHR is needed for hydrogen GWP estimates.

How to cite: Yang, L., Jacob, D., Lin, H., Dang, R., Bates, K., East, J., Travis, K., Pendergrass, D., and Murray, L.: Assessment of Hydrogen’s Climate Impact Is Affected by Model OH Biases, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1429, https://doi.org/10.5194/egusphere-egu25-1429, 2025.

Atmospheric hydrogen sources and sinks vary greatly with latitude and season. In particular, the major sink is deposition into soils for which there is a strong seasonality and inter-hemispheric asymmetry. However, it is understood that there is a positive global warming potential (GWP) when hydrogen is oxidised in the atmosphere.

We have formulated a conceptual model based on hydrogen fluxes that were calculated in a comprehensive atmospheric chemistry simulation as part of the HECTER project. We have used this model to extensively probe the sensitivities of the GWP and distribution of hydrogen to the time of year of emissions and their latitude, and to asymmetries in the atmosphere’s oxidising capacity. Examining these sensitives helps us to understand the discrepancies between different atmospheric chemistry models and with observations, and to further constrain uncertainties in the hydrogen GWP.

How to cite: Tardito Chaudhri, A. and Brown, M.: Conceptual Experiments to Deepen our Understanding of Sensitivities in the Hydrogen Distribution and its Impacts., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2918, https://doi.org/10.5194/egusphere-egu25-2918, 2025.

EGU25-3587 | Orals | AS3.47

Modelling the Climatic Impact of Hydrogen Emissions in SSP scenarios 

Thomas Gasser and Gabriel Baudouin

With a possible transition toward a hydrogen-based economy as an alternative to fossil fuels, concerns arise regarding the environmental impacts of hydrogen emissions. Although hydrogen has no direct radiative forcing, it indirectly contributes to global warming through its interactions with atmospheric components such as methane, ozone, and water vapor. This impact has not been assessed in the SSP scenarios or in the broader AR6 scenario database.

This study integrates a comprehensive hydrogen budget into the OSCAR compact Earth system model, focusing on its sources, sinks, and chemical interactions, to assess its potential climatic impacts under the main SSP scenarios of ScenarioMIP. We evaluated key anthropogenic sources such as fossil fuel combustion, biomass burning, and leakage from hydrogen infrastructure. We parameterised secondary sources such as methane and VOC oxidation. The major sinks, atmospheric oxidation by hydroxyl radicals and soil uptake by bacteria, were modelled using simplified equations calibrated against outputs from complex process-based models.

With our approach, the hydrogen and methane cycles are fully interacting during transient simulations. Our simulations quantify the influence of hydrogen emissions on methane lifetime, tropospheric ozone, and stratospheric water vapor, which combined amount to a slight increase in radiative forcing. Under a leakage rate of 1.8%, the global temperature impact remains minor, altering predictions by a few hundredths of a degree, while a higher leakage rate of 10% amplifies the effect but hardly reaches one tenth of a degree in any scenario. The quantitative impact of hydrogen emissions in terms of global temperature exhibits a widely differing profile across scenarios, strongly influenced by the IAMs’ assumptions regarding future use of hydrogen and by the scenarios’ own emissions of methane.

Although these estimates of the climatic impact of hydrogen are not entirely negligible, especially in low-warming scenarios for which every fraction of a degree counts, our findings suggest that correcting the absence of its quantification in the AR6 scenario database would not lead to a drastic reclassification of these scenarios, which should be reassuring for policy-makers.

How to cite: Gasser, T. and Baudouin, G.: Modelling the Climatic Impact of Hydrogen Emissions in SSP scenarios, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3587, https://doi.org/10.5194/egusphere-egu25-3587, 2025.

EGU25-6850 | Orals | AS3.47

Refining Hydrogen Emission Measurements: Methodological Insights and Pilot Findings  

Malgven Roudot, Victoria Krohl, Tomas Mikoviny, Felix Piel, Nikita Sobolev, and Armin Wisthaler

Hydrogen is expected to be a key contributor to the energy transition. It represents an energy carrier solution for some sectors that are difficult to decarbonize such as industrial processes or long-distance transport.  The hydrogen market is therefore likely to expand rapidly in the coming decades. However, hydrogen has an indirect impact on climate, with an estimated GWP100 around 11.6 ± 2.8 (Sand, 2023). It is thus important to understand how much hydrogen is emitted to the atmosphere during its economic lifecycle (from production, to transport, storage and end-use), as well as design systems to safely minimize the emissions. Frameworks regulating hydrogen emissions are expected in the near future and UK Low Carbon Hydrogen standard already requires measuring, monitoring and reporting hydrogen emissions from hydrogen production facilities.  

To ensure the quality and transparency of reported emissions, Equinor started a project in 2023 to develop and test a method to measure emissions from industrial sites. The instrument chosen was a modified mass spectrometer to allow measurements of small concentrations of hydrogen (<1ppm), with a high precision to detect only minor enhancements (~10ppb) above atmospheric background levels. As the performance of the instrument was very encouraging, 2024 was dedicated to trying to quantify emissions from a point source or an industrial site using the tracer ratio method.  The selection of tracer was guided by Equinor’s safety and sustainability principles adapted to the purposes of this study. Results of small-scale tests, large-scale validation and real-life experiments will be presented. 

How to cite: Roudot, M., Krohl, V., Mikoviny, T., Piel, F., Sobolev, N., and Wisthaler, A.: Refining Hydrogen Emission Measurements: Methodological Insights and Pilot Findings , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6850, https://doi.org/10.5194/egusphere-egu25-6850, 2025.

EGU25-7461 | ECS | Posters on site | AS3.47

Quantifying climate implications of a future hydrogen economy using a two-box model 

Isabella Dressel, Alexander Archibald, Megan Brown, Nicola Warwick, and Paul Griffiths

Hydrogen (H2) provides an alternative to fossil fuel use during the transition to net zero emissions. However, the climate impacts of a H2 economy are dependent on its production method and leakage rates during production, transport, and storage. H2 acts as an indirect greenhouse gas through its impacts on methane (CH4), tropospheric ozone, and stratospheric water vapor. H2 reacts with hydroxyl radicals (OH), the primary sink of CH4, thereby causing the CH4 lifetime to increase. The climate impacts of H2 are not well constrained, largely due to uncertainties in the H2 soil sink, which accounts for ~75% of atmospheric H2 loss.

Here, we develop a two-box model of the CH4–CO–OH–H2 scheme based on the work of Prather (1994). We improve the conventional four-equation system and incorporate data from UK Earth System Model (UKESM1) simulations to generate time-varying OH production and parameterize impacts of nitrogen oxides (NOx) on the system. We evaluate the CH4 lifetime under various H2 leakage rates and SSP scenarios to quantify impacts of changes in carbon monoxide (CO), CH4, volatile organic compounds, and NOx. As the H2 soil sink dominates uncertainty in the H2 budget, we perform a Monte Carlo analysis of uncertainties in H2 soil deposition and quantify impacts on the CH4 lifetime. We estimate the indirect global warming potential of H2 under each scenario relative to both CH4 and CO2 and propose H2 leakage rates required for climate benefits under various SSP scenarios.

How to cite: Dressel, I., Archibald, A., Brown, M., Warwick, N., and Griffiths, P.: Quantifying climate implications of a future hydrogen economy using a two-box model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7461, https://doi.org/10.5194/egusphere-egu25-7461, 2025.

EGU25-8383 | ECS | Posters on site | AS3.47

Future Hydrogen Soil Deposition: Multi-model assessment of hydrogen deposition and lifetime 

Megan Brown, Alex Archibald, and Nicola Warwich

Alternate energy carriers to fossil fuels are needed to mitigate climate change, of which hydrogen is one candidate if generated sustainably. Atmospheric hydrogen indirectly contributes to greenhouse warming by extending methane lifetime, and increasing stratospheric water vapour and tropospheric ozone. Its main sinks are oxidation with OH, and dry deposition via microbial soil uptake. The latter accounts for approximately 50−90% of the sink and is poorly constrained under present day conditions, with very limited studies on its future evolution. The soil sink is a large source of uncertainty in quantifying hydrogen’s climate impact and the H2 global warming potential (GWP).

This work uses an offline hydrogen deposition scheme to perform the first multi-model assessment of deposition velocities driven by physical climate data from 5 models from the Coupled Model Intercomparison Phase 6 project. Deposition values from historical data are compared to observations, and deposition velocities from 4 future scenarios (2015−2100) are assessed. We find hydrogen soil uptake increases over the century, with larger increases under scenarios with stronger climate forcing, leading to shorter hydrogen soil lifetimes. A large discrepancy (20%) between models is attributed to differences in soil moisture and soil porosity, and results in a variation of 33% in the hydrogen GWP under present day condition, with a maximum decrease of 5.3% by the end of the century.

How to cite: Brown, M., Archibald, A., and Warwich, N.: Future Hydrogen Soil Deposition: Multi-model assessment of hydrogen deposition and lifetime, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8383, https://doi.org/10.5194/egusphere-egu25-8383, 2025.

EGU25-9443 | ECS | Posters on site | AS3.47

Controlled-release experiment to optimize emission quantification of H2 point sources 

Iris Westra, Hubertus A. Scheeren, Mareen J. Penninga, Steven M.A.C. van Heuven, and Harro A.J. Meijer

A result of the global energy transition is an expected increase in atmospheric hydrogen, due to fugitive H2 emissions during production, transport, storage and usage. Loss rates are predicted to be up to 10% of the total hydrogen production. The oxidation of hydrogen in the atmosphere leads to the lengthening of the lifetime of methane, enhanced tropospheric ozone production, and increased stratospheric water vapor levels, thereby acting as an indirect greenhouse gas. Until recently, small but climate-relevant hydrogen emissions leading to atmospheric hydrogen concentrations < 1 ppm downwind of emissions sources remained undetected. However, with our newly developed and demonstrated method using an ‘active’ AirCore sampler combined with a Gas Chromatographic system (GC-system) with a Pulsed Discharge Helium Ionization Detector (PDHID), we can detect atmospheric hydrogen emissions with a precision of <2 ppb. The ‘active’ AirCore is an atmospheric sampling system consisting of a long narrow tube (in the shape of a coil) in which atmospheric air samples are collected using a pump during the sampling experiment, in this way preserving a profile of the trace gas of interest along the measurement trajectory. Here, we present first result of a controlled-release experiment to optimize our emission quantification of H2 point sources. As a point source we used a 8 kW electrolyser releasing a constant flow of 1.1 ± 0.1 m3 of hydrogen per hour through a small vent which refers to 1.65 ± 0.15 g min-1 (under standard atmospheric conditions). For our experiments we deployed a newly developed high resolution Agilent 8890 GC-PDHID system that is able to measure H2 (< 2 ppb), CH4 (< 0.5 ppb) and CO2 (< 0.3 ppm), combined with an ‘active’ AirCore as a sampling tool. During our field experiments we deployed two different sampling methods downwind of the plume; the active AirCore was either taken on ground or flown with an UAV up to 35 m altitude. The active AirCore system with a sample volume of 4.1 L, was filled to an end-pressure of up to 1.6 bar over the course of about 2 hours of sampling resulting in up to 200 discrete H2 samples on the new GC-PDHID system. As a control measurement and source apportionment along the measurement trajectory, another sampling technique was involved which uses dried and vacuumized 2.5 L glass flasks to collect discrete samples. The glass flasks samples were further analyzed by Cavity Ring Down Spectroscopy (Picarro G2401) on mole fractions of CO2, CH4, CO, for comparison to the GC-PDHID results. We present first results of our field experiments visualizing the cross sections of the downwind plume up to ~35 m altitude and using these results to optimize our inverse Gaussian plume model. Further work will focus on expanding the inventory of other fugitive hydrogen sources along the hydrogen value chain.

How to cite: Westra, I., Scheeren, H. A., Penninga, M. J., van Heuven, S. M. A. C., and Meijer, H. A. J.: Controlled-release experiment to optimize emission quantification of H2 point sources, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9443, https://doi.org/10.5194/egusphere-egu25-9443, 2025.

EGU25-9572 | Orals | AS3.47

Green Hydrogen from Iceland: A Clean Energy Pathway to Decarbonizing Teesside’s Industry 

David C. Finger, Diego A. Costa, Guðlaugsson Bjarnhéðinn, Jinoop Arackal Narayanan, Robin Thoppurathu Varghese, Zakaria Hmaimid, and Tariq Ahmed

Hydrogen export from Iceland to Teesside, UK, presents a promising opportunity to decarbonize the industrial sector in Teesside. Hydrogen export to Teesside involves storage in containers, transportation via trucks to Reykjavík port, and shipping to Teesside via Rotterdam. Leveraging Iceland's abundant renewable energy resources, including geothermal and hydropower, hydrogen production achieves high full load hours (FLH) compared to intermittent renewables in other countries. Excess electricity in Iceland, which cannot be sold to neighboring countries due to geographic isolation, can be acquired at competitive prices for hydrogen production. Notably, this pricing advantage may reduce hydrogen costs below those of conventional fossil fuels, even when considering the relatively low energy efficiency of hydrogen production processes. This excess energy is particularly available during periods of intense snow and ice melt in summer, further enabling high FLH for hydrogen production.

A full life cycle assessment (LCA) was performed to evaluate the environmental impacts, using secondary data from the ecoinvent database and primary data obtained through research. Additionally, a tool was developed to assess environmental impacts for any transportation chain, ensuring the flexibility and applicability of the analysis. Logistic chains for hydrogen transport, encompassing storage, trucking, and shipping, were identified and validated in collaboration with local stakeholders. Utilizing Polymer Electrolyte Membrane Electrolysis (PEM-EC) and Iceland’s renewable electricity grid mix, hydrogen production emits 13–21 times less greenhouse gases compared to grid-based production in countries like Austria and Belgium.

Transportation of green hydrogen, including liquefaction, storage, and shipping, contributes 25–36% of the carbon footprint for export scenarios but remains a small fraction of the overall emissions compared to grid-based production in fossil-intensive electricity grids. Notably, liquefaction accounts for 81% of the transportation phase’s footprint. Environmental breakeven analyses reveal that Iceland's hydrogen supply chain can offset the emissions of alternative grid-based production within three years, or less than one year when relying solely on geothermal power.

Our results demonstrate the feasibility of establishing a low-emission hydrogen supply chain to support Teesside's industrial decarbonization. Aligning with IEA recommendations, such efforts promote the development of a global green hydrogen infrastructure. Iceland’s renewable energy potential, competitive pricing of excess electricity, and robust logistics planning position it as a pivotal player in the transition to cleaner industrial operations. As an outlook, Iceland plans to further develop its renewable energy infrastructure, increasing its capacity for green hydrogen production and export in the future [2].

[1] Vilbergsson K.V., Dillman K., Emami N., Ásbjörnsson E.J., Heinonen J., D. C. Finger, Can remote green hydrogen production play a key role in decarbonizing Europe in the future? A cradle-to-gate LCA of hydrogen production in Austria, Belgium, and Iceland, International Journal of Hydrogen Energy, Volume 48, Issue 46, 2023, Pages 17711-17728, ISSN 0360-3199, https://doi.org/10.1016/j.ijhydene.2023.01.081

[2] Cabalzar U., Blumer L., Fluri R., Zhang X., Bauer C., Finger D., Bach C., Frank E., Bordenet B., C. Stahel, (2021) Projekt IMPEGA - Import von strombasiertem Gas, Aqua & Gas, 6, 40-45, Schweizerischer Verein des Gas- und Wasserfaches

How to cite: Finger, D. C., Costa, D. A., Bjarnhéðinn, G., Arackal Narayanan, J., Thoppurathu Varghese, R., Hmaimid, Z., and Ahmed, T.: Green Hydrogen from Iceland: A Clean Energy Pathway to Decarbonizing Teesside’s Industry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9572, https://doi.org/10.5194/egusphere-egu25-9572, 2025.

EGU25-9950 | ECS | Posters on site | AS3.47

Development of Instrumentation for Mobile Measurements of Hydrogen Emissions 

Isaac Standen, Rebecca Fisher, James France, Dave Lowry, Mathias Lanoisellé, and Euan Nisbet

In the coming decades, hydrogen infrastructure is expected to expand significantly as our energy supply moves towards net-zero carbon emissions in response to anthropogenic climate change. However, whilst hydrogen itself is not a greenhouse gas, it causes indirect warming. It reacts with other trace gases in the atmosphere, resulting in increased concentrations of tropospheric methane and ozone, and stratospheric water.

This project aims to quantify parts per billion (ppb) level concentration variations in mobile measurements of atmospheric hydrogen in the UK, enabling small leaks to be detected. Molecular hydrogen can be difficult to contain due to its small size and tendency to leak from storage.  Reducing gas analysers require frequent calibration and are generally not portable. Furthermore, hydrogen is not IR active, and therefore cannot be measured using the same techniques as other mobile analysers. 

We are redeveloping an off-the-shelf cavity ring-down spectroscopy (CRDS) analyser to be used for mobile measurements. The instrument contains a catalyst which converts molecular hydrogen within sample gases into water vapour that is measured using CRDS. Due to this measurement method, gases in the analyser must be dried prior to injection. The instrument is regularly flushed with dry nitrogen (N2), and ambient air and calibration standards are passed through a drying inlet that we have designed to reduce moisture within the sample gas. This inlet consists of a flow meter followed by a Nafion dryer, Drierite and magnesium perchlorate; the sample passes through a moisture detector before injection. The air is dried further by an internal drier within the instrument.

Local data will be compared to both continuous and flask measurements taken with the gas chromatography and reducing gas photometer instrument in our laboratory. After this, we will conduct field campaigns at industrial sites across the UK that are likely to be emitting molecular hydrogen. 

A precise, accurate mobile analyser allows for accurate measurements of fugitive emissions from the industrial sector and better constraint of models and hydrogen’s source inventory. The analyser also allows for measurements in remote locations, and could be extremely beneficial in the search for natural hydrogen. This project allows for improvement in our understanding of hydrogen’s impact on the climate and energy sector.

How to cite: Standen, I., Fisher, R., France, J., Lowry, D., Lanoisellé, M., and Nisbet, E.: Development of Instrumentation for Mobile Measurements of Hydrogen Emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9950, https://doi.org/10.5194/egusphere-egu25-9950, 2025.

EGU25-10785 | Posters on site | AS3.47

The UK Environmental Impacts of Hydrogen Energy Programme 

Nicola Warwick, Alex Archibald, Paul Dodds, Eiko Nemitz, Helen ApSimon, and Julia Drewer and the Hydrogen Environmental Impacts Team

This programme examines the climate and air quality implications of transitioning from fossil fuels to hydrogen-based energy systems. It comprises three independent projects – ELGAR, HECTER and COSH-AIR – that investigate various aspects of hydrogen usage and its effects on the atmosphere. The research explores future global and UK energy scenarios, focusing on the development of hydrogen infrastructure and the potential for fugitive hydrogen emissions. It also examines the role of microbial soil processes in removing atmospheric hydrogen, as well as the impacts of hydrogen deployment on climate and air quality. This overview will provide a summary of the research undertaken and the insights gained throughout the programme.

How to cite: Warwick, N., Archibald, A., Dodds, P., Nemitz, E., ApSimon, H., and Drewer, J. and the Hydrogen Environmental Impacts Team: The UK Environmental Impacts of Hydrogen Energy Programme, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10785, https://doi.org/10.5194/egusphere-egu25-10785, 2025.

EGU25-12198 | ECS | Orals | AS3.47

Preliminary results of the characterization of the hydrogen emissions from a water electrolysis plant at pilot scale 

Olivier Lefranc, Julie Clavreul, Alessandro Guzzini, Paolo Piras, Alessandro Saccardi, Cesare Saccani, and Marco Pellegrini

Hydrogen has been identified as an essential energy carrier for a future low-carbon economy. However, recent studies have highlighted the indirect impact of hydrogen emissions on climate change, emphasizing the necessity of quantifying hydrogen emissions. It is within this framework that the NHyRA project is being carried out. The European consortium of 14 entities of NHyRA aims to assess potential current and future hydrogen emissions throughout its entire chain value (from production to end uses), develop methods to detect and measure these emissions and provide an inventory where to collect these measurements in addition to validated data that already exist in the literature. 

This work will focus on the potential hydrogen emission sources from a water electrolysis system. Among existing hydrogen production methods, water electrolysis is a promising technology for converting and storing electricity, making it interesting for harnessing intermittent and fluctuating renewable energy sources. Furthermore, several European countries are implementing challenging development plans regarding the capacity of installed electrolysers. Understanding the various factors that can influence the amount of hydrogen released by this technology before it is deployed on a large scale is crucial to minimizing its environmental impact and then adopting effective mitigation strategies on the technology, e.g., new components or control strategies. 

Herein, we first introduce the fundamentals of water electrolysis, and we present the typical overall design of an electrolysis system, which includes the electrolysis stack and all the auxiliaries needed for its proper work, i.e. the so-called “balance of plant”. We then proceed to qualitatively present and categorize the main potential emission sources. We start with the “Vented emissions”, which are emissions needed for the system's proper operation. The analysis includes the description of the main mechanisms that may lead to these types of hydrogen released to the vent, like physical phenomena (e.g. Hydrogen crossover) or emissions coming from a process step (e.g. Hydrogen vented after a purification unit until the quality required for fuel cell application is reached or related to Start-up/shut down procedures). Last, we present the “fugitive emissions”, which include all uncontrolled emissions that come from connections that are not perfectly sealed or permeation phenomena related.  

As a conclusion of the work, we present a methodology to estimate the amount of hydrogen released considering also different operational conditions. Finally, to put all these different types of emissions in perspective, we perform a preliminary assessment of the emissions that would happen for a specific PEM electrolysis system for different power supply configurations.  

How to cite: Lefranc, O., Clavreul, J., Guzzini, A., Piras, P., Saccardi, A., Saccani, C., and Pellegrini, M.: Preliminary results of the characterization of the hydrogen emissions from a water electrolysis plant at pilot scale, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12198, https://doi.org/10.5194/egusphere-egu25-12198, 2025.

EGU25-12419 | Orals | AS3.47

Modeling Climate Impacts of Hydrogen Transition Pathways 

Christopher Moore, Ansh Nasta, Esther Goita, Emily Beagle, and Micheal Webber

Hydrogen has emerged as a key contender for decarbonizing hard-to-abate sectors, as it has the advantage of emitting no direct carbon dioxide emissions during combustion. However, modeled indirect climate warming impacts from additional hydrogen in the atmosphere have raised questions about its role in achieving net-zero energy transitions. Here we will present findings from two complementary modeling efforts that evaluated the climate implications of hydrogen emissions, and the life cycle impacts across various applications.

The first model effort evaluated emissions in 23 net-zero scenarios from prominent U.S. economy-wide studies, estimating the magnitude of hydrogen emissions relative to residual energy-related carbon dioxide and methane emissions. The model was used to evaluate the potential impact of hydrogen emissions relative to emissions reductions and carbon dioxide removal strategies needed for net-zero scenarios. Then the model was used to estimate energy-related hydrogen and methane emissions rates and global warming potentials with the best available data in literature. Modeling results indicated that hydrogen emissions ranged from 0.02–0.15 GtCO2e/year (using GWP100), with higher emissions in scenarios featuring increased hydrogen production. Despite these emissions, the calculated climate impacts represent less than 15% of combined hydrogen, methane, and carbon dioxide emissions in most scenarios. These impacts can be largely abated through reductions in residual CO2 emissions or enhanced carbon dioxide removal. More specifically, residual CO2 emissions would need to be reduced by 1-25% in scenarios allowing fossil fuels and 32-98% in scenarios restricting fossil fuels to abate the warming effect of H2 emissions.

The second modeling effort involved a life cycle assessment (LCA) of electrolysis and steam methane reforming, highlighting that production methods and feedstock emissions are the dominant factors influencing life cycle emissions, rather than hydrogen leakage. Comparisons of hydrogen-based and fossil fuel-based systems revealed greenhouse gas emission reductions in steel production (800–1400 kgCO2e per tonne of steel) when hydrogen is used in direct reduction steel manufacturing (producing iron from iron ore without melting) rather than fossil fuels in blast furnaces, as well as in heavy-duty transportation (0.1–0.17 kgCO2e per tonne-km of cargo). Importantly, decarbonization potential of hydrogen varies by application, with steel production consistently showing emissions reductions, while benefits in heavy-duty transportation depend on the hydrogen production pathway.

These findings underscore the importance of advancing hydrogen emissions measurement, mitigation strategies, and tailored application areas to maximize its potential climate benefits while addressing indirect warming impacts.

How to cite: Moore, C., Nasta, A., Goita, E., Beagle, E., and Webber, M.: Modeling Climate Impacts of Hydrogen Transition Pathways, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12419, https://doi.org/10.5194/egusphere-egu25-12419, 2025.

EGU25-13708 | ECS | Orals | AS3.47

Comparative Greenhouse Gas Impact Assessment of Well-to-Use Hydrogen and Other Alternative Pathways Across 11 Use Cases 

Stavroula Sartzetakis, Sofia Esquivel-Elizondo, Irving Rettig, and Tianyi Sun

Investments in “clean” hydrogen as an alternative to fossil fuels are driven by anticipated climate benefits. However, most climate impact assessments of hydrogen pathways overlook or underestimate important climate-warming emissions (i.e., hydrogen, methane) and impacts over time. Moreover, hydrogen is often evaluated against conventional fossil fuels without considering alternative decarbonization options, which limits the ability to inform decision-making effectively. This study evaluates the greenhouse gas emissions mitigation potential of 31 well-to-use hydrogen pathways (renewable- and grid-based electrolytic hydrogen and fossil fuel-based hydrogen with carbon capture and sequestration [CCS]) and 14 other alternative pathways (direct electrification, electro-fuels, and CCS) to replace conventional fossil fuels for eleven use cases across various economic sectors. We aim to quantify the effect of hydrogen and methane emissions on the climate benefits of decarbonization pathways and provide guidance on where to deploy hydrogen for maximum climate benefits. Preliminary results show that, across all use cases, hydrogen and methane emissions can considerably reduce the near-term climate benefits of a decarbonization pathway, with an average of a 3% and 12% reduction for every 1% of hydrogen and methane emitted, respectively. Renewable electricity-based pathways (direct electrification, hydrogen, and electro-fuels) consistently offer greater climate benefits than pathways that involve fossil fuel and CCS, but their deployment should consider the efficiency of utilizing renewable electricity. For use cases where direct electrification is available (i.e., light-duty vehicles, buses, trucks, and home heating), it is the most efficient option to reduce climate-warming emissions. Hydrogen and electro-fuels can achieve comparable benefits but demand around 1.4-7 times the renewable electricity capacity. Therefore, they should be reserved for use cases where electrification is limited (i.e., ship, aircraft, industrial heat, power) and where hydrogen serves as a feedstock (i.e., fertilizer, steel, refinery). In these cases, additional renewable capacity buildout is required to avoid diverting resources from other essential decarbonization strategies and inadvertently increasing system level emissions.

How to cite: Sartzetakis, S., Esquivel-Elizondo, S., Rettig, I., and Sun, T.: Comparative Greenhouse Gas Impact Assessment of Well-to-Use Hydrogen and Other Alternative Pathways Across 11 Use Cases, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13708, https://doi.org/10.5194/egusphere-egu25-13708, 2025.

With the proposed increased use of hydrogen energy, a more accurate representation of the atmospheric hydrogen budget is crucial to evaluating potential climate impacts. To this end, we extend the study by Sand et al. (2023), where five different chemical models were used to calculate the global warming potential of hydrogen. A box-model (SimpleH2 model) has been developed using those model results to calculate how atmospheric hydrogen concentrations and hydrogen isotopic compositions change for different sources and sinks. The sources included in the model are anthropogenic sources, biomass burning, nitrogen fixation (over land and ocean), photochemical production in the atmosphere, and geological sources. The two sinks are soil uptake and oxidation by OH. In this study, we will simulate the box model with different combinations of sources and sinks (both in terms of concentrations and isotopic values) to evaluate the feasibility of those inputs, focusing on the contributions of different geological sources and soil sinks. For example, adding a geological source of 20 Tg/year with an isotopic composition of -600 per mil and increasing the soil uptake by 20 Tg/year, will modify the isotopic composition of atmospheric H2 (to ~10 per mil) far from the observed range.  These provide us with useful constraints that can be tested in future measurement campaigns.

How to cite: Krishnan, S.: Constraining potential geological sources of atmospheric hydrogen using a box-model approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15596, https://doi.org/10.5194/egusphere-egu25-15596, 2025.

EGU25-16526 | Posters on site | AS3.47

Volatile Organic Compounds Model Intercomparison Project (VOCMIP)  

Gunnar Myhre, Maria Sand, Ragnhild Skeie, Srinath Krishnan, Marit Sandstad, and Øivind Hodnebrog

Given the significant role of volatile organic compounds (VOCs) on ozone formation, methane lifetime, atmospheric hydrogen formation, secondary organic aerosol formation, overall atmospheric chemistry, and both indirect and direct health impacts, their accurate representation in global atmospheric chemistry models is crucial. In this context, we introduce the Volatile Organic Compounds Model Intercomparison Project (VOCMIP) and invite atmospheric chemistry modeling groups to participate in this collaborative effort. VOCMIP aims to identify model consistencies and discrepancies, enhance parameterizations, and advance our understanding of VOC-related processes in the atmosphere. Global atmospheric chemistry model output will be compared to satellite data and in situ measurements from surface stations and aircraft campaigns for key VOCs. Special emphasis will be placed on formaldehyde (HCHO), examining its chemical sources and sinks, with a particular focus on its role in the atmospheric production of hydrogen.

How to cite: Myhre, G., Sand, M., Skeie, R., Krishnan, S., Sandstad, M., and Hodnebrog, Ø.: Volatile Organic Compounds Model Intercomparison Project (VOCMIP) , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16526, https://doi.org/10.5194/egusphere-egu25-16526, 2025.

EGU25-17780 | ECS | Posters on site | AS3.47

First coupled H2-HD inversion with a 3D chemical transport model (TM5): Constraining the global hydrogen budget 

Firmin Stroo, Wouter Peters, Joram Hooghiem, Maarten Krol, Iris Westra, and Harro Meijer

Hydrogen (H2) is expected to become an increasingly important energy carrier during the energy transition. This will likely cause increased levels of atmospheric H2, due to unavoidable losses during the production, transport, storage, and usage of hydrogen. Multiple studies have shown that through interaction with the hydroxyl radical, global tropospheric and stratospheric composition could be impacted, however, a large uncertainty remains due to a lack of understanding of the global hydrogen budget.

For the first time, we present a comprehensive global hydrogen budget derived using a coupled H2-HD inversion framework embedded within the three-dimensional chemical transport model TM5. This budget is obtained using a global set of 178,640 H2 mole fraction measurements and 540 δD(H2) measurements, which are subsequently supplied to the CarbonTracker data assimilation system. Using its ensemble Kalman filter approach we estimate the magnitude and spatial distribution of monthly global hydrogen emissions, chemical production and losses for 2003–2023. To evaluate the robustness of our results, we compare optimized simulated hydrogen mole fractions with independent observational data from aircraft profiles collected during the IAGOS-CARIBIC, NOAA/ESRL, and ATom campaigns.

How to cite: Stroo, F., Peters, W., Hooghiem, J., Krol, M., Westra, I., and Meijer, H.: First coupled H2-HD inversion with a 3D chemical transport model (TM5): Constraining the global hydrogen budget, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17780, https://doi.org/10.5194/egusphere-egu25-17780, 2025.

EGU25-18263 | ECS | Posters on site | AS3.47

Evaluating Hydrogen Emissions from Incomplete Combustion: Historical Trends and the Role of Policy 

Thiago Brito, Lena Höglund-Isaksson, Peter Rafaj, Robert Sanders, Anna Pauls, Shaohui Zhang, and Zbigniew Klimont

Context: Expanding the use of hydrogen (H2) throughout the economy is widely regarded as a key approach to fossil fuel dependent decarbonizing sectors. However, recent studies have been showing that emissions of hydrogen to the atmosphere are indirectly associated with climate impacts, such as the prolonged lifetime of methane (CH4) as well as the formation of ozone (O3) and stratospheric water vapor (H2O). Despite hydrogen’s short atmospheric lifetime (4-7 years), the studies estimate that hydrogen atmospheric interactions could lead to a Global Warming Potential over 100 years (GWP-100) ranging from 6 to 18. Hydrogen emissions have two main sources: a) direct leakages from related appliances and infrastructure (eg.: electrolyzers, distribution networks, fuel cells); or b) incomplete combustion of fossil fuels or biomass due to poor oxygen supply, where carbon monoxide (CO) and H2 are formed.

Objective: This study aims to quantify historical hydrogen emissions from incomplete combustion from 1990 to 2020 and compare their CO₂-equivalent contribution. In addition, we evaluate the influence of policy measures on reducing these emissions.

Methodology and Data: The current work adopts the Greenhouse Gas and Air Pollution Interactions and Synergies (GAINS) model framework, which takes into account activity level (fuel consumption) by sector, emission factors and the application of control strategies for emissions abatement. We adopt historical fuel consumption from statistical data along with GAINS model’s assumptions. Hydrogen emission factors are derived from carbon monoxide (CO) emission factors by a conversion ratio estimated from the literature. Control strategies represent the countries’ regulations adopted over the period of 1990-2020.

Expected Results: As an indirect greenhouse gas, hydrogen emissions may not be as prominent as CO₂, CH₄, or N₂O, which are commonly monitored. Nevertheless, hydrogen leakage does occur and should be included in emissions inventories. Historical data and future projections could indicate consistent yearly reductions, largely driven by stricter control measures and policies—particularly vehicle standards aimed at reducing a variety of pollutants, including CO. The primary sources of hydrogen emissions from incomplete combustion are gasoline-fueled light-duty vehicles and biomass burning in the domestic sector, although sector-specific contributions may differ across countries.

Discussion: While the expansion of a hydrogen economy may lead to higher emissions from direct leaks, hydrogen has also been released into the atmosphere through past and ongoing fuel combustion. Both sources must be taken into account to ensure these emissions do not undermine the expected benefits of a decarbonized, hydrogen-based economy. This underscores the importance of existing pollution-reduction policies and their co-benefits. Although control strategies have been effective in certain sector, such as transportation, emissions from domestic biomass burning remain difficult to manage and continue to pose challenges in developing countries. Finally, the overall effect of any strategy depends not only on its effectiveness but also on how future activities are distributed across different sectors.

How to cite: Brito, T., Höglund-Isaksson, L., Rafaj, P., Sanders, R., Pauls, A., Zhang, S., and Klimont, Z.: Evaluating Hydrogen Emissions from Incomplete Combustion: Historical Trends and the Role of Policy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18263, https://doi.org/10.5194/egusphere-egu25-18263, 2025.

EGU25-18281 | Orals | AS3.47

Investigating the drivers of microbial H2 uptake: a summary of measured fluxes from a range of soil types and locations 

Nicholas Cowan, Mark Hanlon, Aurelia Bezanger, Josh Dean, Ove Meisel, Grant Forster, Graham Mills, Nicholas Garrard, Eiko Nemitz, and Julia Drewer

The widescale global use of Hydrogen (H2) fuel may result in increasing concentrations of atmospheric H2 gas as a result of diffuse operational leakage. While H2 is not a direct greenhouse gas (GHG), it does exhibit secondary GHG effects and influences several important atmospheric chemistry reactions which could have cascading environmental effects. The dominant process of H2 removal from the atmosphere is uptake by soils; however, this removal mechanism is poorly understood and the fate and impact of increased H2 emissions on the soil sink remain highly uncertain. In order to better understand future impacts of increased H2 concentrations we need to understand current uptake rate of a range of different soils. Models require more information and data to improve the simulation of microbial processes in soils that dominate the global sink of atmospheric H2. Over the past year, we have carried out H2 flux measurements from a number of soils, both in the field (grasslands, arable, forests and peatland soils in the UK) as well as under controlled laboratory conditions, by completing several controlled incubation experiments with soil from the UK and abroad. These studies have provided important information regarding the impact that soil moisture, soil pH, temperature and other soil properties have on H2 fluxes in soils. Our studies highlight that both physical (e.g. soil aeration) and microbial (e.g. pH and temperature) parameters strongly influence the microbial uptake of H2 in soil types, with large differences in fluxes observed between different soil types under relatively similar environmental conditions.

How to cite: Cowan, N., Hanlon, M., Bezanger, A., Dean, J., Meisel, O., Forster, G., Mills, G., Garrard, N., Nemitz, E., and Drewer, J.: Investigating the drivers of microbial H2 uptake: a summary of measured fluxes from a range of soil types and locations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18281, https://doi.org/10.5194/egusphere-egu25-18281, 2025.

EGU25-19715 | Posters on site | AS3.47

Impacts of hydrogen on tropospheric ozone and methane and their modulation by atmospheric NOx 

David Stevenson and Hannah Bryant

Atmospheric hydrogen concentrations have been increasing in recent decades. Hydrogen is radiatively inert, but it is chemically reactive and exerts an indirect radiative forcing through chemistry that perturbs the concentrations of key species within the troposphere, including ozone. Using the atmospheric version of the United Kingdom Earth System Model, we analyse the impact of 10% increased surface concentrations of hydrogen on ozone production and loss. We also analyse the impact of this hydrogen in atmospheres with lower anthropogenic emissions of nitrogen oxides (80% and 30% of present-day anthropogenic surface emissions), as this is a likely outcome of the transition from fossil fuels towards cleaner technologies. In each case, we also assess the changes in hydroxyl radical concentration and hence methane lifetime and calculate the net impact on the hydrogen tropospheric global warming potential (GWP). We find that the hydrogen tropospheric GWP100 will change relatively little with decreases in surface anthropogenic NOx emissions (9.4 and 9.1 for our present day and 30% anthropogenic emissions, respectively). The current estimate for hydrogen GWP100 can therefore be applied to future scenarios of differing NOx, although this conclusion may be impacted by future changes in emissions of other reactive species.

How to cite: Stevenson, D. and Bryant, H.: Impacts of hydrogen on tropospheric ozone and methane and their modulation by atmospheric NOx, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19715, https://doi.org/10.5194/egusphere-egu25-19715, 2025.

EGU25-21824 | ECS | Orals | AS3.47

Changes in climate forcing from hydrogen deployment as a decarbonization strategy 

Patrick O'Rourke, Bryan K. Mignone, Matthew Binsted, Bryan R. Chapman, Olivia E. Clifton, Kalyn Dorheim, Page Kyle, and Steven J. Smith

Hydrogen deployment is projected to expand in energy transition scenarios to decarbonize hard-to-electrify end uses. Hydrogen is an indirect climate forcer, and increased hydrogen production and use may lead to an increase in hydrogen emissions, which could occur during production, delivery, and/or final consumption. At the same time, when hydrogen deploys in the energy system, other energy carriers such as liquid fuels, natural gas, coal, and electricity would be displaced, affecting both CO2 and non-CO2 emissions, including CH4, SO2, NOx, CO, NMVOC, and BC. To our knowledge, the full suite of potential climate forcing changes from hydrogen deployment has not been examined in existing studies, in part because it requires combining information from different fields. This study addresses this gap by using a well-known integrated assessment model (GCAM) to combine (1) credible hydrogen deployment scenarios that illustrate which energy carriers could be displaced by hydrogen; (2) information about hydrogen emission rates and emission factors of other climate forcers by technology, sector, region and time; and (3) a simple climate model capable of translating all relevant emissions, including hydrogen emissions, into changes in climate forcing. Across all scenarios considered, when compared to a scenario without hydrogen deployment for energy, we find that reduced forcing from CO2 emissions dominates all other forcing changes. In addition, the net forcing change excluding CO2 and methane, as well as the net indirect forcing change from CO, NOx, NMVOC, and H2 is negative and small relative to the total forcing change. These results raise important questions for technology and policy assessment regarding the treatment of indirect and aerosol effects.

How to cite: O'Rourke, P., Mignone, B. K., Binsted, M., Chapman, B. R., Clifton, O. E., Dorheim, K., Kyle, P., and Smith, S. J.: Changes in climate forcing from hydrogen deployment as a decarbonization strategy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21824, https://doi.org/10.5194/egusphere-egu25-21824, 2025.

AS4 – Interdisciplinary Processes

EGU25-2877 | ECS | Orals | AS4.1

Atmospheric response to Antarctic coastal polynyas 

Matthias Noel, Sébastien Masson, and Clément Rousset

Antarctic coastal polynyas are ice-free areas forming in sea ice-covered regions, primarily driven by strong katabatic winds that push sea ice offshore. These polynyas enable ocean-to-atmosphere heat exchange, driving intense sea ice production and dense water formation. Despite their role in generating Antarctic Bottom Water (AABW), which constitutes 30-40% of global ocean volume, their atmospheric dynamics remain poorly understood.

This study investigates the atmospheric impacts of Antarctic coastal polynyas using high-resolution (3 km) WRF simulations, focusing on the Prydz Bay region, including the Cape Darnley (CDP) and Mackenzie Bay polynyas (MBP). A sensitivity experiment without polynya, highlights the significant atmospheric changes when polynyas are open: a major heat release toward the atmosphere (up to 1000 W·m⁻²) increases the air temperature (over 5.5°C), creates a low-pressure anomaly (-70 Pa), an acceleration of the surface winds (over 5 m·s⁻¹) and an intense atmospheric convection leading to a thicker boundary layer (+400 m) and more clouds. Two recirculation anomaly cells develop upstream and downstream of the polynya. An analysis of meridional wind trends reveals that the dynamical response of the atmosphere to the polynya opening is controlled by a balance between the pressure gradient forces, the advection and the vertical diffusion, reinforced by the strong vertical turbulent mixing above the polynya. 

These results underline the substantial influence of polynyas on local atmospheric dynamics, and suggest potential feedback mechanisms that could influence polynya dynamics and consequently the AABW formation.

How to cite: Noel, M., Masson, S., and Rousset, C.: Atmospheric response to Antarctic coastal polynyas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2877, https://doi.org/10.5194/egusphere-egu25-2877, 2025.

EGU25-3313 | Posters on site | AS4.1

Decadal time series of high-resolution downwelling spectral radiancemeasurements from Concordia Station, Antarctica 

Giovanni Bianchini, Gianluca Di Natale, Luca Palchetti, and Marco De Pas

In December, 2011 the REFIR-PAD Fourier transform spectroradiometer was installed in Concordia Station, Antarctica to perform continuous monitoring of the atmospheric downwelling emitted radiance in the middle-far infrared region. The spectroradiometer is supported by several auxiliary instruments to monitor ground and sky conditions and, since 2020, by a compact lidar sensor to provide cloud structure in the lower troposphere and boundary layer region, thus establishing a complete and integrated set of sensors for the monitoring of the Antarctic troposphere.

The main product in the data set provided by the observing system consists in high-resolution spectral radiances measured in the 100-1500 cm-1 region with a 0.4 cm-1 resolution. This allows us not only to separate the contributions to the radiation budget due to H2O, CO2, O3 and clouds, but also to retrieve vertical profiles of water vapor and temperature, columnar amounts of minor constituents and cloud properties through a data inversion process.

The production of a consistent long-term dataset needs to front multiple challenges which are intrinsic in long period continuous operation in extreme environment, methods for the correction of systematic effects and to perform automatic data quality assessment had been developed in order to be able to make the data available for use by the atmospheric science community.

An example of the results that can be obtained exploiting the advantage of long term measurement and high temporal resolution provided by the dataset is the identification and analysis of extreme events: not only it is possible to perform a detailed analysis of the most prominent events on an hourly timescale, but also it is possible to search the dataset for the occurrence and statistics of minor events that could be of similar origin.

How to cite: Bianchini, G., Di Natale, G., Palchetti, L., and De Pas, M.: Decadal time series of high-resolution downwelling spectral radiancemeasurements from Concordia Station, Antarctica, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3313, https://doi.org/10.5194/egusphere-egu25-3313, 2025.

EGU25-3634 | Posters on site | AS4.1

Assessment of Long-Term Climatic, Hydrological, and River Ice Dynamics in River Oulankajoki  

Abolfazl Jalali Shahrood, Amirhossein Ahrari, and Ali Torabi Haghighi

This study examines long-term climatic and hydrological trends in River Oulankajoki, in Finland. The aim is to understand the impacts of changing climate conditions on river systems. Using 57 years (1966–2023) of daily air temperature and snow depth data from the Finnish Meteorological Institute (FMI) and hydrological observations from the Finnish Environment Institute (SYKE), the analysis incorporates longwave (LW) and shortwave (SW) radiation data from ERA5, accessed through Google Earth Engine (GEE). The Mann-Kendall trend test was employed to detect significant temporal changes, that reveals a significant decreasing trend in both air temperature values and discharge Phase Change Timing (i.e., PCT) over the study period. The results show that the river ice break-up timing has been shifting about 3-weeks in time, meaning that the break-up season occurs earlier than 57 years ago. These changes indicate potential shifts in regional climate dynamics, likely influenced by global climate change. Correlation heatmaps showed strong positive relationships between air temperature (AT) and river ice Break-Up Days (i.e., BUDs).

How to cite: Jalali Shahrood, A., Ahrari, A., and Torabi Haghighi, A.: Assessment of Long-Term Climatic, Hydrological, and River Ice Dynamics in River Oulankajoki , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3634, https://doi.org/10.5194/egusphere-egu25-3634, 2025.

EGU25-4130 | ECS | Orals | AS4.1

Quantifying the risk of unprecedented Antarctic heatwaves 

Charlie Suitters, James Screen, and Jennifer Catto

It has been widely documented that the East Antarctic heatwave (EAH) in March 2022 featured some of the largest positive temperature anomalies ever recorded anywhere on Earth. The heatwave was extraordinary in both extent and magnitude, where anomalies of at least 30°C were reached widely in the region. This study seeks to determine the likelihood of this event, the risk of even more extreme events occurring in the current state of the Antarctic climate; and whether events of a similar magnitude could occur elsewhere on the continent and at other times of year, with potentially more severe impacts for ice shelf stability. A large ensemble of seasonal hindcasts from multiple forecasting centres is used to assess the simulated occurrence of high temperature extremes over Antarctica, using a technique known as "UNprecedented Simulated Extremes using Ensembles" (UNSEEN).

The March 2022 EAH was outside the range of possible extreme temperatures suggested by the ensemble of hindcasts, signifying that events of this magnitude are incredibly rare. It is also shown with the ensemble that almost everywhere in Antarctica could experience unprecedented March heatwaves in the current climate, at least 5°C higher than has been observed. The UNSEEN method also suggests that temperature anomalies of a similar magnitude to those in the March 2022 EAH could occur widely across the continent in today’s climate. Therefore, Antarctic heatwaves on the scale of the 2022 event could occur almost anywhere, even though they have not yet been observed. This would be particularly problematic over the larger ice shelves of the Ross and Ronne-Filchner. If the extreme temperatures suggested by UNSEEN are realised here, it is shown that these ice shelves would be more susceptible to more frequent, or more severe, melting. This could ultimately result in weaker ice shelves, ice shelf collapse, and rising global sea levels.

How to cite: Suitters, C., Screen, J., and Catto, J.: Quantifying the risk of unprecedented Antarctic heatwaves, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4130, https://doi.org/10.5194/egusphere-egu25-4130, 2025.

EGU25-5718 | Orals | AS4.1

Extreme increases in snow grain size on the Antarctic Plateau from Satellite Observations and Ice Sheet-Atmosphere Interactions 

Claudio Stefanini, Giovanni Macelloni, Marion Leduc-Leballeur, Vincent Favier, Benjamin Pohl, and Ghislain Picard

Grain size variations impact the albedo and have consequence for the energy budget of the surface.  The snow grain size in Antarctica follows a clear seasonal pattern: a summer increase and a winter decrease, which are conditioned by atmospheric processes —namely temperature, wind, snowfall— and by mechanisms acting inside the snowpack leading to water vapour transport thus causing the coarsening of the grains. This study focuses on the evolution of the grain size in the interior part of East Antarctica, where dry metamorphism occurs, by using satellite observations. For this, we use, as proxy for the snow grain size, the Grain Size Index (GSI) inferred from the 89 and 150 GHz radiometer observations collected by the Advanced Microwave Sounding Unit-B (AMSU-B) from 2000 to 2022. Four extreme increase in GSI have been identified over the Antarctic Plateau, along the highest ice divide. In these cases, the ERA5 reanalysis revealed an atmospheric blocking/ridge situation around the onsets of the summer growing of the grain size, conveying the relatively warm and moist air coming from the mid latitudes, often associated with atmospheric rivers. The snow dry metamorphism is facilitated conditions of weak wind, low temperature and low snowfall conditions during the following weeks, leading to grain growth. These conditions determine anomalous high value of the snow grain size at the end of summer. Theoretical analysis have been performed to investigate in detail the extreme snow grain size event happened near Dome Fuji during the summer 2019-2020. The simulations of the AMSU-B observations  confirm that this extreme variation is mainly related to an increase in snow grain size. Results also highlighted  a decrease in snow density during this event. This is supported by independent satellite observations at 1.4 and 36 GHz (from Soil Moisture and Ocean Salinity SMOS and Advanced Microwave Scanning Radiometer 2 AMSR-2, respectively), which showed synchronized variations related to an unusual change in surface snow density.

How to cite: Stefanini, C., Macelloni, G., Leduc-Leballeur, M., Favier, V., Pohl, B., and Picard, G.: Extreme increases in snow grain size on the Antarctic Plateau from Satellite Observations and Ice Sheet-Atmosphere Interactions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5718, https://doi.org/10.5194/egusphere-egu25-5718, 2025.

EGU25-7154 | ECS | Orals | AS4.1

Drivers and impacts of the vertical structure of the troposphere at Villum Research Station, Northeast Greenland 

Jonathan Fipper, Jakob Abermann, Ingo Sasgen, and Wolfgang Schöner

The vertical temperature structure controls atmospheric stability and is a key component for surface energy exchange. However, in situ data for validation of re-analysis data or process studies remain scarce in the Arctic. We collected 130 vertical temperature profiles up to 500 m above ground using uncrewed aerial vehicles (UAVs) over different surface types (ice, snow-free tundra, open water) around the Villum Research Station (VRS) in Northeast Greenland. The VRS is adjacent to Flade Isblink, the largest peripheral ice cap in Greenland. To assess the accuracy of our approach, we conducted 50 ascents and descents next to a meteorological mast equipped with temperature sensors at 2 m, 8 m, 20 m and 80 m above ground. Our UAV-based approach shows good agreement with the mast, with about 90% of the measurements being within the sensor accuracy of 0.6°C. Furthermore, we find a robust agreement between the UAV data and the Copernicus Arctic Regional Reanalysis (CARRA) data set (mean absolute difference of 1°C; r= 0.59) depending on the prevailing wind direction. To understand the influence of different surface properties on the vertical temperature structures and their temporal changes, we focus on daily CARRA data for June, July and August between 1991 and 2024. We show that differences in air temperature between regions of snow-free tundra and glacier ice maximize in July and find the maximum altitude up to which the atmosphere is significantly (α = 0.05) controlled by surface properties at about 100 m above ground. Next, we use K-means clustering to categorize temperature gradients above this threshold of 100 m and 500 m to analyze the associated large-scale atmospheric conditions. We are able to distinguish 5 clusters from the temperature gradients related to distinct patterns of large-scale atmospheric conditions of 850 hPa temperature and 500 hPa geopotential height. These preliminary results suggest that the temperature structures of the lowest 100 m of the troposphere are significantly controlled by surface properties and consequently by the fraction of snow cover in the tundra. Above 100 m, temperature gradients are driven by large-scale synoptic conditions. Finally, we study the effect of surface properties and large-scale circulation on the mass balance of the Flade Isblink ice cap using the Modèle Atmosphérique Régional (MAR).

How to cite: Fipper, J., Abermann, J., Sasgen, I., and Schöner, W.: Drivers and impacts of the vertical structure of the troposphere at Villum Research Station, Northeast Greenland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7154, https://doi.org/10.5194/egusphere-egu25-7154, 2025.

EGU25-9051 | ECS | Posters on site | AS4.1

30 years of Antarctic weather station observations by the IMAU network (1995-2025) 

Maurice Van Tiggelen, Paul Smeets, Carleen Reijmer, Peter Kuipers Munneke, and Michiel van den Broeke

Since 1995, the Institute for Marine and Atmospheric research Utrecht (IMAU) at Utrecht University has operated automatic weather stations (AWS) at 20 different locations on the Antarctic ice sheet. In cooperation with multiple institutes, AWS were installed in Dronning Maud Land, on the East Antarctic Plateau, on the remnants of the Larsen B ice shelf, and on the Larsen C and Roi Baudouin ice shelves.  Besides standard meteorological observations (wind speed, wind direction, air temperature, humidity, surface pressure), these stations also recorded the four components of net surface radiation, as well as surface height change. That allows for a reliable estimation of the surface energy balance (SEB) and surface mass balance (SMB) at hourly temporal resolution. Due to the harsh climatic conditions and limited number of maintenance visits, the data require a thorough quality control procedure and specific sensor corrections.

Here we present the corrections that were applied to the measurements, as well as the procedure that was implemented to flag suspicious samples. We give an overview of the first quantification of the long-term variability in SEB components, as well as the strong contrast between the high-melt locations near the grounding lines of ice shelves and the dry interior of the Antarctic ice sheet.  In total, 152 station-years of observations are available, of which 78% are non-flagged simultaneous observations of all meteorological and radiation parameters.

This dataset may be used for the evaluation of climate models and for the interpretation and validation of remote sensing products, but also for the quantification of climatological changes and for process understanding in general. The data are openly available at  https://doi.pangaea.de/10.1594/PANGAEA.974080.

How to cite: Van Tiggelen, M., Smeets, P., Reijmer, C., Kuipers Munneke, P., and van den Broeke, M.: 30 years of Antarctic weather station observations by the IMAU network (1995-2025), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9051, https://doi.org/10.5194/egusphere-egu25-9051, 2025.

EGU25-9646 | Posters on site | AS4.1

Interconnections between the components of the Antarctic climate system: a causal inference approach 

Sebastian Berghald, Nicole Van Lipzig, Hugues Goosse, and Stef Lhermitte

Antarctica and the Southern Ocean have an important role in Earth's climate, influencing global heat balance and carbon uptake. Recent anomalies, such as drastic sea ice decline, anomalous snowfall, and unprecedented heat waves challenge our understanding of the region's climate response. Both internal (local processes) and external (influence from lower latitudes) factors have been suggested as drivers of this variability, but the relative contributions of these remain unknown due to the lack of observations as well as shortcomings in climate models. We aim to enhance the understanding of this system by making use of recent advances in causal effect estimation. Going beyond correlation, causal network reconstruction aims to detect cause-effect links and their strength from observational datasets, including satellite records and reanalysis data. For selected sectors of Antarctica, the interconnections between ice sheet surface mass balance (SMB), sea ice, ocean temperature, and meridional transport of heat and water from lower latitudes are examined and causal relationships identified and quantified.

How to cite: Berghald, S., Van Lipzig, N., Goosse, H., and Lhermitte, S.: Interconnections between the components of the Antarctic climate system: a causal inference approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9646, https://doi.org/10.5194/egusphere-egu25-9646, 2025.

EGU25-10147 | ECS | Posters on site | AS4.1

Glacier-Climate Interactions across Time: A West Greenland Case Study  

Florina Roana Schalamon, Lindsey Nicholson, Sebastian Scher, Andreas Trügler, Wolfgang Schöner, and Jakob Abermann

Altitude-driven gradients of air temperature, humidity, wind, and surface mass balance play a critical role in understanding glacier-climate interactions, particularly in regions of rapid environmental change like the Arctic. In this study, we compare datasets from Alfred Wegener’s last expedition to the west coast of Greenland in 1930/31 with a modern measurement network established at the same locations in 2022. This unique comparison offers insights into how the atmospheric and glacial conditions have changed within a century.  
The measurement network consists of one automatic weather station at the coast over bare ground in vicinity of the outlet glacier Qaamarujup Sermia and another at 940 m a.sl. on the Greenland Ice Sheet. For both locations observations exist during the Wegener expedition and since 2022. Additionally, temperature and humidity sensors and surface mass balance measurements distributed between these two points provide high-resolution spatial data.  
The observed gradients in air temperature, humidity, wind speed, and wind direction are analysed at multiple temporal scales, from diurnal cycles to annual variations. Preliminary results show that the air temperature gradient between the coastal and the glacier station follows a seasonal cycle by being the smallest in spring (on average –6.5 °C) and the largest in winter (on average –11°C). Although this is true in the historic and modern dataset, the gradient in spring is colder in 2023 and 2024 with –7.0°C and –6.7°C respectively versus –5.7°C in 1931. The summer gradient is warmer in the modern dataset from -8.3°C in 1930, -9.3°C in 1931 to -7.7°C in 2023 and -7.8°C in 2024.  
Our goal is to understand the key factors shaping these gradients, including the influence of large-scale atmospheric patterns such as the Greenlandic Blocking Index and North Atlantic Oscillation and the prevailing regional conditions identified through self-organizing maps. By comparing historical and modern datasets, we further examine how changes in glacier geometry and a frontal retreat of approximately 2 km since the 1930s have shaped climatic gradients. A particular focus is placed on whether this influence is more pronounced at the coastal or the glacier station.  
This work contributes to the broader understanding of how glacier-climate interactions are influenced by both local and large-scale factors and underscores the value of historic observational records in assessing climate change impacts. 

How to cite: Schalamon, F. R., Nicholson, L., Scher, S., Trügler, A., Schöner, W., and Abermann, J.: Glacier-Climate Interactions across Time: A West Greenland Case Study , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10147, https://doi.org/10.5194/egusphere-egu25-10147, 2025.

EGU25-11681 | Posters on site | AS4.1

Surface radiation budget data in a bipolar perspective: observations, comparison and exploiting for products. 

Alice Cavaliere, Claudia Frangipani, Daniele Baracchi, Francesca Becherini, Angelo Lupi, Mauro Mazzola, Simone Pulimeno, Dasara Shullani, and Vito Vitale

Clouds modulate the net radiative flux interacting with both shortwave and longwave radiation, but the uncertainties regarding their effect in polar regions are especially high, because ground observations are lacking and evaluation through satellites is made difficult by the high surface reflectance. In this work, the radiative regimes and sky conditions for five different stations, two in the Arctic (Ny-Ålesund, 78.92°N, 11.93°E,  Barrow, 71.32°N, 156.61° W) and four in Antarctica (Neumayer, 70.68°S, 8.27°W; Syowa,  69.01°S, 39.58°E; South Pole, 90°S, 0°E ; DomeC, 75.01°S, 123.33°E) will be presented, considering the decade between 2010 and 2020. Measurements of broadband shortwave and longwave radiation components (both downwelling and upwelling) are collected within the frame of the Baseline Surface Radiation Network (BSRN) (Driemel et al. 2018). Observations, together with  identification of the clear sky and overcast conditions will be compared with ERA5 reanalysis (Herschbach et al., 2023). Furthermore, the identified conditions based on estimated cloud fraction will serve as labels for a machine learning classification task, leveraging algorithms such as Random Forest and Long Short-Term Memory (LSTM) networks (i.e. Zeng et al., 2021; Sedlar et al., 2021). These models incorporate features including global and diffuse shortwave radiation, downward longwave radiation, solar zenith angle, surface air temperature, relative humidity, and the ratio of water vapor pressure to surface temperature. The Random Forest model will also compute feature importance, identifying the most influential variables in predicting sky conditions and providing insights into the relationships between these meteorological factors.

Bibliography

Driemel et al. (2018): Baseline Surface Radiation Network (BSRN): structure and data description (1992–2017). 

Riihimaki et al. (2019): Radiative Flux Analysis (RADFLUXANAL) Value-Added Product.

Hersbach, H. et al. (2023): ERA5 hourly data on single levels from 1940 to present. Copernicus Climate Change Service (C3S) Climate Data Store (CDS) 

Zeng, Z. et al. (2021): Estimation and Long-term Trend Analysis of Surface Solar Radiation in Antarctica: A Case Study of Zhongshan Station. Adv. Atmos. Sci. 38, 1497–1509. 

Sedlar, J. et al. (2021): Development of a Random-Forest Cloud-Regime Classification Model Based on Surface Radiation and Cloud Products. J. Appl. Meteor. Climatol., 60, 477–491.

How to cite: Cavaliere, A., Frangipani, C., Baracchi, D., Becherini, F., Lupi, A., Mazzola, M., Pulimeno, S., Shullani, D., and Vitale, V.: Surface radiation budget data in a bipolar perspective: observations, comparison and exploiting for products., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11681, https://doi.org/10.5194/egusphere-egu25-11681, 2025.

EGU25-12116 | Orals | AS4.1

Melting energy sources in rainfall conditions over Pine Island Bay, Antarctica. 

Denys Pishniak, Ella Gilbert, Larysa Pysarenko, and Andrew Orr

The case of a strong heat anomaly around Pine Island Bay is examined. This region of west Antarctica is well known for its rapidly thinning and accelerating marine-terminating glaciers. Polar-WRF model simulations were used to investigate the atmospheric structure, dynamic and energy fluxes of this event at high spatial resolution. The modeling discovered a hot spot that formed due to the development of relatively large-scale foehn phenomena at the basin of Pine Island Glacier (PIG). The thickness of the positive temperature layer over this region can exceed 1 km with a maximum of +8ºC. The layering of several warm air masses, accompanied by atmospheric rivers, causes significant liquid precipitation over coastal glaciers and ice shelves.  In such rare cases precipitation makes the main contribution to heat flux directed from atmosphere to the surface. The flux can reach up to 400 W m-2 in the form of latent heat (which may release later). Direct heat transfer is also contributing to surface warming as a negligible part of the heat balance. We also tried to estimate a nonlinear dependence of precipitation heat fluxes in relation to atmosphere warming.  Finally, Noah LSM used in WRF model has some simplicities that make it not an ideal instrument for estimation of precipitation heat fluxes in polar regions. Although precipitation distribution and local wind patterns are sensitive to topography representation and demand high model resolution for estimation accuracy.

How to cite: Pishniak, D., Gilbert, E., Pysarenko, L., and Orr, A.: Melting energy sources in rainfall conditions over Pine Island Bay, Antarctica., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12116, https://doi.org/10.5194/egusphere-egu25-12116, 2025.

EGU25-12294 | ECS | Posters on site | AS4.1

Evolution of precipitations and snow depth over the Arctic sea ice modeled by the regional climate model MAR 

Clara Lambin, Christoph Kittel, Damien Maure, Brice Noël, and Xavier Fettweis

The Arctic is experiencing changes in precipitation, both in terms of amount and phase, due to rising temperatures. Key mechanisms contributing to these changes include increased poleward moisture transport and higher ocean evaporation resulting from the shrinking sea ice cover. In autumn, changes in precipitation over the sea ice can influence its growth by altering the insulation between the ocean and the atmosphere. A reduction in snow cover (which has lower insulating properties) enables the ocean to cool faster by releasing heat into the atmosphere, thus promoting sea ice growth. In spring, variations in snowfall and rainfall can affect the sea ice albedo, influencing its melting rate. Using the regional climate model MAR, which includes a complex snow scheme, we examine trends in precipitation and snow depth over the Arctic sea ice during the growth season. We also conduct sensitivity tests to assess the response of snow depth to changes in sea ice thickness.

How to cite: Lambin, C., Kittel, C., Maure, D., Noël, B., and Fettweis, X.: Evolution of precipitations and snow depth over the Arctic sea ice modeled by the regional climate model MAR, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12294, https://doi.org/10.5194/egusphere-egu25-12294, 2025.

EGU25-13156 | Posters on site | AS4.1

Polar-to-midlatitude teleconnections in a warming world: Statistical relationships from large ensembles 

Carley Iles, Bjørn Samset, and Marianne Lund

How are polar-to-midlatitude teleconnections represented in recent large ensembles of coupled climate model simulations? And how do they evolve with global warming? Using the rich information on internal variability available from large ensembles, we investigate the relationship between sea ice amount and atmospheric circulation for both Arctic and Antarctic sea ice variability in CESM2 and ACCESS-ESM1-5, using a composite analysis. We find that the links between sea ice and sea level pressure (SLP), the midlatitude jet stream and temperature depend on the region in which sea ice varies, for instance with low Barents-Kara sea ice in January being associated with a positive North Atlantic Oscillation SLP pattern and high pressure over Northern Eurasia. These circulation patterns persist with increased levels of global warming, until around 3 or 4°C when they start to evolve in some cases, as sea ice starts to disappear. Surface air temperatures are anomalously high around the region of sea ice retreat with varying patterns of remote cooling elsewhere. Lagged analysis shows that sea-ice circulation relationships when the atmosphere leads sea ice are very similar to the instantaneous relationships, suggesting that the latter largely reflects the atmospheric patterns leading to reduced sea ice. For positive lags (sea ice leading the atmosphere), for some regions the SLP teleconnections persist in a weakened state for subsequent months, whilst for others they evolve, e.g. into a negative Arctic Oscillation response for Barents-Kara sea ice reduction. However, results for positive lags differ between the two models examined. SLP relationships with Antarctic sea ice are model dependent, but feature a negative Southern Annular Mode pattern in ACCESS-ESM1-5. In CESM2, we find a less zonally symmetric pattern which also consists of high pressure over the pole in Autumn and Winter.

How to cite: Iles, C., Samset, B., and Lund, M.: Polar-to-midlatitude teleconnections in a warming world: Statistical relationships from large ensembles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13156, https://doi.org/10.5194/egusphere-egu25-13156, 2025.

EGU25-13164 | ECS | Orals | AS4.1

The Key Role of the Southern Annular Mode During the Seasonal Sea Ice Maximum in Recent Antarctic Sea Ice Loss 

Chloe Boehm, David W.J. Thompson, and Edward Blanchard-Wrigglesworth

Southern Hemisphere sea ice area (SH SIA) exhibited weak increases from the early 1980s until 2015 when it abruptly dropped, setting record low values in 2017, 2022, and 2023. The reasons for the rapid declines in SH SIA remain open to debate, with potential explanations ranging from changes in tropical Pacific climate, warming of the high latitude subsurface ocean, and contemporaneous variations in the extratropical atmospheric circulation. Here we provide novel insights into the role of the extratropical atmospheric circulation in driving year-to-year and long-term changes in Antarctic sea ice, with a focus on the influence of the Southern annular mode (SAM) on recent trends in SH sea ice area. The influence of the SAM on SH SIA exhibits a more pronounced seasonal variation than that indicated in previous work: during the annual sea ice minimum, anomalous circumpolar westerlies associated with the positive polarity of the SAM lead to increases in SH SIA that persistent for several months. In contrast, during the annual sea ice maximum, anomalous circumpolar westerlies associated with the positive polarity of the SAM lead to pronounced decreases in Antarctic sea ice that persist for up to a year. In terms of annual-mean SH SIA, by far the largest impacts arise from variations in the atmospheric circulation during the sea ice maximum. As a result, changes in the SAM during the sea ice maximum have had a marked impact on long-term changes in SH SIA. These linkages are robust in both observationally constrained data products and modeled data, with additional results exploring how this relationship changes as the mean state of the climate changes under global warming.

How to cite: Boehm, C., Thompson, D. W. J., and Blanchard-Wrigglesworth, E.: The Key Role of the Southern Annular Mode During the Seasonal Sea Ice Maximum in Recent Antarctic Sea Ice Loss, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13164, https://doi.org/10.5194/egusphere-egu25-13164, 2025.

EGU25-13984 | ECS | Posters on site | AS4.1

Quality-controlled meteorological datasets from SIGMA automatic weather stations in northwest Greenland 

Motoshi Nishimura, Teruo Aoki, Masashi Niwano, Sumito Matoba, Tomonori Tanikawa, Tetsuhide Yamasaki, Satoru Yamaguchi, and Koji Fujita

In situ meteorological data are essential for a better understanding of the ongoing environmental changes in the Arctic. In order to increase the scientific value of discussions on understanding the actual state of environmental change in a given area, it is necessary to appropriately remove the anomalous values recorded due to external factors resulting from low temperature and icing. Here we present methods for quality control (QC) of meteorological observation datasets from two automatic weather stations in northwest Greenland, where drastic glaciological and meteorological environmental changes have occurred. The stations were installed in the accumulation area of the Greenland Ice Sheet (SIGMA-A site, 1490 m a.s.l.) and near the equilibrium line of the Qaanaaq Ice Cap (SIGMA-B site, 944 m a.s.l.). We describe the two-step sequence of QC procedures we used to produce increasingly reliable data sets by masking erroneous records. This method was developed for the climatic conditions of Greenland, however, it is designed to be as universally applicable as possible, with a basis in meteorology and glaciology, and with the intention of removing the subjectivity of the person performing the QC. The QC is divided into two processes: Initial Control and Secondary Control. Initial Control removes values that violate physical laws and also serves as a preliminary process to improve the accuracy of Secondary Control. Secondary Control removes abnormal values using stricter statistical criteria than Initial Control. As a result of this two-step process, controlled by scientifically objective criteria, we were able to successfully remove erroneous data sets and greatly reduce the time required for QC. In addition, by using a generally applicable process, we were able to successfully establish an algorithm that could be applied to multiple sites. The data sets from both the SIGMA-A and SIGMA-B sites were classified into three levels (Level 1.1 to Level 1.3) according to the stage of data processing. Level 1.1 is the so-called raw data, in which the data for the period when the logger was stopped are masked (processed to flag them as missing or abnormal), the so-called raw data. Level 1.2 and Level 1.3 are datasets to which Initial Control and Secondary Control have been applied to the Level 1.1 and Level 1.2 datasets, respectively, and the Level 1.3 dataset is a dataset from which all abnormal values have been removed. These datasets have been archived in the Arctic Data Archive System (ADS) operated by the National Institute of Polar Research in Japan (e.g., Level 1.3 dataset: SIGMA-A - https://doi.org/10.17592/001.2022041303 and SIGMA-B - https://doi.org/10.17592/001.2022041306).

How to cite: Nishimura, M., Aoki, T., Niwano, M., Matoba, S., Tanikawa, T., Yamasaki, T., Yamaguchi, S., and Fujita, K.: Quality-controlled meteorological datasets from SIGMA automatic weather stations in northwest Greenland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13984, https://doi.org/10.5194/egusphere-egu25-13984, 2025.

EGU25-14448 | ECS | Posters on site | AS4.1

Coupled Influence of Synoptic Weather and Topographic Control on Near-surface Wind Variability in the Denman Glacier Basin, East Antarctica 

Zhaohui Wang, Laurie Menviel, Alex Sen Gupta, Ian Goodwin, Zijian Chen, and Thomas Caton Harrison

Denman Glacier Basin, a critical region for studying polar ice dynamics and climate change impacts, is heavily influenced by the combination of topographic and atmospheric conditions, particularly experiencing strong downslope winds. This study examines the structure and variability of near-surface winds in the basin, focusing on the influence of large-scale circulation, synoptic weathers, and local orographic effects. Through high-resolution atmospheric simulation experiments, we demonstrate the forced components of near-surface winds during prevalent synoptic systems in the area, quantifying the roles of large-scale and locally driven forces in shaping wind structure and variability. We also conduct perturbation experiments with topographies of varying resolutions to examine the orographic controls on the spatial climatology of downslope winds, in response to a range of synoptic systems typical to the region. Our findings can be used to clarify uncertainties in interpreting snow accumulation variability in ice cores and determining whether modern regional mass balance trends result from increased glacial discharge or shifts in synoptic circulation. This research findings will be used to interpret the Denman Glacier discharge, snow accumulation over the basin, aiding in the interpretation of recent ice core data collected in the recent field season.

 

How to cite: Wang, Z., Menviel, L., Sen Gupta, A., Goodwin, I., Chen, Z., and Caton Harrison, T.: Coupled Influence of Synoptic Weather and Topographic Control on Near-surface Wind Variability in the Denman Glacier Basin, East Antarctica, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14448, https://doi.org/10.5194/egusphere-egu25-14448, 2025.

EGU25-14582 | ECS | Orals | AS4.1

Extreme Precipitation in the Cyrosphere: Atmospheric River Interaction with Antarctic Sea Ice 

Gabrielle Linscott, Chelsea Parker, Linette Boisvert, and Elina Valkonen

In 2016, Antarctic sea ice experienced a regime shift when a persisting decreasing trend emerged from a relatively stable annual cycle. Drivers of the sea ice regime shift and future projections of Southern Ocean sea ice remain unresolved. One possible contributing phenomena are atmospheric rivers (ARs), which are long, narrow, and transient features responsible for the majority of global poleward water vapor transport. Though infrequent over Antarctica, ARs wield a substantial influence on the Antarctic ice mass balance. Previous studies highlight their significance, attributing 35% of the interannual precipitation variability over the Antarctic Ice Sheet (AIS) to ARs. The interaction between ARs and Antarctic sea ice has not been as clearly defined. Our ongoing work uses ERA5 reanalysis data, results from an AR tracking algorithm, and passive microwave sea ice concentration data from 1980 to 2023 to examine the relationship between ARs and Antarctic sea ice, especially in the context of the changing sea ice state. In this study, we explore the relationship between AR activity and sea ice area at a region and seasonal scale, then analyse the contribution of ARs to precipitation over sea ice and how that contribution has changed through the 40-year study period. On average, ARs can be attributed with 11% of total precipitation, 11% of snowfall, and 13% of rain over Antarctic sea ice. While the AR contribution to sea ice snowfall is fairly consistent through the year, the predominant AR contribution to rain rotates around the Southern Ocean sequentially by season. The strongest signal of AR precipitation over sea ice is in the Weddell Sea winter, when ARs constitute 25% of winter rain. The trends of these contributions vary by season and by region. For example, while AR precipitation on sea ice has an increasing trend across all types of precipitation in each season in the Weddell Sea, the opposite is true for the Ross Sea. These findings underscore the importance of the AR interaction with Antarctic sea ice, particularly in the context of seasonal and regional variability and change. This work will improve our understanding of the spatiotemporal variability and trends of ARs as precipitation mechanisms, which is vital for understanding and predicting sea ice mass balance in a changing climate.

How to cite: Linscott, G., Parker, C., Boisvert, L., and Valkonen, E.: Extreme Precipitation in the Cyrosphere: Atmospheric River Interaction with Antarctic Sea Ice, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14582, https://doi.org/10.5194/egusphere-egu25-14582, 2025.

EGU25-15568 | ECS | Posters on site | AS4.1

Emulating Greenland Ice Sheet Surface Melt Using Graph Neural Networks 

Ziqi Yin, Aneesh Subramanian, and Rajashree Datta

As global mean temperatures exceeded the 1.5 °C threshold in 2024, the urgency to better quantify the impacts of global warming, including sea level rise contributions from polar ice sheets, has intensified. The Greenland Ice Sheet (GrIS) has experienced significant mass loss over recent decades, primarily driven by surface melting, a process expected to accelerate under continued warming. Surface melt is influenced by a combination of factors and complex interactions between atmosphere and ice sheet surface, but simulating these processes using coupled climate models is computationally expensive and often impractical.

In this study, we develop a graph neural network (GNN) as an emulator for GrIS surface melt, trained on output from the Community Earth System Model version 2 (CESM2), which explicitly calculates surface melt through a downscaled surface energy balance framework. GNNs are uniquely suited to this task, as they capture spatial and relational dependencies across the ice sheet, enabling the emulator to reproduce spatially resolved melt fields and identify the influence of key atmospheric patterns.

We will first evaluate the emulator’s performance in replicating CESM2 simulated melt under different climatic conditions and employ explainability techniques to identify the relative importance of key atmospheric patterns in driving surface melt. This work aims to demonstrate the utility of machine learning emulators in enhancing our understanding of GrIS surface melt dynamics and advancing projections of sea level rise under future climate scenarios.

How to cite: Yin, Z., Subramanian, A., and Datta, R.: Emulating Greenland Ice Sheet Surface Melt Using Graph Neural Networks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15568, https://doi.org/10.5194/egusphere-egu25-15568, 2025.

Greenland's contribution to global mean sea level exhibits decadal variability, driven by interannual surface mass balance (SMB) changes. In this study, we attribute historical Greenland SMB changes to radiative forcings using the Community Earth System Model version 2 Large Ensemble and its single-forcing Large Ensemble simulations (CESM2-LE and CESM2-SFLE), which enables separation of impacts from greenhouse gases and aerosols. We quantify the contribution of radiative forcings to Greenland SMB changes by estimating univariate and multivariate detection and attribution scaling factors through Bayesian total least squares regression implemented via Markov Chain Monte Carlo (MCMC). The MCMC formulation allows us to quantify the uncertainty of the scaling factors using prior knowledge from observation-based simulations and reconstructions, as well as CESM2-LE and CESM2-SFLE. Our results indicate that historical Greenland SMB changes can be attributed to anthropogenic forcings, including anthropogenic aerosols, which affect decadal scale variability superimposed on the greenhouse gas-driven long-term trend. However, CESM2 tends to underestimate the relative contribution of each individual forcing to observed historical Greenland SMB changes. To explore potential reasons for this underestimation, we test a few hypotheses, including the role of internal variability. Our analysis demonstrates that internal variability plays only a minor role in the underestimation of the forced Greenland SMB changes due to individual forcings. Additionally, we find that Greenland runoff changes, rather than precipitation changes, explain both the SMB changes and the underestimation of attributable portions to individual forcings. Our findings emphasize the confounding role of aerosol forcing on the historical SMB trajectory but also highlight outstanding questions regarding the ability of climate models to correctly parse such influences. We will discuss the implications of these issues and steps to address them.

How to cite: Kuo, Y.-N., Culberg, R., and Lehner, F.: Assessing the portion of historical Greenland surface mass balance change attributable to anthropogenic forcing and its uncertainties, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15676, https://doi.org/10.5194/egusphere-egu25-15676, 2025.

EGU25-15824 | ECS | Orals | AS4.1

Exploring atmospheric transport into the Arctic 1940 to 2023 - A Lagrangian Perspective 

Andreas Plach, Lucie Bakels, and Andreas Stohl

The Arctic is a key component of the Earth’s climate system and has received much attention in recent years due to it’s above-average warming (Arctic Amplification). Furthermore, we know that the Arctic is not a closed system, but is influenced by atmospheric transport from lower latitudes, a fact that for example can be observed during spring when polluted air transported from lower latitudes regularly leads to a reduction in visibility (Arctic Haze).

In order to better understand the observed warming and pollution events we investigate circulation and transport patterns in the Arctic by calculating residence times, following air particle trajectories to and from the Arctic, and studying the dynamical characteristics of the Polar Dome. For our investigation we employ a newly created Lagrangian Reanalysis (LARA) dataset which is based on global simulations with the Lagrangian Particle Dispersion Model FLEXPART forced with ERA5 reanalysis data for the period 1940 to 2023.

Similar to a previous study we find average Arctic residence times in the order of one (January) to two weeks (July). Preliminary results indicate that these residence times have changed most during the transition months, especially in spring (e.g., shorter Arctic residence times in April at present than in the mid-20th century). However, we find strong spatial differences in residence times and in their changes over time. In this presentation we aim to discuss the seasonal and spatial characteristic of the residence times, investigate potential pollution source regions, explore the dynamical characteristics of the Polar Dome, and analyze how all of this has changed between 1940 and 2023. Furthermore, we plan to investigate the relation of observed dynamical changes to changes in sea ice, North Atlantic Oscillation, and other observations.

How to cite: Plach, A., Bakels, L., and Stohl, A.: Exploring atmospheric transport into the Arctic 1940 to 2023 - A Lagrangian Perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15824, https://doi.org/10.5194/egusphere-egu25-15824, 2025.

EGU25-15984 | ECS | Posters on site | AS4.1

Pathways of Atmospheric Rivers in the Arctic: Dynamics, Moisture Transport, and Impacts on Sea Ice during April 2020 

Luisa E. Aviles Podgurski, Patrick Martineau, Hua Lu, Ayako Yamamoto, Tony Phillips, Tom Bracegirdle, Amanda C. Maycock, Andrew Orr, Andrew Fleming, Anna E. Hogg, and Grzegorz Muszynski

In recent decades, the Arctic has warmed nearly four times faster than the global average, undergoing profound changes as a result. A key factor in this accelerated warming is the meridional transport of atmospheric water vapour. Particularly, intense intrusions of moisture and heat, so-called atmospheric rivers (ARs), are rare phenomena to reach the high latitudes, but can have severe impacts on the Arctic environment.

In this study, we examine an AR pair in April 2020 using a combination of Eulerian and Lagrangian methods alongside observational data from Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition. The event consisted of two distinct ARs that followed separate pathways - one across Siberia and the other across the Atlantic - before converging in the central Arctic within the span of one week. Large-scale atmospheric circulation patterns associated with these ARs show a combination of low and high pressure systems on the flanks of the ARs, channelling moisture and heat northward. Notably, our results show that the Siberian AR was linked to extreme heat anomalies, whereas the Atlantic AR primarily transported abundant moisture.

Backward air parcel trajectories calculated using LAGRANTO provide new insights into the complex dynamics of Arctic ARs, revealing details of their distinct pathways and moisture source regions. Analysis of these trajectories also uncovers a strong connection between the observed sea ice melt in the Barents-Kara Sea and the interaction of an AR with the ice edge, underscoring the significant influence of ARs on the Arctic climate system.

How to cite: Aviles Podgurski, L. E., Martineau, P., Lu, H., Yamamoto, A., Phillips, T., Bracegirdle, T., Maycock, A. C., Orr, A., Fleming, A., Hogg, A. E., and Muszynski, G.: Pathways of Atmospheric Rivers in the Arctic: Dynamics, Moisture Transport, and Impacts on Sea Ice during April 2020, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15984, https://doi.org/10.5194/egusphere-egu25-15984, 2025.

EGU25-16387 | Posters on site | AS4.1

Characteristics of Strong Winds at Jang Bogo Station in East Antarctica: An 8-Year Observational Study 

Hataek Kwon, Yonghan Choi, and Sang-Jong Park

This study investigates the characteristics and mechanisms of strong winds at Jang Bogo Station (74°37'S, 164°12'E) in Terra Nova Bay, East Antarctica, using 8 years (2015-2022) of Automated Synoptic Observation System (ASOS) data and ERA5 reanalysis data. Analysis of strong wind patterns reveals two distinct strong wind regimes: southwesterly (180-270°) and northwesterly (270-360°) winds. Strong wind events show clear seasonal variation, with peak frequencies occurring in March and July. Synoptic analysis using ERA5 reanalysis data indicates that these strong winds are primarily driven by the interaction between the Amundsen Sea Low and the Antarctic continental high pressure system. The intensity and positioning of these pressure systems significantly influence both wind direction and speed at Jang Bogo Station. Notably, the strongest winds (top 1%) are predominantly northwesterly, associated with enhanced pressure gradients near the station. Case studies of extreme wind events reveal two distinct generating mechanisms: one associated with intense pressure gradients from passing cyclonic systems, and another linked to katabatic flows descending from the Antarctic interior. These findings provide important insights into the wind regime of Terra Nova Bay and contribute to our understanding of Antarctic meteorological patterns, which has implications for both operational forecasting and regional climate studies.

How to cite: Kwon, H., Choi, Y., and Park, S.-J.: Characteristics of Strong Winds at Jang Bogo Station in East Antarctica: An 8-Year Observational Study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16387, https://doi.org/10.5194/egusphere-egu25-16387, 2025.

EGU25-17914 | ECS | Orals | AS4.1

EC-Earth- and ERA5-driven retrospective ensemble hindcasts with the fully coupled ice-sheet–ocean–sea ice–atmosphere–land circum-Antarctic model PARASO 

Florian Sauerland, Pierre-Vincent Huot, Sylvain Marchi, Hugues Goosse, and Nicole van Lipzig

We present 4 retrospective hindcasts using PARASO, a five-component (ice sheet, ocean, sea ice, atmosphere, and land) fully coupled regional climate model over an Antarctic circumpolar domain: a control run forced at its boundaries with reanalysis data from ERA5 and ORAS5, and an ensemble of 3 members forced by 3 different EC-Earth global hindcasts. The ERA5 driven hindcast is shown to accurately simulate the increase in maximum sea ice extent observed prior to 2014. This trend being absent from the EC-Earth driven hindcasts, with strong intra-ensemble agreement, suggests a large influence of mid-latitude forcings, rather than a misrepresentation of local processes in global models. We analyse other factors possibly contributing to the diverging sea ice trends, such as ocean temperature and large-scale circulation patterns, and the spatial pattern of these sea ice changes. It is shown that all simulations display a sea ice retreat in the Amundsen Sea, which has previously been shown to be related to the intensification of the Amundsen Sea Low. Similarly, they all display an increase in sea ice extent in the Indian ocean sector, off of Enderby Land and the Amery Ice Shelf. However, the spatial extent of these areas differs between the ERA5 and EC-Earth driven hindcasts, and the trend diverges around the Antarctic Peninsula and in the Weddell Sea.

Furthermore, we explore how the diverging sea ice extent trends are translating into diverging evaporation trends, which in turn results in diverging moisture transport and surface mass balance trends for the Antarctic continent, even though all hindcasts once again agree on an increasing trend of moisture transport from the mid-latitudes. It is demonstrated that the EC-Earth driven hindcasts agree on most trends affecting the surface climate in Antarctica and the Southern Ocean, both in intensity and spatial pattern. However, the trends seen over the continent are less consistent between the EC-Earth ensemble members, compared to the ones seen over the Southern Ocean, indicating a larger influence of internal variability.

How to cite: Sauerland, F., Huot, P.-V., Marchi, S., Goosse, H., and van Lipzig, N.: EC-Earth- and ERA5-driven retrospective ensemble hindcasts with the fully coupled ice-sheet–ocean–sea ice–atmosphere–land circum-Antarctic model PARASO, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17914, https://doi.org/10.5194/egusphere-egu25-17914, 2025.

EGU25-19587 | ECS | Posters on site | AS4.1

Investigating the drivers of future changes in Arctic aerosols in UKESM1 using a Lagrangian air-mass trajectory framework 

Prerita Agarwal, Laura J. Wilcox, Steven T. Turnock, and Daniel Partridge

Aerosols are well-known climate forcers, yet their climatic impact on the Earth’s radiative budget remains uncertain. One of the reasons for this is poor representation of the aerosol-cloud interaction (ACI) process in the current Global Climate models (GCMs). Aerosol number size distributions in the atmosphere influence key ACI-relevant aerosol and cloud properties and, therefore, need to be accurately represented in GCMs. Understanding aerosol sources and sinks in pristine polar regions is crucial for improving climate projections, as several studies highlight the poor performance of GCMs in these areas. Moreover, it offers the advantage of understanding the impact of future changes in transport patterns on aerosol-climate feedback in sensitive background regions. To this end, improved representation of the regional distribution of aerosol emissions, and their temporal variations in climate models for near-term projections is a crucial gap that needs urgent attention. As the European Union (EU) aims to be climate-neutral by 2050, this study seeks to advance our understanding of aerosol life cycle processes in response to future regional emission changes.

We capitalise on a recently developed framework from the AeroCom Phase III GCM Trajectory (GCMTraj ) experiment, which leverages GCM meteorological fields to calculate the air-mass trajectories (Kim et al., 2020). Our work utilises the free-running and nudged UKESM1-0-LL versions from Regional Aerosol Model Intercomparison Project (RAMIP) simulations to calculate the trajectories and perform a spatio-temporal collocation of aerosol diagnostics. Here, we explore the various shared socioeconomic pathways (SSP370 and SSP370-126aer) from RAMIP to compare the impacts of global warming and aerosol reductions on future aerosol trends. This is the first time the free-running simulations from RAMIP have been used to calculate future air-mass trajectories. Using these trajectories we analyse the changes in source-receptor trends resulting from significant regional emission reductions in the post-fossil Arctic aerosol regime (2050) at Mt. Zeppelin.

We find continental air-mass transport from the northwest, Nordic and Siberian regions, towards the receptor site, Mt. Zeppelin and a strong seasonal variation in the transport patterns between 2010-2014 and 2046-2050. These results contrast with trajectories derived from ERA-Interim, ERA5 reanalysis and UKESM1 (nudged version), which reveal dominant air mass transport from the south-west, Eurasia and the northern Atlantic Ocean between 2010-2014. The results demonstrating seasonal characteristics of aerosol sources and sinks owing to changes in future circulation and emission patterns will be presented. This work will help improve knowledge of ACI evolution in response to changes in regional emission trends in the post-fossil remote aerosol regime. 

How to cite: Agarwal, P., J. Wilcox, L., T. Turnock, S., and Partridge, D.: Investigating the drivers of future changes in Arctic aerosols in UKESM1 using a Lagrangian air-mass trajectory framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19587, https://doi.org/10.5194/egusphere-egu25-19587, 2025.

EGU25-614 | ECS | Posters on site | ITS5.7/AS4.3

Evaluating a Parameterization for Sublimation of Blowing Snow with In-situ Observations in the Arctic 

Lukas Monrad-Krohn, Maximilian Maahn, Markus Frey, and Stephen J. Déry

Surface albedo, sea ice growth and glacier mass balance in the Arctic are all heavily dependent on snow and thus also impacted by blowing snow through redistribution and increased sublimation. The sublimation of blowing snow is significantly higher than that of ground snow due to the larger surface area of the suspended snow crystals and the continuous entrainment of dry air. Thus, sublimation of blowing snow impacts the exchange of energy, moisture and particles between the snow and atmosphere in windy conditions.

Because of the difficulty of modelling such a small-scale process for large areas, parameterizations of sublimation of blowing snow are necessary for snow mass balance and aerosol production studies. The widely used Déry and Yau (2001) parameterization has only been evaluated with model data from the Canadian Prairie, but never for other surface types, where it is applied, or with in-situ observations. Therefore, the goal of this work is to evaluate the parameterization by Déry and Yau (2001) with observations from the MOSAiC expedition in the central Arctic and the Intensive Observation Period for Water (IOP4H20) field measurements in Ny-Ålesund, Svalbard.

Here we show observations of blowing snow events that were detected and characterized by a snow particle counter and the Video In-Situ Snowfall Sensor (VISSS). During these events, measurements of latent heat fluxes from eddy covariance systems are used to evaluate the parameterized sublimation rate. To address challenges with eddy covariance observations in snowy conditions and calculating column-integrated values the observations are complemented with the 1D-column PIEKTUK-D blowing snow model.

In this way, comparing the parameterization with observations brings insights into its uncertainty or possible limitations for two different surface types and thereby improves the estimation of the accuracy of snow mass balance and aerosol production studies that apply this parameterization.

How to cite: Monrad-Krohn, L., Maahn, M., Frey, M., and Déry, S. J.: Evaluating a Parameterization for Sublimation of Blowing Snow with In-situ Observations in the Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-614, https://doi.org/10.5194/egusphere-egu25-614, 2025.

EGU25-731 | ECS | Orals | ITS5.7/AS4.3

Simulating aerosol and cloud properties over coastal Antarctica in a high resolution regional model 

Zhangcheng Pei, Sonya Fiddes, Marc Mallet, Simon Alexander, Kalli Furtado, Calum Knight, Greg Roff, Daniel Smith, Alain Protat, Adrian McDonald, and John French

Global climate models and reanalysis products have revealed large downwelling shortwave radiation biases over the Southern Ocean and Antarctica. The biases are hypothesized to be caused by the incapability of models to accurately simulate the frequent occurrence of low-level mixed-phase clouds in these regions. It’s crucial to elucidate the intricacy of cloud microphysics and aerosol-cloud interaction in climate models over the Southern Ocean and Antarctica in order to better simulate the climate system.

In this study, we use the ground-based observations colleted at Davis, East Antarctica to assess the capability of the high-resolution regional Unified Model (UM) to reproduce precipitating clouds off coastal Antarctica. We found the default configuration of the model can generally simulate the phase, vertical structure, and timing of clouds while exhibiting biases in the simulated water path and surface radiation fluxes compared to observations. A series of sensitivity tests with changed cloud and aerosol properties were conducted. The key findings suggest that: (1) Current monthly aerosol climatology implemented in the UM for cloud droplet activation largely underestimates aerosol concentrations, leading to fewer cloud droplets and worse radiation biases; (2) Increasing the cloud droplet number concentrations to a maximum satellite-based value doesn’t have a significant impact on liquid water path (LWP) and radiation biases; (3) A more realistic ice nucleating particle parameterization significantly increases the LWP and reduces temperature and radiation biases at coastal Antarctica. Moreover, preliminary results from coupling CASIM and GLOMAP aerosol schemes in the UM evaluated with ship-based observations over high-latitude Southern Ocean will be presented.

How to cite: Pei, Z., Fiddes, S., Mallet, M., Alexander, S., Furtado, K., Knight, C., Roff, G., Smith, D., Protat, A., McDonald, A., and French, J.: Simulating aerosol and cloud properties over coastal Antarctica in a high resolution regional model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-731, https://doi.org/10.5194/egusphere-egu25-731, 2025.

EGU25-752 | ECS | Orals | ITS5.7/AS4.3

Local Production of Arctic Sea Spray Aerosol in the Fall-Winter Transition 

Emily J. Costa, Cara Waters, Jessica A. Mirrielees, Hailey E. Kempf, Jun Liu, Jamy Y. Lee, Andrew L. Holen, Judy Wu, Andrew P. Ault, and Kerri A. Pratt

The Arctic is rapidly warming, causing reductions in sea ice extent and thickness. This is resulting in increasing areas of open water, which can act as a source of sea spray aerosol generated by bubble bursting at the sea surface. Changing local marine biogeochemistry is expected to have an increasing impact on the Arctic aerosol population. However, measurements of the Arctic atmosphere under these changing conditions are challenging and limited, especially during the fall-winter transition, when sea ice freeze-up is delayed. As such, there is little knowledge of how the changing ecosystem will influence the regional atmosphere and climate. To investigate Arctic sea spray aerosol particles during the fall-winter transition, we present measurements of individual particles collected during the November – December 2018 Aerosols in the Polar Utqiaġvik Night (APUN) field campaign in coastal Utqiaġvik, Alaska. The morphology and chemical composition of individual atmospheric particles ranging in diameter from 0.1–1.8 μm were measured using computer-controlled scanning electron microscopy with energy dispersive X-ray spectroscopy (CCSEM-EDX) and Raman microspectroscopy. CCSEM-EDX was used to identify individual sea salt aerosol particles and investigate their elemental composition, with an emphasis on quantifying organic carbon content. Using Raman microspectroscopy, we identified marine-derived organics within the individual sea salt aerosol particle coatings. The majority of the sea spray aerosol particles were identified as being produced from nearby open water, rather than being long-range transported. These measurements of sea spray aerosol during the coastal Arctic fall-winter transition will further our understanding of the connections between delayed sea ice freeze-up, seawater microbiology, and aerosol particle composition in the changing Arctic environment.  

How to cite: Costa, E. J., Waters, C., Mirrielees, J. A., Kempf, H. E., Liu, J., Lee, J. Y., Holen, A. L., Wu, J., Ault, A. P., and Pratt, K. A.: Local Production of Arctic Sea Spray Aerosol in the Fall-Winter Transition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-752, https://doi.org/10.5194/egusphere-egu25-752, 2025.

The rapid warming of the Arctic, driven by glacial and sea ice melt, poses significant challenges to Earth's climate, ecosystems, and economy. Recent evidence indicates that the snow-darkening effect (SDE), caused by black carbon (BC) deposition, plays a crucial role in accelerated warming. However, high-resolution simulations assessing the impacts from the properties of snowpack and land‒atmosphere interactions on the changes in the surface energy balance of the Arctic caused by BC remain scarce. This study integrates the Snow, Ice, Aerosol, and Radiation (SNICAR) model with a polar-optimized version of the Weather Research and Forecasting model (Polar-WRF) to evaluate the impacts of snow melting and land‒atmosphere interaction processes on the SDE due to BC deposition. The simulation results indicate that BC deposition can directly affect the surface energy balance by decreasing snow albedo and its corresponding radiative forcing (RF). On average, BC deposition at 50 ng g-1 causes a daily average RF of 1.6 W m-2 in offline simulations (without surface feedbacks) and 1.4 W m-2 in online simulations (with surface feedbacks). The reduction in snow albedo induced by BC is strongly dependent on snow depth, with a significant linear relationship observed when snow depth is shallow. In regions with deep snowpack, such as Greenland, BC deposition leads to a 25–41% greater SDE impact and a 19–40% increase in snowmelt than in areas with shallow snow. Snowmelt and land‒atmosphere interactions play significant roles in assessing changes in the surface energy balance caused by BC deposition based on a comparison of results from offline and online coupled simulations via Polar-WRF/Noah-MP and SNICAR. Offline simulations tend to overestimate SDE impacts by more than 50% because crucial surface feedback processes are excluded. This study underscores the importance of incorporating detailed physical processes in high-resolution models to improve our understanding of the role of the SDE in Arctic climate change.

How to cite: Zhang, Z., Zhou, L., and Zhang, M.: A numerical sensitivity study on the snow-darkening effect by black carbon deposition over the Arctic in spring, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2025, https://doi.org/10.5194/egusphere-egu25-2025, 2025.

EGU25-3641 | ECS | Orals | ITS5.7/AS4.3

Evaluation and Attribution of a Warm Winter Bias Over Arctic Sea Ice in a Climate Model 

Nicolas Michalezyk, Guillaume Gastineau, Martin Vancoppenolle, and Clément Rousset

Biases of the winter near-surface temperature over Arctic sea ice have been reported in climate models, increasing uncertainties in future sea ice and Arctic climate projections. Mitigating these biases in future model versions requires proper evaluation and understanding of their origin. To progress on these matters, we focus on the near surface air temperature simulated in the atmosphere-only and coupled configurations of the IPSL-CM6A-LR climate model. To establish a reliable baseline for evaluating simulations, we identified a linear relationship between the mean surface air temperature from the European Centre for Medium-Range Weather Forecasts 5th generation reanalysis (ERA) and their bias relative to in situ observations from Soviet North Pole drifting stations. This relationship is then used to correct the ERA5 data. We find the winter near-surface temperature bias in the atmosphere-only IPSL-CM6A-LR configuration turns from cold to warm once ERA5 is linearly corrected, reaching +2.2°C over Arctic multiyear ice. The bias increases to +4.8°C in the fully-coupled configuration. Using a pan-Arctic energy budget evaluation, the warm bias in IPSL models is explained by an excessive poleward atmospheric heat transport. In the coupled configuration, the warm bias is increased by the too small sea ice extent, which also acts to reduce the overestimated atmospheric heat transport and leads to a too small poleward oceanic heat transport and surface energy budget. The methods developed here could be used in multi-model evaluations to further progress in understanding and reducing biases in climate models.

 

How to cite: Michalezyk, N., Gastineau, G., Vancoppenolle, M., and Rousset, C.: Evaluation and Attribution of a Warm Winter Bias Over Arctic Sea Ice in a Climate Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3641, https://doi.org/10.5194/egusphere-egu25-3641, 2025.

EGU25-5474 | ECS | Orals | ITS5.7/AS4.3

The importance of oceanic emissions for modelling Arctic aerosols and clouds 

Rémy Lapere, Louis Marelle, Antoine Haddon, Nadja Steiner, Jean-Christophe Raut, and Jennie L. Thomas

Emissions of primary aerosols and aerosol precursors from the ocean are key for the Arctic climate. Among those, secondary aerosols from oceanic dimethylsulfide (DMS) are a key species for aerosol-radiation and aerosol-cloud interactions. However, the representation of DMS in atmospheric models is challenging, which generates large uncertainties in the Arctic aerosol budget. In this work we evaluate the sensitivity of simulated Arctic aerosols and clouds in the WRF-Chem atmospheric chemistry model, over a complete annual cycle, to (1) the representation of DMS chemistry in the atmosphere and (2) the oceanic DMS concentration product used as boundary condition. For (2), we compare the results obtained using the Lana et al. (2011) global climatology versus dedicated simulations of the Arctic Ocean biogeochemistry with NEMO-CSIB.
        We find that aerosol number concentrations can change by up to more than 100%, including over sea ice, depending on the model configuration, with a greater sensitivity to the chemistry mechanism than to the oceanic DMS product. This change is negative in the summer, which leads to decreased cloud droplet number and increased (decreased, respectively) shortwave (longwave, respectively) radiation at the surface over sea ice. The opposite effect is found in late spring and autumn. Overall, we find that using a more complex chemistry and better description of Arctic Ocean DMS has an impact on the surface energy budget of +4 W/m2 on average for the year 2018, both over sea ice and the open ocean. This configuration also performs best compared to observations. Additional experiments evaluating the changes of aerosol number under future oceanic DMS concentrations, potential emissions of DMS through sea ice, and the role of methanesulfonic acid (MSA) nucleation in summertime aerosol number concentration are presented. 
        This work demonstrates the importance of accurately modeling DMS for simulations of the Arctic aerosol budget and climate, and the value-added of forcing atmospheric models with ocean biogeochemistry simulations.

How to cite: Lapere, R., Marelle, L., Haddon, A., Steiner, N., Raut, J.-C., and Thomas, J. L.: The importance of oceanic emissions for modelling Arctic aerosols and clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5474, https://doi.org/10.5194/egusphere-egu25-5474, 2025.

Stable boundary layers (SBL) commonly form during the Arctic polar night, but their correct representation has been posing major challenges for numerical weather prediction (NWP) systems. To enable innovative model verification, we performed measurements of the lower atmospheric boundary layer with airborne fiber-optic distributed sensing (FODS), a tethered sonde, and ground-based eddy-covariance measurements. Here we contrast findings across two representative synoptic forcings leading to structurally different inversion types in a fjord-valley system in Svalbard, namely inflow and outflow conditions during the arctic polar night in early 2024. The strong gradients of the inversions are accompanied by an increased temperature variance, which is related to enhanced buoyancy fluctuations. The observed vertical temperature and wind speed profiles are compared to two configurations of the HARMONIE-AROME system with different horizontal resolutions at 2.5 km and 0.5 km.

The higher-resolution model captures cold pool and low-level jet formation during weak synoptic forcing and valley outflow, resulting in a well-represented vertical temperature profile down to the snow surface, while the coarser model exhibits a warm bias in near-surface temperatures of up to 8 K due to underestimated inversion strength. During changing background flow to valley inflow conditions, the higher-resolution model is more sensitive to misrepresented fjord-scale wind directions and performs less well, while the coarser NWP system has a seemingly better agreement with the observations lending to the underrepresented interaction with the topography.

The results indicate the importance of the ratio between nominal horizontal model resolution and valley width to represent stable boundary layer features in a physically meaningful manner. Our results underline the substantial benefit of the innovative spatially resolving FODS measurements for model verification studies as well as the importance of model and topography resolution for accurate representation of stable boundary layers in complex terrain.

How to cite: Thomas, C., Mack, L., Kähnert, M., Jonassen, M., Batrak, Y., Remes, T., and Pirk, N.: Investigating Stable Boundary-Layer Temperature Profiles Observed from Fiber-Optic Distributed Sensing on a Tethered Balloon and comparing them against NWP Systems at Different Resolutions for an Arctic Fjord-Valley System in Svalbard, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7195, https://doi.org/10.5194/egusphere-egu25-7195, 2025.

EGU25-7289 | Posters on site | ITS5.7/AS4.3

Lagrangian pathways connecting the Weddell and Bellingshausen Seas 

Vladimir Maderich, Roman Bezhenar, Igor Brovchenko, Dias Fabio Boeira, Cecilia Äijälä, and Petteri Uotila

This study aims to assess the connectivity of currents around the Antarctic Peninsula and identify the structure of flows carrying particles from the Eastern to Western Antarctic Peninsula continental shelves. We use circulation data for the Weddell and Bellingshausen Seas from the “Whole Antarctica Ocean Model” to obtain and analyse particle trajectories using the “Probably A Really Computationally Efficient Lagrangian Simulator” (Parcels) model. In addition to the main Parcels kernels and a previously developed kernel that ensures the conservation of the number of particles during flow around irregularities in the bottom relief and the lower edge of ice shelves, we have also developed a kernel to simulate convection in the ocean upper mixed layer. Around 170,000 virtual particles were released at a depth of 10 m during a year with a spatial step of 1° in two shelf and slope sectors in the southern Weddell Sea where depth is less than 1500 m. The first sector covers a shelf area between 71°S and 77°S adjacent to the Filchner-Ronne Ice Shelf. The second sector covers a shelf area between 70°S and 65°S adjacent to the Larsen Ice Shelf.  The pathways of water masses were characterised by the visitation frequency (the percentage of particles P that visit each 10×10 km grid column at least once in a modelling period of 20 years). The proportion of particles crossing 58°W (tip of the Antarctic Peninsula) is 21% of the total amount, while the proportion of particles turning northeast is 70%.  The smaller sector, adjacent to the Larsen Ice Shelf, is the main source of particles transferred to the Bellingshausen Sea (51%). In contrast, particles released in the larger sector were mostly transported to the northeast (75%). Only 3.4% of the released particles were transported to the west of 80°W, while the Amundsen Sea (105°W) is reached only by 0.1% of released particles. This indicates a virtual lack of connectivity between the ocean circulation from the Weddell to the Amundsen Seas.

How to cite: Maderich, V., Bezhenar, R., Brovchenko, I., Boeira, D. F., Äijälä, C., and Uotila, P.: Lagrangian pathways connecting the Weddell and Bellingshausen Seas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7289, https://doi.org/10.5194/egusphere-egu25-7289, 2025.

EGU25-7504 | ECS | Posters on site | ITS5.7/AS4.3

Integrated Analysis of Airborne In-situ Cloud and Aerosol Microphysics Data during the 2022 Chemistry in the Arctic: Clouds, Halogens, and Aerosols (CHACHA) Field Campaign 

Sara Lombardo, Vanessa Selimovic, Sara Lance, Sarah Woods, Daun Jeong, Andrea F Corral, Natasha Garner, Peter Peterson, Carol Costanza, Katja Bigge, Tim Starn, Brian H Stirm, Armin Sorooshian, Jose D Fuentes, William R Simpson, Paul B Shepson, and Kerri Pratt

The Chemistry in the Arctic: Clouds, Halogens, and Aerosols (CHACHA) field project featured a wide collaboration from six universities to enhance the scientific understanding of multiphase halogen chemistry in the Arctic that took place in Utqiaġvik, Alaska during February-April 2022. This project was spurred by the pursuit of strengthening our understanding of how Arctic Sea ice loss and fossil fuel extraction affects atmospheric halogen chemistry.

In this study, cloud flights from the University of Wyoming King Air are evaluated closely to assess the ambient conditions relevant to the Arctic boundary layer during flights targeting clouds emanating from open leads in the Arctic sea ice. During these flights, the Particle into Liquid Sampler (PILS) was utilized using a Roger’s inlet and Counterflow Virtual Impactor (CVI) with low volume (1.5 mL) samples being collected. This study aims to introduce a methodological basis for prioritizing samples and identifying samples that can be safely grouped together to maximize the chemical analysis possible. Instruments are used for this method include Aerosol microphysics data from instruments including Condensation Particle Counters (CPC), Portable Optical Particle Spectrometer (POPS), and Passive Cavity Aerosol Spectrometer Probe (PCASP) and cloud microphysics data from a Cloud Droplet Probe (CDP) and Two-Dimensional Stereo (2D-S). Ultimately, this work is a key step in chemical analysis of cloud flights that will be used to better understand multiphase Arctic halogen chemistry by constraining a Lagrangian chemical box model and cloud parcel modeling.

How to cite: Lombardo, S., Selimovic, V., Lance, S., Woods, S., Jeong, D., Corral, A. F., Garner, N., Peterson, P., Costanza, C., Bigge, K., Starn, T., Stirm, B. H., Sorooshian, A., Fuentes, J. D., Simpson, W. R., Shepson, P. B., and Pratt, K.: Integrated Analysis of Airborne In-situ Cloud and Aerosol Microphysics Data during the 2022 Chemistry in the Arctic: Clouds, Halogens, and Aerosols (CHACHA) Field Campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7504, https://doi.org/10.5194/egusphere-egu25-7504, 2025.

The Asian Water Towers (AWTs), centered on the Tibetan Plateau and its surrounding regions, provide vital water resources for over two billion people but are experiencing rapid glacier retreat. Understanding how atmospheric processes, particularly vertical moisture transport, drive this retreat remains challenging. To address this gap, we conducted a decade of ground-based and tethered balloon observations at key AWTs’ sites. Since 2017, tethered balloon measurements have reached altitudes of up to 9,000 m a.s.l., yielding unique vertical profiles of temperature, relative humidity, water vapor stable isotopes, methane, carbon dioxide, and black carbon at Lulang, Nam Co, Muztagh Ata, and the northern Everest base camp. Our findings reveal how the westerlies and Indian monsoon interact with local moisture sources above and in the atmospheric boundary layer, offering insight into seasonal mixing processes. These observations emphasize the need for comprehensive three-dimensional monitoring of atmospheric water vapor isotopes to refine weather forecasts, strengthen climate projections, and enhance regional water security under a changing climate.

How to cite: Gao, J. and Yao, T.: Unraveling the Atmospheric Water Cycle over the Asian Water Towers through water vapor isotopic observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8439, https://doi.org/10.5194/egusphere-egu25-8439, 2025.

EGU25-10134 | Posters on site | ITS5.7/AS4.3

From the Arctic to Antarctica: Observations of vertical aerosol distribution from tethered balloon measurements 

Julia Schmale, Roman Pohorsky, Michael Lonardi, Yolanda Temel, Joanna Dyson, Radiance Calmer, and Lionel Favre

Vertical profile measurements of aerosol properties in the lower atmosphere still constitute a major observational gap. Focusing on the polar regions, where the planetary boundary layer often forms temperature inversions that inhibit vertical mixing of the lowermost atmosphere, surface measure-ments can often not represent aerosol properties further aloft. However, understanding vertical aerosol distribution is critical for several reasons. From a climate perspective, in the Arctic and Antarctic, cloud formation is often sensitive to aerosol availability. Because clouds strongly influence the surface radiation budget and primarily exert warming, it is important to understand aerosols at cloud level.

Overall, understanding the thermodynamic structure of the lower atmosphere and the dynamics of vertical mixing is critical to answer questions on cloud formation. In situ measurements that describe the (thermo)dynamic, aerosol and cloud variables are indispensible to understand relevant process mechanisms and to improve models that typically struggle to simulate polar lower atmospheric aerosols. 

Here we present results obtained with the Modular Multiplatform Compatible Air Measure-ment System (MoMuCAMS). MoMuCAMS can observe particle number size distributions (8-3000 nm) and overall concentrations, aerosol absorption, cloud droplet size distributions, and trace gas mixing ratios (CO2, CO, O3). Based on filter measurements, aerosol chemical composition and INP number concentrations can be obtained. Wind speed and direction, as well as temperature and relative humidity and video images are recorded.

We deployed MoMuCAMS up to 800 m with a payload of ~20 kg in Fairbanks, Alaska (Jan-Feb 2022), Pallas, Finland (Sep-Oct 2022), the Arctic Ocean (May-Jun 2023), southern Greenland (Jun-Aug 2023), and at Neumayer, Antarctica (Dec 2024 – Feb 2025). Overall, more than 350 profiles were flown. This contribution synthesizes observations of aerosol properties below, in and above clouds, and vertically resolved contributions of local and long-range transported particles.

How to cite: Schmale, J., Pohorsky, R., Lonardi, M., Temel, Y., Dyson, J., Calmer, R., and Favre, L.: From the Arctic to Antarctica: Observations of vertical aerosol distribution from tethered balloon measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10134, https://doi.org/10.5194/egusphere-egu25-10134, 2025.

EGU25-10762 | Orals | ITS5.7/AS4.3

Using Arctic field data and remote sensing BrO data to constrain blowing snow sea salt aerosol production parameterizations 

Xin Yang, Ananth Ranjithkumar, Markus Frey, Eliza Eliza Duncan, Daniel Partridge, Thomas Lachlan-Cope, Xianda Gong, Kouichi Nishimura, Kimberly Strong, Alison Criscitiello, Marta Santos-Garcia, Kristof Bognar, Xiaoyi Zhao, Pierre Fogal, Kaley Walker, Sara Morris, Qidi Li, Yuhan Luo, Bianca Zilker, and Andreas Richter

Field evidence has confirmed a new sea salt aerosol (SSA) source on sea ice, which may significantly affect polar boundary layer chemistry and polar winter climate. While the SSA production rate from blowing snow has been previously parameterised (Yang et al., 2008) and then validated by measurements at both Poles, some key parameters involved are not yet fully constrained, leading to uncertainties when using numerical models to compare with field measurements and assess their environmental and climate impacts. In this presentation, we focus on two key parameters: blowing snow size distribution and snow salinity, which determine SSA production in number and size, respectively. We aim to constrain these factors using the latest field data, supported by remote sensing BrO data and modelling. Blowing snow particles typically follow a two-parameter gamma distribution function with shape factor (alpha) and scaling factor (beta) varying over a large range. However, our recent work focusing on the Arctic Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition data showed that at a given height, beta values increase with wind speeds, while alpha gradually approach a constant value of 1.9 at higher wind speeds (e.g. larger than 10 m/s). This is the first time that we derive such a relationship for blowing snow, which further affirms the aerosol production mechanism from blowing snow and helps elucidate the underlying processes involved. Accordingly, we parameterised the blowing snow particle size distribution as a function of wind speed, accounting for variable wind speeds during storms. In addition, supported by a chemistry transport model (p-TOMCAT), we examined the sensitivities of SSA mass and reactive bromine release rate (in association with the SSA production) to representative snow salinities derived from observations in the central Arctic and coastal regions (at Eureka, Canada). Mean winter/springtime snow salinities that best represent the Arctic were derived by comparing the modelled BrO with ground-based multi-axis differential optical absorption spectroscopy (MAX-DOAS) and air-based satellite-based GOME-2 BrO data at Svalbard and Eureka.   

How to cite: Yang, X., Ranjithkumar, A., Frey, M., Eliza Duncan, E., Partridge, D., Lachlan-Cope, T., Gong, X., Nishimura, K., Strong, K., Criscitiello, A., Santos-Garcia, M., Bognar, K., Zhao, X., Fogal, P., Walker, K., Morris, S., Li, Q., Luo, Y., Zilker, B., and Richter, A.: Using Arctic field data and remote sensing BrO data to constrain blowing snow sea salt aerosol production parameterizations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10762, https://doi.org/10.5194/egusphere-egu25-10762, 2025.

As part of the EU project CRiceS, options have been explored for the improved parameterizations in Earth System Models (ESMs) of air-sea gas exchange and heat exchange in the presence of sea ice. One approach explored the impact of sea ice cover with respect to gas exchange by introducing an "effective sea-ice concentration" (SIC) parameter, that moderates the traditional bulk formula for gas transfer as defined by Wanninkhof (2014), allowing for an increased permeability under sea ice conditions without altering the sea-ice state. Another approach explored the young ice (thin ice) parameterization of increased heat permeability, based on a formula determined by the bulk salinity calculated as a prognostic state variable by the sea-ice model. In this study, both of theses formulations have been implemented in the NorESM2-MM model system, whereby we can explore the combined effect of these parameterizations, and compare with the reference CMIP6 model output.

How to cite: Torsvik, T.: Evaluating new sea-ice parameterizations in NorESM for air-sea gas and heat exchange, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10763, https://doi.org/10.5194/egusphere-egu25-10763, 2025.

EGU25-10952 | ECS | Posters on site | ITS5.7/AS4.3

Aerosol Number Concentration and Cloud Condensation Nuclei Variability During Warm and Moist Intrusions into the Arctic 

Berkay Dönmez, Jakob Boyd Pernov, Eija Asmi, Tak Chan, Radovan Krejci, Andreas Massling, Sangeeta Sharma, Henrik Skov, Peter Tunved, Alfred Wiedensohler, Kay Weinhold, Athanasios Nenes, and Julia Schmale

Recent case studies highlight that warm and moist air intrusion events are significant sources of aerosol particles in the Arctic, influencing cloud properties and thus the resulting radiative forcing in the region. However, the contribution of these short-lived events to different aerosol size modes, cloud condensation nuclei (CCN), and droplet number concentrations remains unconstrained. Here, we investigate the multi-annual aspects of intrusion impacts on aerosol properties using data on aerosol number size distributions, CCN, total particle number concentrations, and optical properties from multiple Arctic stations, including Alert, Tiksi, Utqiaġvik, Villum, and Zeppelin, covering the period 2010-2020.

Preliminary results suggest that particle concentrations change significantly during intrusion episodes, with variations across seasons and stations. For instance, contrary to previous studies, number size distribution data indicate a distinct decrease in accumulation mode concentrations during wintertime intrusion episodes relative to non-intrusion periods at several Arctic stations. In summer, this pattern reverses, although not uniformly across stations. Additionally, at Zeppelin, the average of the yearly mean CCN concentrations during intrusions is increased by 13% compared to non-intrusion periods, with some years showing increases exceeding 40%.

We explore the potential drivers of these observed number size distribution patterns and derive potential source contribution function and removal mechanisms along the trajectories, employing the Lagrangian analysis tool LAGRANTO.

How to cite: Dönmez, B., Pernov, J. B., Asmi, E., Chan, T., Krejci, R., Massling, A., Sharma, S., Skov, H., Tunved, P., Wiedensohler, A., Weinhold, K., Nenes, A., and Schmale, J.: Aerosol Number Concentration and Cloud Condensation Nuclei Variability During Warm and Moist Intrusions into the Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10952, https://doi.org/10.5194/egusphere-egu25-10952, 2025.

Field studies in the high and mid latitudes have demonstrated that snowpack emissions of reactive trace gases driven by photolysis alter regional atmospheric composition, the fate of pollutants and the polar ice core archive of past environmental change. Of particular interest are reactive nitrogen and halogen species released by surface snow, which in turn influence atmospheric levels of O3 and hydroxyl radicals (OH and HO2). Previous field campaigns at South Pole and Dome C showed that surface-near air on the high East Antarctic Plateau in summer is highly oxidising due to the interplay of photolytic snow emissions, a shallow boundary layer and cold temperatures.  However, open questions remain regarding the atmospheric oxidant budget above polar snow. Here we present recent observations carried out as part of the ISOL-ICE project at Kohnen Station (75ºS 0ºW) in austral summer 2017, located at a similar latitude as Dome C. Concurrent measurements of nitrogen oxides (NO and NO2), atmospheric particulate nitrate collected on filters, O3, slant-column bromine oxide (BrO), actinic flux and atmospheric turbulence were carried out for the first time at Kohnen. The bulk ion composition of in surface snow and shallow pits was measured as well.

While diurnal cycles of NOx and turbulent diffusivity were similar to previous observations at Dome C, a distinct and strong diurnal cycle of surface O3 with an amplitude of more than 10 nmol mol-1 was detected. O3 showed also a negative correlation with BrO in the lower atmosphere. These observations may imply O3 photochemical source/sink processes, which are stronger than seen previously on the East Antarctic Plateau. We discuss the role of O3 precursor emissions from the sunlit snowpack and vertical mixing with a view of the implications for our understanding of O3 above polar snow.

How to cite: Frey, M., Winton, H., Savarino, J., and Juranyi, Z.: Unusually strong diurnal variability of ozone (O3) above summer snow in East Antarctica – a discussion of pre-cursor snow emissions and atmospheric transport, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12209, https://doi.org/10.5194/egusphere-egu25-12209, 2025.

EGU25-12366 | ECS | Posters on site | ITS5.7/AS4.3

Arctic response to high-latitude effusive volcanic eruptions depends on the climate state 

Tómas Zoëga, Trude Storelvmo, and Kirstin Krüger

Effusive volcanic eruptions are relatively gentle compared to explosive eruptions, resembling boiling stews rather than fireworks. They often last weeks, or even years, and can emit large amounts of gases into the lower atmosphere, among them sulphur dioxide. Through these emissions, they can impact climate via formation of sulphate aerosols and subsequent impacts on clouds. This was, for example, observed during the 2014-15 Holuhraun eruption in Iceland.

 

Volcanic eruptions with considerable effusive components have been common during the historical period in Iceland (the last ca. 1100 years), with roughly 20% of the more than 200 identified eruptions being either purely effusive or mixed effusive-explosive. The largest of those (e.g. 10th-century Eldgjá and 1783-84 Laki) occurred prior to the industrial revolution, when anthropogenic influences on the climate were smaller than they are today. As different atmospheric conditions modulate the cloud and climate responses to aerosol perturbations, a large pre-industrial effusive eruption might have different climate impacts were it to happen today or in the future. Here we use an Earth system model to simulate the surface climate response to an idealized Icelandic effusive volcanic eruptions, similar to 2014-15 Holuhraun, under pre-industrial (1850; PI), present day (2010; PD), and future (2090, SSP3-7.0; Ft) climate conditions and find that this is indeed the case.

 

The modulating effects of the climate state are especially prominent in the Arctic. During winter, we simulate stronger Arctic surface warming under PI conditions, compared to PD and Ft, as the background PI clouds are thinner and hence more transparent to longwave radiation. During summer, we find that the sea ice area significantly modulates the surface cooling in the Arctic, with more Arctic sea ice under PI conditions resulting in weaker surface cooling compared to PD and Ft conditions. We further model a significant increase in sea ice area, as a result of volcanic perturbations, during summer and fall across climate states through increased shortwave cloud shielding.

 

The different surface air temperature responses in the Arctic between different climate states are rather due to a warmer climate as a result of anthropogenic greenhouse gas emissions, with subsequent changes in cloud properties (during winter) and decreased sea ice (during summer), than changes in the background aerosol state.

How to cite: Zoëga, T., Storelvmo, T., and Krüger, K.: Arctic response to high-latitude effusive volcanic eruptions depends on the climate state, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12366, https://doi.org/10.5194/egusphere-egu25-12366, 2025.

EGU25-12992 | Posters on site | ITS5.7/AS4.3

How well do downscaled Global Climate Models represent SMB in Antarctica? 

Clément Cherblanc and Ruth Mottram

Surface Mass Balance (SMB) is a critical forcing of the long term contribution of the Antarctic Ice Sheet (AIS) to sea level. While most GCMs do not produce SMB as an output, several RCMs, including a new ensemble produced in the PolarRES project do and are used to provide forcing for ice sheet models. There are significant spatial variations between regional climate models forced with reanalysis. RCMs also inherit biases from forcing GCMs when run for historical and future climate pathways which may exacerbate or cancel out biases within the RCM. Since the previous intercomparison, there has been significant regional model development and an expansion of datasets that can be used for evaluating these. We assess the SMB estimates of downscaled GCM and reanalysis simulations over Antarctica, compared to a new updated observational database for the historical period. Our ensemble compares 19 SMB products, generated from 4 different GCMs downscaled by 6 RCMs and SMB models, to observations of SMB gathered in the 2024 SUMup dataset. As 8 datasets do not explicitly calculate SMB, we approximate SMB by subtracting evaporation and melt from precipitation with these models. The various simulations are all pan-Antarctic at resolutions from 11 to 27 km, and span periods from 24 to 64 years, between 1950 and 2023. Fidelity of models to observations varies from product to product. As would be expected given they assimilate observational data, reanalyses perform better overall, with minor biases, whereas climatological SMB from GCM-forced runs  are usually too dry (5/9 GCM, 5/19 total). This is a significant bias in GCMs that will have an impact on modelled future evolution of the Antarctic Ice Sheet. One notable exception is the HIRHAM RCM forced by UKESM. In this case opposing biases appear to cancel out, giving the lowest t-statistic and one of the highest correlation coefficients in the intercomparison, while having the most comparison points due to the length of the simulation. The mean yearly accumulation of the models is 2100 Gt/year on the grounded AIS (Zwally’s mask) with most models predicting about 2000 Gt/year and 3 potential outliers predicting over 2500 Gt/year. Our analysis demonstrates that assessing model performance based on reanalysis driven simulations may provide misleading evidence of model performance for future projections. There are still large divergences in the spatial variability of modelled SMB. We also show the need for observational data with a wide spread in time and space.

How to cite: Cherblanc, C. and Mottram, R.: How well do downscaled Global Climate Models represent SMB in Antarctica?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12992, https://doi.org/10.5194/egusphere-egu25-12992, 2025.

EGU25-13063 | ECS | Orals | ITS5.7/AS4.3

Evolution of the size and composition of ice nucleating particles within the synoptic context of the Arctic melt onset 

Camille Mavis, Sonja Murto, Julia Kojoj, Heather Guy, Paul Zieger, Ian Brooks, Michael Tjerström, Sonia Kreidenweis, and Jessie Creamean

The Arctic region is undergoing rapid changes caused by a warming climate and positive radiative feedback loops associated with rapidly-declining sea ice. Clouds play a key role in melt onset timing and annual extent of sea ice loss by modifying the amount of radiation that reaches the surface. The characteristics of Arctic mixed-phase clouds, including lifetime and partitioning of cloud particle phase, are sensitive to ice nucleating particles (INPs), a cloud-active aerosol capable of initiating freezing of cloud droplets at temperatures above homogeneous freezing (-38 °C). INP concentration and freezing temperature (T) are necessary parameters for modeling and validating observations of cloud ice. Observations of INPs are therefore critical for reducing the uncertainties associated with aerosol-cloud interactions for predicting the future Arctic climate. We present an overview of temperature-resolved INP concentrations observed during the ARTofMELT (Atmospheric rivers and the onset of sea ice melt) expedition from May-June 2023. Included in this overview are concentrations of INPs from total aerosol filters (collected continuously on the icebreaker Oden and directly on the sea ice downwind of open leads) and from size-resolved aerosol collected on Oden. Information regarding particle size is pertinent for revealing the aerosol populations acting as INPs and, alongside back-trajectory and meteorological data, their sources. The concentration of INPs from the Oden total aerosol filters reached a maximum of ~1 L-1 at the coldest detectable temperature (-29 °C) and a minimum of ~0.0001 L-1 at temperatures near -10 °C. The total aerosol filters deployed on the ice were less effective at detecting the warm-temperature (rarest) INPs due to the shorter sampling periods. However, an INP maximum of ~1000 L-1 at T = -29 °C was reached on May 11 downwind of a lead, potentially due to wave breaking in strong winds. The total concentrations of INPs from the size-resolved samples were lower than the concentrations observed from both locations with total aerosol filters, likely due to the size cut-off in the size-resolved samples (0.34-12 μm in particle diameter). The variability in INP size distribution showed associations with wind speed and direction. At T = -20 °C, the largest size stage (2.96-12 μm) had the highest fraction of INPs during a period at the beginning of the expedition that encompassed a series of surface cyclones (May 11-18). The INP number concentrations in the smallest smallest size stage (0.15-0.34 μm) eclipsed those on the largest as a larger storm passed the Oden on May 13. Further analysis into INP size and composition, from heat and chemical treatments of samples, will be used to assess their sources.

How to cite: Mavis, C., Murto, S., Kojoj, J., Guy, H., Zieger, P., Brooks, I., Tjerström, M., Kreidenweis, S., and Creamean, J.: Evolution of the size and composition of ice nucleating particles within the synoptic context of the Arctic melt onset, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13063, https://doi.org/10.5194/egusphere-egu25-13063, 2025.

EGU25-14691 | ECS | Posters on site | ITS5.7/AS4.3

Effects of advanced atmosphere-sea ice exchange coefficient in the Korean Integrated Model (KIM)  

Jin-Yun Jeong and Myung-Seo Koo

The Korea Institute of Atmospheric Prediction Systems (KIAPS) is developing a spatio-temporal integrated coupled modeling system that is capable of forecasting from one week to two months. This system is based on the Korean Integrated Model (KIM) and incorporates the Nucleus for European Modelling of the Ocean (NEMO) framework to simulate ocean and sea ice components. While the coupled model’s mid-term prediction performance is comparable to that of the atmosphere-only model, it exhibits a significant cold bias in the polar regions when evaluated against reanalysis data such as ECMWF reanalysis version 5 (ERA5).
Polar regions, characterized by sea ice, present unique challenges due to the complex interactions between the atmosphere and the ocean. In winter, reduced sea ice formation allows more heat to transfer from the ocean to the atmosphere, further warming the air. Accurate simulation of these regions requires a further understanding of atmosphere-sea ice interaction. In this study, sensitivity tests of the atmosphere-sea ice exchange coefficient were conducted to optimize the momentum and heat transfer in the Arctic and Antarctic. The exchange coefficients were fixed at 0.0014 in the control run, while two parameterization methods, modulating sea ice roughness length, were applied to the experimental run. The results revealed opposing outcomes: one method caused atmospheric warming, while the other resulted in cooling, implying significant uncertainty in calculating the heat exchange coefficient. Further analysis of atmospheric and sea ice dynamics within the coupled KIM will determine the most suitable parameterization approach for accurate polar region simulations.

Acknowledgements. This work was carried out through the R&D project “Development of a NextGeneration Numerical Weather Prediction Model by the Korea Institute of Atmospheric Prediction Systems (KIAPS)”, funded by the Korea Meteorological Administration (KMA2020-02212).

How to cite: Jeong, J.-Y. and Koo, M.-S.: Effects of advanced atmosphere-sea ice exchange coefficient in the Korean Integrated Model (KIM) , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14691, https://doi.org/10.5194/egusphere-egu25-14691, 2025.

EGU25-15432 | Orals | ITS5.7/AS4.3

Vertical measurements of aerosols in the high Arctic during the winter-spring transition using a tethered balloon.  

Radiance Calmer, Lionel Favre, Berkay Dönmez, Joanna Dyson, Roman Pohorsky, Bjarne Jensen, Andreas Massling, Henrik Skov, Lise Lotte Sørensen, Sven-Erik Gryning, Varun Kumar, and Julia Schmale

Aerosol number size distributions, along with thermodynamic and dynamic parameters, were measured from the surface to 600 m using a tethered balloon, the Helikite. The field measurements were carried out at Villum Research Station in Northern Greenland from 23rd March to 2nd May 2024. During the transition from winter to spring, three types of atmospheric regimes were identified: (1) a background regime with a profile of uniformly distributed aerosols, represented by low particle number concentrations as well as number size distributions along the vertical axis similar to the surface number size distribution, (2) a winter-type regime characterized by a pollution layer observable at altitudes above 500 m and not observed at the surface, (3) new particle formation episodes in late April and beginning of May, which accompanied a warm airmass intrusion event that had trigged surface melt. Most of the profiles presented a temperature inversion below 200 m, and a low-level jet was sometimes visible between 50 m and 100 m. These recently acquired measurements helped to clarify when ground-based aerosol observations were representative for higher altitude aerosol populations. By capturing a warm airmass intrusion, a comparison could be established with previous events to better understand its impact on the Arctic climate.

Aerosol number size distributions from the Helikite ranged from 8 nm to 3 µm measured with a Miniaturized Scanning Electrical Mobility Sizer (mSEMS, Brechtel) and a Portable Optical Particle Spectrometer (POPS, Hendix). Wind speed and direction were obtained with a SmartTether (Anasphere), and temperature and relative humidity with SHT85 sensors (Sensirion). Observations from the Helikite were complemented by measurements from the Villum Research Station with a ceilometer (Vaisala CL51) for cloud heights, a Scanning Mobility Particle Sizer (SMPS, TSI) for surface aerosol number size distributions and a stand-alone condensation particle counter (CPC, TSI) for number closure, and a 9-meter meteorological mast (temperature, relative humidity, wind, shortwave radiation). Back trajectories from the Lagrangian Analysis Tool LAGRANTO were also used to shed light on the warm airmass intrusion event. 

How to cite: Calmer, R., Favre, L., Dönmez, B., Dyson, J., Pohorsky, R., Jensen, B., Massling, A., Skov, H., Sørensen, L. L., Gryning, S.-E., Kumar, V., and Schmale, J.: Vertical measurements of aerosols in the high Arctic during the winter-spring transition using a tethered balloon. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15432, https://doi.org/10.5194/egusphere-egu25-15432, 2025.

EGU25-16059 | ECS | Posters on site | ITS5.7/AS4.3

Exploring local and long-range aerosol source contributions to summertime CCN in Southern Greenlandic fjord systems 

Joanna Dyson, Nora Bergner, Lionel Favre, Benjamin Heutte, Mihnea Surdu, Julian Weng, Marta Augugliaro, Patrik Winiger, Athanasios Nenes, Kalliopi Violaki, Silvia Henning, and Julia Schmale

The Greenland Ice Sheet (GrIS) discharges ~1000 Gt yr-1 of freshwater into Arctic coastal oceans in the form of meltwater runoff and glacial discharge, with the majority entering the ocean via fjords. Fjordic ecosystems lie at the nexus of various facets of the environment, the ocean, land, cryosphere, atmosphere and biosphere, all of which are especially sensitive to climate change exacerbated by the rising global temperature. With the increase in length and intensity of the summer melt periods, both marine and land-terminating glaciers are slowly receding leaving altered downstream ecosystems in their wake. As glaciers recede, glacial outwash plains become exposed and the potential of sediment aerosolization increases. Concurrently, triggered by increasing melt-water discharge, marine biological productivity is changing, due to the evolving fjord dynamics, stratification, and composition.  Hence, the composition and sources of atmospheric aerosols responsible for the cloud formation in this region are evolving and we expect this to influence both the Cloud Condensation Nuclei (CCN) and Ice Nucleating Particle (INP) populations. In addition to natural aerosols sources, also local anthropogenic activities can contribute to the CCN and INP populations. Furthermore, distant emissions e.g., from north American boreal forest fires, occasionally reach Greenlandic Fjord systems and can have significant impact on the aerosol properties. 

In this presentation we aim to provide an overview of the processes which influence aerosol populations in Greenlandic fjord systems during Arctic summer. We will show results from a comprehensive and extensive field campaign in the Kujalleq province of Southern Greenland (60.91°N, 46.05°W) in June-August 2023. We will present aerosol size distributions, particle number concentrations, and scattering and absorption measurements from both ground-based and tethered-balloon measurement platforms. We will explore the following questions:

  • What are the local and regional sources of aerosols leading to the formation of CCN in Southern Greenland?
  • What is the current contribution of anthropogenic activities to the aerosol budget and how does this compare to the contribution from natural sources?
  • How do long-range transport, new particle formation and ground-level fog events affect the concentration and vertical distribution of aerosols and subsequent CCN formation?

How to cite: Dyson, J., Bergner, N., Favre, L., Heutte, B., Surdu, M., Weng, J., Augugliaro, M., Winiger, P., Nenes, A., Violaki, K., Henning, S., and Schmale, J.: Exploring local and long-range aerosol source contributions to summertime CCN in Southern Greenlandic fjord systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16059, https://doi.org/10.5194/egusphere-egu25-16059, 2025.

EGU25-17925 | ECS | Posters on site | ITS5.7/AS4.3

Evaluating natural aerosol sources from the Arctic Ocean during the onset of sea ice melt 

Julia Kojoj, Gabriel Pereira Freitas, Camille Mavis, Jessie Creamean, Fredrik Mattsson, Lovisa Nilsson, Jennie Spicker Schmidt, Kouji Adachi, Tina Santl-Temkiv, Erik Ahlberg, Claudia Mohr, Ilona Riipinen, and Paul Zieger

Aerosol-cloud interactions remain one of the most significant challenges in accurately estimating human-induced radiative forcing, as well as projecting the future climate. To address this uncertainty, establishing the baseline levels of natural aerosols in various environments is crucial. The polar regions are ideal locations for studying natural aerosols due to their distances from anthropogenic influences, yet observations in these regions are relatively limited. Specifically, the role of oceans and sea ice in controlling aerosol concentrations, influencing cloud formation, and determining cloud phase remains unclear. A key component is biological aerosol particles that participate in the formation and microphysical modulation of Arctic mixed-phase clouds. Yet, many questions regarding their Arctic sources, emission processes, and ice nucleating properties remain.

We present a detailed study of potential natural sources of aerosols in the high Arctic over the pack ice during the ARTofMELT expedition (May–June 2023). We collected samples of snow, sea ice, seawater, and the sea-surface microlayer (SML) and utilized the comprehensive aerosol instrumentation setup on-board to analyze them immediately after collection for their chemical, microphysical, and fluorescent properties. After the expedition, further analysis of the samples was conducted including measurements of ice-nucleating properties and biological cell quantification.

Our results show that during the late Arctic spring, heightened biological activity in the seawater and the SML increased emissions of fluorescent primary biological aerosol particles (confirmed by increased cell count) and organic-coated sea salt particles. However, concentrations of ice-nucleating particles in liquid samples did not follow the same trend. We will present the clear distinctions found in the biological, chemical, and physical properties of all sample types, and the effect of salinity on the aerosolization process and ice nucleating activity. These results provide valuable information for future studies aimed at improving the source attribution of natural Arctic aerosols, helping to reduce uncertainties in their representation in models, and understanding their influence on Arctic mixed-phase clouds. 

This work is currently in discussion at Freitas et al. (2024).

Freitas GP, Kojoj J, Mavis C, Creamean J, Mattsson F, Nilsson L, Schmidt JS, Adachi K, Šantl-Temkiv T, Ahlberg E, Mohr C. A comprehensive characterisation of natural aerosol sources in the high Arctic during the onset of sea ice melt. Faraday Discussions. 2024. DOI: 10.1039/D4FD00162A 

How to cite: Kojoj, J., Pereira Freitas, G., Mavis, C., Creamean, J., Mattsson, F., Nilsson, L., Spicker Schmidt, J., Adachi, K., Santl-Temkiv, T., Ahlberg, E., Mohr, C., Riipinen, I., and Zieger, P.: Evaluating natural aerosol sources from the Arctic Ocean during the onset of sea ice melt, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17925, https://doi.org/10.5194/egusphere-egu25-17925, 2025.

EGU25-19566 | Orals | ITS5.7/AS4.3

Emission patterns and trends of primary marine organic aerosol in the Arctic 

Bernd Heinold, Anisbel Leon-Marcos, Manuela van Pinxteren, Sebastian Zeppenfeld, Moritz Zeising, and Astrid Bracher

Primary marine organic aerosol (PMOA) is a significant contributor to aerosol concentrations in remote oceanic regions, influencing aerosol-cloud-climate interactions. In the Arctic, sea ice retreat and summer ice loss are key drivers of potential increases in marine aerosol emissions. This study uses an extended version of the aerosol-climate model ECHAM6.3-HAM2.3 to investigate the emission patterns and trends of primary marine organic aerosol in the Arctic from 1990 to 2019 in large detail, considering changing climate and ice conditions. Using the offline results of the biogeochemistry model FESOM2.1-REcoM3, three aerosol-relevant biomolecule groups - polysaccharides (PCHO), amino acids (DCAA), and polar lipids (PL) - are modelled. Their atmospheric transfer is parameterized with OCEANFILMS, which was implemented into the aerosol-climate model ECHAM6.3-HAM2.3 to advance the marine emission scheme. Of the modelled organic groups, PCHO is most abundant in seawater, while PL dominates aerosol particles due to its higher air-seawater affinity. Seasonal variations in both the ocean and aerosol concentrations are pronounced, peaking between May and June, then gradually decreasing by late summer. The modelled PMOA seasonal patterns show reasonable agreement with ground-based measurements, considering the uncertainties in model assumptions and observations. Regional differences within the Arctic are evident in the initiation of biomolecule production in seawater and aerosol emissions. Long-term trends in Arctic PMOA emissions, analysed in this study, reveal a strong dependence on sea ice changes. Over the 30-year period, emissions have increased by at least 24%, with variations among biomolecules and regions. PCHO shows the most pronounced trend.

How to cite: Heinold, B., Leon-Marcos, A., van Pinxteren, M., Zeppenfeld, S., Zeising, M., and Bracher, A.: Emission patterns and trends of primary marine organic aerosol in the Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19566, https://doi.org/10.5194/egusphere-egu25-19566, 2025.

EGU25-21585 | Orals | ITS5.7/AS4.3

Towards Improved Polar Biogeochemistry: Integrating an Explicit Sea-Ice Biogeochemical Model in NEMO/SI3 

Marie Lou Bachélery, Iael Perez, Tomas Lovato, Letizia Tedesco, and Momme Butenschön

Ongoing rapid changes in sea-ice cover require a more accurate representation of their interactions with marine biogeochemistry and cascading impacts on the global carbon cycle. Yet, despite the critical role of polar biogeochemical processes, assessing these interactions remains challenging as sea ice and snow are often treated as biogeochemically inert in most large-scale and climate models.

To address this gap, we present a novel integration of the Biogeochemical Flux Model in Sea Ice (BFMSI) within the three-dimensional global NEMO/SI3 system. This innovative coupling explicitly accounts for dynamic interactions between sea-ice physical properties and biogeochemical processes.

To evaluate this implementation, we perform two sensitivity experiments: one assuming a fixed biologically active layer in the sea ice and another where the thickness of this layer dynamically adjusts based on sea-ice permeability, as derived from the sea-ice model. Model results for 2000–2021 are compared against available observations, providing a brief performance assessment. The two experiments are also analyzed to evaluate the sensitivity of ice and under-ice biogeochemical properties to the biological active layer parameterization and the representation of the light transmission through the ice/snow.

These results aim to provide insights into the interplay between sea-ice properties and ocean biogeochemical processes, informing future studies on the role of sea-ice biogeochemistry in shaping the global carbon cycle and its response to ongoing climatic warming. 

How to cite: Bachélery, M. L., Perez, I., Lovato, T., Tedesco, L., and Butenschön, M.: Towards Improved Polar Biogeochemistry: Integrating an Explicit Sea-Ice Biogeochemical Model in NEMO/SI3, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21585, https://doi.org/10.5194/egusphere-egu25-21585, 2025.

Cold-air outbreaks (CAOs) have an overwhelming influence on global atmospheric and oceanic circulations, yet their cloud regimes remain poorly sampled and are therefore not fully understood nor well-represented in weather models. More data on the vertical dependence of the microphysical and macrophysical properties of clouds in CAOs and its variability and dependence on environmental conditions is crucial for enhancing the understanding of processes occurring in clouds, and for improving and evaluating the performance of models and remote sensing retrievals over high latitudes. The Cold-Air outbreak Experiment in the Sub-Arctic Region (CAESAR) field campaign acquired such in-situ and remote sensing data during 8 flights of the National Science Foundation/National Center for Atmospheric Research (NSF/NCAR) C-130 between 22 February and 7 April 2024 over the Norwegian Sea.

In this study, the vertical dependence of microphysical properties of total number concentration, liquid water content, ice crystal concentration, ice mass content, liquid and ice effective radius, and median volume diameters using data from the Cloud Droplet Probe (CDP), Two-Dimensional Stereo Probe (2D-S) and High Volume Precipitation Sampler (HVPS) is determined as a function of normalized altitude (zn), where zn=0 at cloud base and zn=1 at cloud top. The majority of clouds sampled were either liquid- or mixed-phase, with few entirely ice-phase clouds sampled during the campaign. Case studies from 2 April 2024 (RF09) and 3 April 2024 (RF10) are shown to establish a typical structure of clouds sampled during CAESAR with liquid water content and effective diameter increasing with zn, with graupel, irregular particles and rimed snowflakes occurring in mid-levels for some vertical profiles. However, when examining data from all 70 vertical profiles there was a lack of uniformity on how the parameters varied as a function of zn. Therefore profiles were cataloged according to environmental conditions (e.g., cloud base temperature, updraft/downdraft characteristics, open vs. closed cells, presence of cloud streets, distance from sea ice edge, aerosol concentration) in an attempt to better characterize the variability. Implications for the understanding of processes occurring in CAO clouds will be discussed.  

How to cite: McFarquhar, G., Amundsen, N., and Woods, S.: Quantifying the Dependence of Cloud Vertical Structure during Cold Air Outbreaks on Environmental Conditions: Preliminary Findings from CAESAR, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-174, https://doi.org/10.5194/egusphere-egu25-174, 2025.

EGU25-1061 | ECS | Orals | AS4.4

Bacterial Bioaerosols Involved in Ice Nucleation and Cloud Formation: Connections to Shifting Precipitation Patterns in the Antarctic Peninsula 

Ksenija Vučković, Eva Lopes, Leonor Pizarro, Sharath Chandra Thota, Maria de Fátima Magalhães Carvalho, Claudio Hernán Durán Alarcón, Catarina Magalhães, and Irina Gorodetskaya

With the ongoing warming trend on the Antarctic Peninsula (AP), the amount, intensity, and frequency of precipitation is projected to increase by the end of the 21st century. The future of precipitation phase—whether rainfall will dominate snowfall over the AP—remains uncertain. Warm weather events occurring over the AP have been showing frequent snowfall to rainfall transitions, particularly during atmospheric rivers (AR) (Chyhareva et al., 2021; Wille et al., 2021; Gorodetskaya et al., 2023).

ARs are long corridors of anomalously high water vapour transport, which bring heat and moisture towards polar regions and, notably, can also facilitate the transport of aerosols (Lapere et al., 2021). When the sources of moisture and aerosols co-occur within ARs, aerosols can be scavenged and deposited as precipitation on ice-sheet surfaces.

In pristine environments such as Antarctica, aerosols of natural origin play an important role in cloud and precipitation formation (Mallet et al., 2023). Bioaerosols, specifically bacteria, can serve as potent ice-nucleating particles, facilitating the formation of ice and influencing precipitation formation, especially in mixed-phase clouds.

This study aims to identify culturable bacteria present in precipitation samples—rainfall, snowfall, and surface snow following precipitation events—collected in the northern AP, on King George Island, in the vicinity of the King Sejong station. Bacterial isolates were identified using 16S rDNA gene sequencing, revealing key differences in culturable biodiversity between rainfall and snowfall samples. Genera known for exhibiting ice-nucleating activity, Pseudomonas and Stenotrophomonas, were predominantly recovered from rainfall. Additionally, potentially novel strains were recovered from rainfall samples. Surface snow samples following precipitation events exhibited high culturable biodiversity, including Spirosoma sp. and Bacillus sp. strains, which are adapted to the extreme conditions of aerial and polar environments.

These results highlight a shift from snowfall to rainfall-dominated precipitation in the AP may impact the local biodiversity, and the newly introduced ice-nucleating strains can further impact the Antarctic climate. Bacteria associated with ice nucleating activity were recovered from precipitation, indicating bacteria can impact the polar aerosol budget, cloud dynamics and climate of the AP.

Future analysis of AR-associated precipitation is key to determining the atmospheric transport of bioaerosols and is a necessary component for understanding the current warming trend of the AP.

Acknowledgements:  PROPOLAR (Portuguese Polar Program) projects APMAR/TULIP/APMAR2/APMAR2025 and FCT project MAPS (2022.09201.PTDC) and MicroANT (2023.15890.PEX)

References:

Chyhareva, A., et al (2021). Precipitation phase transition in austral summer over the Antarctic Peninsula. Ukr. Ant. J., https://doi.org/10.33275/1727-7485.1.2021.664

Gorodetskaya, I., et al. (2023). Record-high Antarctic Peninsula temperatures and surface melt in February 2022: A compound event with an intense atmospheric river. npj Clim. Atmos. Sci. https://doi.org/10.1038/s41612-023-00529-6

Lapere, S., et al. (2024). Polar aerosol atmospheric rivers: Detection, characteristics, and potential applications. J. Geophys. Res.: Atmospheres, 129(2). https://doi.org/10.1029/2023JD039606

Mallet, M., et al. (2023). Untangling the influence of Antarctic and Southern Ocean life on clouds. Elementa: Sci. Anthropocene, 11(1). https://doi.org/10.1525/elementa.2022.00130

Wille, J. D., et al. (2021). Antarctic atmospheric river climatology and precipitation impacts. J. Geophys. Res.: Atmospheres, 126(8), e2020JD033788

Keywords: Antarctic Peninsula, precipitation, bioaerosols, culturable biodiversity, ice-nucleation

 

How to cite: Vučković, K., Lopes, E., Pizarro, L., Chandra Thota, S., de Fátima Magalhães Carvalho, M., Durán Alarcón, C. H., Magalhães, C., and Gorodetskaya, I.: Bacterial Bioaerosols Involved in Ice Nucleation and Cloud Formation: Connections to Shifting Precipitation Patterns in the Antarctic Peninsula, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1061, https://doi.org/10.5194/egusphere-egu25-1061, 2025.

EGU25-3274 | ECS | Orals | AS4.4

Extreme precipitation and atmospheric rivers over West Antarctic ice shelves: insights from kilometre-scale regional climate modelling 

Ella Gilbert, Denis Pishniak, José Abraham Torres, Andrew Orr, Michelle Maclennan, Nander Wever, and Kristiina Verro

Extreme precipitation events in the Amundsen Sea Embayment, West Antarctica deposit significant precipitation amounts, often during atmospheric river (AR) events. In this work, we use observations, reanalysis, and three regional climate models (RCMs: MetUM, Polar-WRF, HCLIM) at a spatial resolution of 1 km to evaluate the characteristics of two AR cases: one in winter, and another in summer. We quantify the magnitude of snow and rain falling over the Thwaites and Pine Island ice shelves and explore the drivers and mechanisms of this extreme precipitation. The model results indicate that supercooled liquid precipitation fell during these cases, generated in particular by the interaction of the AR with steep topography. Model estimated snowfall compares well against observed snow height measurements, but ERA5 estimates for both events are severely underestimated (by 3-4 times) compared to the measurements. Our work highlights that kilometer-scale models are useful tools to investigate the total precipitation amount and its partitioning into rain and snow over this globally important and climatically sensitive region, and the critical need for in situ observations of rainfall.

How to cite: Gilbert, E., Pishniak, D., Torres, J. A., Orr, A., Maclennan, M., Wever, N., and Verro, K.: Extreme precipitation and atmospheric rivers over West Antarctic ice shelves: insights from kilometre-scale regional climate modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3274, https://doi.org/10.5194/egusphere-egu25-3274, 2025.

EGU25-6347 | ECS | Posters on site | AS4.4

Assessing the aerosol and moisture transport to the Arctic through atmospheric river and their impact on clouds 

Fathima Cherichi Purayil, Jan Kretzschmar, and Johannes Quaas

The transport of aerosols to the Arctic plays a key role in shaping local climate processes, particularly in the context of Arctic amplification. Here, we utilize an atmospheric river detection algorithm to identify and analyze extreme aerosol and moisture transport events from mid-latitudes to the Arctic over a 43 year period.By examining the combined effects of aerosol and moisture intrusions, we aim to understand how the presence of aerosols alter the cloud properties compared to scenarios with only moisture. Inorder to evaluate the cloud properties, we use the active remote sensing product DARDAR-Nice dataset.

The findings will provide insights into aerosol-cloud interactions in the Arctic, offering a better understanding of the role of aerosol transport in Arctic climate change and thereby improving the accuracy of climate model projections.

How to cite: Cherichi Purayil, F., Kretzschmar, J., and Quaas, J.: Assessing the aerosol and moisture transport to the Arctic through atmospheric river and their impact on clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6347, https://doi.org/10.5194/egusphere-egu25-6347, 2025.

EGU25-6488 | Posters on site | AS4.4

Long-term Analysis of Vertically Resolved Cloud Observations at Ny-Ålesund (Svalbard) using Self-Supervised Deep Learning 

Kerstin Ebell, Nils Risse, Dwaipayan Chatterjee, Andreas Walbröl, Marion Maturilli, Simone Bauer, Mario Mech, and Susanne Crewell

Climate change is particularly evident in the Arctic, where warming between 1979 and 2021 was almost four times faster than the global average (Rantanen et al., 2022). However, this temperature increase is not uniform across the region. For example, the Svalbard archipelago, situated in the warmest part of the Arctic, has experienced the most significant warming (Dahlke and Maturilli, 2017).

The role of clouds in the rapidly changing Arctic climate system, along with the underlying processes, remains a major area of investigation. While detailed cloud observations are crucial, there are few Arctic locations where continuous, high-resolution vertical cloud measurements are conducted. One such site is the German-French Arctic Research Base AWIPEV, located at the Ny-Ålesund Research Station in Svalbard. Since 2016, a 94 GHz cloud radar has been operational here as part of the Transregional Collaborative Research Centre TR172 on Arctic Amplification (AC)³ (http://www.ac3-tr.de; Wendisch et al., 2023). Combined with existing remote sensing tools such as ceilometers and microwave radiometers, this setup enables continuous monitoring of clouds with high temporal and vertical resolution. This presentation will showcase key findings from these multi-year cloud radar observations.

At Ny-Ålesund, clouds are present 78% of the time, with the highest occurrence observed in low-level clouds between 0.5 and 1.5 km altitude. Pure liquid water clouds display a clear seasonal cycle, whereas mixed-phase clouds, containing both liquid and ice, are present throughout the year, averaging 42% of the time. These liquid-containing clouds significantly influence surface radiative fluxes, with an overall net warming effect of clouds of approximately 11 Wm⁻².

A novel approach to efficiently characterize the long-term observations of diverse cloud systems over Ny-Ålesund is by using a self-supervised deep learning framework. This framework is designed to learn the complex relationships within the sub-hourly, multi-scale measurements from radar collected from 2017 to 2021. During training, it captures the non-linear, orthogonal aspects of the clouds' vertical and temporal structure and distributions over the Ny-Ålesund column and extracts the essential low-dimensional features. Sensitivity tests are conducted by combining different measurements and observing the resulting changes in the extracted features. Analyzing this low-dimensional representation of the entire cloud measurement time series provides valuable insights into cloud evolution and its connection to environmental conditions.

Acknowledgment: We gratefully acknowledge the funding by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) – Project Number 268020496 – TRR 172, within the framework of the Transregional Collaborative Research Center “ArctiC Amplification: Climate Relevant Atmospheric and SurfaCe Processes, and Feedback Mechanisms (AC)³”. We also acknowledge the support by AWIPEV for the project AWIPEV_0016.

How to cite: Ebell, K., Risse, N., Chatterjee, D., Walbröl, A., Maturilli, M., Bauer, S., Mech, M., and Crewell, S.: Long-term Analysis of Vertically Resolved Cloud Observations at Ny-Ålesund (Svalbard) using Self-Supervised Deep Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6488, https://doi.org/10.5194/egusphere-egu25-6488, 2025.

Fog is typically a very low cloud touching the ground and consists of tiny liquid droplets or ice particles. Ice fog can form in very cold areas such as polar regions or high mountains at temperatures below -30°C. Few field campaigns have focused on ice fog and fewer have shown the presence of ice fog at warmer temperatures, suggesting that limitation in time and space may lead to an underestimation of this phenomenon with implications on the biosphere and the estimation of the Earth's energy budget.

By analysing CALIOP data from 2006 to 2023, we have found a reduction of both liquid fog (~ -33% up to 0.5km; ~ -32% up to 2km) and ice fog (~ -29% up to 0.5km; ~ -30% up to 2km) over time.
The geographical distribution of ice fog shows that ice fog mainly occurs at latitudes above 50°, where ice is more likely to form due to low temperatures.
Separating the regions with ice fog occurrence into North/South and continental/maritime sub-regions, we have found an increase in ice fog of about 35% (up to 0.5km; +30% up to 2km) over time in the maritime region at latitudes above 60° North, despite a decrease in ice fog in the other areas analysed.
Our results show that the increase in both liquid and ice fog from 2006 to 2023 is well correlated with the increase in aerosols over the same period. However, when ice fog over snow and ice covered surfaces is removed, the correlation between aerosols and ice fog is poor.
The aerosol types provided by CALIOP have been analysed for two temperature ranges to distinguish the homogeneous glaciation (T < -38°C) and the heterogeneous glaciation (-38°C ≤ T ≤ 0°C) of possible ice nucleating particles. This analysis have been used to derive probability density functions of single aerosol types, from which glaciation temperatures have been estimated over continental and maritime surfaces.

How to cite: Bruno, O. and Cermak, J.: Global decrease of ice fog VS increase in the Arctic Ocean: a global analysis of ice fog and aerosols using 17 years of CALIOP measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6541, https://doi.org/10.5194/egusphere-egu25-6541, 2025.

EGU25-8990 | ECS | Posters on site | AS4.4

Diagnosing moisture sources, transport and transformation in the Arctic withwater vapor isotopes in atmospheric modeling 

Hannah Marie Eichholz, Svetlana Botsyun, Jan Kretzschmar, Josefine Umlauft, Stephan Pfahl, and Johannes Quaas

The Arctic has been rapidly moistening over the last forty years, influencing energy fluxes and precipitation. While local changes in
air temperature and sea ice cover partly explain this trend, the role of changing moisture transport to the Arctic is less clear.
Understanding how moisture transport affects Arctic amplification is crucial, as most moisture in the Arctic comes from lower latitudes.
Enhanced warming in the Arctic strengthens meridional transport due to changes in Rossby waves, but current global climate
models struggle to capture these shifts accurately.

The presentation will show results from case studies of moisture transport into the Arctic, analyzing the changing structure of
water vapor isotopes in response to varying moisture transport patterns and phase transition along these transport pathways.
Initial simulations with the isotope-enhanced ICON-ART atmosphere model reveal limitations in its ability to accurately capture
isotopic variations on a global scale. Therefore, the model first needs to be improved and validated for global simulations.
Once these improvements are achieved, case studies are performed to assess phase transition processes in detail and
explore their response to recent warming.

How to cite: Eichholz, H. M., Botsyun, S., Kretzschmar, J., Umlauft, J., Pfahl, S., and Quaas, J.: Diagnosing moisture sources, transport and transformation in the Arctic withwater vapor isotopes in atmospheric modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8990, https://doi.org/10.5194/egusphere-egu25-8990, 2025.

EGU25-9487 | ECS | Posters on site | AS4.4

Model analysis of the changing role of convection in the Arctic climate 

Sophie Vliegen and Johannes Quaas

The pronounced warming observed in the Arctic region has significantly altered the atmospheric energy budget, leading to a transition in the prevailing equilibrium state from radiative-advective to radiative-convective-advective. This study uses data from the Coupled Model Intercomparison Project Phase 6 (CMIP6) to analyze the emergence and characteristics of convective events in the Arctic. Using historical simulations and future projections, we examine the spatiotemporal evolution of convection and its interactions with key climatological parameters such as temperature and humidity. By providing a detailed assessment of these processes, this research contributes to improving our understanding of Arctic climate dynamics and the implications for global climate systems in a warming world.

How to cite: Vliegen, S. and Quaas, J.: Model analysis of the changing role of convection in the Arctic climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9487, https://doi.org/10.5194/egusphere-egu25-9487, 2025.

EGU25-10186 | Orals | AS4.4

Advanced precipitation scheme in ICOLMDZ with improved microphysics and subgrid cloud-hydrometeor interactions to better simulate polar precipitation 

Étienne Vignon, Lea Raillard, Audran Borella, Gwendal Rivière, Meryl Wimmer, and Niels Dutrievoz

The current assessment of the ice sheet surface mass balance and more generally of the atmospheric branch of the high latitude water cycles mostly relies on climate model simulations. The ability of climate models to reproduce the polar precipitation not only depends on the simulation of the atmospheric dynamics and on the advection of moisture towards the poles but also on the representation of the subgrid scale cloud and precipitation processes that govern the formation and growth of snowflakes and rain drops. The ICOLMDZ model, atmospheric component of the IPSL-CM Earth System Model, is intensively involved in polar-oriented studies and recent developments were carried out to improve the representation of mixed-phase and ice clouds. However, recent studies also evidenced substantial shortcomings and biases that persist in the simulation of the polar precipitation, both in the Arctic and in the Antarctic. This study presents the development of a new precipitation scheme in the ICOLMDZ model that includes both an advanced microphysical treatment of snowfall and subgrid vertical overlap considerations to properly account for the interactions between hydrometeors and clouds. Particular attention is also paid to the numerical treatment of the different processes to ensure numerical convergence and stability at typical time steps used in global climate models. The scheme is then evaluated using regional simulations conducted over Adélie Land, East Antarctica and the Svalbard Archipegalo. The simulated vertical profiles of precipitation and microphysical tendencies are compared with observational data from a ground-based polarimetric radar deployed during the APRES3 campaign as well as from airborne radar and lidar data collected during the THINICE campaign. Perturbed parameter ensemble experiments are also conducted to assess the parameteric sensitivity of the model and to disentangle calibration issues from genuine structural biases. Results show that the model is now able to physically capture the vertical evolution of the snowfall and to simulate more realistically the melting layer. Future applications of the new precipitation scheme including simulations of the Antarctic surface mass balance with ICOLMDZ can now be envisaged.

How to cite: Vignon, É., Raillard, L., Borella, A., Rivière, G., Wimmer, M., and Dutrievoz, N.: Advanced precipitation scheme in ICOLMDZ with improved microphysics and subgrid cloud-hydrometeor interactions to better simulate polar precipitation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10186, https://doi.org/10.5194/egusphere-egu25-10186, 2025.

EGU25-11015 | ECS | Posters on site | AS4.4

Observations of the vertical water vapor distribution and the downward, broadband thermal-infrared irradiance at the ground in the Central Arctic during MOSAiC 

Clara Seidel, Dietrich Althausen, Albert Ansmann, Manfred Wendisch, Hannes Griesche, Martin Radenz, Julian Hofer, Sandro Dahlke, Marion Maturilli, Andreas Walbröl, Holger Baars, and Ronny Engelmann

For the first time, measurements of high-resolution water vapor profiles are available for the central Arctic winter North of 85°N. The measurements were conducted with the Raman lidar PollyXT during the MOSAiC-campaign. Using those observations, the impact of the vertical distribution of tropospheric water vapor on the cloud-free downward, broadband thermal-infrared irradiance (FTIR) was quantified.

Values of the integrated water vapor (IWV) were determined from the lidar-derived vertical water vapor profiles up to the tropopause region and correlated to the FTIR at the surface. Colocated radiosonde measurements were used to consider the influence of the temperature of the vertically distributed water vapor on this correlation with means of a water-vapor-weighted mean temperature (representative temperature of the water vapor distribution).

In the study, seven measurement cases of several hours duration were examined representing slowly changing air masses. Furthermore, 53 rather short-term (10 minutes) measurement cases were investigated. The temporal evolution of the slowly changing air masses revealed a linear relationship between FTIR and IWV with slopes between 7.17 and 12.95 W kg−1 and a coefficient of determination larger than 0.95 for most of the selected cases. A dependence of the slopes and ordinate-intercepts on the water-vapor-weighted mean temperature was found with smaller ordinate-intercepts at lower temperatures. A linear relationship was found between the water-vapor-weighted mean temperature and the temperature determined with the Stefan-Boltzmann law from FTIR. The analysis of 53 independent short-term observations of different air masses confirmed the linear relationship between FTIR and IWV at wintertime cloud-free conditions in the Arctic with a coefficient of determination of 0.75 and a slope of 19.95 W kg−1.

The evaluations of the profile measurements showed a clear influence of the temperatures of the water vapor along its profile on the FTIR at the surface and the importance of the vertical water vapor and temperature distribution for radiation investigations at the surface.

How to cite: Seidel, C., Althausen, D., Ansmann, A., Wendisch, M., Griesche, H., Radenz, M., Hofer, J., Dahlke, S., Maturilli, M., Walbröl, A., Baars, H., and Engelmann, R.: Observations of the vertical water vapor distribution and the downward, broadband thermal-infrared irradiance at the ground in the Central Arctic during MOSAiC, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11015, https://doi.org/10.5194/egusphere-egu25-11015, 2025.

EGU25-12746 | Orals | AS4.4

Have three years of observations explained model biases in Southern Ocean clouds? 

Tom Lachlan-Cope and the Southern Ocean Clouds team

Recent climate models have shown biases in surface radiation linked to errors in cloud amount over the Southern Ocean. The NERC funded Southern Ocean Cloud project is trying to explain these biases and has been running for the last three years. It consist of long term measurements of aerosol size and composition at Rothera Station on the Antarctic Peninsula, two airborne campaigns observing cloud properties based out of Rothera and a ship cruise on the Sir David Attenborough, again concentrating on aerosol properties, in the Southern Ocean. The aim of the project is to investigate the sources of aerosols at high southern latitudes and the role they play in clouds. The hope is that this will lead to better representation of these processes within climate models.

Observations made at Rothera Station and on the Sir David Attenborough have identified several distinct types of cloud nuclei and we are working to determine their sources. At the same time these surface based observations, both from Rothera and the ship, are compared with the aircraft observations of cloud properties. These observations are starting to give an insight in to the processes that control clouds over the Southern Ocean and are being used to improve parameterisations of both aerosols and clouds in models.

How to cite: Lachlan-Cope, T. and the Southern Ocean Clouds team: Have three years of observations explained model biases in Southern Ocean clouds?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12746, https://doi.org/10.5194/egusphere-egu25-12746, 2025.

EGU25-13186 | Posters on site | AS4.4

Aerosol particle measurements on the Southern Ocean during the Southern Ocean Clouds (SOC) campaign in November and December 2024 

Leah Williams, James Allan, Michael Flynn, David Beddows, James Brean, Mark Tarn, Manuel Dall'Osto, Amélie Kirchgaessner, and Thomas Lachlan-Cope

We deployed an Aerosol Mass Spectrometer (AMS) on the British Antarctic Survey Research Vessel Sir David Attenborough (SDA) during November and December 2024 as part of the Southern Ocean Clouds (SOC) campaign. The AMS measures sub 1 micron aerosol particle chemical composition and size distributions, using thermal vaporization and electron impact ionization, followed by time-of-flight mass spectrometry.

The cruise track covered a broad area (50 S to 67 S and 70 W to 25 W) and encountered a wide variety of atmospheric environments, including seasonal sea ice zones, open ocean, and areas near islands with penguin colonies and volcanoes. Different ratios of organics, sulphate and methane sulphonic acid (MSA) were observed for different sympagic and pelagic air masses and associated with distinct aerosol size distributions. We also observed distinct plumes of NH4Cl particles from a volcano and we saw aqueous processing of aerosol particles during a multi-day fog event. As is typical of ship campaigns, the AMS organics showed that we were sampling ship emissions, both from the engines and from the kitchen, at least half of the time.

How to cite: Williams, L., Allan, J., Flynn, M., Beddows, D., Brean, J., Tarn, M., Dall'Osto, M., Kirchgaessner, A., and Lachlan-Cope, T.: Aerosol particle measurements on the Southern Ocean during the Southern Ocean Clouds (SOC) campaign in November and December 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13186, https://doi.org/10.5194/egusphere-egu25-13186, 2025.

EGU25-13748 | ECS | Posters on site | AS4.4

Lagrangian single-column modeling of Arctic airmass transformation 

Michail Karalis, Gunilla Svensson, and Michael Tjernström

As warm and moist airmasses are advected into the Arctic, a sequence of turbulent, microphysical and radiative processes is initiated which transfers heat and moisture from the airmass into the Arctic environment, eventually transforming both. Despite the importance of airmass transformation for the evolution of the Arctic climate, it is still relatively poorly understood. In our study, we take on this complex issue from a Lagrangian perspective, using warm-air intrusions captured by different Arctic campaigns (ACSE, MOSAiC, HALO-(AC)3 and ARTofMELT) and the Atmosphere-Ocean Single Column Model (AOSCM). We use trajectory analysis to assess under what conditions and to what extent this Lagrangian AOSCM framework is suitable to study the Arctic airmass transformation. Finally, we use it to simulate the changes in heat-moisture content and vertical structure of the airmass at different stages of the transformation and identify the physical processes that drive them. Comparison with observations, reanalysis and operational forecast data shows that the Lagrangian AOSCM can be used for future model analysis and diagnostics development.

How to cite: Karalis, M., Svensson, G., and Tjernström, M.: Lagrangian single-column modeling of Arctic airmass transformation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13748, https://doi.org/10.5194/egusphere-egu25-13748, 2025.

EGU25-15288 | Posters on site | AS4.4

Investigation of virga with active remote sensing in Ny-Ålesund, Svalbard 

Andreas Foth, Beril Aydin, Maximilian Maahn, and Heike Kalesse-Los

The focus of this work is on sublimation and evaporation of precipitation. Precipitation is an
essential component of the Arctic climate system as part of the hydrological cycle, linking the
atmosphere and cryosphere. Much of the Arctic precipitation sublimates or evaporates before it
reaches the ground due to dry sub-cloud layers.

We use long-term atmospheric observations at Ny-Ålesund with vertically-pointing cloud radars
and backscattering lidars to identify and quantify atmospheric sublimation/evaporation. Radar
observation-based sub-cloud precipitation profiles are studied by employing a virga detection tool,
the so-called Virga-Sniffer (Kalesse-Los et al., 2023). The quantification of the sublimation/
evaporation is based on sub-cloud vertical gradients of radar moments. First statistical results of
precipitation phase, virga depth, and full sublimation/ evaporation altitude above ground will be
shown. Misclassification by the Cloudnet target classification within virga at precipitation edges
will be discussed in detail.

We will also show investigations on wind direction dependence on virga statistics. Air masses
advected from the Arctic Ocean are more humid and lead to more precipitation reaching the ground
and thus less virga. Air masses advected over Ny-Ålesund from Easterly directions (i.e. the island of
Svalbard itself) are often characeterized by low-humidity subcloud layers leading to more
evaporation/sublimation and hence a higher fraction of virga.

References:
Kalesse-Los, H., Kötsche, A., Foth, A., Röttenbacher, J., Vogl, T., and Witthuhn, J.: The Virga-
Sniffer – a new tool to identify precipitation evaporation using ground-based remote-sensing
observations, Atmos. Meas. Tech., 16, 1683–1704, https://doi.org/10.5194/amt-16-1683-2023,
2023.

How to cite: Foth, A., Aydin, B., Maahn, M., and Kalesse-Los, H.: Investigation of virga with active remote sensing in Ny-Ålesund, Svalbard, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15288, https://doi.org/10.5194/egusphere-egu25-15288, 2025.

EGU25-15714 | ECS | Orals | AS4.4

The Microphysical and Radiative Interactions of Arctic Multilayer Clouds  

Gabriella Wallentin, Luisa Ickes, Peggy Achtert, Matthias Tesche, and Corinna Hoose

Multilayer clouds have been found to occur frequently in the Arctic, as determined by ship-based campaigns. Nevertheless, they remain underrepresented in the literature compared to their single-layer counterpart. To deepen our understanding of these clouds regarding microphysics and radiative processes, and to estimate the frequency of occurrence of such phenomena in the Arctic region, we utilise the numerical weather prediction model ICON. 

The model domain, encompassing 71°N-90°N, has been initialised using analysis data from ICON Global and 32 consecutive 24-hour simulations were conducted at a 2.5km grid spacing. The multilayer clouds studied here occurred during the Arctic MOSAiC campaign, active during 2019-2020. The season with the highest number of multilayer clouds, as determined by an observational algorithm, was selected: namely, early autumn (August to September 2020). Model output was acquired at a high temporal resolution following the MOSAiC drifting site and includes full regional coverage of cloud hydrometeors and radiative products. To enhance the representation of Arctic ice nucleating particles (INP), a new immersion freezing parameterisation has been developed, underpinned by extensive Arctic campaigns and station data across the Arctic sector. 

Here, we will present modelled multilayer clouds across the Arctic sector, highlighting a high occurrence of such clouds in the region. We further investigate their microphysical and radiative properties in comparison to single-layer clouds. Using observational products from the MOSAiC campaign for comparison, we further strengthen our modelled understanding of these clouds. Our findings indicate that multilayer clouds differ significantly from single-layer clouds due to both microphysical and radiative interactions. In terms of microphysics, the seeder-feeder mechanism, whereupon frozen precipitation may act as a seed for ice formation in a lower cloud layer, is prevalent, impacting the cloud phase, precipitation and the formation of new cloud particles. In terms of radiative processes, multilayer clouds have been found to have a substantial radiative impact. The presence of upper clouds may efficiently reduce the cloud-top radiative cooling of lower cloud layers, impacting macrophysical cloud properties. Furthermore, we will demonstrate that multilayer clouds exert a surface radiation budget impact that is twice that of single-layer clouds. This emphasises the necessity for further investigation into these cloud systems in this rapidly changing region. 

How to cite: Wallentin, G., Ickes, L., Achtert, P., Tesche, M., and Hoose, C.: The Microphysical and Radiative Interactions of Arctic Multilayer Clouds , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15714, https://doi.org/10.5194/egusphere-egu25-15714, 2025.

EGU25-15924 | ECS | Posters on site | AS4.4

The two Arctic wintertime boundary layer states: Disentangling the role of cloud and wind regimes in reanalysis and observations during MOSAiC 

Sandro Dahlke, Annette Rinke, Matthew D. Shupe, and Christopher J. Cox

The central Arctic atmosphere during winter comprises two distinct synoptic states: a radiatively clear state, which is linked to clear sky, strong surface cooling and temperature inversions; and a radiatively opaque state, which is linked to mixed-phase clouds, weak surface radiative cooling, and more neutrally-buoyant boundary layers. Weather and climate models are often reported to lack the representation of processes associated with these states, but most prior work has treated the problem as an aggregate of synoptic conditions. Here, we disaggregate the Arctic states in an evaluation of ERA5 reanalysis and compare to observations from the MOSAiC drift campaign over the central Arctic sea ice from November 2019 – March 2020. Combining near surface winds and liquid water path (LWP), nine different classes describing synoptic conditions spanning the states are derived. Results show that the clear state is primarily formed by weak and moderate winds and the absence of liquid-bearing clouds, while strong wind cases and enhanced LWP forms the occurrence peak in the radiatively opaque state. ERA5 struggles to reproduce these basic statistics, shows too weak sensitivity of thermal radiation to synoptic forcing, and for similar LWP amounts, it overestimates both upward and downward longwave radiation due to a warm bias near the surface. This warm bias has a pronounced vertical structure and is largest in clear and calm conditions, owing to the lack of surface inversions in ERA5. Under strong synoptic forcing, the warm bias is constant with height and discrepancies in mixed-phase cloud altitude appear. Thus, biases in each state are partially opposing in a manner that makes them overlap unrealistically, masking the distinctions that are known to form the first-order variability of the Arctic winter energy budget. Separating between different synoptic conditions in conjunction with the classical two radiative states classification is therefore regarded a useful step for isolating dominant processes for evaluation of the Arctic troposphere in models.  

How to cite: Dahlke, S., Rinke, A., Shupe, M. D., and Cox, C. J.: The two Arctic wintertime boundary layer states: Disentangling the role of cloud and wind regimes in reanalysis and observations during MOSAiC, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15924, https://doi.org/10.5194/egusphere-egu25-15924, 2025.

EGU25-16621 | ECS | Orals | AS4.4 | Highlight

Marine sources of ice-nucleating proteins in the Arctic and their impact on atmospheric processes 

Lasse Z. Jensen, Christian Castenschiold, Corina Wieber, Claudia Mignani, Anne Ellebæk, Eva Kjærgaard, Dorte Søgaard, Bernadette Rosati, Luisa Ickes, Lars Lund-Hansen, Sigurd Christiansen, Leendert Vergeynst, Malin Alsved, Jakob Löndahl, Thomas Bataillon, Merete Bilde, Kai Finster, and Tina Šantl-Temkiv

The Arctic is particularly vulnerable to climate change due to a decrease in surface albedo caused by declining ice and snow cover. Aerosol-cloud feedbacks modulate Arctic warming, with clouds profoundly affecting the radiative balance of the region through both cooling and warming effects. The concentration and type of ice-nucleating particles (INP) are key factors controlling cloud ice formation which directly influences cloud radiative properties and lifetime. It has recently been proposed that microbially-produced INPs, which come from marine environments and can trigger freezing at low supercooling, are important for the formation of mixed-phase clouds in the Arctic. These clouds commonly form at low altitudes within the temperature range, where biogenic INPs are key drivers of ice formation. Despite their importance, it remains unclear which microorganisms are responsible for the production of marine INPs and under which conditions these are produced. This lack of knowledge limits our quantitative understanding of how high-temperature INPs from marine environments impact cloud formation in the Arctic.

To investigate marine-sourced INPs and their sources, we collected a series of marine- (i.e. seawater, sea-surface microlayer, and sea ice) and atmospheric aerosol samples from the west coast of Greenland between 2016 and 2023. We performed droplet-freezing measurements with the micro-PINGUIN setup to quantify INPs, along with chlorophyll a measurements, δO18 analysis, and amplicon sequencing of marker genes using Illumina MiSeq to determine the composition of bacteria (16S rRNA genes) and microalgae (18S rRNA genes) and identify potential producers of INPs. Using filtration analysis and heat treatments, we investigated the type of INPs identified in marine systems. We carried out field experiments and laboratory simulations using a modified cold-finger to study incorporation of INP from seawater into sea ice. Finally, we employed laboratory simulations using AEGOR the sea-spray tank to study emissions of bioaerosols and marine INP.

In the fjords, we observed a significant contribution of terrestrial sources to INPs in the marine waters during the early melting season with enhanced terrestrial runoff. These reflected in elevated INP concentrations, which were up to 10,000-fold higher that previously reported, with properties distinct from known marine INPs. In the open sea, we found that INP concentrations in seawater increased with latitude, independent of terrestrial freshwater input. While INP concentrations linked to marine microbial communities, they were surprisingly not tightly associated to phytoplankton blooms as previously suggested. We identified annual sea ice as a key reservoir of INPs, which exhibited INP concentrations up to 100-fold higher than the seawater below sea ice. INPs did not preferentially incorporate into the ice from seawater but were likely produced by the heterotrophic bacterial community in the early phase of sea ice growth. As the sea ice melts in the spring, these INPs are released into the surface seawater significantly contributing to the marine INP pool. Finally, through both field measurements and sea-spray experiments, we observed the transfer of marine INPs and microbial cells into the air. Ultimately, our research significantly enhances the understanding of marine microorganisms and their pivotal role in atmospheric processes within the Arctic region.

How to cite: Jensen, L. Z., Castenschiold, C., Wieber, C., Mignani, C., Ellebæk, A., Kjærgaard, E., Søgaard, D., Rosati, B., Ickes, L., Lund-Hansen, L., Christiansen, S., Vergeynst, L., Alsved, M., Löndahl, J., Bataillon, T., Bilde, M., Finster, K., and Šantl-Temkiv, T.: Marine sources of ice-nucleating proteins in the Arctic and their impact on atmospheric processes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16621, https://doi.org/10.5194/egusphere-egu25-16621, 2025.

EGU25-16625 | ECS | Posters on site | AS4.4

Seasonal Dynamics of Bioaerosols and Ice Nucleating Particles in the High Arctic Atmosphere 

Lasse Z. Jensen, Andreas Massling, Lise Lotte Sørensen, Henrik Skov, Frank Stratmann, Heike Wex, Kai Finster, and Tina Šantl-Temkiv

The Arctic is experiencing rapid climate change, with warming rates four times higher than the global average. This warming has a profound impact on the Arctic hydrological cycle, including cloud formation and precipitation processes. Bioaerosols are critical components driving these processes as they can act as high-temperature ice nucleating particles (INPs). Despite their importance, the representation of bioaerosol-cloud interactions in climate models remains highly uncertain, primarily due to limited understanding of biogenic INPs, their sources and specific properties. Recent studies have highlighted the need for long-term studies and detailed source characterization of INPs and their characteristics in the Arctic to bridge these knowledge gaps.

Here, we present preliminary data from the first long-term dataset of bioaerosol concentration and composition in the High Arctic, complementing detailed high-temperature INP measurements. The samples were collected at the Villum Research Station in North Greenland over three years (2021–2023) at a time resolution of 3.5 days. INP concentrations were measured using the Micro-PINGUIN cold-stage setup, focusing on activity between 0°C and -20°C. Simultaneously, bacterial communities in the air were characterized through qPCR and 16S rRNA gene amplicon sequencing. Source-tracking analyses were performed using potential environmental sources, including soils, glacial runoff, plant material, and seawater, supplemented with publicly available Arctic sequence datasets. Meteorological data and aerosol microphysical and chemical data, such as black carbon and particle number size distributions, were incorporated to support the analysis of bioaerosol drivers.

Preliminary results reveal that INP-12 concentrations ranged from 2.2 • 10-5 to 7.2 • 10-2 • L-1, consistent with previous observations in the High Arctic. Airborne bacterial concentrations were exceedingly low, ranging from 2.7 • 100 to 4.2 • 103 • m-3 of air, and the taxonomic diversity varied seasonally. During the Arctic haze season, the microbial community was dominated by spore-forming taxa, such as Bacillus, likely transported via long-range atmospheric transport from mid latitudes. In contrast, post-haze conditions were marked by increased microbial diversity, dominated by phototrophic taxa such as Tychonema and other members of the core cryospheric microbiome, including Sphingomonas and Hymenobacter. These taxa likely originated from regional terrestrial and marine sources, exposed to the atmosphere as snow and ice melted during summer. Both bacterial concentrations and the taxonomic diversity were positively correlated with the warm-temperature INP concentrations (ρ = 0.66, p = 3.6 • 10-12 and ρ = 0.59, p = 1.2•10-9,  respectively), suggesting a direct link between bioaerosol abundance and INP concentration in the Arctic atmosphere. Finally, Spearman rank correlations also revealed significant relationships between warm-temperature INP concentrations and the relative abundances of 177 microbial genera, giving insights into the potential sources of these INPs.

These findings provide new insights into the seasonal dynamics of bioaerosols and their role as INPs in the High Arctic. Our long-term dataset highlights the importance of integrating microbial ecology, aerosol microphysics and chemistry, and meteorological observations to improve our understanding of aerosol-cloud interactions. Future work will focus on disentangling the contributions of source environments and microbial taxa to Arctic INP populations, with the goal of refining aerosol-cloud interaction parameterizations in climate models.

How to cite: Jensen, L. Z., Massling, A., Sørensen, L. L., Skov, H., Stratmann, F., Wex, H., Finster, K., and Šantl-Temkiv, T.: Seasonal Dynamics of Bioaerosols and Ice Nucleating Particles in the High Arctic Atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16625, https://doi.org/10.5194/egusphere-egu25-16625, 2025.

EGU25-17011 | Orals | AS4.4

Precipitation events and atmospheric waves on Greenland's west coast 

Arno Hammann, Ruth Mottram, and Fredrik Boberg

The supply of atmospheric moisture in the Arctic is increasing with the warming global climate, owing both to higher volumes of moisture advection into the region and to enhanced local evaporation. Correspondingly, overall precipitation amounts and the frequency of large individual precipitation events are increasing as well. Due to the relative sparsity of observations in the region, however, the local microphysical and dynamical processes which translate the moisture content into precipitation remain poorly studied and classified. We build on a comprehensive observational dataset from a research site in Qeqertarsuaq, Greenland to characterise the local boundary layer structure during precipitation events. The observations include, besides standard surface climate parameters, atmospheric profiles of temperature and humidity from a microwave radiometer and cloud observations from an optical camera. Dynamical processes are studied by combining observations and the CARRA reanalysis, with a focus on internal gravity waves which trigger precipitation events when they interact with local topography and atmospheric moisture. Both our observations and CARRA are also used to validate and bias-correct simulations of regional atmospheric models (in particular, HIRHAM) performed as part of the PROTECT project, which allow an assessment of how the precipitation-generating processes will change in the future.

How to cite: Hammann, A., Mottram, R., and Boberg, F.: Precipitation events and atmospheric waves on Greenland's west coast, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17011, https://doi.org/10.5194/egusphere-egu25-17011, 2025.

EGU25-17572 | ECS | Posters on site | AS4.4

A calibration method for the UV-Vis-NIR and SWIR spectrometers installed at THAAO and its impact on the retrieval of cloud properties 

Angelica Focardi, Giovanni Muscari, Filippo Calì Quaglia, Monica Tosco, Daniela Meloni, Annalisa Di Bernardino, Virginia Ciardini, Tatiana Di Iorio, Giandomenico Pace, and Alcide di Sarra

A TriOS spectroradiometer (RAMSES-ARC) operating in the UV-Vis-NIR spectral range has been operating at the Thule High Arctic Atmospheric Observatory (THAAO, 76.5° N, 68.8° W, 225 m asl, https://www.thuleatmos-it.it/) in Pituffik, Greenland, since 2021. Its measurements are used to study Arctic cloud characteristics and the cloud optical thickness (COT) in particular. This effort will be extended with additional radiance measurements performed by means of a Zeiss PGS ShortWave InfraRed (SWIR) spectrometer which will be installed at the THAAO in March 2025 in order to further characterise cloud properties.

The RAMSES-ARC is used for in situ hyperspectral light field measurements, operating across a wavelength range of 320–950 nm with a field of view (FOV) of approximately 7° in air. The Zeiss spectrometer covers the 1000–2200 nm spectral range, is thermoelectrically cooled, and will be equipped with a custom-designed input optic to reduce the field of view of its standard fiber optic and with an in-house developed software for the data acquisition.

Ensuring long-term, high-quality measurements in extremely cold environments requires rigorous and repeated calibrations to maintain reliability across the entire spectral range. However, practical challenges, such as high costs and limited access to fully equipped calibration laboratories, often hinder the achievement of optimal calibrations. Furthermore, extended operations in low-temperature environments increase the risk of calibration drifts. This study presents a structured and repeatable calibration procedure that can be easily implemented in settings where advanced laboratory equipment is unavailable.

The calibration method employs a Gigahertz Optik GmbH 250 W halogen calibration lamp powered by a highly stabilised current source. The lamp’s optical axis is aligned perpendicularly to the centre of a Labsphere panel with a reflectance factor of about 0,99 for wavelengths shorter than 1800 nm and between 0,98 and 0,94 for wavelengths between 1800 nm and 2200 nm. The panel is positioned at a distance from the lamp optimised using ANSYS SPEOS software to ensure uniform irradiance distribution across the panel.

Additionally, this presentation will discuss the impact of the new calibration on COT estimates obtained by using the method described in Calì Quaglia et al. (2024).

The primary objective is to prove that the new calibration method maintains measurement integrity while guaranteeing repeatability and accuracy, particularly in scenarios requiring frequent recalibration.

Calì Quaglia, Filippo, et al. (2024), On the Retrieval of Cloud Optical Thickness from Spectral Radiances - A Sensitivity Study with High Albedo Surfaces, Journal of Quantitative Spectroscopy and Radiative Transfer, https://doi.org/10.1016/j.jqsrt.2024.109108.

How to cite: Focardi, A., Muscari, G., Calì Quaglia, F., Tosco, M., Meloni, D., Di Bernardino, A., Ciardini, V., Di Iorio, T., Pace, G., and di Sarra, A.: A calibration method for the UV-Vis-NIR and SWIR spectrometers installed at THAAO and its impact on the retrieval of cloud properties, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17572, https://doi.org/10.5194/egusphere-egu25-17572, 2025.

EGU25-17930 | ECS | Posters on site | AS4.4

What are the most important contributors to Arctic precipitation: When, where and how? 

Melanie Lauer, Annette Rinke, Susanne Crewell, and Awadhesh Pant

To investigate the role of synoptic systems for Arctic precipitation, Lauer et al. (2023) established a new methodology to attribute precipitation to Atmospheric Rivers (AR), cyclones, and also atmospheric fronts and tested it for two field campaigns in the Arctic North Atlantic (ANA) sector (ACLOUD, AFLUX). The results led us to hypothesize that during early summer, precipitation is mainly associated with cyclones, while during early spring, ARs and fronts are more effective. About one-third of the precipitation was classified as residual, which reduced significantly when a precipitation threshold was applied as often used to eliminate “artificial” precipitation. To investigate whether these results can be generalized we now apply the methodology of Lauer et al. (2023) to the long-term (1979-2022) ERA-5 reanalysis record over the full Arctic north of 70 deg.

When: Most precipitation falls in August as a consequence of rain peaking in July and the highest amount of snowfall in September at the time of the sea ice minimum and thus the highest evaporation from the ocean. Where: The ANA region is by far the one with the most precipitation, and the only region with significant rain outside the summer months. How: Cyclone-associated precipitation dominates in all regions, while ARs are more important for summer rainfall and, in some regions, can even bring rain in winter. We can pinpoint the high occurrence of residual precipitation over the ANA region to Marine Cold Air Outbreaks, while in the central Arctic the residual stems from very light precipitation.

How to cite: Lauer, M., Rinke, A., Crewell, S., and Pant, A.: What are the most important contributors to Arctic precipitation: When, where and how?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17930, https://doi.org/10.5194/egusphere-egu25-17930, 2025.

EGU25-18439 | Posters on site | AS4.4

Modelling cloud phase and radiative effects in the European Arctic 

Yaël Le Gars, Jean-Christophe Raut, and Louis Marelle

Arctic clouds, which cover the region for around 70-80% of the year, are a key component of the Arctic climate system, influencing, among others, surface temperature, ice melt and atmospheric dynamics. Mixed-phase clouds, containing both supercooled liquid water and ice crystals, are of particular concern due to their prevalence in the Arctic and their role in the local energy budget. Because their variability and their lifecycle are inaccurately represented in models, they are an important source of uncertainty, as the cloud phase impacts both radiative effects, cloud lifetime and precipitation amounts. Assessing the vertical distribution of clouds, their optical properties and their phase distribution is therefore critical to accurately determine the surface energy balance (SEB). 

 

Here, the mesoscale WRF (Weather Research and Forecasting) updated for application in polar regions is run over the European Arctic from January to June 2015. The simulations are evaluated using observations from the N-ICE campaign, conducted from January through June 2015 in the drifting sea ice north of Svalbard (surface radiation and meteorology, atmospheric profiles), as well as satellite data derived from CALIPSO and CloudSat observations. The simulated SEB as well as low-level cloud distributions and phase partitioning are evaluated to get insight on the limitations of the model to represent Arctic clouds and the factors underlying these biases. 

 

This study reveals strong biases in radiative fluxes at the surface, even when cloudy conditions are successfully represented in the model, with effects varying across seasons. Results show that these discrepancies are likely to be strongly linked to the accurate phase characterization of clouds. Sensitivity tests based on variations in CCN and INP number concentrations reveal moderate effects on the radiative budget through changes in liquid water content, insufficient to account for the observed biases.

How to cite: Le Gars, Y., Raut, J.-C., and Marelle, L.: Modelling cloud phase and radiative effects in the European Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18439, https://doi.org/10.5194/egusphere-egu25-18439, 2025.

EGU25-18587 | Posters on site | AS4.4

Cloud optical thickness measurements in high albedo conditions at the Thule High Arctic Atmospheric Observatory (THAAO), Greenland 

Giovanni Muscari, Filippo Calì Quaglia, Monica Tosco, Daniela Meloni, Annalisa Di Bernardino, Tatiana Di Iorio, Angelica Focardi, Giandomenico Pace, Sebastian K. Schmidt, and Alcide di Sarra

In the Arctic, cloud optical thickness (COT) estimations are scarce due to limited site accessibility, short sunlit seasons, and high surface albedo, which enhances the multiple scattering. This work presents a comparison of estimates of COT obtained by means of different types of measurements collected on the north-western coast of Greenland, an area presenting alternatively high and low surface albedo, depending on the season. Our approach exploits ground-based zenith spectral radiance (ZSR) measurements in the 320-950 nm wavelength range as well as downward shortwave irradiance (DSI, 310-2800 nm) and Liquid Water Path (LWP) measurements. All measurements are carried out at the Thule High Arctic Atmospheric Observatory (THAAO, 76.5° N, 68.8° W, 225 m asl, https://www.thuleatmos-it.it/), where  LWP measurements have been performed from 2016 to 2024, while DSI and ZSR measurements started in 2009 and 2021, respectively, and are still ongoing. The analysis also includes COT values from MODIS aboard Terra/Aqua. 

COT values are calculated for two case studies of low and high surface albedo values, focusing on total cloud cover conditions and liquid clouds. The COT values retrieved from the ZSRs are obtained by using various combinations of transmissivities at different wavelengths. Numerical simulations allowed us to provide uncertainties for the ZSR COT estimates. We found that the use of broadband albedo values in the retrievals instead of spectrally-resolved ones is the largest source of uncertainties. The COT values obtained with the different methods during the two case studies range between 1 and 45.

Results show that the ZSR-based retrievals lack sensitivity for clouds with COT between 6 and 14. Numerical simulations can explain this shortcoming and they will also be presented. For COT larger than 14, the ZSR-based estimates agree very well with the other methods employed. We will discuss in detail how the different estimates compare to one another and show that, given the observatory measurements capabilities, estimates of COT could be performed continuously and with good accuracy in high surface albedo conditions by means of ZSR and DSI measurements.

How to cite: Muscari, G., Calì Quaglia, F., Tosco, M., Meloni, D., Di Bernardino, A., Di Iorio, T., Focardi, A., Pace, G., Schmidt, S. K., and di Sarra, A.: Cloud optical thickness measurements in high albedo conditions at the Thule High Arctic Atmospheric Observatory (THAAO), Greenland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18587, https://doi.org/10.5194/egusphere-egu25-18587, 2025.

EGU25-18624 | ECS | Orals | AS4.4

Properties of Arctic mixed-phase clouds explored by multi-frequency radars 

Linnu Bühler, Sabrina Schnitt, Mario Mech, Janna Rückert, Nils Risse, Pavel Krobot, and Susanne Crewell

Arctic mixed-phase low-level clouds pose a large challenge to weather and climate models. The new G-band radar GRaWAC (G-band Radar Water vapor profiling and Arctic Clouds) is a frequency-modulated continuous wave radar with two frequencies at 167.3 and 174.8 GHz. Measurements at higher frequencies than conventional cloud radars and near the 183 GHz water vapor absorption line enable for extracting water vapor profiles in clouds by making use of the differential absorption technique for measurements at the two frequencies. In combination with radar measurements in the W-band, the high frequencies also make the observations of small hydrometeors in the non-Rayleigh regime possible, enabling future retrievals of hydrometeor phase and size distribution based on differential radar measurements.

We present observations from the ship-based campaign VAMPIRE that took place from August to October 2024 in the Central Arctic Ocean on the research vessel Polarstern and from a ground-based intensive operation period from January to March 2025 at AWIPEV station in Ny-Ålesund, Svalbard. The G-band radar GRaWAC alongside a W-band radar measured in both campaigns, while the observations at AWIPEV were expanded by including a Ka-band radar. First results show the presence of mixed-phase clouds which will be evaluated in their respective environmental conditions, determined by wind and precipitation measurements, and 6- to 12-hourly radiosondes. The contribution will present the post-processed radar data of both intensive measurement periods, including attenuation and ship motion correction, and first analyses of microphysical properties in mixed-phase clouds and water vapor profiles.

How to cite: Bühler, L., Schnitt, S., Mech, M., Rückert, J., Risse, N., Krobot, P., and Crewell, S.: Properties of Arctic mixed-phase clouds explored by multi-frequency radars, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18624, https://doi.org/10.5194/egusphere-egu25-18624, 2025.

EGU25-18964 | ECS | Posters on site | AS4.4

Investigating the Atmospheric and Biological Significance of Ice-Nucleating Macromolecules Produced by Antarctic Mosses 

Nina L. H. Kinney, Floortje van den Heuvel, Amélie Kirchgaessner, Thomas Lachlan-Cope, Mark D. Tarn, Daniel Ballesteros, and Thomas F. Whale

Ice-nucleating particle (INP) concentration in the atmosphere over the Southern Ocean represents a significant source of uncertainty in the representation of clouds in global climate models. A better understanding of the sources, properties and abundance of INPs in this region is essential to reduce this uncertainty (Murray, 2021). There is increasing evidence to suggest that ice nucleators are produced ubiquitously by land plants. Yet, the molecular basis and evolutionary origins of these ice nucleators remain obscure. Adapted for cold- and drought-tolerance, mosses dominate the Antarctic flora, with over one hundred species colonising the ice-free coastal regions of Antarctica and their land cover increasing (Roland 2024). Ice nucleation by moss spores and leaves was recorded separately by Weber (2016) and by Moffett (2015), who suggested that this activity may afford benefit as a means of gathering essential water in dry climates. In the years since, the atmospheric and biological significance of these ice nucleators has remained unexplored. Here we present evidence that mosses produce water-soluble ice-nucleating macromolecules that are present in the gametophyte and sporophyte generations. We hypothesise that the same class of ice-nucleating macromolecules are produced by the spore-producing mosses and ferns and the pollen-producing seed plants, tracing back to an ancient common ancestor. The widespread and variable nature of ice-nucleating activity in plants suggests that this activity is secondary or ‘incidental’ in function (Kinney, 2024). Nevertheless, it is conceivable that such activity may constitute an exaptation, having been selected for in the evolution of taxa adapted to specific environmental conditions. Notably, we find Antarctic moss species exhibit high ice-nucleating activity, reaching temperatures of -7.4 °C, within the range where secondary ice-production may further enhance ice crystal numbers in clouds. As such, we suggest that mosses may represent a previously unknown source of ice nucleators in the atmosphere over the Southern Ocean.

References:

N. L. H. Kinney, C. A. Hepburn, M. I. Gibson, D. Ballesteros, and T. F. Whale. High interspecific variability in ice nucleation activity suggests pollen ice nucleators are incidental. Biogeosciences, 21(13):3201–3214, 2024.

B. F. Moffett. Ice nucleation in mosses and liverworts. Lindbergia, 38(1):14–16, 2015.

B. J. Murray, K. S. Carslaw, and P. R. Field. Opinion: Cloud-phase climate feedback and the importance of ice-nucleating particles. Atmospheric Chemistry and Physics, 21(2):665–679, 2021.

T. P. Roland, O. T. Bartlett, D. J. Charman, et al. Sustained greening of the Antarctic peninsula observed from satellites. Nature Geoscience, 17:1121–1126, 2024.

C. F. Weber. Polytrichum commune spores nucleate ice and associated microorganisms increase the temperature of ice nucleation activity onset. Aerobiologia, 32(2):353–361, 2016.

How to cite: Kinney, N. L. H., van den Heuvel, F., Kirchgaessner, A., Lachlan-Cope, T., Tarn, M. D., Ballesteros, D., and Whale, T. F.: Investigating the Atmospheric and Biological Significance of Ice-Nucleating Macromolecules Produced by Antarctic Mosses, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18964, https://doi.org/10.5194/egusphere-egu25-18964, 2025.

EGU25-19437 | Posters on site | AS4.4

Comparison of ERA5 and CARRA reanalyses with long-term atmospheric measurements at the THAAO, Greenland 

Filippo Calì Quaglia, Giovanni Muscari, Angelica Focardi, Virginia Ciardini, Annalisa Di Bernardino, Tatiana Di Iorio, Daniela Meloni, Giandomenico Pace, Monica Tosco, and Alcide di Sarra

The Thule High Arctic Atmospheric Observatory (THAAO, www.thuleatmos-it.it) is a strategically important site for collecting atmospheric measurements in the Arctic. Located in Pituffik (76.5° N, 68.8° W, 225 m asl) on the Greenland west coast, it experiences harsh environmental conditions and offers invaluable atmospheric measurements otherwise scarce in the region. Over the past decade, increased visits to the observatory have facilitated the expansion, maintenance, and upgrading of its instruments. More than 15 instruments are currently operating at the THAAO, measuring atmospheric and surface climate parameters. Among those are upward- and downward-looking pyranometers and pyrgeometers, radiosondes, microwave spectrometers for atmospheric composition, lidar and ceilometer systems, and a weather station also providing precipitation measurements.

This study compares two prominent reanalysis datasets - ERA5 and the C3S Arctic Regional Reanalysis (CARRA) - produced by the Copernicus Climate Change Service (C3S). Ground-based measurements of various atmospheric parameters, including local and column-integrated variables, are used for this comparison. CARRA delivers higher spatial resolution (2.5 km) but lower temporal resolution (3-hourly) data, concentrating on Greenland and utilising ERA5's global reanalysis (0.25° x 0.25° and hourly) as lateral boundary conditions.

The analysis extends over a period ranging from 3 to 15 years, depending on the parameter, and includes key variables such as temperature, relative humidity, integrated water vapour, radiation components (shortwave and longwave), precipitation, cloud base height, wind speed and direction. In addition, over 50 radiosonde measurements, unevenly distributed between 2016 and 2024, are exploited in the comparison. The data used in this study have not been assimilated into the reanalysis under consideration, allowing an independent evaluation.

The impact of different temporal and spatial resolutions of the reanalyses will be assessed. The climatological length of the reanalyses (> 30 years) allows the assessment of seasonal and annual trends, as well as the regional impact of extreme events over a long time span.

How to cite: Calì Quaglia, F., Muscari, G., Focardi, A., Ciardini, V., Di Bernardino, A., Di Iorio, T., Meloni, D., Pace, G., Tosco, M., and di Sarra, A.: Comparison of ERA5 and CARRA reanalyses with long-term atmospheric measurements at the THAAO, Greenland, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19437, https://doi.org/10.5194/egusphere-egu25-19437, 2025.

EGU25-19981 | ECS | Posters on site | AS4.4

Airborne in-situ cloud observations around the Antarctic peninsula from the Southern Ocean Clouds project  

Floortje van den Heuvel, Dan Smith, Freya Squires, Jonathan Witherstone, Mike Flynn, Jessica Girdwood, Jiawei Xu, and Thomas Lachlan-Cope

Clouds are a major source of uncertainty in climate model projections over the Southern Ocean and Antarctica1. The inaccurate representation of clouds in climate models results in biases in the net radiative balance which has knock-on effects on the ability of models to represent sea surface temperatures, ocean heat uptake, sea ice cover, and ultimately large-scale circulation in the Southern Hemisphere2,3,4,5,6. Evidence suggests that this is due to the poor representation of mixed phase clouds in models—the dominant cloud type in this region.

As part of the Southern Ocean Clouds project, we have conducted two flying campaigns out of Rothera research station which is located on the Antarctic peninsula, in order to investigate the composition of clouds over the Southern Ocean. Over the course of two field seasons (one in the 2022-23, and one in the 2024-25 Antarctic season) we performed more then 40 flights consisting of over 140 flying hours. During these flights we measured ice crystal, water droplet and aerosol number concentrations and sizes. We also collected Ice Nucleating Particles on filters in addition to performing measurements of meteorological parameters, turbulence, and radiative balance. 

Here we will present an overview of the flying campaign of the 2024-25 season, and compare the observations conducted this year to those which were made during our previous campaign in the 2022-23 season. Although we saw higher droplet number concentrations for the 2024-25 campaign than during the 2022-23 campaign, both revealed the presence of higher droplet number concentrations at higher altitudes (> 2000 m asl) indicating a potential long range source for these. 

1 Bodas-Salcedo, A., et al., 2014: Origins of the Solar Radiation Biases over the Southern Ocean in CFMIP2 Models. J. Climate, 27, 41–56, https://doi.org/10.1175/JCLI-D-13-00169.1. 

2 Lauer, A., et al., 2018: Process-level improvements in CMIP5 models and their impact on tropical variability, the Southern Ocean and monsoons. Earth Syst. Dynam., 9, 33–67, https://doi.org/10.5194/esd-9-33-2018. 

3 Frölicher, T. L., et al., 2015: Dominance of the Southern Ocean in Anthropogenic Carbon and Heat Uptake in CMIP5 Models. J. Climate, 28, 862–886, https://doi.org/10.1175/JCLI-D-14-00117.1. 

4 Ferrari and Ferreira 2011: what processes drive the ocean heat transport? Ocean. Model., 38, 171-186, https://doi.org/10.1016/j.ocemod.2011.02.013. 

5: Ceppi P., et al., 2012: Southern Hemisphere Jet latitude biases in CMIP5 models linked to shortwave cloud forcing. Geophys. Res. Lett, 39, 19: https://doi.org/10.1029/2012GL053115. 

6 Y. Hwang, D.M.W. Frierson, 2013: Link between the double-Intertropical Convergence Zone problem and cloud biases over the Southern Ocean, Proc. Natl. Acad. Sci. U.S.A., 110 (13) 4935-4940, https://doi.org/10.1073/pnas.1213302110 

How to cite: van den Heuvel, F., Smith, D., Squires, F., Witherstone, J., Flynn, M., Girdwood, J., Xu, J., and Lachlan-Cope, T.: Airborne in-situ cloud observations around the Antarctic peninsula from the Southern Ocean Clouds project , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19981, https://doi.org/10.5194/egusphere-egu25-19981, 2025.

EGU25-20517 | ECS | Posters on site | AS4.4

Virga Detection Tool based on Micro Rain Radar in Arctic 

Lekhraj Saini, Saurabh Das, and Nuncio Murukesh

Virga known as precipitation that fails to reach to the ground due to evaporation/sublimation beneath the cloud base. Virga is commonly observed in hot and arid regions where dry air helps in the process [1]. In a warming climate, virga is increasingly observed in cold environments such as Antarctica and Switzerland as sublimation of snow [2,3]. Virga precipitation constitutes occurrences over 30% in TRMM, GPM and 50% in Cloudsat in arid regions and accounts for 50% (30%) of false precipitation detections by TRMM (GPM) satellites. Virga plays a crucial role in quantifying total precipitation, particularly in remote regions like the Arctic where virga is poorly studied. Accurate identification of virga is essential to improve precipitation estimates derived from satellite radar observations, which are limited in Arctic regions. This study introduces the Arctic Virga Detection Algorithm (ArViDAM), which uses ground-based vertical precipitation observations from Micro Rain Radar (MRR) deployed at Ny-Ålesund (78° 55' N, 11° 56' E) in the Arctic to identify virga events based on reflectivity and fall velocity profiles up to 6 km.

Figure: (top) Time-height series profile of (a) Ze, (b) W, and (c) SW for 13th–14th June, 2020 includes virga and surface precipitation with detected virga height with black line. (bottom) Seasonal variation of occurrence of virga and surface precipitation during 2020-2023.

A summer event presented in Figure shows the sensibility of the ArViDAM with detected virga height on the time-height profile of reflectivity (Ze), fall velocity (W), and spectral width (SW) during 13th–14th June, 2020. ArViDAM outcomes from 2020–23 indicate that summer has the highest virga occurrence with∼40%, followed by spring and autumn with∼30% and winter with the lowest∼22%. The outcomes are expected to enhance understanding of Arctic precipitation processes and contribute to quantitative precipitation estimation. 

Keywords—Virga, Arctic Precipitation, Sublimation, Micro Rain Radar, Climate Change

 

References

 

[1] Wang, Y. You, and M. Kulie, “Global virga precipitation distribution derived from three spaceborne radars and its contribution to the false radiometer precipitation detection,” Geophysical Research Letters, vol. 45, no. 9, pp. 4446–4455, 2018. [Online]. Available: https://agupubs.onlinelibrary.wiley. com/doi/abs/10.1029/2018GL077891.

 

[2] N. Jullien, E. Vignon, M. Sprenger, F. Aemisegger, and A. Berne, “Synoptic conditions and atmospheric moisture pathways associated with virga and precipitation over coastal ad´elie land in Antarctica,” The Cryosphere, vol. 14, no. 5, pp. 1685–1702, 2020. [Online]. Available: https://tc.copernicus.org/articles/14/1685/2020/. 

 

[3] R. Beynon and K. Hocke, “Snow virga above the swiss plateau observed by a micro rain radar,” Remote Sensing, vol. 14, no. 4, 2022. [Online]. Available: https://www.mdpi.com/2072-4292/14/4/890.

How to cite: Saini, L., Das, S., and Murukesh, N.: Virga Detection Tool based on Micro Rain Radar in Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20517, https://doi.org/10.5194/egusphere-egu25-20517, 2025.

EGU25-21627 | ECS | Posters on site | AS4.4

Landfalling Atmospheric Rivers in the Antarctic Peninsula: Synoptic Evolution and Oceanic Feedback  

Matilde Rafacho, Alizee De Groodt, Paulo Avilez-Valente, Claudio Durán-Alarcón, Sangjong Park, and Irina Gorodetskaya

Atmospheric rivers (ARs), increasingly recognized for their substantial influence on polar regions, are characterized as long, narrow corridors of intense moisture transport that play a crucial role in the redistribution of heat and water vapor toward higher latitudes. These systems profoundly affect precipitation regimes, surface melt dynamics, and, consequently, the surface mass balance of Antarctica (Wille et al., 2021). Additionally, ARs interact with oceanic processes, influencing wave activity, sea spray aerosol production, and feedback mechanisms that can impact cloud microphysics and precipitation. In the Antarctic Peninsula (AP), ARs have been associated with anomalous snowfall, extreme melting events, and transitions between snowfall and rainfall. A notable example occurred in February 2022, when an intense AR event resulted in unprecedentedly high temperatures, extensive surface melting across the AP and anomalously high rainfall amounts in the northern AP, underscoring their significant role in regional climate variability (Gorodetskaya et al., 2023).

Building on prior findings, this study examines a February 2023 AR event using observations at King Sejong Station, King George Island (radiosondes and precipitation radar MRR-PRO), ERA5 reanalysis and WAVEWATCH III model. The AR was driven by a deep low-pressure system west of the AP and a high-pressure ridge to the northeast, creating strong moisture advection and cyclonic uplift. Integrated Vapor Transport (IVT) values exceeded 400–600 kg/m−1 s−1 during peak days, with a distinct influence of baroclinic zones and fronts identified using wet-bulb potential temperature gradients at 850-hPa level. These conditions facilitated enhanced vertical motion, cloud development, and significant precipitation, primarily as snowfall in inland and higher- altitude regions of the AP. Concurrently, the strong winds associated with the AR enhanced wave activity and whitecapping in the surrounding Southern Ocean, increasing sea spray aerosol production, which could potentially influence cloud microphysical properties.

Furthermore, thermodynamic conditions during the AR were characterized by pronounced baroclinicity and the interaction of warm, moist subtropical air with cold polar air, which sustained cloud formation and moisture convergence. Later in February, as cyclonic activity weakened and IVT values decreased below 200 kg/m−1 s−1, precipitation became less intense and spatially confined. However, residual moisture flux and localized thermodynamic forcing supported light snowfall, even as synoptic features transitioned toward zonal flow. The dynamic interplay between AR-driven moisture transport, cyclonic uplift, oceanic feedback, and synoptic transitions underscores the significant role of ARs in modulating cloud and precipitation properties over the AP.

Acknowledgements: We are grateful for financial and logistical support via FCT projects MAPS and MICROANT, PROPOLAR and KOPRI

References:

Gorodetskaya, I.V. et al. “Record-high Antarctic Peninsula temperatures and surface melt in February 2022: a compound event with an intense atmospheric river” (2023) https://www.nature.com/articles/s41612-023-00529-6

Wille, J. D. et al. (2021) “Antarctic atmospheric river climatology and precipitation impacts” J. Geophys. Res. Atmos. 126, e2020JD033788

How to cite: Rafacho, M., De Groodt, A., Avilez-Valente, P., Durán-Alarcón, C., Park, S., and Gorodetskaya, I.: Landfalling Atmospheric Rivers in the Antarctic Peninsula: Synoptic Evolution and Oceanic Feedback , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21627, https://doi.org/10.5194/egusphere-egu25-21627, 2025.

EGU25-21662 | Posters on site | AS4.4

Atmospheric Rivers and Antarctic Peninsula Precipitation Phase Transitions 

Irina V. Gorodetskaya, Claudio Durán-Alarcón, Xun Zou, Penny Rowe, Vincent Favier, and Sangjong Park

Atmospheric rivers (AR) are long, narrow, transient corridors of intense atmospheric moisture transport affecting many regions around the world including Antarctica, where they play an important role in surface mass and energy balance. Over the Antarctic Peninsula (AP), one of the most rapidly warming regions, ARs have been increasing in frequency and intensity causing major heatwaves, anomalous precipitation and surface melt [1,2]. The impact of ARs would not be as intense without global warming [3] and thus it is urgent to understand processes driving ARs and their impacts using observations and improve their representation in the models used for weather forecasts and for future climate projections. One of the most worrying impacts is the increasing frequency of rain both during summer and winter seasons over the AP, which can drastically change surface energy and mass balance as well as impact fragile ecosystems. Understanding processes driving the transitions from snowfall to rainfall in time, location and in vertical profile - during all-weather events and particularly during ARs - is one of our key goals for collecting precipitation and radiosonde measurements at King Sejong station on King George Island, north of the AP. Since February 2023, we have been operating MRR-PRO, a 24-GHz vertically profiling precipitation radar from which we can derive effective reflectivity, Doppler velocity, melting layer height and precipitation rates. King Sejong is also equipped with automatic weather stations providing near-surface meteorological parameters, broadband surface radiation, precipitation-gauge measurements and snow height. Cloud lidar measurements using miniMPL at Escudero station are available via NASA’s MPLnet [4]. Here we present the evolution of ARs and associated snowfall and rainfall properties during two years of observations (2023-2024). The spatial distribution of precipitation from ERA5 and high-resolution Polar-WRF simulations for specific events demonstrates a transition from rainfall in the northern AP to snowfall in its southern part with significant orographic enhancement over the western upwind side of the AP. Vertical profiling with MRR at King Sejong shows significant variability in the melting layer attaining higher altitudes (up to 3km) during AR events. Combining MRR and radiosonde observations during a selected AR in February 2024 showed strong temperature inversions in the first 3 km with a melting layer varying in height between 3 km and near surface, accompanied by a sharp transition from snowfall to rain. Observations are used to evaluate representation of precipitation in ERA5 and in Polar WRF.

Acknowledgements: We thank FCT (projects MAPS/MICROANT); PROPOLAR; KOPRI; ANR (project ARCA).

References:

[1] Wille, J.D., et al. (2019): West Antarctic surface melt triggered by atmospheric rivers. Nat. Geosci.

[2] Gorodetskaya et al. (2023): Record-high Antarctic Peninsula temperatures and surface melt in February 2022: a compound event with an intense atmospheric river. npj Clim Atmos Sci.

[3] González-Herrero et al. (2022): Climate warming amplified the 2020 record-breaking heatwave in the Antarctic Peninsula. Commun. Earth Env..

[4] Rowe et al. (2025) Observations of Clouds and Radiation Over King George Island and Implications for the Southern Ocean and Antarctica, JGR, in review.

How to cite: Gorodetskaya, I. V., Durán-Alarcón, C., Zou, X., Rowe, P., Favier, V., and Park, S.: Atmospheric Rivers and Antarctic Peninsula Precipitation Phase Transitions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21662, https://doi.org/10.5194/egusphere-egu25-21662, 2025.

EGU25-957 | ECS | Posters on site | CL4.4

Exploring Dynamics of Climate and Atmosphere Employing the Temperature Indices Using Bias-Corrected GCMS and Ensemble Model Approach 

Gupta Abhishek Rajkumar, Manish Kumar Nema, and Deepak Khare

Urban areas significantly influence planetary processes by altering heat, moisture and chemical budgets and it plays a pivotal role in modifying planetary processes through their unique interactions with the environment. The reduction in natural vegetation and permeable surfaces limits evapotranspiration and alters the hydrological balance, often leading to increased surface runoff, reduced groundwater recharge and changes in local humidity levels. The current study evaluates the spatial and temporal variation of temperature extremes for the historical period (1951–2014) and the future scenarios of two Shared Socioeconomic Pathways; SSP245 and SSP 585 for the future periods of 2015-2100, divided into two periods; near future (2015-2050) and far future (2051-2100) for the major tributary of The River Godavari; The Wainganga Basin, India. The temperature data for the basin is sourced from five General Circulation Models (GCMs) and an ensemble model derived from them. The ensemble model incorporates climate forecasts and accounts for anticipated space-weather-related atmospheric perturbations, resulting in a more complete knowledge of fluctuations in temperature in the Wainganga River Basin. The temperature variation due to climate change is evaluated using the extreme climate indices influenced by minimum and maximum temperature, recommended by the Expert Team on Climate Change Detection and Indices (ETCCDI) and Expert Team on Sector-Specific Climate Indices (ET-SCI). These indices provide a standardized framework for assessing the impacts of driving forces of dynamic temperature and atmospheric processes. The findings will showcase the impact of changes in temperature and their effects temporally, and spatially on the sub-basin level also address the change in atmosphere strongly with the type of driver, time, and location. As global urbanization continues, insights from studies like this are crucial for developing and evaluating adaptive strategies. Conclusively, findings can inform policies aimed at climate resilience, drawing parallels with urban climate adaptation efforts. 

How to cite: Rajkumar, G. A., Nema, M. K., and Khare, D.: Exploring Dynamics of Climate and Atmosphere Employing the Temperature Indices Using Bias-Corrected GCMS and Ensemble Model Approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-957, https://doi.org/10.5194/egusphere-egu25-957, 2025.

Understanding future changes in temperature variability and extremes is an important scientific challenge. Here, the response of daily near-surface temperature distributions to warming is explored using an idealised global climate model.  Simulations of a wide range of climate states are performed with a slab-ocean aquaplanet configuration and with a simple land continent using a bucket-style model for hydrology. In the tropics, the responses of temperature extremes (i.e., high percentiles of daily near-surface temperature) to climate change contrast strongly over land and ocean. Over land, warming is amplified for hot days relative to the average day. But over ocean, warming is suppressed for hot days, implying a narrowing of the temperature distribution. 

Previous studies have developed theories based on convective coupling to interpret changes in temperature extremes over land. Building on this work, here the contrasting temperature distribution responses over land and ocean are investigated using a new theory based on strict convective equilibrium, which assumes moist adiabatic lapse rates. The theory highlights four physical mechanisms with the potential to drive differential warming across the temperature distribution: hot-get-hotter mechanism, drier-get-hotter mechanism, relative humidity change mechanism, and the free tropospheric temperature change mechanism.  Hot days are relatively dry over land due to limited moisture availability, which drives the drier-get-hotter mechanism and  amplified warming of the warm tail of the distribution. This mechanism is the dominant factor explaining the contrasting responses of hot days over land and ocean to climate change. An extended version of the theory, which relaxes the strict convective equilibrium assumption, is introduced and applied to the simulations to understand the influence of convective available potential energy (CAPE) on changes in the temperature distribution. 

How to cite: Duffield, J. and Byrne, M.: Tropical temperature distributions over a range of climates: theory and idealised model simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1397, https://doi.org/10.5194/egusphere-egu25-1397, 2025.

EGU25-1648 | ECS | Orals | CL4.4

Different Roles of Land-atmosphere Coupling in Compound Drought-heatwave Events 

Donghyuck Yoon, Jan-Huey Chen, Hsin Hsu, and Kirsten Findell

Droughts and heatwaves are inherently linked through land-atmosphere (L-A) coupling, where the interactions between surface energy and water availability play critical roles in their evolution. In energy-limited regimes, anomalously high surface air temperature (T) intensifies evapotranspiration (ET), leading to rapid depletion of soil moisture (SM). Conversely, in water-limited regimes, reduced SM suppresses ET, exacerbating surface warming. The transition between these two regimes, characterized by critical soil moisture thresholds, governs the progression of compound drought-heatwave events.

This study analyzed the spatiotemporal variability of L-A coupling mechanisms during six extreme compound drought-heatwave events. In all cases, SM exhibited a consistent negative temporal correlation with T, declining from the onset to the peak of the heatwave and recovering during the decay phase. However, the behavior of ET varied, with SM-ET coupling dominating in some cases and T-ET coupling prevailing in others. These distinctions in coupling regimes demonstrated regional heterogeneity, even within individual events. As regimes shifted from T-ET to SM-ET coupling, evaporative fraction (EF) on heatwave peak days significantly decreased, underscoring that the drivers of drought-heatwave interactions differ spatially. Furthermore, correlation analysis between SM and EF revealed that critical soil moisture thresholds are key determinants of these coupling behaviors. This highlights the role of critical soil moisture in modulating L-A feedbacks and controlling the transition between coupling regimes.

Using the GFDL SHiELD global 13-km model configuration, we evaluated the predictability of two prominent events in 2022 and 2023, which displayed contrasting dominant regimes. SHiELD effectively captured the spatial distribution and temporal evolution of L-A coupling regimes in both cases. Notably, the SM-ET coupling-dominated 2023 event demonstrated superior forecast skill for SM and TMAX compared to the T-ET coupling-dominated 2022 event. This result emphasizes the importance of soil moisture memory in water-limited regions for enhancing predictability in compound drought-heatwave scenarios.

How to cite: Yoon, D., Chen, J.-H., Hsu, H., and Findell, K.: Different Roles of Land-atmosphere Coupling in Compound Drought-heatwave Events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1648, https://doi.org/10.5194/egusphere-egu25-1648, 2025.

EGU25-1850 | ECS | Orals | CL4.4

Nonlinear interactions amplify the most extreme midlatitude heatwaves  

Yinglin Tian, Jiangong Liu, Yu Huang, Pierre Gentine, and Kai Kornhuber

Recent occurrences of record-breaking heat extremes and their profound societal impacts on health, infrastructure, food systems, and the energy sector underscore the urgent need to improve our physical understanding and modeling capacities for future projections. In mid-latitude regions, persistent high-pressure systems and dry soils have been identified as key contributors to heatwave severity. Moreover, non-linear interactions between these two drivers and temperature have been suggested to play a critical role in some of the most extreme recent heat events, such as the 2021 Pacific-North America heatwave (Bartusek et al., Nat. Clim., 2022). However, the universality and regional significance of such non-linear interactions remain largely unquantified.

Using an explainable machine learning approach, we quantitatively decompose surface air temperature anomalies during heat extremes into three components: direct contributions from (i) geopotential height anomalies, (ii) soil moisture deficits, and (iii) the interaction between the two. Our analysis reveals that non-linear interactions make statistically significant contributions across 19% of the land area in the northern hemisphere mid-latitudes (40°N–60°N). In these regions, the interactive contribution increases with temperature at a rate of 0.1 K/K when temperatures exceed a critical threshold of 4.0 K above the local summer mean. Hotspots of such behavior are especially pronounced in Central Europe, where 40% of the land area exhibits significant non-linear interactions, amplifying the most extreme heatwave events by up to 13%.

Furthermore, we identify a 2.4-fold increase in the regional mean non-linearity of interactions in Central Europe over the past 45 years, accompanied by a 25% expansion in the affected area. This accounts for 18% of the observed widening in the temperature distribution’s upper tail reported in other studies (Kornhuber et al., PNAS, 2024). Additionally, our findings show that CMIP6 climate models underestimate the non-linearity of extratropical interactions by 80%, contributing to biases in projections of extreme heat changes. Our findings underscore the critical role of these non-linear physical processes in amplifying extreme heatwave events, emphasizing the need to account for these processes in climate models to better anticipate and mitigate the impacts of climate extremes in current and future climates.

How to cite: Tian, Y., Liu, J., Huang, Y., Gentine, P., and Kornhuber, K.: Nonlinear interactions amplify the most extreme midlatitude heatwaves , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1850, https://doi.org/10.5194/egusphere-egu25-1850, 2025.

EGU25-2239 | ECS | Orals | CL4.4

A simple complementary framework for evaluating evaporation base on land-atmosphere coupling 

Zhuoyi Tu, Yuting Yang, Michael Roderick, and Tim McVicar

Evaporation (E) is a key process in land-atmosphere water and energy exchanges. Among the evaporation methods, the complementary relationship (CR) approach builds upon the dynamic feedbacks of water and heat fluxes between the land-atmosphere interface, providing a straightforward framework for estimating evaporation using basic meteorological inputs, without relying on complex land surface information. Although CR is a simple and effective method, traditional CR mechanisms/models still face two main challenges. First, the wet boundary condition of CR is inaccurately characterized. When the land surface is not water-limited, evaporation is defined as potential evaporation (Epo). However, Epo estimates using conventional methods often do not align with its fundamental definition, as meteorological variables observed under real conditions differ from those over a hypothetical wet surface. Here, we estimate Epo using the maximum evaporation approach (Epo_max) that does follow the original Epo definition. Our findings show that using Epo_max significantly reduces the asymmetry in the CR. Second, traditional CR mechanisms focus on the feedback between water vapor and temperature in the land-atmosphere system, while overlooking the impact of these changes on radiation. As the surface transitions from dry to wet, enhanced actual evaporation and reduced sensible heat flux lead to cooler and wetter air above the surface, reducing the vapor pressure deficit and further decreasing atmospheric evaporative capacity (or apparent potential evaporation, Epa). Building on this, we found temperature reduction overall increases the radiation term in Epa and partially offsets the traditional view that water vapor weakens the aerodynamic term. Based on the above modifications, we developed a physically-based, calibration-free CR model, which requires few input variables and thus facilitates evaporation estimation. More importantly, the CR method, grounded in land-atmosphere coupling, offers a simpler framework for studying the feedback of evaporation on climate, making it a promising tool compared to complex coupled climate models.

How to cite: Tu, Z., Yang, Y., Roderick, M., and McVicar, T.: A simple complementary framework for evaluating evaporation base on land-atmosphere coupling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2239, https://doi.org/10.5194/egusphere-egu25-2239, 2025.

Tropical regions have undergone extensive deforestation in recent decades, significantly impacting local, regional, and global water cycles; however, detailed studies on their hydroclimatic effects remain limited. This study employs a regional climate model coupled with a water vapor tracking tool to investigate the effects of deforestation on local and regional precipitation from 2000 to 2020 in three major tropical deforestation hotspots: the Amazon, Africa, and Southeast Asia. Results indicate that deforestation affects precipitation with distinct scale-dependent and seasonal variations. In the Amazon, contrasting precipitation responses to deforestation were observed between wet and dry seasons (Yingzuo Qin et al., Nature, 2025, in press). During the wet season, deforested areas exhibited a notable increase in precipitation (0.96 mm month-1 per percentage point of forest loss), primarily due to enhanced mesoscale atmospheric circulation (i.e., nonlocal effects). These nonlocal effects weakened with distance from deforested areas, resulting in significant precipitation reductions beyond 60 km. Conversely, during the dry season, precipitation decreased in deforested areas and across all analysis buffers, with local effects from reduced evapotranspiration (ET) dominating. In Africa, due to the dispersibility of deforestation across the continent, the scale-dependency and seasonality of precipitation effects caused by deforestation are influenced by elevation and deforestation patch size. In Southeast Asia, under the strong influence of oceanic water vapor, deforestation-induced positive precipitation effects prevail throughout the year. These findings underscore the complex interplay between local and nonlocal effects in driving tropical deforestation-precipitation responses across different seasons and scales, highlighting the urgent need to address the rapid and extensive loss of forests in tropical regions to mitigate their nonnegligible climatic impacts.

How to cite: Qin, Y.: Tracking tropical deforestation impacts on local and regional hydroclimate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2431, https://doi.org/10.5194/egusphere-egu25-2431, 2025.

EGU25-3078 | Orals | CL4.4

Soil moisture controls on convective initiation across the diverse landscapes and hydro-climates of Africa 

Christopher Taylor, Cornelia Klein, and Emma Barton

A wealth of studies exist analysing the feedback between soil moisture and convective precipitation across a broad range of time and space scales, encompassing theoretical, numerical modelling and observational approaches. A critical step in this feedback is an understanding of how soil moisture, via its control on sensible and latent heat fluxes, influences the initiation of deep convective clouds. Knowledge of where soil moisture conditions favour triggering of new storms is also important for short-term weather forecasting. Whilst many analyses consider how soil moisture affects the vertical profiles of temperature and humidity (1-D perspective), other studies examine the role of spatially-varying soil moisture on convective initiation via surface-induced mesoscale circulations. Here we use a 20-year observational dataset of convective initiations across sub-Saharan Africa to draw more general conclusions about how soil moisture impacts convective initiation and subsequent rainfall across a diversity of hydro-climatic, topographic and wind conditions.

We use cloud-top temperature data from the geostationary Meteosat Second Generation (MSG) series of satellites to identify afternoon convective initiations for the period 2004-2023 and relate these to pre-storm observations of land surface state (land surface temperature from MSG, and surface soil moisture from the Advanced Scatterometer). Both datasets reveal a consistent Africa-wide picture of initiations favoured at the downwind end of elliptical dry soil structures, as found in previous analyses over the Sahel (Taylor et al, Nature Geoscience, 2011). The soil moisture signal weakens with stronger topographic variability, and in wetter climates and times of year, but outside of the Congo Basin and East African Highlands, the signal of initiation over locally dry soils is clear. Moreover, we show that the along-wind length scale of the dry soil feature increases with low-level wind speed. Our results, valid on scales of up to ~200km, fit with understanding of mesoscale circulations driven by soil moisture heterogeneity, and cannot be explained by 1-D consideration of thermodynamic profiles alone. We also show how the overall soil moisture-precipitation feedback from these events is influenced by wind conditions at storm steering level. In regions (including the Sahel) where winds at low and steering levels are in opposing directions, the feedback is strongly negative. Alternatively, when low and mid-level winds are aligned, the negative feedback weakens, and can become positive.

How to cite: Taylor, C., Klein, C., and Barton, E.: Soil moisture controls on convective initiation across the diverse landscapes and hydro-climates of Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3078, https://doi.org/10.5194/egusphere-egu25-3078, 2025.

The vegetation-temperature feedback significantly influences local climate variability. While previous studies have assessed the responses of local temperature to vegetation biomass changes, they often suffer from the mix of long-term global warming trends and localized vegetation-temperature interactions. More importantly, the temporal evolutions of this feedback remain elusive. Here, we use a novel approach to analyze spatiotemporal variations of this local feedback while controlling for global warming trends. Our findings reveal a weakening role of vegetation in cooling the earth over the past four decades, with a nonlinear feedback change modulated by background climatologic conditions. Furthermore, an evaluation of state-of-the-art climate models shows a systematic overestimation of vegetation cooling effects, particularly in densely vegetated regions. This overly optimistic bias contributes to a significant underestimation of global warming, highlighting the need to improve the representation of vegetation-climate interactions in climate models.

How to cite: Liu, Z., Peng, X., and He, X.: Spatiotemporal dynamics in vegetation-temperature feedback and overly optimistic representations in climate models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3628, https://doi.org/10.5194/egusphere-egu25-3628, 2025.

EGU25-4252 | Orals | CL4.4

Soil moisture–precipitation feedbacks in Central Europe: Fully coupled WRF-Hydro simulations evaluated with cosmic-ray neutron soil moisture measurements 

Joël Arnault, Benjamin Fersch, Martin Schrön, Heye Reemt Bogena, Harrie-Jan Hendricks Franssen, and Harald Kunstmann

The skill of regional climate models partly relies on their ability to represent land–atmosphere feedbacks in a realistic manner, through the coupling with a land surface model. However, these models often suffer from insufficient or erroneous information on soil hydraulic parameters. In this study, the fully coupled land–atmosphere model WRF-Hydro driven with ERA5 reanalysis is employed to reproduce the regional atmospheric conditions over Central Europe with a horizontal resolution of 4 km for the period 2017–2020. Simulated soil moisture is compared with data from cosmic-ray neutron sensors (CRNS) at three terrestrial environmental observatories of the TERENO network. Soil hydraulic parameters from the European digital soil dataset EU-SoilHydroGrids, together with hydraulic conductivity functions from the Campbell and van Genuchten–Mualem models, are used to test the impact of different representations of soil infiltration on modeled land–atmosphere feedbacks. An updated method to disentangle the proportion of convective precipitation being favored over wet, dry and mixed soils is provided, in order to shed more light on the soil moisture–precipitation feedback mechanism. It is found that WRF-Hydro with van Genuchten–Mualem and EU-SoilHydroGrids best reproduces CRNS soil moisture daily variations, in association with enhanced soil moisture in the root zone and a larger proportion of convective precipitation favored over wet soils. This study demonstrates the importance of adequately considering infiltration processes to realistically reproduce land–atmosphere feedbacks.

How to cite: Arnault, J., Fersch, B., Schrön, M., Bogena, H. R., Hendricks Franssen, H.-J., and Kunstmann, H.: Soil moisture–precipitation feedbacks in Central Europe: Fully coupled WRF-Hydro simulations evaluated with cosmic-ray neutron soil moisture measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4252, https://doi.org/10.5194/egusphere-egu25-4252, 2025.

EGU25-4419 | ECS | Posters on site | CL4.4

Identification of climatic extremes by multi-fractal analysis of long climate data series 

Carl Tixier, Pierre-Antoine Versini, and Benjamin Dardé

Shrinking and swelling of clays (SSC), occur as a result of water content fluctuations in expansive clayey soils, governed by seasonal cycles of precipitation and drought. This hazard causes ground movement, which can affect foundations and infrastructures. In France, where 54% of constructions are exposed to this hazard, SSC is the second largest category for natural disaster compensation.

With climate change, modification in the intensity and frequency of droughts, heat waves and precipitation are likely to exacerbate this phenomenon. In this context, further research is needed to anticipate the influence of climatic changes on the evolution of the SSC hazard and its impact on constructions in the next decades.

In particular, it is crucial to understand soil-atmosphere interactions on some appropriate spatial and temporal scales, but also through scales. Climate impact studies use hydrological or agricultural models, fed by global climate data adapted locally by statistical adjustments or downscaling. These methods improve local accuracy but increase bias and uncertainty, as they are often based on stationarity assumptions, which are not always valid in the context of climate change. The modeling of extreme values, essential for risk management, thus becomes more complex.

In response to the difficulties of climate models in representing extreme events at high spatio-temporal resolutions, and in understanding hydro-climatic interactions with clay soil, several geostatistical approaches are proposed.

An in-depth study of the existing literature has enabled us to compare the various downscaling methods. This state of the art is complemented by the study of data (extreme meteorological phenomena, humidity, soil displacements, etc.) acquired by various organizations concerned by the SSC problem (sources: BRGM, INRAE, SNCF, Météo-France, etc.).

This presentation will include the results of geostatistical analyses based on (multi)fractals conducted on this data (spatiotemporal variability, scale breaks, estimation of extreme values, spectral analysis, etc.). The data analyzed will cover the main parameters influencing soil moisture, i.e., precipitation and temperature.

These analyses may reveal the statistical signatures of climatic extremes. By identifying them, it will then be possible to research the different climate scenarios, and thus represent the extremes with precision. This step is essential to understanding SSC phenomena.

The final objective of this research work is to propose a soil-atmosphere interaction model, capable of generating the input data required for a numerical SSC behavior model. This model will take into account the various hydro-climatic parameters mentioned above, focusing mainly on evaporation and infiltration processes, as well as soil heterogeneity.

How to cite: Tixier, C., Versini, P.-A., and Dardé, B.: Identification of climatic extremes by multi-fractal analysis of long climate data series, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4419, https://doi.org/10.5194/egusphere-egu25-4419, 2025.

Tibetan Plateau has been experiencing profound warming and slight wetting over recent decades, which have contradictive effects on soil organic carbon by enhancing plant growth and thereafter carbon input into the soil and increasing the soil organic carbon (SOC) decomposition rate. In this study, we developed a SOC model (WetlandC model) for wetlands, considering also the process of litterfall decomposition and parameterizing the effect of grazing on SOC accumulation. We also established a modelling framework to combine WetlandC model with TEM (Terrestrial Ecosystem Model) model to simulate the changes in SOC of the alpine wetlands on the Tibetan Plateau from 2000 to 2018. Results showed that spatially, the soil organic carbon density (SOCD) of alpine wetlands was higher in the southeast and lower in the northwest, ranging from 1358.22 to 22571.81 g C m-2. The SOCD spatial pattern coincided with the northernmost and southernmost northern boundary of Asian summer monsoon. The SOCD was higher in region with precipitation ranging from 450 to 900 mm, suggesting that the precipitation played an important role in regulating the spatial heterogeneity of SOCD. The temporal trends of SOCD varied from -55.84 to 407.59 g C m-2 yr-1 over the plateau, and 97.98% of the wetland area was accumulating SOC. Temperature, precipitation and actual livestock carrying capacity, as the top influencing factors of the temporal trend of SOCD, accounted for 35.06%, 34.52% and 30.41% of the area in the alpine wetlands, respectively. The 0–30 cm SOC stock of the alpine wetlands on the Tibetan Plateau increased from 518.06 Tg C in 2000 to 607.67 Tg C in 2018. Surface soil in the alpine wetlands acts as a carbon sink of 4.98 Tg C yr-1. Our results indicated that in the context of climate change, additional soil carbon sequestration in the alpine wetlands was facilitated by enhanced plant growth, in spite that grazing consumed the above-ground biomass. Future climate warming and wetting is likely to benefit the SOC accumulation in the alpine wetlands on the Tibetan Plateau if not overgrazed.

How to cite: Zhang, Q.: Effects of climate change and grazing on soil organic carbon stock of alpine wetlands on the Tibetan Plateau, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4887, https://doi.org/10.5194/egusphere-egu25-4887, 2025.

Soil moisture (SM) is a crucial factor in land-atmosphere interactions and climate systems, affecting surface energy, water budgets, and weather extremes. In the Three Rivers Source Region (TRSR) of China, rapid climate change necessitates precise SM monitoring. This study employs a novel UNet-Gan model to integrate and downscale SM data from 17 CMIP6 models, producing a high-resolution (0.1◦) dataset called CMIP6UNet−Gan. This dataset includes SM data for five depth layers (0-10 cm, 10-30 cm, 30-50 cm, 50-80 cm, 80-110 cm), four Shared Socioeconomic Pathways (SSP1-2.6, SSP2-4.5, SSP3-7.0, SSP5-8.5). The UNet-Gan model demonstrates strong performance in data fusion and downscaling, especially in shallow soil layers. Analysis of the CMIP6UNet−Gan dataset reveals an overall increasing trend in SM across all layers, with higher rates under more intense emission scenarios. Spatially, moisture increases vary, with significant trends in the western Yangtze and northeastern Yellow River regions. Deeper soils show a slower response to climate change, and seasonal variations indicate that moisture increases are most pronounced in spring and winter, followed by autumn, with the least increase observed in summer. Future projections suggest higher moisture increase rates in the early and late 21st century compared to the mid-century. By the end of this century (2071-2100), compared to the Historical period (1995-2014), the increase in SM across the five depth layers ranges from: 5.5% to 11.5%, 4.6% to 9.2%, 4.3% to 7.5%, 4.5% to 7.5%, and 163.3% to 6.5%, respectively.

How to cite: Luo, S. and Li, Z.: Trend Analysis of High-Resolution Soil Moisture Data Based on GAN in the Three River Source Region During the 21st Century, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5586, https://doi.org/10.5194/egusphere-egu25-5586, 2025.

The representation of snow in land surface models is critical for accurate seasonal forecasting, yet traditional single-layer snow schemes fail to capture the full insulating properties of deep snowpacks. These limitations result in pronounced seasonal biases, including excessive winter cooling and springtime warming. This study explores the impact of introducing a multi-layer snow scheme within the Global Seasonal Forecast System (GloSea) to address these biases. Using 24 years of retrospective forecasts (1993–2016), we compare the latest version, GloSea6, incorporating the multi-layer scheme, with GloSea5, which relies on a single-layer approach. The multi-layer snow scheme in GloSea6 improves the onset of snowmelt, delaying it by approximately two weeks. This delay moderates spring soil moisture depletion, promoting greater latent heat flux and surface evaporative cooling. The wetter surface reduces the overestimation of water-limited processes and mitigates near-surface warming biases during summer. Additionally, the enhanced representation of snow improves the simulation of precipitation, particularly in snowmelt-driven regions such as the Great Plains, Europe, and South and East Asia, leading to substantial error reductions. These findings highlight the critical role of a multi-layer snow scheme in advancing seasonal forecast accuracy, not only for temperature and precipitation during snowmelt but also for subsequent summer climatic conditions through improved land-atmosphere feedback processes.

How to cite: Seo, E. and Dirmeyer, P.: Unveiling the influence of multi-layer snowpack in seasonal forecast system on model climatological bias, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5714, https://doi.org/10.5194/egusphere-egu25-5714, 2025.

EGU25-5959 | ECS | Orals | CL4.4

Recurring and Co-Occurring Climate Extremes in Eastern Africa. A Normalcy? 

Peter K. Musyimi, Tamás Weidinger, Tímea Kalmár, Lucia Mumo, and Balázs Székely

Recurring and co-occurring extreme climate events exacerbate adverse effects on human livelihoods, regional and local economy, and the environment. Previous studies have extensively researched on the frequency, intensity, and duration of single climate extremes. However, recurring and co occurrence compound extremes remain scantly addressed in the East Africa Region. Here, we examine spatial variations of the precipitation and temperature extremes events from 1991 to 2022 (32 years) in East Africa, where agriculture is the main economic mainstay. We used high-resolution (0.25° x 0.25°) precipitation and temperature ERA5-reanalysis data. Three agriculturally relevant precipitation events: consecutive dry days (CDD), consecutive wet days (CWD), annual total precipitation that is wet-days annual amount (RR ≥ 1 mm)(PRCPTOT),  and three core temperature metrics: summer days with temperature > 25°C (SU25), extremely hot days with maximum temperature > 35°C (SU35) and diurnal temperature range (DTR) are examined. Our results show that the mean annual CDD ranges between 0 and 240 days in DR Congo, Uganda, Kenya, and the Ethiopian Highlands. The CWD annual averages were the longest, and the maximum was observed in some parts of DR Congo, Ethiopian, and Kenya highlands (365 days). However, minimum CWD events were experienced in the whole of Somalia and arid and semi-arid lands (ASALs) of Kenya, Southern Sudan, and Tanzania. The highest PRCPTOT was experienced in high altitudes and rainforest biomes. Mean annual SU25 were low, predominating in mountainous regions with less than 100 days. Most parts of Kenya show the annual DTR between 10 °C to 12 °C, and few areas with values between 8 °C to 10 °C and between 12 °C and 15 °C. Rwanda and Burundi had values between 8 °C and 10 °C while Tanzania experienced values between 8 °C to 10 °C and between 10 °C and 12 °C. These agriculturally relevant climate extremes threaten people’s livelihood, which is highly dependent on rainfed agriculture. Therefore, contextual-specific adaptation strategies are imperative in minimizing socioeconomic loss and damaging adverse effects in the agriculture and water sectors. Early warning systems should be enforced over East Africa to minimize compounded climate risks.

Keywords: Climate Extremes; East Africa region; ERA5; Precipitation; Temperature.

How to cite: Musyimi, P. K., Weidinger, T., Kalmár, T., Mumo, L., and Székely, B.: Recurring and Co-Occurring Climate Extremes in Eastern Africa. A Normalcy?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5959, https://doi.org/10.5194/egusphere-egu25-5959, 2025.

EGU25-7299 | ECS | Orals | CL4.4

Land climate under warming in radiative-convective equilibrium simulations 

Tara Gallagher and Kaighin McColl

A simple way to model Earth’s climate is to assume radiative-convective equilibrium (RCE), where surface fluxes transport heat and water vapor away from the surface, and radiative cooling balances this energy in the atmosphere. This framework has provided basic insight into the effect of warming on climate over oceans with both fixed and interactive surface temperatures, but it is seldom applied over land. Unlike oceans, land surfaces have a limited water supply and a small heat capacity, and may respond quite differently given these features. Here, we run a suite of cloud-permitting simulations in RCE over land both with interactive soil moisture and fixed at saturation. In contrast to the most relevant previous studies, our simulations span a wide range of climates, obtained by varying the top-of-atmosphere insolation and atmospheric CO2 concentrations. Several notable patterns emerge as surface temperatures rise including non-monotonic trends in precipitation and steady declines in soil moisture, neither of which can be explained with existing theory. The results demonstrate distinctions between land and ocean responses to warming, with implications for land climate sensitivity and hydrological sensitivity.

How to cite: Gallagher, T. and McColl, K.: Land climate under warming in radiative-convective equilibrium simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7299, https://doi.org/10.5194/egusphere-egu25-7299, 2025.

EGU25-7752 | ECS | Orals | CL4.4

Causal Dynamics of Land–Atmosphere Coupling under Compound Dry–Hot Events 

Yikui Zhang, Daniel Hagan, Diego G. Miralles, Klaus Goergen, and Stefan Kollet

The increasing frequency and magnitude of compound dry–hot events (CDHEs) pose significant risks to natural and managed systems. While the role of land–atmosphere coupling in determining the magnitude and evolution of CDHEs has been highlighted, the causal interactions between variables within the coupled system under external forcing remain poorly understood. This study investigates the causal relationships between soil moisture and 2m air temperature, as well as between absorbed shortwave solar radiation and 2m air temperature during CDHEs, based on information flow theory. Using two fully coupled simulations with the Terrestrial Systems Modeling Platform (TSMP), one with and one without irrigation, the information flow analysis provides an interpretable framework to characterize the spatiotemporal variability of the land–atmosphere coupling strength in response to the perturbations such as CDHEs and irrigation. 

The results show that concurrent dry and hot conditions are characterized by temporal shifts in the evaporative regime towards increased soil moisture–temperature information flow driven by the shift in surface energy partitioning, such that decreases in soil moisture lead to increased temperatures. Meanwhile, irrigation can significantly reduce the frequency and magnitude of CDHEs by directly increasing soil moisture variability and indirectly affecting surface energy fluxes, and thus altering land–atmosphere coupling. However, the impact of irrigation in Europe is predominantly local and limited by the volumes applied. These findings highlight the potential of targeted, region-specific irrigation strategies to attenuate dry and hot extremes. In addition, the information flow framework provides a robust and interpretable tool for diagnosing the functional performance of regional climate models under perturbations, offering new insights for analyzing the impacts of human interventions on the climate system and enhancing our understanding of extreme hydroclimatic events in future studies.

How to cite: Zhang, Y., Hagan, D., Miralles, D. G., Goergen, K., and Kollet, S.: Causal Dynamics of Land–Atmosphere Coupling under Compound Dry–Hot Events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7752, https://doi.org/10.5194/egusphere-egu25-7752, 2025.

EGU25-8597 | ECS | Orals | CL4.4

Dynamic Impacts of Eurasian Spring Snowmelt on Summer Heat Extremes in Northern East Asia 

Yulong Yang, Qinglong You, and Taylor Smith

Eurasian spring snowmelt (ESS) significantly influences climate, yet its effects on climate extremes and their dynamic variations remains poorly understood. This study investigates the dynamic impact of ESS on summer heat extremes in Northern East Asia (NEA) during 1979–2018 and examines the underlying mechanisms driving long-range links between snowmelt and temperature anomalies. We find that ESS has a notable positive impact on NEA summer heat extremes, primarily driven by snow-hydrological effects (soil-moisture). Increased ESS drives positive local soil-moisture anomalies in summer, which cool the near-surface atmosphere, facilitating the eastward propagation of anomalous wave patterns. This process strengthens the anomalous anticyclone over NEA, amplifying summer heat extremes. We also find that the Atlantic Multidecadal Oscillation modulates this impact, with its positive phase significantly enhancing the ESS effect by altering atmospheric circulation, strengthening the coupling between spring snowmelt and summer soil moisture, and intensifying NEA heat extremes. This study underscores the critical role of ESS in driving atmospheric circulation over wide regions, and highlights the coupled impacts of multi-scale and multi-temporal climate variability.

How to cite: Yang, Y., You, Q., and Smith, T.: Dynamic Impacts of Eurasian Spring Snowmelt on Summer Heat Extremes in Northern East Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8597, https://doi.org/10.5194/egusphere-egu25-8597, 2025.

EGU25-8944 | ECS | Posters on site | CL4.4

How shallow and deep groundwater impact environmental parameters correlated with global heatwaves 

Anastasia Vogelbacher, Mehdi H. Afshar, Milad Aminzadeh, Kaveh Madani, Amir AghaKouchak, and Nima Shokri

Heatwaves present serious challenges to ecosystems, human health, and a wide range of socioeconomic activities. As the frequency and intensity of heatwaves increase, understanding the mechanisms driving their dynamics and interactions with land surface processes become more important. While extensive research has investigated the influence of various land and atmospheric parameters on heatwaves, less is known about how groundwater depth influences heatwave dynamics through their effects on soil moisture and surface evaporative fluxes (Vogelbacher et al., 2024, Sadeghi et al., 2012). To address this knowledge gap, we investigated how the groundwater depth affects the key parameters controlling heatwave dynamics on a global scale. Specifically, we developed more than 200,000 localized Artificial Intelligence (AI) models to represent the spatial distribution of heatwave frequency over the past 21 years across the world. For each model, a radius of 1.5 degrees (approximately 149 neighboring pixels) is considered in the computation to identify key parameters contributing to heatwaves in that region. We analyzed surface fluxes, as well as atmospheric, hydrological, and local environmental variables, to understand their correlation to heatwaves. Our findings suggest that geopotential height representing atmospheric drivers, is the key predictor of heatwave events in regions with deep groundwater tables (>100 m). In contrast, in areas with shallow groundwater (<10 m), surface fluxes emerge as important contributor to the onset of heatwaves. These findings highlight the less-discussed impact of groundwater depth on atmospheric processes and the important role of soil in linking groundwater and the atmosphere. Our results have important implications for water and land management, emphasizing the need for integrated approaches to understand and address the increasing risks posed by heatwaves.

 

References:
Sadeghi, M., Shokri, N., Jones, S.B. (2012). A novel analytical solution to steady-state evaporation from porous media. Water Resour. Res., 48, W09516, https://doi.org/10.1029/2012WR012060

Vogelbacher, A., Aminzadeh, M., Madani,K., Shokri, N. (2024). An analytical framework to investigate groundwater‐ atmosphere interactions influenced by soil properties. Water Resour. Res., 60, e2023WR036643. https://doi.org/10.1029/2023WR036643

How to cite: Vogelbacher, A., Afshar, M. H., Aminzadeh, M., Madani, K., AghaKouchak, A., and Shokri, N.: How shallow and deep groundwater impact environmental parameters correlated with global heatwaves, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8944, https://doi.org/10.5194/egusphere-egu25-8944, 2025.

The global land carbon sink is reduced by climate change, in particular by extreme events such as droughts, heatwaves, and fires1,2. Soil moisture, including its feedback on atmospheric conditions (SA), was identified as one of key drivers of these climate extremes3-6 and contributes to the negative climate effects on the land carbon uptake7,8. However, the extent to which the total climate impact on land carbon uptake can be explained by SA feedback remains unknown. Here, we develop an analytical framework utilizing multiple factorial model experiments to show that SA feedback contributes more than half (–61.6 ± 10.4%) of the total climate effect on land carbon uptake at a global scale during 1981–2014, with the largest contributions from hot and dry regions. The strengthened SA feedback has shifted the climate impact on land carbon uptake from near-neutral during 1981–1997 to largely negative during 1998–2014, primarily by weakening photosynthesis. By the end of the twenty-first century, projected reductions in land carbon uptake caused by the SA feedback could even double under a high emission scenario relative to the historical period, driven by increased soil moisture variability. Our findings highlight that SA feedback will potentially dominate the response of long-term land carbon uptake to climate change.

How to cite: Zeng, Z.: Soil moisture-atmosphere feedback controls more than half of total climate effects on land carbon uptake, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10175, https://doi.org/10.5194/egusphere-egu25-10175, 2025.

EGU25-12031 | ECS | Orals | CL4.4

Buffering of climate extremes within riparian forest corridors: a theoretical study with practical applications 

Myrtille Grulois, Sylvain Dupont, Caroline Bidot, Rémi Lemaire-Patin, and Jérôme Ogée

Riparian forests in tropical and temperate regions often act as climatic microrefugia for many species and taxa, buffering climate extremes relative to their surroundings. For example, during a summer heatwave, maximum air temperatures can vary by several degrees between the edge and the core of the riparian forest understory. This buffering of climate extremes within riparian corridors is well documented, but the processes behind it are not well understood because they involve complex turbulent air flows throughout the convective atmospheric boundary layer interacting with the forest canopy and landscape microtopography. To better understand how forest cover and microtopography influence the microclimate within and above riparian corridors, we performed in silico experiments using a 3-dimensional Large Eddy Simulation (LES) vegetation-atmosphere model to simulate air flows and microclimate below and above the trees, and across the entire convective boundary layer. Simulations were performed for different atmospheric stability conditions, and for different corridor widths. The tree species composition in the riparian corridor and its microtopography (slope, aspect) were chosen to be representative of an old-growth temperate riparian forest known to act as a climate refugium for European beech in south-west France. In this context, we first investigated the effect of microtopography alone on the air flows below and above the forest canopy during a typical summer heatwave. We also investigated the impact of replacing maritime pine plantations on the plateau with a strip of deciduous trees extending beyond the riparian corridor, with the aim to evaluate the minimum strip size required to mitigate climate extremes in the riparian understory.

How to cite: Grulois, M., Dupont, S., Bidot, C., Lemaire-Patin, R., and Ogée, J.: Buffering of climate extremes within riparian forest corridors: a theoretical study with practical applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12031, https://doi.org/10.5194/egusphere-egu25-12031, 2025.

EGU25-12438 | Orals | CL4.4

Identifying regional drivers shaping daily maximum temperatures and their extremes   

Sarosh Alam Ghausi and Axel Kleidon

Daily maximum air temperatures (Tmax) are shaped by radiation, advection, atmospheric circulation, and land-surface processes, all interacting through complex feedbacks but essentially reflecting changes in the local surface energy budget. Here, we use a land-atmosphere systems approach to derive an analytical expression for daily maximum temperatures that depends solely on observed radiative and surface-evaporative conditions, requiring no additional parameters. We do this by accounting for the surface energy balance, heat storage variations within the lower atmosphere and explicitly constrain vertical turbulent exchange using the thermodynamic limit of maximum power. This approach reproduces observations very well with residual errors comparable to the reanalysis data. We then applied it to understand variations in Tmax and found that its day-to-day variability is predominantly shaped by shortwave cloud radiative effects and longwave water-vapor emissivity in the humid tropics, while heat advection and storage effects are the primary contributors in drier subtropics and high latitudes. Hot extremes, however, are mostly shaped by anomalies in land-surface characteristics including soil water stress and turbulent fluxes, with secondary contributions from heat advection and radiative effects. Both variability and extremes in the tropics were linked to changes in moisture, while the heat-storage and advective effects dominate in dry subtropics and high-latitude regions. These findings reveal the regional radiative and hydrological drivers of temperature variations within the thermodynamic energy budget and provide a baseline for understanding biases and inter-model variability in climate models. It can further help in assessing first-order changes in daily maximum temperatures due to various aspects of global change.

How to cite: Ghausi, S. A. and Kleidon, A.: Identifying regional drivers shaping daily maximum temperatures and their extremes  , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12438, https://doi.org/10.5194/egusphere-egu25-12438, 2025.

EGU25-12862 | Orals | CL4.4

Tailoring Land Use, Land-Use Change, and Forestry (LULUCF) Impacts for Stakeholder-Centric Climate Policy 

Julia Pongratz, Suqi Guo, Felix Havermann, Michael Windisch, Steven De Hertog, Amali Amali, Fei Luo, Iris Manola, Quentin Lejeune, and Carl-Friedrich Schleussner

The land sector plays an important role in addressing global climate change: Land use, land-use change, and forestry (LULUCF) is currently responsible for about 10-15% of annual anthropogenic CO2 emissions, including the only notable origins of negative emissions to date; both emissions and removals aspects make LULUCF a key focus of future climate mitigation policies. However, LULUCF also acts via changing albedo, roughness and other surface properties and thus impacts the surface energy balance and water fluxes (the biogeophysical (BGP) effects). Through the BGP effects, LULUCF has a direct impact on local climate and may counteract global warming through local cooling and mitigate extreme weather events like heatwaves and droughts. LULUCF thus also plays a role in helping communities adapt to its effects.

However, decision-makers often focus only on direct emissions and carbon storage from LULUCF. These are called local biogeochemical (BGC) effects. To make sound climate policies, it is important to consider other processes of LULUCF as well: (i) Local BGP effects, which are BGP effects acting at the site the LULUCF happens; (ii) nonlocal BGP effects, which are remote climate changes caused by advection and large-scale changes in atmospheric circulation; (iii) nonlocal BGC effects, which are remote changes in carbon storage driven by the climate changes from nonlocal BGP effects.

The complexity of these LULUCF effects, with their different spatial scales and mechanisms, often prevents stakeholders from fully incorporating them into decision-making. In this study, we create a system that helps tailor the assessment of LULUCF effects to the specific concerns of different stakeholders. This system makes it possible to distinguish the combinations of LULUCF effects that should be considered in decision-making of different purposes: For example, the interest of a farmer will focus more on the local changes in climate (predominantly influenced by BGP effects) and additionally, if farmers get credits for emission reductions or CO2 removals, on local BGC effects. International negotiations under the UNFCCC, by contrast, focus predominantly on the combined local and nonlocal BGC effects.

In our study, we carefully identify different combinations of LULUCF effects exemplarily for 5 key stakeholders’ perspectives. We analyze model results from three advanced Earth system models to give an idea of how important the negligence or incorporation of one or the other LULUCF effect is. We do so for stylized large-scale scenarios of three common forms of LULUCF: global cropland expansion, global cropland expansion with irrigation, and global afforestation. We show that the answer to whether or not a LULUCF change brings desirable effects to climate and may help mitigation and/or adaptation is very much dependent on the perspective, with our system providing a tool to translate between the different perspectives.

This study gives a detailed look at how LULUCF affects both climate and the carbon cycle, providing a foundation for incorporating these impacts into policy at different levels. It helps guide climate action that balances land use with the Sustainable Development Goals, especially considering the growing interest in nature-based solutions for future climate strategies.

How to cite: Pongratz, J., Guo, S., Havermann, F., Windisch, M., De Hertog, S., Amali, A., Luo, F., Manola, I., Lejeune, Q., and Schleussner, C.-F.: Tailoring Land Use, Land-Use Change, and Forestry (LULUCF) Impacts for Stakeholder-Centric Climate Policy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12862, https://doi.org/10.5194/egusphere-egu25-12862, 2025.

EGU25-13001 | ECS | Orals | CL4.4

The delayed onset of South American monsoon under global warming in convection-permitting regional climate simulations. 

Jerry B Samuel, Marcia T Zilli, Neil C G Hart, and Fran Morris

Under a warmer scenario, several monsoon regimes are projected to have a delayed onset
of the rainy season. We employ state-of-the-art convection permitting regional climate
model (CPRCM) simulations performed at the UK Met Office to explore potential drivers of
this projected delay over South America. The simulations correspond to a present-day
climate (CPRM-PD) and an RCP8.5 scenario (CPRCM-2100). CPRCM-PD is downscaled
from an atmospheric general circulation model (AGCM) simulation forced with sea surface
temperatures (SSTs) for the period 1998-2007. CPRCM-2100 is driven by an AGCM
simulation forced with SSTs and greenhouse gas concentrations corresponding to an
RCP8.5 scenario. In CPRCM-2100, the onset of the rainy season is delayed, with several
regions exhibiting a delay of up to one month. The rainfall during September and October
shows approximately 50% decline over Central East Brazil, accompanied by coherent
changes in atmospheric thermodynamics. A larger relative increase in near-surface moist
static energy (MSE) is required of atmospheric destabilization in the RCP8.5 scenario, which
however, crosses the necessary threshold for significant rainfall to begin only in late
October/early November. The increase in MSE is primarily due to low-level moisture
enhancement during the onset phase which is also found to be delayed in the RCP8.5
scenario. Precipitation-moisture relationship over the region during the onset phase
indicates a 20% increase (relative to present-day) in near-surface specific humidity
requirement for a daily rainfall rate of 5 mm/day in the RCP8.5 scenario. However, there is a
substantial reduction in evapotranspiration during September and October, in addition to
the absence of any significant changes in moisture flux convergence. This hampers the
moisture build-up and delays the transition to the rainy season in these months. The decline
in evapotranspiration is despite larger soil moisture content in the soil column which
suggests reduced plant transpiration. An increase in stomatal closure in the future
environmental conditions leads to this decline in the RCP8.5 simulation. These changes are
also accompanied by changes in both surface and top of the atmosphere energy fluxes. The
results call for the urgency to develop land use policies to mitigate climate change effects,
given the increasing intensity of droughts in Brazil during recent times. The findings also
highlight the role of local processes in modulating climate projections and the necessity to
improve their representation in climate models.

How to cite: Samuel, J. B., Zilli, M. T., Hart, N. C. G., and Morris, F.: The delayed onset of South American monsoon under global warming in convection-permitting regional climate simulations., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13001, https://doi.org/10.5194/egusphere-egu25-13001, 2025.

EGU25-13687 | Orals | CL4.4

What is the compound effect of re/af-forestation and extreme heat on summer land-atmosphere coupling across Europe?    

Rita M. Cardoso, Luana C. Santos, Elena García Bustamante, Daniela C.A. Lima Lima, Pedro MM Soares, Carlos da Camara Camara, Diana Rechid, and Ana Russo and the Lucas Team

Through soil moisture and vegetation exchanges, land-atmosphere coupling contributes significantly to the evolution of extreme events. Land use/land cover changes (LUC) modify local land surface properties that control the land-atmosphere mass, energy, and momentum exchanges. The Flagship Pilot Study LUCAS (Land Use & Climate Across Scales) provides a coordinated effort to study LUC using an ensemble of 11 regional climate models (RCMs). In the first phase of the project, three reanalyses-driven experiments were performed for continental Europe: eval (with each RCM using its standard land use / land cover distribution), forest (maximised forest cover), and grass (trees replaced by grassland. An analysis of the impact on the coupling between temperature and evapotranspiration is performed using the usual correlation metric, while a new coupling metric based on the product of normalised variables was developed to analyse the coupling between extreme heat (TX90p) or heat wave (TX90p for at least five consecutive days) and evapotranspiration (LH) or soil moisture (TX90p*LH or TX90p*SMOIS). Whenever its values are lower than -1, then LH (SMOIS) is concurrently in deficit, and soil is uncoupled from the atmosphere. Conversely, when its values are greater than 1, then land-atmosphere coupling occurs.

For all RCMs, a positive correlation between near-surface maximum temperature and latent heat prevails over northern Europe, while the negative correlation dominates over southern and southeastern Europe. Forestation (forest-grass) will lead to higher correlations between latent heat and near-surface maximum temperature due to the different transition zone belt locations and weaker correlations in the grass experiment.

Extreme heat and evapotranspiration are positively coupled in forests across the whole continent except in the Mediterranean.  In the grass experiment, the Mediterranean areas are negatively coupled in most models, whilst northern Europe is positively coupled. This coupling (positive/negative) is amplified under heat wave events. Overall, forestation induces increased coupling in central Europe.  In the forest experiment, extreme temperature and soil moisture are negatively coupled across Europe, indicating that the increase in evapotranspiration is associated with the ability of the trees to source water from deeper soil layers.  In the grass experiment, the ensemble mean shows very weak un/coupling in central/ southern Europe, indicating the inability of grasses to source water in deeper soil layers and a broadening of the transition zone.

 

Acknowledgements

The authors wish to acknowledge the financial support  from the Portuguese Fundação para a Ciência e Tecnologia, (FCT, I.P./MCTES) through national funds (PIDDAC): UID/50019/2025 and LA/P/0068/2020 (https://doi.org/10.54499/LA/P/0068/2020), DHEFEUS (https://doi.org/10.54499/2022.09185.PTDC), and through project references https://doi.org/10.54499/UIDB/00239/2020, https://doi.org/10.54499/UIDP/00239/2020 ,  LS, RMC, AR, and DCAL are supported by FCT, financed by national funds from the MCTES through grant UI/BD/154675/2023, and https://doi.org/10.54499/2021.01280.CEECIND/CP1650/CT0006, https://doi.org/10.54499/2022.01167.CEECIND/CP1722/CT0006, and https://doi.org/10.54499/2022.03183.CEECIND/CP1715/CT0004, respectively

How to cite: Cardoso, R. M., Santos, L. C., García Bustamante, E., Lima, D. C. A. L., Soares, P. M., Camara, C. D. C., Rechid, D., and Russo, A. and the Lucas Team: What is the compound effect of re/af-forestation and extreme heat on summer land-atmosphere coupling across Europe?   , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13687, https://doi.org/10.5194/egusphere-egu25-13687, 2025.

EGU25-13907 | ECS | Posters on site | CL4.4

How do land-use changes shape the occurrence of extreme temperatures across Europe?    

Luana Santos, Rita Cardoso, Elena García Bustamante, Daniela C.A. Lima, Pedro MM Soares, Carlos da Camara, Diana Rechid, and Ana Russo and the Lucas Team

In recent years, an increase in the frequency of occurrence of heatwaves and in the number of hot days in Europe is undeniable. Hence, there is an increased need to understand the feedback mechanisms relevant to their development. Due to their localised impact and although they modify local land surface properties that control the land-atmosphere mass, energy, and momentum exchanges, the influence of land use/land cover changes (LUC) at regional scales still needs to be better represented in coordinated downscaling experiments. The Flagship Pilot Study LUCAS (Land Use & Climate Across Scales) provides a coordinated effort to study LUC using an ensemble of 11 regional climate models (RCMs). In the first phase of the project, three experiments were performed for continental Europe: eval (current climate), grass (trees replaced by grassland), and forest (grasses and shrubs replaced by trees). Heat events can be defined using percentiles, and heat waves are periods of consecutive hot days where temperatures exceed a certain percentile. Here, we use P85, P90 and P95 for maximum temperature thresholds and consider durations of 5, 7, and 10 days.  To facilitate the comparison of the intensity of these extreme events and their evolution over time, we normalise the daily maximum temperature, latent heat and soil moisture using a seasonal interquartile range. An analysis of frequency, magnitude, duration and extension is performed for the three percentiles and for the different land covers.

The results suggest that model responses to afforestation and deforestation exhibit some variability, particularly during summer months. While a substantial proportion of the models indicate a potential enhancement in the intensity and magnitude of heat extremes under forest scenarios, others demonstrate more muted or contrasting effects. The objective of the present analysis is to understand these discrepancies among models and their implications for land-atmosphere interactions under various land use scenarios. The findings will be discussed in terms of their relevance to climate extremes, providing insights into the role of LUC in modulating heat events across Europe.

How to cite: Santos, L., Cardoso, R., García Bustamante, E., Lima, D. C. A., Soares, P. M., Camara, C. D., Rechid, D., and Russo, A. and the Lucas Team: How do land-use changes shape the occurrence of extreme temperatures across Europe?   , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13907, https://doi.org/10.5194/egusphere-egu25-13907, 2025.

EGU25-14418 | Posters on site | CL4.4

Estimating the impact of irrigation and groundwater pumping on regional hydroclimate using an Earth System Model 

Yusuke Satoh, Yadu Pokhrel, Hyungjun Kim, Tomohiro Hajima, and Tokuta Yokohata

Irrigation is a significant anthropogenic forcing to the Earth system, altering water and heat budgets at the land surface and inducing changes in regional hydro-climate conditions across various spatiotemporal scales. These impacts of irrigation are expected to intensify in the future due to growing food demand and the pervasive effects of climate change. Therefore, it is imperative to better understand its nature, extent, and mechanisms through which irrigation affects the Earth system. However, despite its increasing importance, irrigation remains an emerging component in Earth system modeling community, necessitating further advancements in modeling approaches and a deeper understanding.

Our research aims to improve the quantitative understanding of how irrigation and groundwater use, as anthropogenic drivers, affect regional climate and environmental changes. To achieve this, we developed an enhanced Earth system modeling framework based on MIROC-ES2L (Hajima et al., 2020, GMD), integrated with hydrological human-activity modules (Yokohata et al., 2020, GMD). This framework enables simulations of coupled natural-human interactions, including hydrological dynamics associated with irrigation processes. Using this Earth system model, we carried out numerical experiments at T85 spatial resolution with an AMIP-style setup. Our large ensemble simulations allow statistical quantification of irrigation impacts, statistically distinguishing them from uncertainties arising due to natural variability.

Our investigation identified specific regions and seasons where irrigation exerts notable influences on regional hydro-climate. In particular, our results reveal substantial disparities—comparable to or exceeding inter-annual variability—between simulations with and without irrigation processes, especially in heavily irrigated regions such as Pakistan and India. Our model demonstrates that artificially wet soils due to irrigation alter the land surface hydrological balance, which consequently impacts the overlying atmosphere. However, significant uncertainties remain in the impact estimates for several variables in some regions, even those heavily irrigated, including the central United States and eastern China. This highlights the necessity of employing appropriate statistical approaches to evaluate irrigation impacts, accounting for inherent natural variability.

Additionally, our study estimates regional variations in the contributions of groundwater and surface water use to irrigation impacts. Our estimate indicates that approximately two-fifths of global irrigation water depend on groundwater resource, while this groundwater dependency ratio may still be underestimated. By emphasizing the importance of understanding regional and seasonal characteristics, our study underscores the importance of comprehending the complex interactions between irrigation-related human activities and the Earth's climate system. Nevertheless, we may still underestimate the full impacts of irrigation because irrigation water demand estimated by our coupled simulations is lower than that derived from preceding offline simulations or reported statistics. In this presentation, we will discuss this challenge as well.

How to cite: Satoh, Y., Pokhrel, Y., Kim, H., Hajima, T., and Yokohata, T.: Estimating the impact of irrigation and groundwater pumping on regional hydroclimate using an Earth System Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14418, https://doi.org/10.5194/egusphere-egu25-14418, 2025.

Human activities have a significant impact on the climate by altering vegetation types and modifying surface properties, resulting in more frequent and intense extreme weather events, which pose a threat to the sustainable development of the environment. However, the specific effects of vegetation change on extreme temperature events are not fully understood. To address this gap, we conducted evaluations with both in-situ observations and the regional climate model to determine the contributions of different vegetation transitions to extreme temperature changes over China. Our findings indicate that vegetation plays an important role in local heatwaves. Cropland have a stronger heating effect than grassland and forests in lifting the daily maximum temperature but present shorter hot day durations. Uncertainties are high in grassland than those of forest due to more diverse background climatic conditions of grassland sites. Numerical simulations revealed a decrease in extreme temperatures such as a 0.85℃ decrease in the daily maximum temperature and 2.65 fewer hot days, which can be attributed to changes of cloud radiation and sensible heat flux resulting from large-scale deforestation in the southern region and cropland expansion in central China. Converting forests to woody savannas led to a significant reduction in leaf area index and latent heat flux in the southern and northeastern regions. Changes in surface property have a stronger relationship with the average temperature changes than with extreme temperature changes. Overall, our study quantitatively evaluates the impact of different vegetation types and their property changes on regional extreme temperature changes, which have important implications for ecological protection and policy-making in China.

How to cite: Dong, N. and Liu, Z.: Comparing responses of summer extreme temperature to vegetation changes in China between satellite observations and numerical simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14702, https://doi.org/10.5194/egusphere-egu25-14702, 2025.

EGU25-15325 | ECS | Posters on site | CL4.4

Role of Pre-Monsoon Showers in the Evolution of Indian Heatwaves 

Manali Saha, Vishal Dixit, and Karthikeyan Lanka

Heatwaves constitute one of the most lethal weather phenomena, presenting substantial risks to millions of individuals. Characterized by extended periods of extreme temperatures, these events significantly impact ecosystems, economies, and human mortality rates. When coupled with high humidity, these events pose high heat stress over the heatwave domain. India, being one of the significant hotspots, experiences heatwaves during the pre-monsoon season. These heatwaves are associated with both moist and dry mechanisms. Moist heatwaves have high wet bulb temperatures and cause high fatalities among humans and mammals. With high population loading and the context of climate change, the origin or source of these moist heat waves has not been examined thoroughly till now. 

In the study, we investigate the precursors of the moist and dry heat waves in the Indo-Gangetic Plains using the Eulerian temperature decomposition equation to find out the dominant processes responsible for the formation of these events. The past literature says that advection is the major component in triggering these events, but our analysis proves that the effect of advection is minimal and supports the weak temperature gradient (WTG) theory in the tropics. To study the precursors, we extend our analysis from the pre-heatwave time to the onset of the heatwaves. Our analysis shows that pre-monsoon showers are responsible for forming moist heat waves. These showers are associated with nighttime low-level clouds that trap the outgoing long-wave radiation, further accumulating the heat content and causing the temperatures to rise. Further, these rainfall activities must be supported by the mid-tropospheric dryness (MTD) for it to be sustained throughout the period. The MTD helps the low-level clouds resulting from shallow convection remain as they are and does not promote deep convection. We emphasize the importance of local atmospheric conditions along with large-scale activities (that trigger anticyclones in the upper troposphere) in sustaining the heatwave intensity. The findings of this study will help in developing heatwave early warning systems at localized scales.

Keywords: Moist heatwaves, Pre-Monsoon showers, Mid Tropospheric Dryness, Weak Temperature Gradient, Advection

How to cite: Saha, M., Dixit, V., and Lanka, K.: Role of Pre-Monsoon Showers in the Evolution of Indian Heatwaves, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15325, https://doi.org/10.5194/egusphere-egu25-15325, 2025.

EGU25-15489 | ECS | Orals | CL4.4

Revisiting the link between soil moisture deficits and heatwaves 

Dominik L. Schumacher, Emanuele Bevacqua, Mathias Hauser, and Sonia I. Seneviratne

Severe heatwaves tend to strike during drought conditions, primarily considered a consequence of persistent, often quasi-stationary anticyclonic circulation. A key mechanism for heatwave intensification is the positive feedback between rapidly desiccating soils through elevated atmospheric evaporative demand and the associated enhanced surface sensible heating. The effect of such enhanced sensible heating is often quantified by comparing the evolution of heatwaves in climate model simulations with freely evolving soil water to additional simulations in which soil moisture is kept at climatological levels, and can reach up to several degrees Celsius. With this approach, one can gauge the effect of deviations from present-day average soil moisture, but this becomes increasingly hypothetical as we shift away from climatological norms and toward a future marked by widespread projected increases in agro-ecological drought during summer months. In such a climate change context, a general key question to address is: How does heatwave intensity depend on the initial state of soil moisture? To investigate this, we re-simulate historical heatwaves using CESM2, a state-of-the-art global Earth System Model, and examine how these events would have unfolded under different land surface conditions. We also explore the long-noted — yet never fully quantified — effect of soil drought on anticyclonic circulation itself.

How to cite: Schumacher, D. L., Bevacqua, E., Hauser, M., and Seneviratne, S. I.: Revisiting the link between soil moisture deficits and heatwaves, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15489, https://doi.org/10.5194/egusphere-egu25-15489, 2025.

EGU25-16332 | Orals | CL4.4

How much does afforestation’s impact on local land surface temperature vary in space, in time, and during dry and hot extreme events?  

Gregory Duveiller, Daniel E. Pabon-Moreno, Luca Caporaso, Daniel Loos, Di Xie, Melanie Weynants, Alexander J. Winkler, and Alessandro Cescatti

Changing the properties of the land surface may be one of the most direct ways to modulate local (and possibly non-local) land-atmosphere interactions, which in turn is of great interest for designing proper land-based climate mitigation and adaptation strategies. When we change the type of vegetation across a landscape, the biophysical properties of that land surface will change, potentially altering both radiative and non-radiative fluxes. Land surface temperature (LST), as measured from remote sensing satellites, provides a useful diagnostic, integrating the effects of these changes in fluxes. When combined with space-for-time substitution approaches, it is possible to derive data-driven estimations of what a given land cover transition could lead to in terms of LST before the actual land cover change occurs. However, the interannual variability of such biophysical effects of land use and land cover change is still understudied, which is an important prerequisite to understand the role these effects may have in alleviating or aggravating the occurrence and impacts of extreme events. 

In this study we present a global analysis of potential afforestation on local afternoon clear-sky LST across the MODIS Aqua record (from 2002 until 2024). This allows us to explore the interannual variability of local increases in forest cover on local LST, which in turns helps us estimate the sensitivity of the effects of afforestation in a changing climate. By combining these results with a dedicated dataset identifying hot and dry extremes from ERA5, we further explore how the effect of afforestation on LST changes under extreme conditions, which the trees would be increasingly more susceptible to encounter once they reach maturity.

Additionally, we take the opportunity to present the processing pipeline that has been developed within the Open-Earth-Monitor cyberinfrastructure (OEMC) project to make such analysis possible and reproducible. This includes improvements to better handle local topographic effects and testing the capacity to run the entire pipeline within a Discrete Global Grid System (DGGS) framework that preserves area and neighbourhood properties within the space-for-time moving window. We expect that these tools will facilitate data integration and model evaluation, thereby assisting research in land-atmosphere interactions and climate extremes.

How to cite: Duveiller, G., Pabon-Moreno, D. E., Caporaso, L., Loos, D., Xie, D., Weynants, M., Winkler, A. J., and Cescatti, A.: How much does afforestation’s impact on local land surface temperature vary in space, in time, and during dry and hot extreme events? , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16332, https://doi.org/10.5194/egusphere-egu25-16332, 2025.

EGU25-16372 | Orals | CL4.4

On the definition of extreme evaporation events 

Yannis Markonis

Even though evaporation is a crucial component of the energy and water cycles, its extremes remain largely unexplored. To address this gap, this study introduces a statistical framework defining Extreme Evaporation Events (ExEvEs) as individual events with onset and termination. Despite their statistical definition, ExEvEs are shown to have a physical basis, as they relate to radiation and/or precipitation—the main energy and water sources for land evaporation. By applying this methodological approach over Czechia, we can see that ExEvEs tend to form clusters of heightened evaporation lasting several days which fluctuate differently than the average evaporation resulting to significant implications for water availability and regional water cycle's acceleration. The proposed event-based framework provides a systematic way to detect, characterize, and analyse evaporation extremes, which helps to improve our understanding of their drivers and impacts.

How to cite: Markonis, Y.: On the definition of extreme evaporation events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16372, https://doi.org/10.5194/egusphere-egu25-16372, 2025.

EGU25-16413 | Posters on site | CL4.4

A Holistic Multi-Index Approach to Quantify Land Feedback Strength Across Evapotranspiration Regimes 

Sandipan Paul and Karthikeyan Lanka

Soil moisture (SM) is a critical Earth system variable that regulates the cyclicity of water, energy, and carbon, through which SM determines the evolution and thermodynamic state of the atmosphere. Land and atmospheric is tightly coupled in the water-limited regime (WLR), while the coupling strength diminishes in the energy-limited regime (ELR). Specifically, in response to progressive SM drying in the WLR, SM fractionates the net insolation into a greater proportion of sensible heat flux (SHF) and a smaller amount of latent heat flux (LHF), owing to the depletion of moisture. This phenomenon results in reduced land surface cooling, increased air temperature, expansion of the boundary layer, and subsequently enhances the land-atmosphere feedback. Further continuation of SM depletion leads to dry hydroclimatic extremes such as droughts and heatwaves. Consequently, understanding regime-specific coupled water-energy dynamics is fundamental to comprehending such extremes.

We propose a new metric called Land Feedback Strength (LFS) that combines three indices: sensitivity index (SI), variability index (VI) and regime persistence index (RPI). This formulation over the past attempts facilitates to effectively characterise the important components of LFS, which holistically quantify the terrestrial leg of land-atmospheric coupling. SI quantifies the responsiveness of SM to surface energy partitioning and is defined as the slope between SM and EF (LHF/LHF+SHF) in the WLR. Specifically, we observe higher SM sensitivity in semi-arid and sub-humid regions than in wet regions, indicating that the landscape rapidly responds to SM losses and begins influencing the atmosphere instantaneously. In addition, VI quantifies the sufficiency of SM to act as a dominant forcing and is calculated as the ratio of the standard deviation of SM in the WLR to WLR and ELR. While strong coupling is expected where higher sensitivity and sufficient SM variation are present, the coupling strength is exacerbated with the increasing persistence of the WLR. Thus, the RPI is formulated to indicate the likelihood of a landscape remaining in the WLR within a certain period. Furthermore, to quantify the LFS, we initially delineate global regimes using the coverability of SM and EF data pairs during drydowns.

This study’s findings indicate the following: (1) the highest sensitivity is observed during the dry seasons, whereas sensitivity is lowest during the summer; (2) SM variability is predominantly confined to WLR during winter and spring, with approximately equal variability in both regimes noted during autumn, and variability predominantly occurring in ELR during summer; (3) ELR is prevalent during summer in response to precipitation pulses, WLR and ELR demonstrate comparable likelihood in autumn, and WLR becomes predominant during winter and spring; (4) consequently, LFS is at its lowest during summer, increases in autumn, and further intensifies in winter; (5) LFS has facilitated the identification of two groups of strong coupling hotspots – with relatively higher intensity over the western USA and Austrian shrubland, African and Brazilian savannah, and lower intensity over Sahelian grassland, and peninsular India (6) LFS is found to be higher in semi-arid and sub-humid regions or savanna and grassland areas than forested or humid regions.

How to cite: Paul, S. and Lanka, K.: A Holistic Multi-Index Approach to Quantify Land Feedback Strength Across Evapotranspiration Regimes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16413, https://doi.org/10.5194/egusphere-egu25-16413, 2025.

EGU25-16565 | ECS | Orals | CL4.4

Expanding Amazon dry-hot season under anthropogenic climate change 

Mengxin Pan, Shineng Hu, Mark M. Janko, Benjamin F. Zaitchik, and William K. Pan

The Amazon rainforest, a crucial global carbon sink, plays a vital role in the global climate system. As ongoing climate change and local deforestation push the Amazon toward a critical tipping point, understanding the region's changing climate patterns becomes increasingly important. In this study, we reveal a significant expansion of the dry-hot season across the Amazon rainforest from 1980-2022, creating prolonged adverse climate conditions for the ecosystem and local communities. A machine learning clustering algorithm is used to define the dry-hot season automatically by considering the temperature, precipitation, and soil moisture simultaneously.

The land-atmosphere interaction predominates the dry-hot season expansion in the Amazon. During the dry season (Aug-Oct), the daily maximum temperature has warmed by ~1 degree per decade, much faster than that in the wet seasons (~0.4 degree per decade). By the surface heat budget analysis, we found that intensive dry-season warming is predominantly driven by reduced evapotranspiration, leading to decreased surface latent heat flux and increased shortwave radiation due to diminished cloud cover. The declining evapotranspiration rates stem from a combination of increasing soil moisture deficits and local deforestation.

By large-ensemble climate model simulations, we further demonstrate that this dry-hot season expansion is highly unlikely to occur without anthropogenic climate change and this expansion will exacerbate under future warming scenarios. By single-forcing experiment, we further confirm the critical role of local deforestation in amplifying this expansion. These findings emphasize the urgent need for targeted mitigation and adaptation strategies to protect this vital ecosystem from the compounding effects of climate change and deforestation.

How to cite: Pan, M., Hu, S., Janko, M. M., Zaitchik, B. F., and Pan, W. K.: Expanding Amazon dry-hot season under anthropogenic climate change, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16565, https://doi.org/10.5194/egusphere-egu25-16565, 2025.

EGU25-16957 | Orals | CL4.4

Heat capacity, cooling efficiency and drought stress of vegetated surfaces 

Matteo Zampieri, Matteo Piccardo, Guido Ceccherini, Marco Girardello, Ibrahim Hoteit, and Alessandro Cescatti

Drought stress has profound impacts on ecosystems and societies, particularly in the context of climate change. Traditional drought indicators, which rely on integrated surface water budget anomalies at various time scales and thresholds derived from past climate variability, provide valuable insights but often fail to deliver clear and direct real-time assessments of drought stress on vegetation.

This study introduces the Cooling Efficiency Factor (CEF), a novel metric derived from geostationary satellite observations, to detect drought stress by analyzing daytime surface warming anomalies. The CEF is based on the principle that dry surfaces warm more rapidly than wet ones under identical radiative forcing due to reduced evapotranspiration caused by soil moisture limitation and by stomatal closure, altering the effective heat capacity of the land surface.

By leveraging high-frequency, high-resolution retrievals of land surface temperature (LST) and radiation data from geostationary satellites, this study demonstrates the CEF's ability to assess drought stress conditions. The CEF correlates strongly with evapotranspiration anomalies from established datasets, including GLEAM, ERA5-Land, and TerraClimate. Results underscore the CEF's sensitivity to vegetation type, soil moisture variability, and environmental conditions, illustrating its effectiveness in identifying drought stress compared to traditional indicators.

The CEF represents a promising tool for real-time drought monitoring and integration into early warning systems, particularly for arid and semi-arid regions. By complementing existing drought assessment methods, the CEF paves the way for advancements in land-surface process studies and improved drought risk management.

How to cite: Zampieri, M., Piccardo, M., Ceccherini, G., Girardello, M., Hoteit, I., and Cescatti, A.: Heat capacity, cooling efficiency and drought stress of vegetated surfaces, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16957, https://doi.org/10.5194/egusphere-egu25-16957, 2025.

EGU25-17114 | ECS | Orals | CL4.4

Increases in extreme ET leading to a higher risk of flash droughts 

Marius Egli, Vincent Humphrey, Sebastian Sippel, and Reto Knutti

Evapotranspiration (ET) is a crucial process liking the surface energy balance, the hydrological and the carbon cycles. However, ET often remains underexplored due to climate model limitations as well as sparse and poor observational coverage.

While mean ET projections of CMIP6 models are highly uncertain, we explore whether climate models are in clearer agreement in terms of extreme ET, similar to what has been shown for mean versus extreme precipitation. We first define extreme ET (ETxx) as the annual 7-day ET maximum and investigate the physical drivers behind such events in a mid-latitude region (Central Europe). Typically, extreme ET events are characterized by high temperatures and incoming surface radiation, characteristic of a heat wave.  

We find an increase in extreme ET during the recent historical period and throughout scenario SSP5-8.5 in most CMIP6 models, together with a shift of these extremes from summer towards spring. We also find a higher degree of climate model agreement in the ET extremes, partially due to constraints in the boundary conditions of such an event, meaning that the drivers behind an extreme ET event are better constrained than the drivers of annual mean ET. This is a somewhat expected result due to the increase in vapor pressure deficit with higher temperature. The agreement also extends to all considered observational products, which agree on an increase in extreme ET, however the magnitude of this increase remains uncertain across observations-based products. We find that the observed trends lie outside the likely range of trends found in unforced climate simulations, indicating that the recent shift in observed extreme ET is attributable to climate change. We further find that records in extreme ET have been disproportionally set in more recent years, compared to what would be expected in a stationary climate in both observations and CMIP6 models.

Overall, mean ET projections and trends are complex and notoriously uncertain. Here we show that extreme ET events are better constrained than mean ET projections, making them a natural target for more robust inference from observations, attribution studies and emergent constraints. Our findings indicate an elevated risk for flash drought due to higher evaporative demand. The fact that future changes in peak water demand are less uncertain than changes in the mean demand is a highly relevant information for decision-makers and for the design of future water supply infrastructure (such as irrigation systems).

How to cite: Egli, M., Humphrey, V., Sippel, S., and Knutti, R.: Increases in extreme ET leading to a higher risk of flash droughts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17114, https://doi.org/10.5194/egusphere-egu25-17114, 2025.

EGU25-18334 | ECS | Posters on site | CL4.4

Assessing soil moisture-induced changes in land carbon sink projections of CMIP6 models 

Lea Gabele, Petra Sieber, Mathias Hauser, Martin Hirschi, and Sonia Seneviratne

The terrestrial biosphere absorbs about one third of anthropogenic carbon dioxide emissions and thereby dampens human-induced climate change. However, its capacity to act as a carbon sink depends on climate conditions, including temperature and water availability. Uncertainties in both future climate conditions and the response of the terrestrial biosphere lead to greatly diverging projections of the land carbon sink among state-of-the-art Earth System Models (ESMs).

Previous research identified soil moisture (SM) as a critical factor that can restrict land carbon uptake through water limitation and the intensification and prolongation of heat extremes. Green et al. (2019) demonstrated the severe negative impact of reduced SM on long-term land carbon sink projections of the 5th Coupled Model Intercomparison Project (CMIP5) using dedicated experiments isolating the effects of SM.

Here, we use equivalent experiments performed with four ESMs participating in CMIP6 to investigate the impact and uncertainty of SM-induced changes in land carbon sink projections by the end of the century (2070-2099). Our results demonstrate a substantial reduction in the negative impact of SM on the global land carbon sink compared to the previous model generation. Models agree on a SM-induced reduction in land carbon uptake in summer, consistent with an overall SM decline across models, while intermodel uncertainty remains high in spring, particularly regarding the effects of SM variability at mid-to-high latitudes. Additionally, high uncertainty in SM-induced impact on annual carbon uptake persists in the tropics and northern mid-latitudes, driven by differences in the sensitivity of carbon uptake to SM but also disagreement in SM projections across models.

We extend our analysis to a larger ensemble of CMIP6 models that have not performed the SM experiments. To this end, we employ the methods of Schwingshackl et al. (2018), which utilize the distinct link between SM and the evaporative fraction in the different SM regimes. Using this relationship we emulate the impact of SM on the land carbon sink in regions where land carbon uptake is controlled by SM.

The study aims to gain insights into SM-induced impacts and related uncertainties in land carbon sink projections of CMIP6 models, highlighting the ongoing challenge of accurately projecting SM-induced changes in the land carbon sink.

 

References:


Green, J. K., Seneviratne, S. I., Berg, A. M., Findell, K. L., Hagemann, S., Lawrence, D. M., & Gentine, P. (2019). Large influence of soil moisture on long-term terrestrial carbon uptake. Nature, 565(7740), 476-479. https://doi.org/10.1038/s41586-018-0848-x 

Schwingshackl, C., Hirschi, M., & Seneviratne, S. I. (2018). A theoretical approach to assess soil moisture–climate coupling across CMIP5 and GLACE-CMIP5 experiments. Earth System Dynamics, 9(4), 1217-1234. https://doi.org/10.5194/esd-9-1217-2018

How to cite: Gabele, L., Sieber, P., Hauser, M., Hirschi, M., and Seneviratne, S.: Assessing soil moisture-induced changes in land carbon sink projections of CMIP6 models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18334, https://doi.org/10.5194/egusphere-egu25-18334, 2025.

EGU25-19778 * | ECS | Orals | CL4.4 | Highlight

Observed and projected increase of extreme precipitation events on dry soils 

Damián Insua Costa, Chiara M. Holgate, and Diego G. Miralles

Dry soils are associated with low infiltration capacity and increased runoff due to surface crust formation. Therefore, the occurrence of heavy rainfall on dry soils poses a higher risk of flooding. In recent years, abrupt changes from extremely dry to extremely wet conditions have attracted the attention of researchers, and terms such as precipitation whiplash or precipitation volatility have gained currency to refer to these phenomena. Most studies have focused on investigating these episodes on seasonal or annual scales, i.e. changes from very dry to very wet seasons or years. Here, we focus on analysing these events on a daily scale, i.e. the change from very dry to very wet conditions from one day to the next. For this purpose, dry conditions are detected using a threshold in soil moisture and not the rainfall deficit, which would be meaningless on a daily scale. We argue that this approach is more closely related to flash flood risk. Our results based on reanalysis data show that the global frequency of extreme precipitation events on dry soils has increased dramatically in recent decades, at a rate higher than predicted by historical climate model simulations. Furthermore, we show that this trend will continue to increase based on future projections. Specifically, we estimate that the global probability of such an event will more than double by the end of the present century compared to the pre-industrial era under a high-emissions scenario. Finally, we shed light on whether this trend is dominated by an increase in the probability of occurrence of extreme precipitation and dry soils independently, or rather is related to an increase in the probability of concurrence of both, which could be indicative of a negative soil moisture–precipitation feedback.

How to cite: Insua Costa, D., M. Holgate, C., and G. Miralles, D.: Observed and projected increase of extreme precipitation events on dry soils, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19778, https://doi.org/10.5194/egusphere-egu25-19778, 2025.

EGU25-1122 | ECS | Posters on site | BG1.1

Forest Fire Variability Over the Central India Region from 2001–2020 

Saurabh Sonwani, Pallavi Saxena, and Madhavi Jain

Large-scale, frequent forest fires have a detrimental effect on the environment, the quality of the air, and human health. In the present study, from 2001 to 2020, March (1,857.5 counts/month) and April (922.8 counts/month) saw around 70% of the region's annual forest fires. Unusually high numbers of forest fires have been reported in some years, including 2009, 2012, and 2017. A thorough investigation is conducted into the contribution of numerous climate extremes and persistently rising temperatures to the rise in forest fire activity over central India. Forest fire activity doubled and tripled during the non-fire (July–January) and forest fire (February–June) seasons, respectively, over the warmer period from 2006 to 2020. A severe heat wave, an unusual drought, and an exceptionally powerful El Nino occurred in central India between 2015 JASONDJ and 2018 FMAMJ. These events are thought to have contributed to an upsurge in forest fires. The quinquennial spatiotemporal changes in forest fire characteristics, including average fire intensity and fire count density, were also evaluated. Significantly high soil temperature, low soil moisture content, poor evapotranspiration, and low normalized difference vegetation index are statistically associated with high near-surface air temperature and low precipitation during FMAMJ. This makes the climate much drier, which encourages a lot of forest fires in the Central Indian region.

How to cite: Sonwani, S., Saxena, P., and Jain, M.: Forest Fire Variability Over the Central India Region from 2001–2020, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1122, https://doi.org/10.5194/egusphere-egu25-1122, 2025.

EGU25-1314 | ECS | Orals | BG1.1

Exploring the effect of straw burning on urban ozone levels based on multi-source satellites in northern China 

Wannan Wang, Ronald van der A, Jieying Ding, Tianhai Cheng, and Chunjiao Wang

China is a significant region for crop cultivation. For a long time, there has been a common practice of burning crop residues during the post-harvest period (from May to October). The smoke emitted from straw burning contains both types of ozone precursors, including nitrogen oxides (NOx=NO+NO2) and volatile organic compounds (VOCs), and can be transported over long distances. During the transport process, secondary formation or consumption of ozone precursors occurs within the smoke plumes. After the smoke plume mixes with the atmosphere in the downwind urban area, it will lead to changes in the local ozone formation sensitivity. However, due to the nonlinear relationship between ozone and its precursors, the changes in ozone levels in downwind cities are not as straightforward as expected.

Here, we explore the temporal evolution of urban ozone and its precursors on smoke-affected days using multi-source satellite-derived fire event tracking datasets, which are screened by a semi-quantitative absorbing aerosol index (AAI), tropospheric NO2 and HCHO columns measurements from OMI, fire points from Himawari-8, and ground-level O3 monitoring dataset. We aimed to understand the associations between urban ground-level O3 concentrations and crop residue burning events in China. Our analysis revealed that no consistent changes were shown in urban O3 on smoke-affected days. In addition, there was an increase in NO2, while HCHO and O3 decreased in cities after mixing with smoke that had taken a long transport time. Our findings suggest that the O3 formation sensitivity within aged smoke tends to be controlled by VOC-limited regime. We hypothesize that the large amount of NOx carried by aged smoke consumes urban VOCs and O3, while producing NO2 locally. When fresh smoke, which is mainly controlled by the NOx-limited regime, enters urban environments rich in NOx, it leads to an increase in O3 concentration. Our analysis may contribute to an improved understanding of the influence of straw burning on urban ozone levels in China.

How to cite: Wang, W., van der A, R., Ding, J., Cheng, T., and Wang, C.: Exploring the effect of straw burning on urban ozone levels based on multi-source satellites in northern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1314, https://doi.org/10.5194/egusphere-egu25-1314, 2025.

The global wildland fire management community faces pressing climate change and operational challenges and requires improved capabilities in existing modelling tools or the development of novel decision support tools to limit the negative impact of wildfires and to increase use of prescribed burning where appropriate. This presentation will discuss limitations in the existing approaches to incorporating fuel structure effects in different model types (empirical, semi-empirical, detailed physics-based). In particular, novel experimental data will be presented addressing previously identified limitations [1] in the description of surface fuel beds in one of the most widely-used semi-empirical models; the Rothermel model, which underpins many current operational models.

The Rothermel model [2] involves a conservation of energy approach, incorporating separate terms to describe energy release rate in the combustion zone (reaction intensity) and energy transferred to the unburnt fuel (propagating flux), and incorporates a number of empirical closure terms.  The reaction intensity is empirically based, with the underpinning experimental measurements described in Frandsen and Rothermel [3]. By measuring the mass loss rate in a section of a fuel bed, Frandsen and Rothermel were able to characterize the intensity distribution within the combustion zone. However, the interacting effects of simultaneously varying fuel loading and packing ratio were not systematically considered, complicating efforts to understand the interacting effects of fuel loading and bulk density.

This study presents a series of laboratory-based flame spread experiments (no wind) involving excelsior fuel beds of varying structural conditions (Fuel Height: 0.02 to 0.12 m, Bulk Density: 3.3 to 20 kg/m3, Fuel Loading: 0.2 to 0.4 kg). The reaction intensity was calculated via a similar procedure to that described by Frandsen & Rothermel [2] as ‘Method 2’, in which the longitudinal length of the mass measurement region is greater than or equal to the combustion zone depth.

Clear trends in the peak mass loss rate and profile with bulk density were observed with a significant reduction at lower fuel loadings (0.2 kg/m2), and the reaction time was observed to increase at higher bulk densities along with a lengthening in the reaction intensity distribution region (further behind the combustion wave front). These results, along with existing observations of the trailing, in-depth combustion region in porous fuel beds, can be used to further investigate the observed tendency for underprediction of spread rates when the Rothermel model is applied to compressed fuel bed scenarios and has practical implications for other fire behaviour modelling applications. For example, improved characterisation of the overall combustion wave may enable improved modelling of smoke generation, surface-to-crown fire transition, and fuel consumption (e.g. to evaluate prescribed fire effectiveness).

[1] Z. Campbell-Lochrie, M. Gallagher, N. Skowronski, R.M. Hadden, The effect of fuel bed structure on Rothermel model performance, Int. J. of Wildland Fire. 33 (2023).

[2] R.C. Rothermel, A Mathematical Model for Predicting Fire Spread in Wildland Fuels, Research Paper INT-115, USDA Forest Service.,1972.

[3] W.H. Frandsen, R.C. Rothermel, Measuring the energy-release rate of a spreading fire, Combust Flame 19 (1972) 17–24.

How to cite: Campbell-Lochrie, Z.: Revisting Intensity of Combustion Waves to Address Outstanding Issues in Wildfire Modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1390, https://doi.org/10.5194/egusphere-egu25-1390, 2025.

EGU25-1707 | ECS | Posters on site | BG1.1

Modeling Fire-Atmosphere Feedbacks: Insights from the 2019/2020 Australian Wildfires 

Lisa Muth, Bernhard Vogel, Heike Vogel, and Gholamali Hoshyaripour

Wildfire emissions are a significant environmental concern, especially as climate change is expected to increase the frequency and intensity of extreme wildfires. Numerical weather and chemical transport models often struggle to reliably capture the injection height of wildfire plumes, a key parameter for transport that determines the impact on air quality and climate.

This study uses the ICON-ART numerical model to analyze fire-atmosphere feedbacks and their impact on the aerosol plume. The Australian New Year’s wildfire event of 2019/2020, a period of extreme wildfires and pyro-convection, is chosen as the case study. The simulations are performed with a grid spacing of 6.6 km. At this resolution, convection cannot be resolved, so a plume rise model is employed to parameterize the injection height. However, the resolution is sufficiently fine to account for the impact of the fire on meteorological variables.

Our simulations reveal that fire-induced moisture release leads to increased cloud formation under near-saturation conditions, but the overall impact on plume development is small. In contrast, fire-induced heat release significantly increases the mass-weighted height from the start, driven by sensible heat release, increased injection height, and enhanced convective cloud formation.

Comparison with observations shows that accounting for the heat release by the fire enables the simulation of the observed plume heights. These implementations have the strongest effect on the first simulation day, when the fires are most intense, and are negligible on the last simulation day. For fires with lower intensity, the plume rise model performs well without additional implementations.

How to cite: Muth, L., Vogel, B., Vogel, H., and Hoshyaripour, G.: Modeling Fire-Atmosphere Feedbacks: Insights from the 2019/2020 Australian Wildfires, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1707, https://doi.org/10.5194/egusphere-egu25-1707, 2025.

EGU25-1776 | ECS | Orals | BG1.1

Spatiotemporal changes in global cropland fire activity from 2003 to 2020 

Jiaming Wang, Jiasheng Li, Jie Zhao, Xiaoting Zhong, Mengyu Wang, Junhao He, and Chao Yue

Agricultural straw burning is a significant source of greenhouse gas emissions, adversely affecting regional human health and air quality. Understanding the spatiotemporal patterns of agricultural fires is crucial for developing effective emissions reduction strategies in cropland to mitigate climate change. Although it is reported that cropland fires have been decreasing over the past two decades, the trends of global cropland fires on seasonal and diurnal scales remain poorly quantified, limiting a complete understanding of their spatiotemporal dynamics. This study analyzes global cropland fire activity from 2003 to 2020 at annual, seasonal, and diurnal scales, using multiple satellite-based burned area datasets, active fire products, and cropland classification datasets. The results show that from 2003 to 2020, global cropland burned area, active fire detections, and fire intensity all exhibited significant decreasing trends (p < 0.05), with relative changes of -43.5%, -30.3%, and -3.5%, respectively. The most significant decreases in cropland burned area and active fire detections occurred in Africa, while the largest decline in fire intensity was observed in Asia. Moreover, cropland fire activity displayed notable seasonal and diurnal variations. On the seasonal scale, the largest declines in cropland burned area, active fire detections, and fire intensity were observed in December, August, and November, respectively. Notably, fire intensity showed a significant increasing trend (p < 0.05) in April and September. On the diurnal scale, the decrease in cropland active fire detections was primarily driven by daytime activity; however, the rate of decline in fire intensity at night was about 1.5 times that during the day. These findings offer valuable insights into the comprehensive spatiotemporal patterns of global cropland fires, providing a foundation for more effective cropland management and carbon mitigation strategies.

How to cite: Wang, J., Li, J., Zhao, J., Zhong, X., Wang, M., He, J., and Yue, C.: Spatiotemporal changes in global cropland fire activity from 2003 to 2020, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1776, https://doi.org/10.5194/egusphere-egu25-1776, 2025.

EGU25-2016 | ECS | Posters on site | BG1.1

Wildfires and biomass burning in northern Thailand: Observations from ASIA-AQ Campaign 

Sayantee Roy, Francesca Gallo, Elizabeth B. Wiggins, Luke D. Ziemba, Carolyn Jordan, Edward L. Winstead, Michael A. Shook, Joshua P. DiGangi, Glenn S. Diskin, Yonghoon Choi, Jason A. Miech, Wojciech Wojnowski, Felix Piel, Stefan J. Swift, Armin Wisthaler, and Richard H. Moore

Southeast Asia experiences widespread wildfires and biomass burning events during the dry season (January to April), leading to poor air quality, haze, and smog. NASA conducted the Airborne and Satellite Investigation of Asian Air Quality (ASIA-AQ) flight campaign in February and March 2024 to study the contribution of smoke to urban air quality through a multi-faceted observational approach (aircraft, satellite, and ground). The campaign deployed the NASA DC-8 aircraft, equipped with instruments from the Langley Aerosol Research Group (LARGE) and other teams, to measure real-time aerosol microphysical and optical properties, trace gases, and meteorological parameters. During the campaign in the Philippines, South Korea, Thailand, and Taiwan, it was noted that the northern region of Thailand was predominantly impacted by agricultural residue burning and wildfires. Here, we present the variations of vertical and horizontal profiles of aerosol properties and biomass burning tracers, alongside meteorological data to assess the impacts of local conditions and potential pollution pathways. Key findings will include observed variability in aerosols properties, the role of absorbing and scattering aerosols, boundary layer dynamics, and regional pollution transport across the ASIA-AQ domain.

How to cite: Roy, S., Gallo, F., Wiggins, E. B., Ziemba, L. D., Jordan, C., Winstead, E. L., Shook, M. A., DiGangi, J. P., Diskin, G. S., Choi, Y., Miech, J. A., Wojnowski, W., Piel, F., Swift, S. J., Wisthaler, A., and Moore, R. H.: Wildfires and biomass burning in northern Thailand: Observations from ASIA-AQ Campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2016, https://doi.org/10.5194/egusphere-egu25-2016, 2025.

EGU25-2253 | ECS | Posters on site | BG1.1

Near-field atmospheric dispersion of a gas emitted from a hot source : a comparison between analytical modelling and in situ measurements 

Anthony Mendez, Gée Manon, Sylvain Dupont, and Philippe Laguionie

Incidents in nuclear facilities can lead to the emission of a radioactive plume dis-
persing into the atmosphere. In such events, the highest radionuclide concentration
is usually located near the source at distances ranging from a few meters to several
hundred meters. It is, therefore, crucial to be able to accurately predict these levels
of near-source concentrations.
One challenge arises from the thermal characteristics of the source, which regulate
the initial dispersion of the plume. In the case of a non-thermal gas release, the
dispersion of the plume is driven by atmospheric conditions, related to wind and
atmospheric instability, and is influenced by local surface characteristics such as
roughness and the presence of obstacles. In contrast, when the gas is emitted from
a hot source such as a fire, the released gas first rises in the atmosphere up to a
so-called ‘injection height’ due to buoyant forces. The injection height is reached at
a certain distance from the source and doesn’t only depends on the properties of the
hot source but also on the atmospheric conditions (e.g. downdraft effects). The gas
then disperses like in a non-thermal gas release.
While CFD modelling can offer an accurate description of the plume dispersion, its
processing speed is not suitable for use in emergency situations. In contrast, existing
analytical models can provide rapid results, but their injection height parametriza-
tions may lack comprehensive coverage. So far, analytical models have rarely been
validated against field measurements, and few field experiments have been conducted
to improve their parameterization.
The goal of this presentation is twofold, first to present a field experiment on the
atmospheric plume dispersal of a gas released from a hot source, and second to
evaluate an analytical model of plume dispersal against the experiment, with a
particular focus on the Atmospheric Transfer Coefficient of the released gas.
The field experiment was conducted in May 2024 on a flat terrain near Vire (Nor-
mandy, France), under unstable and neutral atmospheric conditions.

The source comprised a burner (PYROS) that generated a propane fire with an average heat
release rate of between 450 kW and 750 kW . Helium was injected into the plume
to serve as a tracer gas. During 15-minute observation periods, helium concentra-
tions in the air were measured at ground level at distances from the source ranging
from 40 m to 400 m, as well as at various altitudes, using air sampling points at-
tached to a rope lifted vertically by a drone. Additionally, atmospheric turbulence
characteristics were also measured using ultrasonic anemometers.
The analytical model employs Heskestad’s formulas to determine the fire character-
istics and Briggs’ dispersion parameters to characterise the Gaussian dispersion of
the plume when buoyant forces become negligible.

 

 

 

How to cite: Mendez, A., Manon, G., Dupont, S., and Laguionie, P.: Near-field atmospheric dispersion of a gas emitted from a hot source : a comparison between analytical modelling and in situ measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2253, https://doi.org/10.5194/egusphere-egu25-2253, 2025.

EGU25-2313 | ECS | Orals | BG1.1

Determining the human signal in burned area under a changing climate 

Bikem Ekberzade, Aydoğan Avcıoğlu, and Tolga Görüm

In this study, we report the preliminary findings from a series of sans-human wildfire simulations using a process based dynamic global to regional vegetation model (DGVM), LPJ-GUESS v 4.1, coupled with the SIMple FIRE Model (SIMFIRE) and the wildfire combustion model (BLAZE), where we investigate the performance of the DGVM to reenact a specific wildfire instance in a Mediterranean catchment. For this, we compared the simulated burned area (BAs) to that in the actual event (BAo) in Manavgat, Antalya, Türkiye. The DGVM spatially captured the fire instance, albeit with a much smaller BA as a result. In July 2021, the largest single wildfire incidence for this region for the last two centuries occurred. The wildfire scorched an area of 60.000 ha.s where the dominant vegetation types were fire adapted dry conifer forests (mainly Pinus brutia) and Mediterranean shrubs. Previous years’ precipitation patterns had encouraged fuel build up, and the extreme heat of the summer of 2021, coupled with the seasonal drought and strong winds provided suitable environmental conditions for the wildfire’s spread. The ignitions in this specific case were intentional, majority were targeted arsons, and a plausible reason behind the ultimate extent of the BA. Here, we show the simulation results from our sans-human model runs using ERA5-Land reanalysis dataset, and compare BAs to BAo for this catchment for 2021. Our ultimate aim in these series of experiments where the ignition source is non-human is initially to decipher the dynamics, and later to develop a methodology to assess the human influence in BA in Mediterranean type ecosystems in the Eastern Mediterranean Basin, under a changing climate. 

How to cite: Ekberzade, B., Avcıoğlu, A., and Görüm, T.: Determining the human signal in burned area under a changing climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2313, https://doi.org/10.5194/egusphere-egu25-2313, 2025.

EGU25-2467 | ECS | Orals | BG1.1

The contribution of fires to PM2.5 and population exposure in Pacific Asia 

Hua Lu, Min Xie, Nan Wang, and Bojun Liu

Forest and vegetation fires are one of the major sources of air pollution and have triggered air quality issues in many regions of Pacific Asia. Here we isolate the fire-specific PM2.5 from monitoring concentrations using an observation-driven approach in the region. The total PM2.5 in Pacific Asia exhibited a rapid declining trend from 2014 to 2021, while fire-specific PM2.5 decreased in early years but begun to reverse, leading to an increasing proportions of fire-specific PM2.5 in recent years. The inconsistency between the decreasing number of fire points and the rising levels of fire-specific PM2.5 may be attributed to a shift in dominant sources of fire emissions in Pacific Asia, moving from anthropogenic agriculture fires to wildfires. Fire-related PM2.5 poses a significant public health threat in Pacific Asia, contributing to approximately 334,300 premature deaths each year. Our assessment highlights the disproportionate impact of fire-specific PM2.5 on poverty populations, indicating a pressing need for more attentions and researches in these regions. Based on the positive correlation between vapor pressure deficit and fire-specific PM2.5, this study suggests that without further regulation and policy intervention, the contributions of fire-specific PM2.5 to air pollution in Pacific Asia are likely to continue increasing under the influence of future climate change.

How to cite: Lu, H., Xie, M., Wang, N., and Liu, B.: The contribution of fires to PM2.5 and population exposure in Pacific Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2467, https://doi.org/10.5194/egusphere-egu25-2467, 2025.

EGU25-3090 | ECS | Orals | BG1.1

Identifying Ignition Drivers of Lightning-Ignited Wildfires in Boreal Forests 

Brittany Engle, Ivan Bratoev, Morgan A. Crowley, Yanan Zhu, and Cornelius Senf

Forest fires are the primary disturbance agent in global boreal forests, and they play a significant role in shaping their composition and structure. Boreal forests are also considered a carbon sink but rising temperatures in high-latitude regions are likely increasing wildfire activity, raising concerns that they may become net carbon emitters. Climate change has also increased the frequency and intensity of fire weather in high-latitude boreal forests and is expected to increase the frequency of lightning, a major source of ignition, which could potentially lead to a substantial increase in burned areas. Lightning-ignited wildfires (LIW) pose unique challenges due to their ability to (i) smoulder for long periods of time undetected, (ii) form fire clusters, and (iii) resist suppression efforts. Understanding drivers of ignition is critical for ignition prediction and for optimizing resource allocation for fire managers. Understanding the dynamics of LIWs is, however, challenging due to lack of spatially explicit data that would allow for pan-Boreal analyses of ignition drivers.  

Current LIW research is thus heavily concentrated in regions with detailed fire data (like North America). In a past study, we filled this data gap by introducing the Temporal Minimum Distance (TMin) method, a new approach to match lightning strikes to wildfires without ignition location data (Engle et al. 2024). The TMin method outperformed current methodologies like the Daily Minimum Distance and the Maximum Index A by identifying 74.71% of fires in boreal forests. Using this method, a comprehensive dataset - BoLtFire - was developed, encompassing 6,228 fires larger than 200 ha spanning across the entire boreal forest from 2012 to 2022. When benchmarked to agency reference datasets, BoLtFire performed reasonably well, with an overall commission error of 30.06% and omission error of 53.63%, but global extent. 

To model lighting ignition efficiency, the BoLtFire dataset was enhanced to include location data for over 6,000 lightning strikes that did not result in a fire. This expanded dataset also now integrates “ignition drivers,” identified through modelling over 80 different lightning characteristic, climatic, topographic, and fuel-related variables to identify the most influential factors in the ignition process. This enriched dataset provides valuable insights into why certain lightning events trigger wildfires, while others do not. It thus enables more accurate ignition prediction and improved wildfire management strategies. This expanded dataset provides new opportunities to model ignition and spread dynamics for wildfires in boreal forests, deepening our understanding of lightning-driven fire activity. By addressing key knowledge gaps and advancing methodological approaches, this research contributes to a more comprehensive framework for mitigating the growing risks of wildfires in boreal regions and their potential impacts on one of the most important land carbon sinks. 

References: 
Engle, B., Bratoev, I., Crowley, M. A., Zhu, Y., and Senf, C.: Distribution and Characteristics of Lightning-Ignited Wildfires in Boreal Forests – the BoLtFire database, Earth Syst. Sci. Data Discuss. [preprint], https://doi.org/10.5194/essd-2024-465, in review, 2024. 

How to cite: Engle, B., Bratoev, I., Crowley, M. A., Zhu, Y., and Senf, C.: Identifying Ignition Drivers of Lightning-Ignited Wildfires in Boreal Forests, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3090, https://doi.org/10.5194/egusphere-egu25-3090, 2025.

EGU25-3113 | ECS | Posters on site | BG1.1

Biomass Burning Organic Aerosols as a Pool of Atmospheric Reactive Triplets to Drive Multiphase Sulfate Formation 

Zhancong Liang, Liyuan Zhou, Yuqing Chang, Yiming Qin, and Chak Keung Chan

Biomass-burning organic aerosol(s) (BBOA) are rich in brown carbon (BrC), which significantly absorbs solar irradiation and potentially accelerates global warming. Despite its importance, the multiphase photochemistry of BBOA after light absorption remains poorly understood due to challenges in determining the oxidant concentrations and the reaction kinetics within aerosol particles. In this study, we explored the photochemical reactivity of BBOA particles in multiphase S(IV) oxidation to sulfate. We found that sulfate formation in BBOA particles is predominantly driven by photosensitization involving the triplet excited states (3BBOA*) instead of iron, nitrate, and S(IV) photochemistry. Rates in BBOA particles are three orders of magnitude higher than those observed in the bulk solution, primarily due to the fast interfacial reactions. Our results highlight that the chemistry of 3BBOA* in particles can greatly contribute to the formation of sulfate, as an example of the secondary pollutants. Photosensitization of BBOA will likely become increasingly crucial due to the intensified global wildfires.

How to cite: Liang, Z., Zhou, L., Chang, Y., Qin, Y., and Chan, C. K.: Biomass Burning Organic Aerosols as a Pool of Atmospheric Reactive Triplets to Drive Multiphase Sulfate Formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3113, https://doi.org/10.5194/egusphere-egu25-3113, 2025.

EGU25-3285 | ECS | Orals | BG1.1

Linking fire synchronicity in Europe to persistent weather regimes 

Xinhang Li, Raul Wood, and Manuela Brunner

Synchronous fires, that is fires co-occurring at different geographical locations within a few days of each other, challenge the distribution of firefighting resources among regions and can have more severe impacts on human health, infrastructure and environmental systems than individual fire events. However, so far very little is known about the occurrence, spatial patterns and the atmospheric drivers of synchronous fires in Europe.

In this work, we use fire observations from a global fire event dataset FRYv2.0 to (1) detect fire synchronicity between ten European regions during 2001–2020 and (2) link the occurrence of synchronous fires to seven dominant European-Atlantic weather regimes. To detect fire synchronicity, we apply complex network theory and an event synchronicity statistical framework to identify significant links between the ten regions. To analyze the relationship between synchronous fire events and dominant weather regimes, we use a conditional probability-based measure calculating the dependency of synchronous fires –between each region pair– on seven common European weather regimes. We perform 2000 block permutations to test the statistical significance of these dependencies. Lastly, we use the CERRA reanalysis data to analyze the seasonal anomalies of relevant atmospheric variables under each weather regime, including temperature, wind speed, precipitation and relative humidity.

We find multiple significant connections between regions across Europe showing fire synchronicity in spring, summer and fall. We show that (1) northern and western regions in Europe experience fire synchronicity in spring under the influence of blocking regimes (i.e., European and Scandinavian Blocking) which promote warm and dry conditions; (2) eastern regions show fire synchronicity in spring and fall during the Zonal Regime under warm and dry conditions; and (3) fire synchronicity in southern regions are significantly modulated by Scandinavian Troughs due to positive wind speed anomalies and dry conditions in spring and fall as well as by Atlantic Ridges due to positive wind speed anomalies in summer.

Our work reveals significant fire synchronicity across Europe with significant links to atmospheric circulation patterns. As the seven weather regimes have predictability on weekly to monthly time scales, our work might help to develop early warning systems for elevated risks of synchronous fires under climate change and improve fire emergency preparedness across different European regions. 

How to cite: Li, X., Wood, R., and Brunner, M.: Linking fire synchronicity in Europe to persistent weather regimes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3285, https://doi.org/10.5194/egusphere-egu25-3285, 2025.

EGU25-3308 | ECS | Orals | BG1.1

Global Drivers of Post-Fire Ecosystem Recovery: Insights from Solar-Induced Chlorophyll Fluorescence 

Yicheng Shen, Colin Prentice, and Sandy Harrison

The recovery time of ecosystems following wildfire significantly influences carbon sequestration rates, land-atmosphere exchanges, and hydrological processes. Post-fire recovery has been studied at local scales but there is a lack of comprehensive global-scale analyses. We used solar-induced chlorophyll fluorescence (SIF) to quantify the recovery of photosynthetic activity after more than 10,000 fires from diverse ecosystems. We used the relaxed lasso technique to identify key determinants of the length of time required for post-fire recovery, and used these to build a linear regression model. Our results show that vegetation characteristics, fire properties, and post-fire climatic conditions all influence recovery time. Gross primary production (GPP) is the most important determinant of recovery time: ecosystems with higher GPP recover faster. Fires with greater intensity and duration, which cause more extensive vegetation damage, are associated with longer recovery times. Post-fire climate also affects recovery time: anomalously high temperatures and temperature seasonality, and increased number of dry days, cause slower recovery, while above-average precipitation accelerates recovery. Recovery times vary between different biomes, potentially reflecting variations in plant fire adaptations: ecosystems with a higher abundance of resprouting plants recover more rapidly. These findings provide a global perspective on how vegetation responds to fire disturbances, offering insights into carbon and water cycle dynamics under changing climatic conditions.

How to cite: Shen, Y., Prentice, C., and Harrison, S.: Global Drivers of Post-Fire Ecosystem Recovery: Insights from Solar-Induced Chlorophyll Fluorescence, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3308, https://doi.org/10.5194/egusphere-egu25-3308, 2025.

EGU25-3335 | Orals | BG1.1

A new probabilistic method to identify fire-igniting lightning events 

Jose V. Moris, Hugh G.P. Hunt, Pedro Álvarez-Álvarez, Marco Conedera, Francisco J. Gordillo-Vázquez, Jeff Lapierre, Francisco J. Pérez-Invernón, Nicolau Pineda, Gianni B. Pezzatti, Sander Veraverbeke, and Davide Ascoli

Lightning-induced ignitions play a major role shaping the frequency, patterns and characteristics of wildfires in several regions across the globe, including extreme wildfire events (e.g., Góis wildfire in 2017 in Portugal) and fire seasons, such as 2019-20 in Australia, 2020 in California, and 2023 in Canada. The attention to lightning-ignited wildfires has been growing in recent years. Studies on LIWs frequently associate lightning and wildfire data to discern or approximate the place and moment of fire ignition. This typically requires to select the lightning strike responsible for the ignition.

Currently, several methods are applied to select the most likely lightning strike causing the ignition. However, this selection is complicated by, at least, two aspects. First, the spatial uncertainty of fire and lightning data (e.g., the location errors of detected lightning events). Second, the holdover phenomenon. Holdover time, commonly defined as the time between lightning-induced fire ignition and fire detection, can range from a few minutes to several days, and more rarely to some weeks or even months. Long holdover times are associated to the presence of a smoldering phase that hinders the detection of these lightning fires.

Here, we present a novel method that uses location accuracy information from lightning location networks, as well as expected distributions of holdover time, to assess the probabilities of lightning igniting wildfires. Our method computes a probability metric, which is the product of two independent probabilities: a spatial and a temporal probability. The spatial component assesses the probability of a cloud-to-ground lightning event striking within a given area surrounding the fire discovery point, while the temporal component evaluates the probability of a lightning-ignited wildfire undergoing a certain holdover time. The lightning event with the maximum probability metric value is then selected as the most likely ignition source. We applied this method in three study areas: Switzerland, Catalonia (Spain), and California and Nevada (USA). The results were compared with lightning selections identified by the index of proximity, one of the currently most common methods to select the most likely ignition source of lightning-induced wildfires.

The initial results indicate that the probability metric yields a different selection of lightning events, in comparison with the index of proximity, for a great proportion of wildfires, with considerable differences across the study areas. We suggest that the probability metric provides a solid alternative to current methods. The probability metric offers some advantages: (1) it simplifies some methodological decisions despite the need for additional computations; (2) it is flexible and can be adapted to different types of lightning and fire data (e.g., fire perimeters); (3) it has a more robust theoretical basis than current methods; and (4) the lightning selection can be enhanced over time due to continuous improvements in lightning and fire databases.

How to cite: Moris, J. V., Hunt, H. G. P., Álvarez-Álvarez, P., Conedera, M., Gordillo-Vázquez, F. J., Lapierre, J., Pérez-Invernón, F. J., Pineda, N., Pezzatti, G. B., Veraverbeke, S., and Ascoli, D.: A new probabilistic method to identify fire-igniting lightning events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3335, https://doi.org/10.5194/egusphere-egu25-3335, 2025.

EGU25-4352 | ECS | Orals | BG1.1

Rising Synchronicity of Extreme Fire Weather Across Europe in a Warming Climate  

Andrina Gincheva, Miguel Ángel Torres-Vázquez, Francesca Di Giuseppe, Alberto Moreno Torreira, Sonia Jerez, and Marco Turco

Synchronous extreme fire weather significantly heightens wildfire ignition and spread risk, potentially overwhelming firefighting efforts. Despite evidence of increasing fire weather extremes in a warming climate, the spatial-temporal synchronicity of these conditions remains understudied outside North America. This research investigates historical and projected changes in the synchronicity of extreme fire weather in Europe, employing the Fire Weather Index (FWI) from 1981–2022 and climate scenarios representing temperature increases (1°C to 6°C) and precipitation changes (-40% to +60%). 

Our findings reveal Central Europe as a significant hotspot, with synchronicity increases up to 389%, and the Mediterranean region experiencing a 66% rise. Synchronicity trends are driven by rising temperatures and shifting atmospheric circulation patterns, particularly in summer and autumn. Future projections suggest compounded fire risks across broader regions, requiring enhanced transnational coordination. This study emphasizes the growing need for proactive fire management strategies tailored to increasing synchronicity, including shared resource mechanisms like RescEU, and highlights the value of integrating synchronicity assessments into regional climate adaptation planning. This abstract is based on findings from a study accepted for publication in Environmental Research Letters.  

Acknowledgements 

A.G. thanks to the Ministerio de Ciencia, Innovación y Universidades of Spain for Ph.D. contract FPU19/06536. A.G., M.A.T-V., and M.T. acknowledge the support of the ONFIRE project, grant PID2021-123193OB-I00, funded by MCIN/AEI/10.13039/501100011033 and by “ERDF A way of making Europe”. M.T. acknowledges funding by the Spanish Ministry of Science, Innovation, and Universities through the Ramón y Cajal Grant Reference RYC2019-027115-I. This work was supported by the project ‘Climate and Wildfire Interface Study for Europe (CHASE)’ under the 6th Seed Funding Call by the European University for Well-Being (EUniWell). 

How to cite: Gincheva, A., Torres-Vázquez, M. Á., Di Giuseppe, F., Moreno Torreira, A., Jerez, S., and Turco, M.: Rising Synchronicity of Extreme Fire Weather Across Europe in a Warming Climate , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4352, https://doi.org/10.5194/egusphere-egu25-4352, 2025.

Fires have great ecological, social, and economic impact. However, fire prediction and management remain challenges due to a limited understanding of their roles in the Earth system. Fires over southern Mexico and Central America (SMCA) are a good example of this, greatly impacting local air quality and regional climate. Here we report that the spring peak (April–May) of fire activities in this region has a distinct quasi-biennial signal based on multiple satellite datasets measuring different fire characteristics. The variability is initially driven by quasi-biennial variations in precipitation. Composite analysis indicates that strong fire years correspond to suppressed ascending motion and weakened precipitation over the SMCA. The anomalous precipitation over the SMCA is further found to be mostly related to the East Pacific–North Pacific (EP-NP) pattern 2 months prior to the fire season. The positive phase of the EP-NP leads to enhanced precipitation over the eastern US but suppressed precipitation over the SMCA, similar to the spatial pattern of precipitation differences between strong and weak fire years. Meanwhile, the quasi-biennial signals in precipitation and fires appear to be amplified by their interactions through a positive feedback loop at short timescales. Model simulations show that in strong fire years, more aerosol particles are released and transported downstream over the Gulf of Mexico and the eastern US, where suspended light-absorbing aerosols warm the atmosphere and cause the ascending motion of the air aloft. Subsequently, a compensating downward motion is formed over the region of the fire source and ultimately suppresses precipitation and intensifies fires. Statistical analysis shows the different durations of the two-way interaction, where the fire suppression effect of precipitation lasts for more than 20 d, while fire leads to a decrease in precipitation at shorter timescales (3–5 d). This study demonstrates the importance of fire–climate interactions in shaping the fire activities on an interannual scale and highlights how precipitation–fire interactions at short timescales contribute to the interannual variability in both fire and precipitation.

How to cite: Liu, Y., Qian, Y., and Wang, M.: Fire–precipitation interactions amplify the quasi-biennial variability in fires over southern Mexico and Central America , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5454, https://doi.org/10.5194/egusphere-egu25-5454, 2025.

EGU25-6847 | ECS | Posters on site | BG1.1

Changes in atmospheric oxidising capacity cause teleconnections between biomass burning and NH4NO3 formation 

Damaris Y. T. Tan, Mathew R. Heal, Massimo Vieno, David S. Stevenson, Stefan Reis, and Eiko Nemitz

Open biomass burning affects many aspects of the Earth system, including atmospheric chemistry and composition. Due to its impact on human health, we focus on the contribution of biomass burning emissions to fine particulate matter (PM2.5) concentrations on a global, annual mean basis, particularly the lesser-studied secondary inorganic component. We use the EMEP MSC-W WRF atmospheric chemistry transport model to show that biomass burning leads to increased ammonium nitrate (NH4NO3) concentrations in densely populated regions not necessarily associated with large-scale fire activity. This is prominent in the eastern USA, northwestern Europe, the Indo-Gangetic Plane and eastern China, where NH4NO3 contributes between 29 and 51% to annual mean biomass burning-derived PM2.5. Pyrogenic CO and NOx (NO and NO2) emissions alter the global-scale oxidising capacity of the atmosphere, affecting how local-scale anthropogenic NOx and NH3 emissions lead to formation of NH4NO3. These teleconnections can locally increase, by up to a factor of two, the contribution of biomass burning emissions to PM2.5 concentrations, which measurements alone cannot detect. This will become relatively more important as anthropogenic sources of PM2.5 are reduced, and with potentially intensified biomass burning occurrences under climate change.

How to cite: Tan, D. Y. T., Heal, M. R., Vieno, M., Stevenson, D. S., Reis, S., and Nemitz, E.: Changes in atmospheric oxidising capacity cause teleconnections between biomass burning and NH4NO3 formation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6847, https://doi.org/10.5194/egusphere-egu25-6847, 2025.

EGU25-7107 | ECS | Orals | BG1.1

Development of a Wildfire Risk Prediction System based on Deep Learning Methods and Remote Sensing 

Jhony Alexander Sanchez Vargas, Johannes Heisig, Marco Painho, and Mana Gharun

Wildfires pose a significant threat to ecosystems, human life, and infrastructure, particularly in South America, where diverse climatic and environmental factors contribute to their occurrence. Climate change has exacerbated extreme weather conditions such as intense heat and drought, leading to a global increase in the frequency and intensity of wildfires. Countries like Brazil have experienced significant rises in wildfire damage, highlighting the urgent need for predictive models that accurately assess future wildfire risks to mitigate their impact effectively. This thesis addresses this need by developing a wildfire risk prediction system leveraging deep learning methods and remote sensing data.

Using Earth Observation (EO) APIs, the system avoids downloading and storing vast amounts of satellite imagery, enabling efficient data acquisition and preprocessing. The study focuses on key variables that influence wildfire activity, including dynamic variables such as Land Surface Temperature (LST), Normalized Difference Vegetation Index (NDVI), Enhanced Vegetation Index (EVI), radiation, Leaf Area Index (LAI), evapotranspiration (ET), wind speed, and temperature, as well as static variables like land cover, Digital Elevation Model (DEM), and population density. The system is designed to predict wildfire risk for the next day and up to eight days, offering a robust tool for proactive wildfire management.

Given the stochastic and nonlinear nature of wildfire phenomena, this research employs advanced deep learning techniques, including Random Forests (RF), Long Short-Term Memory networks (LSTM), and Convolutional LSTM (ConvLSTM) models, to predict wildfire risk in near real-time. Active fire data from MODIS products, along with their burn dates, serve as the basis for training datasets. Non-fire points are generated by mapping the land cover distribution of fire points, ensuring balanced datasets for model training. Variables are extracted and classified into dynamic and static categories to capture both temporal variability and fixed geographical characteristics.

The objectives of this research are threefold: (1) to investigate existing remote sensing-based wildfire management methodologies and identify enhancements through the integration of data cubes and deep learning; (2) to develop a scalable platform for efficient data acquisition, preprocessing, and risk prediction using deep learning algorithms; and (3) to evaluate the system’s accuracy, efficiency, and scalability with real-world datasets and disaster scenarios.

Preliminary results highlight the effectiveness of integrating remote sensing data with deep learning models for wildfire risk prediction. Dynamic variables such as EVI, LST, and NDVI, along with human influence factors like Global Human Modification Index (gHM), emerged as key predictors, demonstrating the interplay of environmental and anthropogenic drivers in wildfire occurrences. Seasonal analysis from 2021 to 2024 revealed a strong correlation between fire activity, elevated temperatures, and declining vegetation indices from November to April. The Random Forest model achieved 83% accuracy, while the LSTM model showed promise with 75% accuracy, emphasizing the potential of both static and temporal data. These findings lay a robust foundation for enhancing wildfire risk management through advanced machine-learning approaches.

How to cite: Sanchez Vargas, J. A., Heisig, J., Painho, M., and Gharun, M.: Development of a Wildfire Risk Prediction System based on Deep Learning Methods and Remote Sensing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7107, https://doi.org/10.5194/egusphere-egu25-7107, 2025.

Wildfire smoke is increasingly recognized as a significant source of air pollution that leads to public health issues. Over the past few decades, air pollution in Canada has been reduced due to effective regulations. However, fine particulate emissions (i.e., particles with an aerodynamic diameter of less than 2.5 μm (PM2.5)) from wildfires have shown upward trends as climate change exacerbates the frequency and likelihood of wildfires. According to the Canadian Interagency Forest Fire Centre (CIFFC) in 2021, there were 18% more fire starts and nearly a 61% increase in the total area burned compared to the past 10-year average in Canada. The emissions inventories used for modeling the impact of fires on air quality and climate exhibit several discrepancies in emissions estimates, primarily due to the different types of satellite products used for identifying fires and measuring burned area, as well as differences in emission factors describing the vegetative fuels burned. This variability of fire emission inventories leads to uncertainties in  predicting air quality. Using the GEOS-Chem chemical transport model, we studied how differences in emissions estimates among three commonly used global biomass burning inventories—the Global Fire Emissions Database 4 (GFED4), the Global Fire Assimilation System (GFAS), and the Quick-Fire Emissions Database 2 (QFED2)—and a newly developed  regional biomass burning emission inventory, the Canadian Forest Fire Emissions Prediction System (CFFEPS), affect modeled concentrations of PM2.5 during the 2021 wildfire season in Canada. To examine the sensitivity of simulated PM2.5 to different biomass burning emission datasets, we compared them with ground based PM2.5 data from 70 NAPS (National Air Pollution Surveillance) stations across Canada, from east to west. The simulated PM2.5 concentrations showed significant variation in model performance based on the geographic location of the monitoring stations, particularly between the western and eastern regions of Canada. These findings indicate the importance of considering the strengths and weaknesses of each fire inventory, as some inventories may more accurately represent fire emissions in certain regions than others.

How to cite: Ashraf, S., Hayes, P., Stevens, R., and Chen, J.: Evaluating the Effect of Variability in Biomass Burning Emissions Inventories on Modeled Smoke Concentrations: Insights from the 2021 Canadian Wildfire Season, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7351, https://doi.org/10.5194/egusphere-egu25-7351, 2025.

EGU25-8307 | ECS | Orals | BG1.1

Vegetation fires as a source of soil-dust particles – a global model perspective 

Robert Wagner, Ina Tegen, and Kerstin Schepanski

Vegetation fires are well known as an important source of aerosol particles originating from the combustion of carbonaceous material. Much less known is that these fires can also efficiently inject soil-dust particles into the atmosphere, raised by the strong fire-induced winds. These soil-dust particles and the likely co-emitted biogenic particles are potent cloud condensation nuclei (CCN) and ice nucleating particles (INPs), and can substantially alter the cloud microphysics and thus impact the Earth’s radiation budget. Fires are an integral component of the Earth system that affect different landscapes around the globe. As they are supposed to get more frequent and more severe along with the ongoing global warming, a better knowledge of these specific fire emissions is crucial to understand their impacts on weather and climate.

Therefore, this work investigates the potential of wildfires to emit soil-dust particles on a global scale as a part of the newly established Leibniz ScienceCampus “BioSmoke” (‘smoke and bioaerosols in a changing climate’). As this particular dust emission pathway is not considered by the state-of-the-art dust emission models, a parameterization describing fire-induced dust emission fluxes has been developed and implemented into the global aerosol-climate model ICON-HAM. Fire-dust emissions are modelled as a function of the fire radiative power (FRP), the ambient wind conditions, and further soil-surface properties, including the soil type and a vegetation-dependent surface roughness correction.

Multi-year ICON-HAM simulations have revealed that fire-related dust emissions can account for up to one fifth of the total global dust emissions with strong regional and seasonal variations, both as the result of a varying fire activity and the local soil-surface conditions that can foster or impede also fire-dust emission significantly. In regions where the classic wind-driven dust emissions from arid, unvegetated soil surfaces are rather low but wildfires occur frequently, e.g., in large parts of the Southern hemisphere, fire-related dust emissions can add substantially to the atmospheric aerosol load and affect the local radiation budget there.

How to cite: Wagner, R., Tegen, I., and Schepanski, K.: Vegetation fires as a source of soil-dust particles – a global model perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8307, https://doi.org/10.5194/egusphere-egu25-8307, 2025.

EGU25-8637 | Orals | BG1.1

The real drivers of the ML revolution in fire forecasting 

Francesca Di Giuseppe, Joe Mc Norton, Fredrik Wetterhall, and Anna Lombardi

Recent advancements in machine learning (ML) have significantly broadened its applications, including the potential to transition from forecasting fire weather to predicting actual fire activity. In this study, we demonstrate the feasibility of this transition using an operational forecasting system. By integrating data on human and natural ignitions along with observed fire activity, data-driven models effectively address the persistent overprediction of fire danger in fuel-limited biomes. This results in fewer false alarms and more informative outputs compared to traditional methods.

A key factor driving this improvement is the availability of global datasets for fuel dynamics and fire detection, which were not accessible during the development of earlier physics-based models. We find that the enhanced predictive skill of ML models stems largely from the comprehensive characterization of fire processes provided by these datasets, rather than from the complexity of the ML methods themselves.

As enthusiasm gather around  data-driven approaches, our findings highlight the critical importance of high-quality training data in improving forecast accuracy. While the rapid advancement of ML techniques generates excitement, there is a risk of undervaluing the essential role of data acquisition and, where necessary, its creation through physical modeling. Our results underscore that investing in robust datasets is indispensable and should not be overlooked in the pursuit of  very complex algorithm.

How to cite: Di Giuseppe, F., Mc Norton, J., Wetterhall, F., and Lombardi, A.: The real drivers of the ML revolution in fire forecasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8637, https://doi.org/10.5194/egusphere-egu25-8637, 2025.

EGU25-8708 | Orals | BG1.1

Evaluation of fire emissions for HTAP3 with CAMS GFAS and IFS-COMPO 

Johannes Kaiser, Vincent Huijnen, Samuel Remy, Martin A. Ytre-Eide, Mark C. De Jong, Bo Zheng, and Christine Wiedinmyer

The Copernicus Atmosphere Monitoring Service CAMS is using ECMWF's Integrated Forecasting System IFS-COMPO with fire emissions from its Global Fire Assimilations System GFAS to monitor and forecast the effect of smoke from vegetation fires, resp. biomass burning, on atmospheric composition. The simulated atmospheric composition fields are routinely validated against observations including from satellites, aircraft and ground stations.

The emissions calculation by the operational GFAS version 1.2 have recently been updated for use in the upcoming HTAP3 multi-model, multi-pollutant study of fire impacts (Whaley et al. 2024), creating the dataset GFAS4HTAP. It is based on the dry matter burnt estimates of GFASv1.2, and uses an updated spurious signal mask, ESA CCI land cover data for 2018, a global peat map (Xu et al. 2018) and emission factors from NEIVA (Shahid et al. 2024) to calculate emission fluxes for various smoke constituents for 2003-2024. An additional GFAS-based dataset has been created by calibration against GFED5beta.

Global comparisons of dry matter, resp. biomass, combustion rates of the three GFAS-based inventories with GFED4s, GFED5beta, and the two variants of FINN2.5 reveal that these inventories can be roughly classified into one group of "traditional" inventories with lower fire activity, resp. emissions, and another of "more recent" inventories with higher fire activity. The pyrogenic carbon monoxide emission estimates from an inversion of satellite observations of atmospheric composition (Zheng et al. 2019) lie between these two groups in terms of global annual values. However, at a global level, they are more consistent with the "more recent" inventories during the late boreal summer peak of the global fire activity and with the "traditional" inventories during periods of lower fire activity.

In order to gain more insight from independent validation, we here present simulations with IFS-COMPO for 2019 based on the three GFAS-based inventories and compare these with atmospheric observations of carbon monoxide, nitrogen dioxide and aerosol optical depth. We find that the best agreement of simulation and observations is achieved by different inventories for different regions, seasons and smoke constituents. However, the emissions of the GFAS4HTAP dataset appears to lead to the overall most balanced atmospheric composition simulation. This supports the group of "traditional" inventories mentioned above.

How to cite: Kaiser, J., Huijnen, V., Remy, S., Ytre-Eide, M. A., De Jong, M. C., Zheng, B., and Wiedinmyer, C.: Evaluation of fire emissions for HTAP3 with CAMS GFAS and IFS-COMPO, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8708, https://doi.org/10.5194/egusphere-egu25-8708, 2025.

As the climate warmings, the frequency and intensity of wildfires have escalated in recent decades.  While the adverse effects of wildfires on air quality are well-documented, their influence on atmospheric ozone in China remains unclear. Here, we apply deep learning and a trajectory-fire interception method (TFIM) to estimate wildfire contributions to ozone concentrations in Chinese cities from 2015 to 2023. Our findings indicate that wildfires influenced 15.1 ± 9.3% of all days during this period, with a wildfire-induced ozone concentration averaging 6.8 μg m-³. Over the nine-year study period, these concentrations exhibited a modest upward trend, increasing by 0.091 μg m⁻³ annually. Regions such as Southwest China, the Qinghai-Tibet Plateau, and Northwest China experienced the highest levels of wildfire-induced ozone. We further utilize SHapley Additive exPlanations algorithms to investigate driving factor behind wildfire-induced ozone. The burnt area, aging hour, and injection height of smoke have a large effect on wildfire-induced ozone concentrations. Finally, we evaluated the health impacts of wildfire-induced ozone, highlighting its significant implications for public health in affected regions.

How to cite: Liu, S.: Explainable deep learning reveal the contribution of wildfire to ozone in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8751, https://doi.org/10.5194/egusphere-egu25-8751, 2025.

EGU25-9010 | ECS | Posters on site | BG1.1

Global fire regimes, their non-fire characteristics, and changes in time. 

Eleanor Butler, Sebastian Sippel, and Ana Bastos

Fires as a disturbance regime are an important component of ecosystems, and are involved in many feedback loops within these systems such as climate-carbon feedbacks. The changing climate can influence fire regimes in multiple ways, both directly and indirectly. For example, changing weather patterns can directly alter the occurrence and timing of fire weather days. Weather patterns also influence vegetation growth and ecosystem composition, leading to changes in fuel availability and flammability. Meanwhile, humans also partially shape fire regimes via accidental and managed ignitions as well as various suppression measures.

In this study, we use 35 years of remote sensing data to establish global pyromes; regions of similar fire regimes, via their fire characteristics. This length of data period allows for the allocation of pyromes across multiple time segments, and for changes in their prevalence and spatial distribution to be observed. We have found that the majority of pyrome transitions occurring are shifts towards smaller or less frequent fires, and these transitions are widespread across the globe. However, some regions such as the Northern high latitudes, the Western United States, and Northern Australia are shown to experience larger or more frequent fires in the final observation segment of the study.

Following on from this, we use statistical methods to investigate relationships between pyromes and a wide variety of non-fire properties, including climate, vegetation, and human influence. This allows for inference of the most relevant drivers of pyrome change, both climatic and non-climatic. Initial results suggest for example, that population density is a more important predictor for pyromes with small and medium sized fires. However, there are significant challenges to disentangling the effects of such complex drivers within a relatively short observational period. Nevertheless, it is possible to build a picture of plausible fire regime evolution in regions with shifting environmental components.

How to cite: Butler, E., Sippel, S., and Bastos, A.: Global fire regimes, their non-fire characteristics, and changes in time., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9010, https://doi.org/10.5194/egusphere-egu25-9010, 2025.

EGU25-9049 | Posters on site | BG1.1

The Sensitivity of High Latitude Wildfires and their impacts on Atmospheric Composition to underlying driving processes in the UK’s Earth System Model (UKESM) 

Steven Turnock, João Teixeira, Chantelle Burton, Katie Blackford, Stephen Arnold, and Fiona O'Connor

Wildfires have a significant influence on the Earth system through perturbing the carbon cycle and also emitting large quantities of short lived climate forcers (SLCFs) such as aerosol precursors (black and organic carbon) and gases that can lead to ozone formation (carbon monoxide, nitrogen oxides). SLCFs are important as they affect the Earth’s radiative balance, influencing climate, and also can have important impacts on air quality in the near-surface atmosphere. Climate change and human interference also have important effects on the size, magnitude and duration of wildfires, which are important to understand further, particularly in the context of a changing climate. Such influences are potentially important in the northern high latitudes, where wildfires have been increasing in magnitude and frequency over the last few decades. Here, we present an evaluation of the representation of high latitude wildfires in a configuration of UKESM with an interactive fire module (INFERNO) coupled to chemistry, aerosol and radiation schemes.  We also show results from sensitivity studies analysing the influence of model process drivers on high latitude wildfires and their impacts on atmospheric composition over the recent past, including from changes in climate, socio-economic factors and underlying vegetation properties.

The baseline configuration of UKESM coupled with INFERNO shows an underestimation of burnt area from high latitude wildfires over the period 2000 to 2015 compared to that reported by GFED4s. The sensitivity scenarios show that this underestimation is found to be strongly driven by the human suppression factor included within INFERNO. The underestimation in burnt area is also reflected in the emission of SLCFs from high latitude wildfires e.g. CO, with implications for both climate and air quality. The INFERNO fire scheme does not currently include the representation of peat fires, which are important sources in the high latitude. When we include a representation of SLCF emissions from high latitude peat fires, the magnitude and temporal variability of such emissions are much improved in the model and compare better with those in GFED4s. Including this additional source also increases the contribution of wildfires to particulate air pollution and the degradation in surface air quality simulated by the model over the northern high latitudes. The interactive fire model coupled within UKESM is shown to underestimate high latitude wildfires due to missing sources and the representation of human interactions in this region. This has important consequences for regional air quality and climate in an area of the world experiencing rapid changes to its climate.

How to cite: Turnock, S., Teixeira, J., Burton, C., Blackford, K., Arnold, S., and O'Connor, F.: The Sensitivity of High Latitude Wildfires and their impacts on Atmospheric Composition to underlying driving processes in the UK’s Earth System Model (UKESM), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9049, https://doi.org/10.5194/egusphere-egu25-9049, 2025.

The backscattering linear depolarization ratio (LDR) is a key parameter to identify particle types. Previous studies on smoke LDR have shown significant differences in their measurements, with the magnitudes varying widely under different study scenarios. Single-particle models involving internally mixed black carbon (BC) are applied to assess the LDR of smoke aerosols. However, handicaps have been found to apply such models to describe the bulk optical properties of aerosols, because of their overlook of the contribution of externally mixed organic carbon (OC) to the LDR. Smoke aerosols typically consist of a low proportion of BC particle population and a high proportion of externally mixed OC particle population. If the spherical assumption is applied to the calculation of smoke LDRs, the LDRs turned to be extremely low even approach zero. This leads to difficulties in explaining the observed variability and higher levels of smoke LDR. We conducted a prescribed burning experiment in Xichang, Sichuan Province, China, and did onsite measurement on the LDR of smoke at a wavelength (λ) of 532 nm using atmospheric laser lidar. Field smoke particles were collected using a single-particle sampler and the morphology of particles was then characterized by the transmission electron microscope (TEM). The results indicated that the LDR of local smoke varied between 0 and 20.1%, with rapid fluctuations. The TEM images confirmed the coexistence of both internally mixed BC and externally mixed OC in the smoke aerosols, with OC displaying an ellipsoidal morphology even on copper grids. Using the discrete dipole approximation, we subsequently evaluated the LDR of individual BC and OC. Based on light scattering theory, we further quantified the bulk LDRs of the aerosol aerosols. The results shown that the smoke LDR ranged from 0.0% to 28.2% in λ = 532 nm while accounting for the effect of externally mixed OC. The LDR is slightly influenced by BC and is significantly affected by the externally mixed OC. Furthermore, the LDR is primarily governed by the morphology and particle size distribution of the externally mixed OC. It is concluded that the high levels and rapid variations in the LDRs of smoke can be largely attributed by the non-sphericity and particle size distribution of externally mixed OC. This study advances the methodologies for LDR measurements and evaluations of smoke aerosols from biomass burning.

How to cite: Qin, Z., Zhang, Q., Wang, H., and Zhang, Y.: The role of non-sphericity of externally mixed organic carbon in altering the backscattering linear depolarization ratio of smoke aerosols from biomass burning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9452, https://doi.org/10.5194/egusphere-egu25-9452, 2025.

EGU25-10591 | Posters on site | BG1.1

Fire proneness of Mediterranean pyroregions is positively linked to tree functional traits indicative of fire-modulated responses 

José Maria Costa-Saura, Gabriele Midolo, Carlo Ricotta, Mara Baudena, Carlo Calfapietra, Mario Elia, Paolo Fiorucci, Simone Mereu, Costantino Sirca, Donatella Spano, Giana Vivaldo, and Gianluigi Ottaviani

Fire is a natural phenomenon that modulates form, function, diversity and distribution of plant species affecting ecosystem dynamics. Global warming and land use change are altering fire regimens potentially threating ecosystem functioning and species persistence. However, pyrogeographical studies aiming to understand differences across fire regimens are usually not considering the role played of plant functional traits. Here, based on a recent pyroregionalization in Italy and using species distribution data from the Italian National Forest Inventory and trait values from public databases we assessed if: 1) species distribution across different pyroregions is affected by fire regime, 2) species in different pyroregions exhibit distinct fire-related trait values, and, if so, 3) trait differences suggest better abilities to cope with fire in species distributed in more fire-prone regions (e.g. thicker bark). Our results tend to positively answer our questions suggesting the necessity of including fire-related traits when studying pyroregions. Noticeably, our study showed that the most fire-prone pyroregions collapse into one region from a functional perspective, with species characterized by highly similar trait values and indicative of fire adaptations.

How to cite: Costa-Saura, J. M., Midolo, G., Ricotta, C., Baudena, M., Calfapietra, C., Elia, M., Fiorucci, P., Mereu, S., Sirca, C., Spano, D., Vivaldo, G., and Ottaviani, G.: Fire proneness of Mediterranean pyroregions is positively linked to tree functional traits indicative of fire-modulated responses, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10591, https://doi.org/10.5194/egusphere-egu25-10591, 2025.

EGU25-12104 | ECS | Orals | BG1.1

Large eddy simulations of the Williams Flat Fire: Aqueous chemistry in pyrocumulous clouds 

Simon Rosanka, Timothy Juliano, Ann Marie Carlton, and Mary Barth

Wildfires are an increasing concern for climate change, air quality and recognized for their substantial impacts on atmospheric composition. In addition to significant emissions of carbon dioxide (CO2) and particular matter (PM), biomass burning events are characterized by substantial non-CO2 emissions, which encompass a wide range of species. These emissions significantly influence atmospheric chemistry at a regional to global scale. Particularly in regions with ample fuel sources and hot, dry, or windy meteorological conditions, surface fires can lead to high-intensity crown fires and frequent downwind spotting. In certain circumstances, the intense formation of crown fires triggers the development of pyrocumulonimbus (PyroCb) atop smoke columns, which ascend to the upper troposphere and lower stratosphere (UTLS) and thus promote the dispersion of the fire emissions within wide regions. On August 2, 2019, the Williams Flats Fire ignited due to lightning from early morning thunderstorms in eastern Washington, USA. The main fire activity occurred between August 2 and August 9. On August 8, the high intensity crown fires led to the formation of a PyroCb. This event was observed and probed by the joint NOAA and NASA FIREX-AQ field campaign, providing a unique observation dataset. In this study, we utilize the Weather Research and Forecasting Model (WRF) to assess the impact of the Williams Flats fires on the atmospheric composition. In particular, we couple the representation of detailed multi-phase chemistry (WRF-CHEM) with WRF’s fire spread model (WRF-FIRE), employing WRF’s Large Eddy Simulation capabilities to resolve turbulence at resolutions of 100 m. In this presentation, results from WRF-FIRE-CHEM simulations with and without aqueous-phase chemistry will be shown to isolate its effects on the long-range transport of trace gases and aerosols.

How to cite: Rosanka, S., Juliano, T., Carlton, A. M., and Barth, M.: Large eddy simulations of the Williams Flat Fire: Aqueous chemistry in pyrocumulous clouds, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12104, https://doi.org/10.5194/egusphere-egu25-12104, 2025.

Machine learning (ML) models are widely used to predict wildfire occurrence and susceptibility (Brys et al., 2025). However, while these models excel at prediction, they often fail to provide insights into their inner workings or uncover the causal pathways driving wildfires. This study addresses this limitation by extending ML models beyond prediction to explore the drivers and causal pathways underlying wildfire occurrence. Our primary aim is to identify meaningful, interpretable patterns from wildfire data.

We developed a novel multi-stage clustering methodology inspired by Cooper et al. (2021) and Cohen et al. (2024). This approach integrates feature attribution (SHAP values), dimensionality reduction (UMAP), hierarchical clustering (HDBSCAN), and causal discovery methods: PC and FCI (Spirtes et al., 2001), and DirectLiNGAM (Shimizu et al., 2011). The causal methods were enhanced with prior background knowledge to derive meaningful insights. We used datasets from Italy (Cilli et al., 2022) and the Netherlands.

A central feature of our methodology is the use of SHAP values to define subgroups and derive causal pathways. SHAP values reduce noise in the feature space while preserving critical information for clustering. By reducing multidimensional SHAP values to two dimensions with UMAP, we improved clustering performance and interpretability. The resulting clusters were described using concise, non-overlapping decision rules based on the original variables, eliminating the need for manual filtering commonly required in clustering raw feature space. The identified clusters revealed specific relationships between wildfire drivers and occurrence. For each cluster, we applied advanced causal discovery techniques to derive probable causal pathways, aligning the findings with the knowledge of stakeholders and domain experts. These actionable and interpretable explanations offer practical utility.

Findings from the case studies demonstrate that supervised clustering effectively characterizes wildfire occurrence by linking it to influencing factors. Furthermore, the approach provides valuable insights into cluster-specific causal pathways. The methodology translates complex relationships into simple causal logic, offering stakeholders and domain experts the necessary context to understand the model's behavior.

 

Brys, C., La Red Martínez, D.L. & Marinelli, M. Machine learning methods for wildfire risk assessment. Earth Science Informatics 18, 148 (2025). https://doi.org/10.1007/s12145-024-01690-z

Cilli, R., Elia, M., D’Este, M., Giannico, V., Amoroso, N., Sanesi, G., Lombardi, A., Pantaleo, E., Monaco, A., Tangaro, S., Bellotti, R. & Lafortezza, R. (2022). Explainable artificial intelligence (XAI) detects wildfire occurrence in the Mediterranean countries of Southern Europe. Scientific Reports 12, 16349. https://doi.org/10.1038/s41598-022-20347-9

Cohen, J., Huan, X. & Ni, J. (2024). Shapley-based explainable AI for clustering applications in fault diagnosis and prognosis. Journal of Intelligent Manufacturing, 35, 4071-4086. https://doi.org/10.1007/s10845-024-02468-2

Cooper, A., Doyle, O. & Bourke, A. (2021). Supervised clustering for subgroup discovery: An application to covid-19 symptomatology. Communications in Computer and Information Science, 1525, 408–422. https://doi.org/10.1007/978-3-030-93733-1_29

Shimizu, S., Inazumi, T., Sogawa, Y., Hyvärinen, A., Kawahara, Y., Washio, T., Hoyer, P. O., & Bollen, K. (2011). DirectLiNGAM: A direct method for learning a linear non-Gaussian structural equation model. The Journal of Machine Learning Research, 12, 1225–1248. https://doi.org/10.48550/arXiv.1101.2489

Spirtes, P., Glymour, C. & Scheines, R. (2001). Causation, Prediction, and Search. Second Edition. MIT Press. https://doi.org/10.7551/mitpress/1754.001.0001

 

How to cite: Korving, H. and Van Marle, M.: Decoding Wildfires - Extracting Interpretations and Causal Pathways of Catalysts for Wildfire Occurrence from Machine Learning Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12889, https://doi.org/10.5194/egusphere-egu25-12889, 2025.

EGU25-13378 | ECS | Posters on site | BG1.1

Using AI-enabled wildfire risk maps to communicate risk: the role of labelling, information presentation, perceived trustworthiness and emotion in shaping perceived risk in Veluwe, Netherlands 

Milica Mijailovic, Alyson Ranucci, Christoph Geib, Bettina Nardelli, Eva Koppen, Futaba Tamura, and Paul Kandathil Parambil

Rising temperatures and changing climate conditions have increased wildfire risk across the world, including in regions such as The Netherlands that have not historically faced these threats. With this trend expected to continue, understanding risk perceptions among individuals with little to no wildfire experience becomes crucial for mitigating the impacts and designing effective risk communication strategies.

Recent advancements in Artificial Intelligence (AI) wildfire mapping tools have proven highly effective in identifying areas susceptible to wildfires, particularly in detecting low-probability incidents by uncovering subtle patterns often missed by traditional methods. For example, machine learning (ML) wildfire risk maps developed by MEJOR Technologies have accurately predicted wildfire locations in The Netherlands in the past. Despite the potential, the use of these tools as communication instruments to improve wildfire risk perception among the public remains largely unexplored.

Through an online randomised experiment conducted among a sample of residents in the Veluwe area of The Netherlands, we empirically assess how AI-generated labelling (AI label, ML label, or no label) and information presentation formats (map, text, or combined) affect individuals’ perceived wildfire risk. Additionally, we investigate whether perceived trustworthiness in technologies and emotion mediate these effects, providing deeper insights into the cognitive and affective processes that shape how individuals in this area perceive wildfire risk. By leveraging our results, policy makers and AI mapping developers can design effective communication interventions and improve public preparedness in the face of wildfires. While our findings are specific to wildfires in the Veluwe area, they may also hold relevance for understanding the perception of other low-probability hazards among individuals with little to no prior exposure.

How to cite: Mijailovic, M., Ranucci, A., Geib, C., Nardelli, B., Koppen, E., Tamura, F., and Kandathil Parambil, P.: Using AI-enabled wildfire risk maps to communicate risk: the role of labelling, information presentation, perceived trustworthiness and emotion in shaping perceived risk in Veluwe, Netherlands, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13378, https://doi.org/10.5194/egusphere-egu25-13378, 2025.

EGU25-13774 | Orals | BG1.1

Modelling interactive fires: climate-fire feedbacks on fire characteristics and multi-model projects 

Cynthia Whaley, Ruth Digby, Vivek Arora, Jack Chen, Paul Makar, Kerry Anderson, Debora Griffin, Terry Keating, Tim Butler, Jacek Kaminski, and Rosa Wu

There are multiple feedback mechanisms between wildfires and climate, such as temperature, emissions, cloud interactions, deposition, and land cover changes. Wildfires can also have large societal and ecological impacts and are considered as an extreme climate event. Despite this, most Earth System Models have, until recently, used prescribed fire emissions and fire plume injection heights for input into their atmospheric models that were unresponsive to climate changes. Fire plume heights, in particular, have a great influence on the radiative forcing and long-range transport of pollutants. This presentation will show recent results from global modelling of interactive fires (land-atmosphere) in the Canadian Earth System Model (CanESM), with a focus on key wildfire characteristics, such as aerosol emissions and fire plume height. These model improvements introduce the capacity to more accurately simulate future projections of wildfire characteristics under different climate scenarios. The upcoming applications of these improvements include experiments for the Hemispheric Transport of Air Pollution (HTAP) Fires project, AerChemMIP2, and Aerocom. HTAP Fires is a multi-model, multi-pollutant study with the goal of improving global fire modelling and using the multi-model ensembles to provide estimates of fire-related pollution for impact studies and policy makers.

How to cite: Whaley, C., Digby, R., Arora, V., Chen, J., Makar, P., Anderson, K., Griffin, D., Keating, T., Butler, T., Kaminski, J., and Wu, R.: Modelling interactive fires: climate-fire feedbacks on fire characteristics and multi-model projects, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13774, https://doi.org/10.5194/egusphere-egu25-13774, 2025.

EGU25-13861 | ECS | Posters on site | BG1.1

Interactive Fire Emissions Coupled with Climate and Chemistry in GFDL’s Earth System Model version 4.1 

Arman Pouyaei, Paul Ginoux, Elena Shevliakova, and Sergey Malyshev

Fire plays a critical role in the Earth system, both as a driver and responder to climate change. Variations in vegetation cover and ignition patterns, influenced by climate, affect fire behavior, while fire emissions impact climate by altering radiative fluxes and cloud properties. Despite these interactions, most global climate models fail to fully represent the dynamic interplay between vegetation, fire, and climate. In this study, we leverage the prognostic fire module from GFDL’s Land Model (LM4.1), which includes dynamic vegetation processes, to interactively calculate biomass burning emissions and injection heights. Emissions are then coupled with the atmospheric chemistry and aerosol component (AM4.1) in GFDL’s Earth System Model version 4.1 (ESM4.1). The model calculates fire radiative power (FRP) from fire spread rates and fuel content, using it alongside atmospheric parameters like boundary layer height and Brunt-Väisälä frequency in the Sofiev injection height scheme. Fire emissions are calculated using carbon release rates from biomass estimated by the land model and emission factors from Akagi et al. (2011) and Andreae and Merlet (2001), and these emissions are integrated directly into the atmospheric model for interactive coupling. 

We conducted a coupled simulation in AMIP mode and compared the modeled emissions with the observation-based Global Fire Emissions Database (GFED4.1s). Preliminary results show a promising agreement for global fire emissions of trace gases and aerosols during the 1997–2014 period, with seasonal variability falling within the error margins of observed emissions. We then compared results from interactive fire emissions experiment with a fixed fire emission experiment to analyze the direct radiative effects of fire-emitted aerosols. By treating fire emissions as an interactive component of the Earth system, rather than as a prescribed external forcing, this approach enables a more comprehensive representation of fire-climate feedback and enhances the assessment of radiative effects from fire aerosols.

How to cite: Pouyaei, A., Ginoux, P., Shevliakova, E., and Malyshev, S.: Interactive Fire Emissions Coupled with Climate and Chemistry in GFDL’s Earth System Model version 4.1, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13861, https://doi.org/10.5194/egusphere-egu25-13861, 2025.

EGU25-14193 | ECS | Posters on site | BG1.1

Understanding Wildfire Emissions: From Composition to Variability, and their Link to Fire Characteristics  

Yingxiao Zhang, Mary Barth, Louisa Emmons, Makoto Kelp, Timothy Juliano, Wenfu Tang, Rebecca Hornbrook, and Eric Apel

Wildfires emit a complex mixture of trace gases and aerosols that significantly impact air quality, climate, and atmospheric chemistry. Key trace gases include carbon dioxide (CO₂), carbon monoxide (CO), nitric oxide (NO), methane (CH₄), and volatile organic compounds (VOCs). Wildfire-generated aerosols predominantly consist of organic carbon (OC), black carbon (BC), and secondary organic aerosols (SOA). Over recent decades, the frequency and intensity of wildfires, particularly in the western United States, have risen due to warmer temperatures and prolonged periods of drought. This trend has led to increased fire activity and smoke emissions, causing wildfires to be a growing contributor to regional and global aerosol forcing, in turn affecting the Earth's radiation budget and climate system. However, substantial uncertainties remain in estimating the composition and quantity of wildfire emissions.

Large variability in biomass burning aerosol estimates across different fire emission inventories poses challenges for accurate air quality and climate impact assessments. To address these challenges, we leverage observational data from the FIREX-AQ and WE-CAN campaigns to investigate how wildfire characteristics such as individual fire size, fire radiative power, and fuel composition influence the chemical composition of wildfire emissions, particularly VOCs. We then develop and apply an artificial neural network in tandem with dimensionality reduction methods to estimate smoke chemistry utilizing fire characteristics. Our machine learning model's results are compared with existing observations and current fire emission inventories to improve our understanding of wildfire emissions and their impacts.

How to cite: Zhang, Y., Barth, M., Emmons, L., Kelp, M., Juliano, T., Tang, W., Hornbrook, R., and Apel, E.: Understanding Wildfire Emissions: From Composition to Variability, and their Link to Fire Characteristics , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14193, https://doi.org/10.5194/egusphere-egu25-14193, 2025.

EGU25-14573 | Orals | BG1.1

Intense transport of smoke to the Central Andes: Insights from a unique set of instruments located in the Bolivian Andean Cordillera 

Marcos Andrade, Laura Ticona, Fernando Velarde, Decker Guzman, Luis Blacutt, Ricardo Forno, Rene Gutierrez, Isabel Moreno, Fabricio Avila, Gaelle Uzu, Philippe Goloub, Michel Ramonet, Olivier Laurent, Alfred Wiedensohler, Kay Weinhold, Radovan Krejci, Diego Aliaga, David Whiteman, and Paolo Laj

In 2024, Bolivia experienced the worst year of fires since 2002, when Aqua MODIS began collecting data. According to estimates, more than 15 million hectares were burned this year. A sunphotometer sitting in the Bolivian lowlands recorded AOD values higher than two for several continuous days indicating the degradation of the air quality in the region. A unique set of instruments located in the Bolivian Andes recorded the transport of smoke produced by this biomass burning. Very high values of atmospheric tracers like carbon monoxide, equivalent black carbon, and others have been measured as high as 5240 m asl  at the Chacaltaya GAW station (CHC, 16.35ºS, 68.13ºW, 5240 m asl) and other sites around it both in the Altiplano and adjacent high altitude valleys. Although transport to these sites was observed previously, usually the events lasted one or two days. However, in 2024 longer periods of consecutive days with smoke arriving from the lowlands were observed for a second year in a row. Similar high values were observed in CHC in October of 2023, a year with less than half of fires in the country. The conditions that led to the transport of smoke to the mountains in the Andean Cordillera will be discussed, as well as the possible effects of the associated deforestation in terms of water availability for the central Andes.

How to cite: Andrade, M., Ticona, L., Velarde, F., Guzman, D., Blacutt, L., Forno, R., Gutierrez, R., Moreno, I., Avila, F., Uzu, G., Goloub, P., Ramonet, M., Laurent, O., Wiedensohler, A., Weinhold, K., Krejci, R., Aliaga, D., Whiteman, D., and Laj, P.: Intense transport of smoke to the Central Andes: Insights from a unique set of instruments located in the Bolivian Andean Cordillera, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14573, https://doi.org/10.5194/egusphere-egu25-14573, 2025.

EGU25-15236 | ECS | Orals | BG1.1 | Highlight

Modelling global burned area with deep learning 

Seppe Lampe, Lukas Gudmundsson, Basil Kraft, Bertrand Le Saux, Stijn Hantson, Douglas Kelley, Vincent Humphrey, Emilio Chuvieco, and Wim Thiery

The temporal coverage from ˜2000 to present of global burned area satellite observations limits many aspects of fire research. As a result, global fire models are often being used to investigate past and future fire behaviour. Unfortunately, the limited temporal coverage of the observations also hinders the development and evaluation of these fire models. The current generation of global fire models are capable of simulating some characteristics of regional fire behaviour, such as mean state and seasonality, well. However, the performance of these models differs greatly from region to region, and aspects such as extreme fire behaviour are not well represented yet.

Here, we propose a new, data-driven fire model that predicts burned area from the same input parameters that are passed to global fire models. We trained LSTMs to model burned area from GFED5. We split our data according to the IPCC regions and perform a region-based cross-validation, that is, we train different LSTMs on different region-splits of the data. We then compose the predictions of these different models so that for each region the predictions are made by LSTMs that have never seen any data during training and validation from that region before. Our model outperforms all fire models on a global scale and in most IPCC regions. With our model, we can improve our understanding of past fire behavior and simulate future fire trends.

How to cite: Lampe, S., Gudmundsson, L., Kraft, B., Le Saux, B., Hantson, S., Kelley, D., Humphrey, V., Chuvieco, E., and Thiery, W.: Modelling global burned area with deep learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15236, https://doi.org/10.5194/egusphere-egu25-15236, 2025.

EGU25-15318 | ECS | Orals | BG1.1

Carbon emissions of an unprecedented Greenland wildfire 

Sonja Granqvist, Lucas Diaz, Sander Veraverbeke, Elmiina Pilkama, Minna Väliranta, and Meri Ruppel

In recent years, large wildfires have spread in Arctic regions as a consequence of ongoing climate change. Arctic organic soils are comparatively shallow but may be ancient, thus thousands of years old carbon may be released in smoldering and deeply burning fires. In Greenland, a land known for its icy expanse, fires are extremely rare. However, in summer 2019, the second-largest wildfire ever recorded on the island occurred at the Kangerluarsuk Tulleq fjord in southwestern Greenland. This study aims to produce pioneering in-field data on this tundra fire, focusing on three key aspects: 1) combustion, 2) burn depth, and 3) the age of the carbon released. Understanding whether the released carbon is modern or old is crucial due to different implications for the global carbon cycle and climate. To estimate carbon losses from the Kangerluarsuk Tulleq tundra fire, we established 14 sampling plots in burned areas and at unburned control sites. The selection of sampling plots was guided by a differenced Normalized Burn Ratio (dNBR) map generated using Sentinel-2 data and field reconnaissance. Within each plot, we assessed fire severity to estimate the above-ground carbon loss. For below-ground carbon loss estimation and burn depth analysis, organic soil samples were collected at burned plots and compared with unburned ones. To explore the vegetation succession and burned vegetation type, organic soil profiles (n=10) were extracted down to the mineral ground using a soil box corer and were studied by light-microscopy. Subsamples (n=20) from burned soil horizons were selected for radiocarbon dating to determine the age of carbon released in the fire. Our preliminary results suggest that soil carbon loss was higher than previously reported at an Alaskan tundra fire site with a mean value of 6.718 ± 0.9 kg of C m-2. The mean burn depth was 9.0 ± 1.8 cm, and soil thaw depths during the 2024 summer were approximately 24 cm deeper in the 2019 burned area compared to unburned tundra. Expected radiocarbon results will indicate the maximum age of the carbon released by the fire. Vegetation succession measurements show that post-fire surfaces were predominantly colonized by pioneering non-Sphagnum bryophytes, Cyperaceae, and Ericaceae. The acquired results are first of a kind from a Greenland tundra fire and produce essential data for global climate modeling to assess the climate impacts of increasing Arctic wildfires.

How to cite: Granqvist, S., Diaz, L., Veraverbeke, S., Pilkama, E., Väliranta, M., and Ruppel, M.: Carbon emissions of an unprecedented Greenland wildfire, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15318, https://doi.org/10.5194/egusphere-egu25-15318, 2025.

EGU25-15841 | ECS | Orals | BG1.1

Modeling peat burned area and understanding its drivers with machine learning 

Jonas Mortelmans, Gabrielle De Lannoy, Devon Dunmire, Sander Veraverbeke, James Waddington, Rebecca Scholten, and Michel Bechtold

Peatland fires pose significant environmental and societal challenges. We recently advanced the Canadian Fire Weather Index (FWI) system for northern peatlands by integrating peatland-specific hydrological data derived from assimilating Soil Moisture and Ocean Salinity (SMOS) L-band brightness temperature observations into the NASA Catchment Land Surface model with its peatland modules, ‘PEATCLSM’. This novel FWIpeat (Mortelmans et al. 2024) was evaluated using satellite-based fire presence data over boreal peatlands from 2010 through 2018, demonstrating improved estimation of peatland fire presence.

Here, we extend the use of this renewed FWIpeat system by integrating it into a machine learning framework to gain deeper insights into when, where, and why peatlands burn. We utilize an XGBoost algorithm trained on peatland burned area data from 2012-2023, incorporating a suite of predictors, including (i) peatland distribution characteristics, (ii) peatland groundwater table, (iii) lightning occurrence, (iv) meteorological data, (v) vegetation properties, and (vi) socio-economic factors. This approach enables proactive fire risk management strategies and contributes to a comprehensive assessment of peatland fire vulnerability and resilience. Preliminary results indicate the importance of peatland groundwater table and lightning occurrence in estimating peat burned area.

Mortelmans, J., Felsberg, A., De Lannoy, G. J. M., Veraverbeke, S., Field, R. D., Andela, N., and Bechtold, M.: Improving the fire weather index system for peatlands using peat-specific hydrological input data, Nat. Hazards Earth Syst. Sci., 24, 445–464, https://doi.org/10.5194/nhess-24-445-2024, 2024.

How to cite: Mortelmans, J., De Lannoy, G., Dunmire, D., Veraverbeke, S., Waddington, J., Scholten, R., and Bechtold, M.: Modeling peat burned area and understanding its drivers with machine learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15841, https://doi.org/10.5194/egusphere-egu25-15841, 2025.

EGU25-16179 | ECS | Posters on site | BG1.1

Climate feedback of forest fires amplified by atmospheric chemistry 

Wei Chen, Yuzhong Zhang, Yufei Zou, and Zhen Zhang

The recent surge in forest fires has significantly impacted atmospheric chemistry, carbon cycles, and climate. Wildfires release CO2 along with various reactive species such as CO, volatile organics, and nitrogen oxides. While the effects of CO2 emissions on the carbon cycle and climate, as well as the impact of reactive species emissions on air quality and health, have been extensively studied, this research demonstrates that reactive species emitted from wildfires create a positive climate feedback through the “fire-chemistry-methane” mechanism. In this process, chemical reactions of reactive carbon species suppress the concentration of hydroxyl radicals, extending the lifetime of heat-trapping methane. The significance of this feedback is suggested by observations of multiple proxy gases for global atmospheric oxidation (i.e., methyl chloroform, methane, and CO) during recent extreme forest fire events. By coupling a fire-ecosystem model and an atmospheric chemistry model, we quantify the effect of this feedback in the future. We find that additional warming caused by this mechanism rivals that of wetland methane feedback and fire CO2 feedback by the 2050s under an intermediate climate scenario. Our analysis highlights the critical role of atmospheric chemistry in regulating fire-climate interactions and the methane budget.

How to cite: Chen, W., Zhang, Y., Zou, Y., and Zhang, Z.: Climate feedback of forest fires amplified by atmospheric chemistry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16179, https://doi.org/10.5194/egusphere-egu25-16179, 2025.

EGU25-16840 | ECS | Orals | BG1.1

Morphological drivers of flammability in canopy and litter contexts across conifer families 

Rebecca Koll and Claire Belcher

Wildfires have shaped ecosystems for millions of years, with plant functional traits playing a key role in fire behaviour and severity. Morphological and physiological traits, particularly at the leaf and shoot levels, influence flammability by determining fuel composition and structure within both canopy and litter layers. These traits are hypothesized not only to affect critical fire dynamics, such as the likelihood of surface fires transitioning into crown fires, with significant consequences for fire intensity and ecosystem impacts, but also influence the evolution of fire-related traits.

This study investigates how leaf- and shoot-level morphology influences flammability in canopy and litter contexts across six dominant conifer families: Araucariaceae, Cupressaceae, Pinaceae, Podocarpaceae, Taxaceae, and Taxodiaceae. Flammability properties were assessed using fire calorimetry to measure ignitability, flame spread, and variability in the rate of energy release from combustion. Results indicate that while shed plant parts (e.g., leaves and shoots) shape fire behaviour by influencing bulk density, aeration, and flame spread rate—ultimately affecting burn sustainability and total energy release—shoot-level traits in isolation, including leaf shape and the arrangement of leaves within shoots, do not consistently predict flammability in canopy material.

Our findings highlight the dynamic interplay between plant morphology, fire regimes, and evolutionary pressures. Traits such as leaf size, shape, and arrangement contribute to fuel structure, driving patterns of fire behaviour that influence long-term plant fitness and survival. This underscores the importance of reconciling fire behaviour, plant functional traits, and the evolutionary history of fire adaptations across phylogenies.

With global change drivers intensifying fire regimes, understanding the relationship between plant flammability, fire regimes, and the acquisition of fire-related traits is increasingly critical. Non-fire-adapted species may face heightened extinction risks, threatening ecosystem stability. Quantifying the intrinsic flammability of plant traits is therefore essential for informing fire management, guiding conservation strategies, and ensuring the long-term sustainability of vegetative communities in a changing climate.

How to cite: Koll, R. and Belcher, C.: Morphological drivers of flammability in canopy and litter contexts across conifer families, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16840, https://doi.org/10.5194/egusphere-egu25-16840, 2025.

The interactions of different components of the Earth system, such as between the biosphere and the atmosphere, are still poorly understood. A major issue is understanding the consequences of increasing wildfire  activity in a changing climate. Smoke particles and gases emitted from such fires affect air quality and the Earth’s radiation balance, and can potentially affect the formation of clouds and precipitation. Understanding links between biodiversity and type of vegetation, smoke emission and the atmospheric distribution and processing of these particles and gases is key for assessing potential impacts and future changes. Addressing the depth of processes in the interconnected atmosphere-climate-vegetation system requires a combination of expertise from various scientific disciplines. The new Leibniz ScienceCampus “Smoke and bioaerosols: Release, processes, and impacts in a changing climate” (BioSmoke) located in Leipzig, Germany will combine expertise in atmospheric and biodiversity research as well as atmospheric processes at several research institutions including the Leibniz Institute for Tropospheric Research and Leipzig University to study effects of the release of aerosol particles from vegetation. To this end, combustion experiments in the laboratory, field measurements of aerosol properties, and remote sensing and modelling of particle emission, transport, and atmospheric effects are envisioned. We will present an overview of the planned projects within the ScienceCampus.

How to cite: Tegen, I., Wagner, R., and Tesche, M.: Introducing the Leibniz Science Campus “Smoke and bioaerosols: Release, processes, and impacts in a changing climate”, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17284, https://doi.org/10.5194/egusphere-egu25-17284, 2025.

EGU25-17646 | ECS | Orals | BG1.1

Investigation of the intense wildfire events and NH3 levels over the Eastern Mediterranean 

Serra Saracoglu, Aykut Mehmet Alban, Seda Tokgoz, and Burcak Kaynak

South eastern Mediterranean region of Türkiye is well known with intense industrialization, shipping activities, agriculture and livestock production in addition to urban emission sources, thus struggle with significant air pollution problems. In addition to criteria pollutants, combination of these sources also results in high ammonia (NH3) levels in the region.

NH3 is released into the atmosphere mainly from agriculture, including nitrogen-based fertilizer applications and livestock farming as well as from several industries and from biomass burning. Atmospheric NH3 plays a significant role in the formation of secondary inorganic particulate matter (PM), which negatively impacts on human health and ecosystems and indirectly influences climate change by altering radiative forcing. Climate change has increased the frequency and intensity of wildfires globally, which became another significant source of NH3 over the Eastern Mediterranean, because the region is among the most sensitive regions. Besides wildfires, agricultural residue burning, although prohibited, also contributes to overall NH3 levels.

Biomass burning contributes to atmospheric pollutants, as the combustion process emits nitrogen and carbon compounds from organic matter. In this study, multi-satellite derived retrievals were utilized, including IASI Level-2 NH3 and CO, TROPOMI Level-2 NO2, CO, and HCHO along with VIIRS S-NPP Fire Radiative Power product to investigate biomass burning related NH3 levels. Products were processed at a 1x1km2 gridded resolution to analyse spatio-temporal variations from 2019 to 2023, especially focusing on intense fire time intervals. While NH3 levels were generally high during the summer over the region, the 2021 summer stood out with exceptionally high levels, coinciding with intense wildfires recorded that year. Similarly, CO levels revealed elevated levels during the same period, further strengthening the common impact of these extreme events. Further, fires detected over some areas by the VIIRS product were associated with residue-burning practices, as the area predominantly consists of agricultural lands.

The aim of the study is to investigate the impacts of fire-related NH3 levels and quantify NH3 enhancements during these fire events in the region. In this context, NH3 to other pollutant ratios will be examined and temporal variation between different biomes will be classified. Air quality and climate change impact studies over the Mediterranean are critically important, with the absence of ground-based NH3 measurements, satellite retrievals have to be utilized more to investigate the sensitivity of the region to extreme biomass burning events with the growing impacts of climate change.

Keywords: ammonia, carbon monoxide, nitrogen dioxide, biomass burning, wildfires

Acknowledgements: IASI is a joint mission of EUMETSAT and the Centre National d'Etudes Spatiales (CNES, France). The authors acknowledge the AERIS data infrastructure for providing access to the IASI data in this study and ULB-LATMOS for the development of the retrieval algorithms. This study was supported by the Scientific and Technological Research Council of Türkiye under the grant number 123Y364.

How to cite: Saracoglu, S., Alban, A. M., Tokgoz, S., and Kaynak, B.: Investigation of the intense wildfire events and NH3 levels over the Eastern Mediterranean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17646, https://doi.org/10.5194/egusphere-egu25-17646, 2025.

EGU25-17962 | Orals | BG1.1

Assessing the impact of climate change on boreal high latitude wildfire using a storyline approach 

Lars Nieradzik, Hanna Lee, Xavier Levine, Paul Miller, Priscilla Mooney, Ruth Mottram, and David Wårlind

Within the framework of the project PolarRES  (POLAR Regions in the Earth System) we assess the impact of climate change on the ecosystems of the terrestrial northern high latitudes by making use of a range of high resolution regional climate simulations. These regional simulations were themselves driven by global climate simulations selected following the storyline approach described in Levine et al. 2024 from the set of CMIP6 SSP3-7.0 simulations, namely NorESM2-MM and CNRM-ESM2-1. These define two extremes in the climatic envelope of the CMIP6 simulations. While NorESM2-MM shows a high warming of the Barents-Kara seas but a low Arctic tropospheric warming CNRM-ESM2-1 shows the opposite. The storyline approach is a comprehensive way of defining pathways for physical outcomes of climate change that are observable in the region of interest and can directly be linked to certain consequences.

The 2nd generation Dynamic Global Vegetation Model (DGVM) LPJ-GUESS with its wildfire model SIMFIRE-BLAZE was applied using the high-resolution meteorological forcing from the regional climate models (RCMs) to investigate the potential impacts on both vegetation and the development of wildfires as well as the role of uncertainty implied by the variability of the forcing data.

It can clearly be stated that wildfire activity will increase significantly under the given scenarios driven mainly by shifts in vegetation distribution, i.e. northward migration of both treeline as well as shrubs and grasses. These effects differ regionally, depending on both, the storyline and the RCMs.

We present the findings from an envelope of potential future climate forcings depicting the impact of climate depending on the regionally observable effects of Arctic tropospheric warming and the Barents-Kara Seas warming, making use of the storyline approach as a comprehensive indicator for regional future change.

The results of this assessment will directly influence the research conducted in the project GreenFeedBack (GREENhouse gas fluxes and earth-system FEEDBACKs), which focusses on enhancing the knowledge on GHG dynamics in the boreal high latitude terrestrial and marine ecosystems.

 

Levine, X. Jet al. : Storylines of summer Arctic climate change constrained by Barents–Kara seas and Arctic tropospheric warming for climate risk assessment, Earth Syst. Dynam., 15, 1161–1177, https://doi.org/10.5194/esd-15-1161-2024, 2024

How to cite: Nieradzik, L., Lee, H., Levine, X., Miller, P., Mooney, P., Mottram, R., and Wårlind, D.: Assessing the impact of climate change on boreal high latitude wildfire using a storyline approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17962, https://doi.org/10.5194/egusphere-egu25-17962, 2025.

EGU25-18252 | Orals | BG1.1

Impact of wildfires on air quality as seen by IAGOS in-situ measurements 

Yasmine Bennouna, Hannah Clark, Pawel Wolff, Valérie Thouret, Romain Blot, Philippe Nédélec, and Damien Boulanger

For thirty years, the European Research Infrastructure IAGOS (In-Service Aircraft for a Global Observing System) has been equipping commercial aircraft with instruments to measure atmospheric composition on long-haul flights around the world.  Ten aircraft are currently equipped with IAGOS instruments to measure ozone, and the precursors carbon monoxide and nitrous oxides from the surface to the upper-troposphere during landing and take-off at worldwide airports,  and at cruise altitude where we observe the long-range transport of polluted airmasses. We analyse the transport of biomass burning pollutants from the intense Canadian wildfire seasons of 2023 and 2024 which impacted air-quality in North America and in Europe, and the extreme wildfires over the Amazon in 2024 that impacted air quality in South American cities.  The significance of these events is interpreted within the context of the 30-year climatology. The events will be compared with forecasts and analyses from the Copernicus Atmosphere Monitoring Service's global and regional models (projects CAMS2_82 and CAMS2_83) and we further  highlight the role of IAGOS  in developing air-quality networks in susceptible urban areas (project RI-URBANS) and the impacts of heatwaves and wildfires on air-quality in a changing climate (project IRISCC).

How to cite: Bennouna, Y., Clark, H., Wolff, P., Thouret, V., Blot, R., Nédélec, P., and Boulanger, D.: Impact of wildfires on air quality as seen by IAGOS in-situ measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18252, https://doi.org/10.5194/egusphere-egu25-18252, 2025.

EGU25-18640 | ECS | Orals | BG1.1 | Highlight

Adapting to fire in a warming climate: towards global assessment of prescribed grazing and prescribed fire 

Oliver Perkins, Olivia Haas, Matthew Kasoar, Doug Kelley, João C. M. Teixeira, Apostolos Voulgarakis, and James D.A. Millington

Whilst global burned area continues to decline, recent climate warming has led to an increase in the occurrence and intensity of extreme fires. Humanity must adapt to this new reality. Two proposed management options are a) prescribed livestock grazing, and b) prescribed fire use. Both methods promise cost-efficient means to reduce fire intensity, fire-induced vegetation mortality, and carbon emissions by reducing and fragmenting fuel loads. However, at present, there has been no systematic global assessment of the efficacy of these interventions. Reasons for this include a lack of data to understand their present-day distribution and impact as well as a lack of formal model structures to represent their uptake under future scenarios.

Here, we present two applications of the newly developed global, agent-based Wildfire Human Agency Model (WHAM!)1 to assess the potential effect of prescribed grazing and prescribed fire as adaptations to future fire regimes. Firstly, to explore the effect of prescribed livestock grazing on global fire regimes, we share a representation of livestock grazing intensity in WHAM! and its integration with the generalised linear models of Haas et al., (2). Secondly, we present work on a tight coupling of WHAM! with the JULES-INFERNO dynamic global vegetation model, focusing on parameterisation of how managed human fire use reduces fire-induced vegetation mortality.

Overall, early results suggest both management options already play a significant role in reducing global fire intensity and highlight the importance of considering dynamic human responses to a changing climate in global projections of future fire regimes.

1Perkins, O… et al. (2024). GMD.

2Haas, O. et al., (2022). Env. Res let.

How to cite: Perkins, O., Haas, O., Kasoar, M., Kelley, D., Teixeira, J. C. M., Voulgarakis, A., and Millington, J. D. A.: Adapting to fire in a warming climate: towards global assessment of prescribed grazing and prescribed fire, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18640, https://doi.org/10.5194/egusphere-egu25-18640, 2025.

EGU25-18688 | ECS | Orals | BG1.1

Satellite observation of long-range transport of wildfires plumes in the northern hemisphere in 2008-2023 

Antoine Ehret, Solène Turquety, Gilles Lecomte, Bruno Franco, Maya George, Lieven Clarisse, Martin Van Damme, Cathy Clerbaux, and Pierre Coheur

Wildfires exert a important influence on the chemical composition of the atmosphere, thereby impacting air quality, ecosystem, and climate forcing. The substantial emission of pollutants from such fires, coupled with their long-range transport, has the potential to counteract the progress achieved in reducing anthropogenic emissions. Numerous studies show that the increase in the frequency and intensity of fires offsets the general trend towards improved air quality observed in regions influenced by wildfires. These studies also caution of an increasing risk of the population being exposed to extreme levels of aerosols and ozone. In addition to their regional impacts, the plumes from the most intense fires can be transported on a continental or even hemispheric scale, thereby imposing health constraints on regions that are not generally affected by widespread, frequent or intense fires.

The northern hemisphere is home to a group of biomes that are particularly sensitive to hydro-meteorological conditions, and therefore to the effects of climate change on burned areas. The majority of the most intense fires of the last two decades have occurred in North America and in the boreal regions of Asia.

This study assesses the impact of fires on the variability of total CO, total PAN and AOD in the Northern Hemisphere using 16 years (2008-2023) of observations from the IASI/MetOp and MODIS/Terra and Aqua satellite instruments. More specifically, the variability in the number of detected plumes of extreme values of CO, PAN and aerosol from fires is studied.

The trajectories of these plumes are estimated using only satellite observations and are used to assess the contribution of the different regions of the Northern Hemisphere to the variability of atmospheric composition. The potential impact of the long-range transport of the identified plumes on air quality is estimated using observations of the altitude of the plumes obtained from both active CALIOP observations and passive IASI observations.

The chemical composition of the identified plumes is characterised using IASI observations of ammonia (NH3), formic acid (HCOOH), methanol (CH3OH) and ozone (O3).

How to cite: Ehret, A., Turquety, S., Lecomte, G., Franco, B., George, M., Clarisse, L., Van Damme, M., Clerbaux, C., and Coheur, P.: Satellite observation of long-range transport of wildfires plumes in the northern hemisphere in 2008-2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18688, https://doi.org/10.5194/egusphere-egu25-18688, 2025.

EGU25-18848 | ECS | Posters on site | BG1.1

An improved approach for simulating peat ignition probability using experimental data 

Dimitra Tarasi, Matthew Kasoar, Hafizha Mulyasih, Alexander Castagna, Guillermo Rein, and Apostolos Voulgarakis

Peatlands, despite covering only 3% of the terrestrial surface, are one of the world's most important carbon storage environments, accumulating around 25% of the total soil carbon. However, climate change is increasing the vulnerability of these carbon-rich ecosystems to fire, with potentially severe implications for the global climate. Warmer and drier conditions, driven by climate change, are expected to intensify and increase the frequency of peat fires, potentially transforming peatlands from carbon sinks into net sources of greenhouse gas emissions. Such a shift could trigger a positive feedback loop, accelerating climate change through the release of vast amounts of sequestered carbon into the atmosphere.

While incorporating peatland fire feedbacks into Earth System Models (ESMs) is essential for accurate climate projections, the majority of the existing models lack a representation of peat fires, limiting their ability to predict future climate dynamics effectively. Understanding the smouldering behaviour of organic soils, their ignition probability, and how these processes can be represented at a global scale is essential. The current state-of-the-art approach to compute peat combustibility, established by Frandsen (1997) and applied in recent peat fire modelling efforts (e.g., INFERNO-peat), relies on a parameterization derived from a single peat type, hampering its global applicability. Frandsen (1997), by conducting experiments on natural peat samples developed an empirical model for smouldering ignition probability based on three key properties of peat: moisture content, inorganic content, and bulk density.

Our study proposes an improved method for calculating peat combustibility by optimizing the coefficients in Frandsen’s model and investigating the ignition limits of diverse peat samples. The optimization process utilized experimental data from seven distinct peat types. First, we established through inverse modelling a link between inorganic content, bulk density and critical moisture content, the moisture threshold above which smouldering cannot be self-sustained. Then we determined the probability distribution of self-sustained smouldering, as a function of moisture content, around the critical moisture content, also employing inverse modelling. The combination of both optimizations yielded consistent coefficients, providing a more robust framework for modelling peat ignition probability.

By improving the representation of peat ignition probability using experimental data from both previous studies and our own experiments, this work aims to upgrade the simulation of peat fires in fire models and ESMs, enhancing our understanding of the impacts of such fires on future atmospheric composition, radiative forcing, and climate.

How to cite: Tarasi, D., Kasoar, M., Mulyasih, H., Castagna, A., Rein, G., and Voulgarakis, A.: An improved approach for simulating peat ignition probability using experimental data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18848, https://doi.org/10.5194/egusphere-egu25-18848, 2025.

EGU25-19104 | Orals | BG1.1

A new measurement site in northern Botswana to observe savanna fire plumes 

Ville Vakkari, Baagi T. Mmereki, Daniel Koolebogile, Christiaan P. E. van Niekerk, Viet Le, Mabala Letsatle, Kerneels Jaars, and Pieter G. van Zyl

Globally, approximately half of landscape fire emissions originate from savannas and grasslands. Furthermore, our observations in South Africa indicated major secondary aerosol formation in near-fire plume ageing. However, the measurements in South Africa are affected by anthropogenic emissions from the Highveld region, except for a clean sector towards the semi-arid Karoo region. Aiming for a savanna environment with minimal anthropogenic influence we set up a new measurement site in the Okavango delta area in northern Botswana in August 2024.

For the active savanna fire season in 2024, we operated online measurements of aerosol chemical composition with an aerosol chemical speciation monitor (ACSM), an online gas chromatograph coupled to an MS detector (GC-MS) for volatile organic compounds and a single particle soot photometer (SP2) for refractive BC. Measurements of aerosol particle size distribution with a differential mobility particle sizer (DMPS), aerosol absorption with a multi angle absorption photometer (MAAP), as well as CO and CO2 concentrations will continue for the next couple of years at least.

For fresh plumes, initial analysis shows a strong decrease in submicron aerosol emission factor (EFPM1) with increasing modified combustion efficiency, i.e. with increasing flaming fraction. The EFPM1 values are in good agreement with previous observations in southern African savanna and with recent laboratory experiments that we carried out in collaboration with University of Eastern Finland. Analysis of ageing effects on the fire plumes in a clean savanna environment is ongoing.

How to cite: Vakkari, V., Mmereki, B. T., Koolebogile, D., van Niekerk, C. P. E., Le, V., Letsatle, M., Jaars, K., and van Zyl, P. G.: A new measurement site in northern Botswana to observe savanna fire plumes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19104, https://doi.org/10.5194/egusphere-egu25-19104, 2025.

Wildfires increasingly threaten European ecosystems and communities, highlighting the necessity for effective predictive metrics to enhance fire risk management strategies. This study aims to compare the effectiveness of Vapor Pressure Deficit (VPD) and the Fire Weather Index (FWI) in forecasting wildfire occurrence and the extent of burned areas across various European forest types. Utilizing the European Forest Fire Information System (EFFIS) for comprehensive fire event data and the ERA5 reanalysis dataset from the European Centre for Medium-Range Weather Forecasts (ECMWF) for meteorological variables, daily VPD and FWI values will be derived for multiple fire seasons spanning from 2000 to 2024.

The research will explore how VPD and FWI each predict wildfire occurrence and burned area, with a focus on different forest types are categorized according to the CORINE Land Cover classification into broadleaf, conifer, and mixed forests while encompassing a range of climatic regions across Europe. VPD calculation methods are generally more straightforward and require fewer input parameters. In contrast FWI system is more complex, requiring a broader range of input data to compute its numerous indices.

By comparing these two metrics across diverse forest types and biomes, the study seeks to determine the most effective indicators for wildfire prediction in Europe. The findings are intended to inform policymakers and fire management agencies, aiding in the development of targeted early warning systems and adaptive fire management strategies. This comparative assessment will contribute to a deeper understanding of the climatic drivers of wildfires and support efforts to mitigate their impacts under changing environmental conditions.

How to cite: Shatto, C. and Samimi, C.: Comparative Assessment of Vapor Pressure Deficit and Fire Weather Index in Predicting Wildfire Occurrence and Burned Area Across European Forest Types Using EFFIS and ERA5 Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19262, https://doi.org/10.5194/egusphere-egu25-19262, 2025.

EGU25-19493 | Orals | BG1.1

The role of dry and heat extremes on vegetation dynamics in the recent fire seasons in Southern Europe 

Célia Gouveia, Mariana Finuras, Ana Russo, and Tiago Ermitão

Rural fires are recurrent in Southern Europe due to climate conditions, land use change, or a combination of both. Wet and mild winters and dry and warm summers favour the growth of vegetation and its subsequent low moisture content, increasing fuel availability. In Portugal, between 15 and 20 September 2024, severe wildfires burned more than 145,000 hectares and caused the death of more than 9 people. In Greece a major fire, stated as the largest recorded in the EU, started near the city of Alexandroupolis on August 21, with around 80.000 hectares burnt, mainly affecting the Dadia Forest and causing the death of almost two tens of migrants. Despite the crucial role played by dry fuel conditions fostering the propagation of wildfires, favourable meteorological conditions and fuel accumulation are related to the recorded fire activity and burned area. The influence of spring meteorological conditions on fire season burned area through their effect on fuel accumulation and dryness is assessed. The link between hot temperature and water availability in spring and the increased risk of summer flammability and fire spread through their influence on vegetation gross productivity is evaluated using satellite-derived data. The important role of fuel accumulation during the early growing season in fire-prone regions is highlighted in the case of Portugal in 2024 and Greece in 2023 and reinforces the crucial importance of fuel management for the definition of effective fire prevention measures in the context of warmer and drier conditions forecasted for southern European Countries.

Acknowledgements: This work is supported by the Portuguese Fundação para a Ciência e Tecnologia, FCT, I.P./MCTES through national funds (PIDDAC): UID/50019/2025 and LA/P/0068/2020 https://doi.org/10.54499/LA/P/0068/2020 and also on behalf of DHEFEUS -2022.09185.PTDC and the project FAIR- 2022.01660.PTDC).

How to cite: Gouveia, C., Finuras, M., Russo, A., and Ermitão, T.: The role of dry and heat extremes on vegetation dynamics in the recent fire seasons in Southern Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19493, https://doi.org/10.5194/egusphere-egu25-19493, 2025.

EGU25-20164 | ECS | Posters on site | BG1.1

Assessing increased turbidity in reservoirs due to wildfires 

Andressa Karen da Silva Nemirovsky, Lino Augusto Sander de Carvalho, and Renata Libonati

After a wildfire event, ashes and pollutants from burns are transported to public supply reservoirs and other water systems, altering the physical and chemical properties of the water. Turbidity is a water parameter that can be applied in environmental monitoring studies to assess water quality in  public supply reservoirs, especially in fire-prone regions such as the Brazilian Cerrado. So, this work aims to answer the following question: What is the impact of the increase in burned area on water turbidity in public supply reservoirs? This study aims to investigate the relationship between environmental variables obtained through remote sensing, such as the burned area product (MODIS-MCD64A1) and turbidity data derived from the red band (620-670 nm) of MODIS Terra Surface Reflectance (Daily Global, 250m resolution), using a global algorithm and statistical analyses to derive insights over the period from 2001 to 2023 in public supply reservoirs of Cerrado.There is variability in both positive and negative turbidity anomalies from 2001 to 2023. However, in some years, positive turbidity anomalies were observed along burned areas. The insights provide the initial understanding of the relationship between burned areas and water quality, and also provide valuable support for water supply managers and the public. 

How to cite: da Silva Nemirovsky, A. K., Augusto Sander de Carvalho, L., and Libonati, R.: Assessing increased turbidity in reservoirs due to wildfires, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20164, https://doi.org/10.5194/egusphere-egu25-20164, 2025.

EGU25-283 | ECS | Orals | OS1.9

Drivers of sensible heat flux in the Southern Ocean and their relationship to submesoscale fronts 

Johan Edholm, Hanna Rosenthal, Louise Biddle, Sarah Gille, Matthew Mazloff, Marcel du Plessis, and Sebastiaan Swart

Advances in uncrewed surface vehicles (USVs) enable expanded observations in the Southern Ocean, a region vital for global heat uptake yet critically undersampled. Using data from three USVs that sampled the Pacific sector of the Southern Ocean in both summer and winter, we evaluate processes and decorrelation scales driving sensible heat flux variability. High flux variability is linked to synoptic-scale southwesterly winds, with sensible heat flux decorrelation scales of 40–60 km and 6–10 hours, consistent across seasons and variables. Fine-scale (<1–10 km) oceanic processes, including fronts, filaments, and boundaries, further influence flux variability: Our datasets reveal over 8,000 temperature fronts ranging from <1 km to >20 km in width. While wind-related variability dominates sensible heat flux changes across the smallest fronts, the ocean’s role becomes increasingly significant with front width, reaching parity at ~4 km. However, due to their abundance, the total change of sensible heat flux over smaller (~1 km) fronts is an order of magnitude greater than that of larger (>4 km) fronts. These results highlight the role of fine-scale atmosphere-ocean interactions in driving heat flux variability in the Southern Ocean, offering valuable insights for enhancing flux estimates in this critical region.

How to cite: Edholm, J., Rosenthal, H., Biddle, L., Gille, S., Mazloff, M., du Plessis, M., and Swart, S.: Drivers of sensible heat flux in the Southern Ocean and their relationship to submesoscale fronts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-283, https://doi.org/10.5194/egusphere-egu25-283, 2025.

EGU25-1399 | Orals | OS1.9

 Dependence of dense filament frontogenesis in a hydrostatic model  

Yalin Fan and Zhitao Yu

 

 In this study, a hydrostatic model - the Navy Coastal Ocean Model (NCOM) is used to analyze the temporal evolution of a cold filament under moderate wind (along / cross filament) and surface cooling forcing conditions. The experimental framework adhered to the setup used in large eddy simulations by Sulllivan and McWilliams (2018). For each forcing scenario, the impact of horizontal resolutions is systematically explored through varies model resolutions of 100 m, 50 m, and 20 m; and the influence of horizontal mixing is investigated by adjusting the Smagorinsky constant within the Smagorinsky horizontal mixing scheme. The role of surface gravity waves is also assessed by conducting experiments both with and without surface wave forcing. 

The outcomes of our study revealed that while the hydrostatic model is able to predict the correct characteristics/physical appearance of filament frontogenesis, it fails to capture the precise dynamics of the phenomenon. Horizontal mixing parameterization in the model was found to have marginal effect on frontogenesis, and the frontal arrest is controlled by the model’s subgrid-scale artificial regularization procedure instead of horizontal shear instability. Consequently, higher resolution is corresponding to stronger frontogenesis in the model. Thus, whether the hydrostatic model can produce realistic magnitude of frontogenesis is purely dependent on the characteristic of the front/filament simulated and model resolution. Moreover, examination of the parameterized effect of surface gravity wave forcing through vertical mixing unveiled a limited impact on frontogenesis, suggesting that the parameterization falls short in representing the real physics of wave-front interaction. 

How to cite: Fan, Y. and Yu, Z.:  Dependence of dense filament frontogenesis in a hydrostatic model , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1399, https://doi.org/10.5194/egusphere-egu25-1399, 2025.

EGU25-2211 | Orals | OS1.9

ODYSEA: a satellite mission to advance knowledge of ocean dynamics and air-sea interaction 

Tong Lee, Sarah Gille, Fabrice Ardhuin, Mark Bourassa, Paul Chang, Sophie Cravatte, Gerald Dibarboure, Tom Farrar, Melanie Fewings, Fanny Girard-Ardhuin, Gregg Jacobs, Zorana Jelenak, Florent Lyard, Jackie May, Elisabeth Rémy, Lionel Renault, Ernesto Rodriguez, Clément Ubelmann, Bia Villas Bôas, and Alex Wineteer

Ocean-surface vector winds, currents, and their interaction play critical roles in shaping many aspects of the Earth’s environment (e.g., weather, climate, marine ecosystems, and ocean health), affecting human safety and wellbeing both on land and at sea. However, there are significant capability gaps in observing winds, currents, and their interaction. At present, global gridded products of surface currents have coarse (~150 km) feature resolutions and rely on theoretical assumptions that break down near the equator. Moreover, there is no satellite that provides simultaneous wind-current measurements that are important for studying wind-current coupling and its impact on weather and climate. The “Ocean DYnamics and Surface Exchange with the Atmosphere” (ODYSEA) satellite mission concept is designed to alleviate these capability gaps. ODYSEA, proposed to NASA’s Earth System Explorers program in mid-2023, aims to provide the first-ever global measurements of total surface currents and simultaneous winds with 5-km data postings and near-daily coverage of the global ocean. ODYSEA builds on NASA’s heritage of scatterometry and the success of the airborne Doppler scatterometer flown as part of the Sub-Mesoscale Ocean Dynamics Experiment (S-MODE), NASA’s Earth Venture Suborbital-3 (EVS-3) mission. ODYSEA also leverages strong domestic and international partnerships. Here we present ODYSEA’s objectives, anticipated capabilities, and expected contributions to advance the understanding of surface current dynamics and air-sea interaction.

 

How to cite: Lee, T., Gille, S., Ardhuin, F., Bourassa, M., Chang, P., Cravatte, S., Dibarboure, G., Farrar, T., Fewings, M., Girard-Ardhuin, F., Jacobs, G., Jelenak, Z., Lyard, F., May, J., Rémy, E., Renault, L., Rodriguez, E., Ubelmann, C., Villas Bôas, B., and Wineteer, A.: ODYSEA: a satellite mission to advance knowledge of ocean dynamics and air-sea interaction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2211, https://doi.org/10.5194/egusphere-egu25-2211, 2025.

EGU25-3214 | Orals | OS1.9

Contribution of the air entrainment to the gas transfer processes in wave-breaking events 

Alessandro Iafrati, Sergio Pirozzoli, and Simone Di Giorgio

Gas exchange processes at the air-sea interface play a crucial role in regulating the climate and sustaining human and marine life. It is known that a large portion of anthropogenic carbon dioxide is absorbed by the ocean, which, in turn, releases nearly half of the oxygen we breathe through the photosynthesis of marine flora in the sunlit upper ocean layer. 

Despite its relevance, the processes governing the gas transfer across the ocean surface are not fully understood. Although there is evidence that the bubbles generated by the wave breaking enhances significantly the gas transfer rate, in particular for low-solubility species, the parameterization of their contribution is inaccurate.

To investigate the phenomenon, the gas transfer occurring at the free surface of progressive waves is simulated by using high-fidelity simulations. A multiphase flow solver is employed to model the gas flux across the air-water interface and the diffusion processes in the air and water domains, making available data with a level of detail unattainable in experiments. Waves of different initial steepness leading to regular wave patterns, mild spilling, and intense plunging breakers are examined and comparisons in terms of the gas flux across the interface and the gas concentration in the two fluids are established. 

It is shown that the amount of gas transferred from the air to the water domain increases remarkably when wave breaking occurs, particularly in the presence of bubble entrainment. The availability of such detailed information allows us to compute the gas transfer velocity. Critical in this respect is the availability of the air-water interface actual area, a quantity generally unavailable in experiments. The increase in the gas transfer velocity is higher than the increase in the interface area across which the exchange takes place, meaning that there is an additional effect related to the enhanced turbulence associated with the bubble entrainment and the subsequent fragmentation process. It is also observed that provided the actual air-water interface area is accounted for, the gas transfer velocity scales approximately as the one-fourth power of the dissipation rate of the energy content in water, consistently with previous theoretical predictions.

How to cite: Iafrati, A., Pirozzoli, S., and Di Giorgio, S.: Contribution of the air entrainment to the gas transfer processes in wave-breaking events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3214, https://doi.org/10.5194/egusphere-egu25-3214, 2025.

EGU25-3897 | ECS | Posters on site | OS1.9

Different Trajectory Patterns of Ocean Surface Drifters Modulated by Near-inertial Oscillations 

Yuhang Zheng, Wei Wu, Minyang Wang, Yuhong Zhang, and Yan Du

Near-inertial oscillations (NIOs) are widely observed dynamic motions in the global ocean, with a frequency related to earth’s rotation. Using a particle trajectory model, we found the combined influence of mesoscale eddies and NIOs could produce distinctive flower-like trajectories, which are a special case of near-inertial trajectories and were observed by surface drifters released within an anticyclone eddy in the South China Sea in 2021. The energy budget indicates that wind and geostrophic eddy currents are crucial in generating near-inertial energy during the flower-like trajectories. Furthermore, the particle trajectory model revealed variations in periods and widths of the near-inertial trajectory with latitudes. The width of near-inertial trajectories can exceed 8km in the near-equatorial region and reach 3-6km in the mid-latitude region (20°-50°). The ratios of near-inertial velocity to background velocity, defined as NITSIs, lead to arc-shaped (0.5<NITSI<1.0), overlapping semi-circular (NITSI>1.0), and near-circular trajectories (NITSI>>1.0). Globally, approximately 1/3 of the drifters’ lifespan featured clear near-inertial trajectories, with a significant presence in most middle latitudes and the largest NITSI in the north Pacific westerly. These findings highlight the importance of NIOs and suggest their substantial impact on local surface matter distribution, trajectory prediction, and marine rescue operations.

How to cite: Zheng, Y., Wu, W., Wang, M., Zhang, Y., and Du, Y.: Different Trajectory Patterns of Ocean Surface Drifters Modulated by Near-inertial Oscillations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3897, https://doi.org/10.5194/egusphere-egu25-3897, 2025.

EGU25-5067 | ECS | Posters on site | OS1.9

Ocean-Atmosphere Coupling Processes during Typhoons in the East China Sea 

Bowen Du and Hui Wu

Typhoons, as intense ocean-atmosphere interaction events, exert profound impacts on coastal regions. The path and intensity of typhoons are predominantly governed by oceanic and atmospheric processes. While extensive research has been conducted in deep ocean regions, the mechanisms of ocean-atmosphere heat exchange during typhoon events remain inadequately understood in shallow shelf regions. It’s particular in the East China Sea, which is distinguished by its expansive continental shelf, shallow depths, overlapping surface and bottom mixed layers, and the influences of shelf circulation and the Yangtze River plume. In this region, tides are one of the key driving forces influencing ocean dynamics, however, they are rarely considered in ocean-atmosphere coupling studies. Basing on these, we have developed a high-resolution ocean-atmosphere coupled model for the coastal waters of China using the COAWST (Coupled-Ocean-Atmosphere-Wave-Sediment Transport) modeling system. This effort builds upon our research group's established high-resolution ocean model. Through simulations and validations of typhoon events, preliminary results demonstrate that ocean-atmosphere coupling significantly improves the prediction of typhoon tracks and intensities. This study will further analyze the dynamics of ocean-atmosphere heat flux exchanges during typhoons under the influence of shelf processes and examines their impacts on typhoon paths and intensities, with particular attention to the role of tides. These findings provide new insights into the dynamic processes induced by typhoons in coastal shelf regions and advance our understanding of their interactions with shallow ocean systems.

How to cite: Du, B. and Wu, H.: Ocean-Atmosphere Coupling Processes during Typhoons in the East China Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5067, https://doi.org/10.5194/egusphere-egu25-5067, 2025.

With the growth in computing power and the advancement in numerical algorithms, computational fluid dynamics (CFD) is playing an increasingly important role in the study of many fluid mechanics problems in geophysical sciences.  Built on highly accurate numerical schemes and utilizing high-performance computing, high-fidelity CFD is especially valuable for faithfully capturing the flow physics of turbulence in complex environments, such as water waves.  This talk will introduce some of our recent developments in numerical methods for nonlinear wave fields and turbulence in the wave environment.  The flow physics of wave-turbulence interaction will be illustrated, focusing on the turbulent boundary layers and multiphase flows at the wave surface.  Innovative theoretical analyses and modeling will be presented to reveal the underlying flow dynamics. 

How to cite: Shen, L.: Simulation-Based Study of Turbulent Flows in Wave Environment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5153, https://doi.org/10.5194/egusphere-egu25-5153, 2025.

EGU25-5418 | ECS | Posters on site | OS1.9

Impacts of Dust on Surface-Radiative Fluxes, and Sea Surface Temperatures in the Red Sea 

Sravanthi Nukapothula, Hari Prasad Dasari, Ravi Kumar Kunchala, Vassilis P. Papadopoulos, Ibrahim Hoteit, and Yasser Abualnaja

This study examines the impact of dust on surface and radiative fluxes, as well as sea surface temperature (SST), over the Red Sea during the dust season (March to August) from 1980 to 2024 using reanalysis and satellite datasets. We first identfied the extreme dust days (EDDs) across the Arabian Peninsula using MERRA-2 reanalysis data, employing the mean and two-sigma standardized deviation method. A total of 1,083 EDDs were detected during the study period, with 394, 103, and 39 days exclusively affecting the southern Red Sea, northern Red Sea, and the entire Red Sea, respectively.

We analysed the key variables, including dust aerosol optical depth, wind patterns, surface fluxes (latent and sensible heat), radiative fluxes (longwave and shortwave), and SST anomalies for the Red Sea and its sub-regions during EDDs. Positive anomalies in dust aerosol optical depth were observed over all three regions during EDDs, and further identified the dust transport pathways based on wind analyses. The results show significant radiative impacts, including increased longwave radiation (+16 W/m²) and reduced shortwave radiation (-30 W/m²) with suppressed latent heat flux (-50 W/m²) and sensible heat flux (-10 W/m²), indicating substantial ocean heat loss through surface evaporation during EDDs.

The SST anomalies also revealed a notable cooling across the Red Sea, with the northern region cooling up to -1.4°C, and the southern region exhibited milder cooling ranging between -0.3°C and +0.2°C. The average cooling across the entire Red Sea is approximately -0.8°C reflects the combined effects of stronger cooling in the northern and moderate cooling in the southern Red Sea region during EDDs. These findings highlight the critical role of dust in modulating surface energy budgets and SST variability in the Red Sea under three different EDD scenarios.

Key words: Arabian Peninsula, Extreme Dust Days, The Red Sea, Suraface-Radiative Fluxes, and Sea Surface Temperature.

How to cite: Nukapothula, S., Dasari, H. P., Kunchala, R. K., Papadopoulos, V. P., Hoteit, I., and Abualnaja, Y.: Impacts of Dust on Surface-Radiative Fluxes, and Sea Surface Temperatures in the Red Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5418, https://doi.org/10.5194/egusphere-egu25-5418, 2025.

EGU25-5512 | Posters on site | OS1.9

Development and evaluation of the probability density distribution for mixed layer depth over the global oceans 

Sergey Gulev, Vladimir Kukushkin, and Anne Marie Treguier

Development of theoretical probability density function (PDF) for MLD over the oceans is important, as such a function provides a novel avenue for diagnostics of the numerical experiments with ocean GCMs and for comparison of the model results with observational data such as Argo floats. We built a new PDF based upon the Censored Modified Fisher-Tippet distribution (CMFT PDF herein). CMFT PDF represents a 2.5 – parameter distribution with the shape and location parameters steering the PDF and a pre-defined minimum of sample. CMFT distribution provides explicit equations for the mean and variance and also allows for estimating extreme values of MLD corresponding to high percentiles. A newly developed CMFT PDF was applied to GLORYS12 reanalysis to diagnose the characteristics of MLD in terms of MLD statistics. For application we used 3-degree spatial averaging of GLORIS12 profiles to provide the results which can further analyzed and intercompared to different alternative MLD estimates. This provided quite a rich sample which was further used for computation of the PDF parameters and higher order percentiles over the global oceans. This analysis shows that characteristics of probability density distributions are quite different for different regions with e.g. Labrador Sea demonstrating much heavier tails compared to the Irminger Sea and the NAC. Extreme values of MLD for March can amount to more than 3000 meters in the Labrador Sea. This provides an effective diagnostic approach for intercomparison of different model experiments and also for validation of the model results against observational data, such as e.g. Argo buoys. We also provide the analysis of climate variability of MLD statistics derived from CMFT PDF demonstrating in particular different tendencies in the mean and extreme MLD values. Further we also discuss the links between the statistics of the ocean MLD with those of surface fluxes as well as atmospheric variability.

How to cite: Gulev, S., Kukushkin, V., and Treguier, A. M.: Development and evaluation of the probability density distribution for mixed layer depth over the global oceans, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5512, https://doi.org/10.5194/egusphere-egu25-5512, 2025.

Observations of Argo profiles and TAO/TRITON array confirm the significant seasonality of the barrier layer (BL) and temperature inversion (TI) in the northeastern tropical Pacific (NETP). Statistical result of the occurrence based on the Argo profiles reveals a bimodal variability of the BL, with two peaks in July and October. This bimodal seasonality of BL is attributed to the out-of-phase variations of the eastern Pacific fresh and warm pools. The fresh and warm pools both expand westward from May to July, when the Inter-Tropical Convergence Zone (ITCZ) becomes intense and broad. Heavy rainfall is the dominant contributor to the extension of the fresh and warm pools, leading to a high frequency of thick BL (40%). This frequent thick BL provides a precondition for its another development after August. The fresh pool is stable from August to November, while the warm pool contracts sharply. The cold tongue becomes active due to a prevailing trade wind and horizontal advection transports surface cold water to the northeastern warm pool. This cold advection deepens the isothermal layer and contributes to a frequent TI (30%) and thick BL (46%). The results suggest that the ITCZ rainfall and northward cold advection from equator dominate the upper layer stratification of NETP in summer and autumn, respectively 

How to cite: Chi, J.: The Impact of the Eastern Pacific Fresh and Warm Pools on the Bimodal Seasonality of Barrier Layers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5569, https://doi.org/10.5194/egusphere-egu25-5569, 2025.

EGU25-5682 | ECS | Orals | OS1.9

Toward a better understanding of the effects of mesoscale air-sea interactions on the Antartic Circumpolar Current dynamics using coupled ocean-atmosphere models 

Anjdy Borg, Lionel Renault, Guillaume Lapeyre, Guillaume Morvan, Julien Jouanno, and Sallée Jean-Baptiste
Strong westerly winds blowing in the Southern Ocean enhance a unique oceanic dynamic composed of the world's strongest ocean current, the Antarctic Circumpolar Current (ACC), and a vertical circulation, the Overturning Circulation. Although these currents play a central role in shaping our climate, and despite numerous international observational and modeling programs, the processes controlling their strength and variability remain poorly understood, especially those related to fine-scale oceanic processes and their interactions with the atmosphere. To fill this gap, this study aims to understand both the direct and indirect effects of air-sea interactions on the dynamics of the ACC, including the large-scale, mesoscale (10-100 km), and eddy mean flow interactions (the inverse and direct energy cascade). We focus on two main air-sea interactions: the current feedback (CFB), which corresponds to the influence of surface ocean currents on the overlying atmosphere, and the thermal feedback (TFB), which is essentially the influence of ocean surface temperature and its gradients on heat and momentum fluxes. To achieve our goals, we developed a first set of coupled ocean (CROCO) - atmosphere (WRF) simulations of an idealized atmospheric storm track coupled to an idealized ACC with a spatial resolution up to 4 km for the ocean and 10 km for the atmosphere for a period of 75 years. We will present our first results, focusing in particular on the mean oceanic and atmospheric dynamics and the exchange of kinetic and potential energy between the ocean and the atmosphere.

How to cite: Borg, A., Renault, L., Lapeyre, G., Morvan, G., Jouanno, J., and Jean-Baptiste, S.: Toward a better understanding of the effects of mesoscale air-sea interactions on the Antartic Circumpolar Current dynamics using coupled ocean-atmosphere models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5682, https://doi.org/10.5194/egusphere-egu25-5682, 2025.

Mesoscale eddies are ubiquitous features of the global ocean circulation. Tradiontally, anticyclonic eddies are thought to be associated with positive temperature anomalies while cyclonic eddies are associated with negative temperature anomalies. However, our recent study found that about one-fifth of the eddies identified from altimeter data are surface cold-core anticyclonic eddies (CAEs) and warm-core cyclonic eddies (WCEs). Idealized numerical model experiments highlight the role of relative wind-stress-induced Ekman pumping, surface mixed layer depth, and vertical entrainment in the formation and seasonal cycle of these unconventional eddies. The abundance of CAEs and WCEs in the global ocean calls for further research on this topic.

How to cite: Zhai, X.: Cold anticyclonic eddies and warm cyclonic eddies in the ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5720, https://doi.org/10.5194/egusphere-egu25-5720, 2025.

EGU25-5858 | ECS | Orals | OS1.9

Intensification of Pacific tropical instability waves over the recent three decades 

Minyang Wang, Shang-Ping Xie, Hideharu Sasaki, Masami Nonaka, and Yan Du

Tropical instability waves (TIWs), one of the most prominent mesoscale oceanic phenomena in the tropical Pacific, play important roles in climate and ecosystem. Due to limited observations and the difficulty in estimating equatorial current velocity, long-term changes in TIWs remain unknown.

 

Rather than the geostrophic equilibrium (Bonjean and Lagerloef, 2002), the TIW currents exhibit a momentum balance between inertial forces (local accelerations and advections), the Coriolis force and the pressure gradient force. Using a shallow water diagnostic model that retains the inertial forces, we have produced the TIW surface currents since 1993 based on the satellite altimetry sea surface height observations. The results have been well validated with moored observations of ocean velocities in TAO array (Wang et al., 2020, https://doi.org/10.1175/JPO-D-20-0063.1).

 

The satellite altimetry-derived TIW currents (1993-2021) have shown that TIWs have strengthened during this period, with their eddy kinetic energy (EKE) increasing by 12% per decade (~10 J m-3 per decade). The trend has been corroborated by other three independent datasets: satellite-observed sea surface temperature (1982-2021), moored currents from TAO (1980s-2020), and a global eddy-resolving ocean circulation model data (OFES2, 1958-2021). They consistently imply that the intensification is concentrated on the equatorial Yanai-mode TIWs. EKE budget based on OFES2 model data suggests that the increased EKE is attributed to the increased barotropic (primary) and baroclinic (secondary) instabilities. The former is due to the strengthened south equatorial currents (SEC), and the latter is due to the decreased mixed layer stratification and increased equatorial buoyancy fronts. The underlying mechanism is an enhanced cross-equatorial asymmetric warming in the eastern tropical Pacific since the 1990s that forces the changes in the equatorial multiscale ocean dynamics. As a feedback effect on the heat budget of cold tongue SST, the intensified TIWs lead to increased eddy dynamic heating effects of ∼70% since the 1990s near the equator, with implications for predicting and projecting tropical Pacific climate changes. (https://doi.org/10.1038/s41558-023-01915-x)

How to cite: Wang, M., Xie, S.-P., Sasaki, H., Nonaka, M., and Du, Y.: Intensification of Pacific tropical instability waves over the recent three decades, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5858, https://doi.org/10.5194/egusphere-egu25-5858, 2025.

EGU25-6892 | Orals | OS1.9

Mechanical Air-Sea Interactions at submesoscale and Wind Rolls Scales 

Lionel Renault, Enesto Rodriguez, Carlos Conejero, Igor Uchoa, Patrick Marchesiello, Marcela Contreras, and Jacob Wenegrat

In this study, we use in situ observations and high-resolution coupled ocean-atmosphere simulations to investigate the mechanical coupling between the ocean and the atmosphere (referred to as Current Feedback, CFB) at the oceanic submesoscale (O(10 km)) and wind roll scales. First, we show that while the CFB remains active at the submesoscale with a stronger effect on the surface stress during the winter, its effect on submesoscale energetics is weaker than at the mesoscale. This effect is further weakened by energy contributions from thermal feedback and the highly transient nature of submesoscale flow. In addition, using in situ observations from DopplerScat and very high resolution (dx = 80 m) coupled simulations, we show that wind rolls can obscure the imprint of surface currents on surface stress and low-level winds. This interaction induces an energy transfer from the atmosphere to the ocean that overwhelms the energy transfer from submesoscale currents to the atmosphere, and generates currents coherent with the wind rolls down to 20 m depth.

How to cite: Renault, L., Rodriguez, E., Conejero, C., Uchoa, I., Marchesiello, P., Contreras, M., and Wenegrat, J.: Mechanical Air-Sea Interactions at submesoscale and Wind Rolls Scales, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6892, https://doi.org/10.5194/egusphere-egu25-6892, 2025.

EGU25-6934 | ECS | Posters on site | OS1.9

Shallow open-ocean convection in the Weddell Sea: A case study using observations and modelling techniques 

Rowan Brown, Alexander Haumann, Martin Losch, Carsten Rauch, and Markus Janout

Water mass transformations in the Southern Ocean serve as a lynchpin in the global overturning circulation. Among them, the transformation of Circumpolar Deep Water into Antarctic Winter and Surface Water is uniquely critical for the export of Intermediate Waters north of the Polar Front, the exchange of carbon dioxide between the atmosphere and the subsurface ocean, and the upwards flux of oceanic heat, which inhibits sea ice growth. However, our understanding of the processes responsible for the upwelling of Circumpolar Deep Water and its destruction remains incomplete. We hypothesize that shallow open-ocean convective plumes, only extending into or just below the pycnocline, are underrepresented in both the observational record and in global Earth System Models (ESMs), due to their elusive spatial and temporal scales and the hydrostatic approximation made by all ESMs. Therefore, they play a hitherto undervalued role in setting the water mass structure of the Southern Ocean. We present evidence from a unique year-round upper ocean mooring in the Weddell Sea of a shallow open-ocean convective plume extending into the pycnocline during winter 2021. Using the MITgcm ocean model, we simulate an analogous plume in both hydrostatic and non-hydrostatic configurations. Preliminary results suggest that the conditions necessary to form such plumes can be expected with some regularity in the Weddell Sea. We also note differences between the non-hydrostatic and hydrostatic simulations, highlighting the expected biases associated with the hydrostatic approximation in ESMs.

How to cite: Brown, R., Haumann, A., Losch, M., Rauch, C., and Janout, M.: Shallow open-ocean convection in the Weddell Sea: A case study using observations and modelling techniques, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6934, https://doi.org/10.5194/egusphere-egu25-6934, 2025.

Metre-scale boundary layer turbulence and kilometer-scale submesoscale mixed layer eddies play crucial roles in upper ocean stratification. It is well established that the former generates significant vertical fluxes that mix the upper ocean, while the latter acts to restratify it. However, the interaction between these two multi-scale processes is not well understood, particularly when atmospheric forces are non-negligible. MPAS-Ocean was firstly used to investigate the influence of boundary layer turbulence on submesoscale eddy-induced restratification under various initial conditions. Two parametrizations K-Profile Parametrization (KPP) and k-ε were used to represent different forms of turbulence-induced destratification under the same forcing conditions. Comparison analysis was carried out by comparing the resulting submesoscale eddy-induced restratification. Among all cases, KPP exhibited a larger magnitude of vertical buoyancy flux than k-, indicating stronger turbulence-induced destratification. This enhanced destratification can lead to more intense submesoscale eddy-induced restratification, which largely compensates the turbulence-induced destratification. Furthermore, the value of the mixed layer eddy-induced streamfunction strongly depends on the strength of boundary layer turbulence, suggesting that parameterizations of these two processes may need to consider their interactions. To further explore the bidirectional interactions between these two processes, we are currently employing large-eddy simulation to resolve both. A spatial filter is used to separate the flow into submesoscales and small-scale turbulence. Preliminary results of the large eddy simulations, aiming to elucidate the interactions between these two processes, will be discussed.

How to cite: Jiang, X. and Li, Q.: interaction between boundary layer turbulence and submesoscale mixed layer eddies and its influence on upper ocean stratification, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7745, https://doi.org/10.5194/egusphere-egu25-7745, 2025.

EGU25-8009 | ECS | Orals | OS1.9

AMOC sensitivity to air-sea fluxes parametrization 

Clément Dehondt, Pascale Braconnot, Sebastien Fromang, and Olivier Marti
The Atlantic Meridional Overturning Circulation (AMOC) is a large scale circulation of about 18 Sv and 1.2 PW at 26°N characterized by upper waters flowing northward, losing heat and becoming cold deep waters before flowing back southward. The Deep Water Formation (DWF) and the Subpolar gyre circulation are key aspects of AMOC intensity [1] but strongly depend on air-sea fluxes, thus the need to quantify their influence.

To do so, we compare 5 air-sea fluxes parametrizations within the IPSL General Circulation Model (GCM) [2] based on the new DYNAMICO atmospheric dynamical core [3] and the ocean engine NEMO [4]. We show that the spread in AMOC is more than 2 Sv, confirming the high sensitivity to air-sea fluxes. Furthermore, we manage to explain these discrepancies by assessing (i) winter time buoyancy fluxes in DWF area and (ii) subtropical and subpolar gyres intensity which drives the circulation. We also analyse the ocean-atmosphere feedbacks (mainly wind and sea surface temperature) that may be responsible for changes in AMOC, hence paving the way to a better representation in GCMs.
 
 
[1] Buckley, M. W. and J. Marshall (2016), Observations, inferences, and mechanisms of Atlantic Meridional Overturning Circulation variability: A review, Rev. Geophys., 54, 5–63, doi:10.1002/2015RG000493.
 
[2] Boucher O., Servonnat, J., Albright, A. L., Aumont, O., Balkanski, Y., Bastrikov, V., et al. (2020). Presentation and evaluation of the IPSL‐CM6A‐LR climate model. Journal of Advances in Modeling Earth Systems, 12, e2019MS002010. https://doi.org/10.1029/2019MS002010
 
[3] Dubos, T., Dubey, S., Tort, M., Mittal, R., Meurdesoif, Y., and Hourdin, F.: DYNAMICO-1.0, an icosahedral hydrostatic dynamical core designed for consistency and versatility, Geosci. Model Dev., 8, 3131–3150, https://doi.org/10.5194/gmd-8-3131-2015, 2015.
 
[4] “NEMO ocean engine”, Scientific Notes of Climate Modelling Center, 27 — ISSN 1288-1619, Institut PierreSimon Laplace (IPSL), doi:10.5281/zenodo.1464816

How to cite: Dehondt, C., Braconnot, P., Fromang, S., and Marti, O.: AMOC sensitivity to air-sea fluxes parametrization, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8009, https://doi.org/10.5194/egusphere-egu25-8009, 2025.

EGU25-9247 | Orals | OS1.9

Dynamics of sea breezes: Analysis of recent events in Southwest Spain 

Esther Luján-Amoraga, Carlos Román-Cascón, Marina Bolado-Penagos, Pablo Ortiz-Corral, Juan Alberto Jimenez-Rincón, Alfredo Izquierdo, Miguel Bruno, and Carlos Yagüe

Coastal breezes are mesoscale meteorological phenomena primarily driven by the thermal contrast between land and sea surfaces, creating a dynamic system that influences local circulation. These phenomena, common in coastal regions, have a significant impact on various environmental aspects, such as regulating extreme temperatures, transporting atmospheric pollutants, and modifying coastal surface ocean currents. This study aims to characterize the sea breeze system along the southwest coast of Spain, using a combination of observational data to provide a more detailed understanding of these phenomena in the region.

The analysis of sea breeze events focused on the summers of 2023 and 2024, using data obtained from coastal meteorological stations and radiosondes launched specifically in the study area to gather vertical information on the breezes. To detect breeze events, an objective algorithm based on the work of Borne et al. (1988), Arrillaga et al. (2018), and Román-Cascón et al. (2019) was used. This algorithm facilitated the identification of breeze events based on atmospheric conditions, providing a basis for further analysis.

A key contribution of this study is the proposal of a new classification of breeze types, enabling a more accurate characterization of different breeze events, by considering variables such as intensity, duration, and associated synoptic conditions. Furthermore, statistics of the recorded events are presented, offering a deeper insight into the frequency, intensity, and temporal characterization of breezes in the study area. The study also explored the relationship between turbulent variables during breeze events and different tidal moments, which is particularly relevant due to the large intertidal zone affecting one of the stations used. This observational approach enhances the understanding of the coastal breeze system in the study area and contributes to the broader knowledge of these phenomena.

How to cite: Luján-Amoraga, E., Román-Cascón, C., Bolado-Penagos, M., Ortiz-Corral, P., Jimenez-Rincón, J. A., Izquierdo, A., Bruno, M., and Yagüe, C.: Dynamics of sea breezes: Analysis of recent events in Southwest Spain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9247, https://doi.org/10.5194/egusphere-egu25-9247, 2025.

Interannual variability of surface mixed-layer near-inertial energy (NIE, representing the intensity of near-inertial waves) in the South China Sea and western North Pacific (WNP) is investigated using satellite-tracked surface drifter data set. It is found that NIE in the study region correlates negatively with El Niño-Southern Oscillation (ENSO) with a correlation coefficient of R = −0.44 and a time lag of 5 months, mainly because the variation of local wind stress lags behind El Niño by 4 months. By separating summer and winter seasons, the correlation is significantly improved. The summer NIE correlates positively with El Niño (R = 0.62), since tropical cyclones over the WNP tend to be stronger and longer-lived during the El Niño developing phase. The winter NIE correlates negatively with El Niño (R = −0.65), since the winter monsoon is weakened by the ENSO-related WNP anomalous anticyclone. This is the first time that interannual variability of NIE is studied by direct current velocity observations. 

How to cite: lu, H.: Interannual Variability of Near-Inertial Energy in the SouthChina Sea and Western North Pacific, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10164, https://doi.org/10.5194/egusphere-egu25-10164, 2025.

Near-inertial internal waves (NIWs) are among the primary drivers of turbulence that sustains the ocean stratification. To propagate downward into the ocean interior, NIWs typically need horizontal scales L∼100 km. Therefore, it is commonly held that NIWs generated by basin-scale midlatitude storms depend on refraction by background vorticity gradients to become horizontally compact and then propagate into the thermocline. This contrasts with NIWs generated by tropical cyclones (TCs), which can rapidly propagate downward regardless of background ocean conditions. Here, we study the upper ocean response to midlatitude storms and TCs using a dynamical framework whose equations of motion are written in terms of vorticity and divergence rather than velocity vectors. We show that patterns of wind stress curl and convergence that are inherently linked to atmospheric convection necessarily generate NIWs that are horizontally compact and can induce substantial downward energy fluxes within the first inertial cycle after storm passage. The vorticity-divergence dynamical framework elucidates this because it allows us to account for spatial wind patterns even when solving motion linearly and for a single point in space. With this, we argue that the morphology of mesoscale convective systems allows them to drive downward propagation of NIWs in their wakes, whether ocean storms take the shape of a TC or a midlatitude storm.

How to cite: Brizuela, N. and D'Asaro, E.: Morphology of atmospheric convective systems facilitates rapid transmission of near-inertial energy into the ocean thermocline, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11271, https://doi.org/10.5194/egusphere-egu25-11271, 2025.

EGU25-11742 | Posters on site | OS1.9

Two-particle dispersion in the Gulf of Gabès using a high resolution nested ocean model  

Maher Bouzaiene, Milena Menna, A. Fehmi Dilmahamod, Damiano Delrosso, Simona Simoncelli, and Claudia Fratianni

Measuring relative dispersion in coastal ecosystems is important for both ocean health and society. Submesoscale dynamics interacting with mesoscale eddies influence mixing processes and phytoplankton blooms dispersion. Two-particle dispersion statistics over an initial spatial scale (0.7 - 1 km) are analysed in the Gulf of Gabès (central-southern Mediterranean Sea) using a high-resolution ocean model through a multiple nesting approach. The model is forced by ERA5 atmospheric fields, while the lateral boundary conditions and initial conditions are provided by daily fields from a Mediterranean Sea reanalysis. The analysis focuses on the turbulent fluid aspects of phytoplankton dispersion in coastal areas under bloom and non-bloom conditions. The results are presented in terms of kurtosis (normalized fourth moment of the pair separation distances), relative diffusivity (particles’ spreading velocity) and time scale-dependent pair separation rate (pair velocity scales normalized by separation distance). At the submesoscale (0.7 – 2km), the non-local exponential regime is absent in both bloom and non-bloom conditions, where the dispersion is locally driven by energetic submesoscale structures. For scales ranging 2-15 km, the two-particle statistics follow the theoretical Richardson regime, which is well detected in the case of a bloom. This regime implies the presence of an inverse energy cascade range where energy is transferred from small to large scales. The diffusive regime is absent for all scales and in both bloom and non-bloom conditions.

How to cite: Bouzaiene, M., Menna, M., Dilmahamod, A. F., Delrosso, D., Simoncelli, S., and Fratianni, C.: Two-particle dispersion in the Gulf of Gabès using a high resolution nested ocean model , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11742, https://doi.org/10.5194/egusphere-egu25-11742, 2025.

EGU25-12896 | Posters on site | OS1.9

Near surface bubble, gas and flow measurements during the Bubble Exchange in the Labrador Sea (BELS) cruise – early results 

Helen Czerski, Intesaaf Ashraf, Ian Brooks, and Steve Gunn

The bubbles formed by breaking waves are thought to play an important role in increasing gas transfer across the atmosphere-ocean surface during high wind conditions (>15 m/s).  However, real world data on near-surface bubbles with sufficient resolution in space, time and bubble size to understand exactly how the transfer mechanisms work is rare. In addition, there are almost no data showing the relationship between bubble size distributions and the local flow and gas saturation conditions, although data from the HiWinGS cruise suggests that these structures could be very important for gas transfer. The BELS project data was collected during five weeks in November/December 2023, and includes tracer-based gas flux measurements, physical oceanography, and ocean chemistry.  Hourly averaged wind speeds were 5-30 m/s, with maximum significant wave height of 11 m.  Here, we will present early results from the part of the project monitoring near-surface bubbles and their relationship to flow patterns and dissolved gas concentrations in the top five metres of the ocean. Data will be presented from a free-floating buoy carrying specialised bubble cameras at 1m and 3m, ADCPs and oxygen optodes. We will show measured bubble size distributions, and the spatial relationship of these bubbles to Langmuir circulation patterns and dissolved oxygen concentrations. We will also present an early analysis of the relationships between gas carried by both the water itself and the bubbles, and how this relates to the advection of these two gas reservoirs in the top few metres of the ocean.  

How to cite: Czerski, H., Ashraf, I., Brooks, I., and Gunn, S.: Near surface bubble, gas and flow measurements during the Bubble Exchange in the Labrador Sea (BELS) cruise – early results, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12896, https://doi.org/10.5194/egusphere-egu25-12896, 2025.

EGU25-13975 | Orals | OS1.9

Assessment of satellite-derived sea surface salinity using in-situ measurements in the Southeast Asia 

Kaushik Sasmal, Sumit Dandapat, Xingkun Xu, Pavel Tkalich, Bijoy Thompson, Rajesh Kumar, Kalli Furtado, and Hugh Zhang

Advances in satellite microwave remote sensing have demonstrated an unprecedented capability to observe global ocean sea surface salinity (SSS) from space since 2009. Satellite-based SSS observations provide a unique monitoring capability for the interfacial water exchanges between the atmosphere and the upper ocean, as well as salinity redistribution due to climate and global water cycle variability, and land-ocean interactions.

Satellite measurements of sea surface salinity (SSS) started in November 2009 with the Soil Moisture and Ocean Salinity (SMOS) mission launched by the European Space Agency (ESA). The Aquarius/SAC-D, launched in June 2011 by NASA and the Argentinean Space Agency (CONAE), was the first satellite mission designed to measure SSS. Meanwhile, the Soil Moisture Active and Passive (SMAP) was launched by NASA in January 2015, and it provides SSS as a derived product. SMAP is configured with a larger swath coverage, providing a higher spatial resolution (~40 km) than that (~100 km) in Aquarius.  

Satellite remote sensing of SSS encounters many challenges, such as contamination of microwave signals near coastal areas or dependance of SSS accuracy on the quality of temperature and wind speed measurements. As such, the satellite-derived SSS data needs to be validated against in-situ measurements.

Here we used in-situ measurements of salinity and temperature from ARGO data for three oceanic basins i.e., Bay of Bengal (BOB), South China Sea (SCS), and Western North Pacific Ocean (WNPAC). The ARGO data from Sep 2011 to Dec 2022 were utilized for analysis due to the consistency of the period with the available satellite-derived salinity data. The number of ARGO profiles varies significantly among these three oceanic basins with the largest profiles available in the WNPAC and the least number of profiles in the SCS.

ARGO SSS climatology, although available at a coarser resolution than the satellite-derived SSS, captured the spreading of the low salinity water in the BOB during Oct-Dec. This feature is consistent with the satellite-derived SSS spatial distribution. For the BOB, the agreement between ARGO and satellite SSS data is reasonably good with an RMSE of 0.58 psu. In comparison, the SCS and WNPAC achieve RMSE of 0.22 psu and 0.14 psu, respectively. It should be noted that the number of near-surface ARGO observations is much higher in the WNPAC (37,207) compared to that in the BOB (15,305) and in the SCS (9,722) from Sep 2011 to Dec 2022. The BOB reveals strong seasonality and the largest variation in SSS from ~25-35 psu. Whereas, the SCS and WNPAC recorded variations in the range ~32-35 psu. The SCS and WNPAC exhibit freshening and salinification in specific years. The monthly mean SSS from ARGO and satellite data are highly correlated and show consistent variation in salinity in all three oceanic basins. Therefore, the satellite-derived SSS data could provide great insight for understanding ocean dynamics, circulation, water cycle, and could be useful for validating ocean models.  

How to cite: Sasmal, K., Dandapat, S., Xu, X., Tkalich, P., Thompson, B., Kumar, R., Furtado, K., and Zhang, H.: Assessment of satellite-derived sea surface salinity using in-situ measurements in the Southeast Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13975, https://doi.org/10.5194/egusphere-egu25-13975, 2025.

EGU25-14006 | ECS | Posters on site | OS1.9

Relating surface signatures to modeled turbulence dynamics in open channel flow 

Boqi Tian, C. Chris Chickadel, and Ramsey R. Harcourt

In open channel flow (OCF), expressions and patterns at the water surface may represent underwater turbulent phenomena. In this study, we seek to connect the surface signatures with the turbulence beneath it through the prediction of the time and length scales of turbulent structures in second moment closure (SMC) models. In the simplest scenario, the unforced free surface OCF is driven by a uniform horizontal pressure gradient and the only source of turbulence is the bottom shear. Working with Neumann surface boundary conditions for turbulence quantities, the traditional ‘return-to-isotropy’ for turbulent kinetic energy (TKE) components is modified to decay – in the absence of local TKE production – to a specified anisotropy profile as a function of depth below the surface, rather than to isotropy. This gives rise to distinct vertical and horizontal length scales, formed from the TKE components and the turbulence decay timescale. It also results, through changes in the algebraic closure solution, in a modification of vertical diffusivity consistent with more ad-hoc proposals in other studies to address excessive flux predictions using depth-dependent damping functions. An examination of results from these model changes is presented for weak equilibrium k - ε SMC models. The weak equilibrium k - ε SMC model solves for turbulent second moments by combining prognostic equations for TKE (k) and dissipation (ε) with an algebraic model to obtain eddy viscosity and diffusivity. SMC predictions for TKE components, dissipation, and horizontal turbulent length scales at the free surface are compared with observations obtained in a tidally modulated river, as well as with published results from OCF lab experiments and direct numerical simulations.

How to cite: Tian, B., Chickadel, C. C., and Harcourt, R. R.: Relating surface signatures to modeled turbulence dynamics in open channel flow, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14006, https://doi.org/10.5194/egusphere-egu25-14006, 2025.

EGU25-14246 | ECS | Orals | OS1.9

Spatial Extent and Variability of Equatorial Deep-Cycle Turbulence in the Pacific Cold Tongue 

Jofia Joseph, Anna-Lena Deppenmeier, Daniel B Whitt, Frank O. Bryan, William S. Kessler, LuAnne Thompson, and Elizabeth Thompson

Deep-cycle turbulence (DCT) is a critical mechanism driving vertical mixing in the equatorial Pacific, playing a pivotal role in modulating heat and nutrient transport within the Pacific Cold Tongue. DCT arises from diurnal variations in stratification and shear, leading to turbulence that extends below the mixed layer. DCT generates significant heat fluxes into the ocean, averaging O(100 W m⁻²) and peaking at ~1000 W m⁻² during nighttime bursts, which contribute to surface cooling and thermocline warming. This process helps maintain cool sea surface temperatures (SSTs) and net heat uptake in the eastern Pacific Cold Tongue, influencing SST dynamics on interannual, seasonal, and subseasonal timescales. These dynamics significantly impact air-sea interactions, as DCT regulates the exchange of heat, momentum, and gases, which play a critical role in shaping tropical weather patterns and global climate variability.

 Despite previous studies elucidating the temporal variability and mechanisms of DCT on the equator, its spatial extent and variability across the equatorial Pacific remain poorly understood due to limited observations.

This study examines the spatial and temporal variability of DCT in the Cold Tongue region using Large Eddy Simulations (LES), which explicitly resolve sub-grid-scale mixing processes. The LES cover a meridional array of seven latitudinal points (1.5°S to 4.5°N) along 140°W and a zonal array spanning the central to eastern Pacific (165°W to 100°W) along the equator during contrasting periods influenced by Tropical Instability Waves (TIWs) and the seasonal cycle. Complementary hourly turbulence outputs from a 20-year MITgcm simulation are utilized to examine parameterized turbulence at these locations, enabling a comparison between sub-grid-resolved turbulence in LES and parameterized turbulence in the MITgcm.

Diurnal composite analyses reveal that parameterized turbulence in the MITgcm overestimates diapycnal heat flux compared to LES-resolved turbulence. The relationship between Richardson number, shear, stratification, and mixing is explored to understand the transition from the marginally stable regime near the equator (0°N, 140°W) to more stable conditions farther from the equator. Preliminary findings illustrate spatial asymmetries in mixing-related variables, with notable differences between the northern and southern hemispheres. These results highlight the need for further exploration of hemispheric asymmetries and their implications for mixing processes.

This study sets the stage for a comprehensive evaluation of mixing representation in the Pacific Cold Tongue region across diurnal to longer timescales, leveraging a hierarchy of model outputs, from LES to regional and global high-resolution simulations.

How to cite: Joseph, J., Deppenmeier, A.-L., B Whitt, D., O. Bryan, F., S. Kessler, W., Thompson, L., and Thompson, E.: Spatial Extent and Variability of Equatorial Deep-Cycle Turbulence in the Pacific Cold Tongue, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14246, https://doi.org/10.5194/egusphere-egu25-14246, 2025.

EGU25-14275 | ECS | Posters on site | OS1.9

Ocean-atmosphere coupling regimes in the tropical area 

Ruyan Chen

Tropical ocean-atmosphere coupling plays a pivotal role in regulating the global climate system. Variability and mechanisms of the coupling exhibit significant regional differences due to variations in the background states and thermodynamic processes across the tropical basins. While previous studies mostly focused on the specific time scales and localized regions, a broader view of the tropical air-sea coupling “picture” remains incomplete. This project first utilizes an energy balance model of the coupled ocean-atmosphere system to diagnose the coupling characteristics for each tropical grid point across timescales through the “heat flux—sea surface temperature” relationship. Subsequently, a clustering algorithm is used to classify spatial differences into distinct coupling regimes. Finally, decomposition of the flux calculation is applied to identify critical variables and processes underlying each regime. This approach progressively reveals the mechanisms behind the regional differences in tropical ocean-atmosphere coupling features. Our findings also highlight that current high-resolution climate models still face challenges in accurately reproducing the coupling characteristics of some regimes, which would further limit the accuracy of climate simulation and prediction.

How to cite: Chen, R.: Ocean-atmosphere coupling regimes in the tropical area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14275, https://doi.org/10.5194/egusphere-egu25-14275, 2025.

EGU25-14613 | ECS | Orals | OS1.9

Resolving Langmuir Turbulence in a Coupled Wind-Wave System 

Yankun Liu and Qing Li

Langmuir turbulence, arising from the nonlinear interaction between surface gravity waves and wind-driven shear currents, significantly contributes to ocean mixing and the air-sea transfer of mass, momentum, and energy. Previous studies have either prescribed surface wind stress in single-phase flow simulations or left surface waves indeterminate in two-phase flow simulations. To better understand the generation and evolution of Langmuir turbulence, and to quantify the momentum and energy transfer across the air-sea interface, a series of two-phase wave-resolved direct numerical simulations are conducted across various Langmuir numbers. In these simulations, fully developed pressure gradient-driven turbulence on the air side is acted upon prescribed surface gravity waves. The results reveal characteristic structures of Langmuir cells at varying scales, including pairs of counter-rotating vortices and elongated streamwise streaks on the water surface. By decomposing flow velocity into mean current, wave orbital motion, and turbulence fluctuation, the impact of wave-induced phase-dependent strain on underlying turbulence and the enhancement of streamwise vorticity are analyzed in detail. Additionally, the momentum flux across the air-sea interface is calculated and its transfer mechanism is discussed, providing insights for parameterization in climate models.

How to cite: Liu, Y. and Li, Q.: Resolving Langmuir Turbulence in a Coupled Wind-Wave System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14613, https://doi.org/10.5194/egusphere-egu25-14613, 2025.

EGU25-16290 | ECS | Orals | OS1.9

The role of small-scale ocean mixing processes in regional sea surface temperature 

Audrey Delpech and Anne-Marie Tréguier
The advances of numerical performances over the last decades have opened the way for km-scale climate modelling, which not only improve the representation of the state of the climate globally, but also allows to downscale climate information at a local scale where climate adaptation strategies are decided. In this context, it is interesting to evaluate the performance of such models at a regional scale.
In this study, we evaluate the capabilities of km-scale coupled climate simulations delivered by the EERIE (European Eddy-RIch Earth system models) project on the North Atlantic coastal shelfs in the representation of sea surface temperature and air surface temperature. Our findings suggest that eddy-rich coupled simulations can alleviate some of the large-scale biases found at coarser resolution but at the same time points out towards persistent model biases at local-scale due to unresolved or poorly parameterized mixing processes. We subsequently evaluate the nature and impact of unresolved oceanic mixing processes in climate models on the sea surface temperature mean state, variability and extremes.
 

How to cite: Delpech, A. and Tréguier, A.-M.: The role of small-scale ocean mixing processes in regional sea surface temperature, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16290, https://doi.org/10.5194/egusphere-egu25-16290, 2025.

EGU25-16435 | Posters on site | OS1.9

Three-dimensional Ocean Surface Layer Response to Rain, Wind Bursts and Diurnal Heating 

Lars Umlauf, Mira Schmitt, Knut Klingbeil, and Radomyra Shevchenko

In the tropical ocean, diurnal heating and the formation of atmospheric convection cells associated with local precipitation events, cold pools and wind bursts, have been shown to impact air-sea exchange and the structure of the ocean surface layer. Here, we use a high-resolution regional ocean model, forced by an atmospheric Large Eddy Simulation (LES) that explicitly resolves these processes in a realistic scenario in the tropical north-east Atlantic Ocean, to study their impact on the ocean surface layer and parameterized air-sea fluxes.  We find that in our study area, located in the trade wind zone, the oceanic heat loss is, unexpectedly, reduced in the presence of cold pools by on average 30 W m-2 due to the higher air humidity, weaker mean winds, and increased cloud cover. Our results also show that the total non-solar heat flux is dominated by the diurnal cycle of the trade winds, rather than by diurnal heating. In the ocean surface layer, local wind bursts, rain layers, and cloud shading induce a strong lateral variability of Diurnal Warm Layers (DWLs), questioning the local applicability of available DWL bulk parameterizations. From a series of numerical tracer experiments, we identify a new shear-dispersion mechanism, induced by the diurnal jet, that is reflected in an extreme anisotropy of horizontal dispersion with diffusivities of order 10-100 m2 s-1. These findings are likely relevant also in other regions in the trade wind zone.

How to cite: Umlauf, L., Schmitt, M., Klingbeil, K., and Shevchenko, R.: Three-dimensional Ocean Surface Layer Response to Rain, Wind Bursts and Diurnal Heating, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16435, https://doi.org/10.5194/egusphere-egu25-16435, 2025.

EGU25-17338 | ECS | Posters on site | OS1.9

Leveraging automatic differentiation for calibrating vertical mixing parameterizations  

Gabriel Mouttapa, Julien Le Sommer, Emmanuel Cosme, Anne Durif, Bruno Deremble, Alexandre Legay, and Gregory LeClaire Wagner

Fine-scale turbulence in the upper ocean boundary layer (OSBL) governs ocean surface stratification, and vertical exchanges of heat, momentum and matter in the ocean, which are key in the response of the oceans to changing environmental conditions. However, these turbulent processes are not explicitly represented in ocean models and their parameterization remains a significant source of uncertainty in climate models and operational prediction systems. Increasingly, systematically leveraging diverse data sources is becoming standard practice for developing and assessing OSBL parameterizations. Over the past years, data-driven automated procedures have for instance been used for calibrating the parameters of physics-based models, for developing parameterizations embedding ML components, and for proposing pure ML-based parameterizations of OSBL processes. 

This study explores the advantages of the emerging paradigm of differentiable programming for the calibration of OSBL parameterizations . We developed a benchmark tool, Tunax, implemented in JAX, a differentiable framework for Python. This benchmark includes a fully differentiable single-column model with various possible OSBL parameterizations, alongside a calibration module which tunes the coefficients of these parameterizations against a reference database. The differentiability of the model enables the application of variational techniques for parameter calibration. The reference database is a collection of  Large Eddy Simulations (LES) covering a range of typical physical conditions.

Here, we focus on the k-ε closure (Umlauf and Burchard, 2005), widely used in global ocean circulation models, and calibrate its parameters using a dataset of LES. These simulations have been designed to model the evolution of the oceanic mixed layer under various surface conditions (wind, heat fluxes and rotation). This work highlights the potential of differentiable calibration techniques to address uncertainties inherent to turbulence closures by enabling more flexible and data-informed parameterizations. Although this approach does not yet consistently outperform traditional calibration methods, it provides a promising avenue for reducing model biases associated with sub-grid scale parameterizations.

 

How to cite: Mouttapa, G., Le Sommer, J., Cosme, E., Durif, A., Deremble, B., Legay, A., and LeClaire Wagner, G.: Leveraging automatic differentiation for calibrating vertical mixing parameterizations , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17338, https://doi.org/10.5194/egusphere-egu25-17338, 2025.

There is a large number of mesoscale eddies in the ocean, which play a significant role in ocean circulation and climate change. Recent studies have indicated that mesoscale eddy activity in most regions will become more active under the influence of global warming, but changes in the characteristics of these eddies remain unclear. This study utilizes satellite observational data and reanalysis datasets, focusing on the Agulhas Leakage region, which is rich in mesoscale eddies and has become a research hotspot due to its unique geographical position. The study finds that the changes in the characteristics of anticyclonic eddies in this region are related to variations in the Atlantic Meridional Overturning Circulation (AMOC). Some of the eddy characteristics exhibit dynamic adjustments, with a turning point around 2005, which may be associated with sea temperature differences between the South Indian Ocean and the South Atlantic, as well as changes in the local wind field. The findings of this study will provide insights for future predictions of AMOC variability.

How to cite: Wei, L. and Wang, C.: Why do warm anticyclonic eddies in the Agulhas Leakage undergo dynamic adjustments?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17915, https://doi.org/10.5194/egusphere-egu25-17915, 2025.

EGU25-17994 | Posters on site | OS1.9

On the way towards understanding the effect of sea-water surfactants on gas transfer velocity  

Jacek Piskozub, Violetta Drozdowska, Iwona Wróbel-Niedźwiecka, Karol Kuliński, Przemysław Makuch, Fernando Aguado Gonzalo, Piotr Markuszewski, and Małgorzata Kitowska

Gas flux across the sea surface is proportional to the difference of partial pressure between the sea-water and the overlying atmosphere and also to a parameter called gas transfer velocity k, a measure of the, the measure of efficiency of the gas exchange. Although it depends mostly in in-water and atmospheric turbulence, the usual way to parametrize it is by the wind speed, the source of the turbulence which has the advantage of being easily available from ship base measurements and reanalyses. Unfortunately, measured values of gas transfer velocity at a given wind speed have a large spread in values. It has been long suspected that the coverage of the sea surface with variable amounts of surface-active substances (or surfactants). It has been shown that surfactants may decrease the CO2 air-sea exchange by up to 50%. However the labour intensive methods used for surfactant study make it impossible to collect enough data to map the surfactant coverage or even create a gas transfer velocity parametrization involving a measure of surfactant activity. This is why we decided check the possibility of using optical fluorescence as a proxy of surfactant activity.

 

We are in the third year of a 4-year research grant funded by the Polish National Science Centre, NCN (grant number 2021/41/B/ST10/00946). Our group has previously showed that fluorescence parameters allow estimation the surfactant enrichment of the surface microlayer, as well as types and origin of fluorescent organic matter involved. In order to study their possible usefulness in improving the parametrization of the gas transfer velocity k, we measure from the research ship of the Institute, R/V Oceania, all the variables needed for its calculation, namely CO2 partial pressure both in water (PiCCARO G2101-i) and in air (Licor 7200, semiclose path with heated tube and Licor 7500, open path) as well as vertical flux of this trace gas (with the GiLL WindMaster and WindMaster Pro for 3D air movement needed for eddy correlation) as well as meteorological conditions. The data are used to calculate gas transfer velocity values which are compared to ones calculated literature from parametrization functions. The differences between the two, together with the surfactant fluorescence parameters are be used to test the hypothesis that surfactants are main reason for the “noisiness” of k measurement results and hopefully to improve the k parametrization by adding a surfactant related variable to the wind speed which at present is the sole independent variable of most parametrizations.

 

After 3 years of the project we have data from six Baltic cruises and to three Atlantic ones, of which 2/3 have been already analysed. The poster will present the early results of the project and show progress towards the main goal of the research: finding a reliable optical proxy for surfactant to be used in gas transfer velocity parametrization.

 

How to cite: Piskozub, J., Drozdowska, V., Wróbel-Niedźwiecka, I., Kuliński, K., Makuch, P., Aguado Gonzalo, F., Markuszewski, P., and Kitowska, M.: On the way towards understanding the effect of sea-water surfactants on gas transfer velocity , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17994, https://doi.org/10.5194/egusphere-egu25-17994, 2025.

EGU25-18385 | Posters on site | OS1.9

Characterizing Wind-Generated Waves Using a Color Imaging Slope Gauge (CISG) 

Julián Marcelo Morales Meabe and Martin Gade

Wind-driven waves play a pivotal role in air-sea interactions, influencing processes such as energy dissipation and turbulent mixing. In this study, we employ a Color Imaging Slope Gauge (CISG) to measure surface wave slopes with high spatiotemporal resolution in the linear wind-wave tank at the University of Hamburg. Complementary techniques include a Laser Doppler Velocimetry (LDV) system for point-wise, two-dimensional velocity measurements; a wire gauge and a laser slope gauge for point measurements of wave height and slope, respectively; and an infrared radiometer capable of capturing surface temperature variations. These tools enable the investigation of thermal gradients and their correlation with wave dynamics. 

This research aims to examine the statistical properties of wind-generated waves and reconstruct their three-dimensional profiles to better understand their physical and kinematic behavior. A particular focus is placed on the mechanisms of microbreaking, which contribute to energy dissipation and capillary wave generation. To explore surface tension effects, surfactants are introduced to dampen gravity-capillary waves, allowing for detailed investigations of energy fluxes between wave regimes and the suppression of high-frequency wave components. 

The combined use of slope imaging, velocity measurements, and thermal detection enhances our ability to study the interplay of different physical processes at the air-sea interface. This work lays the groundwork for further investigations of wave behavior under varying environmental conditions. In particular, the findings of this study will provide critical insights into the small-scale processes driving wave dynamics and contribute to improved parameterizations for wave and climate models. 

 

How to cite: Morales Meabe, J. M. and Gade, M.: Characterizing Wind-Generated Waves Using a Color Imaging Slope Gauge (CISG), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18385, https://doi.org/10.5194/egusphere-egu25-18385, 2025.

EGU25-18410 | ECS | Posters on site | OS1.9

Impact of Submesoscale Dynamics and Turbulent Mixing on the Senegalo-Mauritanian Upwelling System 

Marco Schulz, Florian Schütte, Marcus Dengler, and Peter Brandt

Based on a combination of over 20 years of satellite data with extensive in situ measurements from previous research expeditions, an initial step is taken to differentiate the impact of submesoscale processes and turbulent mixing on the Eastern Boundary Upwelling System (EBUS) off Senegal and Mauritania. EBUS are an essential part of the global carbon cycle and are of central importance for the sustainability of economic and food resources. In the tropical Senegalo-Mauritanian EBUS, sea surface temperatures and net primary production exhibits a pronounced seasonal cycle. It is characterized by coastal upwelling in late boreal winter and an abrupt end in late boreal spring with the onset and strengthening of the poleward Mauritania Current. At first glance, the temporal and spatial development follows the annual cycle of the wind stress curl. However, a closer look reveals a more complex picture with a pronounced spatiotemporal heterogeneity, characterized by the influence of (sub)mesoscale eddies and (non-linear) internal tides.

Integrated cross-shelf tidal energy fluxes towards the coast are locally estimated from observations of multiple short-term moorings. Such fluxes should result in increased mixing near the coast, which is in fact supported by assessment of over 800 microstructure turbulence observations. (Internal) tides are known to drive much of the mixing and vertical exchange on a rather narrow coastal strip. Besides, lateral density gradients which were induced by upwelling are regularly subject to conditions favorable for frontogenesis. The associated secondary circulations can induce strong vertical motions and instabilities and export chlorophyll offshore through frontal jets. A snapshot of ship-based measurements of turbulent kinetic energy dissipation rates indicates an order of magnitude larger dissipation on the cold, dense side of the front, whereby surface heat flux is known to play a crucial role. Spatially high-resolution measurements of sea level deflections from the SWOT satellite show considerable variability on scales smaller than 20 km, but the applicability for balanced motions is hampered by the regular occurrence of solitary waves and topographic effects. Given the significance of these observed small-scale processes for the redistribution and alteration in net primary production and expected general changes of submesoscale processes (e.g. due to changing mixed layer depths in the context of global warming), a more precise quantification of their net impact is essential.

Outlook: An interdisciplinary expedition in spring 2025 will supplement the existing data and will use an adaptive sampling strategy, e.g. to tackle the mutual interaction of tides and internal waves with density fronts. Observed tidal fluxes will be interpreted in the context of a high-resolution 3D baroclinic tidal model. These, as well as the work presented, serve as preparatory work for the unprecedented year-round “FUTURO” campaign, which aims to provide a detailed picture of the annual cycle for this important EBUS.

How to cite: Schulz, M., Schütte, F., Dengler, M., and Brandt, P.: Impact of Submesoscale Dynamics and Turbulent Mixing on the Senegalo-Mauritanian Upwelling System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18410, https://doi.org/10.5194/egusphere-egu25-18410, 2025.

EGU25-18874 | ECS | Orals | OS1.9

Parameterizing Entrainment Induced by Submesoscale Eddies 

Anna Lo Piccolo, Baylor Fox-Kemper, Genevieve Jay Brett, Tomás L. Chor, Jacob O. Wenegrat, and Zhihua Zheng

Submesoscale eddies in the ocean surface layer are known to cause the restratification of the mixed-layer by converting the potential energy stored in the outcropping isopycnals into kinetic energy. Evidence of entrainment and subduction is found associated to submesoscale eddies, suggesting their importance for the biogeochemistry of the global ocean. Submesoscale eddies cannot be resolved in today’s global ocean models and existing parameterizations for baroclinic mixed-layer instabilities (MLIs), which are proven to reproduce the restratification quite well, are not capable to fully capture the vertical exchange of passive tracers across the mixed-layer. In this study, high resolution numerical simulations show the inadequacy of the MLI parameterization of Fox-Kemper, Ferrari, and Hallberg (2008, ‘FFH’) for the entrainment problem. A method for tracer inversion is then used to gain insights on the tracer transport in order to inform the parameterization. Parameter dependence is explored by considering different ocean initial conditions. Finally, the results show that a diffusive (symmetric) component needs to be included to the streamfunction (anti-symmetric) to entirely represent the transport induced by MLIs: the parameterization for entrainment is an update to the FFH parameterization.

How to cite: Lo Piccolo, A., Fox-Kemper, B., Brett, G. J., Chor, T. L., Wenegrat, J. O., and Zheng, Z.: Parameterizing Entrainment Induced by Submesoscale Eddies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18874, https://doi.org/10.5194/egusphere-egu25-18874, 2025.

In this study, we identify regions across the Mexican Pacific waters where the high-frequency variability of daily sea surface temperature (SST) is diminishing and those in which the warm upper-layer thickness increases, analyzing changes in the upper layers' thermal structure along the tropical Pacific Ocean and their relationship with the variability of the upper-layer thickness in the so-called Warm Pool of the Mexican Pacific. Our results reveal a clear, direct relationship between the thickness increase of the warm, upper-ocean layer and the reduction of the high-frequency SST variability, which are related to the long-term trend of SST and ENSO variability. The implications are enormous since extreme positive SST anomalies and increasing warm, upper-layer thickness are optimal oceanic conditions for forthcoming hurricane development and intensification.

How to cite: Martinez-Lopez, B.: Otis intensification and its relationship to El Niño and Climate Change in the eastern Pacific Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20498, https://doi.org/10.5194/egusphere-egu25-20498, 2025.

Sea spray-mediated heat flux plays an important role in air-sea heat transfer. Heat flux integrated over droplet size spectrum can well simulate total heat flux induced by sea spray droplets. Previously, a fast algorithm of spray-flux assuming single-radius droplets (A15) was widely used since the full-size spectrum integral is computationally expensive. Based on the Gaussian Quadrature (GQ) method, a new fast algorithm (SPRAY-GQ) of sea spray-mediated heat flux is derived. The performance of SPRAY-GQ is evaluated by comparing heat fluxes with those estimated from the widely-used A15. The new algorithm shows a better agreement with the original spectrum integral. To further evaluate the numerical errors of A15 and SPRAY-GQ, the two algorithms are implemented into a coupled CFSv2.0-WW3 system, and a series of 56-day simulations in summer and winter are conducted and compared. The comparisons with satellite measurements and reanalysis data show that the SPRAY-GQ algorithm could lead to more reasonable simulation than the A15 algorithm by modifying air-sea heat flux. For experiments based on SPRAY-GQ, the sea surface temperature at mid-high latitudes of both hemispheres, particularly in summer, is significantly improved compared with the experiments based on A15. The simulation of 10-m wind speed and significant wave height at mid-low latitudes of the Northern Hemisphere after the first two weeks is improved as well. These improvements are due to the reduced numerical errors. The computational time of SPRAY-GQ is about the same as that of A15. Therefore, the newly-developed SPRAY-GQ algorithm has a potential to be used for calculation of spray-mediated heat flux in coupled models.

How to cite: Shi, R. and Xu, F.: Accelerated Estimation of Sea Spray-Mediated Heat Flux Using Gaussian Quadrature, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21343, https://doi.org/10.5194/egusphere-egu25-21343, 2025.

Subduction in the Northwestern Pacific produces North Pacific Subtropical Mode Water (NPSTMW) and constitutes an important branch of the Subtropical Cell. Subduction in the Northwestern Pacific occurs typically during March and April. Based on ocean and atmosphere reanalysis products, the subduction of the NPSTMW is calculated using an Eulerian method. It is found that the averaged subduction time of NPSTMW, weighted by the daily detrainment rate, can vary more than two weeks every year. A composite analysis of the early and the late subduction shows that the subduction time is mostly affected by the strength of the surface zonal wind in the subduction region, which is found to be closely related to the strength and meridional shift of the Aleutian Low in March and April. When the Aleutian Low is stronger (weaker) or shifts southward (northward) in March and April, the surface westerly wind in the subduction region is stronger (weaker), which delays (expedites) the shoaling of the mixed layer and leads to a later (earlier) subduction of the NPSTMW. 

How to cite: Zhang, X. and Xu, F.: The Interannual Variability of North Pacific Subtropical Mode Water Subduction Time Modulated by Aleutian Low, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21345, https://doi.org/10.5194/egusphere-egu25-21345, 2025.

EGU25-363 | ECS | Posters on site | AS4.10

Climate, Air Quality, and Health Inequities in Europe: Evidence-Based Policy Implications 

Muhammad Shafeeque, Frank Oliver Glöckner, Sonja Hänzelmann, Rajini Nagrani, Nour Naaouf, Christoph Buck, and Wolfgang Ahrens

Climate change and air pollution are interrelated challenges with profound implications for public health, equity, and resilience in Europe. This study investigates relationships between climate, air quality, and health across European countries (2005-2020) as part of the DataNord/Healthy Planet project. Using reanalysis, remote sensing, and observed datasets (ERA5-Land, MERRA-2, Sentinel-5P, MODIS, OMI, EDGAR v6, EEA health assessments), we employed machine learning and statistical analysis to identify significant warming trends (temperature anomaly: +0.90°C), regional variability in precipitation (e.g., Cyprus: -28% to +15%) and other variables. Air quality improvements varied regionally, e.g., NO2 and PM2.5 concentrations decreased >50% in Sweden, while NO2 increased in Cyprus (+17%) and O3 in Belgium (+21%), reflecting differences in policy effectiveness and local conditions. Context-specific correlations between climate and pollution (-0.86 to 0.79) reflected local variations in meteorological and emission factors. Health assessments revealed substantial reductions in premature mortality, especially from PM2.5 (Estonia: -93%) and NO2 (Germany: -53%, Spain: -58%). Our findings emphasize the need for integrated climate-air quality policies targeting regional challenges. We recommend implementing region-specific emission reduction targets based on local vulnerability indices, supported by enhanced monitoring networks and targeted interventions in areas showing slower progress.

How to cite: Shafeeque, M., Glöckner, F. O., Hänzelmann, S., Nagrani, R., Naaouf, N., Buck, C., and Ahrens, W.: Climate, Air Quality, and Health Inequities in Europe: Evidence-Based Policy Implications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-363, https://doi.org/10.5194/egusphere-egu25-363, 2025.

EGU25-560 | ECS | Posters on site | AS4.10

Impact of nitrogen dioxide pollution on paediatric asthma and premature mortality in South Africa 

Terrence Koena Sepuru, Eloise A. Marais, Mogesh Naidoo, Karn Vohra, Eleanor Gershenson-Smith, and Rebecca M. Garland

Nitrogen dioxide (NO2), a priority pollutant and an indicator for Traffic-Related Air Pollution (TRAP), poses significant health risks including childhood-onset asthma and premature mortality. Routine measurements of NO2 are severely limited in Pretoria and Johannesburg, two large cities in the industrialised Highveld of South Africa that experience severe air pollution due to road traffic. We use tropospheric columns of NO2 observed with the TROPOMI instrument for 2019 and simulated NO2 vertical profiles for the same year from the very high spatial resolution (~6 km) CAMx model driven with a locally developed emissions inventory to estimate ground-level NO2. Near traffic-roadside ground stations, yearly averaged satellite-derived NO2 ranges from 9 to 68 µg/m³, far in excess of the threshold for harm. Satellite-derived values agree with ground stations where sampling conditions are consistent, but validation is limited to a few sites. Underway is the use of the satellite-derived NO2 to attribute asthma incidences and premature mortality to exposure to NO2 and TRAP using state-of-knowledge exposure-response coefficients and Global Burden of Disease baseline rates of mortality and asthma incidences to motivate action to address severe air pollution in the industrialised Highveld.

Keywords

TRAP, Health Impact, satellite-derived, mortality burden, asthma, anthropogenic emissions, South Africa

How to cite: Sepuru, T. K., Marais, E. A., Naidoo, M., Vohra, K., Gershenson-Smith, E., and Garland, R. M.: Impact of nitrogen dioxide pollution on paediatric asthma and premature mortality in South Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-560, https://doi.org/10.5194/egusphere-egu25-560, 2025.

Introduction

Historically, intense underground mining for precious metals was the backbone of the South African economy for many decades. However, due to changing rent value of the targeted material and a shift in focus of the core economic activities, a number of small legacy mining towns are scattered across South Africa. 

In this project, PM2.5 particulates were sampled at two points in Welkom. A residential area and the industrial area, 5.8 Km South of the residential site. A comparison for their total PM2.5, BC, UV-PM and trace elemental composition, sources and geographical origins was performed. The main objective of the study was to determine the air quality in a legacy mining town where past activities, more recent developments and spatial priorities contribute to the sources and matrix of the air pollutants.

Methods

Sampling was performed by gravimetric methods, with PM2.5 and the constituent elements analysed by XRF. The source apportionment and back trajectory transport was performed on EPA-PMF and HYSPLIT models respectively. A total of 75 samples were collected with 5 duplicates per site. Statistical analysis included descriptive statistics, Spearman’s Rank correlation and Kruskal-Wallis test for seasonality.

Results

The annual mean PM2.5 level for the 12-month study period was 14.7 µg.m-3 (11.6 – 66) at the Industrial area and 6.34 µg.m-3 (6.34 – 23.4) at the Residential Site. The daily PM2.5 WHO guidelines (15 µg.m-3) and the daily PM2.5 South African NAAQS (40 µg.m-3) were exceeded on 27 and 5 days of the 75 days, respectively, at the industrial and residential sites. The sum of the trace elements per 12-month period was 2.3 µg.m-3 and 1.5 µg.m-3 and these constitute 12.4% and 10% of the total PM2.5 per year. Of interest is that Cl and K were present at both sites, Mn was present at the residential site and P was present at the industrial only. Although 26% of wind trajectories are from the Westerly direction, the highest recorded particulates are from the Northerly direction with 19% of wind trajectories. The highest three recordings for PM2.5 for the industrial site was 66.1, 61 and 56 µg.m-3 on the 23 August, 6 June and 12 July 2022 respectively.  From the NNE and Easterly directions. At the Industrial site, the highest average concentration (19.9 µg.m-3) recorded for a cluster was from the Northern direction over 13 days despite the cluster from the easterly direction recording 30 days (15.2 µg.m-3).

Conclusion

New spatial development priorities such as rezoning for industrial activities that are currently upwind of the residential sites present new air quality challenges to legacy ‘extractional’ towns such as Welkom in South Africa.

How to cite: Howlett-Downing, C. and Wichmann, J.: A comparative air quality and spatial planning study between two sites in a legacy mining town, Welkom, South Africa 2022-2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-798, https://doi.org/10.5194/egusphere-egu25-798, 2025.

EGU25-1218 | ECS | Orals | AS4.10

Breaking siloes of decision making for effective and systematic air quality solutions 

Nicole Cowell, Aoife Kirk, Roddy Weller, and Audrey de Nazelle

Air pollution is one the great challenges facing urban environments today, with 99% of the global population living in areas where air pollution concentrations are deemed “unsafe” according to the WHO air quality guidelines. Air pollution is also a typically wicked problem. We know there are inequities in exposure to air pollution and the resources available to address it; a heterogeneous nature to the sources and dispersion of pollution; and an array of solutions available to stakeholders. There are synergies between air quality solutions and actions for climate, health, equity and social wellbeing, yet siloed thinking in decision-making is limiting the outcomes of air pollution action. Systems approaches offer opportunities to overcome siloed thinking.

In collaboration with the World Economic Forum, we used structured decision-making as a novel engagement tool to gain systems insights into the synergies, barriers and opportunities facing stakeholders. We invited a diverse array of stakeholders from across urban systems to collaborate in a problem solving workshop, in which we adapted the structured decision making process for systems insights into urban air quality actions. The aim of the workshop was to understand the synergies and conflicts between stakeholders, and to identify the actions that stakeholders believe are feasible and provide co-benefits for climate, health and social wellbeing.

With 24 participants from 15 countries, we gathered the insights from NGOs, Academia, Industry and Policy from sectors such as transport, health, environment and technology. The group agreed on common goals that drive their work: “human health and well-being”, "equity" and "planetary health and climate". In response to these, they identified  over 100 solutions and highlighted the importance of transport and data related solutions, including air quality monitoring , modelling and transparency. The perceived feasibility of transport solutions was varied, however despite this “public transport” and “climate and health promoting transport” were recommended as some of the  top co-created actions by stakeholders. Key barriers to action included lack of data (access, quality and awareness), challenges of siloed thinking and collaboration and misinformation and disinformation.  There was a call from stakeholders for enhanced cross collaboration and systems approaches, but a lack of suggestions of how to practically implement this.    

The process of identifying and agreeing on common goals and co-creating corresponding solutions can help break siloes of decision making and help promote optimal systems-based solutions. There is a clear need for further understanding into how we integrate systems thinking into real world decision making, especially in low and middle income regions where the application of systems thinking is currently understudied.     

How to cite: Cowell, N., Kirk, A., Weller, R., and de Nazelle, A.: Breaking siloes of decision making for effective and systematic air quality solutions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1218, https://doi.org/10.5194/egusphere-egu25-1218, 2025.

EGU25-2439 | Posters on site | AS4.10

Mitigating air pollution benefits multiple sustainable development goals in China 

Yi Zhou, Xiuming Zhang, Chuanzhen Zhang, Binhui Chen, and Baojing Gu

Achieving the United nations 2030 Sustainable Development Goals (SDGs) remains a significant challenge, necessitating urgent and prioritized strategies. Among the various challenges, air pollution continues to pose one of the most substantial threats to the SDGs due to its widespread adverse effects on human health and ecosystems. However, the connections between air pollution and the SDGs have often been overlooked. This study reveals that out of the 169 SDG targets, 71 are adversely impacted by air pollution, while only 6 show potential positive effects. In China, two major atmospheric nitrogen pollutants, ammonia and nitrogen oxides, resulted in an economic loss of 400 billion United States Dollar (USD) in 2020, which could be reduced by 33% and 34% by 2030, respectively. It would enhance the progress towards SDGs in China by 14%, directly contributing to the achievement of SDGs 1 to 6 and 11 to 15. This improvement is estimated to yield overall benefits totaling 119 billion USD, exceeded the total implementation cost of 82 billion USD with ammonia as the preferential mitigation target. This study underscores the importance of robust scientific evidence in integrated policies aimed at aligning improvements in environmental quality with the priorities of sustainable development.

How to cite: Zhou, Y., Zhang, X., Zhang, C., Chen, B., and Gu, B.: Mitigating air pollution benefits multiple sustainable development goals in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2439, https://doi.org/10.5194/egusphere-egu25-2439, 2025.

EGU25-2884 | Posters on site | AS4.10

Health gains from particulate air pollution controls in China 

Aristeidis K. Georgoulias, Jos Lelieveld, Klaus Klingmüller, Dimitris Akritidis, Andrea Pozzer, Georgia Alexandri, Muhammad Bilal, Yafang Cheng, Hang Su, and Prodromos Zanis

Long-term exposure to elevated PM2.5 concentrations (fine particulate matter with a diameter smaller than 2.5 micrometers) poses a significant human health risk, contributing to excess mortality. Global estimates suggest that approximately 4–9 million excess deaths annually are attributable to PM2.5, with China accounting for about one-third of these fatalities. Since the start of the 21st century, China has undergone exceptional industrialization and urbanization, resulting in hundreds of millions of urban residents being exposed to poor air quality.  Recognizing the severity of the issue, Chinese authorities began implementing a series of successive control measures in 2006 to address unprecedented levels of atmospheric pollution. The research presented here, based on satellite observations and a combination of novel trend and mortality analysis methods, highlights the significant achievements of Chinese policies in mitigating the sharp rise in PM2.5 levels. Our results indicate that the reduction of PM2.5 at the levels of 2018–2019 (pre-COVID) prevented more than one million excess deaths annually and avoided an average reduction in life expectancy of over one year. We suggest that maintaining emission reductions at the current rate could drastically diminish the PM2.5-related health burden within the next two decades.

How to cite: Georgoulias, A. K., Lelieveld, J., Klingmüller, K., Akritidis, D., Pozzer, A., Alexandri, G., Bilal, M., Cheng, Y., Su, H., and Zanis, P.: Health gains from particulate air pollution controls in China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2884, https://doi.org/10.5194/egusphere-egu25-2884, 2025.

EGU25-3541 | ECS | Posters on site | AS4.10

Investigating drivers of recent reductions in PM2.5 concentrations across the UK 

Daniel. J Bryant, Alastair. C Lewis, and Sarah. J Moller

Exposure to particulate matter less than 2.5 micrometres in diameter (PM2.5) is the leading environmental risk factor for the global burden of disease and is associated with tens of thousands of deaths in the UK each year. Across the UK, legal compliance and progress towards the PM2.5 targets set out in the Environment Act, are measured using a network of fixed monitoring sites as part of the Automated Urban and Rual Network (AURN) across the country.

Over the last two decades, significant progress has been made in the reduction of PM2.5 concentrations across the UK. However, larger than expected decreases in PM2.5 have been observed recently across the UK. Temporal trends in PM2.5 concentrations across UK sites all show annual reductions in concentrations since 2018 with large reductions across the early part of 2019, before UK and European COVID-19 lockdowns in 2020.

This work utilises the AURN and complementary networks that measure gas-phase PM2.5 precursors including volatile organic compounds and ammonia as well as both inorganic and organic aerosol components. The aim is to investigate the potential drivers of recent reductions in PM2.5 concentrations across the UK to evaluate if the reductions are due to anthropogenic or natural drivers. These drivers could include emission reductions, changes in transboundary sources and atmospheric chemical pathways, as well as the effect of local and regional weather and climate. This analysis will inform assessment of whether the observed reductions may be a transient response to changes in the economy and commodity prices, changes in weather patterns, or whether the reductions represent change that is likely to be sustained. This has implications for both progress towards reducing the health burden of air pollution and future air quality policy.

How to cite: Bryant, D. J., Lewis, A. C., and Moller, S. J.: Investigating drivers of recent reductions in PM2.5 concentrations across the UK, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3541, https://doi.org/10.5194/egusphere-egu25-3541, 2025.

EGU25-3661 | ECS | Posters on site | AS4.10

Spatiotemporal Trends in Anthropogenic NOx Emissions in the Northern Hemisphere: Insights from Satellite Observations and Atmospheric Modeling 

Yu Mao, Fei Jiang, Weimin Ju, Hengmao Wang, Shuzhuang Feng, and Mengwei Jia

Nitrogen oxides (NOx = NO + NO2) are critical atmospheric pollutants with significant implications for human health and are key precursors of ozone and nitrate aerosols. Anthropogenic emissions primarily from sectors such as transportation, industry, and fossil fuel combustion are the main sources of NOx. The temperate regions of the Northern Hemisphere, which host most industrialized countries and densely populated areas, account for 60~70% of global anthropogenic NOx emissions. As the harmful effects of air pollution gain global attention, nations have implemented various clean energy policies to address these threats. Effective monitoring of anthropogenic NOx emissions and control policies relies on accurate, long-term emission inventories. However, existing “bottom-up” inventories suffer from delays in data compilation, making it difficult to timely and accurately monitor the spatiotemporal variations of NOx emissions.  This study presents an effective top-down inversion framework using TROPOMI satellite NO2 observations combined with the GEOS-Chem atmospheric chemical transport model to assess recent NOx emissions. The framework employs a mass balance principle and a two-step inversion approach, extending anthropogenic NOx emissions in the Northern Hemisphere into 2022 and optimizing emissions from 2019 to 2022 for the temperate regions. Our results show a 1.68% decrease in NOx emissions in 2020, followed by a 5.72% rebound in 2021. The recovery in China was faster than in other regions, surpassing 2019 levels by July 2020. In 2022, emissions declined across all regions, driven primarily by the Omicron variant, energy shortages, and clean energy policies. By integrating satellite observations, atmospheric modeling, and emission inversion techniques, our study contributes to the growing body of knowledge on how emissions evolve in response to global disruptions.

How to cite: Mao, Y., Jiang, F., Ju, W., Wang, H., Feng, S., and Jia, M.: Spatiotemporal Trends in Anthropogenic NOx Emissions in the Northern Hemisphere: Insights from Satellite Observations and Atmospheric Modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3661, https://doi.org/10.5194/egusphere-egu25-3661, 2025.

EGU25-4224 | Orals | AS4.10

Atmospheric health burden across the century and the accelerating impact of temperature compared to pollution 

Andrea Pozzer, Brendan Steffens, Yiannis Proestos, Jean Sciare, Dimitris Akritidis, Sourangsu Chowdhury, Katrin Burkart, and Sara Bacer

Anthropogenic emissions alter atmospheric composition and therefore the climate, with implications for air pollution- and climate-related human health. Mortality attributable to air pollution and non-optimal temperature is a major concern, which is subject to change in the future under different climate change and socioeconomic scenarios. We use model outputs from the recent Intergovernmental Panel on Climate Change multi-institution simulations to assess future changes in mortality attributable to long-term exposure to both non-optimal temperature and air pollution. We show that, under a moderate scenario (SSP2-4.5), end-of-century mortality could quadruple from present-day values to around 30 (confidence level 95%:12-53) million/year, potentially reaching 44 million/year in a more pessimistic scenario (SSP5-8.5). While pollution-related mortality is projected to increase five-fold by the end of the century in a moderate scenario, temperature-related mortality will experience a seven-fold rise, making non-optimal temperature exposure more important than air pollution as health risk factor for at least 20% of the world's population. Population aging emerges as the primary driver of increased mortality, countering efforts to improve air quality and mitigate climate change. These findings underscore the urgency not only to improve air quality but, more importantly, to simultaneously implement more effective climate change policies to prevent significant loss of lives in the future.

How to cite: Pozzer, A., Steffens, B., Proestos, Y., Sciare, J., Akritidis, D., Chowdhury, S., Burkart, K., and Bacer, S.: Atmospheric health burden across the century and the accelerating impact of temperature compared to pollution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4224, https://doi.org/10.5194/egusphere-egu25-4224, 2025.

EGU25-4374 | Posters on site | AS4.10

Unraveling the health impacts of local and cross-border air pollution 

Dimitris Akritidis and Andrea Pozzer

Long term exposure to fine particulate matter (PM2.5) is a major health risk associated with excess mortality. Ambient PM2.5 concentrations at a given location are subject not only to local pollution but also to that transported from other regions. To unravel the contribution of local and cross-border pollution to the PM2.5 related excess mortality of each country around the world, numerous simulations are carried out with the chemistry general circulation model EMAC (ECHAM5/MESSy for Atmospheric Chemistry), removing each time the anthropogenic emissions of a country. The simulations are performed at a T106 horizontal resolution (equivalent to 1.1 x 1.1 degree at the equator) for the year 2015, while the anthropogenic emissions of each country are based on CEDS (Community Emissions Data System, 2020-v1). Mortality calculations are performed applying the FUSION exposure-response function, with country-level population and mortality rates obtained from the GBD (Global Burden of Disease). We find that local pollution is the main driver of PM2.5 related excess mortality in China and India, while cross-border pollution is responsible for at least one out of two excess deaths attributable to PM2.5 in many European countries. Our results reveal the limits of health-driven mitigation, supporting policy makers to design and implement actions at both national and international levels.

How to cite: Akritidis, D. and Pozzer, A.: Unraveling the health impacts of local and cross-border air pollution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4374, https://doi.org/10.5194/egusphere-egu25-4374, 2025.

EGU25-4867 | ECS | Orals | AS4.10

An introduction to MethaneMIP: investigating the climate and health benefits of methane mitigation using Earth System Models 

Mark England, Drew Shindell, Fiona O'Connor, Chris Smith, Yangyang Xu, Feng Chuan, Benjamin Gaubert, Rachel Law, Tilo Ziehn, Patrick Jöckel, Franziska Winterstein, Thomas Kleinen, Vaishali Naik, Martin Cussac, Lise Seland Graff, Dirk Olivié, and Michael Sigmond

Methane is a potent greenhouse gas which has substantially contributed to climate change since the pre-industrial era, second only in importance to carbon dioxide. Due to its short atmospheric lifetime and high global warming potential, methane emissions have disproportionately large impacts on near-term climate change. Beyond its direct role as a greenhouse gas, methane also has other important implications for climate, human health, air quality and vegetation, largely due to its impact on tropospheric ozone. Thus, reducing methane emissions has been identified as a key policy lever for delaying the worst impacts of near-term climate change with expected co-benefits for health and air quality. The most notable of these efforts is the Global Methane Pledge which aims to achieve a 30% reduction in global anthropogenic methane emissions by 2030 as compared to 2020. And yet, in many respects, methane mitigation has been overlooked relative to other climate mitigation strategies. Existing modelling evidence for the estimating the potential climate benefits of methane mitigation rely extensively on idealised climate emulators or comprehensive modelling studies based on a limited number of models and ensemble members. Both approaches have important limitations. Hence, there is a pressing need for a co-ordinated intermodel comparison project which uses state-of-the-art ESMs in which all modelling groups prescribe identical reductions in methane concentrations or emissions, all modelling groups use the same baseline scenario, and sufficient ensemble members are simulated to investigate the broader climate and health impacts of methane mitigation. MethaneMIP has been envisioned to undertake these tasks.

In this talk I will introduce the MethaneMIP protocol and the two new methane reduction scenarios ‘Technical Measures’ and ‘Ambitious’, which are both branched from SSP2-4.5 and cover the period 2020-2050. The overarching aim of MethaneMIP is to provide a policy-relevant state-of-the-art estimate of the climate and health impacts of methane mitigation, and a robust quantification of the uncertainties, as well as furthering our understanding of methane’s role in the climate system. Over ten modelling centres from across the world are participating in MethaneMIP, with simulations for the core MethaneMIP experiments currently underway. For the first time, I will present the preliminary results of MethaneMIP as pertaining to the research questions it was set up to address, including: What are the best estimates of the expected climate and health benefits of plausible methane mitigation by mid-century? Which near-term climate events projected to occur may be delayed or avoided by curbing methane emissions? What are potential impacts of successful implementation of the Global Methane Pledge? When should we expect the climate or health signal from reduced methane to be detectable in the presence of internal variability?  I will finish by discussing the implications of MethaneMIP for climate policy, as well as introducing the flagship emissions-driven MethaneMIP simulations which will be performed later this year.

How to cite: England, M., Shindell, D., O'Connor, F., Smith, C., Xu, Y., Chuan, F., Gaubert, B., Law, R., Ziehn, T., Jöckel, P., Winterstein, F., Kleinen, T., Naik, V., Cussac, M., Graff, L. S., Olivié, D., and Sigmond, M.: An introduction to MethaneMIP: investigating the climate and health benefits of methane mitigation using Earth System Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4867, https://doi.org/10.5194/egusphere-egu25-4867, 2025.

EGU25-5146 | ECS | Orals | AS4.10

Household and ambient air pollution mortality risk: global insights from macro-level indicators 

Scott Mark Romeo Mahadeo and Avidesh Seenath

Household and ambient air pollution (HAAP) pose a major global health risk, contributing to over six million premature deaths annually and significantly diminishing quality of life. We examine macro-level socio-economic, environmental, energy, and health determinants of HAAP mortality rates across 150 countries. While prior research often focuses on micro-level factors or single-country analyses, our study provides one of the first comprehensive global assessments, incorporating a wide array of indicators. Our findings highlight critical pathways to reducing HAAP-related deaths. Increased rural access to clean cooking fuels and higher healthcare expenditure emerge as pivotal solutions, while rurality amplifies mortality risks. Advanced economies exhibit greater resilience to HAAP mortality, whereas emerging and developing economies remain highly vulnerable, with notable disparities among them. Contrary to conventional assumptions, males face higher HAAP mortality risks than females, a pattern supported by descriptive statistics and global GIS mapping of predicted probabilities from regression models. Our results are robust across alternative models and consistent over time. To contextualise these findings, we integrate evidence from prior country-specific case studies, bridging local insights with global trends. This research advances understanding of progress toward UN Sustainable Development Goals (SDGs 3, 5, and 7) and provides useful insights for policymakers to mitigate HAAP mortality risks and improve living conditions globally.

How to cite: Mahadeo, S. M. R. and Seenath, A.: Household and ambient air pollution mortality risk: global insights from macro-level indicators, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5146, https://doi.org/10.5194/egusphere-egu25-5146, 2025.

EGU25-5695 | Posters on site | AS4.10

Air pollution and the impact of meteorological factors in air quality of Chalki Island during a winter period of 2023-2024 

Ioannis Logothetis, George Giakoumakis, Adamantios Mitsotakis, and Panagiotis Grammelis

Air quality and climate change are of the dominant challenges for Islandic ecosystems in Mediterranean region. This work studies the air quality and the impact of meteorological conditions in pollution levels of Chalki Island, a small island that is located in the climatic sensitive region of southeastern Aegean basin. The analysis was conducted during a low touristic activity period that covers the days from 24th of November 2023 to 3rd of March 2024. Hourly recording of PM2.5, O3 and SO2 as well as meteorological factors of temperature (T) and relative humidity (HR) from a mobile air quality monitoring system (Haz-Scanner™ Model HIM-6000) which is located in the center of city in combination with meteorological parameters (precipitation, planetary boundary height, atmospheric pressure, wind speed and direction) available from the last generation of ECMWF reanalysis dataset (ERA5) are used for the analysis. The calculation of Air Quality Index (AQI) for the studied pollutants shows that PM2.5 is the dominant factor that determines the air quality in the city center of Chalki. The majority of days is classified in “good” and “moderate” air quality classes (in terms of AQI). Additionally, the analysis shows that climate conditions significantly affect the concentration of pollutants. In particular, the higher height of planetary boundary layer (PBL) and increased ventilation coefficient (as a measure of the dispersive capability) are related to improved air quality conditions. The temperature and relative humidity conditions lead to improved climate sense for the mean population (in terms of Discomfort Index; DI<21). Finally, AQI is positive correlated to DI values (corr. Coef: 0.4) indicating a synergy of degraded air quality and discomfort conditions on human health.

How to cite: Logothetis, I., Giakoumakis, G., Mitsotakis, A., and Grammelis, P.: Air pollution and the impact of meteorological factors in air quality of Chalki Island during a winter period of 2023-2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5695, https://doi.org/10.5194/egusphere-egu25-5695, 2025.

EGU25-6068 | Posters on site | AS4.10

Quantifying the Burden of Air Pollution on Type 2 Diabetes Mellitus in Europe 

Pedro Jiménez-Guerrero, Agustín Ríos-Moreno, and Patricia Tarín-Carrasco

Air pollution is a significant environmental issue affecting human health, with growing evidence linking it to chronic diseases such as Type 2 Diabetes Mellitus (T2DM). T2DM has become a major global health concern, with its prevalence and incidence rising at an alarming rate. This metabolic disorder, characterized by chronic hyperglycemia due to insulin resistance or insufficient insulin production, has traditionally associated with factors such as obesity, sedentary lifestyles, and dietary habits. However, recent research highlights that environmental exposures, particularly to air pollutants, may significantly contribute to the development and progression of the disease. Particulate matter (PM2.5) and nitrogen dioxide (NO2) have been shown to trigger systemic inflammation, oxidative stress, and endothelial dysfunction—key mechanisms in insulin resistance and beta-cell impairment. These findings emphasize the need to consider air pollution as an emerging and modifiable risk factor for diabetes.

However, the relationship between air pollution and T2DM remains underexplored, with limited studies establishing robust exposure-response relationships. Understanding the exposure-response relationship is crucial for accurately estimating the disease burden attributable to air pollution and guiding public health interventions. this study aims to establish the exposure-response function that relates the concentration of two air pollutants (NO2 and PM2.5) to the hazard ratio associated with acquiring T2DM, based on various cohort studies conducted worldwide. To achieve this, a methodology using nonlinear function adjustments will be employed, fitting a specific function dependent on four parameters to a scatter plot of pollutant concentration and hazard ratio data pairs extracted from available cohort studies. Once the specific form of this exposure-response function is determined, it will be applied to the domain of Europe using atmospheric concentrations for the period 1991-2020, obtaining the risk ratio for each cell. From there, the incidence of air pollution on T2DM will be estimated for each age group.

The results indicate a significant nonlinear relationship between air pollution exposure and T2DM incidence, with higher risks observed in areas with elevated levels of NO2 and PM2.5 (specifically, in large European cities and central Europe due to traffic and industrial activities mainly). The results show that NO2 air pollution is responsible for 4,693,000 [4,285,000 – 4,946,000 95% CI] cases of T2DM per year, representing an incidence of 0.64% [0.58 – 0.67 95% CI] relative to the total population of the study area. For PM2.5, the total number of annual cases rises to 5,009,000 [3,957,000 – 6,452,000 95% CI], accounting for an incidence of T2DM of 0.68% [0.54 – 0.87 95% CI] considering the population in the target area. The analysis revealed that PM2.5, despite lower concentrations compared to NO2, had a higher impact on T2DM incidence, especially at lower exposure levels. The findings underscore the need for stringent air quality regulations, particularly in urban and industrial regions, to mitigate the health impacts of air pollution.

How to cite: Jiménez-Guerrero, P., Ríos-Moreno, A., and Tarín-Carrasco, P.: Quantifying the Burden of Air Pollution on Type 2 Diabetes Mellitus in Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6068, https://doi.org/10.5194/egusphere-egu25-6068, 2025.

EGU25-7478 | ECS | Orals | AS4.10

Clean air for some: How satellite-measured NO2 reveals sources and impacts of and equitable solutions to long-standing disparities 

Gaige Hunter Kerr, Susan C. Anenberg, Lulu Chen, Daniel L. Goldberg, Daniel E. Huber, Michelle Meyer, and Joshua Miller

The pollutant nitrogen dioxide (NO2), a tracer for fossil fuel combustion from transportation and industry and commonplace in urban areas, is associated with a growing number of adverse health outcomes. Many of its sources as well as NO2 concentrations themselves are often highest within marginalized and minoritized communities in the United States (U.S.) and throughout the world. The short lifetime and spectral properties of NO2 allow for high-fidelity, space-based measurements, and the increasingly high spatial resolution and complete geographic coverage of satellite-derived NO2 provided by current instruments, such as the TROPOsphere Monitoring Instrument (TROPOMI), attest to recent advances in our ability to surveil NO2 from space. 

Here, we highlight how remotely-sensed observations of NO2 or estimates of NO2 that incorporate satellite data can reveal the extent, sources, and impacts of these disparities. To these points, we show how communities of color in the U.S. face significantly higher levels of NO2 by a factor of ~2.1 than majority white, non-Hispanic communities and trace back this disproportionate exposure to particular NO2 sources such as light- and heavy-duty transportation and the rapidly-growing e-commerce and warehousing industry. These inequitable exposures are associated with a large burden of disease—including an estimated 115,000 new cases of pediatric asthma annually in the U.S.—disproportionately borne by marginalized communities. Despite the concerted efforts of policymakers to reduce these health disparities, we find that the magnitude of disparities has grown in recent years. 

We discuss how new geostationary instruments with complete daytime coverage, such as Tropospheric Emissions: Monitoring of Pollution (TEMPO), may reveal different disparities in NO2 exposure compared with polar-orbiting instruments such as TROPOMI that provide only a single early afternoon snapshot of NO2 levels. We also broaden our exploration of urban air quality, health, and equity to the global scale and discuss how global marginalized communities may face similar, disproportionate exposure to this pollutant as they do within the U.S. Overall, these satellite-enabled insights can spur and inform policies that would not only reduce urban pollution but could have outsized benefits for overburdened communities, and we discuss how actions such as adopting more stringent air quality or engine standards can reduce NO2 emissions and targeted cleanup of emission sources within these overburdened communities could reduce these long-standing disparities. 

How to cite: Kerr, G. H., Anenberg, S. C., Chen, L., Goldberg, D. L., Huber, D. E., Meyer, M., and Miller, J.: Clean air for some: How satellite-measured NO2 reveals sources and impacts of and equitable solutions to long-standing disparities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7478, https://doi.org/10.5194/egusphere-egu25-7478, 2025.

EGU25-7968 | ECS | Orals | AS4.10

Advancing Regional Air Pollution Exposure Assessment: Revealing Underestimated Long-Term Exposure to PM2.5 in Greece 

Martin Otto Paul Ramacher, Anastasia Kakouri, Eleni Athanasopoulou, and Volker Matthias

The estimation of human exposure to air pollution presents well-known methodological challenges. Two major challenges are incorporating population activity and accounting for outdoor pollutant concentrations infiltrating indoor environments. These aspects are often overlooked in current exposure assessments at urban and regional scales, introducing biases that result in non-representative exposure estimates and associated health effects.

In this study, we present a method for regional dynamic exposure estimation by integrating population activity and the infiltration of air pollutants into indoor environments. Using the time-microenvironment-activity concept in combination with open-source datasets for the spatial and temporal distribution of the European population, our framework generates grids of population activity across different microenvironments (home, work, schools, transport, etc.) with a spatial resolution of 1x1 km2 and a temporal resolution of 1 hour for all of Europe. Each microenvironment is assigned seasonal, literature-based outdoor-to-indoor infiltration factors. The resulting dynamic population grids can be created for any urban or regional to domain in Europe and can be applied to air pollutant concentrations derived from any air quality model that match these domains.

To illustrate the impact of regional dynamic exposure estimates compared to static estimates (based on residential addresses), we combined the dynamic population activity data with a high-resolution (1x1 km2) gridded dataset of PM2.5 concentrations across Greece from 2015 to 2022. This dataset was produced using a recently developed and extensively evaluated Random Forest modeling approach to downscale regional to urban pollutant concentrations specifically for Greece. Initial results reveal that regional-scale dynamic estimates incorporating population activity resulted in >10% higher mean exposure to PM2.5 compared to exposure estimates based on static populations but can vary significantly between different microenvironments. These findings suggest that current population exposure estimates to ambient air pollution across Europe are likely to be underestimated.

How to cite: Ramacher, M. O. P., Kakouri, A., Athanasopoulou, E., and Matthias, V.: Advancing Regional Air Pollution Exposure Assessment: Revealing Underestimated Long-Term Exposure to PM2.5 in Greece, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7968, https://doi.org/10.5194/egusphere-egu25-7968, 2025.

EGU25-10552 | ECS | Orals | AS4.10

Using high-resolution TROPOMI NO2 columns to assess health disparities in NO2 exposure across London 

Eleanor Gershenson-Smith, Eloise A. Marais, Karn Vohra, and Rebekah P. Horner

Long-term exposure to air pollution is a major global public health threat. However, the health burden due to air pollution exposure is unequal. In cities, ethnic minorities experience the most severe exposures and adverse health outcomes to air pollution, particularly from traffic. Exposure to traffic-related air pollution is associated with childhood-onset asthma and adult premature mortality. Contemporary data of the location and size of the disparities to determine and address inequities in exposure and health burdens is not readily available for all cities. Here we address this dataset by deriving surface concentrations of nitrogen dioxide (NO2) as proxy for traffic-related air pollution for London at fine spatial scales (~400 m). This is achieved by oversampling 5 years of TROPOspheric Monitoring Instrument (TROPOMI) tropospheric NO2 column data from its nadir resolution of ~5.6 km x 3.5 km. We then subtract off a uniform free-tropospheric NO2 column of 50 pptv determined from cloud-sliced vertically resolved TROPOMI data to isolate the boundary layer. These boundary layer columns are then converted to surface concentrations using an exponential relationship between the TROPOMI boundary layer column and midday mean in-situ network measurements. Midday concentrations are converted to 24-hour concentrations using a midday-to-24h ratio of 1.30, which is calculated from surface network sites in the Greater London Area (GLA). The TROPOMI-derived 24-hour mean surface NO2 concentrations reproduce the NO2 observed by the surface network. We use 2021 census data at the finest resolution for three out of five high-level ethnic groups defined by the UK census: Asian, Black and White. To calculate the health burden, we use borough level baseline mortality rates, the finest scale available, which range between 44 and 2818 per 100,000, and an exposure response coefficient of 1.023 per 10 µg m-3 annual mean NO2 as recommended by the UK’s Committee on the Medical Effects of Air Pollutants (COMEAP). We find premature mortality rates due to traffic-related pollution exposure for each ethnic group exhibit similar spatial variation across the city, with highest mortality in central and central northwest London. The average GLA premature mortality rate is worst for the Black population (59 per 100,000), then the Asian population (57 per 100,000) and least severe for the White population (56 per 100,000), reflecting the ethnic injustices in air pollution exposure. Work is underway to identify specific census-tract areas with the most severe disparities that require immediate regulatory actions and to quantify the disparities in childhood asthma instances across the city. We aim to expand this investigation to four other major UK cities with the greatest traffic-related pollution emissions, according to the UK National Atmospheric Emission Inventory (NAEI). These are Birmingham, Leeds, Manchester and Glasgow.

How to cite: Gershenson-Smith, E., Marais, E. A., Vohra, K., and Horner, R. P.: Using high-resolution TROPOMI NO2 columns to assess health disparities in NO2 exposure across London, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10552, https://doi.org/10.5194/egusphere-egu25-10552, 2025.

EGU25-11546 | ECS | Orals | AS4.10

Inequality in hazardous volatile organic compound (VOC) emissions and concentrations measured over Los Angeles 

Eva Y. Pfannerstill, Jennifer Ofodile, Sally E. Pusede, Cesunica E. Ivey, Caleb Arata, and Allen H. Goldstein

In the United States, PM2.5 and NOx pollution disproportionately burden communities of color and of lower income. However, such information is lacking when it comes to hazardous air pollutants (HAPs) like toxic volatile organic compounds, for which city-wide measurements are more challenging and thus are not available in routine observations.

In this study, we use the highest spatially resolved (~2 km) airborne measurements of emissions and concentrations ever reported of HAPs while covering a whole megacity, and combine these observations with US Census information. We observe higher concentrations and emissions of 17 measured HAPs – such as benzene, naphthalene, and p-chlorobenzotrifluoride (PCBTF) – in California-designated Disadvantaged Communities and census tracts with low-income Hispanics and Asians. While concentrations were on average 32 ± 5% higher for low-income Hispanics compared to high-income non-Hispanic whites, emissions were even 107 ± 21% higher - indicating the proximity of low-income Hispanics to localized emission sources. Low-income Hispanics and Asians share an unequal burden from traffic-related emissions, with benzene, nitrogen oxides (NOx ), and carbon monoxide (CO) concentrations up to 60% higher. However, in Disadvantaged Communities and census tracts with large Hispanic populations (>50%), we observe toluene-to-benzene emission ratios above 3, pointing to inequalities in other HAPs primarily caused by non-traffic emission sources such as industry and solvents. In these communities, regulatory inventories also significantly underestimate the observed emissions. We find that efforts to address HAP inequalities and environmental justice concerns in Los Angeles will need to consider contributions from volatile chemical products, which represent a growing source of emissions driving inequalities in impacted communities.

How to cite: Pfannerstill, E. Y., Ofodile, J., Pusede, S. E., Ivey, C. E., Arata, C., and Goldstein, A. H.: Inequality in hazardous volatile organic compound (VOC) emissions and concentrations measured over Los Angeles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11546, https://doi.org/10.5194/egusphere-egu25-11546, 2025.

Rapid urbanization and high population densities in Latin American cities pose significant challenges for air quality monitoring, particularly for fine particulate matter (PM2.5), recognized as the foremost health risk for urban populations. This study leverages satellite data and machine learning to estimate the spatial-temporal variability of PM2.5 in the Santiago City Metropolitan Area (Chile), providing critical data to enhance public health policies and address environmental injustices.

Our methodology encompassed four stages: data preprocessing, model architecture selection and construction, model validation, and spatial mapping of PM2.5 concentrations. Initially, we processed PM2.5 data from 12 ground monitoring stations (period 2015 to 2024), integrating it with meteorological data (ERA-5), land cover and NDVI products (MODIS), as well as aerosol products from MERRA-2. We employed a variety of modeling techniques, such as Decision Trees, Treebag, Random Forest, and Extreme Gradient Boosting (XGB). The XGB model was ultimately selected for its superior performance metrics (i.e., higher R2 and lower RMSE).

The XGB model captured a significant range of PM2.5 concentrations across Santiago for the test period (2023-2024), with winter months showing the highest levels, peaking at 75 µg/m³ in June 2023. In contrast, the lowest concentrations occurred from February to April and from October to December, with a minimum of 10 µg/m³ in November. The 1 km² resolution maps revealed a pronounced gradient of PM2.5 concentrations from the west (the Coastal Mountain range) to the east (the Andes Mountain range), negatively correlated with elevation. Densely populated communes such as Quinta Normal and Lo Espejo, which have lower socioeconomic standings, recorded the highest average PM2.5 concentrations (67 to 63 µg/m³). In contrast, wealthier and less densely populated areas like Lo Barnechea and Vitacura exhibited lower concentrations (21 to 23 µg/m³). By identifying how socioeconomic disparities intersect with environmental risks, this study provides a solid foundation for policymakers to formulate interventions that not only improve air quality but also promote social equity.

How to cite: Diez, S. and Urquiza, J.: Exploring PM2.5 dynamics in Santiago, Chile: how satellite data and machine learning could inform environmental policy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14015, https://doi.org/10.5194/egusphere-egu25-14015, 2025.

EGU25-17122 | Orals | AS4.10

From temperature observations to mitigation measures: Data-driven approaches to multi-scale climate adaptation in Hesse, Germany 

Susanne A. Benz, Mathias Jehling, Svea Krikau, Sven Wursthorn, and Sina Keller

As urban temperatures rise and the demand for urban densification increases, climate adaptation has become a significant concern for policymakers. However, we face a challenge in today's data-rich environment: How can we effectively manage the vast amounts of information available to make informed decisions for our cities and communities? Accordingly, urban agglomerations in Germany are struggling in allocating measures.

In collaboration with the federal state of Hesse, we have developed a data-driven decision-making method to address two critical questions: Which locations should we focus on for heat mitigation and the protection of cool oases? And which climate adaptation measures are most suitable for each location?

Our method consists of four steps:

  • Identification of Hot Spots and Cold Spots: We identify universal hot and cold spots that consistently experience high or low temperatures during both day and night. This assessment is based on various temperature metrics that capture heat stress and imbalances in surface heat fluxes, which we harmonize using a 100 m grid. We validate our findings using local climate zones and CORINE land cover data.
  • Prioritization of Locations: We prioritize hot and cold spots using a merit- and penalty-based system. Rather than focusing solely on the hottest areas, we emphasize locations where heat impacts vulnerable populations or disrupts cooling patterns over broader regions.
  • Assessment of Mitigation Potentials: Each grid cell is evaluated for its deficits and potentials for climate adaptation using a multitude of contextual data. This includes detailed land cover information obtained from high-resolution aerial imagery segmentation, along with green and blue indicators (such as NDVI, green volume, and water availability), and settlement structure (e.g., types  of historic urban centers or single family housing).
  • Suitability of Adaptation Measures: Based on the results from steps 2 and 3, we rank the suitability of various adaptation measures (e.g., green facades, increased tree coverage) for each grid cell using a second merit- and penalty-based system.

In a close loop with practitioners from local to regional authorities, this integrated approach enables us not only to identify areas in need of climate action, but also to recommend specific, actionable measures. By leveraging data at this level of detail and scale, we facilitate informed, targeted climate adaptation strategies.

How to cite: Benz, S. A., Jehling, M., Krikau, S., Wursthorn, S., and Keller, S.: From temperature observations to mitigation measures: Data-driven approaches to multi-scale climate adaptation in Hesse, Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17122, https://doi.org/10.5194/egusphere-egu25-17122, 2025.

EGU25-18004 | ECS | Orals | AS4.10 | Highlight

Provincial economic and air quality-related health impacts of China’s potential partitioned carbon regulation 

Mingwei Li, Hantang Peng, Da Zhang, Fengwei Wan, and Xiliang Zhang

China has launched the national emissions trading system (ETS) and intends to form a novel mechanism to control provincial carbon emissions. While previous studies have separately analyzed the impacts of ETS and provincial reduction targets on welfare and air quality, how the potential integration of these approaches would impact welfare and air quality-related health remains underexplored. In this study, we employ an integrated modeling framework to compare the economic impacts and health outcomes associated with PM2.5 and ozone under three provincial control mechanisms, all targeting the same national total carbon emissions in 2035. Our findings indicate that ETS improves national welfare by at least 0.12% compared to the conventional provincial control mechanism (PRO_CAP). The partitioned carbon regulation mechanism (PART_REG), which applies national ETS to power and energy-intensive industry sectors while assigning reduction targets to other sectors at the provincial level, achieves 85% of the welfare improvement observed under an ideal mechanism with comprehensive ETS coverage (FULL_ETS). Compared to PRO_CAP, ETS redistributes CO2 and co-emitted air pollutant emissions from northern to southern China, improving air quality in northern provinces but worsening it in central and southern provinces. National premature deaths increase by 32,700 (95% CI: 23,200—41,600) and 44,800 (95% CI: 31,400—57,600) under the PART_REG and FULL_ETS scenario, respectively, compared to the RPO_CAP scenario. When comparing the changes in welfare and monetized health impact, ETS remains cost-effective nationally compared to RPO_CAP, with a median net benefit estimate of US$6.6 billion under the PART_REG—20% larger than that under the FULL_ETS. The northern and southeastern coastal provinces experience net positive benefits, while some central provinces face net negative benefits.

How to cite: Li, M., Peng, H., Zhang, D., Wan, F., and Zhang, X.: Provincial economic and air quality-related health impacts of China’s potential partitioned carbon regulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18004, https://doi.org/10.5194/egusphere-egu25-18004, 2025.

Unequal exposure to air pollution is a systemic issue in the UK. What makes it further challenging to address are the inconsistencies in location and size of these disparities based on the air pollutant and chosen attribute: emissions, exposure or health burden. Missing is a comprehensive assessment in UK air pollution disparities from all three perspectives to inform policy. In this study, we explore how the location and size of disparities evolve from investigating disparities in air pollutant precursor emissions to that in exposure and health burdens.

Here, we use a 2-model setup to simulate meteorology and atmospheric composition over the UK at a spatial resolution of 9 km x 9 km for 2019. The meteorology is simulated using the WRF (Weather Research and Forecasting) model and atmospheric chemistry and transport processes using the CMAQ (Community Multi-scale Air Quality) model. The CMAQ model is updated with the most up-to-date chemistry mechanism CRACMM (Community Regional Atmospheric Chemistry Multiphase Mechanism) and is driven with air pollutant precursor emissions from the UK National Atmospheric Emissions Inventory (NAEI).

Modelled surface concentrations of health-harming fine particles (PM2.5) and nitrogen dioxide (NO2) are evaluated against observations from the extensive national and local ground-based monitoring networks and are then applied to health risk assessment models to quantify PM2.5-attributable premature mortality and NO2-attributable asthma incidences. The emissions (primary PM2.5 and NOx), exposure and attributable health burdens are then used with demographic datasets to examine disparities in these. Work is underway to compare inequities in urban versus rural landscape in the UK. Findings from this comprehensive evaluation of inequities will be used to inform stakeholders to create targeted interventions and action plans.

How to cite: Vohra, K. and Bloss, W.: A Comprehensive Assessment of Disparities in UK Air Pollutant Emissions, Exposure, and Health Burden to Inform Policy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18940, https://doi.org/10.5194/egusphere-egu25-18940, 2025.

Traffic-related air pollution is one of the major sources of exposure in urban areas and an increasingly important contributor to anthropogenic emissions in lower and middle-income countries. Due to a rapid rise in the motor fleet owing to population growth, economic development, the expansion of metropolitan areas, and the increasing dependence on motor vehicles because of changes in land use, the concerns about the health effects of traffic-related air pollutants (TRAPs) have greatly increased. In the light of limited evidence in the Indian context, the present research work involved conducting a crossover panel study on a group of healthy adults in Delhi (security guards on a university campus; sample size ~ 40) to understand the short-term effect of PM2.5 (particles having aerodynamic diameter less than 2.5 microns) and their chemical components on acute changes in cardiovascular health. The study improved the exposure estimates by real-time monitoring of PM2.5 mass, its chemical components like ions and trace metals, black carbon (BC) and size-resolved particle number concentration in a traffic microenvironment instead of using ambient concentrations as a proxy to traffic exposure. The participants were administered questionnaires to gather the background data about socio-economic status, secondary exposures or prevailing health conditions and any potential confounders. The ECG holter systems were used to monitor the real-time changes in heart rate variability (HRV) parameters, which are an indicator of cardiac activity (both time-domain (SDNN- standard deviation of normal-to-normal; pNN50- percent normal-to-normal intervals > 50ms; rMSSD- root mean square of successive differences between normal heart beats) and frequency domain (HF- high frequency; LF- low frequency and LF/HF ratio) were monitored). Mixed models were used to quantify the associations between TRAPs and HRV parameters. A significant decline was observed in all the HRV indices with an increase in the pollutant concentrations. The highest decline in HRV with respect to particle size was observed for the particles with a diameter between 0.03-0.1 µm with negligible change in particles with dia. > 1µm. Similarly, amongst the PM2.5 constituents, BC showed the highest decline in HRV, followed by nitrates and sulfates. The study emphasized the need to study exposures in specific microenvironments due to differences in the pollutant concentrations and composition with respect to ambient. It also highlighted the need to investigate the micro-physical and chemical characteristics of PM2.5 because of their potential to have greater health impacts as compared to the total PM2.5 concentrations.

How to cite: Jain, K. and Habib, G.: Assessing Short-Term Cardiovascular Effects of PM2.5 and Its Components in a Traffic Microenvironment: A Crossover Panel Study in Urban India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20428, https://doi.org/10.5194/egusphere-egu25-20428, 2025.

EGU25-20465 | Posters on site | AS4.10

Fine-scale Climate Projections over Minnesota for the 21st Century  

Stefan Liess, Heidi Roop, Tracy Twine, Alejandro Fernandez, Dhondup Dolma, Jack Gorman, Nathan Meyer, Amanda Farris, and Peter Neff
Global warming has its largest amplitude in the higher latitude regions of the Northern Hemisphere. This is especially the case during winter months when reduced reflectivity from diminished snow cover leads to higher average temperatures. This process has led to warming at twice the rate as the rest of the planet. In addition to accelerated warming from local snow melt, this Arctic warming is contributing to strong warming over Minnesota, especially during winter, when Minnesota is one of the states that is warming the strongest within the contiguous United States. We have previously emphasized this strong warming in our study on high-resolution climate projections over Minnesota with CMIP5, and we are now producing an updated dataset with higher spatial resolution and with input from six CMIP6 global climate models (GCMs), namely BCC-CSM2-MR, CESM2, CMCC-ESM2, CNRM-ESM2-1, IPSL-CM6A-LR, and MIROC-ES2L.

 

We use ensemble climate simulations over Minnesota with the Weather Research and Forecasting (WRF) model to compute downscaled versions of the comprehensive global climate projections for the 20-year periods 2040-2059, 2060-2079, and 2080-2099. We also perform model integrations over the historical period of 1995-2014 in order to assess any systematic model uncertainties.

These projections build on our previous results at 10-km resolution, but now we use a higher 4-km horizontal resolution over Minnesota nested in a 20-km grid over the contiguous USA and southern Canada with 38 vertical levels in the atmosphere and a sophisticated representation of the many lakes that exist in Minnesota.

Our final results will show a more detailed representation of the ongoing warming for individual counties in Minnesota in all seasons, especially in winter. We expect conditions near the end of the 21st century that are significantly different from current climate. Our results will influence regional decision-making related to agriculture, infrastructure, water resources, and other sectors.

How to cite: Liess, S., Roop, H., Twine, T., Fernandez, A., Dolma, D., Gorman, J., Meyer, N., Farris, A., and Neff, P.: Fine-scale Climate Projections over Minnesota for the 21st Century , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20465, https://doi.org/10.5194/egusphere-egu25-20465, 2025.

Coal and lignite mining, along with thermal power generation, are major contributors to air pollution, posing significant risks to human health and the environment. India, ranking fifth globally in coal reserves, is the second-largest producer, consumer, and importer of coal. Currently, 533 active coal mines and 20 lignite mines operate in the country, of which 249 coal mines and all lignite mines are opencast. Approximately 180 coal-based and 9 lignite-based thermal power stations contribute to meeting ~77% of India's energy demands. According to research by the Global Burden of Disease regarding the present state of air pollution, there were an astounding 1.67 million air pollution-related deaths in India alone in 2019. Most of these deaths, or over 0.98 million, were caused by ambient particulate air pollution such as PM2.5. Long-term PM2.5 exposure is associated with adverse health effects, including Chronic Obstructive Pulmonary Disease (COPD)—the third leading cause of mortality globally—contributing to substantial financial burdens. In this study, we evaluated PM2.5concentrations at 10 locations in and around the Neyveli Lignite Mine, India’s largest opencast lignite mine, for over two years (March 2020–February 2022). The mean annual PM2.5 concentrations across the study locations were 41.08 μg/m³ (Year 1) and 41.42 μg/m³ (Year 2), exceeding Indian NAAQS, US EPA, and WHO air quality standards. Meteorological data were obtained from the NCEP-NCAR Reanalysis 1 dataset, and air mass back trajectory clusters were analysed using NOAA’s HYSPLIT model. Conditional Bivariate Probability Function (CBPF) and Potential Source Contribution Function (PSCF) plots were generated to identify potential PM2.5 sources. CBPF 75th percentile plots revealed significant pollution events from the south and southeast directions at wind speeds >4 miles/hour. PSCF 75th percentile plots indicated long-range PM2.5 transport from the Bay of Bengal (summer and winter), the Arabian Sea (monsoon), and nearby urban areas (post-monsoon). Using the Multiple-Path Particle Dosimetry (MPPD) model, PM2.5 deposition in the human respiratory system (Yeh/Schum 5-Lobe) was estimated for exposure scenarios of 8 hours/day, 5 days/week, over a year. The total deposition fraction was 0.8238, with the head region contributing the highest deposition (68.28%), followed by the pulmonary (23.56%) and tracheobronchial regions (8.16%). Health impact assessment using WHO’s AirQ+ software estimated COPD hospitalisations attributable to PM2.5. The Estimated Attributable Proportion (EAP), Excess Attributable Cases (EAC), and Estimated Attributable Cases per 100,000 Population (EACP) ranged from 6.57%–6.63%, 1,085–1,095, and 1,026.35–1,035.59, respectively. The financial burden of COPD, evaluated using the Cost of Illness (COI) and Value of Statistical Life (VSL) methods, was 43.23–43.62 million INR (COI) and 1,768,474 INR (VSL). These results highlight the significant health and economic impacts of PM2.5 exposure, emphasising the critical need for targeted air quality interventions and sustainable practices. Moving forward, these preliminary findings will be expanded through receptor modelling to provide a more detailed source apportionment, offering valuable insights for enhancing air quality through focused interventions and strategies.

How to cite: Mitra, S. and Nagendra, S.: Assessing PM2.5 Exposure and Health Risks in a Mining and Thermal Powerplant Township in Southern India: Impacts on Air Quality and Public Health, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21565, https://doi.org/10.5194/egusphere-egu25-21565, 2025.

EGU25-4545 | Posters on site | ITS3.4/AS4.11

Comparative Insights from Living Labs: Driving Sustainable Urban Behaviors through Participatory Science 

Ivan Marchesini and the I-CHANGE D3.7 Team

Urban areas face a wide range of climate-related challenges, including air pollution, waste management, extreme weather events, and the need for sustainable mobility. These challenges demand need to be addressed through tailored (or customised) approaches that account for local socio-economic context and that empower citizens to play an active role in climate adaptation and mitigation actions.

This study compares the outcomes of multiple Living Labs (LLs) operating in diverse socio-economic and environmental contexts across Europe and other regions. Each LL focused on specific urban climate challenges, such as promoting sustainable transportation to reduce emissions or monitoring air quality through participatory science. To better understand what drives individuals to adopt sustainable behaviors, focus groups and surveys were conducted across the LLs. These tools allowed the identification of key factors - be they local or personal - that influence people's willingness to embrace pro-environmental practices.

Results reveal significant variability in how citizens respond to interventions, shaped by local conditions such as infrastructure, cultural factors, and environmental priorities. Across the LLs, the research sought to identify key drivers that encourage individuals to adopt more sustainable behaviors. Such drivers include experiencing climate-induced disasters, enhancing personal competencies, and gaining social approval. Barriers such as limited resources and skepticism toward systemic solutions were also identified and addressed.

This comparative analysis highlights the potential of participatory science not only to collect valuable environmental data but also to act as a catalyst for behavior change. By integrating citizen contributions into localized strategies, the LLs demonstrated how tailored interventions can effectively motivate sustainable practices.

The contribution highlights the critical need to understand the factors that motivate individuals to adopt sustainable behaviors across diverse local contexts. It provides actionable recommendations for designing interventions that empower citizens, reduce climate risks, and foster resilience in urban areas globally.

How to cite: Marchesini, I. and the I-CHANGE D3.7 Team: Comparative Insights from Living Labs: Driving Sustainable Urban Behaviors through Participatory Science, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4545, https://doi.org/10.5194/egusphere-egu25-4545, 2025.

Several personalized carbon footprint and lifestyle calculators have been developed that can be accessed via a web browser or smartphone applications to raise awareness and educate individuals on promoting sustainable behavioural change. This study uses citizens in an experimental setting in Hasselt (Belgium) (n=55) and Karachi (Pakistan) (n=65) to develop further insights about the capabilities of five largely used smartphone-based applications. These applications are Earth Hero, Klima, Yayzy, Carbon Neutral & CO2 Meter, and 2zero-Sustainable Living. Citizens are invited to download a particular app on their smartphone, and other details of the experiment are provided in an initial workshop. For example, a timeframe of three months is given for the app to be used regularly for at least 10 minutes per day. After three months, participants were invited again to workshops, where a structured discussion was held in a focus group setting to understand the behavioural change capabilities of a particular app.  Participants from Hasselt (Belgium) and Karachi (Pakistan) exhibited diverse responses due to socio-cultural, economic, and infrastructural differences, highlighting the contextual adaptability of each application. EarthHero and Klima, which emphasized actionable sustainability tips, resonated well with users seeking direct and practical interventions. After three months, the structured focus group discussions revealed marginal behavioural change patterns, such as increased awareness of personal carbon footprints, reduced energy consumption, and shifts toward eco-friendly habits like public transport use or waste reduction. These changes were more pronounced among participants in Belgium than in Karachi, mainly due to the limited availability of sustainable alternatives. An issue of access to reliable local data has emerged, especially in Karachi, for quantifying footprint. Participants requested more user engagement features in the apps that increase peer interactions, such as leaderboard, community formation, etc. The findings could provide valuable insights into the role of technology in sustainability education, offering recommendations for app developers to improve user engagement and for policymakers to integrate such tools into broader environmental awareness campaigns.

How to cite: Adnan, M., Outay, F., Ahmed, A., and Ahmed, A.: Carbon Footprint Apps as Catalysts for Climate-Friendly Behavioural Change:  Insights from Citizen Science Experiments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6486, https://doi.org/10.5194/egusphere-egu25-6486, 2025.

EGU25-8084 | Posters on site | ITS3.4/AS4.11

CLIMATE OBJECTIVE: I-CHANGE and UIF amateur photographers' alliance for climate  

Antonio Parodi, Luca Ferraris, Nicola Loglisci, Marina Mantini, Lara Polo, Antonello Provenzale, Rita Visigalli, and Elisa Poggi

I-CHANGE addresses climate challenges by actively involving communities in environmental monitoring activities. The objective of the project is to empower individuals and communities to make informed decisions that reduce their environmental footprint, thus contributing to climate change adaptation and mitigation strategies. I-CHANGE equips individuals with tools, and sensors allowing to collect and analyze data to assess the impact of personal and community choices on the environment. The digital camera, in cooperation with the Unione Italiana Fotoamatori (UIF, https://www.uif-net.com/), has emerged as a crucial tool to involve the public and promote participation in climate change topics. UIF has enabled the participation of 176 authors and collected over 1500 images through photographic competitions: the result is a wonderful photography book ready to be downloaded for entertainment and educational purposes (https://doi.org/10.5281/zenodo.13928716 

How to cite: Parodi, A., Ferraris, L., Loglisci, N., Mantini, M., Polo, L., Provenzale, A., Visigalli, R., and Poggi, E.: CLIMATE OBJECTIVE: I-CHANGE and UIF amateur photographers' alliance for climate , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8084, https://doi.org/10.5194/egusphere-egu25-8084, 2025.

EGU25-9057 | Orals | ITS3.4/AS4.11

Fostering Environmental Awareness Through Innovation: Outcomes from the I-CHANGE Project 

Antonio Parodi, Nicola Loglisci, Massimo Milelli, Silvana Di Sabatino, Erika Brattich, Teresa Carlone, Carlo Cintolesi, Pinhas Alpert, Gabriel Campos, Yoav Rubin, Paolo Mazzetti, Antonella Galizia, Ivan Marchesini, Anna Molter, Grace D'Arcy, Juan Esteban Quintero-Marín, Maria Carmen Llasat, Laura Esbri, Gert-Jan Steeneveld, and Esther Peerlings and the I-CHANGE Team

The I-CHANGE project addresses the critical challenges posed by climate change, focusing on active citizen participation and the enhancement of public awareness through evidence-based methodologies. This paper presents the key achievements of the project, which include the organization of diverse community-oriented initiatives aimed at fostering environmental awareness, the deployment and testing of advanced environmental monitoring sensors, and the development of cutting-edge digital tools, such as an interactive dashboard and the ChallengeYeti mobile application. Additionally, the project analyzed extensive data collected through awareness raising campaigns with surveys on individual environmental behaviour, offering valuable insights into the drivers of environmental consciousness. The results underline a significant increase in awareness levels among participants, the effectiveness of technological solutions in promoting engagement, and the relevance of comprehensive data analysis in understanding and addressing climate-related challenges. I-CHANGE proposes a scalable and replicable model that combines technological innovation and inclusive citizen engagement to support climate adaptation and mitigation efforts. 

How to cite: Parodi, A., Loglisci, N., Milelli, M., Di Sabatino, S., Brattich, E., Carlone, T., Cintolesi, C., Alpert, P., Campos, G., Rubin, Y., Mazzetti, P., Galizia, A., Marchesini, I., Molter, A., D'Arcy, G., Quintero-Marín, J. E., Llasat, M. C., Esbri, L., Steeneveld, G.-J., and Peerlings, E. and the I-CHANGE Team: Fostering Environmental Awareness Through Innovation: Outcomes from the I-CHANGE Project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9057, https://doi.org/10.5194/egusphere-egu25-9057, 2025.

EGU25-9596 | Posters on site | ITS3.4/AS4.11

MeteoTrackers (MT) in Citizens Science -A New Era in Micrometeorology or just an Instrument for education?Lessons from MT operations within I-CHANGE EU project  

Pinhas Alpert, Gabriel Campos, Nitsa Haikin, Yoav Rubin, Massimo Milelli, Antonio Parodi, and Nicola Loglisci

The I-CHANGE (Individual Change of HAbits Needed for Green European transition, 2021-2025) project promotes the active participation of citizens to address climate change. It engages citizens and local stakeholders to take part in science initiatives and support more sustainable behaviour. To this aim, a set of Living Labs located in very different eight cities of socio-economic contexts (Amsterdam, Barcelona, Bologna, Dublin, Genova, Hasselt, Jerusalem and Ouagadougou), were chosen. The I-CHANGE Living Labs address different environmental issues all employing Meteotrackers (MT) in order to perform high-resolution meteorological measurements.

With recent emergence of new types of near-surface meteorological data that are exploding in their big numbers and cover much higher resolution than classical or World Meteorological Organization (WMO) data, much interest is naturally given to the quality and validation of this crowdsourcing data. The present note focuses on MeteoTracker (in brevity, MT) data collected by citizens walking or biking and travelling.

The present note suggests a practical methodology for operating MTs, along with the suggestion of the potential emergence of a new era in micrometeorological measurements that allows high resolution, both spatial and temporal. Micrometeorology in the sense of obtaining data on the scales of ~1 m, ~1 min and ~0.1 deg for temperature etc. A great challenge in such measurements is that there are a multitude of factors influencing surface observations and it is a complex task to define which factors, as well as their potential synergies, are involved, or just which are dominant. Thus, allowing better understanding of the synergies among several microscale factors. Such factors include, among many others, land cover temporal/spatial variations of agriculture, water, soil moisture, trees, urban area, isolated buildings, as well as topographical variations, solar insolation, cloudiness, aerosols, mesoscale dynamical effects, synoptics.

The basic concept here is that although these new data types are still involved with operation challenges and several error types, the very large amounts of MT data compensate when compared to classical measurements. A few examples, based on many measured days, are demonstrated here.

I-CHANGE is funded by EU Horizon 2020 grant 101037193.

How to cite: Alpert, P., Campos, G., Haikin, N., Rubin, Y., Milelli, M., Parodi, A., and Loglisci, N.: MeteoTrackers (MT) in Citizens Science -A New Era in Micrometeorology or just an Instrument for education?Lessons from MT operations within I-CHANGE EU project , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9596, https://doi.org/10.5194/egusphere-egu25-9596, 2025.

EGU25-9681 | Orals | ITS3.4/AS4.11

The I-CHANGE Dashboard: A tool for raising awareness and triggering behavioural change 

Sasa Vranic, Joy Ommer, Milan Kalas, Paolo Mazzetti, Antonella Galizia, Antonio Parodi, Roberto Roncella, Enrico Boldrini, and Simon Smart

As urban areas face increasing threats from climate change, citizen science has emerged as an important tool to engage communities in monitoring and responding to environmental challenges, thus filling in the gap which existing tools are not addressing appropriately. Citizen science initiatives are essential for engaging citizens in climate action, involving them in environmental observations and monitoring human impacts. These participatory initiatives between science and society have gained popularity across various fields, including sociology, astronomy, and environmental protection. By involving students, citizens, and stakeholders, these initiatives foster a sense of ownership and empowerment, encouraging continued engagement and collaboration.

This paper introduces a dashboard developed within the Horizon 2020 project I-CHANGE, designed to involve citizens in the collection and analysis of environmental data. The dashboard empowers urban residents to use low-cost sensors and crowdsourced observations to gather vital information on air quality and climate variables. Co-designed with scientists and stakeholders, the dashboard provides an intuitive platform for citizens to view, understand, and interpret complex collected data. By presenting crowdsourced data in a meaningful manner, the dashboard bridges the knowledge-action gap, fostering greater public awareness and environmental consciousness. Such participatory approach increases the level of understanding of urban climate risks and strengthens adaptation strategies by integrating local insights and vulnerabilities.

Through the active involvement of citizens in data collection, the dashboard promotes hands-on experience with the real effects of climate change, leading to increased awareness and climate-friendly behaviours. This engagement is essential for achieving climate mitigation goals and advancing Europe's climate adaptation strategies. The paper discusses the design, implementation, and data integration of the dashboard, highlighting its role in combating misinformation and supporting community-driven climate action.

How to cite: Vranic, S., Ommer, J., Kalas, M., Mazzetti, P., Galizia, A., Parodi, A., Roncella, R., Boldrini, E., and Smart, S.: The I-CHANGE Dashboard: A tool for raising awareness and triggering behavioural change, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9681, https://doi.org/10.5194/egusphere-egu25-9681, 2025.

EGU25-10030 | ECS | Posters on site | ITS3.4/AS4.11

Indoor heat in Amsterdam during a heatwave: Comparing observed indoor air temperatures from a professional network and from a citizen science approach 

Gert-Jan Steeneveld, Esther Peerlings, Saša Vranic, Joy Ommer, and Milan Kalas

Ongoing climate change is increasing summertime temperatures, and frequency and intensity of heatwaves in Europe, which can threaten human health. Relatively little is known about how quickly outdoor heat penetrates into residences during heatwaves. Long-term and systematic networks recording indoor temperatures are challenging to install and maintain, and therefore scarce. We first report on crowdsourced indoor air temperature data in residences in Amsterdam (The Netherlands) during a heatwave event in September 2023. These data complement professional long-term indoor air temperature observations in 92 houses in Amsterdam. Second, we document the lessons learnt in the design and execution of this citizen science activity. 571 indoor temperature records were collected through the citizen science crowdsourcing approach, with a median value of 28.0 °C on the warmest day in the study period, while outdoor mean minimum and maximum temperatures reached 20.6 °C and 31.1 °C respectively. The results indicate that the crowdsourcing approach reports temperatures that are significantly higher than the professional approach, which supports the need for professional indoor networks. Finally, local media attention was critical in reaching a wide audience.

How to cite: Steeneveld, G.-J., Peerlings, E., Vranic, S., Ommer, J., and Kalas, M.: Indoor heat in Amsterdam during a heatwave: Comparing observed indoor air temperatures from a professional network and from a citizen science approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10030, https://doi.org/10.5194/egusphere-egu25-10030, 2025.

EGU25-10110 | ECS | Posters on site | ITS3.4/AS4.11

Our Climate Story: Exploring local climate challenges and solutions through serious gaming 

Joy Ommer, Catharina Dörr, Antonella Galizia, Mattia Fortunati, Caroline Bertram, and Milan Kalas

Cities are disproportionately affected by climate change due to their dense populations, concentrated infrastructure, and unique urban microclimates, which can exacerbate climate risks such as heatwaves, air pollution, and flooding. The European Climate Adaptation Strategy emphasises the importance of local-level action, community engagement, and innovative tools to foster resilience. In this context, Our Climate Story - a serious game developed under the H2020 I-CHANGE project - serves as an interactive and educational tool to raise awareness, promote sustainable behaviours, and empower citizens to address urban climate risks collaboratively.

Urban climate risks pose significant threats to public health, particularly for vulnerable populations. This current and future challenge underscores the need for a deeper understanding of local vulnerabilities and susceptibilities, which often go beyond what is captured by traditional data-driven risk mapping. Our Climate Story bridges this gap by combining participatory science methods with storytelling and gaming.

The serious game incorporates participatory mapping, a method that invites players to co-create a visual representation of their city, identifying local hazards such as flood-prone areas, pollution hotspots, and heat islands. This mapping process allows participants to draw on their experiences and local knowledge as well as enhance intergenerational learning. In addition, Our Climate Story encourages participants to brainstorm solutions such as enhancing public transportation or adopting Nature-based Solutions to mitigate hazards. These discussions encourage active involvement, critical thinking, and collaborative decision-making.

The participatory nature of Our Climate Story goes beyond simply raising awareness. It instils a sense of responsibility for the environment by making the impacts of climate change tangible and personal. Players witness how their actions such as choosing sustainable transportation or reducing waste contribute to mitigating climate risks. This approach aligns with the European Union’s goals of promoting greater environmental awareness but also citizen-driven action.

By integrating scientific concepts with interactive gameplay, Our Climate Story demonstrates that addressing urban climate risks requires not only top-down policy interventions but also bottom-up community engagement and co-created solutions. It showcases the potential of participatory science and gamification to bridge the gap between knowledge and action, inspiring both individual and collective efforts to build climate-resilient cities.

How to cite: Ommer, J., Dörr, C., Galizia, A., Fortunati, M., Bertram, C., and Kalas, M.: Our Climate Story: Exploring local climate challenges and solutions through serious gaming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10110, https://doi.org/10.5194/egusphere-egu25-10110, 2025.

EGU25-10492 | Orals | ITS3.4/AS4.11

Mapping urban heat islands in Padua (Italy): perspectives and trends of climate extremes in a changing climate 

Salvatore Eugenio Pappalardo, Andrea Santaterra, Francesco Facchinelli, Carlo Zanetti, Massimo De Marchi, and Alessandro Ceppi

The Mediterranean Basin is widely recognized as a significant hotspot for the impacts of climate change. Extreme meteorological events, such as heatwaves, exacerbate the phenomenon of urban heat islands (UHI), dramatically increasing climate risks, particularly in high-density urban areas. The combined effects of heatwaves and UHI are negatively impacting urban infrastructure and public health in numerous metropolitan regions.
This study aims to identify, quantify, and map UHI in the city of Padua (Northeast Italy) over recent decades, with a focus on climate extremes related to heatwaves, such as tropical nights and hot days.
The research analyzes and geovisualizes thermal anomalies in the complex urban environment, emphasizing sealed surfaces, rural areas, and watercourses. A reference dataset from an official weather station in Legnaro, operated by ARPA-Veneto, provides comprehensive data spanning 30 years (1993–2022). To gain a broader perspective on temperature variations across the urban area, the study also incorporates high-resolution data (100 m) from the ERA5 climate model for the period 2008–2017. Additionally, three citizen-science meteorological stations from the Meteonetwork association—located in distinct urban contexts (Portello, Basso Isonzo and Montà districts)—contribute localized climatological data, with particular emphasis on the exceptionally hot summer of 2022, recorded as the hottest on record.
The findings highlight the significant impacts of climate extremes on the city and its residents, including a detailed estimation of the urban population exposed to these conditions.

How to cite: Pappalardo, S. E., Santaterra, A., Facchinelli, F., Zanetti, C., De Marchi, M., and Ceppi, A.: Mapping urban heat islands in Padua (Italy): perspectives and trends of climate extremes in a changing climate, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10492, https://doi.org/10.5194/egusphere-egu25-10492, 2025.

EGU25-10503 | Posters on site | ITS3.4/AS4.11

 ChallengeYeti App: Bridging the Knowledge-Action Gap through Gamification and Digital Engagement  

Milan Kalas, Joy Ommer, Sasa Vranic, Muhammad Adnan, Carlo Trozzi, Laura Polo, Erika Brattich, Silvana Di Sabatino, and Antonio Parodi

Climate change mitigation campaigns aim to raise awareness, increase knowledge, and communicate actions for reducing carbon footprints. Unfortunately, these top-down campaigns often fail to engage the public effectively. To address this issue, the I-CHANGE project developed the ChallengeYeti app, an innovative solution designed to fill the knowledge-action gap by empowering and motivating citizens to take climate action through participatory and gamification approaches. 

The ChallengeYeti app leverages digital tools and gamification to foster behavioural change. Rooted in the COM-B theory of behaviour change, the app focuses on three components: capability, opportunity, and motivation. By incorporating game elements, the app stimulates intrinsic motivation through social interaction and extrinsic motivation through competition and rewards. This approach ensures long-term user engagement and sustainable impact. 

Unlike traditional carbon footprint calculators that focus on specific aspects such as transport or energy efficiency, the ChallengeYeti app offers a comprehensive platform for tracking both avoided and produced carbon footprints. The app presents data in a clear and understandable format, enabling users to grasp the context and take informed actions. Additionally, the app promotes user engagement through a series of challenges and the creation of communities, fostering competition and collective action. 

How to cite: Kalas, M., Ommer, J., Vranic, S., Adnan, M., Trozzi, C., Polo, L., Brattich, E., Di Sabatino, S., and Parodi, A.:  ChallengeYeti App: Bridging the Knowledge-Action Gap through Gamification and Digital Engagement , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10503, https://doi.org/10.5194/egusphere-egu25-10503, 2025.

EGU25-10602 | Posters on site | ITS3.4/AS4.11

The I-CHANGE Environmental Impact Hub (EIH) 

Roberto Roncella, Enrico Boldrini, Fabrizio Papeschi, Paolo Mazzetti, Simon Smart, Thomas Hodson, Saša Vranic, Antonella Galizia, Nicola Loglisci, and Antonio Parodi

The I-CHANGE (Individual Change of HAbits Needed for Green European transition) project is a 3.5-year Innovation Action initiative, funded under the European Union's Horizon 2020 programme, concluding in April 2025. It aims to engage citizens actively in environmental monitoring and climate action, demonstrating that individual behavioral changes, facilitated through citizen science initiatives utilizing sensors and monitoring devices, can significantly reduce environmental footprints. The project establishes Living Labs (LLs) as collaborative spaces where researchers and communities engage in scientific discourse, sharing insights and outcomes.

Central to I-CHANGE is the Environmental Impact Hub (EIH), a comprehensive data infrastructure designed to collect data, provide tools, and support initiatives facilitating citizens to participate in environmental monitoring and action. The EIH is a data hub that effectively shares, manages, and processes diverse datasets, ensuring interoperability and usability of heterogeneous data. It supports machine-to-machine interactions to facilitate the development of desktop and mobile applications through dedicated service interfaces and APIs. The EIH is built of discrete components, including the Data and Information Broker - based on the pre-existing Discovery and Access Broker (DAB) - which facilitates seamless discovery and access to diverse data sources, including in-situ measurements, citizen-provided data, and European infrastructures; the Citizen Observatory Archive which ingests, quality-checks, and stores observations generated by the LLs; the Dashboard which supports visualization of environmental data and empowers citizens to monitor and understand their environmental impact with intuitive and user-friendly interfaces, near real-time analytics, and actionable insights, enabling users to explore the environmental consequences of their actions and track improvements over time. The EIH offers multiple interfaces to support a wide range of use cases and interaction types. These include geospatial interfaces adhering to standards (such as those from OGC and ISO), a Web API for easy web development integration, and a RESTful API for exchanging JSON data across various platforms.

I-CHANGE is predicated on the belief that citizens and civil society play a central role in environmental protection and climate action. As direct involvement of private citizens is considered essential to drive meaningful shifts towards more sustainable behavior, I-CHANGE presents a comprehensive effort to engage citizens in environmental monitoring and action, by providing both advanced technological platforms and participatory Living Labs. The EIH supports this vision by providing the underpinning technical infrastructure. By facilitating access to diverse data and tools, and promoting citizen involvement, I-CHANGE aims to empower individuals to make informed decisions that contribute to environmental sustainability, mitigating environmental challenges, and advancing climate action.

How to cite: Roncella, R., Boldrini, E., Papeschi, F., Mazzetti, P., Smart, S., Hodson, T., Vranic, S., Galizia, A., Loglisci, N., and Parodi, A.: The I-CHANGE Environmental Impact Hub (EIH), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10602, https://doi.org/10.5194/egusphere-egu25-10602, 2025.

EGU25-11243 | ECS | Posters on site | ITS3.4/AS4.11

Integrated modelling chain for tailored traffic policy interventions 

Francesco Barbano, Erika Brattich, Muhammad Adnan, Carlo Trozzi, Enzo Piscitello, Rita Vaccaro, Carlo Cintolesi, Antonio Parodi, and Silvana Di Sabatino

Urbanization brings a set of challenges that demand innovative and comprehensive solutions. Among these, sustainable mobility and air pollution mitigation are the most pressing ones, both tackled by the European Green Deal that advocates for Europe's climate neutrality by 50. The EU framework only sets the target goal for air quality and pollutant emissions, but the single member states are empowered to define their mobility strategy and define national and local policies. Therefore, a proper design and implementation of strategic initiatives must be tailored to the needs of local settlements and communities. Numerical models offer the possibility to test realistic strategies and evaluate their benefits by simulating realistic scenarios, including individuals’ and communities’ behavioural changes in response to strategy implementation. This study proposes an integrated modelling chain developed within the I-CHANGE (Individual Change of Habits Needed for European Green Transition) EU Horizon 2020 project to estimate the role and impact of behavioural change for the mitigation of CO2, greenhouse gases, short-lived climate forcers and air pollutants associated with road traffic. The modelling chain is modular and suitable to simulate the current status and hypothetical policy scenarios: it composes of an activity-based model, deriving the traffic flow generated by the citizens’ daily habits, an emission model, extrapolating the emission inventory of the target atmospheric compounds which are finally used by a dispersion model to derive the air pollutants concentration and spatial distribution. Rooted in numerical models at the state-of-the-art and well-consolidated analytical methods, citizens sustain the chain will and stakeholder needs to frame the necessary policy interventions. ntions. The outcome of the modelling chain is twofold: (i) bringing evidence on the efficiency of designed mitigation strategies and (ii) demonstrating to the public that mitigation can be pursued, incentivizing the necessary behavioural change it might require.  

The methodology here presented is applied to evaluate four policy scenarios tested in the city of Bologna (IT), Dublin (IE) and Hasselt (BE). The output allows to elaborate potential advantages and disadvantages in terms of mobility, air quality and behavioural change the cities would face. Specifically, the policy scenarios envision new bicycle infrastructure in designated areas (policy 1), Low Emission Zones in the city centre (policy 2), time-based restrictions on car and private vehicle usage near schools (policy 3) and flexible working hours/working from home schemes (policy 4). Depending on the scenario, policies implementation can introduce notable impacts on (local) concentrations. Specifically, policy scenarios tend to lead to lower peaks of pollutant concentration levels in the areas where policies are implemented, counterbalanced by minor concentration increases in other areas. These insights facilitate evidence-based policy adjustments, enabling decision makers to address the complexities of urban development while fostering resilient, inclusive, and environmentally conscious communities.  

How to cite: Barbano, F., Brattich, E., Adnan, M., Trozzi, C., Piscitello, E., Vaccaro, R., Cintolesi, C., Parodi, A., and Di Sabatino, S.: Integrated modelling chain for tailored traffic policy interventions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11243, https://doi.org/10.5194/egusphere-egu25-11243, 2025.

EGU25-11392 | Orals | ITS3.4/AS4.11

Drivers and Barriers to Sustainable Behaviors Among Youth in Climate-Vulnerable Urban Areas: Insights from Chiavari, Italy 

Simone Sterlacchini, Debora Voltolina, Umberto Mezzacapo, Christian N. Gencarelli, Giuseppe Esposito, Alessandro Mondini, Paola Salvati, Selene Tondini, Teresa Carlone, Alessandro Sarretta, Antonella Galizia, and Ivan Marchesini

Urban areas, increasingly exposed to climate change, demand innovative strategies for public engagement and adaptive behavior. This research investigates the drivers and barriers influencing sustainable behaviors among young people in Chiavari, Italy, a climate-vulnerable city frequently impacted by extreme weather events such as floods and wildfires. Utilizing the Capability, Opportunity, Motivation-Behavior (COM-B) model, this study sheds light on the personal, social, and contextual factors shaping pro-environmental behaviors, offering a framework for participatory science to address urban climate challenges.

Quantitative surveys and focus groups involving over 470 secondary students (ages 15–17) and 117 young adults (ages 18–35) reveal distinct patterns of awareness, motivation, and behavioral change. A critical finding is the role of lived experience: young adults, many of whom experienced Chiavari’s severe flash floods in 2002 and 2014 or nearby wildfires, exhibit heightened sensitivity and awareness compared to students, who were too young to remember or directly experience these events. This suggests that direct exposure to extreme weather events significantly enhances motivation and fosters a deeper understanding of the importance of sustainable behaviors. "Capability" (knowledge and skills) emerges as the cornerstone for fostering motivation, while substantial barriers—including limited educational integration, insufficient resources, and inadequate community infrastructure—hinder the translation of awareness into impactful actions.

The research highlights the value of participatory tools in bridging knowledge-action gaps. School-driven discussions, citizen science projects, and locally contextualized interventions emerge as critical avenues for empowering youth. Focus group insights reveal that perceived social disapproval, the absence of practical tools, and skepticism about systemic effectiveness (e.g., EU climate goals) further challenge sustainable behavior adoption. However, nearly 70% of students express readiness to adopt sustainable mobility options, such as public transportation and cycling, underscoring their potential as agents of change in climate-resilient urban planning.

Findings advocate for participatory science to elevate awareness and foster local climate adaptation. This approach integrates simple yet effective community tools and data-driven insights to create actionable interventions. The COM-B framework proves instrumental in identifying leverage points, such as linking extreme event experiences (floods and wildfires) to awareness campaigns or targeting reflective motivations to enhance community engagement. Moreover, the research suggests that localized interventions incorporating cultural and socio-economic nuances significantly enhance the efficacy of sustainable behavior programs.

How to cite: Sterlacchini, S., Voltolina, D., Mezzacapo, U., Gencarelli, C. N., Esposito, G., Mondini, A., Salvati, P., Tondini, S., Carlone, T., Sarretta, A., Galizia, A., and Marchesini, I.: Drivers and Barriers to Sustainable Behaviors Among Youth in Climate-Vulnerable Urban Areas: Insights from Chiavari, Italy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11392, https://doi.org/10.5194/egusphere-egu25-11392, 2025.

EGU25-12498 | ECS | Posters on site | ITS3.4/AS4.11

The I-CHANGE MOOC: ensuring cross-fertilisation and knowledge-sharing on citizen science for climate action and risk prevention beyond European Living Labs. 

Juan Esteban Quintero-Marín, Anna Mölter, Nicola Loglisci, Lara Polo, Muhammad Adnan, Maria Carmen Llasat, Laura Esbrí, Francesco Barbano, Erika Brattich, Carlo Cintolesi, Selene Tondini, Teresa Carlone, Silvana Di Sabatino, Gert-Jan Steeneveldg, and Esther E.M Peerlings

The I-CHANGE project aims to demonstrate that individual behavioural change through awareness generated by citizen science activities can ultimately contribute to a collective reduction in environmental footprints. The project, which operates through Living Labs (LLs), has as one of its main challenges to take the learning accumulated in 3.5 years beyond the LLs and reach as many people as possible. To maximise the project's learnings, a Massive Open Online Course (MOOC) was developed. Its objectives include enhancing knowledge of: 1) the global context of climate change, 2) critical local climate change issues and related natural hazards in each LL, 3) the significance of behavioural change, and 4) the role of citizen science in climate awareness and action, as well as accessing information produced by I-CHANGE and other open sources of citizen science data. The I-CHANGE MOOC was co-developed collaboratively by project partners and offers concise and practical lessons encapsulating key project learned lessons. 

The methodology for designing the MOOC involved a first scoping meeting, in which a preliminary table of contents was designed and feedback was received from the project partners. The table of contents was shared and improved over several months. The MOOC topics were distributed among the different LLs according to their local climate-change-related hazards, resulting in specific content about heatwaves, air pollution, and flooding authored by renowned academics. The structure of each topic has been designed innovatively, with three short sections covering the three topics: The Science (defining the issue and its causes), The Action Tools (description and utility of the technological tool used to address specific environmental challenges through citizen science) and The Change (specific actions that citizens can take to tackle this problem and successful examples from the project). 

The MOOC was a successful way to summarise key learnings, maximise the media produced in the project, and disseminate some of the dissemination outputs, including animated videos, interviews, a serious game, the Citizens4Climate dashboard, and the YetiApp for calculating environmental footprints. The production of the MOOC took a total of 8 months from the first draft to publishing the course online. Some of the challenges during the process involved synthesising a large amount of information, writing informative yet concise and engaging texts, and making decisions about accessibility and language. Challenges in the dissemination stage are associated with the number of participants expected to be reached. 

The MOOC is hosted on the Thinkific platform and became publicly available on October 24, 2024. Dissemination efforts are ongoing through the project's social media channels and European citizen science portals. To meet project goals, a target audience of 1,000 participants has been established to be monitored using Thinkific analytics. Further work will continue to disseminate the MOOC to various sectors of society. and the international English-speaking audience. 

How to cite: Quintero-Marín, J. E., Mölter, A., Loglisci, N., Polo, L., Adnan, M., Llasat, M. C., Esbrí, L., Barbano, F., Brattich, E., Cintolesi, C., Tondini, S., Carlone, T., Di Sabatino, S., Steeneveldg, G.-J., and Peerlings, E. E. M.: The I-CHANGE MOOC: ensuring cross-fertilisation and knowledge-sharing on citizen science for climate action and risk prevention beyond European Living Labs., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12498, https://doi.org/10.5194/egusphere-egu25-12498, 2025.

EGU25-13390 | Posters on site | ITS3.4/AS4.11

Citizen science in action: air pollution campaigns and thermal comfort assessment from I-CHANGE Day  

Maria-Carmen Llasat, Laura Esbrí, Montserrat Llasat-Botija, Yolanda Sola, Edson Plasencia, Carlo Guzzón, Gert-Jan Steeneveld, Esther Peerlings, Bio Mohamadou Torou, Muhammad Adnan, Anna Mölter, Juan Esteban Quintero, Pinhas Alpert, Gabriel Campos, Lara Polo, Nicola Loglisci, Carlo Citolesi, Erika Brattich, Silvana Di Sabatino, and Antonio Parodi and the I-CHNAGE Living Labs teams

Citizen science has become an essential tool for addressing urban climate challenges, engaging communities, and fostering behavioural change. The I-CHANGE project (Individual Change of HAbits Needed for Green European transition) integrates participatory approaches across eight international Living Labs (LLs) to enhance urban climate resilience and encourage shifts toward sustainable behaviours. As part of this effort, the I-CHANGE Day initiative promoted awareness and action through coordinated citizen-led experiments 

The event featured two major activities: (1) the Air pollution campaign with Smart Citizen Kits (SCKs) and (2) the Temperature and humidity perception experiment. Both activities were co-designed with LL leaders, whose expertise included urban heat, air quality, sociology, and citizen science, ensuring adaptability across diverse socio-cultural contexts. 

The SCK campaign deployed 14 low-cost sensors in five cities (Barcelona, Bologna, Dublin, Genoa, and Ouagadougou) at representative urban locations volunteered by LL participants and stakeholders. These sensors measured air quality parameters, including particulate matter and CO₂ levels, during a common monitoring period. Data were integrated into the I-CHANGE dashboard to foster discussions on air pollution among LL participants. Results highlighted the critical role of urban green spaces in mitigating air pollution, evidenced by lower pollutant levels in these areas. Community involvement was key, with local stakeholders participating in sensor installation and data interpretation workshops. 

The Temperature and Humidity Perception Experiment engaged over 100 participants in seven LLs (Amsterdam, Barcelona, Bologna, Dublin, Genoa, Hasselt, and Jerusalem). Using portable MeteoTracker devices while biking or walking, participants mapped temperature and humidity in their neighbourhoods, recorded thermal comfort perceptions, and identified vulnerable areas. Discrepancies between perceived and measured temperature, particularly in highly urbanized areas, provided valuable insights for urban planning and climate resilience strategies. 

Both activities demonstrated the transformative potential of citizen science for understanding and addressing urban climate risks. By fostering hands-on engagement, I-CHANGE Day not only enhanced climate literacy but also inspired community-driven solutions for sustainable urban living. This initiative underscores the importance of integrating participatory approaches in scientific research to promote collective climate action. 

 

The I-CHANGE project has received funding from the European Union’s Horizon 2020 Research and Innovation programme under grant agreement 101037193. 

How to cite: Llasat, M.-C., Esbrí, L., Llasat-Botija, M., Sola, Y., Plasencia, E., Guzzón, C., Steeneveld, G.-J., Peerlings, E., Torou, B. M., Adnan, M., Mölter, A., Quintero, J. E., Alpert, P., Campos, G., Polo, L., Loglisci, N., Citolesi, C., Brattich, E., Di Sabatino, S., and Parodi, A. and the I-CHNAGE Living Labs teams: Citizen science in action: air pollution campaigns and thermal comfort assessment from I-CHANGE Day , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13390, https://doi.org/10.5194/egusphere-egu25-13390, 2025.

EGU25-17092 | ECS | Orals | ITS3.4/AS4.11

Best Practices for Citizen Engagement in Climate Change Adaptation 

Eulàlia Baulenas and Samuel Pickard

Effective citizen engagement is pivotal in driving successful climate change adaptation efforts. This study is part of the Mission Adaptation AGORA project (A Gathering place to cO-design and co-cReate Adaptation), which aims to strengthen citizen engagement in climate adaptation by developing innovative methodologies and frameworks that enhance public participation. By focusing on co-creation and knowledge-sharing, AGORA supports the development of climate-resilient communities through the integration of diverse perspectives and local insights. Here, we present the results of our efforts to synthesize findings from two years of research – including expert surveys, interviews, and peer-learning workshops – to identify best practices and challenges in citizen engagement initiatives (CEIs). Our analysis, which covers a wide variety of participatory approaches to citizen engagement, highlights the necessity of a few universal principles to follow in order to foster effective participation. These include setting clear objectives, investing in tailored communication strategies, taking goal-dependent design choices, and the mindful consideration and involvement of the different actors involved in all stages of preparing, carrying out and participating in the CEI. Additionally, the study underscores the importance of understanding contextual factors, such as local socio-economic conditions or the familiarity  of the local political system with  deliberative democratic processes, when designing and implementing impactful CEIs. Despite good intentions and intensive research and hands-on experience attempting to overcome them, we find that persistent challenges remain, particularly in reaching marginalized groups and translating engagement outcomes into policy actions. 

Our recommendations stemming from this study aim to provide adaptable engagement frameworks that strengthen democratic processes, inclusivity, and climate resilience, offering practical guidance for policymakers and practitioners seeking to engage citizens in the field of climate adaptation. By creating tailored guidance depending on the intended goal and context, we hope to inform design choices of a wide range of citizen engagement approaches, ranging from awareness raising and ideation, to citizen science and knowledge co-production, to shared decision making for climate adaptation action. 

How to cite: Baulenas, E. and Pickard, S.: Best Practices for Citizen Engagement in Climate Change Adaptation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17092, https://doi.org/10.5194/egusphere-egu25-17092, 2025.

EGU25-18817 | ECS | Orals | ITS3.4/AS4.11

Community-Centric Rainfall Monitoring for Climate Awareness and Urban Flood Mitigation Advocacy 

Salman Khan, Nasim Eslamirad, Payam Sajadi, and Fiachra O’Loughlin

Accurate rainfall measurement, particularly at high spatiotemporal resolution, is crucial for urban flood monitoring. However, traditional methods of obtaining rainfall data are often inaccessible, costly, or inadequate for capturing localised flooding events. Low-cost weather stations (LCWS) can provide a viable solution, promoting public awareness and engagement with climate-related issues, including flooding, amidst growing urbanisation. This study shows the important role individual citizens can play in monitoring rainfall and contributing to flood mitigation measures. A total of 40 LCWS were deployed across Dublin to monitor rainfall at 5-minute intervals. The recorded rainfall data were compared with measurements from three nearby reference stations (RefS) operated by Met Éireann, as well as satellite rainfall data from the Global Satellite Mapping of Precipitation (GSMaP), focusing on extreme events and hourly scales. Various performance indicators, were used to evaluate the accuracy of LCWS relative to the RefS. Overall, LCWS demonstrated closer alignment with the RefS, achieving higher CC (0.43 vs 0.26) and Probability of Detection (POD) (0.49 vs 0.23) values, along with lower Percent Bias (14.7 vs -48.3%) and False Alarm Ratio (FAR) (0.27 vs 0.38) values, compared to the GSMaP data. Moreover, POD values (FAR values) showed a decreasing (increasing) trend with distance from the RefS, representing the spatial variability of rainfall. Additionally, citizens’ engagement was assessed through a survey with preliminary results revealing that nearly 60% of homeowners observed intense rainfall events being recorded by their stations during the study period. 78.6% of respondents reported an increased interest in climate change and urban flooding, while 57% expressed a growing interest in advocating for climate action and urban sustainability due to their participation in this project. These findings underscore the potential of LCWS in participatory monitoring and their ability to drive advocacy for climate action and urban flood mitigation.

How to cite: Khan, S., Eslamirad, N., Sajadi, P., and O’Loughlin, F.: Community-Centric Rainfall Monitoring for Climate Awareness and Urban Flood Mitigation Advocacy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18817, https://doi.org/10.5194/egusphere-egu25-18817, 2025.

EGU25-20709 | Orals | ITS3.4/AS4.11

Flying Thermometers: How Urban-Dwelling Bats Help Map Urban Heat Islands  

Alexandra Chudnovsky, Aya Goldshtein, Limor Shashua-Bar, Yovel Yovel, and Oded Potchter

This study introduces a novel approach to reconstruct Urban Heat Islands (UHI) by leveraging urban-dwelling bats as biologically-assisted samplers (BAS), offering a unique perspective similar to urban residents. Using Egyptian fruit bats equipped with temperature loggers, we mapped spatial air temperature (Tair) profiles across diverse urban environments. To evaluate the feasibility of this method, we employed mixed-effects models and Geographically Weighted Regression (GWR) to analyze the influence of urban features on Tair distribution. Vegetation emerged as a critical factor in mitigating urban heat, with winter Tair differences of 2–5 °C observed between dense urban areas and adjacent vegetative or open spaces. A prominent UHI hotspot was identified in winter over the Ayalon highway, while differences were less pronounced during summer nights due to coastal cooling from sea breezes. Preliminary results further reveal a unique 3D perspective of UHI: Tair variations above dense urban areas were smaller compared to vegetative zones.

This approach demonstrates that urban bats, as local "residents," can act as efficient agents for atmospheric monitoring, complementing low-cost citizen science initiatives to gather environmental data. However, challenges associated with crowdsourced data collection, such as ensuring data accuracy, coverage, and integration with bat-derived scans, highlight the need for robust data validation frameworks. Despite these challenges, the synergy between bats and citizen science offers valuable insights into local vulnerabilities and informs targeted mitigation strategies, particularly during nocturnal hours when UHI effects are most pronounced.

 

How to cite: Chudnovsky, A., Goldshtein, A., Shashua-Bar, L., Yovel, Y., and Potchter, O.: Flying Thermometers: How Urban-Dwelling Bats Help Map Urban Heat Islands , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20709, https://doi.org/10.5194/egusphere-egu25-20709, 2025.

EGU25-21112 | Orals | ITS3.4/AS4.11

A cross European participatory approach to addressing urban climate risks, lessons learned from the Adaptation AGORA’s pilot regions 

Riccardo Biondi, Alfredo Reder, Paola Mercogliano, Arianna Acierno, Marina Mattera, Marianna Adinolfi, Marta Ellena, and Antonella Mele

Urban areas and their populations across Europe are increasingly dealing with climate change effects, including increased risks of flooding, rising sea levels, heatwaves and more severe storms, which disproportionately affect vulnerable populations. Urbanization further amplifies these effects by significantly altering landscapes and influencing local atmospheric conditions. Addressing these complex dynamics requires a comprehensive understanding of the intricate interplay between urbanization and climate change. Sustainable solutions must integrate climate considerations and resilience measures into urban planning, ensuring cities can adapt to the evolving environmental pressures. 

Adaptation AGORA project engages citizens through participatory methodologies and co-creation strategies to foster, among others, urban climate adaptation initiatives and resilience. By enhancing knowledge and raising awareness among planners, policymakers, and stakeholders, it becomes possible to integrate climate-responsive strategies into the planning process of climate-resilient infrastructure.

Recently in a peer-to-peer learning exchange event, Malmö (pilot city within Adaptation AGORA) and Valencia (one of the project’s Followers), have shared challenges, tools and practices aimed at addressing heat vulnerability and fostering the engagement of vulnerable communities in heatwaves preparedness and response. These initiatives have explored strategies to reduce the impacts of extreme heat, especially on vulnerable populations. Cities need to embed heat adaptation into urban infrastructure and planning, including among others low-tech cooling solutions, and upscaling cooling shelters. By sharing insights and learning from one another, cities like Malmö and Valencia are paving the way for equitable and innovative approaches to urban heat resilience. Their experiences underscore the importance of cross-sector collaboration and community participation in tackling the climate challenges of the future.  

In Rome, another AGORA pilot city, citizens joined the consultation process of the City’s climate adaptation strategy, offering their contribution to the development of the plan. This participatory approach incorporated community insights and needs  into local vulnerabilities, enhancing the relevance and impact of proposed measures. Workshops, focus groups, and collaborative discussions in Rome fostered a deeper understanding of urban climate challenges and empowered communities to play an active role in shaping adaptation solutions.

This presentation will highlight AGORA’s participatory approach to addressing urban climate risks, with a focus on pilot initiatives and community engagement in adaptation planning. It will explore and discuss best practices for involving communities in sustainable adaptation strategies.

How to cite: Biondi, R., Reder, A., Mercogliano, P., Acierno, A., Mattera, M., Adinolfi, M., Ellena, M., and Mele, A.: A cross European participatory approach to addressing urban climate risks, lessons learned from the Adaptation AGORA’s pilot regions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21112, https://doi.org/10.5194/egusphere-egu25-21112, 2025.

EGU25-21125 | Posters on site | ITS3.4/AS4.11

Digital tools for capacity building, a tangible support for citizens to tackle climate disinformation and be more resilient 

Massimo Milelli, Paola Mercogliano, Alfredo Reder, Arianna Acierno, Marina Mattera, Marianna Adinolfi, Marta Ellena, Antonella Mele, Jorge Barba, Spyridoula Markou, and Adam Doulgerakis

Misinformation and disinformation present significant barriers to addressing climate change and effectively communicating risks. While misinformation refers to false or inaccurate information shared without intent to mislead, disinformation involves deliberately false narratives designed to deceive and manipulate. Both phenomena distort public perception, erode trust in scientific and institutional sources, and delay critical action. When people encounter conflicting or false information, they may struggle to discern credible guidance, making them less likely to act appropriately. Furthermore, both phenomena can polarize public opinion, making collective action more difficult. To counter them, it is essential to provide clear, reliable, and timely information while promoting media literacy.

Effective communication must proactively address false narratives while promoting clear, evidence-based messaging that empowers informed decision-making. The empowerment of citizens' role is closely linked to strengthening citizen resilience against climate change disinformation, which is one of the main focuses of the Adaptation AGORA project. Adaptation AGORA supports the overall objectives of the Mission on Adaptation to Climate Change by advancing best practices, innovative approaches, policy instruments and governance mechanisms. These efforts aim to effectively engage communities and regions in climate actions, accelerating and upscaling adaptation processes for building a climate resilient Europe.

In this framework, the project developed a "Digital AGORA", as an integrated discussion and learning space, a living environment co-designed with stakeholders. This resource hub hosts two “Digital Academies” to support citizens and stakeholders to access open-source climate data for adaptation and tackle climate change disinformation.

The AGORA Digital Academy against Climate Change Disinformation is designed to equip participants with reliable, fact-checked data and information from credible sources, enhancing their critical thinking and their ability to counter misleading narratives. Furthermore, the project has been developing a mobile app to tackle climate disinformation. The gamified mobile app aims to support the education of citizens on climate change adaptation and counter disinformation campaigns through an entertaining and engaging approach. The app will be officially released in April 2025. 

The Academy emphasizes improving media literacy and critical thinking skills among citizens, policymakers, and other stakeholders. Through interactive training modules and educational materials, participants gain the tools needed to identify and address the spread of disinformation. Using interactive tools, workshops, and adaptable communication frameworks, they are equipped to apply these skills in their own communities, ensuring that solutions are both actionable and relevant.

This presentation will focus on the AGORA Digital Academy against Climate Change Disinformation as a case study, illustrating its efforts to tackle the growing challenge of disinformation. Drawing on experiences from pilot regions, it will explore effective practices and key takeaways, with a focus on challenges such as cognitive biases, the role of media and enhancing media literacy, and socio-political dynamics.

By emphasizing inclusivity and collaborative approaches, the Adaptation AGORA project demonstrates the power of community engagement in combating misinformation. This session will present innovative tools and methods developed by the AGORA team to support informed decision-making and build resilience against climate disinformation.

How to cite: Milelli, M., Mercogliano, P., Reder, A., Acierno, A., Mattera, M., Adinolfi, M., Ellena, M., Mele, A., Barba, J., Markou, S., and Doulgerakis, A.: Digital tools for capacity building, a tangible support for citizens to tackle climate disinformation and be more resilient, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21125, https://doi.org/10.5194/egusphere-egu25-21125, 2025.

EGU25-21602 | Orals | ITS3.4/AS4.11

Unveiling the climate – health nexus through citizen science: the TRIGGER Climate Health ConnectionLabs 

Maria Carelli, Erika Brattich, Igor Dienberger, Valerio Carelli, Emmanouil Galanakis, Eleni Dimitriou, Andreas Hoffmann, Muhammad Saleem Pomee, Elke Hertig, Alberto Spadotto, Enora Bruley, Anna Scolobig, Anna Pulakka, Sylvain Sebert, and Silvana Di Sabatino

The TRIGGER Horizon Europe project aims to enhance evidence-based connections between climate change and health threats and human well-being.

As clearly emerging in the EXPOSOME paradigm on which the project is rooted, the interactions among climate, health and ecosystems are multiple and complex, and research aiming at identification, monitoring, and quantification of impacts of climate change on human health requires the application of novel and transdisciplinary approaches. To this aim, TRIGGER has envisaged activities in a wide variety of disciplines developed in different real-world contexts considering the climatic, social, economic, and cultural richness of the European continent.

Specifically, TRIGGER has identified a set of five demonstration labs, the Climate Health Connection Labs (CHCLs) in which citizens are part of a codesign mechanism to directly monitor health, weather-climate, environmental and socio-economic data.

These labs operate in five strategically selected cities, Augsburg, Bologna, Geneva, Heraklion, and Oulu, chosen to reflect diverse climatic, socio-economic, and cultural contexts.

The objectives of the TRIGGER CHCLs are to:
• Investigate the complex interplay between climate change and health.
• Define a common language to foster collaboration among stakeholders, including medical, professionals, policymakers, climatologists, patient associations, and citizens, addressing local challenges.
• Provide a platform for interdisciplinary research and robust stakeholder engagement.

To achieve these ambitious aims, the CHCLs implement three interconnected clinical studies—RetroCLAVIS, CrossCLAVIS, and LongCLAVIS, which collectively provide a comprehensive understanding of the climate-health interplay. Each study contributes unique insights while building upon the others to create an integrated, multi-layered approach to identifying risk profiles and actionable interventions.

RetroCLAVIS:
• Retrospectively analyzes pre-existing lifelong health and environmental data.
• Identifies long-term trends and emerging health threats, providing a temporal context to complement acute and longitudinal findings.

CrossCLAVIS:
• Serves as the foundation by analyzing cardiovascular and respiratory disease patterns in real-time across diverse European settings.
• Investigates molecular and microbiological mechanisms, such as the respiratory microbiome and mitochondrial DNA.
• Provides baseline data to inform and validate hypotheses in RetroCLAVIS and LongCLAVIS.

LongCLAVIS:
• Extends CrossCLAVIS findings through a longitudinal study enrolling 300 healthy volunteers.
• Use wearable technology and citizen science to capture detailed data on health, personal and environmental exposures over a one-year period.
• Explores molecular and microbiological pathways underlying climate-driven disease susceptibility.

In this complex scenario, the Bologna CHCL specifically examines how extreme heat and air pollution could trigger cardiovascular and respiratory diseases. This lab combines cross-sectional and longitudinal studies, to analyze environmental exposures and health threats using harmonized datasets.

Overall, this work will present how the CHCL approach in the TRIGGER project provides an innovative, user-centered framework that integrates interdisciplinary collaboration and stakeholder engagement. By enabling capacity-building and deepening the understanding of the climate-health connection, the CHCLs deliver critical insights and practical mitigation and adaptation solutions, advancing societal preparedness for the challenges posed by climate change.

How to cite: Carelli, M., Brattich, E., Dienberger, I., Carelli, V., Galanakis, E., Dimitriou, E., Hoffmann, A., Pomee, M. S., Hertig, E., Spadotto, A., Bruley, E., Scolobig, A., Pulakka, A., Sebert, S., and Di Sabatino, S.: Unveiling the climate – health nexus through citizen science: the TRIGGER Climate Health ConnectionLabs, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21602, https://doi.org/10.5194/egusphere-egu25-21602, 2025.

EGU25-6169 | ECS | Orals | NH11.4

Importance of exposure data quality versus uncertainty in vulnerability and hazard for catastrophe modelling 

Georgios Sarailidis, Francesca Pianosi, and Kirsty Styles

Catastrophe (cat) models are widely used to combine information on the probability distribution of hazard intensity, exposure location, and exposure vulnerability to quantify risk, usually expressed in terms of financial loss. While substantial attention has been paid to improving hazard and vulnerability components (including incorporating climate change), exposure data often lags in terms of quality and detail and may vary widely in granularity and reliability. For instance, reinsurers frequently receive aggregated portfolios from insurers, which may lead to loss of critical information about location-specific risks. This lack of detail undermines the precision of loss estimates, even if hazard and vulnerability components are highly refined. This raises an important question: how influential is the level of detail exposure information on risk estimates with respect to uncertainties in vulnerability and climate change model?

In this presentation we will answer this question via a global sensitivity analysis (GSA) of the JBA flood cat model. GSA is a methodology to systematically investigate the propagation of input uncertainties through mathematical models and quantify the relative importance of those uncertainties on the variability of model outputs. Differently from local sensitivity analyses, in GSA all input uncertainties are varied simultaneously within their plausible variability ranges, instead of being varied one at the time from a baseline. This enables us to capture interaction effects between uncertain inputs and ensure that sensitivity results are not conditional on the chosen baseline. In our application, the three input uncertainties are hazard (including climate change), vulnerability, and exposure data and we quantify their relative influence on financial loss estimates.

Overall, the analysis and the results will highlight how hazard, vulnerability and exposure data quality impact loss estimates guiding cat model developers to prioritize their efforts on model improvement and reinsurers to leverage better quality exposure data.

How to cite: Sarailidis, G., Pianosi, F., and Styles, K.: Importance of exposure data quality versus uncertainty in vulnerability and hazard for catastrophe modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6169, https://doi.org/10.5194/egusphere-egu25-6169, 2025.

EGU25-6304 | ECS | Posters on site | NH11.4

Using an ensemble of flood catastrophe models to explore the interplay of loss variability and the catastrophe model calibration process 

Conor Lamb, Malcolm Haylock, Oliver Wing, and Olivia Sloan

Catastrophe (cat) models are tools, typically used in the (re)insurance industry, that evaluate the risks to a given portfolio by modelling the impact of thousands of years of synthetic hazard events. Of particular interest to users is an evaluation of the low probability (tail) risks. This includes asking questions such as, “what is the worst loss event that will be exceeded, on average, every 200 years?” 

An assessment of tail risks is inherently uncertain. This is compounded by a large number of uncertain or free parameters throughout the modelling chain which may be set via expert (subjective) judgement or via a process of calibration. The calibration process would take a given portfolio with known historical losses and adjust some of the free parameters to match the historical losses. This process may be reframed as creating a structured ensemble of catastrophe models with a range of each of the free or uncertain parameters. The process would then compare the modelled losses from each of the ensemble members to the known historical record and select the model that best represents the historical losses. 

A major limitation of the ensemble approach to catastrophe model calibration is the short historical record from which to select the most representative model. This work uses a flood catastrophe model ensemble to explore the calibration process by creating a short synthetic loss record from a single ensemble member and examining the downstream effects of using this loss record for model selection. 

How to cite: Lamb, C., Haylock, M., Wing, O., and Sloan, O.: Using an ensemble of flood catastrophe models to explore the interplay of loss variability and the catastrophe model calibration process, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6304, https://doi.org/10.5194/egusphere-egu25-6304, 2025.

EGU25-7007 | Orals | NH11.4 | Highlight

Insured Losses from European Natural Catastrophes: Is there a trend over time? 

Charlotte Milner and Kelsey Mulder

Diagnosing the drivers of changing insured losses year on year is an important component of developing a sustainable insurance portfolio. The common assumption is that losses for most perils are increasing year on year. However, there are many factors that could drive the change in losses: economic versus insured losses, impacts of inflation, changes in societal wealth over time, movement toward riskier property locations as well as potential changes in the frequency and severity of European wind and flood events. This presentation will quantify each of the above factors to determine the drivers of changes in insured losses over time.

How to cite: Milner, C. and Mulder, K.: Insured Losses from European Natural Catastrophes: Is there a trend over time?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7007, https://doi.org/10.5194/egusphere-egu25-7007, 2025.

EGU25-7030 | Posters on site | NH11.4

Disaster Risk Reduction through innovative insurance solutions  

Francesco Lo Conti, Glauco Gallotti, Antonio Tirri, Antonio Santoro, Guido Rianna, Valentina Bacciu, and Michele Calvello

The HuT (The Human-Tech Nexus) project aims at finding effective strategies to manage the risks associated with extreme climate events by means of specific demonstrators over the European territory in which different Disaster Risk Reduction strategies are prototyped and tested. In this context, we show here two distinct innovative insurance prototypes to cope with risks associated with wildfires and landslides over two peculiar areas in Sardinia and Campania regions (Italy). While the hazard posed by the two perils show distinct characteristics and origins, in both cases an insurance product can play a crucial role in the aftermath of the events for communities and private stakeholders. Since the risk assessment is crucial both in terms of financial structure and pricing strategies of a natural hazard insurance product, prototypes are developed through a Nat Cat modeling-based hazard assessment, while the vulnerability and finance considerations are related to the specific characteristics of the area of interest. Eventually, two prototypes are fully developed: “Landslide First Rescue”, a semi-parametric product designed to cope with the immediate economic needs after a landslide events; and “Fire Safe Community”, proposed as a community-based efficient tools to restore the economic losses related to wildfires. The prototypes present specific discounts if the policy holders are willing to implement risk reduction solutions to cope with the specific natural hazard. Results prove that the final premium associated with the products would be affordable and several consultations with interested stakeholders have shown how these kinds of products could also play a role in the development of nature-based solutions over broader regions.

How to cite: Lo Conti, F., Gallotti, G., Tirri, A., Santoro, A., Rianna, G., Bacciu, V., and Calvello, M.: Disaster Risk Reduction through innovative insurance solutions , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7030, https://doi.org/10.5194/egusphere-egu25-7030, 2025.

EGU25-9693 | Posters on site | NH11.4

First results from the implementation of a new fire-spread model in FireHUB platform 

Nikolaos S. Bartsotas, Themistocles Herekakis, Stella Girtsou, and Charalampos Kontoes

To mitigate the growing intensity, duration, and frequency of wildfires in recent years, leveraging the latest forecasting tools and maximizing their capabilities is essential. The FireHUB platform, provided by Beyond Operational Unit of the National Observatory of Athens, has been a reliable decision-support system utilized by numerous decision-makers and public bodies. It is also a continuously evolving platform. The most recent enhancement, implemented under the framework of the MedEWSa project, involves the deployment of a brand-new fire-spread model, offering several comparative advantages that are presented in this study.

A variety of atmospheric and soil parameters (e.g., wind, air/soil temperature and humidity, fuel density) are necessary to accurately predict fire spread information. Many of these factors are influenced by local topographical features, making high-resolution forecasts crucial. Additionally, the ability of a fire-spread model to ingest and process spatiotemporally variable fields is critical. Deploying the ForeFIRE code in combination with finer grid scales from our atmospheric operational forecasts (2-km resolution) demonstrated significant strengths over the existing system. In a series of simulated fire episodes, predictions from the old model and the new model are compared against satellite-derived burnt scar maps to evaluate their performance. The new system is expected to operate in a pseudo-operational mode alongside the existing service during the 2025 fire season and to fully replace the operational fire-spread model by 2026.

How to cite: Bartsotas, N. S., Herekakis, T., Girtsou, S., and Kontoes, C.: First results from the implementation of a new fire-spread model in FireHUB platform, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9693, https://doi.org/10.5194/egusphere-egu25-9693, 2025.

EGU25-9897 | Posters on site | NH11.4

Modelling Freeze Hazard for the North American Winters  

Mubashshir Ali, Farid Ait-Chaalal, Alison Dobbin, and Juergen Grieser

Freeze hazard represents the costliest peril associated with winter weather in the United States (US). This study focuses on the development and validation of a Freeze Index (FI) to model the impact of freeze effectively. The FI integrates both the intensity and duration of freeze events, offering a more accurate modelling of freeze hazards. The updated FI is used to select US-wide events targeting mainly the spatial scale of cold air outbreaks (CAOs). Validation of the hazard footprints is performed against historical data, including the December 2022 CAO and the Texas freeze of 2021. The findings underscore the importance of considering both temperature and duration in freeze hazards to model the damages accurately.

The freeze events obtained above are used to investigate trends in duration and FI, using 2-metre temperature (T2M) from the reanalysis data (1950 – 2024) and compared with the events from the detrended T2M. In the detrended set, no significant trend is observed in the duration of events from 1950 onwards. The average FI obtained from the footprints of each event also did not show a significant trend. The freeze events obtained from the non-detrended T2M also do not show a significant trend in duration and average FI for the events. However, there is a clear decrease in the occurrence of long-duration events with only four events greater than 10 days from 1990 onwards compared to thirteen events in the 1950 – 1985 period.

How to cite: Ali, M., Ait-Chaalal, F., Dobbin, A., and Grieser, J.: Modelling Freeze Hazard for the North American Winters , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9897, https://doi.org/10.5194/egusphere-egu25-9897, 2025.

EGU25-9927 | ECS | Orals | NH11.4

Quantifying the Impact of Recent Climate Trends on North Atlantic Hurricane Activity and Losses 

Benjamin Hohermuth, Juner Liu, Carmen Steinmann, and David N. Bresch

North Atlantic hurricanes rank among the costliest natural catastrophes globally, fuelled by high sea-surface temperatures (SST) in the main development region (MDR) and neutral to positive El Niño Southern Oscillation (ENSO). Record-high SSTs and a predicted shift to positive ENSO ahead of the 2024 season have raised concerns about a “hurricane season from hell”. A key issue is that catastrophe models used to estimate insured loss in practice are calibrated with observations dating far back and may not adequately reflect hurricane risk in today’s climate. Many scientific models focus long term climate change and are thus not fully fit to assess recent climate trends or are not openly accessible for commercial use. Therefore, we built a simplified, physically-based model conditioned on climate variables to quantify changes in hurricane risk from 1980 to today.

The model uses the physical proxies potential intensity (PI) and cyclone genesis index (CGI) calculated from ERA5, as well as hurricane observations. The number of tropical cyclones is modelled as Poisson process with mean equal to the CGI in the MDR. Locations of lifetime maximum intensities (LMI) are drawn from historical observations conditioned on MDR SST and ENSO. LMI is determined based on PI and historical LMI to PI ratios and translated into landfall activity using a statistical method. The model adequately reproduces observed basin and landfall activity when forced with historical climate conditions. By detrending each grid cell using Theil-Sen regression, we project the climate inputs to any specified year to assess climate driven risk changes.

Our results indicate a 17% increase in hurricane landfalls under the 2020 climate compared to historical forcing from 1980 to 2020, with major hurricanes potentially increasing by 22%. Adjusting landfall rates in a vendor catastrophe model accordingly leads to an increase of around 20% in average annual loss. This increase comes mainly from an increased frequency predicted by the CGI, in line with observations. Keeping CGI constant while incorporating PI increases results in fewer lower-category storms, but more categories 4 and 5 storms. Our approach has limitations, notably in translating basin to landfall activity, where we do not simulate the full tracks but rely on historical ratios to determine the landfall intensity. Consequently, shear and steering effects along the track are only implicitly considered, potentially yielding a conservative risk assessment.

Nevertheless, our results highlight a material increase in hurricane risk in the current climate relative to 1980-2020. Given the lag in most catastrophe models, modelled losses may not fully reflect today’s risk. Our methodology can also be used to extrapolate to 2050, to assess climate change impacts, an area of ongoing research.

How to cite: Hohermuth, B., Liu, J., Steinmann, C., and Bresch, D. N.: Quantifying the Impact of Recent Climate Trends on North Atlantic Hurricane Activity and Losses, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9927, https://doi.org/10.5194/egusphere-egu25-9927, 2025.

Due to its intrinsic exposure to the climate, agriculture is one of the economic sectors most directly affected by climate change. Although long-term average precipitation in Switzerland is sufficient to ensure crop production, summer drought is increasingly posing problems to the agricultural sector, as evidenced by the drought events of 2003, 2011, 2015, 2018, 2020, 2022 and again 2023. It is therefore not surprising that insurance companies in Switzerland and other European countries have added coverage to drought-induced crop yield losses to their product portfolio. However, defining viable insurance strategies for the future, from both an agronomic and economic perspective, depends on knowing the potential level of losses.

 

In this study, we assessed how climate change is likely to impact the yields of summer crops (maize and potatoes) in the four most important cropland regions in in Switzerland. Our analysis is based on the current Swiss climate scenarios (CH2018) targeting the mid-century (2050-2070) and the end of the century (2089-2099). It focuses on a representative concentration pathway (RCP) that does not envisage mitigation measures (RCP 8.5) and considers only one of the most extreme scenarios within the ensemble of available model chains. In this extreme scenario, the summer period presents a drastically negative climatic water balance (‑500 mm by the end of the century), and mean dry spell duration increasing in duration by around 50%. In the Western Plateau, these conditions entail a factor-of-two yield reduction in 60% of the years for maize and in 30% of the years for potatoes. Results further indicate that yield stability is likely to substantially decrease for both crops, as indicated by an increase in the coefficient of variation by a factor of more than two. In general, our findings stress the importance of summer crops as target of future drought-related insurance products.

How to cite: dos Reis Martins, M. and Calanca, P.: Risks from climate change for Swiss cropping systems: assessing the impacts of summer droughts on crop yields and yield stability for informing future insurance strategies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10036, https://doi.org/10.5194/egusphere-egu25-10036, 2025.

EGU25-10365 | Posters on site | NH11.4

Modeling cyclone risk variations in Australia by ENSO phases. 

Vishal Bongirwar, Lijo Abraham Joseph, Rabi Ranjan Tripathy, Daniel Martin Kalbermatter, Tathagata Roy, and Peipei Yang

Historical cyclone data indicate significant variations in cyclone activity during different phases of the El Niño-Southern Oscillation (ENSO). However, the impact of these variations on cyclone risk and damage has not been thoroughly investigated due to limited historical loss record. Understanding these variations could be crucial for effective risk management.

This study examines the variation in cyclone risk associated with ENSO phases, utilizing the cyclone risk assessment model by Impact Forecasting for Australia. The model employs a stochastic event set of cyclones, representing about forty-two thousand years of basin-wide activity, developed using environmental data from reanalysis and machine learning techniques. Our analysis demonstrate that the stochastic event set accurately reflects the seasonal variation in cyclone activity due to ENSO phases, making it a reliable tool for risk assessment.

To evaluate risk by ENSO phases, we segregated the stochastic event set using the Oceanic Nino Index and estimated wind-driven losses for each phase. The model results shows a significant variation in cyclone risk in Australia during El Niño and La Niña. However, the risk during the Neutral phase is found to be comparable with the long-term average. Annual average losses (AAL) during La Niña increases by 40%, while El Niño phases show a 37% reduction compared to the long-term average. Additionally, a one-in-hundred-year event during La Niña can result in 21% higher losses, whereas losses are 28% lower during El Niño compared to the long-term average.

The modeled loss variations across ENSO phases are consistent with observed changes in cyclone activity in Australia and are supported by the historical loss records.

How to cite: Bongirwar, V., Abraham Joseph, L., Ranjan Tripathy, R., Martin Kalbermatter, D., Roy, T., and Yang, P.: Modeling cyclone risk variations in Australia by ENSO phases., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10365, https://doi.org/10.5194/egusphere-egu25-10365, 2025.

EGU25-10429 | ECS | Posters on site | NH11.4

How drought risk evolution impacts crop weather insurance loss ratio in France? 

Léa Laurent, Albin Ullmann, and Thierry Castel

Climate change has modified climatic hazards features and requires to reconsider agro-climatic risks. Among these, drought is one of the risks with the strongest impact on both crop production and crop weather insurance performance (Brisson et al., 2010). Understanding the effects of climate change on agro-climatic risks at regional to local scale is therefore a major challenge for the agricultural sector, specifically for insurers offering crop weather insurance policies. This work, resulting from a collaboration between an insurer and a research laboratory, focuses on the development of a drought index that well explain the evolution of crop weather insurance loss ratio. As maize is a major crop in the company's portfolio, the study focuses on this crop in particular. The aim of this work is to find the optimal set of parameters that maximizes the correlation between the drought index and the drought-related losses on crop weather insurance.

The Safran-Isba-Modcou reanalysis produced by Météo France provides spatially and temporally continuous climate data over metropolitan France of relevant interest to address this topic (Le Moigne et al., 2020; Soubeyroux et al., 2008). At the regional scale, these data allow us to quantify the evolution of climate hazards related to the water cycle from 1960 to present day. Taking into account the vulnerability of the crop of interest through the use of a simplified two reservoirs water balance model provides an opportunity to assess changes in maize water stress (Jacquart and Choisnel, 1995). The definition of a water stress threshold leads to the development of an annual drought index (Laurent et al., under review). The correlation with the crop weather insurance loss ratio due to drought is tested at various spatial scales (municipality, production basin), for different varieties, different sowing dates and different stress thresholds.

Our results indicate that climate change has affected the frequency and intensity of drought risk on maize crops in France, depending on the French production area studied. The significance of the correlation depends on maize variety, sowing date and hydric stress threshold. It seems that using drought index computed with low stress thresholds and analyzing correlations at large spatial scales gives the best results.

For non-irrigated maize area at production basin scale, our drought index can explain a significant part of drought-related losses in crop weather insurance. The results suggest that such an index may be relevant to improve the actuarial loss model of the insurer. However, further analysis is required in areas where correlations are weaker, particularly in production basins with high irrigation levels.

References:

Brisson et al., 2010. Field Crops Res. 119, 201–212. https://doi.org/10.1016/j.fcr.2010.07.012
Jacquart, Choisnel, 1995. La Météorologie 8ème série, 29–44. https://doi.org/10.4267/2042/51939
Laurent et al., under review. J. Agric. For. Meteorol.
Le Moigne et al., 2020. Geosci. Model Dev. 13, 3925–3946. https://doi.org/10.5194/gmd-13-3925-2020
Soubeyroux et al., 2008. La Météorologie 8, 40. https://doi.org/10.4267/2042/21890

How to cite: Laurent, L., Ullmann, A., and Castel, T.: How drought risk evolution impacts crop weather insurance loss ratio in France?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10429, https://doi.org/10.5194/egusphere-egu25-10429, 2025.

EGU25-11503 | Posters on site | NH11.4

Analysis of the insurance impacts of storm clusters: a case study with Generali France 

Laura Hasbini, Pascal Yiou, and Laurent Boissier

Clusters of storms are defined as sequences of multiple storms occurring within a short time frame and a limited spatial extent. In this study, storm clusters are identified using a Lagrangian approach combined with an absolute frequency metric within a 96-hour time window, reflecting reinsurance contract specifications for an insurance company. Compound storms are further constrained to affect a common area, determined by the intersection of their footprints. Those footprints can be delineated using various radii of different sizes, depending on the desired granularity for compounding analysis.

The motivation for this definition stems from the potentially severe impacts of such events on the insurance sector. Storms are known to be among the costliest events for Insurance in Europe, with an average annual insured loss of €217 billion [Copernicus, 2023]. The repetition of such intense wind and strong precipitation events is no exception. The successive storms Lothar and Martin in December 1999 remain the costliest events observed in France with an estimated loss of €17 billion [EEA, 2023]. Despite the substantial risks associated with these compound events, few studies have investigated their role in amplifying both the hazard and the vulnerability.

We apply this approach to Generali, an Italian insurance company with approximately 5% market share in France. Using Generali’s historical claims data from 1998 to 2024, we propose a novel methodology linking high-resolution claims to individual storm events. This approach represents a significant advance in understanding loss drivers. Applied to storm clusters, the methodology distinguishes the relative contribution of each storm in a cluster to the total observed loss. By comparing the findings with Generali’s portfolio from 2018 to 2024, we identify key factors contributing to the additional damages caused by storm clusters. These insights are crucial for enhancing risk prevention and adapting current insurance strategies to better address compound storm events.

How to cite: Hasbini, L., Yiou, P., and Boissier, L.: Analysis of the insurance impacts of storm clusters: a case study with Generali France, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11503, https://doi.org/10.5194/egusphere-egu25-11503, 2025.

EGU25-16606 | Orals | NH11.4

Tropical Cyclone Rapid Intensification & it’s Impact for (Re)insurers 

Andrew Robson and Iain Willis

The rapid intensification (RI) of tropical cyclones (whereby the maximum sustained wind increases by 30 kt (15.4 m s−1) or over in a 24-period) has garnered particular attention in recent years, with insurers and risk managers increasingly concerned that warmer ocean basins are fuelling increasingly intense landfalling hurricanes (Kaplan et al 2010).

RI was a notable characteristic of both Hurricanes Helene and Milton during the 2024 North Atlantic Hurricane Season. These two storms caused 78bn and 35bn in economic losses respectively (Gallagher Re), with Helene undergoing explosive RI of 55mph in the 24-hours ahead of landfall, increasing its windspeed upon impacting the Florida coast to 140mph, classifying it as a category 4 storm (Saffir-Simpson scale).

In this study, key trends have been analysed in the pattern of RI of Tropical Cyclones globally over the period 1990-2023, including the response of different ocean basins as well as the critical impact of teleconnection patterns such as the El Nino Southern Oscillation (ENSO) in modulating the geographic dispersion of intensifying cyclones. The study shows that while most Tropical Cyclones (>90%) in recent decades have exhibited some form of RI in their development prior to landfall, there is a clear upward trend in recent years in some ocean basins towards a pattern of so-called ‘Explosive’ Rapid Intensification (whereby a storm intensifies at a rate >50 kt in 24 hours).

With the most extreme Tropical Cyclones undergoing explosive RI and potentially landfalling with greater intensity than in previous decades, this research studies the potential economic and (re)insured loss implications for global risk management. Particular focus is given to the North Atlantic as well as the strong signal of RI occurrence changes under ENSO and over the study period in the North-West and Eastern Pacific basins.

Kaplan, J., DeMaria, M., & Knaff, J. A. (2010). A revised tropical cyclone rapid intensification index for the Atlantic and eastern North Pacific basins. Weather and forecasting25(1), 220-241.

How to cite: Robson, A. and Willis, I.: Tropical Cyclone Rapid Intensification & it’s Impact for (Re)insurers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16606, https://doi.org/10.5194/egusphere-egu25-16606, 2025.

EGU25-17961 | Posters on site | NH11.4

Designing representative European storm surge scenarios for insurance risk assessment: challenges, results, and limitations 

Anyssa Diouf, Ignatius Ryan Pranantyo, Mathis Joffrain, and Nicolas Bruneau

Storm surge, a coastal flooding phenomenon driven by high-speed winds pushing water onshore poses a significant natural hazard across the globe. In recent decades, Europe has experienced several destructive extratropical cyclones that have severely impacted coastal communities and economies, such as Eunice (2022), David (2018), or Xaver (2013). Storm Xynthia in 2010 was especially notable, with substantial fatalities and material losses in France, highlighting the need for accurate storm surge risk assessment for societies and the (re)insurance industry involved. Yet, current modelling solutions are limited. Main commercial models only provide partial coverage of the risk in Europe, with a primary focus on the United Kingdom. To address this gap, AXA proposes a scenario-based approach to assess storm surge risk across North-Western Europe. Using the SCHISM 2D hydrodynamic model, we reproduced 10 significant historical events notably affecting France, Germany, and the United Kingdom, then perturbed them along three parameters: wind speeds, storm sizes and tide timings, generating 480 scenarios. The study presents the challenges of scenario selection and variability representation. It further provides findings on the modelling results by parameter and country, and on the estimation of the loss potential using a representative North-Western Europe insured market portfolio. Finally, key limitations are discussed, related to unmodelled defences and Digital Elevation Model accuracy. The approach provides valuable insights for AXA’s risk assessment and is a crucial step towards building a robust understanding of our risk.

How to cite: Diouf, A., Pranantyo, I. R., Joffrain, M., and Bruneau, N.: Designing representative European storm surge scenarios for insurance risk assessment: challenges, results, and limitations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17961, https://doi.org/10.5194/egusphere-egu25-17961, 2025.

EGU25-18013 | Posters on site | NH11.4

Evaluating the relationship between wind and storm surge risk in the Philippines and Hong-Kong, an insurance industry perspective. 

Mathis Joffrain, Ignatius Ryan Pranantyo, and Nicolas Bruneau

Due to intense destructive winds and heavy rainfall associated with storm surges, large waves and flooding, tropical cyclones are one of the most damaging natural catastrophes. They are a major threat to human lives and properties across the globe. When travelling over the ocean and approaching shallow water regions, tropical cyclones generate storm surge and waves that can devastate coastal communities and local economies.

In the recent years, Typhoons Hato (2017) and Mangkhut (2018) produced material surge damages to insurers in the Northwest Pacific basin, and therefore raised the need for accurate natural catastrophe models. Cat models consist of very large catalogues of synthetic but realistic events also called “event sets”. These event sets are consistent with experienced historical data but allow extrapolation beyond what was observed. 

In this study, we focus in winds and surges on the Philippines and Hong Kong regions. Driven by an existing tropical cyclone wind event set, over 10k full-physic simulations of storm surge and waves are computed for each region to estimate the complete distribution of coupled wind and surge losses over an exposure dataset. Due to computationally expensive dynamical simulations of storm surges and waves,  we first rank and select a subset of events (10k) based on an IKE (Integrated Kinetic energy) index. For each of these 10k event, the Semi-implicit Cross-scale Hydroscience Integrated System Model (SCHISM; Zhang & Baptista, 2008, Zhang et al., 2016) is forced by atmospheric winds and pressure fields to derive wave and surge footprints.

Second, we use adjusted Hazus (FEMA) damage functions to convert the water heights and windspeeds from the simulated events into damage factors. These factors are then multiplied to the considered exposure to derive losses. Third, we study the relationship between the wind and the surge modeled losses based on two criteria, (i) the event level correlation between IKE and surge losses, to ensure this index stands as a robust risk representation, and (ii) the event level proportion of surge losses out of the wind losses, which provides a set of reusable inter perils correlation factors.

How to cite: Joffrain, M., Pranantyo, I. R., and Bruneau, N.: Evaluating the relationship between wind and storm surge risk in the Philippines and Hong-Kong, an insurance industry perspective., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18013, https://doi.org/10.5194/egusphere-egu25-18013, 2025.

EGU25-18168 | Posters on site | NH11.4

Development of a climate-driven stochastic event catalogue for Wildfire in Europe 

Frédéric Azemar, Marie Shaylor, Nicolas Bruneau, Thomas Loridan, Daniel Swain, and Mathis Joffrain

Recent years have seen wildfires causing widespread environmental and economic damage as well as numerous fatalities globally. With record breaking yearly burnt areas, longer fire seasons, and more extreme events, wildfire is emerging as a growing concern for populations, governments and the private sector alike. In Europe, destruction and disruption have been historically more prominent in southern countries where key sectors of the economy like tourism, forestry, and agriculture can remain severely affected for years in the aftermath of catastrophic events.  

Over the last 30 years, catastrophe modelling solutions have been crucial in aiding the understanding of the economic impacts of natural risks like wildfire, making them essential tools for the (re)insurance industry for managing their exposure and quantifying potential losses. Such solutions typically involve the development of large scale and physically-based probabilistic models. 

We present here a climate-driven stochastic event catalogue for wildfire in Europe. The model allows us to expand on the limited historical records by generating millions of synthetic event footprints. For this, we first consider how climate conditions drive spatio-temporal patterns of wildfire activity in terms of yearly burnt area (fire activity module). In a second step, events are sampled via an ignition module that leverages machine learning algorithms and draws correlations between anthropogenic and bio-climate factors, and historical events. Finally, a propagation module generates event footprints given the local topography, fuel data, and meteorological conditions. The stochastic catalogue consists of 50K synthetic years and about 25M unique footprints at 100m resolution. This allows us to estimate hazard metrics like event frequency, event size, and tail risk over the whole continent as well as performing impact analyses. Lastly, we present an evaluation of structures at risk in France by intersecting our catalogue with a representative dataset of buildings. 

How to cite: Azemar, F., Shaylor, M., Bruneau, N., Loridan, T., Swain, D., and Joffrain, M.: Development of a climate-driven stochastic event catalogue for Wildfire in Europe, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18168, https://doi.org/10.5194/egusphere-egu25-18168, 2025.

EGU25-18838 | ECS | Posters on site | NH11.4

Development of a Globally Connected, Climate-Driven, Stochastic Drought Model for Hazard Assessment using Machine Learning Techniques 

Marie Shaylor, Nicolas Bruneau, Frédéric Azemar, and Thomas Loridan

With global temperatures continuing to rise year on year, drought conditions are becoming increasingly frequent and severe, across all continents. More and more, the negative effects of these worsening drought conditions are being experienced by people across the world both directly, through damage to agricultural systems, water scarcity or damage to homes from subsidence, as well as indirectly, through cascading effects on other perils such as heatwaves and wildfires, which in turn may devastate communities and drive great economic losses. For these reasons, drought is of growing concern to the (re)insurance industry, as an emerging peril. It is therefore essential that reinsurers have access to tools which can aid in their understanding of drought hazard and risk in a changing climate. One such tool we present here – a climate driven, globally connected stochastic drought hazard model, which responds dynamically to the climate of any given year, enabling this understanding of how drought conditions change with the climate.

In this presentation, we describe the novel methodology applied to generate this globally connected and climate-driven stochastic drought model. The model is generated in two stages, the first addressing global variability in drought trends and teleconnections, and the second looking at continental scale patterns. In the first instance, we apply a dimensionality reduction to a selection of historical drought indexes over different time scales, allowing extraction of the key modes of variability of drought at the global scale. We then condition the top key modes of variability to the climate state using reanalysis (ERA5) data, allowing us to drive our stochastic set at the global scale, based on the global climate state.

Once these global patterns have been determined, we use the residual drought signal to condition a regional (continental) model using similar reduction and conditioning techniques. This regional layer is then effectively layered onto the global model, allowing us to recreate globally and regionally consistent drought variability in the stochastic set. A Bayesian framework is used to sample a range of realistic drought conditions, aligned with the climate of any given year. Global and regional drought conditions are then combined in order to generate >100K stochastic years of global drought severity as well as duration of drought for three severity levels (moderate, severe, extreme). This framework can also be applied to any other climate model data (for example, CESM LENS2) to generate a stochastic event set up to the year 2100. Here we present initial results from this stochastic catalogue, showcasing the spatial and temporal variation in drought hazard from 1950 – 2100, return periods, and comparisons to historical records. This work also builds upon a previous, continental only version of the drought model.

How to cite: Shaylor, M., Bruneau, N., Azemar, F., and Loridan, T.: Development of a Globally Connected, Climate-Driven, Stochastic Drought Model for Hazard Assessment using Machine Learning Techniques, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18838, https://doi.org/10.5194/egusphere-egu25-18838, 2025.

EGU25-19732 | ECS | Orals | NH11.4

Country-level energy demand for cooling using CMIP6 and world population projections 

Albert Martinez-Boti, Lorenzo Sangelantoni, Daniele Peano, Silvio Gualdi, Stefano Tibaldi, and Enrico Scoccimarro

Cooling Degree Days (CDD) are commonly used to quantify energy demand for cooling and recent works highlighted the importance of population weighting to better represent energy load distribution. This study builds on the work of Scoccimarro et al. (2023), who assessed country-level cooling demand from 2000 to 2020 using both standard dry CDDs and humid CDDs (CDDhum), corrected with population weighting (CDD values are averaged at the national level, weighted by population). The humidity correction uses perceived temperature, which combines both temperature and humidity effects, rather than relying on temperature only. This adjustment offers a more accurate representation of cooling needs, as humidity plays a significant role in human stress and the demand for cooling.

This study aims to assess future cooling demand by utilising a selection of CMIP6 global climate models (GCMs), combined with country-level population projections from the United Nations World Population Prospects 2024. We analyse future trends (2015–2100) for the two mentioned metrics—standard cooling degree days (CDD) and humidity-adjusted cooling degree days (CDDhum) — both weighted by country-level population projections. Temporal evolution of these two metrics is assessed according SSP1-2.6 and SSP5-8.5 societal/emission scenarios, applying a consistent population weighting for both. GCM biases affecting population-weighted CDD and CDDhum are also assessed by considering ERA5 as reference product.

Preliminary results —calculated over Europe during the reference period 1971-2000 and without the application of humidity correction or population weighting — show that, despite some biases in the trend magnitude, the CMIP6 GCMs generally capture the spatial pattern of ERA5 CDD showing a general increasing trend in the energy required for cooling buildings during summer season. In particular, the Mediterranean Basin is projected to experience the most significant increase in CDDs, with considerable inter-model variability. In contrast, some northern European regions, such as the Scandinavian Peninsula and Iceland, show no trend in CDDs.

This work is based on ERA5 and CMIP6 data, collected and tailored as part of the H2020 BlueAdapt project (Grant agreement action Number 101057764), and on analysis codes developed under the Copernicus-funded contract (C3S2_520).

How to cite: Martinez-Boti, A., Sangelantoni, L., Peano, D., Gualdi, S., Tibaldi, S., and Scoccimarro, E.: Country-level energy demand for cooling using CMIP6 and world population projections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19732, https://doi.org/10.5194/egusphere-egu25-19732, 2025.

We present a novel method to construct a 10,000-year event set for European weather using expired ensemble forecasts from ECMWF [1]—requiring no additional computational effort. Derived from the same numerical model underlying ERA5, this approach naturally extends it more than two orders of magnitude, whilst inherently overrepresenting the climates of the 2010s and 2020s. Hence, it provides a valuable resource for quantifying risks in today’s already-warmed climate

Our evaluation focuses on extreme wind speeds from extra-tropical cyclones impacting major European cities. With a rigorous order statistics framework, we confirm that this dataset replicates the statistical tails of ERA5 for return periods up to RP40 and extends exceedance probability (EP) curves up to RP10,000. Crucially, its physical consistency enables robust analysis of joint distributions across space and time, offering precise insights into compound and correlated risks. Using empirical copulas, we quantify critical conditional probabilities, such as P(Paris = RP100 London = RP50), a task infeasible with only the weather record beyond RP5.

This method leverages years of historical computational investments by ECMWF, that created a vast global low-bias source of simulated weather data, fully interchangeable with ERA5 for seamless integration into existing pipelines. Following two years of archive extraction efforts, we compiled a subset of surface variables (t2m, 10m/100m wind, runoff,...) and make it widely available to the community [2]. 

[1] European Centre for Medium-Range Weather Forecasts (ECMWF) __Atmospheric Model Ensemble extended forecast__ https://www.ecmwf.int/en/forecasts/datasets/set-vi
[2] Dolezal P., Expired ECMWF ENSemble Extended forecasts and Reforcasts for Renewable power in Europe. NERC EDS Centre for Environmental Data Analysis,
https://catalogue.ceda.ac.uk/uuid/7783f79c7080456088d98a34ca238bfa

How to cite: Dolezal, P. and Shuckburgh, E.: Spatial Coincidence of Extreme Wind Across European Cities: Evidence from 10,000 Years of Expired ECMWF Forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19805, https://doi.org/10.5194/egusphere-egu25-19805, 2025.

EGU25-20119 | Orals | NH11.4

Projected Impacts of Climate Change on High Temperatures for Tomato Cultivation 

Ana Maria Tarquis, Alfredo Rodriguez, Esther Hernández-Montes, Ernesto Sanz, Andres F. Almeida-Ñauñay, and Alberto Garrido

Climate change poses significant challenges to agricultural systems worldwide, including increased agroclimatic risks that threaten crop productivity and sustainability. This study investigates how climate change will influence the agroclimatic risk of high temperatures on tomato cultivation in Malta, a region already experiencing Mediterranean climatic pressures. Using climate projections under different greenhouse gas emission scenarios, we analyzed temperature trends, heat stress events, and their potential impacts on key growth stages of tomatoes, including flowering and fruit development. The results indicate a marked increase in the frequency and intensity of high-temperature events, particularly during critical phenological phases, which could significantly reduce yields and quality. Our findings also reveal spatial variability in risk levels across Malta, emphasizing the need for localized adaptation strategies. To mitigate these risks, we propose targeted interventions such as selecting heat-tolerant tomato varieties, optimizing irrigation schedules, and implementing shading techniques. This research underscores the urgency of integrating climate-resilient practices into tomato production systems to ensure sustainable agricultural productivity in Malta amidst a changing climate.

How to cite: Tarquis, A. M., Rodriguez, A., Hernández-Montes, E., Sanz, E., Almeida-Ñauñay, A. F., and Garrido, A.: Projected Impacts of Climate Change on High Temperatures for Tomato Cultivation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20119, https://doi.org/10.5194/egusphere-egu25-20119, 2025.

EGU25-473 | ECS | Orals | NP6.1

Turbulent Lagrangian fCO2 time series statistics in the Southern Ocean 

Kévin Robache and François G. Schmitt

The Southern Ocean plays a crucial role in regulating Earth's climate, absorbing approximately 10 % of annual human CO2 emissions (DeVries, 2014; Friedlingstein et al., 2023). However, it is still a challenge to fully understand its carbon dynamics due to significant observational gaps, particularly during winter. Furthermore, the dynamics on small spatial and temporal scales are also poorly understood, despite their potential importance in shaping the overall carbon budget of the region (Guo & Timmermans, 2024). Between 2001 and 2012, researchers from the LOCEAN laboratory in Paris deployed 15 CARIOCA Lagrangian drifting buoys in this region to gain a deeper understanding of its spatial carbon dynamics (Boutin et al., 2008; Resplandy et al., 2014) at high-frequency (1-hour time resolution). In this study, we analyzed the time series of six of these buoys in the framework of Lagrangian turbulence (Kolmogorov, 1941; Landau & Lifschitz, 1944; Inoue, 1951). This is done using Lagrangian data on CO2 fugacity (fCO2), chlorophyll a, sea surface temperature (SST), and sea surface salinity (SSS) along their trajectories. Additionally, we examined the dynamics of the buoys' drifting speeds estimated from buoys location data.

Through Fourier spectral analysis and structure function analysis, we demonstrated that these time series exhibit scaling and intermittent behaviour, in agreement with the Lagrangian vision of the turbulent Richardson-Kolmogorov energy cascade in fully developed turbulence. Notably, at least two distinct spectral regimes were identified. Chlorophyll a and fCO2 behave as active turbulent scalars, while SST and SSS depicted statistics compatible with passive scalars with a higher intermittency on timescales shorter than 4 days. The links between these time series were also investigated, using the generalized correlation functions (GCFs) and exponents (GCEs).

References :

DeVries, T. (2014). The oceanic anthropogenic CO2 sink: Storage, air‐sea fluxes, and transports over the industrial era. Global Biogeochemical Cycles28(7), 631-647.

Friedlingstein, P. et al. (2023). Global carbon budget 2023. Earth System Science Data, 15(12), 5301-5369.

Guo, Y., & Timmermans, M. L. (2024). The role of ocean mesoscale variability in air‐sea CO2 exchange: A global perspective. Geophysical Research Letters51(10), e2024GL108373.

Boutin, J. et al. (2008). Air‐sea CO2 flux variability in frontal regions of the Southern Ocean from CARbon Interface OCean Atmosphere drifters. Limnology and Oceanography53(5part2), 2062-2079.

Resplandy, L. et al. (2014). Observed small spatial scale and seasonal variability of the CO2 system in the Southern Ocean. Biogeosciences11(1), 75-90.

Kolmogorov, A. N. (1941). On degeneration (decay) of isotropic turbulence in an incompressible viscous liquid. In Dokl. Akad. Nauk SSSR (Vol. 31, pp. 538-540).

Landau L.D. & Lifshitz E.M. (1944). Fluid Mechanics (MIR), first russian edition.

Inoue, E. (1952). Turbulent fluctuations in temperature in the atmosphere and oceans. Journal of the Meteorological Society of Japan. Ser. II30(9), 289-295.

How to cite: Robache, K. and Schmitt, F. G.: Turbulent Lagrangian fCO2 time series statistics in the Southern Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-473, https://doi.org/10.5194/egusphere-egu25-473, 2025.

EGU25-1290 | Posters on site | NP6.1

Dispersal of invasive species larvae within the Orust-Tjörn fjord system 

Sandra-Esther Brunnabend, Lars Arneborg, and Sam Fredriksson

The Orust-Tjörn fjord system is located on the west coast of Sweden and consists of several fjords connected by shallow and narrow straits. It is home to nature reserves, harbors, leisure areas, and aquaculture farms, and biodiversity is threatened by invasive species, for example brought in through shipping. Therefore, it is important to understand how larvae of invasive species are dispersed by the currents within the fjords system in order to find efficient methods for management of existing and future harmful invasive species. 

A connectivity study is performed in order to identify dispersion patterns, assuming that larvae are passively transported by surface currents. For the years 2016 and 2022, the dispersion of larvae is simulated using the open source Opendrift software (Dagestad et al., 2018). The model is forced by velocity fields modeled with a high resolution regional Nemo3.6 ocean model with lateral resolution of ~50m. A large number of particles (~700,000) are seeded with four-day intervals, covering the whole fjord system and areas of open waters near the entrances of the fjord system. For each seeding, the dispersion model runs for 3 weeks where larvae that reach a shore are transported away again when currents change (pelagic phase). This is followed by a one-week period where larvae settled as soon as they reach a shore (settling phase). On the basis of this ensemble, we perform a connectivity analysis indicating the probabilities of larvae, released at one location, settling in other locations within the fjord system.

Results show that larvae seeded inside the Orust-Tjörn fjord system mostly remain there with some even remaining in the same local fjord basin during the four-week period. Connectivity matrices also show that some larvae travel far. Larvae seeded outside the Orust-Tjörn fjord system are likely to leave the model domain as they are transported within the generally northward flowing swift Baltic current. 

How to cite: Brunnabend, S.-E., Arneborg, L., and Fredriksson, S.: Dispersal of invasive species larvae within the Orust-Tjörn fjord system, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1290, https://doi.org/10.5194/egusphere-egu25-1290, 2025.

EGU25-1454 | ECS | Posters on site | NP6.1

An Adaptive Masking Time Series Transformer based Representation Learning Model for Well Log Curves 

Pin Li, Jun Zhou, Yubo Liu, Juan Zhang, Guojun Li, and Yuange Zhou

Well log curves, acquired from downhole logging tools during well logging, are pivotal for reservoir characterization and formation evaluation in oil and gas exploration and production. However, manual feature extraction from raw curves remains essential for constructing effective machine learning models, presenting time-consuming challenges and stringent labeling requirements. Concurrently, the transformer architecture, prevalent in NLP and computer vision, offers promise for representation learning. This paper proposes a self-supervised transformer based methodology for extracting well log curves representations, aiming to expedite downstream model development.

While transformer models have gained prominence in handling text and image data, well log curves present a distinct challenge as they resemble time series data. Despite the nascent development of time series transformer models, we conducted an extensive review of current progress and adopted the best-performing time series transformer model for extracting representations from well log curves. Importantly, given the challenges posed by factors such as borehole conditions and instrument failure, certain types of well log curves may occasionally be missing or distorted. To address this issue, our proposed methodology introduces an adaptive masking mechanism, which selectively applies masking to patches of curves where data quality is poor, thereby effectively mitigating data quality concerns.

Data from 2000 wells are utilized for model training, with an additional 100 wells reserved for validation purposes. Our study observed a consistent decrease in both training and test losses until convergence during the training stage. Initially, mean squared error (MSE) and mean absolute error (MAE) are employed to quantify reconstruction errors between reconstructed curves and raw curves, low values of MSE (0.08) and MAE (0.07) indicate effectiveness of the learned representations. Subsequently, a downstream task involving oil and gas identification is undertaken, wherein a classification model is developed based on representations learned by the transformer model. Performance comparison between models utilizing learned representation and those employing statistical features highlights the superior performance of the former (98% accuracy), emphasizing the efficacy of our representation learning methodology. This paper introduces a novel self-supervised methodology based on transformer architecture for well log curve representation learning. The method automates information extraction without requiring logging expertise and substantially enhances downstream machine learning model performance.

How to cite: Li, P., Zhou, J., Liu, Y., Zhang, J., Li, G., and Zhou, Y.: An Adaptive Masking Time Series Transformer based Representation Learning Model for Well Log Curves, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1454, https://doi.org/10.5194/egusphere-egu25-1454, 2025.

EGU25-3171 | ECS | Orals | NP6.1

Lagrangian tracking of particles settling through the atmosphere: influence of particle shape on its dispersion 

Taraprasad Bhowmick, Florencia Falkinhoff, Eberhard Bodenschatz, and Gholamhossein Bagheri
All solid particles in the atmosphere – such as ash, dust, ice crystals, pollen and microplastics – are non-spherical, which affects their atmospheric transport. However, studies of their dispersion are often based on models derived from measurements in stationary fluids or on field data distorted by atmospheric fluctuations. To address these limitations, the IMPACT (In-situ Measurement of Particles, Atmosphere, Cloud, and Turbulence) field campaign was conducted in northern Finland during May and June 2024. As part of this initiative, we launched an innovative experiment to track the dispersion of small, non-spherical particles released at altitudes between 2 and 7 km. Their trajectories were monitored until they reached the ground.
 
The experiment used particles of consistent mass (8.5 grams) and volume but varying shapes, including icosahedrons (representing near-spherical forms), as well as circular and elliptical discs, some with perforations. Up to 20 paperboard particles equipped with miniaturized, battery-powered electronics were placed inside a biodegradable helium balloon for each launch. At the target altitude, the balloon burst, releasing the particles from a single point. Throughout the particles' ascent within the balloon and their descent after release, GPS data on their position and altitude were transmitted via radio to ground stations. Over the course of the campaign, we tracked up to 150 particles across six distinct shapes. In addition, particle-resolved direct numerical simulations are carried out to determine the settling behavior in still air as a function of particle shape. In this presentation, we will share preliminary findings on particle dispersion patterns and explore the influence of atmospheric turbulence on the behavior of non-spherical particles.

How to cite: Bhowmick, T., Falkinhoff, F., Bodenschatz, E., and Bagheri, G.: Lagrangian tracking of particles settling through the atmosphere: influence of particle shape on its dispersion, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3171, https://doi.org/10.5194/egusphere-egu25-3171, 2025.

EGU25-4715 | Orals | NP6.1

Nonlinear causal dependencies as a signature of the complexity of the climate dynamics 

Stéphane Vannitsem, X. San Liang, and Carlos A. Pires

Nonlinear quadratic and linear dynamical dependencies of large-scale climate modes are disentangled through the analysis of the rate of the information transfer. That is performed in a joint analysis of eight dominant climate modes, covering the tropics and extratropics over the North Pacific and Atlantic. A clear signature of nonlinear and compound influences at low-frequencies (time scales larger than a year) are emerging, while high-frequencies are only affected by linear dependencies. These results point to the complex nonlinear collective behavior at global scale of the climate system at low-frequencies, supporting earlier views that regional climate modes are local expressions of a global intricate low-frequency variability dynamics, which is still to be fully uncovered.

How to cite: Vannitsem, S., Liang, X. S., and Pires, C. A.: Nonlinear causal dependencies as a signature of the complexity of the climate dynamics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4715, https://doi.org/10.5194/egusphere-egu25-4715, 2025.

EGU25-5726 | ECS | Posters on site | NP6.1

Manifold Embeddings for Multispectral Time-Series Land Disturbance Detection 

Mengyao Li and Jianbo Qi

Dimensionality reduction techniques have been successfully applied in remote sensing to reduce redundant information. However, achieving dimensionality reduction and lossless recovery for multispectral data at any global location remains a challenge, particularly given the complex and variable nature of surface conditions. Furthermore, it is still unclear if the reduced features maintain temporal continuity and can be effectively integrated with existing time series algorithms for disturbance detection. This study trains a Uniform Manifold Approximation and Projection (UMAP) model based on Harmonized Landsat Sentinel-2 (HLS) imagery to accomplish multispectral dimensionality reduction. Subsequently, the manifold embeddings are used in the Continuous Change Detection and Classification (CCDC) algorithm for land disturbance detection. Two key conclusions are drawn from this study: 1) a general multispectral dimensionality reduction model was constructed based on UMAP, which is applicable to all global land surfaces and any seasons. The manifold embeddings exhibit a stable value range and preserve the coherence of the time series. 2) compared to full-spectrum multispectral data, the manifold embeddings achieved comparable performance in image prediction and disturbance detection. Our study demonstrates the potential of manifold learning-based representation of global land surface reflectance spectra for lightweight storage and processing of dense satellite image time series, while keeping the ability to detect any kinds of land disturbance.

How to cite: Li, M. and Qi, J.: Manifold Embeddings for Multispectral Time-Series Land Disturbance Detection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5726, https://doi.org/10.5194/egusphere-egu25-5726, 2025.

EGU25-5876 | Orals | NP6.1

Relative dispersion at the surface of the ocean: role of balanced motions and internal waves 

Stefano Berti, Michael Maalouly, Guillaume Lapeyre, and Aurélien Ponte

Ocean flows at scales smaller than few hundreds of kilometers display rich dynamics, mainly associated with quasi- geostrophic motions and internal gravity waves. Although both of these processes act on comparable lengthscales, the former, which include meso and submesoscale turbulent flows, are considerably slower than the latter, which take part in the ocean fast variability. Understanding how their effects overlap is crucial for several fundamental and applied questions, including the interpretation and exploitation of new, high-resolution satellite altimetry data, and the characterization of material transport at fine scales.

In this study we investigate these points by examining Lagrangian pair-dispersion statistics in a high-resolution global-ocean numerical simulation including high-frequency motions, such as internal gravity waves. In particular, we aim at assessing the sensitivity of the particle relative-dispersion process on ageostrophic, fast fluid motions. For this purpose we select a study area close to Kuroshio Extension, characterized by energetic submesoscales, and focus on the seasonal variability of the Lagrangian dynamics.

We find that in winter pair dispersion is predominantly influenced by meso and submesoscale motions, meaning nearly balanced dynamics. The behavior of the different Lagrangian indicators considered agrees in this case with the theoretical predictions, based on the shape of the kinetic energy spectrum, in quasi-geostrophic turbulent flows. Conversely, in summer, when high-frequency motions gain importance and submesoscales are less energetic, the situation is found to be more subtle, and the usual relations between dispersion properties and spectra do not seem to hold. We explain this apparent inconsistency relying on a decomposition of the flow into nearly-balanced motions and internal gravity waves. Through this approach, we show that while the latter contribute to the kinetic energy spectrum at small scales, they do not impact relative dispersion, which is essentially controlled by the nearly-balanced, mainly rotational, flow component at larger scales.

How to cite: Berti, S., Maalouly, M., Lapeyre, G., and Ponte, A.: Relative dispersion at the surface of the ocean: role of balanced motions and internal waves, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5876, https://doi.org/10.5194/egusphere-egu25-5876, 2025.

EGU25-6863 | ECS | Posters on site | NP6.1

Spatiotemporal Causal Effect Estimation in Complex Dynamical Systems 

Rebecca Herman and Jakob Runge

Causal Inference is essential for identifying and quantifying causal relationships in systems where randomized controlled experiments are infeasible, but the high dimensionality and co-variability structure of spatiotemporal dynamical systems such as the climate system pose special challenges for causal effect estimation. It is standard for climate scientists to reduce the dimension of their data with pre-processing procedures such as regional means and principal component analysis, but taking a regional mean may mask differences in spatial pattern – such as the difference between Eastern Pacific and Central Pacific El Niño events – that may be relevant for causal relationships. Similarly, principal component analysis may obscure true causal relationships because the spatial pattern associated with maximum co-variability may not be the causally relevant information. Instead of using these preprocessing techniques, the basic procedure of time series causal effect estimation can be simply extended to multivariate time series, but this introduces new complications and heightens already existing complications of time series causal effect estimation. Here, we discuss these complications and present practical solutions. Complications for multi-variate as well as univariate time series include: (1) neighboring points in time and space may be very similar if the scale of the spatiotemporal sampling rate is small relative to the characteristic scale of the variance, resulting in unstable estimations, (2) the do-calculus expression for estimating the response to a hard intervention may include calculations with spatiotemporal gradients so strong they would result in instabilities in the system, and finally, (3) it is often not possible to actually perform a hard intervention in dynamical systems, making the interpretation of the causal effect unclear. The first complication may be addressed using L2 regularization, and the second and third complications may be addressed by focusing on soft interventions of reasonable magnitude that approach zero on their spatiotemporal boundaries. A unique complication of multi-variate causal effect estimation is that, when using L2 regularization, the total causal influence of a climate variable will be penalized inverse-proportionally to the number of spatial datapoints. This complication can be addressed by scaling variables so that the total spatiotemporal variance, rather than the component-wise variance, is one. We showcase the power of the technique by quantifying the spatiotemporal causal effect of El Niño-related sea surface temperature variability on atmospheric pressure variability in the North Atlantic in unforced Community Earth System Model simulations. We demonstrate that spatiotemporal causal effect estimation allows us to simultaneously determine the relevant spatial patterns and more accurately quantify a pattern-dependent causal effect between ENSO and NAO that has thus far proven difficult to measure in observational studies.

How to cite: Herman, R. and Runge, J.: Spatiotemporal Causal Effect Estimation in Complex Dynamical Systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6863, https://doi.org/10.5194/egusphere-egu25-6863, 2025.

EGU25-6918 | ECS | Orals | NP6.1

New ABL measurements of Lagrangian relative dispersion by means of radiosonde clusters 

Niccolo' Gallino, Shahbozbek Abdunabiev, John Craske, Ben Devenish, Jennyfer Tse, and Daniela Tordella

Turbulent relative dispersion is a phenomenon of fundamental interest both for its theoretical implications and for its immediate applications, which in geophysical sciences range from pollutant spreading in the atmosphere to nutrient transport in the oceans. We present new results in the measurement of turbulent relative dispersion in the atmospheric boundary layer, which enrich the picture with respect to the current framework. The measurements were carried out using clusters of miniaturized radiosondes, carried by small (~40 cm in diameter) helium balloons [1]. These clusters enable the effective investigation of relative dispersion by computing inter-particle distances among radiosondes. This methodology represents a concrete attempt at realising the type of analysis originally conceived by L. F. Richardson in his 1926 paper [2], often regarded as the one that initiated the field of study of relative dispersion.

The current accepted framework for the discussion of relative dispersion is the Kolmogorov-Obukhov scaling theory, which on dimensional grounds allowed for the derivation of the result (called the Richardson-Obukhov law) according to which the mean square distance in between particles advected by a turbulent flow field scales like the cube of time, , where ε is the energy dissipation rate and g is called the Richardson constant. However, this result is only valid for the case of homogeneous, isotropic turbulence, specifically in the inertial range of scales [2, 3]. Atmospheric turbulence, instead, is far from homogeneity and isotropy, and is characterized by local intense intermittency and entrainment [4, 5].
We conducted six cluster launches across three distinct topographical environments: the near-maritime plains at Chilbolton Observatory, the western Alps near the Astronomical Observatory of Aosta Valley, and the hilly region surrounding Udine. The results reveal not only deviations from the RO law but also significant variations between launches and distinct dispersion regimes within each launch (Fig. 1). The implication is, as expected, that the dispersion law for the atmosphere does not have a universal character, and depends on specific details of the boundary layer flow. The next step in the analysis will be the identification of the relevant flow features which impact the dispersion law, which is especially challenging due to the wide range of possibly participating phenomena.


Fig. 1. Mean square separation distance between mini-radiosondes within the cluster during six field experiment flights in different environmental topologies. Cross symbols show results from the MET OFFICE NAME dispersion model [6].

1. Abdunabiev S. et al., Measurement 224, 113879 (2024)
2. Richardson LF, Proc. R. Soc. Lond. A 110, 709 (1926)
3. Devenish, BJ, Thomson DJ. JFM 867, 877–905 (2019)
4. Van Reeuwijk M, Vassilicos JC, Craske J. JFM 908 (2021)
5. Fossa’ L., Abdunabiev S., Golshan M., Tordella D., Physics of fluids 34, (2022)
6. Turbulence_&_Diffusion_Note_288, Met Office, UK (2003)

How to cite: Gallino, N., Abdunabiev, S., Craske, J., Devenish, B., Tse, J., and Tordella, D.: New ABL measurements of Lagrangian relative dispersion by means of radiosonde clusters, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6918, https://doi.org/10.5194/egusphere-egu25-6918, 2025.

In past decades, increasing robust causal models were proposed, making causal inference under different scenarios and data limitations feasible. On one hand, these causal model are all based on time series data sources. On the other hand, in Earth Science, some variables, such as soil features and elevation, do not present a time series or the time series of these variables do not present sufficient temporal variations. In this case, traditional temporal causal models may fail to identify these clearly existing causalities in Earth Science.  To fill these gaps, here we show a Geographical Convergent Cross Mapping (GCCM) model for spatial causal inference with spatial cross-sectional data based cross-mapping prediction in reconstructed state space. Three typical cases, where clearly existing causations cannot be measured through temporal models, demonstrate that GCCM could detect weak-moderate causations when the correlation is not significant. And when the coupling between two variables is significant and strong, GCCM is advantageous in identifying the primary causation direction and better revealing the bidirectional asymmetric causation, overcoming the mirroring effect. The principle and some cases of GCCM are briefly introduced.  

How to cite: Chen, Z.: Causal Inference in GeoScience: From the Temporal to Spatial Dimensions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7326, https://doi.org/10.5194/egusphere-egu25-7326, 2025.

EGU25-11012 | Posters on site | NP6.1

Enhanced Ocean Model Predictability through Integration of High-Frequency Radar Observations and 2DVAR Data Assimilation: A Case Study of Pasaia Port 

Guillermo García Sánchez, Irene Ruiz, Anna Rubio, and Lohitzune Solabarrieta

Accurate ocean state forecasting is fundamental for effective port operations and coastal zone management. In the southeastern Bay of Biscay, particularly Pasaia port, high-resolution ocean condition forecasts directly impact navigation safety, port logistics, and environmental monitoring capabilities. The integration of observational data with numerical models represents a critical advancement in improving forecast accuracy for operational oceanography applications.

This study addresses the challenge of enhancing ocean model performance through a systematic approach to data assimilation. We focus on incorporating high-frequency (HF) radar observations into the Iberian-Biscay-Irish (IBI) regional model framework to optimize boundary conditions of the MOHID model that is available in the area. The motivation stems from the need to reduce forecast uncertainties in coastal areas where complex bathymetry, tidal forcing, and meteorological conditions interact. By implementing a two-dimensional variational (2DVAR) assimilation scheme, we aim to minimize the discrepancies between model outputs and observational data, ultimately providing more reliable ocean state estimates for local maritime operations. To validate the improved model outputs, we will compare them against Lagrangian drifter trajectories using a skill score metric, ensuring the assimilation’s effectiveness in capturing complex ocean dynamics.

How to cite: García Sánchez, G., Ruiz, I., Rubio, A., and Solabarrieta, L.: Enhanced Ocean Model Predictability through Integration of High-Frequency Radar Observations and 2DVAR Data Assimilation: A Case Study of Pasaia Port, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11012, https://doi.org/10.5194/egusphere-egu25-11012, 2025.

EGU25-11509 | ECS | Orals | NP6.1

Sparse pre-whitening operators for regression of climatic time series 

Donald P. Cummins and Mengheng Li
Regression methods are used extensively in climate science and are commonly applied to output from numerical climate models, e.g. for detection and attribution of climate change trends and for diagnosing emergent properties of climate models such as Equilibrium Climate Sensitivity (ECS). Output from climate models can have complex spatiotemporal dependence structures and, in practice, the assumptions of the Gauss-Markov Theorem seldom hold. Under such conditions, the application of Ordinary Least Squares (OLS) is inefficient and can lead to biased inference, with implications for model selection and evaluation.

The detection and attribution community has traditionally addressed this problem using a Generalised Least Squares (GLS) approach, whereby a pre-whitening operator is estimated from a climate model's pre-industrial control (piControl) simulation, typically using an unstructured sample covariance matrix or regularised version thereof.

We show how, for low-dimensional collections of climate variables, the dependence structure can be parsimoniously parameterised as a Vector AutoRegression (VAR) and the resultant sparse pre-whitening operator efficiently computed. For the first-order VAR(1) model, this procedure is analogous to a multivariate Prais-Winsten estimation. An example application to calibration of Simple Climate Models (SCMs) is discussed, shedding new light on the problem of choosing an appropriate model complexity.

How to cite: Cummins, D. P. and Li, M.: Sparse pre-whitening operators for regression of climatic time series, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11509, https://doi.org/10.5194/egusphere-egu25-11509, 2025.

EGU25-11547 | ECS | Posters on site | NP6.1

Vortex dynamics on Rotating Penetrative Convection 

Gabriel Meletti, Thierry Alboussière, Jezabel Curbelo, Stéphane Labrosse, and Philippe Odier

This work presents experimental results regarding rotating penetrative convection. The focus is on how convection driven by thermal or salty composition interacts with a stably stratified region. In such systems, as convection overshoots into the stratified layer, complex feedback loops arise, leading to the generation of internal waves that propagate in the stably stratified region. In rotating systems, Coriolis effects can further modify the dynamics, giving rise to inertial-gravity waves in the stably stratified region. Furthermore, the convective cells can change into different patterns of elongated vortices, changing how convection overshoots, and how it can drive internal waves. These phenomena are relevant to different geophysical and astrophysical applications, such as in the Earth's atmosphere, where internal gravity waves are excited in the stratosphere by convective motions in the troposphere. These interactions are also relevant to planetary and stellar interior applications, where convection can drive waves in stably stratified layers such as the radiative zone of stars or in the (possibly existing) stratified layer at the Earth's external core, where rotation effects are even more significant due to the small Rossby numbers, of the order of $10^{-5}$ to $10^{-4}$. This indicates that rotational forces dominate over inertial forces, highlighting the importance of better understanding the effects of rotation in the dynamics of penetrative convection and wave interactions.

Our experimental setup, named \textit{CROISSANTS (Convective ROtational Interactions with Stable Stratification Arising Naturally in Thermal Systems)}, found at the Physics Laboratory of the Ecole Normale Supérieure (ENS) de Lyon, is mounted on a rotating table and investigates the dynamics of rotating systems using water with a temperature gradient. The temperature ranges from approximately $30^oC$ at the top of a $30$cm-high cubic cavity and decreases to $0^oC$ at the bottom. Since water exhibits a density inversion between $0^oC$ and $4^oC$, the system naturally develops convection at the bottom, beneath a stably stratified region that extends from the convective interface to the top of the cavity. Measurements were performed using techniques such as Particle Image Velocimetry (PIV), Schlieren techniques, and Laser-Induced Fluorescence (LIF), to capture the convective and wave motions in both vertical and horizontal planes. Numerical simulations complement the experiments, exhibiting similar behavior to the observed experimental results. Both experiments and numerical simulations show that the elongated vortices in the convective region can be observed in higher regions of the stable density stratified zone. These long-lasting vortices move slowly in the flow (compared to the rotation of the experiment). Lagrangian-Averaged-Vorticity-Deviation (LAVD) techniques are then applied to track the dynamics of these long-lasting vortices elongated in the stable region. Understanding these processes provides a framework for interpreting how convective motion transfers energy across scales, impacting large-scale magnetic fields and planetary evolution.

How to cite: Meletti, G., Alboussière, T., Curbelo, J., Labrosse, S., and Odier, P.: Vortex dynamics on Rotating Penetrative Convection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11547, https://doi.org/10.5194/egusphere-egu25-11547, 2025.

Natural magnetic field measurement is essential for discovering fundamental physical mechanisms in space. Both the CSES mission and the DEMETER satellite equipped with the search coil magnetometer to observe the magnetic field waves. The CSES mission’s search coil magnetometer was developed by the School of Space Sciences Department of Beihang University. But the accuracy of these measurements is often degraded by artificial interference from reaction wheels on satellites. These wheels produce complex harmonic interference, often overlapping with the natural signal in both time and frequency domain, which makes it difficult to observe natural signals.

Traditional methods usually construct filters to separate interference. Advanced signal technologies have focused on reducing interference using self-adaptive signal decomposition methods in either time or frequency domain. In this field, Finley and Robert have used singular spectrum analysis to remove interference from in situ magnetic field data from the CASSIOPE/Swarm-Echo mission. But they did not settle the time-frequency overlap problem. In fact, most signal decomposition methods do not work well. These methods usually damage the natural signal because the overlapping areas remain indistinguishable.

In this paper, a novel method named the Instantaneous Phase Discontinuity (IPD) method is proposed to address this issue. Based on the sensitivity of instantaneous phase to variation of signal frequency, this method utilizes the discontinuities in the phase function to identify overlapping time-frequency regions. Subsequently, the natural signal within the overlapping region is carefully separated through frequency band contraction and envelope correction. IPD holds broad application prospects. As an example, IPD effectively separates interference from the time-frequency overlapping regions while preserving the integrity of natural signals when applied to data obtained from the CSES mission.

How to cite: Shi, F., Zeng, L., and Fu, Y.: An Innovative Technique for Reaction wheel Interference Separation in Satellite Magnetic Field Signals, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11558, https://doi.org/10.5194/egusphere-egu25-11558, 2025.

EGU25-11897 | Posters on site | NP6.1

Numerical studies of connectivity and Lagrangian transport in the world’s oceans 

Viacheslav Kruglov and Ulrike Feudel

Particles transport can be used to study flow fields on different scales in geophysics. Tracer and inertial particle transport can highlight the connectivity between different locations in the ocean or describe changes in flow fields based on the visualization of the flow by tracers. Of particular interest are long-range transport properties to either identify changes in flow paths due to climate change or to study the transport of seeds over long distances to identify sources of plants in different parts of the world. Such studies require particle tracking algorithms which are capable to work properly on a global scale of the Earth, i.e. on a spherical geometry. 

We have created a sophisticated software tool that simulates the movement of large numbers of tracer and inertial particles within interpolated oceanic velocity fields, in our examples based on the publicly available HYCOM data. Built in C++ and parallelized with Intel Threading Building Blocks (Intel TBB), it achieves high performance when dealing with substantial computational loads. To accelerate nearest-neighbor searches, we organize the grid points into a kd-tree, making it quick to locate grid points near any particle. We then interpolate the eastward and northward velocity components using a Gaussian-shaped weight function — an effective choice that avoids the singularities sometimes encountered in inverse distance interpolation. Since planar projections can introduce significant distortions on a global scale, we also account for Earth’s spherical geometry. Specifically, we solve two-dimensional tracer equations and the Maxey–Riley equation for inertial particles on a local tangent plane. Afterward, we revert the computed particle positions to latitude-longitude coordinates via an azimuthal equidistant projection, mitigating large-scale errors in simulations that may span thousands of kilometers.

The software is capable of simulating the dispersal of seeds and algae by ocean currents, easily managing hundreds of thousands of particles under varied initial conditions. It reconstructs connectivity maps between distant coasts, identifies transport barriers through finite-time Lyapunov exponent calculations, and can compute derivatives of the velocity field — such as divergence, vorticity, and the Okubo–Weiss parameter — broadening its range of oceanographic applications.

We highlight the software’s capabilities with two representative examples. First, we track the origins of particles (such as plant seeds) and explore their possible routes to Hawaii. Second, we assess the likelihood that harmful algal blooms could drift into the Baffin Bay during the warmest parts of the summer.

How to cite: Kruglov, V. and Feudel, U.: Numerical studies of connectivity and Lagrangian transport in the world’s oceans, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11897, https://doi.org/10.5194/egusphere-egu25-11897, 2025.

EGU25-13384 | Orals | NP6.1

Confinement and shedding 

Bernard Legras, Aurélien Podglajen, Mariem Rezig, and Clair Duchamp

Large-scale atmospheric vortices like the polar vortex or the Asian monsoon anticyclone are known to confine compounds for several months in the corresponding regions of the stratosphere with many consequences on the transport and the resulting atmospheric composition, the chemical activity and radiative properties.

It was recently discovered that confinement over the same time scale occurs also in much smaller mesoscale anticyclonic vortices generated within the absorbing plumes of smoke or ash generated by large forest fires and some volcanic eruptions.

As a rule, the atmosphere dissipates rapidly all inertial structures and these vortices are all maintained by a sustained forcing. We will discuss the similarities and differences among those vortices, the smoke vortices being distinguished by their autonomy as they carry their own source of forcing when they travel around the globe.

We will discuss the phenomenon of isentropic vortex shedding which is a main mechanical dissipation factor and show that it behaves very similarly at all scales. In the vertical direction, the flux processor of the large vortices will be compared to and distinguished from the leaking process of the rising smoke vortices. Other processes associated with radiative relaxation of thermal anomalies play role both to maintain and dissipate.

Although the state of understanding of smoke vortices is still very incomplete, a discussion of their condition of formation, maintenance and stability will be offered based on observations and idealized numerical simulation.

How to cite: Legras, B., Podglajen, A., Rezig, M., and Duchamp, C.: Confinement and shedding, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13384, https://doi.org/10.5194/egusphere-egu25-13384, 2025.

EGU25-14793 | ECS | Orals | NP6.1

On uniting Eulerian and Lagrangian mesoscale eddy perspectives 

Stella Bērziņa, Aaron Wienkers, Nicolas Gruber, and Matthias Münnich

Mesoscale eddies play a pivotal role in oceanic dynamics, influencing transport, mixing, and energy distribution. Current detection methods are primarily divided into Eulerian and Lagrangian approaches, each highlighting unique eddy characteristics. Eulerian methods rely on instantaneous fields, such as sea surface height, Okubo–Weiss parameter or vorticity, to identify the eddy boundaries. In contrast, Lagrangian approaches utilize water parcel trajectories to compute metrics like the Lagrangian Average Vorticity Deviation (LAVD) or Finite-Time Lyapunov Exponents (FTLE), identifying rotationally coherent Lagrangian vortices (RCLVs) with minimal exchange across the boundary. Eulerian eddies, however, are inherently "leaky", allowing for fluid exchange due to the fact that their boundaries are non-material. Despite these differences, both approaches capture complementary aspects of the same physical phenomenon. This study aims to bridge the gap between the two eddy detection methods by combining their strengths and leveraging high-resolution simulations from the coupled climate model ICON. Here, we identify daily RCLVs from evolving LAVD fields to find the time at which each Eulerian eddy loses coherence. In doing so, we will be able to explore how eddy coherence changes though its lifecycle and geographical location. This combined methodology can deepen our understanding of mesoscale ocean transport by quantifying realistic eddy trapping ability.

How to cite: Bērziņa, S., Wienkers, A., Gruber, N., and Münnich, M.: On uniting Eulerian and Lagrangian mesoscale eddy perspectives, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14793, https://doi.org/10.5194/egusphere-egu25-14793, 2025.

EGU25-17867 | ECS | Posters on site | NP6.1

An Intensive Biomass Burning Aerosol Observation phase in 2022, over Skukuza, South Africa: CO transport and balance over Southern Africa 

Marion Ranaivombola, Nelson Bègue, Gisèle Krysztofiak, Lucas Vaz Peres, Venkataraman Sivakumar, Gwenaël Berthet, Fabrice Jegou, Stuart Piketh, and Hassan Bencherif

The Biomass Burning Aerosol Campaign (BiBAC) was conducted in the Kruger National Park (KNP), at Skukuza in South Africa during the 2022 biomass burning season. The campaign included an Intensive Observation Phase (IOP) from September to October, aiming to quantify aerosol optical properties and plume transport.(Ranaivombola et al., 2024). The combination of ground-based (sun-photometer), satellite observations (MODIS, IASI and CALIOP), and CAMS reanalysis show a significant aerosol and carbon monoxide (CO) loading linked to biomass burning activity. Using AOD data from sun-photometer observations, Ranaivombola et al., (2024) define two events of biomass burning plume over the Southwestern Indian Ocean (SWIO) basin: September 18 to 23 and October 9 to 17, called here after event 1 and event 2, respectively.

During Event 1, the plume was transported toward the SWIO basin as a "river of smoke" phenomenon. As reported previously in the literature (Swap et al., 2003 and Flamant et al., 2022), the meteorological conditions were influenced by the passage of westerly waves associated with a cut-off low (COL) that favored the eastern transport pathway. However, it was not the case during Event 1. There were two troughs which supported the formation of two frontal systems and contributed to the transport of aerosols and CO plumes from South America (SAm) towards Southern Africa (SA). This transport was driven by a westerly baroclinic wave through the mid-tropospheric layers.

Event 2 involved a more complex synoptic setup with three frontal systems supported by three distinct troughs, allowing the recirculation of plumes over SA. This dynamic system enhanced the transport of CO plumes from SAm, which merged with African plumes over the Mozambique Channel. The sustained activity of the baroclinic wave generated new troughs, keeping aerosol levels high for an extended period of 1.5 week. The progression of baroclinic waves and frontal system development were essential in driving regional and intercontinental transport of aerosols and CO plumes.

These two events allowed to reveal two transport mechanisms of aerosol plumes and CO between SAm and SA towards the SWIO basin. It shows also that SA is a target region for aerosols and CO from SAm biomass burning. To assess and quantify the contributions of SA and SAm sources to observed CO concentrations over SA, we used the FLEXPART model (version 10.4) coupled with CO emissions database (biomass burning and anthropogenic emission from CAMS: GFAS and CAMS-GLOB-ANT, respectively). Each simulation tracked particles representing CO back in time over a period of 20 days, during the IOP. The setup included daily releases of 20,000 particles over six sites in Southern Africa (Skukuza, Durban, Maun, Upington, Mongu and Gobabeb). Both SA and SAm sources significantly influenced the CO balance over SA. The contribution of biomass burning emissions from SA were higher than those from SAm. Nevertheless, the biomass burning emission from SAm were more variable and could occasionally match or exceed those from SA. This quantification confirmed the predominance of African sources but also highlighted the presence of intercontinental transport which is poorly investigated until now.

How to cite: Ranaivombola, M., Bègue, N., Krysztofiak, G., Vaz Peres, L., Sivakumar, V., Berthet, G., Jegou, F., Piketh, S., and Bencherif, H.: An Intensive Biomass Burning Aerosol Observation phase in 2022, over Skukuza, South Africa: CO transport and balance over Southern Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17867, https://doi.org/10.5194/egusphere-egu25-17867, 2025.

EGU25-19212 | Posters on site | NP6.1

A Lagrangian Estimate of the Mediterranean Outflow's Origin 

Giulia Vecchioni, Paola Cessi, Nadia Pinardi, Louise Rousselet, and Francesco Trotta

The Mediterranean Sea is characterized by an anti-estuarine circulation, with Atlantic Water entering the Strait of Gibraltar at the surface and denser waters, formed within the basin, exiting at depth as the Mediterranean Outflow. Early studies identified the Western Mediterranean Deep Water, formed in the Gulf of Lions, as the primary source of the dense water masses contributing to the Outflow. While confirming this finding, more recent analyses of in-situ observations have highlighted additional contributions from other intermediate and deep water masses, such as Western Intermediate Water, Levantine Intermediate Water and Tyrrhenian Deep and Intermediate Waters.

In this study, the origin of the Mediterranean Outflow is investigated by deploying six million Lagrangian parcels at the Strait of Gibraltar, and advecting them backward in time using velocity estimates from an eddy-permitting reanalysis. Trajectories are integrated until parcels reach one of three origin sections within a maximum time of 78 years. To estimate the transport exchange between the origin sections and the Strait of Gibraltar, each parcel is tagged with a small volume transport, which is conserved along the trajectories due to the non-divergence of the velocity field.

The results indicate that 86% of the Outflow's transport originates from the Gulf of Lions, associated with Western Mediterranean Deep Water and Western Intermediate Water; 13% from the Strait of Sicily, related to Levantine Intermediate Water; and 1% from the Northern Tyrrhenian, related to Tyrrhenian Deep and Intermediate Waters. Mediterranean dense waters all recirculate in the Algerian Basin and in the deep Tyrrhenian basin, where stirring and mixing processes are hypothesized to occur. Before exiting the Strait of Gibraltar, anticyclonic recirculation induced by the western Alboran gyre decreases the density and depth of the water mass, ultimately shaping the characteristics of the Mediterranean Outflow. Temperature-salinity histograms at each origin section exhibit broad distribution, with peaks corresponding to expected water-mass types. The median transit times from the sections to the Strait of Gibraltar range from 5 years (Gulf of Lions) to 8 years (Strait of Sicily).

How to cite: Vecchioni, G., Cessi, P., Pinardi, N., Rousselet, L., and Trotta, F.: A Lagrangian Estimate of the Mediterranean Outflow's Origin, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19212, https://doi.org/10.5194/egusphere-egu25-19212, 2025.

This study investigates the 3-D Lagrangian evolution of Madagascar cyclonic eddies and their interaction with the Agulhas Current, combining targeted Argo float experiments, satellite altimetry data, and ocean modeling, following three in situ experiments. The region of interest spans from southwest Madagascar, where the South East Madagascar Current detaches from the continental shelf and generates dipoles, to the KwaZulu-Natal Bight, where the Agulhas Current flows southward.

The first two experiments, conducted in April and July 2013, deployed eight Argo floats configured to measure temperature and salinity at high temporal resolutions (daily and five-daily) and at varying park depths (300, 500, 650, and 1,000 m). These deployments assessed float retention within two cyclonic eddies that propagated southwestward over 130 days at an average speed of 11 km/day, undergoing growth, maturity, and decay phases before interacting with the Agulhas Current. A third experiment, conducted from May to September 2022, deployed two Euro-Argo ERIC-managed Core Argo floats southwest of Madagascar to further explore eddy dynamics. These floats drifted at non-standard depths of 650 m and 800 m, with adaptive cycle intervals (daily, 2-daily, and 5-daily) based on the eddy's proximity to the Agulhas Current. This experiment also captured the eastward propagation of the cyclonic eddy and its interaction with the current. In all three experiments, the floats exited the eddy when positioned below the depth at which the eddy's nonlinearity ratio dropped below 1. Complementary numerical simulations used an eddy identification and tracking algorithm with the GLORYS12V1 reanalysis product. Virtual particle releases and Lagrangian tracking at depths matching the above Argo float parking levels replicated the field experiments. Numerical results aligned with observations, showing that cyclonic eddies exhibited greater trapping depths during their mature phase and shallower depths during the growth and decay phases.

By integrating targeted float experiments, satellite data, and numerical simulations, this study provides a comprehensive understanding of eddy trapping dynamics southwest of Madagascar and their role in transporting heat, salt, and biogeochemical properties into the Agulhas Current. These findings demonstrate the potential of GLORYS12V1 combined with numerical Lagrangian particle tracking to address observational gaps in traditionally undersampled regions and underscore the benefits of combining ad hoc Argo configurations and numerical simulations for studying 3-D eddy dynamics.

How to cite: Aguiar González, B. and Morris, T.: Assessing the Trapping Dynamics of Madagascar Cyclonic Eddies Through Non-Standard Argo Float Experiments and Numerical Lagrangian Particle Tracking, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19267, https://doi.org/10.5194/egusphere-egu25-19267, 2025.

EGU25-334 | ECS | Posters on site | NP2.2

A new process-based carbon cycle for the FaIR simple climate model 

Alejandro Romero-Prieto, Camilla Mathison, Piers Forster, Glen Harris, Chris Jones, Ben Booth, and Chris Smith

Simple Climate Models (SCMs) provide an efficient way to explore potential climate futures by quickly evaluating emissions and mitigation scenarios.  This efficiency enables applications beyond the capabilities of complex Earth System Models (ESMs), such as integration with integrated assessment models and reactive policy analysis. A prominent example of this type of models is the FaIR SCM, which has gained popularity in recent years and been applied in various contexts. However, the current implementation of FaIR’s carbon cycle lacks detail, as it does not resolve the carbon fluxes between different ecosystem components. This limitation reduces the model’s flexibility and prevents it from participating in carbon-focused research.

Here, we present a new simple carbon cycle model that simulates the evolution of the global carbon stocks and fluxes across the atmosphere, ocean, soil and vegetation pools. The model calibration used data from 13 ESMs participating in the 6th Coupled Model Intercomparison Project (CMIP6), including all model simulations for the Shared Socioeconomic Pathways (SSP) scenarios. We evaluate the model’s performance in emulating ESM carbon cycles and discuss the integration with the FaIR SCM. By using the calibrations to CMIP6 ESMs and sampling the uncertainty parameters in our carbon cycle model, we can obtain posterior sets that compare well with best available observations, such as the growth in land, ocean and atmospheric stocks from the annual Global Carbon Budget. This enhancement to FaIR to include a process-based carbon cycle significantly strengthens its carbon cycle capabilities, unlocking new research opportunities.

How to cite: Romero-Prieto, A., Mathison, C., Forster, P., Harris, G., Jones, C., Booth, B., and Smith, C.: A new process-based carbon cycle for the FaIR simple climate model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-334, https://doi.org/10.5194/egusphere-egu25-334, 2025.

EGU25-1288 | ECS | Orals | NP2.2

The influence of freshwater biases on AMOC stability and consequences for CMIP6 models 

Amber Boot and Henk Dijkstra

The Atlantic Meridional Overturning Circulation (AMOC) modulates global climate and has been identified as a potential tipping element that might collapse under future climate change. Such a collapse would have strong global consequences for the climate system, ecosystems and society. The IPCC AR6 report states that it is unlikely that the AMOC will collapse in the 21st century which is mostly based on CMIP6 type Earth System Model results. However, these models have strong biases that can affect AMOC stability. If these models are biased towards a too stable AMOC, they might underestimate the probability of an AMOC collapse this century. To better understand the effects of freshwater biases on AMOC stability we perform experiments with the intermediate complexity Earth System Model CLIMBER-X. By introducing both positive and negative freshwater biases in the Atlantic and Indian Ocean we can gain a better understanding on how these biases affect AMOC stability. We find that introducing fresh biases in the Indian Ocean leads to an increase in stability, whereas fresh biases in the Atlantic Ocean lead to a decrease in stability. The combined effect of the biases in the Atlantic and Indian Ocean is near linear. We project the results of CLIMBER-X onto CMIP6 model biases such that we can assess whether CMIP6 models are likely simulating a too stable or too unstable AMOC.    

How to cite: Boot, A. and Dijkstra, H.: The influence of freshwater biases on AMOC stability and consequences for CMIP6 models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1288, https://doi.org/10.5194/egusphere-egu25-1288, 2025.

EGU25-2101 | Orals | NP2.2

TSformer: A Non-autoregressive Spatial-temporal Transformers for 30-day Ocean Eddy-Resolving Forecasting 

Guosong Wang, Xinrong Wu, Zhigang Gao, Min Hou, and Mingyue Qin

Ocean forecasting is critical for various applications and is essential for understanding air-sea interactions, which contribute to mitigating the impacts of extreme events. State-of-the-art ocean numerical forecasting systems can offer lead times of up to 10 days with a spatial resolution of 10 kilometers, although they are computationally expensive. While data-driven forecasting models have demonstrated considerable potential and speed, they often primarily focus on spatial variations while neglecting temporal dynamics. This paper presents TSformer, a novel non-autoregressive spatiotemporal transformer designed for medium-range ocean eddy-resolving forecasting, enabling forecasts of up to 30 days in advance. We introduce an innovative hierarchical U-Net encoder-decoder architecture based on 3D Swin Transformer blocks, which extends the scope of local attention computation from spatial to spatiotemporal contexts to reduce accumulation errors. TSformer is trained on 28 years of homogeneous, high-dimensional 3D ocean reanalysis datasets, supplemented by three 2D remote sensing datasets for surface forcing. Based on the near-real-time operational forecast results from 2023, comparative performance assessments against in situ profiles and satellite observation data indicate that, TSformer exhibits forecast performance comparable to leading numerical ocean forecasting models while being orders of magnitude faster. Unlike autoregressive models, TSformer maintains 3D consistency in physical motion, ensuring long-term coherence and stability in extended forecasts. Furthermore, the TSformer model, which incorporates surface auxiliary observational data, effectively simulates the vertical cooling and mixing effects induced by Super Typhoon Saola.

How to cite: Wang, G., Wu, X., Gao, Z., Hou, M., and Qin, M.: TSformer: A Non-autoregressive Spatial-temporal Transformers for 30-day Ocean Eddy-Resolving Forecasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2101, https://doi.org/10.5194/egusphere-egu25-2101, 2025.

EGU25-2501 | Posters on site | NP2.2

A Residual Ordering of SST Koopman Spectra for the Identification of Fundamental Modes 

Paula Lorenzo Sánchez and Antonio Navarra

El Niño-Southern Oscillation (ENSO) is a prominent driver of global climate variability, with significant impacts on ecosystems and societies. While existing empirical-dynamical forecasting methods, such as Linear Inverse Models (LIMs), are limited in capturing ENSO's inherent nonlinearity, Koopman operator theory offers a framework for analyzing such complex dynamics. Recent advancements in Koopman-based methods, such as DMD-based methods, have enabled exploration of nonlinear ENSO-related modes. However, they often suffer from challenges in robustness and interpretability. Specifically, k-EDMD algorithms tend to produce a large number of modes, complicating their physical relevance and reliability. In this study, we address these limitations by employing Colbrook’s Residual EDMD (Res-EDMD) framework as a tool to classify and prioritize modes based on their residuals. This approach enables us to systematically identify robust and physically meaningful modes, distinguishing them from less reliable counterparts. Furthermore, leveraging the property that eigenfunctions of Koopman operators can generate higher-order harmonics through powers and multiplications, we introduce a methodology to detect fundamental modes and their associated harmonics. Applying this framework to tropical Pacific SST data, we demonstrate that k-EDMD, together with Res-EDMD, are capable of isolating fundamental modes of tropical SST dynamics. These fundamental modes provide insights into the system's physical evolution and facilitate the retrieval of meaningful dynamical information. By systematically identifying and interpreting the modes, we establish a pathway to overcome the limitations of conventional Koopman-based methods, thereby enhancing their applicability for studying and forecasting complex climatic systems like ENSO. This study underscores the potential of Res-EDMD to refine mode selection in Koopman spectral analysis, paving the way for robust, physically interpretable insights into tropical SST variability.

How to cite: Lorenzo Sánchez, P. and Navarra, A.: A Residual Ordering of SST Koopman Spectra for the Identification of Fundamental Modes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2501, https://doi.org/10.5194/egusphere-egu25-2501, 2025.

EGU25-2814 | ECS | Orals | NP2.2

Ensemble simulation of the AMOC collapse in a conceptual climate model 

Dániel Jánosi, Ferenc Divinszki, Reyk Börner, and Mátyás Herein

The Atlantic Meridional Overturning Circulation (AMOC) is a mechanism of great importance, as its possible collapse would constitute a dramatic response to Earth’s changing climate. The AMOC is particularly important for Northern Europe, as it plays a central role in regulating the region’s climate, and a slowdown or collapse would lead to a significant cooling of the region. This critical transition has been the subject of many studies over the years, both from the aspects of climate modeling and dynamical systems theory. In the context of the latter, climate change is nothing but a complex, chaotic-like system, which possesses a time-dependent parameter, in the shape of e.g. the growing CO2 concentration. It has been known for some time now, that such systems not only have a chaotic attractor, but one which is also time-dependent, a so-called snapshot attractor. Such objects, and thus the systems they describe, can only be faithfully represented by statistics over an ensemble of trajectories, a single one does not suffice. We perform such ensemble simulations on a conceptual climate model of the AMOC, constructed by coupling the Lorenz84 and the Stommel box models. We find that the difference between the ensemble members in the point when the collapse occurs can be up to hundreds of years, and that some trajectories can even survive with the AMOC remaining in the “on” state.  This highlights the fact that that a single trajectory is unreliable, however, with the proper ensemble statistics (e.g. standard deviations, time-dependent Lyapunov exponents, etc), a probabilistic description of the collapse can be given.

How to cite: Jánosi, D., Divinszki, F., Börner, R., and Herein, M.: Ensemble simulation of the AMOC collapse in a conceptual climate model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2814, https://doi.org/10.5194/egusphere-egu25-2814, 2025.

EGU25-3266 | ECS | Orals | NP2.2

Non-Equilibrium Thermodynamics and Climate Predictability: Investigating Entropy Production and Frenesy 

Roberta Benincasa, Jeffrey B. Weiss, Danni Du, Gregory S. Duane, and Nadia Pinardi

Assessing climate predictability remains a central challenge in modeling and forecasting the climate system. Approaches from nonequilibrium statistical mechanics, particularly stochastic thermodynamics, have provided insights into non-equilibrium properties of stochastic models, which have proven useful in representing patterns of climate variability. In this work, we investigate the potential of entropy production and frenesy as tools for quantifying the predictability of non-equilibrium fluctuations in the climate system. Entropy production, a measure of the irreversibility of the system’s dynamics, is explored as an intrinsic indicator of predictability and its possible connections to the Anomaly Correlation Coefficient (ACC). Frenesy, a lesser-known quantity derived from active matter studies that captures kinetic fluctuations and dynamical activity, is assessed for its potential role in explaining non-equilibrium processes within the climate system. Thus, we aim to better understand the relationships between these thermodynamic quantities and climate oscillations, such as the El Niño-Southern Oscillation and the Madden-Julian Oscillation, with the ultimate goal of defining a new measure of climate predictability and better comprehending non-equilibrium processes in the ocean and the atmosphere.

How to cite: Benincasa, R., Weiss, J. B., Du, D., Duane, G. S., and Pinardi, N.: Non-Equilibrium Thermodynamics and Climate Predictability: Investigating Entropy Production and Frenesy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3266, https://doi.org/10.5194/egusphere-egu25-3266, 2025.

EGU25-3480 | ECS | Posters on site | NP2.2

Causal analysis of time series data for modeling nonlinear phenomena 

Kazuki Kohyama, Rin Irie, and Masaki Hisada

In typhoon forecasting, air-only and coupled air-sea models have similar accuracy in predicting typhoon trajectories. However, air-sea interactions must be considered to accurately forecast typhoon intensity [1]. Although coupling between multiple modules, including turbulence, waves, ecosystem, and chemistry, has been suggested to improve forecast accuracy, the modules and their individual model equations for typhoon forecasting are still determined empirically. Accurate modeling of the interactions between phenomena across multiple modules is an essential determinant of simulation accuracy. To determine critical factors within each module, parameterizations should be determined quantitatively, not empirically. However, it is challenging to impose preconditions on models that accurately capture the many complex interactions between air and sea.

In this study, we propose a modeling method to identify these critical factors using a causal analysis based on information theory. The causality of typical causal network models depends on the precondition network shape, but by using information theory, it is possible to extract causality comprehensively without preconditions. This allows for a quantitative assessment of causality without making the assumptions necessary for causal networks, such as Bayesian networks. In the proposed method, the information flux T, also known as transfer entropy, is defined as the difference in the Shannon entropy for multi-elements Q over two timesteps tn and tn+1 [2], as follows

TJI = H(Qjn+1Q≠in ) − H(Qjn+1Qn),

= ∑i,j p(in+1,in,jn) log p(in+1in,jn) / p(in+1in),

where H(Q) = Σ p(q) log p(q) is Shannon entropy, and we define Q as containing two elements Q = (I,J). Information flux quantifies the causality and amount of information flow between two time series. The magnitude of T corresponds to the parameter value indicating the interactions within and between the models. For example, recently, this method of quantifying causality was also applied to turbulence [3], which is one of the most chaotic phenomena, and used to clarify the causality of interactions between scales in the transport of scales in developed turbulence [4]. As a first step, we apply this method to a simplified non-linear model, and try to reconstruct its original model equation for test cases of the Lotka-Volterra model and the Lorenz model. For combinations of time series data for multiple variables generated by the models as multi-dimensional ordinary differential equations, we calculated the information flux according to the equation to extract the causal relationships of combinations with high T values. Then, by selectively rebuilding the model with only the variables of the elements that cause a high Tcause→effect value as the basis of the model function, the cost of parameter optimization is reduced, and the optimal parameter values are determined by fitting with the original time series data. In the presentation, we will discuss possibilities of the proposed method and its potential applications in climate simulations.

 

References
[1] L. R. Schade and K. A. Emanuel, J. Atmos. Sci. 56, pp. 642–651 (1999).
[2] T. Schreiber, Phys. Rev. Lett. 85, pp. 461–464 (2000).
[3] A. Lozano-Durán and G. Arranz, Phys. Rev. Res. 4, 023195 (2022).
[4] R. Araki, A. Vela-Martín, and A. Lozano-Durán, J. Phys.: Conf. Ser. 2753, 012001 (2024).

How to cite: Kohyama, K., Irie, R., and Hisada, M.: Causal analysis of time series data for modeling nonlinear phenomena, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3480, https://doi.org/10.5194/egusphere-egu25-3480, 2025.

EGU25-6571 | Orals | NP2.2

Challenging the hierarchy: what could a pluralist ecosystem of climate modelling strategies look like? 

Erica Thompson, Marina Baldissera Pacchetti, and Julie Jebeile
The predominant strategy of climate modelling is to continually increase resolution and complexity of general circulation models (GCMs). At present, there are calls to double down on this strategy and invest a lot more financial and computational resource into GCM resolution and complexity, with the assumption that this will improve the usefulness of climate predictions to support climate adaptation decision making.
We argue that this is not the best use of scientific effort.  Because there are many different kinds of questions encompassed within climate decision making - involving different individuals, communities and organisations with plural value systems - many different climate modelling strategies are needed which have different methodological aims and do not necessarily form a simple linear “hierarchy”, but can still learn from and complement each other.  We contrast the strengths and weaknesses of approaches such as GCMs, machine learning methods, EMICs, toy models, and narrative or storyline approaches as well as physics-informed models such as IAMs, ecosystem models and climate fiction.
We outline some ideas for what a (more) pluralist ecosystem of climate modelling strategies would look like, and how it could more effectively answer adaptation decision questions.

How to cite: Thompson, E., Baldissera Pacchetti, M., and Jebeile, J.: Challenging the hierarchy: what could a pluralist ecosystem of climate modelling strategies look like?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6571, https://doi.org/10.5194/egusphere-egu25-6571, 2025.

EGU25-6658 | ECS | Orals | NP2.2

Dealing with bugs is part of climate modeling 

Ulrike Proske

Numerical models are not just numerical representations of physical phenomena. They are also software files written by humans. As such they contain unintended coding errors, termed bugs. While the size of climate model code and human imperfection suggest that these are frequently present in climate models (Pipitone and Easterbrook, 2012), bugs are seldom acknowledged in the literature. However, missing understanding of model bugs hinders our understanding of model results as well as our ability to improve modeling workflows.

With a case study of the ICON general circulation model (GCM), I elucidate the practices and considerations around model debugging. Specifically, I give examples for bugs detected in that GCM's development and report on qualitative in-depth interviews I conducted with 11 model developers (domain scientists and scientific programmers). The interviews show that dealing with bugs is not a standardised process. While the technical testing of ICON code developments is highly standardised, and for example the assignment of responsibility is standardised implicitly, the scientific testing resists standardisation. The missing standardisation makes dealing with bugs a laborious process that takes time and effort and where human influence is common.

While this study focusses on the meaning of bugs for GCMs, similar considerations may be at play for models from different rugs of the model hierarchy. Where they differ, the model hierarchy may offer a way to more systematically detect and fix bugs in models of any rug.

 

 

Pipitone, J. and Easterbrook, S.: Assessing climate model software quality: a defect density analysis of three models, Geosci. Model Dev., 5, 1009–1022, https://doi.org/10.5194/gmd-5-1009-2012, 2012.

How to cite: Proske, U.: Dealing with bugs is part of climate modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6658, https://doi.org/10.5194/egusphere-egu25-6658, 2025.

EGU25-9070 | ECS | Orals | NP2.2

Physics-aware kernel Koopman operator estimation for consistent nonlinear mode decomposition 

Nathan Mankovich and Gustau Camps-Valls

Nonlinear dynamical systems are ubiquitous across scientific disciplines, yet their analysis and predictive modeling remain challenging due to their inherent complexity. Koopman operator estimation and Koopman mode decomposition are common tools for emulating and extracting modes of variability from such systems. In this work, we propose a novel method for Koopman operator estimation called the Physics-Aware Koopman Operator (PAKO). Our approach is tailored for physical consistency by introducing a regularization term based on the Hilbert-Schmidt Independence Criterion (HSIC) to enforce independence between predictions and sensitive or protected physical variables. In addition to Koopman operator estimation, we extract Koopman modes and eigenvalues through a Koopman mode decomposition. We validate PAKO on the ClimateBench dataset, demonstrating superior accuracy, robustness, and interpretability for estimating the internal variability of climate systems. Our results showcase the potential of PAKO for advancing Koopman operator estimation of complex nonlinear dynamical systems.

How to cite: Mankovich, N. and Camps-Valls, G.: Physics-aware kernel Koopman operator estimation for consistent nonlinear mode decomposition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9070, https://doi.org/10.5194/egusphere-egu25-9070, 2025.

EGU25-9917 | ECS | Orals | NP2.2 | Highlight

An unsupervised method for extracting coherent spatiotemporal patterns in multi-scale data 

Karl Lapo, Peter Yatsyshin, Brigitta Goger, Sara Ichinaga, and J. Nathan Kutz

The unsupervised and principled diagnosis of multi-scale data is a fundamental obstacle in earth sciences. Here we explicitly define multi-scale data as being characterized by spatiotemporal processes (i.e. processes acting along time and space simultaneously) with process scales acting across orders of magnitude, non-stationarity, and/or invariances such as translation and rotation. Existing methods, such as traditional analytic approaches, data-driven modeling like Dynamic Mode Decomposition (DMD), and even deep learning, are not well-suited to diagnosing multi-scale data, usually requiring supervised strategies such as human intervention, extensive tuning, or selection of ideal time periods.

We present the multi-resolution Coherent Spatio-Temporal Scale Separation (mrCOSTS), a data-driven method capable of overcoming the challenges of multi-scale data. It is a hierarchical variant of Dynamic Mode Decomposition (DMD) that enables the unsupervised extraction of spatiotemporal features in multi-scale data. It operates by decomposing the data into bands of temporal frequencies associated with coherent spatial modes. The method requires no training and functions with little to no hyperparameter tuning by instead taking advantage of the hierarchical nature of multi-scale systems.

We demonstrate mrCOSTS on multi-scale data from a range of disciplines and scales: 1) sea surface temperature of the El-Nino Southern Oscillation (ENSO), 2) Antartic sea ice concentration, and 3) directly evaluating a numerical weather model against LIDAR observations of wind speed. In each example we demonstrate how mrCOSTS can be used to gain insights into the underlying dynamics of each system, revealing missing components in the description of each system's variability, diagnosing extreme events, and provide a pathway forward for building better physical representations in models.

Using mrCOSTS, we show that ENSO is the result of 6 coherent spatio-temporal bands and use these results to explain the difference in intensity and spatial pattern of extreme 2015-2016 ENSO event relative to other extreme ENSO events. In the second example, we show that the dynamics of Antarctic sea ice concentration were found to have a negligible interannual component until 2012 when a long-term decline initiated and interannual dynamics at a decadal-scale started contributing. The large decline in sea ice concentration between 2014-2017 was almost entirely the result of the new interannual dynamics while the recent record low sea ice concentrations had a strong climate change signal. Finally, we demonstrate how mrCOSTS enables the evaluation of models directly against spatially-explicit observations. We evaluated an eddy-resolving numerical model against LIDAR observations of wind speed. The scale-aware model evaluation allowed us to easily reveal that errors at the largest scales dominated the system despite the agreement of lower order statistical moments. In each case using mrCOSTS we trivially retrieved complex dynamics that were previously difficult to resolve while additionally extracting previously unknown patterns or complexities of systems characterized by multi-scale processes.

How to cite: Lapo, K., Yatsyshin, P., Goger, B., Ichinaga, S., and Kutz, J. N.: An unsupervised method for extracting coherent spatiotemporal patterns in multi-scale data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9917, https://doi.org/10.5194/egusphere-egu25-9917, 2025.

Connecting the different levels of the hierarchy of complexity in which climate models operate, and comparing the assumptions that apply at each level, has led to much progress in climate science. A particularly notable success was Klaus Hasselmann’s use of Brownian motion to inspire his linear Markovian stochastic energy balance model (EBM), the history of which was recently summarised by Watkins [2024]. Another informative, but lateral, connection and comparison is that between either studying climate through the lens of stochastic physical models or doing so via statistical methods. This presentation showcases how comparing these approaches can sometimes surprise us.

It has been asserted that because the Hasselmann stochastic EBM has a mean-reverting term due to feedbacks, this property must also be detected in global mean temperature time series by statistical models such as the well-known Box-Jenkins ARIMA family. Conversely its absence has been taken as an indication of fundamental difficulties with anthropogenic driving. By fitting Hasselmann models, with and without anthropogenic driving, to an ARFIMA model with automatically selected parameters we show that in fact the absence of a prominent autoregressive term has precisely the opposite meaning, and is, rather, a clear indication of strong driving.

We will also report preliminary findings about the extent to which the presence of long range memory due to the multiple time scales present in the coupled ocean-atmosphere can affect the above conclusions, updating  the work summarised by Watkins et al [2024]. We thank Nick Moloney for many insightful suggestions.

Watkins, N. W., "Brownian motion as a mathematical superstructure to organise the science of climate and weather", In Foundational Papers in Complexity Science, Volume 3, pp. 1481–1510. Edited by David C. Krakauer. Santa Fe, NM: SFI Press. DOI: 10.37911/9781947864542.51 (2024).

Watkins, N. W., R. Calel, S. C. Chapman, A. Chechkin, R. Klages and D. Stainforth,   The Challenge of Non-Markovian Energy Balance Models in Climate.  Chaos. 34, 072105 . DOI:10.1063/5.0187815 (2024).

 

How to cite: Watkins, N. W. and Stainforth, D.:  Comparing the views of the driven climate system through the lenses of statistical time series analysis  and stochastic EBMs: Apparent absence of mean reversion can be evidence of anthropogenic driving., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12353, https://doi.org/10.5194/egusphere-egu25-12353, 2025.

EGU25-12960 | ECS | Orals | NP2.2

Data-driven Discovery of Predictive Spatiotemporal Patterns leading to Tropical Cyclogenesis 

Frederick Iat-Hin Tam, Tom Beucler, and James Ruppert

The early intensification (genesis) of tropical cyclones (TCs) is challenging to predict accurately in operational settings. The difficulty in predicting TC genesis stems from an insufficient understanding of the thermodynamic-kinematic characteristics involved in the multiscale interaction between clouds and TC circulations leading to genesis. Cloud-radiative feedback (CRF) has been shown to play a critical role in accelerating intensification during genesis by initiating secondary circulations that drive moisture and momentum convergence. However, it is still challenging to identify the exact pattern in radiation that could benefit genesis the most. Traditional diagnostic approaches to isolate CRF, such as the Sawyer-Eliassen Equation, require steady-state, axisymmetric thermal forcing. As such, these diagnostics methods are likely suboptimal in studying the response of weak TCs to intermittent, spatially asymmetric thermal forcing. 

 

This presentation utilizes novel data-driven methodologies to identify complex three-dimensional radiative patterns and approximate the thermodynamic-kinematic feedback between such patterns and early TC intensification. Specifically, we tasked a stochastic Variational Encoder-Decoder (VED) framework to discover different predictive patterns in radiative heating and quantify how these patterns affect early TC intensification. Applying the proposed framework to ensemble WRF simulations of Typhoon Haiyan (2013), longwave radiation anomalies in the downshear quadrants of Haiyan are shown to be particularly relevant to the early intensification of that TC. The extracted patterns provide new insights into how deep convective and shallow clouds should distribute spatially to best accelerate genesis. Apart from analyzing the extracted pattern, the stochastic nature of the proposed ML architecture brings additional insights into the radiatively-driven TC genesis research problem. We can use uncertainty in the prediction of intensification rates to track the time evolution of the relevance of radiation in tropical cyclone intensification. Furthermore, the uncertainty in the extracted pattern allows us to pinpoint trustworthy regions in the discovered predictive patterns for scientific interpretation.

 

Our study underscores the potential use of data-driven methodologies to quantify the impact of asymmetric radiative forcing on early TC formation without relying on axisymmetric or steady-state assumptions. The successful application of VED in this presentation reveals a promising way to use data-driven methods to uncover new knowledge in weather dynamics.

Reference:

Iat-Hin Tam, F., Beucler, T., & Ruppert, J. H., Jr. (2024). Identifying three-dimensional radiative patterns associated with early tropical cyclone intensification. Journal of Advances in Modeling Earth Systems, 16, e2024MS004401. https://doi.org/10.1029/2024MS004401

 

How to cite: Tam, F. I.-H., Beucler, T., and Ruppert, J.: Data-driven Discovery of Predictive Spatiotemporal Patterns leading to Tropical Cyclogenesis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12960, https://doi.org/10.5194/egusphere-egu25-12960, 2025.

EGU25-14237 | Orals | NP2.2

The Role of Internal Climate Variability in Noise-Shaped Hysteresis Cycles of the AMOC Under Rising CO2 Forcing 

Susanna Corti, Matteo Cini, Giuseppe Zappa, and Francesco Ragone

The Atlantic Meridional Overturning Circulation (AMOC), is a key tipping element of the climate system. A tipping point typically results from the interplay between external forcing (such as increased GHGs concentration or freshwater input) and the intrinsic internal variability of the system. While most studies mainly focus on identifying a critical forcing threshold (i.e. the minimal CO2 concentration or anomaly freshwater input needed for the collapse), the role of the internal climate variability remains less explored. Investigating the role of the internal variability requires performing large ensemble simulations which are  typically unfeasible with state-of-the-art models and traditional approaches. In our study, using an intermediate complexity model (PlaSIM-LSG, T21), once we assessed noise-induced collapse with a rare event algorithm, we investigated at which extent climate variability affects AMOC stability when CO2 forcing is applied. Traditionally, the AMOC stability landscape is investigated using single-realization hysteresis diagrams, driven by freshwater input in the North Atlantic. However, the effects of gradual CO2 forcing and, in particular, the impact of internal climate variability on the timing of AMOC tipping points have been less studied.  We conducted three independent hysteresis simulations, applying a slow CO2 ramp-up and ramp-down (0.2 ppm/year). Our findings reveal that internal variability strongly affects the timing of the AMOC tipping and the shape of the hysteresis cycle. In one simulation, we observed a reversed cycle, where the AMOC recovers at higher CO2 levels than at collapse. While statistical Early Warning Signals (EWS) provide some indication of approaching tipping points, the internal variability considerably reduces their predictability and introduces false positives. This suggests that AMOC behavior, when internal climate variability is considered, can differ significantly from characteristics of simpler models, and that caution is needed when interpreting results from a single-experiment realization. Moreover, the role of internal climate variability suggests that a probabilistic approach is necessary to define AMOC’s “safe operating space”, since it might not be possible to define a single critical CO2 threshold to prevent AMOC collapse.

How to cite: Corti, S., Cini, M., Zappa, G., and Ragone, F.: The Role of Internal Climate Variability in Noise-Shaped Hysteresis Cycles of the AMOC Under Rising CO2 Forcing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14237, https://doi.org/10.5194/egusphere-egu25-14237, 2025.

EGU25-14642 | ECS | Posters on site | NP2.2

Using Deep Learning to Identify Initial Error Sensitivity for Interpretable ENSO Forecasts 

Kinya Toride, Matthew Newman, Andrew Hoell, Antonietta Capotondi, Jakob Schlör, and Dillon Amaya

We introduce an interpretable-by-design method, optimized model-analog, that integrates deep learning with model-analog forecasting which generates forecasts from similar initial climate states in a repository of model simulations. This hybrid framework employs a convolutional neural network to estimate state-dependent weights to identify initial analog states that lead to shadowing target trajectories. The advantage of our method lies in its inherent interpretability, offering insights into initial-error-sensitive regions through estimated weights and the ability to trace the physically-based evolution of the system through analog forecasting. We evaluate our approach using the Community Earth System Model Version 2 Large Ensemble to forecast the El Niño-Southern Oscillation (ENSO) on a seasonal-to-annual time scale. Results show a 10% improvement in forecasting equatorial Pacific sea surface temperature anomalies at 9-12 months leads compared to the unweighted model-analog technique. Furthermore, our model demonstrates improvements in boreal winter and spring initialization when evaluated against a reanalysis dataset. Our approach reveals state-dependent regional sensitivity linked to various seasonally varying physical processes, including the Pacific Meridional Modes, equatorial recharge oscillator, and stochastic wind forcing. Additionally, forecasts of El Niño and La Niña are sensitive to different initial states: El Niño forecasts are more sensitive to initial error in tropical Pacific sea surface temperature in boreal winter, while La Niña forecasts are more sensitive to initial error in tropical Pacific zonal wind stress in boreal summer. This approach has broad implications for forecasting diverse climate phenomena, including regional temperature and precipitation, which are challenging for the model-analog approach alone.

How to cite: Toride, K., Newman, M., Hoell, A., Capotondi, A., Schlör, J., and Amaya, D.: Using Deep Learning to Identify Initial Error Sensitivity for Interpretable ENSO Forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14642, https://doi.org/10.5194/egusphere-egu25-14642, 2025.

EGU25-15878 | Posters on site | NP2.2

Spatiotemporal Similarity-Based Approach for Analyzing the Relationship Between Sea Fog Occurrence and Sea Level Pressure Distributions 

Sung-Hwan Park, Hojin Kim, Ki-Young Heo, and Nam-Hoon Kim

This study presents a novel methodology for analyzing the relationship between sea level pressure (SLP) distributions and sea fog occurrences, focusing on a spatiotemporal similarity-based approach. Using SLP data from 2001 to 2019 and visibility observations from Baengnyeong Island (BYI), Yellow Sea, the proposed framework quantifies the connection between atmospheric pressure patterns and sea fog formation. The methodology integrates three key components: defining temporal and spatial domains, calculating weighted similarities, and validating the results using sea fog occurrence data. The temporal domain was set to a 7-hour period, determined by analyzing visibility trends prior to sea fog events. This period captures the critical atmospheric changes leading to fog formation. Spatially, a 2D weighted map was constructed using Pearson correlation coefficients between SLP variations at BYI and other locations in the study area. This weighting emphasizes regions with strong correlations, ensuring the analysis focuses on areas most relevant to sea fog dynamics. The Spatiotemporal Similarity Measure (STSM) method was then applied to compare reference SLP maps from 2017–2019 with historical SLP data from 2001–2015. By identifying historical cases with high similarity to reference conditions, the study examined the likelihood of sea fog occurrences under similar atmospheric setups. These similarities were categorized into thresholds, and their connection to sea fog events was evaluated using Probability of Detection (POD) and False Alarm Ratio (FAR) metrics. The results demonstrate that higher SLP similarity corresponds to increased POD and decreased FAR, validating the effectiveness of the STSM method. This approach highlights the role of recurring SLP patterns in sea fog formation and underscores the utility of historical data in improving sea fog forecasting.

How to cite: Park, S.-H., Kim, H., Heo, K.-Y., and Kim, N.-H.: Spatiotemporal Similarity-Based Approach for Analyzing the Relationship Between Sea Fog Occurrence and Sea Level Pressure Distributions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15878, https://doi.org/10.5194/egusphere-egu25-15878, 2025.

EGU25-16465 | ECS | Posters on site | NP2.2

Simplifying Earth System Projections: Mimicking ESM Results with a Diffusion Model 

Edward Gow-Smith, Roberta Benincasa, Marco M. De Carlo, Evgeny Ivanov, Simone Norberti, and Will Chapman

Ensemble simulations using Earth System Models (ESMs) have historically been used to gain insights into future climate scenarios. However, they present notable disadvantages, particularly their long computing times and the high technical threshold required for accessibility. The recent rise of data-driven approaches offers a promising alternative, making long-term climate projections more efficient, accessible to policymakers and regional planners, and scalable for specific regions.

During the Winter School “Data-Driven Modeling and Predictions of the Earth System,” we compared the results of a simple diffusion model with the ensemble results from the CESMv.2.1.5 Large Ensemble from model year 2015 to 2090. The diffusion model, trained on CESM data, uses only CO₂ concentration and the month of the year as context channels to predict spatially-resolved, monthly averaged air temperature, precipitation, and atmospheric pressure on a global scale. The project aimed to demonstrate how effectively the diffusion model simulates global and regional variability and long-term trends in these atmospheric variables compared to the ESM. Particular attention was given to its representation of the El Niño–Southern Oscillation (ENSO) region. Additionally, a bias correction was applied to the diffusion model results against the ESM to evaluate distortions in trends and variability.

The study concluded that even a simple diffusion model has significant potential for predicting meteorological parameters based solely on projected greenhouse gas emissions and the time of year. However, its performance weakened near the poles in reproducing ESM results, highlighting the importance of incorporating additional geographic variables (e.g., grid cell size) during training. Despite these limitations, combining the strengths of coupled ESMs with diffusion models can leverage the physical accuracy of ESM outputs and the computational efficiency and adaptability of diffusion models, offering a more comprehensive understanding of Earth system dynamics.

How to cite: Gow-Smith, E., Benincasa, R., De Carlo, M. M., Ivanov, E., Norberti, S., and Chapman, W.: Simplifying Earth System Projections: Mimicking ESM Results with a Diffusion Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16465, https://doi.org/10.5194/egusphere-egu25-16465, 2025.

EGU25-17680 | Orals | NP2.2

Climate-carbon cycle modelling hierarchy 

Chris Jones

Much climate science relies on numerical modelling to both understand the processes of the Earth system and to make predictions or projections of how it may change in the future. International climate policy relies on the outcomes of these models to make decisions which will affect the lives and livelihoods of billions of people – so it is vital that they are well understood and their use is based on robust understanding of what they can (and also what they cannot) tell us.

Spatially resolved General Circulation Models (GCMs) have evolved over recent decades in both their spatial resolution (allowing finer detail to be studied) and their process complexity (including but not limited to biogeochemistry and feedbacks between climate and ecosystems). This expansion of their capability makes them more useful and relevant than ever, but they are extremely slow to run on even the worlds most powerful super computers. Conversely very simple models exist which can be run thousands (or millions) of times, but do not include the full detail of the GCMs. Finally there are models of intermediate complexity which sit between these extremes and also make valuable contributions through differing combinations of comprehensiveness and computational efficiency.

All classes of models have something to offer – it is important to understand their strengths and weakness and to choose the most suitable tool for the job. Moreover, use of these models together can be very powerful. For example IPCC reports tend to draw firstly on complex GCMs but then through thorough calibration processes propagate their information to larger numbers of scenarios using simplified climate emulators.

In this talk I will briefly outline how this mode of use of the full modelling hierarchy has developed in the field of carbon cycle feedbacks and in quantifying the remaining carbon budget – which allows detailed planning of climate mitigation policy aligned with the goals of the Paris Agreement. I will show the development of our understanding of climate-carbon cycle feedbacks from complex models and how these have been used first to determine a simple relationship between cumulative CO2 emissions and global warming (so called TCRE: transient climate response to carbon emissions), and then how simple models have been used in conjunction with complex models to explore the processes behind this relationship and begin to allow propagation of observational constraints.

I will end by outlining emerging knowledge on the strengths and weakness of each class of model (e.g. how simple is too simple?) and identifying research gaps for moving forward.

How to cite: Jones, C.: Climate-carbon cycle modelling hierarchy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17680, https://doi.org/10.5194/egusphere-egu25-17680, 2025.

There is a long history of global climate model (GCM) studies of the response of the Atlantic Meridional Overturning Circulation to changing greenhouse gases (GHGs). Alongside this is an almost separate branch of the literature studying the AMOC’s response to fresh water input (‘hosing’) with fixed GHGs, focusing on the potential for ‘tipping’ behaviour. Some common model responses are observed among models (e.g. in GHG experiments an initial AMOC weakening associated with warming of the subsurface North Atlantic), but also considerable diversity, especially in the long-term response following stabilisation of GHG concentrations or hosing.

In recent years a few studies have emerged that use in-depth analysis frameworks to give insight into individual model responses, or into the differences between model responses. However the two branches of the literature (GHG and hosing response) have remained largely independent, and there is an increasing recognition that in real-world climate change the ‘smooth’ response to GHGs and potential abrupt ‘tipping’ responses need to be considered together. Given the diversity of model responses it will be valuable to establish whether there is a simple model framework that captures the potential mechanisms of response to GHGs and hosing that have been identified in GCMs. Such a model can then be used to characterise the types of qualitative behaviour that are possible in the more relevant scenario of tipping in a warming climate.   

We present a simple box model of thermally- and haline-driven AMOC change that aims to capture in as simple a form as possible many of the mechanisms of the AMOC responses to GHGs and hosing that have been identified in the literature. To develop this from an earlier model (that captured purely the hosing response), it was found necessary to add both a simple representation of basin-scale energy and water balances, and a simple representation of varying stratification in the sub-polar North Atlantic, increasing the dynamical degrees of freedom of the model.

We show that the model captures a wide range of behaviours seen in GCM experiments, and use it to identify circumstances in which AMOC tipping may be possible without requiring unrealistic additional water input from the Greenland Ice Sheet.

How to cite: Wood, R.: Towards a unified understanding of AMOC changes under warming and fresh water forcing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17881, https://doi.org/10.5194/egusphere-egu25-17881, 2025.

EGU25-19443 | ECS | Orals | NP2.2

Linking response to forcing to natural variability using a Koopman operator formalism 

John Moroney, Valerio Lucarini, and Niccolò Zagli

Response theory has been shown to be a powerful tool in determining the impact of external forcing on the earth’s climate. High sensitivity to perturbations and the slow decay of response functions is associated with critical behaviour and tipping points. Despite the nonlinear nature of the climate dynamics, a generalisation of the fluctuation-dissipation theorem provides a direct connection between these response functions and the natural variability of the system. We show how response functions for a complex dynamical system may be written as a sum of terms that depend on the eigenvalues and eigenfunctions of the Koopman operator of the system, each term corresponding to a mode of variability. We demonstrate in a number of low-dimensional examples how extended dynamic mode decomposition may be used to accurately compute response and correlation functions of various observables, given only a set of snapshot data.

How to cite: Moroney, J., Lucarini, V., and Zagli, N.: Linking response to forcing to natural variability using a Koopman operator formalism, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19443, https://doi.org/10.5194/egusphere-egu25-19443, 2025.

EGU25-19722 | Orals | NP2.2

A stable hothouse triggered by a tipping mechanism 

Erik Chavez, Michael Ghil, and Jan Rombouts

The climate system is nonlinear and affected by both natural variability and several types of forcing. The impact of anthropogenic forcing and environmental change on several of the system's nonlinear processes has led to considerable concern about the tipping of regional subsystems (e.g. Lenton, 2016), due to their potentially irreversible consequences. On the global level, these nonlinear effects have been shown to give rise to bistability (Stommel, 1961} and chaotic behavior (Lorenz, 1963) in the system's past (e.g., Boers et al, 2022), as well as having been proposed conceptually as due to occur in its future, too (e.g., Steffen et al, 2018). However, specific mechanisms for a sudden tipping to an alternate stable “hothouse”, several degrees warmer than the present climate, have not been explored so far to a satisfactory extent with ESM-based studies using aqua planets (e.g., Ferreira et al 2011, Popp et al, 2016).

   Here we show that a highly simplified energy balance model (EBM) of globally averaged temperature T representing the radiative budget, coupled with a three box-type model of global carbon dynamics, does exhibit such an alternate stable hothouse climate with T higher by roughly 10 °C than the present. This TCV model also captures quite accurately the fluxes of carbon between the separate reservoirs of the coupled atmosphere-land-ocean system, when compared with observations and with simulations by high-end models. The model includes two regional mechanisms, that trigger a global tipping to such a hothouse. The two regional mechanisms are (i) the decrease of terrestrial albedo due to the darkening of ice sheets by pervasive glacial micro algal growth (e.g., Williamson et al, 2020) not included in ESMs to date; and (ii) the limits of vegetation adapting to increased environmental stress and, hence, the reduction of its carbon absorbtion (e.g., Hammond, 2022).

    These findings and the mechanistic understanding of the processes leading to a global tipping can contribute to a fruitful dialogue between the conceptual-model and ESM communities. Such a dialogue can greatly enhance our understanding of the climate system’s potential for global tipping in response to anthropogenic greenhouse gas emissions.  

How to cite: Chavez, E., Ghil, M., and Rombouts, J.: A stable hothouse triggered by a tipping mechanism, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19722, https://doi.org/10.5194/egusphere-egu25-19722, 2025.

EGU25-20182 | Orals | NP2.2

Morphological cellular analysis of Pockets of Open Cells on Marine 

Jan Haerter and Diana Monroy

More of Earth’s surface is covered by Stratocumulus clouds (Sc) than by any other cloud
type making them extremely important for Earth’s energy balance, mostly due to reflection of
solar radiation. However, representing Sc and their radiative impact is one of the largest chal-
lenges for global climate models because these cannot resolve the length scales of the processes
involve in its formation and evolution. For this reason, Sc clouds represent a large uncertainty
for climate projections [1].
The challenge becomes more intricate due to the organizational complexity that Sc clouds
present in a broad range of spatial scales. In particular, Sc fields over the oceans display
characteristic mesoscale patterns that can present both organized and unorganized structures.
Between these morphological types, cellular convection receives particular attention given than
cloud decks self-organize into honeycomb-like hexagonal patterns composed by closed and
open convective cells fields.
The purpose of this project is to analyze satellite images of a particular tendency of Sc to orga-
nize into spatially compact, cellular-patterned, low-reflectivity regions of open cells embedded
in closed cellular cloud fields called as pockets of open cells (POCs) [2].
We aim to propose a segmentation, cell tracking and quantitative analysis of cell shape and
behavior changes in closed and open cell fields, in particular the interaction of both cells when
POCs are formed. A statistical analysis of different POCs will be carried to describe the time
and spatial contributions of cell shape changes, transitions and rearrangements in the evolution
of cellular patterns on Sc clouds considering the local dynamics between individual cells.
We hypothesize that the interaction between cold pools that are formed when open cells pre-
cipitate triggers a rapid dynamics on open cells fields. For its part, closed cells fields present
steady morphology until perturbations are formed triggering the formation of POCs.

How to cite: Haerter, J. and Monroy, D.: Morphological cellular analysis of Pockets of Open Cells on Marine, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20182, https://doi.org/10.5194/egusphere-egu25-20182, 2025.

EGU25-20523 | Posters on site | NP2.2

Seasonal Forecasts with Transformers methods 

Antonio Navarra

Transformer-based approaches to seasonal forecasting have emerged as powerful tools in predicting climate patterns by leveraging deep learning techniques. These models, initially designed for natural language processing, excel in capturing long-range dependencies and complex temporal patterns, making them suitable for climate data characterized by intricate temporal relationships. In seasonal forecasting, transformers can process sequential data such as surface temperature and SST, learning from historical patterns to predict future seasonal variations.

A crucial enhancement to this approach is the exploitation of spatial coherence, which is often captured by variance modes. Variance modes, such as those derived from empirical orthogonal functions (EOFs), identify dominant spatial patterns in climate data, encapsulating the spatial correlations across different regions. By integrating these modes into transformer models, it becomes possible to enhance the model’s understanding of spatial dependencies, leading to more accurate and coherent seasonal forecasts.
Furthermore, the model allows to focus on the predictability of time means, from monthly to seasonal, and also on specific sectors of the variabilith as they are identified by EOFs. This approach aligns with practical forecasting needs, where average conditions over extended periods are often more relevant than short-term fluctuations. By combining transformers, spatial coherence, and time-averaged data, this method holds significant promise for advancing seasonal climate forecasting.

How to cite: Navarra, A.: Seasonal Forecasts with Transformers methods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20523, https://doi.org/10.5194/egusphere-egu25-20523, 2025.

The influence of structural errors in general circulation models (GCMs) — stemming from missing physics, imperfect parameterizations of subgrid-scale processes, limited resolution, and numerical inaccuracies — results in systematic biases across various components of the Earth system.

 

In this talk, we develop an approach to correct biases in the atmospheric component of the Community Earth System Model (CESM) using convolutional neural networks (CNNs) to create a corrective model parameterization for online bias reduction. By learning to predict systematic nudging increments derived from a linear relaxation towards the ERA5 reanalysis, our method dynamically adjusts the model state, significantly outperforming traditional corrections based on climatological increments alone. Our results demonstrate substantial improvements in the root mean square error (RMSE) across all state variables, with precipitation biases over land reduced by 25-35%, depending on the season. Beyond reducing climate biases, our approach enhances the representation of major modes of variability, including the North Atlantic Oscillation (NAO) and other key aspects of boreal winter variability. A particularly notable improvement is observed in the Madden-Julian Oscillation (MJO), where the CNN-corrected model successfully propagates the MJO across the maritime continent, a challenge for many current climate models. Using trio-interaction theory, we explore the dynamic improvements to the MJO and assess whether these enhancements arise from accurate physical processes.

 

This advancement underscores the potential of using CNNs for real-time model correction, providing a robust framework for improving climate simulations. Our findings highlight the efficacy of integrating machine learning techniques with traditional dynamical models to enhance climate prediction accuracy and reliability. This hybrid approach offers a promising direction for future research and operational climate forecasting, bridging the gap between observed and simulated climate dynamics.

How to cite: Chapman, W. and Berner, J.: Improving climate bias and variability via CNN-based state-dependent model-error corrections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20624, https://doi.org/10.5194/egusphere-egu25-20624, 2025.

EGU25-1069 | ECS | PICO | AS4.17

Study on long-range transport of dust-associated airborne bacteria over Eastern Himalayas in India 

Antara Pramanick, Shahina Raushan Saikh, Md Abu Mushtaque, and Sanat Kumar Das

Transboundary movement of atmospheric microorganisms through dust transportation plays a pivotal role in influencing human health, agricultural productivity, and climate dynamics by participating in cloud condensation processes. Present study investigates long-range transported atmospheric bacteria along with dust particlesover Darjeeling (27°03′N, 88°26′E), a high-altitude region (2.2 km amsl) in the Eastern Himalayas, India. 27 samples are collected in winter (Temp: 6.2± 1.5°C; RH: 85.2 ± 9.6%) and summer 2022 (Temp: 16 ± 1.5°C; RH: 93.5 ± 6.5%). Total bacterial cell count is found tobe increased by 24 ± 0.4% in summer compared to that in winter. Concurrently, particle number concentrations, measured using a Scanning Mobility Particle Sizer (SMPS) within the size range of 8-350 nm, showed 70% increasein summer, with modal size shifting from 110 nm to 150 nm.Satellite observations from MODIS on-board Aqua, Terra, and OMI on-board Aura reveal an increase in Aerosol Optical Depth (AOD) from 0.4 in winter to 0.7 in summer, alongside decline in Angstrom Exponent from 1.6 to 0.3, indication of coarser aerosol abundances. Aerosol Index also rises from 0.8 to 2.1, indicating dust dominance. CALIPSO data identifies a 1 km thick dust layer within 2 to 3 km altitude above the Eastern Himalayas. Air mass back-trajectory analysis suggests dust particles travel at an altitude of 2 to 3 km from the Thar Desert to Eastern Himalayas.Seasonal shifts in microbial communities are evident, with higher Shannon diversity in summer (4.4 ± 0.8) compared to winter (2.3 ± 0.6). Beta diversity analyses confirm distinct community compositions in summer that is due to transport of unique bacteria attached with desert dust. In summer, predominant bacterial genera included Flavobacterium (5.4 ± 3.6%), Nocardioides (4.2 ± 3%), and Corynebacterium (4.2 ± 1.4%), while Corynebacterium (2.4 ± 0.5%), Acinetobacter (1.8 ± 0.9%), and Massilia (1.3 ± 0.3%) in winter. Notably, pathogenic genera such as Afipia and Clostridium, linked to human and animal infections, are detected with dust exclusively in summer.Presentresult highlights the role of transported dust-associated microbes in altering the airborne bacterial composition in the Himalayas, providing critical insights into the sources and biodiversity changes over the Eastern Himalayas in India.

How to cite: Pramanick, A., Saikh, S. R., Mushtaque, M. A., and Das, S. K.: Study on long-range transport of dust-associated airborne bacteria over Eastern Himalayas in India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1069, https://doi.org/10.5194/egusphere-egu25-1069, 2025.

EGU25-1414 | ECS | PICO | AS4.17

 Cyanobacteria and climate change: Insights from Atmospheric and Heritage Studies  

Alessandra Mascitelli, Piero Chiacchiaretta, Fernanda Prestileo, Eleonora Maria Stella, Eleonora Aruffo, Pasquale Simeone, Paola Lanuti, Silvia Di Lodovico, Mara Di Giulio, Simone Guarnieri, Piero Del Boccio, Maria Concetta Cufaro, Valentina Gatta, Federico Anaclerio, Stefano Dietrich, and Piero Di Carlo

The atmosphere plays a pivotal role in modulating the interactions between microorganisms and their surrounding environments, influencing ecological cycles, heritage conservation, and providing opportunities for novel applications. Recent studies have highlighted the role of microbial responses to atmospheric conditions as indicators of environmental change [1]. This study highlights the potential of cyanobacteria as biosensors for detecting and monitoring climate change, using the Majella Massif region of Central Italy as a case study. The region’s rock art, characterized by red and black schematic motifs, is increasingly impacted by microbial colonization, driven by climate-induced temperature variations. These impacts align with broader research showing the link between microbial growth patterns and climatic factors [2]. 

Laboratory analyses were performed on cyanobacteria samples collected near rock paintings in Lama dei Peligni, Abruzzo. Using BG11 culture medium under controlled conditions, the growth rates of cyanobacteria were compared at two temperature regimes: 14.3 °C, representing historical mean temperatures (1930-1970), and 18.6 °C, reflecting current averages (2023). Results revealed a significant increase in growth rates at the higher temperature (40 cfu/ml vs. 35 cfu/ml), demonstrating their sensitivity to climatic shifts. Similar findings have been reported in studies of microbial ecology, emphasizing the value of cyanobacteria as biosensors [3]. This sensitivity positions cyanobacteria as effective biosensors for tracking environmental changes over time. 

These findings underscore the dynamic role of atmospheric factors in shaping microbial survival and propagation. Beyond their implications for heritage conservation, cyanobacteria’s responsiveness to temperature changes offers a unique avenue for monitoring broader climate dynamics. The enhanced growth of cyanobacteria due to rising temperatures also poses a challenge: while serving as indicators of change, their proliferation can degrade cultural heritage sites, threatening their preservation. This duality has been widely documented, where microorganisms act as both agents of degradation and ecological indicators [4,5]. 

This research advocates for interdisciplinary approaches that integrate atmospheric sciences, microbial ecology, and heritage studies to explore the dual role of cyanobacteria as both threats and tools. By leveraging their biological traits, cyanobacteria can provide valuable insights into climate dynamics while emphasizing the urgency for proactive strategies to mitigate environmental impacts on vulnerable ecosystems and heritage sites. 

[1] Decho, A. W., et al. (2010). "Microbial indicators of environmental change." 

[2] Pointing, S. B., et al. (2009). "Microbial growth patterns linked to climatic factors." Colwell, R. R., et al. (2008). "Microbial responses to atmospheric shifts." 

[3] Paerl, H. W., & Huisman, J. (2008). "Cyanobacteria as biosensors for climate monitoring." Whitton, B. A. (2012). "Ecological roles of cyanobacteria." 

[4] Gu, J. D., et al. (2021). "Microorganisms in heritage conservation." Mitchell, R., et al. (2013). "Dual roles of microorganisms in degradation and ecology." 

[5] Foster, P. L., et al. (2021). "Cyanobacteria in environmental monitoring." Singh, A., et al. (2020). "Applications of cyanobacteria in climate studies." 

How to cite: Mascitelli, A., Chiacchiaretta, P., Prestileo, F., Stella, E. M., Aruffo, E., Simeone, P., Lanuti, P., Di Lodovico, S., Di Giulio, M., Guarnieri, S., Del Boccio, P., Cufaro, M. C., Gatta, V., Anaclerio, F., Dietrich, S., and Di Carlo, P.:  Cyanobacteria and climate change: Insights from Atmospheric and Heritage Studies , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1414, https://doi.org/10.5194/egusphere-egu25-1414, 2025.

EGU25-1548 | ECS | PICO | AS4.17

Hidden Ecosystems Above: Unraveling Viral-Bacterial Interactions in Cloudwater 

Janina Rahlff, Ritam Das, Rebecca Büschel, Julia Micheel, and Manuela van Pinxteren

Clouds have been regarded as atmospheric oasis for microbes including psychrophilic bacteria (Delort et al., 2017; Péguilhan et al., 2023). However, adaptations of bacteria to the cloud environment and interactions with viruses are not fully understood. In this study, cloudwater was sampled with six compact Caltech active strand cloud water collectors (Demoz et al., 1996) on the Mount Verde, a mountain of 744 m height on the São Vicente island in the tropical Atlantic Ocean (van Pinxteren et al., 2020) and stored frozen. From iron-flocculated and filtered cloudwater samples, DNA was short-read sequenced for metagenomics, and 24 bacteria were additionally isolated from these samples on Luria-Bertani (LB) and Reasoner's 2A (R2A) agar. After purification, the bacterial DNA was subjected to whole-genome sequencing, revealing a diverse array of microbial taxa. The isolate genomes were identified as belonging to Gram-positive species, including Agrococcus sp., Alkalihalobacillus_A gibsonii_A, Arthrobacter sp., Bacillus spizizenii, Cytobacillus oceanisediminis, Curtobacterium spp., Deinococcus sp., Micrococcus luteus, and Rossellomorea spp., as well as Gram-negative species such as Paracoccus marcusii, and Sphingomonas sp. This microbial diversity highlights the presence of spore-forming, halotolerant, and marine-associated bacteria in cloudwater. The genomes had an average GC content of 58.3% (range 41% – 73%) and encoded for cold-shock genes probably supporting survival during sample freezing and in supercooled cloudwater. The presence of 24 prophages and a diverse arsenal of antiviral defense systems, including adaptive CRISPR immunity targeting viral operational taxonomic units (vOTUs), indicates ongoing bacterial-viral interactions in cloudwater. On average, bacterial strains encoded for five defense systems, with restriction-modification systems being the most common. Interestingly, the isolated strain Sphingomonas sp. MPC37 encoded for the highest number of defense systems (12), indicating its potential ecological significance in this unique environment. Metagenomic sequencing identified 458 vOTUs, with major bacterial hosts predicted as Sphingomonas spp. (75 vOTUs), Deinococcus spp. (15), Novosphingobium spp. (14), and Methylobacterium spp. (13). Analysis of air mass trajectories for the cloudwater suggests a marine origin for certain samples, which were associated with the highest counts of both unique and total vOTUs. We also find genetic variability within a population of closely related viruses (microdiversity). Viral variants arise sequentially during different cloud events and are shared among temporally proximate events. Our results reveal clouds as dynamic microbial and viral ecosystems with complex survival strategies and interactions.

References

Delort, A. M., Vaïtilingom, M., Joly, M., … & Deguillaume, L. (2017). Clouds: a transient and stressing habitat for microorganisms. Microbial ecology of extreme environments, 215-245. https://doi.org/10.1007/978-3-319-51686-8_10

Demoz, B. B., Collett, J. L., & Daube, B. C. (1996). On the Caltech Active Strand Cloudwater Collectors. Atmospheric Research, 41(1), 47-62. https://doi.org/10.1016/0169-8095(95)00044-5

Péguilhan, R., Rossi, F., Joly, M., … & Amato, P. (2023). Clouds, oases for airborne microbes – Differential metagenomics/ metatranscriptomics analyses of cloudy and clear atmospheric situations. bioRxiv, 2023.2012.2014.571671. https://doi.org/10.1101/2023.12.14.571671

van Pinxteren, M., Fomba, K. W., Triesch, N., . . . & Herrmann, H. (2020). Marine organic matter in the remote environment of the Cape Verde islands – an introduction and overview to the MarParCloud campaign. Atmos. Chem. Phys., 20(11), 6921-6951. https://doi.org/10.5194/acp-20-6921-2020

 

How to cite: Rahlff, J., Das, R., Büschel, R., Micheel, J., and van Pinxteren, M.: Hidden Ecosystems Above: Unraveling Viral-Bacterial Interactions in Cloudwater, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1548, https://doi.org/10.5194/egusphere-egu25-1548, 2025.

Airborne microorganisms (bioaerosols) play crucial roles in global biogeochemical cycles and ecosystem dynamics. We have developed a novel dual-chamber atmospheric simulation system to investigate the physicochemical properties and survival mechanisms of bioaerosols under controlled conditions.

The system is installed in a BSL-2 compliant Class 100 clean room and features two interconnected stainless steel chambers. The material selection and surface treatment of the chambers have been optimized to minimize microbial adhesion while preventing electrostatic losses of aerosol particles. Each chamber is equipped with UV irradiation systems and precise temperature control mechanisms. The chambers are connected by dampers, enabling separate control of environmental conditions. This design allows for bioaerosol generation in one chamber while conducting exposure experiments with various environmental factors (disinfectants, temperature, humidity, UV radiation, etc.) in the other.

A distinctive feature of our system is its capability to simultaneously evaluate both the physical characteristics of aerosol particles and the biological activity of bioaerosols. By combining real-time particle counter monitoring with SEM-EDS analysis of particle morphology and composition, we can comprehensively characterize the properties of particles acting as microbial carriers. This approach has enabled novel insights into size-dependent effects of disinfectants and environmental stresses on airborne microbial survival strategies.

The system's unique infrastructure allows for segregation and size-specific analysis of particles and bioaerosols, making it a crucial platform for studying atmospheric microorganisms. We have validated the system through experiments with various environmental microorganisms, demonstrating its effectiveness in maintaining stable experimental conditions while enabling precise measurements of both biological and physical parameters.

Current research utilizing this facility focuses on understanding the transport processes of airborne microorganisms and their interactions with atmospheric components. The findings are expected to contribute significantly to our understanding of microbial transport processes and global biogeochemical cycles.

How to cite: Maruyama, F. and Fujiyoshi, S.:  Development of a Dual-Chamber Atmospheric Simulation System for Bioaerosol Research: Size-Dependent Analysis and Surface Interaction Studies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1931, https://doi.org/10.5194/egusphere-egu25-1931, 2025.

Atmospheric microorganisms play a crucial role in cloud formation and climate processes, yet understanding their spatial and temporal dynamics remains a significant challenge. To advance our knowledge of atmospheric microbial ecology and transport processes, our research team initiated a multi-dimensional study in 2023 that examines the complex interactions between airborne microorganisms and their atmospheric environment. The study encompasses five integrated components: continuous real-time bioaerosol monitoring coupled with meteorological measurements, weekly microbiological community analysis using high-volume air samplers, monthly high-altitude microbial sampling via light aircraft at 1600 m above sea level, multi-level atmospheric monitoring using a 123-meter tower, and planned sampling in cloud-prone regions.

Our monitoring efforts revealed distinct temporal patterns in microbial abundance and distribution. While total particle concentrations showed minimal diurnal variation, biological particle counts exhibited pronounced daily fluctuations during the late summer and early autumn months (August-October), with this pattern notably absent during the winter period (November-March). Spatial analysis across monitoring sites demonstrated consistent total particle distributions but heterogeneous biological particle patterns, suggesting strong influences of local environmental factors on microbial dynamics. Community structure analysis indicated that under typical conditions, atmospheric microorganisms predominantly originated from local sources rather than long-range transport, highlighting the importance of surface-atmosphere exchange processes.

These findings contribute to our understanding of the atmosphere as a dynamic component of Earth's microbiome, where microorganisms actively participate in biological, chemical, and physical processes. Future research will focus on elucidating the mechanisms governing microbial survival and activity in the atmosphere, including their responses to environmental stressors and their potential influence on atmospheric processes.

How to cite: Fujiyoshi, S. and Maruyama, F.: Temporal and spatial dynamics of bioaerosol particles through integrated monitoring approach of local air distribution patterns, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2115, https://doi.org/10.5194/egusphere-egu25-2115, 2025.

Fungi are among the most important biota on the planet, mediating ecosystem processes and contributing to the global bioaerosol budget and pollution even when metabolically inactive. Despite this, diversity and transport of fungi in the atmosphere are poorly explored. Here I show that the atmosphere contains diverse fungi with varied ecological roles and recruitment reflecting underlying habitats. The atmospheric mycobiome is dominated by decomposers and pathogens; over 40% of the total airborne mycobiota are known pathogens of plants or animals, including humans, with the capacity to transfer antibiotic resistance genes. Using aircraft surveys between 2022-2023 and unprecedented comprehensive environmental datasets, I found that remote sensing and meteorological data can predict diversity of fungi comprising the rare/transient portion of the atmospheric mycobiome. Vegetative decay/turnover is linked to increased fungal richness in the atmosphere, strengthening the view that phenology is a major determinant of atmospheric biodiversity. Additionally, ecological selection and niche effects can shape vertical assembly of the atmospheric mycobiome. Forward trajectory models predict air masses carrying the sampled fungi will reach Africa, Europe, and Asia as far as east as Kazakhstan, with global impacts and long-range transport beyond 11,000-km possible. This work sheds light on how genomic and environmental datasets acquired by aircraft and satellites can be used for multipronged data forecasts and dispersal predictions to allow proactive measures, clarify aerobiology questions, and provide a unified view of fungal ecology for planetary protection.

How to cite: Metris, K.: Fungus above us: Eco-environmental drivers of fungal diversity and transport in the atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2599, https://doi.org/10.5194/egusphere-egu25-2599, 2025.

EGU25-3895 | ECS | PICO | AS4.17

Impact of Yellow Dust Event on PM2.5 Microbial Communities during Spring in Ulaanbaatar, Mongolia 

Ian Cho, Sookyung Kang, Amgalan Natsagdorj, Jiyi Lee, and Kyung-Suk Cho

The Ulaanbaatar region in Mongolia exhibits a characteristic increase in particulate matter (PM) concentrations during spring, due to yellow dust events. This phenomenon has emerged as a significant air pollution issue across Asia. Among air pollution indicators, PM2.5 has substantial impacts on human health and plays a crucial role in microbial community structures and ecological interactions. This study investigated the characteristics of PM2.5 microbial communities during spring, including a yellow dust event, in Ulaanbaatar, Mongolia. The bacterial and fungal metagenomes of PM2.5 samples collected in Ulaanbaatar over a week from April 6 to April 12, 2022 were analyzed. DNA was extracted from PM2.5 filters, and bacterial 16S rRNA gene regions were amplified using 515F/806R primers. For fungi, ITS2 gene regions were amplified using ITS3/ITS4 primers. Subsequently, sequence analysis was performed using Illumina MiSeq. The study examined the impact of air pollutants (NOx, NO) and meteorological factors (relative humidity (RH), temperature) on microbial diversity indices (Chao1, Shannon) and the characteristics of dominant species during the investigation period. Based on the sequencing results, the relative abundance of bacteria and fungi in PM2.5 at the genus level was assessed, and changes in microbial abundance before and after the yellow dust event were compared using a heatmap. Additionally, Spearman correlation analysis was conducted to explore the relationships between the Top 5 dominant bacterial and fungal species on the yellow dust event day and the air pollutants as well as meteorological factors. The results indicated that the diversity indices of bacterial and fungal communities during spring tended to be higher with increasing concentrations of air pollutants and temperature; however, higher RH was associated with lower diversity indices. Changes in dominant microorganisms throughout the study period were confirmed through heatmap analysis, revealing that the composition of dominant microorganisms altered before and after the yellow dust event. On the yellow dust day, the Top 5 dominant bacterial genera were identified as Nitrososphaera, Arthrobacter, Nocardioides, Sphingomonas, and Chthoniobacter, while the Top 5 dominant fungal genera were Trichosporon, Cladosporium, Ascochyta, Alternaria and Vishniacozyma. On the event day, the dominant bacterial genera exhibited positive correlations with PM10 concentrations and temperature, while showing negative correlations with RH. Most of these genera are typically found in soil environments and are known to survive in arid conditions. In the case of fungi, the Top 5 fungal species on the yellow dust day, except for Trichosporon, also showed negative correlations with RH. This study may serve as fundamental data for future management strategies of PM2.5 air quality.

How to cite: Cho, I., Kang, S., Natsagdorj, A., Lee, J., and Cho, K.-S.: Impact of Yellow Dust Event on PM2.5 Microbial Communities during Spring in Ulaanbaatar, Mongolia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3895, https://doi.org/10.5194/egusphere-egu25-3895, 2025.

EGU25-6447 | ECS | PICO | AS4.17

Photoheterotrophy provides increased fitness in airborne bacteria: Aerosol simulation chamber studies 

Frédéric Mathonat, Federico Mazzei, Marie Prévot, Virginia Vernocchi, Elena Gatta, Muriel Joly, Mariline Théveniot, Barbara Ervens, and Pierre Amato

The atmosphere harbors a great diversity of microorganisms. Among them, some taxa of bacteria, such as Methylobacterium species are abundant and recurring members of the viable fraction (Amato et al., 2017; Woo and Yamamoto, 2020). These include non-obligate light-users, and we postulate that this function could be linked with their prevalence and survival capacity in the atmosphere. The alternative use of light to generate biochemical energy (ATP) through photoheterotrophy and anoxygenic photosynthesis is known to enhance survival under nutrient-deficient conditions (Soora and Cypionka, 2013). The use of light could therefore be beneficial and favor survival by supporting the maintenance of metabolic activity in the atmospheric environment,  with dispersed droplets or particles where access to substrates is limited.

To test the hypothesis that photoheterotrophy is beneficial to the survival of airborne bacteria, two distinct phenotypes of the same strain (with or without the photosynthetic pigment bacteriochlorophyll; [BChl+] or [BChl-], respectively, which can be controlled by growing cells under dark or light conditions, respectively) of a facultative photoheterotrophic strain of Methylobacterium sp. (R17b-9), isolated from clouds, were injected into the atmospheric simulation chamber (ASC) "ChAMBRe" (Vernocchi et al., 2023). Their survival was monitored for 2 hours while being exposed to different light intensities. During experimentation in the ASC, cell viability, cultivability, ATP concentration and residence time were measured.

Bacteria containing bacteriochlorophyll retained greater viability and cultivability than those lacking this photosynthetic pigment.  Light exposure on [BChl-] phenotype had a negative impact on cultivability, but not on viability. The mean half-lives (measuring by cultures) of bacteria [BChl-] was ~100-700 min depending on light intensity whereas there was no loss of cultivability over time for bacteria with pigment independently from light exposure. The ATP/cell ratio was 3 times greater for bacteria with bacteriochlorophyll than without. In addition, bacteria with bacteriochlorophyll sedimented 1.71 times faster than their counterparts without the pigment. This study supports the idea that not all bacteria are equal to atmospheric transport, and that specific phenotypic traits can be involved. It is possible that the widespread distribution, at low level, of photoheterotrophy in bacteria in the global environment could be promoted by their increased ability to disperse aerially.

 

Reference

Amato, P., Joly, M., Besaury, L., Oudart, A., Taib, N., Moné, A. I., Deguillaume, L., Delort, A.-M., and Debroas, D.: Active microorganisms thrive among extremely diverse communities in cloud water, PLOS ONE, 12, e0182869, https://doi.org/10.1371/journal.pone.0182869, 2017.

Soora, M. and Cypionka, H.: Light Enhances Survival of Dinoroseobacter shibae during Long-Term Starvation, PLOS ONE, 8, e83960, https://doi.org/10.1371/journal.pone.0083960, 2013.

Vernocchi, V., Abd El, E., Brunoldi, M., Danelli, S. G., Gatta, E., Isolabella, T., Mazzei, F., Parodi, F., Prati, P., and Massabò, D.: Airborne bacteria viability and air quality: a protocol to quantitatively investigate the possible correlation by an atmospheric simulation chamber, Atmospheric Measurement Techniques, 16, 5479–5493, https://doi.org/10.5194/amt-16-5479-2023, 2023.

Woo, C. and Yamamoto, N.: Falling bacterial communities from the atmosphere, Environmental Microbiome, 15, 22, https://doi.org/10.1186/s40793-020-00369-4, 2020.

How to cite: Mathonat, F., Mazzei, F., Prévot, M., Vernocchi, V., Gatta, E., Joly, M., Théveniot, M., Ervens, B., and Amato, P.: Photoheterotrophy provides increased fitness in airborne bacteria: Aerosol simulation chamber studies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6447, https://doi.org/10.5194/egusphere-egu25-6447, 2025.

EGU25-7510 | PICO | AS4.17

Preliminary study of Microbiology in Clouds at Whiteface Mountain in New York 

Sara Lombardo, Archana Tripathy, Sridar V Chittur, Diana Gentry, Andrew Hayden, Marcy L Kuentzel, Paul W Casson, Rudra Patel, Lily Hammond, and Sara Lance

Whiteface Mountain (WFM) in northern NY State is the site of a historic mountaintop atmospheric observatory with an ongoing cloud water chemistry monitoring program that has been operating every summer (June through September) since 1994. Though long-term chemical analysis has been conducted, no analysis on the microbiome has been completed at WFM. Over the years, a new chemical regime has been reported in the cloudwater with missing analytes. Knowing how microbes can interact with chemicals, we hypothesize microbes are partially responsible for this shift and are crucial in understanding the chemical background of clouds.

To start this study, cloudwater filters have been analyzed both chemically and microbially. Chemically, weighted averages have been calculated for each cloudwater filter based on the chemical composition of the clouds. Microbially, we have begun DNA extractions and subsequent metagenomic analysis using the Oxford Nanopore MinION using a select number of cloud water filters from 2024. Overall, this study aims to build upon microbial work accomplished by the Puy de Dôme groups and discuss the collection, storage, and analysis of cloudwater filters to connect the chemical to the microbial at WFM.

How to cite: Lombardo, S., Tripathy, A., Chittur, S. V., Gentry, D., Hayden, A., Kuentzel, M. L., Casson, P. W., Patel, R., Hammond, L., and Lance, S.: Preliminary study of Microbiology in Clouds at Whiteface Mountain in New York, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7510, https://doi.org/10.5194/egusphere-egu25-7510, 2025.

EGU25-11035 | ECS | PICO | AS4.17

In-depth analysis of the origin of Primary Biological Aerosol Particles in a temperate forest of Leipzig 

Bhavana Valath Bhuan Das, Martina Herrmann, Beate Michalzik, Susanne Dunker, and Beatriz Sánchez-Parra

Primary Biological Aerosols (PBAPs) or bioaerosols are airborne particles originating from biological sources that are directly emitted from the biosphere into the atmosphere. These include bacteria, archaea, viruses, pollen, fungal spores, and fragments of plants and animals (Després, 2012) PBAPs play a significant role in atmospheric processes, climate regulation, and human health, making it essential to investigate their sources, composition, and emission mechanisms.

Bioaerosols can be transported over short or long distances, influenced by factors such as atmospheric turbulence, and environmental conditions (Fröhlich-Nowoisky, 2016) However, the mixing of locally emitted particles with those transported over long distances complicates the accurate identification of their emission sources. This challenge hinders our ability to fully understand their real influence on the atmosphere and ecosystem of origin.

To better elucidate the exchange of particles between these interconnected systems, in this study we investigated the plant and soil litter composition of a temperate floodplain forest thanks to the Leipzig Canopy Crane facility, located in the Leipzig Auwald, along with the dynamics of bioparticles in the air between the spring and autumn seasons.

Relevant data were obtained through sequencing the samples. By comparing the sequences with their potential sources, we obtained temporal and source-specific variations in the bioaerosol community structure across the different months. In Bacteria there is an increase in the overall diversity from spring to autumn, similar seasonal variation is observed in the fungal population. Ascomycota, one of the more dominant groups in the microbial community, varies in abundance with seasonal shifts, being consistently more abundant in the air samples when compared to Basidiomycota which are more prevalent in source communities, likely contributed by their individual dispersion properties.

 

References-

  • Després, V. R., Huffman, J., et al. (2012). Primary biological aerosol particles in the atmosphere: A review. Tellus B: Chemical and Physical Meteorology, 64(0), 15598. https://doi.org/10.3402/tellusb.v64i0.15598
  • Fröhlich-Nowoisky, J., et al. (2016). Bioaerosols in the Earth system: Climate, health, and ecosystem interactions. Atmospheric Research, 182, 346–376. https://doi.org/10.1016/j.atmosres.2016.07.018

How to cite: Valath Bhuan Das, B., Herrmann, M., Michalzik, B., Dunker, S., and Sánchez-Parra, B.: In-depth analysis of the origin of Primary Biological Aerosol Particles in a temperate forest of Leipzig, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11035, https://doi.org/10.5194/egusphere-egu25-11035, 2025.

EGU25-13349 | PICO | AS4.17

Airborne microalgae: investigating their aerosolization potential and gaseous emissions 

Bernadette Rosati, Jane Tygesen Skønager, Marat Bektassov, Merete Bilde, Marta Barbato, Kasper Vita Kristensen, and Sylvie V.M. Tesson

Atmospheric aerosols influence the Earth’s radiation balance and play a significant role in cloud formation, as well as air quality. Among biological aerosols, there is a clear lack of understanding the impact airborne microalgae have on climate.  To date, most studies have focussed on the associated health and environmental effects when microalgae disperse to new environments; their interactions with sunlight and potential role in cloud seeding have so far been largely neglected.

In this work, we performed detailed laboratory measurements to mimic the potential release of microalgae from the oceans into the atmosphere.  For this purpose, we utilized a sea spray simulation chamber with a plunging jet. We selected microalgae strains from saltwater and freshwater environments that have previously been found to be important for the release of dimethyl sulphide, a compound that is imperative for new particle formation in the atmosphere in marine regions. We focussed on the investigation of the emission of the microalgae themselves and volatile organic compounds (VOCs) that are simultaneously released. Aerosol particle concentrations and size distributions were tracked online by using an aerosol size spectrometer; additionally, the emitted particles were sampled with an impinger and counted using microscopy. A proton-transfer-reaction mass spectrometer continuously measured the VOCs, which were also periodically sampled with Tenex sorbent tubes and analysed using mass spectrometry. Furthermore, we analysed whether microalgae viability was affected by the water-air transfer.

How to cite: Rosati, B., Skønager, J. T., Bektassov, M., Bilde, M., Barbato, M., Kristensen, K. V., and Tesson, S. V. M.: Airborne microalgae: investigating their aerosolization potential and gaseous emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13349, https://doi.org/10.5194/egusphere-egu25-13349, 2025.

EGU25-15888 | PICO | AS4.17

Lipidome of Saharan dust aerosols 

Kalliopi Violaki, Christos Panagiotopoulos, Pierre Rossi, Ernest Abboud, Maria Kanakidou, Nikolaos Evangeliou, Christine Groot Zwaaftink, and Athanasios Nenes

Lipidomics, a subfield of metabolomics, is an emerging field where hundreds to thousands of lipid species are simultaneously identified. Given the ubiquity and diverse biological roles of lipids, lipidomics offers valuable insights into mechanisms and the discovery of biomarkers related to environmental stressors that affect the cellular physiology and their numerous biochemical pathways. The major source of lipids in the atmosphere are the biogenic particles (bioaerosols) e.g., bacteria, fungi, pollen, plant fragments and viruses. Specifically, the terrestrial ecosystems including deserts, are the major sources of the atmospheric bioaerosols with urban environments and areas with agricultural and industrial activity being particularly important. The desert dust aerosols contain high concentrations of bioaerosols mainly composed of soil microorganisms and plant detritus. Agricultural dust can contain significantly more amounts of biological material, which subsequently can be enriched with additional biogenic particles when they are transported across terrestrial and aquatic environment through their coagulation with other airborne bioaerosols. The lipidome of airborne biogenic particles is unexplored to date, yet it can provide unique insights on bioaerosols, their stress state and oxidant exposure history. During this study we used lipidomics as a novel tool for the atmospheric research, to study the lipid changes in bioaerosols systems induced by their exposure to air pollutants and other atmospheric aging factors.

To achieve this, Saharan dust aerosols (n= 15) were sampled from East Mediterranean (Crete, Greece) using a high-volume (85 m3 h−1) TSPs sampler (TISCH). Dust atmospheric particles were collected on precombusted (450 °C for 5 h) 20 × 25 cm quartz filters (Pall, 2500QAT-UP). A reliable analytical protocol was established for lipidomics analysis of Saharan dust aerosols, which allowed us to identify approximately 60 lipid species, primarily phosphatidylcholines (PC), phosphatidylethanolamines (PE), triglycerides (TG), and their oxidation products, ceramides (Cer), and monogalactosyldiacylglycerols (MGDG). In addition to lipid analysis, biological identification and chemical analysis, including metals, major ions, and sugars, was also performed and will be discussed in detail.

Each dust event has a distinct signature, reflecting not only the chemical composition of the Saharan soil but also the atmospheric processing during its long-range transport. Preliminary results indicate a higher percentage contribution from the oxidation products of TG (OxTG, 33%) and PCs (OxPC, 22%) to the total identified lipids. The significant correlation between PCs and mannitol indicates a fungal contribution to airborne cholines. Furthermore, the correlation between anthropogenic metals (e.g., V, Ni, As, Cr, Pb) and galactolipids (MGDG), which are common plant membrane lipids, indicates a complex mixture of anthropogenic emissions and plant material in the dust aerosols due to long range transport of Saharan soil.

 

How to cite: Violaki, K., Panagiotopoulos, C., Rossi, P., Abboud, E., Kanakidou, M., Evangeliou, N., Groot Zwaaftink, C., and Nenes, A.: Lipidome of Saharan dust aerosols, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15888, https://doi.org/10.5194/egusphere-egu25-15888, 2025.

EGU25-16671 | ECS | PICO | AS4.17

Isolation and characterization of potentially pathogenic bacteria from mountainous regions in France 

Masoumeh Kashiri, Athanasios Zervas, Florian H. H. Brill, Jörg Steinmann, and Alexandre M. Anesio

Introduction:

High-altitude snowy regions are recognized as unique biomes hosting diverse microbial communities. Microorganisms in these environments have evolved adaptations to survive extreme conditions, such as low temperatures, high UV radiation, and limited nutrient availability. These adaptations may include antibiotic resistance and virulence factors, which could pose ecological and public health risks if transferred to human pathogens or clinically relevant ecosystems. 

This study aimed to isolate and identify bacterial strains from these environments, assess their temperature tolerance, hemolytic activity, and potential antibiotic resistance profiles and to investigate the presence of antibiotic resistance genes (ARGs) and their potential public health risks.

 

Methods:

Snow samples were collected from Chamrousse Ski Resort (Grenoble, France) and cultivated on R2A agar at 4°C, 15°C, and 37°C, with morphologically distinct colonies isolated and purified. Growth was monitored over 7 days at 4°C, 15°C, 25°C, and 37°C by measuring OD600 at 24-hour intervals to assess temperature tolerance. Hemolytic activity was evaluated on sheep and horse blood agar plates incubated at 15°C, 25°C, and 37°C, with patterns of alpha, beta, or gamma hemolysis recorded. Genomic DNA was extracted, and 16S rRNA sequencing was used to identify the isolates at the species level. Whole genome sequencing was conducted using the Oxford Nanopore method, and antibiotic resistance genes (ARGs) were identified via the CARD database. Minimum inhibitory concentration (MIC) testing is planned as a follow-up to validate resistance profiles and assess the functional expression of the identified ARGs.

 

Results:

Sanger sequencing of the 16S rRNA gene identified Peribacillus simplex for isolates 1, 2, and 3, and Sphingomonas faeni for isolate 4, with 100% sequence homology. Growth monitoring revealed that Peribacillus isolates grew best at 25°C, with Peribacillus 1 showing moderate growth at 37°C, while Sphingomonas exhibited psychrotolerant traits, thriving at 15°C and 25°C but performing poorly at other temperatures. Hemolytic activity tests showed that Peribacillus 1 exhibited alpha hemolysis on both sheep and horse blood agar, whereas Peribacillus 2 and 3 showed gamma hemolysis, and Sphingomonas did not grow on blood agar. Whole genome sequencing identified several antibiotic resistance genes (ARGs) linked to multidrug resistance and virulence, including blaZ and vanY in Peribacillus spp., and acrB and mexA in Sphingomonas spp.

 

Conclusion:

This study highlights the adaptability of microbial communities in snowy alpine environments to changing climates and their potential to spread ARGs and hemolytic features into ecosystems. The presence of such traits in these microorganisms underscores their possible role as reservoirs of antibiotic resistance and virulence factors in natural habitats. Further studies, including MIC testing and pathogenicity assessments, are crucial to fully understanding the ecological and public health implications of these findings.

How to cite: Kashiri, M., Zervas, A., H. H. Brill, F., Steinmann, J., and M. Anesio, A.: Isolation and characterization of potentially pathogenic bacteria from mountainous regions in France, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16671, https://doi.org/10.5194/egusphere-egu25-16671, 2025.

EGU25-17716 | PICO | AS4.17

Microorganisms in the air through the lenses of atmospheric chemistry and microphysics  

Barbara Ervens, Pierre Amato, Kifle Aregahegn, Muriel Joly, Amina Khaled, Tiphaine Labed-Veydert, Frederic Mathonat, Leslie Nuñez-López, Raphaelle Peguilhan, and Minghui Zhang

Microorganisms in the atmosphere comprise a tiny fraction (~10-8%) of the Earth’s microbiome. A significant portion of this ‘aeromicrobiome’ consists of bacteria that typically remain airborne for a few days before being returned to the ground through wet or dry deposition. Unlike bacteria in the other Earth surface spheres (e.g., litho-, hydro-, phyllo-, cryospheres), atmospheric bacteria are aerosolized, residing in individual particles and separated by considerable distances (a few centimeters) from each other. Within these small isolated microcosms, bacteria are exposed to particular chemical and physical conditions that potentially affect their stress levels, survival and general functioning. Using fundamental chemical and microphysical concepts of atmospheric aerosol particles and cloud droplets, we examine these specific environmental conditions. In particular, we challenge the concept of clouds as microbial oases by illustrating the water amounts and time scales inside clouds. In addition, we suggest that the small volumes of cloud droplets may cause greater nutrient limitations but simultaneously reduce oxidative stress compared to other aquatic environments. Various chemical and microphysical factors may act as microbial stressors (e.g., oxidative, osmotic, and UV-induced) in the atmosphere, which may either enhance or diminish the survival and diversity of atmospheric bacteria. Based on established atmospheric chemical and microphysical principles, we discuss that observed trends of bacterial community properties and pollutant concentrations may lead to incorrect interpretations due to confounding factors. In summary, our presentation aims to motivate future experimental and modeling studies to disentangle the complex interplay of chemical and microphysical factors with the atmospheric microbiome. Such studies are important to eventually allow for a comprehensive understanding of the atmosphere’s role in affecting airborne microorganisms, a small yet rapidly evolving component of the Earth’s microbiome.

 

Ervens, B., Amato, P., Aregahegn, K., Joly, M., Khaled, A., Labed-Veydert, T., Mathonat, F., Nuñez López, L., Péguilhan, R., and Zhang, M.: Ideas and perspectives: Microorganisms in the air through the lenses of atmospheric chemistry and microphysics, Biogeosciences, 22, 243–256, https://doi.org/10.5194/bg-22-243-2025, 2025.

How to cite: Ervens, B., Amato, P., Aregahegn, K., Joly, M., Khaled, A., Labed-Veydert, T., Mathonat, F., Nuñez-López, L., Peguilhan, R., and Zhang, M.: Microorganisms in the air through the lenses of atmospheric chemistry and microphysics , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17716, https://doi.org/10.5194/egusphere-egu25-17716, 2025.

EGU25-18147 | PICO | AS4.17

Characterization of the Atmospheric Microbiome in a Semi-Rural Area of Central Europe Using Flow Cytometry 

Ernest Abboud, Pierre Rossi, Benoit Crouzy, Athanasios Nenes, and Kalliopi Violaki

The abundance, characterization, and identification of biological aerosol particles (bioaerosols) are important for understanding their impact on the Earth system in terms of biogeochemical cycles of phosphorus and nitrogen, cloud formation, precipitation, and human health. Bioaerosols consist of all airborne prokaryotes or eukaryotes ranging in size from a few nanometers to hundreds of micrometers.

In this study, a flow cytometry protocol was optimized in order to quantify and characterize the biogenic particles collected from a semi-rural site in central Europe (Payern, Switzerland). Samples collection (n = 39) was performed using a high-volume wet-cyclone over a period of 5 months (April to August 2024). Specifically, a live/dead protocol for atmospheric samples was optimized using two nucleic acid stains: Syto13 to stain all live cells and propidium iodide to stain all dead cells. The simultaneous use of the dyes and the subsequent application of an automated clustering algorithm after acquisition (FlowSOM, Bioconductor - FlowSOM) allowed us to identify populations characterized by a high nucleic acid (HNA) content (e.g., fungal spores and protists) and a low nucleic acid (LNA) content (e.g., bacterial cells and dead protists).

Preliminary results showed that the average concentration of bioaerosols was 2.25x104 ± 2.99x104 microorganisms m-3. The HNA population was dominant during the sampling period (detected in 79% of the samples) while the LNA population dominated the bioaerosols fraction on rainy days. The intact population dominated the bioaerosol fraction (92.6 ± 12.3%) compared to the dead population (7.4 ± 12.3%). A significant high correlation was found between the LNA and the dead populations (rspearman = 0.88), indicating that the dead population is a component of the LNA population (rspearman = 0.50 with the HNA population).

The populations quantified by flow cytometry will be identified taxonomically using Oxford Nanopore sequencing. The results will be discussed in detail.

How to cite: Abboud, E., Rossi, P., Crouzy, B., Nenes, A., and Violaki, K.: Characterization of the Atmospheric Microbiome in a Semi-Rural Area of Central Europe Using Flow Cytometry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18147, https://doi.org/10.5194/egusphere-egu25-18147, 2025.

EGU25-18628 | PICO | AS4.17

Microorganisms from North African deserts persist in Southern Europe’s atmosphere 

Joan Cáliz, Mateu Menéndez-Serra, Xavier Triadó-Margarit, Anna Avila, and Emilio O. Casamayor

Long-range atmospheric processes facilitate global dispersal of microorganisms, with significant implications for Earth’s ecosystems functioning and global health. While traditional aerobiological studies have focused on low troposphere aerosols, assuming airborne communities are primarily influenced by neighbouring ecosystems, our study challenges this perspective. We analysed nearly three decades of aerosol particles present in rainwater samples collected at a mountain site located in South Europe (Iberian Peninsula, NE Spain). Coupling this data with analyses of high troposphere air mass provenances and genetic data of topsoils from North Africa and from a global public bacterial database, we revel a persistent influence of desert microorganisms from North Africa in Southern European sky. Remarkably, desert-derived microorganisms dominate even in rain originating from the Atlantic Ocean, despite sea spray being the largest source of global aerosols. The frequency of dust outbreaks, altitude reached, and long residence times of fine-sized particulates are postulated as critical factors that significantly shape the long-range and persistence of aerial assemblages, while air mass provenance playing a secondary role. Our findings highlight the profound and long-lasting impact of desert aerosols on terrestrial ecosystems, calling for further exploration of intercontinental aerial connections with deserts and drylands elsewhere, and the ecological implications of desert immigrants on worldwide ecosystems.

How to cite: Cáliz, J., Menéndez-Serra, M., Triadó-Margarit, X., Avila, A., and O. Casamayor, E.: Microorganisms from North African deserts persist in Southern Europe’s atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18628, https://doi.org/10.5194/egusphere-egu25-18628, 2025.

EGU25-18717 | ECS | PICO | AS4.17

Temporal Dynamics of Atmospheric Microbial Communities in the Alps: Insights from 11-Years of High-Altitude Sampling 

Marie Labat Saint Vincent, Patrik Winiger, Julian Weng, Stephan C. Schuster, Christoph Hueglin, Sophie Darfeuil, Pauline Bros-Rolere, Patrick Ginot, Claudia Mohr, Jean-Luc Jaffrezo, Imad El-Haddad, Aurélien Dommergue, and Catherine Larose

Temporal Dynamics of Atmospheric Microbial Communities in the Alps: Insights from 11-Years of High-Altitude Sampling

Marie Labat Saint Vincent1; Patrik Winiger2; Julian Weng2; Stephan C. Schuster3; Christoph Hueglin4; Sophie Darfeuil1; Pauline Bros-Rolere1; Patrick Ginot1; Claudia Mohr2,5; Jean-Luc Jaffrezo1; Imad El-Haddad2; Aurélien Dommergue1; Catherine Larose1

1: Institut des Géosciences de l’Environnement (IGE) CNRS, UGA, IRD, INRAE, Grenoble INP, 38058, Grenoble CEDEX, France

2 : PSI Center for Energy and Environmental Sciences (PSI-CEES), Paul Scherrer Institute, Villigen, 5232, Switzerland

3 : Singapore Centre for Environmental Life Sciences Engineering (SCELSE), Nanyang Technological University Singapore, Singapore, Singapore

4 : Swiss Federal Laboratories for Materials Science and Technology (EMPA), Dübendorf, 8600, Switzerland

5 : Department of Environmental Systems Science, ETH Zurich, 8092 Zürich, Switzerland

 

Atmospheric microbial communities play a significant role in biogeochemical cycles and serve as a key source of microorganisms deposited onto glacial surfaces, where they may be preserved for millennia. Understanding the dynamics of these communities and their responses to environmental factors is critical for assessing their transfer and preservation in glacial archives. In this study, we leverage a unique dataset collected by the Swiss National Air Pollution Monitoring Network (NABEL), consisting of 11 years (2010–2021) of atmospheric particulate samples from Jungfraujoch (3500m a.s.l., Switzerland). This sampling site provides a rare opportunity to unravel atmospheric microbial community dynamics at high altitude as well as providing information on the pool of microorganisms that can potentially be deposited onto glaciers in the Alps.

DNA extraction and quantitative PCR (qPCR) were performed on atmospheric filters collected every four days (>1000 samples) to quantify microbial abundance. These data allow us to investigate the temporal trends in abundance in the Alpine atmosphere over more than a decade, highlighting seasonal variations over time. Additionally, correlations with geo-physico-chemical environmental parameters, like temperature, pollution events, and atmospheric composition, were carried out to identify key factors driving these dynamics.

This time series represents one of the most comprehensive temporal datasets of atmospheric microbial dynamics at high altitude available. In addition to providing a unique opportunity to characterize the drivers of microbial communities in the atmosphere over longer time scales, this data also represents an important step towards understanding the processes governing microbial deposition and preservation in Alpine ice. This work lays the foundation to the broader goal of validating ice cores as reliable archives of past atmospheric microbial diversity and environmental conditions.

How to cite: Labat Saint Vincent, M., Winiger, P., Weng, J., Schuster, S. C., Hueglin, C., Darfeuil, S., Bros-Rolere, P., Ginot, P., Mohr, C., Jaffrezo, J.-L., El-Haddad, I., Dommergue, A., and Larose, C.: Temporal Dynamics of Atmospheric Microbial Communities in the Alps: Insights from 11-Years of High-Altitude Sampling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18717, https://doi.org/10.5194/egusphere-egu25-18717, 2025.

EGU25-19389 | PICO | AS4.17

Metabolic activity and inaZ gene expression during atmospheric dispersal of plant pathogen Pseudomonas syringae  

Tina Šantl-Temkiv, Corina Wieber, María Palomeque Sánchez, Anton Legin, Arno Schintlmeister, Stefanie Imminger, Sigurd Christiansen, Meilee Ling, Augusta Kjelstrup Isaksen, Merete Bilde, Thomas Boesen, Dagmar Woebken, Bernadette Rosati, and Kai Finster

Pseudomonas syringae is a common plant pathogen, posing significant threats to the global crop production. By producing ice-nucleating proteins (INpro), encoded by the inaZ gene, cells can inflict frost injuries to plants, gaining access to nutrient-rich plant tissue. Furthermore, P. syringae can impact cloud formation and interfere with atmospheric chemistry through their metabolic and ice-nucleation activity. Both metabolic activity and inaZ gene expression under atmospheric conditions remain poorly understood, limiting our ability to accurately predict the atmospheric impact and dispersal success of P. syringae.

 

Our fist aim was to investigate the metabolic activity of P. syringae at simulated atmospheric conditions. We exposed single cells placed on polycarbonate filters to RH 94-100% in presence of D2O. We used the incorporation of deuterium as an activity marker detected via nanoscale secondary ion mass spectrometry (NanoSIMS). Cells exhibited metabolic activity when liquid water was available (RH 100%) without the addition of carbon sources, suggesting that P. syringae can maintain activity based on storage compounds. While we observed a significant decrease in deuterium incoorporation when water was supplied through the vapor phase (<100% RH), likely due to reduced viability, a fraction of cells remained metabolically active at 97% and 94% RH. Interestingly, we observed deuterium incorporation in non-viable cells, likely because of residual enzymatic activity. Such residual enzymatic activity in dead airborne cells may have unknown impacts on atmospheric chemistry, which remain to be determined. Altogether, the results suggest that metabolic activity is possible both in cloud droplets and in dry atmosphere based on storage compounds available in cells, which could support cells in actively modifying their surface properties, by e.g. synthesizing novel INpro while airborne.

 

Our second aim was to investigate the effect of aerosolization on the inaZ gene expression in P. syringae. Using bubble-bursting aerosolization combined with immunofluorescence staining we found a significantly larger proportion of INpro-bearing cells in the aerosolized fraction (33.2%) compared to pre-aerosolization (10.7%). Using microbial adhesion to hydrocarbon test in combination with a droplet-freezing assay to quantify INpro-bearing cells, we found that cell surface hydrophobicity did not vary between INpro-bearing and other cells, suggesting that our observation was not linked to preferential aerosolization of INpro-bearing cells. Finally, we assessed the relation between cell viability and the number of INpro-bearing cells, to decipher whether INpro synthesis is triggered in aerosolized cells. Here, cells were aerosolized using a Sparging Liquid Aerosol Generator into a flow tube at varying RH and were recollected using different methods which both affected cell viability. Viability was determined by live/dead staining and flow cytometry. We found that the increase in INpro-bearing cell fraction after aerosolization, as determined via the droplet-freezing assay, correlated with the fraction of viable cells, suggesting that a stress response triggered inaZ gene expression leading to the synthesis of novel INpro.

 

Overall, we demonstrated that metabolic activity and inaZ gene expression is feasible in airborne P. syringae and leads to a significant increase in INpro-bearing cells. These processes may have profound impacts on cloud formation,  atmospheric chemistry, and the dispersal success of P. syringae.

How to cite: Šantl-Temkiv, T., Wieber, C., Sánchez, M. P., Legin, A., Schintlmeister, A., Imminger, S., Christiansen, S., Ling, M., Isaksen, A. K., Bilde, M., Boesen, T., Woebken, D., Rosati, B., and Finster, K.: Metabolic activity and inaZ gene expression during atmospheric dispersal of plant pathogen Pseudomonas syringae , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19389, https://doi.org/10.5194/egusphere-egu25-19389, 2025.

The atmospheric dust cycle serves as a global conduit for microorganisms, with implications for environmental processes, ecosystem health, and human well-being. This study investigates the growth dynamics of dust-borne bacteria, focusing on their ability to thrive on atmospheric dust substrates, the characterization of the microbiome, their localization, and interactions. Dust samples collected from the eastern Mediterranean were cultured to identify selected bacterial with versatile metabolic capacities that are often associated with significant ecological and health impacts. We will present our findings of their growth patterns, substrate utilization, and environmental tolerance, explored under laboratory conditions. Our preliminary findings highlight the diversity of dust-borne bacterial community, their potential interactions, and their durability in different environmental conditions and anthropogenic effects.

How to cite: Lahav, E. and Lang-Yona, N.: Growth Dynamics of Dust-Borne Bacteria on Atmospheric Dust Substrates and Potential Implications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19919, https://doi.org/10.5194/egusphere-egu25-19919, 2025.

EGU25-20514 | PICO | AS4.17

Influence of climatic variables on the production and dispersion of allergenic pollen in Mexico City. 

Maria del Carmen Calderon-Ezquerro, Benjamín Martínez-López, and César Guerrero-Guerra

Climate change has diverse biological impacts on plants, significantly altering their reproductive processes. These alterations are reflected in flowering phenology and pollen production rates, which are highly sensitive to climatic variations and are frequently used as bioindicators in temperate regions.

Pollen data analysis is essential to assess the effects of climate change on plants at a regional level. Temperature emerges as a key factor influencing changes in flowering phenology, and advances in reproductive stages are increasingly linked to global warming. Likewise, water availability significantly influences plant productivity.

Global warming due to increased greenhouse gas emissions, especially CO2, is the primary driver of climate change in vast regions of our planet. Increased surface air temperatures, changes in water availability, and high atmospheric CO2 concentrations directly impact plant biology, affecting photosynthesis and thus modifying plant growth and development. Furthermore, temperature and precipitation variations related to some patterns of interannual climate variability, such as the North Atlantic Multidecadal Oscillation and El Niño-Southern Oscillation, can influence plant phenology. These changes have public health implications, as they can modify pollen production and increase the prevalence and severity of pollen-related allergic diseases.

How to cite: Calderon-Ezquerro, M. C., Martínez-López, B., and Guerrero-Guerra, C.: Influence of climatic variables on the production and dispersion of allergenic pollen in Mexico City., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20514, https://doi.org/10.5194/egusphere-egu25-20514, 2025.

EGU25-12575 | Posters on site | ITS3.20/AS4.19 | Highlight

Artificial Intelligence as  a tool for upholding human rights in disaster management: A Case Study of Wayanad landslides 

Dr Sanju v k, Dr sajikumar n l, and saina s asok

Artificial intelligence as a tool for upholding humanrights in disaster management: A case study of wayanad landslides

            Dr n l  sajikumar ,Associate Professor, Government Law College, Kerala, India

                    Dr Sanju.V.K Associate Professor, GovernmentLaw College, Kerala, India

                   saina S Asok, LL.M, Arbitration, Jindal Global Law School, Haryana, India

                            

The study is based on the report and assessment of materials collected from various sources with respect to the landslide disaster in Waynad ,Kerala, India  that occurred in 2024,wherein there were loss of human lives as well as property that resulted in huge commercial loss endangering human rights. This incident led the researchers to explore the application of artificial intelligence in detecting the possibility of such disasters and protecting the human rights of the people.

Approximately 24% of the Earth's land features uneven surfaces, which are home to around 12% of the global population. In areas characterized by such irregular landscapes, the likelihood of soil and rock mass movement, referred to as landslides, is significantly increased due to the direct effect of gravity. In this scenario the researchers intend to explore the application of Artificial Intelligence (AI) in enhancing human rights protection during disaster management, focusing on the Wayanad landslides in Kerala,, the Gods own country in India. . In India, areas like Wayanad in Kerala are prone to landslides due to their unique topography and climatic conditions. A Case Study of Wayanad Landslides natural disasters pose significant threats to human rights, particularly in vulnerable regions of the world The catastrophic landslides in Wayanad in 2024   underscored the necessity for innovative disaster management approaches that leverage technology to protect lives and uphold human rights. Artificial Intelligence (AI) has emerged as a pivotal tool in disaster management, offering predictive analytics, resource optimization, and effective response strategies. This article explores the potential of AI in enhancing disaster management practices, specifically focusing on the case of the Wayanad landslides and its implications for human rights .Disasters can severely infringe on human rights, including the right to life, health, and a safe environment. The United Nations Office for Disaster Risk Reduction emphasizes the need to integrate human rights considerations into disaster risk reduction and management strategies. In the case of Wayanad, the landslides resulted in widespread destruction of homes, displacement of communities, and loss of life, highlighting the urgent need for effective disaster preparedness and response mechanisms. In this scenario the researchers intent to introspect the need for leveraging Artificial intelligence technology to forecast landslides  for an early warning systems employing AI algorithms can significantly improve response times and enable communities to evacuate before disasters strike, thereby protecting lives and minimizing human rights violations.

Keywords-Artificial intelligence-Landslides-Waynad-Disaster management-Human Rights

How to cite: v k, D. S., n l, D. S., and s asok, S.: Artificial Intelligence as  a tool for upholding human rights in disaster management: A Case Study of Wayanad landslides, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12575, https://doi.org/10.5194/egusphere-egu25-12575, 2025.

EGU25-16460 | ECS | Posters on site | ITS3.20/AS4.19

Advanced Diagnostic and Forecast System of Icing Conditions for UAV Operational Safety 

Satyanarayana Tani, Helmut Paultisch, Robin Deutsch, Arno Fallast, Thomas Neubauer, Markus Kucera, and Reinhard Puffing

The increasing use of Unmanned Aerial Vehicles (UAVs) across various sectors underscores the necessity for thorough testing under diverse meteorological conditions to ensure operational safety and reliability. The IFIRE project, led by AIRlabs Austria in collaboration with Pegasus Research & Development GmbH, Graz University of Technology, and FH JOANNEUM, addresses this important challenge by focusing on assessing UAV performance in adverse weather conditions, particularly in relation to icing.

The primary objective of the project is to enhance aviation safety and efficiency by integrating advanced weather diagnostic and forecasting capabilities into UAV operations. A comprehensive methodology is proposed, which includes developing a sophisticated weather forecast model, machine learning approaches, conducting flight tests to collect critical data, and evaluating natural icing conditions at the Steinalpl test site in Austria. IFIRE aims to establish new safety and reliability benchmarks for UAVs by creating a state-of-the-art flight-testing area specifically designed for natural icing conditions. The multidisciplinary consortium brings together technical, regulatory, environmental, and operational expertise to address the challenges of UAV testing in icy environments. Information on the initial phase of the project and future steps will be presented.

How to cite: Tani, S., Paultisch, H., Deutsch, R., Fallast, A., Neubauer, T., Kucera, M., and Puffing, R.: Advanced Diagnostic and Forecast System of Icing Conditions for UAV Operational Safety, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16460, https://doi.org/10.5194/egusphere-egu25-16460, 2025.

EGU25-17964 | Posters on site | ITS3.20/AS4.19

City Climate Monitoring System for Zürich, Basel and Tallinn 

Heinrich Walter Denzer, Karl Grutbrod, Nico Bader, and Sebastian Schloegl

A fully automated IoT measurement network was installed in these 3 cities' urban areas (as well as in the surrounding rural areas), measuring air temperature and precipitation at typically ≥50 different locations selected according to scientific and social criteria, covering all local climate zones and points of interest, in places where the (much more costly) official WMO-standard stations can not operate due to technical restrictions. Where available, data from existing measurement systems were be integrated into the processing chain. The real-time IoT monitoring system was calibrated with local WMO-standard quality-controlled measurements,  utilised satellite data and micro-scale models developed by meteoblue,  to generate special city climate maps (e.g., heat maps which detect and visualise the urban heat island effect at the spatial resolution of 10 m, cold air flow maps, or precipitation risk maps). The real-time monitoring system and resulting maps were integrated into existing city management platforms.

Applications include using these data with a surface energy balance model to calculate possible options for climate change adaptation measures (e.g., roof greening, irrigation, de-sealing of surfaces) for urban hot-spots, to select the best adaptation strategies for parts of the city. Additionally, the effectiveness of  climate change adaptation measures in the process of being implemented can be tracked, so the economic effectiveness of the measures can be assessed, by comparing with other locations where no adjustment took place.

The combination of IoT network and Microscale modelling provides better results of modelling, cold air flow tracking and  measuring adaptation effectiveness at a significantly lower cost of implementation and operation than alternative methods.

How to cite: Denzer, H. W., Grutbrod, K., Bader, N., and Schloegl, S.: City Climate Monitoring System for Zürich, Basel and Tallinn, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17964, https://doi.org/10.5194/egusphere-egu25-17964, 2025.

This presentation shows the role of weather informatics in addressing critical societal challenges by integrating meteorological science with advanced data analytics and user-centric geospatial visualization tools. Key innovations include high-resolution weather forecasting, radar and satellite data processing, and real-time sensor network integration with robust visualization platforms designed to meet operational demands.

At the core of this approach is the Weather Image Information System (WIIS), a weather informatics platform created to process, analyse, and share extensive volumes of meteorological image data. By integrating diverse data sources—including satellite systems, ground-based radars, and real-time sensor networks—WIIS generates high-resolution imagery, enabling precise monitoring of weather patterns. This system offers interactive geospatial maps, dynamic weather animations, and customizable overlays, facilitating detailed analysis of atmospheric phenomena and enhancing real-time situational awareness.

WIIS also provides advanced decision-support capabilities, allowing users to set customizable alert thresholds for severe weather events. These features enable proactive disaster preparedness, safeguard operational continuity, and support critical infrastructure in the energy and transport sectors.

How to cite: Paulitsch, H. and Tani, S.: Advancing Weather Informatics for Meteorological Data Management and Decision Support Systems in the Energy and Transport Sectors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18359, https://doi.org/10.5194/egusphere-egu25-18359, 2025.

EGU25-922 | ECS | Posters on site | AS4.20

Meteoric 10Be as a Tracer of Chemical Weathering in Glacial Sediments 

Aaditya Nath Kapil, Jon Telling, Ana Carracedo, Vasile Ersek, and Joseph Graly

Subglacial environments are hotspots for chemical weathering with dynamic hydrological and microbial systems interacting with freshly produced meltwater and sediments. These chemical weathering processes can either drawdown or release atmospheric CO2 depending on the type and extent of weathering pathways. This study delves into chemical weathering processes in subglacial environments and their broader implications for global geochemical cycling.

We employ meteoric 10Be, a cosmogenic nuclide, to assess the neoformation of silicate weathering products as the isotope can be incorporated into the crystal structure of clays, oxides, and oxyhydroxides. This study aims to determine the extent to which chemical weathering products within glacial sediments originated during the glacial period, distinguishing them from detrital minerals derived from underlying bedrock and modern soil formed in interglacial settings. Additionally, we aim to address an observational gap in the meteoric 10Be fallout measurements in the 50° – 70° latitude and high altitude. i.e., northern Britain and Ladakh respectively, thereby enhancing our understanding of the general distribution and behaviour of the isotope.­­­­

We measured the contemporary fallout rates from the upper horizon of moraines in glacial sediments, while the inherited portion of meteoric 10Be within the lower horizons serve as archives of sub-glacial and proglacial weathering processes. Sequential extractions were performed to quantify extent of chemical weathering by isolating and measuring meteoric 10Be in three forms: adsorbed in aqueous solution, precipitated with oxides/oxyhydroxides, and/or inside the crystal structure of authigenic clay minerals. The distribution of the isotope was assessed across different grain sizes to examine its dependence on grain size and its association with various chemical and mineral species examined through ICP-MS and XRD.

This is a novel approach to identify minerals of subglacial origin in post-glacial settings. The quantification of the abundance of synglacial silicate weathering products in these glacial sediments will allow inference to a chemical weathering rate under the British Ice Sheet – a heretofore unsolved problem that offers crucial insights into the effect of glaciation on climate dynamics.

How to cite: Kapil, A. N., Telling, J., Carracedo, A., Ersek, V., and Graly, J.: Meteoric 10Be as a Tracer of Chemical Weathering in Glacial Sediments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-922, https://doi.org/10.5194/egusphere-egu25-922, 2025.

EGU25-1711 | ECS | Posters on site | AS4.20

New Opportunities for Modeling Cosmogenic Isotopes Using the Chemistry-Climate Model SOCOL  

Kseniia Golubenko, Eugene Rozanov, Melanie Baroni, and Ilya Usoskin

We present new opportunities for modeling cosmogenic isotopes using the chemistry-climate model (CCM) SOCOL, including recent advancements in the modeling of 10Be and 14C. A state-of-the-art SOCOL-AERv2 model (coupled with the CRAC production model) has been developed to simulate cosmogenic isotope atmospheric transport and deposition. The model incorporates all relevant atmospheric processes, enabling precise calculations of isotope concentrations across different locations and times. 
Validation of SOCOL-AERv2-Be against 10Be data from five Antarctic and Greenland ice cores demonstrates a reasonable agreement, capturing large-scale atmospheric dynamics while averaging synoptic-scale variability. This work reveals that most 10Be production occurs in the stratosphere, with >60% of 10Be deposited on the Earth's surface within a year. Additionally, a simplified parameterization of the full-model results is introduced, offering quick and practical estimates for polar regions. 
Extending these capabilities, the new SOCOL:14C-Ex model allows for the study of extreme solar particle events (ESPEs) beyond the Holocene based on 14C, which was previously limited by the lack of models applicable to glacial climates. Using this model we analyzed the strongest known ESPE, dated to approximately 12350 BC. This event, nearly twice as powerful as the widely studied 775 AD event, likely occurred between January and April 12350 BC, with a peak in early March. 
These developments demonstrate how advanced chemistry-climate modeling with the SOCOL framework opens new frontiers in understanding cosmogenic isotopes, solar-terrestrial interactions, and the climatic implications of extreme solar events.

How to cite: Golubenko, K., Rozanov, E., Baroni, M., and Usoskin, I.: New Opportunities for Modeling Cosmogenic Isotopes Using the Chemistry-Climate Model SOCOL , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1711, https://doi.org/10.5194/egusphere-egu25-1711, 2025.

EGU25-2277 | ECS | Orals | AS4.20

Modelling the modern oceanic cycle of beryllium-10 and beryllium-9 

Kai Deng, Gregory de Souza, and Jianghui Du

Beryllium isotopes, i.e. cosmogenic meteoric 10Be and stable 9Be, enter the oceans through distinct pathways. Beryllium-10 is produced in the atmosphere and enters the oceans mainly via precipitation, while 9Be is sourced from continents. Beryllium isotopes with a short oceanic residence time (102-103 yrs) display non-conservative behaviour in seawater. The 10Be/9Be proxy has been utilized as a powerful tool for quantifying diverse processes, including geomagnetism, sedimentation, continental input, and ocean circulation. Substantial effort has been invested in understanding external sources and internal cycling of Be isotopes in the recent decade, such as constraints on the global distribution of 10Be depositional fluxes and on riverine and benthic 9Be inputs. Hence, it offers an excellent opportunity to revisit their modern oceanic cycle. Here, we investigate the controls on the modern oceanic cycling of Be isotopes using a three-dimensional ocean biogeochemical model constrained by water-column distributions of 9Be and 10Be compiled from the literature. In addition to modelling the previously identified controls, we highlight the critical role of marine benthic fluxes and scavenging on particulate organic matter and opal in governing the mass balance and spatial distribution of Be isotopes. The transport of Be isotopes between basins by circulation is of lesser importance compared to external inputs at continent/atmosphere–ocean boundaries, except in the South Pacific. Consequently, the basin-wide 10Be/9Be ratio predominantly reflects the pattern of external inputs across most basins in the modern ocean. Based on our data-constrained oceanic model, we can further assess the sensitivity of basin-wide 10Be/9Be ratios to changes in external sources, such as continental denudation, and internal cycling, such as particle scavenging. The mechanistic understanding developed from this Be cycling model provides important insights into the various applications of marine Be isotopes, and offers additional tools to assess the individual effects of geomagnetism and environment on cosmogenic 10Be/9Be records in marine sediments.

How to cite: Deng, K., de Souza, G., and Du, J.: Modelling the modern oceanic cycle of beryllium-10 and beryllium-9, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2277, https://doi.org/10.5194/egusphere-egu25-2277, 2025.

EGU25-2464 | Orals | AS4.20

An overview of available models for simulations of the life cycle of cosmogenic isotopes 

Eugene Rozanov, Tania Egorova, Kseniia Golubenko, Mélanie Baroni, Timofei Sukhodolov, and Ilya Usoskin

Measurements of the cosmogenic isotope concentrations in the natural archives are valuable sources of information about the variability of solar activity and parameters of explosive events in the solar system and our galaxy. The retrieval and understanding of the forcing peculiarities from the data requires detailed modeling of all relevant processes. Therefore, any applied model should be able to treat the production, transport, chemical transformation, and deposition of cosmogenic isotopes and atmospheric state parameters regulating their life cycle. A hierarchy of such models ranging from simple box models to full-scale Erath system models has been developed and utilized since 1990th. This lecture will briefly present the critical turning points in model development. Then I will discuss contemporary approaches to simulate the transport, chemistry, mixing, and deposition of different cosmogenic isotopes produced by galactic cosmic rays and solar proton events and the most promising ways of further development. Special attention will be paid to the influence of volcanic eruptions and integrating 10Be modeling with other species such as 36Cl and 14C.

Acknowledgement: Support from Oulu University (Project GERACLIS #24304650) and collaborative Swiss French project AEON (grant no. 200020E_219166).

How to cite: Rozanov, E., Egorova, T., Golubenko, K., Baroni, M., Sukhodolov, T., and Usoskin, I.: An overview of available models for simulations of the life cycle of cosmogenic isotopes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2464, https://doi.org/10.5194/egusphere-egu25-2464, 2025.

EGU25-3110 | Posters on site | AS4.20

Denudation and weathering rates of carbonate landscapes from meteoric 10Be/9Be ratios 

Hella Wittmann, Julien Bouchez, Damien Calmels, Jerome Gaillardet, Daniel Frick, Karim Keddadouche, Georges Aumaitre, Fawzi Zaidi, and Friedhelm von Blanckenburg

Quantifying the rates at which carbonate rocks are denuded, the balance between chemical weathering and physical erosion, and their responsiveness to climate, vegetation, and tectonic activity is crucial for revealing feedback mechanisms in the carbon cycle and the dynamics of karst landscapes that provide vital services to humans. However, no existing method effectively partitions denudation into erosion and weathering fluxes. To estimate total denudation rates in carbonate terrains across spatial scales from soil to entire watersheds, we adapted a previously established framework that utilizes cosmogenic meteoric 10Be as an atmospheric flux tracer together with stable 9Be released during rock weathering. We employed the new method to the limestone-rich French Jura Mountains. By analyzing water, soil, sediment, travertine, and bedrock for 10Be/9Be ratios, as well as major and trace elements, stable carbon isotopes, and radiogenic strontium, we were able to quantify the contributions of beryllium from both primary and secondary carbonate phases and its release during the weathering of carbonate bedrock versus silicate impurities. We determined the partitioning of beryllium between solids and solutions and calculated rates of catchment-wide denudation (from sediment) and point source denudation (from soil), along with weathering and erosion rates. Our findings suggest that the average denudation rates range from 300 to 500 t/km2/yr, with denudation primarily driven by weathering intensity (W/D) ratios exceeding 0.92. These rates are consistent within a factor of two when compared to decadal-scale denudation rates derived from combined suspended and dissolved fluxes, underscoring the substantial potential of this method for Earth surface research in karst landscapes.

How to cite: Wittmann, H., Bouchez, J., Calmels, D., Gaillardet, J., Frick, D., Keddadouche, K., Aumaitre, G., Zaidi, F., and von Blanckenburg, F.: Denudation and weathering rates of carbonate landscapes from meteoric 10Be/9Be ratios, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3110, https://doi.org/10.5194/egusphere-egu25-3110, 2025.

EGU25-6701 | ECS | Posters on site | AS4.20

Insights on Denudation Controls of Volcanic Tropical Islands from Meteoric 10Be/9Be Ratios 

Adrien folch, Lukas Rowald, Julien Bouchez, Eric Gayer, Celine Dessert, Anne Bernhardt, and Hella Wittmann

Weathering of volcanic rocks accounts for approximately one third of global CO2 consumption in the silicate weathering cycle1. Tropical volcanic islands contribute to this process due to their extreme denudation rates, thought to be mainly driven by high and episodic precipitation, which may sustain high weathering fluxes. However, how total denudation (D) divides into erosion (E) and weathering (W) fluxes, and the factors governing their long-term rates on tropical islands remain unclear. This uncertainty arises from the lack of methods to quantify these rates over centennial to millennial timescales. Common approaches face challenges like absence of quartz for in situ-10Be or unevenly-distributed olivine for in situ-3He analysis, limited long-term observational data for gauging, and the impacts of caldera collapse and infilling of river valleys from eruptions that complicate erosion rate estimates from topographic reconstructions. The recently developed meteoric 10Be/9Be ratio that uses meteoric 10Be as an atmospheric flux tracer alongside stable 9Be released during rock weathering provides an alternative to estimate D and weathering intensity across scales, from soils to entire watersheds, independent of specific minerals.

We applied this method to Réunion and Guadeloupe, two islands with extreme precipitation regimes (respectively up to 11000 and 8000 mm/yr), steep slopes, high elevations, and warm mean annual temperatures. Both islands have catchments on lavas of similar emplacement ages (5 Kyr to 1.8 Myr), but differ mainly in lithology: Réunion's hotspot volcanism produces basalts, whereas Guadeloupe's arc volcanism generates mainly andesites. To isolate key controlling parameters, we sampled catchments with uniform lava deposition ages across varying precipitation regimes.

Preliminary results reveal a stark contrast in denudation (D). On Réunion, catchment-averaged D´s are 4000 t/km²/yr (n=11, ranging from 11 t/km²/yr in very small catchments to 15000 t/km²/yr), while Guadeloupe´s average D is 300 t/km²/yr (n=13, ranging from 100 to 1000 t/km²/yr). Weathering intensities measured on sediment from Guadeloupe are, on average, significantly higher than for Reunion. This result aligns with the observation that lower erosion rates promote more intensive soil leaching. Our denudation rates generally align well with gauging-based rates2,3and topographic reconstructions4,5,6, although the latter estimates are consistently higher by a factor of 2-5, depending on each island.

Our preliminary findings suggest that volcanic emplacement age does not control D, while the role of lithology requires further investigation. Future work will involve determining local depositional fluxes of meteoric 10Be, and analyzing additional data from weathering profiles and river sediments.

References : 1. Dessert et al., 2003; 2. Louvat et al., 1997 ; 3. Rad et al., 2006 ; 4. Salvany et al., 2012; 5. Gayer et al., 2019; 6. Samper et al., 2007.

How to cite: folch, A., Rowald, L., Bouchez, J., Gayer, E., Dessert, C., Bernhardt, A., and Wittmann, H.: Insights on Denudation Controls of Volcanic Tropical Islands from Meteoric 10Be/9Be Ratios, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6701, https://doi.org/10.5194/egusphere-egu25-6701, 2025.

EGU25-7851 | ECS | Posters on site | AS4.20

Authigenic beryllium isotopes in maar lake sediments response to climate change since the last deglaciation 

Ye Yang, Sheng Xu, Zhen-Ping Cao, and Cong-Qiang Liu

The timing, amplitude, and mechanisms of rapid climate changes since the last deglaciation remain elusive. Here we present well dated, high resolution lacustrine sediment 10Be/9Be ratio and major elements records of East Asia’s climate variability from Maar Lake Xiaolongwan, Northeast China. The abrupt increase in concentrations of Al, Ca, and Ti, considered proxies for aeolian dust flux, intriguingly coincides with a significant enhancement of the East Asian summer monsoon since the onset of the Bølling-Allerød interstadial. Combining previous analyses of dust provenance, we argue that this pattern likely attributes to heightened Central Asian dust input driven by winter-spring southwest winds and increased precipitation controlled by summer monsoon. The abrupt vegetation prosperity at the beginning of the Holocene Optimum, as evidenced by an increase in total organic carbon and total nitrogen, could have reduced the concentration of Mg, Fe, Al, and 9Be derived from the weathering of surrounding basaltic bedrock. The identified abrupt decreases in precipitation in northeastern China, inferred from our 10Be/9Be precipitation proxy, are consistent with known Dansgaard-Oeschger and Bond events in the North Atlantic region since the last deglaciation. This supports that global cooling events since the last deglaciation may be linked to a complex interplay between the intertropical convergence zone, El Niño events, and the Atlantic meridional overturning circulation.

How to cite: Yang, Y., Xu, S., Cao, Z.-P., and Liu, C.-Q.: Authigenic beryllium isotopes in maar lake sediments response to climate change since the last deglaciation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7851, https://doi.org/10.5194/egusphere-egu25-7851, 2025.

EGU25-10115 | ECS | Posters on site | AS4.20

Thermoremanent magnetic, 10Be and 14C data provide no convincing evidence for longterm solar variability in the Holocene 

Maximilian Arthus Schanner, Andreas Nilsson, and Raimund Muscheler
The longterm evolution of the Sun's activity is of crucial interest, when trying to understand both recent and historical climatic changes. On timescales beyond the direct observation through sunspots, one has to rely on records of cosmogenic radionuclides, such as 14C and 10Be. These radionuclides can be found, for example, in tree rings and ice cores. Their production rates are modulated by solar activity, but also by the Earth's magnetic field, and thus contain an entangled signal of their evolution.

We constructed a joint statistical model of solar activity and the global geomagnetic field, accounting for a possible bi-modality in solar modulation, due to the occurrence of grand solar minima. Inversion of 10Be data from Greenland (GRIP) and Antarctica (EDML), 14C data from IntCal20 and global thermoremanent magnetic data from GEOMAGIA provides no convincing evidence for longterm solar variability over the Holocene, apart from possible clustering of grand solar minima. Additionally, the radionuclide records do not provide strong constraints on the time-averaged symmetry of the global geomagnetic field, due to a lack of calibration and lack of magnetic data from the southern hemisphere.

How to cite: Schanner, M. A., Nilsson, A., and Muscheler, R.: Thermoremanent magnetic, 10Be and 14C data provide no convincing evidence for longterm solar variability in the Holocene, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10115, https://doi.org/10.5194/egusphere-egu25-10115, 2025.

EGU25-12244 | Orals | AS4.20

Production rates of atmospheric cosmogenic nuclides 3H, 7Be, 10Be, 14C, 22Na, 36Cl calculated for the 20th and early 21st centuries 

Stepan Poluianov, Gennady Kovaltsov, Ilya Usoskin, and Naoyuki Kurita

Galactic cosmic rays constantly bombard the Earth’s atmosphere and induce cascades of nuclear reactions that produce various particles. One of the products of such interactions is cosmogenic nuclides, very useful tools for researches in different areas, such as solar physics, atmospheric physics, geomagnetic studies, hydrology, archeology, and many others. Their production rates are not uniform over the globe. Due to the changing shielding effect of the Earth’s geomagnetic field from cosmic rays, the production is higher in polar regions than near the equator. Furthermore, the production of cosmogenic nuclides varies greatly with altitude. In addition, the cosmic ray flux changes over time, following variations in solar activity. Several production models are available that account for all these effects (Poluianov et al., 2016, 2020), but their use requires some learning of computational details. To simplify the application of these models, we present calculated time series of the production rates for 3H, 7Be, 10Be, 14C, 22Na, and 36Cl, covering more than a century up to the present day. The results provide altitude-longitude-latitude resolution for each nuclide, include recent cosmic-ray data for the beginning of the 20th century, and account for the slow evolution of the geomagnetic field.

How to cite: Poluianov, S., Kovaltsov, G., Usoskin, I., and Kurita, N.: Production rates of atmospheric cosmogenic nuclides 3H, 7Be, 10Be, 14C, 22Na, 36Cl calculated for the 20th and early 21st centuries, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12244, https://doi.org/10.5194/egusphere-egu25-12244, 2025.

EGU25-13118 | ECS | Orals | AS4.20

Meteoric 10Be/9Be as a Proxy for Denudation and Uplift in the active Albanides orogenic belt 

Chiara Bazzucchi, Hella Wittmann, Silvia Crosetto, Paolo Ballato, Claudio Faccenna, and Francesca Rossetti

Cosmogenic nuclides are invaluable tools for quantifying denudation and uplift rates and thus decoding geological processes that act over different timescales and leave distinct imprints on the Earth’s surface. Among these, meteoric ¹⁰Be has emerged as a particularly powerful proxy due to its unique capability of being measured independently of lithology. Meteoric 10Be is an atmospheric flux tracer, and when normalized to stable 9Be, a trace element released by rocks during weathering, the 10Be/9Be ratio emerges. This ratio can be measured on small sample amounts and is independent of the presence of quartz which provides a benefit over the “sister” nuclide in situ 10Be that has been widely used in landscapes of felsic rocks.

The Albanides orogenic belt is a tectonically active region characterised by a remarkable lithological diversity, including carbonates, ophiolites, siliciclastics, metamorphics, and volcanic rocks distributed over short distances. In the Albanides´quartz-bearing sector, in situ ¹⁰Be-derived denudation rates were recently measured, but large areas of this belt remained unexplored due to lack of quartz. Meteoric 10Be/9Be -derived denudation rates fill this gap. When combined with geomorphic analyses to investigate uplift patterns in equilibrated river systems, results from both cosmogenic nuclides systems are consistent, and reveal significant spatial variability in denudation and uplift rates ranging from 0.1 to over 1.5 mm/yr. These results suggest that the Albanides are undergoing rapid landscape evolution, with rates and uplift mechanisms varying considerably across the belt. Our findings underscore the versatility of the meteoric ¹⁰Be/⁹Be method as a robust approach providing key information for quantifying erosional processes, sediment transport dynamics, landscape development and tectonic evolution. The consistency between the two datasets strengthens the reliability of the meteoric ¹⁰Be/⁹Be technique across regions with diverse geological compositions. Overall, our approach paves the way for future studies aimed at exploring the interplay between tectonics, climate, and surface processes using cosmogenic nuclides in complex lithological settings.

How to cite: Bazzucchi, C., Wittmann, H., Crosetto, S., Ballato, P., Faccenna, C., and Rossetti, F.: Meteoric 10Be/9Be as a Proxy for Denudation and Uplift in the active Albanides orogenic belt, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13118, https://doi.org/10.5194/egusphere-egu25-13118, 2025.

EGU25-14118 | Posters on site | AS4.20

Concentrations of Be-7 cosmogenic radionuclide in aerosols in connection with geomagnetic storms of CIR/HSSWS origin with atmospheric influences. 

Kateřina Podolská, Michal Kozubek, Miroslav Hýža, and Tereza Šindelářová

We investigate the coupling of concentrations of the cosmogenic radionuclide Be-7 (time series of activity concentration of Be-7 in aerosols evaluated by the corresponding activity in aerosols on a weekly basis at the National Radiation Protection Institute Monitoring Section in Prague) with reliable indicators of various atmospheric processes primarily determined by the solar activity level and space weather conditions influenced by coupling processes between the neutral atmosphere, ionosphere including sporadic E layers, magnetosphere and other geospace environment. We try to contribute to better understanding of the dynamics of these processes by associating them with new catalogue of over two hundred geomagnetic storms initiated by co-rotating Interaction Region (CIR)/High-Speed solar wind Stream (HSSWS) during the years 2016 – 2023. The catalogue CIR/HSSWS allows analysis of geomagnetic storms effects on ionosphere and troposphere which were clearly caused by CIR/HSSWS and or sudden stratospheric warmings or various significant tropospheric events like convection associated with frontal passages over European region. We also compare Be-7 concentrations during periods of strong solar and geomagnetic storms with periods of low solar activity in the longitudinal view in years 1986 – 2023.

How to cite: Podolská, K., Kozubek, M., Hýža, M., and Šindelářová, T.: Concentrations of Be-7 cosmogenic radionuclide in aerosols in connection with geomagnetic storms of CIR/HSSWS origin with atmospheric influences., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14118, https://doi.org/10.5194/egusphere-egu25-14118, 2025.

EGU25-15088 | ECS | Orals | AS4.20

An assessment of modern and past Circumpolar Deep Water presence beneath Shackleton Ice Shelf, East Antarctica: insights into using Meteoric Beryllium-10 

Matthew Jeromson, Molly Husdell, Helen Bostock, David Fink, Krista Simon, Ole Rieke, Sarah Thompson, Madi Rosevear, Luke Nothdurft, Laura Herraiz–Borreguero, and Duanne White

Perched precariously upon the deepest continental location on Earth, East Antarctica’s Denman Glacier is hypersensitive to changes in both air and ocean temperatures. Shackleton Ice Shelf buttresses Denman Glacier, regulating the rate at which it flows into the Southern Ocean. However, under warming ocean conditions along the continental shelf – a function of increased upwelling of warm Circumpolar Deep Water (CDW) in many places around Antarctica – Shackleton Ice Shelf may become unstable and collapse. Loss of the ice shelf would destabilise the glacier in turn, and a complete collapse of the Denman System could contribute +1.5 m to global sea level. Besides what began 15 years ago, observational ocean data show that the interactions between upwelling CDW and regional calving margins is otherwise unprecedented in historical records, and of unknown influence on longer timescales. Here we aim to resolve two questions: is warm CDW currently reaching the glacier’s grounding line? And is there any evidence of CDW presence within the Shackleton Ice Shelf on a Holocene timescale? Utilising a Conductivity-Temperature-Depth (CTD) profile and a 1m sediment core collected from the seafloor beneath Shackleton Ice Shelf during the 2023-24 Denman Terrestrial Campaign, we employ meteoric-10Be signatures from sediment samples – which have been shown to reflect upwelling circumpolar deep-water conditions along the Antarctic continental shelf – to discuss the modern and paleo-ocean conditions within the Shackleton Ice Shelf cavity.

How to cite: Jeromson, M., Husdell, M., Bostock, H., Fink, D., Simon, K., Rieke, O., Thompson, S., Rosevear, M., Nothdurft, L., Herraiz–Borreguero, L., and White, D.: An assessment of modern and past Circumpolar Deep Water presence beneath Shackleton Ice Shelf, East Antarctica: insights into using Meteoric Beryllium-10, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15088, https://doi.org/10.5194/egusphere-egu25-15088, 2025.

EGU25-15588 | Posters on site | AS4.20

Orographic and convective precipitation control meteoric 10Be wet depositional fluxes at low latitude 

Rose Paque, Angus Moore, Jean Dixon, Yessenia Montes, Marcus Christl, and Veerle Vanacker

Meteoric beryllium-10 (10Bem) is a valuable tracer for investigating land surface processes, and numerous studies have used it to assess soil ages and residence time, date sedimentary archives and quantify soil erosion rates at the hillslope and catchment scales. The flux of 10Bem to the Earth's surface is influenced by e.g. solar activity, the Earth’s magnetic field, stratosphere-troposphere exchange dynamics and atmospheric circulation patterns that control 10Bem production, transport, and deposition.

The control of precipitation on the flux of 10Bem to Earth’s surface remains unclear at low latitude, where there is little observational data available. To study the impact of precipitation on deposition of 10Bem at low latitude, we determined 10Bem concentrations in rainwater along a 10-fold precipitation gradient on Santa Cruz Island in the Galápagos Archipelago (Ecuador) over one meteorological year. To elucidate spatial and temporal variations in 10Bem concentrations, rainwater was collected at five sites spanning the precipitation gradient during the cool and warm seasons.

Our findings reveal a rise in 10Bem deposition rates with precipitation that exceeds a linear increase, indicating a super-additive effect of precipitation on 10Bem deposition. We attribute this to the presence of an inversion layer on Santa Cruz Island during the cool season, which limits atmospheric mixing. Furthermore, we observed a clear decline in 10Bem concentrations with increased convective precipitation during the warm and rainy season. This suggests a dilution effect on atmospheric 10Bem deposition during intense precipitation events. Our study highlights the spatial variability of 10Bem deposition along a precipitation gradient and deepens understanding of how different types of precipitation influence 10Bem fluxes.

How to cite: Paque, R., Moore, A., Dixon, J., Montes, Y., Christl, M., and Vanacker, V.: Orographic and convective precipitation control meteoric 10Be wet depositional fluxes at low latitude, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15588, https://doi.org/10.5194/egusphere-egu25-15588, 2025.

EGU25-17083 | Orals | AS4.20

Combining meteoric 10Be and U-series isotopes to decode weathering intensity in East Antarctica’s subglacial environment 

Joseph Graly, Adi Torfstein, Eiríka Arnardóttir, Kathy Licht, and Marc Caffee

We investigated chemical weathering in the subglacial environment of East Antarctica through studies of two isotope systems: meteoric 10Be and (234U/238U). We sampled blue ice moraines as a window into Antarctica’s subglacial environments. Here vapour-starved winds ablate near-stagnant ice, allowing sediment-rich basal ice to be thrust against mountains and nunataks. These moraines form across a wide swath of the continent. Many blue ice moraine sediments are substantially altered by chemical weathering; sediment grains are often coated in a mix of clays, oxides, and amorphous material that does not resemble soil but speaks to a chemical weathering regime specially found in the subglacial environment.

Meteoric 10Be works as a tracer in this system because its concentration in ice is relatively well known from ice cores, it is very unlikely to occur in detrital minerals, and it has a strong propensity to become incorporated in authigenic minerals, such as clays and oxyhydroxides. The total abundance of meteoric 10Be therefore traces meltwater input over the sediment residence time and the speciation of meteoric 10Be traces the formation of authigenic minerals.

In developing the meteoric 10Be tracer, we initially focused on Mt. Achernar Moraine, a site in the central Transantarctic Mountains containing highly weathered fine sediments of subglacial origin. We tested a variety of extraction procedures to most effectively extract 10Be from minerals formed during chemical weathering. At Mt. Achernar Moraine, the total meteoric 10Be strongly correlates to the abundance of authigenic minerals (particularly smectite clay) and aligns well with mass balance calculations for meltwater input.

The use of (234U/238U) as a tracer relies on the loss of 234U due to alpha recoil. As a result, (234U/238U) in residual detrital silt and clay particles drops below equilibrium and progresses towards a low steady state value. By contrast, the surrounding solutions and authigenic minerals that precipitate from them display (234U/238U) ratios higher than equilibrium.

Analyses of several samples from Mt. Achernar Moraine, show that U series isotopes confirm recent (i.e. within 100 ka) authigenic weathering at the site. Clay mineral (234U/238U) ratios are higher than those of silt, suggesting a mix of detrital and authigenic clay. Adsorbed species, carbonates, and oxyhydroxides display (234U/238U) higher than equilibrium, reflecting their precipitation from 234U-enriched solutions.

The results in total are very promising for both isotope systems. The U series system can constrain the time frame of chemical alteration to within a glacial-interglacial cycle.  The 10Be system trace the meltwater input and also confirm the presence of authigenic mineral phases. These tracers, especially in combination, allow us to define the relationship between meltwater input and weathering intensity across Antarctica and make large scale influences about the ice sheet’s influence on its substrate and on global biogeochemical cycles.

How to cite: Graly, J., Torfstein, A., Arnardóttir, E., Licht, K., and Caffee, M.: Combining meteoric 10Be and U-series isotopes to decode weathering intensity in East Antarctica’s subglacial environment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17083, https://doi.org/10.5194/egusphere-egu25-17083, 2025.

Cosmogenic nuclide records can in principle allow for the estimation of the behaviour of the heliospheric magnetic field (HMF) in the distant past. This study focuses on understanding how magnetic field turbulence uncertainties impact cosmic ray (CR) transport modeling on long time scales. We present a 3D time-dependent ab initio CR modulation code that utilizes theoretically and observationally motivated temporal profiles of heliospheric parameters that influence CR transport, emphasizing both large-scale parameters (such as the tilt angle) and small-scale turbulence parameters. The model is validated against spacecraft observations of galactic CR proton differential intensities for 1977-2001, showing good agreement with observed CR intensity profiles. To investigate pre-space age cosmic ray modulation, we applied historic HMF estimates from McCracken & Beer (2015) as model inputs, revealing clear evidence of drift effects during the Dalton Minimum. The study demonstrates the critical role of magnetic turbulence characterization in understanding historic cosmic ray modulation, and the uncertainties therein

How to cite: Moloto, K.: Modeling Long-Term Cosmic Ray Transport: The Role of Magnetic Turbulence Uncertainties in Heliospheric Field Reconstruction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19388, https://doi.org/10.5194/egusphere-egu25-19388, 2025.

EGU25-20054 | ECS | Orals | AS4.20

Volcanic modulation of Beryllium-10 atmospheric transport 

Andrin Jörimann, Timofei Sukhodolov, Louise Harra, Mélanie Baroni, Eugene Rozanov, and Tatiana Egorova

Cosmogenic 10Be isotope is an important proxy for past solar activity that can be measured from natural archives such as ice cores. It is mostly produced in the stratosphere and its atmospheric lifetime until the deposition to the surface depends on different transport processes. In the troposphere, 10Be deposition to natural archives occurs comparatively quickly, being dominated by scavenging, with weather patterns causing regional variations. The stratospheric and cross-tropopause transport of the isotopes is affected by their attachment to the stratospheric aerosol particles, presenting an additional effect of size-dependent gravitational sedimentation.  Strong volcanic eruptions massively increase the stratospheric aerosol loading, thus increasing its effect on the 10Be transport and deposition, which has been proposed as a major complication term in the interpretation of proxy records. In our study, we address this effect by employing the state-of-the-art aerosol-chemistry-climate model SOCOL-AERv2-Be that has a full 10Be atmospheric cycle, including its attachment to aerosol particles. We isolate the effects of sedimentation by comparing simulations with and without it for the 10Be tracer. In these simulations we examine the long-term climatological effects of a background aerosol layer on the 10Be distribution in the atmosphere and the resulting deposition maps. In another set of simulations we specifically focus on the influence of the enhanced stratospheric aerosol layer after volcanic events of various magnitudes, including their large-scale dynamical effects on the 10Be transport induced by the lower stratospheric heating. The results are compared with ice core data from the Greenland and Antarctic stations.

How to cite: Jörimann, A., Sukhodolov, T., Harra, L., Baroni, M., Rozanov, E., and Egorova, T.: Volcanic modulation of Beryllium-10 atmospheric transport, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20054, https://doi.org/10.5194/egusphere-egu25-20054, 2025.

EGU25-20720 | Orals | AS4.20

 Ocean 10Be/9Be as denudation rate proxy. Does 9Be deliver? 

Friedhelm von Blanckenburg

The ratio of meteoric cosmogenic 10Be to that of stable 9Be in seawater has been suggested to serve as a proxy for terrestrial weathering and denudation rates (D), in the modern ocean [1], and in the past when measured in chemical sediment of known age [2, 3]. The principle is remarkably simple. The only input of 10Be is atmospheric deposition into seawater. This flux is well-known at the scale of ocean basins. The trace metal9Be enters the oceans after continental weathering via two potential pathways: a) direct riverine input into the coastal ocean (both dissolved and mobilised from particles); b)  the release of “reactive” terrigenous Be from particles into seawater during early marine diagenesis, called “boundary exchange”. When the dissolved 9Be is mixed with seawater, the unknown weathering and denudation input flux of 9Be can be calculated from the 10Be/9Be ratio.

However, because Be is an element that readily attaches to reactive particles, not all riverine 9Be escapes the coastal zone. We have estimated this delivery fraction (fdel) to be about 6% of the dissolved and adsorbed riverine Be [1]. For pathway a) we already suggested the possibility that with changing sediment delivery to the coastal ocean, fdel might potentially be a function of D itself [1]. However, global river data show that river particle concentration and D are not correlated. Yet, this erroneous assumption was made to suggest that 10Be/9Be fails to serve as a denudation rate proxy [4].

In any case such dependence does not affect pathway b) “boundary exchange” [5]. This pore water input may even dominate the marine 9Be budget [6].

Research is thus required to evaluate all of these potential input pathways of 9Be, how strongly sediment delivery onto the seafloor, also being a function of particulate riverine input flux, controls the release flux of 9Be, and whether its release is buffered in any way. Given the simple pathway of the known 10Be input, the 10Be(meteoric)/9Be ratio offers much potential to explore these fluxes, both in the terrestrial and the marine domain, and to evaluate their dependence on denudation and delivery – even three decades  after the first introduction of this system [7].

  • von Blanckenburg, F. and J. Bouchez, Earth and Planetary Science Letters, 2014. 387
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  • Li, S., S.L. Goldstein, and M.E. Raymo, Proc Natl Acad Sci USA, 2021. 118
  • von Blanckenburg, F., Bouchez, J., Willenbring, J.K., Ibarra, D.E., Rugenstein, J.K.C., Proc Natl Acad Sci USA, 2022. 119
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How to cite: von Blanckenburg, F.:  Ocean 10Be/9Be as denudation rate proxy. Does 9Be deliver?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20720, https://doi.org/10.5194/egusphere-egu25-20720, 2025.

The oceans are filled with acoustic waves, which are trapped in a low-velocity layer at about 1 km water depth. The sound speed of these waves strongly depends on the temperature. An increase in temperature will lead to an increase in the sound speed and hence shorter travel times. IMS hydro-acoustic stations measure these waves continuously and travel times can be obtained through the cross correlation of transient signals between different hydrophones. IMS hydro-acoustic station H10 near Ascension Island has been operational for nearly two decades. Although in place to detect nuclear-test explosion for the CTBT, H10 appeared well equipped to measure deep ocean temperature change. A decrease in the travel time between the two arrays was derived, being -0.002 s/yr. This corresponds to a deep ocean warming of 0.007 degC/yr, at about 900m water depth. As such, acoustic waves provide an independent and passively acquired measure of the temperature change in the deep ocean.

How to cite: Evers, L. G.: Decadal observations of deep ocean temperature change passively probed with acoustic waves, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2547, https://doi.org/10.5194/egusphere-egu25-2547, 2025.

Throughout the recent period of announced nuclear testing by the Democratic People's Republic of Korea there has been a series of small magnitude seismic events detected in the vicinity of the test site. These events, reported by the International Data Centre of the Comprehensive Nuclear Test-Ban-Treaty Organisation, are only detected at regional seismic stations. It is of interest to the global CTBTO community if these events and the announced nuclear tests can be characterised using regional observations. We investigate the ratio of P- to Lg-wave amplitudes to discriminate between announced nuclear tests and presumed earthquakes in the vicinity of the test site. Investigating amplitude ratios independently at seismic stations overcomes path effects assuming that the events of interest are all located near to each other. There is a clear separation between the P/Lg ratios of announced nuclear tests and presumed earthquakes on the 3-component sensors at USRK and MDJ for events within 50km of the test site. Interestingly, the signals in the vicinity of the test site have low coherence across the USRK seismic array, likely due to effects from local geology at the array site. Effective discrimination comes from averaging the root-mean-square amplitudes of all three-components of the seismometer, and not on the beam made using vertical array elements. The Pg/Lg amplitude ratios are more consistent over the range of passbands investigated (1-18Hz) compared to Pn/Lg ratios. The P/Lg ratios of assumed mining events (the majority generating infrasound detections) in the vicinity of the test site are higher than earthquakes, however being more than 100km from the test site could generate different path effects to USRK. Discrimination between earthquakes and explosions in the vicinity of the DPRK test site using regional signals supports the technical verification of the CTBT.

© British Crown Owned Copyright 2024/AWE

How to cite: Merrett, M. and Selby, N.: The characterisation of announced nuclear tests and seismic events in the vicinity of the DPRK test site using P/Lg ratios at regional seismic stations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3160, https://doi.org/10.5194/egusphere-egu25-3160, 2025.

Infrasound measurements play a critical role in global bolide detection and accurate location determination. However, significant mismatches frequently emerge between observed back azimuth angles and theoretical predictions derived from a bolide’s brightest emission point, especially under shallow entry conditions. In such instances, elongated acoustic traces across multiple trajectory segments induce large variations in back azimuth residuals. An investigation to quantifies the effects of varying entry angles on azimuth deviations over distances up to 15,000 km was carried out. The results show that shallow-angle entries can produce substantial discrepancies, complicating reliable geolocation at extended ranges. Conversely, steeper trajectories yield more consistent azimuth measurements, minimizing uncertainties. These findings demonstrate the necessity of incorporating entry geometry in infrasound analyses to refine bolide detection and bolster planetary defense. Additionally, this framework offers important considerations for other high-energy atmospheric phenomena, such as spacecraft re-entries, where accurate geolocation remains paramount.

SNL is managed and operated by NTESS under DOE NNSA contract DE-NA0003525.

How to cite: Silber, E.: Reducing uncertainties in bolide and space debris detection: The role of entry geometry in infrasound analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4030, https://doi.org/10.5194/egusphere-egu25-4030, 2025.

EGU25-4487 | PICO | SM8.5

Time residuals at HA11 and HA03 for T-phases from deep earthquakes in the Ring of Fire 

Tiago Oliveira, Urtnasan Khukhuudei, and Rodrigo Chi-Durán

This work investigates the T-phase time residuals (defined as differences between the observed arrival times and their theoretical values) at IMS hydrophone stations HA11 and HA03 in the Pacific Ocean.  The work is focused on T-phases from earthquakes in the Ring of Fire recorded between 2001 and 2024. Time residuals of T phases from these regions can typically range from minus 150 to 150 seconds. These disparities between expected and observed arrival times can present significant challenges when associating hydroacoustic signals to events built by automatic processing systems or by human analysts based on signals recorded by the IMS network. In this work, we shed light on the reasons for these high time-residual variabilities. We show that the time residuals in these regions depend on the location of the hypocentre along the subduction plate. Overall, time residuals go from negative (T phases arrive earlier than expected) to positive (later than expected) as the earthquake depth decreases along the subduction and approaches the Ocean Trench. We present general results for the Ring of Fire and detailed analyses for regions with different subduction angles in the trenches of Kermadec-Tonga, Mariana, Philippines, Nansei-Shoto, Kuril, Aleutian, and Peru-Chile.   

How to cite: Oliveira, T., Khukhuudei, U., and Chi-Durán, R.: Time residuals at HA11 and HA03 for T-phases from deep earthquakes in the Ring of Fire, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4487, https://doi.org/10.5194/egusphere-egu25-4487, 2025.

EGU25-4857 | PICO | SM8.5

Comparative Analysis of IDC REB Bulletins with NEIC Seismological Bulletin 

Ehsan Qorbani Chegeni, Fekadu Kebede Alamneh, Gerard Rambolamanana, and Gerhard Graham

The International Data Centre (IDC) of the Comprehensive Nuclear Test Ban Treaty Organization (CTBTO) processes and analyses data from the International Monitoring System (IMS). This effort culminates in the daily production of the Reviewed Event Bulletin (REB), recognized as one of the most comprehensive global seismic bulletins.

This study compares the IDC REB bulletins with those produced by the National Earthquake Information Center (NEIC), one of the major organizations producing seismological bulletins, over a 20-year period (2004–2024). Specifically, we assess the consistency of events with IDC magnitudes (mb) greater than 4, identifying events that are either missed or uniquely included by the IDC. By examining discrepancies in epicenter locations, we aim to pinpoint regions with significant location differences and investigate whether these discrepancies correlate with global and regional network coverage or are randomly distributed.

Additionally, we explore potential connections between location discrepancies and the use of travel time, azimuth, and slowness correction models. Our findings aim to enhance the understanding of global seismic monitoring accuracy, contributing to improved data integration, event detection, and correction models.

How to cite: Qorbani Chegeni, E., Kebede Alamneh, F., Rambolamanana, G., and Graham, G.: Comparative Analysis of IDC REB Bulletins with NEIC Seismological Bulletin, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4857, https://doi.org/10.5194/egusphere-egu25-4857, 2025.

EGU25-5270 | ECS | PICO | SM8.5

Hydroacoustic observations of a submarine landslide along Trou Sans Fond Canyon offshore Ivory Coast in March 2024 on CTBTO network 

Vaibhav Vijay Ingale, Ross Parnell-Turner, Wenyuan Fan, Peter J Talling, and Jeffrey Neasham

Underwater communication cables are critical components of global infrastructure, carrying over 99% of international data traffic. On 14 March 2024, a significant disruption to this network occurred due to a cable break offshore Ivory Coast, leading to widespread internet outages in the west African region. To investigate the cause of this cable break, we analyze hydroacoustic data recorded between 6 March and 22 March on the two hydrophone triads (H10N and H10S) installed near Ascension Island by the International Monitoring System of the Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO). We detect a low-frequency (< 60 Hz) signal on three northern and two southern triad hydrophones on 12 March 2024. The signal had a duration of 85 seconds on the north triad compared to 45 seconds on the south triad. We used the Generalized Cross-Correlation with Phase Transform method to show that the detected signal originated at a bearing of 38.8 ± 4.6°, consistent with the location of the cable break off Ivory Coast, and with steep bathymetric slopes mapped in the Trou Sans Fond Canyon. We do not observe associated signals on the nearby land-based seismic stations in Ghana and Ivory Coast, confirming the marine origin of this event. Additionally, template matching shows that the same signal was not recorded in the preceding and following 8 days, implying that this event was an isolated case. Given the scarcity of natural earthquakes offshore Ivory Coast, this combination of evidence suggests that the hydroacoustic signals are likely caused by a submarine landslide in the Trou Sans Fond Canyon. Our results show that investigating the causative submarine landslide events is also needed to realize the potential of these hydroacoustic methods for hazard risk assessment.

How to cite: Ingale, V. V., Parnell-Turner, R., Fan, W., Talling, P. J., and Neasham, J.: Hydroacoustic observations of a submarine landslide along Trou Sans Fond Canyon offshore Ivory Coast in March 2024 on CTBTO network, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5270, https://doi.org/10.5194/egusphere-egu25-5270, 2025.

EGU25-7096 | PICO | SM8.5

Deep learning based phase picking on seismological IMS stations 

Andreas Steinberg and Peter Gaebler

We present our work on training and the application of deep learning algorithms for the automated phase picking of body waves on the the IMS network. We train new IMS data based seismic phase pickers from both EQT and PhaseNet architectures. Phase picking is a necessary step before event localization and characterization and deep learning based models have been proven to perform well at this task. PhaseNet and EQTransformer are two prominent state-of-the-art phase picking algorithms that have been retrained on several different datasets.

Waveform data from primary and auxiliary stations is used in the training and evaluation. For training we use good quality picks from REB events between 2013 until 2023. We evaluate the performance in comparison with unseen evaluation REB phase picks and manual phase picks. We compare the performance with applying other pre-trained phase pickers to the IMS data to determine if already pre-trained models can be used satisfactory out of the box for seismological IMS data. We also evaluate the generalization ability of the two IMS data trained models by applying them to other non IMS seismological stations of the German Regional Seismic Network (GRSN).

We  further train new phase pickers based on the PhaseNet architecture and a database of 20 years listed in the earthquake catalog of BGR. The models are trained and evaluated with manual phase picks of BGR analysts. We compare the performance of the newly trained models by also applying other pre-trained PhaseNet and EQTransformer based phase pickers on unseen data.  We determine if existing pre-trained models can satisfactorily be used out of the box for phase picking on waveforms of the GRSN.

How to cite: Steinberg, A. and Gaebler, P.: Deep learning based phase picking on seismological IMS stations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7096, https://doi.org/10.5194/egusphere-egu25-7096, 2025.

EGU25-7200 | PICO | SM8.5 | Highlight

Combined (DAS/Seismometers) Seismic Analysis of an Underwater Explosion in the Baltic Sea 

Aurélien Mordret, Tine Larsen, Peter Voss, Emil Jensen, Trine Dahl-Jensen, Nicolai Rinds, Björn Lund, Michael Roth, Stefanie Donner, and Andreas Steinberg

In November 2024, an Ml ~1.5-2.0 underwater explosion occurred in Danish waters north of Bornholm Island. It was recorded by the Danish and Greenlandic national seismic networks as well as the Swedish national network. In addition, the event was captured by a nearby Distributed Acoustic Sensing (DAS) system deployed along a 120 km-long underwater fiber-optic cable. We investigated the event location by integrating data from these complementary recording systems, systematically assessing the trade-off between the number of DAS channels with respect to the number of permanent seismometers and the quality of the picks. Our results indicate horizontal uncertainties on the order of 2–3 km for the final event location. To further constrain the depth of the explosion and its yield, we conducted a spectral analysis of the seismograms, joined with a non-linear inversion of the P-waveforms at the closest station. The inferred source parameters are consistent with the known water depth and velocity at the explosion site, revealing that the event probably involved two distinct detonations located less than 10 m above the seafloor, each with an approximate 30 kg TNT equivalent yield. These findings highlight the advantages of combining conventional permanent seismic instrumentation with underwater DAS, thereby improving the detection and characterization of anthropogenic seismic sources and offering enhanced protection for critical submarine infrastructures.

How to cite: Mordret, A., Larsen, T., Voss, P., Jensen, E., Dahl-Jensen, T., Rinds, N., Lund, B., Roth, M., Donner, S., and Steinberg, A.: Combined (DAS/Seismometers) Seismic Analysis of an Underwater Explosion in the Baltic Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7200, https://doi.org/10.5194/egusphere-egu25-7200, 2025.

EGU25-8540 | PICO | SM8.5

Infrasound observation and propagation of recent meteoroid events  

Christoph Pilger and Patrick Hupe

Large meteoroids entering Earth’s atmosphere are a well-known source of infrasound. During the supersonic entry of space material into the atmosphere, shock waves are emitted from the trajectory as a line source. Explosive fragmentation of the meteoroid may additionally produce one or multiple point source events. Both types of shock waves propagate as low-frequency acoustic waves, also known as infrasound, within the atmosphere and to the Earth’s surface. Such infrasound signals can be detected by adequate instrumentation at distances of hundreds to thousands of kilometers, after long range sound propagation within atmospheric ducts.

Using microbarometer arrays of national observation networks, like e.g. the Central and Eastern European Infrasound Network, and the International Monitoring System for the Comprehensive Nuclear-Test-Ban Treaty, such meteoroid events can be remotely identified, localized and characterized. Array signal processing using the Progressive Multi-Channel Correlation method and propagation modeling using Ray-Tracing and Parabolic Equation approaches are applied to estimate the origin of the acoustic signals along the meteoroid trajectories and to derive information about entry parameters and explosive yield.

This study focuses on the infrasound observation, event analysis and sound propagation of recent meteoroid events, including the Southern Atlantic Ocean fireball on the 7th of February, 2022, the El Hakimia fireball over Northern Algeria on the 7th of May, 2023 and the Ribbeck fireball over Eastern Germany on the 21st of January, 2024.

How to cite: Pilger, C. and Hupe, P.: Infrasound observation and propagation of recent meteoroid events , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8540, https://doi.org/10.5194/egusphere-egu25-8540, 2025.

The global verification system established under the Comprehensive Nuclear-Test-Ban Treaty (CTBT) is designed to detect all nuclear explosions on Earth. Seismic monitoring, one of the four verification technologies, relies on the International Monitoring System (IMS), a global network of sensor stations, to identify nuclear explosion signals. This study presents an application of Moment Tensor (MT) inversion analysis to assist individual States Parties through expert technical analysis (ETA) of IMS data and any additional datasets provided by the requesting State Party. MT inversion enables precise determination of parameters such as total seismic moment, focal mechanism, and source depth. 


To evaluate this approach, we analyzed data from declared nuclear events in the Democratic People’s Republic of Korea (DPRK). For the most recent event, DPRK6 (2017/09/03), two methodologies were applied: (1) a regional moment tensor inversion in the time domain (TDMT, Dreger, 2003) and (2) a joint inversion using regional waveforms and teleseismic firstmotion polarities (Nayak and Dreger, 2015; Chi-Durán et al., 2024). The analysis included 4 regional waveforms (filtered between 20–50 s) and 81 teleseismic first-motion polarities from CTBTO stations. Known regional velocity models were used to model the synthetic waveforms (Ford et al., 2010; Dreger et al., 2021).


The TDMT approach achieved a high waveform fit and revealed a predominantly isotropic mechanism with a minor double-couple component. These findings are consistent with previous studies using other station datasets (e.g., Alvizuri and Tape, 2018; Chiang et al., 2018). The joint inversion further improved the waveform fit, with the isotropic component remaining dominant. The source-type lune plot confirmed a mechanism primarily characterized by isotropy. Current efforts aim to incorporate additional data, such as teleseismic waveforms, to refine the depth and other characteristics of the event across all declared DPRK events.

How to cite: Chi-Durán, R.: Moment Tensor Inversion Analysis of DPRK6 Nuclear Events Using CTBTO/IMS Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9831, https://doi.org/10.5194/egusphere-egu25-9831, 2025.

EGU25-11325 | ECS | PICO | SM8.5

Automatic identification of sources recorded by the hydroacoustic stations of the International Monitoring System 

Hugo Fauvel, Sentia Oger, Dorian Cazau, Sara Bazin, and Julien Vergoz

As part of the Comprehensive Nuclear Test Ban Treaty Organisation (CTBTO), six hydroacoustic stations were installed. Although few in number, they record underwater acoustic waves that propagate over long distances via the SOFAR (SOund Fixing And Ranging) channel. Low-frequency coherent waves (< 40 Hz) are detected automatically by the PMCC (Progressive Multi-Channel Correlation) method. An average of 306 daily detections, with a Maximum Amplitude (MaxAmp) above 1 Pa, are reported. At this point, there is no identification made by any analyst of the source type (e.g. earthquake, volcanism, cryosphere, whales, airgun, anthropophonic explosion). Thus, the aim of this study is to develop an automatic source discrimination tool to support operational monitoring.

We analyze PMCC extractions from stations in the Atlantic (HA10), Indian (HA01, HA04, HA08) and Pacific (HA03, HA11) oceans over a period spanning January to Decembre 2023. The association to a source type is made in two stages. (i) We apply wave parameter and acoustic indices conditional statements to select typical signals with MaxAmp above 1.5 Pa for each type of source, except for airgun with MaxAmp of 1 Pa. (ii) The resulting catalog of extracted records are used to train a convolutional neural network of two layers and calibrate it by conformal prediction with Least Ambiguous set-value Classifier (LAC) score and a nominal error level of 0.05. All detections with a MaxAmp greater than 1 Pa are associated with one or more source types.

Over the year 2023, 111,260 coherent waves were extracted by PMCC on the 8 hydrophone triplets, of which 14,028 were associated to a source type using the ad hoc conditional statements. These records are associated to the right source type by the trained neural network at 92.5%. Overall, the classifier associated 75 ± 6% of records with one source. Significant differences in performance were observed between the hydrophone triplets. Results were lowest at hydrophone triplet HA10N (< 65%), while they were highest at HA04N (> 80%). This difference is due to the soundscape, with certain sources (earthquakes, volcanoes and croyspheres) being more difficult to discriminate. The criteria used to compile the reference catalog need to be improved to discriminate more accurately detections by source type.

How to cite: Fauvel, H., Oger, S., Cazau, D., Bazin, S., and Vergoz, J.: Automatic identification of sources recorded by the hydroacoustic stations of the International Monitoring System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11325, https://doi.org/10.5194/egusphere-egu25-11325, 2025.

Analysis of seismic records of local earthquakes and a series of underground chemical explosions conducted during the Source Physics Experiment (SPE) at the Nevada National Security Site (NNSS) have shown that at local distances (<200 km) the effectiveness of the single-station P/S ratio source discriminant is reduced, especially when seismic recordings from a sparse network of stations is used.

We used high performance computing to model high-frequency (0-10Hz) waveforms for 12 selected local earthquakes, with magnitudes ranging from 2.05 to 3.54, recorded by a network of seismic stations in the Rock Valley at NNSS. In addition, we performed a series of simulations of collocated isotropic and double-couple explosion sources in the Rock valley. The high-frequency wave propagation scattering was simulated by adding correlated small-scale stochastic perturbations to the Seismic Velocity Model of the Rock Valley (SVM). The recorded and synthetic waveforms were then analyzed to investigate the effects of source radiation and wave scattering effects on the simulated waveforms and P/S source discriminant.

The inclusion of correlated depth-dependent stochastic velocity perturbations in the GFM, improved the quality of simulated source radiation and local waveforms, which resulted in better reproduction of the observed spatial variations of the P/S discriminant. We found that the shallow wave scattering deforms the radiation pattern and amplitude of source generated P and S waves, thus reducing the efficiency of the P/S discriminant. Our simulations suggest that a good azimuthal stations coverage and the network averaging can improve the performance of the P/S discriminant at local distances.

How to cite: Pitarka, A., Walter, W., and Pyle, M.: Broad-band Modeling of Earthquakes in the Rock Valley, Nevada: Implication of Wave Propagation Effects on the P/S Source Discriminant , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12763, https://doi.org/10.5194/egusphere-egu25-12763, 2025.

Radionuclide monitoring is complementary to seismic, hydroacoustic, and infrasound wave monitoring technologies used in verification, and it is the only one that can discriminate and confirm whether an explosion detected and located is indicative of a military nuclear explosion. Therefore, to understand radioactive particles and noble gas prompt releases from underground nuclear explosions, their transport in the atmosphere to radionuclide monitoring stations, and to discriminate nuclear explosion generated radioisotopes from artificially produced ones, generated and released by nuclear reactors, particle accelerators, or radionuclide generators, one must accurately and numerically simulate the explosion phase, the interaction of the explosive energy released with the fractured hosting rock, and cavity formation, the radionuclide generation and their circulation within the cavity, and the eventual prompt release or seepage of the radionuclide gases to the atmosphere. To support this daunting task, LLNL has developed an HPC-based comprehensive numerical framework to simulate, from source-to-atmosphere, the radioisotope gas releases by coupling a non-linear explosion hydrocode to a geomechanical code that converts explosion-induced damage to rock permeability, which is a key parameter to subsurface and surface coupled gas transport codes. The resulting gas releases source to the atmosphere is then used as an input to a global atmospheric circulation code to reach the monitoring stations. We illustrate the onset of the different regimes and their combined effect of flow, heat and mass transport of different gas species, the fraction of molten rock and their impact on the noble gas fractionation. We also present a sensitivity analysis of the effect of the outer cavity boundary condition on the heat loss and cooling to the adjacent rock formation and its eventual release to the atmosphere. We demonstrate several scenarios of underground prompt releases to the atmosphere using a first-ever fully coupled prompt subsurface-to-atmospheric transport without ad-hoc boundary conditions between physics-based domains, or handshakes between different numerical codes. We also demonstrate using HPC-empowered numerical hypothetical explosion scenarios, the benefits of the proposed technology versus the common approaches. We will conclude by exploring physics informed ML schemes for developing surface responses of the end-to-end simulation framework to anthropogenic explosions. This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

How to cite: Ezzedine, S., Vorobiev, O., Herbold, E., Sun, Y., Hao, Y., and Myers, S.: End-to-End HPC Numerical Simulations of Underground Explosions, Cavity Formation and Circulation Processes, Subsurface Gas Transport, and Prompt Atmospheric Releases, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14449, https://doi.org/10.5194/egusphere-egu25-14449, 2025.

At the International Data Centre (IDC), data received from the International Monitoring System (IMS) network goes through a three-step process (station processing, network processing and interactive review) to determine if a combination of detections can be built into an event. One of the major steps in determining if an event can be built or not, is the phase classification of the detected signals. For acoustic data, phases are determined during each process where in the first two steps, algorithms will automatically name and rename phases based on a set of criteria and thresholds. In the interactive review, analysts can change or rename phases for a final time to build or not build an event. Here, we analyze the number of phase changes at each IMS Infrasound and hydroacoustic station and compare the number of detections in each process database to examine how a detection contributes to building an event. Furthermore, the expansion of the operational stations of the IMS network is examined to understand how additional stations have altered the ability of the automatic and interactive processes to classify phases and build events. Ultimately, the results of this analysis can be used to improve the automatic IDC pipeline for acoustic phase classification and building events. 

How to cite: Walsh, B. and Oliveira, T.: Understanding phase classification throughout the International Data Centre acoustic pipeline, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15641, https://doi.org/10.5194/egusphere-egu25-15641, 2025.

The radionuclide network of the International Monitoring System for the Comprehensive Nuclear-Test-Ban Treaty is in place for the detection of tiny atmospheric traces of radioactive fission and activation products generated by nuclear explosions.  Atmospheric transport modelling supports the assessment of potential source regions and checks for consistency with explosion sites.

All radionuclide station sniff for particulate radionuclides, a part of it is additionally equipped with noble gas systems measuring radioactive xenon isotopes. Those are of particular importance as they are more likely to escape from underground nuclear explosions and the inert character is advantageous for simulating atmospheric transport.

A central challenge of radioxenon monitoring remains to classify radioactive xenon emissions originating from other sources as isotope production facilities and other reactors. This attribution was also crucial for the interpretation of radioxenon detections in the aftermath of the announced North Korean nuclear test explosions.  

Another radioactive noble gas isotope krypton-85. It is not part of the list of CTBT relevant isotopes due to its large background (half-life 10.8 years) and smaller nuclear yield. Large quantities of krypton-85 have been released into the atmosphere by nuclear fuel reprocessing both for military and civilian purposes. This created a significant atmospheric background due to the long krypton-85 half-life. In the context of discussing monitoring possibilities for a future fissile material cut-off krypton-85 is potentially suitable as indicator for the detection of clandestine plutonium separation. The “Bundesamt für Strahlenschutz” (BfS, Federal Office for Radiation Protection) has been operating a network with weekly air sample collection at up to 26 locations in Germany and worldwide since 1973. For the data from 2005-2024 backward ATM is performed for more than 10000 samples from about 10 stations. Taking advantage of the long time series we analyse if backward atmospheric transport modelling allows even in the coarse time resolution of weekly samples for attribution to different emitters on the Northern Hemisphere.  The effect of the shutdown of the Selllafield reprocessing facility on the European network is analysed as example.

How to cite: Ross, J. O. and Brander, S.: Assessment of emissions from noble gas background sources: what can we learn from atmospheric transport modelling for long term krypton-85 measurements?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19799, https://doi.org/10.5194/egusphere-egu25-19799, 2025.

EGU25-20246 | PICO | SM8.5

Reducing Uncertainty in Nuclear Test Detection: An Analysis of Multiple IMS Detections 

Anne Tipka, Jonathan Bare, Robin Schoemaker, and Monika Krysta

The Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO) relies on its International Monitoring System (IMS) to detect radionuclide releases, which can indicate potential nuclear tests. By using atmospheric transport modelling (ATM), the CTBTO aims to establish links between detecting stations and corresponding source locations. When detection is limited to a single event within a narrow time window or between neighbouring stations, operational analysis typically generates large possible source regions that require further refinement. Multiple detections offer a unique opportunity for a more detailed analysis, allowing advanced methods to be applied for more accurate identification of the source location.

Recently, elevated levels of radioxenon were detected at multiple IMS locations in and around the Japanese region, including Takasaki, Wake Island, and the non-IMS system at Horonobe. These detections exceeded historical levels, emphasizing the need for a more detailed analysis. The dense network of measurement stations in this area presents an opportunity to explore advanced methods for source localization, reducing the uncertainty, and to discuss the implications of these findings on the monitoring of radioxenon isotopes.

How to cite: Tipka, A., Bare, J., Schoemaker, R., and Krysta, M.: Reducing Uncertainty in Nuclear Test Detection: An Analysis of Multiple IMS Detections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20246, https://doi.org/10.5194/egusphere-egu25-20246, 2025.

EGU25-3877 | Orals | NP1.3

The Typicality of Regimes Associated with Northern Hemisphere Heatwaves 

Christopher Chapman, Didier Monselesan, James Risbey, Abdelwaheb Hannachi, Valerio Lucarini, and Richard Matear

We study the hemispheric to continental scale regimes that lead to summertime heatwaves in the Northern Hemisphere. By using a powerful data mining methodology -archetype analysis - we identify characteristic spatial patterns consisting of a blocking high pressure systems embedded within a meandering upper atmosphere circulation that is longitudinally modulated by coherent Rossby Wave Packets. Periods when these atmospheric regimes are strongly expressed correspond to large increases in the likelihood of extreme surface temperature. Most strikingly, these regimes are shown to be typical of surface extremes and frequently reoccur. Three well publicised heatwaves are studied in detail - the June-July 2003 western European heatwave, the August 2010 "Russian" heatwave, and the June 2021 "Heatdome" event across western North America. We discuss the implications of our work for long-range prediction or early warning, climate model assessment and post-event diagnosis.

How to cite: Chapman, C., Monselesan, D., Risbey, J., Hannachi, A., Lucarini, V., and Matear, R.: The Typicality of Regimes Associated with Northern Hemisphere Heatwaves, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3877, https://doi.org/10.5194/egusphere-egu25-3877, 2025.

EGU25-5631 | Orals | NP1.3

TurboMeter: attributing aviation turbulence events to climate change 

Tommaso Alberti, Lia Rapella, Erika Coppola, and Davide Faranda

Turbulence remains a pressing challenge for aviation safety and efficiency, as highlighted by recent incidents involving Singapore Airlines, Qatar Airways, and Scandinavian Airlines. Among the various types, Clear Air Turbulence (CAT) poses the greatest hazard due to its occurrence in clear skies, rendering it difficult to detect and predict. Furthermore, the unprecedented changes in Earth's climate are reshaping atmospheric dynamics on a global scale, with profound implications on aviation. As a companion of ClimaMeter, a platform designed to assess and contextualize extreme weather phenomena in relation to climate change, we introduce here TurboMeter. It is designed to use ERA5 reanalysis data to investigate the meteorological drivers of turbulence events by comparing them with historical analogues under similar atmospheric conditions. Turbulence diagnostics, including Ellrod’s indices, are used to evaluate the roles of jet streams, wind shear, and convective activity at typical cruising altitudes.

To illustrate TurboMeter, we present some recent aviation turbulence events occurred during 2024. Our findings reveal that they are closely linked to intensified jet streams and enhanced convective activity, influenced by the growing impacts of anthropogenic climate change. These results highlight a concerning trend: changing climatic patterns are altering the atmospheric drivers of turbulence, particularly CAT, with significant implications for flight safety and operational planning. Our study evidences the urgent need for improved weather forecasting and turbulence prediction models to mitigate aviation risks in a rapidly warming climate.

How to cite: Alberti, T., Rapella, L., Coppola, E., and Faranda, D.: TurboMeter: attributing aviation turbulence events to climate change, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5631, https://doi.org/10.5194/egusphere-egu25-5631, 2025.

EGU25-5780 | Posters on site | NP1.3

ClimaMeter: a rapid attribution framework for weather extreme events 

Davide Faranda and the The ClimaMeter team
Climate change is a global challenge with manifold and widespread consequences, including the intensification and increased frequency of numerous extreme weather phenomena. In response to this pressing issue, we introduce ClimaMeter, a platform designed to assess and contextualize extreme weather phenomena in relation to climate change. The platform provides near-real-time information on the dynamics of extreme events, serving as a resource for researchers, policymakers, and acting as a scientific outreach tool for the general public. ClimaMeter currently analyzes heatwaves, cold spells, heavy precipitation, and windstorms.Our methodology is based on looking for weather conditions similar to those that caused the extreme event of interest with physics-informed machine-learning methodologies. We focus on the satellite era, namely the period since 1979, when widespread observations of climate variables from satellites have become available. The object studied (i.e. "the event") is asurface-pressure pattern over a certain region and averaged over a certain number of days, that has lead to a extreme weather conditions. We split the dataset 1979-Present in two parts of equal length and consider the first half of the satellite era  as "past" and the second part as "present" separately. We use data from MSWX. We then compare how the selected weather conditions have changed between the two periods, and whether such changes are likely due to natural climate variability or anthropogenic climate change.
This presentation sheds light on the methodology, data sources, and analytical techniques that ClimaMeter relies on, offering a comprehensive overview of its scientific foundations. To illustrate ClimaMeter, we present some examples of recent extreme weather events. Additionally, we highlight the role of ClimaMeter in promoting a profound understanding of the complex interactions between climate change and extreme weather phenomena, with the hope of ultimately contributing to informed decision-making and climate resilience. Follow us on the social-media @ClimaMeter and visit www.climameter.org.

How to cite: Faranda, D. and the The ClimaMeter team: ClimaMeter: a rapid attribution framework for weather extreme events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5780, https://doi.org/10.5194/egusphere-egu25-5780, 2025.

EGU25-7645 | ECS | Orals | NP1.3

Advancing the understanding of extreme events through the lens of dynamical system theory 

Chenyu Dong, Adriano Gualandi, Valerio Lucarini, and Gianmarco Mengaldo

Since Lorenz's pioneering work, dynamical systems theory has provided a powerful framework for studying complex systems. Among these, the study of their instantaneous properties is particularly significant for understanding short-lived yet impactful extreme events. Here, we propose an analogues-based index to measure the instantaneous predictability of dynamical systems over different forecasting horizons. We demonstrate its application in both classical dynamical systems and the Euro-Atlantic sector atmospheric circulation. Furthermore, recognizing that the onset of extreme events often involves processes operating across different scales, we introduce a novel framework that enables the exploration of scale-dependent dynamical properties. Given the flexible and generalizable nature of these methods, we believe they open new research avenues for studying extreme events from a dynamical systems perspective and will serve as valuable tools for deepening our understanding of extreme events.

How to cite: Dong, C., Gualandi, A., Lucarini, V., and Mengaldo, G.: Advancing the understanding of extreme events through the lens of dynamical system theory, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7645, https://doi.org/10.5194/egusphere-egu25-7645, 2025.

EGU25-7685 | Orals | NP1.3

Progress and Challenges in the Study of Extreme Weather 

Gianmarco Mengaldo

Extreme weather events, including heatwaves, extreme precipitation, tropical cyclones, and other hazards, pose significant risks to society and ecosystems. Recent advancements in observational techniques, numerical modeling, theoretical frameworks, and AI methods have greatly improved our understanding and prediction of extreme weather events. However, despite significant progress, key challenges remain unresolved, particularly in achieving a thorough understanding of the physical drivers of extreme events, improving the transparency of AI-based prediction methods, and evaluating the vulnerability and resilience of cities to their impacts. To address these challenges, we present various approaches drawn from different fields, including dynamical systems theory, explainable AI, and NLP-based methods. Given the flexible and generalizable nature of these methods, we believe they may pave the way toward more robust solutions for addressing the challenges posed by extreme weather events.

How to cite: Mengaldo, G.: Progress and Challenges in the Study of Extreme Weather, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7685, https://doi.org/10.5194/egusphere-egu25-7685, 2025.

Compound climate and weather extremes have received significant attention in recent years due to the increased risks that they pose to the environment, human societies, and the economy. While prior studies have identified associations between various hazards in disaster databases, investigations focussing on droughts and floods remain rare. In this study, we analyze the impacts of concurrent or sequential drought-flood extremes from two widely used disaster databases: the Emergency Events Database (EM-DAT) and its geocoded version (GDIS), as well as the DesInventar database. The analysis focuses on the period from 1960 to 2018, aligning with GDIS temporal coverage. We define concurrent or sequential hazards as instances where a flood occurs during a drought period or within four months following a drought.  


Our findings for the global extratropics reveal that the economic losses and the number of affected people resulting from the identified drought-flood events are two to eight times higher than those ascribed to isolated droughts or floods, with a confidence interval ranging from two to twelve. Specifically, in DesInventar, the impact ratio (the mean impact of concurrent or sequential events divided by the mean impact of isolated events) for indirectly affected individuals and financial losses is approximately three. In EM-DAT, the impact ratio reaches three for economic damages and eight for affected individuals. Furthermore, the impact ratios are notably higher in the last 30 years of the study period compared to earlier decades, emphasizing the increasing severity of the drought-flood compound events.


These results highlight the amplified negative impacts when droughts and floods occur concomitantly or sequentially, highlighting the need for more robust policies to address their socio-economic risks, particularly under changing climatic conditions.

How to cite: Worou, K. and Messori, G.: Amplified Socio-Economic Impacts of Concurrent or Sequential Drought-Flood Events: Insights from Disaster Databases (1960–2018), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8719, https://doi.org/10.5194/egusphere-egu25-8719, 2025.

EGU25-10235 | ECS | Orals | NP1.3

Assessing the impact of climate change on wildfire development: insights from analogues and regional climate models 

Chen Lu, Rita Nogherotto, Tommaso Alberti, Gabriele Messori, Erika Coppola, and Davide Faranda

Climate change is an ongoing process that is modifying weather patterns and influencing weather phenomena and extreme events such as heatwaves, droughts, and floods. In this study, we investigate whether climate change can also play a role in enhancing wildfires by focusing on a set of three recent wildfires in Europe (i.e., events occurred in Central Sweden in July 2018, France in July 2022, and in Sicily and Greece in July 2023). We employ the concept of analogues to assess the influence of climate change on the atmospheric conditions underlying wildfire development monitored through the fire weather index, by comparing past and present atmospheric patterns similar to those that occurred during the wildfire. Our analysis focuses on both reanalysis data and high-resolution regional climate models to attribute the observed changes and provide future projections. Our findings show that climate change has altered critical factors supporting wildfire development, such as temperature, humidity, and wind patterns. The results from our sample of three events point out that climate change has increased wildfire hazards in Europe, which is projected to further increase for similar fire weather conditions in the future.

How to cite: Lu, C., Nogherotto, R., Alberti, T., Messori, G., Coppola, E., and Faranda, D.: Assessing the impact of climate change on wildfire development: insights from analogues and regional climate models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10235, https://doi.org/10.5194/egusphere-egu25-10235, 2025.

EGU25-10570 | Posters on site | NP1.3

VORTEX project: The role of the polar vortex on the predictabIlity of extreme events in the Northern Hemisphere 

Carmen Alvarez-Castro, Cristina Peña-Ortiz, David Gallego, and Davide Faranda

Extreme weather and climate events, marked by unexpected and severe conditions at the edges of historical distributions, significantly impact human health, society, and ecosystems. With global warming driving an increase in the frequency and intensity of these extremes, there is an urgent need to enhance weather prediction beyond the typical 7–10-day range. Among the atmospheric and oceanic components studied for improving predictability, the stratosphere stands out due to its slower and more predictable changes, which can have persistent impacts on surface weather patterns.

Research has highlighted the stratosphere's role in driving weather and climate extremes, particularly in the extratropical Northern Hemisphere. Events involving a weak or strong stratospheric polar vortex can precede the occurrence of surface extremes, making the polar vortex a key link between stratospheric variability and surface climate predictability. While various studies have previously identified this teleconnection, the processes connecting anomalous vortex states to extreme surface events are not yet fully understood.

In VORTEX project we employ a methodology based on advancements in dynamical systems theory to explore the relationship between anomalous polar vortex states and extreme precipitation and temperature events. This approach characterizes each vortex-extreme event's recurrence, persistence, and predictability, providing dynamic insights that traditional methods cannot. By identifying the intrinsic predictability of stratospheric patterns tied to extremes, this methodology offers a pathway to improve sub-seasonal to seasonal climate models, focusing future efforts on better representing critical patterns that influence extreme weather.

How to cite: Alvarez-Castro, C., Peña-Ortiz, C., Gallego, D., and Faranda, D.: VORTEX project: The role of the polar vortex on the predictabIlity of extreme events in the Northern Hemisphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10570, https://doi.org/10.5194/egusphere-egu25-10570, 2025.

EGU25-10822 | ECS | Orals | NP1.3

Exploring a new methodology to quantify natural variability in conditional extreme event attribution 

Clara Naldesi, Mathieu Vrac, Nathalie Bertrand, and Davide Faranda

Anthropogenic climate change (ACC) is one of the most demanding challenges facing our society. The intensification and increased frequency of many extreme events due to ACC are among its most impactful consequences, threatening human health, infrastructure, and ecosystems. In this context, raising the awareness of the general public of the relationship between ACC, extremes, and associated impacts becomes a crucial task.

This work is grounded in attribution science and focuses on quantifying and understanding the influence of internal climate variability on extreme events. Among the many tools available for attribution, we use ClimaMeter [Faranda et al. 2023], a rapid framework designed to provide context for extreme events in relation to ACC. ClimaMeter’s approach emphasizes the dynamics associated with extreme events and identifies weather conditions similar to those characterizing the event of interest, leveraging the analogues methodology for conditional attribution [Yiou, 2014]. The analysis provided by such a framework enables the evaluation of significant changes over time of the event’s dynamics and associated meteorological hazards and links them to ACC.

An essential part of ClimaMeter’s methodology is quantifying the influence of natural variability relative to ACC in explaining the changes associated with the event. Specifically, three modes of Sea Surface Temperature variability are taken into account: the El Niño-Southern Oscillation, the Atlantic Multidecadal Oscillation and the Pacific Decadal Oscillation. These three modes are considered with equal weight and changes not explained by them are assumed to be due to ACC [Faranda et al., 2023]. While the methodology is rapid and easy to communicate, it also has some limitations. In this work, we investigate the implications of this approach. First, we test it on a pre-industrial simulation of the IPSL climate model to evaluate its performance under stationary climate conditions. Additionally, we explore a generalization of the current methodology, aiming to refine the quantification of natural variability by weighing the three modes based on the event region and associated hazard. This generalized approach has the potential to expand ClimaMeter’s methodology and provide new insights into the complex mechanisms linking natural variability and extremes.

How to cite: Naldesi, C., Vrac, M., Bertrand, N., and Faranda, D.: Exploring a new methodology to quantify natural variability in conditional extreme event attribution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10822, https://doi.org/10.5194/egusphere-egu25-10822, 2025.

EGU25-10966 | ECS | Posters on site | NP1.3

Winter cyclones drive stronger surface wind extremes in the North Atlantic than in the Southern Ocean 

Aleksa Stanković and Rodrigo Caballero

Hemispheric symmetries, including those in zonal-mean eddy kinetic energy and in hemispheric-mean planetary albedo, are a characteristic feature of Earth’s climate. Whether such a symmetry also holds for extreme surface windspeeds driven by midlatitude cyclones is currently unclear. We address this question by focusing on the regions with the peak of storm tracks over the North Atlantic, North Pacific and Southern Ocean. We analyse reanalysis and satellite datasets and employ objectively calculated storm tracks to associate cyclones with surface winds they produce. Additionally, we check for existence of trends in extreme windspeeds of each basin. Results show a statistically distinguishable hemispheric asymmetry in extreme surface windspeeds, with the North Hemisphere having stronger extremes, driven primarily by extreme windspeeds occurring during winter and in proximity to cyclones. This implies that cyclones in the North Hemisphere drive stronger surface windspeed extremes than in the South Hemisphere. The North Hemisphere also has higher extreme windspeeds above the boundary layer (700 hPa), pointing to the role of large-scale processes in driving these differences. Lastly, trends in the extreme surface windspeeds across all basins are positive in the reanalysis dataset, and statistically significant in the North Pacific and Southern Ocean.

How to cite: Stanković, A. and Caballero, R.: Winter cyclones drive stronger surface wind extremes in the North Atlantic than in the Southern Ocean, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10966, https://doi.org/10.5194/egusphere-egu25-10966, 2025.

EGU25-12284 | ECS | Orals | NP1.3

Comparative predictability of eastern and western north pacific blocking events 

Anupama K Xavier, Oisín Hamilton, Davide Faranda, and Stéphane Vannitsem

North Pacific blocking patterns, defined by persistent high-pressure systems that disrupt atmospheric circulation, are pivotal elements of mid-latitude weather dynamics. These blocking events play a significant role in shaping regional weather extremes, such as prolonged cold spells or heatwaves, and can redirect storm tracks across the Pacific. For instance, the 2021 Pacific Northwest heatwave demonstrated the profound impact of blocking on terrestrial temperatures, where an upstream cyclone acted as a diabatic source of wave activity, intensifying the blocking system. This led to heat-trapping stable stratification, which elevated surface temperatures to unprecedented levels (Neal et al., 2022). Similarly, marine heatwaves in the Northeast Pacific have been linked to high-latitude blocking events, which weaken westerly winds, suppress southward Ekman transport, and enhance ocean stratification, thereby increasing sea surface temperatures (Niu et al., 2023). The predictability of North Pacific blocking events is governed by the intricate interplay of large-scale atmospheric dynamics, ocean-atmosphere interactions, and internal variability (Smith et al., 2020).

This study investigates the differences in predictability between eastern and western North Pacific blocking events, using a modified version of the Davini et al. (2012) blocking index to distinguish their geographical locations. Identified blocking events were tracked using a block-tracking algorithm until they dissipated. Predictability was assessed by identifying an analogue pair for each blocking event. Specifically, after classifying blocks as eastern or western, geopotential height maps for each event were compared to all other days in the dataset. The analogue pair for an event was defined as the day with the smallest root mean square (RMS) distance. Predictability was then evaluated by averaging the error evolution of the tracks between events in each analogue pair.

Using CMIP6 model simulations and ERA5 reanalysis data, the study revealed that eastern blocks are significantly more persistent and stable than their western counterparts. Eastern blocks exhibited longer durations and greater resistance to atmospheric variability, resulting in improved forecast accuracy. In contrast, western blocks were found to be more transient and challenging to predict due to their susceptibility to dynamic instabilities.

References

Davini, P., Cagnazzo, C., Gualdi, S. and Navarra, A., 2012. Bidimensional diagnostics, variability, and trends of Northern Hemisphere blocking. Journal of Climate, 25(19), pp.6496-6509.

Neal, E., Huang, C.S. and Nakamura, N., 2022. The 2021 Pacific Northwest heat wave and associated blocking: Meteorology and the role of an upstream cyclone as a diabatic source of wave activity. Geophysical Research Letters, 49(8), p.e2021GL097699.

Niu, X., Chen, Y. and Le, C., 2023. Northeast Pacific marine heatwaves associated with high-latitude atmospheric blocking. Environmental Research Letters, 19(1), p.014025.

How to cite: K Xavier, A., Hamilton, O., Faranda, D., and Vannitsem, S.: Comparative predictability of eastern and western north pacific blocking events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12284, https://doi.org/10.5194/egusphere-egu25-12284, 2025.

EGU25-13213 | ECS | Orals | NP1.3

Sensitivity of Dynamical Coupling to Large-Scale Circulation in European Winter Extremes 

Ane Carina Reiter, Martin Drews, Gabriele Messori, Davide Faranda, and Morten Andreas Dahl Larsen

The physical mechanisms underlying climate-induced extreme events are inherently complex, arising from the compounding nature of multiple drivers and/or hazards. Leveraging the chaotic nature of the atmosphere, a novel approach, based on results from dynamical system theory, has recently been adopted to reveal the drivers of both individual and compound extremes. Central to this approach is the co-recurrence ratio, which quantifies the instantaneous dynamical coupling between multiple variables in terms of joint recurrences of atmospheric configurations to similar ones in the past.

While the co-recurrence ratio has demonstrated potential in revealing the atmospheric drivers of certain extremes, its performance may depend heavily on factors such as the choice of geographical domain(s), selection of variables, and the thresholds used to define extremes. These sensitivities remain underexplored, limiting the broader applicability of this approach.

In this study, we aim to address these gaps by assessing the sensitivity of the co-recurrence ratio in a European setting, focusing on daily winter extremes in temperature, wind, and precipitation. For this analysis, we adopt a bivariate focus, diagnosing the coupling between large-scale circulation patterns and single hazard variables.

By exploring these sensitivities, this work seeks to enhance the understanding of the robustness of the co-recurrence ratio and its effectiveness in diagnosing the atmospheric drivers of various types of extremes.

How to cite: Reiter, A. C., Drews, M., Messori, G., Faranda, D., and Dahl Larsen, M. A.: Sensitivity of Dynamical Coupling to Large-Scale Circulation in European Winter Extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13213, https://doi.org/10.5194/egusphere-egu25-13213, 2025.

EGU25-13374 | ECS | Posters on site | NP1.3

Causality and predictability of the Pan Atlantic compound extremes 

Meriem Krouma and Gabriele Messori

The co-occurrence of wintertime cold spells in North America and wet, windy extremes in Europe, known as the Pan-Atlantic compound extremes, is linked to distinct dynamical pathways. One of those dynamical pathways involves the presence of a persistent high-pressure system west of Greenland. This high-pressure anomaly tends to simultaneously induce a southward displacement of a trough over the eastern United States and sustain an upper-level trough over southwestern Europe, creating conditions that induce both cold spells in North America and extreme precipitation in Europe. The co-occurrence of the Pan-Atlantic compound extremes has been investigated in previous studies. However, the causal association between extremes on both sides of the Atlantic has yet to be verified. In this study, we aim to assess the relationship between these compound extremes and to uncover the causal mechanisms driving their co-occurrence. Preliminary findings indicate that high-pressure anomalies over Greenland are a main driver of both phenomena, providing a coherent dynamical link that bridges these geographically distinct extreme events. The study further seeks to clarify the underlying dynamics and improve predictability for such interconnected extreme weather events, which can help to better manage and mitigate their impacts.

How to cite: Krouma, M. and Messori, G.: Causality and predictability of the Pan Atlantic compound extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13374, https://doi.org/10.5194/egusphere-egu25-13374, 2025.

EGU25-13784 | ECS | Orals | NP1.3

RHITA: a framework for real-time detection and characterization of weather extremes 

Greta Cazzaniga, Adrien Burq, Mathieu Vrac, and Davide Faranda

Extreme weather events such as heatwaves, droughts, thunderstorms, and cyclones threaten human lives, ecosystems, and economic stability. Tracking and characterizing the spatiotemporal dynamics of such events is essential for understanding their cascading impacts on socioeconomic and environmental systems. When the detection and characterization of extremes are done in real-time, they can provide critical information that benefits many sectors, including agriculture, emergency management, and regulatory authorities.

To offer a tool for operational monitoring of weather-related hazards across Europe, we developed RHITA (Real-time Hazards Identification and Tracking Algorithm), an online framework designed for the rapid, automated, and objective spatiotemporal detection of hazards driven by extreme weather events. RHITA is intended for a wide range of users, including scientists, policymakers, authorities, and the general public. It leverages the ERA5 dataset for real-time detection, and the algorithm is calibrated using the EM-DAT dataset, which documents global disaster occurrences and impacts.

RHITA currently offers two main features: (1) real-time tracking and spatiotemporal characterization of extreme weather events such as heatwaves, droughts, cold spells, cyclones, and storms, focusing on associated hazards like extreme temperatures, water deficits, heavy precipitation, and strong winds; and (2) publicly available, up-to-date, transboundary historical spatiotemporal hazard catalogs for Europe.

How to cite: Cazzaniga, G., Burq, A., Vrac, M., and Faranda, D.: RHITA: a framework for real-time detection and characterization of weather extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13784, https://doi.org/10.5194/egusphere-egu25-13784, 2025.

EGU25-13891 | Posters on site | NP1.3

Ensemble Random Forest for Tropical Cyclone Tracking 

Pradeebane Vaittinada Ayar, Stella Bourdin, Davide Faranda, and Mathieu Vrac


Even though tropical cyclones (TCs) are well documented from the moment they reach a certain intensity to the moment they start to evanesce, many physical and statistical properties governing them are not well captured by gridded reanalysis or simulated by earth system models. Thus, the tracking of TCs remain a matter of interest for the investigation of observed and simulated tropical. Many cyclone tracking schemes are available. On the one hand, there are trackers that rely on physical and dynamical properties of the TCs and users prescribed thresholds, which make them rigid, and need numerous variables that are not always available in the models. On the other hand, there are trackers leaning on deep learning which, by nature, need large amounts of data and computing power. Besides, given the number of physical variables needed for the tracking, they can be prone to overfitting, which hinders their transferability to climate models. In this study, the ability of a Random Forest (RF) approach to track TCs with a limited number of aggregated variables is explored. Hence, it becomes a binary supervised classification problem of TC-free (zero) and TC (one) situations. Our analysis focuses on the Eastern North Pacific and North Atlantic basins, for which respectively 514 and 431 observed tropical cyclones tracks record are available from the IBTrACS database over the 1980-2021 period. For each 6-hourly time step, RF associates TC occurrence or absence (1 or 0) to atmospheric situations described by predictors extracted from the ERA5 reanalysis. Then situations with TC occurrences are joined for reconstructing TC trajectories. Results show good ability of the method for tracking of tropical cyclones over both basins and good ability for spatial and temporal generalization as well. It also shows similar TC detection rate as trackers based on TCs' properties and significantly lower false alarm rate. RF allows us to detect TC situations for a range of predictor combinations, which brings more flexibility than threshold based trackers. Last but not least, this study shed light on the most relevant variables allowing to detect tropical cyclone.

How to cite: Vaittinada Ayar, P., Bourdin, S., Faranda, D., and Vrac, M.: Ensemble Random Forest for Tropical Cyclone Tracking, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13891, https://doi.org/10.5194/egusphere-egu25-13891, 2025.

EGU25-14873 | ECS | Orals | NP1.3

Large-scale atmospheric circulation as a source of uncertainty in western European heat extreme projections  

Shutong Liu, Yinglin Tian, and Kai Kornhuber

Europe has been identified as a heatwave hotspot, where heatwave intensities have outpaced other mid-latitude regions in the Northern Hemisphere (Rousi et al. Nat. Comms. 2022). Accelerated European heatwave trends have been found to be associated with the increased persistence of Eurasian double jets, a specific set-up of the large-scale circulation in which the Northern hemisphere polar and subtropical jets occur as two clearly separated branches. However, if observed trends are projected to continue with anthropogenic warming and to what degree the present generation of climate models constitute useful tools to assess changes in the atmospheric circulation has not yet been ascertained.

In this study, we benchmark 11 CMIP6 climate models to evaluate their ability to reproduce the main characteristics of double jets and their relationship to heat extremes, aiming to identify the best-performing models for future projections. Our findings show that, on average, the models tend to underestimate the frequency of double jets by 80%. Moreover, half of the climate models underestimate the intensity of double-jet-associated heatwaves over Western Europe, with the remaining models even showing a negative anomaly in heatwave intensity during double jet events in the region. Furthermore, climate models fail to capture the growth rate of double jet persistence, with the model mean trend at -0.4 days per decade, while the observed rate is approximately 1.5 days per decade. The bias in the persistence trend of double jet in models is strongly correlated with the underestimation of the western European heat extreme trend, with an R2 value of 0.42.

Despite this, some models show reasonable agreement with the observations, and these models are further analyzed to project circulation-driven changes in extreme heat. Using EC-Earth3-Veg-LR, we observe an increase in double jet frequency from 2020 to 2060, at a rate of 0.2 days per decade. Our work highlights the need for better representation of double jet characteristics and their relationship with heat extremes in climate models to enhance preparedness for future heat risks.

How to cite: Liu, S., Tian, Y., and Kornhuber, K.: Large-scale atmospheric circulation as a source of uncertainty in western European heat extreme projections , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14873, https://doi.org/10.5194/egusphere-egu25-14873, 2025.

EGU25-15668 | ECS | Posters on site | NP1.3

High-risk atmospheric circulation patterns for Italian precipitation extremes 

Cristina Iacomino, Salvatore Pascale, Giuseppe Zappa, Marcello Iotti, Federico Grazzini, Alice Portal, and Paolo Ghinassi

Extreme precipitation events (EPEs) are meteorological phenomena that are likely to intensify as a result of climate change. They are a major concern for our society, especially in densely populated areas, as they can have significant economic and environmental impacts. Therefore, identifying large-scale atmospheric circulation that lead to EPEs is crucial for detecting geographical areas at risk and mitigating their adverse impacts.

To achieve this objective, we study the circulation patterns associated with EPEs in Italy. Initially, we focus on North-Central Italy and we identify the precipitation extremes in three datasets: ARCIS 3.0, MSWEP, and CERRA LAND. Circulation types associated with the EPEs are obtained by applying Self Organizing Maps (SOMs), an unsupervised artificial neural network widely used in synoptic climatology, to anomalies of geopotential height at 500 hPa and mean sea level pressure. Since ArCIS, the reference dataset, is limited to North-Central Italy, we extend the analysis to the whole of Italy using CERRA-Land. Such choice is based on the fact that it produced the most similar results to ArCIS in North-Central Italy compared to MSWEP.

We then generate composites of various variables (all retrieved from ERA5) for each SOM pattern to better understand the circulation patterns and characterize the atmospheric dynamics associated with extreme events. Additionally, we analyze the probability of exceeding the 99th percentile of wet-days to identify the areas impacted by each pattern. Composites for the different circulation types show variations in the synoptic pattern's position within the Mediterranean basin, as well as differences in the direction and intensity of moisture flux. These patterns influence distinct regions and display varying frequencies across seasons.

In future works the classification obtained by this study will be applied to climate model simulations, aiming to investigate the role of anthropogenic climate change in the dynamics leading to EPEs in Italy. 

How to cite: Iacomino, C., Pascale, S., Zappa, G., Iotti, M., Grazzini, F., Portal, A., and Ghinassi, P.: High-risk atmospheric circulation patterns for Italian precipitation extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15668, https://doi.org/10.5194/egusphere-egu25-15668, 2025.

EGU25-17645 | Orals | NP1.3

Graph neural networks based climate emulator for kilometer scale hourly precipitation : a novel hybrid imperfect approach 

Erika Coppola, Valentina Blasone, Serafina Di Gioia, Guido Sanguinetti, Viplove Arora, and Luca Bortolussi

Regional climate emulators provide computationally efficient tools for generating high-resolution climate projections, bridging the gap between coarse-scale models and the detailed resolution required for local-scale hazard assessments. Climate hazards from extreme precipitation events are projected to increase in frequency and intensity under global warming, emphasizing the need for accurate modeling of convective processes. However, traditional numerical methods are constrained by low resolution or the high computational costs of kilometer-scale simulations.

To overcome these limitations, we introduce GNN4CD, a novel deep learning emulator that estimates kilometer-scale (3 km) hourly precipitation from coarse atmospheric data (~25 km). The model leverages graph neural networks and a hybrid imperfect approach (HIA) for downscaling, initially trained on ERA5 reanalysis and observational data, and applied using regional climate model (RegCM) data for present-day and future projections.

GNN4CD demonstrates exceptional performance in reproducing precipitation distributions, seasonal diurnal cycles, and extreme percentiles across Italy, even when trained on northern Italy alone. The model captures shifts in precipitation distributions, particularly for extremes, across historical, mid-century, and end-of-century scenarios. Additionally, evaluations using an ensemble of convection-permitting regional models confirm GNN4CD's ability to replicate ensemble spreads for both present-day and future projections essential for estimating the uncertainty in the future climate change signal..

How to cite: Coppola, E., Blasone, V., Di Gioia, S., Sanguinetti, G., Arora, V., and Bortolussi, L.: Graph neural networks based climate emulator for kilometer scale hourly precipitation : a novel hybrid imperfect approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17645, https://doi.org/10.5194/egusphere-egu25-17645, 2025.

EGU25-17852 | ECS | Posters on site | NP1.3

The impact of the upward trend in the NAO index on precipitation dynamics in the Mediterranean region 

Emma Schultz, Barend Spanjers, and Dim Coumou

The North Atlantic Oscillation (NAO) is the dominant pattern of atmospheric variability over the North Atlantic region, having its greatest influence on Europe during the winter months. In winter, positive NAO index values are linked to warmer temperatures and increased precipitation in western and northern Europe, whereas southern Europe tends to experience colder and drier conditions. These drier conditions can pose significant challenges for agriculture and livelihoods. An overall positive trend in the NAO index has been observed in winter in recent decades. However, how precipitation dynamics in the Mediterranean region respond to the shift towards a higher NAO index are largely unknown, partly due to the poor capture of NAO’s upward shift in climate models. 

Here we examine the impact of the shift towards a higher NAO index on precipitation dynamics in the Mediterranean region in winter. We employ a novel statistical model to analyse next-day precipitation conditional on past observations. The analysis focuses on conditioning drought persistence on different NAO states to assess their influence on the distributional characteristics of drought durations across the Mediterranean region. We present preliminary analyses that contribute to the growing body of evidence that long-term positive trends in the NAO index have an impact on rainfall patterns and drought occurrence in Europe. Understanding the role of teleconnections in regional climate variability and long-term trends is essential for robust regional climate projections for improved risk assessment and policy planning.

How to cite: Schultz, E., Spanjers, B., and Coumou, D.: The impact of the upward trend in the NAO index on precipitation dynamics in the Mediterranean region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17852, https://doi.org/10.5194/egusphere-egu25-17852, 2025.

EGU25-17937 | ECS | Orals | NP1.3

Impact Attribution for Climate Law: The Case of Storm Irene 

Mireia Ginesta, Shirin Ermis, Rupert Stuart-Smith, and Benjamin Franta

People are increasingly turning to courts to combat climate crisis. In the early 2000s, fewer than 10 climate change litigation cases had been filed globally. By 2024, this number has grown to over 2,500, with more than half originating in the United States. Some of these cases rely on extreme weather attribution science to link damages to anthropogenic climate change. Developing rigorous, legally useful assessments of damage attributable to climate change is an increasingly pressing need.

We present a framework for forecast-based impact attribution which can link physically consistent hazards to impacts, providing evidence for legal cases and climate cost recovery laws. As a case study, we analyze the severe impacts of Storm Irene in August 2011 when it was undergoing extratropical transition in the north-eastern USA. In the state of Vermont, Irene caused rainfall of up to 180 mm within a few hours, leading to fluvial and pluvial flooding with catastrophic consequences that caused $850 million in economic damages. By integrating an operational weather forecast model (ECMWF’s IFS) and hydrological models with economic impact assessments, we assess the extent to which these damages can be attributed to anthropogenic climate change.

This research underscores the potential of interdisciplinary attribution methodologies to enhance the scientific basis for judicial adjudication on climate change and climate law-making.

How to cite: Ginesta, M., Ermis, S., Stuart-Smith, R., and Franta, B.: Impact Attribution for Climate Law: The Case of Storm Irene, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17937, https://doi.org/10.5194/egusphere-egu25-17937, 2025.

EGU25-17947 | Orals | NP1.3

Towards an impact-based approach to the detection of analogues: the case study of Emilia-Romagna floods in May 2023 

Valerio Lembo, Mireia Ginesta, Tommaso Alberti, Roberta D'Agostino, and Davide Faranda

The framework of weather analogues is a powerful methodology for the detection of the climate change fingerprint on weather extremes, that has been widely used in several contexts. The procedure has several advantages compared to standard model-based attribution exercises, being fast and not computationally expensive. Here we address whether the detection of analogs based on impacts (e.g., environmental, socio-economic) of a severe weather event can provide added value on the attribution of the event intensity or likelihood to climate change.

As a case study, we analyse the twin Emilia-Romagna flood event of May 2023. It caused a sizable amount of casualties, widespread destruction and substantial economic damage. We detect analogues of the river runoff as an impact-based observable of interest, addressing it in an univariate context, but also jointly with other observables (i.e., in a multivariate framework), such as mean sea-level pressure, total precipitation, and 850 hPa vorticity. We therefore detect the optimal set of variables for performing multivariate analysis and the appropriate analysis domain. We suggest that by combining river runoff with other observables by carefully selecting the spatial domain, we obtain a clearer view of the role played by anthropogenic climate change for this event, also including the additional vulnerability linked to the environmental impact of human activities, such as land-use change and freshwater diversion.

How to cite: Lembo, V., Ginesta, M., Alberti, T., D'Agostino, R., and Faranda, D.: Towards an impact-based approach to the detection of analogues: the case study of Emilia-Romagna floods in May 2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17947, https://doi.org/10.5194/egusphere-egu25-17947, 2025.

EGU25-18710 | Orals | NP1.3

The predictable chaos of rare events in geophysical and complex systems 

Tommaso Alberti, Davide Faranda, and Valerio Lucarini

Many natural systems show emergent phenomena at different scales, leading to scaling regimes with signatures of chaos at large scales and an apparently random behavior at small scales. These features are usually investigated quantitatively by studying the properties of the underlying attractor. This multi-scale nature of natural systems makes it practically impossible to get a clear picture of the attracting set as it spans over a wide range of spatial scales and may even change in time due to non-stationary forcing.

Here we present a review of some recent advancements in characterizing the number of degrees of freedom and the predictability horizon of geophysical and complex systems showing non-hyperbolic chaos, randomness, state-dependent persistence and predictability. We compare classical approaches, based on Lyapunov exponents and correlation dimension, with novel approaches based on combining adaptive decomposition methods with concepts from extreme value theory. We demonstrate that the properties of the invariant set depend on the scale we are focusing on and that the proposed formalism can be generally helpful to investigate the role of multi-scale fluctuations within complex systems, allowing us to deal with the problem of characterizing the role of stochastic fluctuations across a wide range of physical systems as well as the role of different dynamical components in determining the predictability of rare events in complex systems.

How to cite: Alberti, T., Faranda, D., and Lucarini, V.: The predictable chaos of rare events in geophysical and complex systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18710, https://doi.org/10.5194/egusphere-egu25-18710, 2025.

EGU25-18740 | ECS | Orals | NP1.3

Analyzing the Historical and Projected Evolution of the Global Diurnal Temperature Range (DTR) 

Muskula Sai Bargav Reddy, Vinnarasi Rajendran, and Mukul Tewari

The Diurnal Temperature Range (DTR) serves as a crucial meteorological indicator, reflecting the difference between daily maximum and minimum temperatures and the magnitude of diurnal extremes. The anomalous values of DTR are often linked to the occurrence of various climatic extremes such as droughts, heatwaves, and wet spells, which make it necessary to understand the evolution of DTR both historically and for the future. This study focuses on analyzing the evolution of DTR globally by employing the non-stationary Multidimensional Ensemble Empirical Mode Decomposition (MEEMD) method. To accomplish this, historical temperature data spanning 69 years (1951-2019) and CMIP6 Bias corrected data covering 150 years (1951-2100) were utilized. The non-linear trend characteristics in temperature are computed using CRU 0.50 x 0.50 gridded temperature data for historical trends and five different bias-corrected climate projection datasets of NASA Earth Exchange Global Daily Downscaled Projections (NEX-GDDP-CMIP6) for the assessment of trends in future DTR by considering two SSP scenarios, i.e., SSP 245 and SSP 585, each corresponding to intermediate and high emissions scenarios. The CMIP6 models that are considered are CanESM5, GFDL CM4, MIROC6, NorESM2-MM, and MPI-ESM1-2-HR. The results from the analysis reveal the decrease in global DTR, with a faster rate of increase in minimum temperature than in maximum temperature. However, the southern regions of Australia and Africa showed an increase in DTR. The CMIP6 simulations showed that CanESM5 and MPI-ESM1-2-HR showed a decreasing trend in global DTR for both scenarios of ssp, with an increase in DTR for South America and the southern part of Africa for CanESM5, while GFDL CM4, MIROC6, and NorESM2-MM showed a decrease in global DTR. The findings underscore the importance of understanding regional climatic variations when assessing global temperature trends. The observed contrasting regional patterns in DTR highlight the influence of localized hydroclimatic factors, including land-use changes, aerosols, and atmospheric feedback mechanisms. These insights are crucial for refining climate models and improving future climate projections under different emission pathways. Overall, the study emphasizes the necessity of incorporating non-linear approaches like MEEMD to capture complex climatic trends and underscores the role of DTR as a key indicator of climate change and its impacts at both global and regional scales.

How to cite: Reddy, M. S. B., Rajendran, V., and Tewari, M.: Analyzing the Historical and Projected Evolution of the Global Diurnal Temperature Range (DTR), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18740, https://doi.org/10.5194/egusphere-egu25-18740, 2025.

EGU25-19577 * | Orals | NP1.3 | Highlight

Unraveling the Rising Threat of Atmospheric and Marine Heatwaves in the Mediterranean Region 

Samira Khodayar Pardo, Paco Pastor, and Laura Paredes-Fortuny

Heatwaves (HWs) are extreme climate events increasingly magnified under climate change, posing significant risks to both human and environmental systems. The Mediterranean region, recognized as a climate change hotspot, is experiencing a worrying amplification of both atmospheric and marine heatwaves. In this presentation we will discuss the evolution and interplay of these phenomena emphasizing their compounding effects when occurring simultaneously.

Our findings reveal a clear increase in HW frequency, intensity, and duration, with the concurrence of atmospheric and marine heatwaves resulting in a significant local amplification of marine heatwave intensity. While atmospheric heatwaves remain largely unaffected by this interaction. This interaction has become more prominent in recent years, highlighting the increasing complexity of extreme climate phenomena in this region.

The results underscore the urgent need for regionally tailored strategies to mitigate the cascading impacts of compounding heatwaves, as their intensification under climate change exacerbates threats to Mediterranean ecosystems and communities.

 

How to cite: Khodayar Pardo, S., Pastor, P., and Paredes-Fortuny, L.: Unraveling the Rising Threat of Atmospheric and Marine Heatwaves in the Mediterranean Region, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19577, https://doi.org/10.5194/egusphere-egu25-19577, 2025.

EGU25-19698 | Orals | NP1.3

 January 2025 Wildfires in Southern California are attributable to Anthropogenic Global Warming 

Rita Nogherotto, Chen Lu, Greta Cazzaniga, Coppola Erika, and Davide Faranda

Starting January 7, 2025, devastating wildfires have swept through the Los Angeles metropolitan area and nearby regions. By January 10, the fires had caused ten deaths, destroyed thousands of structures, displaced nearly 180,000 residents, and scorched approximately 30,000 acres. This study employs the extended ClimaMeter (climameter.org <http://climameter.org/>) protocol to explore the potential role of climate change in exacerbating the severity of this event. Specifically, we examine whether climate change has modified the atmospheric conditions, represented by the mean sea level pressure, that contribute to wildfire occurrence, represented by the fire weather index, by analyzing historical and current weather patterns similar to those observed during the fires. Our methodology integrates both reanalysis datasets and high-resolution regional climate models to assess observed changes and project future fire risk scenarios. The results indicate a significant increase in the fire weather index across much of California and surrounding regions, which suggests that this event can be ascribed to human-driven climate change. The models show a similar signal in the present climate and project increases in fire weather hazard in the future.

How to cite: Nogherotto, R., Lu, C., Cazzaniga, G., Erika, C., and Faranda, D.:  January 2025 Wildfires in Southern California are attributable to Anthropogenic Global Warming, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19698, https://doi.org/10.5194/egusphere-egu25-19698, 2025.

EGU25-20545 | ECS | Orals | NP1.3

Characterizing ENSO Through Topological Analysis of Jin-Timmermann Model's Chaotic Regimes 

Maria Sanchez Muniz, Margaret Brown, and Pushpi Paranamana

The El Niño-Southern Oscillation (ENSO) represents one of the most significant drivers of global climate variability. This study investigates the chaotic parameter regimes of the Jin-Timmermann model, particularly focusing on the dynamics identified by Guckenheimer et al. where chaotic attractors emerge. We analyze the reduced three-dimensional system with specific attention to the critical parameters δ = 0.225423, ρ = 0.3224, which govern the time-scale interactions between oceanic and atmospheric processes. Using topological data analysis (TDA), we characterize the structural transitions between periodic and chaotic behaviors in the model's parameter space. Our methodology combines persistent homology with dynamical systems theory to identify distinct topological signatures associated with strong El Niño events. We validate these theoretical findings against observational data from the ERA5 reanalysis and NOAA/ERSSTv5 Niño 3.4 index, focusing particularly on the relationship between topological features and prolonged dry conditions in Southeast Asia. This approach provides new insights into the non-systematic relationship between strong El Niño events and regional climate impacts, while establishing a novel framework for comparing theoretical models with observational data. Our results demonstrate the utility of topological methods in understanding complex climate phenomena and suggest new possibilities for improving ENSO prediction capabilities.

How to cite: Sanchez Muniz, M., Brown, M., and Paranamana, P.: Characterizing ENSO Through Topological Analysis of Jin-Timmermann Model's Chaotic Regimes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20545, https://doi.org/10.5194/egusphere-egu25-20545, 2025.

Extreme rainfall events during the Indian monsoon season pose significant challenges due to their socioeconomic and environmental impacts. Understanding the spatial and temporal dynamics of these events requires robust analytical and statistical methods capable of capturing complex relationships within rainfall generating systems. Complex network approaches have emerged as powerful tools for analyzing spatiotemporal patterns in climate data, offering new insights into extreme weather phenomena.

This study compares two methodologies for constructing and analyzing climate networks to study the spatiotemporal structure and dynamics of heavy precipitation events in India during the monsoon season across multiple time scales. Specifically, we introduce a novel combination of Discrete Wavelet Decomposition with Event Coincidence Analysis (ECA), referred to as Multi-Scale Event Coincidence Analysis (MSECA) and compare the results with the existing Multi-Scale Event Synchronisation (MSES). From a conceptual perspective, MSECA appears to be a more reasonable method compared to MSES, as it mitigates certain undesired effects of temporal clustering of rainfall extremes across various timescales.

Our results reveal distinct differences in network properties depending on the methodology used, highlighting the sensitivity of network-based analyses to the choice of construction technique. These differences affect the identification of dominant heavy rainfall patterns and their underlying drivers, such as large-scale atmospheric circulation and/or local feedback mechanisms at daily to monthly temporal scales.

Our work underscores the importance of methodological rigor and the potential of complex network approaches in advancing the understanding of extreme rainfall events in monsoon-dominated regions. This comparison provides a foundation for developing standardized practices for network-based climate studies, enabling more robust assessments of extreme weather phenomena.

How to cite: Bishnoi, G., Dhanya, C. T., and Donner, R. V.: A Comparison of Methodologies for Studying Heavy Precipitation Events during the Summer Monsoon Season in India Using Complex Network Approaches, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21222, https://doi.org/10.5194/egusphere-egu25-21222, 2025.

AS5 – Methods and Techniques

EGU25-2059 | ECS | Orals | CL4.7

Coupling techniques in the new high resolution SHiELD + MOM6 model for extreme weather prediction 

Joseph Mouallem, Kun Gao, Lauren Chilutti, Brandon Reichl, Lucas Harris, Rusty Benson, Niki Zadeh, and Cheng Zhang

We present a new model that couples GFDL’s FV3-based weather model SHiELD, GFDL’s ocean model MOM6, and NCEP’s wave model WAVEWATCH III. This model is specifically designed for high-resolution simulations of air-sea interactions during extreme coastal weather events. It aims to address the critical need for accurate representation of fine-scale processes in air-sea interactions, which are not resolved in current-generation global  models. By combining SHiELD, MOM6, and WAVEWATCH III, we seek to capture the complex dynamics of atmosphere, ocean, and wave interactions at kilometer-scale resolutions.

We will discuss the methodology and present the infrastructure used to seamlessly couple these models, ensuring efficient data exchange and synchronization among the atmospheric, oceanic, and wave components. The coupling technique leverages GFDL’s in-house Flexible Modeling System (FMS) infrastructure which is employed for GFDL's suite of world-leading coupled climate models and those developed for kilometer-scale modeling of extreme weather events, enhancing the model's ability to accurately simulate the feedback mechanisms between the ocean surface and the atmosphere. We believe this new model will be a valuable tool for researchers and meteorologists, improving disaster preparedness and response strategies for coastal communities.

How to cite: Mouallem, J., Gao, K., Chilutti, L., Reichl, B., Harris, L., Benson, R., Zadeh, N., and Zhang, C.: Coupling techniques in the new high resolution SHiELD + MOM6 model for extreme weather prediction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2059, https://doi.org/10.5194/egusphere-egu25-2059, 2025.

EGU25-2254 | Orals | CL4.7

Spectral Causal Analysis of Air-Sea Coupling Feedbacks through the Mesoscale 

Aaron Wienkers, Dian Putrasahan, and Nicolas Gruber

Ocean–atmosphere interactions play a crucial role in global climate & weather dynamics, yet our understanding of the interplay between mesoscale thermal and current air–sea feedbacks remains incomplete. The strength of this coupling influences heat and kinetic energy fluxes at different length-scales and locations across the global oceans. Eddy-parameterising climate models can resolve the large-scale energy input into the ocean, which is then transferred into eddy kinetic energy through parameterised hydrodynamic instabilities. These models, however, struggle to accurately capture the spatial patterns of energy transfer, both kinetic and thermal, back into the atmosphere from the ocean mesoscales. Here, we present insight from a mesoscale-resolving global coupled climate model that elucidates the physical mechanisms driving air–sea current and thermal feedbacks at the mesoscale, in comparison to the large-scale air–sea coupling. Spectral analysis further reveals how these feedbacks are suppressed when either the ocean or atmosphere fails to resolve a local critical coupling length-scale. Extending beyond these traditional regression-based methods, we employ a novel causal analysis framework to uncover a hybrid thermal–current mesoscale feedback which enhances kinetic energy injection directly into ocean mesoscales. This mechanism involves localised heat fluxes enhancing vertical convection and downward momentum transport within the atmospheric boundary layer, leading to increased local wind stress and consequently wind work into eddy kinetic energy. These results highlight the critical role of mesoscale air–sea coupling in accurately representing the energetic ocean mesoscales, which in turn influence the global oceanic circulation and climate. 

How to cite: Wienkers, A., Putrasahan, D., and Gruber, N.: Spectral Causal Analysis of Air-Sea Coupling Feedbacks through the Mesoscale, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2254, https://doi.org/10.5194/egusphere-egu25-2254, 2025.

EGU25-4489 | ECS | Posters on site | CL4.7

Quantifying Ensemble Divergence in Large-Domain Convective-Scale Simulations over Africa 

Fran Morris, Marcia Zilli, Neil Hart, and Jerry Samuel

Evidence indicates that since convective-scale simulations can explicitly resolve motion around deep convection, they may improve representation of coupling between small-scale moist convection and upscale modes of atmospheric variability.  Prior studies indicate that there can be a shift in the mean state of large-scale tropical circulations in convective-scale simulations relative to models with parameterised deep convection. However, it is uncertain whether this shift is systematic in convective-scale simulations or simply the response in a single model realisation.

To resolve this uncertainty, we run a 9-member ensemble of simulations over tropical southern and eastern Africa, using the Met Office Unified Model on a 2.2km grid with no deep convection parameterisation. ERA5 forces the lateral boundaries and simulations use FLake, a lake scheme to reduce over-lake biases in precipitation. The ensemble will be compared to a similar configuration which uses a deep convection parameterisation and a 12km grid.

Our ensemble experiments quantify the internal variability associated with varying initial conditions in the tropics and subtropics, relative to the variability induced by lateral boundary forcings. The ensemble divergence will be compared for the simulations with and without convection parameterisations to explore implications of ensemble design for high-resolution simulations of large domains. Furthermore, the hypothesis that there is a systematic mean-state shift in large-scale tropical circulations in kilometre-scale simulations relative to coarser GCMs will be evaluated using the two ensembles.

Effects of incorporating FLake and the role of soil moisture in initialisations will also be discussed, as well as their implications for predictability in kilometre-scale simulations. Model outputs will be compared to in-situ observations over northwest Zambia obtained during the 2022 DRYCAB field campaign, and we will outline how these results inform the design of planned further simulations to investigate monsoon onset predictability on subseasonal-to-seasonal timescales.

How to cite: Morris, F., Zilli, M., Hart, N., and Samuel, J.: Quantifying Ensemble Divergence in Large-Domain Convective-Scale Simulations over Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4489, https://doi.org/10.5194/egusphere-egu25-4489, 2025.

EGU25-4874 | Orals | CL4.7

High-Resolution Simulations with the Community Earth System Model (CESM): An Update 

Gokhan Danabasoglu, Ping Chang, Fred Castruccio, Dan Fu, Teagan King, Xue Liu, Nan Rosenbloom, Justin Small, Xiaoqi Wang, Gaopeng Xu, Steve Yeager, Qiuying Zhang, Andreas Prein, and Julio Bachmeister

As impacts of climate change are being felt by the society through sea level rise, increased intensity and occurrences of heat waves, droughts, extreme rainfall events and / or tropical cyclones (TCs), just to list a few, decision makers and stakeholders need reliable weather and climate information at increasingly finer spatial and temporal scales. Beyond such actionable aspects, there are numerous science questions regarding representation of and changes in importance of various processes with increased model resolution as well as their interactions with each other such as how TCs and oceanic mesoscale eddies interact with each other and with large-scale circulations. It is generally anticipated that with less reliance on uncertain parameterizations and their parameter choices, high-resolution models will represent various processes and coupled interactions of the Earth system with increased fidelity. To address these needs and challenges, we have made significant advances in high-resolution global climate modeling and predictions. Specifically, we have performed an unprecedented set of simulations at a TC-permitting and ocean-eddy-rich horizontal resolution using the Community Earth System Model (CESM 1.3), with additional modifications and improvements (hereafter referred to as CESM-HR). CESM-HR uses a 0.25° grid in the atmosphere and land and a 0.1° grid in the ocean and sea-ice components. These simulations include: a 500-year pre-industrial control simulation; 150-year 1%CO2 per year increase and 4xCO2 simulations; a 10-member ensemble of historical simulations; 10-member ensembles each of RCP8.5 and RCP6.0 future scenario simulations; 1 member each of RCP4.5 and RCP2.6 future scenario simulations; all HighResMIP coupled and AMIP simulations; and 10-member ensembles of 5-year decadal prediction simulations for the 1980-2023 period with May and November start dates for each year. The presentation will introduce these simulations and provide a few highlights from our extensive analysis. In general, high‐resolution simulations show significant improvements in representing global-mean surface temperature, oceanic heat uptake, sea level changes, extreme events such as TCs and winter-time extreme precipitation, and recent cooling and expanding sea-ice trends in the Southern Ocean. There are also improvements in prediction skill for several fields of interest. Our analysis shows that the projected increase in daily extreme precipitation over global land by the end of this century under the business-as-usual scenario is nearly double in the high-resolution simulations compared to its low-resolution counterpart, suggesting that current low-resolution models may significantly underestimate the future threat. Moreover, high-resolution simulations suggest that future precipitation intensifications arise from both moisture and circulation changes. This finding is in contrast with low-resolution simulations which primarily attribute such changes to increased moisture with warming. While not a panacea to address all the biases, these high-resolution simulations certainly offer promising potential to reduce model biases and uncertainties in comparison with their low-resolution counterparts and to improve our understanding of processes. Datasets from many of these simulations are now available to the broader community.

How to cite: Danabasoglu, G., Chang, P., Castruccio, F., Fu, D., King, T., Liu, X., Rosenbloom, N., Small, J., Wang, X., Xu, G., Yeager, S., Zhang, Q., Prein, A., and Bachmeister, J.: High-Resolution Simulations with the Community Earth System Model (CESM): An Update, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4874, https://doi.org/10.5194/egusphere-egu25-4874, 2025.

EGU25-5848 | ECS | Posters on site | CL4.7

Improvement of large-scale circulation simulation in an ocean-sea ice model with high-resolution 

Yiwen Li, Hailong Liu, Pengfei Lin, Mengrong Ding, and Zipeng Yu

The impact of the resolution on the large-scale features in an ocean-sea ice coupled model is represented in this paper through three aspects. Firstly, refined resolution accelerates temperature and salinity drifts at a basin-averaged scale by facilitating exchanges among basins, subsequently reducing global-averaged drifts. This amplification of basin-scale exchanges is associated with an accelerated large-scale circulation, leading to a more rapid equilibration of temperature and salinity above 300 meters. Secondly, the refined resolution yields improved simulations of large-scale temperature, salinity, and currents, particularly evident in regions such as the Gulf Stream and its extension. Enhanced current simulations and corresponding temperature distributions contribute to more accurate representations of wind stress through ocean currents and sea surface temperature feedback. This feedback, in turn, influences wind-driven currents, establishing positive feedback loops. Despite little impact on the temporal variability of phenomena such as ENSO, IOD, PDO, and AMO, the refined resolution enhances the strengths of their variabilities. However, spatial patterns of PDO and AMO do not exhibit improvement with refined resolution, potentially attributed to the coarse resolution of the reference dataset.

How to cite: Li, Y., Liu, H., Lin, P., Ding, M., and Yu, Z.: Improvement of large-scale circulation simulation in an ocean-sea ice model with high-resolution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5848, https://doi.org/10.5194/egusphere-egu25-5848, 2025.

EGU25-6699 | Posters on site | CL4.7

Multi-year simulations at kilometre scale with the Integrated Forecasting System coupled to FESOM2.5 and NEMOv3.4 

Thomas Rackow, Tobias Becker, Rohit Ghosh, Aleksei Koldunov, Xabier Pedruzo-Bagazgoitia, and Daisuke Takasuka

We report on the first multi-year kilometre-scale global coupled simulations using ECMWF's Integrated Forecasting System (IFS) coupled to both the NEMO and FESOM ocean–sea ice models, as part of the H2020 Next Generation Earth Modelling Systems (nextGEMS) project. We focus mainly on an unprecedented IFS-FESOM coupled setup, with an atmospheric resolution of 4.4 km and a spatially varying ocean resolution that reaches locally below 5 km grid spacing. A shorter coupled IFS-FESOM simulation with an atmospheric resolution of 2.8 km has also been performed. A number of shortcomings in the original numerical weather prediction (NWP)-focused model configurations were identified and mitigated over several cycles collaboratively by the modelling centres, academia, and the wider nextGEMS community. The main improvements are (i) better conservation properties of the coupled model system in terms of water and energy budgets, which also benefit ECMWF's operational 9 km IFS-NEMO model; (ii) a realistic top-of-the-atmosphere (TOA) radiation balance throughout the year; (iii) improved intense precipitation characteristics; and (iv) eddy-resolving features in large parts of the mid- and high-latitude oceans (finer than 5 km grid spacing) to resolve mesoscale eddies and sea ice leads. New developments at ECMWF for a better representation of snow and land use, including a dedicated scheme for urban areas, were also tested on multi-year timescales. We provide first examples of significant advances in the realism and thus opportunities of these kilometre-scale simulations, such as a clear imprint of resolved Arctic sea ice leads on atmospheric temperature, impacts of kilometre-scale urban areas on the diurnal temperature cycle in cities, and better propagation and symmetry characteristics of the Madden–Julian Oscillation.

How to cite: Rackow, T., Becker, T., Ghosh, R., Koldunov, A., Pedruzo-Bagazgoitia, X., and Takasuka, D.: Multi-year simulations at kilometre scale with the Integrated Forecasting System coupled to FESOM2.5 and NEMOv3.4, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6699, https://doi.org/10.5194/egusphere-egu25-6699, 2025.

Tropical waves are key drivers of weather and climate variability, yet their accurate simulation remains challenging due to the complexities of moist convection. This study investigates the impact of model resolution and convection treatment on tropical wave representation in a global non-hydrostatic model. Six simulations, with resolutions of 3.75 km, 15 km, and 120 km and convection treatments ranging from fully explicit to fully parameterized, are analyzed for their ability to capture wave-induced rainfall and three-dimensional wave structures. Results indicate that explicit convection outperforms parameterized convection in replicating rainfall anomalies, dynamic and thermodynamic wave structures, and rainfall-wind coupling. The 3.75-km explicit convection simulation performed best overall, indicating that explicit convection requires high resolution for optimal performance. A 15-km simulation using an alternative cumulus scheme produced wave signals nearly as accurate as the 3.75-km run, but with a significant rainfall bias, suggesting that the right results can sometimes be obtained for the wrong reasons. The study concludes that high resolution and explicit convection are essential for accurate tropical wave representation, with profound implications for weather forecasting and climate projections.

How to cite: Judt, F. and Rios-Berrios, R.: Sensitivity of Tropical Wave Structure to Resolution and Convection Treatment in a Global Non-Hydrostatic Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7071, https://doi.org/10.5194/egusphere-egu25-7071, 2025.

EGU25-7755 | ECS | Posters on site | CL4.7

Convergent Response in Aquaplanet Climate Change Experiments with Increasing Horizontal Resolution  

Angel Peinado Bravo, Daniel Klocke, and Bjorn Stevens

General Circulation Models (GCMs) are widely used to understand our climate and to simulate and predict the effects of global warming. They have shown persistent biases in the large-scale features of the general circulation and basic climate statistics, which are attributed mainly to parameterizations, especially the convection parameterization. To address this, Global storm-resolving models (GSRMs) provide an alternative approach to parameterization by explicitly resolving convection and its interaction with other processes through the refinement of the horizontal gridIn a prior study, we showed the physical convergence of the tropical and general circulation structure at a horizontal grid spacing of 2.5 km using aquaplanets. However, questions linger: Does the response to climate warming converge in a simplified framework as aquaplanets? 

 

We will present the effect of increasing horizontal grid spacing on the convergence of the climate change response in aquaplanet experiments. We will focus on the convergence of the storm tracks and jet stream in terms of their location and intensity using the global storm-resolving model ICON. Control runs, and idealized climate change experiments (increasing sea-surface temperature by 4 Kelvin) were conducted at horizontal grid spacing from 160 km to 2.5 km using an aqua-planet configuration. We adopt an aquaplanet configuration to focus on atmospheric phenomena, specifically convection and cloud feedback while reducing the effect of complex interaction with land, topography, sea ice, and seasons. We will discuss the convergence rate of the large-scale circulation, the eddy-driven jet, the subtropical jet, and the storm track and their response to climate warming, characterized by the location, width, and intensity.

How to cite: Peinado Bravo, A., Klocke, D., and Stevens, B.: Convergent Response in Aquaplanet Climate Change Experiments with Increasing Horizontal Resolution , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7755, https://doi.org/10.5194/egusphere-egu25-7755, 2025.

EGU25-8534 | ECS | Posters on site | CL4.7

Storm-Resolving Model ICON at the Air-Sea Interface: Insights into Momentum Dynamics and Parameterization Challenges 

Marius Winkler, Juan Pedro Mellado, and Bjorn Stevens

Storm-resolving models, such as the ICON model at 5 km resolution, are transforming our understanding of the Earth’s climate system by explicitly resolving key small-scale processes. This study highlights the dual nature of this modeling revolution: the advantages of improved representation of subgrid-scale dynamics and the challenges posed by existing parameterizations in capturing air-sea interactions.
On the one hand, a detailed momentum analysis of equatorial boundary layer winds using the coupled storm-resolving model ICON reveals dynamics that deviate from traditional assumptions. We identify two persistent wind patterns—zonal and meridional—governed by SST-driven pressure gradients, vertical turbulent flux, and horizontal momentum transport. These transport terms, largely overlooked in conventional models, and resolving the fine-scale interaction between SST gradients and boundary layer dynamics play a decisive role in shaping surface winds. A revised wind model, incorporating these findings, demonstrates strong agreement with storm-resolving model outputs.
On the other hand, storm-resolving models expose limitations in parameterizations of small-scale processes at the air-sea interface. For instance, the surface exchange coefficients—such as drag (cD) and heat exchange (cH)—are shown to be inadequate under low-wind regimes, leading to biases in surface pressure distribution and convection patterns. Using the ICON atmosphere-land-only "OptiFlux" configuration, we demonstrate that even small adjustments to these coefficients can substantially improve the representation of surface fluxes, strengthen pressure gradients, and enhance atmospheric dynamics.
These two aspects of this study illustrate the transformative potential and pressing challenges of storm-resolving models in further research.

How to cite: Winkler, M., Mellado, J. P., and Stevens, B.: Storm-Resolving Model ICON at the Air-Sea Interface: Insights into Momentum Dynamics and Parameterization Challenges, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8534, https://doi.org/10.5194/egusphere-egu25-8534, 2025.

EGU25-9092 | Orals | CL4.7

An overview of findings from km-scale simulations of the Destination Earth Climate Adaptation Digital Twin: successes, limitations and future challenges  

Paolo Davini, Jost von Hardenberg, Matteo Nurisso, Silvia Caprioli, Natalia Nazarova, Supriyo Ghosh, Ingo Wagner, Nuno Rocha, Marc Battle, Pablo Ortega, Leo Arriola, Rene Redler, Daniel Klocke, Jenni Kontkanen, and Sebastian Milinski

The Destination Earth Climate Adaptation Digital Twin represents a groundbreaking initiative aimed at achieving operational kilometer-scale global climate simulations for climate adaptation. During Phase 1 (Oct 2022 - Apr 2024), significant technological and scientific advancements have been made, resulting in the production of high-resolution historical (1990-2019, at 10 km) and SP370 scenario (2020-2039, at 5 km) datasets using two state-of-the-art models: IFS-NEMO and ICON.

These high-resolution simulations have demonstrated positive results in capturing extreme precipitation events and provide a realistic representation of the mean climate. The historical simulations outperform the CMIP6 model ensemble across various metrics, as assessed by the Reichler and Kim (2008) Performance Indices. In particular, IFS-NEMO exhibits well-defined precipitation patterns and vertical zonal wind structures, despite a persistent cold temperature bias. Meanwhile, ICON’s simulations - while showing more realistic temperature patterns - are characterized by an overly marked warming rate.

Both ICON and IFS-NEMO biases have been traced to suboptimal initialization strategies and oceanic tuning, both of which are being addressed in preparation for Phase 2. The ongoing efforts aim to refine these models further, enhancing their accuracy and reliability for climate adaptation policies.

How to cite: Davini, P., von Hardenberg, J., Nurisso, M., Caprioli, S., Nazarova, N., Ghosh, S., Wagner, I., Rocha, N., Battle, M., Ortega, P., Arriola, L., Redler, R., Klocke, D., Kontkanen, J., and Milinski, S.: An overview of findings from km-scale simulations of the Destination Earth Climate Adaptation Digital Twin: successes, limitations and future challenges , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9092, https://doi.org/10.5194/egusphere-egu25-9092, 2025.

EGU25-9160 | ECS | Posters on site | CL4.7

Mediterranean extreme precipitation events in storm-resolving NextGEMS Earth System Models 

Paolo Lanteri and Simona Bordoni

This study evaluates the ability of global storm-resolving simulations in reproducing extreme precipitation events (EPEs) over the Mediterranean basin, with a specific focus on the Italian peninsula. We use multi-decadal simulations provided by two coupled models, ICON and IFS-FESOM, both developed under the EU’s Horizon 2020 Next Generation Earth Modelling Systems (NextGEMS) project. Thanks to the synergy between large-scale circulation patterns and km-scale atmospheric dynamics, it is expected that such models better represent precipitation distribution and intensity.

In this work we apply a classification of EPEs based on a set of thermodynamic parameters representative of the regional-scale environmental conditions, following  Grazzini et al. (2020), to classify EPEs over central-northern Italy in three main categories, based on the main uplift mechanism. 

We validate model simulations against the results of Grazzini et al. (2020) based on ArCIS/ERA5 data over central-northern Italy. The analysis is then extended to other Mediterranean regions, providing insights into the models’ capabilities and limitations in capturing extreme events under different large-scale conditions. 

How to cite: Lanteri, P. and Bordoni, S.: Mediterranean extreme precipitation events in storm-resolving NextGEMS Earth System Models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9160, https://doi.org/10.5194/egusphere-egu25-9160, 2025.

EGU25-9386 | ECS | Posters on site | CL4.7

Scientific developments of IFS-NEMO for Destination Earth’s Climate Adaptation Digital Twin 

Nuno Rocha, Pablo Ortega, Marc Batlle, Ingo Wagner, Kai Keller, Charles Pelletier, Xabier Pedruzo, Thomas Rackow, Tobias Becker, Dmitry Sidorenko, Matteo Nurisso, Silvia Caprioli, Natalia Nazarova, Supriyo Ghosh, and Sebastian Milinski

The Climate Adaptation Digital Twin within the Destination Earth project represents an innovative initiative aimed at achieving operational kilometer-scale global climate simulations to support climate adaptation efforts. Three state-of-the-art Earth System Models (ESMs) are used separately and we are focusing on the scientific advancements and simulation results of the IFS-NEMO model throughout the project's duration.

During the first phase of the project, two main simulations were produced: a historical experiment (1990–2019) at 10 km resolution, and a SSP3-7.0 scenario (2020–2039) at 5 km resolution. Phase 2 aims to enable the operationalization of these simulations. Analysis of phase 1 IFS-NEMO results revealed a notable cold bias in the model’s mean state. To address this issue, a newly tuned version of the model was developed, significantly reducing the cooling trends. Key adjustments to achieve this improvement, first tested at a 25 km resolution version of the model, included refinements to sea-ice parameterization within the NEMO model,  and the introduction of MACv2-SP forcings in IFS, which enabled the representation of time-varying aerosols in the future scenarios. Additional enhancements were made to couple the river runoff to the ocean.

The outcomes of these efforts highlight the potential for substantial advancements in global climate modeling. Looking ahead, the integration of kilometer-scale simulations into operational workflows promises to deliver unprecedented detail and accuracy in climate projections. This will enable more precise assessments of climate impacts and provide critical insights for policymakers and stakeholders striving to implement effective climate adaptation strategies. The continued refinement of the IFS-NEMO model and its components will play a pivotal role in achieving these ambitious goals.

How to cite: Rocha, N., Ortega, P., Batlle, M., Wagner, I., Keller, K., Pelletier, C., Pedruzo, X., Rackow, T., Becker, T., Sidorenko, D., Nurisso, M., Caprioli, S., Nazarova, N., Ghosh, S., and Milinski, S.: Scientific developments of IFS-NEMO for Destination Earth’s Climate Adaptation Digital Twin, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9386, https://doi.org/10.5194/egusphere-egu25-9386, 2025.

EGU25-10848 | ECS | Posters on site | CL4.7

Assessing the impact of anthropogenic aerosols in a kilometer-scale Earth system model 

Philipp Weiss and Philip Stier

Aerosols influence Earth's climate directly by scattering or absorbing radiation and indirectly by serving as nuclei for cloud droplets or ice crystals. Earth system models have significantly improved our understanding of aerosols, clouds, and radiation. The resolution of these models has increased from above 100 kilometers to below 10 kilometers in recent years. With that, important atmospheric processes like deep convective motions are explicitly resolved.

To perform kilometer-scale (km-scale) simulations with the Earth system model ICON-MPIM, we developed the one-moment aerosol module HAM-lite. In HAM-lite, aerosols are represented as an ensemble of log-normal modes with prescribed properties. There are two pure modes, one composed of dust and one composed of sea salt, and two internally mixed modes, both composed of organic carbon, black carbon, and sulfate. The first mixed mode includes aerosols from biomass burning emissions and the second mixed mode includes aerosols from anthropogenic and volcanic emissions. The four modes are transported through the atmosphere and are coupled with various processes such as radiation, convection, and precipitation.

To assess the impact of anthropogenic aerosols, we performed two km-scale simulations over one year with different emission scenarios. The present-day scenario is based on emissions from the Community Emissions Data System (CEDS) and the Global Fire Assimilation System (GFAS). The pre-industrial scenario is based on the historic biomass burning emissions for CMIP6 (BB4CMIP). In both simulations, the sea surface temperature and sea ice are prescribed with the boundary conditions of AMIP, and the initial conditions of the atmosphere and land are derived from the operational analysis of ECMWF. Based on these two scenarios, we analyze how anthropogenic aerosols interact with radiation and clouds over one year. 

How to cite: Weiss, P. and Stier, P.: Assessing the impact of anthropogenic aerosols in a kilometer-scale Earth system model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10848, https://doi.org/10.5194/egusphere-egu25-10848, 2025.

Mesoscale convective systems are a crucial feature in Sahel, a water vulnerable semi-arid region in West Africa. Observational studies have shown that they are responsible for bringing approximately 90% of the rainfall during the summer monsoon season, and play an especially important role in extreme rainfall events. Despite of their important impacts on society and climate, traditional general circulation models, with their coarse horizontal resolution and parameterized convection schemes, struggle to properly simulate these organized convective systems. However, the newer generation of km-scale convection-permitting climate models have been shown to much more accurately capture the characteristics of mesoscale convective systems, showing great potential for studies of future climate change in vulnerable regions such as the Sahel.

In this study we analyze the latest simulations run with IFS and ICON within the NextGEMS project, with a horizontal resolution up to 9 km. Using a lagrangian tracking algorithm to identify the mesoscale convective systems, we investigate how they and their related weather are represented in the models, how well they scale in strength with known amplifying factors and if any trends can be identified in the simulation.

How to cite: Berntell, E.: Representation of West African mesoscale convective systems in NextGEMS km-scale simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10993, https://doi.org/10.5194/egusphere-egu25-10993, 2025.

EGU25-11001 | ECS | Orals | CL4.7

Unveiling global haboob behavior with a kilometer-scale aerosol-climate model 

Rumeng Li, Philipp Weiss, Andreas Baer, Carlos Pérez García-Pando, Philip Stier, and Martina Klose

Haboob dust storms, formed by the cold pool outflow from moist convection, play a significant role in global dust emissions. However, they are largely absent in current global climate models, as most do not explicitly resolve convection processes, leading to considerable inaccuracies in modeling global dust and its impacts. Therefore, the global influence of haboobs on the dust cycle and the Earth system remains poorly understood. With the advent of kilometer-scale Earth system models, there is a unique opportunity to unveil the global haboob behavior and advance our understanding of their impacts.

In this study, we implemented physics-based dust emission schemes in the ICON-HAM-lite model, a new kilometer-scale Earth system model developed in the nextGEMS project. A one-year model simulation was conducted globally at a 5 km resolution including online dust simulation. A haboob detection algorithm was developed and applied to track haboobs, allowing us to analyze their global characteristics and variability. This includes their spatial distribution, seasonal and diurnal cycles, duration, and size. Additionally, the contribution of haboobs to global dust emissions was evaluated.

This study provides what is, to our knowledge, the first comprehensive analysis of haboobs on a global scale based on the current literature, shedding light on their critical role in the global dust cycle. These findings highlight the benefits of using global kilometer-scale models, specifically emphasizing their potential to improve dust simulation accuracy in climate models by explicitly including convection.

How to cite: Li, R., Weiss, P., Baer, A., Pérez García-Pando, C., Stier, P., and Klose, M.: Unveiling global haboob behavior with a kilometer-scale aerosol-climate model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11001, https://doi.org/10.5194/egusphere-egu25-11001, 2025.

EGU25-11145 | ECS | Posters on site | CL4.7

Assessing the impacts of climate change in Iberian mountains using the NextGEMS km-scale global climate simulations 

Diego García-Maroto, Luis Durán, Elsa Mohino, and Álvaro González-Cervera

Mountain areas play a pivotal role in the hydrological cycle of vast regions of the world, largely due to local processes such as orographic precipitation and the presence of seasonal or permanent snow cover. In the context of climate change, some of these processes are expected to be disrupted causing significant impacts to local ecosystems and nearby populations. This is particularly relevant for regions like the Iberian Peninsula, where the development of a persistent winter-spring snowpack confined to the various medium sized mountain ranges is key to offsetting water deficits during the dry summer season. Knowing the future climate of these mountains is therefore vital both for water resource management and for economic interests.

However, these mountain ranges are often characterized by medium heights and a small horizontal extent, making them very difficult to represent in most conventional coarse resolution global climate models and demanding thus the use of regional to local dynamical and statistical downscaling methods. Considering this, the new km-scale global climate simulations developed in the context of the European H2020 NextGEMS project and other similar initiatives may open up unprecedented opportunities to readily study future impacts of climate changes on these regions. These models allow the representation of local and regional processes while retaining the benefits of homogeneous global simulations. 

The present study firstly evaluates the capacity of historical km-scale simulations (1990-2019) to represent the climate of the main mountainous areas of the Iberian Peninsula, with a particular emphasis on variables impacting seasonal snow cover which are compared with different historical data sources, including local observations, reanalyses and satellite observations. We show a fairly acceptable agreement between the model climatology and regional reanalysis products specially for the annual number of days with snow cover. Regarding snow depth, however, the model shows a small positive bias in all regions except Sierra Nevada, where it has a negative bias. Following the assessment of potential model biases, the differences between the historical climatology and a 2020-2049 projection under scenario SSP3-7.0 are analysed. Among others, we show that in the projection significant decreasing trends are present in most snow cover metrics for all the considered mountain regions, even though they are more extreme at Sierra Nevada, where a significant reduction of total winter precipitation is also present. 

How to cite: García-Maroto, D., Durán, L., Mohino, E., and González-Cervera, Á.: Assessing the impacts of climate change in Iberian mountains using the NextGEMS km-scale global climate simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11145, https://doi.org/10.5194/egusphere-egu25-11145, 2025.

EGU25-11236 | ECS | Posters on site | CL4.7

The ICON-ParFlow coupling: Integrating a continental-scale hydrological model into an Earth system model 

Jan Weinkaemmerer, Reiner Schnur, Klaus Goergen, and Stefan Kollet

3D prognostic groundwater flow on a global scale is currently lacking in Earth system models. In order to prepare Earth system models for kilometer-scale simulations with integrated continental hydrology, the ParFlow hydrological model has been coupled to the land model of the ICON modelling framework. Global simulations of atmosphere and land were conducted with a two-way coupling between ParFlow and the soil hydrological scheme of ICON-Land over the Pan-European region. In this first configuration, ParFlow and ICON-Land exchange surface moisture fluxes and liquid soil water. Analyzing simulations covering the extended summer months, it is found that the coupling with ParFlow significantly reduces the soil-water variability in the deeper soil layers by resolving actual shallow aquifers. In ParFlow, surface runoff and infiltration are more physical resulting in a more realistic response of soil moisture to weather patterns on longer time scales. Correlations of soil moisture with surface latent heat flux and atmospheric moisture transport show that this results regionally in an increased land-atmosphere coupling strength. Also, the lateral flow of near-surface groundwater, which is intrinsically linked to the formation of river networks, influences atmospheric variables related to cloud formation by increasing their horizontal heterogeneity. Apart from these results, which demonstrated the importance of an integrated hydrological model for shallow groundwater in Earth system modelling, first results of high-resolution coupled simulations with an extended ParFlow coverage on a latitude belt over the tropical zone at 1 km resolution are presented. 

How to cite: Weinkaemmerer, J., Schnur, R., Goergen, K., and Kollet, S.: The ICON-ParFlow coupling: Integrating a continental-scale hydrological model into an Earth system model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11236, https://doi.org/10.5194/egusphere-egu25-11236, 2025.

EGU25-11601 | Orals | CL4.7

Are global km-scale climate models becoming indistinguishable from observations? 

Lukas Brunner, Rohit Ghosh, Leopold Haimberger, Cathy Hohenegger, Dian Putrasahan, Thomas Rackow, Reto Knutti, Aiko Voigt, and Jana Sillmann

Simulating global climate has been a challenge and aspiration ever since the advent of numerical modeling. Today, global climate models have become essential tools to understand the climate system, project future changes, and inform mitigation and adaptation decisions. In that, they build on a long history of development, from the first attempts to couple atmospheric and ocean models in the late 1960s, to the emergence of Earth system models in the 2000s, and the development of the first km-scale models today.

In this talk, we show that the latest models provide global climate information with previously unprecedented accuracy. The two next-generation km-scale models included in our analysis (ICON Sapphire and IFS) even simulate temperature fields indistinguishable from observation-based references for the first time. We place this step-change in model fidelity in the context of nine observation-based datasets (20CR, ERA40, ERA-Interim, ERA5, JRA55, MERRA, MERRA2, NCAR-NCEP) and over 150 global climate models developed over the past three decades (from CMIP2 to CMIP6) in an extensive model evaluation. Based on this comparison, we discuss emerging challenges for model evaluation as the choice of the reference dataset starts to dominate model error for the latest models. 

 

How to cite: Brunner, L., Ghosh, R., Haimberger, L., Hohenegger, C., Putrasahan, D., Rackow, T., Knutti, R., Voigt, A., and Sillmann, J.: Are global km-scale climate models becoming indistinguishable from observations?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11601, https://doi.org/10.5194/egusphere-egu25-11601, 2025.

Here we investigate tropical precipitation biases in the novel kilometer-scale Earth system models (ICON and IFS) developed by the EU-funded H2020 nextGEMS project. Despite the much higher resolution, these km-scale models still feature biases that are common to CMIP models: first, tropical precipitation is systematically overestimated. Second, the double ITCZ (Intertropical Convergence Zone) bias is not ameliorated, with too little rain falling close to the Equator and too much rain in the southern branch relative to the northern branch. The double ITCZ bias is consistent with Hadley circulations that feature secondary cells close to the equator. Third, both the northern and the southern ITCZ branches are displaced poleward relative to observations. 

Focusing on the tropical precipitation distribution, we more explicitly quantify existing biases through a symmetric and an antisymmetric precipitation index. Leveraging the well-established atmospheric energy balance framework, we show how hemispherically symmetric biases are positively corellated with biases in the equatorial net energy input (NEI), once any residual in its global average is removed. In both models, equatorial NEI biases primarily arise from surface latent heat fluxes. Hemispherically antisymmetric biases are instead negatively correlated with the cross-equatorial atmospheric energy transport, which is in turn linked to biases in the NEI hemispheric asymmetry. The leading sources of asymmetric biases are top-of-atmosphere radiative fluxes in IFS and surface radiative fluxes in ICON.

Finally, although we find that notorious GCM precipitation biases are not mitigated when employing km-scale grids, we also see that the atmospheric energy balance holds great potential for improving tropical precipitation patterns. In this regard key candidates for improving the energy balance are surface flux schemes, particularly for latent heat over the oceans, and cloud-radiative effects. 

How to cite: Müller, S. K. and Bordoni, S.: Understanding tropical precipitation biases in kilometer-scale global climate models using the atmospheric energy balance framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11818, https://doi.org/10.5194/egusphere-egu25-11818, 2025.

EGU25-12756 | ECS | Posters on site | CL4.7

Comparing biases in the earth system model ICON-ESM-ER with its predecessor MPI-ESM-ER 

Chathurika Wickramage, Jürgen Kröger, and Fabian Wachsmann

The resolution of climate models significantly influences their ability to simulate physical processes and reduce biases, especially in oceanic and atmospheric systems. The Eddy-Rich Earth System Models (EERIE) project focuses on developing next-generation Earth System models at kilometer-scale resolution. In this study, we compare the control simulations of one of the EERIE models, the ICOsahedral Non-hydrostatic Earth System Model (ICON-ESM-ER), with those of its eddy-rich predecessor, the Max Planck Institute Earth System Model (MPI-ESM-ER). The ICON-ESM-ER features a 5 km ocean resolution coupled with a 10 km atmospheric resolution, while the MPI-ESM-ER employs a 10 km ocean resolution and a 100 km atmospheric resolution. Additionally, the ICON-ESM-ER uses an unstructured icosahedral grid, whereas the MPI-ESM-ER is based on a tripolar curvilinear grid. As models gradually move to finer spatial resolution, we naturally expect to improve simulations of atmospheric and oceanic flows. However, things become particularly interesting when new thresholds are crossed, as it enables the explicit simulation of previously unresolved phenomena. This can also introduce new complexities and challenges. The analysis reveals distinct differences in biases between the two models. For instance, focusing on the Southern Ocean, ICON-ESM-ER exhibits overall warmer biases than its predecessor MPI-ESM-ER and shows very large positive dynamic sea level biases. Additionally, ICON-ESM-ER produces large positive zonal surface wind biases in this region. On a more positive note, the sea surface salinity biases in the South Atlantic and Indian Ocean are negligible in ICON-ESM-ER. The ICON-ESM-ER does not outperform MPI-ESM-ER and, in some cases, introduces larger biases in key climate variables. Understanding these biases, particularly in comparison to its predecessor, is essential to guide future model development and improve the representation of critical processes in the Earth system.

How to cite: Wickramage, C., Kröger, J., and Wachsmann, F.: Comparing biases in the earth system model ICON-ESM-ER with its predecessor MPI-ESM-ER, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12756, https://doi.org/10.5194/egusphere-egu25-12756, 2025.

EGU25-13120 | ECS | Posters on site | CL4.7

Discovering convection biases in global km-scale climate models using computer vision 

Lilli Freischem, Philipp Weiss, Hannah Christensen, and Philip Stier

Convective clouds are a key component of the climate system, impacting the hydrological cycle, and leading to the redistribution of heat, moisture, and momentum. Traditional low-resolution climate models rely on parameterisations to represent convection and thus struggle to realistically capture convective processes. In contrast, km-scale models can directly simulate deep convection, improving the accuracy of cloud and precipitation fields. However, significant uncertainties remain, due to parameterisations of remaining unresolved subgrid-scale processes, which must be addressed.

Traditional model evaluation methods rely on aggregated spatial and temporal statistics, which overlook the fine-grained details critical to understanding the physical processes underlying convection. In addition, conventional dimensionality reduction techniques (e.g., principal component analysis) cannot capture the non-linear relationships of small-scale physical processes.

To address these limitations, we use computer vision models to learn meaningful low-dimensional embeddings of outgoing longwave radiation (OLR) fields and evaluate km-scale models in this new embedding space. More specifically, we use contrastive learning, a self-supervised technique that trains machine learning models to distinguish between similar and dissimilar data points, to train a deep neural network to generate compact representations of OLR fields.

We present results from a case study evaluation of two km-scale models, the Integrated Forecasting System (IFS) and the Icosahedral Nonhydrostatic Model (ICON), developed as part of the nextGEMS project. The simulations are compared to observations from the Geostationary Operational Environmental Satellites (GOES-16). We quantitatively assess the realism of km-scale models by comparing the embedding distributions of models and observations using vector quantisation. Finally, we use explainability methods to identify key factors influencing the accuracy of simulated convection. Our results highlight the value of our approach in understanding and improving the performance of high-resolution climate models, contributing to more reliable climate projections at finer spatial scales.

How to cite: Freischem, L., Weiss, P., Christensen, H., and Stier, P.: Discovering convection biases in global km-scale climate models using computer vision, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13120, https://doi.org/10.5194/egusphere-egu25-13120, 2025.

EGU25-15682 | Orals | CL4.7

Tales of Storms: Climate Storylines of Extreme Precipitation Events in Autumn 2024 

Thomas Jung, Amal John, Sebastian Beyer, Marylou Athanase, Antonio Sanchez Benitez, Helge Gößling, and Jan Wehner

The autumn of 2024 witnessed a series of extreme precipitation events that caused widespread impacts, highlighting the importance of investigating the role of climate change in impacting these phenomena. This study employs novel kilometre-scale (km-scale) storyline simulations using the IFS-FESOM coupled climate model to examine three major events—Hurricane Helene in the United States, severe flooding in Valencia, Spain, and Storm Boris that brought extreme precipitation to Central and Eastern Europe—under preindustrial, present-day, and future climate forcings. By nudging the evolution of large-scale atmospheric dynamics to ERA5, the storyline approach isolates thermodynamic changes due to anthropogenic warming while maintaining consistency with the observed event structures. The km-scale resolution enables a detailed representation of topographical influences, local-scale processes such as moisture convergence, and convective dynamics, providing critical insights into how the intensity, spatial distribution, and other characteristics of heavy precipitation may unfold in different climates. This study lays the foundation for a comprehensive set of storylines of high-impact extreme precipitation events, offering actionable information for decision-makers and increasing public understanding of the impact of climate change on extreme weather risks.

How to cite: Jung, T., John, A., Beyer, S., Athanase, M., Sanchez Benitez, A., Gößling, H., and Wehner, J.: Tales of Storms: Climate Storylines of Extreme Precipitation Events in Autumn 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15682, https://doi.org/10.5194/egusphere-egu25-15682, 2025.

EGU25-17342 | Orals | CL4.7

A global-regional hierarchy approach to exploring upscale processes in km-scale Earth System models 

Huw Lewis, Richard Jones, Sally Lavender, Claudio Sanchez, Dasha Shchepanovska, and Calum Scullion

Exploitation of more powerful supercomputers has unlocked the potential to run kilometre-grid scale global simulations. Reaching convection-permitting resolution has been highlighted as a means to both transform local-scale weather prediction and reduce long-standing biases in global climate models. The dynamical downscaling benefits of delivering convection-permitting predictions, have been long established for weather and climate applications. Explicitly representing many of the key dynamical convective processes leads to better representation of several aspects of the mesoscale phenomena that lead to high impact weather than is achievable in coarser grid-scale models which require convection to be fully parametrized. GSRM potentially unlock representation of this upscale interaction within models, not currently simulated in global models in which the influence of convection is parametrized, or in nested limited-area models in which smaller scales do not feedback onto the general circulation. By doing so, it is hypothesized that long-standing model biases, such as in large-scale circulations and their effect on global precipitation patterns, might be resolved or reduced.

In the UK, Met Office and university partner K-Scale research has been focussed on assessment of this upscale hypothesis. A traceable global-regional model hierarchy has therefore been established, exploiting the Unified Model seamless modelling framework and model development foundations. The hierarchy spans global and limited area atmosphere-only simulations across a range of grid resolutions and model physics. We exploit the hierarchy to demonstrate the influence of upscale processes on the predicted strength and variability of upper-level winds. Enabling upscale growth in our simulations results in a relative strengthening of the tropical easterly jet. Over S. America, there is evidence of a weakening of the westerly jet over the eastern Pacific and stronger easterlies over the tropical Atlantic in vicinity of the Atlantic ITCZ. Over SE Asia, there is a general strengthening of upper-level easterly winds.

We describe the further evaluation of the hierarchy, including its sensitivity to model physics choices, in the context of new year-long simulations adopting the DYAMOND3 protocol, and discuss plans and challenges of how the Met Office is looking to apply Earth system models at km-scale in the context of evolving operational NWP, climate research and machine learning capability and service development.

How to cite: Lewis, H., Jones, R., Lavender, S., Sanchez, C., Shchepanovska, D., and Scullion, C.: A global-regional hierarchy approach to exploring upscale processes in km-scale Earth System models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17342, https://doi.org/10.5194/egusphere-egu25-17342, 2025.

As the climate continues to warm, hydrometeorological extremes are extracting a greater toll from society both economically and socially. The need for accurate extreme event projections during acute dry spells was recently highlighted by the January 2025 devastating wildfires in the Los Angeles region. Current CMIP-style global climate models broadly project an increasing frequency and intensity of heavy precipitation and drought. However, the relatively coarse resolution, lack of ocean-atmosphere coupling, and parameterization of convection means they do not capture the spatial heterogeneity and mesoscale processes of complex coasts and topography relevant for simulating extreme events which often introduces model biases.

The ongoing H2020 Next Generation Earth Modelling Systems (nextGEMS) project aims to address these issues with the development of convection-permitting, fully-coupled, Earth-system models. Using the ECMWF Integrated Forecast System (IFS) and Icosahedral Nonhydrostatic Weather and Climate Model (ICON), we examine detailed dry spell characteristics in the Mediterranean region of Europe and then expand our analysis globally. These results are compared against a suite of observations (station and satellite based), reanalysis datasets, and CESM2 simulations.

Using ICON and IFS with about 6 km and 4 km spatial resolution, respectively over a five-year period in the Mediterranean, we find the increased resolution and hybrid/explicit representation of convection improves the representation of dry hour frequency and alleviated the long-standing drizzle bias observed in many GCMs, here illustrated for CESM2. For simulating the maximum length of dry spells over land, switching off the convective parameterization scheme in ICON improves accuracy with similar dry spell lengths as observations and reanalysis. However, the annual maximum length of dry spells over the sea for both ICON and IFS is excessive by 30-50 days. The depiction of dry spells in the Mediterranean region is representative of the nextGEMS’ models performance across the whole mid-latitudes. Ongoing research using recently developed 30-year transient ICON and IFS simulations (2020-2050) looks to investigate how dry extremes evolve globally in a warming world.

How to cite: Wille, J. and Fischer, E.: Dry spell representation on regional and global scale using convection-permitting models within the nextGEMS project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17833, https://doi.org/10.5194/egusphere-egu25-17833, 2025.

EGU25-18012 | ECS | Posters on site | CL4.7

4.4-km global climate projections with IFS-FESOM 

Sebastian Beyer, Thomas Rackow, Dmitry Sidorenko, Nikolay Koldunov, Amal John, Rohit Ghosh, Jan Streffing, Suvarchal Kumar Cheedela, Maqsood Mubarak Rajput, Miguel Andrés-Martínez, Mohammed Hussam Al Turjman, Razvan Aguridan, Matteo Nurisso, Jan Wehner, and Thomas Jung

We present the current IFS-FESOM model configuration of the Destination Earth (DestinE) project, which we used to compute a coupled climate projection (SSP-3.70) from 2020 to 2040 with unprecedented storm-resolving resolution. The atmospheric resolution of 4.4 km allows us to replace previously necessary parametrizations with explicitly resolved atmospheric dynamics. The unstructured NG5 ocean mesh, which locally reaches below 5 km resolution, resolves mesoscale ocean eddies and sea ice leads.

IFS-FESOM consists of the Integrated Forecasting System (IFS, developed by ECMWF) coupled to the Finite Volume Sea Ice-Ocean Model FESOM2. It utilizes the IO-server and post-processing toolkit multIO, providing hourly outputs and statistical processing of numerous variables. It also takes advantage of recent improvements to the IFS, including enhanced representations of snow and land use, as well as a dedicated scheme for urban areas and cities worldwide.

We present initial results from analyzing the simulation, addressing technical challenges and scientific questions related to running km-scale simulations over multiple decades.

How to cite: Beyer, S., Rackow, T., Sidorenko, D., Koldunov, N., John, A., Ghosh, R., Streffing, J., Cheedela, S. K., Rajput, M. M., Andrés-Martínez, M., Al Turjman, M. H., Aguridan, R., Nurisso, M., Wehner, J., and Jung, T.: 4.4-km global climate projections with IFS-FESOM, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18012, https://doi.org/10.5194/egusphere-egu25-18012, 2025.

EGU25-18760 | Orals | CL4.7

Eddy activity in the high-latitude Southern Ocean and its response to climate change 

Nathan Beech, Thomas Rackow, Tido Semmler, and Thomas Jung

Eddy activity in the high-latitude Southern Ocean is linked to critical drivers of the global climate such as Antarctic Bottom Water (AABW) formation, seasonal sea ice cover, and shoreward heat transport. Yet, no comprehensive description of eddy activity poleward of the Antarctic Circumpolar Current (ACC) exists and the mesoscale processes in the region are missing from virtually all major projections of climate change. Using a high-resolution ocean model and cost-reducing simulation design, eddy activity in the high southern latitudes is characterized with unprecedented detail, including 3-dimensional spatial distribution and characteristics, unobstructed information beneath sea ice, and projections of future conditions after prolonged anthropogenic warming. A rich mesoscale field is detected, with eddy activity closely linked to large-scale circulation features like gyres and the Antarctic Slope Current. Eddy activity exhibits a strong seasonal cycle in which the presence of sea ice decreases the eddy population and increases the proportion of anticyclones. Anthropogenic warming is projected to increase the eddy population, particularly in winter. Projected impacts of climate change are regionally diverse; ACC eddy activity shifts poleward, Antarctic Slope Current eddy activity intensifies, and the seasonal cycle affecting the eddy population and rotational direction is reduced.

How to cite: Beech, N., Rackow, T., Semmler, T., and Jung, T.: Eddy activity in the high-latitude Southern Ocean and its response to climate change, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18760, https://doi.org/10.5194/egusphere-egu25-18760, 2025.

EGU25-20426 | Posters on site | CL4.7

Regionally focused aerosol-climate modelling at kilometer scale 

Anne Kubin, Bernd Heinold, Philipp Weiss, Philip Stier, and Ina Tegen

Aerosol particles from natural and anthropogenic sources play an important role in the Earth's climate through their interactions with radiation and clouds. However, the underlying mechanisms and their climate impacts remain poorly understood. Kilometer-scale high-resolution climate simulations provide a powerful tool to tackle these uncertainties and reveal new details about the effects of aerosols, e.g., on moist convective clouds and fine-scale atmospheric dynamics. Recently, the reduced-complexity aerosol module HAM-lite was developed for global simulations within the ICON-MPIM Earth system model. While based on the proven but complex aerosol module HAM, HAM-lite represents aerosols as a group of logarithmic-normal modes with predefined sizes and compositions. It uses one mode each for pure dust and sea salt particles, and two internally mixed modes with organic carbon, black carbon, and sulfate. Now, this coupled model system has been further advanced to support limited-area mode (LAM) applications, enabling faster, targeted simulations of specific source and target regions and their associated aerosol processes.

We showcase the enhanced capability of ICON-MPIM and HAM-lite through LAM case studies. Regional simulations are performed at a resolution of approximately 2.5 kilometers over several months, using AMIP boundary conditions for sea surface temperature and sea ice. Initial and lateral boundary conditions for the atmosphere are sourced from ECMWF operational analysis, while aerosol boundary data are derived from either the Copernicus Atmosphere Monitoring Service reanalysis (EAC4 CAMS) or global ICON-MPIM-HAM-lite simulations. In this study, we present LAM applications for case studies of air pollution in Central Europe and Eastern Australia, densely populated regions with extensive aerosol measurement networks for model evaluation in the northern and southern hemispheres, respectively. Further analyses include aerosol processes at high-latitudes in the Fram Strait-Svalbard Arctic region, investigating the effects of sea ice on sea-spray emissions and polar air mass exchange; and low-latitude events in West Africa, focusing on the transport and impacts of dust and biomass burning smoke on regional climate and air quality.

How to cite: Kubin, A., Heinold, B., Weiss, P., Stier, P., and Tegen, I.: Regionally focused aerosol-climate modelling at kilometer scale, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20426, https://doi.org/10.5194/egusphere-egu25-20426, 2025.

Recently, hierarchical finite element spaces were constructed using the subdivision algorithm
to generalize well-established concepts in isogeometric analysis to irregular meshes, for example of
the sphere. This talk illustrates the suitability of these function spaces for structure-preserving
simulations of the shallow water equations with local refinement. We focus on quantifying the
observed accuracy gains and the scaling of the compute time by comparison to established finite
elements without local refinement.
A key benefit of the hierarchical spaces is that they maintain a discrete de Rham complex
under local refinement and thus yield structure-preserving numerical methods. This property is
crucial for discretisations of atmospheric models as it allows us to locally increase the resolution
whenever necessary without changing characteristic features of the simulated systems, such as mass,
total energy or vorticity. Thus, the evolution of the discrete system mirrors the continuous system
faithfully and the simulation results are physically meaningful. We will present simulation results
that confirm these theoretical results.

How to cite: Piel, R. and Bauer, W.: An adaptive, structure-preserving numerical method for the rotating shallow water equations using hierarchical finite elements generated through subdivision, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-449, https://doi.org/10.5194/egusphere-egu25-449, 2025.

EGU25-1213 | Orals | AS5.2

Improving performance of ICON-O through parallel-in-time integration and dynamic super-resolution 

Daniel Ruprecht, Philip Freese, Sebastian Götschel, Thibaut Lunet, Fabricio R. Lapolli, Peter Korn, Max Witte, Christopher Kadow, and Martin Schreiber

Global ocean simulations at very high resolution are extremely time consuming. Representing sub-mesoscale eddies on a numerical grid requires local resolutions of around 600m and is currently only possible in simulations over a few weeks or months. We will investigate two approaches to increase the throughput of ICON-O with the aim of enabling sub-mesoscale resolving simulations of climatologically relevant timescales.

The first approach replaces the current Adams-Bashforth time stepping method with parallelizable spectral deferred correction (SDC) methods. SDC is an iterative method that computes the stages of a fully implicit Runge-Kutta method by multiple “sweeps’’ with a low-order integrator, often an implicit-explicit Euler. It delivers arbitrary, tunable order of accuracy and possesses good stability properties. Proper selection of method parameters allows for small-scale parallelization of each sweep, using threads up to the number of computed stages. We will investigate stability, accuracy and efficiency for a parallel SDC implementation in ICON-O and the research code SWEET. Benchmark results on a single node of JUSUF at Jülich Supercomputing Center demonstrate speedups over the currently used Adams-Bashforth-2 algorithm.

The second approach is based on super-resolution techniques from image enhancement. We propose a dynamic super-resolution technique, where the numerical solution is frequently modified by a U-net-type neural network to correct it towards the restriction of a higher resolution simulation. For the Galewsky test case we demonstrate that our approach can deliver L2 errors comparable to a 10km resolution on a 20km resolution mesh while correctly conserving mass.

How to cite: Ruprecht, D., Freese, P., Götschel, S., Lunet, T., Lapolli, F. R., Korn, P., Witte, M., Kadow, C., and Schreiber, M.: Improving performance of ICON-O through parallel-in-time integration and dynamic super-resolution, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1213, https://doi.org/10.5194/egusphere-egu25-1213, 2025.

The limitations of high-performance computing (HPC) often impose significant constraints on the development and performance of numerical models. While double precision ensures high accuracy in traditional models, it comes with substantial computational costs. Lower precision can reduce computational expenses but may introduce round-off errors that degrade model accuracy. The Quasi double-precision (QDP) algorithm addresses these errors by maintaining corrections, thereby improving result accuracy. Building on previous work where the QDP method demonstrated effective enhancement in the dynamics core of the Model for Prediction Across Scales-Atmosphere (MPAS-A), this study explores the potential of extending the QDP approach to both the dynamics core and tracer components. The impact of the QDP method on these two components is explored through a series of planned experiments using idealized and real-data cases. By applying QDP to both the dynamics and tracer components, this research aims to assess the joint effects on model accuracy and efficiency, seeking to demonstrate the feasibility of further enhancing model performance without significantly increasing computational resources. This study offers a promising path toward more cost-effective simulations in numerical weather prediction and climate modeling.

How to cite: Lai, J. and Wang, L.: Enhancing Numerical Model Accuracy with Quasi Double-Precision: Extending the Application to Dynamics and Tracers in MPAS-A, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2641, https://doi.org/10.5194/egusphere-egu25-2641, 2025.

Global numerical modeling is entering the era of kilometer-scale, non-hydrostatic, and AI-powered. Meanwhile, heterogeneous computing is the trend in HPC. As a strong candidate for the next-generation global kilometer-scale GCM, the A-grid dynamical core based on LMARS (Low Mach number Approximate Riemann Solver) needs to address the following three issues: 1. The strong-gradient problem is particularly significant at high resolutions. Although LMARS can use higher-order numerical schemes, it cannot guarantee monotonicity. 2. The large discrepancy between vertical and horizontal grid spacings severely limits the time integration step size of the non-hydrostatic model. 3. Classic models are written in FORTRAN, and algorithms designed for CPUs may not be suitable for GPUs. This study builds a prototype model LMARSpy with specific solutions to these issues: addressing the strong-gradient problem through a high-order monotonicity limiter, to solve the non-hydrostatic problem with a conserving vertical implicit solver, and building a Python-based high-performance computing platform to address heterogeneous computing challenge. A series of benchmark tests show that: 1. The monotonicity limiter effectively eliminates non-physical oscillations and maintains high-order accuracy in discontinuous regions, with a computational cost increase of only 10.4% on GPUs. 2. The vertical implicit solver relaxes CFL limitations in cases where vertical grid spacing is much larger than horizontal grid spacing, improving computational efficiency by at least an order of magnitude. 3. The Python high-performance computing platform supports the efficient operation of the dynamical core on both CPU and GPU computing platforms. The performance of a single GPU-based system can rival large computing clusters with over 325 standard CPU cores. Last but not least, with the PyTorch backend built-in, LMARSpy is born with efficient compatibility with machine learning.

How to cite: Wei-Kang, Z. and Xi, C.: A GPU-Ready LMARS-Based Nonhydrostatic Dynamical Core with a Monotonicity Limiter and a Vertical Implicit Solver, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2801, https://doi.org/10.5194/egusphere-egu25-2801, 2025.

EGU25-2978 | ECS | Orals | AS5.2

Impact of a New Submesoscale Parameterization Scheme on the Simulation of Kuroshio Extension in a High-Resolution OGCM 

Ziyi Zhang, Bo An, Zhiwei Zhang, and Yongqiang Yu

Impact of a New Submesoscale Parameterization Scheme on the Simulation of Kuroshio Extension in a High-Resolution OGCM

Ziyi Zhang1,2, Bo An1, Zhiwei Zhang3 and Yongqiang Yu1,2

  • Key Laboratory of Earth System Numerical Modeling and Application, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029
  • University of Chinese Academy of Sciences, Beijing 100049
  • Ocean University of China, Qingdao 266100

ABSTRACT

    In this study, we investigate the impact of a new submesoscale parameterization scheme developed by Zhang et al. (2023; Zhang23 parameterization hereafter) on the simulation performance of the regional version of the 1/10° ocean model LICOM3.0 in the North Pacific. Specifically, a set of numerical experiments with and without Zhang23 parameterization scheme are conducted to study changes in thermal and dynamic characteristics in the Kuroshio Extension region resulting from the submesoscale processes. Compared to the control experiment, the deeper bias in the winter mixed layer depth(MLD) is significantly reduced in the sensitivity one with Zhang23 parameterization in the Kuroshio Extension region, by 26.7m (24.0%) on average. The simulated Kuroshio Extension shifts southward by about one degree of latitude from 36.5°N to 35.5 °N, closer to the observations.

    The simulated SST in the sensitivity run is much cooler than in the control run in the KE region. This contradicts the change in net surface heat flux, implying that the internal dynamical mechanism dominates these changes. Further analyses suggest that the vertical heat fluxes caused by parameterized submesocale processes are mainly concentrated at 39-40°N, 140-150°E in winter. This results in significant warming in the upper 100 m and cooling below, contributing to mixed layer restratification. The ocean heat content decreases in the region where the most energic mesoscale eddy exist in KE region, resulting in a weaker meridional thermal gradient at 37°N. This leads to a southward shift of the ocean front in the upper ocean and KE axis, which weakens meridional heat transport, and thus exacerbates the SST cooling north of 37°N. Although the vertical heat flux of the Zhang23 parameterization occurs primarily in winter, the cold SST anomalies in the subsurface are maintained throughout the year via the reemergence mechanism. The parameterization scheme directly affects winter temperatures by promoting upward heat transport, which warms the surface and cools the subsurface, leading to a southward shift and weakening of the WBC. In other seasons, it influences temperatures via current changes, maintaining a cooling anomaly in the north surface and subsurface layers. Overall, this results in a highly variable surface layer and a relatively stable cold subsurface layer. 

    This study demonstrates the good performance of Zhang23 submesoscale parameterization in improving the simulation of Kuroshio extension in the eddy-resolving OGCM. It reveals the key role of vertical heat transport by submesoscale processes and other oceanic dynamical mechanisms in modulating the sea temperature and its seasonal variation in the Kuroshio Extension region.

How to cite: Zhang, Z., An, B., Zhang, Z., and Yu, Y.: Impact of a New Submesoscale Parameterization Scheme on the Simulation of Kuroshio Extension in a High-Resolution OGCM, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2978, https://doi.org/10.5194/egusphere-egu25-2978, 2025.

In this study, the characteristics of Western North Pacific tropical cyclones (TCs) simulated in 1985 to 2014 by a climate system model FGOALS-f3-H that participated in the HighResMIP are evaluated. The simulations from the stand-alone atmospheric and fully coupled versions are inspected to explore the effects of ocean coupling. Results show that the model can capture the main TC characteristics in tracks, amounts, and genesis locations. The seasonal and interannual variation of TC genesis frequency (TCGF) are reasonably simulated, as well as the wind-pressure relationship (WPR), horizontal structures, and TC-induced precipitation. However, some obvious biases remain in both versions, mainly in the TC intensity and TCGF distributions. The simulation shows a much smaller number of super typhoons (SSTY) and tropical storms (TS), and a larger number of severe typhoons (STY), typhoons (TY), and severe tropical storms (STS). The TCGF shows underestimated biases in the west of 140E with less genesis of all categories, and overestimated biases in the east of 140E with more genesis of STY, TY, and STS, corresponding to the biases of intensity distributions. The overestimated TCGF biases are more obvious in coupled simulation which can be explained by the TC genesis potential index (GPI). The stronger biases of relative humidity, potential intensity and vertical wind shear contribute to the higher GPI biases together with warm sea surface temperature (SST) biases and weak Western Pacific subtropical high (WPSH). The model shows a stronger seasonal cycle in atmospheric simulation which is improved in coupled simulation but remains stronger. Meanwhile, the TCGF interannual variation in atmospheric simulation shows a better correlation with the observation (coefficient of 0.44 vs 0.14). The annual TCGF shows similar patterns in empirical orthogonal function (EOF) analysis, and the first principal component (PC1) is relevant to the Nino3.4 index, suggesting that TCGF is simultaneously modulated by the El Niño-Southern Oscillation (ENSO). Therefore, the poor interannual variation in coupled simulation can be attributed to a weak ENSO. For WPR, the simulation shows a larger wind speed with same sea level pressure, but the coupled simulation shows a closer WPR to the observation. The simulated horizontal structures of winds and pressure are similar in atmospheric and coupled simulation, while the warm core of intense TCs is stronger in coupled simulation. The simulated precipitation is overestimated which can be weakened in coupled simulation. The coupled simulation can also capture the observed SST cooling of TCs, while the atmospheric simulation cannot, showing more reasonable atmosphere-ocean interactions. Overall, ocean coupling can improve some details of the simulated TCs but not the climatology due to ocean biases and coupled interactions, the better TC simulation in a coupled model requires improvements on both atmospheric and ocean models.

How to cite: Guo, Y. and Yu, Y.: The simulation of tropical cyclones in the Western North Pacific by a climate system model FGOALS-f3-H and the effects of ocean coupling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3460, https://doi.org/10.5194/egusphere-egu25-3460, 2025.

EGU25-4105 | Orals | AS5.2

The sensitivity of a climate model to numerical mixing in its ocean component 

Alex Megann, Dan Copsey, Amber Walsh, and Ollie Tooth

We describe the sensitivity of an ensemble of integrations of the HadGEM3-GC5 coupled model, with a ¼° ocean and N96 (~130km) atmosphere, to settings in the ocean component that have been demonstrated to affect the numerical mixing in forced simulations. This configuration is closely related to the UK contribution to CMIP7. The ensemble is integrated for 60 years with constant present-day greenhouse forcing.

The ocean surface temperature has a robust response to numerical mixing, with increased mixing leading consistently to warming over the global ocean by up to 0.5°C, while reducing mixing cools the surface by a similar degree. The response of the surface air temperature is closely similar to that of the SST, and is seasonally amplified at high latitudes in the respective winter. We present large-scale ocean and atmospheric metrics, and discuss mechanisms for the counter-intuitive sign of the sensitivity of surface temperatures in these simulations to numerical mixing in the ocean, in which more mixing warms the surface and vice versa.  This sensitivity is significant, since it is comparable with the surface temperature changes expected in a simulation with historical or future greenhouse scenario forcings, and we shall speculate on the implications for modelling future climates.

How to cite: Megann, A., Copsey, D., Walsh, A., and Tooth, O.: The sensitivity of a climate model to numerical mixing in its ocean component, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4105, https://doi.org/10.5194/egusphere-egu25-4105, 2025.

EGU25-4566 | Posters on site | AS5.2

Fully implicit timestepping methods for the rotating shallow water equations 

Werner Bauer and Colin J. Cotter

Fully implicit timestepping methods have several potential advantages for atmosphere/ocean simulation. First, being unconditionally stable, they degrade more gracefully as the Courant number increases, typically requiring more solver iterations rather than suddenly blowing up. Second, particular choices of implicit timestepping methods can extend energy conservation properties of spatial discretisations to the fully discrete method. Third, these methods avoid issues related to splitting errors that can occur in some situations, and avoid the complexities of splitting methods. Fully implicit timestepping methods have had limited application in geophysical fluid dynamics due to challenges of finding suitable iterative solvers, since the coupled treatment of advection prevents the standard elimination techniques. However, overlapping Additive Schwarz methods, as introduced for geophysical fluid dynamics by Cotter and Shipton (2023), provide a robust, scalable iterative approach for solving the monolithic coupled system for all fields and Runge-Kutta stages. In this study we investigate this approach applied to the rotating shallow water equations, facilitated by the Irksome package (Farrell et al, 2021) which provides automated code generation for implicit Runge-Kutta methods. We compare various schemes in terms of accuracy and efficiency using an implicit/explicit splitting method, namely the ARK2 scheme of Giraldo et al (2013), as a benchmark. This provides an initial look at whether implicit Runge Kutta methods can be viable for atmosphere and ocean simulation.


References:

Cotter, Colin J., and Jemma Shipton. "Mixed finite elements for numerical weather prediction." Journal of Computational Physics 231, no. 21 (2012): 7076-7091.

Farrell, Patrick E., Robert C. Kirby, and Jorge Marchena-Menendez. "Irksome: Automating Runge–Kutta time-stepping for finite element methods." ACM Transactions on Mathematical Software (TOMS) 47, no. 4 (2021): 1-26.

Giraldo, Francis X., James F. Kelly, and Emil M. Constantinescu. "Implicit-explicit formulations of a three-dimensional nonhydrostatic unified model of the atmosphere (NUMA)." SIAM Journal on Scientific Computing 35, no. 5 (2013): B1162-B1194.

How to cite: Bauer, W. and Cotter, C. J.: Fully implicit timestepping methods for the rotating shallow water equations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4566, https://doi.org/10.5194/egusphere-egu25-4566, 2025.

EGU25-4636 | ECS | Posters on site | AS5.2

Land Components Control the ENSO Representation in the Earth System Model MIROC-ES2L 

Keiichi Hashimoto, Tomohiro Hajima, Hiroaki Tatebe, Takahito Kataoka, and Hiroaki Miura

Terrestrial vegetation affects the atmosphere through both biogeochemical and physical processes. Radiative forcing is affected by carbon uptake and release, while albedo, evapotranspiration, and surface roughness also depend on vegetation. In Earth system models (ESMs), vegetation growth is often represented by prognostic simulations of the leaf area index (LAI). MIROC-ES2L, an ESM version of the MIROC climate model, simulates a larger El Niño-Southern Oscillation (ENSO) amplitude compared to simulations that prescribe observed LAI.

To investigate the cause of this enhanced ENSO amplitude in MIROC-ES2L, we compared the feedback processes contributing to El Niño growth in two experiments: one with observed LAI and the other with model-prognosed LAI. The prognosed LAI experiment showed stronger zonal advection, Ekman, and meridional advection feedbacks, associated with warmer sea surface temperatures (SSTs) in the eastern equatorial Pacific.

Sensitivity experiments were conducted to identify the regions where LAI contributes most significantly to SST changes. These experiments constrained LAI to observed values in specific regions, while using model-prognosed values elsewhere. The results show that the ENSO amplitude is particularly sensitive to LAI over South America, where the model overestimates LAI along the west coast.

We conclude that the underlying mechanism is as follows: increased LAI over South America induces surface cooling due to enhanced latent heat release. This modifies the tropospheric circulation, weakening the local Walker circulation over the Andes and consistently altering the SST distributions. The resulting SST warming off the coast of Peru enhances the convective response to SST anomalies, strengthening the effective Bjerknes feedback and amplifying ENSO.

How to cite: Hashimoto, K., Hajima, T., Tatebe, H., Kataoka, T., and Miura, H.: Land Components Control the ENSO Representation in the Earth System Model MIROC-ES2L, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4636, https://doi.org/10.5194/egusphere-egu25-4636, 2025.

EGU25-5694 | ECS | Orals | AS5.2

Development of a GPU-accelerated, Finite Element based Dynamical Core for Sea Ice 

Robert Jendersie, Christian Lessig, and Thomas Richter

Sea ice is an import part of Earth's climate system. Yet, an accurate, highly resolved simulation of sea ice dynamics remains challenging. As the development of faster processors has slowed down, a turn to more specialized hardware is needed to achieve more accurate simulations at higher resolutions. Graphics processing units (GPUs) offer an order of magnitude higher floating-point performance and efficiency compared to CPUs. However, their full utilization often also requires significant engineering effort. Therefore, several frameworks have emerged in recent years which aim to simplify general-purpose GPU programming. In particular, heterogeneous compute frameworks such as SYCL and Kokkos make it possible to develop a unified code base that works accross GPUs and CPUs. Similarly, machine learning frameworks like PyTorch combine an easy to use interface with highly specialized backends that can make it possible to transparently exploit new hardware features to accelerate large-scale linear algebra workloads. Furthermore, their use provides a simple path-way to integrate machine learning components into simulations.

In this talk, we compare available options for the GPU-parallelizaton of the novel sea-ice code neXtSIM-DG. Its dynamical core is based on higher-order finite elements for the momentum equation and discontinous Galerkin elements for the advection. This makes the code highly parallezible. We discuss characteristics of our discretization and its consequences for the GPU implementation. For the full port of the dynamical core we use Kokkos as, based on our assessement, it combines usability with good performance. With moderate changes compared to the OpenMP-based CPU code, the new implementation achieves a sixfold speedup on the GPU while being as fast as the reference on the CPU.

How to cite: Jendersie, R., Lessig, C., and Richter, T.: Development of a GPU-accelerated, Finite Element based Dynamical Core for Sea Ice, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5694, https://doi.org/10.5194/egusphere-egu25-5694, 2025.

EGU25-5990 | ECS | Posters on site | AS5.2

Biases in model simulations of Indian Summer monsoon low-pressure systems  

Mahendra Singh, Govindasamy Bala, and Ashwin K. Seshadri

Monsoon low-pressure systems (LPSs) during the Indian Summer monsoon season are crucial synoptic-scale phenomena over the Indian subcontinent.  An average of about 14 LPSs per summer monsoon season form contributing approximately 60-70 percent of rainfall over large parts of India. Many previous modelling studies have shown a systematic bias of a southward shift in LPS activity and a dry bias over the monsoon core zone of ISM.  This study is an attempt to account for these biases in the NCAR Community Earth System Model (CESM2.1.3) simulation. Our present-day simulation using the fully coupled configuration of the model shows a southward shift in LPS activity compared to ERA5 reanalyses, consistent with prior studies showing similar biases in CMIP5 (Coupled Model Intercomparison Project Phase 5) model simulations relative to various reanalysis datasets.

We show that biases in simulating LPS activity in CESM2.1.3 are related to a southward bias in the latitude of the low-level westerly jet as well as a dry bias over northwestern India. The simulated monsoon low-level jet, typically located poleward of the zero absolute vorticity contour, is more east-west oriented and biased southward in the model simulation compared to ERA5. This is due to enhanced meridional advection of negative absolute vorticity over the central Indian Ocean below the zero absolute vorticity contour from increased cross-equatorial flow and reduced meridional advection of positive absolute vorticity over the western Arabian Sea above the zero absolute vorticity contour. Further, it is likely that a bias towards larger dry air intrusion from the north and west of Arabian Sea into India leads to a southward displacement of the monsoon low-level jet. This shift adversely affects LPS genesis and growth in northern and northwestern India, leading to a southward bias in LPS activity in model simulations as compared to reanalysis data. We also offer evidence to show that the southward shift in LPS activity and the dry air intrusion into northwest India are nearly common biases across the three generations (CMIP3, CMIP5 and CMIP6) of climate models, contributing to a dry bias over the monsoon core zone of the Indian summer monsoon.

How to cite: Singh, M., Bala, G., and Seshadri, A. K.: Biases in model simulations of Indian Summer monsoon low-pressure systems , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5990, https://doi.org/10.5194/egusphere-egu25-5990, 2025.

EGU25-6374 | ECS | Posters on site | AS5.2

Impact of vertical velocity damping on the numerical stability and atmospheric representation in ICON 

Tat Chi Wong, Clarissa Kroll, and Robert Jnglin Wills

The upper portion of atmospheric models typically employ a damping (sponge) layer to absorb upward-propagating wave energy, thereby preventing spurious wave reflections from the rigid model top. In the Icosahedral Nonhydrostatic Weather and Climate Model (ICON), implicit Rayleigh damping is applied on the vertical velocity following the approach of Klemp et al., 2008. In high-resolution simulations, the waves resolved in the model can increase substantially. Insufficient damping leads to more frequent model crashes due to numerical instability. While increasing the amount of damping might be a simple and intuitive adjustment, excessive damping can also induce back reflections from the damping layer itself, causing spurious standing oscillations. It is therefore crucial to carefully adjust the damping settings with sensitivity experiments. 

We analyze a set of ICON simulations with different damping settings. These are 1-month simulations with a horizontal resolution of 10 km. The goal is to provide insights into the optimal damping settings that can improve numerical stability in high-resolution simulations without compromising the atmospheric representation. Evaluation of the mean wind field outside of the damping layer shows no significant changes across different damping settings. However, spurious standing oscillations are observed in the tropical stratosphere. Further examination demonstrates that these oscillations align with the vertical grids, an indication that they can possibly be caused by vertical discretization error rather than back reflections from the damping layer. Investigation of Eliassen-Palm (EP) flux using Transformed Eulerian Mean (TEM) analysis also shows no significant change in the mean EP flux at the damping layer height due to changing damping coefficient. This suggests no major change in back reflections from the damping layer. Overall, our current results show that increasing the amount of damping could improve numerical stability with no indication of severely altered atmospheric representation over the 1-month time frame. Further analysis through long-term simulations will be necessary to assess the possible impact on longer timescales. 

References
Klemp, J. B., Dudhia, J., and Hassiotis, A. D. (2008). An Upper Gravity-wave Absorbing Layer for NWP Applications. Mon. Wea. Rev., 136(10), 3987–4004. doi: 10.1175/2008MWR2596.1

How to cite: Wong, T. C., Kroll, C., and Jnglin Wills, R.: Impact of vertical velocity damping on the numerical stability and atmospheric representation in ICON, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6374, https://doi.org/10.5194/egusphere-egu25-6374, 2025.

EGU25-6960 | Orals | AS5.2

Rational Approximation of Exponential Integration (REXI) for dynamical cores 

Martin Schreiber and Jed Brown

This presentation focuses on numerical solutions for Initial Value Problems (IVPs) involving linear PDEs dominating the time step size, as is the case for dynamical cores. We investigate using Rational Approximation of Exponential Integration (REXI). REXI replaces sequential time-stepping with a sum of rational terms, enabling parallelization and exploiting additional scalability on supercomputers for spatially limited problems.

We introduce the "unified REXI" method, showing its algebraic equivalence to methods developed decades ago, such as implicit Runge-Kutta methods, Cauchy-contour integration, and direct approximations. Our studies involve basic test cases for dynamical cores, offering a detailed numerical investigation, discussion, and comparisons of REXI methods. We address numerical issues and propose workarounds where feasible. Performance comparisons are conducted using nonlinear shallow-water equations on a rotating sphere on high-performance computing systems.

In addition to exposing more parallelism for faster solutions, we evaluate resource efficiency at prescribed accuracy. Our findings reveal that diagonalized lower-order Gauss Runge-Kutta methods (formulated as REXI) achieve a 64x reduction in computational resource requirements compared to prior work.

How to cite: Schreiber, M. and Brown, J.: Rational Approximation of Exponential Integration (REXI) for dynamical cores, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6960, https://doi.org/10.5194/egusphere-egu25-6960, 2025.

EGU25-7001 | ECS | Orals | AS5.2

Parameterization adaption needed to unlock the benefits of increased resolution for the ITCZ in ICON 

Clarissa Kroll, Andrea Schneidereit, Robert Jnglin Wills, Luis Kornblueh, and Ulrike Niemeier

The double Inter-Tropical Convergence Zone (ITCZ) feature is a prominent bias in the precipitation distribution simulated by most weather and climate models. Its persistence over several CMIP generations without substantial improvements is one factor motivating the investigation of whether higher resolution and the discard of parameterizations can solve the misrepresentation of large-scale atmospheric circulation. In this work, we analyze uncoupled simulations with the Icosahedral Nonhydrostatic Weather and Climate Model, ICON, in the eXtended Predictions and Projections configuration (XPP), spanning horizontal resolutions from 160 km up to 5 km. Although improvements in the precipitation bias are apparent due to the better representation of orography starting at 40 km horizontal resolution, we demonstrate that the double ITCZ feature persists over the entire resolution spectrum – even if deep convective parameterization is discarded at 5 km. In a subsequent sensitivity study, we can tie the emergence of the double ITCZ to biases in the near surface humidity arising from the turbulence scheme. We perform a physically motivated parameter optimization to correct for the bias in near surface specific humidity and can reduce tropcial precipitation biases over the entire resolution hierarchy. Our findings not only showcase the benefits of models supporting various resolutions but also underline the importance of further developing indispensable parameterizations.

How to cite: Kroll, C., Schneidereit, A., Jnglin Wills, R., Kornblueh, L., and Niemeier, U.: Parameterization adaption needed to unlock the benefits of increased resolution for the ITCZ in ICON, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7001, https://doi.org/10.5194/egusphere-egu25-7001, 2025.

EGU25-7497 | Posters on site | AS5.2

Effects of the high-resolution river routing model on seasonal prediction model 

Suryun Ham, Johan Lee, and Beomcheol Shin

To improve the prediction skill of Korea Meteorological Administration climate prediction system (KMA-GloSea6), high-resolution river routing model in land surface model are implemented. The characteristics of the current river routing model were investigated and pointed out the weakness. It was found that GloSea6 uses a relatively simple river routing model, and the simulated river storage is overestimated compared to the observation. To simulate accurate river flow and air-land-sea interaction, it is most desirable to coupling a sophisticated and realistic river routing model. As a simple method, it was tried to reduce the amount of freshwater flowing into the ocean by increasing the resolution in same river routing model. The GloSea6, which can replace the existing 1-degree resolution with 0.5-degree and 0.125-degree resolution for river routing model, was newly constructed. Also, as the resolution of the river routing model changed, the setting coefficients for the meandering and river flow velocity were optimized. It is clear that the newly conducted system reduces errors in river flow and discharge compared to existing operational system. The simulation with optimized high-resolution river routing model shows reduced biases in ocean circulation and temperature, especially in the Pacific and Indian Oceans. These results can be useful in improving seasonal prediction due to more accurate air-sea interaction and in applied and policy research on water resources.

How to cite: Ham, S., Lee, J., and Shin, B.: Effects of the high-resolution river routing model on seasonal prediction model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7497, https://doi.org/10.5194/egusphere-egu25-7497, 2025.

This study investigates a climate dynamics model that incorporates topographical effects and the phase transformation of water vapor. The system comprises the Navier–Stokes equations, the temperature equation, the speciffc humidity equation, and the water content equation, all adhering to principles of energy conservation. Applying energy estimation methods, the Helmholtz–Weyl decomposition theorem, and the Brezis–Wainger inequality, we derive high-order a priori estimates for state functions. Subsequently, based on the initial data assumptions V0 ∈ H4 (Ω), T0, q0, mw0 ∈H2 (Ω), we can prove that a strong solution to this system exists globally in time and establish the uniqueness of the global strong solution.

How to cite: Lian, R., Ma, J., and Zeng, Q.: Global existence of the strong solution to the climate dynamics model with topography effects and phase transformation of water vapor, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7966, https://doi.org/10.5194/egusphere-egu25-7966, 2025.

EGU25-14018 | ECS | Posters on site | AS5.2

A composable climate model in pure Julia  

Simone Silvestri, Gregory Wagner, Milan Klower, Maximilian Gelbrecht, and Navid Constantinou

Coupled general circulation models of atmosphere and ocean form the heart of every earth-system model. Currently,  the only languages used to write a model at that complexity are Fortran and C, which are limited by traditional programming patterns. However, modern languages like Python and Julia shine with interactivity, accessibility, and extensibility, yet a coupled model of that complexity, written in a modern language, has not yet been attempted. Here, we present a coupled climate model implemented entirely in the Julia programming language. The model integrates an atmospheric component based on the SpeedyWeather.jl library with the ClimaOcean.jl package for ocean and sea-ice dynamics. This approach leverages Julia's strengths combining computational efficiency with a high-level programming interface. The result is a climate modeling framework that maintains computational efficiency without sacrificing flexibility. The dynamical core employs high-order numerical methods, combining Weighted Essentially Non-Oscillatory (WENO) advection schemes in the ocean and spectral methods in the atmosphere, ensuring a robust and accurate representation of transport processes. A high-level interface for coupling the codes is introduced, which is distinctly more flexible than traditional couplers. This interface allows running coupled simulations on laptops as well as high-performance computing (HPC) resources. We will present initial results from coupled idealized simulations, highlighting key features such as boundary currents in the ocean, convective patterns in the atmosphere, and air-sea interactions.

How to cite: Silvestri, S., Wagner, G., Klower, M., Gelbrecht, M., and Constantinou, N.: A composable climate model in pure Julia , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14018, https://doi.org/10.5194/egusphere-egu25-14018, 2025.

The Amundsen Sea Low (ASL) is a connection between the tropical variabilities and climate changes in the Antarctic. The combination of negative trend of the Interdecadal Pacific Oscillation (IPO) and the positive trend of the Atlantic Multidecadal Oscillation (AMO) is recognized to result in the strengthening of the Amundsen Sea Low (ASL) as well as the change of the Antarctic sea ice in recent decades. In this study, we demonstrate that models in the Coupled Model Intercomparison Project phase 6 (CMIP6) largely underestimate the combined influence of IPO and AMO on the ASL variability. The unrealistic relationship between IPO and AMO among coupled models, which potentially cancels out their effects on the ASL each other, is one potential factor for the underestimated ASL variability. Another factor is the large inconsistent AMO-related teleconnection patterns among models. Further analysis is carried out to explore the origin of the large model spread, and the result suggests that the cool mean SST biases over the northern tropical Atlantic Ocean and the warm mean SST biases over the southeastern Pacific are both found to be the dominant source for the underestimated ASL change. These results emphasize the collaborative effect of the IPO and AMO to the Southern Ocean region and the related model biases among the coupled models.   

How to cite: Cai, D.: Underestimated trends of Amundsen Sea Low associated with unrealistic interdecadal tropical variability in CMIP6 models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14770, https://doi.org/10.5194/egusphere-egu25-14770, 2025.

EGU25-15654 | ECS | Orals | AS5.2

Towards dynamic adaptive mesh refinement in Earth system models 

Kerstin Hartung, Benedict Geihe, Chiara Hergl, Johannes Holke, Patrick Jöckel, Johannes Markert, and Michael Schlottke-Lakemper

The currently available computing power severely limits the spatial resolution in chemistry climate simulations, even on upcoming exascale machines. This is mainly due to the large number of prognostic variables which includes chemical tracers. To further enhance the reliability and accuracy of climate projections, small scales need to be better resolved.

Adaptive methods enable a continuously re-adjusted focus of computational power in time and space. This increases the achievable level of detail considerably, while reducing the time to solution and resource consumption. However, adaptivity requires a sophisticated selection of adaptation criteria, algorithms, memory layouts, and communication patterns to fully utilize modern HPC infrastructures.

Additionally, discontinuous Galerkin methods promise to increase the effective resolution, i.e. by employing high order polynomials, so that prognostic variables are better resolved, even on coarser meshes. Most of the additional computation is done locally, so that the overall algorithm is ideally suited for parallel execution. The typical lack of robustness of higher-order methods can be remedied by utilizing state-of-the-art entropy stable schemes.

In this conference contribution, we will present the setup and the interfaces between MESSy, Trixi.jl and t8code as well as results from a prototypical simulation that showcases the interaction, application, and challenges of dynamic adaptive meshes.
 Here, MESSy is a software framework that allows to integrate multiple numerical model components to build regional and global chemistry climate models. t8code is a parallel mesh management library written in C++. Finally, Trixi.jl is a computational fluid dynamics solver, build around a modern Discontinuous Galerkin method, and written in the Julia programming language.
 This work was performed within the project ADAPTEX (ADAPtive Earth system modelling with strongly reduced computation time for EXascale-supercomputers), which aims to evaluate the potential benefit of dynamic adaptive meshes in ESM.

How to cite: Hartung, K., Geihe, B., Hergl, C., Holke, J., Jöckel, P., Markert, J., and Schlottke-Lakemper, M.: Towards dynamic adaptive mesh refinement in Earth system models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15654, https://doi.org/10.5194/egusphere-egu25-15654, 2025.

EGU25-16648 | Posters on site | AS5.2

Fast-wave slow-wave spectral deferred correction methods applied to the compressible Euler equations 

Jemma Shipton, Alex Brown, Joscha Fregin, Thomas Bendall, Thomas Melvin, Thomas Baumann, and Daniel Ruprecht

In numerical weather prediction and climate modelling, semi-implicit time-stepping methods have long been favoured for their ability to take large time steps without excessively damping slow-moving waves. Fast-Wave Slow-Wave Spectral Deferred Correction (FWSW-SDC) methods offer an attractive alternative, achieving arbitrary-order accuracy by iteratively solving a collocation problem, akin to implicit Runge-Kutta methods. Similar to semi-implicit methods, FWSW-SDC improves stability compared to fully explicit schemes, enabling large time steps while retaining accuracy. Additionally, the rich literature on parallel-in-time SDC methods presents opportunities for both parallelization within the correction process and across time steps.

In this poster, we extend prior work with FWSW-SDC from linear systems to the nonlinear compressible Euler equations, evaluating its potential for numerical weather prediction and climate modelling applications. We apply SDC methods to standard dynamical core test cases, including the non hydrostatic gravity wave, moist rising bubble, and baroclinic wave tests, to assess stability, accuracy, and computational performance. Finally, we explore the implementation of parallelisable SDC preconditioners in the FWSW framework.

How to cite: Shipton, J., Brown, A., Fregin, J., Bendall, T., Melvin, T., Baumann, T., and Ruprecht, D.: Fast-wave slow-wave spectral deferred correction methods applied to the compressible Euler equations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16648, https://doi.org/10.5194/egusphere-egu25-16648, 2025.

EGU25-16827 | ECS | Posters on site | AS5.2

Developing ECMWF’s portable next-generation atmospheric dynamical core 

Sara Faghih-Naini, Till Ehrengruber, Christian Kühnlein, Lukas Papritz, and Peter Dueben

Numerical weather prediction directly benefits from advancements in the accuracy, efficiency, and scalability of the atmospheric model. We present the development of a performance-portable high-level Python-based framework for the next-generation ECMWF global atmospheric dynamical core, enabling simulations at unprecedented numerical resolutions. This new model framework, called the Portable Model for Multi-Scale Atmospheric Prediction (PMAP), is an advancement of the Finite-Volume Module (FVM) originally developed in Fortran at ECMWF.

A key feature of the global PMAP is its implementation with the latest version of the GridTools for Python (GT4Py) domain-specific library, named gt4py.next. This library is tailored to the efficient implementation of conservative finite-volume discretization methods that support, among others, ECMWF’s operational octahedral grid. Co-developed with various Swiss partners, the gt4py.next library itself is under continuous extension, optimization, and refinement alongside the PMAP. The model runs distributed across multiple nodes, enabling large-scale simulations on modern supercomputers with accelerators.

We present recent model validation results and provide an analysis of its performance, portability, and scalability on latest European supercomputing platforms.

How to cite: Faghih-Naini, S., Ehrengruber, T., Kühnlein, C., Papritz, L., and Dueben, P.: Developing ECMWF’s portable next-generation atmospheric dynamical core, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16827, https://doi.org/10.5194/egusphere-egu25-16827, 2025.

EGU25-17712 | Posters on site | AS5.2

Technical improvements with the GLOBO atmospheric model, through collaboration with ESiWACE3 

David Guibert, Loris Lucido, Erwan Raffin, Alessio Bellucci, Paolo Davini, Frederico Fabiano, Antenolla Galizia, Valerio Lembo, and Daniele Mastrangelo

GLOBO is an atmospheric general circulation model developed at the Institute of Atmospheric Sciences and Climate of the National Research Council of Italy (CNR-ISAC). It is largely equivalent to the BOLAM atmospheric model, used for synoptic-scale operational numerical weather prediction. The GLOBO model is currently part of the S2S multi-model initiative for prediction at the sub-seasonal to seasonal timescale range. 

Here, we present improvements to the performance of GLOBO that were obtained through collaboration with the ESiWACE3 initiative. This service is aimed at supporting the exascale preparations for the weather and climate modelling community in Europe through the establishment of short collaborative projects between Research Software Engineers (RSEs) and model development groups. These collaborations provide guidance, engineering, and advice to improve model efficiency and port models to existing and upcoming computing infrastructures

The main tasks that were carried out throughout the collaboration were aimed at:

  • getting a better vectorized instruction set on AMD processors using the Intel compilers
  • improving the efficiency of inline functions called inside some loops
  • gathering parallel communications before waiting for the data to be exchanged
  • reducing the number of unnecessary or redundant communications;

The model was tested at a 78km horizontal resolution with a number of processors ranging  between 8 and 240. An improvement in the scalability of the model was observed, leading up to 25-34% speedup (on 240 or 160 processors resp.).

How to cite: Guibert, D., Lucido, L., Raffin, E., Bellucci, A., Davini, P., Fabiano, F., Galizia, A., Lembo, V., and Mastrangelo, D.: Technical improvements with the GLOBO atmospheric model, through collaboration with ESiWACE3, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17712, https://doi.org/10.5194/egusphere-egu25-17712, 2025.

EGU25-19121 | ECS | Posters on site | AS5.2

FRIDOM: A new modular Python based framework for geophysical fluid simulations 

Silvano Rosenau and Carsten Eden

Numerical modeling frameworks are essential for advancing our understanding of oceanic and atmospheric processes. Traditional ocean models, often written in Fortran, offer high computational efficiency but can be challenging for young scientists due to their complexity and lack of GPU support.

We present the Framework for Idealized Ocean Models (FRIDOM), a Python-based and modular framework for fluid simulations. Inspired by machine learning frameworks like TensorFlow and PyTorch, FRIDOM’s flexible design supports applications beyond ocean-specific contexts or idealized setups. Realistic setups with complex topography and realistic forcings are already possible. Currently, it includes implementations of the 2D shallow water equations and 3D nonhydrostatic Boussinesq equations, compatible with both rectilinear Arakawa C-grids and spectral grids. The framework is designed for seamless integration of new governing equations, grid types, such as unstructured grids used in FESOM, and discretization methods.

FRIDOM also provides advanced flow decomposition tools, including Optimal Balance and Nonlinear Normal Mode Decomposition, for separating balanced and wave components in flow fields. Comprehensive documentation, tutorials, and examples ensure accessibility, making FRIDOM a powerful and user-friendly framework for fluid modeling and analysis, with the capability of performing high-resolution simulations to address important questions in geophysical fluid dynamics.

How to cite: Rosenau, S. and Eden, C.: FRIDOM: A new modular Python based framework for geophysical fluid simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19121, https://doi.org/10.5194/egusphere-egu25-19121, 2025.

EGU25-19435 | Orals | AS5.2

Analysis of a Seamless Semi-Implicit Finite Volume Method for Atmospheric Flows 

Gottfried Hastermann and Rupert Klein

In this contribution, we present a non-standard, functional analytic framework to rigorously analyze the properties of the semi-implicit second-order finite volume discretization for the compressible Euler equations developed by Benacchio and Klein (2019). In experiments, this method shows favorable stability properties for geophysically relevant benchmarks and is capable of approximating the pseudo-incompressible and/or hydrostatic limit regime without changing the underlying discretization.
Our main results are the consistency and stability of the implicit projection step, which we achieve by choosing discontinuous velocity and continuous pressure variables. As a consequence, the classical divergence is replaced by its natural analogue, i.e., by line integrals along the boundary of a dual cell.
In contrast to preceding work, we consider general quadrilateral and cuboid meshes, and we provide an interpolation operator that is compatible with the natural divergence on the dual grid.
Aiming for a rigorous stability estimate of the overall scheme, we furthermore discuss a choice of advection operator that ensures compatibility.

How to cite: Hastermann, G. and Klein, R.: Analysis of a Seamless Semi-Implicit Finite Volume Method for Atmospheric Flows, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19435, https://doi.org/10.5194/egusphere-egu25-19435, 2025.

EGU25-19830 | Posters on site | AS5.2

Automating the construction of time-parallel 4DVar data assimilation systems for finite element models. 

Josh Hope-Collins, Jemima Tabeart, and David Ham

Data assimilation (DA) has made a significant contribution to the increase in forecast skill in recent decades by leveraging real-world observations to improve the states used in the forecasting system. However, the DA stage comprises a large part of the computational work of the system. Therefore, improving DA efficiency is crucial for continued improvements in forecast skill, which in turn requires high productivity software to be available for DA researchers.

 

4D variational assimilation (4DVar) is a DA method in common use operationally. 4DVar optimises an objective function (agreement with observations and prior forecasts) by updating a control (initial conditions) using the adjoint method. This requires running the linearised system forwards in time, and the system adjoint backwards in time, at every optimisation step. Weak constraint 4DVar is a modification that allows an "inexact model" and splitting the time-series into chunks. This enables reformulating each optimisation step as a saddle point problem, where the forward and adjoint models on each time-chunk can be run in parallel. This time-parallelism can potentially greatly decrease the time required for the optimisation.

 

The adjoint method is highly effective but requires differentiating every operation in the system. Manually differentiation requires high developer effort for new system components, while automatic numerical differentiation is often computationally inefficient. This is particularly problematic in the development stage, where researchers want to run a variety of methods on a variety of equations. This causes a gap between simple equations (e.g. Lorenz and heat) often used in research, and the fluids models in operational systems.

Symbolic differentiation aims to achieve the efficiency of manual differentiation with the automation of numerical differentiation, and provides a route to closing this gap.

 

We present a library for constructing the 4DVar system using symbolic automatic differentiation. This is achieved using: Firedrake, a finite element library which provides symbolic differentiation using UFL, a high level DSL; and pyadjoint, a library for symbolically recording code execution and automatically constructing the forward and adjoint models.

To construct the 4DVar system, the user need only run the forward model (i.e. dynamical core) and the observation operators once. Firedrake and pyadjoint record this run and calculate the linearised forward model and the adjoint model, from which all components of 4DVar can be constructed.

The implementation is both space and time parallel, enabling the real performance of the methods to be tested on HPC machines. Because pyadjoint is model agnostic, this library can be used for any equation simply by changing the finite element model. Minimising the code modification required for different models is key for improving researcher productivity. This not only allows a smoother transition up the model hierarchy, but also allows straightforward testing of different dynamical core discretisations. We will demonstrate the software API and discuss the design choices taken, and present preliminary results on different equations.

How to cite: Hope-Collins, J., Tabeart, J., and Ham, D.: Automating the construction of time-parallel 4DVar data assimilation systems for finite element models., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19830, https://doi.org/10.5194/egusphere-egu25-19830, 2025.

EGU25-252 | ECS | Orals | ITS1.16/AS5.4

A Comprehensive Assessment of Climate Data Bias-Adjustment Techniques Over Australia 

Alicia Takbash, Damien Irving, Justin Peter, Thi Lan Dao, Arpit Kapoor, Andrew Gammon, Andrew Dowdy, Mitchell Black, Ulrike Bende-Michl, Doerte Jakob, and Michael Grose

The National Partnership for Climate Projections (NPCP) aims to develop a consistent approach to deliver comparable, robust, fit-for-purpose future climate information to assess climate risks and inform adaptation planning. The NPCP climate projections roadmap identifies a number of priority areas of collaboration, including the delivery of national and regional downscaled climate projections. This involves selecting global climate models (GCMs), downscaling using regional climate models (RCMs), bias-adjusting model outputs, and conducting secondary and next-level analysis (e.g., impact modelling).

The focus on bias-adjustment is an acknowledgement of the fact that GCM and RCM outputs often show significant discrepancies when compared to observations. These systematic errors, or biases, can render raw outputs unsuitable for direct use in downstream impact models such as those for hydrology and agriculture, as well as in climate risk assessments. For the NPCP bias-adjustment intercomparison project, we evaluated various bias-adjustment techniques currently in use in the Australian climate research community. These include Equi-distant/ratio Cumulative Density Function matching (ECDFm), Quantile Matching for Extremes (QME), N-Dimensional Multivariate Bias Correction (MBCn), and Multivariate Recursive Nesting Bias Correction (MRNBC).

While previous studies have assessed some of these techniques for specific metrics and applications in Australia, our evaluation aimed to be broad and comprehensive. The participating techniques were applied to daily RCM data from the CORDEX-CMIP6 project for a baseline task, where bias-adjusted data were produced for the 1980-2019 period using 1980-2019 as a training period, as well as a cross-validation task, where data were produced for 1990-2019 using 1960-1989 for training. These bias-adjusted data were then compared to observations across Australia on various metrics relating to temperature and precipitation climatology, variability, statistical distribution and extremes. The impact of bias-adjustment on simulated trends was also assessed by producing bias-adjusted data for the 2060-2099 period. Additionally, we compared the bias-adjustment techniques with a simple quantile delta change approach and investigated scenarios where it may be sufficient to directly bias-adjust GCM data without the need for computationally expensive downscaling.

Based on the results of the intercomparison, the best-performing techniques were subsequently used by the Australian Climate Service (ACS) to bias-adjust outputs from the CORDEX-CMIP6 archive. This ensures the availability of a consistent set of high-resolution, bias-adjusted products for the Australian community to evaluate climate hazards and risks, and support adaptation planning.

How to cite: Takbash, A., Irving, D., Peter, J., Dao, T. L., Kapoor, A., Gammon, A., Dowdy, A., Black, M., Bende-Michl, U., Jakob, D., and Grose, M.: A Comprehensive Assessment of Climate Data Bias-Adjustment Techniques Over Australia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-252, https://doi.org/10.5194/egusphere-egu25-252, 2025.

EGU25-4123 | ECS | Orals | ITS1.16/AS5.4

Leveraging Deep Learning for Downscaling GOME-2 Atmospheric Data Using TROPOMI Observations 

Riccardo Ratta, Simone Mantovani, Maximilien Houël, Samuele Beccarini, Sebastiano Fabio Schifano, and Federico Fierli

The Global Ozone Monitoring Experiment 2 (GOME-2) and the TROPOspheric Monitoring Instrument (TROPOMI) are two significant satellite-based instruments dedicated to monitoring Earth’s atmosphere. GOME-2, part of the MetOp platform, has been operational since 2006, and was originally developed to monitor the ozone layer in the atmosphere. However, its onboard spectrometer can also detect pollutant gases, including NO2, which we will use as an initial example in this study.

GOME-2 spatial resolution is very coarse: a single data point is representative of an area of approximately 40 km x 80 km, which provides a broad view of atmospheric composition at global scale but limits its effectiveness in capturing fine-scale variations over cities and other human activity areas.

This study investigates whether TROPOMI high-resolution data can be utilized to downscale GOME-2 observations, potentially yielding insights into atmospheric changes dating back to 2006. We explore the implications of this process on spatial and radiometric accuracy and consider its broader significance for the future of satellite observations.

Given the abundance of available training data, we propose a novel approach involving deep learning. In particular, we used a combination of Residual Dense Blocks (RDBs) which state-of-the-art studies have shown to outperform similar Convolutional Neural Networks (CNNs) and Generative Neural Networks (GNNs) but still relies on the convolution operation, unlike transformers architectures (e.g., Vision Transformers ViTs). Then, to effectively train our model, we addressed challenges such as the resolution disparity between GOME-2 and TROPOMI (approximately a factor of 10), which requires working with a large pixel space, significantly increasing the memory needed for training. And the significant issue of missing data in atmospheric acquisition, e.g., due cloud cover.

Aside from the technical challenges of developing such model, the output validation plays a crucial role in ensuring the reliability and scientific utility of our results. We therefore evaluated our model performance on an independent dataset to verify the consistency of absolute reported NO2 values.

The approach involved training the model on one year of data (2023) over 10 selected locations and evaluate its performance using the ground-based Pandonia Global Network (PGN), a network of well-calibrated instruments designed to provide high-quality measurements of atmospheric trace gases at specific locations.

Results show an improvement not only limited to the reconstruction of fine details but also on the agreement of the absolute reported NO2 value between PGN data and the output from our model. We are currently working on expanding the dataset to further test the limits of our approach at global scale. Another active research area is the extension of the proposed approach to other common trace gases common between the two instruments. We hope to enhance the utility of this approach for broader applications in atmospheric science and to highlight the potential of leveraging deep learning downscaling for atmospheric data.

How to cite: Ratta, R., Mantovani, S., Houël, M., Beccarini, S., Schifano, S. F., and Fierli, F.: Leveraging Deep Learning for Downscaling GOME-2 Atmospheric Data Using TROPOMI Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4123, https://doi.org/10.5194/egusphere-egu25-4123, 2025.

EGU25-7043 | Posters on site | ITS1.16/AS5.4

Statistical downscaling applied to the CMCC Seasonal Prediction System 3.5 

Leonardo Aragão and Silvio Gualdi

The Italian Peninsula's climate is highly influenced by its complex topography and diverse regional weather systems, making high-resolution (HiRes) seasonal forecasting crucial for agriculture, water management, and energy sectors. Traditional seasonal prediction models, such as the CMCC Seasonal Prediction System (SPS3.5), provide valuable insights but lack the spatial resolution necessary to capture local-scale climatic details. Recent advances in Statistical Downscaling (SD) promise enhancing these coarse-resolution forecasts by generating more localised and accurate predictions. Thus, this study aims to provide a HiRes seasonal forecast for the Italian Peninsula by enhancing the SPS3.5 model through SD techniques tailored to the region's demand for finer-scale climate information.
The downscaling method involves a three-step process that utilises historical observational datasets and machine-learning techniques to refine SPS3.5 forecasts. The first regards the ground truth, composed of HiRes observational data from ERA5 reanalysis for 2m temperature (T2m), sea surface temperature, and 10m wind components, and from CHIRPS for precipitation. Then, SPS3.5 daily forecasts are spatially interpolated from 1º to 1/4° to match the observation data's grid. Finally, both data are combined through a machine-learning method based on the k-Nearest Neighbours (kNN) technique, which translates SPS3.5 into HiRes fields by matching forecasted conditions to observed patterns. The kNN algorithm utilises a set of k days of similar weather conditions (five predictors mentioned before) determined by the Euclidean distance to capture seasonally relevant weather analogues. Once the analogue days are defined, the kNN can forecast any meteorological field within the observational dataset. Finally, the SD method was accessed over the Italian Peninsula domain through cross-validation along the 24-year hindcast period available for SPS3.5 (1993-2016).
Preliminary results indicate that SD significantly enhances seasonal forecasts for the Italian Peninsula, achieving biases about 5-6 times smaller than the original SPS3.5 for all evaluated predictands. The main component of this improvement is the spatial accuracy promoted by downscaling, allowing the identification of domain characteristics unnoticed in SPS3.5. Even though the statistical indices show appreciable values for the domain as a whole when we evaluate smaller portions of this same domain, the original seasonal forecasts are still far from the desired. As expected, forecast bias increases with lead time also for kNN, with accuracy declining progressively from lead month 1 onward. For example, T2m bias increased from -0.14/-0.85°C in lead month 1 to -0.68/-1.41°C in month 6 (kNN/SPS3.5). This trend highlights the ongoing challenge of maintaining forecast skills over extended periods and the importance of adaptive correction strategies to extend lead-time reliability.
Integrating SD techniques with SPS3.5 outputs provides a promising solution for generating HiRes seasonal forecasts, offering valuable support for climate-sensitive applications by reducing forecast bias and enhancing spatial accuracy. This work demonstrates the potential of SD as an effective tool for bridging the gap between coarse seasonal forecasts and the localised weather information necessary for effective decision-making.

How to cite: Aragão, L. and Gualdi, S.: Statistical downscaling applied to the CMCC Seasonal Prediction System 3.5, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7043, https://doi.org/10.5194/egusphere-egu25-7043, 2025.

EGU25-8914 | Posters on site | ITS1.16/AS5.4

Adjusting the Weather Generator for Use in Operational Forecasting Weather-Dependent Processes 

Martin Dubrovský, Miroslav Trnka, Lenka Bartošová, and Petr Štěpánek

Weather generators (WGs) produce synthetic weather series, which are statistically similar to the real world weather series. The generators are used in assessing responses of weather-dependent processes on climate change (CC) or variability. Individual types of generators may differ in various parameters: (a) they may be parametric or non-parametric, (b) single-site or multi-site, (c) they differ in number of weather variables being generated and (d) the time step. Choice of these parameters depends on the purpose of their use. For example, in agrometeorology, single site (4-6)-variate daily generators are used to assess CC impacts on crop yields, which may include assessment of the sensitivity of the yields to changes in various climate characteristics.

In this contribution, we present our approach to using the generator in crop yield forecasting. Specifically, the crop yields are simulated by crop models, while the input weather series consisting of observational data till day D0 (when the forecast is made) are seamlessly followed by the synthetic series produced by the parametric single-site daily weather generator M&Rfi. Two approaches were implemented in M&Rfi to produce such series: (1) In the first, “operational” mode, the synthetic series are “forced” to exactly fit the available weather forecast, which accounts for the possible uncertainties and spans for the rest of the growing season; to make a probabilistic crop yield forecast, large number of possible weather series realisations is produced. (2) In the second, “research” mode, we do not assume to have a specific weather forecast, but we rather assume to have a knowledge on the accuracy of the available weather forecasts, which may be expressed as a function of the weather forecast error on the lead time. Having this function, we may produce a large ensemble of possible weather forecasts and corresponding ensemble of synthetic weather series.

Our methodology of producing synthetic weather series, which fit available weather forecasts, may be applied also for other weather dependent processes, for example in hydrological applications.

Acknowledgements: The experiment was made within the frame of projects PERUN (supported by TACR, no. SS0203004000) and YiPeeO (supported by ESA, no. 4000141154/23/I-EF).

How to cite: Dubrovský, M., Trnka, M., Bartošová, L., and Štěpánek, P.: Adjusting the Weather Generator for Use in Operational Forecasting Weather-Dependent Processes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8914, https://doi.org/10.5194/egusphere-egu25-8914, 2025.

EGU25-9167 | Posters on site | ITS1.16/AS5.4

Statistical downscaling of climate models for the Mediterranean region combining convolutional neural network and quantile delta mapping 

Marco D'Oria, Valeria Todaro, Daniele Secci, and Maria Giovanna Tanda

Regional climate projections are essential for guiding local governments in developing effective mitigation strategies. A common technique for downscaling General Circulation Model (GCM) outputs is dynamical downscaling, but its high computational demands have motivated the search for alternative approaches, including statistical downscaling. This study presents a two-phase statistical downscaling framework to improve the spatial resolution and accuracy of precipitation and temperature projections. In the first phase, a Convolutional Neural Network (CNN), trained to learn spatial patterns from ERA5 reanalysis data, is employed to refine the coarse grid of GCMs. In the second phase, bias correction is performed using a quantile delta mapping technique, with ERA5 still serving as the reference dataset. The resulting downscaling framework is applied to outputs from five GCMs participating in the Coupled Model Intercomparison Project Phase 6 (CMIP6) under two Shared Socioeconomic Pathways (SSPs): SSP1-2.6 and SSP3-7.0. This work is part of the OurMED PRIMA project, which focuses on the Mediterranean region, a recognized climate change hotspot. Results indicate substantial improvements in the accuracy of temperature and precipitation projections compared to other downscaling methods. The proposed approach effectively captures fine-scale spatial variability, a crucial aspect for regional climate studies in complex regions like the Mediterranean region. The downscaled climate data are used to assess climate extremes by computing the indices defined by the Expert Team on Climate Change Detection and Indices (ETCCDI). These indices can offer valuable insights into evolving climate trends and extremes throughout the 21st century. The proposed methodology demonstrates significant potential for broader applications in regions requiring high-resolution climate data to support adaptation strategies and policy development.

This work was supported by OurMED PRIMA Program project funded by the European Union’s Horizon 2020 research and innovation under grant agreement No. 2222. Valerio Todaro acknowledges financial support from the PNRR MUR project ECS_00000033_ECOSISTER.

How to cite: D'Oria, M., Todaro, V., Secci, D., and Tanda, M. G.: Statistical downscaling of climate models for the Mediterranean region combining convolutional neural network and quantile delta mapping, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9167, https://doi.org/10.5194/egusphere-egu25-9167, 2025.

EGU25-9367 | ECS | Posters on site | ITS1.16/AS5.4

Three Decades of high-Resolution ERA5 Downscaling over the Italian domain: Validation and Applications in Hydrology, Meteorology, and Climate Analysis 

Mohsin Tariq, Francesco Cavalleri, Silvio Davolio, Michele Brunetti, Stefania Camici, Daniele Mastrangelo, and Paolo Stocchi

This study presents a detailed assessment of very high-resolution reanalysis data covering the entire Italian territory and the broader Alpine domain for the three-decade period 1990-2020. The dataset was generated using a dynamical downscaling of ERA5 reanalysis with the convection-permitting model MOLOCH, implemented at a fine grid spacing of 1.8 km.

Validation against high-resolution observational datasets (GRIPHO, ARCIS, and the ISAC-CNR precipitation and temperature dataset) and comparisons with similar downscaled reanalysis products (ERA5-LAND, CERRA, MERIDA-HRES, and SPHERA) confirm the dataset’s reliability in reproducing key meteorological variables, such as temperature and precipitation. Importantly, the dataset leads in capturing higher-order statistics, including intensity and extremes.

The dataset’s versatility is illustrated through multi-disciplinary applications. In hydrology, it enables high-resolution drought characterization; in meteorology, it supports the analysis of extreme weather events and orographic effects. In climate research, it provides valuable insights into long-term trends and variability.

This work underscores the importance of very high-resolution datasets in advancing our understanding of the complex interactions between natural processes and human activities, especially in regions with challenging topography like the Alps. It establishes a strong foundation for future research and practical applications, including disaster risk management, water resource planning, and climate adaptation strategies.

How to cite: Tariq, M., Cavalleri, F., Davolio, S., Brunetti, M., Camici, S., Mastrangelo, D., and Stocchi, P.: Three Decades of high-Resolution ERA5 Downscaling over the Italian domain: Validation and Applications in Hydrology, Meteorology, and Climate Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9367, https://doi.org/10.5194/egusphere-egu25-9367, 2025.

EGU25-11322 | ECS | Posters on site | ITS1.16/AS5.4

A Two-Stage  Downscaling Approach using Machine Learning and image super-resolution techniques for high-resolution seasonal climate forecasts in the Alpine region  

Suriyah Dhinakaran, Alice Crespi, Mariapina Castelli, Iacopo Ferrario, and Alexander Jacob

The Alpine region faces heightened risks from climate change due to its complex terrain and ecosystems, highlighting the significant global challenge posed by a warming climate. The region is particularly susceptible to the effects of global warming, which not only intensifies weather extremes but also significantly impacts hydrological processes. These changes increase the frequency and severity of extreme events like droughts and floods, further heightening the region's vulnerability. Accurate local climate predictions are essential for effectively managing these risks, as they provide the spatial and temporal precision necessary for hydrological simulations. Such high-resolution data enable detailed modelling of water availability, runoff patterns, and flood risks, facilitating improved planning and adaptation strategies. However, existing global datasets often lack the resolution needed for these assessments. To address this gap, this research aims to generate high-resolution seasonal climate forecasts specifically designed for the Alpine region, providing an essential tool for understanding climate variability, managing hazards, and supporting hydrological analyses. The study proposes a novel two-stage downscaling approach within the perfect prognosis framework to enhance the spatial resolution of ECMWF (European Centre for Medium Range Weather Forecasts) SEAS5 (Seasonal Forecast System 5) seasonal forecasts from native 0.25°x0.25° to 1 km for the Alpine region. Key variables include daily temperature, precipitation, and downward surface solar radiation. In the first stage, pixel-by-pixel downscaling is performed though LGBM (Light Gradient Boosting Machine) regression applied to ERA5 reanalysis predictor fields matched against CHELSA-W5E5 (v1.1) fields, conservatively interpolated to 6-km resolution. Predictors are selected through feature importance analysis via cluster-based regression and is optimized for the 2005–2016 training period. The trained model is then applied to the 51 ensemble members of SEAS5 predictors, generating target variables at a 6 km resolution. In the second stage, the 6-km downscaled outputs, along with additional static predictors such as elevation, aspect, and cyclically encoded day of the year, are passed to a sliding-window Enhanced Super-Resolution Generative Adversarial Network (ESRGAN). This image super-resolution technique trained and optimized using CHELSA-W5E5 at its native 1-km resolution, further refines the forecasts to produce high-resolution seasonal predictions with 51 ensemble members at 1 km resolution. The two-stage scheme was found to improve the downscaling performance with respect to the application of one-step method. The contribution will present the overall methodology and the results of the model evaluation. The outcomes of this study are expected to play a key role as critical inputs for a drought prediction module within the framework of the EU-funded interTwin project. This research has been funded by the European Union through the interTwin project (101058386).

How to cite: Dhinakaran, S., Crespi, A., Castelli, M., Ferrario, I., and Jacob, A.: A Two-Stage  Downscaling Approach using Machine Learning and image super-resolution techniques for high-resolution seasonal climate forecasts in the Alpine region , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11322, https://doi.org/10.5194/egusphere-egu25-11322, 2025.

EGU25-11385 | ECS | Orals | ITS1.16/AS5.4

Statistical Downscaling and Emulators: Can Generative Machine Learning add Value to Extrapolation and Bias? 

Mikel N. Legasa, Redouane Lguensat, and Mathieu Vrac

Besides regional climate models (RCMs), there exist two main approaches to tackle the insufficient resolution of global climate models: emulators and statistical downscaling. While both approaches are similar in the techniques they use (statistical and machine learning, ML, methods), they differ in their objectives and underlying assumptions. Emulators are intended to provide a cost-effective alternative to RCMs by emulating their downscaling functions. Alternatively, statistical downscaling (SD) models learn the empirical (observed) relationships that link a set of key large-scale predictors, to the local high-resolution predictand of interest. There is a key tradeoff between these two approaches: emulators are unconstrained by observed climate records, yet they also inherit RCM biases; conversely, SD methods are able to produce potentially bias-free simulations (at least when driven by reanalyses), but with extrapolation constrained by observed relationships.

This tradeoff between extrapolation and bias is a key research perspective, especially when compounded with the usual additional challenges ML methods face, like representation of extremes or the temporal/spatial consistency of the predictions. Within this context, the added value of generative/stochastic methods is highly relevant and timely. Indeed, recent studies using deterministic ML methods (such as Wang et al. 2023; Doury et al. 2024) have highlighted that emulating high-resolution fields does require generative/stochastic approaches, specially when it comes to representing extreme weather events for complex variables like precipitation (Watson, 2022, 2023). However, while generative methods such as diffusion models may offer an advantage when it comes to simulating extremes (Addison et al. 2024; Aich et al. 2024), they are also subject to more potential instability (e.g., diffusion models are known to have hallucinations, Aithal et al. 2024), hence also increasing the biases.

In this study we aim to address the added value and potential downsides generative/stochastic ML methods can bring to the field of statistical downscaling and emulation, by targeting the tradeoff between extrapolation and bias. Therefore, we will address both already well-established generative deep learning techniques and the latest generation diffusion models, and focus on how well they fare when capturing aspects beyond mean statistics, including extremes, which are of particular interest in terms of climate impacts.

 

References:
Addison, H. et al. (2024). Machine learning emulation of precipitation from km-scale regional climate simulations using a diffusion model. Preprint. DOI: https://doi.org/10.48550/arXiv.2407.14158

Aich, M. et al. (2024). Conditional diffusion models for downscaling & bias correction of Earth system model precipitation. Preprint. DOI: https://doi.org/10.48550/arXiv.2404.14416

Aithal, S. K. et al. (2024). Understanding Hallucinations in Diffusion Models through Mode Interpolation. Preprint. DOI: https://doi.org/10.48550/arXiv.2406.09358

Doury, A. et al. (2024). On the suitability of a convolutional neural network based RCM-emulator for fine spatio-temporal precipitation. Climate Dynamics, 62(9), 8587-8613. DOI: https://doi.org/10.1007/s00382-024-07350-8

Watson P. A. G. (2022). Machine learning applications for weather and climate need greater focus on extremes. Environmental Research Letters 17(11). DOI: https://doi.org/10.1088/1748-9326/ac9d4e

Watson, P. (2023). Machine learning applications for weather and climate predictions need greater focus on extremes: 2023 update. NeurIPS 2023 Workshop on Tackling Climate Change with Machine Learning.

 

Acknowledgement:

This work is funded by the National Research Agency under France 2030 bearing the references ANR-22-EXTR-0005 (TRACCS-PC4-EXTENDING project) and ANR-22-EXTR-0011 (TRACCS-PC10-LOCALISING project).

How to cite: Legasa, M. N., Lguensat, R., and Vrac, M.: Statistical Downscaling and Emulators: Can Generative Machine Learning add Value to Extrapolation and Bias?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11385, https://doi.org/10.5194/egusphere-egu25-11385, 2025.

EGU25-11589 | Posters on site | ITS1.16/AS5.4

A Comprehensive Approach for Evaluating Downscaled Climate Model Projections from Multiple Perspectives: A Case Study of Hydrological Germany 

Mohammad Hadi Bordbar, Philip Lorenz, Frank Kreienkamp, and Theresa Schellander-Gorga

Unprecedented climatic events have been occurring more frequently, highlighting the role of anthropogenic climate change and the need for accurate regional climate projections for adaptation planning. Such projections require high spatial resolution, typically achieved by downscaling global climate model outputs. However, evaluating climate model outputs remains challenging, as they represent statistical features of climate change and do not evolve consistently with observations.

In this study, we conduct an empirical statistical downscaling of a large number of historical (1951-2014) CMIP6 global climate projections using different configurations of the statistically downscaling method EPISODES. The domain covers Hydrological Germany, including Germany and its main rivers' basins. 

We provide a comprehensive assessment of the performance of each downscaled projection. We evaluate the statistical characteristics of each model run against observational data from four key perspectives. Specifically, we assess the performance of each projection for six key climate variables based on annual and seasonal climate means, as well as internal variability across various timescales. To estimate the ability of each run to capture the persistence of weather regimes, we also compare the lagged autocorrelation function across the entire domain for daily mean variables. Additionally, we divide our domain into nine zones and compute the histograms of daily mean variables. We use various widely adopted statistical metrics and have developed new indices. This approach enables a comprehensive evaluation of the performance of each realization from multiple perspectives, facilitating the identification of the optimal configuration of EPISODES, which can serve as a key tool for climate model evaluation.

How to cite: Bordbar, M. H., Lorenz, P., Kreienkamp, F., and Schellander-Gorga, T.: A Comprehensive Approach for Evaluating Downscaled Climate Model Projections from Multiple Perspectives: A Case Study of Hydrological Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11589, https://doi.org/10.5194/egusphere-egu25-11589, 2025.

EGU25-13504 | ECS | Orals | ITS1.16/AS5.4

Downscaling a heat stress index in southern South America using deep-learning  

Candela Sol Glatstein, Rocio Balmaceda-Huarte, and Maria Laura Bettolli

Empirical-statistical Downscaling (SD) techniques are valuable tools able to generate high-resolution climate information needed to carry out impact studies. In this regard, Convolutional Neural Networks (CNNs) are promising SD techniques capable of handling large amounts of data and extracting relevant predictor information for each particular site. These characteristics of the CNN represent a major advantage over traditional SD methods, which typically rely on human-guided predictor selection. Notwithstanding, an adequate tuning of the CNN is key for optimising their potential.

In southern South America (SSA), CNNs has proven to be skilful in representing daily extreme temperatures and extrapolating into future scenarios. Although the selection of the activation function introduces a source of uncertainty in the future projections. 

In this context, this study aims to explore the use of CNNs as a statistical downscaling tool to simulate the wet bulb temperature (Tw) over SSA, a multivariate heat-stress index estimated from temperature and humidity. Tw has been widely used as a heat-stress proxy in different parts of the world, however, its characterisation and modelling in SSA remain as a pending task. To this end, four different CNN architectures regarding the activation function (ReLU or linear), domain size and configuration of the CNN layers were tested. All CNN models were trained during summer days using a cross-validation (CV) scheme in the period 1991-2020 and then evaluated in four unseen summers between 2021 and 2024. For comparison purposes, CNN models were similarly trained and validated to simulate maximum temperature (Tx). 

Overall, CNN models well represented all the features evaluated, including the heat-waves that took place in the summers evaluated independently. In particular, CNN models presents a better performance in simulating Tw than Tx with smaller errors in terms of mean and extremes aspects. Regarding the domain size, for both temperatures, the configuration with the smaller domain yields the best results. Also in this latter case, the reduction of the number of filter size in the last layer slightly improves the representation of Tx. When considering the large domain, the differences between the CNNs based on different activation functions increase, and CNN models with linear configuration outperform the ones with ReLu. 

The findings of this work reinforces the potential of CNNs for climate downscaling in SSA, especially for its use to simulate multivariate impact indices.

How to cite: Glatstein, C. S., Balmaceda-Huarte, R., and Bettolli, M. L.: Downscaling a heat stress index in southern South America using deep-learning , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13504, https://doi.org/10.5194/egusphere-egu25-13504, 2025.

The large computational cost of Regional Climate Models (RCMs) means that only one ensemble member per climate model is typically downscaled; subsequently, internal variability uncertainty is generally not explicitly accounted for in coordinated regional climate downscaling efforts (e.g., CORDEX). Surrogate Artificial Intelligence-based emulators are several orders of magnitude faster than RCMs and have been well-tested in their ability to generate reliable regional climate projections. This study employs a Generative AI-based approach using Generative Adversarial Networks (GANs) to downscale daily precipitation from a large ensemble of climate projections from CanESM5 (n=20) and ACCESS-ESM-1-5 (n=40) at a 12km resolution for New Zealand. We show that this AI-based approach can reproduce key features including rainfall extremes and their increases in future climates with useful accuracy. Similar to previous studies using low-resolution climate models, our results show robust future changes in winter precipitation across the ensemble members, but significant uncertainty during summer. The large ensemble of downscaled climate projections better samples extremely rare localized extreme events, which are not adequately sampled using a single ensemble member. Using this ensemble, we can calculate the relative contributions of internal variability and model structural uncertainty (both GCM and downscaling) in climate projections of local-scale impact-relevant weather events. Overall, our study highlights the significant potential of AI to complete dynamical downscaling and allow quantification of internal variability uncertainty at regional scales.

How to cite: Sherwood, S., Rampal, N., and Gibson, P.: Quantifying Internal Variability Uncertainty in Regional Climate Projections using Artificial Intelligence, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14590, https://doi.org/10.5194/egusphere-egu25-14590, 2025.

Global gridded land use projection data is essential for the investigation of various research topics in global environmental change. Such information is commonly provided by various integrated assessment models (IAMs) at a relatively coarse resolution. For example, the Land Use Harmonization 2 (LUH2) provided future global land use data at 0.25-degree for CMIP 6. However, the demand for higher resolution land use projection data has been increasing in recent years for more granular analysis of various topics. The Asia-pacific Integrated Model (AIM), which is a widely known IAMs for climate policy study, could so far provide global gridded land use data at 0.5-degree resolution under the SSP-RCP scenario framework. In this study, I constructed a downscaling framework for the AIM land use model system, that combines an empirical land use change model and a cross-entropy minimization method and aimed to downscale land use projection from half-degree to 5 arcminutes or even higher resolution. The empirical land use change model is estimated by multinominal logit regression method with historical data from 1995 to 2015, which allows the land use change driven by various biophysical and socio-economic factors and provides prior land use distribution information for the cross-entropy minimization process. Validation for the period of 2015 to 2020 showed the effectiveness of the downscaling model. This newly developed downscaling model could provide high-resolution gridded land use projection information for global environmental change research community.  

How to cite: Wu, W.: The development of a high-resolution global land use projection downscaling model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15262, https://doi.org/10.5194/egusphere-egu25-15262, 2025.

EGU25-15411 | ECS | Posters on site | ITS1.16/AS5.4

How to Make Downscaling Model Inputs Closer to Real Distribution Patterns? 

Zitong Wen, Lu Zhuo, Jiaqi Yu, and Dawei Han

Due to the excellent temporal continuity, reanalysis datasets are often used as input data for downscaling models. However, because of the relatively coarse spatial resolution, reanalysis datasets often exhibit significant value differences between adjacent pixels, making it challenging to accurately capture the distribution of meteorological parameters in heterogeneous urban areas. Although many downscaling studies have utilized reanalysis data, none have explored how to preprocess these datasets to achieve smoother patterns in the distribution of meteorological parameters at the urban level, making them closer to real distribution patterns. To address this limitation, this study proposes a novel iterative Gaussian filtering method. This method applies iterative Gaussian filtering while keeping the mean values unchanged within the coarse-resolution pixels to generate fine-resolution data with smoother distribution patterns. In this study, the 1-km land surface temperatures obtained from MODIS and its reprojected 0.1˚ resolution data are assumed to represent the true fine-resolution values and coarse-resolution values, respectively, to validate the effectiveness of the proposed method. The results indicate that, compared to the coarse-resolution data, the fine-resolution data processed through iterative Gaussian filtering achieves higher accuracy, with RMSE and MAE improvements of 11.06% and 11.89%, respectively. The distribution patterns of the fine-resolution data are also closer to real distribution patterns than those of the coarse-resolution data. These findings suggest that our proposed method could serve as a valuable tool for enhancing the accuracy of downscaling models in future studies.

How to cite: Wen, Z., Zhuo, L., Yu, J., and Han, D.: How to Make Downscaling Model Inputs Closer to Real Distribution Patterns?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15411, https://doi.org/10.5194/egusphere-egu25-15411, 2025.

EGU25-16520 | ECS | Orals | ITS1.16/AS5.4

AI for high-resolution climate data: downscaling climate projections and decadal predictions with a deep learning Latent Diffusion Model  

Elena Tomasi, Gabriele Franch, Sandro Calmanti, and Marco Cristoforetti

Over the past decade, advancements in high-performance computing have led Machine Learning (ML) to play a key role in enhancing Earth System Models (ESMs), enabling progress beyond the current state-of-the-art. Downscaling techniques to generate high-resolution data starting from the results of large-scale models are one of the most promising Deep Learning (DL) applications for ESMs. This approach offers a computationally efficient alternative to numerical dynamical downscaling, particularly for climate projections.  

In this study, we present the application of a state-of-the-art DL model to emulate the dynamical downscaling of 6-hourly climate data, focusing on precipitation and minimum and maximum temperatures. The model is trained to reconstruct fields at a 4 km resolution, starting from dynamical predictors at ~100 km resolution. Training data consists of coarsened ERA5 reanalysis data (Hersbach et al., 2018) as predictors and high-resolution target data from the COSMO-CLM dynamical reanalysis for Italy (Raffa et al., 2021). We utilize 40 years of 6-hourly data (1981–2020) for training. 

This training setup is designed to prepare the model for inference on low-resolution outputs from a selection of diverse climate projections and decadal predictions. The ultimate goal is to generate an ensemble of high-resolution projections that deliver additional insights, particularly into extreme values, at a fraction of the computational cost of regional climate models. 

The DL architecture employed is a recently developed Latent Diffusion Model applied with a residual approach (Tomasi et al. 2024), which has demonstrated exceptional performance in downscaling continuous variables, such as 2-m temperature and 10-m wind speed components. Results are compared against other ML models (e.g., UNET) and available numerical regional climate models for benchmarking. Preliminary results are presented, highlighting (i) the enhancements introduced by the LDM architecture compared to baseline models, (ii) its ability to reconstruct coherent structures and extreme values, and (iii) the added value of the high-resolution data obtained by the application of the LDM to low-resolution climate projections. 

How to cite: Tomasi, E., Franch, G., Calmanti, S., and Cristoforetti, M.: AI for high-resolution climate data: downscaling climate projections and decadal predictions with a deep learning Latent Diffusion Model , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16520, https://doi.org/10.5194/egusphere-egu25-16520, 2025.

EGU25-17918 | Orals | ITS1.16/AS5.4

Comparative Analysis of Daily Precipitation Using High-Resolution Reanalysis Data 

Esteban Rodríguez-Guisado, Jesús Gutiérrez-Fernández, María Ortega, Irene Rodríguez-Muñoz, Alfonso Hernanz, and Carlos Correa-Guinea

As part of its responsibilities within the Spanish National Climate Change Adaptation Plan (PNACC) 2021-2030, AEMET generates and makes available to the public, through its website, climate change scenario information for Spain using statistical methods. These methods require a robust and sufficiently long observational database to enable proper training and validation, which has traditionally constrained their application to temperature and precipitation. However, the adaptation community requires information on a broader set of essential climate variables to adequately characterise the impacts of climate change on each sector. Recent studies using Artificial Intelligence show potential to generate downscaled information for a broader set of variables. However, long records from other ECV are scarce, relying on reanalysis information for training the methods.

Advances in modelling, on the other hand, have made available regional reanalysis products sich as COSMO reanalysis (Bollmeyer et al., 2015), CERRA (Schimanke et al., 2021), and ERA5-LAND (Muñoz-Sabater et al., 2024). These types of products provide historical information on a wide range of Essential Climate Variables (ECVs), offering extensive spatial coverage and physical consistency.

This study evaluates the performance of various available reanalysis products as a preliminary step towards selecting the most suitable dataset for generating high-resolution scenario information for a comprehensive set of Essential Climate Variables. Despite the focus on a complete set of ECVs, the study will focus on precipitation, as it is the variable for which AEMET has the most comprehensive data network. Different domains across the Iberian Peninsula will be analysed, with particular 

How to cite: Rodríguez-Guisado, E., Gutiérrez-Fernández, J., Ortega, M., Rodríguez-Muñoz, I., Hernanz, A., and Correa-Guinea, C.: Comparative Analysis of Daily Precipitation Using High-Resolution Reanalysis Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17918, https://doi.org/10.5194/egusphere-egu25-17918, 2025.

EGU25-18397 | ECS | Posters on site | ITS1.16/AS5.4

Assessing the added value of statistical downscaling to the predictive skill of global subseasonal temperature forecasts during the Paris 2024 Olympics 

Eren Duzenli, Jaume Ramon, Verónica Torralba, Sam Pickard, Dragana Bojovic, Paloma Trascasa-Castro, and Ángel G. Muñoz

Global warming is increasing the frequency and intensity of extreme temperature events, posing significant risks to human health during major outdoor events such as the Summer Olympics. Providing decision-makers with robust, high-resolution extreme temperature forecasts well in advance is crucial to anticipate risks on the health of both athletes and spectators. Global subseasonal forecasts can play a key role in addressing this challenge because they offer data with relatively high temporal resolution (i.e., weekly) several weeks ahead. However, the coarse spatial resolution of these forecasts limits their utility for the types of localized decision-making required for major events, necessitating the use of downscaling methods to improve resolution.

Although numerous downscaling approaches exist, their ability to skillfully downscale subseasonal data has not been systematically evaluated. To address this gap, this study assesses the performance of 27 statistical downscaling methods – including bias correction, linear regression, logistic regression, and analogs – in enhancing the spatial resolution of subseasonal temperature hindcasts. We use Climate Prediction System version 2 (CFSv2) data at 100 km resolution as the raw hindcast product and downscale these hindcasts to a 5 km resolution. The process is conducted separately for temperature hindcasts from models initiated 1, 2, 3, and 4 weeks prior to the three target weeks of the Paris 2024 Olympics (starting from 22 July, 29 July and 5 August). In addition to using CFSv2 temperature outputs as predictors, we explore the added value of incorporating atmospheric patterns into the downscaling process. Models are constructed using both daily and weekly data, enabling a comparative analysis of performance across two temporal scales.

The results show that downscaling methods can successfully transfer the predictive skill of CFSv2 to the 5 km resolution. However, the choice of downscaling method is crucial to the performance, as some methods degrade the predictive skill of CFSv2, while others enhance it. Notably, methods that incorporate atmospheric patterns show promise in improving forecasts with longer lead times. Additionally, daily data models using analogs outperform their weekly counterparts, while regression-based methods perform better with weekly data.

In summary, this study demonstrates the potential of statistical downscaling to enhance coarse-resolution subseasonal temperature forecasts. However, it also highlights the significant variability in forecast skill depending on the choice of predictors and methods, which can either improve or degrade performance.

How to cite: Duzenli, E., Ramon, J., Torralba, V., Pickard, S., Bojovic, D., Trascasa-Castro, P., and Muñoz, Á. G.: Assessing the added value of statistical downscaling to the predictive skill of global subseasonal temperature forecasts during the Paris 2024 Olympics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18397, https://doi.org/10.5194/egusphere-egu25-18397, 2025.

EGU25-19329 | ECS | Orals | ITS1.16/AS5.4

Statistical bias adjustment and the usability of climate information: a perspective on strategies and underlying assumptions 

Jakob B. Wessel, Fiona R. Spuler, Julie Jebeile, and Theodore G. Shepherd

Statistical bias adjustment of climate models has become widespread practice to bridge the usability gap of climate information for impact studies and other societal applications. However, the application of bias adjustment offers potential for misuse and comes with several fundamental issues which have been highlighted in the literature. In this tension between widespread use and fundamental issues, different strategies for the application of statistical bias adjustment have developed, ranging from selecting a consistent bias adjustment method across applications to ensure comparability, to applying an ensemble of available methods in a given case study. In this contribution, we examine the specific methodological assumptions of different approaches to bias adjustment, such as the relevance and potential for trend preservation, and propose an evaluative framework based on recent literature in philosophy of science to assess the understanding of usability underlying different approaches to bias adjustment. We find that both methodological assumptions about bias adjustment, as well as the understanding of usability in the context of climate information determine the choice of bias adjustment strategy in current practice. For example, global application of a bias adjustment method generates information that is salient and credible and thus usable mostly for the purpose of model intercomparison, whilst local adaptation improves credibility, but compromises on the ease-of-use. With neither the methodological assumptions nor the understanding of what usable climate information is and who it is generated for often explicitly stated in practice, we hope to contribute to enhanced methodological practice and reflection through this discussion.

How to cite: Wessel, J. B., Spuler, F. R., Jebeile, J., and Shepherd, T. G.: Statistical bias adjustment and the usability of climate information: a perspective on strategies and underlying assumptions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19329, https://doi.org/10.5194/egusphere-egu25-19329, 2025.

EGU25-19866 | Posters on site | ITS1.16/AS5.4

Enhancing Bias Correction and Downscaling of Rainfall Pattern Over Taiwan with a Deep Learning Neural Network Over Complex Terrain 

Yi-Chi Wang, Chia-Hao Chiang, Wan-Ling Tseng, and Ko-Chih Wang

This study evaluates the application of a deep learning approach employing a multi-head attention mechanism within a deep neural network (DNN) framework to enhance bias correction and downscaling of the fifth-generation European Centre for Medium-Range Weather Forecasts (ECMWF) reanalysis rainfall datasets. The proposed Encoder-Decoder with multi-head Attention (EDA) model leverages gridded 5-km daily rainfall observations and auxiliary inputs, such as surface wind data and high-resolution topography, to generate local-scale daily rainfall estimates across Taiwan—a mountainous subtropical island with complex terrain.

The model's performance is assessed using mean rainfall patterns, rainfall statistics, extreme climate indices, and interannual variations during Taiwan's rainy seasons. Results demonstrate that the EDA model effectively corrects biases in low-intensity rainfall and resolves inaccuracies in orographic rainfall placement present in reanalysis datasets, outperforming conventional quantile-mapping methods. Additionally, the integration of auxiliary surface wind information significantly improves the model's downscaling accuracy across various metrics.

This study highlights the potential of deep learning architectures, particularly those incorporating attention mechanisms and auxiliary data, for statistical bias correction and downscaling in regions characterized by intricate interactions between synoptic and local circulations modulated by topography.

How to cite: Wang, Y.-C., Chiang, C.-H., Tseng, W.-L., and Wang, K.-C.: Enhancing Bias Correction and Downscaling of Rainfall Pattern Over Taiwan with a Deep Learning Neural Network Over Complex Terrain, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19866, https://doi.org/10.5194/egusphere-egu25-19866, 2025.

EGU25-21537 | Orals | ITS1.16/AS5.4

Global Location Transferability of Generative Deep Learning Models for Precipitation Downscaling 

Paula Harder, Christian Lessig, Matthew Chantry, Francis Pelletier, and David Rolnick

Generative deep learning models have shown remarkable skill in the probabilistic downscaling of climate and weather forecasts, with generative adversarial networks (GANs) as a particularly effective approach for precipitation downscaling. However, most existing methods are trained for specific regions, and their performance on unseen geographic areas remains largely unexplored. In our work, we evaluate the transferability of generative models to new locations outside their training domain. Using a global experimental setup, we employ ERA5 as the predictor dataset and IMERG as the high-resolution target dataset at 0.1° resolution. To systematically assess the performance across diverse regions, we design a hierarchical location split with 16 regions. We then train networks independently on the 16 regions and evaluate each of them on all others. Our findings provide insights on the robustness and limitations of generative models for global-scale precipitation downscaling, revealing challenges such as poor generalization to unseen orography and decreased performance in tropical regions, both for models applied in these areas and for those trained in the tropics and transferred elsewhere.

How to cite: Harder, P., Lessig, C., Chantry, M., Pelletier, F., and Rolnick, D.: Global Location Transferability of Generative Deep Learning Models for Precipitation Downscaling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21537, https://doi.org/10.5194/egusphere-egu25-21537, 2025.

Tropical cyclones (TCs) pose signif­icant risks, particularly in coastal regions, making accurate prediction of their track and intensity is crucial for effective disaster preparedness and response. Traditional numerical models struggle with balancing accuracy and computational efficiency, although TC track prediction has achieved substantial progress, challenges remain in forecasting TC intensity, especially rapid intensification (RI). This study aims to (1) develop a Transformer-based deep learning (DL) model to predict TC track, intensity, and 24-hour future intensity change simultaneously, and (2) investigate the relative importance of input variables to the contribution of improving model forecast ability. Based on 2001–2021 best track data and ERA5 reanalysis data over the western North Pacific (WNP), we develop an optimal model called OWZP-Transformer, which leverages the multi-head self-attention mechanism and incorporates the 13 input parameters categorized into four factors: basic, environmental, gradient, and structural. Specifically, our study incorporates structural parameters, which is represented by Okubo-Weiss-Zeta Parameter (OWZP). Our OWZP-Transformer model achieves competitive results for track prediction and shows excellent performance in intensity forecasting for the next 6 hour, with an overall root mean square error (RMSE) of 0.91 m/s. This result represents an improvement of 61.9% to 68.4% compared to existing DL models, which generally have RMSE values above 2 m/s. In addition, our model demonstrates superior performance in predicting 24-hour future intensity change, achieving an overall lower mean absolute error (MAE) of 1.57 m/s, which is 63.5% to 74.6% lower than existing DL models. Furthermore, our model successfully identifies all 11 RI events out of 30 TCs samples from WNP test dataset during 2020-2021. We further evaluate the contributions of each parameter for the first time using two explainable feature importance methods: DeepLIFT and DeepLiftShap. The results indicate that self-contributions and the basic factors play a dominant role in short-term forecasts, while the OWZ parameter plays a significant role following them. This study is the first attempt to comprehensively predict a broad range of TC forecasting tasks using a single DL model, highlighting the potential the OWZP-Transformer model as a reliable tool for enhancing both the accuracy and efficiency of TC predictions.

How to cite: Lin, Z. and Chu, J. E.: Enhancing tropical cyclone track and intensity predictions with the OWZP-Transformer model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-80, https://doi.org/10.5194/egusphere-egu25-80, 2025.

EGU25-628 | ECS | Posters on site | AS5.5

Development of a Novel ANN-Based Predictive Model for Multi-Site ILCR Estimation Using Weather Parameters and PM2.5 

Shivam Singh, Pratibha Vishwakarma, and Tarun Gupta

This study introduces a novel artificial neural network (ANN)-based methodology for predicting the Incremental Lifetime Cancer Risk (ILCR) in urban environments, leveraging weather parameters and PM2.5 concentrations. The innovative approach addresses the limitations of conventional ANN models, enabling superior performance and applicability across diverse geographical locations. The model incorporates a unique method to preprocess wind direction and speed into a singular representative factor, enhancing its adaptability and generalizability to different sites.

To validate the proposed methodology, one year of weather data and polycyclic aromatic hydrocarbons (PAHs) data were collected from two distinct sites in India. PAHs were analyzed using gas chromatography-mass spectrometry (GC-MS) to calculate ILCR. These data served as inputs for the ANN models. The conventional ANN model yielded a coefficient of determination (R²) of 0.73 and a mean squared error (MSE) of 0.0100. In contrast, the proposed method achieved significantly improved performance, with an R² of 0.93 and an MSE of 0.0031.

This improvement highlights the efficacy of the novel preprocessing technique, which optimally integrates meteorological parameters, particularly wind-related factors, into the modelling framework. Moreover, the proposed model’s ability to generalize across multiple sites allows it to be trained on larger datasets, thereby enhancing its robustness and reliability for predicting ILCR in various urban areas.

The study's findings emphasize the importance of refining input parameter representation in ANN-based environmental risk models to achieve superior accuracy and broader applicability. This work not only demonstrates the feasibility of using advanced AI techniques to assess public health risks but also offers a scalable solution for multi-site applications, paving the way for better-informed environmental and public health policies.

How to cite: Singh, S., Vishwakarma, P., and Gupta, T.: Development of a Novel ANN-Based Predictive Model for Multi-Site ILCR Estimation Using Weather Parameters and PM2.5, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-628, https://doi.org/10.5194/egusphere-egu25-628, 2025.

Aerosol composition information is crucial for determining the detrimental effects of aerosols on climate, air quality, and human health, given the differential effects of varying aerosol types. Conversely, developing south Asian countries lack systematic data on aerosol composition, with the available composition information limited to a few sites and a limited time. Moreover, the large spatio-temporal coverage of satellite observations is relatively unexplored for aerosol characterization.

In this study, we utilize satellite sensor Multi-angle Imaging Spectro-Radiometer (MISR) Level 2 version 23 aerosol products (spatial resolution = 4.4 km x 4.4 km) to calculate fractional aerosol optical depths (fAODs) for 2015-2016. These fAODs represent the proportion of total AOD attributable to the eight aerosol models assumed in MISR's aerosol retrieval algorithm, categorized based on size, shape, and refractive indices. The fractional AOD of aerosol model i is represented by fAODi. In this study, we use these eight fAODs, EDGAR emission data, together with land use and meteorological variables, as predictors in a machine learning (ML) model. The model is trained on a quarter-degree grid covering south Asia, using the chemical model simulated aerosol species mass fraction as the target variable.

We train models to predict six aerosol species-sulfate, nitrate, ammonium, black carbon (BC), organic carbon (OC) and dust. We employ two models: Random Forest with out-of-bag bootstrap sampling for cross-validation and Support Vector Regression (SVR) with a 5-fold cross-validation, utilizing 80% of the data for training and 20% for testing. The SVR model shows a mean cross-validation R² of 0.79, 0.83, 0.72, 0.81, 0.73 and 0.81 for sulfate, nitrate, ammonium, dust, OC and BC, respectively, with corresponding RMSE values of 0.02, 0.03, 0.01, 0.05, 0.04 and 0.01 on the test data. The Random Forest model performs better, with R² values of 0.87, 0.92, 0.85, 0.89, 0.90 and 0.88 for the same aerosol species and RMSE values of 0.02, 0.03, 0.01, 0.001, 0.03 and 0.01 for the test data. Permutation feature importance analysis shows that MISR-derived fAODs significantly influence the model’s predictions. The model anticipates aerosol composition to strengthen climate and health effect assessments of aerosols by focussing on their differential effects in low-income south Asian countries.

How to cite: Srivastava, S. and Dey, S.: Estimation of surface-based aerosol composition from satellite data-driven machine learning model over south Asia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-873, https://doi.org/10.5194/egusphere-egu25-873, 2025.

EGU25-1413 | Posters on site | AS5.5

Inland Ozone Production Due to Nitrogen Dioxide Transport Downwind of a Coastal Urban Area: A Neural Network Assessment  

Piero Chiacchiaretta, Eleonora Aruffo, Alessandra Mascitelli, Carlo Colangeli, Sergio Palermi, Sebastiano Bianco, and Piero Di Carlo

 The rapid advancement of Information Technology is transforming research in atmospheric and environmental sciences, with Artificial Intelligence and Machine Learning (AI/ML) offering novel tools to explore complex environmental systems. AI/ML techniques have demonstrated significant potential in atmospheric research and pollutant dynamics [6]. Machine learning’s capability to capture non-linear relationships among environmental variables has been validated in prior studies [5]. 

This study leverages a feed-forward neural network (FFNN) to investigate nitrogen dioxide (NO2) transport from a coastal urban environment in Central Italy to an inland rural area, leading to increased ozone (O3) production downwind. Such transport phenomena underscore the need to address both direct and transported emissions, as observed in urban-rural gradients worldwide [4,6]. 

By integrating observational data and meteorological parameters, including wind speed and direction alongside NOx and O3 levels, the FFNN model effectively predicted O3 concentrations at the inland site.  Results showed consistently higher O3 levels at the rural site compared to the urban area, reflecting significant O3 production during transport. The model exhibited a high correlation (R = 0.82) between observed and predicted O3 concentrations, underscoring AI’s value in enhancing air pollution dynamics understanding. These findings align with broader research demonstrating AI’s role in refining air quality predictions and improving source attribution [1,2]. 

This study highlights the effectiveness of AI techniques in environmental research, particularly in elucidating interactions between transportation emissions and secondary pollutants like O3. The results stress the importance of regional air quality modeling and advanced computational approaches in supporting environmental policy and decision-making. AI-driven insights can inform more effective mitigation strategies, enhance air quality forecasting, and assist policymakers in addressing public health concerns related to air pollution [1,2]. Recent reviews emphasize the necessity of integrating AI into air quality management frameworks [7]. 

Additionally, this research underscores the potential of hybrid AI methods and physics-informed machine learning to further improve atmospheric models and source attribution accuracy. Such innovations are critical for advancing air quality modeling and developing targeted strategies to mitigate environmental and public health impacts [7]. 

[1] World Health Organization. (2021). Air pollution and health.

[2] Lelieveld, J. et al. (2019). The contribution of outdoor air pollution sources to premature mortality on a global scale. Nature, 525(7569), 367-371.

[3] Heal, M. R., et al.  (2013). Particles, air quality, policy, and health. Chemical Society Reviews, 41(19), 6606-6630.

[4] Crutzen, P. J. (2006). The role of NO and NO2 in the chemistry of the troposphere and stratosphere. Annual Review of Earth and Planetary Sciences, 7, 443-472.

[5] Jacob, D. J. (1999). Introduction to Atmospheric Chemistry. Princeton University Press.

[6] Monks, P. S., et al. (2015). Tropospheric ozone and its precursors from the urban to the global scale. Atmospheric Chemistry and Physics, 15(15), 8889-8973.

[7] Kumar, P., et al. (2018). Ambient volatile organic compounds in urban environments: Techniques for sampling, analysis, and implications for air quality. Progress in Environmental Science and Technology, 2(1), 3-13.

How to cite: Chiacchiaretta, P., Aruffo, E., Mascitelli, A., Colangeli, C., Palermi, S., Bianco, S., and Di Carlo, P.: Inland Ozone Production Due to Nitrogen Dioxide Transport Downwind of a Coastal Urban Area: A Neural Network Assessment , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1413, https://doi.org/10.5194/egusphere-egu25-1413, 2025.

EGU25-2638 | Orals | AS5.5 | Highlight

Deep learning-based surface O3 responses to anthropogenic and meteorological changes 

Zhe Jiang, Xiaokang Chen, Min Wang, and Tai-Long He

The applications of deep learning (DL) technique in atmospheric environment research are expanding rapidly. Here we developed a DL framework to quantify the responses of surface ozone (O3) to anthropogenic and meteorological changes in China. The DL-based analysis suggests volatile organic compound (VOC)-limited regimes in urban areas over northern inland China, and thus, reductions of nitrogen oxide (NOx) emissions have resulted in increases in surface O3 concentrations. In contrast, changes in meteorological conditions led to a dramatic decrease in surface O3 concentrations in 2019-2021, particularly, in the North China Plain, whereas the decline in surface O3 concentrations driven by beneficial meteorological conditions in 2019-2021 has been completely reversed due to the occurrence of long-lasting heatwave in 2022, particularly in central China. The DL framework, developed in this work, provides a novel data-driven pathway to assess the causes of surface O3 changes, and is helpful for a comprehensive understanding of the driving factors of surface O3 evolution in China.

How to cite: Jiang, Z., Chen, X., Wang, M., and He, T.-L.: Deep learning-based surface O3 responses to anthropogenic and meteorological changes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2638, https://doi.org/10.5194/egusphere-egu25-2638, 2025.

EGU25-2682 | ECS | Posters on site | AS5.5

Comparison of LSTM and Bi-LSTM Models for Predicting PM2.5 Concentration in Seoul 

Kwon Jang, Ju-Yong Lee, Seung-Hee Han, Kyung-Hui Wang, and Hui-Young Yun

The importance of predicting fine particulate matter (PM2.5) concentrations has grown significantly due to deteriorating urban air quality. Seoul presents unique modeling challenges due to its intensive industrial activities, high population density, significant data variability between monitoring stations, and numerous missing values. This study analyzes and compares the predictive performance of LSTM (Long Short-Term Memory) and Bi-LSTM (Bidirectional LSTM) models using hourly PM2.5 concentration data collected from 25 monitoring stations in Seoul from 2018 to 2022.

In the data preprocessing phase, we employed the MICE (Multiple Imputation by Chained Equations) method to handle missing values, which effectively preserved the data's structural characteristics by considering inter-variable relationships. The predictive performance of both models was evaluated using metrics such as RMSE (Root Mean Square Error) and MAE (Mean Absolute Error). While LSTM focuses on forward learning, Bi-LSTM can capture complex time series patterns by utilizing both forward and backward information.

The results demonstrated that Bi-LSTM effectively captured complex time series patterns through its bidirectional learning structure, and optimal learning rates and dropout ratios were determined through various parameter tuning experiments. These findings present the characteristics and potential applications of both models in PM2.5 concentration prediction, expected to contribute to improved air quality forecasting systems and policy decision support.

Future research will focus on enhancing model accuracy through the implementation of additional algorithms and exploring applications for PM2.5 prediction in other cities. This aims to increase the spatial resolution of air pollution prediction and contribute to broader air quality improvements.

Acknowledgement 

"This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)"

How to cite: Jang, K., Lee, J.-Y., Han, S.-H., Wang, K.-H., and Yun, H.-Y.: Comparison of LSTM and Bi-LSTM Models for Predicting PM2.5 Concentration in Seoul, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2682, https://doi.org/10.5194/egusphere-egu25-2682, 2025.

EGU25-2683 | ECS | Posters on site | AS5.5

A Transfer Learning-Based Model for PM2.5 Prediction in Seoul 

Seung-Hee Han, Ju-Yong Lee, Kwon Jang, Kyung-Hui Wang, and Hui-young Yun

Predicting PM2.5 concentrations using air quality data is often hindered by the presence of missing values, which can compromise accuracy and reliability. Traditional prediction models frequently suffer significant data loss during the handling of missing values, necessitating new approaches that address data quality issues while improving prediction performance.

This study proposes an efficient prediction methodology leveraging transfer learning to minimize the impact of missing values. A pre-trained model was constructed using integrated data from all monitoring stations in Seoul, followed by fine-tuning for specific monitoring stations to develop a PM2.5 prediction model. Transfer learning is a machine learning technique that utilizes knowledge from previously trained models to enhance learning efficiency and performance in new tasks or domains. Unlike traditional approaches that require training from scratch, transfer learning reuses the weights and structure of pre-trained models, reducing training time and improving performance.

In this study, a deep neural network (DNN) pre-trained model was built using data from all monitoring stations in Seoul, and fine-tuning was applied using specific station data. The model was trained on six-hour average PM2.5 data to predict the next six hours, effectively addressing missing values.

Preliminary results indicate that the transfer learning-based model effectively handles missing values and demonstrates improved prediction accuracy compared to independently modeled traditional approaches. By leveraging domain-wide information, the model compensates for the limitations of individual monitoring station data, achieving higher accuracy and reliability.

This study provides a scalable solution for addressing data gaps in air quality prediction and contributes to research on the health impacts of air pollution and urban air quality management. Future research will explore the application of this methodology to other pollutants and regions, further enhancing its generalizability and effectiveness.

Acknowledgement

"This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)"

How to cite: Han, S.-H., Lee, J.-Y., Jang, K., Wang, K.-H., and Yun, H.: A Transfer Learning-Based Model for PM2.5 Prediction in Seoul, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2683, https://doi.org/10.5194/egusphere-egu25-2683, 2025.

EGU25-3633 | ECS | Orals | AS5.5

Deep Learning for Accurate Global Dust Aerosol forecasting 

Shikang Du and Siyu Chen

Dust aerosol forecasting is of significant scientific and societal importance. Currently, the most accurate forecasting systems rely on numerical weather prediction methods, which solve differential equations to simulate the physical and chemical processes of dust aerosols and predict dust concentrations. However, errors introduced by initial and boundary conditions, along with the complex nonlinear interactions between aerosol physical-chemical processes and atmospheric dynamics, result in uncertainties and high computational costs in numerical prediction methods. In recent years, artificial intelligence (AI) methods have demonstrated significant potential in the field of weather forecasting. However, AI-based approaches for addressing such challenging extreme weather events remain in their infancy. Here, we introduce DustWatcher, an AI-based forecasting method for global dust aerosols. DustWatcher integrates spatiotemporal Transformers with conditional generative networks to develop a neural network framework that optimizes forecasting errors in an end-to-end manner. Compared to current state-of-the-art global and regional aerosol forecasting systems, DustWatcher, trained on 41 years of global reanalysis aerosol data, delivers more accurate deterministic forecasts for most aerosol variables including surface dust concentration and aerosol optical depth. DustWatcher provides skillful forecasts every three hours for the next seven days at a resolution of 0.5°×0.625°. Our results demonstrate the potential of AI in improving the dust forecasts accuracy and advancing its application in dust aerosol forecasting field.

How to cite: Du, S. and Chen, S.: Deep Learning for Accurate Global Dust Aerosol forecasting, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3633, https://doi.org/10.5194/egusphere-egu25-3633, 2025.

EGU25-4569 | ECS | Orals | AS5.5

An AI System to Predict Street-Level Air Quality: Introduction to the QUALARIA Project 

Cathy Wing Yi Li, Victória M. L. Peli, Mario E. Gavidia Calderón, Gabriel M. P. Perez, Thomas C. M. Martin, Amanda V. de Lucena, Edson L. S. Y. Barbosa, Matthias Schindler, Felix Laimer, Maria de Fátima Andrade, Edmilson Dias de Freitas, and Guy Brasseur

Here we present the joint German-Brazilian project QUALARIA (Artificial Intelligence based system for sub-urban scale air quality prediction/Sistema baseado em Inteligência Artificial  para previsão de qualidade do ar em escala sub-urbana). 

Through joint effort between research and business partners in Brazil and Germany, QUALARIA proposes to develop an operational artificial intelligence-based system for monitoring, simulating and predicting air quality in urban environments with unprecedented spatial resolution availability (https://meteoia.com/qualaria/). New downscaling approaches based on artificial intelligence have recently shown promising performance to simulate sub-grid atmospheric processes. This approach is designed to monitor and predict atmospheric pollutant concentrations and air quality indexes with high spatial resolution, through the development of the QUALARIA system. Advanced global and regional chemical-meteorological models, such as reanalysis data from ERA5 and EAC4, and WRF-Chem simulations are applied to derive the climatological state of air composition, specifically the average levels of air pollutant based on existing emission inventories. Measurements of PM10, PM2.5 NO2, and O3 concentrations from Air Quality Automatic Stations of the Environmental Company of São Paulo State (CETESB) are used to train the downscaling AI algorithm to capture the sub-grid spatial variations of the pollutant concentrations. Low-cost sensors are deployed to increase and complement the spatial coverage of the CETESB network. Artificial intelligence will transform air quality maps at a horizontal resolution of 10 km to street-level maps with an increased resolution of 100 m. From its simulated and predicted downscaled pollutant concentration fields, QUALARIA will provide its users with relevant air quality indicators, informing about the impacts of air pollution in human health and activities via an online dashboard. To achieve the optimal dashboard design, public and private sector stakeholders are being engaged and consulted for the co-development of the dashboard design and features.

How to cite: Li, C. W. Y., Peli, V. M. L., Calderón, M. E. G., Perez, G. M. P., Martin, T. C. M., de Lucena, A. V., Barbosa, E. L. S. Y., Schindler, M., Laimer, F., Andrade, M. D. F., Dias de Freitas, E., and Brasseur, G.: An AI System to Predict Street-Level Air Quality: Introduction to the QUALARIA Project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4569, https://doi.org/10.5194/egusphere-egu25-4569, 2025.

EGU25-6004 | Orals | AS5.5

DIRESA – A Deep Learning-based, nonlinear "PCA"​ 

Geert De Paepe and Lesley De Cruz

A deep ANN-based dimension reduction (DR) method, called DIRESA (distance-regularized Siamese twin autoencoder), has been developed to capture nonlinearities while preserving distance (ordering) and producing statistically independent latent components. The architecture is based on a Siamese twin autoencoder, with three loss functions: reconstruction, covariance, and distance loss. An annealing method is used to automate the otherwise time-consuming process of tuning the different weights of the loss function. DIRESA has been compared with PCA and state-of-the-art DR methods for two conceptual models, Lorenz ’63 and MAOOAM (Modular Arbitrary-Order Ocean-Atmosphere Model), and significantly outperforms them in terms of distance (ordering) preservation KPIs and reconstruction fidelity. The latent components have a physical meaning as the dominant modes of variability in the system. DIRESA correctly identifies the major coupled modes associated with the low-frequency variability of the coupled ocean-atmosphere system. Next to the conceptual model results, the first DIRESA results for reanalysis data will be presented.

DIRESA is provided as an open-source Python package, based on Tensorflow. With one line of code convolutional and/or dense layers DIRESA models can be build. On top of that, the package allows the use of custom encoder and decoder submodels to build a DIRESA model. The DIRESA package acts as a meta-model, which can use submodels with various kinds of layers, such as attention layers, and more complicated designs, such as graph neural networks. Thanks to its extensible design, the DIRESA framework can handle more complex data types, such as three-dimensional, graph, or unstructured data. Its flexibility and robust performance make DIRESA an promising new tool in weather and climate science to distil meaningful low-dimensional representations from the ever-increasing volumes of high-resolution climate data, for applications ranging from analog retrieval to attribution studies.

Tutorial: https://diresa-learn.readthedocs.io/

Preprint: https://arxiv.org/abs/2404.18314

How to cite: De Paepe, G. and De Cruz, L.: DIRESA – A Deep Learning-based, nonlinear "PCA"​, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6004, https://doi.org/10.5194/egusphere-egu25-6004, 2025.

Cloud fraction significantly affects the short- and long-wave radiation. However, its realistic representation in models has been difficult due to inadequate understanding of the sub-grid scale cloud processes. Recently, we have developed a neural network-based scale-adaptive (NSA) cloud-fraction scheme using the CloudSat data and found that the new scheme could greatly improve the simulation of cloud spatial distribution and vertical structure. In this study, we present two applications of the NSA scheme in the WRF model. The first is the simulation of the regional winter climate of the Tibet Plateau, where the NSA scheme was shown to significantly reduce the longstanding bias of too-cold surface temperature. The second is a tropical cyclone simulation, showing that the NSA scheme better simulated the track of In-Fa (2021). The underlying mechanisms will be presented.

How to cite: Chen, G.: The application of a neural network-based scale-adaptive cloud-fraction scheme in the WRF model , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7683, https://doi.org/10.5194/egusphere-egu25-7683, 2025.

EGU25-7915 | ECS | Orals | AS5.5

An Alternative Large-scale Sea Surface Wind Field Reconstruction Method Using Sparse Scatterometer Data Based on Physics-informed Neutral Network 

Ran Bo, Zeming Zhou, Huadong Du, Pinglv Yang, Xiaofeng Zhao, Qian Li, and Zengliang Zang

Satellite-based research on global sea surface wind is essential for understanding and monitoring the air-sea interface dynamical processes, driving the need for accurate and efficient assessment. Spaceborne scatterometers, which are among the most relevant sensors for sea surface wind observation, play a vital role in obtaining global ocean surface wind information. However, a significant challenge associated with polar-orbiting satellites lies in data gaps caused by their orbital paths, resulting in missing observations between swaths. While several satellite-derived sea surface wind products have been developed using data assimilation (DA) techniques, these existing methods are time-consuming and require large amounts of diverse data, rendering them computationally expensive. Additionally, the iterative steps of variational algorithms can only perform linear or weakly nonlinear adjustments to the governing equations, which may pose challenges given the highly non-linear nature of these equations.

In this study, we leveraged physics-informed neural networks (PINNs) techniques to reconstruct large-scale sea surface wind fields with sparse scatterometer observations from different satellites, integrating observations and filling gaps. By incorporating physical constraints into the loss function, specifically the Navier-Stokes equations, we efficiently fill the data gaps and reconstruct wind fields that not only match observational data but also adhere to physical principles. Another objective of this work is to introduce the wind speed gradient and direction parallel consistent constraints into the loss function in order to enhance the detail of the reconstructed wind field and increase the accuracy of both wind speed and direction. Structurally, the PINN resembles a fully connected neural network (FCNN), offering the advantage of automatic feature extraction. Our model not only extracts valuable information from existing data but also uncovers complex patterns and correlations in data that are difficult for traditional algorithms to capture. This approach provides a novel perspective and an alternative methodology for wind field reconstruction.

The results show that PINNs can reconstruct wind fields that closely resemble realistic wind patterns, capturing large-scale structures while preserving fine-scale details, thanks to the introduction of wind speed gradient and direction parallel consistent constraints. The training time for this model is about 3 hours, using only a single GPU core. This efficiency is partly due to the fact that PINNs do not rely on ensemble methods or large datasets to produce results. Unlike traditional DA methods, PINN does not depend on an initial best-guess field for assimilating observations. While we use only a small amount of scatterometer observation data, no initial field is required to complete the reconstruction. Additionally, since the PINN represents a continuous and differentiable function, it can produce outputs at any spatial or temporal point within the training domain.

Recognizing their potential for forecast models and data integration, PINNs offer a promising approach for accurate sea surface wind field reconstruction and could serve as an effective alternative to current methods.

How to cite: Bo, R., Zhou, Z., Du, H., Yang, P., Zhao, X., Li, Q., and Zang, Z.: An Alternative Large-scale Sea Surface Wind Field Reconstruction Method Using Sparse Scatterometer Data Based on Physics-informed Neutral Network, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7915, https://doi.org/10.5194/egusphere-egu25-7915, 2025.

EGU25-8958 | ECS | Posters on site | AS5.5

Reconstruction of Radar Composite Reflectivity Based on Satellite Observations and Deep Learning 

Jianyu Zhao, Sheng Chen, Jinka Tan, Qiqiao Huang, Liang Gao, Yanping Li, and Chunxia Wei

Ground-based weather radar provides crucial information for severe weather monitoring and forecasting, but it faces coverage limitations in regions with complex terrain, especially for oceanic and mountainous regions. To address the limitation, this study proposes "Echo Reconstruction UNet (ER-UNet)", a novel deep learning approach that reconstructs radar composite reflectivity (CREF) using Fengyun-4A geostationary satellite observations with broad coverage. The proposed ER-UNet enhances the UNet architecture by integrating wavelet transforms and multi-scale feature extraction mechanisms, significantly improving the network's capacity to capture detailed radar echo characteristics. Experimental results demonstrate that ER-UNet achieves superior performance compared to UNet, with improvements in statistical metrics that include root mean square error (RMSE), mean absolute error (MAE), and structural similarity index measure (SSIM), as well as categorical verification scores including probability of detection (POD), false alarm rate (FAR), critical success index (CSI), and Heidke skill score (HSS). Case studies further reveal ER-UNet's enhanced capability in reconstructing strong echo features, particularly in terms of intensity distribution and spatial structure. The proposed method shows potential for providing reliable radar reflectivity estimates in areas with limited radar coverage, offering valuable support for severe weather monitoring and early warning services.   

How to cite: Zhao, J., Chen, S., Tan, J., Huang, Q., Gao, L., Li, Y., and Wei, C.: Reconstruction of Radar Composite Reflectivity Based on Satellite Observations and Deep Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8958, https://doi.org/10.5194/egusphere-egu25-8958, 2025.

EGU25-10253 | ECS | Posters on site | AS5.5

Utilizing a residual neural network ensemble for ground-based cloud classifications 

Markus Rosenberger, Manfred Dorninger, and Martin Weissmann

Clouds of any kind play a substantial role in a wide variety of atmospheric processes. They are directly linked to the formation of precipitation, and significantly affect the atmospheric energy budget via radiative effects and latent heat. Hence, knowledge of currently occurring cloud types allows the observer to draw conclusions about the short-term evolution of the state of the atmosphere and hence also the weather. However, the number of operational cloud observations is rather decreasing than increasing due to high monetary and personnel expenses.

To show that automatized methods can be used to close this emerging gap, we trained an ensemble of 10 identically initialized residual neural network architectures from scratch to classify clouds from ground-based RGB pictures into 30 different classes. 4 pictures are used as input at each instance, so that the whole visible sky is covered. Operational manual cloud classification reports at the nearby station Vienna HoheWarte are used as ground truth, where for each instance up to 3 out of 30 categories are reported according to the state-of-the-art WMO cloud classification scheme for operational synoptic observations, making this a multi-label classification task. To the best of our knowledge we are the first to automatically classify clouds based on this elaborate classification scheme. Weutilize class specific resampling to reduce prediction biases because of highly imbalanced observation frequencies among categories. Results show that precision and recall scores are high in all classes, although in initially small classes overfitting is supposed to be the reason for exceptionally high accuracy. Still, every member of our ensemble outperforms both random and climatological predictions in each class. A substantial ratio of wrongly assigned pictures is made up by false negative predictions, where the model recognized the correct class in the input but the assigned probability was too small. For further improvement of current results, we aim to include also satellite images and measurement data, e.g. cloud base height, into our classifier. Though additional data is not supposed to solve overfitting issues, we expect to reduce the number of false negative and false positive predictions substantially.

Autonomy and output consistency are the main advantages of such a trained classifier, hence we consider operational cloud monitoring as main application. Either for consistent cloud class observations or to observe the current state of the weather and its short time evolution with high temporal resolution, e.g. in proximity of solar power plants. There, upcoming clouds can substantially change the possible energy output, which leads to the necessity of taking precautions.

How to cite: Rosenberger, M., Dorninger, M., and Weissmann, M.: Utilizing a residual neural network ensemble for ground-based cloud classifications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10253, https://doi.org/10.5194/egusphere-egu25-10253, 2025.

Understanding the interplay between weather conditions and fine particulate matter (PM2.5) is crucial for improving air quality management and public health. This study investigates the diurnal, seasonal, and spatial variability in the influence of weather factors on PM2.5 concentrations across Poland during 2015–2024. Hourly PM2.5 data from a nationwide network of monitoring stations were analyzed alongside meteorological parameters derived from the Weather Research and Forecasting (WRF) model. Key weather variables included wind speed and direction, precipitation, temperature, atmospheric pressure, relative humidity, solar radiation, and planetary boundary layer (PBL) height.

The machine learning model, XGBoost, was employed to predict PM2.5 concentrations, and the SHAP (SHapley Additive exPlanations) method, optimized using TreeSHAP, was used to assess variable importance and uncover patterns in the data. The results reveal complex, nonlinear relationships between meteorological factors and PM2.5, with notable variability across time and space. Seasonal and diurnal analyses highlight that weather influences are context-dependent: for instance, precipitation has negative impact on PM2.5 concentrations in winter, but its effect diminishes during summer months. Additionally, the role of PBL height was found to vary diurnally, reflecting their influence on pollutant dispersion. Spatial differences in weather-PM2.5 relationships were also observed, emphasizing the role of local topography, urbanization, and emission sources.

The comprehensive analysis provides a decade-long perspective on how weather factors influenced PM2.5 concentrations in Poland, offering valuable insights for regional air quality modeling and policy interventions aimed at mitigating air pollution under varying climatic conditions.

How to cite: Vovk, T. and Kryza, M.: Diurnal, seasonal, and spatial patterns of weather influences on PM2.5 concentrations in Poland: An explainable machine learning approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10255, https://doi.org/10.5194/egusphere-egu25-10255, 2025.

EGU25-10282 | ECS | Orals | AS5.5

Error bounded compression for weather and climate applications 

Langwen Huang and Torsten Hoefler


Weather and climate simulations produce petabytes of high-resolution data that are later analyzed by researchers to understand climate change or severe weather. We propose a new error-bounded compression method targeting for weather and climate data. It contains a JPEG2000 compression layer to capture the bulk part of the data, and a sparse wavelet layer to record the sparse signal that excess the given error bound. The sparse wavelet layer encodes the wavelet coefficients using the SPIHT algorithm. We test our method with established compression methods on a suite of benchmarks including basic statistics, case study of the hurricane data, derived variable computation, and Lagrangian trajectory simulation. Our method is favourable in most benchmark cases at given range relative error targets from 0.1% to 10% achieving compression ratios from 10x to more than 800x. It can reconstruct the derivatives of the compressed data with a best fidelity and does not add high frequency artifacts found in other compression methods. In Lagrangian trajectory simulations, our method can produce less distortion in trajectories and distribution of particles compared with SZ3. We are able to produce a 16x compressed wind data achieving less error metric than adding 5% random noise to the data, making it ready for practical use.

How to cite: Huang, L. and Hoefler, T.: Error bounded compression for weather and climate applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10282, https://doi.org/10.5194/egusphere-egu25-10282, 2025.

EGU25-10297 | ECS | Orals | AS5.5

MeshGraphNets for 3D atmospheric flow in Urban Environment for Atmospheric Dispersion 

Armand de Villeroché, Vincent Le Guen, Rem-Sophia Mouradi, Patrick Massin, Marc Bocquet, Alban Farchi, Sibo Cheng, and Patrick Armand

Urban and industrial areas are vulnerable to accidental releases of pollutants. To accurately determine the pollutant's plume position and affected areas, it is essential to estimate the atmospheric flow around the affected site. This flow can be precisely computed using numerical methods of Computational Fluid Dynamics (CFD). However, CFD computation is expensive and slow, making it unsuitable for emergency response. As reduced order approximations, machine learning surrogates offer a promising alternative as they are usually much faster; but they must first be trained on CFD-generated data. In this study, we propose a database of atmospheric simulations with varying meshes and atmospheric stability conditions. Meshes are built by randomly sampling buildings and positioning them in space. For each mesh, values of the Monin-Obukhov length and of the ground roughness are sampled, leading to different turbulent regimes and overall atmoshperic flow behaviour. We then train a MeshGraphNet on this database, i.e. a graph neural network built on the mesh structure. The performance of the trained neural network on unseen scenarios with different initial conditions has been evaluated and will be presented.

How to cite: de Villeroché, A., Le Guen, V., Mouradi, R.-S., Massin, P., Bocquet, M., Farchi, A., Cheng, S., and Armand, P.: MeshGraphNets for 3D atmospheric flow in Urban Environment for Atmospheric Dispersion, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10297, https://doi.org/10.5194/egusphere-egu25-10297, 2025.

EGU25-10486 | ECS | Posters on site | AS5.5

Objective characterization of mesoscale cloud patterns from graph theory and an Ising-like model (BICIM). 

Faustine Mascaut, Olivier Pujol, and Peter Forkman

The organization of mesoscale cloud fields is crucial for understanding atmospheric dynamics and their modeling. 
The role played by these cloud structures on their direct environment and, more generally, on the climate remains challenging to incorporate in climate models. 
In this contribution, we propose a methodology for automatically identifying and studying these cloud organizations, combining two innovative approaches: 
(1) an Ising-like model (called BICIM) capable of reproducing cloud fields with specific organization patterns, and 
(2) graph theory, applied to the outputs of this model and satellite observations, which allows us to derive distributions of surfaces and perimeters of clouds as well as inter-cloud distance distributions. 
For the first point, sensitivity tests on input data and fluxes revealed that BICIM consistently responds to changes, produces realistic results, and highlights humidity and wind as key factors in the formation of cloud organizations.
From the second point, we propose a new quantity, denoted as M, as a Metric for Assessing Similarity between Cloud Organization Layouts (MASCOL). 
As its name suggests, M quantifies the similarity between two cloud fields. 
We apply this methodology to satellite data, identifying cloud structures, with MASCOL aiding in classifying cloud fields relative to reference organizations (from BICIM).
This approach therefore enables a faster and more objective identification of each structure compared to visual methods. 
The reason is that it is based on graph theory, which is an efficient mathematical tool.
Furthermore, the methodology's reliance on graph theory and robust pattern recognition metrics makes it particularly well-suited for integration with machine learning and artificial intelligence techniques, opening avenues for automated analysis and large-scale applications.

How to cite: Mascaut, F., Pujol, O., and Forkman, P.: Objective characterization of mesoscale cloud patterns from graph theory and an Ising-like model (BICIM)., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10486, https://doi.org/10.5194/egusphere-egu25-10486, 2025.

EGU25-10865 | ECS | Orals | AS5.5

Developing Neural Operators for Modeling PM2.5 and CO over India 

Sanchit Bedi, N.M. Anoop Krishnan, and Sri Harsha Kota

Machine Learning (ML) has been widely explored for its potential in modelling air quality in numerous studies in the past. However, these approaches approximated function that maps the finite-dimensional input and output vectors. This restricts their extrapolation to unseen data and different discretization. Neural operators, a class of neural networks approximate the operator between infinite dimensional input and output functions. These models learn the underlying operator between input functions and their time-evolved state directly from data. In this work, we introduce our contribution to the field of neural operators termed Complex Neural Operator (CoNO) to learn the evolution of PM2.5 and CO concentrations over India. We trained our models using WRF-Chem simulated data over India for the years 2016-2018 and evaluated it for the year 2019. We assess our models for forecasting high pollution events, long-term forecasting (up to 72 hours) and city-level forecasts for six cities targeting two key pollutants.

How to cite: Bedi, S., Krishnan, N. M. A., and Kota, S. H.: Developing Neural Operators for Modeling PM2.5 and CO over India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10865, https://doi.org/10.5194/egusphere-egu25-10865, 2025.

EGU25-11971 | Posters on site | AS5.5

Estimating Anthropogenic NOx Emissions Using Convolutional Neural Networks with Horizontal Transport Considerations 

Yucong Zhang, Steffen Beirle, Leon Kuhn, Thomas Wagner, and Liangyun Liu

Nitrogen oxides (NOx = NO + NO₂) are significant air pollutants, mainly emitted from anthropogenic sources. Bottom-up methods for the estimation of anthropogenic NOx emissions are based on energy consumption data, which, if outdated, result in a delayed response in the produced emission inventories. The TROPOspheric Monitoring Instrument (TROPOMI) provides high-resolution NO₂ column densities, offering valuable data for estimating NOx emissions. Given the short atmospheric lifetime of NOx, horizontal transport influences over distances within a few tens to a few hundred kilometers must be taken into account. To address this, we developed a convolutional neural network (CNN) which incorporates the NO₂ divergence and horizontal transport features to estimate the anthropogenic NOx emissions. Our model operates on a monthly timescale with a spatial resolution of 0.1°, utilizing TROPOMI NO₂ column densities and ERA5 wind field data as inputs, and the EDGARv8.1 0.1° gridded NOx inventories as targets. The training set comprised data from 2019 and 2020, of which 70 % were used for training, and the remaining 30 % for testing of the model. The model achieved an R² of 0.922 and an RMSE of 11.214 Mg/month on the test set when estimating NOx emissions in Europe and the USA. Additionally, the model demonstrated temporal generalization capabilities, achieving an average R² of 0.853 (±0.066) and an average RMSE of 16.545 (±3.804) Mg/month in monthly estimations for Europe and the USA during 2021-2022. The proposed method integrates satellite observations with emission inventories, employing CNNs to facilitate rapid updates of anthropogenic NOx emissions.

How to cite: Zhang, Y., Beirle, S., Kuhn, L., Wagner, T., and Liu, L.: Estimating Anthropogenic NOx Emissions Using Convolutional Neural Networks with Horizontal Transport Considerations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11971, https://doi.org/10.5194/egusphere-egu25-11971, 2025.

EGU25-13106 | ECS | Posters on site | AS5.5

Physics-Informed AI for Enhanced Climate Downscaling and Extreme Event Prediction in the Energy Sector 

Pascal Léon Thiele, Jasmin Lampert, Marianne Bügelmayer-Blaschek, Katharina Baier, Kristofer Hasel, Theresa Schellander-Gorgas, and Irene Schicker

Climate change is a pressing reality, with increasing extreme weather events such as droughts, floods, and heatwaves causing significant damages and casualties [1]. To mitigate these impacts, climate neutrality has become a global priority. This requires a transition to renewable energy, necessitating accurate weather and climate models [2]. High-resolution Regional Climate Models (RCMs) offer detailed projections but are computationally expensive. Statistical downscaling techniques provide a more efficient alternative but have limitations, such as the inability to capture relevant climate change signals and underestimating extreme events. To address these issues, we propose a physics-informed artificial intelligence (AI) model bridging the gap between data-driven and model-driven approaches, by incorporating known physical principles and domain knowledge into the learning and prediction process [3,4].

In this research, we focus on developing a physics-informed AI model for efficient downscaling of climate and weather data, enabling high-resolution projections that enhance renewable energy predictions. More specifically, we aim for improving downscaling techniques, reducing uncertainties, and accurately representing extreme weather events. Key research questions include identifying suitable datasets for downscaling, evaluating errors, and improving multivariate downscaling from coarse (100 km for GCM, 10 km for RCM) to high resolutions (5 km to 1 km). Our developed method is compared against dynamical downscaling techniques across different temporal and spatial resolutions. This research aims to advance climate and weather predictions for impact sectors in need of very high spatial resolutions through providing an efficient and fast AI-based downscaling method, particularly for renewable energy applications, aiming at supporting decision-making and adaptation strategies in the face of climate change.

References

[1] IPCC, 2021 IPCC, 2021: Climate Change 2021: The Physical Science Basis. Contribution of Working Group I to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change [Masson-Delmotte, V., P. Zhai, A. Pirani, S.L. Connors, C. Péan, S. Berger, N. Caud, Y. Chen, L. Goldfarb, M.I. Gomis, M. Huang, K. Leitzell, E. Lonnoy, J.B.R. Matthews, T.K. Maycock, T. Waterfield, O. Yelekçi, R. Yu, and B. Zhou (eds.)]. Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, In press, doi:10.1017/9781009157896.

[2] Schaeffer, Roberto, Alexandre Salem Szklo, André Frossard Pereira De Lucena, Bruno Soares Moreira Cesar Borba, Larissa Pinheiro Pupo Nogueira, Fernanda Pereira Fleming, Alberto Troccoli, Mike Harrison, and Mohammed Sadeck Boulahya. 2012. ‘Energy Sector Vulnerability to Climate Change: A Review’. Energy 38 (1): 1–12. https://doi.org/10.1016/j.energy.2011.11.056.

[3] Harder, Paula, Alex Hernandez-Garcia, Venkatesh Ramesh, Qidong Yang, Prasanna Sattigeri, Daniela Szwarcman, Campbell Watson, and David Rolnick. 2022. ‘Hard-Constrained Deep Learning for Climate Downscaling’. arXiv. https://doi.org/10.48550/ARXIV.2208.05424.

[4] Karniadakis, George Em, Ioannis G. Kevrekidis, Lu Lu, Paris Perdikaris, Sifan Wang, and Liu Yang. 2021. ‘Physics-Informed Machine Learning’. Nature Reviews Physics 3 (6): 422–40. https://doi.org/10.1038/s42254-021-00314-5.

How to cite: Thiele, P. L., Lampert, J., Bügelmayer-Blaschek, M., Baier, K., Hasel, K., Schellander-Gorgas, T., and Schicker, I.: Physics-Informed AI for Enhanced Climate Downscaling and Extreme Event Prediction in the Energy Sector, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13106, https://doi.org/10.5194/egusphere-egu25-13106, 2025.

EGU25-13224 | ECS | Orals | AS5.5

Diffusion models for image-based nowcasting of desert dust for West Africa 

Kilian Hermes, John Marsham, Martina Klose, Franco Marenco, Melissa Brooks, and Massimo Bollasina

Diffusion models have been shown highly capable for image generation tasks and more recently have been adapted for weather forecasting, allowing sharper predictions than forecasts generated by previous methods, and straight-forward generation of ensemble predictions. Their value for image-based predictions is evident. Dust storms are frequent high-impact weather phenomena in West Africa that directly impact human life, e.g., by disrupting land and air traffic, posing health threats, and affecting energy delivery from solar-energy systems. Timely and precise prediction of these phenomena is crucial to mitigate adverse impacts.

State-of-the-art machine learning-based weather prediction (MLWP) models do not predict dust since they are limited by computational constraints and by the need of high-quality aerosol reanalyses. Moreover, the current operational numerical weather prediction (NWP) models for Africa still need improvement for resolving the short-scale dynamics and surface properties which leads to the formation of convective dust storms, and also often the convection itself. This is where observation-based short term forecasts (“nowcasts”) become particularly valuable. Nowcasts can provide greater skill than NWP on short time-scales, can be frequently updated, and have the potential to predict phenomena currently operational NWP and MLWP models do not reproduce. However, despite routine high frequency and high resolution observations from satellites, as of January 2025, no nowcast of dust storms is available.

In this study, we present an image-based approach for nowcasting dust storms: we apply a diffusion model to predict next frames of the SEVIRI desert dust RGB composite, a product of false-colour satellite images highlighting both dust and deep convection. We create nowcasts of this RGB composite for a large domain over West Africa up to 6 hours ahead and show that our nowcasts can predict both convective storms and convectively generated dust storms which currently operational NWP may not reliably reproduce. Furthermore, we create ensemble predictions, allowing a probabilistic forecast assessment.

Our approach provides a valuable tool that could be used in operational forecasting to improve the prediction of convective storms, dust storms, and indeed other weather events. Due to the technical similarity of RGB composite imagery from geostationary satellites, this approach could also be adapted to nowcast other RGB composites, such as those for ash, or convective storms. In the wider context, such nowcasts of brightness temperatures and brightness temperature differences, which the RGB composites are based on, could be used for predicting other products which use these satellite retrievals.

How to cite: Hermes, K., Marsham, J., Klose, M., Marenco, F., Brooks, M., and Bollasina, M.: Diffusion models for image-based nowcasting of desert dust for West Africa, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13224, https://doi.org/10.5194/egusphere-egu25-13224, 2025.

We use machine learning (ML) to map column-integrated water vapor (IWV) to characterize atmospheric rivers (ARs) and to map planetary boundary layer (PBL) height given Global Navigation Satellite Systems (GNSS) radio occultation (RO) data. GNSS RO of the Earth’s atmosphere obtains vertical profiles of microwave refractivity with vertical resolution approaching 100 meters. RO is effectively a water vapor sounder in the lower troposphere and is especially sensitive to vertical gradients associated with the top of the PBL. RO soundings undersample synoptic variability of the atmosphere with severe nonuniformity in spatial and solar angle distribution, making the creation of atmospheric model-agnostic level 3 climatologies a complicated task. ML methods have already shown great promise for mapping RO retrieved quantities in the horizontal and time. We present two applications of ML to RO data, the first to characterize ARs, and the second to map PBL height.

In a mission architecture trade study, we use an ML approach to determine what type of small-satellite constellation would be appropriate to map ARs with detail sufficient for atmospheric process studies and for the prediction of the severe weather on the U.S. Pacific coast that results from ARs. Because ARs are high-volume flows of water vapor in filaments within the PBL and RO sounds water vapor, RO data are ideally suited as input to ML algorithms for the study of ARs. How many low-Earth orbiting RO sounders would be needed to gain desired information on ARs remains an open question, as does our ability to map ARs with existing program-of-record RO data. We answer these questions by formulating ML algorithms to map ARs in the North Pacific Ocean from simulated and real RO data. Simulated RO sounding geolocations are defined by various sizes and types of Walker constellations, realistic GNSS orbits, and the interpolation of refractivity profiles from the ECMWF operational forecast system. We develop two neural networks, one to convert refractivity soundings between 0 and 10 km to IWV and another to map IWV in the horizontal in 1-hr time windows. We find that optimal performance is obtained with Walker constellations of 36 or more RO satellites in near-polar orbits, appropriate orbits for temporal uniformity of the RO’s sampling density. The advent of GNSS RO satellites in micro-satellite and nano-satellite form factors makes such constellations feasible and affordable in the very near future.

We then use ML to map PBL height. The PBL is the part of the atmosphere closest to the Earth’s surface. In the PBL, turbulent processes often affect the vertical redistribution of heat and moisture and their exchange influences cloud evolution and large- to meso-scale circulation. The PBL height can be used to describe climatological processes in a specific region, including cloud characterization. The high vertical resolution of RO observations is suitable to model PBL height in individual profiles. Initially, we use the changes in refractivity to model the PBL height at RO locations and times. Then, we apply ML to produce global PBL heights with a high temporal resolution.

How to cite: Shehaj, E., Leroy, S., and Cahoy, K.: A machine learning framework to map Atmospheric Rivers and Planetary Boundary Layer height from GNSS radio occultation observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13623, https://doi.org/10.5194/egusphere-egu25-13623, 2025.

EGU25-14109 | Orals | AS5.5

Large-Scale Deep Learning for Global Precipitation Type Classification 

Marko Orescanin, Dalton Duvio, and Veljko Petkovic

Accurate classification of precipitation type (convective vs. stratiform) from passive microwave satellite observations is fundamental for understanding global precipitation patterns and improving weather prediction models. While previous studies have demonstrated the effectiveness of deep learning approaches with accuracies above 90% on smaller temporal windows, questions remain about model generalization across extended time periods and different surface types. This study presents a comprehensive analysis using a nine-year Global Precipitation Measurement (GPM) mission dataset, followed by a detailed investigation of surface-type specialization. 

Our primary analysis leverages over 400 million samples from 2014-2022, using 32x32 pixel patches and a ResNet architecture. This large-scale model achieved an accuracy of 85% on a holdout test-year, with balanced performance across both precipitation types (F1-score of 0.85 for both convective and stratiform classes). While matching the general performance range of previous approaches, these results demonstrate robust generalization capabilities across a much longer temporal span and diverse global conditions, using a significantly larger training dataset. 

To further investigate model generalization, we conducted a specialized analysis to examine performance across different surface types creating distinct datasets for land and ocean. ResNet-50 architectures were trained for three comparative models: a baseline model using combined data, a land-only, and an ocean-only model. Analysis revealed that the baseline model achieved robust performance across both surface types (82 % accuracy over land, 86 % over ocean). Surprisingly, surface-specific models showed minimal improvement, with the land-specific model achieving 81% and the ocean-specific model reaching 85% accuracy on their respective domains. This suggests that larger, diverse datasets enable models to learn more robust features that generalize well across data subsets. 

These findings demonstrate that deep learning models can effectively maintain consistent performance when scaling to multi-year global datasets, and suggest that investing in larger, more diverse training datasets provides robust generalization across both temporal and spatial dimensions without requiring specific subsetting. The approach could lead to more efficient operational systems while maintaining reliable classification accuracy across different surface types and extended time periods. 

How to cite: Orescanin, M., Duvio, D., and Petkovic, V.: Large-Scale Deep Learning for Global Precipitation Type Classification, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14109, https://doi.org/10.5194/egusphere-egu25-14109, 2025.

EGU25-14355 | Orals | AS5.5

Physics-Constrained Machine Learning Model Enhances Weather Forecast Accuracy and Physical Consistency 

qiusheng huang, xiaohui zhong, xu fan, and hao li

Data-driven weather forecasting models, such as FuXi and Pangu-Weather, have made significant advancements in global forecasting accuracy and computational efficiency. However, these models lack physical constraints, a limitation that traditional numerical weather prediction (NWP) models address through the dynamical core and physical parameterization schemes. Recent efforts, like NeuralGCM and PINNs, have successfully integrated the dynamical core or Navier-Stokes equations with machine learning models. Yet, effective integration of physical parameterization schemes remains uncharted in this field, primarily due to the greater uncertainty and complexity of physical processes compared to the dynamical core. To bridge this gap, we integrated the shortwave radiative transfer scheme with FuXi, by modeling the Rapid Radiative Transfer Model for General Circulation Models Applications (RRTMG) as a neural network. This represents the first successful integration of a physical parameterization scheme with large-scale weather forecasting models. This integration yielded substantial improvements in forecasting performance and physical consistency, reducing root mean square error (RMSE) by approximately 15% for radiatively related variables, such as albedo and cloud water mixing ratio, especially for longer lead times.  Moreover, the optimized model demonstrated significantly enhanced atmospheric moisture energy conservation.  This work provides a promising pathway for integrating physical processes into machine learning based weather forecasting models, paving the way for more accurate and physically consistent weather forecasts.

How to cite: huang, Q., zhong, X., fan, X., and li, H.: Physics-Constrained Machine Learning Model Enhances Weather Forecast Accuracy and Physical Consistency, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14355, https://doi.org/10.5194/egusphere-egu25-14355, 2025.

EGU25-14604 | ECS | Orals | AS5.5

Multilevel Deep Learning for Non-Local Prediction of ABL Flow Fields Across Varying Stability Regimes 

John Keithley Difuntorum, Marwan Katurji, Jiawei Zhang, and Peyman Zawar-Reza

Understanding and predicting wind flow structures within the atmospheric boundary layer (ABL) across varying stability conditions remains a key challenge in atmospheric science and environmental modeling. Although large-eddy simulation (LES) provides high-fidelity insights, it is computationally prohibitive for near-real-time or large-scale applications. To address this, we propose a deep learning framework that predicts the two-dimensional wind flow fields in the u, v, and w components at a target height z, using corresponding flow fields at three levels above z. By integrating vertical flow correlations and continuity principles, our approach captures essential turbulent features while reducing input dimensionality and eliminating the need for full 3D simulations.

A modified convolutional neural network (CNN) forms the core of this framework, capturing complex spatial and temporal patterns from high-resolution LES datasets. Mass conservation is embedded in the training process to ensure physically consistent results. Preliminary results indicate that the model preserves large-scale turbulence features and captures the influence of higher-elevation dynamics, although smaller high-frequency turbulent features require further refinement. To address this, our ongoing work includes adopting a scale-specific approach to explicitly handle the diverse turbulent length scales observed in the ABL. We are also incorporating multitemporal dynamics and attention mechanisms into the architecture of our model to better account for long-range dependencies over time, thereby enabling the model to adapt to different stability regimes and transitions among them. To enhance interpretability, we will employ explainable AI (XAI) tools such as SHAP and GradCAM, revealing how specific regions in the input influence the emergence of particular turbulent footprints in the predicted flow. These insights guide improvements in both model design and understanding of atmospheric processes governing ABL flow development.

This research underscores the transformative potential of deep learning in boundary layer meteorology. By significantly reducing computational demands while retaining essential flow dynamics, our model enables real-time, high-resolution predictions of ABL flows. This scalable and efficient framework opens new possibilities for diverse applications, including weather forecasting, wind energy optimization, and environmental analysis.

How to cite: Difuntorum, J. K., Katurji, M., Zhang, J., and Zawar-Reza, P.: Multilevel Deep Learning for Non-Local Prediction of ABL Flow Fields Across Varying Stability Regimes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14604, https://doi.org/10.5194/egusphere-egu25-14604, 2025.

EGU25-14723 | ECS | Orals | AS5.5

Efficient machine learning frameworks for prediciting China’s future air quality trends 

Fengwei Wan, Lu Shen, and Zhe Jiang

Fine particulate matter (PM2.5) and ozone pollution cause a significant number of premature deaths in China each year. Evaluating the effects of emission mitigation and climate change on air quality with climate-chemistry models is computationally expensive. In this study, we develop two machine learning models — a deep learning framework based on U-Net image segmentation and long short-term memory (LSTM) neural networks, and an extreme value model — to predict China’s future air quality trends. These models are trained using model simulation results from 2014 to 2022 under high to low anthropogenic emission scenarios. The deep learning model yields promising results for PM2.5, with an R2 of 0.79 and root mean squared error (RMSE) of 12.58 ug/m3. The extreme value model for ozone episode exceedance rates achieves an R2 of 0.97 and RMSE of 1.43%. This work demonstrates the potential of deep learning and extreme value models in efficiently modeling air quality, offering robust tools for future air quality assessments.

How to cite: Wan, F., Shen, L., and Jiang, Z.: Efficient machine learning frameworks for prediciting China’s future air quality trends, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14723, https://doi.org/10.5194/egusphere-egu25-14723, 2025.

EGU25-15264 | ECS | Posters on site | AS5.5

Deep learning for global three-dimensional ocean modeling with physical response consistency 

Jeong-Hwan Kim, Daehyun Kang, Young-Min Yang, and Jae-Heung Park

With the advent of the AI era, deep learning has been actively applied to global weather prediction, achieving remarkable progress. Furthermore, these deep learning-based global prediction models are being utilized for seasonal forecasting, with efforts underway to extend the forecast lead time. Leveraging the memory effect of the ocean is essential for such advancements. In this study, we developed a deep learning-based global three-dimensional ocean model, incorporating three key innovations: (1) expanding the receptive field and reducing the number of parameters using a visual attention network, (2) eliminating ocean/land boundary effects through the application of partial convolution, and (3) aligning prediction value distributions with observations using adversarial loss. Compared to persistence forecasts and NMME models, our model demonstrated global three-dimensional ocean simulation capabilities comparable to state-of-the-art coupled general circulation models, achieving significant improvements, particularly in predicting horizontal ocean currents. Furthermore, the model realistically simulated the ocean’s response to surface boundary forcing. These results highlight the potential for developing a deep learning-based ocean-atmosphere coupled general circulation model.

How to cite: Kim, J.-H., Kang, D., Yang, Y.-M., and Park, J.-H.: Deep learning for global three-dimensional ocean modeling with physical response consistency, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15264, https://doi.org/10.5194/egusphere-egu25-15264, 2025.

EGU25-15746 | ECS | Posters on site | AS5.5

From Prediction to Causation: Understanding theDrivers of Maximum Deep Convective Systems Area 

Alejandro Casallas, Andrea Polesello, Caroline Muller, and Sophie Abramian

Deep convective systems (DCSs) play a crucial role in the tropical hydrological cycle and radiative budget (Stephens et al., 2023; Roca et al., 2014). In particular, the largest and longest-lived of those cloud systems contribute to a high fraction of the extreme precipitation in the Tropics (Roca and Fiolleau, 2020). Therefore understanding what drives these types of systems is crucial. To that end, Abramian (2023) developed a new method to predict the maximum area of DCSs using the DYAMOND-Summer simulation with the cloud-resolving global model SAM, and the TOOCAN algorithm to track cloud systems. The method uses simple machine learning models, trained on information on the early stage of the systems and their surrounding environment, including dynamical and thermodynamical variables, morphological features of the systems and the characteristics of their neighbors.
We improve this method by incorporating an integrated gradients (IG) approach, which provides a more precise quantification of the importance of each input variable directly from the neural network model. Furthermore, we embedded the neural network outputs into a causal discovery framework by identifying the variables that explain the most variance, using the IG method. These key variables were then subjected to a causal discovery analysis, enabling the identification of causal drivers that influence the maximum extent of the systems at various stages of their lifecycle.
This approach improves both interpretability and includes causal inference to avoid non-causal relations. Preliminary results suggest that during the early stages (0.5 hours after the onset of the DCS), the strength of vertical velocity and upper tropospheric saturation explain most of the variance in the system’s maximum area. Interestingly, the presence of neighboring systems also plays a significant role, likely because a smaller number of neighbors allows more moisture and energy to be available for the DCS to grow. In contrast, during the later stages (around 3.5 hours after the DCS onset), when the area reaches its maximum, neighboring systems no longer contribute significantly to the variance. At this stage, thermodynamic factors, particularly
moisture and temperature, emerge as the primary drivers, with the 2-meter temperature playing a particularly important role, suggesting a potential role of cold pools in determining the maximum area of the system.

How to cite: Casallas, A., Polesello, A., Muller, C., and Abramian, S.: From Prediction to Causation: Understanding theDrivers of Maximum Deep Convective Systems Area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15746, https://doi.org/10.5194/egusphere-egu25-15746, 2025.

EGU25-16620 | ECS | Posters on site | AS5.5

Deep Learning based Bias Correction of Forecast Products with Fusion of Geographical Information 

Sai Zhang, Ruyan Chen, Yuxiang Huang, and Xin Zhang

Accurate numerical weather prediction is a prerequisite for disaster prevention and mitigation. Based on the numerical ocean-atmosphere-wave coupling forecasting model developed by our team, artificial intelligence technology is introduced to correct prediction bias, addressing the systematic forecast error inherent in numerical models, and further enhancing the accuracy and reliability of our forecast products. This study aims to establish a bias correction model for the numerical forecast products and integrate multi-source geographic information, such as elevation, land cover, and soil type, to improve the forecast results. Convolutional Neural Networks (CNNs) effectively extract spatial features through the computational mechanisms of their convolutional modules, making them well-suited for tasks like meteorological forecast correction, where spatial correlations have a significant impact. We employ a Residual Convolutional Neural Network to efficiently extract the spatial features from numerical model forecast results, leading to improved correction performance compared to traditional correction methods. A spatiotemporal feature extraction module is utilized to adaptively detect terrain and surface features at different scales, addressing the extraction and fusion of multi-source heterogeneous features. We further evaluate and optimize the impact of terrain and land surface features at different resolutions on model correction effectiveness, maximizing prediction accuracy. This research will provide strong technical support for enhancing the precision of ocean-atmosphere-wave coupling forecasting products and offer reliable data assurance for disaster prevention and mitigation efforts.

How to cite: Zhang, S., Chen, R., Huang, Y., and Zhang, X.: Deep Learning based Bias Correction of Forecast Products with Fusion of Geographical Information, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16620, https://doi.org/10.5194/egusphere-egu25-16620, 2025.

EGU25-17016 | Orals | AS5.5

Towards machine learning-based Earth system models 

Christian Lessig

Large scale machine learning is currently revolutionizing Earth system modeling and the next generation of models will likely be machine learning-based or contain substantial machine learning components. The lack of a complete equation-based description of the Earth system as well as the availability of a plethora of high-quality data make this a tantalizing possibility to obtain models with unprecedented capabilities. In the first part of the talk, we will discuss grand challenges for building machine learning-based Earth system models and what milestones have already been achieved in the last years. We will also examine cases where machine learning models already surpass state-of-the-art equation-based models, e.g. for medium range weather forecasting. In the second half of the talk, we will introduce the WeatherGenerator project that aims to build a next generation, machine learning-based Earth system model. Led by leading European modeling centers but open-source from day-1, the project will train on a wide range of datasets to build a seamless prediction model that can faithfully represent Earth system dynamics from sub-km scale, short term processes to multi-decadal projects. The project will also consider selected applications to ensure the real-world applicability of the developed model.

How to cite: Lessig, C.: Towards machine learning-based Earth system models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17016, https://doi.org/10.5194/egusphere-egu25-17016, 2025.

EGU25-18422 | ECS | Posters on site | AS5.5

Bias Correction of Maximum Temperature Forecasts for Ensemble-Based model using Various Machine Learning Techniques for Hyderabad Station 

Sakshi Sharma, Arun Chakraborty, Anumeha Dube, Harvir Singh, and Raghavendra Ashrit

The increasing frequencies of extreme weather events like heavy precipitation, drought, heatwaves, etc, have been associated with climate change in recent years. The reliability of air temperature forecasts at 2 meters above the surface is vital when trying to prepare for potential weather-related disasters, such as heat waves. In recent years, there has been a lot of emphasis placed on the prediction of heatwave conditions over India by using deterministic Numerical Weather Prediction (NWP) models. Despite improvements in model physics and resolution, deterministic NWP models have difficulties predicting extreme events at longer lead times. As the model integrates over time, errors grow due to the uncertainty associated with the initial conditions. This uncertainty is taken into account using ensemble prediction systems (EPSs). Heatwaves are now being predicted in India using EPSs due to their better performance in predicting events with longer lead times. The intensity of extreme events is typically underestimated by these models because EPSs typically have a low resolution and are also affected by the systematic biases present in the parent deterministic models. So to make the forecast more reliable, bias correction of the maximum temperature forecasts from EPSs is required.

This study focuses on the comparative assessment of various machine learning techniques for bias correction of maximum temperature from ensemble forecasts of maximum temperature for Hyderabad station. Three machine learning techniques were used in this study, namely Random  Forest,  Gradient Boost, and Support Vector Machine. The temperature forecasts used in this study were obtained from the National Centre for Medium Range Weather Forecasting (NCMRWF) global ensemble prediction system (EPS—called the NEPS). The NEPS configuration is based on the UK Met Office Global and Regional Ensemble Prediction System (MOGREPS).  The climatology used in this study is obtained from the MOGREPS data available on TIGGE and the observations for the maximum temperature are from the Indian Meteorological Department (IMD) station data (1985-2021), this data is used as the training set. The objective of this research study is to improve the accuracy of temperature forecasts by utilizing machine learning techniques for the bias correction of maximum temperature in order to improve model performance, primarily based on metrics such as Root Mean Square Error (RMSE). The initial raw RMSE values for Day 3, Day 5, and Day 7 are recorded as 2.1461, 2.4741, and 2.811, respectively. By examining the refined RMSE values for these specific forecast days, model corrections are revealed using Support Vector Machines (SVM), Gradient Boosting (GB), and Random Forest (RF) . After correction, the SVM model achieves improvements of 18.42%, 26.29%, and 27.42% in RMSE, demonstrating its increased predictive accuracy for Days 3, 5, and 7. Similarly, the RMSE reductions for GB on Day 3, Day 5, and Day 7 are observed at 18.77%, 26.23%, and 28.16%, while RF exhibits reductions of 39.21%, 28.24%, and 22.5% for the corresponding forecast days.  The percentage reductions indicate the improved accuracy attained by bias correction employing various machine learning methods.

Keywords: Heat Waves, Ensemble Prediction Systems, Support Vector Machine, Random Forest, Gradient boost.

How to cite: Sharma, S., Chakraborty, A., Dube, A., Singh, H., and Ashrit, R.: Bias Correction of Maximum Temperature Forecasts for Ensemble-Based model using Various Machine Learning Techniques for Hyderabad Station, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18422, https://doi.org/10.5194/egusphere-egu25-18422, 2025.

EGU25-18459 | ECS | Orals | AS5.5

Leveraging observations to bias-correct the Arctic surface energy budget in reanalysis through machine learning 

Akil Hossain, Paul Keil, Harsh Grover, and Felix Pithan

The Arctic Ocean plays a critical role in global climate dynamics, yet direct observations of its surface energy budget are sparse and largely constrained to individual field campaigns. Current estimates often rely on reanalysis data, notably ERA5, which demonstrates systematic biases in boundary-layer properties and surface fluxes over Arctic sea-ice. In this study, we train an artificial neural network (ANN) to predict surface fluxes observed during MOSAiC, SHEBA, Arctic Ocean 2018 and ARTofMELT expeditions using ERA5 data as input. Data from shorter field campaigns, such as N-ICE, are used for testing our model against unseen data. Our results indicate that ERA5 Arctic surface fluxes exhibit very low correlations with observations and are characterized by large RMSE values. Our predictions demonstrate significant error reductions across key variables: sensible heat flux (~39%), 2m temperature (~39%), net shortwave radiation (~37%), downward longwave radiation (~21%) and net longwave radiation (~17%). Furthermore, we find a higher correlation (~0.58) with observations compared to ERA5 (~0.24) and approximately 50% reductions in RMSE of the hourly total surface energy budget, i.e. the sum of the individual fluxes. We produce a bias-corrected estimate of surface energy fluxes over Arctic sea-ice. We use our bias correction to revise previous estimates of the climatological surface energy budget over Arctic sea ice. We will make the trained weights available to allow for the custom derivation of bias-corrected fluxes in individual case studies and for climate model evaluation.

How to cite: Hossain, A., Keil, P., Grover, H., and Pithan, F.: Leveraging observations to bias-correct the Arctic surface energy budget in reanalysis through machine learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18459, https://doi.org/10.5194/egusphere-egu25-18459, 2025.

Urban heat islands (UHI) exacerbate health and environmental challenges, disproportionately affecting vulnerable populations. This study identifies high-risk areas for UHI effects in the Americas, including their metropolitan regions, using a suitability analysis model. It highlights the interplay between urban expansion, social vulnerability, and climate stress, emphasizing the urgency of addressing these issues in rapidly urbanizing contexts.

High-resolution satellite imagery and geospatial data were used to build the model. Key criteria included population density (dasymetric layers from WorldPop), relative wealth index, land surface temperature (LST) from MODIS, land cover from MODIS, PM2.5 and NO2 concentrations (Sentinel-5P), and road network layers derived for the analysis. Each criterion was reclassified, transformed to a common scale, and weighted equally to ensure consistency and comparability.

The suitability index was generated using raster algebra (weighted sum), producing a continuous map where higher values indicate greater susceptibility to heat stress and lower socioeconomic status. The analysis revealed spatial patterns that highlight areas with high potential impacts due to UHI characteristics.

The suitability index serves as a tool for identifying priority areas for targeted interventions and climate mitigation actions. This integrative approach highlights the need for sustainable urban development policies that reduce socio-environmental disparities and promote resilience in vulnerable communities

How to cite: Rocha, T.: Identifying Urban Heat Island Risk Areas with Vulnerable Populations: A Suitability Analysis Approach to support Health Interventions in the Americas, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-742, https://doi.org/10.5194/egusphere-egu25-742, 2025.

EGU25-1299 | Posters on site | ESSI1.6

Building a framework for the design and deployment of digital twins: the Digital Twin Factory project 

Thibault Xavier, Dawa Derksen, Vincent Martin, and Pierre-Marie Brunet

The digital twin is a useful tool for scientists and decision makers to understand the present (what now), explore future trajectories (what next) to to investigate the future impacts of current risk mitigation actions (what if), or of a system. Working at the local scale allows detailed physics to be implemented in an approach that better captures the complexity of the study site (city, watershed, etc.) in an approach that complements the global scale. The availability of very high-precision spatial products (optical, 3D, thermal, etc.) enables this high-precision local analysis anywhere on the Earth.This growing interest is leading a number of actors to build digital twins at the local scale. However, building this type of representation requires a dedicated effort from the user, usually a scientist, which prevents him from focusing on the scientific added value he could bring with his thematic expertise.
The Digital Twin Factory (DTF, 2024-2026) project, coordinated by the French National Centre of Space Studies (CNES), aims to provide users with a framework capable of building, deploying and operating a digital twin at the scale of the site. It is designed as a Digital Twin as a Service API (PaaS) to abstract the underlying infrastructure, with possibility of accessing both the HPC resources and usual Cloud providers. The DTF also provides users with methodological building blocks to access (catalogue harvester), manipulate (ingester, data processing pipeline), visualize and analyze (plot, dashboarding) the data. In this way, the instantiators of the digital twin can focus on their thematic expertise and deploy their physical solvers with access to multi-source data.
While high performance computing resources can be made available to run these physical models, parametric studies or climate trajectories may require high cost and long simulation times. Partial or full data based surrogate model is an approach that can overcome this barrier and provide results in a reactive manner. Part of the DTF's work is therefore aimed at providing users with methodological building blocks for surrogate modelling, based on the expertise of the scientific community.
This contribution presents the multi-layered architecture of the DTF project, its different components and the services offered to users. We illustrate this work with the construction of the digital Twin of Nokoué Lake in Benin that integrates flood forecasting, pollution control, salinity management, long-term risk evolution, risk governance, and adaptation measures. Satellite data are used as input for a hydrodynamic code, on which first developments of surrogate models are presented.

How to cite: Xavier, T., Derksen, D., Martin, V., and Brunet, P.-M.: Building a framework for the design and deployment of digital twins: the Digital Twin Factory project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1299, https://doi.org/10.5194/egusphere-egu25-1299, 2025.

An Earth System Digital Twin (ESDT) is a dynamic, interactive, digital replica of the state and temporal evolution of Earth systems. It integrates multiple models along with observations, and connects them with analysis, AI, and visualization tools. Together, these enable users to explore the current state of the Earth system, predict future conditions, and run hypothetical scenarios to understand how the system would evolve under various assumptions. To establish a sustainable, extensible, and expandable ESDT solution, a formal software architecture is needed. Through the collaboration across multiple NASA centers, the teams partnered with the Apache Software Foundation to establish the professional open-source Integrated Digital Exploratory Analysis System (IDEAS) framework for digital twins. IDEAS is designed with three basic concepts. 

  • Design to Exploit– ESDT architect needs to be aware of existing freely available provisioned data, model, and visualization services that the ESDT could benefit from. In computer science, we instructed our students the simple Don’t Repeat Yourself (DRY) principle. The is especially true for ESDT, because ESDT is aiming for operational big data solutions, not just a quick demonstration. If an organization is already actively making their curated data, analysis, or model outputs available, the ESDT should find ways to exploit them. Software reuse is another form of exploitation. Why reinvent? Exploiting existing services and software reuse would significantly reduce future operation costs. An ESDT should also be prepared to be exploited by other ESDTs. It will be discussed in the Design to Expand principle. 
  • Design to Extend– An ESDT needs to be extensible to support new measurements, models (both numeric and AI-based), and interfaces. As we are connecting our digital assets, we will encounter gaps and limitations, both in data and technology. As we identify new climate phenomena or scientific needs, the ESDT needs to be prepared for these changes in technology and requirements. 
  • Design to Expand– It would be unrealistic to expect a single ESDT is capable to replicate the complex Earth System that is equipped with all the past and present observations, to drive all possible global and regional numerical models, and process all AI capabilities concerning instruments, data, and predictions. We could try to acquire all publicly available data, but an ESDT should also be able to integrate private, commercial data. The Babel-like ESDT would require significant computing and store, and well as staff (science and technical) to operate. This is the motivation behind the open-source IDEAS framework, to encourage collaboration to set up common public-facing architecture. Imagine being able to orchestrate a federation of ESDTs using exploration tools like a Jupyter notebook without having to setting up a local ESDT instance. We think federated ESTDs is the answer to making actionable science available to Disadvantaged Communities. 

The presentation will discuss IDEAS architecture, its latest progress, and its growing portfolio of digital twins for the Earth including air quality, wildfire, hydrology, and coastal zone.

How to cite: Huang, T.:  Integrated Digital Exploratory Analysis System (IDEAS) – An Open-Source Software Framework for Digital Twins, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2622, https://doi.org/10.5194/egusphere-egu25-2622, 2025.

EGU25-3702 | ECS | Posters on site | ESSI1.6

What if Data story telling was the corner stone for environmental digital twins? 

Faten EL outa and Guillaume Dechambenoit

Environmental digital twins face significant interdisciplinary challenges in their development and operation, particularly in managing complex environmental data and facilitating effective communication among diverse stakeholders. While these virtual representations of environmental systems offer powerful capabilities for monitoring and decision-making, they often struggle to bridge the communication gap between technical experts, decision-makers, and end-users.

Data storytelling is the practice of narrating messages derived from data to address specific needs and visually communicating these messages to an audience in an ordered manner that is easily understandable. Interestingly, digital twins share a similar objective: both aim to simplify and communicate complex data through intuitive and meaningful narratives.

Building on this shared characteristic, we propose an approach that adapts data storytelling techniques to the creation of digital twins. This abstract focuses on how data storytelling can enhance the creation and communication of digital twin data through visual formats tailored to specific audiences, addressing their unique needs to support monitoring, decision-making, and actionable insights.

This innovative integration of data storytelling and environmental digital twins establishes a comprehensive approach to address three key challenges:

  • Documenting and structuring the development process  from data to communication to incorporate stakeholder needs and communication requirements from the outset.
  • Facilitating collaboration among interdisciplinary teams through shared narrative frameworks.
  • Ensuring environmental insights are effectively translated into actionable knowledge.

We present a methodology that leverages data storytelling techniques to enhance the accessibility and impact of environmental digital twins, ultimately improving their effectiveness in environmental monitoring, decision-making, and stakeholder engagement.

 

How to cite: EL outa, F. and Dechambenoit, G.: What if Data story telling was the corner stone for environmental digital twins?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3702, https://doi.org/10.5194/egusphere-egu25-3702, 2025.

EGU25-4499 | ECS | Orals | ESSI1.6

Coupling approaches for data-driven Earth system models 

Lorenzo Zampieri, Harrison Cook, Rachel Furner, Sara Hahner, Florian Pinault, Baudouin Raoult, Nina Raoult, Mario Santa Cruz, and Matthew Chantry

Machine learning models have emerged as powerful tools for simulating Earth system processes. Following their successful application in capturing atmospheric evolution for medium-range weather forecasts, attention has increasingly shifted towards other components of the Earth system, such as the marine and land environments. This interest is further driven by the potential to enhance forecasting capabilities beyond the medium range. Machine learning frameworks offer remarkable flexibility in integrating these model components to achieve a coherent Earth system representation. At one end of the spectrum, model components can be trained jointly within a unified framework optimised using a shared loss function. At the other end, components may be developed independently and coupled by exchanging physically relevant information at multiple interfaces, mirroring the traditional coupling strategies employed in numerical models. In this presentation, we will examine the advantages and challenges of these approaches, with a particular emphasis on coupling the atmospheric, land, and marine components within the deterministic AIFS model, the machine learning-based forecast system developed at ECMWF. Furthermore, we will compare the coupling strategies of data-driven models with those of traditional numerical models, highlighting their strengths and limitations.

How to cite: Zampieri, L., Cook, H., Furner, R., Hahner, S., Pinault, F., Raoult, B., Raoult, N., Santa Cruz, M., and Chantry, M.: Coupling approaches for data-driven Earth system models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4499, https://doi.org/10.5194/egusphere-egu25-4499, 2025.

EGU25-5110 | Orals | ESSI1.6

Digital twin for weather-induced extremes 

Roger Randriamampianina and the DestinE Extremes Digital Twin Team

Our presentation aims to describe the development and operationalisation of the Destination Earth (DestinE) Extremes Digital Twin (DT), including the On-Demand component, a system designed to improve the prediction and management of extreme weather events in Europe. The system leverages high-resolution weather models using information from Extreme Detection (EDF) and Triggering (DTF) Frameworks, as well as ECMWF ensemble, incorporating impact-specific models for hydrology, air quality, renewable energy, and more. A key component is a configuration lookup table prioritising end-user needs and available resources. The system incorporates various masking techniques (ACCORD models configurations, geographical, capacity, event type) to refine forecasts. The presentation describes the system's architecture, data sources, and workflow, emphasising the integration of multiple models and data sources, and the use of cutting-edge technologies such as GPUs and machine learning for enhanced forecasting and efficient resource utilisation. Pilot regions are used for testing and operationalisation, with a phased approach planned for broader deployment. The project addresses challenges in forecasting accuracy, communication of uncertainty, and the integration of forecasts into decision-making processes across various sectors.

How to cite: Randriamampianina, R. and the DestinE Extremes Digital Twin Team: Digital twin for weather-induced extremes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5110, https://doi.org/10.5194/egusphere-egu25-5110, 2025.

EGU25-5909 | ECS | Orals | ESSI1.6

Enhancing the Skill of Medium Range Forecasts with a Machine Learning Based Multi-Model Super-Ensemble (MMSE) 

Karan Purohit, Mitali Sinha, Aniruddha Panda, Subhasis Banerjee, and Ravi S Nanjundiah

In recent years, medium-range AI weather forecasting models have improved significantly, now offering forecasting accuracy comparable to classical numerical weather prediction (NWP) models, while also being faster and (once trained) less computationally demanding.

Due to inherent assumptions and limitations, all weather prediction models exhibit some degree of persistent systematic errors, also called biases, in their forecast output, with certain models performing better than others for specific variables and regions.

To address these persistent biases, we introduce a machine learning-based multi-model super-ensemble (MMSE), which collectively reduces model biases by combining the complementary strengths of each model. The MMSE assigns optimized weights to each model's forecast based on its historical performance to leverage each model’s strengths under different conditions (both spatial and temporal) rather than equally weighting models as in a simple ensemble mean.

In this work, we developed two regional MMSE models tailored to specific regions, seasons, and variables of interest. One model targets 2-meter air temperature and 10-meter wind components in Germany’s winter season, while the other targets Indian summer monsoon rainfall.

We trained the MMSE using an Extreme Gradient Boosting framework (XGBoost) to capture spatiotemporal features more effectively. The training data consisted of past forecasts from multiple AI models (FourCastNet, Pangu-Weather, GraphCast) and relevant climatology and topology data. ERA5 reanalysis served as the ground truth. The details of MMSE development will be presented.

Our MMSE developed for 2-meter temperature over Germany showed approximately a one-day improvement in forecast gain time compared to the best-performing individual model. In other words, the MMSE’s 11th-day forecast matched the accuracy of the 10th-day forecast from the best-performing model, effectively adding an extra day of reliable lead time. These findings suggest that the proposed MMSE offers a promising, computationally efficient alternative to traditional ensembles for real-time weather forecasting, with potential applications in domains requiring high-precision predictions. With a view to make these results interpretable and to identify the relative strengths of participating models, we will also present the analysis of SHAP values for various variables and regions.

How to cite: Purohit, K., Sinha, M., Panda, A., Banerjee, S., and S Nanjundiah, R.: Enhancing the Skill of Medium Range Forecasts with a Machine Learning Based Multi-Model Super-Ensemble (MMSE), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5909, https://doi.org/10.5194/egusphere-egu25-5909, 2025.

EGU25-6965 | ECS | Posters on site | ESSI1.6

Global post-processing of ERA5 precipitation product via graph-based neural networks  

Patrick Ebel, Linus Magnusson, and Rochelle Schneider

Total precipitation is a key variable of the weather state, accumulated over a given period. Beyond their direct relevance, high-quality precipitation data are of importance for driving downstream applications in hydrology, e.g. river streamflow and runoff forecasting. However, common measurements of precipitation are either precise but sparse (as for in-situ recordings) or global but uncertain (as for spaceborne observations). Though reanalysis products such as ECMWF’s ERA5 provide a best estimate of the state of the atmosphere, the quality of their total precipitation reconstruction is imperfect. Following reports that ERA5 is prone to overestimating the occurrence of drizzle at the cost of underestimating extreme precipitation, prior work explored data-driven models for local post-processing to address the latter. However, the local models employed in preceding work do not easily extend to a global post-processing setup and an exclusive emphasis on outliers limits the ability to represent the full distribution of precipitation intensity, which limits their relevance.

 

In this work, we propose a novel approach for precipitation post-processing which models the entire globe in a single forward pass and models dryness, light rain and heavy rain alike. The post-processer is based on a graph neural network architecture, trained on decades of gauge-calibrated multi-source weighted estimates of precipitation. We demonstrate that our model learns to bias-correct ERA5 total precipitation information and consistently improves upon the baseline while maintaining its global applicability. Further experiments will detail the nature of its improvements and may explore its benefits for downstream applications.  

How to cite: Ebel, P., Magnusson, L., and Schneider, R.: Global post-processing of ERA5 precipitation product via graph-based neural networks , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6965, https://doi.org/10.5194/egusphere-egu25-6965, 2025.

Developing region-specific radar quantitative precipitation estimation (QPE) products for South China (SC) is crucial due to its unique climate and complex terrain over there. Deep learning (DL) has emerged as a promising avenue for radar QPE, especially graph neural networks (GNNs). Many studies have tested the DL models in radar QPE, but virtually no studies have evaluated the performance of DL models in different precipitation intensities, types, or organizations. Moreover, limited attention has been given to whether DL-based methods can mitigate radar QPE errors caused by orographic influences in complex terrains, such as those in SC.

This study investigates the advantages of DL methods for QPE tasks in South China, utilizing nearly three years of hourly gauge data as labels and ground-based radar reflectivity as inputs. Firstly, multi-layer perceptron (MLP), Convolutional Neural Networks (CNNs), and GNNs with similar architectures are constructed and compared to traditional Z-R relationships considering precipitation types. DL methods outperform traditional Z-R relationships and GNNs perform the best. More importantly, this study conducts a systematic evaluation of the proposed GNN. For extreme precipitation (>30 mm/h), GNN achieves the smallest MAE, highlighting its potential for hazardous event estimation. It also demonstrates stable performance for stratiform and organized precipitation, with minimal bias and standard deviation. However, GNN is less effective for isolated precipitation, whereas CNNs are a better choice due to their ability to estimate scattered rainfall accurately. Last but not least, the Z-R relationship shows systematic spatial biases, overestimating precipitation in coastal plains and underestimating it in inland high-altitude regions. DL methods alleviate these terrain-induced biases by incorporating spatial information. Overall, this study highlights the advantages of DL methods across different precipitation scenarios and demonstrates their ability to mitigate systematic biases from complex terrain.

How to cite: Zhu, K. and Xu, W.: Deep Learning for Radar Quantitative Precipitation Estimation over Complex Terrain in Southern China, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8155, https://doi.org/10.5194/egusphere-egu25-8155, 2025.

EGU25-8169 | ECS | Orals | ESSI1.6 | Highlight

Exploring AI-Driven Event-based Storylines 

Amal John, Thomas Rackow, Nikolay Koldunov, Sebastian Beyer, Antonio Sanchez Benitez, Helge Gößling, Marylou Athanase, and Thomas Jung

Artificial Intelligence-based Numerical Weather Prediction (AI-NWP) models have recently emerged as powerful tools for weather forecasting, offering computational efficiency and high accuracy. This study explores the extreme weather events simulated by the Artificial Intelligence Forecasting System (AIFS), initialised with conditions derived from kilometer-scale storyline experiments using the IFS-FESOM model where the atmospheric circulation is constrained to observations. We present two case studies: the 2023 South Asian humid heatwave and the 2024 Storm Boris. These two events are reproduced in the present climate, but also simulated if they were to unfold in pre-industrial and +2K future climates, effectively creating AI-driven storylines. The methodology we employ offers a complementary framework, where the use of AI-driven ensembles provides a scalable and rapid way to assess the potential uncertainty and variability associated with such events, by enabling us to explore a broader range of plausible outcomes at very low computational costs. By combining the strengths of physics-based modelling with the efficiency and flexibility of AI-driven simulations, this dual approach offers a pathway to operationalise ensemble-based extreme weather storylines.

How to cite: John, A., Rackow, T., Koldunov, N., Beyer, S., Sanchez Benitez, A., Gößling, H., Athanase, M., and Jung, T.: Exploring AI-Driven Event-based Storylines, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8169, https://doi.org/10.5194/egusphere-egu25-8169, 2025.

EGU25-9956 | ECS | Orals | ESSI1.6

 Xaurora: Advancing subseasonal-to-seasonal forecasting by fine-tuning foundation weather models with spectral consistency  

Eliot Walt, Wessel Bruinsma, Maurice Schmeits, Efstratios Gavves, and Dim Coumou

Sub-seasonal to seasonal (S2S) timescales range from two weeks to three months and are crucial to make informed climate change-related decisions, including renewable energy resources allocation, extreme events’ risks mitigation, and the development of effective early warning systems. Unfortunately, traditional physics-based forecasting systems achieve poor skill on these lead times. Recently, deep learning (DL) has shown promising results in weather forecasting on timescales up to 10 days, reaching performance competitive with that of physical models. However, these DL approaches currently struggle on S2S timescales.  

Following previous studies on neural solvers for partial differential equations and weather forecasting, we propose a fine-tuning framework aimed at improving the S2S prediction skill of foundation weather models. Our approach has two core components. First, we implicitly condition the latent space embeddings to retain the predictable signals at a given lead time using an additional regression head. Second, we design a novel frequency-domain decoder and loss function to ensure spectral consistency. These steps should ensure that the model focuses on the most predictable frequencies. We apply this methodology to the recently published Aurora foundation model and propose Xaurora, standing for “extended Aurora”. Our fine-tuning approach represents an important milestone in data-driven S2S forecasting, addressing key challenges in the field while remaining broadly applicable with minimal assumptions on the underlying model’s architecture. 

The relevance of our framework is evaluated through ablation studies, comparing our spectral consistency fine-tuning to the original Aurora model. Furthermore, we provide standard deterministic and probabilistic skill scores on S2S timescales, as well as relevant teleconnection indexes. We present preliminary outputs of this analysis. 

How to cite: Walt, E., Bruinsma, W., Schmeits, M., Gavves, E., and Coumou, D.:  Xaurora: Advancing subseasonal-to-seasonal forecasting by fine-tuning foundation weather models with spectral consistency , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9956, https://doi.org/10.5194/egusphere-egu25-9956, 2025.

EGU25-10817 | ECS | Orals | ESSI1.6

MLOps on DestinE Data Lake – Towards Reproducible AI on Edge Services 

Sina Montazeri, Miruna Stoicescu, Oriol Hinojo Comellas, Danaële Puechmaille, and Michael Schick

Destination Earth (DestinE) is European Commission’s initiative to gradually develop highly accurate Digital Twins (DT)s of the Earth with unprecedented accuracy and resolution. DestinE will initially provide DTs for adapting to climate change, forecasting extreme events and interactive use of high-resolution climate data. Insights from these models support scientists and policymakers to study and plan for future weather- and climate-induced events. 

Stakeholders implementing what-if scenarios and/or ready to use applications on DestinE require the optimum storage and the seamless provision of access to a sheer volume of heterogeneous data often available from different data origins. EUMETSAT has implemented the DestinE Data Lake (DEDL) to address the above challenges. The DEDL offers the Harmonised Data Access (HDA) service that enables access to diverse data from the DEDL data portfolio via a unified STAC API. Furthermore, it offers, for power users, DEDL edge services on request, which are a dynamic suite of distributed big data processing components that operate close to DestinE’s massive data repositories. The edge services offered  are:  STACK (DEDL-managed software applications such as JupyterHub, DASK and Open Data Cube), ISLET (project-managed compute and storage services such as configurable virtual machines and S3 object storage) and HOOK (schedule and run pre-defined or user-defined high-level workflows, such as setting up a data processing pipeline). 

To efficiently exploit the wealth of data available on DestinE, DEDL edge services will extend their abilities to accommodate the necessary infrastructure and software to enable Artificial Intelligence/Machine Learning (AI/ML) activities. DEDL will offer an ML Operations (MLOps) service tailored to Earth Observation (EO) data, which allows users to engage in various steps of AI/ML such as data preprocessing, model training and evaluation, experiment tracking, model deployment, model inference and monitoring. The modularized DEDL MLOps architecture will allow the users to use components as required without the need to be bound to pre-defined workflows and pipelines. The users, furthermore, can develop their AI/ML algorithms according to CI/CD best practices and have multiple environments for development, staging and production. 

A specific focus of DEDL will be to define and work with highly flexible data pipelines. The framework will allow to convert DestinE data portfolio datasets to AI-ready formats, which can readily be used as inputs for various AI/ML models. The framework will have the capability to combine and harmonise data from various sources and formats and provides typical EO-based pre-processing steps such as data collocation, re-projection, and re-gridding among other operations. 

This presentation will highlight the AI/ML and MLOps capabilities of the DEDL, demonstrating how they empower users to efficiently analyse data and derive valuable insights. By seamlessly integrating with DestinE’s data ecosystem, these advancements enable users to focus on innovation and address critical challenges such as climate adaptation and extreme event forecasting, rather than on managing complex workflows or infrastructure. 

How to cite: Montazeri, S., Stoicescu, M., Hinojo Comellas, O., Puechmaille, D., and Schick, M.: MLOps on DestinE Data Lake – Towards Reproducible AI on Edge Services, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10817, https://doi.org/10.5194/egusphere-egu25-10817, 2025.

EGU25-11883 | ECS | Orals | ESSI1.6

Developing a data-driven global ocean model at ECMWF  

Rachel Furner, Rilwan Adewoyin, Mario Santa Cruz, Sara Hahner, Sarah Keeley, Kristian Mogensen, and Lorenzo Zampieri

Machine learning (ML) techniques have emerged as a powerful tool for predicting weather and climate systems, particularly in predicting the short-term evolution of the atmosphere. Here, we look at the potential for ML to predict the evolution of the 3d-ocean. 

We present a data-driven global ocean model, developed within the Destination Earth project, to form the ocean component of a fully data-driven earth system model. Following the skill shown by the AIFS (Lang et al, 2024), we use a graph-based encoder-decoder design, with a transformer backbone. Our model is trained on the ECMWF ORAS6 reanalysis dataset (Zuo et al, 2024). Work focuses on short-term predictions, up to a 2-week forecast period. The model predicts temperature, salinity, zonal and meridional current components throughout the full ocean depth, along with sea-surface height and sea-ice. 

In this presentation we will discuss the design choices of our network architecture, including comparisons between networks trained to predict future fields, and those trained to predict increments to fields. We will show results from our data-driven model and put these into the context of other similar models. 

Simon Lang, Mihai Alexe, Matthew Chantry, Jesper Dramsch, Florian Pinault, Baudouin Raoult, Mariana C. A. Clare, Christian Lessig, Michael Maier-Gerber, Linus Magnusson, Zied Ben Bouallègue, Ana Prieto Nemesio, Peter D. Dueben, Andrew Brown, Florian Pappenberger, and Florence Rabier (2024). AIFS – ECMWF’s data-driven forecasting system. arXiv preprint https://arxiv.org/abs/2406.01465.  

Hao Zuo, Magdalena Alonso-Balmaseda, Eric de Boisseson, Philip Browne, Marcin Chrust, Sarah Keeley, Kristian Mogensen, Charles Pelletier, Patricia de Rosnay, Toshinari Takakura (2024). ECMWF’s next ensemble reanalysis system for ocean and sea ice: ORAS6. ECMWF newsletter. https://doi.org/10.21957/hzd5y821lk  

How to cite: Furner, R., Adewoyin, R., Santa Cruz, M., Hahner, S., Keeley, S., Mogensen, K., and Zampieri, L.: Developing a data-driven global ocean model at ECMWF , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11883, https://doi.org/10.5194/egusphere-egu25-11883, 2025.

EGU25-11988 | Orals | ESSI1.6

Development of an offline and online hybrid model for the Integrated Forecasting System 

Marcin Chrust, Alban Farchi, Massimo Bonavita, Marc Bocquet, and Patrick Laloyaux

Systematic model errors significantly limit the predictability horizon and practical utility of the current state-of-the-art forecasting systems. Even though accounting for these systematic model errors is increasingly viewed as a fundamental challenge in the field of numerical weather prediction, estimation and correction of the predictable component of the model error has received relatively little attention. Modern implementations of weak-constraint 4D-Var are an exception here and a promising avenue within the variational data assimilation framework, showing encouraging results. Weak-constraint 4D-Var can be viewed as an online hybrid data assimilation and machine learning approach which gradually learns about model errors from partial and imperfect observations, allowing to improve the state estimation. We propose a natural extension of this approach by applying deep learning techniques to further develop the concept of online model error estimation and correction.

In this talk, we will present recent progress in developing a hybrid model for the ECMWF Integrated Forecasting System (IFS). This system augments the state-of-the-art physics-based model with a statistical model implemented via a neural network, providing flow dependent model error corrections. While the statistical model can be pre-trained offline, we demonstrate that by extending the 4D-Var control vector to include the parameters of the neural network, i.e. the model of model error, we can further improve its predictive capability. We will discuss the impact of applying the flow dependent model error corrections in the medium range forecasts on the forecast quality.

How to cite: Chrust, M., Farchi, A., Bonavita, M., Bocquet, M., and Laloyaux, P.: Development of an offline and online hybrid model for the Integrated Forecasting System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11988, https://doi.org/10.5194/egusphere-egu25-11988, 2025.

EGU25-12042 | Posters on site | ESSI1.6

Implementing FAIR Agrobiodiversity Workflows for the Destination Earth Data Lake 

Claus Weiland, Daniel Bauer, Desalegn Chala, Dag Endresen, Jonas Grieb, Marcella Orwick Rydmark, and Gabriela Zuquim

The Horizon Europe project “Biodiversity Digital Twin for Advanced Modelling, Simulation and Prediction Capabilities” (biodt.eu) combines state-of-the-art supercomputing resources with FAIR data practices to address biodiversity grand challenges such as the loss of diversity at genetic, species and ecosystem levels driven by factors such as anthropogenic climate change, intensified land use and the spreading of alien invasive species.

Key tools for the integration and assessment of such information in BioDT are so-called prototype Digital Twins (pDTs) which provide digital replicas of particular phenomena of the biosphere. The data produced by pDTs and the computational workflows themselves are annotated with rich machine-interpretable metadata, notably schema.org and its Bioschemas and Croissant (high-level metadata format for machine learning datasets) extensions to enable discovery and interaction with the data for humans and machines. 

The crop wild relatives digital twin developed in BioDT for the identification of novel genetic resources in crop wild relatives (CWR) aims to support the development of mitigation strategies against food-related crises associated with climate change (doi:10.3897/rio.10.e125192). Underutilised crops and CWR are a valuable source of untapped genetic diversity for implementing such strategies because their greater genetic diversity in relation to crops makes adaptation to droughts, cold waves, heavy precipitation or other weather-induced extreme events possible. They are therefore of particular importance to guarantee food security.  

We developed a pilot study to migrate and functionally integrate the pDT CWR in the Destination Earth Data Lake (DEDL) to increase its availability and, more importantly, use both data provided in the data space and the near data processing features of DEDL to improve models and prediction. The framework makes use of web-based technologies such as RO-Crates and FAIR Signposting to facilitate reuse and repurposing of the data within and across different data spaces as well as orchestrated interplay of multiple digital twins (involving the Climate Change Adaptation Digital Twin). 

Building on this blueprint, we will showcase in this presentation the deployment of FAIR agrobiodiversity workflows in DEDL’s compute service Islet and the subsequent publication of results in a lightweight service framework (figure).

How to cite: Weiland, C., Bauer, D., Chala, D., Endresen, D., Grieb, J., Orwick Rydmark, M., and Zuquim, G.: Implementing FAIR Agrobiodiversity Workflows for the Destination Earth Data Lake, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12042, https://doi.org/10.5194/egusphere-egu25-12042, 2025.

EGU25-12349 | Orals | ESSI1.6

How Destination Earth Data Lake support Destination Earth users 

Patryk Grzybowski, Marcin Ziółkowski, Aubin Lambare, Christoph Reimer, and Michael Schick

Destination Earth (DestinE) is a flagship initiative led by the European Commission, implemented by EUMETSAT, ESA and ECMWF. It aims to create highly detailed Digital Twins (DTs) of the Earth, enabling precise simulations for a variety of uses. Currently, the initiative focuses on two primary Digital Twins:  the Weather Extremes Digital Twin (ExtremeDT) and the Climate Change Adaptation Digital Twin (ClimateDT). Over the coming years, the scope of DTs is set to expand, necessitating improved access to data and streamlined methods for working with it. This is where the Destination Earth Data Lake (DEDL) plays a pivotal role, offering comprehensive data discovery, access, and processing services tailored to the needs of DestinE users.

The DEDL operates on two key levels: ‘Data Discovery and Access’ and ‘Edge Services’. DEDL Discovery and Data Access services is provided by Harmonized Data Access (HDA) tool which provides a single, federated entry point to the services and data, including resources from existing datasets and complementary sources such as in-situ and socio-economic data. Notably, it also provides access to the unique datasets generated by DestinE’s DT’s. The services rely on use of the SpatioTemporal Asset Catalogs (STAC) standard which means:

  • The search in the dataset is done according to the STAC protocol;
  • The Federated Catalog search proxy component converts STAC queries into queries adapted to the underlying catalog and returns the results to the user in STAC format.

The cloud computing service is powered by the ISLET infrastructure, a distributed Infrastructure as a Service (IaaS) built on OpenStack. It allows users to manage virtual machines, s3 storage, and run advanced computations via a graphical user interface or command-line interface. A standout feature of ISLET is its proximity to data sources, operating near High-Performance Computing (HPC) facilities. This is achieved through data bridges, enabling efficient processing of large datasets, including those from Digital Twins, in conjunction with HPC systems.

The STACK environment supports application development using JupyterHub and DASK, with Python, and R languages. Users can create DASK clusters on selected infrastructure (sites) to process data directly where it resides, removing the need for extensive local setup and optimization.

Hook Services is a set of pre-defined workflows which could be used by users as a ready-to-use processors like: Sentinel-2: MAJA Atmospheric Correction; Sentinel-1: Terrain-corrected backscatter. It also enables workflow functions to generate on-demand higher-level products, such as temporal composites.

DEDL is a transformative initiative that revolutionizes how Earth Observation data is managed and utilized. By integrating innovative infrastructure (ISLET), data services (HDA), reliable processors (Hook Services), and user-friendly development tools (STACK), DEDL enables unprecedented levels of data harmonization, federation, and processing. Moreover, the DEDL plays a crucial role in empowering DestinE users by providing them with seamless access to vast datasets and advanced computational tools. It simplifies the process of data exploration, integration, and analysis, enabling researchers, policymakers, and developers to focus on innovation and decision-making rather than technical barriers. This cutting-edge system enhances climate research capabilities and supports sustainable development efforts on a scale previously unattainable.

How to cite: Grzybowski, P., Ziółkowski, M., Lambare, A., Reimer, C., and Schick, M.: How Destination Earth Data Lake support Destination Earth users, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12349, https://doi.org/10.5194/egusphere-egu25-12349, 2025.

EGU25-13817 | Posters on site | ESSI1.6

Real-time Prediction of Global Tropical Deciduous Ecosystem Phenology with Deep Learning 

Minchao Wu, Torbern Tagesson, Zhanzhang Cai, and Zheng Duan

Tropical deciduous ecosystems play a critical role in terrestrial ecological processes and the global carbon cycle, influencing seasonal climates through phenology-induced biophysical and biogeochemical feedbacks. Phenological processes for tropical deciduous ecosystems are complex with multiple intertwining climatic and physiological factors that co-shape the underlying dynamics. Here, we present a deep learning framework based on Temporal Fusion Transformer for predicting tropical deciduous phenology globally in real-time with high accuracy. The framework integrates long-term AVHRR-derived vegetation greenness data, high-resolution climate data from ERA-Land, and land surface features including physical and chemical properties to account for terrestrial spatial heterogeneities that affect phenological processes. Our preliminary results demonstrate the ability of the developed framework to accurately predict historical phenological dynamics across 35 growing seasons in the pan-tropical regions. Key phenological metrics, including the start, peak, and end of the growing season, are identified with high accuracy. We believe the framework provides a powerful tool for real-time predictions and reconstructions of phenological states for tropical deciduous ecosystems, especially in regions where human activities like deforestation and agriculture heavily influence the estimates of tropical carbon cycle potential. With insight into the potential phenological states, this framework may help inform sustainable land management practices in pan-tropical regions.

How to cite: Wu, M., Tagesson, T., Cai, Z., and Duan, Z.: Real-time Prediction of Global Tropical Deciduous Ecosystem Phenology with Deep Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13817, https://doi.org/10.5194/egusphere-egu25-13817, 2025.

EGU25-14658 | Posters on site | ESSI1.6

Comparison of the Minimum Bounding Rectangle and Minimum Circumscribed Ellipse of Rain Cells from TRMM 

HongKe Cai, YaQin Mao, XuanHao Zhu, YunFei Fu, and RenJun Zhou

Based on the TRMM dataset, this paper compares the applicability of the improved MCE (minimum circumscribed ellipse), MBR (minimum bounding rectangle), and DIA (direct indexing area) methods for rain cell fitting. These three methods can reflect the geometric characteristics of clouds and apply geometric parameters to estimate the real dimensions of rain cells. The MCE method shows a major advantage in identifying the circumference of rain cells. The circumference of rain cells identified by MCE in most samples is smaller than that identified by DIA and MBR, and more similar to the observed rain cells. The area of rain cells identified by MBR is relatively robust. For rain cells composed of many pixels (N > 20), the overall performance is better than that of MCE, but the contribution of MBR to the best identification results, which have the shortest circumference and the smallest area, is less than that of MCE. The DIA method is best suited to small rain cells with a circumference of less than 100 km and an area of less than 120 km2, but the overall performance is mediocre. The MCE method tends to achieve the highest success at any angle, whereas there are fewer “best identification” results from DIA or MBR and more of the worst ones in the along-track direction and cross-track direction. Through this comprehensive comparison, we conclude that MCE can obtain the best fitting results with the shortest circumference and the smallest area on behalf of the high filling effect for all sizes of rain cells.

How to cite: Cai, H., Mao, Y., Zhu, X., Fu, Y., and Zhou, R.: Comparison of the Minimum Bounding Rectangle and Minimum Circumscribed Ellipse of Rain Cells from TRMM, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14658, https://doi.org/10.5194/egusphere-egu25-14658, 2025.

EGU25-14783 | ECS | Posters on site | ESSI1.6

A Unified Model of Forecasting Ozone by Deep Learning 

Zhenze Liu

We propose a simple yet effective framework for real-time surface ozone forecasting using deep learning. The framework highlights three key modules: independent channel encoders, frequency information extraction, and fine-tuning, all of which consistently enhance model performance. This unified model is built well to autonomously capture different spatial and temporal patterns of ozone concentrations, with an averaged RMSE of 8 ppb for day 1 forecasting. The performance of day 4 forecasting is slightly lower. We find that chemistry becomes less important than meteorology over time, indicating their different roles in short-term and long-term forecasting. Most high ozone episodes can be simulated, though capturing extremely high ozone values remains a challenge. Observations from China are trained and tested to demonstrate our model.

How to cite: Liu, Z.: A Unified Model of Forecasting Ozone by Deep Learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14783, https://doi.org/10.5194/egusphere-egu25-14783, 2025.

EGU25-15162 | ECS | Posters on site | ESSI1.6

Uncertainty Evaluation of Deep Learning Models Using an Artificial Rainfall 

Younghun Kim and Giha Lee

Accurate rainfall prediction is essential not only for water resource management but also for forecasting and mitigating the impacts of climate change-driven weather events such as floods and droughts. Due to the high spatiotemporal variability of complex meteorological phenomena like rainfall, effective prediction necessitates in high-quality data collection, model application, and uncertainty analysis. Unlike existing studies that focus primarily on developing deep learning models to improve rainfall prediction accuracy, this study evaluates the uncertainty of rainfall predictions using pre-existing deep learning models, U-Net and ConvLSTM, with artificially generated elliptical rainfall data. Artificial rainfall data were designed with four temporal patterns: constant, gradually increasing, gradually decreasing, and time-varying. These patterns were applied in horizontal, vertical, and diagonal movements to evaluate the models' ability to handle spatiotemporal complexity. The results indicate that both deep learning models exhibited spatial smoothing issues on rainfall predictions over time. However, the U-Net model demonstrated superior spatiotemporal performance compared to ConvLSTM. While this study focuses solely on deep learning models for rainfall prediction, future research will consider factors such as data complexity and loss functions to conduct a comprehensive evaluation of prediction uncertainty. This work is expected to contribute to the development of methodologies for rainfall modeling using deep learning approaches.

 

Funding: This research was supported by Disaster-Safety Platform Technology Development Program of the National Research Foundation of Korea(NRF) funded by the Ministry of Science and ICT. (No. 2022M3D7A1090338)

How to cite: Kim, Y. and Lee, G.: Uncertainty Evaluation of Deep Learning Models Using an Artificial Rainfall, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15162, https://doi.org/10.5194/egusphere-egu25-15162, 2025.

EGU25-15669 | ECS | Orals | ESSI1.6

Post-Processing Neural Weather Model Outputs for Tropical Cyclone Intensity Forecasts 

Milton Gomez, Tom Beucler, Alexis Berne, and Louis Poulain--Auzéau

Numerical Weather Prediction (NWP) models, which integrate physical equations forward in time, are the traditional tools for simulating atmospheric processes and forecasting weather in modern meteorology. With recent advancements in deep learning, Neural Weather Models (NeWMs) have emerged as competent medium-range NWP emulators with reported performances that compare favorably to state-of-the-art NWP models. However, they are commonly trained on reanalysis with limited spatial resolution (e.g., 0.25° horizontal grid spacing) and thus smooth out key features associated with a number of weather phenomena. For example, tropical cyclones—among the most impactful weather events due to their devastating effects on human activities—are challenging to forecast, as extrema like wind gusts, which serve as proxies for tropical cyclone intensity, are smoothed in deterministic forecasts at 0.25° resolution. To address this, we use our best global observational estimate of wind gusts and minimum sea level pressure to train models that post-process NeWM outputs and enable accurate and reliable forecasts of TC intensity. We present a tracking-independent post-processing algorithm and show that even naïve, linear models extract useful information from NeWM model outputs beyond what is present in the initial conditions used to roll out NeWM predictions. We explore how the NeWM’s spatial context may further improve the forecast through masking and convolutional architectures. Our post-processing framework thus presents a step towards democratization of tropical cyclone intensity forecasting, given the reduction in computational requirements for producing global weather forecasts with NeWMs compared to traditional NWP approaches and the algorithmic simplicity of the tracking-independent approach.

How to cite: Gomez, M., Beucler, T., Berne, A., and Poulain--Auzéau, L.: Post-Processing Neural Weather Model Outputs for Tropical Cyclone Intensity Forecasts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15669, https://doi.org/10.5194/egusphere-egu25-15669, 2025.

EGU25-15811 | Orals | ESSI1.6

Climate Adaptation Digital Twin – building an operational climate information system to support decision-making 

Jenni Kontkanen, Mario Acosta, Pierre-Antoine Bretonnière, Miguel Castrillo, Paolo Davini, Francisco Doblas-Reyes, Barbara Früh, Jost von Hardenberg, Thomas Jung, Heikki Järvinen, Daniel Klocke, Nikolay Koldunov, Pekka Manninen, Sebastian Milinski, Jarmo Mäkelä, Devaraju Naraynappa, Suraj Polade, Irina Sandu, Outi Sievi-Korte, and Stephan Thober

The Climate Change Adaptation Digital Twin (Climate DT) is part of the Destination Earth (DestinE) initiative, developing Digital Twins of Earth to increase resilience against environmental changes. More specifically, Climate DT provides capabilities supporting climate change adaptation at regional and national levels at multi-decadal time scales. We present here an overview of Climate DT, highlighting the added value for the users and discussing the transition of the system towards the operations.  

The development of Climate DT has started in Phase 1 of DestinE, during which the first prototype of the new climate information system has been developed. A key innovation of Phase 1 was the introduction of a generic state vector (GSV), which is evolved by the Earth system models (ESMs) and streamed to applications from climate adaptation impact sectors.  This has created a basis for a pioneering climate information system that enables (i) provision of global climate information at an unprecedented granularity, (ii) scaling the system across a number applications that have access to all the data they need, (iii) user-centric approach with new ways of co-design and opportunities for enhancing interactivity. In Phase 2, which started in May 2024, our focus is on operationalizing Climate DT to deliver high-quality climate and impact-sector information regularly while incorporating new interactive features.

The operational model of the Climate DT is built around three storm- and eddy resolving ESMs; ICON, IFS-NEMO and IFS-FESOM. The operational framework utilizes a DevOps-like cycle, including three set-ups: d-suite for development, e-suite for testing the operational set-up and o-suite for operating the system. The o-suite simulations will provide data covering both past (1990-2020) and future periods (2020-2050) with a 5 km global grid. Additionally, capabilities for special simulations are developed, including story-line simulations for future periods of extremes as well as what-if scenario simulations enabling a new level of interactivity.

The added value of Climate DT to users is demonstrated through four impact sector applications. These applications operate on the streamed GSV as part of the operational framework, and they are improved in co-design with key users. The impact sector applications cover societally relevant climate change adaptation domains, including wind energy management, disaster risk management (with regards to wildfires and floods), as well as agriculture and water management. Climate DT output, including high-resolution climate simulations, storyline simulations, user-relevant indicators and impact assessments are made available to users via DestinE Service Portal.

How to cite: Kontkanen, J., Acosta, M., Bretonnière, P.-A., Castrillo, M., Davini, P., Doblas-Reyes, F., Früh, B., von Hardenberg, J., Jung, T., Järvinen, H., Klocke, D., Koldunov, N., Manninen, P., Milinski, S., Mäkelä, J., Naraynappa, D., Polade, S., Sandu, I., Sievi-Korte, O., and Thober, S.: Climate Adaptation Digital Twin – building an operational climate information system to support decision-making, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15811, https://doi.org/10.5194/egusphere-egu25-15811, 2025.

EGU25-15912 | Orals | ESSI1.6

ClimateBenchPress: A Benchmark for Compression of Climate Data 

Tim Reichelt, Juniper Tyree, Milan Kloewer, Peter Dueben, Bryan Lawrence, Dorit Hammerling, Alisson Baker, Sara Faghih-Naini, and Philip Stier

The rapid growth of weather and climate datasets is increasing the pressure on data centres and hinders scientific analysis and data distribution. For example, kilometre-scale weather and climate models can generate 20 gigabytes of data per second when run operationally, making it generally infeasible to store all output unless advanced compression is applied. 

To address this challenge, novel lossy compression techniques, including recently so-called neural compressors which learn smaller representations of climate data, have been proposed with compression factors beyond 100x. However, if applied without care, lossy compression can remove valuable information from a dataset for often unknown downstream applications. It is therefore important to validate that the compression process does not alter scientific conclusions drawn from the data. Whether the compression error is tolerable is often easier to assess for domain experts and rarely well defined. 

Here, we address this challenge by presenting a benchmark suite for lossy compression of climate data (atmosphere, ocean, and land). We are defining data sets that can be used to train neural compressors as well as corresponding evaluation methods. Compressors have to pass a set of tests for each data set while compressing into the smallest file size possible at a reasonable (de)compression speed. To ensure evaluation on a diverse set of inputs, the benchmark covers climate variables following various statistical distributions at medium to very high resolution in time (hourly to yearly) and space (~1 km to 150 km). Evaluation tests are for single and multi-variable compression of gridded data with stable or changing statistics, random data access or large archives, in medium to very large datasets.

To provide references towards what compression levels can be achieved with current state of the art lossy compressors, we also evaluate a set of baseline compressors (SZ3, ZFP, Real Information) on our benchmark tasks. The benchmark is a quality check for new compressors towards a standardization of climate data compression, aiming to make compressors with high compression factors safe to use and widely supported.

How to cite: Reichelt, T., Tyree, J., Kloewer, M., Dueben, P., Lawrence, B., Hammerling, D., Baker, A., Faghih-Naini, S., and Stier, P.: ClimateBenchPress: A Benchmark for Compression of Climate Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15912, https://doi.org/10.5194/egusphere-egu25-15912, 2025.

EGU25-16981 | ECS | Posters on site | ESSI1.6

Flow matching for in situ, spatially consistent weather forecast downscaling 

David Landry, Anastase Charantonis, and Claire Monteleoni

Weather forecast downscaling, the problem of recovering accurate local predictions given a lower resolution forecast,  is commonly used in operational NWP pipelines. Its purpose is to recover some of the sub-grid processes that could not be represented by the underlying numerical model due to a limited resolution. This misrepresentation provokes statistical mismatches between the observation data gathered from stations and the nearest grid point in the numerical simulation.

Using a downscaling model typically requires making a compromise between spatial consistency and statistical calibration. Traditionally, these models are trained to target a traditional verification metric. Consequently, they suffer from the double penalty issue and fail to correctly model spatial correlation structures by becoming overly smooth. This is detrimental to downstream modeling tasks such as power grid management, which require a good assessment of spatially-correlated phenomena. 

Recently, the finer details of the atmospheric state have successfully been recovered using generative models such as denoising diffusion [2-4]. We propose a similar strategy for in situ downscaling by introducing a flow matching [1] model for that task. A cross-attention transformer [5] backbone allows us to build an internal representation for the gridded numerical forecast as well as the in situ downscaled forecast. 

Our model avoids the numerical instability and mode collapse issues related to Generative Adversarial Networks. It produces well-calibrated forecasts that better represent the spatial correlations between the stations when compared to non-generative alternatives. Our model makes no assumptions about the underlying forecast, and thus can be thought of in two ways. It can be considered a hybrid NWP/AI model, where we first run a numerical simulation and then downscale it. It can also be considered a supplementary forecasting product in a full machine learning pipeline.

Using our flow matching weather forecast downscaling model, we run experiments on the EUPPBench post-processing dataset to predict surface temperature and wind speed. Particular care is given to evaluating the model, where we assess both the marginal performance (via the CRPS, reliability histogram, and spread-error ratio) and the joint performance (via the Energy Score, local Variogram Score and forecast spatial frequency content). The accurate representation of extreme events is evaluated using Brier scores. Further experiments discuss the pitfalls of fitting the Energy Score directly without a generative model.

 

[1] Lipman, Y. et al. (2023) ‘Flow Matching for Generative Modeling’. arXiv. Available at: https://doi.org/10.48550/arXiv.2210.02747.

[2] Couairon, G. et al. (2024) ‘ArchesWeather & ArchesWeatherGen: a deterministic and generative model for efficient ML weather forecasting’. arXiv. Available at: https://doi.org/10.48550/arXiv.2412.12971.

[3] Price, I. et al. (2023) ‘GenCast: Diffusion-based ensemble forecasting for medium-range weather’. arXiv. Available at: https://doi.org/10.48550/arXiv.2312.15796.

[4] Lang, S. and Chantry, M. (2024) ‘Enter the ensembles’, AIFS Blog, 21 June. Available at: https://www.ecmwf.int/en/about/media-centre/aifs-blog/2024/enter-ensembles (Accessed: 15 January 2025).

[5] Vaswani, A. et al. (2017) ‘Attention is All you Need’, in Advances in Neural Information Processing Systems. Curran Associates, Inc. Available at: https://proceedings.neurips.cc/paper/2017/hash/3f5ee243547dee91fbd053c1c4a845aa-Abstract.html (Accessed: 17 May 2022).

How to cite: Landry, D., Charantonis, A., and Monteleoni, C.: Flow matching for in situ, spatially consistent weather forecast downscaling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16981, https://doi.org/10.5194/egusphere-egu25-16981, 2025.

EGU25-17080 | ECS | Orals | ESSI1.6

Spatial Gap Filling in a Geostationary Land-Surface Temperature Product with a Masked Autoencoder 

Matthias Karlbauer, Florian M. Hellwig, Thomas Jagdhuber, and Martin V. Butz

With the increasing availability and demand of remote sensing data from Earth observation satellites, the accuracy of weather prediction models can be improved substantially. Satellite products, such as Land-Surface Temperature (LST), however, suffer from missing data, either caused by clouds that cover the ground, by missing spatial coverage of the mission, or by outages of the sensors. Such spatial data gaps in LST products impose strict limitations when aiming to process the data further with, e.g., numerical weather prediction models assuming spatial continuity with gapless input data. We therefore propose a gap-filling algorithm based on a masked autoencoder that only receives a small percentage from a 32x32 LST snapshot and learns to reconstruct the missing patches. We use the spatial domain defined by the Land Atmosphere Feedback Initiative (LAFI) over central Europe and operate on geostationary LST data from the Copernicus Global Land Service in June 2023 at 5 km resolution. Our approach indicates considerable potential when filling spatial gaps in LST products, however, we emphasize one critical aspect. The LST estimates below clouds cannot be expected to be realistic and would require a sophisticated atmospheric correction. To mitigate this limitation, we aim to incorporate microwave data in future that penetrates clouds and therefore could help to estimate LST below clouds. In its current formulation, our algorithm can be used to fill gaps in LST products as if there were no clouds. We will show the potential and limitations of the autoencoder-based gap-filling algorithm for several showcases across Europe. 

How to cite: Karlbauer, M., Hellwig, F. M., Jagdhuber, T., and Butz, M. V.: Spatial Gap Filling in a Geostationary Land-Surface Temperature Product with a Masked Autoencoder, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17080, https://doi.org/10.5194/egusphere-egu25-17080, 2025.

The Children’s Climate Risk Index (CCRI) was first released in 2021, providing a comprehensive, global view of children’s exposure and vulnerability to the impacts of climate change. The CCRI is a composite index that aims to rank countries where children are exposed to climate and environmental hazards. The CCRI 2.0 builds on the previous index by integrating two pillars; Pillar 1 focusing on climate hazards and Pillar 2 on inherent vulnerabilities to WASH, health, education and other relevant dimensions. 

 

We highlight our contributions to CCRI 2.0, using a cluster methodology for quantifying children’s exposure to climate risks including riverine and coastal flooding, tropical storms, heatwaves, and drought. Using unsupervised learning, we allow for a data-driven approach to provide an interpretation of the ranking of children’s exposure to climate risks on a global scale between countries, as well as at the sub-national and local levels. It complements the previous method of constructing the synthesized index, which involved calculating the simple average of multiple indicators. We further discuss our techniques in tackling the challenges of multisource data processing, analysis, and visualization of geospatial data for user insight.

How to cite: Kim, D. and Doerksen, K.: Quantifying Children’s Exposure to Climate Risks using Unsupervised Learning with Multi-Source Geospatial Datasets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17875, https://doi.org/10.5194/egusphere-egu25-17875, 2025.

EGU25-18447 | ECS | Orals | ESSI1.6

ArchesClimate: Ensemble Generation for Decadal Prediction using Flow Matching 

Graham Clyne, Guillaume Couairon, Juliette Mignot, Guillaume Gastineau, Anastase Charantonis, and Claire Monteleoni

Sampling from climate models to generate ensembles of predictions is computationally expensive (Hawkins et al., 2015). Climate model ensembles are used to understand probabilities of climatic events and identify internal variability in climate models. In the short term, model uncertainty and inter-annual variability dominate uncertainty in climate predictions (Smith et al., 2019). A typical approach to address these uncertainties is to use large ensembles of non-learned, physical numerical global circulation models (GCM) (Eade et al., 2014). These ensembles allow for statistical analysis of distributions and determination of internal variability in the climate model.

Our approach demonstrates that we can efficiently learn to emulate a GCM. We use ensembles generated by the IPSL submission to the Decadal Climate Prediction Project (DCPP). The dataset ranges from 1960-2016 and produces 10-member, 10-year forecast ensembles for each year. On this dataset, we train a modified version of ArchesWeatherGen, a Swin Transformer based on PanguWeather that can be used in a generative way using flow matching (Couairon et al. 2024). The model was modified to predict additional climatic variables (e.g. air temperature, specific humidity, ocean potential temperature at depth, sea surface temperature, sea level pressure) at a monthly temporal resolution. Once trained, the model probabilistically generates ensemble members rapidly which can be auto-regressively rolled out. We show that they are physically reliable via evaluation methods that assess physical processes derived from the variables represented in the machine learning model, such as by evaluating it on El Niño/La Niña events. This model demonstrates that machine learning can enhance climate models by expanding ensemble sizes to improve our understanding of climatic processes. We aim to output physically realizable month-to-month trajectories to estimate future climate and its uncertainties across various domains, including land, ocean, and atmospheric processes.



Couairon, G., Singh, R., Charantonis, A., Lessig, C., & Monteleoni, C. (2024). ArchesWeather & ArchesWeatherGen: a deterministic and generative model for efficient ML weather forecasting. arXiv preprint arXiv:2412.12971.

Eade, Rosie, Doug Smith, Adam Scaife, Emily Wallace, Nick Dunstone, Leon Hermanson, et Niall Robinson. « Do Seasonal-to-Decadal Climate Predictions Underestimate the Predictability of the Real World? » Geophysical Research Letters 41, no 15 (2014): 5620‑28. https://doi.org/10.1002/2014GL061146.

Hawkins, Ed, Robin S. Smith, Jonathan M. Gregory, et David A. Stainforth. « Irreducible Uncertainty in Near-Term Climate Projections ». Climate Dynamics 46, no 11 (1 juin 2016): 3807‑19. https://doi.org/10.1007/s00382-015-2806-8.

Smith, D. M., R. Eade, A. A. Scaife, L.-P. Caron, G. Danabasoglu, T. M. DelSole, T. Delworth, et al. « Robust Skill of Decadal Climate Predictions ». Npj Climate and Atmospheric Science 2, no 1 (17 mai 2019): 1‑10. https://doi.org/10.1038/s41612-019-0071-y.

How to cite: Clyne, G., Couairon, G., Mignot, J., Gastineau, G., Charantonis, A., and Monteleoni, C.: ArchesClimate: Ensemble Generation for Decadal Prediction using Flow Matching, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18447, https://doi.org/10.5194/egusphere-egu25-18447, 2025.

EGU25-19021 | ECS | Posters on site | ESSI1.6

RAINA - High-resolution nowcasting of precipitation and wind extremes with a foundation model for the atmosphere 

Erik Pavel, Michael Langguth, Martin G. Schultz, Christian Lessig, Stefanie Hollborn, Jan Keller, Roland Potthast, Britta Seegebrecht, Sabrina Wahl, Juergen Gall, Anas Allaham, Mohamad Hakam Shams Eddin, and Ilaria Luise

Data-driven weather prediction models based on deep learning have been on the rise for several years and have outperformed traditional physics-based numerical models in various benchmark forecasting scores. However, a significant challenge remains: accurately predicting extreme events on a local scale, such as thunderstorms and wind gusts. Previous models struggle in this area, as they were primarily developed for medium-range forecasting and operate at relatively coarse spatio-temporal resolutions. However, the capability of weather models to predict extreme events at a local level is essential for preventing severe consequences for communities, ecosystems, and the financial and material losses they entail. Recently, task-agnostic foundation models, trained on extensive and diverse datasets using self-supervised methods, have demonstrated remarkable skill and robustness, especially in their ability to generalize to rare extreme events. 

The RAINA project aims to develop a foundation model for the atmosphere, with an emphasis on delivering reliable, high-resolution forecasts of extreme wind and precipitation events. In partnership with the EU Horizon-funded WeatherGenerator project, which aims to create advanced digital twins for Destination Earth, RAINA will extend the pioneering AtmoRep model (Lessig et al., 2023) by employing a multi-modal learning approach.
The foundation model seeks to develop a comprehensive, statistically robust, and multi-scale understanding of atmospheric dynamics by incorporating a wide range of meteorological datasets from both models and observations. Innovative deep learning methods, including diffusion models and test-time adaptation, will be investigated to facilitate short-range forecasts of temperature, wind, and precipitation at kilometer-scale resolution over Germany.

In a first demonstrator, short-range forecasts are generated using the AtmoRep model and subsequently refined with the CorrDiff downscaling approach (Mardani et al., 2024) that combines a generative diffusion model with a residual approach. This two-step strategy delivers high-resolution forecasts with a maximum lead time of six hours while disentangling uncertainties inherent in the forecasting and downscaling processes, a separation that can enhance training quality when properly applied. By using ERA5 and COSMO REA2 reanalysis data, the approach enhances the precision of high-resolution forecasts over Germany. 
Initial results from the first demonstrator will be presented in a poster, along with the overall timeline and key milestones of the RAINA project.

How to cite: Pavel, E., Langguth, M., Schultz, M. G., Lessig, C., Hollborn, S., Keller, J., Potthast, R., Seegebrecht, B., Wahl, S., Gall, J., Allaham, A., Shams Eddin, M. H., and Luise, I.: RAINA - High-resolution nowcasting of precipitation and wind extremes with a foundation model for the atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19021, https://doi.org/10.5194/egusphere-egu25-19021, 2025.

EGU25-19238 | Orals | ESSI1.6

Destination Earth Data Lake user story on Danube Delta water reservoir  

Charlotte Delmas, Aubin Lambaré, and Arnaud Le Carvennec

The Danube Delta, the second-largest delta in Europe and a critical economic waterway, represents a dynamic yet fragile ecosystem requiring effective preservation strategies. Monitoring water reservoirs is crucial for both ecological sustainability and socio-economic management. The increasing availability of diverse datasets from multiple sources offers new opportunities to enhance real-time observation and forecasting efforts. 

Implemented by EUMETSAT, the Destination Earth Data Lake (DEDL) provides seamless access to these datasets and integrates high-performance computing for complex scientific modeling. Its edge services provide efficient, scalable data processing, empowering researchers to analyze environmental phenomena with speed and precision. 

Leveraging DEDL services enables to consolidate key hydrological datasets offering important features to monitor the ecosystem’s health state: 

  • Daily live in situ data: Real-time measurements of water level, temperature, and discharge from DanubeHIS ground stations along the river and its delta, has been retrieved via the DEDL Harmonized Data Access (HDA). 
  • Outputs from existing scientific algorithms: The integration and evolution of the Surfwater algorithm within the DEDL environment allows leveraging Earth Observation data (Landsat 8/9) to detect water bodies in the area. This makes it possible to generate time series of surface areas, volumes, and fill rates of water bodies within the region. 
  • Hourly radar data: Rainfall rates are computed using OPERA radar observations on the European Weather Cloud instances. 
  • Precipitation forecasts: Predictive data from ECMWF (Destination Earth Digital Twin Outputs), accessed via HDA, are leveraged to provide valuable forecasting insights. 

The outcome of those algorithms and analysis are provided live through a dashboard. By enabling cross-referencing of diverse data streams, it allows stakeholders to obtain a complete view of the Danube Delta’s environmental conditions, supporting informed decision-making for ecosystem preservation. 

Leveraging advanced geoscience tools, this integrated approach highlights the transformative power of modern data platforms in tackling global environmental challenges. 

How to cite: Delmas, C., Lambaré, A., and Le Carvennec, A.: Destination Earth Data Lake user story on Danube Delta water reservoir , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19238, https://doi.org/10.5194/egusphere-egu25-19238, 2025.

EGU25-19942 | Orals | ESSI1.6

A Spatial Multi-Grid Neural Operator-Transformer Mdoel for High-Resolution Climate Modeling 

Maximilian Witte, Johannes Meuer, and Kadow Christopher

High-resolution machine learning faces the challenge of balancing local computation with large physical context windows. GPU memory limitations and the slow training process when distributing the model across multiple GPUs further complicate this task. 

We present a transformer model for high-resolution climate-related tasks that uses neural operators within a multi-grid architecture. This approach allows resolution independence, large physical context windows, and the handling of discontinuities such as coastlines.

The model is spatially flexible, supporting both regional and global training schemes. It is also independent of the number of input variables, allowing training to be scaled to large numbers of input variables.

We demonstrate the ability of the model to scale, both spatially and in terms of variables. The model forms the foundation of an approach to learn from the rich and diverse climate data available, enabling high-resolution downscaling, infilling, and predictions.

How to cite: Witte, M., Meuer, J., and Christopher, K.: A Spatial Multi-Grid Neural Operator-Transformer Mdoel for High-Resolution Climate Modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19942, https://doi.org/10.5194/egusphere-egu25-19942, 2025.

EGU25-20187 | Orals | ESSI1.6

TWINE: TWInning capability for the Natural Environment 

Joana Mendes, Edward Pope, Zorica Jones, Andrew Cottrell, Michael Eastman, Joshua Wiggs, Hannah Findley, Angela Heard, Paul Hallett, Emilie Vanvyve, Remy Vandaele, Hywell Williams, Milto Miltiadou, Finley Gibson, Kirstine Dale, Anna Angus-Smyth, Simon Gardner, and Sam Tailby

Digital twins are an exciting and rapidly developing research area, with the potential to provide a step change in the way we understand our evolving environment and its impact on sensitive systems.

The TWInning Capability for the Natural Environment (TWINE) programme is being co-delivered by the Met Office and Natural Environment Research Council (NERC) to explore the potential of this technology for transforming environmental science and across priority areas including climate change adaptation and mitigation, biodiversity and ecosystems, and natural hazards and their mitigation.

Through the TWINE programme, NERC and the Met Office have funded six digital twin pilot projects across a range of applications, including harmful algal blooms, flooding and coastal overtopping, optimising data collected by ocean gliders and aircraft, and multi-objective land-use decisions.

We will introduce the TWINE programme, giving a brief overview of the projects which are advancing our understanding of how we can harness the potential of digital twinning technology. These include cross-sector challenges such as: risk to natural resources, Net Zero targets, and addressing the science-to-policy lag.

How to cite: Mendes, J., Pope, E., Jones, Z., Cottrell, A., Eastman, M., Wiggs, J., Findley, H., Heard, A., Hallett, P., Vanvyve, E., Vandaele, R., Williams, H., Miltiadou, M., Gibson, F., Dale, K., Angus-Smyth, A., Gardner, S., and Tailby, S.: TWINE: TWInning capability for the Natural Environment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20187, https://doi.org/10.5194/egusphere-egu25-20187, 2025.

EGU25-1266 | Posters on site | AS5.8

First deployment of a drone-borne active AirCore in a volcanic plume at Mount Etna 

Tanja Schuck, Johannes Degen, Nicole Bobrowski, Mélisende Bossard, Lucie Boucher, Huilin Chen, Bastien Geil, Giovanni Giuffrida, Steven van Heuven, Thorsten Hoffmann, Gianluigi Ortenzi, and Andreas Engel

Uncrewed Aircraft Systems (UAS) are by now established platforms for measurements in volcanic plumes. Trace gases of interest range from sulfur dioxide and halogenated substances to carbonaceous trace gases including carbon monoxide (CO) and carbon dioxide (CO2). However, sophisticated measurement techniques for high-precision observations of trace gases often require instrumentation that cannot be used on board UAS due to the high weight and power consumption of the devices

Originally developed for stratospheric observations, air sampling with long coiled tubes in AirCores, has proven to be a light-weight sampling technique to probe parts of the atmosphere that are otherwise difficult to access. Trace gas analysis of sampled air is done post-flight, most commonly with fast high-precision optical methods, delivering high-quality and high-resolution trace gas mixing ratios. While balloon-borne AirCore setups perform so-called passive sampling, making use of natural pressure differences, in 2018, a team at Groningen University developed a UAS-deployable small active AirCore device collecting air with a small pump.

In July 2024, we deployed this AirCore setup on a UAS to probe the volcanic plume of Mt. Etna (Sicily, Italy), which was particularly active at the time of the measurements. This was to our knowledge the first time that the AirCore sampling technique was used to sample air inside a volcanic plume. The air sample was successfully analysed with cavity-ring down spectroscopy for CO, CO2 and methane (CH4). While CO and CO2 mixing ratios were markedly enhanced in the plume and signals correlated well with SO2 enhancements observed by an electro-chemical sensor, no significant enhancement of CH4 was observed. The observed trace gas mixing ratios will be used in further studies to model the chemistry in the plume of Mt. Etna.

How to cite: Schuck, T., Degen, J., Bobrowski, N., Bossard, M., Boucher, L., Chen, H., Geil, B., Giuffrida, G., van Heuven, S., Hoffmann, T., Ortenzi, G., and Engel, A.: First deployment of a drone-borne active AirCore in a volcanic plume at Mount Etna, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1266, https://doi.org/10.5194/egusphere-egu25-1266, 2025.

EGU25-4415 | ECS | Orals | AS5.8

Cloud Sampling with UAS during the #CHOPIN Campaign at Mount Helmos in October 2024 

Anna Voss, Alkistis Papetta, Franco Marenco, Spyros Bezantakos, Marine Goret, Leo Håkansson, Konstantinos Michailidis, George Biskos, Maria Kezoudi, Nikolaos Mihalopoulos, and Jean Sciare

Uncrewed Aircraft Systems (UAS) have gained a strong presence in atmospheric sciences in recent years due to their flexibility, cost-effectiveness, and ability to access areas that are challenging for manned aircraft. As part of the #CHOPIN (CleanCloud Helmos OrograPhic Site ExperimeNt) campaign, the Unmanned Systems Research Laboratory (USRL) of the Cyprus Institute deployed UAS on Mt. Helmos, Greece, from October 11 to November 1, 2024, providing valuable data for the study of clouds.  

The #CHOPIN campaign, conducted in collaboration with NCSR Demokritos and FORTH/EPFL, was hosted at the Kalavryta Ski Center with a base altitude for the UAS takeoffs and landings of 1690 m ASL. The campaign aimed to improve the understanding of aerosol-cloud interactions and to evaluate remote sensing algorithms and models. Located in a rapidly changing "climate hotspot" at the intersection of various air masses, Mount Helmos is particularly sensitive to environmental changes, with interactions between wildfire smoke, pollution, sea salt, and Saharan dust. This unique setting provides an ideal location to study the dynamics of aerosol-cloud interactions.

This study presents an overview of the UAS operations held at Mount Helmos, highlighting collection of vertical profiles of particle size distribution from the ground (1.7km ASL) up to 3.5 km ASL, both inside and outside the clouds. In contrast to point measurements from ground-based stations, UAS can follow cloud movement and sample the entirety of the cloud, capturing aerosol particle size distributions below, within, and above the clouds, and cloud droplet size-distributions. These measurements provide valuable insights into aerosol properties and cloud-aerosol interactions at different altitudes. Additionally, consecutive UAS flights helped study the evolution of the Boundary Layer Height (BLH) at the Helmos site. The data collected can fill the vertical resolution gap of aerosol size distributions and provide additional datasets for comparison with fixed station observations. 

How to cite: Voss, A., Papetta, A., Marenco, F., Bezantakos, S., Goret, M., Håkansson, L., Michailidis, K., Biskos, G., Kezoudi, M., Mihalopoulos, N., and Sciare, J.: Cloud Sampling with UAS during the #CHOPIN Campaign at Mount Helmos in October 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4415, https://doi.org/10.5194/egusphere-egu25-4415, 2025.

EGU25-4488 | Posters on site | AS5.8

Added value of off-the-shelf UAS for exploring Alpine valley flows 

Alexander Gohm

Scanning Doppler wind lidars have become an important tool for investigating the kinematic structure of the mountain boundary layer and associated local flows. However, currently, no appropriate remote sensing technique exist that can capture the thermodynamic structure (temperature and humidity) in the lowest hectometres above ground at a sufficient spatiotemporal resolution. Hence, uncrewed aircraft systems (UAS) have become a prominent tool to fill this gap.

In this work, we report how a single off-the-shelf UAS (DJI Mini 2) equipped with a temperature and humidity logger (iMet-XQ2) can provide added value for the interpretation of Doppler wind lidar observations of complex winds in a narrow Alpine valley. The study site is located at Nafingalm, a mountain pasture located at the end of the Weer Valley in Tyrol, Austria. This location will be one of the target areas of the TEAMx Observational Campaign (TOC) in summer 2025. We present data from a short campaign conducted on 01 and 02 September 2023 to test the feasibility of combined UAS and Doppler lidar measurements at this remote site. The UAS performed vertical profiles over more than 24 hours of the lowest 120 m above ground at a 30-minute interval during daytime and an hourly interval during nighttime to capture the whole boundary layer evolution.

We will show the characteristics of daytime upvalley and nighttime downvalley winds as captured by the Doppler wind lidar and the corresponding temperature structure depicted by the UAS observations. In this context, the UAS measurements were crucial for correctly interpreting the transient warming phases during early evening as turbulent mixing events resulting from the interaction of a cross-mountain airflow with the stable boundary layer in the valley. The observations indicate that the early evening transition phase is characterized by high complexity and presents an interesting phase for studying turbulent processes in more detail within the framework of the TOC.

How to cite: Gohm, A.: Added value of off-the-shelf UAS for exploring Alpine valley flows, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4488, https://doi.org/10.5194/egusphere-egu25-4488, 2025.

EGU25-4779 | Posters on site | AS5.8

Towards sensible heat flux measurements with multicopter UAS 

Norman Wildmann and Laszlo Györy

This study demonstrates the feasibility of measuring temperature variance and sensible heat flux with self-calibrated fine-wire platinum resistance thermometers (FWPRT) on multicopter drones. The sensors are especially designed for light-weight, fast response-times and to be carried on miniature drones for turbulence measurements.
A significant improvement was found in vertical profiling of temperature gradients compared to slower solid-state sensors, demonstrating reduced hysteresis between ascent and descent phases and accurate representation of strong gradients. 
More than 100 single flights with the sensors attached to drones of the SWUF-3D fleet were carried out in vicinity to a meteorological mast array at the WiValdi wind energy research park in Northern Germany. The comparison to sonic anemometers shows that mean temperature and temperature variance can be accurately measured within the background flow variability. The same applies for sensible heat flux, which was measured for the first time with multicopter UAS and the eddy covariance method. An uncertainty of 50 W m-2 was determined with the constraint that only low wind speed conditions could be used to guarantee accurate vertical wind speed measurements. The results indicate that the temperature sensors are suited for sensible heat flux measurements, but further improvements are necessary with regard to vertical wind speed estimates to decrease the overall uncertainty.

How to cite: Wildmann, N. and Györy, L.: Towards sensible heat flux measurements with multicopter UAS, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4779, https://doi.org/10.5194/egusphere-egu25-4779, 2025.

EGU25-5595 | ECS | Posters on site | AS5.8

UAV-based methodologies for quantifying methane emissions from point sources 

Abdullah Bolek, Martin Heimann, and Mathias Göckede

Uncrewed aerial vehicles (UAVs) are increasingly becoming complementary monitoring tools in various scientific fields, particularly in atmospheric and climate science, as they are versatile, relatively cheap, and can provide data at various spatial scales. However, UAV-based methodologies are still in their early stages and require extensive effort to fully exploit the potential of UAVs. Accurate quantification of emission rates from point or localized sources, such as geologic seeps or oil and gas production sites, is important for understanding emission processes and mitigating climate change. Conventional greenhouse gas monitoring platforms (i.e., flux chambers and eddy-covariance towers) have a significant sampling gap as they struggle to provide the spatial extent needed to accurately estimate emission rates from point or localized sources. UAV platforms carrying greenhouse gas analyzers for CO2 and CH4, along with an anemometer to measure 2D wind speed, air temperature, humidity, and pressure, allow capturing the spatial extent of a plume originating from a point source, and therefore accurately quantify its source strength.

The UAV platform employed for this study was used to sample a geological methane seep located in the Mackenzie Delta, Canada. Geological methane seeps can act as super emitters, releasing methane at rates significantly higher than typical biogenic sources; hence, accurate quantification of their emission rates is crucial to estimate the overall CH4 budget of the area. In July 2024, different flight strategies were tested to monitor point sources, including several curtain flights and a grid flight conducted at varying downwind distances from the seep. Using these flight data, the emission rate of the methane seep was quantified using two different methods: a mass-balance approach and a Gaussian plume inversion technique. The CH4 plume released from the seep showed concentrations about ten times higher than the atmospheric CH4 background levels, underscoring the significant potential impact of the geological seeps on the overall Arctic carbon budget.

How to cite: Bolek, A., Heimann, M., and Göckede, M.: UAV-based methodologies for quantifying methane emissions from point sources, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5595, https://doi.org/10.5194/egusphere-egu25-5595, 2025.

EGU25-6449 | ECS | Orals | AS5.8

Development of an airborne Eddy covariance system dedicated to greenhouse gases (CO2/CH4) and energy fluxes measurements of heterogeneous landscapes onboard fixed-wing UAV 

Ngoc Minh Hoang, Jean-Louis Bonne, Nicolas Dumelié, Florian Parent, Vincent Moncourtois, Grégory Albora, Jérémie Burgalat, Thomas Lauvaux, Charbel Abdallah, Pedro-Henrique Herig-Coimbra, Benjamin Loubet, Ludovic Donnat, and Lilian Joly

Climate change poses significant threats to ecosystems and human activities, necessitating urgent efforts to reduce greenhouse gas emissions. This requires new tools able to monitor and quantify emissions at the meso-scale, applicable to large industrial facilities, agricultural sites, landfills or natural areas such as forests or peatlands. To address this challenge, our project aims at developing a lightweight (< 4 kg) eddy covariance (EC) system embarked on a fixed-wing vertical take-off and landing (VTOL) uncrewed aircraft system, enabling precise measurements of greenhouse gases (CO2, CH4) and energy fluxes between the surface and the atmosphere over large and heterogeneous areas. 

The system combines a five-hole turbulence probe (ADP) to measure three-dimensional wind and air temperature, along with a custom-fabricated diode laser spectrometer for CO2, CH4 and H2O concentrations. The gas analyzer is lightweight (2.1 kg), highly accurate (< 0.5 %), capable of rapid measurements (100 Hz) and optimized for high-speed mobile platforms. 

A preliminary mobile EC system (comprising the ADP, a reference sonic anemometer and the custom gas analyzer) was mounted on a vehicular platform to evaluate the integrated sensor suite under real atmospheric conditions. Comparative analyses of instantaneous relative velocity components and turbulence spectra show close agreement between the two wind sensors, confirming the ADP’s suitability for integration into our VTOL-based EC system. Furthermore, the water vapor and CO2 concentration spectra indicate that the concentration sensor is well-suited for measuring atmospheric gases within a mobile EC setup. A continuous wavelet transform approach was applied to compute surface fluxes on agricultural fields near the road trip. Combined with a footprint analysis to study landscape heterogeneity, this lays the groundwork for a transition to a drone-based EC system.  

A flight maneuver was conducted with the ADP-equipped VTOL under unstable atmospheric conditions to validate wind and air temperature measurements. Spectral analysis indicates that the airborne platform can capture actual atmospheric turbulence. Sensible heat flux was computed for this test flight, demonstrating our drone-based EC system’s potential to generate surface fluxes and emissions maps over heterogeneous landscapes. 

As part of our future work, flight trials will be carried out to measure greenhouse gases (CO2 and CH4) and energy fluxes. These measurements will be compared against tower-based EC fluxes to evaluate the performance of the UAV-based system. 

How to cite: Hoang, N. M., Bonne, J.-L., Dumelié, N., Parent, F., Moncourtois, V., Albora, G., Burgalat, J., Lauvaux, T., Abdallah, C., Herig-Coimbra, P.-H., Loubet, B., Donnat, L., and Joly, L.: Development of an airborne Eddy covariance system dedicated to greenhouse gases (CO2/CH4) and energy fluxes measurements of heterogeneous landscapes onboard fixed-wing UAV, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6449, https://doi.org/10.5194/egusphere-egu25-6449, 2025.

EGU25-9080 | ECS | Orals | AS5.8

Quantifying methane emissions from UK Landfills Using Unmanned Aerial Vehicles 

Maria Tsivlidou, Jamie McQuilkin, Hugo Ricketts, Kieran Wood, Han Yong, and Grant Allen

Methane (CH₄) is a potent greenhouse gas, with a global warming potential 27.2 to 29.8 times greater than carbon dioxide (CO₂) over a 100-year timescale. Accurate quantification of methane emissions is crucial for developing effective climate change mitigation strategies and meeting international agreements on greenhouse gas reduction. However, significant uncertainties remain in estimating methane emissions, particularly from anthropogenic sources such as landfills, due to spatial heterogeneity and complex atmospheric interactions.

Landfills are known as significant contributors to anthropogenic methane emissions. In recent years, the use of unmanned aerial vehicles (UAVs) equipped with high-precision methane sensors has developed into a promising approach for quantifying these emissions. This method offers advantages such as improved spatial coverage, reduced operational costs and dynamic monitoring. The field of emissions quantification by UAV survey has rapidly expanded over the past decade, with a growing international academic community refining and validating methods, and an emerging commercial sector driving technological advancements.

Our study focuses on quantifying methane emissions from three UK landfills in 2024/25 using drone-based spatial sampling of in situ gas concentrations, wind speed and direction. We apply and compare different mass balance methods with varying approaches to spatial interpolation, to test the sensitivity of emission quantification to the selected approach. This analysis aims to assess the strengths and limitations of each method when applied to landfill environments. Additionally, we conduct an error analysis, examining the main sources of uncertainty such as wind measurements and background methane concentrations. 

By addressing these challenges, our research contributes to improving the accuracy and robustness of drone-based methane quantification for landfill applications (and similar local scale sources). This work supports the development of methods for measuring emissions directly, which is crucial for setting emission reduction targets and improving national greenhouse gas inventories in waste management.

How to cite: Tsivlidou, M., McQuilkin, J., Ricketts, H., Wood, K., Yong, H., and Allen, G.: Quantifying methane emissions from UK Landfills Using Unmanned Aerial Vehicles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9080, https://doi.org/10.5194/egusphere-egu25-9080, 2025.

EGU25-9677 | ECS | Posters on site | AS5.8

Improving the accuracy of particle concentration measurements of an optical particle counter (UCASS) for balloon soundings 

Sina Jost, Ralf Weigel, Konrad Kandler, Luis Valero, Jessica Girdwood, Chris Stopford, Warren Stanley, Luca K. Eichhorn, Christian von Glahn, and Holger Tost

Since the Earth's energy balance is also influenced by aerosols and cloud droplets, knowledge concerning their size, number and vertical distribution is essential. To enable frequent, continuous, and cost-effective observations, a balloon-borne optical particle counter (“Universal Cloud and Aerosol Sounding System” (UCASS)) was developed by the University of Hertfordshire (UK). Hitherto, GPS or pressure-based measurements of the balloon’s ascent rate have been used to calculate the air’s flow velocity and volume flow rate through the UCASS, from which aerosol and cloud droplet concentrations were obtained. However, it appeared reasonable to modify the UCASS set-up by directly measuring the flow velocity in the immediate vicinity of the particle detection region within the UCASS with the aid of a thermal flow sensor (TFS), such that the volume flow within the UCASS can be measured continuously and in real time.

Consequently, a modification of the UCASS instrument has been conducted, including an internal TFS within the instrument for a more accurate determination of the probed (analyzed) air volume. This study shows that the TFS, located in a UCASS extending housing, has negligible influence on the flow velocity in the detection region within the UCASS. Field tests (in the framework of “TPChange”, DFG TRR301) have demonstrated that the ascent rates derived from GPS and pressure rarely match the TFS-based ascent rates and deviate by up to 30 %. Laboratory experiments show that with an isoaxial flow (between 2 and 8 m/s) towards the UACSS, the flow velocity within the UCASS is generally increased by ~11.3 % compared to the external flow velocity. Only if the angle of attack of the UCASS is changed to values between 20°-30°, the flow velocities within the UCASS correspond approximately to the external flow. In contrast to GPS and pressure-based ascent rates, the TFS-measured volume flow within the UCASS allows for obtaining true volume flow rates despite flow distortions (caused by the UCASS housing) and in particular the deflection of the UCASS body from an isoaxial orientation. In this way, the UCASS extension including the TFS represents an improvement of the UCASS measurements in the sense of more accurate recordings of volume flows and, thus, particle concentrations up to 7.5 km altitude.

How to cite: Jost, S., Weigel, R., Kandler, K., Valero, L., Girdwood, J., Stopford, C., Stanley, W., Eichhorn, L. K., von Glahn, C., and Tost, H.: Improving the accuracy of particle concentration measurements of an optical particle counter (UCASS) for balloon soundings, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9677, https://doi.org/10.5194/egusphere-egu25-9677, 2025.

EGU25-9787 | Posters on site | AS5.8

Using uncrewed aerial systems for investigating the vertical aerosol particle distribution close to German airports 

Lutz Bretschneider, Anna Voß, Barbara Harm-Altstädter, Konrad Bärfuss, Ralf Käthner, Falk Pätzold, Andreas Schlerf, Malte Schuchard, Markus Hermann, Ulf Winkler, and Astrid Lampert

Ultrafine aerosol particles (UFP, particles < 100 nm diameter) can contribute to respiratory and cardiovascular diseases. Aircraft engines have been found to emit significant amounts of UFP. The vertical and horizontal distribution of these particles in the vicinity of airports depends mainly on the wind speed, the local wind direction and the stability of the atmospheric boundary layer (ABL). To investigate the vertical distribution of UFP emissions depending on these parameters, TU Braunschweig conducted measurement flights with the uncrewed aerial system (UAS) ALADINA near the Berlin Brandenburg Airport (BER) in October 2021 during the ULTRAFLEB project and near the Frankfurt Airport (FRA) in October 2024 as part of the SOURCE FFR project.
During the two field campaigns, 140 and 110 vertical profiles were conducted at BER and FRA, respectively, at varying periods during the day. The results indicate that UFP concentrations are higher compared to the background conditions downwind of the airport plume. This behaviour can also be seen in the preliminary data analysis of the FRA campaign. During stable conditions of the ABL, the measured UFP remain within the inversion layer, as vertical mixing is suppressed. This is also the case for the relatively larger particles with a size diameter between 300 and 500 nm, which were mainly emitted from car traffic close to the site.
The UAS measurements performed downwind of FRA provide a profound understanding of the vertical distribution of UFP and the interaction with meteorological conditions will allow to relate this results to the in parallel performed particle dispersion and wake vortex modeling.

Acknowledgement:
This research is part of the project ULTRAFLEB (DE: Ultrafeinstaubbelastung durch Flughäfen in Berlin; EN: UFP caused by airports in Berlin) and is funded by the German Environment Agency (Umweltbundesamt) under grant RE FOPLAN FKZ 3720 52 201 0 and the work was carried out as part of the UFP exposure study SOURCE FFR (Study On Ultrafine Particles in the Frankfurt Airport Region) commissioned by the Umwelt und Nachbarschaftshaus (UNH).

How to cite: Bretschneider, L., Voß, A., Harm-Altstädter, B., Bärfuss, K., Käthner, R., Pätzold, F., Schlerf, A., Schuchard, M., Hermann, M., Winkler, U., and Lampert, A.: Using uncrewed aerial systems for investigating the vertical aerosol particle distribution close to German airports, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9787, https://doi.org/10.5194/egusphere-egu25-9787, 2025.

EGU25-11744 | ECS | Posters on site | AS5.8

Enhancing High Resolution Atmospheric Profiling Using UAS: Deployment and Validation of the PARASITE Sensor Package 

Yann Büchau, Martin Schön, Kjell zum Berge, Samantha Gallatin, Jens Bange, and Andreas Platis

Uncrewed Aircraft Systems (UAS) are an invaluable tool for atmospheric profiling due to their mobility and capability to operate in the lower atmosphere and boundary layer. These regions represent an observational gap between ground-based stations and remote sensing instruments and satellites, which tend to be less accurate at lower altitudes. To fill this gap, while prioritising usability, versatility and safety, we have developed a custom meteorological sensor suite integrated into commercially available UAS, specifically multicopters.

The custom sensor package, called the Portable Aircraft Rucksack for Atmospheric Sensing and In-situ Turbulence Estimation (PARASITE), integrates data from the aircraft's positioning system and external meteorological sensors, including fast measurement of temperature, relative humidity and barometric pressure. We demonstrated the capabilities of this sensor package in flight on a DJI Mavic 3 multicopter with dimensions of 350 mm × 290 mm and a total take-off weight of 1 kg.

The three-dimensional wind vector is calculated using an improved method that combines a physical model based on meteorological and aircraft data - such as attitude, rotor frequencies, ground speed and air density - with machine learning techniques. The accuracy of the system was validated during the VITAL field campaign against ground-based in situ and remote sensing instruments, including Doppler wind lidars, differential absorption lidar, a 120 m meteorological tower and radiosondes.

The VITAL campaign was organised by the Hans-Ertel Centre for Weather Research of the German Weather Service (DWD) at Forschungszentrum Jülich, Germany in August 2024 and was also part of the World Meteorological Organisation's (WMO) global UAS Demonstration Campaign. During the campaign, PARASITE collected more than 100 vertical profiles, which were automatically transmitted wirelessly to a central data server after landing.

The system demonstrated compliance with WMO requirements by delivering processed data products in BUFR (Binary Universal Form for the Representation of Meteorological Data) format within minutes of each flight. The PARASITE system's rapid data processing and reliable performance highlight its potential to advance atmospheric profiling and support global meteorological initiatives.

 

How to cite: Büchau, Y., Schön, M., zum Berge, K., Gallatin, S., Bange, J., and Platis, A.: Enhancing High Resolution Atmospheric Profiling Using UAS: Deployment and Validation of the PARASITE Sensor Package, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11744, https://doi.org/10.5194/egusphere-egu25-11744, 2025.

EGU25-11881 | ECS | Posters on site | AS5.8

Combined measurement of Saharan dust, meteorological variables and space charge with the uncrewed aircraft system MASC-3 over Cyprus 

Martin Schön, Vasilieos Savvakis, Matteo Bramati, Andreas Platis, and Jens Bange

Mineral dust, especially Saharan dust, has a significant impact on atmospheric processes by influencing radiative forcing and cloud formation. To improve the representation of dust events in numerical weather prediction models, high-resolution in-situ measurements are required. In this study, the MASC-3 unmanned aircraft system (UAS) was used to perform simultaneous vertical profiling of meteorological variables, turbulence, aerosol particles and space charge during an intense dust event over Cyprus in April 2022. The UAS, equipped with an optical particle counter payload (OPC-Pod), provided high-resolution measurements of aerosol number concentration, with observed peaks of 45 counts/ml at 2500 m above sea level (a.s.l.), consistent with concurrent remote sensing observations, satellite imagery and back-trajectory simulations, as well as measurements from other UAS. The space charge distribution within the dust layer showed distinct patterns at the upper and lower boundaries, consistent with theoretical expectations. This study demonstrates the capability of MASC-3 for simultaneous meteorological, aerosol and charge measurements at altitudes up to 5500 m, providing valuable data for improving dust transport models. The results highlight the value of in-situ observations with UAS in characterising the vertical structure and electrical properties of dust layers, contributing to a more accurate understanding of dust-atmosphere interactions.The measurements were part of a project supported by the European Commission under the Horizon 2020 - Research and Innovation Framework Programme, H2020-INFRADEV-2019-2, Grant Agreement number: 871115.

How to cite: Schön, M., Savvakis, V., Bramati, M., Platis, A., and Bange, J.: Combined measurement of Saharan dust, meteorological variables and space charge with the uncrewed aircraft system MASC-3 over Cyprus, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11881, https://doi.org/10.5194/egusphere-egu25-11881, 2025.

In support of obtaining accurate, high-resolution meteorological and climatological observations, over remote regions, uncrewed stratospheric platforms are a potential breakthrough in capability in support of improving weather forecasting of extreme weather events. They offer cost effective and unique observations using micro-dropsondes. They can profile the entire atmospheric column from the lower stratosphere to sea-level with high vertical resolution data.

Voltitude Ltd., uses long endurance micro-high-altitude balloons (mHAB) and is developing fixed-wing solar electric stratospheric drones, also known as High Altitude Pseudo Satellites (HAPS), for delivering and dispensing micro-dropsondes over remote regions. The new micro-dropsonde has been compared with profiles from market leading radiosondes and other dropsonde systems and offers high quality data products featuring extremely high vertical resolution. The presentation “Dropsondes from the Stratosphere” will review the global weather observation challenges, priority use cases, and how new stratospheric technological innovations are impacting this field and will discuss the emerging capabilities offered by low-cost long endurance stratospheric platforms.

Results from resent weather observation data gathering field trials using the StratoSonde® mHAB system will be presented. This is a lightweight (<3kg) self-navigating, long endurance stratospheric balloon incorporating a dispenser containing up to ten, 20g, micro-dropsondes. This mHAB is capable of accurate altitude control and can target specific wind layers to drift in desired directions towards data sparse regions of interest, with its payload of micro-dropsondes. Once dispensed the dropsondes take approximately 20-minutes to descend to sea-level, measuring Temperature, Pressure, Relative Humidity, Wind speed and Wind Direction in high vertical resolution all the way from stratosphere to sea-level. Data is transmitted to the dispensing balloon, which disseminates this in near-real-time via SATCOM. Presentation of results will include 2023 and 2024 field campaigns across the tropical Atlantic, operating out of the Cabo Verde islands, off the west coast of Africa. This valuable in-situ data is permitting new research relating to potential intensity and the role of the outflow layer in the rarely observed upper troposphere, in structural evolution and intensification of tropical cyclones.  More recently, mHAB have been deployed from Iceland to navigate to arctic regions, gathering polar observations from the 2024-2025 season, and supporting research into high latitude, short lived and intense polar low phenomena.

The presentation will conclude with results from new research into reducing the vulnerability of fixed-wing solar electric drones a.k.a. High-Altitude Pseudo Satellites (HAPS), to gusts and turbulence. The new “Gust Alleviation” technique has successfully expanded the operating envelope of HAPS for launch, recovery and flight through the troposphere to and from the relative safety of the stratosphere. This is a key enabling technology and permits HAPS to take-off and land more frequently, to enable new applications including micro-dropsonde delivery from the stratosphere, where it is critical to be able to land and restock the dropsonde payload every couple of weeks. This disruptive new capability is highly complementary to wide area, high density services currently offered by lighter-than-air mHAB and provides a higher value targeted observation of specific meteorological features of interest.

How to cite: Stevens, P.: Dropsondes from the Stratosphere: Targeted Observations Over Remote Regions Using Uncrewed Stratospheric Platforms., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13017, https://doi.org/10.5194/egusphere-egu25-13017, 2025.

EGU25-13819 | ECS | Orals | AS5.8

Max PlanckWinDarts: High-resolution measurements in the planteray boundarylayer with a tethered balloon 

Venecia Chávez-Medina, Hossein Khodamoradi, Eberhard Bodenschatz, and Gholamhossein Bagheri

Uncrewed Aircraft Systems (UAS) and tethered balloon systems (TBS) are transforming atmospheric research by enabling high-resolution, multi-instrument observations. To address long-standing gaps in planetary boundary layer (PBL) observations, particularly in the mixed layer and entrainment zone, we employed the Max Planck CloudKite, a tethered kite-balloon hybrid system, equipped with the latest generation of WinDarts. These versatile instruments provide continuous multi-parameter measurements of PBL dynamics for up to 20 hours. Each WinDart measures three-dimensional wind velocity, temperature, relative humidity, pressure, particle concentration (0.3–40 μm), carbon dioxide, and volatile organic compounds, offering unparalleled insights into PBL processes.

During the Pallas Cloud Experiment (September 2022) and the IMPACT campaign ("In-situ Measurement of Particles, Atmosphere, Cloud and Turbulence," May–June 2024) in Pallas, Finland, we deployed successive generations of WinDarts, achieving a cumulative flight time of nearly 370 hours. These campaigns yielded high-resolution datasets capturing turbulent fluxes of heat and momentum and interactions between the PBL and the free atmosphere.

This contribution presents findings from the IMPACT campaign, focusing on velocity-temperature interactions and their role in turbulence and vertical transport. The results demonstrate the value of TBS-based platforms in complementing UAS systems for atmospheric research and advancing our understanding of PBL processes.

To the left, the image shows two kite-balloons deployed with three WinDarts during a flight as part of the IMPACT field campaign. To the right, we show a lateral visualization of a WinDart highlighting its different components.

How to cite: Chávez-Medina, V., Khodamoradi, H., Bodenschatz, E., and Bagheri, G.: Max PlanckWinDarts: High-resolution measurements in the planteray boundarylayer with a tethered balloon, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13819, https://doi.org/10.5194/egusphere-egu25-13819, 2025.

EGU25-14053 | Posters on site | AS5.8

Tethered Helikite Observatories 

Eberhard Bodenschatz and Gholamhossein Bagheri

 It is impossible to build measurement towers that are several kilometers high. Traditionally, aircraft have been used for atmospheric measurements. Due to their high true air speed, time-resolved measurements from manned aircraft are very challenging. This is especially true for measurements in clouds. Dropsondes and sounding balloons are regularly used to measure atmospheric profiles. However, it is not possible to measure the transport properties of moisture, temperature and aerosols. Unmanned aerial vehicles and drones can be used to measure atmospheric properties. However, due to either the high true air speed or the downwash from the propeller system, measurements of 3D wind speed are quite limited. In addition, the payload of these systems is modest. It is impossible to measure for many hours or days.  It would therefore be desirable to have a system that can serve the same purpose as a tower, but can reach heights of several kilometers. 

In this talk I will present the Max Planck Cloud Kite Observatory. It is a tethered helikite system operated from a winch on the ground or from a research vessel. The tether holding the helikite is made of very low weight, high or low density pre-stretched polyethylene. The helikite is both a helium balloon and a kite. By this it is not pushed towards the ground at high windspeeds nor does it fall to the ground when the wind stops. By mounting two 250m^3 helikites on top of each other, we achieved a safe lift of 150kg on the tether. Remotely operated instruments can be easily mounted anywhere on the tether.  The system is certified for wind speeds up to 25m/s. Due to its stationary location it has shown to supplement measurements with UAVs perfectly.   In addition multiple tethered helikite observatories can be employed in close vicinity to each other. In other words, the Max Planck Cloud Kite is a mobile observatory platform with the same utility as a multi kilometer high tower.

 I will present the system: winch, helikite, mounting strategies, the helium recovery system and the instruments we have developed to measure eddy covariances, aerosols, and cloud particle dynamics by holographic particle image velocimetry. I will give an outlook on how such a system can be used to highly resolve stratocumulus clouds and other situations. 

 

How to cite: Bodenschatz, E. and Bagheri, G.: Tethered Helikite Observatories, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14053, https://doi.org/10.5194/egusphere-egu25-14053, 2025.

EGU25-15058 | Orals | AS5.8

Improving weather forecasts through an operational network of Meteomatics Meteodrones 

Fabiola Ramelli, Lukas Hammerschmidt, Brad Guay, Melanie Kobras, Julie Thérèse Villinger, Johannes Rausch, Lukas Umek, and Martin Fengler

Weather significantly impacts a wide range of industries and influences many aspects of our daily lives. However, weather models often lack sufficient and reliable observations in the atmospheric boundary layer, which limits their accuracy, particularly in forecasting local weather phenomena over complex terrain. To fill this observational gap, Meteomatics has developed the Meteodrone-Meteobase-system.

Meteodrones are hexacopters equipped with meteorological sensors that collect high-resolution vertical profiles of temperature, humidity, wind speed and wind direction up to 6000 meters AMSL. The Meteobase acts as a base station, enabling the automatic launch and landing of the Meteodrones. Since 2020, Meteomatics has been operating a growing network of 3-10 Meteobase stations across Switzerland that is remotely controlled by a pilot. The data collected by the Meteodrones is automatically integrated into our high-resolution weather model EURO1k (1 km2 resolution), to close the observational gap and improve weather forecasts. Building on the success and experience gained from the Swiss network, Meteomatics will install and deploy a network of 30 Meteobase stations across Norway between 2024 and 2027.

Here we assess the quality of the Meteodrone measurements against the World Meteorological Organization's (WMO) observation requirements for high-resolution numerical weather prediction. Furthermore, we evaluate the impact of the Meteodrone data on forecasting local weather phenomena, such as stratus clouds, by comparing observations to model simulations with and without assimilated drone data. These findings showcase the operational capabilities of automatic Meteodrones for meteorological profiling and its contribution to improving numerical weather forecasts.

How to cite: Ramelli, F., Hammerschmidt, L., Guay, B., Kobras, M., Villinger, J. T., Rausch, J., Umek, L., and Fengler, M.: Improving weather forecasts through an operational network of Meteomatics Meteodrones, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15058, https://doi.org/10.5194/egusphere-egu25-15058, 2025.

EGU25-17032 | ECS | Orals | AS5.8

Real-time identification of flow structures in the atmospheric boundary layer using UAV-borne measurements and neural networks 

Louis Alsteens, Matthieu Duponcheel, and Philippe Chatelain

The accurate identification and classification of wind structures in the atmospheric boundary layer (ABL) are promising to address the challenges of surface fluxes estimations and improving our understanding of the atmosphere dynamics. Traditionally, the Eddy-Covariance method is used to estimate those fluxes but it struggles to achieve the energy balance closure in specific atmospheric conditions such as day-time convective conditions. Those inaccuracies are possibly due to the presence of localized wind structures such as updrafts or other coherent structures in the vicinity of the measurement tower.

The present study was performed on numerical simulation databases to develop the methodology and will be applied to field data in the upcoming future.

First, an innovative framework that combines real-time data acquisition using unmanned aerial vehicle (UAVs) and signal reconstruction via Fourier mode decomposition is going to be presented. The UAV is flying on a predefined path to gather measurements that are then used to reconstruct the velocity field based on a limited number of Fourier modes. The solenoidal constraint is applied to the velocity field to get more accurate results. The determination of the Fourier modes is handled as a minimization problem while the limited number of modes ensures a good computational efficiency while trying to preserve the key features of the flow. The time-history of the measurements is considered up to a certain sample age but the location of the samples from the past is advected in a Lagrangian fashion according to the reconstructed field. This reconstruction process is performed in near real-time which is critical for practical applications.

Second, we will focus on the identification of the flow structures. It is handled by a neural network trained on an extensive data sets of more than 100 million samples taken from Large Eddy Simulations (LES) of convective boundary layer with various atmospheric conditions (mean Temperature going from 15 to 25°, geostrophic wind speed ranging from 0 to 4m/s...). This neural network has demonstrated good performance reaching an accuracy of 84% in structure identification according to the classification of Park et al. [1], even for ABL conditions unseen during the training process. These results showcase the robustness of the neural network and its ability to adapt to varying convective scenarios and its ability to identify various structures such as updrafts, downdraft and other coherent structures.

Finally, the two approaches are combined. Within a LES flow flied, a virtual UAV takes measurements on a predefined path, reconstructs the velocity field based on the Fourier modes approach and identifies the structures. The results of the identification problem are then compared to the actual features in the LES in order to evaluate the accuracy and effectiveness of the combined method.

[1] Park, S., P. Gentine, K. Schneider, and M. Farge, 2016: Coherent Structures in the Boundary and Cloud Layers: Role of Updrafts, Subsiding Shells, and Environmental Subsidence. J. Atmos. Sci.73, 1789–1814, https://doi.org/10.1175/JAS-D-15-0240.1.

How to cite: Alsteens, L., Duponcheel, M., and Chatelain, P.: Real-time identification of flow structures in the atmospheric boundary layer using UAV-borne measurements and neural networks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17032, https://doi.org/10.5194/egusphere-egu25-17032, 2025.

EGU25-17544 | ECS | Orals | AS5.8

Hovering a Microscope on a Drone: Development of UAV Based Systems for High-resolution Imaging of Falling Snow 

Koen Muller, Mario Camenzind, Ilja Shesterikov, Simone Morandi, and Filippo Coletti

From single crystal formation high in the atmosphere down to precipitating snowfalls at ground level no snowflake takes the same path through the air column. During descent snow-crystals grow, coalesce, break, and rime into graupel while interacting with the surrounding air. Among the well-studied effects of temperature and humidity super-saturation, the specific role of the various turbulence activities throughout the atmosphere remains elusive. This work uses uncrewed aerial vehicles (UAVs) as a flexible platform to study snowfall up to 120 meters above ground level during their most ‘turbulent end-of-lifetime’ as they descend through the atmospheric surface layer. The work is twofold. Firstly, a smaller commercially available DJI Mavic3E quadcopter equipped with an onboard telelens and CZZI GL10 searchlight is used to gather aerial photography of snowfall 3 meters away from the drone. Automated flight paths executed in an hourly deployment scan the air column and harvest 13407 snowflakes from 3351 images taken during nighttime experiments. Building on previous ground-imaging studies, we extract snowflake metrics for size, aspect ratio, complexity, and orientation angle at a 160μm-per-pixel image resolution. Our data suggests that snowflakes of high aspect ratio tend to glide in horizontal orientation while interacting with the turbulent atmosphere. Mapping our data over various height positions we find an overall 30% percent variability in snowflake growth, while variation in shape is found less prominent. Secondly, we present developments on an airborne microscopy system to shed further light on the intricate details of the snowflakes concerning their freefall behavior. Equipping a larger DJI Matrice600Pro hexacopter capable of carrying a 6kg payload with an Infinity K2-Distamax long-range microscope telescopic lens we increase the image resolution by a factor of ten and reach 16μm-per-pixel. We will present the various subsystems involved in imaging snowflakes outside the drone's flow envelope, including synchronizing a pulsed LED circuit to compensate for the large image distance and low numeric aperture. We will present the first snowflakes captured in freefall during the start of the 2024 snow season to demonstrate the feasibility of our airborne microscopy system in hovering flight.

How to cite: Muller, K., Camenzind, M., Shesterikov, I., Morandi, S., and Coletti, F.: Hovering a Microscope on a Drone: Development of UAV Based Systems for High-resolution Imaging of Falling Snow, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17544, https://doi.org/10.5194/egusphere-egu25-17544, 2025.

EGU25-19551 | Posters on site | AS5.8

A multi-gas sensor system lifted by a tethered aerostat for real time in-situ investigation of volcanic plumes 

Salvo Marcuccio, Stefano Corradini, Riccardo Biondi, Francesco Ciancitto, Alessandro Filippeschi, Gaetano Giudice, Matteo Gemignani, Lorenzo Guerrieri, Linda Lambertucci, Irene Marsili, Luca Merucci, Camilo Naranjo, Simona Scollo, and Dario Stelitano

Volcanic eruptions eject a large amount of aerosols and gases in the atmosphere with severe implications on the environment, climate and life on Earth and, in recent times, human society and aviation. Currently, the main technique for observing volcanic clouds relies on remote sensors both from satellites and ground observatories, also using multispectral cameras. However, the composition of volcanic clouds is difficult to assess due to physical limitations of the instruments’ detection capability: satellite and ground based remote sensing systems, generally used to detect and retrieve plume particles and gases, are limited by instrument sensitivity, spatial resolution and uncertainties of particles optical properties and size distribution. Moreover, the presence of high concentration of some gases in the atmosphere (e.g. CO2) makes their estimation impossible inside the volcanic cloud. Therefore, in-situ measurements are necessary to collect ground truth data to validate the remote sensing models and obtain an accurate characterization of a volcanic cloud.

Drone-mounted sensors could compromise the measurements within the plume due to the disturbances caused by the propellers. Additionally, the drone could be contaminated and damaged by the ash. As a less invasive and less expensive alternative, our groups at the Space Systems Laboratory of the University of Pisa together with INGV developed a novel method for in-situ measurements in volcanic clouds: a custom multi-gas sensor package (“Volcanosonde”) lifted by a tethered aerostat inside the plume. A volcanosonde is composed of a set of sensors, integrated on a circuit board, which record the concentrations of the main constituents of a volcanic plume (SO2, HCl, CO2, PM1 – 10) together with the atmospheric parameters (pressure, relative humidity and temperature). In the volcanosonde, data packets are acquired with a frequency of 1 Hz and stored onto an onboard memory, while a timewise subsampled subset of the data is transmitted to a ground station for real-time visualization via LoRa protocol over the 868 MHz ISM band.

We tested the developed apparatus during a measurement campaign in August 2024 on Mt. Etna, Sicily, in the frame of “VOLANDO”, a PRIN project funded by the European Union- Next Generation EU. The system consisted of a sounding balloon including three volcanosondes attached at 50 m intervals on the retaining rope, a stand-alone Optical Particle Counter and a GNSS receiver. The helium-inflated aerostat was raised to 400 m a.g.l. allowing the sondes to enter the plume and make uninterrupted measurements for 3 hours. The experiment was repeated on different days, effectively collecting in-situ data.

The system showed excellent flight behavior and was relatively easy to handle, even in no flat volcanic terrain, allowing for quick re-location of the flying balloon and the attached sondes over several areas of interest. Real time monitoring of the measurements provided the operators with indication of the quality of data collected and guided the right positioning of the flying platform so to achieve an optimal positioning of the volcanosondes within the plume. We estimate that a crew of two with minimal trraining can operate the tethered balloon autonomously under good weather conditions.

How to cite: Marcuccio, S., Corradini, S., Biondi, R., Ciancitto, F., Filippeschi, A., Giudice, G., Gemignani, M., Guerrieri, L., Lambertucci, L., Marsili, I., Merucci, L., Naranjo, C., Scollo, S., and Stelitano, D.: A multi-gas sensor system lifted by a tethered aerostat for real time in-situ investigation of volcanic plumes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19551, https://doi.org/10.5194/egusphere-egu25-19551, 2025.

EGU25-19785 | Posters on site | AS5.8

Greenhouse gas emissions from wastewater treatment plants using drone-based measurements 

Magnus Gålfalk and David Bastviken

Using a drone-based method for simultaneous flux measurements of greenhouse gases (GHGs) we assessed methane (CH4) and nitrous oxide (N2O) at several wastewater treatment plants (WWTPs) with anaerobic digestion.  Results showed unexpectedly high fluxes and discovered that N2O emissions from sludge storage are at least as important as CH4 emissions in terms of global warming. Despite this, N2O emissions from anaerobic digestion sludge are usually assumed to be negligible and therefore not measured routinely at WWTPs. The CO2-equivalent total emissions of CH4 and N2O were 3-fold higher than the IPCC-recommended emission-factor-based estimates. The drone-method works in a wide variety of environments for simultaneous measurements of the major GHG fluxes (CH4, N2O, and CO2) without the need to do repeated flight patterns to cover all gases, alleviating the problem of flux potentially changing between flights which would otherwise make flux comparisons between the different GHGs less reliable.

The drone method used is a further developed version of our previous method (Gålfalk et al 2021 - https://pubs.acs.org/doi/10.1021/acsearthspacechem.1c00106) with longer flight time, higher payload, all major GHGs measured simultaneously, improved logging with all measurements needed for flux calculations being measured on-board the drone without any need for ground-based auxiliary measurements, and more convenient post-processing to calculate fluxes.

How to cite: Gålfalk, M. and Bastviken, D.: Greenhouse gas emissions from wastewater treatment plants using drone-based measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19785, https://doi.org/10.5194/egusphere-egu25-19785, 2025.

EGU25-20658 | Orals | AS5.8

UAV-based measurement of natural gas seeps using a newly developed ultra-lightweight high-sensitivity methane sensor in the western Canadian Arctic 

Jalal Norooz Oliaee, Meghan Beattie, Roger MacLeod, Chase Sun, Joel Corbin, and Peter Morse

Airborne eddy-covariance measurements over the outer Mackenzie River delta in the western Canadian Arctic have linked significant methane (CH4) emissions to geological sources from subsurface reservoirs. However, few natural gas seeps have ever been mapped. Efforts by airborne imaging spectroscopy to locate these methane ‘hotspots’ primarily attributed higher emissions to biogenic CH4 from wetlands as a function of the water table. Resolving the discrepancies between these findings requires identifying seeps within areas of high background emissions. Conducting ground-based measurement surveys to achieve this is challenging in wetlands due to the impedance of widespread bodies of water and the risk of releasing CH4 when disturbing the soil during on-foot surveys.

To aid in identifying methane seeps that have not been mapped before, we present an ultra-lightweight in-situ methane sensor, and its deployment on a common commercially available Uncrewed Aerial Vehicle (UAV) – a DJI Matrice 300 RTK. This system was tested in a location in the Mackenzie River delta where CH4 is known to seep to the surface through conduits in thin, thawing permafrost overlying underground hydrocarbon reservoirs. The easily transportable UAV permits non-invasive, near-surface flight capabilities with highly flexible flight plans, while the sensor’s lightweight and power-efficient design permits high sensitivity for detecting and quantifying subtle variations in atmospheric CH4 concentrations, even in remote and challenging environments.

Our miniaturized, mid-infrared tunable diode laser absorption spectroscopy CH4 sensor targets CH4’s strongest rotational-vibrational transition at the 3270 nm wavelength. Employing the wavelength modulation technique and a small open-path gas absorption cell, the sensor is able to resolve atmospheric CH4 concentrations as low as 10 ppb (parts per billion) with a near-instantaneous response time (100 Hz sample rate) making it suitable for deployment on fast moving aerial platforms. The entire standalone instrument package weighs 1.2 kg and is ideal for integration on consumer UAVs which have limited payload capacities.

We flew the UAV in horizontal grid patterns typically used in source detection and localization scenarios, as well as vertical “curtain” patterns to sample cross sections of the CH4 plume arising from a known gas seep to quantify the flux rate. Preliminary data analysis using a Gaussian plume inversion technique yields a CH4 emission flux estimate near 8 kg hr-1, which is comparable to fugitive emissions from some oil and gas production facilities in Canada. Our results emphasize the significance of this approach to reliably, effectively, and precisely quantify CH4 emission from natural sources, as it will enable us to identify sources of CH4 hotspots and test our hypothesis that the magnitude and frequency of these emissions will increase throughout the study region as the climate warms.

How to cite: Norooz Oliaee, J., Beattie, M., MacLeod, R., Sun, C., Corbin, J., and Morse, P.: UAV-based measurement of natural gas seeps using a newly developed ultra-lightweight high-sensitivity methane sensor in the western Canadian Arctic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20658, https://doi.org/10.5194/egusphere-egu25-20658, 2025.

EGU25-20826 | Orals | AS5.8 | Highlight

Preliminary results of World Meteorological Organization Uncrewed Aircraft Systems Demonstration Campaign (WMO UAS DC) 

Debbie OSullivan, James Pinto, and Nicolas Rivaben

The WMO Uncrewed Aircraft Systems Demonstration Campaign (UAS-DC) was organised to measure the ability of a range of UAS to meet the requirements for operational upper air observations and to assess their ability to fill observational gaps in WIGOS GBON and/or RBON. Data were collected over a 7-month period from March to September 2024 and 3 Special Observing Periods were performed: during US March 2024 Eclipse, Paris Olympics and during 2024 ISARRA Flight Week Campaign in September, using WMO NetCDF data format standard, which were automatically converted to the BUFR format. These two standardised formats facilitated the widespread use of UAS weather observations by researchers and NWP modelling centres around the world. In addition to deploying a distributed trial network of UAS to test the concept, the campaign used the WMO Information System (Version 2.0, WIS 2.0) to provide real-time data to participating subscribers during the campaign. These highly flexible, accurate and environmentally friendly weather sensing UAS provide a new innovative observing system for National Meteorological and Hydrological Services (NMHSs) to fill observational gaps and subsequently improve numerical weather prediction capabilities. The UAS-DC provided insight into the potential use of crowd-sourced data from observations of opportunity collected by the delivering UAS. We present in this work an overview of the campaign, including a discussion of the methods, and the potential impact that UAS observations collected at regional scales may have, as indicated by initial studies conducted by NWP centres.

How to cite: OSullivan, D., Pinto, J., and Rivaben, N.: Preliminary results of World Meteorological Organization Uncrewed Aircraft Systems Demonstration Campaign (WMO UAS DC), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20826, https://doi.org/10.5194/egusphere-egu25-20826, 2025.

Air pollution is the second cause of death from non-communicable diseases. In Guanajuato, Mexico, the brick industry is the main means of life and source of polluting emissions, with health impacts (short stature, neurological deterioration, cardiorespiratory diseases and asthma). This sector has initiated regulatory changes but now there is no monitoring and its impact on health. As a first pilot phase, the objective was to measure the main air pollutants in a rural community in Guanajuato, Mexico, using a low-cost ATMOTUBE® monitor and describe the area and population group at greatest risk of exposure.  Analytical and longitudinal design from September 2023 to February 2024, with the ATMOTUBE® measurement parameters, VOC, PM1, PM2.5, PM10, temperature, humidity and pressure. During the six months of measurement, the results were VOC 4.15±11.79 ppm, AQS 65.17±30.11, PM1 4.90±18.43 ug/m3. From January to February 2024 was the period of highest concentration of pollutants with a maximum concentration of PM2.5 of 664±12.5μg/m3, PM10 of 650±14.8μg/m3 and low humidity value (34.1 ± 5.2) where they are near two schools. The first inventory of the main air pollutants in a rural community is presented, with children and women being the population at greatest risk. With this data from this pilot phase, it is recommended to begin with surveillance measures as well as health and nutrition indicators.

How to cite: Monroy-Torres, R.: Pilot Study About Inventory of Air Pollutants in a Rural Community of Guanajuato, Mexico using a Low-Cost ATMOTUBE® Monitor, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-127, https://doi.org/10.5194/egusphere-egu25-127, 2025.

Investigating the Awareness of Risks of Exposure to Atmospheric Aerosol and the Potentials of Low-Cost Air Quality Sensors at Quarry Site in Ebonyi State-Nigeria

1Ibeh, Gabriel Friday, 2Lawrence Ibeh, 3Vwavware, O.J., 4Akande-Roland, P.I., 5Edebeatu C. C, and 6Njoku E. I

Corresponding Author: gabriel.ibeh@gmail.com

Abstract

The study is aimed at investigating the awareness of risks associated with the exposure to atmospheric aerosol at quarry site and its health implication in Ebonyi state, and to examines how low-cost air quality sensors can enhance monitoring and management efforts. The questionnaire used covers the demographic information, awareness of occupational health hazards, use of personal protective equipment, health effects experienced by workers, and suggestions for improvement. A total of three hundred and fifty (350) questionnaire were distributed to respondents. a sample of one hundred and eighty-five (185) for quarry workers, quarry owners/managers, community members living near quarry sites, sixty-five (65) healthcare providers, fifty-five (55) environmental protection agencies and forty-five (45) policymakers was selected through random sampling.  the data collected was statistically analyzed using frequency counts and mean. a total of three hundred and forty-seven (348) were returned, two (2) were torn and five (5) were wrongly filed. a total of three hundred and forty-three (343) were accepted and assembled for analysis. The findings on the awareness of occupational health hazards among quarry workers indicate a concerning lack of knowledge and training in this field. The findings from assessing the use of personal protective equipment (PPE) among workers indicate varying levels of compliance with safety measures. The findings from investigating the health effects of workers' exposure to aerosols at a quarry site reveal significant impacts on their well-being. The findings from the investigation aimed at identifying suggestions for improving a conducive work environment at the quarry indicate enhancement of health care. The responses from questionnaire provide valuable insights into the current state of occupational health and safety at quarry sites in Ebonyi State and help identify areas for improvement.  The research reviewed that lack of low-cost air quality sensors for monitoring of aerosol from quarry station is hindering the awareness of risk of exposure. Low-cost air quality sensors offer a practical solution for monitoring these risks, enabling real-time data collection that informs both operational practices and community engagement efforts.  The integration of low-cost air quality sensors into the environmental management framework at quarry sites in Ebonyi State can significantly enhance the understanding and control of air pollution. By providing real-time data and fostering community involvement, these sensors can play a pivotal role in mitigating the adverse effects of quarrying on air quality and public health. Therefore, collaborative approaches to help in having access to low-cost air quality sensors in Nigeria, research grants and sponsorship for training are the panacea for clean air quarry sites of Ebonyi State. 

 

How to cite: Ibeh, Dr. G. F.: Investigating the Awareness of Risks of Exposure to Atmospheric Aerosol and the Potentials of Low-Cost Air Quality Sensors at Quarry Site in Ebonyi State-Nigeria, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-279, https://doi.org/10.5194/egusphere-egu25-279, 2025.

EGU25-298 | ECS | Orals | AS5.9

Ammonia miniaturized sensors: Are they ready to be used in outdoor environments? 

Pablo Espina-Martin, Sarah Leeson, Robert Nicoll, Karen Yeung, Neil Mullinger, Nathalie Redon, Graham Spelman, Hilary Costello, and Christine F. Braban

NH3 is the major alkaline gas in the atmosphere and the third most abundant N-containing species, after N2 and N2O. It is an important target pollutant due to its role in N deposition processes impacting over ecosystems, and it is also a precursor of fine particulate matter (PM), known to cause several impacts on human health. Being able to detect and quantify NH3 is essential for determining the best mitigation policies to reduce these impacts, yet this is challenging given the high spatial and temporal variabilities of this pollutant.

Miniaturized sensors in theory combine the high time resolution with the flexibility in size and cost, however they have associated challenges including high or undefined LODs, variable response times, unspecified cross–interferences with other pollutants and degradation with usage time. The NH3 sensor market is less developed than some pollutants for ambient air applications, with most suppliers offering indoor applications at ppm level concentrations, while ambient NH3 concentrations are in the ppb range.

The results of a campaign comparing five NH3 sensors (four electrochemical and one chemiresistive) against a Picarro G2103 are reported. The campaign was carried out over 1 month at the Whim Bog, Scotland, which releases NH3 if specific wind speed and direction conditions are fulfilled simulating a small chicken farm. Local ambient concentrations are ~1-2 ppb. The commercial suppliers do not provide practical guidelines on how to properly use, maintain and clean the data for these sensors however the sensors were set-up accordingly to their technical capabilities, either sampling from a weatherproof enclosure or directly outdoor air. NH3 concentrations were <10 ppb up to 3 ppm from the Picarro data. The sensors had variable responses, with only two correlating with the NH3 release and the Picarro data (R2= 0.59 and 0.70). However, they underestimated the concentration levels (slopes = 0.26 and 0.6) and response times are still not satisfactory.

The study shows that only two out of five sensors were fit for measuring NH3 in the ambient air. Nonetheless, these two sensors data are to be used only as qualitative information and would need significant improvement before use in situations which require quantitative data. Specific technical challenges need to be addressed, including sensor orientation, housing, and the airflow inside of and quantification of the concentration range.

How to cite: Espina-Martin, P., Leeson, S., Nicoll, R., Yeung, K., Mullinger, N., Redon, N., Spelman, G., Costello, H., and Braban, C. F.: Ammonia miniaturized sensors: Are they ready to be used in outdoor environments?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-298, https://doi.org/10.5194/egusphere-egu25-298, 2025.

A CALM:ER approach to air quality education: low-cost sensors as a tool to increase awareness and invite behavioural change.

The Clean Air Living Matters – Exploring Reading collaborative programme aims to drive behavioural change and deliver air quality education to local schools and communities in Reading Borough Council UK.

The programme provides day-to-day solutions to pupils, parents and the wider community to improve air quality and reduce exposure to polluted air. The CALM:ER team utilise various approaches to engage with pupils, including exploring air quality using handheld low-cost devices. Low-cost sensors have also been used to map pollution in and around schools, all of which supports parts of the curriculum and encourages the development of various STEM skills, critical thinking and data analysis.

How to cite: O'Brien, M. and the CALM:ER Project team: A CALM:ER approach to air quality education: use of low-cost sensors to increase awareness and invite behavioural change., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-542, https://doi.org/10.5194/egusphere-egu25-542, 2025.

Air pollution is a critical global challenge, impacting quality of life and public health of vulnerable communities in low- and middle-income countries (LMICs), due to absence of monitoring devices, weak policies and fragmented institutions for effective air quality (AQ) management. Carbon monoxide (CO), nitrogen dioxide (NO2) and ammonia (NH3), are among the gaseous pollutants found in urban cities with potential to cause respiratory illnesses or cardiovascular diseases. The metal oxide low cost sensors are among the emerging air pollutants measuring devices for indicative measurements in urban areas, because they provide fast cheap results and allow to attain good spatial coverage at a low cost even in areas with no reference monitors. The low cost of these sensors comes with low performances and low qualities of data recorded as compared to reference grade sensors and thus with requirements for frequent calibrations. Frequent calibration necessitates availability of computational resources with skills for data analysis and modeling. The low-cost sensor systems (LCS) are solution for LMICs in building local capacities for addressing these challenges but strong local and international collaboration to improve AQ management is required.

The study focuses on calibrations and performance evaluations of MICS 6814 based gaseous low cost sensors using datasets collected in laboratory and field settings. The calibration is based on testing the performances of model equation for transforming sensor responses into air pollutants measurements in laboratory and field deployments. The results of linear calibration procedures in laboratory showed the transformation of sensor responses into air pollutant concentration to be significantly good with coefficient of determination R2 ranging from 0.55 – 1, for all gaseous pollutants. The performance evaluation results for sensor deployments in field across the city showed varying results depending on site categories and time of day such that the coefficient of determination R2 for CO, ranged from 0.82 – 1; for NH3, R2 ranging from 0.23 - 0.98, and for NO2 , R2 ranged from 0.52 – 0.9. Variations of coefficient of determination R2 during sensor calibrations in field, poses challenges in developing network wide calibration models for real time air pollutants monitoring. Further challenge, comes from the fact that the trends for individual field observations datasets, showed varying picking levels of pollutions during morning and evening rush hours for all categories of sensor location. Over all, the observed indicative measure of air pollutants across the city were sufficient for public awareness and policy making purposes. 

How to cite: manyele, A. and Mkiramweni, M.: Calibrations and Performance Evaluations of Metal Oxide Low- Cost Air Sensor for NH3, CO and NO2 Detections: Case study for Laboratory and Field Calibration of across Dar es Salaam City, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-778, https://doi.org/10.5194/egusphere-egu25-778, 2025.

EGU25-788 | ECS | Orals | AS5.9

Statistical Modelling of low cost PM2.5 sensor data in Dar es Salaam City  

Triphonia Jacob Ngailo

The rapid urbanization and industrialization in many parts of the world have made air pollution a global public health problem. Exposure to air pollutants has both acute and chronic impacts on health. In low and middle income countries like Tanzania have experienced accelerated population growth and urbanization in which air quality is generally poor and there is a lack of long-term reliable air quality monitoring.

Among the major air pollutants, particulate matter 2.5 (PM2.5) is the most harmful, and its long-term exposure can impair lung functions. Low-cost sensors (LCS) are becoming increasingly popular for measuring the level of particulate matter (PM) in the air. However, issues with reliability require calibrations before the sensors can be used in regulatory settings. The aim of this paper was to develop a statistical model for determining the accuracy of low-cost sensor network data. Considering PM2.5 adverse health impacts, especially on people’s respiratory systems. We therefore, developed a low-cost PM2.5 sensor calibration model for measuring PM2.5 concentrations using maximum likelihood method. Moreover, we used the model to predict the PM2.5 with its driving forces that is temperature and humidity, and estimated its parameters. The PM2.5 data used for the developed model were collected from LCS network of five stations from Dar es Salaam City including Kigamboni, Vingunguti primary, Jangwani, Ubungo, and Buza recorded from April 2022 to May 2023. The data was fitted to a regression model using Maximum-Likelihood (MLR). Descriptive and trend analysis was also performed using Mann-Kendall Trend analysis to describe the pollutant characteristics and identify significant trends in the selected stations in Dar es Salaam. The model performed well with high accuracy and performance with root mean of 3.58 and mean squared errors of 12.846, a coefficient of determination of 0.967, and mean absolute errors of 2.8.The results for MLR showed a high value of coefficient determination (R2=0.82) and low error measure.

Our results will aid in improving the accuracy of low-cost sensors for measuring PM2.5 concentrations, thereby providing cost-effective solutions for enhancing people’s health and well-being in Tanzania.

How to cite: Jacob Ngailo, T.: Statistical Modelling of low cost PM2.5 sensor data in Dar es Salaam City , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-788, https://doi.org/10.5194/egusphere-egu25-788, 2025.

EGU25-829 | ECS | Posters on site | AS5.9

Improving PM2.5 Exposure Modeling by Hyperlocal Monitoring Using Low-Cost Sensors in the Kolkata Metropolitan Area 

Kirtika Sharma, Sagnik Dey, Rijurekha Sen, and Sachin Chauhan

Personal exposure to PM2.5 poses a significant health risk, necessitating assessments at very high spatial and temporal resolutions. However, existing monitoring techniques, like Continuous Ambient Air Quality Monitoring Systems (CAAQMS), provide highly accurate data but are expensive and limited by their sparse distribution. Low-cost sensors (LCS) offer dense spatial data but often encounter reliability challenges and need extensive calibration. These limitations prevent the precise tracking of PM2.5 exposure at the personal level. To overcome these challenges, we have developed a hybrid framework integrating calibrated LCS data with CAAQMS observations. This approach aims to generate a unified, high-resolution spatiotemporal PM2.5 database, bridging existing gaps and significantly improving exposure assessments at the personal scale.

This study developed a high spatial (1 km × 1 km) and temporal (1 h) scale PM2.5 estimates by integrating calibrated static low-cost sensor (LCS) data with hourly ground-based PM2.5 measurements from CAAQMS across Kolkata, India, for the winter season (1st December 2023–31st January 2024). To harmonize these datasets and create a spatiotemporal database of PM2.5 estimates, we utilized hourly PM2.5 data from seven CAAQMS stations and calibrated data from 22 static LCS stations. The LCS calibration incorporated meteorological data, precisely temperature (T) and relative humidity (RH), sourced from the nearest CAAQMS stations. 

We employed a Random Forest machine learning model, an ensemble algorithm that effectively captures complex non-linear relationships in the data and improves accuracy by combining multiple decision trees. Our model achieved an approximately 24% reduction in RMSE and an R² of 0.90, validated using an 80:20 train-test split, ensuring robust evaluation of its accuracy. This reduction demonstrates the efficacy of the integrated approach for high-resolution air quality mapping. On 4th December 2023, PM2.5 exposure estimates for a common grid point (88.34°E, 22.54°N) were derived using two approaches: one with only CAAQMS data and another with a hybrid of CAAQMS and LCS data. Without LCS, the exposure range at this grid point was 51.34 µg/m³, with an average exposure of 89.40 µg/m³. By integrating LCS data with CAAQMS, the exposure range was reduced to 30.02 µg/m³, and the average exposure increased to 103.39 µg/m³. This increase suggested that LCS might have captured more localized variations, contributing to the higher average exposure value. The reduction in the exposure range indicated a more consistent exposure pattern, highlighting the importance of integrating sparse, accurate CAAQMS data with spatially dense LCS data. This integration enhanced the spatial variability of PM2.5 and provided a more accurate estimate for personal exposure assessments.

How to cite: Sharma, K., Dey, S., Sen, R., and Chauhan, S.: Improving PM2.5 Exposure Modeling by Hyperlocal Monitoring Using Low-Cost Sensors in the Kolkata Metropolitan Area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-829, https://doi.org/10.5194/egusphere-egu25-829, 2025.

EGU25-881 | ECS | Orals | AS5.9

A Multipollutant Low-Cost Sensor Network in Bengaluru, India: Long-Term Performance Evaluation and High-Resolution Mapping of Particulate and Gaseous Pollutants 

Emil Varghese, Nirav Lekinwala, Kavyashree N Kalkura, Nidhi Malik, Vinod Shekar, Srinivas Sridharan, Yashwant Pratap S.Y., Swagata Dey, and Subramanian Ramachandran

Hybrid air quality monitoring integrating reference-grade instruments, low-cost sensors (LCS) and satellite data is revolutionising the air quality monitoring standards globally. The current study is from Bengaluru, a metropolitan city in southern India, where a multipollutant (particulate and gaseous) sensor network comprising 60 LCS (5-25 nodes each from five different Indian integrators) has been deployed across the city. Before deployment, these sensor nodes were initially collocated with reference-grade instruments at the India Sensor Evaluation and Training (Indi-SET) centre in Bengaluru. Correction models for PM2.5, PM10, NO2, and O3 were developed using regression and machine learning methods to improve sensor data reliability. The sensors used include electrochemical sensors (Alphasense (A4 or B4 series) or EC Sense TB600 series) for the gases and optical sensors (Plantower (PMS7003 or PMS5003), Tera Sense New Gen OEM, Sensirion SPS30 and/or Alphasense (OPC-R2 or OPC-N3)) for particulate matter (PM). One node from each integrator was collocated for a year to assess the long-term performance of these multipollutant sensors. During this period, an Aerodyne Time-of-Flight Aerosol Chemical Speciation Monitor (ToF-ACSM) is operated to evaluate the real-time performance of PM sensors with varying aerosol chemical composition. The localised correction of sensors reduced errors to 10-40 %, achieving a correlation with reference instruments greater than 0.7 and ensuring uniform performance across different integrators. Initial analysis of the deployed sensors indicated that PM2.5 levels exhibit significant monthly temporal variation but minimal spatial variation. In contrast, NO2 showed both spatial and diurnal variations across different nodes, with peaks in the morning and evening traffic rush hours. Additionally, spatial maps of various particulate and gaseous pollutants are being developed using the Land-Use Regression (LUR) model to estimate population exposure. The presentation will cover the long-term performance of multipollutant sensors, the performance of PM sensors with varying aerosol chemical compositions, the most effective long-term correction model, and the high-resolution mapping of pollutants using low-cost sensors and reference-grade instruments.

How to cite: Varghese, E., Lekinwala, N., N Kalkura, K., Malik, N., Shekar, V., Sridharan, S., Pratap S.Y., Y., Dey, S., and Ramachandran, S.: A Multipollutant Low-Cost Sensor Network in Bengaluru, India: Long-Term Performance Evaluation and High-Resolution Mapping of Particulate and Gaseous Pollutants, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-881, https://doi.org/10.5194/egusphere-egu25-881, 2025.

EGU25-1084 | ECS | Orals | AS5.9

Challenges and opportunities in using low-cost sensors for PM2.5 monitoring in urban transport microenvironments: a study case in Barranquilla Metropolitan Region, Colombia 

Sandra Maldonado, María José Nieto-Combariza, Julián Arellana, Julio Dávila, Daniel Oviedo, Santiago Torreglosa, Alexander Parody, and Dayana Agudelo-Castañeda

Air pollution constitutes a significant environmental justice challenge, particularly affecting vulnerable communities in low- and middle-income countries (LMICs). Urban mobility plays a substantial role in personal exposure to pollutants, notably PM2.5, exacerbating health disparities among transport users. Effective monitoring of these exposures is essential for understanding and addressing these inequities; however, traditional air quality measurement infrastructures are often inadequate in LMIC contexts. The growing availability of low-cost sensors (LCS) presents a promising avenue for bridging data gaps in urban air quality monitoring. Nonetheless, the reliability and applicability of these sensors in dynamic urban transport environments require thorough evaluation. This study, executed as part of an interdisciplinary collaboration among experts in urban policy, air quality, and transport studies, investigates the deployment of an LCS for PM2.5 monitoring in Soledad, Colombia. The research aims to assess the potential of LCS to capture exposure disparities among various modes of transport while addressing associated technical and logistical challenges. The primary focus is to evaluate the feasibility of utilizing LCS to measure personal exposure to PM2.5 in urban transport microenvironments, emphasizing calibration accuracy, adaptability to local conditions, and the potential to inform equitable transport policies. The AirBeam3 sensor was employed across motorized three-wheelers, buses, and private cars during predetermined urban routes. A rigorous 15-day calibration process against a reference-grade station was conducted to ensure data accuracy, achieving a correlation coefficient of R² = 0.87. Data collection strategies were tailored to account for transport-specific dynamics, including variations in ventilation, proximity to emission sources, and traffic conditions. The study encountered several challenges, including adaptation to high humidity, protection of equipment in high-risk environments, and correction of measurement biases. Notably, the sensor identified significant PM2.5 exposure disparities among transport modes, with motorized three-wheeler users exhibiting the highest exposure levels. Adjusted data indicated that environmental conditions, traffic density, and vehicle type emerged as critical determinants of exposure. Despite certain limitations, the LCS provided robust, high-resolution exposure data, demonstrating its suitability for capturing real-world variability in LMIC contexts. This research underscores the challenges and opportunities presented by the deployment of LCS for air quality monitoring in resource-constrained urban settings. While technical hurdles, such as calibration and environmental sensitivity, persist, the affordability and accessibility of LCS render them invaluable tools for addressing environmental justice issues. The findings emphasize the potential of LCS to enhance local air quality initiatives, inform sustainable transport policies, and promote equitable health outcomes through data-driven interventions.

Keywords: low-cost sensors, air quality, PM2.5, urban mobility, personal exposure, environmental justice, LMICs.

How to cite: Maldonado, S., Nieto-Combariza, M. J., Arellana, J., Dávila, J., Oviedo, D., Torreglosa, S., Parody, A., and Agudelo-Castañeda, D.: Challenges and opportunities in using low-cost sensors for PM2.5 monitoring in urban transport microenvironments: a study case in Barranquilla Metropolitan Region, Colombia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1084, https://doi.org/10.5194/egusphere-egu25-1084, 2025.

EGU25-1095 | ECS | Posters on site | AS5.9

Leveraging Open Data and Land Use Regression Models for Scalable Air Quality Monitoring: Integrating Low-Cost Sensors for Global Applicability 

Gabriel Oduori, Chiara Cocco, Payam Sajadi, and Francesco Pilla

The growing availability of open geospatial data presents significant opportunities to address spatial and temporal gaps in air quality (AQ) monitoring. This is particularly crucial in resource-limited and underserved regions. In this study, we introduce a novel framework that combines low-cost sensor (LCS) measurements with Land Use Regression (LUR) models, utilising publicly accessible datasets to improve the spatial and temporal resolution of AQ estimates. By integrating empirical sensor data with open, openly available model predictors, the framework enhances the accuracy of air quality predictions, particularly in areas with limited high-density monitoring infrastructure.

The open LUR model uses freely available data, such as traffic density, land cover, population distribution, and meteorological information, from OpenStreet Map and OpenWeatherMap, to predict local pollutant concentrations. These predictions are dynamically calibrated with real-time LCS measurements through machine learning regression techniques, which adjust for sensor biases, reduce noise, and quantify uncertainties. This integration allows for a more accurate, real-time representation of air pollution levels, especially in urban areas where traditional monitoring is often inadequate or nonexistent.

To demonstrate our framework's capability in refining Nitrogen Dioxide (NO₂) and Particulate Matter (PM₂.₅) estimates, we conduct a study in a dense population area in Nairobi, Kenya. Our result achieves a significant improvement in alignment with regulatory-grade measurements. By relying on open data and open-source LUR models, this approach is scalable, adaptable, and transferable, making it a cost-effective solution for AQ monitoring in diverse geographic and socio-economic settings.

This work emphasises the transformative potential of open data and open LUR models in democratising access to high-resolution, real-time air quality monitoring tools. By combining low-cost sensors with these open-source data and models, the framework offers actionable insights for urban planning, public health initiatives, and environmental policy. It underscores the broad applicability of this solution in addressing global air pollution challenges, providing scalable tools for effective air quality management and policy-making across various regions.

 

Keywords:

Low-cost sensors (LCS), open data, open Land Use Regression (LUR) models, air quality monitoring, Nitrogen Dioxide (NO₂), Particulate Matter (PM₂.₅), urban planning, public health, environmental policy, data fusion, scalability, global applicability, open-source models.

 

 

How to cite: Oduori, G., Cocco, C., Sajadi, P., and Pilla, F.: Leveraging Open Data and Land Use Regression Models for Scalable Air Quality Monitoring: Integrating Low-Cost Sensors for Global Applicability, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1095, https://doi.org/10.5194/egusphere-egu25-1095, 2025.

EGU25-1232 | ECS | Posters on site | AS5.9 | Highlight

Establishing a Nationwide Ambient Air Quality Monitoring Network: The Clean Air Initiative and PM2.5 Monitoring in The Gambia 

Julius David, Dawda Badgie, Mariatou Dumbuya, Awa Sabally Touray, Isatou Touray, Saikou Camara, Buba Manjang, and Sunkaru Touray

Background: Air pollution is a major global health risk, causing seven million deaths each year. In The Gambia, the use of firewood and charcoal for household energy, along with harmattan dust, significantly increases exposure to harmful particulate matter (PM2.5). Women and children are particularly vulnerable to these health risks.

To address the air quality data gaps in The Gambia, we launched the Clean Air Initiative in 2023. Our goal was to set up a nationwide ambient air quality monitoring network using low-cost sensors. Led by the Permian Health Lung Institute (PHLI) and the National Environment Agency (NEA) in collaboration with various stakeholders, the initiative aimed to systematically tackle air pollution challenges.

Methodology: We began with stakeholder mapping to identify the multifaceted challenges of air pollution. Key participants included government ministries of health and environment, private construction companies, and academic institutions. The process involved installing air quality sensors, conducting education workshops, and integrating scientific data with actionable plans.

Results: Over 12 months, we deployed 17 low-cost air quality sensors (IQAir AVO) across all seven regions of The Gambia. This network helped identify air quality trends and assess their health impacts. Challenges such as sensor security and cellular network reliability were addressed through community engagement and solar panel installations. Our focus on the densely populated Greater Banjul Area enabled crucial observations and set the stage for nationwide expansion.

Data from our initial four sensors showed a 12-month average PM2.5 concentration of 36.9 µg/m³ (95% Confidence Interval: 31.9 - 42.0 µg/m³), which is seven times higher than the World Health Organization (WHO) guideline of 5 µg/m³. Seasonal variations were significant, with dry season levels (November to May) averaging 44.9 µg/m³ (95% CI: 39.7 - 50.2 µg/m³), compared to 25.8 µg/m³ (95% CI: 18.6 - 32.9 µg/m³) during the rainy season.

Discussion: A key outcome of the initiative was The Gambia's first Air Quality State Report, bolstered by continuous PM2.5 monitoring and capacity building at the National Environment Agency through international partnerships. Funding from the University of Chicago Energy Policy Institute was crucial for our success. Collaborations with regional entities like Makerere University are improving data accessibility across Africa. Despite these advances, challenges such as connectivity issues with remote sensors and environmental impacts on equipment remain, especially during seasonal transitions.

Conclusion: The Clean Air Initiative marks a significant leap in managing air quality in The Gambia. By establishing a comprehensive monitoring network and creating foundational policies, we are paving the way for improved public health and governance. Continued collaboration and overcoming operational hurdles are essential for sustained progress. Future plans for expansion and regional data integration offer promising pathways for effective air quality management in the region.

Keywords: Air pollution, PM2.5, The Gambia

How to cite: David, J., Badgie, D., Dumbuya, M., Sabally Touray, A., Touray, I., Camara, S., Manjang, B., and Touray, S.: Establishing a Nationwide Ambient Air Quality Monitoring Network: The Clean Air Initiative and PM2.5 Monitoring in The Gambia, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1232, https://doi.org/10.5194/egusphere-egu25-1232, 2025.

Overview

The Operational Network of Air Quality Impact Resources (OPENAIR) project set out to address a common issue for local governments concerned about poor air quality in their communities.

Local governments and community organisations are becoming aware of the availability of  affordable air quality sensors and are keen to use them to support evidence based policy and interventions.  To date however they have lacked the skills and capability to design, procure and operate air quality monitoring systems.

OPENAIR set out to address this through four goals, all of which have been achieved:

  • Develop air quality sensing best practise guidance materials. Over 50 resources have been published covering topics including business case development,  sensing system design and implementation, data interpretation and stakeholder engagement. These are freely available for all to use.
  • Have participating local governments use affordable air quality sensors to address local community air quality issues. With expert support they each led and undertook projects focused on bushfire smoke, wood fire heater smoke, transportation pollution, coal dust, heat and building community STEM and technology literacy.   
  • Develop an online collaboration hub (openair.org.au) to host best practise resources and foster ongoing collaboration.
  • Develop a “harmonised” data feed that ingests air quality measurements from a range of commercially available sensing devices and makes that data available via a single, open API or use by researchers, policy makers and the general public

The project was led by the New South Wales Smart Sensing Network (NSSN) - a research innovation network sponsored by the NSW Office of the Chief Scientist and Engineer.  It involved experts from the NSW Department of Climate Change, Energy and the Environment and Water (DCCEEW), nine local governments, five universities and three small businesses.

Impact

This initiative has enabled more evidence based policy making in local government.  It has led to ongoing collaboration between local governments, university and government researchers.   The harmonised data feed has provided air quality and climate researchers with a great deal more data than they previous had access to.  It has raised awareness of low cost environmental sensing more generally.

OPENAIR has been recognised for its innovation and impact by winning a number of national and state awards in Australia related to air quality, sustainability, environment outcomes and research innovation.  See https://www.nssn.org.au/awards for more details.

A project overview is available at https://www.nssn.org.au/openairproject.

Future

The project team published a discussion paper describing 35 specific recommendations in four categories:

  • Promoting and supporting the use of smart, low-cost air quality sensing
  • Enhancing state government air quality information products and services
  • Enabling improved data sharing
  • Application to other environmental measurements

Several of these have commenced, including initiatives to:

  • include other types of environmental measurements relating to heat, water and wildfires (soil and fuel moisture, fire ignitions and monitoring).
  • explore international research and government collaboration focused on best practises, data sharing, data quality and international standards development.

 

How to cite: Runcie, P.: OPENAIR - Low Cost Air Quality Sensing Best Practises and Open Data Platform, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1550, https://doi.org/10.5194/egusphere-egu25-1550, 2025.

EGU25-3891 | Orals | AS5.9

Quantifying long-term exposures to fine particulate matter (PM2.5) using real-time, low-cost sensors to assess the impact of household air pollution on birthweight in two cohort studies in southern India  

Naveen Puttaswamy, Sreekanth Vackacherla, Santu Ghosh, Sudhakar Saidam, Saritha Sendhil, Divya Jayakumar, Sneha Patil, Ajay Pillarisetti, and Kalpana Balakrishnan

Personal exposure to fine particulate matter (i.e., PM2.5) istypically measured for 24 or 48 hours in health effects research. Real-time, low-cost sensors (LCS) offer long-term PM monitoring solutions with potentially high spatiotemporal resolution that can facilitate better exposure – response analysis. We assessed long-term exposures to PM2.5 among pregnant women in the Tamil Nadu Air Pollution and Health Effects-II (TAPHE-II) and Reproductive effects from Exposure to Airborne Chemicals in urban Homes (REACH) cohorts using such real-time LCS.

Battery-operated real-time PM sensors equipped with PMS7003™ (Plantower Inc., China) were used to monitor living-room PM2.5 levels for a period of 21-days and 7-months in the TAPHE-II (n=80) and REACH (n=15) cohort homes, respectively. Further, pregnant women wore a portable ultrasonic personal air sampler (UPAS™ v2.1) for 24 hours, equipped with a 37-mm PTFE filter, to measure PM mass concentration. The LCS recorded PM, temperature, and relative humidity at 1-minute time intervals and transmitted data in real-time to the cloud. Sensors were collocated with gravimetric samplers for a period of 24-h on three consecutive days in 25 homes to develop indoor-specific calibration equations. In addition, all sensors were collocated with a reference-grade beta attenuation monitor pre- and post-monitoring period; linear models were used to derive ambient calibration coefficients.

Continuous PM data was monitored on average 21 (SD 3) days; data availability ranged between 97 to 100% across rural and urban homes in the TAPHE-II cohort. Precision across all sensors was satisfactory, with a standard deviation of 2.6 µg/m3 and a coefficient of variation of 15.6%. The normalized root mean square error (NRMSE) for indoor and ambient collocation was 31.6% (r=0.86) and 43.2% (r=0.80), respectively. Correlation (NRMSE) between measured personal daily exposures and 21-day real-time PM2.5 measures was 0.62 (47.9%). Long-term averages (min–max) of indoor PM2.5 levels were high among biomass users (n=20, 49.8 µg/m3 (35.8 – 80.6)), followed by mixed-fuel (n=14, 28.7 µg/m3 (29.4 – 61.9)), and liquefied petroleum gas (LPG) (n=46, 25.7 µg/m3 (21.3 – 39.5)) users.

We demonstrate the applicability of LCS for long-term indoor PM monitoring to assess health risks associated with indoor air pollution. Indoor-specific calibrations capture the true range of PM exposures and temporal variability, minimizing uncertainty in exposure – response relationships in health effects research. To more accurately assess the exposure of urban pregnant women, we are using LCS to measure indoor PM throughout most of the gestational period (i.e., up to 7 months). This data will be used to evaluate the representativeness of the 24-hour and 21-day average PM2.5 levels as a proxy of gestational exposure.

How to cite: Puttaswamy, N., Vackacherla, S., Ghosh, S., Saidam, S., Sendhil, S., Jayakumar, D., Patil, S., Pillarisetti, A., and Balakrishnan, K.: Quantifying long-term exposures to fine particulate matter (PM2.5) using real-time, low-cost sensors to assess the impact of household air pollution on birthweight in two cohort studies in southern India , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3891, https://doi.org/10.5194/egusphere-egu25-3891, 2025.

EGU25-4367 | ECS | Posters on site | AS5.9

Challenges and Opportunities in Monitoring Indoor Air Quality with Low-Cost Sensors  

Juncheng Qian, Yuqing Dai, Bowen Liu, and Zongbo Shi

Low-cost air quality sensors offer promising, cost-effective solutions for monitoring indoor air quality (IAQ). However, their utility is often constrained by challenges in accuracy and data reliability, including those related to inadequate calibration. This is particularly important considering the large variabilities in indoor environmental conditions, in terms of temperature, humidity, and PM2.5 levels. To address this, we developed an experimental chamber using a container to calibrate two types of low-cost particulate matter (PM) sensors against a reference-grade instrument (Fidas 200) using machine learning methods. Sensors from two brands were tested in controlled conditions simulating common indoor pollutant sources such as cooking, smoking, and incense burning. Calibration revealed clear performance variability between sensor brands, with sensors underestimating or overestimating pollutant concentrations at different levels. Sensor correction using machine learning greatly improved sensor accuracy and data reliability. Calibrated sensors will be deployed to monitor PM concentrations (PM2.5 and PM10), temperature, relative humidity, and carbon dioxide (CO2) levels continuously over two years in retrofitted and control homes, capturing pre- and post-retrofit IAQ changes. Future recalibration is planned to evaluate long-term sensor drift. Our preliminary findings highlight the critical role of rigorous calibration in ensuring reliable IAQ monitoring using low-cost sensors. This study provides valuable insights into the practical applications and limitations of such sensors in retrofitted environments.

How to cite: Qian, J., Dai, Y., Liu, B., and Shi, Z.: Challenges and Opportunities in Monitoring Indoor Air Quality with Low-Cost Sensors , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4367, https://doi.org/10.5194/egusphere-egu25-4367, 2025.

Air quality monitoring networks in the Global South often face challenges due to data scarcity and limited resources, which can hinder effective air quality management. This study presents a methodology for optimizing the spatial distribution of air quality monitoring stations in urban areas of the Global South, aiming to improve data representativeness for population exposure and inform evidence-based policies.

Building upon existing monitoring network design literature (Kanaroglou et al., 2005; Gupta et al., 2018), our approach integrates high-resolution population data with a modified K-means clustering algorithm. We combine the center of gravity concept with standard K-means to determine monitor locations, prioritizing areas of high population density. The methodology incorporates a two-tier approach, categorizing areas into low and high population density zones and applying weighted K-means clustering separately to each category. To enhance applicability across diverse urban landscapes, we implement geospatial considerations in distance calculations, addressing limitations of standard Euclidean distance-based methods in geographic coordinate systems.

We applied this methodology to rapidly growing urban centers including Lahore (Pakistan), Lagos (Nigeria), and Dhaka (Bangladesh). Results suggest potential improvements in representing population exposure compared to current monitoring configurations.

Limitations of our approach include its reliance on population data, which may overlook other important air quality determinants. The current method also does not account for land use patterns, emission sources, or meteorology. However, the proposed methodology provides a foundation for further development of air quality monitoring network design, potentially enhancing urban air quality management by optimizing air quality monitor placement in data-sparse regions of the Global South.

How to cite: Omar, A. and Naveed, M.: Population-Centric Optimization of Air Quality Monitoring Networks in Data-Sparse Urban Regions: A Weighted K-Means Approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4723, https://doi.org/10.5194/egusphere-egu25-4723, 2025.

Low-cost sensor networks (LCSNs) have attracted widespread attention as valuable monitoring tools for environment science and air quality management, revolutionizing traditional air monitoring systems. However, previous studies concentrated on the urban pollution hotspots monitoring, leaving a gap in understanding the performance and application of LCSN for long-term regional monitoring in extreme environments.

This study presents a novel and challenging application of LCSN to investigate the causes and sources of ozone pollution in the unique and remote Tibetan Plateau, characterized by rapid temperature and humidity fluctuations and significant diurnal variations. Since 2023, a real-time and high-density LCSN with 40 sites has been gradually established in Tibet, covering 6 cities including Nagri and Lhasa. The sensors are designed to mitigate the influence of temperature and humidity from both hardware and algorithm adjustments. Calibration and side-by-side tests against reference-grade instruments are conducted to characterize the sensitivity and baseline of the sensors based on the variation in pollutant concentrations in the real-world atmosphere. The spatial-temporal characteristics, production and transport patterns of ozone were preliminarily interpreted in combination with meteorological data and the HYSPLIT model.

The results show that the optimized and calibrated low-cost sensors were consistent with standard equipment in long-term monitoring, indicating the accuracy and stability of sensors in the extreme plateau environment. LCSN can provide reliable real-time data with high temporal and spatial resolution to support the exploration of regional ozone and its precursor production and transport patterns. Tibet ozone pollution is dominated by regional contributions with favorable weather conditions, while locally generated pollution has little impact. Different cities and regions show variability in ozone pollution pattern. For instance, in Nagri, located near the western border, approximately 70% of ozone pollution is attributed to regional transport, which is affected by the cross-border transport accompanied by westerly winds; while Lhasa, with a larger population and more transportation and industrial activities, has an increased proportion of local contributions influenced by precursors. These findings reveal the robustness and applicability of LCSN in extreme environments, showcasing its potential to provide actionable insights into dynamic air pollution. This study highlights the opportunities and challenges of utilizing LCSN for air quality monitoring in remote regions and extreme environments, providing scalable solutions for global air quality management and sustainable development strategies.

How to cite: Chen, W.: Application of Low-cost Sensor Network in Extreme Environment: A Case Study of Ozone Pollution in Tibetan Plateau, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5007, https://doi.org/10.5194/egusphere-egu25-5007, 2025.

EGU25-5634 | ECS | Orals | AS5.9

FILTER: Framework for Improving Low-Cost Sensor Network Data for Air Quality Monitoring 

Amirhossein Hassani, Vasileios Salamalikis, Philipp Schneider, Kerstin Stebel, and Núria Castell

Over the last decade, low-cost sensors (LCSs) have improved air quality monitoring by enabling widespread, community-driven data collection, particularly in regions with limited resources. Although these LCSs have increased public engagement and enriched datasets for understanding pollution dynamics, challenges related to data quality, standardization, and interoperability have hindered their full integration into regulatory frameworks and large-scale environmental monitoring (Barkjohn et al., 2024; Carotenuto et al., 2023). The lack of consistent Quality Control (QC) processes and correction methodologies limits the reliability of LCS-derived data for applications such as public health assessments, modeling, and policymaking.
To address these issues, we introduce FILTER (Framework for Improving Low-cost Technology Effectiveness and Reliability), a scalable, multi-level QC, and correction framework designed to improve the reliability of PM2.5 data from citizen-operated LCS networks. FILTER employs spatial “correlation” and “similarity” QC tests, allowing for in-situ correction of LCS data in different environments. The FILTER framework’s effectiveness is validated using large-scale European data from the sensor.community and PurpleAir networks, two of Europe’s largest citizen-driven air quality networks, covering the period 2018 – 2023. The final dataset, including 521,115,762 hourly PM2.5 measurements from 37,085 locations, was categorized into “high quality,” “good quality,” and “other quality” groups. At the raw data stage, applying QC steps through the spatial similarity level results in a ~50.3% decrease in median RMSE (from 7.61 to 3.78 µg m⁻³) across 483 LCSs. For corrected data, applying the same QC steps reduces the median RMSE by ~49.5% (from 7.59 to 3.83 µg m⁻³) across 456 LCSs. These enhancements enable LCS data to be more effectively integrated into scientific research, regulatory datasets, and policy development.
FILTER demonstrates several key advantages: independence from sensor-specific designs, geospatial scalability, adaptability to real-time processing, and applicability to other pollutants with spatial patterns similar to PM2.5. However, its utility is constrained for pollutants like NO₂, which exhibit hyper-local variability, or scenarios requiring sub-hour temporal resolution. FILTER also demonstrates the potential of on-site calibration techniques that do not require co-location to generate accurate data from LCS networks. This is particularly important for developing large LCS networks that can contribute to both science and policy, especially in light of the new European Air Quality Directive. 

References
Barkjohn, K. K., Clements, A., Mocka, C., Barrette, C., Bittner, A., Champion, W., et al. (2024). Air Quality Sensor Experts Convene: Current Quality Assurance Considerations for Credible Data. ACS ES&T Air. 
Carotenuto, F., Bisignano, A., Brilli, L., Gualtieri, G., & Giovannini, L. (2023). Low‐cost air quality monitoring networks for long‐term field campaigns: A review. Meteorological Applications, 30(6), e2161. 

We acknowledge funding for CitiObs project from the European Union’s Horizon Europe research and innovation programme under grant agreement No.101086421. We also acknowledge the contributions of sensor.community (https://sensor.community/en/, accessed October 2024) and PurpleAir (https://www2.purpleair.com/, accessed October 2024) sensor networks where the original sensor data come from, as well as the citizens who provided the low-cost sensor data.

How to cite: Hassani, A., Salamalikis, V., Schneider, P., Stebel, K., and Castell, N.: FILTER: Framework for Improving Low-Cost Sensor Network Data for Air Quality Monitoring, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5634, https://doi.org/10.5194/egusphere-egu25-5634, 2025.

EGU25-5687 | Posters on site | AS5.9

Improving Zimbabwe’s capacity for air quality monitoring from the ground and by TROPOMI  

Marloes Penning de Vries, Martin de Graaf, Munyaradzi Davis Shekede, and Ntandokamlimu Nondo

Zimbabwe is one of the African countries severely affected by high air pollution levels with significant impacts on human health and the environment. To develop mitigation strategies and sustainable policies, monitoring of air quality (AQ) is essential. However, Zimbabwe has few air quality monitoring stations, and these are concentrated in the densely populated industrial area of Harare. This results in significant data gaps, limited assessment of air quality, ineffective health and environmental policies. We present the progress made within the “AQ4Zim” project, funded by ESA within the EOAFRICA framework, of which the objectives are: 1) expand the AQ monitoring network through installation of low-cost sensors; 2) explore the spatial and temporal variations in Aerosol Optical Thickness (AOT) patterns across Zimbabwe using TROPOMI on the Sentinel-5p platform; and 3) develop and evaluate a smoke-dust discriminator for TROPOMI. The satellite data will be compared with ground-based data from the low-cost sensors as they become available. Relating satellite measurements to the measurements at ground level, ensures that they can be used to routinely monitor air quality efficiently. The data will form a basis for the calculation of the UN Sustainable Development Goals (SDG) target indicators 11.6.2 and 3.9.1.

How to cite: Penning de Vries, M., de Graaf, M., Shekede, M. D., and Nondo, N.: Improving Zimbabwe’s capacity for air quality monitoring from the ground and by TROPOMI , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5687, https://doi.org/10.5194/egusphere-egu25-5687, 2025.

Low-cost air quality sensing holds the promise to transform how we address air pollution by providing more information and more science that can drive public interest, political will, and policy toward cleaner, healthier air. Crucially, through a combination of its price point and transportability, the technology also makes it feasible for more people to do this work in more places.

However, technology alone cannot fulfill this promise. Realizing its potential requires the low-cost sensing community of people who build sensors, measure data, generate analyses, and use insights from those analyses to actively and strategically work together toward shared goals.

This presentation will explore what could be possible in the coming decade for the low-cost sensing community to accomplish, in terms of influencing policy and public engagement — and ultimately, cleaner healthier air.

The presentation will also define three actionable opportunities for the low-cost sensing community to shape itself toward that greater impact:

  • Advocate for greater software, hardware, and data transparency policies, along with stronger consumer ownership rights from air quality sensing companies to better support the community — particularly those in low-resource settings
  • Collaborate on open-source quality assurance/quality control (QA/QC) technical and community frameworks that minimize inefficient duplication of effort and allow for adaptability across a range of sensor array sizes
  • Attract and allocate financial resources to expand accessibility and utility of low-cost sensing, especially in places with high air pollution levels yet low existing air quality management infrastructure and resources

How to cite: Hasenkopf, C.: How can the low-cost air quality sensor community maximize its positive impact? , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6193, https://doi.org/10.5194/egusphere-egu25-6193, 2025.

We reviewed 60 sensor networks and 17 related efforts (sensor review papers and data accessibility projects) to better understand the landscape of stationary low-cost gas-phase sensor networks deployed in outdoor environments worldwide. We found that particulate matter (PM) is more commonly studied globally than gas-phase compounds, and coverage gaps are most severe in the Global South and rural areas. Data quality and availability were also found to be barriers to access, with the highest quality data typically emanating from research institutions, which also tend to have the least straightforward data access for the public. In response, we aim to harmonize sensor networks by amalgamating measurements from a multitude of networks into one open access database hosted by NASA’s Atmospheric Science Data Center. As of early 2025, data from 12 unique US-based sensor networks have been collected for redistribution in the archive, and we are currently recruiting global network participants. Data from each network will be reformatted in a common data format with metadata embedded to streamline data processing. A key feature is a tier system in which we critically review each sensor network by their calibration efforts and subsequent data quality, providing data quality flags to help end users determine which sensor data best meets their target application. The accessible and inclusive open science platform will allow users to search based on calibration criteria in addition to location, date range, and pollutant of interest. The sensor database is aimed at scientific end users seeking ground-based validation data for satellites and models alike, but is also accessible to community scientists. Future iterations will include data from global sensor networks, and assimilation with satellite and ground-based remote sensing data.

How to cite: Okorn, K. and Iraci, L.: Development of an Open-Source Harmonized Low-Cost Sensor Data Archive to Maximize Scientific Return from Existing Networks, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7017, https://doi.org/10.5194/egusphere-egu25-7017, 2025.

EGU25-7223 | ECS | Orals | AS5.9

Validating low-cost indoor air quality monitors to improve exposure monitoring in nail salons 

Rachel Thompson, Samantha Fisher, A. Michael Ierardi, and Brian Pavilonis

In the US, approximately 200,000 nail salon workers face chronic exposure to airborne chemicals. Health effects among this sector have been well documented and public health laws aimed at exposure reduction have been implemented across the US. In this study, we evaluated the accuracy and feasibility of using commercially available low-cost sensors as tools for workers to monitor and reduce their daily exposures. We compared the performance and utility of six commercially available low-cost total volatile organic compound (TVOC) sensors (Awair Omni, Kaiterra Sensedge, UHoo Smart Air Monitor, Airthings View Plus, Atmotube, and Atmocube) to validated reference instruments. Sensors were collocated in at least 4 different salons for 7 consecutive days during an initial baseline measurement period. Salons then received an intervention on methods to reduce exposure by utilizing existing controls and another 7 days of exposure measurements were collected. TVOC measurements from low-cost sensors exhibited moderate to strong correlations (rs ~ 0.54 - 0.88) with readings from validated reference instruments. Accuracy of the low-cost sensors varied, especially at higher TVOC concentrations and after repeated days of use. Low-cost sensors on average underestimated TVOC concentrations at the highest quartile of exposure (Mean Absolute Error (MAE) Q4: 16.19 – 28.49 ppm) but performed more similarly to reference instruments at lower quartiles of exposure (MAE Q1: 0.69 –  2.53 ppm, Q2: 1.60 – 2.75 ppm, Q3: 5.55 – 6.85 ppm). Despite some limitations, these sensors can be valuable tools for exposure assessment, including monitoring nail salon workers' daily exposures and studying the health effects of chemical exposures in longitudinal epidemiologic studies among this group.

How to cite: Thompson, R., Fisher, S., Ierardi, A. M., and Pavilonis, B.: Validating low-cost indoor air quality monitors to improve exposure monitoring in nail salons, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7223, https://doi.org/10.5194/egusphere-egu25-7223, 2025.

EGU25-8701 | ECS | Posters on site | AS5.9

Democratizing Access to Accurate Air Quality Measurements with Open-Source Tools 

Anika Krause and Siriel Saladin

Resource-constrained regions often face the highest levels of air pollution yet lack the infrastructure to monitor and mitigate its impacts effectively. Reliable air quality (AQ) data is critical for understanding and addressing the adverse effects of air pollution. While low-cost monitors can reduce equipment and maintenance costs, ensuring the accuracy of the collected data presents challenges, often requiring more expertise and effort than conventional reference equipment.

This presentation introduces open-source tools designed to address these challenges, democratizing access to accurate AQ monitoring. Focusing on outdoor PM2.5 sensors, our work highlights three key innovations that enhance the reliability and accessibility of low-cost air quality monitoring systems.

Calibration Strategies Without a Reference Instrument
The accuracy of low-cost sensors can be significantly enhanced by calibrating them against a local reference instrument. However, many regions lack access to such equipment. To address this gap, AirGradient has developed multiple calibration methods, including:

  • In-house calibration using a Federal Equivalent Method during monitor assembly.
  • Calibration via background extraction from sensor networks (see Point 2).
  • Application of a generalized correction formula, which is the focus of this discussion:
    The U.S. Environmental Protection Agency has devised a comprehensive correction formula for Plantower PM2.5 sensors. This algorithm accounts for relative humidity effects and the sensors’ non-linear response at high concentrations. When applied to AirGradient sensors deployed in nine global locations, the formula delivered significant improvements in accuracy. Average R2 values increased from 0.899 (raw) to 0.923 (corrected), while the normalized root mean square error (nRMSE) was reduced from 86% to 34%. 

Sensor Networks for Enhanced Calibration and Maintenance
Beyond granular pollution mapping, AQ sensor networks offer advanced capabilities for calibration and maintenance. A network of 16 AirGradient monitors deployed in Pai, Thailand, was used to extract regional background PM2.5 concentrations. With no local reference instruments available, calibration data from Mae Hong Son (a city 50 km away) was leveraged to adjust sensor readings, demonstrating the potential for regional calibration strategies.

Automatic Detection of Sensor Failures
A robust AQ dataset requires the detection and removal of anomalous data. Using a combination of AirGradient-owned co-location datasets and user-contributed public data, we identified various artefacts, including outliers, missing data, extended periods of high-concentration readings, and physically implausible values. An automated data cleaning algorithm was developed to identify and flag these anomalies effectively. While the system reliably enhances data quality, challenges remain in distinguishing short-term real emission events from artefacts. The integration of duplicate PM sensors into individual monitors could help address this issue, providing further reliability.

By improving the accuracy, reliability, and usability of low-cost AQ sensors, these open-source tools empower a wide range of users —such as schools, environmental organizations, and local governments— to generate actionable AQ data. This democratization of air quality monitoring fosters local engagement and equips resource-constrained regions with the tools needed to combat air pollution effectively.

How to cite: Krause, A. and Saladin, S.: Democratizing Access to Accurate Air Quality Measurements with Open-Source Tools, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8701, https://doi.org/10.5194/egusphere-egu25-8701, 2025.

Air pollution poses a significant global health concern, particularly for children, who are especially vulnerable due to their developing bodies1. This research examines particulate matter (PM) levels and their sources at three schools in Port Harcourt, the largest and capital city of Rivers State in Nigeria. It is the fifth most populous city in Nigeria with air quality highly impacted by the oil and gas industry. Low-cost source apportionment techniques were employed that use the size distribution of PM to fingerprint air pollution sources2. The approach allows for a highly detailed understanding of the risks of exposure faced by both students and staff across rainy and dry seasons. By employing affordable sensors, PM1, PM2.5, and PM10 levels were measured, revealing frequent exceedances of WHO air quality standards. During school hours, indoor PM concentrations were found to surpass outdoor levels, influenced by internal sources and the penetration of outdoor pollutants. Seasonal differences were evident, with elevated PM levels during the dry season largely attributed to Harmattan desert dust, while anthropogenic emissions were the primary contributors during the rainy season. These findings highlight the pressing need for interventions to reduce PM exposure in schools and comparable urban environments affected by natural and anthropogenic pollution. This study offers practical recommendations to minimize exposure risks and enhance air quality in educational spaces globally.

 

1 Rose, O.G., D. Bousiotis, C. Rathbone and F.D. Pope (2024) Investigating Indoor Air Pollution Sources and Student’s Exposure Within School Classrooms: Using a Low-Cost Sensor and Source Apportionment Approach, Indoor Air, vol. 2024, Article ID 5544298, https://doi.org/10.1155/2024/5544298

2 Bousiotis, D., Allison, G., Beddows, D.C., Harrison, R.M. and Pope, F.D., 2023. Towards comprehensive air quality management using low-cost sensors for pollution source apportionment. npj Climate and Atmospheric Science6(1), p.122. https://doi.org/10.1038/s41612-023-00424-0

How to cite: Pope, F., Nwokorie, V., and Bousiotis, D.: Investigating the influence natural and anthropogenic air pollution sources upon school environments in a Global South metropolis using a low-cost source apportionment approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8927, https://doi.org/10.5194/egusphere-egu25-8927, 2025.

EGU25-9303 | ECS | Orals | AS5.9

Space-Time Air Quality Disparities in Sub-Saharan Africa: PM₂.₅, PM₁₀, and Black Carbon Trends in the Greater Accra Metropolitan Area 

James Nimo, Ibrahim-Anyass Yussif, Mathias A. Borketey, Emmanuel K-E Appoh, Benjamin Essien, Selina Amoah, Joanna Modupeh Hodasi, and Allison F. Hughes

Particulate matter (PM₂.₅ and PM₁₀) and black carbon (BC) significantly affect climate and public health, especially in rapidly urbanizing regions. This study examines the spatial and temporal variations of PM₂.₅, PM₁₀, and BC in the Greater Accra Metropolitan Area (GAMA), Ghana, from January to December 2021. Measurements were conducted at a busy, high-density residential site and a low-density residential background site using two federal equivalent monitors, alongside meteorological parameters (relative humidity, temperature, wind speed, and wind direction).

Annual mean concentrations of PM₂.₅, PM₁₀, and BC were significantly higher at the high-density site characterized by heavy traffic and residential congestion than at the predominantly residential background site. These discrepancies underscore the influence of distinct land-use patterns, local emissions, and site-specific activities on air quality. Seasonal differences were also evident, particularly during the Harmattan—a dry, dusty trade wind unique to sub-Saharan Africa that substantially degrades air quality. During this period, both sites experienced elevated pollutant levels, with consistently higher measurements at the urban site, highlighting the marked increase in PM₂.₅ and BC concentrations in busy urban areas.

Analysis of the PM₂.₅/PM₁₀ ratio showed lower values during the Harmattan, reflecting the predominance of coarse dust particles from natural sources, whereas higher ratios during the wet season indicated greater contributions from fine particles generated by anthropogenic activities such as traffic and industrial processes. Conditional Bivariate Polar Plot analysis further revealed that pollutant levels at the urban site were more strongly driven by wind speed, indicating substantial local emissions and particle resuspension due to heightened human activity. In contrast, concentrations at the background site remained relatively uniform, indicating minimal local emissions and a stronger influence of regional background levels.

Overall, this study illustrates the significant spatial and temporal variability of air pollution in GAMA, with important implications for public health and climate change. The elevated levels of PM₂.₅ and BC during the Harmattan period underscore the need for targeted air quality management strategies to mitigate health risks and environmental impacts in sub-Saharan Africa’s rapidly urbanizing environments

How to cite: Nimo, J., Yussif, I.-A., Borketey, M. A., Appoh, E. K.-E., Essien, B., Amoah, S., Modupeh Hodasi, J., and Hughes, A. F.: Space-Time Air Quality Disparities in Sub-Saharan Africa: PM₂.₅, PM₁₀, and Black Carbon Trends in the Greater Accra Metropolitan Area, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9303, https://doi.org/10.5194/egusphere-egu25-9303, 2025.

The advancement of low-cost sensors provides new opportunities in aerosol research. After calibrating the low-cost sensors in the laboratory and in the fields with research-grade instruments, the accuracy concern of the data quality is resolved. With these research-grade low-cost sensors, PM2.5 and PM1 in a time-resolution of minutes can be obtained. This presentation demonstrates the application of research-grade low-cost sensors in source evaluation for community and indoor PM sources, personal PM exposure assessment, and panel-type epidemiological studies which investigates the associations of peak PM exposure and heart rate variability (HRV). HRV is a marker of cardiac autonomic balance; the reduced HRV indicators were found to be associated with an increased risk of myocardial infarction.

 

Cases studies conducted in Asia will be presented. The sensor application on evaluating the contribution of community PM sources was conducted in the Central Taiwan in 2017. The sensor application on assessing indoor PM sources was conducted in the Taipei metropolitan area in the northern Taiwan in 2018. The PM exposure assessment and panel-type of epidemiological studies were conducted in the southern Taiwan and Indonesia in 2018 to 2020. Research-grade low-cost sensors, namely AS-LUNG-O, AS-LUNG-I, and AS-LUNG-P, were used for outdoor, indoor, and personal monitoring in these studies, respectively. The medical-certified RootiRx® sensors were used for HRV monitoring.

 

The results showed that incremental contribution from the stop-and-go traffic, market, temple, and fried chicken vendor to PM2.5 levels at 3–5m away were 4.38, 3.90, 2.72, and 1.80 μg/m3, respectively. Significant PM spatial variations observed further emphasized the importance of conducting community air quality assessment. For indoor sources, cooking occurred most frequently; cooking with and without solid fuel contributed to high PM2.5 increments of 76.5 and 183.8 μg/m3 (1 min), respectively. Incense burning had the highest mean PM2.5 indoor/outdoor (1.44 ± 1.44) ratios at home and on average the highest 5-min PM2.5 increments (15.0 μg/m3) to indoor levels, among all single sources. In exposure assessment and epidemiological studies, it was found that for a 10 μg/m3 increase in PM2.5, HRV indicators were reduced 1.3-4.0% in Taiwan subjects in summer and 1.8 -5.7% in Indonesia subjects in dry season. The low-cost sensors used and methodology demonstrated in this presentation can be applied in resource-limited countries to conduct PM and health research.

How to cite: Lung, S.-C. C., Liu, C.-H., Wen, T.-Y. J., Shui, C.-K., and Tsou, M.-C. M.: Evaluating contributions of community and indoor PM sources, assessing personal PM exposure, and conducting panel-type epidemiological studies in Asia with research-grade low-cost sensors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9426, https://doi.org/10.5194/egusphere-egu25-9426, 2025.

Exposure to impaired ambient air quality, including fine particulate matter (PM2.5), poses significant risks to human health. Monitoring air pollutants is essential for understanding pollution trends, assessing exposure risks, and informing mitigation strategies. However, traditional regulatory-grade air quality monitoring networks are often sparse and costly to operate, limiting their ability to provide data at high spatial resolution. Low-cost sensors offer an alternative by enabling the deployment of localized monitoring stations with broader coverage, but their accuracy can be compromised under variable environmental conditions. To address this, data fusion techniques can be used to integrate data from multiple sensors and improve air quality predictions. However, integrating multimodal data presents challenges, including incompatible measurement units, spatial and temporal resolutions, and inherent uncertainties.

Here, we propose a probabilistic spatiotemporal model based on the stochastic advection-diffusion (SAD) equation for data fusion in air quality monitoring. The SAD model offers computational efficiency and flexibility, allowing it to handle large datasets while accounting for prediction uncertainties in air quality data. This probabilistic approach is well-suited for air quality managers and policymakers, as it not only predicts air quality with high accuracy but also provides interpretable model parameters that offer insights into the underlying processes driving air pollution. The approach is then evaluated using PM2.5 data from the Coastal Bend Region of Texas, an area facing growing environmental concerns due to expanding industrial development. When the spatiotemporal model is integrated with data from both regulatory-grade stations and low-cost sensors, error is reduced by 40% compared to the nearest regulatory-grade monitor located 20 km away and 11% compared to the nearest low-cost sensor located 1 km away. The model captures 78% of observed data within a 75% confidence interval, demonstrating its ability to accurately represent uncertainty. This method provides a promising framework for integrating diverse air quality data sources, addressing uncertainties, and enhancing community-engaged pollution monitoring efforts.

How to cite: Hummel, M. and Choi, B.: Enhancing Low-Cost Sensor Networks through Multimodal Data Fusion: Application of a Probabilistic Spatiotemporal Air Quality Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10518, https://doi.org/10.5194/egusphere-egu25-10518, 2025.

EGU25-11078 | ECS | Orals | AS5.9

Assessing low-cost sensor performance at varying temporal resolution against reference instruments for the measurement of NO2 

Seán Schmitz, Alexandre Caseiro, and Erika von Schneidemesser

Air pollution continues to be a major global health concern, with nitrogen dioxide (NO2) significantly contributing to negative health impacts. Low-cost sensors (LCS) present promising opportunities for accessible, high-resolution air quality monitoring but are often questioned for their accuracy and reliability. This study assesses the performance of electrochemical LCS for NO2 measurements compared to high-precision reference instruments—cavity attenuated phase shift (CAPS) and chemiluminescence NO2 monitors—across eleven temporal resolutions (ranging from 10 seconds to 6 hours). Data were collected over six months at an urban-traffic air quality monitoring site in Berlin using three EarthSense Zephyr sensor systems equipped with electrochemical sensors. Statistical metrics, including R², relative error (%), and mean bias error (MBE), were used to evaluate sensor performance. The results indicate that LCS demonstrate strong agreement with reference instruments at coarse time resolutions (≥1-hour averages, R² > 0.8), but their accuracy declines considerably at higher resolutions (<1-minute, R² < 0.5). Performance improves when sensors are calibrated against CAPS monitors compared to chemiluminescence monitors. Factors such as chemistry and emissions play a significant role, with poorer performance during the day than at night, a discrepancy that is further amplified at finer temporal resolutions. CAPS-calibrated predictive models also excel in capturing short-term concentration peaks compared to those calibrated with chemiluminescence monitors. These findings highlight that while LCS are effective for coarse-resolution NO2 monitoring, their limitations in dynamic environments at high temporal resolutions pose challenges for use in exposure studies and mobile applications. The study recommends careful calibration, strategic experimental design, and a focus on lower time-resolution applications to enhance LCS deployment.

How to cite: Schmitz, S., Caseiro, A., and von Schneidemesser, E.: Assessing low-cost sensor performance at varying temporal resolution against reference instruments for the measurement of NO2, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11078, https://doi.org/10.5194/egusphere-egu25-11078, 2025.

EGU25-12322 | ECS | Orals | AS5.9

Characterization of low-cost sensors via simultaneous field measurements: a case study 

Lorenzo Gentile, Eleonora Aruffo, Alessandra Mascitelli, Piero Chiacchieretta, and Piero Di Carlo

The use of low-cost sensors is continuously increasing as more evidence appears of their benefits: from the wide range of applications to the ease of use and accessible costs. Still, they are extensively studied to rightfully understand their range of use and the right way to handle their data. The first part of this work focuses on one month of simultaneous measurements of temperature, relative humidity, pressure, CO, NO, NO2, O3, OX, VOCs, PM2.5 and PM10 by three different low-cost sensors and a Pollution PyxisGC BTEX. Dataset acquired by ARTA (Agenzia Regionale per la Tutela dell’Ambiente) and ITAF (Italian Air Force) have been used as reference for the comparison. Vaisala AQT530, while also being part of the characterized instruments, has been used as reference for those quantities that were not present in the mentioned dataset and a 2B Ozone Monitor has also been used for O3 characterization.

Aside from a discrepancy in temperature and RH for AirSensEUR, the meteorological quantities for all the sensors show high correlation values (R ∼ 0.9). NO, NO2 and VOCs have high correlation with the same compounds observed by ARTA instruments (R ≥ 0.8), except for Libelium Smart Environment PRO NO2 that has a lower value (R = 0.348). Pollution PyxisGC BTEX VOCs comparison shows low slope values (∼ 0.16 against 1 hoped). CO measurements have a high similarity between the three low-cost sensors, differently OX values show a generally lower similarity with the reference instruments (with R ∼ 0.8 for Vaisala while being R ∼ 0.5 for the others). Libelium Smart Environment PRO measurement of NO, NO2 and O3 are affected by an extremely high bias (with values ≥ 100), a peculiar result considering how the sensors mounted where all factory-new and already calibrated by the manufacturer. PM values have only been compared averaging over the entire day (due to the kind of reference data available), showing a general matching with ARTA measurements only for AirSensEUR, which, at the same time, has the highest standard deviation.

Moreover, the dataset has also been used as a case study to investigate the ability of these instruments to catch signals from different near sources: 1) the local regional airport, 2) heavily used highway and roads. Analysis during rush hours, weekdays vs weekends, during the Christmas Holiday and with the help of wind data have been conducted. The results prove the ability of these low-cost sensors to detect rush hours measurements as well as the contribution to CO, NO, NO2, VOCs and PM emission due to the presence of the near highway.

How to cite: Gentile, L., Aruffo, E., Mascitelli, A., Chiacchieretta, P., and Di Carlo, P.: Characterization of low-cost sensors via simultaneous field measurements: a case study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12322, https://doi.org/10.5194/egusphere-egu25-12322, 2025.

EGU25-12373 | ECS | Orals | AS5.9

Monitoring Fog Evolution of Air Quality in Central Taiwan Mountain Area Using Air Quality Boxes 

Wei-Chieh Huang and Hui-Ming Hung

Increased industrialization has led to heightened exposure to poor air quality, raising the risk of cardiovascular diseases. Forest environments are increasingly valued for their ability to improve human mental and physical health by releasing phytoncide and reducing air pollutants. Xitou Experimental Forest of National Taiwan University (23.40°N, 120.47°E, 1178 m a.s.l.), a cloud forest in central Taiwan, located in a valley linked to industrial and metropolitan areas to the northwest, experiences air pollutant transport influenced by land-sea and mountain-valley breezes. These local circulation patterns bring urban air pollutants inland during the day, causing higher daytime concentrations compared to nighttime levels. To evaluate the contributions of physical transport and chemical reactions across different seasons, we applied five home-built Air Quality Box (AQB) systems along the valley. Each AQB integrates low-cost sensors to monitor ambient gaseous pollutants (CO, NO, NO2, O3, SO2, CO2, and non-methane hydrocarbon), ambient particle number size distribution (0.38-17 μm diameter), and meteorological parameters (temperature, relative humidity, and pressure). The particle size distribution shifts toward larger sizes with elevation, driven by hygroscopic growth as relative humidity increases during parcel ascent. Aerosols might act as cloud condensation nuclei, forming fog droplets predominantly around 5 μm in diameter in the Xitou area. With Mie scattering calculations, the extinction effect of aerosols and visibility in the study area can be estimated. CO concentrations, a marker of local pollutant transport, increase with the development of sea breeze and valley wind but decrease as the cleaner mountain wind prevails. Seasonal variations show that the mountain wind develops earlier in winter than in summer, leading to earlier pollutant reductions. Furthermore, agglomerative hierarchical clustering of diurnal CO patterns shows how pollutant concentrations rise with the development of valley winds and decrease with mountain wind onset around 17:00. These results demonstrate the utility of AQBs in providing high temporal-spatial resolution data to analyze complex transport dynamics and fog formation processes in mountain environments.

How to cite: Huang, W.-C. and Hung, H.-M.: Monitoring Fog Evolution of Air Quality in Central Taiwan Mountain Area Using Air Quality Boxes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12373, https://doi.org/10.5194/egusphere-egu25-12373, 2025.

Black Carbon (BC) is a crucial indicator of combustion-related pollution with significant health and climate implications; however, affordable, reliable, and easy-to-operate BC monitoring solutions remain limited. This presentation explores the integration of a novel BC Module into Clarity’s low-cost sensor (LCS) platform, and its implications for air quality management in the European Union and beyond.

Long-term collocated measurements of the Clarity BC Module across varied environmental conditions in California, Colorado, and Florida demonstrate high accuracy (R2 > 0.8) when benchmarked against a research-grade aethalometer. In early 2024, nine BC Modules were deployed in Perth, Australia to supplement the existing network of Clarity PM2.5 sensors. Using a source apportionment model, we found that diurnal and spatial variability in BC mass concentrations linked to fossil fuel combustion was greater than that of PM2.5, suggesting that city-wide BC monitoring can highlight spatial and temporal hotspots in local traffic emissions. Additionally, a strong correlation between PM2.5 and BC levels attributed to biomass burning emerged during periods impacted by nearby brush fires. While monitoring PM2.5 mass concentration is essential for evaluating air quality, integrating BC measurements can provide deeper insights into spatial, temporal, and source-specific air quality variability, enhancing our ability to manage and mitigate pollution sources effectively.

This session highlights how LCS, especially when integrated with black carbon measurement, can enhance air quality management in urban and rural areas across Europe and beyond. In the wake of the European Parliament’s adoption of the revised Ambient Air Quality Directive (April 2024), this session will explore the joint role of LCS and black carbon measurement in achieving Europe’s ambitious air quality goals. The directive mandates stricter pollution limits for particulate matter (PM2.5 and PM10) and introduces a requirement for BC monitoring, acknowledging its pivotal role in source attribution and pollution reduction strategies. By incorporating BC monitoring into existing PM2.5 networks, cities, and regions can achieve a more detailed understanding of pollution sources, such as traffic and biomass burning, enabling targeted interventions to reduce emissions and meet stricter limits.

How to cite: Micalizzi, P.: Integrating Low-Cost Sensors and Black Carbon Measurement for Better Air Quality Management in Europe and Beyond, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14392, https://doi.org/10.5194/egusphere-egu25-14392, 2025.

Over the past decade, I have had the privilege of collaborating with multiple teams in the USA, Europe, Africa, and Asia on projects to develop, characterise, and use low-cost sensors for air quality studies. These experiences and lessons for the future will be summarised in this talk.

In 2015, we partnered with SenSevere (now part of Sensit) to develop the Real-time Affordable Multi-Pollutant (RAMP) monitor, showing that startups can quickly enter this field with innovative ideas. However, extensive field testing by an academic group was required to make the devices usable, following which a network of 50 RAMPs was deployed across Pittsburgh, Pennsylvania. The high spatial density, high time resolution monitoring enabled by the sensor network revealed the impact of a large point source outside the city, while also highlighting hyperlocal pollution and street canyon effects. The extended deployment also showed that electrochemical sensors for nitrogen dioxide have a relatively high detection limit (~15 ppb) at odds with laboratory data and need to be replaced annually.

Hurricane Maria critically impaired traditional monitoring in San Juan, Puerto Rico, but the portability and low power requirements of sensor-based devices enabled rapid, solar-powered deployments of RAMPs that found significant sulfur dioxide pollution from generator usage across the city.

Sensing with RAMPs and Modulair-PM nodes and on-site observations identified hyperlocal sources of pollution at stadiums in Qatar and justified mitigation actions to ensure that football fans breathed cleaner air. Multi-year sensor-based monitoring in Kigali, Rwanda; Nairobi, Kenya; Abidjan, Côte d'Ivoire; and Accra, Ghana (coupled with CHIMERE air quality modelling over East Africa and 3D satellite data over West Africa) identified key sources of local air pollution, the influence of regional transport including Saharan dust in West Africa, and the need to develop local emission inventories.

The West African and Middle-Eastern experiences also showed the inability of low-cost PM sensors to detect supermicron dust. Evaluations at the first India Sensor Evaluation and Training (Indi-SET) facility in Bengaluru, India over 2024 showed that more expensive OPCs can better detect supermicron construction dust, but using similar internal sensors does not guarantee similar performance across device integrators.

Field collocation with reference monitors is ideal to improve sensor data quality, but this is not always possible especially in the Global South. Global reanalysis data sets can help reduce known artifacts in PM sensors. Establishing more facilities like Afri-SET (Accra, Ghana) and Indi-SET can also help improve sensor data quality.

This work would not be possible without international collaborations and networks like AfriqAir, CAMS-Net, ASIC, IGAC/Allin Wayra, and WMO/GAFIS. Collaborators, especially early-career researchers, will be acknowledged on the respective slides.

I will conclude with key learnings and prospects for the use of low-cost air quality sensors to address the grand challenge of clean air for all.

(Note: I have no financial interest in any sensor company.)

How to cite: Subramanian, R. S.: A decade of research with low-cost air quality sensors: air pollution insights, key learnings, and the road ahead, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14577, https://doi.org/10.5194/egusphere-egu25-14577, 2025.

EGU25-14757 | ECS | Posters on site | AS5.9

Optical Signals From Confined Materials At Nanometer Scales: Miniaturization As The Future Of Contaminant Detection 

Cesar A. Guarin Duran, Felipe Navarro Sanchez, Juan Galicia López, Jose Luis Hernández Pozos, Luis Guillermo Mendoza Luna, and Emmanuel Haro Poniatowski

Air pollution has become a critical public health issue in recent years, contributing significantly to the rise of respiratory diseases across large segments of the population and reducing average life expectancy. Although regulations exist to limit the emission of gases and particulate matter, there is a pressing need for more effective and comprehensive monitoring strategies. These strategies should enable real-time and large-scale detection of pollutant levels with greater accuracy. While monitoring stations are present in both developed and developing regions, more frequent and reliable data collection is essential to improve coverage and enhance data reliability.

This study focuses on pollutant monitoring and the development of innovative networks using miniaturized, low-cost sensor systems (LCS). It emphasizes research grounded in basic science, particularly the use of nanomaterials as sensors to selectively detect harmful gases and particles at low concentrations [1]. The study also explores the influence of local electric fields on the photophysical behavior of molecules near miniaturized systems [2], enabling the measurement of radiative and non-radiative processes triggered by device perturbations. This research aims to establish the foundation for building miniaturized sensors by integrating nanometer-scale devices into lab-on-a-chip systems [3], marking a significant step toward advancing low-cost, portable sensor technology.

The author are grateful to SECIHTI (CONAHCYT) for funding through grant CBF2023-2024-3073. The authors gratefully acknowledge the computing time granted by LANCAD and CONAHCYT on the supercomputers Yoltla (grant 21-2025) at LSVP UAM-Iztapalapa and UNAM.

[1] Experimental and computational investigation on the surface plasmon resonance of copper thin-films produced via pulsed laser deposition. Luis Mendoza-Luna, Cesar A. Guarin, Estefania Castañeda, Felipe Navarro Sánchez, Emmanuel Haro-Poniatowski, José L. Hernández-Pozos. Results in Optics. In review.

[2]Li, J.-F.; Li, C.-Y.; Aroca, R. F., Plasmon-enhanced fluorescence spectroscopy. Chem. Soc. Rev. 2017,46(13), 3962-3979

[3] Anderrsson, Helene; Van den berg, Albert. Microfluidic devices for cellomics: a review. Sensors and actuators B: Chemical, 2003, vol. 92, no 3, p. 315-325.

How to cite: Guarin Duran, C. A., Navarro Sanchez, F., Galicia López, J., Hernández Pozos, J. L., Mendoza Luna, L. G., and Haro Poniatowski, E.: Optical Signals From Confined Materials At Nanometer Scales: Miniaturization As The Future Of Contaminant Detection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14757, https://doi.org/10.5194/egusphere-egu25-14757, 2025.

EGU25-15040 | Orals | AS5.9

Enhancing Citizen Observatories for healthy, sustainable, resilient and inclusive cities 

Nuria Castell, Amirhossein Hassani, Uta Wehn, Joan Maso, João Tavares, and Alexios Chtzigoulas

Citizen Observatories (COs) empower residents to become active contributors to the observation and management of their local environments. Instrumented with low-cost sensors, communities can monitor the environment. However, the data and insights from COs do not always contribute to policy development. To address this challenge, the CitiObs project (www.citiobs.eu) is developing tools, methodologies and approaches to enhance COs in observing, monitoring, and protecting the urban environment, with a focus on air quality.  

CitiObs employs a co-creation framework, working closely with 85 COs to develop, test, and scale its tools and methodologies. Activities such as needs assessment workshops, capacity-building sessions, and strategic roadshows ensure the broad participation of stakeholders, from local citizens to EU policymakers.   

We follow a socio-technical approach, aiming to drive societal transformation by integrating technical innovations with participatory governance, enabling localized citizen-led actions. CitiObs technical approach focuses on advancing the use of sensors, generating Analysis Ready Data (ARD), and creating Decision Ready Information (DRI) to support environmental monitoring and policymaking. To make data FAIR the project uses Sensor Thing API (and the Citizen Science extension: STAplus). To create ARD, the project has developed automated calibration methods to improve sensor accuracy and has proposed a unified terminology for data quality levels to ensure consistency and interoperability across datasets. The validated data is then used to generate DRI, as, for example, high-resolution maps of air pollution and thermal stress (e.g., integrating sensor data with satellite observations and CAMS models). The ARD and DRI can then be used for customized analytics, and it facilitates the uptake of policy makers and scientists as it ensures that citizen-collected data is reliable, or of known-quality. CitiObs social approach emphasizes inclusive citizen engagement, participatory governance, and citizen-led actions to foster sustainable urban environments. The project is developing four toolkits. 

The Leaving No One Behind Toolkit helps COs enhance diversity and inclusion with practical guidance and resources for more inclusive initiatives. The Participation Dynamics Toolkit supports COs in fostering strong stakeholder relationships, addressing conflicts, and building trust. The Citizen Led Action Toolkit empowers communities to drive environmental protection through co-creation tools for planning impactful actions, often with artists and creatives. Lastly, the Environmental Monitoring Toolkit (https://github.com/citiobs) provides resources for affordable, open environmental monitoring, covering sensor selection, data quality, and interoperability. 

The project’s outcomes include the development of a comprehensive Knowledge Platform and the CitiObs Cookbook, which will serve as resources for communities and practitioners in Europe and worldwide to establish or enhance their own Citizen Observatories. We are currently collaborating with the Citizen Science Global Partnership to transfer the know-how generated in the project to other countries in Africa, Latin America and Asia. 

We acknowledge funding for CitiObs project from the European Union’s Horizon Europe research and innovation programme under grant agreement No.101086421. 

How to cite: Castell, N., Hassani, A., Wehn, U., Maso, J., Tavares, J., and Chtzigoulas, A.: Enhancing Citizen Observatories for healthy, sustainable, resilient and inclusive cities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15040, https://doi.org/10.5194/egusphere-egu25-15040, 2025.

EGU25-15277 | Posters on site | AS5.9

Calibration of integrated low-cost environmental sensors based on machine learning 

Chao Zeng, Fang Nan, Huifang Li, Jie Li, and Xiaobin Guan

Monitoring urban microenvironments using low-cost sensors effectively addresses the spatiotemporal limitations of conventional monitoring networks. However, their widespread adoption is hindered by concerns regarding data quality. Calibrating these sensors is crucial for enabling large-scale deployment and increasing confidence among researchers and users. This study focuses on an Internet of Things (IoT) application in Wuhan, China, aiming to enhance the quality of long-term hourly air quality and air temperature data collected by low-cost sensors through on-site calibration.

Standard weather stations operated by meteorological regulatory agencies at various locations served as reference points for calibrating the sensors. Multiple linear regression (MLR) and machine learning (ML) algorithms were employed for calibration, with leave-one-out cross-validation (LOOCV) used for model evaluation. Factors, such as environmental conditions, spatial distances, and seasonal variations were also examined for their influence on long-term data calibration. Experimental findings revealed that the random forest (RF) model consistently outperformed other methods. Calibration using this approach markedly improved sensor data quality, with the R-squared value of a sensor with the poorest raw data increasing from 0.416 to 0.980, mean absolute error (MAE) decreasing from 6.255 to 1.002, and root mean square error (RMSE) reducing from 7.881 to 1.447. The study also investigated the effects of multiple scenes and distances on calibration through three experimental scenarios. Results indicated that calibrated models using training sites with the same surface type as testing sites performed better when distances were similar. However, due to a limited number of sites with similar surface types, there are insufficient experiments on the impact of distance when the surface types are similar.

The ML-based calibration model developed in this study has the potential to enhance the utility of low-cost sensors for urban environmental monitoring. It enables real-time monitoring, cost-effective and reliable data collection, supporting research on urban regional environments and urban residents’ health.

How to cite: Zeng, C., Nan, F., Li, H., Li, J., and Guan, X.: Calibration of integrated low-cost environmental sensors based on machine learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15277, https://doi.org/10.5194/egusphere-egu25-15277, 2025.

EGU25-15372 | Orals | AS5.9

From Workplace Safety to Behavioral Change: Diverse Applications of Low-Cost Sensors in Indoor Environments 

Stig Koust, Morten Stoltenberg, Thor-Bjørn Ottosen, Søren Møller, Freja Rasmussen, Jonas Andersen, Julie Rasmussen, Halfdan Clausen, Pia Viuf Ørby, and Ulrich Gosewinkel

Low-cost sensors (LCS) have emerged as versatile tools for air quality monitoring across diverse applications. This presentation synthesizes some of our work and findings from multiple projects, demonstrating the adaptability and effectiveness of LCS in various monitoring scenarios.

We have investigated the usefulness of low-cost sensors for continuous monitoring of particle exposure as a tool for workplace interventions. Through a systematic study across four companies, we have benchmarked the performance of LCS against reference-grade equipment in realistic work environment settings. LCS with sufficient accuracy potentially enables organizations to perform their own air quality management. We have provided such a system to the companies and are currently assessing how access to real-time LCS data has changed the safety cultures in the workplaces. Moreover, we have utilized LCS sensors to validate the performance of novel air cleaning technology in diverse environments such as garbage truck cabins and elder care facilities.

Another initiative aimed to develop an early warning system for fungal spores in greenhouse environments, to reduce the use of preventive fungicide. The system achieved an accuracy of 83% with less than 5% false positives in identification of “high” greymold spore-counts. This system demonstrated the potential for LCS in preventing crop diseases while reducing fungicide use.

In another project, we utilized CO2 sensors to study user behavior modifications in office environments, while also looking at its effects on the indoor climate. Revealing a simple case of how data analysis of simple measurements and the implementation of LCS itself provided insights into nudging humans to improve their working environment while determining the potential effects. Lastly, we have utilized LCS in schools and daycares to evaluate indoor air quality (IAQ) and correlate IAQ to the transmission of airborne patogens and thereby spread of disease.   

These diverse applications highlight a small part of the versatility and strengths of LCS, while demonstrating practical solutions for data quality challenges, calibration procedures, and long-term reliability. Our experiences provide insights for implementing LCS across various scenarios, particularly in resource-constrained environments.

How to cite: Koust, S., Stoltenberg, M., Ottosen, T.-B., Møller, S., Rasmussen, F., Andersen, J., Rasmussen, J., Clausen, H., Ørby, P. V., and Gosewinkel, U.: From Workplace Safety to Behavioral Change: Diverse Applications of Low-Cost Sensors in Indoor Environments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15372, https://doi.org/10.5194/egusphere-egu25-15372, 2025.

Particulate matter (PM), particularly PM2.5 and PM10, poses significant risks to human health, with concentrations varying across time and space. While conventional sources of PM are well-known, domestic wood burning may also substantially influence air quality, particularly in residential areas. In this study, we use publicly available citizen-owned low-cost air quality sensor data (e.g., PM2.5 and PM10) and a web-scraping dataset on woodburning devices to investigate the effect of domestic wood burning on air quality in The Netherlands. We retrieved and analyzed large volumes of sensor data, which we compared with data from calibrated sensors. By examining the temporal and spatial patterns of PM data, we assessed the potential link between domestic wood burning and air quality. We will discuss specific results but also the opportunities and challenges of the use of citizen-owned sensors, including for the integration of environmental and health research.

How to cite: Veldhuijzen, P., Schultner, J., and Hein, L.: Using citizen-owned sensors for integrating environmental and health research: an exploration of domestic wood burning and air quality in The Netherlands, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17566, https://doi.org/10.5194/egusphere-egu25-17566, 2025.

EGU25-18970 | ECS | Orals | AS5.9

Investigating In-Cabin Air Quality in Public Utility Buses in the Philippines Using Small-Sensors 

Roy Emmanuel Pineda, Aldon Cris Galido, John Jairus Eslit, Uziel Rein Agub, Jomari Ganhinhin, Miguel Carlos Menguito, Percival Magpantay, Marc Rosales, Isabel Austria, Jaybie de Guzman, Maria Theresa de Leon, Rhandley Cajote, Paul Jason Co, and John Richard Hizon

This study investigates in-cabin air quality on Philippine public utility buses (PUBs) by measuring particulate matter (PM) and carbon dioxide (CO2) concentrations to assess potential exposure levels among daily commuters. Using compact air quality monitors with small-sensor technology, measurements were taken inside two types of PUBs: regular buses in the EDSA carousel and the smaller modern jeepneys currently being deployed across different routes in the metro. Data was collected across different routes with varying traffic and occupancy conditions to evaluate how these factors influence the variability and range of PM and CO2 concentrations. The air quality aboard the EDSA Carousel bus was assessed along its bus rapid transit route on EDSA, extending to the Parañaque Integrated Terminal Exchange (PITX). Meanwhile, the modern jeepney route began at its terminal near EDSA-Shaw Boulevard and ended in Antipolo City. The bus route covered approximately 28 kilometers (~2 hrs), while the modern jeepney route spanned 14 kilometers (~1 hr). Elevated CO2 levels were observed in both types of PUBs during rush hours increasing from 1039.51 ppm to 2284.03 ppm and 3806.9 ppm to 6150.44 ppm for the carousel bus and modern jeepney, respectively. This effect can be attributed to higher passenger occupancy and is more pronounced in the modern jeepney, which has a smaller cabin and often experiences passenger overloading, compared to the EDSA carousel bus, which features a larger cabin and enforces stricter passenger limits. CO2 concentrations also read higher at the rear of the buses, farther from the bus doors. Additionally, PM2.5 levels were elevated during periods of heavier road traffic, with levels climbing from 7.12 µg/m3 to 10.39 µg/m3 and 6.66 µg/m3 to 18.79 µg/m3 for the carousel bus and modern jeepney, respectively. The observed increase suggests that traffic conditions contribute considerably to indoor particulate matter exposure within the PUBs, which is likely due to the diffusion of outdoor air pollution when the doors open during stops.

How to cite: Pineda, R. E., Galido, A. C., Eslit, J. J., Agub, U. R., Ganhinhin, J., Menguito, M. C., Magpantay, P., Rosales, M., Austria, I., de Guzman, J., de Leon, M. T., Cajote, R., Co, P. J., and Hizon, J. R.: Investigating In-Cabin Air Quality in Public Utility Buses in the Philippines Using Small-Sensors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18970, https://doi.org/10.5194/egusphere-egu25-18970, 2025.

EGU25-19054 | ECS | Orals | AS5.9

Short-Term PM2.5 Exposure and Health Impacts: Insights from the AMRIT Low-Cost Sensor Network in the Indo-Gangetic Plains of India 

Navdeep Agrawal, Nimit Godhani, Anandh P. Chandrasekaran, Anil Kumar, Sachchida N. Tripathi, Sourangsu Chowdhury, and Piyush Rai

Air pollution remains a critical global challenge, exerting significant health and economic burdens, particularly in developing nations. A key obstacle to effective air quality management is the limited availability of monitoring infrastructure, compounded by insufficient spatial coverage. This shortfall is largely due to the high costs associated with establishing and maintaining regulatory air quality monitoring stations. However, the advent of Internet-of-Things (IoT)-based monitoring devices equipped with low-cost sensors (LCS) has opened new avenues for air quality assessment. These devices, which leverage cellular networks for connectivity, offer a cost-effective alternative and can be deployed across geographic locations. Over India, this development presents a valuable opportunity to enhance our understanding of air quality beyond the urban regions, where monitoring stations are scarce.
In this context, a state-wide sensor-based Ambient Air Quality Monitoring (SAAQM) network has been established under the project “Ambient Air Quality Monitoring Over Rural Areas using Indigenous Technology” (AMRIT) to investigate the current levels of fine particulate matter (PM2.5) pollution across the state of Bihar, located in the eastern part of Indo-Gangetic Plains, India. This initiative has expanded the air quality monitoring infrastructure from 35 regulatory-grade monitors to 539 SAAQM nodes, enhancing monitoring infrastructure coverage by a factor of 15. This enables a more granular assessment of PM2.5 exposure and associated health impacts, reaching down to the census tract level.
To generate continuous sub-daily PM2.5 concentration maps at a spatial resolution of 0.5 km², we employed a machine learning framework that integrates meteorological variables and satellite imagery-based predictors with SAAQM observations. Our findings indicate that the dense SAAQM network is considerably more effective in capturing localized variations in PM2.5 exposure, which are often overlooked by other high-resolution global datasets. We found significant spatiotemporal heterogeneity in the PM2.5 exposure distribution, with elevated PM2.5 exposure levels over the northern tracts of Bihar. The population-weighted concentration ranged from 55 (±14) μg/m³ in pre-monsoon (March-May), 110 (±30) μg/m³ in post-monsoon (October-November), and 136 (±40) μg/m³ in winter months (December-February). Furthermore, we evaluated the associated health impacts using an India-specific exposure-response function, identifying a short-term mortality rate of 50 per lakh population (95% CI: 33–64) in the region. These findings emphasize the critical importance of hyperlocal air quality monitoring in understanding PM2.5 exposure and mitigating its health risks.

How to cite: Agrawal, N., Godhani, N., P. Chandrasekaran, A., Kumar, A., N. Tripathi, S., Chowdhury, S., and Rai, P.: Short-Term PM2.5 Exposure and Health Impacts: Insights from the AMRIT Low-Cost Sensor Network in the Indo-Gangetic Plains of India, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19054, https://doi.org/10.5194/egusphere-egu25-19054, 2025.

EGU25-19153 | ECS | Posters on site | AS5.9

Optimal data framework for large-scale application of low-cost sensor networks in African cities 

Deo Okure, Richard Sserunjogi, Joel Ssematimba, Usman Abdul-Ganiy, Julia Brown, and Engineer Bainomugisha

Many cities in Low and Middle Income Countries (LMICs), particularly in Africa lack access to timely data from continuous networks due to the prohibitive costs of setting up conventional networks. Low-cost sensors (LCS) costing less than $2,000 have the potential to close the data gaps in data-hungry cities because of the advances in sensing technology, computational capability and affordability. Application of LCS has gained traction over the years, increasingly recognised by regulatory and international agencies including the World Meteorological Organisation, US EPA, and the recent UNEA-6/10 resolution on regional cooperation for improved air quality globally recognises the need to leverage LCS and digital platforms. However, there are contextual bottlenecks including data reliability and availability, limited internet and electricity, and local capacity for network management that hinder successful deployments of large-scale networks. These challenges are intricately linked to local environmental conditions and logistical circumstances in African settings. The current work based on AirQo’s experience across Africa seeks to unlock the barriers to the adoption of low-cost sensors for continuous monitoring through contextualization, firstly, by untangling the requirements for custom-sensor applications in an African context that transcends beyond the choice of technology. We demonstrate from ongoing case studies in major African cities including Kampala, Nairobi, Kisumu, Yaounde, and Lagos, that achieving a robust LCS network requires integration of four key pillars; (i) custom technology for autonomous portable air quality sensors, (ii) decentralised sensing network (iii) data management platform and (iv) community ownership. The current work advances the case for replicating real-life case studies across diverse settings in different data-hungry cities across Africa.

How to cite: Okure, D., Sserunjogi, R., Ssematimba, J., Abdul-Ganiy, U., Brown, J., and Bainomugisha, E.: Optimal data framework for large-scale application of low-cost sensor networks in African cities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19153, https://doi.org/10.5194/egusphere-egu25-19153, 2025.

EGU25-19203 | ECS | Posters on site | AS5.9

From monitoring to mitigating: the role of data in reducing air pollution levels in low- and middle-income countries 

Camille Fournier de Lauriere, Ella Henninger, E. Keith Smith, Vally Kouby, and Thomas Bernauer

Outdoor air pollution is responsible for more than 4 million premature deaths annually, with disproportionate impacts in low- and middle-income countries. Despite the human and economic cost of air pollution, many cities worldwide lack reliable air pollution data, even in regions suspected of having the highest levels of pollution. The publication of air quality information has been widely advocated as a critical step towards reducing pollution and improving public health, as it can raise awareness, drive regulatory action, and empower citizens to demand effective policies.

In practice, China’s extensive Air Quality Monitoring (AQM) campaigns have successfully raised public attention and awareness while reducing pollution levels. Similarly, it is documented that reference-grade monitors at U.S. embassies have led to significant pollution reductions. Despite these examples, we lack a systematic understanding of how AQM campaigns translate into pollution reductions. Notably, the role of ‘low-cost’ sensors -that are cheaper, easier to deploy and maintain and show increasing accuracy to measure air pollution levels- is not yet broadly documented.

This research is a quantitative evaluation of the extent to which reference-grade monitors and low-cost sensors might be associated with reductions in pollution levels. We also explore how socio-economic and political contexts may mediate the effectiveness of AQM, particularly in developing regions where regulatory enforcement and public responsiveness vary. Understanding how AQM in different developing contexts may or may not lead to improved air quality could prove invaluable in designing new successful campaigns without hindering economic development.

How to cite: Fournier de Lauriere, C., Henninger, E., Smith, E. K., Kouby, V., and Bernauer, T.: From monitoring to mitigating: the role of data in reducing air pollution levels in low- and middle-income countries, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19203, https://doi.org/10.5194/egusphere-egu25-19203, 2025.

EGU25-19762 | Orals | AS5.9

Long-term aerosol measurements of the Alphasense OPC-N3 in arctic regions: Sensor performance and corrections 

Kilian Schneiders, Lasse Moormann, Sylvain Dupont, Daniel Koenen, Jan Rabe, Pavla Dagsson Waldhauserová, Kerstin Schepanski, Agnesh Panta, Martina Klose, Hannah Meyer, Cristina González-Flórez, Adolfo González-Romero, Xavier Querol, Andres Alastuey, Jesús Yus-Díez, Carlos Pérez García-Pando, and Konrad Kandler

With the decrease of electronic component prices, powerful yet low-cost optical particle counters (OPCs) gain in popularity and are frequently used in citizen science as well as classical science projects. The application of OPCs in large numbers can yield higher spatial resolution and, thus, offers great opportunities for studies of spatial distribution and development, e.g. of dust or air pollution. As a consequence, sensor performance and long-term accuracy must be evaluated in order maintain data quality.

During the HiLDA campaign, a measurement campaign focused on Arctic dust emission, we deployed seven measurement stations at Arctic locations (Jan Mayen, Northern and Southern Iceland, Southern Svalbard, North West Norway, South East Greenland, Faroe Islands). Each station was equipped with a compact weather station and four Alphasense OPC-N3 low-cost OPCs, among others. Data was collected for different periods of one to over three years between 2020 and 2025.

During the deployment under occasionally severe weather conditions, most of the sensors age significantly, which was to be expected at the time of deployment. Therefore, of the four instruments at each station, only one system was operated permanently, while a second one was switched on every week for a short time period to allow for a detection of this aging. The other two served as spare, which were used when the continuously running system was deemed to be degraded. The findings from a total of 28 low-cost OPCs are presented. We observed a combination of continuous aging due to soiling and sudden degradations, probably linked to single extreme events. We present a correction scheme for the continuous aging and point out quality markers for the degradation, as well as observed instrument variation. This information can be used to develop adapted measurement strategies and yield an overall increased data quality.    

How to cite: Schneiders, K., Moormann, L., Dupont, S., Koenen, D., Rabe, J., Dagsson Waldhauserová, P., Schepanski, K., Panta, A., Klose, M., Meyer, H., González-Flórez, C., González-Romero, A., Querol, X., Alastuey, A., Yus-Díez, J., Pérez García-Pando, C., and Kandler, K.: Long-term aerosol measurements of the Alphasense OPC-N3 in arctic regions: Sensor performance and corrections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19762, https://doi.org/10.5194/egusphere-egu25-19762, 2025.

EGU25-19930 | Posters on site | AS5.9

Opportunities and challenges of sensor technology for indoor air quality monitoring 

Vasileios Salamalikis, Amirhossein Hasani, Nuria Castell, Stelios Kephalopoulos, Óscar González, Thanos Nenes, Maria Figols, Kostas Eleftheriadis, Mario Lovrić, Alessandro Battaglia, Pieter De Beule, and Sywert Brongersma and the IDEAL CLUSTER - WG5 Memebers

Indoor air quality (IAQ) plays a vital role in providing healthier indoor environments, especially considering that most human activities occur indoors.  Since indoor and outdoor air pollutants are closely interrelated, monitoring both can provide insights into IAQ dynamics.  

The IDEAL (Indoor Air Quality Health) Cluster comprises seven Horizon-Europe funded projects (InChildHealth, INQUIRE, LEARN, K-HealthinAIR, SynAir-G, TWINAIR, and EDIAQI) and the Working Group (WG) on Sensors aims to enhance understanding of knowledge gaps in IAQ, identifying IAQ determinants and to assess their health impacts using various sensor technologies. The goal of the WG on Sensors is to develop common documentation on sensor types, operation modes, characterization, calibration, performance, assessment and validation methods for indoor air quality monitoring and health impact assessment.  

The documentation is informed by the different technologies and methodologies used across the seven EU-projects. We have found that the most commonly measured parameters include particulate matter, total volatile organic compounds (TVOC), CO2 and comfort parameters (temperature and relative humidity) although other parameters are also monitored based on the specific needs of each project.  Low-cost sensors for indoor air quality monitoring are used across all the IDEAL cluster’s projects, although they come from different manufacturers. For example, VOCs are monitored using metal oxide sensors from Sensirion, Alphasense, and Figaro, with non-distinction of the VOC species to be the common challenge across all low-cost sensors. All the projects have planned for co-location to understand the data quality. Sensor-measured particulate matter is mainly validated against reference measurements in the field, and in two out of seven projects co-location campaigns conducted in various European countries to assess how the sensors respond in different indoor environments. 

In this transfer learning approach, all projects share their experiences, highlighting the advantages, limitations, and challenges associated with using different sensor technologies to measure air pollutants. All information gathered is mapped to identify possible similarities and challenges in measuring common parameters across the seven IDEAL Cluster’s projects. This information can be proven useful also to projects pertaining to other citizen science initiatives that are interested in monitoring IAQ. 

 

Acknowledgments: We acknowledge funding for INQUIRE project from the European Union’s Horizon Europe Research and Innovation programme under grant agreement No.1011057499. 

How to cite: Salamalikis, V., Hasani, A., Castell, N., Kephalopoulos, S., González, Ó., Nenes, T., Figols, M., Eleftheriadis, K., Lovrić, M., Battaglia, A., De Beule, P., and Brongersma, S. and the IDEAL CLUSTER - WG5 Memebers: Opportunities and challenges of sensor technology for indoor air quality monitoring, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19930, https://doi.org/10.5194/egusphere-egu25-19930, 2025.

EGU25-20256 | Orals | AS5.9

Performance of low-cost sensors to measure PM10: do they also measure coarse particles? 

Martine Van Poppel, Jelle Hofman, Jan Peters, Jo Van Laer, Borislav Lazarov, Michel Gerboles, and Sinan Yatkin

Low-cost sensor can be key additional tools to fixed air quality monitoring stations (AQMS)for more extended AQ assessment. Sensors can be deployed at a higher density due to their lower cost. However, the data quality of sensors is still unknown and can be function of location and meteorological conditions.

One of the issues that PM sensors are dealing with is the ability to measure coarse fractions of PM. It is known that some low-cost sensors calculate PM10 concentrations based on the measured concentrations of PM2.5. The main issue with the evaluation of PM sensors for PM10 in the field, is that PM10-2.5 fractions at most AQMS are relatively small, and relying on only field test for PM10 would not identify the problem, whereas the sensor would largely underestimate the PM10 concentrations when deployed at areas or specific events with high coarse fractions.

Coarse particles are defined here as PM10-2.5 = PM10 – PM2.5. A laboratory test was developed for PM sensors (as part of the CEN/TS 17660-2:2024) and will evaluate the potential of the PM10 sensor system to correctly measure the coarse fraction. This presentation presents the lab test to evaluate if sensor systems can measure also coarse PM fractions and can measure PM10 rather than calculating it from the PM2.5 signal.

The sensor systems under test are placed in the test chamber in close vicinity of the optical monitor (as equivalent method) and particles are generated and mixed so that sensor systems and optical monitor are exposed to the same PM concentrations and fractions.

The sensor systems are exposed to two different PM fractions over two tests (‘Coarse test’ and ‘Fine test’) to evaluate their response to PM. The size fractions generated inside the test chamber will fulfil the following requirements:

  • Coarse test: >80% PM10-2.5 in PM10
  • Fine test: <20% PM10-2.5 in PM10

For each test, a monodisperse aerosol with respectively coarse and fine size restrictions (and with the same composition) is used to generate these conditions. Based on these tests, the sensor response (ratio of the output of the sensor versus the equivalent method) is calculated for PM10-2.5 (coarse test) and PM2,5 (fine test). When the sensor measures the PM10 concentration it is assumed that the sensor response will not change significantly between the two conditions. An example to illustrate this approach will be given using the AirsensEUR (version 3.0) sensor system. The AirsensEUR sensor system has two sensors included.  Laboratory test results will also be compared to field observations for this sensor system; data collected as part of the sensEURcity project.

 

How to cite: Van Poppel, M., Hofman, J., Peters, J., Van Laer, J., Lazarov, B., Gerboles, M., and Yatkin, S.: Performance of low-cost sensors to measure PM10: do they also measure coarse particles?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20256, https://doi.org/10.5194/egusphere-egu25-20256, 2025.

EGU25-20302 | ECS | Orals | AS5.9

Improving indoor air quality in schools: Evidence from an air purifier intervention with low-cost sensors 

Stefania Renna, Jacopo Bonan, Francesco Granella, and Luis Sarmiento

Poor air quality disproportionately affects children's health, causing both clinical and subclinical effects including respiratory infections, asthma, allergies, absenteeism, and cognitive impairment. This challenge is particularly acute in developing countries and urban areas, where air pollution frequently exceeds the World Health Organization's global air quality guidelines. Leveraging innovative low-cost sensor technology, we designed a cluster randomized control trial to evaluate the effectiveness and economic feasibility of classroom portable air purification systems, while simultaneously developing a framework for continuous air quality monitoring in educational settings. We randomly assigned 95 classrooms (~2000 students) across five primary schools in Milan, Italy, to treatment and control groups, implementing a comprehensive monitoring system that integrated indoor and outdoor air quality sensors with health outcome data. Our sensor network collected continuous measurements of air quality parameters while enabling real-time data analysis and integration with survey data on health symptoms and air quality perception. Results demonstrate that air purifiers reduced indoor air pollution by 28%, corresponding to an 11% reduction in student absences. The impact was most pronounced among vulnerable students with higher pre-treatment absences and those of non-Italian nationality. Notably, the purifiers' effectiveness showed an inverse relationship with outdoor pollution levels, suggesting limitations in their ability to maintain healthy indoor air quality during severe pollution events. Our intervention also revealed improved self-reported respiratory health, enhanced awareness of air quality issues, and increased support for urban air quality policies among treated students. This study not only demonstrates the cost-effectiveness of school-based air purifiers but also establishes a replicable framework for implementing and evaluating air quality interventions in resource-constrained educational settings using affordable sensor technologies.  

How to cite: Renna, S., Bonan, J., Granella, F., and Sarmiento, L.: Improving indoor air quality in schools: Evidence from an air purifier intervention with low-cost sensors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20302, https://doi.org/10.5194/egusphere-egu25-20302, 2025.

EGU25-20418 | ECS | Orals | AS5.9

Beyond Data: Leveraging Low-Cost Sensors for Policy Impact and Regulatory Acceptance   

Faith Nangila Wafula, Nuria Castell, and Libby Hepburn

Low-cost sensors are revolutionizing air quality monitoring, especially in under-resourced regions like Kenya. These devices enable affordable, localized data collection, which allows communities to identify pollution hotspots, raise awareness, and advocate for action. However, their integration into formal regulatory frameworks remains limited due to concerns over data reliability and perceived shortcomings compared to traditional systems (Lewis et al., 2016).

Many African cities face mounting air pollution challenges but lack consistent urban air quality monitoring. Although Kenya enacted Air Quality Regulations in 2014, data on particulate pollutants in Nairobi remains scarce. This gap is common across many African nations, hindering efforts to assess pollution impacts, inform policy, and respond effectively to deteriorating air quality. The global Air Quality Community of Practice (CoP) of the Citizen Science Global Partnership (CSGP) actively addresses these challenges by working to scale up air quality monitoring in under-resourced regions and demonstrating evidence-based policymaking through citizen science.

This presentation proposes actionable strategies to enhance the credibility and impact of low-cost sensors in policymaking and regulatory contexts in such regions. First, establishing universal calibration and validation protocols in collaboration with academic and industry stakeholders can significantly bolster the credibility of sensor data by ensuring alignment with regulatory standards (Crilley et al., 2018). The Air Quality CoP is collaborating with the WorldFAIR+ Project and the CitiObs project to create interoperability frameworks based on FAIR principles for citizen science air quality monitoring. Second, creating effective data communication strategies can maximize the visibility and impact of sensor-derived insights. Platforms that transform complex datasets into accessible visualizations and narratives can engage policymakers and the public, fostering broader support (Kumar et al., 2022).

Integrating citizen science into policy through multi-stakeholder collaborations institutionalizes community-driven data collection. Open-access platforms, such as OpenAQ, bridge local monitoring efforts with policy-level interventions, building stakeholder trust and cooperation. Finally, advocating for adaptive regulatory systems that position low-cost sensors as complementary tools to traditional monitoring methods and not replacements can drive innovation and amplify impact.

Drawing from case studies within the CoP and successful implementations, this session explores how these solutions can bridge the gap between citizen-driven data and institutional action. By tackling technical, communication, and policy challenges, low-cost sensors can be repositioned as essential tools for community agencies, filling data gaps, raising awareness, and impactful policy change.

 

We acknowledge funding for the CitiObs project from the European Union’s Horizon Europe research and innovation programme under grant agreement No.101086421.   

 

References:  

Lewis, A., et al. (2016). Evaluating low-cost sensors for air quality monitoring. Faraday Discussions. https://doi.org/10.1039/C5FD00201J  

Crilley, L., et al. (2018). Calibration of low-cost air quality sensors for urban environments. Atmospheric Measurement Techniques. https://doi.org/10.5194/amt117092018  

Kumar, P., et al. (2022). Bridging the gap between citizen science and policymaking. Environmental Monitoring and Assessment. https://doi.org/10.xxxxxx  

Code for Africa. (2019, October 21). Measuring Nairobi’s air quality using locally assembled low-cost sensors. Medium. https://medium.com/code-for-africa/measuring-nairobis-air-quality-using-locally-assembled-low-cost-sensors-94a356885120

Hasenkopf C. et al (2024) Energy Policy Institute at Chicago. The Case for Filling Air Quality Data Gaps with Local Actors: A Golden Opportunity for the Philanthropic Community  

How to cite: Nangila Wafula, F., Castell, N., and Hepburn, L.: Beyond Data: Leveraging Low-Cost Sensors for Policy Impact and Regulatory Acceptance  , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20418, https://doi.org/10.5194/egusphere-egu25-20418, 2025.

EGU25-20628 | Posters on site | AS5.9

The climate-health cascade: Assessing the impact of rising temperature and particulate pollution on hospital admissions 

Ricardo HM godoi, Felipe Baglioli, Camila B Carpenedo, isabelle O Silva, and Ana F L Godoi

Recent research from across the globe has unveiled a growing trend towards more frequent and intense climate events, marked by increasingly higher temperature peaks. Additionally, escalating human activities in urban areas are amplifying air pollution levels, notably particulates such as PM10 and PM2.5, which are closely linked to significant health problems and subsequent hospitalizations. These environmental concerns — heightened levels of particulates and more extreme climate events — have been definitively associated with adverse health outcomes, leading to an uptick in hospital admissions. This study seeks to explore the interconnections between these environmental factors and public health, assessing how human-induced climate change impacts healthcare systems. By integrating meteorological data, public health records, and readings from particulate matter sensors in Curitiba, Southern Brazil, we have constructed a comprehensive dataset that spans these three domains. Our statistical analysis reveals that average monthly concentrations of PM10 and PM2.5 exhibit a slight negative correlation with hospital admissions in the same month. Intriguingly, this relationship turns positive when analyzed with a one-month delay. Furthermore, we found that hospitalization rates increase in months when pollution levels exceed the World Health Organization's Air Quality Guidelines. Similarly, we observed that maximum temperature values show a negative correlation with hospital admissions initially but correlate positively when delayed by a month. These correlations suggest a synergistic effect between rising temperatures and increased levels of particulate matter, underscoring a direct link to hospital admissions with a one-month lag. 

How to cite: godoi, R. H., Baglioli, F., Carpenedo, C. B., Silva, I. O., and Godoi, A. F. L.: The climate-health cascade: Assessing the impact of rising temperature and particulate pollution on hospital admissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20628, https://doi.org/10.5194/egusphere-egu25-20628, 2025.

Exposure to high levels of particulate matter (PM) could result to adverse health effects.
The use of fireworks during the New Year celebration result to the rapid increase in
ground-level air pollution which could linger for a few hours or longer depending on the
prevailing meteorological conditions. The rapid increase in the air pollution levels caused
by this event could affect vulnerable groups with underlying health conditions. This
research explores the variations of air pollution levels in select residential areas in Iloilo
City, Philippines during the 2025 New Year celebration. The sensors used are
AirGradient outdoor monitors managed by the Urban Air Quality Monitoring Group at
Central Philippine University. The observation period spanned from December 10, 2024
and January 10, 2025 and is focused on PM2.5 levels to give insight on the overall air
pollution condition. The data shows a total increase in pollution levels throughout all the
stations during the event followed by the subsequent reduction in air pollution levels
hours after the event. The observed PM2.5 concentration ranged from below 35 μg/m 3
prior to the event and up to greater than 500 μg/m 3 in some stations immediately after the
event. At the highest peak, some stations register values more than 40 times greater than
the WHO guideline value for 24-hr exposure. The research offers valuable information
on the air pollution levels in Iloilo City particularly during the New Year celebration. The
use of a network of low-cost sensors gives valuable insight on the characteristic
variations and trends on the air pollution in low-income urban communities and cities in
the Philippines and beyond.

How to cite: Magtulis, V. J.: PM2.5 level observations during New Year Celebration inIloilo City, Philippines using low-cost sensors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20880, https://doi.org/10.5194/egusphere-egu25-20880, 2025.

EGU25-21629 | Orals | AS5.9

Integrating Low-cost Sensor Systems and Networks to Enhance Air Quality Applications 

R subu Subramanian, Sara Basart, Carl Malings, Kofi Amegah, Sebastian Diez, Colleen Rosales, and Naomi Zimmerman

 Low-cost air quality sensor systems (LCS) represent a transformative tool in modern air quality management strategies, offering unprecedented opportunities to complement traditional monitoring approaches. The integration of LCS data with established monitoring systems, including satellite observations and reference-grade instrumentation, has the potential to significantly enhance the reliability and applicability of air quality data. In regions lacking comprehensive monitoring networks, LCS can bridge critical gaps by identifying local factors affecting air quality, thus guiding targeted monitoring efforts and informing policy development.

A key advantage of LCS lies in their capacity to extend the spatial and temporal coverage of existing monitoring networks. By deploying LCS in underserved areas, policymakers can gain actionable insights into localized pollution patterns, which are essential for designing effective mitigation strategies. Furthermore, the use of LCS promotes community engagement by empowering local stakeholders to participate in air quality monitoring and advocacy.

Despite their potential, the application of LCS data must account for inherent limitations in accuracy and precision. Co-locating LCS with reference-grade monitors is a critical step to quantify measurement uncertainties and ensure data quality. This approach facilitates the calibration of LCS, enabling their use in advanced applications such as air quality forecasting, source impact analysis, and public health assessments.

The World Meteorological Organization (WMO) has played a pivotal role in coordinating global efforts to standardize and optimize the deployment of LCS technologies. Through the development of guidelines, best practices, and frameworks for integration, the WMO has provided critical support for national and regional initiatives aimed at improving air quality management. Recent developments, overviewed in the WMO’s 2024 report (WMO, 2024), highlight the organization’s leadership in promoting the use of LCS as integral components of comprehensive air quality management frameworks. This report underscores the importance of integrating LCS with traditional and emerging data sources, offering practical guidance on network design, calibration protocols, performance evaluation, and data communication. These insights align with previous WMO publications that establish foundational principles for LCS operation and deployment.

The continued refinement of LCS technologies, alongside efforts to standardize their use within monitoring networks—coordinated by institutions such as the WMO—will be pivotal in unlocking their full potential and fostering a more equitable approach to air quality management worldwide.

The present contribution will overview the main outcomes of the WMO’s 2024 report on the use of LCS for different air quality applications from supporting air quality management strategies to promoting social awareness of air pollution issues.

How to cite: Subramanian, R. S., Basart, S., Malings, C., Amegah, K., Diez, S., Rosales, C., and Zimmerman, N.: Integrating Low-cost Sensor Systems and Networks to Enhance Air Quality Applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21629, https://doi.org/10.5194/egusphere-egu25-21629, 2025.

EGU25-3546 | ECS | Posters on site | HS1.2.2

Innovative Lagrangian Radiosonde Clusters for ABL Observations 

Shahbozbek Abdunabiev, Niccolo' Gallino, and Daniela Tordella

We present a novel method to track fluctuations in the atmospheric boundary layer (ABL) using a cluster of mini-radiosondes. Each radiosonde is lightweight, expendable and carried by biodegradable balloons. This system collects statistics of turbulence fluctuations in the ABL and warm clouds within it. The first operational prototype of the radiosonde cluster developed at POLITO was tested in several field campaigns from November 2022 to September 2024. These campaigns, which included six cluster launch experiments, were conducted in collaboration with CNR-INRIM, MET-OFFICE, NCAS, ARPA Piemonte, ARPA-FVG, and OAvdA (see Fig. 1). The system provides critical insights for modeling ABL dynamics and dispersion, a major source of uncertainty in climate and meteorological simulations [1].

Figure 1: In-field experiments with the radiosonde cluster network. LoRa P2P radio transmission, 12 km range, 868 MHz, 0.2 Hz data acquisition frequency. Left: radiosonde trajectories. Middle: vertical profiles of temperature and mean Brunt-Vaisala frequency from 3 radiosondes. The purple color indicates positive temperature gradients, while green indicates negative ones. Right: wind speed, magnetic field, and acceleration fluctuation spectra. A) Alpine environment, St. Barthelemy, Aosta, Italy, November 2023. B) Rural near-maritime Atlantic coast, Chilbolton, UK, July 2023, WESCON campaign. C) Subalpine region, Udine, Italy, June 2024. D) Rural near-maritime Atlantic coast, Chilbolton, UK, September 2024. Ground-level wind speeds: A: 1 m/s, B: 17 m/s, C: 0.5 m/s, D: 10 m/s.

Each radiosonde is a radioprobe board [1, 2] mounted on a biodegradable balloon [3] filled with a helium-air mixture, allowing a float time of several hours. It measures air temperature, pressure, humidity, and four vector quantities (position, velocity, acceleration, and Earth's magnetic field) along each trajectory (Fig. 1). Passive tracking of multiphase cloud parcels provides a multi-point view of flow structures. Recent experiments have explored turbulent dispersion analysis using a distance neighbor graph algorithm [4], addressing aspects of atmospheric turbulence not previously measured in field observations. The system can advance models for cloud microphysics and turbulence schemes for atmospheric tracer dispersion [5]. Our methodology uses high-frequency atmospheric data and improves understanding of turbulence. This enables advances in cloud modeling, weather prediction, and climate simulation. The biodegradable balloon has a volume of ~40 liters and weighs ~18 grams. Optimizing the size and weight of the circuit board (halving both dimensions) will reduce the balloon volume by 30%, allowing for simultaneous deployment of swarms of ~100 mini-radiosondes. The future radioprobe will have sensors for VOCs, greenhouse gases, and UV radiation integrated into the PCB to expand its use cases. An energy harvesting module will extend the lifetime of the probe.

1. Abdunabiev S. et al., Measurement 224, 113879 (2024)

2. Paredes et al., Sensors 21, 1351 (2021)

3. Basso et al., Mat. Chem. Phys. 253, 123411 (2020)

4. Richardson, Proc. R. Soc. Lond. A 110, 709 (1926)

5. Mirza et al., Q. J. R. Meteorol. Soc. 150, 761 (2024)

How to cite: Abdunabiev, S., Gallino, N., and Tordella, D.: Innovative Lagrangian Radiosonde Clusters for ABL Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3546, https://doi.org/10.5194/egusphere-egu25-3546, 2025.

EGU25-3756 | Posters on site | HS1.2.2 | Highlight

Sampling spores and microorganisms in the stratosphere 

Jérôme Kasparian, Sara Leoni, Océane Devisme, Maxime Hervo, Gonzague Romanens, and Katia Gindro

Spores are the survival and dissemination units of fungi. Many are designed for optimal airborne dispersal while maintaining long-term survival. Depending on the chemical and structural nature of their walls, they are highly resistant to extreme temperatures and UV radiation. For example, Botrytis cinerea conidia stored dry at -80°C are still able to germinate after more than 20 years in storage. Given their anemochorous nature and resistance to abiotic factors, it would therefore be possible for spores of pathogenic fungi to be aeroported through the stratosphere. However, little is known about the spread of pathogenic fungi in high-altitude airspace.

 

In order to investigate the presence of fungal spores in the stratosphere and explore the diversity of viable and non-cultivable fungi, we designed a low-cost sampling device capable of sampling particles in the stratosphere. It consists in a sealed polystyrene box with two ports on the top and bottom sides, allowing air circulation. A rotating arm sampler spins in the resulting airflow, with four sticks coated with petroleum jelly. The opening of the ports is controlled by mobile covers driven by servomotors, managed by an Arduino Uno microcontroller connected to a high-pressure pressure sensor. Moreover, an on-board radiosonde continuously transmits GPS position, relative humidity, and temperature data. An internal camera captures the opening, closing, and sampling processes during the desired altitude segment. Additionally, a control box, that never opens during flight,  monitors potential contamination below the stratosphere.

 

Both the measurement and control boxes are sterilized under UV-C, sealed and attached to a meteorologic radiosonding balloon. Upon reaching an altitude of 12,000 meters, the covers open, and airborne particles are collected. Once the balloon bursts (at around 35,000 m; -63°C), a parachute deploys during the descent, and the cover closes at 12,000 meters.  The prompt recovery of the sample at landing is assisted by a specifically dedicated mobile app, that extrapolates the descent trajectory and guides the crew to the expected landing location.

 

Five test flights between October 2023 and June 2024 up to 35,000 meters altitude, allowed us to optimize and validate the device, the sampling conditions, and the sample recovery procedures and analysis. The collected samples were both cultured on fungal medium and prepared for deep DNA sequencing. The control box remained sterile, confirming the absence of contamination. Furthermore, several species of cultivable fungi were identified in the sample, demonstrating the viability of spores despite low pressure and temperature, while the DNA sequencing revealed the presence of many species, including exotic ones.

 

This setup opens the way to routine monitoring of stratospheric airborne fungi spores and other biological aerosols, in view of a better understanding of their dispersal and survival.

How to cite: Kasparian, J., Leoni, S., Devisme, O., Hervo, M., Romanens, G., and Gindro, K.: Sampling spores and microorganisms in the stratosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3756, https://doi.org/10.5194/egusphere-egu25-3756, 2025.

EGU25-12080 | Posters on site | HS1.2.2

Cryoegg, Cryowurst and Hydrobean: wireless instruments for glaciology and hydrology 

Michael Prior-Jones, Hawkins Jonathan, Lisa Craw, Elizabeth A Bagshaw, Christine F Dow, Allan Mason-Jones, Hashem Alnader, Elena von Benzon, Luke Copland, Dorthe Dahl-Jensen, Brittany Main, Josh James, Stephen Livingstone, Sarah Mann, Matthew Peacey, Rupert Perkins, and Sophia M Rahn

Observations of conditions within and beneath the ice of glaciers and ice sheets are required to better constrain models of glacier dynamics and provide more reliable forecasts of how ice responds to a changing climate. We have developed and deployed two wireless instruments intended to provide long-term observations of englacial and subglacial environments.  A third instrument has been developed for use in streams and rivers – this may be used in either glacial or temperate environments.

Cryoegg is a spherical instrument deployed in subglacial channels via boreholes, or in moulins. It measures temperature, water pressure and electrical conductivity and provides data live by radio link through the ice to a receiver on the surface. The spherical shape allows it to travel within water channels and report on conditions within the hydrological system. We demonstrate how it has provided 5 months of data from within a glacier moulin in west Greenland, and that the radio link can operate through 2,500m of ice in north-east Greenland.

Cryowurst is a cylindrical instrument deployed in a borehole and measures both subglacial hydrological parameters (water pressure, temperature and electrical conductivity) but also its tilt and orientation change as the ice moves. It also reports wirelessly to a datalogger on the glacier surface. It has provided 5 months of data during a deployment in Yukon, Canada.

Hydrobean is an instrument intended for citizen scientists studying streams and small rivers in temporate regions. It shares some common technology with the two cryospheric instruments. Hydrobean consists of a hemispherical unit deployed on the river bed, which sends data by radio link to a data logger on the bank. It measures water pressure, water temperature and electrical conductivity and is intended to help identify pollution events (which may raise both the temperature and electrical conductivity of the water). Hydrobean has been tested in the River Usk in Wales and the river Dart in south-west England. We also intend to deploy Hydrobean in supraglacial streams during future glaciological fieldwork.

The data loggers which receive the data from all three wireless instruments store the data locally but can also forward data to a web portal using cellular or satellite links. This has allowed us to closely monitor and retrieve data in close to real time and reduces the risk of data loss from equipment damage in a harsh environment.

How to cite: Prior-Jones, M., Jonathan, H., Craw, L., Bagshaw, E. A., Dow, C. F., Mason-Jones, A., Alnader, H., von Benzon, E., Copland, L., Dahl-Jensen, D., Main, B., James, J., Livingstone, S., Mann, S., Peacey, M., Perkins, R., and Rahn, S. M.: Cryoegg, Cryowurst and Hydrobean: wireless instruments for glaciology and hydrology, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12080, https://doi.org/10.5194/egusphere-egu25-12080, 2025.

EGU25-13702 | ECS | Posters on site | HS1.2.2

SPYCE: A Multi-Modal Rodent Monitoring Device for Enhanced Detection, Monitoring, and Behavior Analysis 

Chirag Padubidri, Ioannis Louloudakis, Ioannis Daliakopoulos, Sukru Esin, and Andreas Kamilaris

Rodents pose a significant threat to agriculture, causing extensive damage to crops, infrastructure, and ecosystem health. This pressing issue necessitates innovative, sustainable management solutions. SPYCE, a rodent-monitoring device (RMD), is designed to provide a flexible, adaptable solution for rodent detection, monitoring, and behavior-analysis. Developed as part of the MED4PEST project, which focuses on advancing ecologically based rodent management by reducing reliance on synthetic pest-control methods and promoting sustainable, eco-friendly farming systems tailored to the Mediterranean-region. SPYCE’s modular, customizable configuration allows users to select sensors based on operational requirements and budget constraints, emphasizing open accessibility, tailored functionality, and cost-effective deployment.


SPYCE is a T-shaped device designed for flexible deployment at greenhouse entry points and fenced agricultural fields. Its design allows rodents to enter and exit freely, facilitating precise monitoring. The T-joint structure includes a horizontal base pipe equipped with PIR sensors at each entrance to detect movement. A housing at the top of the vertical pipe contains critical sensors such as an ultrasonic sensor, ultrasonic microphone, and infrared camera oriented downward toward the T-joint, all integrated with a Raspberry-Pi. A mmWave-radar sensor monitors external movement signatures. A temperature-humidity sensor collects environmental data, while a protective top cover shields the electronics from dust and water.

The system firmware, developed in Python, supports three operational modes for various monitoring needs. In Mode-1, PIR sensors at the entrances activate the system, which waits for ultrasonic-sensor confirmation to initiate data collection. In Mode-2, the ultrasonic sensor detects motion at the central joint, directly triggering data acquisition. In Mode-3, the infrared camera operates continuously, detecting motion through background changes and activating other sensors when a rodent is detected. Across all modes, temperature-humidity data are recorded at regular intervals. Additionally, separate code records movement signatures using the mmWave radar. SPYCE’s modular design adapts to diverse operational requirements while maintaining accuracy and reliability in data collection. Furthermore, SPYCE is open-source, with hardware designs, scripts, and implementation details available on GitHub (https://github.com/superworld-cyens/MED4PEST), enabling researchers and practitioners to replicate and customize SPYCE for rodent monitoring.

SPYCE is currently deployed at pilot sites in Greece and Turkey, actively collecting rodent-activity data. This data will serve as the foundation for developing a multi-modal deep-learning model capable of detecting, counting, and analyzing rodent behavior with high precision. Additionally, multi-modal anomaly-detection techniques will investigate behavioral changes in rodents under EBRM and non-EBRM conditions, providing valuable insights. These pilot deployments will validate SPYCE’s potential as an effective tool for assessing EBRM strategies. This work can also extend to broader rodent-management applications, including population estimation, behavioral analysis, and ecological monitoring.

Funding: This work is part of MED4PEST, funded under the PRIMA Programme, an Art.185 initiative co-funded by Horizon-2020, the EU’s Research and Innovation Programme. Additional funding was provided by the General Secretariat for Research and Innovation, Greece; the Scientific and Technological Research Council of Turkey; the EU Horizon-2020 Research and Innovation Programme (grant No. 739578); and the Government of the Republic of Cyprus through the Directorate General for European Programmes, Coordination, and Development.

How to cite: Padubidri, C., Louloudakis, I., Daliakopoulos, I., Esin, S., and Kamilaris, A.: SPYCE: A Multi-Modal Rodent Monitoring Device for Enhanced Detection, Monitoring, and Behavior Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13702, https://doi.org/10.5194/egusphere-egu25-13702, 2025.

EGU25-14559 | ECS | Posters on site | HS1.2.2

The Open Digital Environmental Lab 

Elad Levintal, Elyasaf Freiman, Thi Thuc Nguyen, Devi Orozco, Tom Norman, Robel Kahsu, and Ariel Altman

The development of new affordable sensors, and the ability to log high-resolution data for long periods of time can potentially revolutionize environmental sciences. Collecting high-resolution spatiotemporal data requires sensor grids that are often costly and not necessarily modular enough to fit a specific experimental objective. These are limiting factors that can be solved using open-source hardware. In our Open Digital Environmental Lab, we develop and integrate complex sensor arrays into our research that simultaneously measure multiple parameters, such as water content and CO2  and O2  concentrations. We rely on integrating IoT (Internet of Things) concepts and aim to meet not only our current research goals, but also to enable new capabilities at a fraction of traditional sensor costs but with similar accuracy. Our vision is that open-source sensors will: (1) “Democratize science” by reducing cost limitations, and (2) Be game-changers for measuring environmental parameters with the ability to capture process-related heterogeneity. At the conference, we will present various projects, ranging from lab-oriented devices to field networks for real-time monitoring of soil and river parameters that allow new modeling and mechanistic understandings.

How to cite: Levintal, E., Freiman, E., Nguyen, T. T., Orozco, D., Norman, T., Kahsu, R., and Altman, A.: The Open Digital Environmental Lab, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14559, https://doi.org/10.5194/egusphere-egu25-14559, 2025.

EGU25-18431 | Posters on site | HS1.2.2

Open Hardware in the UK Floods and Droughts Research Infrastructure (FDRI) 

Wouter Buytaert, Alejandro Dussaillant, and Will Veness

The UK Floods and Droughts Research Infrastructure (FDRI) is a £38 million investment from the UK Government to support transformative research and applications on flood and drought resilience. The infrastructure will consist of a combination of in-situ monitoring infrastructure, an overarching digital infrastructure to support telemetry, analytics, and data integration, and an extensive portfolio of capacity development, training and community building activities.

FDRI aims to be a state-of-the-art infrastructure that supports transformative research. This means that innovation sits at the heart of the infrastructure – both technological innovation using novel and emerging technologies, but also social innovation to explore novel arrangements for data collection, analysis, and knowledge co-production.

Open hardware provides unprecedented opportunities to support such innovation, not only as a source of new sensing and data processing technologies and setups, but also as a catalyst for engaging makers, inventors, entrepeneurs, citizen scientist and other innovation communities in FDRI.

Here we give an overview of the vision and implementation strategy of FDRI, as well as the specific opportunities for engagement, from early experimentation and prototyping to contributing to designing for cost-effectiveness, accuracy, robustness, longevity and long-term sustainability.

How to cite: Buytaert, W., Dussaillant, A., and Veness, W.: Open Hardware in the UK Floods and Droughts Research Infrastructure (FDRI), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18431, https://doi.org/10.5194/egusphere-egu25-18431, 2025.

EGU25-18763 | ECS | Posters on site | HS1.2.2

Automated wetting of a fiber-optic cable for forest evaporation partitioning 

Gijs Vis and Miriam Coenders-Gerrits

Measuring evaporation through Bowen ratios requires measuring a wet and a dry air temperature, something that is challenging to reliably accomplish in outdoor field conditions. In the context of forest evaporation, the desire to estimate Bowen ratios as a function of height (e.g., to partition evaporation above and below the canopy) adds another dimension of complexity to this measurement challenge.

As part of the Ruijsdael Observatory in the Loobos, Netherlands, we aim to continuously measure evaporation throughout a forest profile, using a dry and a wetted fiber-optic table along a 40 m tower to measure temperature profiles using Distributed Temperature Sensing (DTS). Previous studies have used continuous pumping with relatively large flow rates to ensure wetness, but this is not feasible for long term installations because of large water volume requirements.

In this contribution a smart and open-source solution for keeping a wet temperature wet and a dry temperature dry over a 40 m profile is presented. Two peristaltic pumps are regulated using two microcontrollers that modulate the pumping rate along different environmental conditions. For instance, no pumping could be needed at nighttime since there is negligible evaporation and pumping is stopped at low temperatures to prevent frost damage. A capacitive method is presented to attempt to quantify wetness, tank levels are monitored, and solutions for recycling water to limit the water volume requirements are introduced. Microcontrollers are connected to WiFi to enable convenient monitoring from the office.

With this contribution we hope to contribute to generalized solutions to measure evaporation or, in general, to inspire on methods about how to keep hydrological sensors wet or dry.

How to cite: Vis, G. and Coenders-Gerrits, M.: Automated wetting of a fiber-optic cable for forest evaporation partitioning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18763, https://doi.org/10.5194/egusphere-egu25-18763, 2025.

EGU25-19559 | ECS | Posters on site | HS1.2.2

Signal Transmission from the Water Surface for Plastic Pollution Tracking 

Marc Schneiter, Rolf Hut, and Erik Van Sebille

We use surface drifters to sample individual traces of floating macro plastic. These in-situ measurements provide input for the development of Lagrangian simulations to analyze both the dispersion patterns, and the physical transport processes of the plastic. An important component of drifters is the transmission of data directly from the water surface. This is challenging both due to the remoteness of the locations where the transmissions take place, and due to the dynamical movement of the water, which impedes signal transmission. For this reason, expensive satellite modems are often used, with careful design considerations that make the communication possible. The aims of our current research project are twofold: We want to test established and alternative terrestrial communication technologies at tens of kilometers from shore, and extend the knowledge about these data transmissions in challenging environments. This is done with a custom waterproof instrument that can be deployed and kept next to a research vessel. The instrument contains transition modems for satellite, cellular and LoRa communication. We present the construction of the instrument and results of a recent measurement campaign in the North Sea, off the Dutch coast.

How to cite: Schneiter, M., Hut, R., and Van Sebille, E.: Signal Transmission from the Water Surface for Plastic Pollution Tracking, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19559, https://doi.org/10.5194/egusphere-egu25-19559, 2025.

EGU25-2495 | Posters on site | AS5.11

Examining the effect of horizontal gradients in trace gas distributions during the intercomparison campaign CINDI-3 

Steffen Ziegler, Janis Pukite, Robert Gilke, Simona Ripperger-Lukosiunaite, Bianca Lauster, Lucas Reischmann, Sebastian Donner, and Thomas Wagner

The third Cabauw intercomparison of DOAS-type instruments (CINDI-3) campaign took place at the CESAR measurement site near Cabauw, Netherlands in June 2024. Stationary DOAS instruments were supported by mobile platforms: cars, a bike and an airplane mapped the horizontal distribution of trace gases in the regions around Rotterdam and Cabauw. In this work, we combine the information gained from all mobile platforms to obtain the horizontal distribution of nitrogen dioxide (NO2). During the campaign additional MAX-DOAS instruments were set up along the main viewing azimuth direction to investigate the retrieval of horizontal gradients from MAX-DOAS instruments using a tomographic approach. Here, we present NO2 maps obtained from the mobile measurements, the differences between the stationary instruments and the resulting implications for the tomographic approach.

How to cite: Ziegler, S., Pukite, J., Gilke, R., Ripperger-Lukosiunaite, S., Lauster, B., Reischmann, L., Donner, S., and Wagner, T.: Examining the effect of horizontal gradients in trace gas distributions during the intercomparison campaign CINDI-3, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2495, https://doi.org/10.5194/egusphere-egu25-2495, 2025.

Retrieving the vertical distribution of tropospheric Ozone (O3) based on ground-based Multi-AXis Differential Optical Absorption Spectroscopy (MAX-DOAS) observations presents challenges due to the interference of stratospheric O3 absorption. A Convolutional Neural Networks (CNN) method is proposed for retrieving the vertical distribution of tropospheric O3 based on ground-based MAX-DOAS observations. This method circumvents the issue of stratospheric O3 absorption interference when obtaining tropospheric O3 profiles by using CNN to extract features from MAX-DOAS spectral segments, enabling the retrieval of tropospheric O3 profiles. The core optimizations of this method are reflected in the following three aspects: (1) Enhancement of MAX-DOAS spectral features and establishment of a dataset with multiple features. To improve the feature extraction capability of the CNN model, mathematical methods are employed to enhance the features of the 320-340 nm spectral segments, which exhibit strong absorption characteristics for O₃. Additional datasets of various sensitive factors are incorporated to improve model inversion accuracy. The Z-Score normalization method is applied to unify dimensions and expedite model convergence, addressing inversion errors resulting from disparate dataset dimensions; (2) Constructing a PCA-F_Regression-SVR hybrid model to screen the optimal ancillary dataset for modeling. Principal Component Analysis (PCA) is utilized to reduce the dimensionality of all sensitive factors. A combination of Support Vector Regression (SVR) and the F_Regression function comprehensively evaluates and screens features sensitive to the tropospheric O₃ profiles retrieval. These features include profiles of temperature, specific humidity, fraction of cloud cover, eastward and northward winds, SO₂, NO₂, HCHO, as well as seasonal and temporal features; (3) The CNN inversion model is developed to extract the enhanced features from MAX-DOAS spectral segments and sensitive factors, enabling the retrieval of tropospheric O3 profiles. Aiming to minimize the loss function of the Mean Absolute Percentage Error (MAPE), the hyperparameters of the CNN inversion model are determined through cross-validation. The enhanced MAX-DOAS spectral features, along with sensitive factors, are used as the model inputs. The EAC4-CNEMC hybrid O3 profiles serve as the model outputs, resulting in a decrease in MAPE from 26% to 19%. The CNN inversion model is applied to independently retrieve tropospheric O3 profiles, and effectively reproduced the O3 profiles of the EAC4 dataset, exhibiting a Gaussian-like vertical distribution with peaks mainly around 950 hPa, and Absolute Percentage Errors (APEs) are generally controlled below 20%. In conclusion, leveraging MAX-DOAS spectra enables the retrieval of tropospheric O3 vertical distribution through the established CNN inversion model.

How to cite: Wang, Z., Tian, X., Xie, P., and Xu, J.: A Convolutional Neural Networks Method for Tropospheric Ozone Vertical Distribution Retrieval from Multi-AXis Differential Optical Absorption Spectroscopy Measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3930, https://doi.org/10.5194/egusphere-egu25-3930, 2025.

Bromine oxides (BrO) play a critical role in ozone depletion and boundary layer chemistry. During the spring-summer period of 2024 (May 1 to June 15), Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) measurements were conducted in Hangzhou Bay Area, China, to observe the presence of BrO, aerosols, and other trace gases (NO₂, HCHO, etc.). The average BrO volume mixing ratio (VMR) during the observation period was 2.14 ppt, increasing to 4.24 ppt during pollution episodes. High concentrations of BrO were primarily observed in the boundary layer at altitudes of 1.5–2.5 km, while other trace gases are mainly concentrated between 0-1 km near the surface. BrO concentrations tended to peak during the morning hours (7:00 am–10:00 am local time), showing a clear correlation with aerosol variations, indicating significant photochemical activation. A anti-correlation was observed between BrO and ozone (O₃), revealing a bromine-mediated O₃ depletion mechanism.

Furthermore, the overall pollutant concentration in June was higher than in May, and this change is closely related to seasonal meteorological factors, particularly variations in wind direction and temperature, which are considered the main factors influencing BrO levels.

Validation conducted during the CINDI-3 campaign demonstrated the high reliability of MAX-DOAS measurements, confirming the robustness of the MAX-DOAS technique for monitoring coastal air quality. These findings enhance our understanding of BrO dynamics in coastal regions and their impact on atmospheric chemistry.

How to cite: Lv, C., Li, A., and Hu, Z.: Observations of BrO and other trace gases in typical regions of China based on MAX-DOAS network, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4556, https://doi.org/10.5194/egusphere-egu25-4556, 2025.

EGU25-4660 | ECS | Orals | AS5.11

Trace gas and aerosol profile measurements from MAX-DOAS in South Korea during ASIA-AQ 

Hyeong-Ahn Kwon, Soi Ahn, Jan-Lukas Tirpitz, Alessandro Franchin, Jason St Clair, Pawan Gupta, Elena Lind, Jhoon Kim, and Ukkyo Jeong

The Airborne and Satellite Investigation of Asian Air Quality (ASIA-AQ) campaign was conducted from February to ­March 2024 to investigate air quality in Asia. One of the primary scientific objectives of the ASIA-AQ campaign was satellite validation and interpretation, especially for the Geostationary Environment Monitoring Spectrometer (GEMS) products. To achieve this goal, nitrogen dioxide (NO2), formaldehyde (HCHO), aerosols, and other trace gases were measured using airborne and ground-based instruments. Here, we present trace gas and aerosol profile measurements from the ground-based Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) SkySpec instruments in South Korea during ASIA-AQ. We use the RAPSODI (Retrieval of Atmospheric Parameters from Spectroscopic Observations using DOAS Instruments) algorithm to retrieve profiles from MAX-DOAS measurements. The NO2 surface concentrations retrieved from MAX-DOAS are in good agreement with in-situ measurements, showing correlation coefficients of 0.63 (north direction) and 0.88 (south direction), but with negative biases of –48% and –15%, respectively. In comparison with airborne in-situ measurements, MAX-DOAS NO2 concentrations below 1 km are lower than those measured by in-situ instruments (NASA GSFC CANOE and NCAR NOx and O3 Chemiluminescence) onboard NASA’s DC-8 aircraft. These negative biases in comparison with surface and aircraft measurements are influenced by the heterogeneity of NO2 concentrations due to the differing locations of MAX-DOAS and in-situ instruments. Aerosol optical depths (AODs) derived from MAX-DOAS are well correlated with those from the Aerosol Robotic Network (AERONET). Using these MAX-DOAS measurements, we validate GEMS NO2 and AOD products. GEMS NO2 version 3 products reduce positive biases occurring in the version 2 products but remain lower than those from MAX-DOAS NO2 products. GEMS AOD products are in good agreement with AERONET and MAX-DOAS products.

How to cite: Kwon, H.-A., Ahn, S., Tirpitz, J.-L., Franchin, A., St Clair, J., Gupta, P., Lind, E., Kim, J., and Jeong, U.: Trace gas and aerosol profile measurements from MAX-DOAS in South Korea during ASIA-AQ, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4660, https://doi.org/10.5194/egusphere-egu25-4660, 2025.

EGU25-6583 | Posters on site | AS5.11

Estimation of tropospheric water vapor using differential attenuation at microwaves and comparison with other measurements 

Luca Facheris, Fabrizio Argenti, Fabrizio Cuccoli, Ugo Cortesi, Samuele Del Bianco, Francesco Montomoli, Marco Gai, Massimo Baldi, Flavio Barbara, Andrea Donati, Elisa Castelli, Enzo Papandrea, Andre' Achilli, Maurizio Busetto, Francescopiero Calzolari, Samantha Melani, Massimo Viti, Alberto Ortolani, Andrea Antonini, and Luca Rovai and the Team of the University of Pisa, Dept. of Civil and Industrial Engineering, Pisa, Italy

Measuring water vapor (WV) in the troposphere, where nearly all atmospheric WV is concentrated, is critical for understanding atmospheric composition and dynamics comprehensively. A particularly challenging issue is conducting systematic WV measurements in the lower troposphere (approximately 5–6 km) on a global scale, as this would significantly enhance both climate modeling and numerical weather prediction (NWP) capabilities over short time scales.

Based on theoretical studies conducted for the European Space Agency (ESA), some of the authors proposed an innovative approach - the Normalized Differential Spectral Attenuation (NDSA) - capable of retrieving integrated water vapor (IWV) from attenuation measurements taken in the 17–21 GHz frequency band along microwave links crossing the troposphere. The NDSA technique relies on estimating a parameter, called spectral sensitivity (S), which quantifies the differential attenuation experienced by a pair of tone signals separated by a fractional bandwidth of less than 2%. It has been demonstrated that S can be directly converted into IWV using a linear relationship. Through the aforementioned ESA studies, the authors have also shown that the NDSA method can successfully estimate WV vapor from space by utilizing sets of co-rotating or counter-rotating Low Earth Orbit (LEO) satellites.

Recently, the Italian Space Agency supported the SATCROSS project, aimed at demonstrating the feasibility of a future space mission and to develop a prototype for NDSA measurements along terrestrial links operating at 19 GHz. A critical step toward consolidating progress and advancing the realization of a space-based measurement project using the NDSA approach is the performance analysis of the IWV estimates provided by prototype instruments. This includes validating those estimates by comparing them with results from other sensors and techniques, which was the objective of a four-month measurement campaign conducted from July to November 2024.

In this work, we present the main results of the campaign, conducted in a ground-to-ground configuration, designed to compare IWV measurements from the NDSA prototype instrument with those obtained using the Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) technique. MAX-DOAS retrieves IWV in the visible spectral range, specifically at about 445 nm. The independent optical device used in this study was configured to observe the same air volume as the NDSA instrument. Measurements were made along a link connecting the meteorological station "Giorgio Fea," located at the rural site of St. Pietro Capofiume, Bologna, 10 m above sea level, to the WMO/GAW (World Meteorological Organization/Global Atmosphere Watch) Climate Observatory “Ottavio Vittori” at Mount Cimone, 2165 m above sea level.

The link length is 91 km, with no physical obstacles interposed. In addition to MAX-DOAS data, measurements were also acquired and processed from radiosondes, hygrometers, GNSS (Global Navigation Satellite Systems) and a tethered balloon.

The research activities presented in this work were carried out with contribution of the Next Generation EU funds within the National Recovery and Resilience Plan (PNRR), Mission 4-Education and Research, Component C2-From Research to Business (M4C2), Investment Line 1.1-Fund for the National research program and projects of significant national interest (PRIN), Project 2022JJJYTE -``Measuring tropospheric water vapor through the Normalized Differential Spectral Attenuation (NDSA) technique''

How to cite: Facheris, L., Argenti, F., Cuccoli, F., Cortesi, U., Del Bianco, S., Montomoli, F., Gai, M., Baldi, M., Barbara, F., Donati, A., Castelli, E., Papandrea, E., Achilli, A., Busetto, M., Calzolari, F., Melani, S., Viti, M., Ortolani, A., Antonini, A., and Rovai, L. and the Team of the University of Pisa, Dept. of Civil and Industrial Engineering, Pisa, Italy: Estimation of tropospheric water vapor using differential attenuation at microwaves and comparison with other measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6583, https://doi.org/10.5194/egusphere-egu25-6583, 2025.

EGU25-7208 | Orals | AS5.11

Aerosol vertical profile measurements using passive radiometric measurements 

Elena Lind, Marcos Herreras-Giralda, Masahiro Momoi, Thomas Eck, Aliakxandr Sinyuk, and Oleg Dubovik

Aerosol vertical profiles in the lowest 1-2 km of the atmosphere are not very well studied due to technology limitations (e.g. LIDARs) and air space restrictions (e.g. manned and unmanned aircrafts). This study investigates sensitivity of the radiance measurements in UV-VIS part of the spectrum to the aerosol profiles from the standard columnar almucantar and direct sun measurements combined with low elevation sky scanning (from the horizon to zenith direction).

GRASP algorithm is used to simulate scattered sky radiances and conduct aerosol profile inversions. Radiance measurements are conducted by the sun-sky radiometer at subset of standard AERONET wavelengths (340, 380, 440, 500, 675, 870). AErosol RObotic NETwork (AERONET) is a network of sun-sky-moon photometers that measure solar radiation at 9 wavelength bands (centered at 340, 380, 440, 500, 675, 870, 937, 1020, 1640 nm, 2-25 nm FWHM filter transmission). The main AERONET products are columnar aerosol optical depth, Angstrom exponent (from direct sun measurements), single scattering albedo and size distribution (from Almucantar and hybrid scans). The additional products investigated in this study are volume density and aerosol extinction coefficient profiles. This study evaluates CIMEL 318T pointing accuracy (near horizon), effect of surface albedo on the inversions and ability of radiance measurements to invert vertical profiles both from synthetic and real measurements at 2 locations: Greenbelt, MD and Rotterdam, NL.

How to cite: Lind, E., Herreras-Giralda, M., Momoi, M., Eck, T., Sinyuk, A., and Dubovik, O.: Aerosol vertical profile measurements using passive radiometric measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7208, https://doi.org/10.5194/egusphere-egu25-7208, 2025.

EGU25-7990 | ECS | Posters on site | AS5.11

UV-Vis remote sensing of shipping emissions and atmospheric pollutants at the North Sea 

Gytha Mettepenningen, Caroline Fayt, Frederik Tack, Cato Van Doorne, Lars Jacobs, Sophie Berkenbosch, Aurélien Aubry, Filip Desmet, Martine De Mazière, and Michel Van Roozendael

Ship emissions comprise up to 15% of global transport pollution. To regulate this pollution, Nitrogen Emission Control Area (NECA) and Sulphur Emission Control Area (SECA) zones have been introduced in the North Sea, which define a threshold for shipping emissions of respectively NOx and SOx. The current method of control of these regulations in the Belgian North Sea uses an aircraft equipped with sniffers to fly through the plume. As this is an intensive method, only a limited number of ships can be evaluated. The Ship Emission Monitoring by Passive Absorption Spectroscopy (SEMPAS) project develops a UV-Visible Differential Optical Absorption Spectroscopy (DOAS) instrument to permanently monitor ships from a Belgian offshore windfarm and to complement the aircraft-based measurements.

As part of a preparatory stage prior to its deployment on an off-shore wind farm conversion platform, the imaging DOAS system with a field of view of 0.2x3 degrees is installed in the port of Zeebrugge at the Belgian North Sea coast. From there, it measures slant columns of both SO2 and NO2 in the UV at a spectral resolution of 0.4 nm, as proxies for NOx and SOx. The aim of the project is to use these measurements to quantify shipping emission factors, to check for compliance of the emission factors as defined in NECA and SECA zones. Additionally, the instrument will be used as a MAX-DOAS system, to study the variability of atmospheric trace gases and contribute to the validation of satellite measurements in a marine environment.

To enhance sensitivity of the ship plume, an image recognition AI-based algorithm identifies ships on a camera accompanying the instrument. By accurate pointing of the system, ships can be tracked actively in their course. This enlarges the time in view of the instrument and as such increases the measurement signal. With this technique, we explore whether the sensitivity required for monitoring of the current strict regulations can be reached.

The poster addresses the installation of the instrument and finetuning of the ship-tracking algorithm. We discuss the identification of shipping emissions based on the DOAS technique and show first results.

How to cite: Mettepenningen, G., Fayt, C., Tack, F., Van Doorne, C., Jacobs, L., Berkenbosch, S., Aubry, A., Desmet, F., De Mazière, M., and Van Roozendael, M.: UV-Vis remote sensing of shipping emissions and atmospheric pollutants at the North Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7990, https://doi.org/10.5194/egusphere-egu25-7990, 2025.

EGU25-8524 | ECS | Posters on site | AS5.11

Comparison of Cloud Classification methods 

Robert Gilke, Lucas Reischmann, Steffen Ziegler, Elaheh Bastani, Sebastian Donner, Simona Ripperger-Lukošiūnaitė, Stefan Kinne, Vinod Kumar, and Thomas Wagner

Cloud properties play an important role in the evaluation and interpretation of Multi-AXis Differential Optical Absorption Spectroscopy (MAX-DOAS) measurements. Clouds strongly influence the length of atmospheric light paths, and are thus important for deriving the aerosol optical depth (AOD) and vertical column density (VCD) of trace gases from MAX-DOAS measurements. As such, information about the cloud properties is important to interpret the data.
This study focuses on comparing three methods to derive information on cloud properties which can be run in conjunction with MAX-DOAS measurements, allowing for a more comprehensive characterisation of cloud effects: a ceilometer, an infrared camera and information derived from the MAX-DOAS measurements themselves. All instruments are located at the Max-Planck Institute for Chemistry in Mainz, Germany. We investigate, under which cloud conditions MAX-DOAS inversions might yield reasonable results and under which cloud conditions inversion results have large uncertainties. One focus of our investigation is the effect of cloud altitude on the MAX-DOAS retrievals.

How to cite: Gilke, R., Reischmann, L., Ziegler, S., Bastani, E., Donner, S., Ripperger-Lukošiūnaitė, S., Kinne, S., Kumar, V., and Wagner, T.: Comparison of Cloud Classification methods, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8524, https://doi.org/10.5194/egusphere-egu25-8524, 2025.

EGU25-8855 | ECS | Posters on site | AS5.11

Horizontal Gradients of Aerosols and Trace Gases: Insights from MAX-DOAS Measurements in Mainz 

Elaheh Bastani, Steffen Ziegler, Robert Gilke, Sebastian Donner, Steffen Beirle, and Thomas Wagner

This study investigates horizontal gradients of aerosols and trace gases using a rooftop-mounted MAX-DOAS instrument located at the Max Planck Institute for Chemistry in Mainz. Horizontal inhomogeneities, especially in urban areas or near strong emission sources, can significantly affect the accuracy of MAX-DOAS profile retrievals, as these typically assume horizontally homogeneous atmospheric conditions. The experimental setup allows for measurements in two azimuthal directions (possibly extended to 4 azimuth directions), focusing on gradients between opposing directions (180° apart). By analyzing the retrieved differential slant column densities (dSCDs) at low elevation angles horizontal gradients will be identified and quantified. They are compared to the temporal variability of the dSCDs at high elevation angles, taking into account also wind speed and direction. From the MAX-DOAS observations also trace gas and aerosol profiles are retrieved.  Retrievals under conditions of strong and weak gradients are contrasted to assess their influence on the atmospheric profile retrievals. As a result, we give recommendations which situations might be favorable or not favorable for MAX-DOAS profile inversions, particularly relevant in areas influenced by complex emission sources.

How to cite: Bastani, E., Ziegler, S., Gilke, R., Donner, S., Beirle, S., and Wagner, T.: Horizontal Gradients of Aerosols and Trace Gases: Insights from MAX-DOAS Measurements in Mainz, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8855, https://doi.org/10.5194/egusphere-egu25-8855, 2025.

EGU25-10395 | ECS | Posters on site | AS5.11

Feasibility of volcanic CO2, HF, and HCl remote sensing measurements using Fourier-transform infrared spectrometry in scattered sunlight geometry 

Moritz Sindram, Tobias Dieter Schmitt, Nicole Bobrowski, Ralph Kleinschek, Benedikt Löw, Lukas Weis, and André Butz

Carbon dioxide (CO2) is usually the second most abundant gas in volcanic plumes. Its early dissolution from rising magmas can allow insights into magmatic source regions and subsurface volcanic structures. Due to its chemical inertness, CO2 measurements are particularly valuable for studying plume chemistry using CO2 as a mixing tracer. The also relatively abundant volcanic gases, hydrogen fluoride (HF) and hydrogen chloride (HCl), dissolve at shallower depths. Their measurements, along with those of other halogen and sulfur compounds, complement the insights into the volcanic system and plume composition. Continuous measurements of volcanic CO2, HF, and HCl emissions could therefore enhance our understanding of volcanic activity and improve hazard assessment.

Remote sensing measurements of volcanic gases in the shortwave infrared (SWIR) spectral range offer the potential for automated, continuous data acquisition of the above-mentioned gases. However, current studies are limited to direct sun geometry which restricts measurement opportunities to cases where the volcanic plume is positioned between the instrument and the sun. Therefore, we investigated the feasibility of operating a portable Fourier-transform infrared (FT-IR) spectrometer in scattered sunlight geometry for CO2, HF, and HCl measurements. This approach would enable greater measurement flexibility but introduces the challenge of a significantly weaker light source in the SWIR spectral range.

We present a framework for calculating the required averaging time to achieve specific detection limits for CO2, HF, and HCl based on instrument parameters (e.g. detector specifications, field of view, beam diameter). For Bruker’s EM27/SUN instrument, modified and optimized for scattered sunlight measurements, we estimate an averaging time of several hours to detect CO2 slant column densities at levels typical for Mt. Etna (Italy). This makes the setup studied highly impractical for volcanic CO2 measurements. In contrast, the required averaging times for HF and HCl detection are of the order of 10 minutes.

These results underscore the utility of performance calculations in guiding instrument design while highlighting the challenges associated with scattered sunlight being a weak light source in the SWIR spectral range.

How to cite: Sindram, M., Schmitt, T. D., Bobrowski, N., Kleinschek, R., Löw, B., Weis, L., and Butz, A.: Feasibility of volcanic CO2, HF, and HCl remote sensing measurements using Fourier-transform infrared spectrometry in scattered sunlight geometry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10395, https://doi.org/10.5194/egusphere-egu25-10395, 2025.

EGU25-12396 | Orals | AS5.11

MAX-DOAS observations of spatial variability of NO2 in Athens 

Andreas Richter, Kai Krause, Myrto Gratsea, André Seyler, Folkard Wittrock, John P. Burrows, and Hartmut Bösch

Nitrogen dioxide is a key pollutant in the troposphere. Most of its sources are anthropogenic and linked to the burning of fossil fuels, but wildfires, lightning and soil emissions also contribute to the overall NOx (NO + NO2) loading.

Using passive remote sensing in the UV and visible spectral range, NO2 columns can be retrieved with both ground-based MAX-DOAS and satellite instruments. As a result of the multitude of sources and the short atmospheric lifetime of NOx, spatial and temporal variability of NO2 in the troposphere is large. This variability complicates the interpretation of satellite measurements, which integrate over relatively large areas, and also has to be considered in satellite validation.

The University of Bremen, in collaboration with the National Observatory of Athens (NOA), has been operating a MAX-DOAS instrument at the NOA premises on Penteli Hill in the northeast of Athens since 2012. The measurement location allows for several viewing directions over the city of Athens and towards less polluted background regions. The measurements are, therefore, ideal to investigate an inhomogeneous NO2 distribution and its impact on satellite validation.

Using the data from the MAX-DOAS instrument, the temporal and spatial variability of NO2 is evaluated, and simple parametrisations are developed and tested to characterise the degree of variability. Comparing the results from variations in time and those in azimuth direction, interesting similarities and differences are found. The derived inhomogeneity parameters can be used to classify situations where the MAX-DOAS data is particularly well suited for satellite validation and which days should be excluded from such evaluations.

How to cite: Richter, A., Krause, K., Gratsea, M., Seyler, A., Wittrock, F., Burrows, J. P., and Bösch, H.: MAX-DOAS observations of spatial variability of NO2 in Athens, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12396, https://doi.org/10.5194/egusphere-egu25-12396, 2025.

EGU25-13109 | Orals | AS5.11

Overview of the Third Cabauw Intercomparison of UV-Vis DOAS instruments (CINDI-3) 

Michel Van Roozendael, Arnoud Apituley, Karin Kreher, Diego Alves Gouveia, Alexander Cede, Udo Friess, Martina M. Friedrich, Elena Spinei Lind, Alexis Merlaud, Ankie Piters, Andreas Richter, Frederik Tack, Thomas Wagner, and Steffen Ziegler

The third Cabauw Intercomparison of UV-Vis DOAS Instruments (CINDI-3) took place from May 21st to the 24th of June 2024 at the Cabauw Experimental Site for Atmospheric Research (CESAR), a semi-rural observational facility managed by the Dutch Meteorological Institute close to the cities of Rotterdam and Utrecht in the Netherlands. Its main objective was to intercompare UV-Vis MAX-DOAS instrument types targeting nitrogen dioxide, ozone, aerosols and several other reactive gases such as formaldehyde, glyoxal and BrO, with the aim to assess their performance under a range of observational conditions, and to progress towards the understanding of the measurement technique through community effort. The stationary UV-Vis observations were complemented with a range of additional measurements including ozone and aerosol lidars, NO2 and ozone sondes, long-path DOAS and in-situ instruments. Furthermore, mobile instruments were deployed around Cabauw, De Bilt and Rotterdam during selected days with favourable weather conditions using cars and bikes as well as a small research aircraft, to provide a more complete picture of the distribution of pollutants from the industrial and urbanised area around Rotterdam.

CINDI-3 was organised under the umbrella of NDACC and the European Research Infrastructure ACTRIS with additional support from ESA and NASA. In total, over 100 researchers from 16 countries participated to the field deployment. In this presentation, we provide an overview of the main on-site activities and we highlight first results of the post-campaign data evaluation with a focus on the ACTRIS/NDACC semi-blind intercomparison exercise and activities under way in various working groups addressing calibration, trace gas and aerosol vertical profiling, spectral retrieval improvements, and the joint exploitation of mobile and airborne measurements.

How to cite: Van Roozendael, M., Apituley, A., Kreher, K., Alves Gouveia, D., Cede, A., Friess, U., Friedrich, M. M., Spinei Lind, E., Merlaud, A., Piters, A., Richter, A., Tack, F., Wagner, T., and Ziegler, S.: Overview of the Third Cabauw Intercomparison of UV-Vis DOAS instruments (CINDI-3), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13109, https://doi.org/10.5194/egusphere-egu25-13109, 2025.

EGU25-14161 | ECS | Orals | AS5.11

Surface NO2 Derived from Pandora Column Measurements in Toronto and Detroit-Windsor 

Darby Bates, Ramina Alwarda, Kimberly Strong, Xiaoyi Zhao, Vitali Fioletov, Sum Chi Lee, and Yushan Su

Atmospheric trace gases near the Earth’s surface can have important human and environmental health impacts. In particular, the trace gas nitrogen dioxide (NO2), which is commonly emitted by traffic, biomass burning, and industrial sources, can be a major threat to human respiratory health, leading to increased rates of asthma, lung cancer, and overall mortality. In the Greater Toronto Area (GTA) and in the Detroit-Windsor Area (DWA), NO2 and other trace gases are being measured by ground-based Pandora UV-visible spectrometers that are part of the Pandonia Global Network. We present NO2 surface volume mixing ratios derived from Pandora direct sun total column measurements to monitor air quality in these two urban areas. The conversion method uses three inputs in addition to the Pandora total columns: (1) the stratospheric NO2 column from the Ozone Monitoring Instrument (OMI), (2) the free troposphere NO2 column from the GEOS-Chem chemical transport model, and (3) the ratio of NO2 surface volume mixing ratio to planetary boundary layer column from Environment and Climate Change Canada’s regional air quality forecast model, Global Environmental Multi-scale-Modelling Air quality and Chemistry (GEM-MACH). The derived estimates of surface NO2 are compared with in situ measurements, and their level of agreement is assessed for dependence on meteorological conditions, including wind speed and direction, temperature, and boundary layer height. The mean bias between the derived estimates and in situ measurements ranges from -1.0 ppbv to -2.6 ppbv. This bias has been found to vary with boundary layer height, so a method to account for this dependence has been developed to improve the results. This presentation will provide an overview of this column-to-surface conversion method, a summary of results for each site in the GTA and DWA, and an outline of plans toward using this approach to improve and validate satellite estimates of surface NO2.

How to cite: Bates, D., Alwarda, R., Strong, K., Zhao, X., Fioletov, V., Lee, S. C., and Su, Y.: Surface NO2 Derived from Pandora Column Measurements in Toronto and Detroit-Windsor, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14161, https://doi.org/10.5194/egusphere-egu25-14161, 2025.

EGU25-15190 | Posters on site | AS5.11

GEMS L2 data validation during ASIA-AQ campaign 

Hyunkee Hong, Ukkyo Jeong, Limseok Chang, Hanlim Lee, Serin Kim, and Donghee Kim

To understand the dominant chemical mechanisms driving wintertime secondary PM2.5 formation and to validate GEMS L2 data, the National Institute of Environmental Research and the National Aeronautics and Space Administration (NASA) conducted the Airborne and Satellite Investigation of Asian Air Quality (ASIA-AQ) campaign across four Asian countries (Korea, the Philippines, Malaysia, and Thailand) from February to March 2024. During this campaign, we deployed six Pandora instruments, two AQProfilers, and five AERONET systems around the Seoul metropolitan region. Using these ground-based instruments, we retrieved nitrogen dioxide, ozone and formaldehyde vertical column densities, as well as aerosol properties, and compared the results with GEMS L2 products. A comparison of NO₂ observed by GEMS with that from ground-based remote sensing instruments revealed a correlation coefficient of over 0.6 across all regions. Additionally, a performance comparison of GEMS NO₂ across different versions showed that the overestimation observed in GEMS v2 results was improved in the v4 results. Furthermore, we also compared results from NASA GeoTASO with those from GEMS during this period.

How to cite: Hong, H., Jeong, U., Chang, L., Lee, H., Kim, S., and Kim, D.: GEMS L2 data validation during ASIA-AQ campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15190, https://doi.org/10.5194/egusphere-egu25-15190, 2025.

EGU25-16039 | ECS | Orals | AS5.11

CINDI-3 glyoxal intercomparison 

Kai Krause, Andreas Richter, Simon Bittner, Udo Frieß, Steffen Ziegler, Robert Gilke, Thomas Wagner, Sebastian Donner, Robert Ryan, Elisa Castelli, André Achilli, Paolo Pettinari, Erna Frins, Roberto Barragán, Gaia Pinardi, Michel van Roozendael, Hugo Wai Leung Mak, Hyeong-Ahn Kwon, Kimberly Strong, Ramina Alwarda, Kevin Joshy, Darby Bates, Chaonan Lv, Ang Li, Zhaokun Hu, Dimitris Karagkiozidis, Alkis Bais, Cristina Prados-Roman, Monica Navarro-Comas, Olga Puentedura Rodriguez, Margarita Yela Gonzalez, Ka Lok Chan, Cheng Liu, Shiyao Tang, Chengzhi Xing, Xiangguang Ji, Johannes Lampel, and Hartmut Bösch

Glyoxal (CHOCHO) is an intermediate product of the oxidation of volatile organic compounds (VOCs) and has anthropogenic, biogenic and pyrogenic sources. It is an indicator of formation of secondary organic aerosols in the atmosphere and plays a role in the photochemical reactions of ozone in the troposphere. Additionally, at high concentrations glyoxal is harmful for humans. The lifetime of glyoxal in the atmosphere is short (a few hours) and it is removed from the atmosphere by photolysis, oxidation by OH, and deposition. Due to the different sources and short lifetime of glyoxal, its abundance in the atmosphere can vary between several parts per trillion (ppt) e.g., in remote parts of the oceans, to parts per billion (ppb) in the presence of strong sources, like biomass burning, industrial processes, fossil fuel combustion or over tropical rainforest regions.

Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) instruments are capable of measuring glyoxal, but the retrieval is difficult due to its relatively weak absorption compared to other trace gases. Therefore, further improvements of current MAX-DOAS glyoxal retrievals are needed.

Glyoxal was one of the target species during CINDI-3, the third semi-blind intercomparison campaign of UV-Vis DOAS instruments in Cabauw, The Netherlands. Based on the large scatter of the measurements among the participating instruments, it was identified as one of the more challenging trace gases to retrieve. A task group has been formed to develop a common and improved approach to retrieve glyoxal, using the data collected by several instruments and institutes during the campaign, and applying different retrieval software. In this study, we present the initial glyoxal retrievals from the campaign, and outline the development of improved retrieval settings, which we want to propose as a new standard for future glyoxal measurements.

How to cite: Krause, K., Richter, A., Bittner, S., Frieß, U., Ziegler, S., Gilke, R., Wagner, T., Donner, S., Ryan, R., Castelli, E., Achilli, A., Pettinari, P., Frins, E., Barragán, R., Pinardi, G., van Roozendael, M., Mak, H. W. L., Kwon, H.-A., Strong, K., Alwarda, R., Joshy, K., Bates, D., Lv, C., Li, A., Hu, Z., Karagkiozidis, D., Bais, A., Prados-Roman, C., Navarro-Comas, M., Puentedura Rodriguez, O., Yela Gonzalez, M., Chan, K. L., Liu, C., Tang, S., Xing, C., Ji, X., Lampel, J., and Bösch, H.: CINDI-3 glyoxal intercomparison, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16039, https://doi.org/10.5194/egusphere-egu25-16039, 2025.

EGU25-16804 | ECS | Posters on site | AS5.11

AOTF-based NO2 camera: CINDI-3 results 

Cedric Busschots, Pierre Gramme, Emmanuel Dekemper, Gytha Mettepenningen, Alexis Merlaud, and Michel Van Roozendael

In recent years, a novel type of passive remote sensing instrument has been under development at the Royal Belgian Institute for Space Aeronomy (BIRA-IASB). The aim of this instrument, known as the NO2 camera, is to improve the spatio-temporal resolution of ground-based-observed NO2 slant column densities which are usually measured by azimuth and elevation scanning spectrometers. As a result, NO2 emitted in polluted environments can be better characterized. 


The working principle of this so-called NO2 camera is based on an acousto-optical tunable filter (AOTF), a crystal whose lattice is modulated by a propagating acoustic wave. The elasto-optic effect taking place in the crystal allows the selection of any single wavelength from the incoming light bundle with a spectral resolution between 0.6 and 0.8 nm. Within this imaging optical setup, the AOTF records spectral images of a scene (in this case the atmosphere) in successive wavelengths. For our instrument, a crystal operating in the 435 to 455 nm band was selected. The resulting hyperspectral images are then processed using the DOAS technique.


Between May 21 and June 24, 2024, the BIRA-IASB NO2 camera participated in the Third Cabauw INtercomparison of DOAS-type Instruments (CINDI-3), providing an opportunity to benchmark its performance against state-of-the-art instruments. During the campaign, the camera operated in close synchronization with other participating DOAS-type instruments. Additionally, outside of the prescribed campaign protocol, the camera sampled the NO2 field in the direction of Rotterdam and Utrecht. We present the first results of these measurements, discuss their performance and highlight preliminary findings.

How to cite: Busschots, C., Gramme, P., Dekemper, E., Mettepenningen, G., Merlaud, A., and Van Roozendael, M.: AOTF-based NO2 camera: CINDI-3 results, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16804, https://doi.org/10.5194/egusphere-egu25-16804, 2025.

EGU25-16842 | ECS | Posters on site | AS5.11

Intercomparison of MAX-DOAS, FTIR and direct sun DOAS HCHO retrievals in Xianghe (China) 

Gaia Pinardi, Michel Van Roozendael, Martina M. Friedrich, Bavo Langerock, Corinne Vigouroux, Isabelle De Smedt, François Hendrick, Ting Wang, Pucai Wang, Minqiang Zhou, and Steffen Beirle

MAX-DOAS, direct sun DOAS and FTIR measurements are increasingly used as fiducial reference measurements (FRM) for the validation of HCHO satellite observations. Understanding their strengths and limitations, and assessing their consistency is therefore crucial to produce robust and consolidated validation results. So far, only a few studies have explored the complementarity between MAX-DOAS and FTIR HCHO measurements.

In the present study, we take benefit of MAX-DOAS and FTIR instruments being simultaneously operated at the Xianghe station (39.75° N, 116.96° E, approximately 55 km southeast of Beijing) to compare HCHO vertical columns (VCDs) retrieved from both instruments during one full year in a site under the influence of strong VOC emissions from biogenic and anthropogenic origins. In addition to its standard MAX-DOAS geometry, the IAP/BIRA instrument also provides regular direct sun measurements suitable for comparison with FTIR solar absorption data. The two direct sun measurements, in the UV and IR, show an excellent agreement and form a reliable HCHO VCD reference.

We investigate results obtained using MMF and MAPA MAX-DOAS algorithms and their combined use within the FRM4DOAS centralized processing facility, assessing the agreement reached with respect to the direct sun reference data and investigate the reasons for the observed differences. A good correlation (~0.96) but with a systematic under-estimation of about -20% is found for all the MAX-DOAS approaches. We explore whether this discrepancy can be understood by the known lack of sensitivity of MAX-DOAS measurements in the free-troposphere, above 4 km of altitude. Changing the MMF a-priori profiles to monthly averaged profiles coming from CAMS or TM5 models shows a reduction of the bias of 10 to 15% with respect to the direct sun reference data. By further considering the MAX-DOAS and FTIR respective vertical sensitivities through application of their averaging kernels, we reduce the remaining bias to -2% for the different MAX-DOAS datasets.

How to cite: Pinardi, G., Van Roozendael, M., Friedrich, M. M., Langerock, B., Vigouroux, C., De Smedt, I., Hendrick, F., Wang, T., Wang, P., Zhou, M., and Beirle, S.: Intercomparison of MAX-DOAS, FTIR and direct sun DOAS HCHO retrievals in Xianghe (China), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16842, https://doi.org/10.5194/egusphere-egu25-16842, 2025.

EGU25-17520 | Posters on site | AS5.11

Airborne Measurements of NO2, HONO, and HCHO Emissions from Canadian Wildfires and the Oil Industry 

Alexis Merlaud, Frederik Tack, Nicolas Theys, Michel Van Roozendael, Farrer Owlsey-Brown, Callum Middleton, Will Maslanka, Toby Wainwright, Luke Richardson-Foulger, Martin Wooster, and Dirk Schuettemeyer


In August 2023 and September 2024, King’s College London (KCL) conducted airborne campaigns in Canada to investigate emissions from wildfires and the oil industry. The British Antarctic Survey (BAS) Twin Otter aircraft was equipped with an array of in-situ and remote sensing instruments, including the SWING instrument. Developed by the Royal Belgian Institute for Space Aeronomy (BIRA-IASB), SWING is a compact whiskbroom imager designed to map trace gases that absorb in the UV-visible spectral range (300-550 nm).

We present the integration of SWING into the BAS Twin Otter and its operations during the airborne campaigns. On 14 and 19 August 2023, the aircraft sampled the plume from a wildfire in Ontario, measuring NO2. On 11 September 2024, the aircraft flew over a fire in Saskatchewan, where we detected NO2 together with HCHO and HONO. In the same 2024 campaign, we observed NO2 emissions from flaring at oil facilities in Alberta: Fort McMurray, Fort McKay, and from chemical plants near Edmonton. These airborne measurements are compared with satellite-based air quality data from TROPOMI and TEMPO, for which we are close to the northern edge of the field of view. We also estimate the HONO/NO2 from the fire and investigate how such measurements may help to quantify the emissions from wildfires and from natural gas flaring. 

How to cite: Merlaud, A., Tack, F., Theys, N., Van Roozendael, M., Owlsey-Brown, F., Middleton, C., Maslanka, W., Wainwright, T., Richardson-Foulger, L., Wooster, M., and Schuettemeyer, D.: Airborne Measurements of NO2, HONO, and HCHO Emissions from Canadian Wildfires and the Oil Industry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17520, https://doi.org/10.5194/egusphere-egu25-17520, 2025.

EGU25-18486 | Orals | AS5.11

Urban Pollution Monitoring with the AOTF-based NO2 Camera: Validation Campaign in Rome 

Pierre Gramme, Cedric Busschots, Emmanuel Dekemper, Stefano Casadio, Paolo Pettinari, Elisa Castelli, and André Achilli

The NO2 camera is a novel instrument, developed by the Royal Belgian Institute for Space Aeronomy. It consists in an AOTF-based hyperspectral imager and DOAS-based data processing algorithms enabling to measure the differential slant column densities (dSCD) of NO2 along each pixel’s line of sight.  

In the framework of IDEAS-QA4EO, a measurement campaign was organized in an urban environment at the BAQUNIN supersite in Rome, in March 2024. The NO2 camera was compared to two collocated reference NO2 remote sensing instruments: a PANDORA spectrometer from LuftBlick deployed at the BAQUNIN supersite, and a SkySpec-2D Max-DOAS spectrometer from Airyx, operated by CNR Isac. All instruments were synchronized to a common pointing schedule, measuring the dSCD at low elevation angles (-2° to +10°) and around 4 agreed azimuth angles with unobstructed view of the horizon. The PANDORA and SkySpec obtained their measurements by scanning in elevation and in azimuth, up to 10° left and right of each reference direction. To the best of our knowledge, this is the first time these two instruments have been compared in this manner. All dSCDs were computed using as fixed reference a zenith spectrum acquired by each instrument at the same specified time. Three days of synchronized data are available for comparison, with clear to partly cloudy weather conditions. 

A total of 156 hyperspectral cubes were obtained by the NO2 camera during the synchronized periods. Several local enhancements were captured by the NO2 camera, showing the inhomogeneity of the Roman NO2 field. In total, about 6000 dSCD values from the NO2 camera were compared to the SkySpec, and about 700 values were compared to the PANDORA. The tolerance margins for inclusion in the comparison were set to 5 minutes for the acquisition time, and to 0.1° for the azimuth and elevation. Overlaying the retrievals from all instruments showed how the additional visual context captured by the camera may help understanding the location of NO2 emission sources. This can be seen in the example image below, as well as the good qualitative agreement between the instruments. More formally for the whole campaign, the measured dSCDs ranged from -2e16 to +22e16 molecules/cm². The disagreement between the camera and the SkySpec (resp. PANDORA) has mean -0.7e16 (resp. -0.01e16) molecules/ cm² and standard deviation 1.6e16 (resp 2.5e16) molecules/cm² for all points above the horizon. 

We will present more details on the campaign setup and results. 

 


How to cite: Gramme, P., Busschots, C., Dekemper, E., Casadio, S., Pettinari, P., Castelli, E., and Achilli, A.: Urban Pollution Monitoring with the AOTF-based NO2 Camera: Validation Campaign in Rome, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18486, https://doi.org/10.5194/egusphere-egu25-18486, 2025.

EGU25-19146 | Posters on site | AS5.11

SEICOR - Ship Emission Inspection with Calibration-free Optical Remote sensing 

Folkard Wittrock, Andre Daubinet, Christoph Haisch, Kai Krause, Denis Pöhler, Jan Poppe, Andreas Richter, Markus Rieker, and Stefan Schmitt

Ship emissions of particles, SO2 and NOx (the sum of NO and NO2) are a significant contribution to air pollution, in particular in coastal areas and close to busy in-land shipping routes. Therefore, national and international regulations have been put in place to limit emissions and thereby minimize the impact of shipping on air quality. However, the monitoring of ship emissions is challenging, and so far, no automated systems are operational for systematic surveillance of compliance with regulations.

Active Optical Remote Sensing is one possible approach to measuring ship emissions. Briefly, a light source is set-up on one side of a river or port, and a reflector on the other side. The light path is positioned in such a way that the emission plume of passing ships is sampled. Using spectroscopic methods, the amounts of trace gases in the plume can be determined. With Automated Identification System (AIS) data, the plumes can be assigned to individual ships. The advantage of remote sensing over in-situ observations is a reduced dependence on wind direction, increasing the rate of successful measurements. A second important advantage is the self-calibration of the method, facilitating long-term autonomous operation without the need for on-site calibration.

This method has been successfully used in the UV/Vis wavelength range to detect SO2 and NO2 at the location of Wedel, a small town at the river Elbe, 10 km downriver of the port of Hamburg, Germany. Based on these data and a plume model, emission rates of NOx and SO2 in g s-1 could be determined with an automated method (Krause et al., 2021).

While this type of measurement is useful in determining emission rates, often specific emissions relative to the amount of fuel burnt are of interest. This is particularly the case for SO2, where regulations are based on limits for the fuel sulphur content. In order to extend the method to these quantities, an additional channel measuring CO2 in the IR part of the spectrum has to be added to the instrument. The CO2 can be used as a proxy of the amount of fuel burnt, and thereby also the energy used. In addition, direct NO measurements in the IR would reduce the uncertainties of the NOx measurements.

The SEICOR project aims at developing such a system for automated long-term surveillance of emissions from ships and other, similar sources. It is based on the experience and tools from the measurements performed in Wedel. The new system will cover all parts of the measurements, from the instrument over data analysis of the emission factors to direct generation of warnings in case of high emissions. An automated reporting to the authorities, port operators and / or ship owners is planned. Here we present technical details and first results of the measurement and validation campaign which takes place in April 2025 in Wedel at the river Elbe.

The SEICOR project is funded by the Federal Ministry for economic affairs and climate action.

How to cite: Wittrock, F., Daubinet, A., Haisch, C., Krause, K., Pöhler, D., Poppe, J., Richter, A., Rieker, M., and Schmitt, S.: SEICOR - Ship Emission Inspection with Calibration-free Optical Remote sensing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19146, https://doi.org/10.5194/egusphere-egu25-19146, 2025.

EGU25-19196 | ECS | Posters on site | AS5.11

First retrievals of aerosol microphysical properties from polarisation-sensitive MAX-DOAS measurements 

Kirsten Blohm, Udo Frieß, Elena S. Lind, Jan-Lukas Tirpitz, and Ulrich Platt

Characterizing the microphysical properties of aerosols is crucial for understanding their impacts on air quality, climate change, and human health. In this study, we present a novel approach for determining aerosol size distribution, refractive index, and single-scattering albedo using a polarization-sensitive Multi-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) instrument. Extracting the polarimetric state of the atmosphere through polarization-sensitive solar almucantar measurements improves the accuracy and resolution of the derived aerosol parameters.

The RAPSODI retrieval algorithm employs a bimodal size distribution within the aerosol Mie model, coupled with the VLIDORT vector forward model and inversion via the optimal estimation method. Measurements conducted at the IUP Heidelberg during the second half of 2024 provided a dataset of polarization-dependent differential slant column densities (dSCD) and differential slant optical thicknesses (dSOT), which were analyzed to derive the vertical distribution of NO₂, aerosol extinction, and the microphysical properties of the aerosols. Good correlation between measured and modeled dSCDs and dSOTs is achieved, providing confidence that microphysical aerosol parameters can be retrieved reliably with our novel remote sensing method.

The results demonstrate that the polarization-sensitive MAX-DOAS technique improves the information content for characterizing spherical aerosol particles. For validation, we performed comparisons with a co-located CIMEL sun-photometer from the Aerosol Robotic Network (AERONET). This study highlights the potential of polarization-sensitive MAX-DOAS in advancing both data collection and our understanding of aerosol properties.

How to cite: Blohm, K., Frieß, U., Lind, E. S., Tirpitz, J.-L., and Platt, U.: First retrievals of aerosol microphysical properties from polarisation-sensitive MAX-DOAS measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19196, https://doi.org/10.5194/egusphere-egu25-19196, 2025.

The emergence of spectral imaging concepts that are both sensitive and snapshot open up new perspectives in response to major challenges, such as air quality monitoring and greenhouse gas emissions. The imSPOC concept (Brevet n° : FR16/56162) is a static Fourier transform spectral imager. Its compactness, robustness, and lightness make it a promising concept for measuring greenhouse gases from space or assessing air quality. This concept is based on a paradigm shift, as it enables the acquisition of only portions of interferograms [1]. Consequently, it is necessary to transfer optimal estimation algorithms into the interferogram space: since spectral radiances cannot be retrieved from partial interferograms, it is necessary to directly fit measured interferograms to simulated interferograms in order to retrieve total columns from its measurements. Within the framework of the European Space Carbon Observatory project (H2020 SCARBO), it was demonstrated that the relevant geophysical information (CO2 column for one camera and CH4 column for the other) is indeed present in the identified interferogram portions [2]. In parallel, two prototypes were built, one dedicated to CO2 and the other to CH4. To improve the designs of these cameras, a co-design code allowing the propagation of instrumental errors to gas columns is essential.


In this work, we demonstrate how an approach based on the Cramer-Rao Lower Bound enabled a sensitivity increase of more than a factor of two for both the CO2 and CH4 cameras. The design of such instrumentation relies on both the selection of shape and spectral position of the filter, as well as the properties of the interferometric plate, which is an array of Fabry-Perot interferometers. We evaluated the impact of several design parameters: (i) the selection of the spectral shape and position of the filter, (ii) the selection of the maximum optical path difference, and (iii) the Fabry-Perot finesse of the interferometer, which enhances discrimination between different gas signatures. Further refinement of the design was achieved using the MEDOC retrieval model, incorporating additional parameters such as engraving depths, leading to an optimized repartition of the available optical path difference acquired by the spectral imaging sensor. Finally, the newl design for the CO2 camera was benchmarked against the earlier CO2 SCARBO design. The study found that the CO2 scale factor random error has been reduced by more than a factor of two. Furthermore, performance has become more consistent across varying incidence angles. Additionally, correlation between albedo and retrieved CO2 products has also decreased. This work received funding from the European Union’s H2020 research and innovation program under grant agreements No 769032 (SCARBO) and No 101135301 (SCARBOn).

[1] S. Gousset, L. Croizé, E. Le Coarer et al., “NanoCarb hyperspectral sensor: on performance optimization and analysis for greenhouse gas monitoring from a constellation of small satellites”, CEAS Space J., 11, pages 507–524 (2019)

[2] M. Dogniaux, C. Crevoisier, et al., “The Space CARBon Observatory (SCARBO) concept: Assessment of XCO2 and XCH 4 retrieval performance”. Atmospheric Measurement Techniques Discussions, 1-38.

How to cite: Croize, L. and Ferrec, Y.: Impact of the design of a spectral imager based on partially sampled interferograms on the retrieve products, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21657, https://doi.org/10.5194/egusphere-egu25-21657, 2025.

EGU25-2908 | Posters on site | AS5.12

Models, In situ, and Remote sensing of Aerosols (MIRA)International Working Group: An Update 

Charles Trepte, Vassilis Amiridis, Elisabeth Andrews, Maria Obiminda Cambaliza, Mian Chin, Claudia Di Biagio, Oleg Dubovik, Sang Woo Kim, Eleni Marinou, Jens Redemann, Masanori Saito, Gregory Schuster, Ping Yang, and Luke Ziemba

There is a natural partitioning of scientific interest amongst three focus areas of aerosol research: modeling, in situ measurements, and remote sensing observations. The community benefits when these groups interact, with overall benefits towards advancing our understanding of climate, weather, and air quality. To this end, MIRA seeks to foster international collaborations across disciplines and regional boundaries and offers a complementary association with established international working groups.  A special focus is on collaborations that help advance operational services and products for near term benefits to society. 

Within the present framework, MIRA has identified four initial focus areas. One effort advances knowledge of the aerosol lidar ratio for different aerosol compositions and locations to improve backscatter lidar retrievals from satellites and ground-based instruments. Another effort seeks to improve aerosol and cloud optical parameters used by climate and radiative transfer models. A third effort focuses on harmonizing aerosol assimilation models with satellite measurement retrievals, and a fourth interest seeks to develop retrievals of aerosol particulate matter from satellite remote sensing measurements.

The grassroots working group was formed in 2021 and includes more than 250 participants with representatives from Asia, Europe, Australia, and North America. A newsletter is published quarterly and webinars are held bi-monthly on topics of interest to the members.  A workshop in Greece is also planned for June 2025.  The presentation will provide an overview on MIRA and ways for the community to engage.

How to cite: Trepte, C., Amiridis, V., Andrews, E., Cambaliza, M. O., Chin, M., Di Biagio, C., Dubovik, O., Kim, S. W., Marinou, E., Redemann, J., Saito, M., Schuster, G., Yang, P., and Ziemba, L.: Models, In situ, and Remote sensing of Aerosols (MIRA)International Working Group: An Update, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2908, https://doi.org/10.5194/egusphere-egu25-2908, 2025.

EGU25-3192 | ECS | Posters on site | AS5.12

Drone-Based Aerosol Profiling: Calibration Using an In Situ Multi-Sensor System 

Ilya Bruchkouski, Artur Szkop, Jakub Wink, and Aleksander Pietruczuk

Aerosol profile measurements are crucial for validating and improving atmospheric models, satellite remote sensing algorithms, and regional dynamic models that consider the fine vertical structure of boundary layer dynamics. The boundary layer, where the atmosphere interacts with the Earth’s surface, is characterized by rapid changes in temperature, humidity, and turbulence. These thermodynamic conditions influence aerosols’ hygroscopic growth, mixing, and their roles in global atmospheric processes such as cloud formation and radiative transfer. The applying of unmanned aerial vehicles (UAVs) offers the potential for high-resolution in-situ profiling of aerosol parameters, enabling the capture of fine-scale variations often missed by traditional methods such as satellite observations or ground-based instruments. Since aerosols in the boundary layer are rarely uniformly distributed, their spatial heterogeneity significantly impacts air quality assessments and pollutant transport modeling.

In coastal regions, aerosol PM measurements are particularly valuable for evaluating the combined effects of marine and terrestrial emissions on air quality, ecosystem health, and nearby populations. However, deploying rotary UAVs as air quality sensor platforms presents unique challenges. The turbulence generated by UAV propellers can alter the sampled aerosol concentrations, potentially leading to quasi-systematic inaccuracies. Addressing this issue requires careful calibration of UAV-based sensors in the field.

Given study presents the results of vertical aerosol profile measurements, focusing on PM1, PM2.5, and PM10 concentrations, conducted during a short measurement campaign above the sea surface near Hel (54°44'25.9" N, 18°34'02.5" E), Poland. Data were collected using an OPC-N3 sensor mounted on a UAV at altitudes ranging from 5 to 120 m. Calibration of the drone-based measurements was performed using the specially designed Integrated Aerosol Monitoring Unit (IAMU), which houses three aerosol sensors (SPS30, OPC-N3, and OPS 3330) within a single enclosure [1]. All IAMU sensors as well as drone-based sensor are sensitive to hygroscopic growth of aerosol because of the absence of sample drying. However, the calibration approach formulated in [1] allows for approximating aerosol grow factor coefficient. This assessment was supported by auxiliary observations from a nephelometer Aurora 4000, Sun photometer and meteorological station. A calibration technique is proposed for the OPC-N3 sensor, incorporating synchronous IAMU data and accounting for aerodynamic losses in the sampling inlet tubes.

  • Bruchkouski, I.; Szkop, A.; Wink, J.; Szymkowska, J.; Pietruczuk, A. Multi-Sensor Instrument for Aerosol In Situ Measurements. Atmosphere 2025, 16, 42. https://doi.org/10.3390/atmos16010042

How to cite: Bruchkouski, I., Szkop, A., Wink, J., and Pietruczuk, A.: Drone-Based Aerosol Profiling: Calibration Using an In Situ Multi-Sensor System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3192, https://doi.org/10.5194/egusphere-egu25-3192, 2025.

EGU25-3484 | Orals | AS5.12

The Mass Extinction Coefficient for Dust: challenges in the link between mass and optical properties for models, reanalyses, in-situ and satellite observations 

Claire Ryder, Natalie Ratcliffe, Alcide Zhao, Nicolas Bellouin, Laura Wilcox, Helen Dacre, Clément Bézier, Vassilis Amiridis, Eleni Marinou, Emmanouil Proestakis, Bernadett Weinzierl, Stephanie Woodward, Ben Johnson, and Anthony Jones

The latest range of CMIP6 model dust simulations shows a greater diversity than previous generations of models in terms of dust emission, deposition, burden and dust optical depth (DOD) (Zhao et al., 2022). Validation of dust models is crucial for understanding the impact of dust on climate and climate change, as well as for quantifying socio-economic and health impacts of dust.

While models (and reanalyses) mostly provide output in terms of mass, satellite observations used for model validation are optical measurements. Thus we require good knowledge of the dust mass extinction coefficient (MEC) to successfully validate our dust models. However, the MEC is intricately linked to the dust size distribution, fraction of coarse particles and composition, all of which may vary regionally, in the vertical and in time.

This presentation will provide a perspective on some recent efforts exploring the challenges in model validation relating to dust size, composition, optical depth and dust mass loading in climate models (Zhao et al., 2024; Ratcliffe et al., 2024), reanalyses (Ryder et al., 2024), space-borne lidar, space-borne optical depth and in-situ measurements, demonstrating the critical importance and uncertainty of the dust MEC.

References

Ratcliffe, N.G., Ryder, C.L., Bellouin, N., Woodward, S., Jones, A., Johnson, B., Wieland, L.-M., Dollner, M., Gasteiger, J., Weinzierl, B. Long range transport of coarse mineral dust: an evaluation of the Met Office Unified Model against aircraft observations, Atmos. Chem. Phys., 24, 12161–12181, https://doi.org/10.5194/acp-24-12161-2024, 2024.

Ryder, C.L., Bézier, C., Dacre, H., Clarkson, R., Amiridis, V., Marinou, E., Proestakis, E., Kipling, Z., Benedetti, A., Parrington, M., Rémy, S., Vaughan, M., Aircraft Engine Dust Ingestion at Global Airports, https://doi.org/10.5194/nhess-24-2263-2024, 24, 7, Natural Hazards and Earth System Science, 2024.

Zhao, A., Ryder, C.L., Wilcox, L., How well do the CMIP6 models simulate dust aerosols?, Atmos. Chem. Phys., 22, 2095–2119, https://doi.org/10.5194/acp-22-2095-2022, 2022.

Zhao, A., Wilcox, L., Ryder, C.L., The key role of atmospheric absorption in the Asian Summer Monsoon response to dust emissions in CMIP6 models, Atmos. Chem. Phys., https://doi.org/10.5194/acp-24-13385-2024, 2024.

How to cite: Ryder, C., Ratcliffe, N., Zhao, A., Bellouin, N., Wilcox, L., Dacre, H., Bézier, C., Amiridis, V., Marinou, E., Proestakis, E., Weinzierl, B., Woodward, S., Johnson, B., and Jones, A.: The Mass Extinction Coefficient for Dust: challenges in the link between mass and optical properties for models, reanalyses, in-situ and satellite observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3484, https://doi.org/10.5194/egusphere-egu25-3484, 2025.

There are 9 Fengyun (FY) meteorological satellites on the orbit to obtain the global meteorological observation data. The validation is fundamental for satellite product and the quantitative application. At present, China Meteorological Administration (CMA) maintains the huge ground-based meteorological observation network with nearly 80,000 sets of ground-based equipment spanning over 340 types to measure over 100 items of meteorological parameters. This network provides the independent means to assess the accuracy of the data products derived from the FY satellites. An operation-oriented validation system for FY-3 polar orbiting satellites has been designed and established since 2022. This system is named as the Integrated Space-Ground System for Calibration and Validation (ISGS4CV).

The objective of ISGS4CV is to assess the FY satellite products routinely and to generate the integrated dataset by data fusion as well. With the data fusion, ISGS4CV can generate the integrated dataset to better describe the digital Earth. The new dataset will inherit the advantages of the space-based measurement in spatiotemporal resolution and the ground-based measurement in high accuracy. The current CMA ground-based meteorological observation network will be selected to support ISGS4CV. For example, the surface network, the upper-air network, the new generation weather radar network, the atmospheric composition network, the ground-based remote sensing network, and the airborne observation system and field campaigns will be included.

How to cite: Zhang, P.: Chinese Integrated Meteorological Observation Network for FY Satellite Validation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4707, https://doi.org/10.5194/egusphere-egu25-4707, 2025.

In order to solve the problem of insufficient monitoring capabilities of water vapor transport (WVT) induced by low-level jets (LLJs), which restricts the improvement of regional extreme rainfall forecasting capabilities, the atmospheric water vapor as one of the key variables to monitor WVT will be synergistically estimated through ground-based, airborne and space-borne multi-platform including ground-based GNSS, microwave radiometer, lidar, radiosonde, high-altitude unmanned aerial vehicles and Fengyun satellites and so forth. The estimates of atmospheric water vapor from different platforms will be compared to clarify the advantages and disadvantages of different monitoring methods, observation error characteristics and optimal applicable conditions. The GNSS tomography method will be developed to retrieve three-dimensional water vapor distribution. The observation network and observation mode will be optimized and the technology to synergistically monitor atmospheric water vapor through multiple instruments will be developed. In addition, the methods to combine and fuse the retrievals of water vapor from multi-platform will be developed. The fusion datasets of water vapor will be established. This datasets and wind datasets provided by another program will be used to compute integrated water vapor transport induced by LLJs. To sum up, this study would be of great help to advance LLJs monitoring and improve the accuracy of regional extreme rainfall forecasts induced by LLJs.

How to cite: Liang, H., Zhang, P., Zhou, L., Zhao, P., Bu, Z., and Mao, J.: Estimating atmospheric water vapor synergistically through ground-based, airborne and space-borne observations for monitoring water vapor transport induced by low-level jets during regional extreme rainfall events, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5381, https://doi.org/10.5194/egusphere-egu25-5381, 2025.

EGU25-6160 | Orals | AS5.12

Advanced retrieval of aerosol vertical profiles using synergy of EarthCARE ATLID and passive spaceborne observations 

Anton Lopatin, Anna Gialitaki, Chong Li, Alexandra Tsekeri, Paul Tytgat, Konstantinos Rizos, Eleni Marinou, Vassilis Amiridis, Oleg Dubovik, and Edward Malina

We present the “EarthCARE ATLID and MSI Instruments Synergy for Advanced Retrieval of Aerosol Vertical Profiles” (ECAMS) project, which aims to enhance the integration of passive and active observations by combining Level 1 (L1) data from EarthCARE and various imagers. This project focuses on aerosol retrieval through the fusion of L1 observations from lidar (ATLID) and imagers on EarthCARE (MSI) and PACE (SPEXone, HARP-2). This approach, though methodologically promising, presents significant technical challenges and requires substantial resources.

Atmospheric aerosols are major drivers of climate change and have significant impacts on human health. Global information on aerosol properties is primarily obtained from space-based measurements. Passive remote sensing involves spectral observations of top-of-atmosphere reflectance at various angles, providing data on aerosol quantity, particle size and morphology, with limited sensitivity to its vertical distribution. Conversely, active lidar observations excel in detecting aerosol vertical distribution but lidar stand-alone retrievals require assumptions about aerosol size and morphology, making collocated radiometric measurements crucial for their comprehensive interpretation.

Current methods for synergetic aerosol property retrievals mainly focus on ground-based active and passive observations and do not fully leverage recent advancements in lidar technology, such as high spectral resolution lidars (HSRLs). Moreover, existing methods lack the flexibility to integrate various lidar configurations with passive measurements for space-based observations. ECAMS aims to address these limitations by developing new methods for generating global aerosol vertical distribution products with improved accuracy, aiding climate model validation. The project’s synergetic retrieval approach uses highly optimized forward models (including aerosol and surface reflectance) and the statistical estimation framework of the open-source GRASP (Generalized Retrieval of Atmosphere and Surface Properties) software.

The ECAMS framework is designed for adaptability, enabling the synergistic processing of various active and passive satellite observations across different spatial, vertical, and spectral resolutions and ranges. It serves as platform for advancing remote sensing of atmospheric and surface structures, providing a virtual laboratory for diverse remote sensing research and applications.

One of the project’s objectives is to support and complement synergy developments in the context of ESA AIRSENSE project and its studies on aerosol-cloud interactions, in collaboration with the EC CleanCloud and CERTAINTY projects. Ongoing developments and results will be presented and discussed.

How to cite: Lopatin, A., Gialitaki, A., Li, C., Tsekeri, A., Tytgat, P., Rizos, K., Marinou, E., Amiridis, V., Dubovik, O., and Malina, E.: Advanced retrieval of aerosol vertical profiles using synergy of EarthCARE ATLID and passive spaceborne observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6160, https://doi.org/10.5194/egusphere-egu25-6160, 2025.

EGU25-7503 | Posters on site | AS5.12

Tailoring TPTRS for Operational Thermodynamic Retrieval in the Complex Terrain of Korea 

Youn Choi, Kwan-Ho Kim, Yung-Lin Teng, and Yu-Chieng Liou

The Korea Meteorological Administration Weather Radar Center (WRC) has collaborated with Taiwan National Central University (NCU) and ported the multiple-Doppler radar wind field retrieval technique (WISSDOM) and thermodynamic variable retrieval technique. WISSDOM utilizes a variational method to overcome the limitations of conventional wind retrieval techniques. It determines the optimal wind vector from radial velocities of multiple weather radars through iterative calculations of control variables (horizontal and vertical wind components) to minimize the cost function of dynamic constraints. Consequently, WISSDOM produces a 3D wind field that satisfies the physical equations and reflects the influence of observational data. WRC has tuned the algorithm to suit the complex terrain of Korea, enabling real-time operation. As a next step, we aim to develop a radar wind field-based thermodynamic variable retrieval technique called the Terrain-Permitting Thermodynamic Retrieval Scheme (TPTRS). TPTRS retrieves thermodynamic variables such as pressure, temperature, and water vapor mixing ratio using a 3D wind field synthesized from multiple Doppler radars in complex terrain. To address the challenges posed by complex terrain, TPTRS applies the Immersed Boundary Method to constrain the flow of fluids on the ground and utilizes a cost function composed of momentum and thermodynamic equations. By iteratively minimizing the cost function, TPTRS retrieves significant 3D thermodynamic variables. In this study, we implemented a radar-based TPTRS algorithm suitable for the complex terrain of Korea and analyzed its results. We conducted experiments to determine the optimal number of iterations for real-time operation and obtained meaningful results with over 1000 iterations. A case study was conducted on a heavy rainfall event that occurred on 31 July 2019, analyzing the potential temperature, mixing ratio, and pressure fields. In the cross-section of the developing major precipitation system, we observed an increase in potential temperature with altitude, accompanied by high and thick mixing ratios. This aligns with the characteristics of a developing system and is considered a significant result. We plan to develop a system for retrieving thermodynamic variables across the entire Korean Peninsula in the future.

This research was supported by the " Development of radar based severe weather monitoring technology (KMA2021-03121)" of "Development of integrated application technology for Korea weather radar" project funded by the Weather Radar Center, Korea Meteorological Administration.

How to cite: Choi, Y., Kim, K.-H., Teng, Y.-L., and Liou, Y.-C.: Tailoring TPTRS for Operational Thermodynamic Retrieval in the Complex Terrain of Korea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7503, https://doi.org/10.5194/egusphere-egu25-7503, 2025.

EGU25-7797 | Posters on site | AS5.12

Estimation of Satellite-Based Air Temperature Using Land Surface Temperature 

Dahwan Shin and Sang Seo Park

Air temperature is an important parameter in both icing and fog, and thus plays a critical role in assessing the operational stability of Urban Air Mobility (UAM) during takeoff, landing, and routine operations. However, there has been relatively little research focused on directly retrieving air temperature from satellite observations. This study estimated air temperature over the Korean Peninsula in East Asia using satellite-based land surface temperature (LST). This study employed the fine-resolution LST (~100 m), which was derived from coarse-resolution temperature of the Geostationary Korea Multi-Purpose Satellite-2A (GK-2A) and Landsat 8 using Taylor series expansions and surface characteristic indices. To mitigate the atmospheric effects, the surface indices, derived from Landsat 8, included the Normalized Difference Vegetation Index (NDVI) and the Normalized Difference Moisture Index (NDMI). The fine-resolution LST was then incorporated into the surface energy balance budget equation to estimate air temperature. It is anticipated that this study will enable the derivation of high-resolution atmospheric temperatures and that obtaining these directly from satellite observations will greatly aid research on modeling fog and icing formation.

 

This work was funded by the Korea Meteorological Administration Research and Development Program under Grant RS-2024-00404042.

How to cite: Shin, D. and Park, S. S.: Estimation of Satellite-Based Air Temperature Using Land Surface Temperature, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7797, https://doi.org/10.5194/egusphere-egu25-7797, 2025.

EGU25-9642 | ECS | Orals | AS5.12

Satellite Aerosol Composition Retrieval from a Combination of three different Instruments 

Ulrike Stöffelmair, Thomas Popp, Marco Vountas, and Hartmut Bösch

The influence of aerosols on climate is determined not only by their global distribution but also by their specific composition. Knowledge of the aerosol component distribution on a global scale is important (among other factors) for the radiation balance and the hydrological cycle due to the different influence of different components on the direct and indirect aerosol effect. Ideally, the component distribution should be known globally. For this reason, we propose a novel approach to derive the components using satellite observations.  Since no single instrument can provide a comprehensive analysis, we integrate data from three satellite-based instruments with complementary information content to achieve a synergistic aerosol retrieval. Our approach utilizes measurements with varying observational characteristics, including different spectral ranges (UV, VIS, thermal IR) and viewing geometries (nadir and oblique). The instruments involved are the dual-view SLSTR (Sea and Land Surface Temperature Radiometer) aboard Sentinel 3A and 3B, the Infrared Atmospheric Sounding Interferometer (IASI), and the Global Ozone Monitoring Experiment-2 (GOME-2), both on METOP A/B/C. The data are averaged onto a common grid of 40x80 km², temporally aligned within a 60-minute window, and subjected to cloud masking.

This study aims to extract the total Aerosol Optical Depth (AOD) as well as the AOD of major aerosol components from the satellite data using an optimal estimation framework. An information content analysis showed that an upper limit of up to 22 parameters (surface albedo at different wavelengths, surface temperature, Aerosol Optical Depth (AOD) and the AOD for up to 15 different aerosol components) with their uncertainties can be retrieved out of the combined dataset depending on the aerosol amount and the surface properties. For the a priori values of the retrieval parameters, we utilize climatological data: the GOME-2 surface LER database for albedo values, which contains Lambertian-equivalent reflectivity (LER), and climatological MERRA-2 reanalysis data for AOD and aerosol composition.

This combination of instruments thus has the potential to accurately ascertain aerosol composition and with this additional information to refine our understanding of their climate impact. In this study we show first promising results of the retrieval in different scenarios. 

How to cite: Stöffelmair, U., Popp, T., Vountas, M., and Bösch, H.: Satellite Aerosol Composition Retrieval from a Combination of three different Instruments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9642, https://doi.org/10.5194/egusphere-egu25-9642, 2025.

EGU25-9959 | Posters on site | AS5.12

Multi-term LSM as methodological platform for advanced multi-sensor  remote sensor synergy  

Oleg Dubovik, Pavel Litvinov, David Fuertes, Anton Lopatin, Tatyana Lapyonok, Chong Li, and Christian Matar

The presentation discusses the Multi-term Least Square Method (LSM) as a methodological platform for realizing of the multi-instrument synergy. As discussed  by Dubovik et al. (2021), the Multi-term LSM has been used to develop complex inversion algorithms for a number of years and have been successfully applied to aerosol retrievals from diverse  satellite, ground-based and laboratory measurements. Theoretically, the approach unites the advantages of a variety of approaches and to provide transparency and flexibility in development of efficient retrievals. It provides a methodology for using multiple a priori constraints to atmospheric problems. One of the most important  practical features of the approach is that it allows for synergy processing of observations that are not fully coincident nor fully co-located. Specifically, synergy of such observation can be realized following the multi-pixel approach (Dubovik et al., 2011), when the large groups of satellite observations (pixels) are inverted simultaneously. By processing observations from multiple pixels together, the retrieval efficiently incorporates prior knowledge about the temporal and spatial variability of the retrieved parameters.

Indeed, while the  synergy of  not coincident or not co-located observation is less intuitive, it is very promising.  Whereas the fusion of co-incident multi-angular polarimeter and lidar observations is considered as efficient approach, in practice the coincidence of such observations can be limited. For example, the trajectories of currently operating EarthCARE and PACE have very limited overlaps, therefore the possible synergy product of these two satellites can only be very sparse. In contrast, the synergy of not fully coincident or co-located observations can be applied always for combining any observations from operating satellites with different trajectories. Based on our current experience such synergy, realized using multi-pixel approach, allows for substantial improvement of aerosol characterization due to two phenomena: (i) propagation of superior information about aerosol details from more sensitive observations to less sensitive, and (ii) overall increase of observations volume of the same aerosol event in different times and locations. The benefits of such synergy of non-coincident observations have been demonstrated in the framework of ESA SYREMIS project (https://www.grasp-earth.com/portfolio/syremis/), where the synergetic multi-instrument retrieval approach was developed for characterizing aerosol and surface properties using different combinations of S-3A, S-3B, S-5p, polar and HIMAWARI  geo observations. It was shown that realized methodology helped the information  from polar satellite to propagate geo retrieval and made possible the retrieval of AE and SSA for the pixel with HIMAWARI observations reasonable accuracy, while processing these observations separately does not provide these parameters. In these regards, the combined processing of PACE, EarthCARE and HIMAWARI could also be used to provide enhanced aerosol global product.

Dubovik, O., M. Herman, A. Holdak, et al., “Statistically optimized inversion algorithm for enhanced retrieval of aerosol properties from spectral multi-angle polarimetric satellite observations”, Atmos. Meas. Tech., 4, 975-1018, https://doi.org/10.5194/amt-4-975-201, 2011.

Dubovik, O., D. Fuertes, P. Litvinov, et al. , “A Comprehensive Description of Multi-Term LSM for Applying Multiple a Priori Constraints in Problems of Atmospheric Remote Sensing: GRASP Algorithm, Concept, and Ap-plications”, Front. Remote Sens. 2:706851. doi: 10.3389/frsen.2021.706851, 2021

How to cite: Dubovik, O., Litvinov, P., Fuertes, D., Lopatin, A., Lapyonok, T., Li, C., and Matar, C.: Multi-term LSM as methodological platform for advanced multi-sensor  remote sensor synergy , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9959, https://doi.org/10.5194/egusphere-egu25-9959, 2025.

EGU25-10732 | ECS | Orals | AS5.12

Satellite retrievals of aerosol water uptake and their validation using ground-based, in-situ, and airborne campaign data 

Jasper Mens, Bastiaan van Diedenhoven, and Otto Hasekamp

Aerosols affect climate in two main ways: directly, through scattering and absorption of solar radiation, and indirectly, through affecting cloud formation and cloud properties. Combined, these effects result in a net cooling, partially offsetting the warming caused by greenhouse gases (GHGs). While there is consensus about the existence of this cooling effect, its magnitude remains uncertain. This is problematic; as anthropogenic aerosol emissions decrease, we expect the cooling effect to diminish, leading to an enhanced warming effect from GHGs in the near future. Therefore, the accuracy of future warming projections strongly depends on our understanding of aerosols.

In particular, the hygroscopicity (i.e., efficiency of water uptake) of aerosols is a poorly understood property, yet highly influential on both cloud droplet nucleation capacity and light scattering. Typically, aerosols are complex mixtures of particles which themselves are a mixture of various materials, some of which are hydrophilic, and others hydrophobic. The distribution of these species, both within and among aerosol particles, is a key factor determining the effect of water uptake. As a result, different model treatments of aerosol compositions produce widely varying radiative forcing estimates. This strongly contributes to the uncertainty on the aerosol cooling term.

Global hygroscopicity data is crucial to inform model choices and thereby improve forcing estimates, except the available data is sparse and limited. Our goal is to address this gap by compiling polarimetric satellite observations from POLDER-PARASOL (for 2006-2010) and SPEXone-PACE (2024+) into the first ever global climatology of aerosol hygroscopicity. We use the RemoTAP algorithm to retrieve the aerosol refractive index, among other properties, from the multi-angle polarimeters. Through comparison of the retrieved refractive index to the known refractive indices for dry material and of water, a volume fraction of water in the aerosol is derived.

Given the novelty of our approach, validation of the retrievals is of particular importance. First, we compare the satellite retrievals to ground-based measurements such as refractive indices derived from AERONET observations. Furthermore, to validate our method of deriving the water fraction from the refractive index in general, we compare the retrievals to aerosol water fractions derived from ground-based in-situ nephelometer measurements of particle growth in response to changes in humidity, combined with ambient relative humidity measurements.

Another fundamental pillar of this validation is the PACE-PAX campaign, which was conducted in September 2024 with the express purpose of validating PACE and EarthCARE results. The campaign involved a high-altitude aircraft serving as a direct satellite proxy, which included the SPEX airborne instrument. Furthermore, one low-altitude aircraft gathering in-situ measurements, two boats, and a glider participated in the campaign. Observation targets included AERONET stations and satellite overpasses, providing ample opportunities for intercomparison between high-altitude aircraft observations and ground-based, aircraft in-situ, and satellite measurements.

We discuss our validation strategies and results, demonstrating the accuracy and limitations of our approach

How to cite: Mens, J., van Diedenhoven, B., and Hasekamp, O.: Satellite retrievals of aerosol water uptake and their validation using ground-based, in-situ, and airborne campaign data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10732, https://doi.org/10.5194/egusphere-egu25-10732, 2025.

Mineral dust aerosol is important in the Earth system, and the correct representation of its size distribution is fundamental for shaping the current state and evolution of the climate. Despite many observational dust size data that are available in the literature, using this body of information to properly guide the development and validation of climate models and remote sensing retrievals remains challenging. In this study we collect, evaluate, harmonize, and synthesize 58 size distribution data from the past 50 years of in situ field observations with the aim of providing a consistent dataset to the community for use in constraining the representation of dust size across its life cycle.

Four levels (LEVs) of data treatment are defined, going from original data (LEV0), data interpolated and normalized on a standardized diameter grid (LEV1), and data in which original particle diameters are converted to a common geometrical definition under both spherical (LEV2a) and aspherical (LEV2b) assumptions. Size distributions are classified as emission or source (SOURCE, < 1 d from emission; number of datasets in this category N = 12), mid-range transport (MRT, 1–4 d of transport; N = 36), and long-range transport (LRT, > 4 d of transport; N = 10). The harmonized dataset shows consistent features suggesting the conservation of airborne particles with time and a decrease in the main coarse-mode diameter from a value on the order of 10 μm (in volume) for SOURCE dust to a value on the order of 1–2 μm for LRT conditions. An additional mode becomes evident below 0.4 μm for MRT and LRT dust. Data for the three levels (LEV1, LEV2a, and LEV2b) and the three categories (SOURCE, MRT, and LRT), together with statistical metrics (mean, median, 25th and 75th percentiles, and standard deviation), are publicly available and distributed on the DATA TERRA EasyData portal.

The significance of the dataset for remote sensing and modelling of mineral dust will be discussed.

 

How to cite: Formenti, P. and Di Biagio, C.: Large synthesis of in situ field measurements of the size distribution of mineral dust aerosols across their life cycles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11368, https://doi.org/10.5194/egusphere-egu25-11368, 2025.

EGU25-11446 | ECS | Orals | AS5.12

Introducing random mixtures of irregular hexahedrals and spheroids to reproduce polarimetric lidar observations of desert dust 

Anna Gialitaki, Alexandra Tsekeri, Matthew O’Callaghan, Dimitra Kouklaki, Kyriaki Papachristopoulou, Maria Kezoudi, Alkistis Papetta, Franco Marenco, Konrad Kandler, Sudharaj Aryasree, Melanie Eknayan, and Vassilis Amiridis

In this work, we present the use of random shape mixtures of irregular hexahedrals and spheroids to simulate the spectral dependence of lidar-derived dust depolarization ratio and lidar ratio in 3 wavelengths traditionally used in aerosol research: 355, 532 and 1064nm.

Vertically-resolved polarimetric remote sensing provides a comprehensive understanding of atmospheric dust properties and its’ effects on radiation, weather and climate. Optical property profiles derived from polarimetric lidar observations such as the lidar ratio (Sp) and the depolarization ratio (dp), are sensitive to the particles’ morphology. However, in order to extract particle microphysical properties from these observations, accurate modelling of dust scattering properties is required. Dust particles appear to be highly-irregular and while complex shape models have been developed to describe them (e.g. Gasteiger et al. 2011), the scattering calculations are expensive in terms of computational power, which limits their applicability.

Thus, in most cases dust particle shapes are modelled using simplified representations such as spheroids. Spheroid shape mixtures have been demonstrated to successfully reproduce the angular dependence of light scattering from dust aerosols, nevertheless deviations are observed, particularly close to backscattering angles (Dubovik et al., 2006). Recent developments show that irregular hexahedral ensembles can better reproduce the measured dust lidar-relevant properties (Saito & Yang, 2021; Saito et al., 2021), however it is still challenging to reproduce their spectral dependence.

In all cases, additional assumptions are made with respect to the distribution of the different particle shapes considered in the ensemble (i.e. a shape distribution).

Herein we explore a different pathway, using random shape mixtures of irregular hexahedrals and spheroids to simulate the spectral dependence of lidar-derived dust dp and Sp. Since the considered particle shapes are not realistic, we do not constrain the simulations with measured shape distributions, but rather allow the different particle shapes to vary randomly in the mixtures. For the simulations we utilize the MOPSMAP (Gasteiger & Wiegner, 2018) and the TAMUdust2020 (Saito & Yang, 2021; Saito et al., 2021) scattering databases.

The size distributions and complex refractive indices considered for the calculations, are provided by AERONET retrievals collocated with the lidar observations, and height-resolved airborne in-situ data, acquired during the ASKOS-ESA campaign, implemented in Mindelo, Cabo Verde (Marinou et al., 2023). The simulated dp and Sp for dust particles are evaluated against multi-wavelength polarization lidar data from ASKOS and lidar-derived climatological values.

As an independent consistency check of the simulation results, the derived random spheroids/hexahedral mixtures are utilized in radiative transfer calculations to simulate multi-wavelength sky-radiances from AERONET almucantar sequences. More specifically, the sun-photometer observational geometry is considered for two cases: i) assuming the spheroid shape distribution used in AERONET (Dubovik et all, 2006) and ii) assuming the random spheroids/hexahedral mixture found to better reproduce the lidar data. The modelled sky radiances are then compared to the co-located sun-photometer measurements.  

First results show that the random hexahedral/spheroid shape mixtures can accurately reproduce the spectral dependence of dp and Sp for a selected dust case study of ASKOS, while the results are also within the uncertainty of the corresponding climatological lidar data.

How to cite: Gialitaki, A., Tsekeri, A., O’Callaghan, M., Kouklaki, D., Papachristopoulou, K., Kezoudi, M., Papetta, A., Marenco, F., Kandler, K., Aryasree, S., Eknayan, M., and Amiridis, V.: Introducing random mixtures of irregular hexahedrals and spheroids to reproduce polarimetric lidar observations of desert dust, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11446, https://doi.org/10.5194/egusphere-egu25-11446, 2025.

EGU25-11541 | ECS | Orals | AS5.12

Simultaneous profiling of aerosol and tropospheric nitrogen dioxide from synergetic ground-based observations of sun-sky photometer and spectrometer 

Masahiro Momoi, Oleg Dubovik, Elena Lind, Marcos Herreras-Giralda, Tatyana Lapyonok, Anton Lopatin, Wushao Lin, Fernando Rejano, Marie Charlotte Stöckhardt, Axel Kreuter, and Alexander Cede

Trace gasses (e.g., NO2, SO2, HCHO) and aerosols play an important role in atmospheric chemistry and physics. They also negatively affect human and ecosystem health. Vertical distribution of these gasses in the lower troposphere (up to 3-4 km) is often monitored using MAX-DOAS (Multi-AXis Differential Optical Absorption Spectroscopy) technique. Conversion of the trace gas slant absorption (from different viewing angles) into vertical concentration profile requires information about aerosol optical properties and their vertical distribution. Aerosol extinction coefficient profiles are retrieved from the MAX-DOAS measurements of absorption induced by oxygen collision complex (O2O2). The missing Information about columnar aerosol properties is typically taken, with some simplification, from the closest AERONET sun-sky photometer measurements.

This study investigates the possibility of simultaneous aerosol and tropospheric NO2 concentration profile retrievals from synergetic ground-based observations by AERONET sun-sky photometer and Pandonia Global Network spectrometer. We consider standard AERONET sun-sky photometer measurements at 440, 675, 870, and 1020 nm, as well as, available additional observations at 340, 380, 500, and 1640 nm.

We use GRASP (Generalized Retrieval of Atmosphere and Surface Properties, Dubovik et al., 2021) to implement simultaneous retrieval of tropospheric NO2 and vertical aerosol properties from multi-axis differential slant column densities of NO2 and O2O2, and radiance measurements (almucantar and vertical scanning).

The GRASP algorithm was modified to include trace gases (NO2, HCHO, O2O2) differential slant column density measurements and pseudo spherical correction of Earth curvature. In addition, a flexible gas absorption calculation based on optimized correlated k-distribution method (Momoi et al., 2022) was implemented. This presentation demonstrates advantages of synergetic observations for the aerosol and tropospheric NO2 vertical profile retrievals in comparison to the current MAX-DOAS only inversion approaches.

 

Reference:

Dubovik, O., D. Fuertes, P. Litvinov, et al., “A Comprehensive Description of Multi- Term LSM for Applying Multiple a Priori Constraints in Problems of Atmospheric Remote Sensing: GRASP Algorithm, Concept, and Applications”, Front. Remote Sens. 2:706851. doi: 10.3389/frsen.2021.706851, 2021.

Momoi, M., H. Irie, M. Sekiguchi, et al., “Rapid, accurate computation of narrow‑band sky radiance in the 940 nm gas absorption region using the correlated k‑distribution method for sun‑photometer observations”, Prog. Earth Planet. Sci., 9, 10, 1 - 22, https://doi.org/10.1186/s40645-022-00467-6, 2022.

How to cite: Momoi, M., Dubovik, O., Lind, E., Herreras-Giralda, M., Lapyonok, T., Lopatin, A., Lin, W., Rejano, F., Charlotte Stöckhardt, M., Kreuter, A., and Cede, A.: Simultaneous profiling of aerosol and tropospheric nitrogen dioxide from synergetic ground-based observations of sun-sky photometer and spectrometer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11541, https://doi.org/10.5194/egusphere-egu25-11541, 2025.

EGU25-12468 | Posters on site | AS5.12

Optical and microphysical properties of fire smoke aerosol from in-situ polar nephelometry using GRASP  

Fernando Rejano Martínez, Daniel Pérez-Ramírez, Chong Li, Elena Bazo, David Fuertes, Vanderlei Martins, Oleg Dubovik, Antonio Valenzuela, Sonia Castillo, Gloria Titos, and Francisco José Olmo

Advances in aerosol characterization through remote sensing rely on improved inversion algorithms. Scattering phase matrix measurements of ambient aerosols, now feasible with advanced polar nephelometry, are key to these advancements. The Polarized Polar Imaging Nephelometer (PI-Neph, GRASP-Earth PIN-100) has been operating continuously since 2022 in Granada (Spain) providing direct measurements of the phase function (F11) and the degree of linear polarization (−F12/F11) at three wavelengths (405, 515, and 660 nm).

During an extreme biomass-burning event from September 10–12, 2022, surrounding Granada, PM10 and PM2.5evels reached 100–150 µg/m3. Aerosol scattering and absorption coefficients peaked at 500 and 150 Mm−1, respectively. Chemical analysis of PM10 revealed elevated carbonaceous species concentrations, with organic carbon (OC) and elemental carbon (EC) reaching 14 µg/m3 and 3 µg/m3, respectively. Microscopy analyses identified spherical carbonaceous particle agglomerates.

This study explores different configurations of the Generalized Retrieval of Aerosol and Surface Properties (GRASP) algorithm to retrieve aerosol optical and microphysical properties during this biomass-burning event using multiwavelength F11 and F12 measurements. Three inversion approaches were evaluated: a classical scheme assuming a uniform refractive index for all aerosol modes, a bimodal scheme allowing distinct refractive indexes for each mode, and a novel approach incorporating multiwavelength absorption coefficients from Aethalometer measurements.

The classical inversion yielded modal radii of r1=0.13 μm  and r2=8.1 μm, with a refractive index of 1.66+2.70⋅10−4i at 515 nm. The bimodal scheme produced smaller radii (r1=0.12 μm, r2=0.44 μm) and refractive indexes of 1.66+2.01⋅10−4i and 1.50+6.30⋅10−5i, respectively Both approaches showed single scattering albedo (SSA) values above 0.99 but underestimated the measured absorption coefficients.

Incorporating Aethalometer data improved agreement with measured absorption. This method retrieved modal radii of r1=0.11 μm and r2=0.30 μmand refractive indexes of 1.65+6.70⋅10−2i and 1.70+3.10⋅10−4i for each modes respectively. The derived total SSA was 0.85 (with values of 0.75 and 0.99 for each mode), accurately reproducing measured absorption coefficients.

In all cases, inversion residuals were below 2%, highlighting the effectiveness of these retrieval approaches in characterizing aerosols during intense biomass-burning events.

How to cite: Rejano Martínez, F., Pérez-Ramírez, D., Li, C., Bazo, E., Fuertes, D., Martins, V., Dubovik, O., Valenzuela, A., Castillo, S., Titos, G., and Olmo, F. J.: Optical and microphysical properties of fire smoke aerosol from in-situ polar nephelometry using GRASP , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12468, https://doi.org/10.5194/egusphere-egu25-12468, 2025.

EGU25-12682 | ECS | Posters on site | AS5.12

Quantifying dust concentration and mineralogy in the atmosphere, by combining remote sensing and airborne (UAV) in-situ, during the ASKOS campaign 

Maria Tsichla, Alexandra Tsekeri, Konrad Kandler, Holger Baars, Moritz Haarig, Anna Gialitaki, Maria Kezoudi, Athena Floutsi, Alkistis Papetta, Franco Marenco, Eleni Marinou, Kalliopi-Artemis Voudouri, Nikolaos Mihalopoulos, and Vassilis Amiridis

Airborne dust plays a significant role in influencing weather phenomena, climate dynamics, and human health. Accurate quantification of dust concentration and its vertical distribution in the atmosphere, as well as accurate monitoring of dust microphysical properties including chemical composition, is essential for understanding dust impacts on radiation, cloud formation, weather and climate, and for developing corresponding mitigation strategies. Various observational methods have been developed to measure atmospheric dust properties, utilizing remote sensing (e.g. lidar and sun-photometers) and in-situ techniques. These techniques use different assumptions and their combination is a challenging task (e.g. Tsekeri et al., 2017). Herein, we try to harmonize their outputs for dust concentration profiles, using an extensive dataset gathered during the ASKOS campaign in the Cabo Verde Islands, a region uniquely positioned to observe dust outbreaks.

The ASKOS campaign (Marinou et al., 2023) was the ground-based component of the JATAC campaign organized by ESA and NASA in the islands of Cabo Verde (Fehr et al., 2023) during 2021 and 2022. Its main aim was to provide data for the calibration and validation of the Aeolus mission, with a focus on aerosol products. Over the course of these two years, a combination of aircraft, UAV, and ground-based remote sensing measurements was conducted.

The instruments deployed during ASKOS included a multiwavelength Raman-polarization lidar (PollyXT), an AERONET sun-photometer, and in-situ sampling performed using optical particle counters (OPCs) and impactors onboard UAVs (Kezoudi et al., 2023). The UAV in-situ measurements were acquired from ground level up to 5 km above sea level, collocated with the remote sensing data. The OPCs provided measurements of particle size distribution, and the impactors of particle mineralogy.

The dust concentration profiles were calculated from lidar data using the POLIPHON method (Mamouri & Ansmann, 2014). This method utilizes extinction-to-mass conversion factors derived from AERONET data for various aerosol types (including dust), and calculates the mass concentration profiles from the extinction coefficient profiles provided by the lidar.

Dust mass concentration at different altitudes was also derived by using in-situ observations of the number size distribution of the particles. First, the corresponding volume size distribution and the total volume of the particles, are calculated. The dust mass concentration is calculated based on the percentage of dust particles in the volume (provided by the impactor chemical composition observations), using a mean density for dust particles, equal to 2.6 g/cm3.  For cases for which no in-situ observations are available, the volume size distribution of AERONET is utilized, though providing column-effective values.

The initial results indicate that the integrated mass concentration across the dust layer, as determined by both techniques, lies within the uncertainty ranges of the respective methods. Also, the analysis from the impactors provides information on the mineralogical composition of the dust particles that are transported from the Sahara.

Our work will assess each technique’s validity and identify the conditions under which the remote sensing method can be used independently.

This research was supported by the REVEAL project (GA 7222) funded by the Hellenic Foundation for Research & Innovation and by the PANGEA4CalVal project (GA 101079201) EU-funded.

How to cite: Tsichla, M., Tsekeri, A., Kandler, K., Baars, H., Haarig, M., Gialitaki, A., Kezoudi, M., Floutsi, A., Papetta, A., Marenco, F., Marinou, E., Voudouri, K.-A., Mihalopoulos, N., and Amiridis, V.: Quantifying dust concentration and mineralogy in the atmosphere, by combining remote sensing and airborne (UAV) in-situ, during the ASKOS campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12682, https://doi.org/10.5194/egusphere-egu25-12682, 2025.

EGU25-14129 | Orals | AS5.12

Overview of French efforts for the innovative characterisation of aerosols and cloud interactions with the future Atmosphere Observing System 

Juan Cuesta, Anton Lopatin, Cyrille Flamant, Laaziz El Amraoui, Joel Ferreira De Brito, Marc Mallet, Michaël Sicard, Solène Turquety, Claudia Di Biagio, Paola Formenti, Sergey Khaykin, Irène Xueref-Remy, Valérie Gros, Vincent Noël, Jean-Eudes Petit, Benjamin Torres, Fazzal Qayyum, and Abou Merdji

Aerosols and clouds play a major role in the Earth Climate systems, while the quantification and clear understanding of their variabilities, interactions and feedbacks remain a great challenge. In particular, aerosols strongly impact the energy budget by direct modification of solar and infrared radiation, alteration of cloud properties and their formation processes as well as the thermodynamic properties of the atmosphere. Aerosols are also the most harmful air pollutant, being responsible of several millions of premature deaths worldwide each year. Even though diverse observation and modelling approaches of aerosols exist, numerous unknowns remain concerning the chemical and physical mechanisms that affect them, their vertical redistribution in the atmosphere, the quantification of their environmental impacts and their interactions with clouds and convective processes.

In order to tackle these major environmental issues at global scale, a new spaceborne Atmosphere Observing System (AOS) has been conceived as an international cooperation between NASA from USA, CNES from France, JAXA from Japan, CSA from Canada and ASI from Italy. This mission is built as a constellation of several satellites following two orbits, a polar orbit with global coverage in the continuity of the A-Train constellation and an inclined designed to document the diurnal variation of convection in the Tropics and mid-latitudes. They satellites will carry new generation active and passive instruments for sounding aerosols, clouds, convection, and precipitation, including an advanced multiwavelength lidar in tandem with a multi-angular polarimeter, whose launching period is planned for 2030.

In the current presentation, we will provide an overview of French efforts for the innovative characterization of aerosols and its interactions with clouds  for preparing the scientific exploitation of AOS. They gather relevant contributions from 8 French scientific laboratories: LISA, LOA, LATMOS, CNRM, LAERO, LACy, CERI EE and LSCE and a French industrial partner: GRASP-SAS. These efforts are threefold: (i) the development of innovative French aerosol satellite products based on AOS observations, (ii) suborbital measurements for feeding both the aerosol products and conceiving a synergetic exploitation with AOS and (iii) synergism with chemistry-transport models. The AOS aerosol observations will provide a new quantification of the vertical profile of aerosol concentration simultaneously for different particle types and chemical species. This information will be derived from lidar only and the synergism of lidar and polarimeter measurements using a so-called GRASP retrieval approach. Additional products aim the quantification of cloud condensation nuclei for studying aerosols/cloud interactions. The suborbital contribution will characterize aerosol optical, microphysical, and chemical properties from airborne, ground-based from several French sites and laboratory instrumentation. While documenting aerosols properties for different aerosol types and species, they provide a scientific framework for studying complex interactions such as the impact of aerosols on convective activity in specific regions. This is the case of the BACCOPA French field campaign aiming the studying of the impact of biomass burning aerosols emitted from Central Africa on convective activity. Finally, synergetic approaches with chemistry transport-models aim the development of data assimilation methods of AOS measurements and the use of these last ones for evaluating their numerical simulations.

How to cite: Cuesta, J., Lopatin, A., Flamant, C., El Amraoui, L., Ferreira De Brito, J., Mallet, M., Sicard, M., Turquety, S., Di Biagio, C., Formenti, P., Khaykin, S., Xueref-Remy, I., Gros, V., Noël, V., Petit, J.-E., Torres, B., Qayyum, F., and Merdji, A.: Overview of French efforts for the innovative characterisation of aerosols and cloud interactions with the future Atmosphere Observing System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14129, https://doi.org/10.5194/egusphere-egu25-14129, 2025.

EGU25-14616 | ECS | Posters on site | AS5.12

Improving Black Carbon Emission Estimates at Global Scale Using GEOS-Chem model and 4D-Var assimilation of TROPOMI/GRASP data 

Abhinna Behera, Cheng Chen, Oleg Dubovik, Pavel Litvinov, Yixuan Gu, Daven Henze, Tatyana Lapyonok, François Thieuleux, and Benjamin Guinot

Radiative forcing by light-absorbing aerosols, particularly black carbon (BC), a major climate forcing agent alongside CO2 and CH4, remains poorly constrained due to insufficient characterisation of their optical properties and highly variable spatio-temporal distributions. Here we aim to refine BC’s spatio-temporal variability using the GEOS-Chem 3D Eulerian chemistry-transport model, which incorporates BC’s well-defined physical and chemical properties. The model includes aerosol-phase chemistry relevant to urban atmospheres, such as desert dust, BC, organic carbon, sea salts, SiO2, metal oxides, SO4²⁻, NO3-, NH4⁺, Na⁺, and Ca²⁺, at a global resolution (2°×2.5°) with primary aerosols only. Our primary objective is to precisely map BC’s spatial and temporal distributions, which is critical for evaluating the long-term impact of absorbing aerosols on net radiative forcing.

Using the 4D-Var assimilation method with TROPOMI/GRASP aerosol optical depth (AOD) and aerosol absorption optical depth (AAOD) data, we adjust global-scale emissions at an hourly resolution from March 2019 to November 2020. From a satellite remote sensing perspective, this characterization of aerosols via a single-viewing spectrometer is unprecedented. The GRASP open-source algorithm has generated this novel dataset. The GEOS-Chem model is driven by 3-hourly meteorological fields obtained from GEOS-FP reanalysis data. Our study includes the extreme events of the Australian bushfire season and Canadian forest fire events, where we identify emission sources absent from the GFED3 inventories (1996–2012) used in the forward run. Assimilation of TROPOMI/GRASP AOD and AAOD data into the model allows to reproduce carbonaceous aerosol emissions. These results are validated using MODIS and VIIRS RGB imagery. Ground-level BC concentrations are further validated against in situ measurements from France in the frame of the ANR BLACKNET project and from AERONET. 

This framework will enable creating a global particulate matter (PM) database with high temporal resolution, spanning several years. Satellite data alone cannot achieve this level of detail. High-resolution BC distribution via inverse modelling will benefit from future spaceborne multi-angular polarimetric sensors, such as 3MI, CO2M MAP, and PACE. Additionally, aerosol vertical distributions will be studied to assess their influence on temperature profiles and atmospheric stability. This work will aid in validating and comparing suborbital measurements. The inverse modelling approach aligns closely with LiDAR-based observations from the EarthCARE mission. 

How to cite: Behera, A., Chen, C., Dubovik, O., Litvinov, P., Gu, Y., Henze, D., Lapyonok, T., Thieuleux, F., and Guinot, B.: Improving Black Carbon Emission Estimates at Global Scale Using GEOS-Chem model and 4D-Var assimilation of TROPOMI/GRASP data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14616, https://doi.org/10.5194/egusphere-egu25-14616, 2025.

EGU25-14885 | ECS | Posters on site | AS5.12

Aerosol Optical Properties in the Eastern Arabian Peninsula from Direct Sun Observations 

Ersin Tutsak, Mohamed M. Mahfouz, Imran Shahid, Jassem A. Al-Thani, Oğuz Yiğiterhan, and Ebrahim M.A.S. Al-Ansari

The Eastern Arabian Peninsula experiences elevated atmospheric particle loads due to anthropogenic emissions from the extraction and use of fossil fuels, as well as natural dust events, resulting in significant aerosol optical thickness (AOT). However, despite the region's significance, there is a lack of studies focusing on the optical and microphysical characterization of aerosols, leaving critical gaps in understanding their radiative effects. This study examines the optical properties of atmospheric particles over Qatar using more than one-year sun photometer data, with an emphasis on temporal variations and source origins. Measurements of direct sunlight were recorded every 5 minutes across wavelengths from 340 to 1020 nm between March 2023 and November 2024. Aerosol optical thickness (AOT) was calculated from these measurements using the Beer-Lambert-Bouguer law, while the Angstrom Exponent (AE) was derived to assess particle size. The results revealed notable daily variability, with average AOT values at 440 nm of 0.41 ± 0.21 and AE values averaging 0.87 ± 0.35. Seasonal patterns showed higher AOT during the summer months and a transition from dust-dominated to anthropogenic aerosols between March and December. Aerosols were classified into three categories: mineral dust-dominated (AE < 0.5), mixed (0.5 < AE < 1), and anthropogenic (AE > 1), accounting for 18%, 44%, and 38% of the total observations, respectively. These findings provide new insights into the aerosol composition over the region and emphasize the need for further research using radiative transfer models to evaluate aerosol-induced changes to the radiation budget.

How to cite: Tutsak, E., M. Mahfouz, M., Shahid, I., A. Al-Thani, J., Yiğiterhan, O., and M.A.S. Al-Ansari, E.: Aerosol Optical Properties in the Eastern Arabian Peninsula from Direct Sun Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14885, https://doi.org/10.5194/egusphere-egu25-14885, 2025.

EGU25-15230 | Orals | AS5.12

Enhancing Atmospheric Profiling with the AMETHYST Hyperspectral Inversion System 

Steven Businger and Paolo Antonelli

In this talk, we will discuss plans to maximize the extraction of information from the inversion of hyperspectral infrared (IR) and microwave data obtained from polar-orbiting instruments.  Hyperspectral remote sensing, which involves capturing Earth’s emitted energy in the IR spectrum, has become a pivotal tool for understanding atmospheric and surface conditions. A central challenge in this field is the efficient and accurate inversion of hyperspectral IR data to extract quantitative physical and chemical properties. The AdaptiveMETeo HYperSpectral Transformer (AMETHYST) inversion system represents a significant advancement in this regard. It enables the characterization of vertical atmospheric columns by considering variables such as temperature, pressure, and humidity at various altitudes. By comparing observed hyperspectral IR data with simulated radiance, AMETHYST adjusts model parameters to accurately retrieve vertical atmospheric structures.

AMETHYST leverages both hyperspectral data and numerical weather prediction (NWP) model forecasts to produce thermodynamic profiles and transformed retrievals (TRs). These TRs, developed using Migliorini’s transformation, are particularly suited for regional model assimilation due to their reduced data volume, instrument-specific adaptations, and simplified observation error covariance. Recent studies, including Cherubini et al. (2023), have demonstrated the effectiveness of TR assimilation in improving moisture field characterization over the central North Pacific Ocean, particularly at mid-atmospheric levels. This improvement is crucial for refining cloud and precipitation predictions.

Additionally, our team is extending the capabilities of AMETHYST to analyze physical profiles above cloud tops in the Arctic by integrating cloud masks and properties from various satellite instruments, differentiating it from its predecessor, MIRTO.

How to cite: Businger, S. and Antonelli, P.: Enhancing Atmospheric Profiling with the AMETHYST Hyperspectral Inversion System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15230, https://doi.org/10.5194/egusphere-egu25-15230, 2025.

The influence of aerosols on climate is determined not only by their global distribution but also by their composition. However, a large fraction of the development efforts for satellite-based aerosol retrievals has focused on inverting the total column aerosol optical depth (AOD) from different single instruments. As the information content of single instruments is smaller than necessary to retrieve a comprehensive quantification of all parameters of the atmospheric aerosol, there is a need for using auxiliary information to fill this gap (e.g. pre-defined optical aerosol properties, climatological vertical profiles, ...). Retrievals inverting further aerosol parameters from one instrument (e.g. Fine Mode or Dust AOD) depend on the auxiliary assumptions and on the sensitivity of the available instrument channels to the various aerosol properties. This leads to inconsistencies even between AOD results and certainly for additional parameters inverted from different sensors. Examples of consequential inconsistencies are the step in the AOD Climate Data Record built from subsequent pieces from similar instruments but with opposing viewing directions in the “dual view radiometer” series (A)ATSR(-2) and SLSTR) or the combined use of retrieval results from thermal with UV-VIS instruments at the same wavelength (usually 550 nm). For both examples, synergetic retrievals hold the potential to reduce the dependence on assumed properties and thus improve consistency.

It can be argued that each new generation of satellite instruments offers new additional capabilities so that the most recent era of multi-angle, multi-spectral polarimeters provide significantly larger information content and are thus able to invert more aerosol parameters. However, the wealth of satellite-based aerosol climate-relevant time series dating back to early 1980s comes from much simpler instruments. Here I see the largest field of synergetic retrievals, ranging from combinations of AVHRR with TOMS over combinations of MODIS and MISR or AATSR / MERIS / SCIAMACHY (and IASI) and their successor instruments.

One alternative road to achieve this could be in data assimilation of single-sensor aerosol retrieval results. However, any inconsistency of those separate pieces ingested into an atmospheric model will create difficulties and, in addition, the effort for including several independent satellite aerosol products (error covariance matrices, bias corrections) has put a stringent limitation so far. Ultimately, the use of all available information from different sensors offers the perspective of “self-consistent” results.

Building on lessons from the decade of Aerosol_cci developments and my own early and simplistic synergetic retrievals (SYNAER with AATSR and SCIAMACHY), this work presents a conceptual framework for advancing synergetic aerosol retrieval methodologies. Key elements include multi-sensor information content analysis, strategies for addressing historical data gaps and practical challenges (e.g. cross-calibration, cross-channel correlations, colocations and differences in field of views). In combination with priorities for needed parameters and length and gaps in historic records, this paper aims to establish a roadmap for synergetic aerosol retrievals, paving the way for more robust and comprehensive, i.e. self-consistent climate data records.

How to cite: Popp, T.: A concept for synergetic retrievals of self-consistent aerosol property climate data records, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15893, https://doi.org/10.5194/egusphere-egu25-15893, 2025.

EGU25-15896 | ECS | Posters on site | AS5.12

Vertical distribution of the concentrations of multiple aerosol types derived from the multiwavelength spaceborne lidar of the future Atmosphere Observing System  

Fazzal Qayyum, Juan Cuesta, Abou Bakr Merdji, Anton Lopatin, Oleg Dubovik, Durgesh Nandan Piyush, Laaziz El Amraoui, and Richard Ferrare

Atmospheric aerosols play a key role in influencing the Earth's radiation budget. Still, their impacts remain poorly quantified due to the complex mechanisms involved in the interaction between aerosols and clouds. Indeed, aerosols act as ice-nucleating particles and cloud condensation nuclei, significantly altering the formation of precipitation and clouds. These environmental impacts of aerosols are strongly dependent on their composition, origin, and types. Moreover, high concentrations of aerosols in the atmosphere degrade air quality, posing large health risks which are also highly dependent on their composition (which is related to their types).

In recent decades, a space-borne lidar called the cloud–aerosol lidar with orthogonal polarization (CALIOP) onboard cloud–aerosol lidar and infrared pathfinder satellite observation (CALIPSO) satellite was providing aerosol vertical distribution from space using two wavelengths, namely 532 nm which provides attenuated backscatter and depolarization profiles and 1064 nm which deliver attenuated backscatter profile. Combining its 3 channels, CALIOP measurements provide a purely qualitative aerosol typing detection, indicating the presence or absence of a single aerosol type at each altitude of the atmosphere. To provide a more detailed and quantitative characterization of aerosols and to gain new insights into the interactions between aerosols, clouds, convective processes and precipitation, the upcoming mission called Atmosphere Observing System (AOS), which includes contributions from the space agencies NASA (United States), CNES (France), ASI (Italy), JAXA (Japan) and CSA (Canada) is currently in preparation for launching in a horizon near 2030. AOS payload will include an advanced high-energy 3-wavelength lidar with Raman capabilities during nighttime, called CALIGOLA.

In our present work, we examine the potential of CALIGOLA lidar during the daytime (three wavelength attenuated backscatter and depolarization measurements) and nighttime (one additional Raman channel in the UV which is suitable for nighttime measurements) flying in a polar orbit. By utilizing our newly developed retrieval approach, we quantitatively discriminate the concentration vertical profiles of five distinct aerosol types, such as smoke, continental, oceanic, dust and urban polluted. The development and first implementation of the method were performed using the pseudo-reality simulations obtained from the chemistry-transport model called Modèle de Chimie Atmosphérique de Grande Echelle (MOCAGE). In addition, the first tests of our innovative retrieval approach are planned using real lidar measurements from the High Spectral Resolution Lidar-2 (HSRL-2) airborne lidar from NASA Langley Research Center (LaRC).

How to cite: Qayyum, F., Cuesta, J., Merdji, A. B., Lopatin, A., Dubovik, O., Nandan Piyush, D., El Amraoui, L., and Ferrare, R.: Vertical distribution of the concentrations of multiple aerosol types derived from the multiwavelength spaceborne lidar of the future Atmosphere Observing System , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15896, https://doi.org/10.5194/egusphere-egu25-15896, 2025.

EGU25-16550 | ECS | Posters on site | AS5.12

Daily aerosol variation revealed by synergetic multi-satellite GRASP retrieval 

Siyao Zhai, Pavel Litvinov, Oleg Dubovik, Christian Matar, Chong Li, David Fuertes, Cheng Chen, Zhen Liu, Tatyana Lapyonok, Manuel Dornacher, Arthur Lehner, Alexandru Dandocsi, Daniele Gasbarra, Elody Fluck, and Christian Retscher

In this study, we analyze the daily aerosol variability from synergetic multi-satellite GRASP retrieval. On a regional to local scale, aerosol diurnal concentration and microphysical properties can change rapidly due to inherent short lifespan, intense source emissions and weather processes. To observe the aerosol diurnal variability of a region, it is necessary to have multiple satellite measurements (greater than two measurements per day), and desirable to have per-hour satellite measurement. The capability to observe aerosol diurnal patterns is of interest to many research and applications such as: basic research of the aerosol global spatial distribution, variability and climate effects; aerosol transport modelling; Assimilation into atmospheric circulation models, etc. To meet these needs, it is essential to utilize all available satellite measurements to increase the sampling in time, in scattering angle and in spectral space.

 

In the ESA SYREMIS project, we performed a pioneering attempt of synergetic retrieval combining OLCI/Sentinel-3(A and B), TROPOMI/Sentinel-5p and AHI/Himawari-8 measurements using the GRASP algorithm. Such synergy of instruments from different satellite platforms greatly expands the spectral range, observation angle range and temporal observation density compared to existing synergy/merged satellite products. This led to much enhanced observation capability and retrieval accuracy for the merged instrument network. Among the aerosol products from synergetic retrieval, Aerosol Optical Depth (AOD) show very good fit to AERONET AOD diurnal time series, aerosol microphysical parameters such as Angstrom Exponent (AE) and Single Scattering Albedo (SSA) also show very good fit to the corresponding AERONET diurnal time series. Lateral comparison with the XAERDT merged aerosol products (MODIS+VIIRS+AHI) were made, and GRASP synergetic aerosol products show superior performance, especially in terms of the temporal stability of all aerosol parameters, and accuracy of the aerosol microphysical parameters. The improved synergy aerosol product should greatly benefit downstream applications such as aerosol transport modelling, assimilation into atmospheric circulation models and air quality forecast models.

How to cite: Zhai, S., Litvinov, P., Dubovik, O., Matar, C., Li, C., Fuertes, D., Chen, C., Liu, Z., Lapyonok, T., Dornacher, M., Lehner, A., Dandocsi, A., Gasbarra, D., Fluck, E., and Retscher, C.: Daily aerosol variation revealed by synergetic multi-satellite GRASP retrieval, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16550, https://doi.org/10.5194/egusphere-egu25-16550, 2025.

EGU25-16759 | ECS | Orals | AS5.12

Object-based characterization of continental Shallow Cumulus using synergistic decameter-scale observations 

Oscar Ritter, Sebastian Bley, Rusen Oktem, David M. Romps, and Hartwig Deneke

Shallow convective cumulus clouds (ShCu) play a crucial role in weather and the global climate system. These clouds are characterized by spatial and temporal variability on a wide range of scales, making ShCu an important contributor to the uncertainty in determining the local and global radiation budget as well as mass transport. Since individual remote sensing instruments can only capture a small part of this variability, a synergy of several observations is beneficial.

By combining very high spatial resolution, multispectral observations from the polar-orbiting Sentinel-2 satellite with a stereo camera-based 4D cloud product, Clouds Optically Gridded by Stereo (COGS), we will analyze 15 scenes of continental ShCu in a 6x6x6km3 domain around the Central Facility of the ARM Southern Great Plains site in the United States. Using an object-based approach, we will highlight the three-dimensional geometric properties of individual ShCu and the relationship to their multispectral reflectances and their cloud shadows. The meteorological influences on the geometric properties, and the relationship between cloud size, cloud thickness and cloud volume will be discussed.

Furthermore, considering the 270km wide observation path of the Sentinel-2 satellite, we will discuss the influence of cloud geometry, meteorological conditions and the organization of ShCu on the variability of cloud fraction and cloud size distributions, as an important step towards the parameterization of ShCu in climate models. The results will also be placed in the context of temporal cloud development.

How to cite: Ritter, O., Bley, S., Oktem, R., Romps, D. M., and Deneke, H.: Object-based characterization of continental Shallow Cumulus using synergistic decameter-scale observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16759, https://doi.org/10.5194/egusphere-egu25-16759, 2025.

EGU25-16761 | ECS | Orals | AS5.12

Can bimodal aerosol size distribution be retrieved from AURORA4000 polar integrating nephelometer data? 

Justyna Szymkowska, Artur Szkop, and Aleksander Pietruczuk

Atmospheric aerosols are tiny liquid and solid particles suspended in the air. They can scatter and absorb electromagnetic radiation, thus affecting the Earth’s radiative balance and climate. Additionally, aerosols can influence air quality, leading to respiratory and cardiovascular health problems.

To acquire information about the space-time variability of atmospheric aerosols and their optical and microphysical properties, various techniques are employed. In situ methods are typically performed at ground level, while remote methods use light to determine optical aerosol parameters.

This study focuses on the polar integrating nephelometer Aurora 4000 (Chamberlain-Ward and Sharp, 2011), which measures aerosol light scattering at different angles ranging from 10° to 170° across three wavelengths: 450, 525, and 635 nm. The main objective is to conduct sensitivity studies of the nephelometer by simulating theoretical signals for varying sets of optical and microphysical aerosol parameters. Thus examining the influence of various particle distribution parameters on light scattering measured by the nephelometer.

To simulate the nephelometer signals, the an advanced and versatile retrieval algorithm is employed. The Generalized Retrieval of Atmosphere and Surface Properties (GRASP) software (Dubovik et al., 2014; Lopatin et al., 2021) represents a state-of-the-art approach to integrating multi-source remote aerosol data, capable of retrieving atmospheric properties based on active (LIDAR) and passive (sun-sky photometer) remote techniques, as well as ground-based nephelometers.

Statistical parameters of aerosol size distributions (ASD) are derived from measurement data recorded by a ground-based system of aerosol size spectrometers, which includes a mobility particle size spectrometer (MPSS) and an aerodynamic particle size spectrometer (APSS). This combination allows for the determination of particle sizes within 10 nm to 10 μm. The synergy of these two instruments enables the acquisition of high-quality and wide range aerosol size distribution spectra.

Chamberlain-Ward, Steve, and Felicity Sharp. "Advances in nephelometry through the Ecotech Aurora nephelometer." The Scientific World Journal 11.1 (2011): 2530-2535.

Dubovik, Oleg, et al. "GRASP: a versatile algorithm for characterizing the atmosphere." SPIE Newsroom 25.10.1117 (2014): 2-1201408.

Lopatin, Anton, et al. "Synergy processing of diverse ground-based remote sensing and in situ data using the GRASP algorithm: applications to radiometer, lidar and radiosonde observations." Atmospheric Measurement Techniques 14.3 (2021): 2575-2614.

This work is supported by the National Science Centre grant number 2021/41/B/ST10/03660.

How to cite: Szymkowska, J., Szkop, A., and Pietruczuk, A.: Can bimodal aerosol size distribution be retrieved from AURORA4000 polar integrating nephelometer data?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16761, https://doi.org/10.5194/egusphere-egu25-16761, 2025.

EGU25-16773 | Orals | AS5.12

Multi-sensor Aerosol Product from EPS-SG – Consideration for the Operational Aerosol Product 

Soheila Jafariserajehlou and Bertrand Fougnie

With the launch of EPS-SG in 2025, EUMETSAT will operate a space platform hosting a series of instruments among which VII, 3MI, IASI-NG and UVNS (Sentinel-5). The potential of a synergistic approach combining 3 instruments has been already demonstrated with the release of the EPS/PMAp product, operational as a Near-Real-Time aerosol product since 2014. After a colocation of all the measurements provided by the instruments, the synergistic retrieval becomes possible. For EPS-SG, an important step forward will be made with the polarimeter 3MI which will allow the provision of many aerosol properties. The synergistic use of the other instruments will contribute to improve this characterisation from 3MI. The spectral extension to UV and TIR, the sub-pixel information, but also the use of absorption bands. The pre-design of this synergistic product will be presented.

How to cite: Jafariserajehlou, S. and Fougnie, B.: Multi-sensor Aerosol Product from EPS-SG – Consideration for the Operational Aerosol Product, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16773, https://doi.org/10.5194/egusphere-egu25-16773, 2025.

EGU25-17053 | ECS | Posters on site | AS5.12

Vertical Profiles of Aerosol Chemical Species Concentrations derived from the Synergism of the Future Spaceborne Lidar and Polarimeter of the Atmosphere Observing System 

Abou Bakr Merdji, Juan Cuesta, Fazzal Qayyum, Anton Lopatin, Oleg Dubovik, Durgesh Nandan, Laaziz El Amraoui, and Richard Ferrare

The Atmosphere Observing System (AOS), a collaborative initiative from the international cooperation of NASA, CNES, JAXA, ASI, and CSA, aims to substantially enhance the observation of aerosols and clouds through the deployment of an advanced spaceborne lidar and a multi-angular polarimeter, expected to fly in tandem. Within this framework, we present a novel methodology for retrieving vertical concentration profiles of aerosol chemical species by synergistically leveraging measurements from co-located lidar and polarimeter instruments. This approach, named Aerosol Chemical Profiling (AEROCHEMPro), extends the GRASP (Generalized Retrieval of Aerosol and Surface Properties) framework to provide vertically resolved profiles of aerosol modes: (i) a fine mode containing black carbon, brown carbon, inorganic salts, and water content; (ii) a coarse desert dust mode composed of iron oxide and quartz; and (iii) a coarse sea salt mode with associated water content.

First, the AEROCHEMPro methodology is developed and implemented on synthetic observations from an Observing System Simulation Experiment (OSSE). Synthetic lidar and polarimeter measurements are simulated by radiative transfer code using a pseudo-reality built from the MOCAGE chemistry-transport model. We consider the instrumental configuration of AOS: the high energy 3-wavelength elastic backscatter lidar called CALIGOLA and the 8-wavelength ultraviolet-to-near-infrared multi-angular polarimeter of the AOS-Sky mission. These case studies demonstrate the capability of AEROCHEMPro to accurately retrieve the vertical profiles of aerosol chemical species, along with their optical and microphysical properties, offering a robust foundation for real-world applications.

In a second stage, a first adaptation of the AEROCHEMPro approach to real measurement is conducted. We use real airborne measurements from the Research Scanning Polarimeter (RSP) and NASA's High Spectral Resolution Lidar-2 (HSRL-2). While the RSP delivers complementing passive observations of polarized radiances across many spectral bands, the HSRL-2 offers high-resolution active aerosols remote sensing. HSRL-2 measurements are used to derive elastic backscatter signals as those that will be performed by CALIGOLA and level 2 products for comparison with respect to AEROCHEMPro output.

The proposed presentation will provide results of AEROCHEMPro based on both OSSE synthetic measurements and first implementations with airborne real measurements.

 

Keywords: AEROSOL OBESERVING SYSTEM; LIDAR; POLARIMETER; AEROSOL SPECIES PROFILE; GRASP; AEROCHEMPro

How to cite: Merdji, A. B., Cuesta, J., Qayyum, F., Lopatin, A., Dubovik, O., Nandan, D., El Amraoui, L., and Ferrare, R.: Vertical Profiles of Aerosol Chemical Species Concentrations derived from the Synergism of the Future Spaceborne Lidar and Polarimeter of the Atmosphere Observing System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17053, https://doi.org/10.5194/egusphere-egu25-17053, 2025.

With the launch of EPS-SG in 2025, a new era for a long-term operational Near-Real-Time provision of aerosol product is starting. If most of the potential for such a new remote sensing polarimetry has been demonstrated since 1996 with the 3 POLDER and PARASOL missions, the recent advance in term of retrieval but also analysis and exploitation of the data reveal more and more the potential. Indeed, polarimeters allow the observation of aerosols with a significantly improved information content which will feed the retrieval. On top of the aerosol optical thickness classically retrieved, an additional set of parameters characterizing the aerosol properties can now be derived such as the fraction of aerosol chemical components, which contributes to filling the gap between satellite retrieval and modelling community by going beyond aerosol typing, the new retrieved parameters also highlights the need for in-situ measurements to support on one hand the assumptions that could be needed in the algorithm (constraints, definition of aerosol chemical components…), and on the other hand contribute to the validation of the products. This set of new parameters is also stimulating new discussion about aerosol modelling.    

How to cite: Jafariserajehlou, S. and Fougnie, B.: New Space-borne Remote Sensing Capabilities Based on Polarimetry and the Implication in term of Aerosol Chemical Components and the needs for in-situ Measurements , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18328, https://doi.org/10.5194/egusphere-egu25-18328, 2025.

EGU25-18448 | ECS | Posters on site | AS5.12

Enhancing WRF-Chem Dust Predictions Through Assimilation of Satellite-Based MIDAS Dust Optical Depth Data 

Eleni Drakaki, Antonis Gkikas, Thanasis Georgiou, Hesham El-Askary, and Vassilis Amiridis

Accurately modelling the distribution of mineral dust in the atmosphere is a complex task that poses significant challenges. Dust aerosols influence critical atmospheric processes, such as the radiation balance and nutrient deposition, making their study essential for understanding Earth’s dynamics. However, the inherent variability and complexity of dust emissions, transport, and deposition contribute to large uncertainties in aerosol numerical predictions.

This study combines advanced numerical modelling with satellite observations, to tackle these challenges and enhance dust forecasts over the Mediterranean region. We use the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) to simulate dust activity during September 2021. The simulations are improved by assimilating satellite-based dust optical depth data from the MIDAS (Mineral Dust Aerosol Satellite) product, which provides observations at a spatial resolution of 1°×1°.

By integrating MIDAS data, we significantly refine the model’s dust predictions, aligning them more closely with observed conditions. The improved forecasts demonstrate clear benefits, especially for applications in air quality management and solar energy optimization. Additionally, a more accurate representation of dust aerosol provides a solid base for studying aerosol-cloud interactions.

These findings highlight the value of blending high-quality observational datasets with sophisticated modelling approaches to address uncertainties in dust aerosol studies.

Acknowledgements. This research work has been supported by the EU-funded programme CiROCCO under Grant Agreement No 101086497. Α part of this work has been supported by AIRSENSE (Aerosol and aerosol cloud Interaction from Remote SENSing Enhancement) project, funded from the European Space Agency under Contract No. 4000142902/23/I-NS.

How to cite: Drakaki, E., Gkikas, A., Georgiou, T., El-Askary, H., and Amiridis, V.: Enhancing WRF-Chem Dust Predictions Through Assimilation of Satellite-Based MIDAS Dust Optical Depth Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18448, https://doi.org/10.5194/egusphere-egu25-18448, 2025.

EGU25-18680 | ECS | Posters on site | AS5.12

Development of a flexible module accounting gas absorption in GRASP allowing simultaneous retrieval of gases and aerosols 

Wushao Lin, Marcos Herreras-Giralda, Masahiro Momoi, Tatyana Lapyonok, Anton Lopatin, Fernando Rejano, Oleg Dubovik, Andrew Barr, and Jochen Landgraf

Accurate modeling of gas absorption is essential for understanding atmospheric radiative transfer and enabling reliable retrievals of atmospheric composition. To address this need, we have developed a new gas computation module into the GRASP (Generalized Retrieval of Atmosphere and Surface Properties, Dubovik et al., 2021) code, extending its capability for simultaneous retrieval of atmospheric gases and aerosols.

The new gas module primarily employs an optimized correlated k-distribution method (Momoi et al., 2022) to efficiently calculate gas absorption optical thickness with high accuracy across a wide spectral range. Additionally, the module supports the line-by-line method as a complementary approach for comparison and validation, ensuring high accuracy and flexibility for a variety of atmospheric scenarios. The implementation of the gas module significantly expands GRASP’s capabilities, making it a more comprehensive tool for simultaneous retrieval of atmospheric gas vertical profiles and aerosol properties. 

Preliminary results regarding the combination of multi-angular polarimeters and SWIR spectrometers (e.g., CO2M, S5 and 3MI) highlight the module's computational efficiency, precision, and adaptability, making it well-suited for operational deployment. Its ability to handle diverse atmospheric scenarios enables the development of advanced retrieval algorithms. Integrating this advanced gas module into GRASP code marks a transformative advancement, enhancing the capacity of remote sensing sensors to monitor aerosol and gases and address environmental challenges effectively.

How to cite: Lin, W., Herreras-Giralda, M., Momoi, M., Lapyonok, T., Lopatin, A., Rejano, F., Dubovik, O., Barr, A., and Landgraf, J.: Development of a flexible module accounting gas absorption in GRASP allowing simultaneous retrieval of gases and aerosols, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18680, https://doi.org/10.5194/egusphere-egu25-18680, 2025.

EGU25-18930 | Orals | AS5.12

Towards Advanced Sentinel-3 Near Real Time (NRT) L2 synergy aerosols capabilities - On-going Day 2 & Day 3 developments 

Julien Chimot, Edouard Martins, Jaap Onderwater, Bertrand Fougnie, Pavel Litvinov, and Oleg Dubovik

As an operational user-driven Earth observation satellite agency, EUMETSAT is the reference European provider of Near Real Time (NRT - < 3h from the sensing time) Level 2 (L2) aerosol satellite observations from a constellation combining both Low Earth Orbit (LEO), with Metop / Sentinel-3 and EPS-SG, and GEOstationary (MSG & MTG). Primary users are operational air quality and climate services. Notably, for several years, EUMETSAT has closely interacted with the Copernicus Atmospheric Monitoring Service (CAMS) and provided expertise to support the uptake of all its observations into the modelling and assimilation processes.

With two multi-spectral optical sensors and observations acquired at a high spatial resolution at 10:00, Sentinel-3 is the main Copernicus mission mandated by the European Commission (EC) to provide a high quality of Aerosol Optical Depths (AODs) at global coverage during morning overpass time for the long future. As such, EUMETSAT is mandated since 2014 by its Member States and Copernicus to develop, enhance and ensure the Copernicus NRT Sentinel-3 Aerosol product. This is the 2nd European product delivering Aerosol Optical (AOD) after Metop with PMAP (Polar Multi-sensor Aerosol optical Properties). Since 2020, it is derived from the OSSAR-CS3 (Optimized Simultaneous Surface Aerosol Retrieval for Copernicus Sentinel-3) algorithm, jointly specified & developed by EUMETSAT scientific experts & the Swansea University team led by Prof. Dr. Peter North (Chimot et al., 2021). Furthermore, EUMETSAT intensively works with the European Centre for Medium-Range Weather Forecasts (ECMWF) by exchanging the necessary expertise to support the future operational assimilation by the Copernicus Atmospheric Monitoring Service (CAMS), as done with PMAP.

The latest evolution, called Collection 3.1, compiles several major developments: 1) a sophisticated classification mask (called Naïve probabilistic) leading to enhanced coverage over all waters, and better cloud, snow, dust / ash, and dark vs. inland waters distinction, 2) more accurate 1st guess of land vegetation reflectance, 3) revised underlight scattering caused by Ocean Colour features by using the Sentinel-3 Level 2 OLCI water reflectance, 4) improved constraints for bare soils in the dual-angular land model, and 4) a new Quality Indicator (QI) system integrated in the L2 product to guide further the users.

Based on lessons learned, EUMETSAT is now leading a major redesign of this algorithm, structured in two steps: first a Day-2 solely based on SLSTR, and a Day-3 intended as a NRT synergy (OLCI + SLSTR) to be based on the future Sentinel-3 NRT L1C under study and generated by EUMETSAT (De Bartolomei, 2014). As such, enhanced aerosol typing and further understanding of interaction with clouds are being investigated. This redesign also covers the development of Aerosol Layer Height (ALH) retrieval from the OLCI O2-A bands.

This presentation will summarise an extensive set of validation results including match-up with ground-based AERONET, inter-comparison of time series with MODIS/VIIRS from NASA and NOAA, and exchanges with the oeprational user community. Then, it will share the details of the plans of developments of the NRT Sentinel-3 Synergy and the major algorithm redesign items under specification, implementation, and testing.

How to cite: Chimot, J., Martins, E., Onderwater, J., Fougnie, B., Litvinov, P., and Dubovik, O.: Towards Advanced Sentinel-3 Near Real Time (NRT) L2 synergy aerosols capabilities - On-going Day 2 & Day 3 developments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18930, https://doi.org/10.5194/egusphere-egu25-18930, 2025.

EGU25-18977 | ECS | Posters on site | AS5.12

Observations informed European Black Carbon emission estimates for 2022 

Saurabh Annadate, Sabine Eckhardt, Stephen Platt, Rona L. Thompson, Ignacio Pisso, Nikolaos Evangeliou, Enrico Mancinelli, Jgor Arduini, and Michela Maione

Black Carbon (BC) is an important aerosol species with a strong positive radiative forcing and severe health impacts. In the last decades, the enforcement of European air quality policies has reduced aerosol ambient levels and altered aerosol composition, with implications on aerosol-radiation interaction. Therefore, a comprehensive BC emission inventory is needed for a good understanding of the radiative forcing and associated climate feedback. It is also critical to minimize the uncertainty in predicting the current and future climate influence of BC. Under the Horizon Europe project Process Attribution of Regional Emissions (PARIS), in collaboration with the sister project Verifying Emissions of Climate Forcers (EYE-CLIMA), we aim to provide a top-down, observation-informed estimate of European BC emissions.

In this study, we used inverse modelling to derive emission estimates of BC using the FLEXPART transport model and the FLEXINVERT Bayesian inversion framework. Here, we present our initial results for 2022, utilising harmonised BC observations from 14 European measurement sites operated under the ACTRIS network. We employed different bottom-up emission inventories from ECLIPSE, EDGAR-HTAP, and LRTAP as prior emissions. The inversion results showed a pronounced seasonality in BC emissions, with peaks during winter, likely driven by increased residential combustion activities. Significantly high emissions were estimated in March compared to other months, with the majority of emissions originating from central and southeastern Europe. The high emissions were in line with the large number of wildfires reported in this region.

 

How to cite: Annadate, S., Eckhardt, S., Platt, S., Thompson, R. L., Pisso, I., Evangeliou, N., Mancinelli, E., Arduini, J., and Maione, M.: Observations informed European Black Carbon emission estimates for 2022, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18977, https://doi.org/10.5194/egusphere-egu25-18977, 2025.

EGU25-19313 | Posters on site | AS5.12

Aerosol layer height constrained by micro-lidar to enhance space borne push-broom spectrometer measurements of CH4 and CO2 

Daria Stepanova, Errico Armandillo, Marcos Herreras-Giralda, Oleg Dubovik, Anton Lopatin, Sergio Tomás, Manuel Queißer, and David Vilaseca

The greenhouse gases (GHG) methane (CH4) and carbon dioxide (CO2) have been emitted at an increasing rate since the Industrial Revolution, leading to amplified global warming. The Paris agreement, signed by 175 nations, represents the world’s first sound political framework to regulate GHG emissions. It entails a need to quantify GHG fluxes, ideally with global coverage. 

Since the pioneering missions able to detect and quantify trace gases in the Troposphere, green gas monitoring instrument (GMI) and scanning imaging absorption spectrometer for atmospheric cartography (SCIAMACHY) almost 30 years ago, a number of satellite missions that provide global coverage have been launched and are used to serve that need. There is, however, a significant discrepancy between bottom-up GHG emission estimates from inventories and top-down estimates using a combination of space-borne GHG concentration measurements and atmospheric dispersion modeling. Over the last 12 years or so, a new generation of satellites-borne imaging spectrometers emerged with sub-kilometre pixel resolution, able to map trace gas plumes and thus able to quantify GHG fluxes directly at the source, contributing to improved GHG inventories. Among those are the first commercial Earth observation missions to monitor GHG sources.

The commercial AIRMO mission aims to quantify GHG fluxes, notably CH4, in the planetary boundary layer, over regions that may contain significant aerosol concentrations, such as sulfate, marine and desert aerosols and aerosols from biomass burning. These aerosols exhibit extinction of solar photons by scattering and absorption, which may significantly modify the path of solar photons so that apparent and actual column lengths differ, leading to a possible over or underestimation of GHG column densities from passive spectroscopy. 

To correct for this bias in the retrieval algorithm, employing full physical modeling of light extinction by aerosols in the forward model is envisaged. Sensitivity tests are performed using the GRASP (Generalized Retrieval of Atmosphere and Surface Properties) retrieval and simulation code to assess the sensitivity of three crucial model parameters: The aerosol concentration parametrized as aerosol optical depth (AOD), the bidirectional surface reflectance (BRDF) and the aerosol layer height (ALH). A conceptually straightforward way to constrain the model aerosol parameters is a lidar co-located to the spectrometer, operating in a spectral region where the gases of interest have absorption lines. Consequently, a pulsed micro-lidar is simulated as a tool to constrain ALH. The benefits of this input information in the retrieval against methodologies based on oxygen A-band absorption bands are assessed. Furthermore, work is underway that assesses the overall benefits of the lidar, including those for other model parameters and mission objectives.

How to cite: Stepanova, D., Armandillo, E., Herreras-Giralda, M., Dubovik, O., Lopatin, A., Tomás, S., Queißer, M., and Vilaseca, D.: Aerosol layer height constrained by micro-lidar to enhance space borne push-broom spectrometer measurements of CH4 and CO2, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19313, https://doi.org/10.5194/egusphere-egu25-19313, 2025.

EGU25-19758 | Posters on site | AS5.12

High-Resolution Retrieval of Local Road Emissions from Coarse Satellite Images Using CFD Modeling 

Konstantin Kuznetsov, Oleg Dubovik, Pavel Livinov, and David Fuertes

Accurately quantifying local road emissions is crucial for understanding urban air quality and its health impacts. This study presents a novel approach for retrieving high-resolution emissions data, achieving up to 1-meter resolution, from relatively coarse resolution satellite images (500 meters). The methodology integrates Computational Fluid Dynamics (CFD) to simulate wind fields and pollution dispersal from selected road segments in complex urban conditions.
The model is based on several key assumptions: emission rates remain constant along each road segment, pollution dynamics are treated as a passive scalar without considering chemical transformations, and the pollution field within the domain is defined solely by the selected road segments and boundary conditions. The CFD simulation covers a domain of 1km by 1km with a vertical extent of 800 meters, achieving a resolution of 1 meter near buildings to accurately capture fine-scale variations in the pollution field, different surface types are using in this model: buildings, water, vegetations and roads. 
For each road segment, we calculate the Aerosol Optical Depth (AOD) from the pollution field. Given that the pollution patterns are linear with respect to the velocity field, we can scale the pollution field according to emission values, allowing for flexible adaptation to varying emission rates. Our approach considers the 25 largest road segments, constructing a basis set from their respective AOD patterns. By using a linear combination of these AOD patterns, we develop a regression model where the weights correspond to the emission values for each road segment.
To solve this regression problem, we employ the Non-Negative Least Squares (NNLS) method, ensuring physically plausible, non-negative emission values. This technique provides a robust and scalable framework for transforming coarse satellite imagery into high-resolution emission maps, significantly enhancing the spatial granularity and accuracy of urban air quality assessments. Our approach represents a significant advancement in environmental monitoring, offering valuable insights for urban planners and policymakers aiming to mitigate pollution and improve air quality.

How to cite: Kuznetsov, K., Dubovik, O., Livinov, P., and Fuertes, D.: High-Resolution Retrieval of Local Road Emissions from Coarse Satellite Images Using CFD Modeling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19758, https://doi.org/10.5194/egusphere-egu25-19758, 2025.

EGU25-20416 | ECS | Orals | AS5.12

Hourly Seamless Retrieval of Near-Surface PM2.5 and O3 Concentrations across China from 2018 to 2023 

Lin Zang, Yuqing Su, Yi Zhang, Feiyue Mao, and Zengxin Pan

In recent years, China’s air pollution control efforts have significantly reduced fine particulate matter (PM2.5) concentrations. However, ozone (O3) pollution has emerged as a key issue, becoming the second major pollutant affecting air quality. During certain periods, simultaneous high concentrations of PM2.5 and O3 lead to “dual-high” compound pollution. Understanding the dynamic evolution of these pollutants is essential for precise control strategies.

Existing observational data on PM2.5 and O3 are insufficient for research and applications. Ground-based monitoring stations provide temporally continuous data but have limited spatial coverage, while geostationary satellites offer wide spatial coverage but suffer from data gaps due to cloud interference, retrieval algorithm limitations, and the lack of nighttime observations. These challenges highlight the need for spatiotemporally continuous, all-weather data.

This study develops a high-precision retrieval model for near-surface PM2.5 and O3 concentrations, integrating AI algorithms with multispectral data from Himawari-8/9, reanalysis meteorological data, and geographic parameters. By incorporating the spatiotemporal autocorrelation of pollutants as a physical constraint, the model innovatively combines Gaussian smoothing adjustment and discrete cosine transform to create a data fusion framework. This framework generates seamless, all-weather datasets, addressing data gaps and correcting systematic biases in satellite retrievals.

Independent validation shows strong model performance, with hourly R² values exceeding 0.85. Using retrieval results from 2018 to 2023, we analyzed the spatiotemporal distribution of PM2.5 and O3 across four major urban agglomerations in China (Beijing-Tianjin-Hebei, Yangtze River Delta, Pearl River Delta, and Central China) before, during, and after the COVID-19 outbreak. The findings reveal the effects of emission reductions and the post-pandemic pollution recovery.

This study demonstrates the potential of integrating remote sensing, AI, and mathematical modeling to achieve spatiotemporally continuous monitoring of PM2.5 and O3. It offers critical support for air pollution control and environmental policy evaluation.

How to cite: Zang, L., Su, Y., Zhang, Y., Mao, F., and Pan, Z.: Hourly Seamless Retrieval of Near-Surface PM2.5 and O3 Concentrations across China from 2018 to 2023, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20416, https://doi.org/10.5194/egusphere-egu25-20416, 2025.

EGU25-20466 | Posters on site | AS5.12

Real-time environmental monitoring system architecture using distributed networks of low-cost and high-end sensors combined with remote sensing and data assimilation  

Marina Georgiou, Ilias Romas, Chrysoula Papathanasiou, Marios Vlachos, Marios Sophocleous, Kleanthis Erotokritou, Eleni Drakaki, Georgios Grivas, Panagiotis Kosmopoulos, Mehrdad Ghanad, Hesham Al-Askary, Omar Elbadawy, Petros Mouzourides, Giorgos Alexandrou, Minučer Mesaroš, Francisco Alcalá, and Raúl Segura

The impacts of climate change on desert ecosystems are profound and far-reaching, influencing not only local environments but also neighbouring regions, where dust storms transport pollutants and particulate matter over thousands of kilometers. These phenomena pose significant challenges to environmental monitoring and policy-making, requiring innovative approaches to data collection and analysis. In the Horizon Europe CiROCCO project, we have adopted an approach ensuring comprehensive environmental monitoring by leveraging the strengths of high-end sensors offering precise and reliable measurements and low-cost sensors, enabling extensive spatial coverage and high-frequency data acquisition. This integration creates a robust and scalable network, which enhance data accuracy and consistency, can support real-time monitoring and long-term environmental research and conservation efforts. The CiROCCO system architecture has been designed to facilitate the deployment and exploitation of this advanced monitoring framework across diverse environments, addressing the specific needs of four pilot sites in Cyprus, Egypt, Serbia and Spain. It incorporates state-of-the-art data fusion techniques, remote sensing integration, and a flexible modular design, ensuring adaptability to various ecological and socio-economic contexts. Our presentation will provide an overview of the CiROCCO system architecture, emphasising its potential to support not only environmental conservation and research but also evidence-based policy-making and climate adaptation strategies.

Acknowledgement:

The CiROCCO project is funded by the European Union’s Horizon Europe Programme. Views and opinions expressed are, however, those of the author(s) only and do not necessarily reflect those of the European Union or REA. Neither the European Union nor the granting authority can be held responsible for them.

How to cite: Georgiou, M., Romas, I., Papathanasiou, C., Vlachos, M., Sophocleous, M., Erotokritou, K., Drakaki, E., Grivas, G., Kosmopoulos, P., Ghanad, M., Al-Askary, H., Elbadawy, O., Mouzourides, P., Alexandrou, G., Mesaroš, M., Alcalá, F., and Segura, R.: Real-time environmental monitoring system architecture using distributed networks of low-cost and high-end sensors combined with remote sensing and data assimilation , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20466, https://doi.org/10.5194/egusphere-egu25-20466, 2025.

EGU25-20475 | Orals | AS5.12

Polarimetric measurements for characterization of aerosol properties with CIMEL instruments: photometer and LiDAR 

Stephane Victori, Ioana Popovici, Philippe Goloub, Luc Blarel, Thierry Podvin, Maria Fernanda Sanchez Barrero, Yenny Gonzalez Ramos, Qiaoyun Hu, and Igor Veselovskii

CIMEL is well known for its CE318 photometer, equipping AERONET network. The polarized sun/sky/lunar photometer (CE318-TP) is maybe less known, but it offers polarization measurements in 9 channels in a wide spectral range (340-1640 nm) and it has been shown to improve the retrieval of the real part of the refractive index, the fine mode of the size distribution and the particle shape parameter, especially for small particles, and to reduce inversion errors by 30% [1,2]. If polarizers alignment issues have been observed in the mechanical setup before, on older instruments, these have been addressed, leading to improved polarization measurements accuracy in current instruments. We believe that commercial polarized photometers such as the CE318-TP can be a key tool for ground-based validation of future polarimetric space missions. On the vertical scale of the atmosphere, lidars equipped with polarization channels offer insights into the discrimination of aerosol types vertically: dust, ash, smoke etc. We produce two types of polarization lidars. The CE376-GPN lidar (GP stands for Green Polarized, N for near-infrared channel), which is a compact, eye-safe, automatic dual-wavelength, polarization lidar, demonstrating its capability to distinguish dust from smoke in several observations in Lille, France [3] and the CE710 high power lidar, a multi-wavelength polarization, fluorescence lidar, giving access to advanced aerosol research in complex scenarios, with 3 depolarization channels at 355, 532 and 1064 nm and which allowed to study the depolarization of aerosol fluorescence and water vapor Raman backscatter [4].

Finally, a 360°x180° linearly polarized filter-based fisheye camera funded by ESA is being developed in order to help the satellite community with instantaneous sky and sun measurements. In this work, we propose to present examples of real measurements from our panel of polarimetric instruments and what added value they bring to the aerosol community and for future polarimetric space missions.

References

[1] Li, Z., Goloub, P., Dubovik, O., Blarel, L., Zhang, W., Podvin, T., et al., 2009: Improvements for ground-based remote sensing of atmospheric aerosol properties by additional polarimetric measurements. JQRST 110, issue 17, 1954-1961.

[2] Fedarenka, A., Dubovik, O., Goloub, P., Li, Z., et al., 2016: Utilization of AERONET polarimetric measurements for improving retrieval of aerosol microphysics: GSFC, Beijing and Dakar data analysis. JQRST 179, 72-97.

[3] Sanchez Barrero, M. F., Popovici, I. E., Goloub, P., Victori, S., Hu, Q., et al., 2023: Enhancing mobile aerosol monitoring with CE376 dual-wavelength depolarization lidar, EGU sphere [preprint], https://doi.org/10.5194/egusphere-2023-2579

[4] Veselovskii, I., Hu, Q., Goloub, P., Podvin, T., Boissiere, W., et al., 2024: Derivation of depolarization ratios of aerosol fluorescence and water vapor Raman backscatters from lidar measurements, Atmos.Meas. Tech., 17, 1023–1036.

How to cite: Victori, S., Popovici, I., Goloub, P., Blarel, L., Podvin, T., Sanchez Barrero, M. F., Gonzalez Ramos, Y., Hu, Q., and Veselovskii, I.: Polarimetric measurements for characterization of aerosol properties with CIMEL instruments: photometer and LiDAR, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20475, https://doi.org/10.5194/egusphere-egu25-20475, 2025.

EGU25-20704 | Posters on site | AS5.12

ARM Mobile Observatory Recent and Field Studies 

Heath Powers

The U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) user facility aims to improve climate and earth system models through providing detailed observations of the atmosphere to the scientific community.  These observations are provided by ARM's atmospheric observatories which combine dozens of remote and in situ sensors for characterizing many atmospheric parameters relating to clouds, precipitation, aerosols, and radiation balance.  This presentation will focus on the recent and upcoming deployments of two of ARM's ground based observatories, the ARM Mobile Facility (AMF) 1 & 2.  These AMFs travel the globe to collect observations from diverse regions and meteorological regimes through proposal-driven deployments.  This will focus on studies in Houston, Texas, USA,; La Jolla, California, USA; Tasmania, Australia, and upcoming deployments of ARM’s AMFs.  

How to cite: Powers, H.: ARM Mobile Observatory Recent and Field Studies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20704, https://doi.org/10.5194/egusphere-egu25-20704, 2025.

EGU25-1170 | ECS | Posters on site | AS5.13

1.57μm Active Laser Heterodyne Spectrometer and CO2 Concentration Measurement 

Xingji Lu, Yinbo Huang, Zhengsong Cao, Haiping Mei, Chaolong Cui, Jun Huang, and Yao Huang

CO2 is an important greenhouse gas(GHG) that affects the Earth's atmosphere, and continuous measurement of CO2 helps understand its sources and sinks. The passive laser heterodyne spectrometer(LHS) has been used in meteorology and environmental monitoring recently, especially in the measurement of the radiation properties of the Earth and the densities of atmospheric greenhouse gases. As well known, the passive LHS uses sunlight, the heterodyne efficiency is low, the heterodyne signal processing is complex, and it cannot be measured without sunlight. Therefore, it is difficult for passive LHS to achieve continuous measurement of the GHG of interest. In order to improve the application field of LHS, a 1.57 μm active LHS is investigated and built by using a tunable DFB laser, acoustic-optic frequency shifter and fiber amplifier. It adopts the reflected laser after amplified and frequency shifted as the input light and mixed with seed laser, which possesses the advantage of high coherence efficiency and continuous observation day and night. The CO2 absorption spectrum measurement in the range of 2.2 km is realized, and the signal-to-noise ratio is about 286. The densities of CO2 are 419.15 ~ 424.48ppmv during the experiment. The research will make up for the deficiency of the passive laser heterodyne spectrometer.

How to cite: Lu, X., Huang, Y., Cao, Z., Mei, H., Cui, C., Huang, J., and Huang, Y.: 1.57μm Active Laser Heterodyne Spectrometer and CO2 Concentration Measurement, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1170, https://doi.org/10.5194/egusphere-egu25-1170, 2025.

EGU25-2361 | Posters on site | AS5.13

High-performance data acquisition and processing system based on SOM-FPGA and its application in optical instruments 

Weixiong Zhao, Shichuan Ni, Jiacheng Zhou, Weijun Zhang, and Weidong Chen

An ideal data acquisition and processing system has the characteristics of high integration, low latency, wide applicability, and scalability. Its development plays a vital role in the advancement of optical instruments. Most of the data acquisition and processing systems currently used are based on digital signal processing (DSP) or system-on-chip (SoC) architectures, which are limited in processor performance, number of interfaces, and edge computing capabilities. In this presentation, we report a data acquisition system (SOM-FPGA lock-in, SFLI) based on modular system-on-module (SOM) and field-programmable gate array (FPGA) architecture. The SFLI system integrates high-speed signal acquisition and processing, digital lock-in amplifier (DLIA), and edge data storage functions, improves the edge computing capability of the system, and has the advantages of high performance, multiple interfaces, and low cost. The system can simultaneously achieve four-channel high-speed acquisition (sampling rate up to 65 MSPS) and digital phase sensitive detector (demodulation frequency from DC to 5 MHz). When the modulation frequency is 20 kHz and the input voltage range is 1 V, the input voltage noise of the SFLI system is about 41 nV/√Hz. The performance of the SFLI system is compared with that of a commercial lock-in amplifier, showing good consistency. The SFLI has been applied to cavity-enhanced spectroscopy technology, providing a new solution for the miniaturization of optical instruments and edge computing in practical applications.

How to cite: Zhao, W., Ni, S., Zhou, J., Zhang, W., and Chen, W.: High-performance data acquisition and processing system based on SOM-FPGA and its application in optical instruments, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2361, https://doi.org/10.5194/egusphere-egu25-2361, 2025.

EGU25-4475 | ECS | Posters on site | AS5.13

Optical sensing platform based on tunable laser absorption spectroscopy for the measurement of carbon dioxide dissolved in seawater 

Yongyong Hu, Patrick Augustin, Jingjing Wang, Kun Liu, Ruyue Cui, Hongpeng Wu, Lei Dong, Xiaoming Gao, Marc Fourmentin, Tong Nguyen Ba, and Weidong Chen

Ocean-atmosphere gas exchange plays a critical role in the global carbon cycle, as the ocean acts as both a major sink and source of atmospheric CO2. This exchange process regulates the Earth's carbon balance and influences climate systems on a global scale. Understanding the mechanisms of CO2 absorption and release at the ocean surface is essential for accurately assessing the ocean’s contribution to carbon fluxes [1].

The present work introduces the development of a optical sensor based on Tunable Diode Laser Absorption Spectroscopy (TDLAS) for measurement of CO2 dissolved in seawater. This approach enables real-time measurement of CO2 concentrations in seawater for evaluation of CO2 distribution and study of exchange processes between ocean and atmosphere. The developed sensing platform involves a 2008 nm distributed feedback laser coupled to a compact 30-m multipass cell with 7-circle spot dense pattern [2] using wavelength modulation spectroscopy approach [Figure 1]. CO2 dissolved in seawater is extracted using a custom-designed membrane contactor extraction device.

Figure 1. Experimental measurements of 2f absorption spectra of CO2 in air and dissolved in seawater.

Performance of the CO2 sensing platform, experimental details and the preliminary results will be discussed and presented.

 

Acknowledgments

This work is partially supported by the French national research agency (ANR) under the Labex CaPPA (ANR-10-LABX-005) and the ICAR-HO2 (ANR-20-CE04-0003) contracts, the EU H2020-ATMOS project (Marie Skłodowska-Curie grant agreement No 872081), the regional CPER ECRIN program, and the National Natural Science Foundation of China (Grant No. 62235010). The Région Hauts-de-France and the Pôle Métropolitain de la Côte d’Opale are gratefully acknowledged for PhD scholarship support.

 

References

[1] Tim DeVries, “The ocean carbon cycle”, Annual Review of Environment and Resources 47 (2022) 317-341.

[2] Kun Liu, Lei Wang, Tu Tan, Guishi Wang, Weijun Zhang, Weidong Chen, Xiaoming Gao, “Highly sensitive detection of methane by near-infrared laser absorption spectroscopy using a compact dense-pattern multipass cell”, Sensors and Actuators B: Chemical 220 (2015) 1000-1005.

How to cite: Hu, Y., Augustin, P., Wang, J., Liu, K., Cui, R., Wu, H., Dong, L., Gao, X., Fourmentin, M., Nguyen Ba, T., and Chen, W.: Optical sensing platform based on tunable laser absorption spectroscopy for the measurement of carbon dioxide dissolved in seawater, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4475, https://doi.org/10.5194/egusphere-egu25-4475, 2025.

EGU25-6525 | ECS | Posters on site | AS5.13

Subpromille measurements of H2 absorption spectra near 1.2 μm 

Hui Liang, Yan Tan, Jing Wang, and Shui Ming Hu

The molecule hydrogen is the most abundant neutral molecule in the universe and dominates the atmosphere of gas giants in the solar system and beyond. Laboratory-measured spectral data of the hydrogen molecule, including transition absorption (?) frequencies, intensities, and related temperature-/pressure-dependent spectroscopic parameters, are the basis for modeling the planetary atmospheres [1].

The present work is based on two high precision cavity enhanced spectroscopy methods. Both absorption and dispersion spectra were recorded with the same frequency-stabilized cavity-enhanced spectroscopy instrument referenced to an optical frequency comb. Doppler-broadened spectra of the first overtone Q(1) line of the H2 molecule near 1.2 µm were measured in the range of 20-80 kPa. The spectrums were fitted by the Hartmann-Tran profile (HTP) [2], which is suitable for molecule hydrogen analysis. The line intensities obtained by the two methods reached an accuracy of 0.15%, and they agree well with theoretical results [3]. It is the first time that subpromille measurements of a rovibrational transition of the hydrogen molecule have been performed with two different methods. The work paves the way for SI-traceable high-precision molecular density measurements based on laser spectroscopy.

The experimental detail and the data analysis results will be presented and discussed.

 

Acknowledgments

This work was jointly supported by the National Natural Science Foundation of China (Grant Nos. 12393825, 12393822, 22327801, 22241302), the Innovation Program for Quantum Science and Technology (Grant Nos. 2021ZD0303102, 2022YFF0606500), and the Chinese Academy of Sciences (Grant No. YSBR-055).

References

[1] Liu, Q. H., Tan, Y., Cheng, C. F., & Hu, S. M. (2023). Precision spectroscopy of molecular hydrogen. Physical Chemistry Chemical Physics25(41), 27914-27925.

[2] Konefał, M., Słowiński, M., Zaborowski, M., Ciuryło, R., Lisak, D., & Wcisło, P. (2020). Analytical-function correction to the Hartmann–Tran profile for more reliable representation of the Dicke-narrowed molecular spectra. Journal of Quantitative Spectroscopy and Radiative Transfer242, 106784.

[3] Komasa, J., Puchalski, M., Czachorowski, P., Łach, G., & Pachucki, K. (2019). Rovibrational energy levels of the hydrogen molecule through nonadiabatic perturbation theory. Physical Review A100(3), 032519.

How to cite: Liang, H., Tan, Y., Wang, J., and Hu, S. M.: Subpromille measurements of H2 absorption spectra near 1.2 μm, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6525, https://doi.org/10.5194/egusphere-egu25-6525, 2025.

EGU25-6779 | ECS | Orals | AS5.13

The ALBATROSS spectrometer for balloon-borne measurements of UTLS water vapor: Laboratory and in-flight validation 

Simone Brunamonti, Alex Weitnauer, Philipp Scheidegger, Lukas Emmenegger, and Béla Tuzson

The amount of water vapor (H2O) in the upper troposphere-lower stratosphere (UTLS) plays a critical role for the Earth's radiative balance. However, due to its low abundance, accurate measurements of H2O in this region (~8‒25 km altitude) are still very challenging, and large discrepancies were often found between different techniques.

Here, we present the validation of a laser absorption spectrometer, ALBATROSS, specifically developed for balloon-borne measurements of UTLS H2O [1]. ALBATROSS is a compact (< 3.5 kg)  instrument using a continuous-wave (cw) distributed feedback quantum cascade laser (DFB-QCL) emitting at 6.014 μm, and a monolithic segmented circular multipass cell [2] with an optical path length of 6 m within a cell diameter of 10.8 cm. The multipass cell is highly resistant to thermal and mechanical stress, and can be operated both in a closed-path (laboratory) and an open-path (flight) configuration.

The performance of the spectrometer was assessed at UTLS-relevant conditions using SI-traceable reference gases generated by a dynamic-gravimetric permeation method [3]. The results show that ALBATROSS achieves an accuracy better than ±1.5 % with respect to the SI-traceable reference at all investigated pressures (30‒250 mbar) and H2O amount fractions (2.5‒35 ppm), and a precision better than 0.3 % at 1 s resolution. The quadratic speed dependent Voigt profile (qSDVP) line shape model was implemented to assure this level of accuracy using first principles.

Further laboratory-based validation activities included the AquaVIT4 intercomparison of atmospheric hygrometers, held at the AIDA cloud simulation chamber in Karlsruhe, Germany. Here, the performance of four airborne hygromenters, including ALBATROSS, was evaluated under a wide range of challenging environmental conditions (pressure 20‒600 mbar, temperature 190‒245 K, H2O amount fraction 0.5‒530 ppm).

Recently, ALBATROSS was deployed in a series of atmospheric test flights conducted from the Meteoswiss Payerne Observatory (Switzerland), within the framework of the Swiss H2O-Hub project. In tandem with ALBATROSS, a cryogenic frospoint hygrometer (CFH) was also deployed as a reference. Good agreement within ±10 % was found between ALBATROSS and CFH up to about 24 km altitude (~30 mbar pressure).

Altogether, our results demonstrate the exceptional potential of mid-IR laser spectroscopy for in-situ measurements of UTLS H2O. This is particularly relevant considering the ongoing reconception of the CFH method, currently used in long-term climate monitoring networks (e.g., the GCOS reference upper air network, GRUAN), due to its use of fluoroform (HFC-23) as cooling agent, which must be phased out due to its high global warming potential.

[1] Graf et al., Atmos. Meas. Tech., 14, 1365–1378, 2021.

[2] Graf et al., Opt. Lett., 43, 2434-2437, 2018.

[3] Brunamonti et al., Atmos. Meas. Tech., 16, 4391–4407, 2023.

How to cite: Brunamonti, S., Weitnauer, A., Scheidegger, P., Emmenegger, L., and Tuzson, B.: The ALBATROSS spectrometer for balloon-borne measurements of UTLS water vapor: Laboratory and in-flight validation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6779, https://doi.org/10.5194/egusphere-egu25-6779, 2025.

EGU25-6846 | ECS | Orals | AS5.13

Laboratory Spectroscopy and Optical Metrology Approaches for Analysis of Atmospheric Constituents 

D. Michelle Bailey, Eric Crump, Joseph Hodges, and Adam Fleisher

Successful evaluation of atmospheric gas composition relies on complementary efforts from experimental campaigns, laboratory metrology, and quantum chemistry theory. When these three areas work in concert, we significantly improve our ability to accurately describe atmospheric composition and understand atmospheric chemical behavior. Here we will discuss techniques employed in NIST’s Optical Measurements Group to perform precise gas sample analysis and provide reference-grade spectroscopic data that is critical for Earth and exoplanet atmosphere observations.

First, we will discuss direct frequency comb spectroscopy (DFCS) methods. A cross-dispersed technique has been demonstrated in the mid-infrared spectral region for rapid and precise measurement of isotopic abundance of nitrous oxide [1] which is the third leading contributor to radiative forcing in Earth’s atmosphere. Leveraging fundamental molecular transitions near 4.5 µm, we can employ a small-volume gas cell with short (7 cm) optical pathlength to analyze pure gas samples. This presentation will introduce initial measurements of nitrous oxide community reference materials [2] which can be used for maintaining isotope abundance scales, a key metrology challenge when discerning and disseminating gas analysis results. Additionally, we will introduce near-infrared DFCS studies focused on benchmarking hydrogen cyanide (HCN) molecular line lists [3] which are relevant for Earth and exoplanetary observing systems that use HCN as a tracer for chemical or physical processes.

Further, we will highlight cavity ring-down (CRD) techniques that provide spectroscopic reference data that describe fundamental physical attributes of atmospheric constituents. These parameters, including molecular transition intensity, are necessary for accurate spectroscopic modelling and can impact the accuracy of experimental retrievals. Here, we will present ultra-precise mid-infrared CRD measurements enabled by state-of-the-art hybrid crystalline mirrors. [4] Recent experimental results for a carbon monoxide transition intensity in the fundamental band will be discussed.

[1] D. M. Bailey, G. Zhao, and A. J. Fleisher, Anal. Chem. 2020, 92 (20), 13759–13766

[2] J. Mohn et al., Rapid Commun. Mass Spectrom. 2022, 36 (13), e9296

[3] D. M. Bailey, E. M. Crump, J. T. Hodges, and A. J. Fleisher, Faraday Discuss. 2023, 245, 368-379

[4] GW. Truong et al., Nat. Comms. 2023, 14, 7846

How to cite: Bailey, D. M., Crump, E., Hodges, J., and Fleisher, A.: Laboratory Spectroscopy and Optical Metrology Approaches for Analysis of Atmospheric Constituents, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6846, https://doi.org/10.5194/egusphere-egu25-6846, 2025.

Fourier Transform Infrared (FTIR) spectroscopy faces significant challenges in detecting volatile organic compounds (VOCs) within complex environments due to cross-absorption and spectral overlap among components. To address these challenges, an enhanced nonlinear least squares algorithm (SN-NNLS) that integrates sparsity and non-negativity constraints is proposed. The sparse regularization term effectively separates gas components with overlapping absorption features, improving the accuracy of multi-component analysis. Meanwhile, the non-negativity constraint ensures physically meaningful results by eliminating negative concentration estimates, enhancing the reliability of the outcomes. Additionally, the algorithm incorporates dynamic polynomial degree adjustments and nonlinear correction techniques to handle the nonlinear characteristics of diverse spectral datasets, further enhancing its adaptability and robustness. Experimental results demonstrate that the SN-NNLS algorithm significantly improves the precision, stability, and robustness of VOC concentration measurements. This method offers a reliable and efficient solution for quantitative infrared spectral analysis in complex environments.

How to cite: Qin, Y.: Sparsity and Non-Negativity Constrained FTIR Spectroscopic Analysis for VOC Detection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8094, https://doi.org/10.5194/egusphere-egu25-8094, 2025.

EGU25-9240 | Posters on site | AS5.13

A net ozone production rate detection system based on dual-channel cavity ring-down spectroscopy 

Renzhi Hu, Chuan Lin, Haotian Cai, Guoxian Zhang, Jinzhao Tong, and Pinhua Xie

A newly constructed cavity ring-down spectroscopy (OPR-CRDS) for measuring net photochemical ozone production rates was developed. The system consists of two chambers (a reaction chamber and a reference chamber) and a dual-channel Ox-CRDS detector. The inner surfaces of both chambers are coated with Teflon film to minimize the wall loss of Ox. It was found that even though the photolysis frequency (J value) decreased by 10%, the decrease in the P(O3) caused by the ultraviolet-blocking film coating was less than 3%. The two chambers had a good consistency in the mean residence time and the measurement of NO2 and Ox under the condition of no sunlight. The detection limit of the OPR-CRDS was determined to be 0.20 ppbv/hr. To further verify the accuracy of the system, the observed values of the OPR-CRDS were compared with the calculation results based on radical (OH, HO2, and RO2) reactions, and a good correlation was obtained. Finally, the developed instrument was applied to the comprehensive field campaign at an urban site in the Yangtze River Delta (China), the time series and change characteristics of the P(O3) were required directly, and the good environmental adaptability and stability of the OPR-CRDS system were demonstrated. It is expected that the new instrument will be beneficial to investigations of the relationship between P(O3) and its precursors.

How to cite: Hu, R., Lin, C., Cai, H., Zhang, G., Tong, J., and Xie, P.: A net ozone production rate detection system based on dual-channel cavity ring-down spectroscopy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9240, https://doi.org/10.5194/egusphere-egu25-9240, 2025.

EGU25-9415 | ECS | Orals | AS5.13

A dual-comb spectrometer for open-path monitoring of greenhouse gases concentrations above an urban area  

Romain Dubroeucq, Tobias D. Schmitt, André Butz, Thomas Pfeifer, and Markus Oberthaler

Remote sensing of trace gases in the atmosphere can be performed with numerous spectrometers relying on different sources of light. Incoherent sources such as those found with typical Fourier transform spectrometers provide broad spectral coverage, thus allowing to measure spectral signatures from multiple species simultaneously. However, this comes at the cost of limited sensitivity and spectral resolution. On the other hand, coherent sources such as lasers offer high spectral brightness and resolution, resulting in high sensitivity and selectivity at the cost of limited spectral coverage. Developed since the advent of the optical frequency comb (OFC) 25 years ago, state-of-the-art spectrometers operating with OFCs as probing light sources combine high sensitivity, high spectral resolution and broad spectral bandwidth. Among all comb-based spectroscopic techniques, dual-comb spectroscopy (DCS) does not require any dispersive or moving optical component to record a spectrum, allowing for relatively small footprints and mechanically robust instruments. This makes dual-comb spectrometers particularly suited for remote sensing [1] and field-deployed operation outside of the optical laboratory [2].

Here, we present the recent technical developments of a near-infrared dual-comb spectrometer for open-path monitoring of greenhouse gases above the city of Heidelberg. The instrument is located at the top of the Institute of Environmental Physics in Heidelberg University campus. The light from two fibered OFCs, spanning 1.58-1.7 µm, is coupled into free space with a telescope, and propagates along a 1.5 km path to a retroreflector array. The reflected signal is picked up by the telescope and coupled back into fiber for detection and data acquisition. We discuss performance of the instrument and the results of our upcoming measurement campaign.

[1] G. B. Rieker et al., "Frequency-comb-based remote sensing of greenhouse gases over kilometer air paths," Optica 1, 290-298 (2014), DOI: 10.1364/OPTICA.1.000290.

[2] S. Coburn et al., "Regional trace-gas source attribution using a field-deployed dual frequency comb spectrometer," Optica 5, 320-327 (2018), DOI: 10.1364/OPTICA.5.000320.

How to cite: Dubroeucq, R., Schmitt, T. D., Butz, A., Pfeifer, T., and Oberthaler, M.: A dual-comb spectrometer for open-path monitoring of greenhouse gases concentrations above an urban area , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9415, https://doi.org/10.5194/egusphere-egu25-9415, 2025.

EGU25-12911 | ECS | Posters on site | AS5.13

Spectroscopy of gas plumes in the laboratory: remote sensing of comets and icy satellites 

Dominik Belousov, Omar Mokhtari, Linus Stöckli, Joël Fritschi, Daniele Piazza, Axel Murk, and Nicolas Thomas

Radiometry is a highly accurate technique of gas spectroscopy, widely used in observations of stellar objects (e.g., molecular clouds, accretion discs), planetary atmospheres, comets and icy satellites. Since observations are usually made far from the object, the spectrum detected is a combination of many gas layers lying between the gas source and the observer. Thus, gas models are needed to properly fit observations, which becomes especially challenging in optically thick layers and with large gradients in gas profiles. In addition, optically thick layers can mask the properties of the gas source which have a direct connection with chemical and physical conditions of subsurface layers. 

Our project, called WEEVIL (the Water Emission of Vapour from Ice in the Laboratory), concerns the spectroscopy of gas plumes arising from the sublimation of icy, porous and dusty media in controlled laboratory experiments, following [1]. Project objectives are: 1) verification/correction of subsurface models of icy bodies by comparing laboratory and space observations; 2) studying the capabilities of radiometry for determining subsurface material properties.  

A heterodyne radiometer operating primarily at the frequency of 557 GHz (water rotational line) is being used to investigate column densities, production rates, temperatures, and outflow gas velocities of sublimed icy samples. An internal cooling system using liquid nitrogen and a cryocooler ensures stable temperature of the sample and radiometer compounds, and mitigates the impact of the vacuum chamber on the gas plume. The radiometer has been developed/procured and is undergoing the necessary sensitivity tests. The vacuum chamber is in the final design/production stage. Measured brightness temperatures by the radiometer will be compared with DSMC (direct simulation Monte Carlo) of gas and radiative transfer calculations. The radiative transfer model includes time dependence due to gas expansion and non-LTE due to non-collisional background, following [2]. 

[1] O. Auriacombe et al. 2022 MNRAS 515 

[2] M. A. Cordiner et al 2022 ApJ 929 38 

 

How to cite: Belousov, D., Mokhtari, O., Stöckli, L., Fritschi, J., Piazza, D., Murk, A., and Thomas, N.: Spectroscopy of gas plumes in the laboratory: remote sensing of comets and icy satellites, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12911, https://doi.org/10.5194/egusphere-egu25-12911, 2025.

EGU25-13275 | ECS | Posters on site | AS5.13

New experimental measurements of the Collision-Induced Absorptions of H2-H2 and H2-He in the 3600-5500 cm-1 spectral range from 120 to 500 K   

Francesca Vitali, Stefania Stefani, Giuseppe Piccioni, Marcel Snels, Davide Grassi, David Biondi, and Angelo Boccaccini

The atmospheres of the gaseous and icy giant planets represent a high-density environment, whose composition is generally dominated by H2 and He.

Consequently, the H2 Collision-Induced Absorption (CIA) represents one of the main sources of opacity in the near-infrared spectral range between 1 and 5 μm, a spectral range widely used by remote sensing instruments.

To reduce the retrieval uncertainty of the atmospheric gases, it is very important to have experimental data on the CIA absorption compared with the available theoretical models. These models are necessary in any case where these are missing due to technological limits in the lab.

We measured in our lab the H2 CIA fundamental band in the [3600, 5500] cm-1 spectral range using an experimental setup called PASSxS (Planetary Atmosphere Simulation for Spectroscopy) (Snels et al, 2021).

This setup consists of a simulation chamber that contains a Multi-Pass cell coupled with a Fourier spectrometer and aligned to reach an optical path of 3.28 m. The chamber can be heated up to 550 K, cooled down to 100 K, and sustain pressures up to 70 bar.

We measured the H2-H2 and H2-He binary absorption coefficients for temperatures going from 120 to 550 K by using a pure H2 gas and an H2-He mixture, as shown in Figures 1 and 2.

Figure 1: H2-H2 binary absorption coefficients

Figure 2: H2-He binary absorption coefficients

A large water vapor absorption can be noted on the band’s wings, highlighted by the two light blue rectangles.

The results obtained have been recently published (Vitali et al., 2024) and the data can be downloaded from the Zenodo platform at the following link https://doi.org/10.5281/zenodo.13142014.

Those measurements can be of particular interest in the field of planetary atmospheres since they can be recombined to obtain the total absorption coefficients, at a fixed temperature, of a H2-He mixture for any desired mixing ratio.

Moreover, these are essential input parameters when using radiative transfer models such as the NASA Planetary Spectrum Generator (PSG).

We plan to extend the investigation of the CIA in a wider spectral range, including the [7500, 9500] cm-1 range interested by the H2 CIA first overtone band, with a more detailed temperature scale for both spectral ranges.

Figures 1 and 2 show the so-called interference dips (Van Kranendonk, 1968) around 4150 cm-1 and 4700 cm-1, which represent a lack of absorption at specific wavelengths not taken into account by the CIA models.

A further investigation of the density dependence of those features is already in progress, by exploiting the new Fourier spectrometer at a higher spectral resolution and the entire optical path in vacuum.

We plan to perform high-resolution measurements at different densities using both a pure H2 gas and a H2-He mixture. We will use the line profile developed by Van Kranendonk to study the dependence of the inter-collisional halfwidth on density. Finally, we will also investigate the dip’s behavior while varying the He mixing ratio.

Acknowledgments: This work has been developed under the ASI-INAF agreement n. 2023-6-HH.0.

How to cite: Vitali, F., Stefani, S., Piccioni, G., Snels, M., Grassi, D., Biondi, D., and Boccaccini, A.: New experimental measurements of the Collision-Induced Absorptions of H2-H2 and H2-He in the 3600-5500 cm-1 spectral range from 120 to 500 K  , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13275, https://doi.org/10.5194/egusphere-egu25-13275, 2025.

EGU25-13660 | ECS | Posters on site | AS5.13

A compact light weight instrument for in situ detection of I2 in the marine boundary layer 

Shogo Saito, Caroline Womack, Steven Brown, and Albert Ruth

The release of molecular iodine (I2) from the oceans into the atmosphere has been recognized to correlate strongly with ozone depletion events and aerosol formation in the marine boundary layer [1,2]. The detailed mechanisms and dominant sources leading to the observed concentrations of I2 and IO in the marine troposphere are still under investigation. One prime source of I2 are brown macro-algae (kelp) such as Laminaria digitata, which release molecular iodine when under oxidative stress [3].

In order to further advance the understanding of I2 exchange processes between the sea and atmosphere near the coast, it is essential to map the spatial and temporal distribution of I2 over the shoreline. For that purpose we developed a low power (~20 W), compact, and light weight (~4 kg) instrument for the deployment in field trials on mobile platforms, including unmanned aerial vehicles. The instrument uses incoherent broadband cavity-enhanced absorption spectroscopy (IBBCEAS) [4] for I2 detection, with a molecule-specific 3𝜎 detection limits of 48 pptv in 1 s, as demonstrated under laboratory conditions.

In this presentation, we outline the mechanical, optical, and electronic design of the instrument and discuss its general engineering features. Laboratory measurements of I2 emitted by Laminaria digitata will be presented together with future applications and envisaged field deployments of the instrument.

Acknowledgement: This work is supported by Research Ireland (21/FFP-A-8973, AtmoTrace)

[1] A. Saiz-Lopez, J.M.C. Plane, Novel iodine chemistry in the marine boundary layer, Geophys. Res. Lett. 31, L04112 (2004).

[2] G. McFiggans et al., Direct evidence for coastal iodine particles from Laminaria macroalgae - linkage to emissions of molecular iodine, Atmos. Chem. Phys. 4, 701–713 (2004).

[3] S. Dixneuf et al., The time dependence of molecular iodine emission from Laminaria digitata, Atm. Chem. Phys. 9, 823–829 (2009).

[4] S.E. Fiedler et al. Incoherent broad-band cavity-enhanced absorption spectroscopy, Chem. Phys. Lett. 371, 284–294 (2003).

Key words: Marine boundary layer, iodine I2, iodine oxide IO, macro-algae, cavity enhanced absorption spectroscopy.

How to cite: Saito, S., Womack, C., Brown, S., and Ruth, A.: A compact light weight instrument for in situ detection of I2 in the marine boundary layer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13660, https://doi.org/10.5194/egusphere-egu25-13660, 2025.

EGU25-14245 | ECS | Orals | AS5.13

Single-photon level detection technique of long open-air path dual-comb spectroscopy 

Ruocan Zhao and Jiangtao Li

Optical frequency combs are important tools in the field of quantum precision measurement. Over the past decade, dual-comb spectroscopy technology has been widely applied in Earth sciences, especially in atmospheric laser remote sensing. It has demonstrated significant advantages in measurement accuracy and interference resistance compared to traditional laser remote sensing technologies. This work aims to address the key technical bottlenecks in current open-air dual-comb spectroscopy (DCS) technology for long-distance detection and non-cooperative target conditions, focusing on the application of single-photon weak signal detection technology in dual-comb spectroscopy. By introducing photon counting technology, we can achieve high-resolution spectral measurement under extremely low light conditions, significantly enhancing the detection capability of dual-comb spectroscopy. This work will conduct laboratory and field dual-comb spectroscopy experiments, focusing on the reconstruction of dual-comb interference spectra based on photon arrival times, precise spectral modulation and synchronization of optical frequency combs, and spectral processing and inversion algorithms. The research results will provide strong technical support for atmospheric science, environmental monitoring, and fundamental physics research, and are expected to promote the development of global atmospheric multi-element remote sensing technology.

How to cite: Zhao, R. and Li, J.: Single-photon level detection technique of long open-air path dual-comb spectroscopy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14245, https://doi.org/10.5194/egusphere-egu25-14245, 2025.

EGU25-14308 | ECS | Posters on site | AS5.13

Open-path, portable, low-power laser methane sensor system using miniature multi-pass cell for methane mobile monitoring 

Gang Wang, Ruyue Cui, Yongyong Hu, Hongpeng Wu, Weidong Chen, and Lei Dong

We demonstrated an open-path, portable, low-power laser methane sensor system based on tunable diode laser absorption spectroscopy (TDLAS) and wavelength modulation spectroscopy (WMS) for monitoring methane concentrations in the atmosphere. The design of the open cavity structure accelerates the gas exchange process, reducing the power consumption and weight of additional equipment such as pumps. The portable methane sensor system achieves a methane concentration detection limit of 94 ppb, with dimensions of 22×20×7 cm3, a weight of 1182 g, power consumption of 1.8 W, and a response time of <1 s. To validate the practicality and portability of this sensor system, it was mounted in the front frame of a bicycle and employed for mobile methane monitoring on a campus.

How to cite: Wang, G., Cui, R., Hu, Y., Wu, H., Chen, W., and Dong, L.: Open-path, portable, low-power laser methane sensor system using miniature multi-pass cell for methane mobile monitoring, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14308, https://doi.org/10.5194/egusphere-egu25-14308, 2025.

EGU25-15148 | ECS | Posters on site | AS5.13

A high-resolution microcavity transmission spectrometer 

Bin Yang and Qin Yin

Spectral analysis is one of the most powerful tools for studying and understanding matter. As a key branch, absorption spectroscopy is widely used in material detection, isotope analysis, trace gas detection, and the study of atomic and molecular hyperfine structures. Traditional mode-locked optical frequency combs, which feature broad spectra and low repetition rates, have enabled high-precision absorption measurements through dual-comb techniques. These combs have found applications in trace gas detection, spectral imaging, and isotope analysis. However, their complexity, bulkiness, and large size limit their use outside laboratories. In contrast, low-noise optical frequency combs generated by optical micro-resonators offer significant potential advantages for spectroscopy due to their chip-scale size and lightweight design. We present a microcavity-based transmission spectrometer using a single silicon nitride microcavity soliton, achieving a 4 THz bandwidth with 200 kHz resolution. This system combines the stable dissipative Kerr soliton (DKS) comb from a silicon nitride micro-resonator with the dual-sideband scanning from an intensity electro-optic modulator (EOM), transferring sub-Hz RF precision to the optical domain. The resulting frequency-modulated (FM) comb inherits the high precision of the RF domain, with optical accuracy dominated by the pump laser and repetition rate stability. The DKS comb allows independent locking of the pump laser and repetition rate, facilitating ultra-precise FM comb generation. The frequency-modulated comb is then imaged onto a 2D CCD array using a VIPA in tandem with a diffraction grating, enabling the recording of a composite spectrum during scanning. It is anticipated that using an ultra-narrow linewidth laser locked to an ultra-stable cavity as the pump source could enable Hz-level precision and stability. Given the integration advantages of the key components in this approach, it holds significant potential for future miniaturization, offering vast possibilities for compact, high-precision spectroscopic measurements.

How to cite: Yang, B. and Yin, Q.: A high-resolution microcavity transmission spectrometer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15148, https://doi.org/10.5194/egusphere-egu25-15148, 2025.

EGU25-15173 | ECS | Posters on site | AS5.13

Atomic Oxygen and Temperature Retrieval in the MLT region by Terahertz Heterodyne Measurements from a Satellite: Single vs. Dual-frequency Scenarios 

Peder Bagge Hansen, Martin Wienold, and Heinz-Wilhelm Hübers

Atomic oxygen is a key component of the mesosphere and lower thermosphere (MLT) in Earth's atmosphere. It plays a crucial role in the energy balance and chemical processes within the MLT region, along with the temperature.

The Keystone mission, which is an upper-atmosphere limb-sounding satellite initiative, has entered its phase-0 study [1]. Operating from a low Earth orbit, Keystone will scan the atmosphere at varying tangential heights to measure several atmospheric gases. Most notably, Keystone aims to observe atomic oxygen through its terahertz (THz) fine-structure transitions at 2.1 THz and 4.7 THz. These transitions, being in local thermodynamic equilibrium (LTE), enable the retrieval of vertical atomic oxygen concentration profiles without reliance on photochemical models, but requiring only the local temperature.

The fine-structure transitions of atomic oxygen can be spectrally resolved using heterodyne spectroscopy technology [2,3]. Temperature can then be derived from either the Doppler broadening of these transitions or from the relative intensities of the two transitions, as they originate from distinct upper electronic levels (0.028 eV for the 2.1 THz transition and 0.020 eV for the 4.7 THz transition).

This study evaluates the retrieval uncertainties in temperature and atomic oxygen density for a limb sounding satellite mission such as Keystone. We use the methodology also presented in [4] to compare scenarios with two THz channels measuring both the 2.1 THz and 4.7 THz transitions against those measuring only one transition. For two channels with similar noise levels we find that measuring both transitions improve the precision in atomic oxygen concentration beyond what is gained from the increased signal by using two detectors.

[1] D. Gerber, webpage, https://ceoi.ac.uk/eo-missions/earth-explorer-11/keystone/, visited 14th January 2025.

[2] Richter, H., et al., Commun Earth Environ 2, 19 (2021).

[3] Wienold, M., et al., IEEE Transactions on Terahertz Science and Technology, vol. 14, no. 3 (2024).

[4] Hansen, P., et al., EGU General Assembly 2024, Vienna, Austria, (2024).

How to cite: Hansen, P. B., Wienold, M., and Hübers, H.-W.: Atomic Oxygen and Temperature Retrieval in the MLT region by Terahertz Heterodyne Measurements from a Satellite: Single vs. Dual-frequency Scenarios, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15173, https://doi.org/10.5194/egusphere-egu25-15173, 2025.

EGU25-15608 | Orals | AS5.13

Quartz-Enhanced Photoacoustic Spectroscopy for Environmental Monitoring 

Pietro Patimisco, Andrea Zifarelli, Raffaele De Palo, Mariagrazia Olivieri, Angelo Sampaolo, and Vincenzo Spagnolo

Air pollution is a critical global issue, contributing to over 4.2 million deaths annually due to stroke, heart disease, lung cancer, and chronic respiratory diseases. It also poses significant economic and social challenges, including increased healthcare costs and reduced productivity. The need for real-time, high-resolution air quality monitoring is essential to minimize public exposure, particularly for vulnerable populations. However, existing ambient pollutant detectors are bulky and impractical for widespread deployment, and current electrochemical sensors lack the stability and sensitivity required for regulatory compliance.

In this context, we report the results obtained within the European Project PASSEPARTOUT in advancing the development of miniature, hyperspectral optical sensors based on Quartz Enhanced Photoacoustic Spectroscopy (QEPAS). QEPAS is trace gas optical detection technique that exploits the photoacoustic effect occurring in a gas sample when a modulated, resonant light is absorbed by the target analytes. A weakly damped propagating acoustic (pressure) wave with wavelengths in the centimeter range is generated in the proximity of the exciting light beam. In QEPAS, these sound waves are detected by a spectrophone, composed of a quartz-tuning fork (QTF) transducer and a pair of millimeter-size resonator tubes, aligned on both sides of the QTF.

Eight different air pollutants, namely CH4, NO2, CO2, N2O, CO, NO, SO2 and NH3 have been detected with the same acoustic detection module (containing the spectrophone) and interchangeable laser sources, to prove the modularity of the technique as well as the adaptability to different lasers. Each gas species was detected with an ultimate detection limit well below their typical natural abundance in air even with a signal integration time as low as 0.1 s.

Two significant advancements have also been achieved. The first involves the development of a portable, field-deployable QEPAS sensor that eliminates the need for free-space optical components, thereby increasing the mechanical stability and robustness of the system. By integrating a single-mode fiber to guide the laser beam into the spectrophone, the sensor achieves enhanced flexibility and ease of deployment. The second innovation consists of a custom-designed three-wavelength laser module, combining three quantum cascade lasers (QCLs) into a single collimated beam, further extends the sensor’s capabilities for multi-gas detection with a single sensor architecture.

These advancements pave the way for the deployment of mobile, high-precision air quality monitoring systems that are scalable, adaptable, and capable of providing real-time data for regulatory compliance and public health protection.

How to cite: Patimisco, P., Zifarelli, A., De Palo, R., Olivieri, M., Sampaolo, A., and Spagnolo, V.: Quartz-Enhanced Photoacoustic Spectroscopy for Environmental Monitoring, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15608, https://doi.org/10.5194/egusphere-egu25-15608, 2025.

EGU25-15692 | ECS | Posters on site | AS5.13

Design of a new cryogenically cooled radiometer for middle atmospheric water vapor measurements:CRYOWARA 

Adrianos Filinis, Gunter Stober, and Axel Murk

Continuous monitoring of atmospheric trace gases in the middle atmosphere presents
significant challenges. Remote sensing instruments are essential for understanding and
characterizing changes in atmospheric chemical composition. Although water vapor is
present in low concentrations in the middle atmosphere, it plays a critical role as one
of the most significant greenhouse gases, profoundly influencing climate change. Water
vapor is a key climate variable, important for radiative balance, and is involved in various
chemical reactions, including ozone depletion through the formation of polar stratospheric
clouds.
With the decommissioning of the AURA-MLS 183 GHz water vapor line, there is an
increasing need to expand the ground-based network of microwave (MW) radiometers.
At the Institute of Applied Physics (IAP), within the Microwave Group (MW), we have
designed a new cryogenically cooled radiometer to measure the emitted radiation from the
22 GHz water vapor line. This instrument, called CRYOWARA, is intended to replace
the existing 22 GHz radiometer known as MIAWARA, which is currently used by the
MW group at the Zimmerwald observatory in Switzerland.
The primary distinction of CRYOWARA is its partially cryogenically cooled front end,
which significantly reduces instrumental noise. This enhancement will enable more ac-
curate water vapor retrievals at higher altitudes, further advancing the study of middle
atmospheric dynamics. At the EGU 2025 conference, we will present the instrument’s
design along with some preliminary results from the breadboard assembly.

How to cite: Filinis, A., Stober, G., and Murk, A.: Design of a new cryogenically cooled radiometer for middle atmospheric water vapor measurements:CRYOWARA, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15692, https://doi.org/10.5194/egusphere-egu25-15692, 2025.

EGU25-16084 | ECS | Posters on site | AS5.13

A compact mid-IR laser absorption spectrometer for water vapor isotopologue measurements in the upper air 

Alex Weitnauer, Lorenz Heilmann, Philipp Scheidegger, Lukas Emmenegger, Dominik Brunner, and Béla Tuzson

Water vapor is the main natural greenhouse gas controlling the Earth's energy balance. It significantly influences atmospheric chemistry and climate dynamics, particularly in the upper troposphere and lower stratosphere (UTLS), which makes it an essential climate variable. Therefore, systematic monitoring of the variability of water vapor in the UTLS is crucial for the understanding of the climate system. However, measurements of its concentration lack important information about the history and origin of the water. This issue can be addressed by considering stable isotopologues of water (e.g. H216O, H218O, and HDO) and quantifying tiny variations in their distribution, which is driven by environmental conditions and chemical/physical processes, making stable water isotopologues an ideal proxy for process studies of the hydrological cycle. Despite the large potential of such measurements, the availability of in-situ data is still very limited due to a lack of adequate analytical tools.

This project focuses on the development of a mobile laser absorption spectrometer (LAS) for airborne in-situ measurements of water vapor isotopologues up to the UTLS region, leveraging on our recent advances in the development of compact instruments [1, 2]. We target the strong absorption features of H216O, H218O, and HDO simultaneously using a single cw-DFB quantum cascade laser (QCL) at around 1359 cm-1. This range was selected after a detailed spectral survey covering the whole infrared domain. We are currently evaluating a laboratory setup using an astigmatic Herriott multipass cell with an optical path length (OPL) of 76 m to assess the performance of the approach.

The mobile design will rely on our succesful concept [1, 2] including a segmented circular multipass cell [3] in open path configuration, which allows for an effective mitigation of memory effects and exhibits the fastest response time. However, the low abundance of the rare water vapor isotopologues needs to be compensated by substantially extending the OPL (30-fold) to enhance the signal-to-noise ratio. Simulations and laboratory tests have shown that this can be achieved while keeping the rigidity, low weight, and tolerance needed for harsh environmental conditions.

Ultimately, our concept should provide an easy-to-deploy tool for isotope-resolved water vapor profiles at high spatio-temporal resolution.

 

[1] Graf et al., Atmos. Meas. Tech., 14, 1365–1378, 2021.

[2] Brunamonti et al., Atmos. Meas. Tech., 16, 4391–4407, 2023.

[3] Graf et al., Opt. Lett., 43, 2434-2437, 2018.

How to cite: Weitnauer, A., Heilmann, L., Scheidegger, P., Emmenegger, L., Brunner, D., and Tuzson, B.: A compact mid-IR laser absorption spectrometer for water vapor isotopologue measurements in the upper air, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16084, https://doi.org/10.5194/egusphere-egu25-16084, 2025.

EGU25-17118 | Orals | AS5.13

Advances in lightweight laser-based analyzers for flying platforms 

Béla Tuzson, Lorenz Heilmann, Simone Brunamonti, Philipp Scheidegger, André Kupferschmid, Alex Weitnauer, and Lukas Emmenegger

Laser absorption spectroscopy is a widely adopted technique for high-precision trace-gas analysis across a broad range of applications. However, commercial instruments remain too bulky for deployment on flying platforms, such as UAVs or balloons. The key challenge thus remains reducing their size  without compromosing their analytical performance.

In this study, we address this challenge and showcase our ongoing developments that have enabled the creation of highly compact mid-infrared trace-gase analyzers. Key innovations include: i) a rapid frequency sweep of the laser using an intermittent continuous wave (icw) driving scheme [1], which reduces the footprint and improves energy and heat management efficiency, ii) a fully monolithic segmented circular multipass cell design [2] that overcomes the size and weight limitations of traditional absorption cells, and iii) an FPGA-based data acquisition system capable of processing large volumes of data in real-time with bandwidths up to 250 MB/s [3].

By combining these groundbreaking developments, we have developed fully autonomous devices that excel in robustness, compactness, rigidity, and lightweight design. Their exceptional in-flight performance is demonstrated through selected field deployments on UAVs and balloons [3-5]. Ongoing developments include multi-species trace-gases detection to monitor ship emissions. This requires a fundamental reconception of the circular multipass cell to increase its optical path length by an order of magnitude.

The versatility and ruggedness of these lightweight and low-footprint spectrometers unlocks new opportunities for applications requiring high spatio-temporal resolution, such as urban or industrial site monitoring and upper atmosphere observation.

 

References:

[1] C. Liu et al., Rev. Sci. Instr. 89, 065107, 2018.

[2] M. Graf et al., Opt. Lett. 43, 2434-2437, 2018.

[3] B. Tuzson et al., Atmos. Meas. Tech., 13(9), 4715-4726, 2020.

[4] M. Graf et al., Atmos. Meas. Tech., 14(2), 1365-1378, 2021.

[5] Brunamonti et al., Atmos. Meas. Tech., 16, 4391–4407, 2023.

How to cite: Tuzson, B., Heilmann, L., Brunamonti, S., Scheidegger, P., Kupferschmid, A., Weitnauer, A., and Emmenegger, L.: Advances in lightweight laser-based analyzers for flying platforms, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17118, https://doi.org/10.5194/egusphere-egu25-17118, 2025.

EGU25-17500 | ECS | Posters on site | AS5.13

A dual-comb spectrometer for remote sensing of greenhouse gases from commercially available devices and components – a progress report. 

Tobias D. Schmitt, Romain Dubroeucq, Thomas Pfeifer, André Butz, and Markus K. Oberthaler

Estimating emissions of trace gases into the lower troposphere requires accurate concentration measurements of the species of interest. Most commonly, they are provided by networks of in-situ sensors or remote sensing instruments on satellites. In high-gradient environments (e.g. urban settings), in-situ instruments are only spatially representative for a small area. On the other hand, many satellites average on the kilometer scale on which also the aggregation of the data for inversion modelling takes place. But satellites can only provide data for sunny weather conditions, at best once a day in a specific region and typically lack sensitivity for local enhancements. Path averaged measurements of trace gases can potentially fill this observation gap. Between all the technological options for such measurements, dual comb spectroscopy (DCS) can provide high resolution spectra at high brightness with basically no instrument line function, all of which have already been demonstrated in the field [1]. But the high costs and the amount of experience required to set up and run such a system limit the application to metrology experts. With developments in recent years, like the commercial availability of turn-key frequency combs, DCS becomes a more realistic option for a wider scientific community and industry.

Here, we present our DCS setup, which is intended for greenhouse gas quantification in the near infra-red. Where possible, we used readily available parts and solutions. We present our current setup and first results obtained, as well as lessons learned and experiences gained in the process.

[1] Sean Coburn et al., "Regional trace-gas source attribution using a field-deployed dual frequency comb spectrometer," Optica 5, 320-327 (2018), DOI: 10.1364/OPTICA.5.000320.

How to cite: Schmitt, T. D., Dubroeucq, R., Pfeifer, T., Butz, A., and Oberthaler, M. K.: A dual-comb spectrometer for remote sensing of greenhouse gases from commercially available devices and components – a progress report., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17500, https://doi.org/10.5194/egusphere-egu25-17500, 2025.

EGU25-17864 | ECS | Orals | AS5.13

Development of a Laser Heterodyne Radiometer for Atmospheric CO₂ and O₂ Measurements: Comparison with FTIR Data 

Adela Collado-Rodríguez, Aldo Moreno-Oyervides, Oscar Elías Bonilla-Manrique, Omaira García, and Pedro Martín-Mateos

There is currently a major global interest in the monitoring of greenhouse gases (GHGs), recognized as the main cause of global warming. At present, the most widely accepted and utilized technique for accurate measurements of GHGs in the atmosphere is Fourier Transform Infrared (FTIR) analysis [1]. These systems are widely used in ground-based monitoring networks, because they provide high accuracy concentration measurements of many trace gases simultaneously. However, the main disadvantage of this type of systems, besides the cost, is its size, which makes it difficult to use for characterizing hot spot GHGs sources.  This has led to a growing interest in the development of new, more portable, and compact GHGs systems. In this context, Laser Heterodyne Radiometry (LHR) is seen as a promising alternative to complement and improve current observation systems. The technique characteristics include high optical resolution, flexibility of operation and a compact instrument design. On the other hand, the optical span is restricted by the tuning range of the local oscillator, which generates certain constraints and challenges that still need to be properly studied and addressed.

In LHR systems, the incoming signal is combined with the local oscillator laser and taken to a photodetector, which provides a downshifted radiofrequency (RF) copy of the spectrum of the optical input signal. The RF signal is amplified and filtered to configure the optical resolution of the instrument and detected by a RF power meter [2]. If the laser emission frequency is swept the spectrum of the optical signal can be retrieved.

This contribution will present the development of a novel, high-performance LHR, with optical frequency comb calibration, which allows the measurement of CO2 and O2 atmospheric concentrations in the field. The results of a measurement campaign, in which the developed system has been compared in detail with the FTIR spectrometer of the TCCON network at the Izaña Atmospheric Observatory (Spain) [3], will be presented and discussed. We believe that the results obtained provide a clear and promising outlook on the future possibilities of using LHR systems for atmospheric composition monitoring.

[1] D. Wunch et al., “The Total Carbon Column Observing Network’s GGG2014 Data Version,” CaltechDATA, Oct. 2015, doi: 10.14291/TCCON.GGG2014.documentation.R0/1221662.

[2] A. Moreno-Oyervides, O. E. Bonilla-Manrique, O. García, and P. Martín- Mateos, “Design and evaluation of a portable frequency comb-referenced laser heterodyne radiometer,” Opt Lasers Eng, vol. 171, p. 107801, Dec. 2023, doi: 10.1016/J.OPTLASENG.2023.107801.

[3] E. Cuevas et al., “Izaña Atmospheric Research Center Activity Report 2019-2020,” State Meteorological Agency (AEMET), Madrid, Spain and World Meteorological Organization, Geneva, Switzerland, NIPO: 666-22-014-0, WMO/GAW Report No. 276, 2022, https://doi.org/10.31978/666-22-014-0.

How to cite: Collado-Rodríguez, A., Moreno-Oyervides, A., Bonilla-Manrique, O. E., García, O., and Martín-Mateos, P.: Development of a Laser Heterodyne Radiometer for Atmospheric CO₂ and O₂ Measurements: Comparison with FTIR Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17864, https://doi.org/10.5194/egusphere-egu25-17864, 2025.

EGU25-18041 | ECS | Orals | AS5.13

Real time monitoring of N2O and CO emissions from vehicles using a quartz-enhanced photoacoustic sensor 

Mariagrazia Olivieri, Andrea Zifarelli, Angelo Sampaolo, Vincenzo Spagnolo, and Pietro Patimisco

Greenhouse gases represent a crucial component of Earth's atmospheric system, playing a fundamental role in maintaining the planet's heat balance through their ability to absorb and emit infrared radiation. Anthropogenic activities have increased the atmospheric concentration of these gases, leading to enhanced global warming effects. The primary greenhouse gases include carbon dioxide (CO₂), methane (CH₄), nitrous oxide (N₂O), and water vapor (H₂O). Among the other pollutants, carbon monoxide (CO) stands out as one of the most hazardous for human health. In urban areas, vehicle emissions represent the primary source of CO, produced through incomplete fuel combustion, with concentrations significantly higher than in unpolluted areas (∼50 ppb). Furthermore, vehicles emissions, particularly from those equipped with catalytic converters, partially contribute to the global atmospheric N2O budget, whose atmospheric concentration is ~300 ppb. The deployment of portable and reliable sensors to monitor these emissions is crucial for understanding their sources, assessing their impact, and developing effective mitigation strategies. 
Quartz Enhanced Photoacoustic Spectroscopy (QEPAS) sensors offer an effective solution for monitoring air pollutants, providing high selectivity and sensitivity, compact dimensions, and rapid response times. Photoacoustic (PAS) basic principle consists in detecting sound waves induced by gas non-radiative energy relaxation as consequence of infrared modulated light absorption. QEPAS represents an evolution of the PAS approach and exploits a quartz tuning fork (QTF) to transduce the acoustic wave into an electric signal. Mid-IR Quantum Cascade Lasers (QCLs) have been employed as light source in QEPAS-based sensor to target the absorption bands of both N2O and CO.
Here we report on the realization of a QEPAS-based system employing a QCL with a central emission wavelength at 4.61 μm and a T-shaped QTF coupled with a pair of acoustic resonator tubes to amplify the sound wave. A ~1 min ramp was added to the fast laser modulation to scan the 2190.6-2188.7 cm-1 spectral range, where well-resolved absorption features of N2O and CO were selected. Laboratory calibrations with certified gas cylinders demonstrated the sensor's ability to detect N₂O and CO at hundreds and tens of ppb level, respectively, at a working pressure of 300 Torr and an integration time of 100 ms. We demonstrated the sensor capability to continuously monitor the QEPAS signal of the two gases both in indoor and outdoor environments. Indoor measurements were carried out over several days by sampling air inside the laboratory, while outdoor measurements took place in a university parking area in Bari to continuously monitor vehicle emissions. During spectral scans, the laser power, the sample temperature and its water vapor content was continuously measured, to eventually compensate for their influence on QEPAS signal. The resulting performances demonstrated its applicability for the realization of a compact and portable sensor for emission monitoring in urban areas.

How to cite: Olivieri, M., Zifarelli, A., Sampaolo, A., Spagnolo, V., and Patimisco, P.: Real time monitoring of N2O and CO emissions from vehicles using a quartz-enhanced photoacoustic sensor, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18041, https://doi.org/10.5194/egusphere-egu25-18041, 2025.

EGU25-18251 | ECS | Posters on site | AS5.13

Heterodyne Spectroradiometer for Precise Measurements of Carbon Dioxide 

Iskander Gazizov and Bernhard Lendl

Recent developments around instrumental control of carbon balance are aimed at accurate evaluation of sources and sinks of major greenhouse gases (GHG) by natural landscapes, cities, industrial and agricultural objects. And we see a significant progress in the development of instruments based on commercial telecom components to make global GHG measurements accessible [1].

Fig. 1. Prototype of MLHS instrument performing measurements in Arctic region.

Here we present the Multichannel Laser Heterodyne Spectroradiometer (MLHS) for exploring the Earth's atmosphere in the near-infrared range, addressing the lack of coverage for greenhouse gases in existing measurement networks. High spectral resolution of solar occultation heterodyne spectroscopy enables us to study the structure and dynamics of the atmosphere while maintaining a compact and low-cost design.

Following the 2022 measurement campaign with a Fourier-spectrometer station for CO2 and CH4, we identified key limitations of the prototype. By improving thermal stability, optimizing optical scheme, and applying accurate sensors for atmospheric parameters, we are presenting the next generation of MLHS.

References

[1] Zenevich, Sergei, et al. "A concept of 2U spaceborne multichannel heterodyne spectroradiometer for greenhouse gases remote sensing." Remote Sensing 13.12 (2021): 2235.

How to cite: Gazizov, I. and Lendl, B.: Heterodyne Spectroradiometer for Precise Measurements of Carbon Dioxide, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18251, https://doi.org/10.5194/egusphere-egu25-18251, 2025.

EGU25-19036 | Posters on site | AS5.13

Potential capabilities of CO2 measurement in the atmospheric column using a near infrared laser heterodyne radiometer (LHR) 

Weidong Chen, Marie Thérèse El Kattar, Tingting Wei, Aditya Saxena, and Hervé Herbin

Vertical concentration distributions of atmospheric trace gases, depending on vertical air transport from the Earth’s surface to the tropopause, play crucial roles in air pollution, ozone depletion and climate change. Accurate determination of the mixing ratios of the greenhouse gases (GHGs) in the lower troposphere, is thus important in the current international context of fighting against global warming and climate change. Laser heterodyne radiometry (LHR) technique, which extracts target molecular absorption information from the broadband sunlight by beating it with a local oscillator for heterodyne measurement, is a highly effective method for ground-based remoting measurement of GHGs’ concentration and vertical profile in the atmospheric column [1].

A transportable, all-fiber-coupled LHR instrument has been developed at the LPCA for ground-based remote sensing of carbon dioxide (CO₂​) [2] in the atmospheric column by using a wide band tunable external-cavity diode laser (1520 – 1620 nm) as local oscillator. The measured LHR spectra of CO2 in the atmospheric column demonstrate strong agreement with spectra recorded by FTIR spectrometer of the TCCON at Paris and simulated from atmospheric transmission model.

The main objective of this study is to quantify the contribution of the LHR to the measurement of tropospheric abundances of CO2 in the atmospheric column from the ground. We present the LHR’s capabilities to measure CO2 vertical profiles through a complete information content analysis, a channel selection and an error budget estimation, using the radiative transfer model ARAHMIS (Atmospheric Radiation Algorithm for High-Spectral Resolution Measurements from Infrared Spectrometers), developed at the LOA [3]. A comparison with the other ground-based instruments like the EM27/SUN and the IFS125HR of the TCCON networks are also presented.

 Acknowledgments

This work is partially supported by the French national research agency (ANR) under the Labex CaPPA (ANR-10-LABX-005) contract, the EU H2020-ATMOS project (Marie Skłodowska-Curie grant agreement No 872081), the regional CPER ECRIN program, and the CNES ATMOSFER project.

 References

[1] D. Weidmann, "Atmospheric trace gas measurements using laser heterodyne spectroscopy", Ch. 4, pp. 159-223, in Advances in Spectroscopic Monitoring of the Atmosphere, eds. by Weidong Chen, Dean S. Venables, Markus W. Sigrist, ISBN: 978-0-12-815014-6, Elsevier (2021).

[2] J. Wang, T. Tu, F. Zhang, F. Shen,J. Xu, Z. Cao, X. Gao, S. Plus, and W. Chen, "An external-cavity diode laser-based near-infrared broadband laser heterodyne radiometer for remote sensing of atmospheric CO2", Optics Express 31 (2023) 9251-9263.

[3] M.T. El Kattar, F. Auriol, H. Herbin, “Instrumental Characteristics and potential greenhouse gas measurement capabilities of the Compact High-Spectral-Resolution Infrared spectrometer: CHRIS”, Atmospheric Measurement Technique 13 (2020) 3769-3786.

How to cite: Chen, W., El Kattar, M. T., Wei, T., Saxena, A., and Herbin, H.: Potential capabilities of CO2 measurement in the atmospheric column using a near infrared laser heterodyne radiometer (LHR), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19036, https://doi.org/10.5194/egusphere-egu25-19036, 2025.

EGU25-19639 | ECS | Orals | AS5.13

Development of Open-Path Incoherent BroadBand Cavity Enhanced Absorption Spectroscopy (OP-IBB-CEAS) instruments for the measurement of trace gases in the Irish Atmospheric Simulation Chamber 

Mixtli Campos-Pineda, Satheesh Chandran, Amir Ben Brik, Niall O'Sullivan, John Wenger, and Andy Ruth

The study of the reactions of volatile organic compounds (VOCs) in the troposphere is important to assess the impact of biogenic and anthropogenic emissions on climate, health and the economy. The challenge of these studies lies, principally, in the difficulty of designing experiments and instruments to measure VOCs and their reaction products under conditions that are significant for the atmosphere (e.g. low concentrations, short lifetimes). The Irish Atmospheric Simulation Chamber (27 m3 Teflon cuboid) is a research facility for the kinetic and mechanistic study of VOC oxidation processes, and a series of open-path incoherent broadband cavity enhanced absorption spectroscopy (OP-IBB-CEAS) setups have been developed for the measurement of different trace gases that are relevant for the study of atmospheric processes. The open-path characteristic of the IBB-CEAS instruments, ensures that there are no sampling losses and that the concentrations measured correspond directly to those of the trace gases in the static chamber. Currently, four OP-IBB-CEAS setups have been developed for measurements of different trace gases: a) A NIR-IBB-CEAS instrument was developed for the measurement of H2O and CO2, b) A visible IBB-CEAS instrument centred at 662 nm for the measurement of H2O, NO3, and NO2, c) A visible IBB-CEAS instrument centred at 450 nm for the measurement of (CHO)2 and NO2, and d) A UV IBB-CEAS instrument for the measurement of HONO, NO2 and MACR. The effective mirror reflectivity of the UV-Vis IBB-CEAS instruments was calibrated with NO2 in a simulated “nighttime” scenario and in a photo-stationary state, using a home-made extractive Cavity Ring-Down Setup. Absorption coefficients for the different instruments range from 10-9 to 10-8 cm-1. A fast retrieval method based on singular value decomposition (SVD) was integrated into an iterative algorithm for fast and robust determination of the concentrations of the different analytes, corresponding to mixing ratios in the range of pptv (e.g. for NO3), to ppbv (e.g. for MACR). In this presentation we will report on a series of NOY production experiments from the reaction of NO2 and O3 was conducted to benchmark the response of the IBB-CEAS instruments, and to study NOY photolysis. These benchmarking experiments shed some light on the importance of the transition stages between "nighttime" and “daytime” chemistry, and their possible impact on the chemistry of nitrogen oxides.

How to cite: Campos-Pineda, M., Chandran, S., Ben Brik, A., O'Sullivan, N., Wenger, J., and Ruth, A.: Development of Open-Path Incoherent BroadBand Cavity Enhanced Absorption Spectroscopy (OP-IBB-CEAS) instruments for the measurement of trace gases in the Irish Atmospheric Simulation Chamber, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19639, https://doi.org/10.5194/egusphere-egu25-19639, 2025.

EGU25-20358 | Posters on site | AS5.13

Design of a Laser Heterodyne Radiometer (LHR) Sensor for Wildfire Detection and Characterization 

J. Houston Miller and Erin McCaughey

Fire detection has traditionally been done optically using tools, ranging from human eyes to modern, advanced hyperspectral cameras.  Both the intensity as well as the spectral signature of the light emitting from fires are important parameters to quantify and characterize. Our laboratory is developing and constructing two sensor platforms to demonstrate a novel technology in Fire Optical Measurements (FOM) for both laboratory and simple “field-scale” demonstrations. The first system, to be described in this presentation, operates in the near-infrared region and will focus on potassium light emissions (K-FOM). Radiative emissions from hot potassium are characteristic of intense fires involving biological materials, distinguishing them from fossil fuel combustion.

The system design for K-FOM is framed by our prior experience in developing Laser Heterodyne Radiometry (LHR) sensors used in solar occultation measurements of greenhouse gases, employing a similar optical design.  In K-FOM, light from a flame containing potassium is collected onto a single-mode optical fiber. The collected radiation is mixed with light from a tunable diode laser (Eblana Photonics),  operating near 770 nm, using a 2x2 combiner. The two output fibers from the combiner arerouted to a a balanced detector (Thorlabs), and the resulting radio frequency (rf) power is measured using a Digikey power sensor.

In this presentation, the design and characterization of the K-FOM sensor will be described, along with tests using laboratory flame burners.  Simple field demonstrations are planned for calendar year 2025.

How to cite: Miller, J. H. and McCaughey, E.: Design of a Laser Heterodyne Radiometer (LHR) Sensor for Wildfire Detection and Characterization, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20358, https://doi.org/10.5194/egusphere-egu25-20358, 2025.

EGU25-1212 | Orals | GI4.3

Mapping horizontal wind speed using a single Doppler Wind Lidar scanning horizontally: a test case over Paris 

Clement Toupoint, Jonnathan Cespedes, Simone Kotthaus, Ludovic Thobois, Martial Haeffelin, and Janna Preissler

Scanning Doppler Wind Lidars are used in a variety of applications, thanks to the versatility brought by their scanning head. Their principal output is the wind speed along the lidar beam, termed the radial wind speed. When used for vertical profiling, the horizontal wind speed and wind direction are obtained from a wind field reconstruction algorithm (DBS or VAD) applied to the radial wind speed along several high-elevation lines of sight.

However, for other scanning strategies (i.e., with low elevation or horizontal scans), the use of such algorithms is not common, making the radial wind speed the sole output of the Doppler Wind Lidar. The radial wind speed is more difficult to interpret visually for a human user, harder to compare with numerical models, and requires more work to be used into advanced algorithms.

Thus, we showcase the Volume Wind wind field reconstruction algorithm, capable of reconstructing the horizontal wind speed and wind direction from measurement points taken at the same elevation and varying azimuth.

We present data taken from the PANAME2022 campaign, in which a Doppler Wind Lidar (WindCube Scan 400S) was set up on an 88m-high tower in Paris city. The lidar performs scans at 0° elevation above the urban area of Paris, measuring radial wind speed from within the Urban Boundary Layer.  Then, we create maps of horizontal wind speed and direction, spanning a large part of the Paris urban area, using the Volume Wind wind field reconstruction algorithm.

This allows us to study the influence of the topography on the wind field at the height of the urban canopy. The effect of the bed of the Seine river is of particular interest, as it is thought to be an important ventilation corridor in periods of extreme heat. These results highlight the potential of remote sensors for studying the Urban Boundary Layer, and the added value of advanced processing algorithms.

How to cite: Toupoint, C., Cespedes, J., Kotthaus, S., Thobois, L., Haeffelin, M., and Preissler, J.: Mapping horizontal wind speed using a single Doppler Wind Lidar scanning horizontally: a test case over Paris, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1212, https://doi.org/10.5194/egusphere-egu25-1212, 2025.

EGU25-2757 | Orals | GI4.3

Multi product comparison during BELLA-ABL Campaign across different Lidar System 

Donato Summa, Paolo Di Girolamo, Marco Di Paolantonio, Benedetto De Rosa, Ilaria Gandolfi, Giuseppe D'amico, Marco Rosoldi, Michail Mytilinaios, Christina Anna Papanikolaou, Nikolaos Papagiannopoulos, Frabrizio Marra, and Lucia Mona

The BELLA measurement campaign took place at the CNR-IMAA Atmospheric Observatory (CIAO), where a large ensemble of instruments, including ceilometers, a Raman lidar, a wind Doppler lidar, a Ka band Doppler radar, a microwave radiometer and different types of in-situ sensors, were operated on a continuous basis over the period April-June 2024. The measurement effort also benefitted from the continous operation throughout the campaign duration of the Raman lidar system CONCERNIG Lidar, located approx. 7 km south-eastward of CIAO, at University of Basilicata in Potenza. All lidar systems involved in the measurement campaign were operated with high space and time resolution, typically 5-10 m and 10 sec, respectively, with vertical profiling capability both in daytime and nighttime for different atmospheric components/variables, including water vapour mixing ratio, CO2 mixing ratio, temperature and particle (aerosol and clouds) optical (backscatter/extinction) properties. This measurement capability, relying on different ABL tracers/properties is very effective in the characterization of the Atmospheric Boundary Layer structure and depth. Estimates of the ABLH obtained from the different parameters measured by CONCERNING are compared with those obtained from the radiosonde and Raman lidar measurements at CIAO, properly revealing differences associated with the different approaches and with atmospheric variability. In this work our attention is focused on two specific case studies (15-16 April 2024 and 28 April-01 May 2024), with results revealing a good agreement, quantified in terms of absolute and percentage BIAS, between the different sensors and approaches. 

Acknowledgment
The authors acknowledge Next Generation EU Mission 4 “Education and Research” - Component 2: “From research to business” - Investment 3.1: “Fund for the realization of an integrated system of research and innovation infrastructures” - Project IR0000032 – ITINERIS.  

How to cite: Summa, D., Di Girolamo, P., Di Paolantonio, M., De Rosa, B., Gandolfi, I., D'amico, G., Rosoldi, M., Mytilinaios, M., Papanikolaou, C. A., Papagiannopoulos, N., Marra, F., and Mona, L.: Multi product comparison during BELLA-ABL Campaign across different Lidar System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2757, https://doi.org/10.5194/egusphere-egu25-2757, 2025.

EGU25-2855 | ECS | Orals | GI4.3

3D Wind Field Retrieval within Thunderstorm Clouds over Piedmont 

Priya Kumari, Massimiliano Burlando, Renzo Bechini, Djordje Romanic, and Alessandro Battaglia

Windstorm, particularly driven by thunderstorms, are among the most destructive natural hazards in Europe causing significant economic losses and causalities. Despite various research, the understanding of thunderstorm outflows and their interaction with built and natural environments remains incomplete, especially in regions prone to intense convective activity, such as the northern Italy. This study focuses on the three-dimensional (3D) structure and dynamics of thunderstorm clouds, emphasizing the formation of downburst and gust fronts that generates damaging surface winds. To construct the 3D wind structure, dual Doppler radar systems are utilized, combining data from operational C-band radar and X-Band radar within the study area. A LiDAR instrument was also operational during the investigated event; however, the scanning LiDAR and C-band radar volume do not overlap due to sheltered positioning of the LiDAR relative to the radar. The inclusion of the X-band radar resolves this issue by covering areas that are blind to C-band radar, thereby re-establishing continuity in measurements across the three instruments. This configuration ensures continuous and comprehensive spatial coverage of wind field measurements, spanning from surface to maximum observation altitude.  To carry this out, historical thunderstorm events that occurred in the Piedmont region, Italy, in 2024 are analysed to enhance present understanding of convective dynamics, and the development of severe wind phenomena. This research will also help identify patterns associated with gust fronts and downbursts, hence facilitating improved nowcasting and risk mitigation strategies for these localized windstorms.

How to cite: Kumari, P., Burlando, M., Bechini, R., Romanic, D., and Battaglia, A.: 3D Wind Field Retrieval within Thunderstorm Clouds over Piedmont, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2855, https://doi.org/10.5194/egusphere-egu25-2855, 2025.

EGU25-3198 | ECS | Orals | GI4.3

An airborne Raman lidar to sample horizontal meteorological fields in the framework of MAESTRO 

Hélène Cassan, Patrick Chazette, Julien Totems, Frédéric Laly, Jeremy Lagarrigue, Valentin Guillet, Laurent Forges, and Sandrine Bony

The Airborne Weather and Aerosol Lidar (A-WALI) is the first airborne meteorological lidar using Raman technology to measure the horizontal fields of water vapour, temperature, clouds and aerosols, as key weather and climate parameters (https://metclim-lidars.aeris-data.fr/). Based on lidar technologies tested in WALI (Totems et al., 2021; Chazette et al., 2014)) and ALiAS (Chazette et al., 2020), it was developed to meet the scientific objectives of ERC project MAESTRO (Mesoscale Organisation of Tropical Convection, https://maestro.aeris-data.fr). This experiment was motivated by the scarcity of observations of convective clouds organisation and their environment over the oceans, whereas this spatial organisation of mesoscale clouds, i.e. the tendency of convective clouds to aggregate and form clusters of varying horizontal and vertical extent, plays an important role in climate and meteorology. One of the objectives of the MAESTRO airborne campaign was therefore to sample the horizontal distribution of meteorological temperature and humidity fields, as well as the spatial distribution of aerosols and clouds. A-WALI was flown on board the ATR-42 aircraft of the SAFIRE unit (https://www.safire.fr/), departing from Sal in Cape Verde. The experiment, which took place between 10 August and 10 September 2024, was part of the international campaign ORCESTRA (Organised Convection Experiments in the Tropical Atlantic) supported by the World Climate Research Programme.

We will give examples of the measurements made by A-WALI and estimates of the associated uncertainties. We will discuss the calibration approach, the lidar sampling capabilities and limitations. Depending on the geophysical parameter under consideration, we will show at which spatial scales the lidar measurement provides relevant information and what its range can be.

How to cite: Cassan, H., Chazette, P., Totems, J., Laly, F., Lagarrigue, J., Guillet, V., Forges, L., and Bony, S.: An airborne Raman lidar to sample horizontal meteorological fields in the framework of MAESTRO, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3198, https://doi.org/10.5194/egusphere-egu25-3198, 2025.

In May 2024 the ESA/JAXA satellite mission EarthCARE was launched into a low Earth orbit. The satellite combines a high spectral resolution lidar and a cloud radar with doppler capability as key instruments on one single platform. Additionally, it is equipped with a multi spectral imager and a broad band radiometer. This unique combination makes EarthCARE the most complex single satellite mission to study aerosol, clouds and precipitation. The successful use of these new data for science application needs a thorough validation of the measurements and the derived data products. A similar EarthCARE-like payload was implemented onboard the German research aircraft HALO (High Altitude and Long range).

This instrumentation was flown during PERCUSION (Persistent EarthCARE underflight studies of the ITCZ and organized convection) campaign. Within its scientific component this field experiment aimed to test factors assumed to control the organization of deep maritime convection, and to investigate the influence of convective organization on the larger-scale environment. The validation part of PERCUSION focused on an as close as possible spatial and temporal co-location of the airborne with the space-borne measurement, which can only be done using an aircraft.

Thus, we included an EarthCARE underpass within each research flight. HALO measurements were performed during the EarthCARE commissioning phase in August 2024 out of Sal, Cape Verde, and out of Barbados in September 2024. In addition, we performed pure validation flights out of Oberpfaffenhofen, Germany in November 2024 for the validation under atmospheric conditions that could not be captured in the two first campaign parts. Altogether, 33 EarthCARE underpasses were performed in different aerosol and cloud situations. Some of the flights were coordinated with in-situ measurements onboard other aircraft (e.g. the French ATR42), with shipborne measurements onboard the German research vessel METEOR, or with ground-based radar and lidar measurements at Mindelo (Cape Verde), Barbados, and the ACTRIS stations Antikythera, Leipzig, Lindenberg and Munich.

In our presentation we will give a short overview of the HALO PERCUSION field experiment. Selected EarthCARE underpasses will be used to exemplify the merits and limitations of the level 1 and some level 2 data products of the ATLID lidar onboard EarthCARE.

How to cite: Wirth, M. and Groß, S.: Validation of EarthCARE lidar products using airborne measurements with the research aircraft HALO during the PERCUSION campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3255, https://doi.org/10.5194/egusphere-egu25-3255, 2025.

EGU25-3463 | Orals | GI4.3

Horizontal wind profiling with Doppler lidars: long-term evaluation of the perpendicular vertical sweeps reconstruction method 

Elsa Dieudonné, Pauline Haezebrouck, Perrine Maynard, Anton Sokolov, Hervé Delbarre, Patrick Augustin, and Marc Fourmentin

Over the last 30 years, the demand for wind profile observations in the lower troposphere has rocketed, carried by weather agencies, airports and the wind energy industry. Doppler lidars are favoured for their compactness, easiness of operation, and versatility in the scanning strategy. Several methods have been developed to reconstruct the horizontal wind profile from the raw radial wind observations recorded in different directions. The most common is the Doppler Beam Swinging (DBS) technique, which is implemented in commercial lidars software. However, DBS leaves a blind zone near the ground that can damper the observation of very low-altitude phenomena like certain low-level jets. 
Another horizontal wind reconstruction method consists in combining observations from two vertical sweeps of the Range-Height Indicator (RHI) type recorded in perpendicular directions, by binning the data into horizontal layers. To our knowledge, this cross-RHI technique has only been used twice [1, 2] and applied to only a few tenth  of hours of lidar scans, so that this method still needs to be fully validated over a longer period and under more varied conditions.
In this study, the cross-RHI and DBS techniques were compared using observations recorded by two Doppler scanning lidars from the Leosphere/Vaisala company, installed at two contrasting sites in France: a flat coastal site (Dunkerque, North Sea coast) for four months, and an urban hilly site (Paris) for two months. Compared to the previous studies and to the DBS method, the cross-RHI technique was improved by adding filtering steps designed to remove range-folded echoes from middle-level clouds. In addition, the flow inclination on the hilly site was taken into account by tilting the wind binning layers and minimizing the total intra-layer variance. 
The horizontal wind speed values retrieved using both techniques were in very good agreement on both sites, with correlation coefficients ~0.92 in the first 200 m above the lidar. The regression slope was 0.93 and the intercept was below 0.4 m/s on both sites, drawn by a small share of points where the DBS grossly overestimated the wind speed due to range-folded echoes. This problem disappeared at higher altitudes, where the correlation coefficients exceeded 0.97, with slopes ~0.97 and intercepts lower than 0.1 m/s. In Dunkerque, where the DBS were averaged over 10 consecutive cycles, the horizontal wind direction difference was smaller than 5° (resp. 10°) for 61% (resp. 83%) of observations in the first 200 m above the lidar, and these numbers also improved with increasing altitude. Additionally, the cross-RHI technique proved to be more efficient to reconstruct the wind in pristine conditions yielding low lidar signal. 
This method’s ability to capture very low-altitude phenomena while providing turbulence information opens new perspectives for urban studies and wind farm site assessment. 

References
[1]    R. M. Banta et al., “Nocturnal Low-Level Jet Characteristics Over Kansas During Cases-99,” Bound.-Lay. Meteorol., 105(2), 221–252, 2002, doi: 10.1023/A:1019992330866.
[2]    T. A. Bonin et al., “Evaluation of turbulence measurement techniques from a single Doppler lidar,” Atmos. Meas. Tech., 10(8), 3021–3039, 2017, doi: 10.5194/amt-10-3021-2017.

How to cite: Dieudonné, E., Haezebrouck, P., Maynard, P., Sokolov, A., Delbarre, H., Augustin, P., and Fourmentin, M.: Horizontal wind profiling with Doppler lidars: long-term evaluation of the perpendicular vertical sweeps reconstruction method, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3463, https://doi.org/10.5194/egusphere-egu25-3463, 2025.

EGU25-3558 | ECS | Posters on site | GI4.3

How can the Latent Heat Flux in a Convective Boundary Layer be Described?  

Linus von Klitzing, Diego Lange, David D. Turner, Andreas Behrendt, and Volker Wulfmeyer

We present ongoing work within the Land-Atmosphere Feedback Initiative (LAFI) [1]. LAFI is funded by the Deutsche Forschungsgemeinschaft (DFG) and is located at the University of Hohenheim, Stuttgart. LAFI's objective is to quantify and understand land-atmosphere feedbacks by utilizing synergetic observations and simulations in an interdisciplinary way. One aspect is covered by this work, which aims to provide a better understanding of fluxes in the convective boundary layer (CBL), especially the latent and sensible heat flux. The focus lies on entrainment fluxes in the interfacial layer (IL), the uppermost layer of the CBL, which marks the transition to the free atmosphere (FA).

A key aspect of this work is setting up a comprehensive dataset. This should capture all relevant variables such as temperature, humidity, and wind of the lower atmosphere at high spatial and temporal resolutions for as many cloud-free CBL situations as possible. Accordingly, simultaneous and high-resolution data from the synergetic use of different lidar systems will be used (see [2]) and processed (see [3]). Next, we will analyze this data for the driving variables and possible parameterizations of the latent and sensible heat flux.

We have already started this work by building a dataset containing data from the Atmospheric Radiation Measurement Climate Research Facility (ARM) Southern Great Plains (SGP) site in Oklahoma, USA, and testing a similarity relationship for the latent heat flux in the IL in [4].

Corresponding first results could not confirm the proposed similarity relationship for the latent heat flux in the IL from [2] and will be presented at the conference. Additionally, correlations of the flux with other measured variables, as well as an example case representative for the pool of selected cases will be shown.

In the coming months, we will expand the dataset to other measurement campaigns, like the synergy of Raman and Doppler lidar systems within LAFI in 2025.

References:

[1] https://www.lafi-dfg.de/

[2] Wulfmeyer, Volker et al. (2016): Determination of Convective Boundary Layer Entrainment Fluxes, Dissipation Rates, and the Molecular Destruction of Variances: Theoretical Description and a Strategy for Its Confirmation with a Novel Lidar System Synergy. In Journal of the Atmospheric Sciences 73 (2), pp. 667–692. DOI: 10.1175/JAS-D-14-0392.1

[3] Behrendt, Andreas et al. (2020): Observation of sensible and latent heat flux profiles with lidar. In Atmos. Meas. Tech. 13 (6), pp. 3221–3233. DOI: 10.5194/amt-13-3221-2020

[4] von Klitzing, Linus (2024): Latent Heat Entrainment Flux Similarity Relationships for the Convective Boundary Layer. Master's dissertation. University of Hohenheim, Stuttgart. Institute of Physics and Meteorology

How to cite: von Klitzing, L., Lange, D., Turner, D. D., Behrendt, A., and Wulfmeyer, V.: How can the Latent Heat Flux in a Convective Boundary Layer be Described? , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3558, https://doi.org/10.5194/egusphere-egu25-3558, 2025.

EGU25-4141 | ECS | Orals | GI4.3

Raman lidar derived WVMR profiles compared to ERA5 - A WaLiNeAs application  

Frédéric Laly and Patrick Chazette

Vibrational Raman lidar measurements of the water vapour mixing ratio (WVMR) were conducted during the WaLiNeAs (Water Vapor Lidar Network Assimilation) field campaigns in the western Mediterranean during autumn and winter 2022–2023 and in southwestern France (Toulouse) between June and September 2023. These campaigns, which spanned different seasons and geographical locations, provided an opportunity to sample various meteorological phenomena, including a dry winter, rainstorms, long-range aerosol transport, and an intense heat wave. Consequently, the water vapour content recorded in the lower troposphere showed significant variability during WaLiNeAs, ranging from less than 1 g kg-1 to more than 17 g kg-1. For operational purposes, a vertical resolution of 100 m and a temporal resolution between 15 and 60 min have been chosen. These resolutions are aligned with the spatio-temporal resolution of the ERA5 dataset from ECMWF's Integrated Forecasting System (IFS) global numerical weather prediction models. The processing of the lidar data has resulted in a scientific publication explaining the methods used to invert the lidar data and recover various atmospheric parameters. Lidar measurements address a critical gap left by operational instruments, which struggle to capture the diurnal cycle of water vapour from the planetary boundary layer to the lower free troposphere. The primary aim of this study is to compare ERA5 data with lidar-derived WVMR profiles. The results reveal altitude-dependent differences in Pearson correlation coefficient (COR), mean bias (MB), and root mean square deviation (RMSD), particularly during periods of high-water vapour content (> 10 g kg⁻¹). Over all periods the MB ranges from 0.1 to 3 g kg⁻¹, and the RMSD varies between 0.6 and 3.7 g kg⁻¹. COR ranges from 0.16 to 0.94, with lower values observed in the free troposphere during warmer periods. These variations underline the differences in the performance of the reanalysis model over different periods and altitudes when compared to lidar profiles. We show that the reanalysis constantly underestimated the WVMR at all altitudes. This study highlights the importance of scrutinising WVMR and the challenges faced by models during high water vapour meteorological events. The results provide valuable insights into the performance of operational numerical weather prediction models and highlight the need to refine their representation of WVMR vertical profiles in the lower troposphere by incorporating ground-based lidar measurements.

We give special thanks to the ANR grant #ANR-20-CE04-0001 for its contribution to the WaLiNeAs programme, to Meteo-France for its help with the measurements in Toulouse, and to the CNRS INSU national LEFE programme for its financial contribution to this project.

How to cite: Laly, F. and Chazette, P.: Raman lidar derived WVMR profiles compared to ERA5 - A WaLiNeAs application , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4141, https://doi.org/10.5194/egusphere-egu25-4141, 2025.

EGU25-4413 | ECS | Posters on site | GI4.3

Evaluating Wind Velocity Measurement Errors in Ground-Based Doppler LiDAR Using Virtual Doppler LiDAR and Large Eddy Simulation 

Veronica Escobar-Ruiz, Janet Barlow, and Zheng-Tong Xie

Doppler Wind LiDARs (DWLs) are remote sensing devices that measure wind speed and direction by analysing the Doppler shift of the light backscattered from atmospheric particles along the lidar beam's line of sight. Hence, DWLs are extensively employed in boundary layer meteorology to analyse wind flow due to their ability to provide high-resolution wind measurements. Recently, there has been growing interest in deploying DWLs in urban environments, where mast-based cup anemometers or sonic anemometers face challenges. However, DWL scanning techniques typically assume a homogeneous, stationary wind field, assumptions which often break down in urban boundary layers due to turbulence caused by buildings and complex topography that significantly influences wind profiles. Moreover, the selection of DWL scanning patterns and their configuration should be carefully tailored to the specific application.

One of the most-used scanning methods for measuring vertical wind velocity profiles is the Velocity Azimuth Display (VAD). The technique involves scanning the laser beam around the zenith in a conical pattern at a fixed elevation angle. However, completing the full 360° requires a finite time, during which the wind speed is assumed to be constant. Additionally, if the wind varies significantly within the sampling volume (e.g., due to turbulence or flow inhomogeneity) the calculated wind profiles may be inaccurate.

Large-Eddy Simulation (LES), with a sufficiently high grid resolution to resolve turbulent motions, provides a means to evaluate potential errors in DWL sampling strategies. This study uses a Virtual Doppler LiDAR (VDL) tool (Rahlves et al., 2022) within the Parallelized Large-Eddy Simulation Model (PALM, version 6.0) to estimate velocity profiles derived from simulated radial velocities along virtual laser beam paths under the VAD scheme. The research is part of the ASSURE Project (Across-Scale Processes in Urban Environments), which focuses on Bristol, UK. The project investigates urban wind flow using DWLs deployed across the city, employing scanning strategies utilised during a one-year field campaign beginning in May 2024.

Bristol was chosen for its compact urban layout and distinct topographic features, including the Avon Gorge and a central valley. The city serves as a case study for examining urban wind dynamics. This study's objectives are twofold: (1) to identify and quantify errors between the vertical wind profile derived from a VAD scan using the VDL and the profile directly taken from the PALM model and (2) to facilitate comparisons between PALM-simulated wind profiles and observations from ground-based DWL. By addressing the discrepancies arising from topographically induced flow, this research aims to enhance the reliability of DWL data in urban settings and improve our understanding of urban boundary layer processes. Results will be presented for a case study of flow channelled by a deep valley interacting with a city-centre boundary layer.

Rahlves, C., Beyrich, F., and Raasch, S. (2022). ‘‘Scan strategies for wind profiling with Doppler lidar – an large-eddy simulation (LES)-based evaluation’’, Atmospheric Measurement Techniques, 15(9), 2839-2856

How to cite: Escobar-Ruiz, V., Barlow, J., and Xie, Z.-T.: Evaluating Wind Velocity Measurement Errors in Ground-Based Doppler LiDAR Using Virtual Doppler LiDAR and Large Eddy Simulation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4413, https://doi.org/10.5194/egusphere-egu25-4413, 2025.

Atmospheric lidar has become a powerful tool for atmospheric detection due to its advantages of high spatiotemporal resolution, multiple parameters and high-precision detection. In this paper, the application status of lidar in China’s meteorological observation is introduced, and the prospects for the development of lidar applications are presented. For better observation of atmospheric clouds, aerosol, and water vapor parameters, the China Meteorological Administration(CMA) has laid out and constructed a Raman-Mie aerosol lidar network with 49 stations from 2021 to 2024 and has solved several key technical problems such as data quality control, parameter inversion, and quantitative calibration. In order to achieve high-precision observations with a time resolution at the minute level, more than 10 standard specifications have been formulated for calibration, observation, and data transmission. The lidars for network applications normally use a three-wavelength laser covering 355 nm, 532 nm, and 1064 nm,and they can achieve a detection distance of more than 10 km, an accuracy of aerosol backscattering coefficient of less than 20%(0.5-2 km)and 40%(2-5 km), and an accuracy of water vapor concentration of less than 1g/kg (0.5-3 km).In the field of wind observation, the CMA has laid out and constructed a wind lidar network with 372 stations by 2024. The lidars use the coherent detection with a laser wavelenth of 1550nm, and they can achieve a maximum detection distance of more than 3km, a horizontal wind speed error less than 0.8m/s, and a horizontal wind direction error less than 8°.The layout and application of aerosol lidar network and wind lidar network have greatly improved China's meteorological observation capability and application levels in aerosol and wind fields. In recent years, the CMA has actively cooperated with various universities and scientific research institutes to carry out key technological studies in atmospheric temperature and humidity lidar, high spectral resolution lidar, middle and upper atmosphere lidar, and airborne/spaceborne lidar. Through planning and constructing meteorological business application platforms in the future, the comprehensive three-dimensional observation of multiple parameters such as temperature, humidity, wind and aerosols will be developed to improve China's meteorological observation ability and provide strong support for research in meteorological services, atmospheric science and climate change.

How to cite: Chen, Y.: Status and Development of Lidar applications in China's Meteorological Observation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5725, https://doi.org/10.5194/egusphere-egu25-5725, 2025.

EGU25-5758 | Orals | GI4.3

Aerosol impacts on cirrus cloud formation and properties using in-situ and lidar measurements during CIRRUS-HL campaign  

Qiang Li, Silke Gross, Martin Wirth, Tina Jurkat-Witschas, Christiane Voigt, Elena De La Torre Castro, and Daniel Sauer

Cirrus clouds cover about 30% of the Earth’s surface and play a crucial role in the Earth’s radiation balance. They are composed of ice crystals with various sizes and nonspherical shapes. Ice crystals can form through either homogeneous freezing or heterogeneous freezing depending on the ambient temperature, humidity, updraft, and the availability of INPs, and hence possess different properties. Their radiative effects strongly depend on the formation processes and cloud microphysical, thermal, and optical properties. Furthermore, global aviation affects the Earth’s radiation balance by increasing cloudiness due to contrail formation and exerting an indirect effect on the microphysical properties of naturally-formed cirrus clouds. Aviation is responsible for 3-4% of anthropogenic effective radiative forcing and more than half of them stems from contrails and contrail-induced cirrus. Experimental and numerical studies have been carried out in the past years to understand contrails and contrail-induced cirrus as well as their climate effects. Unfortunately, however, the parameterization of ice crystal properties in global climate model and the estimate of radiation forcings are still inadequate. Compared with the intensive studies on cirrus clouds in the tropics and midlatitude regions, cirrus cloud measurements and model studies at high latitudes are sparse, although cirrus clouds at high latitudes attract more attention in recent years because the Arctic undergoes faster warming than other regions of the globe. The airborne measurements from the ML-CIRRUS mission revealed that cirrus clouds with enhanced PLDR appear in areas of high aviation emissions. Nevertheless, observational evidence of indirect effects of aviation exhaust on the changes of cirrus properties is still missing. Thanks to the foundational work of ML-CIRRUS, the CIRRUS-HL mission in June-July, 2021, with upgraded instrumentation was designed to characterize cirrus cloud at both high- and midlatitudes and to investigate aviation impact, radiation, and aerosol-cloud interactions. It collected more details in the simultaneous profiling of cirrus cloud and aerosol properties. In this study, we focus on the comparison of particle linear depolarization ratios (PLDR) of cirrus clouds with the airborne lidar WALES from two specific flights under similar cloud formation processes during CIRRUS-HL. Their microphysical properties (i.e. ice crystal size and number concentration) are also determined and compared based on the analysis of simultaneous in-situ measurements. The analysis is also extended to all the flights for statistical results. Furthermore, the characterization of aerosol load, especially aviation soot, will be identified in the regions of ice crystal formation and evolution and their correlations with cirrus cloud properties are finally able to be further determined.  

How to cite: Li, Q., Gross, S., Wirth, M., Jurkat-Witschas, T., Voigt, C., De La Torre Castro, E., and Sauer, D.: Aerosol impacts on cirrus cloud formation and properties using in-situ and lidar measurements during CIRRUS-HL campaign , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5758, https://doi.org/10.5194/egusphere-egu25-5758, 2025.

EGU25-6889 | Orals | GI4.3

Desert dust profiling and applications 

Vassilis Amiridis

Atmospheric remote sensing from space and surface has been advanced during the last decade. Mineral dust is an atmospheric target that provides a strong signature on active and passive polarimetric remote sensing observations, due to its irregular shape. Nowadays, advanced lidar systems operating in the framework of ACTRIS provide quality assured, calibrated multi-wavelength linear particle depolarization ratio measurements, while new developments will provide us elliptical polarization recordings in the near future. Passive polarimeters are already part of ACTRIS and AERONET and their integration in operational algorithms is expected in the near future. This wealth of new information combined with updated scattering databases and sophisticated inversion schemes provide the means towards an improved characterization of desert dust in the future. This kind of information can be used for space-borne lidars such as CALIPSO, CATS, Aeolus, EarthCARE and the future AOS missions.

We present here some examples of how remote sensing facilitates desert dust research during the last decade, aiming to demonstrate the progress on issues such as: (a) the discrimination of desert dust in external mixtures, (b) the estimation of the fine and coarse particle modes, (c) the synergy of passive and active remote sensing for the derivation of dust properties, (d) the provision of dust-related CCN and IN particle concentrations for aerosol-cloud interaction studies, (e) the development of new scattering databases based on realistic particle shapes, (e) the application of these techniques on space lidar datasets for the provision of climatological datasets, and (f) the use of these datasets in data assimilation for improving dust representations in models.

How to cite: Amiridis, V.: Desert dust profiling and applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6889, https://doi.org/10.5194/egusphere-egu25-6889, 2025.

EGU25-7172 | Posters on site | GI4.3

Recent Advances in Automated Temperature and Humidity Lidar 

Andreas Behrendt, Diego Lange, and Volker Wulfmeyer

We will give an update of our recent activities regarding automated high-resolution temperature and humidity lidar.

The Raman lidar ARTHUS (Atmospheric Raman Temperature and HUmidity Sounder) of University of Hohenheim is an automated instrument with continuous operation (Lange et al., 2019; Wulfmeyer and Behrendt, 2022). Besides being operated during several field campaigns elsewhere, ARTHUS is usually located at the LAFO (Land Atmospheric Feedback Observatory) near the agricultural research fields of our university. Here, in addition, three scanning Doppler lidars, a Doppler cloud radar, two meteorological 10-m towers with eddy-covariance stations, as well as surface and sub-surface sensors are collecting routinely data. These data are combined with detailed vegetation analyses.

ARTHUS is an eyesafe Raman lidar using a diode-pumped Nd:YAG laser as transmitter. Only the third-harmonic radiation at 355 nm is – after beam expansion – transmitted into the atmosphere. The laser power is about 20 W at 200 Hz repetition rate. The receiving telescope has a diameter of 40 cm. A polychromator extracts the elastic backscatter signal and four inelastic signals, namely the vibrational Raman signal of water vapor and CO2 molecules, and two pure rotational Raman signals. The raw data is stored with a resolution of 7.5 m and typically 1 to 10 s. All five signals are simultaneously analyzed and stored in both photon-counting (PC) mode and voltage (so-called “analog” mode) in order to make optimum use of the large intensity range of the backscatter signals covering several orders of magnitude. Primary data products are temperature, water vapor mixing ratio, carbon dioxide mixing ratio, particle backscatter coefficient, and particle extinction coefficient. The high resolution allows studies of boundary layer turbulence (Behrendt et al, 2015) and - in combination with the vertical pointing Doppler lidar - sensible and latent heat fluxes (Behrendt et al, 2020).

Further refined lidars like ARTHUS are offered by the company Purple Pulse Lidar Systems (www.purplepulselidar.com). Meanwhile three more systems have been built and are operating.

At the conference, we will present the recent advances in these powerful automated temperature and humidity lidars and show highlights of the measurements.

 

References:

Behrendt et al. 2015, https://doi.org/10.5194/acp-15-5485-2015

Behrendt et al. 2020, https://doi.org/10.5194/amt-13-3221-2020

Lange et al. 2019, https://doi.org/10.1029/2019GL085774

Wulfmeyer and Behrendt 2022, https://doi.org/10.1007/978-3-030-52171-4_25

How to cite: Behrendt, A., Lange, D., and Wulfmeyer, V.: Recent Advances in Automated Temperature and Humidity Lidar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7172, https://doi.org/10.5194/egusphere-egu25-7172, 2025.

EGU25-7552 | Posters on site | GI4.3

Scanning Measurements With an Automated Temperature and Moisture Lidar in the Atmospheric Boundary Layer 

Diego Lange Vega, Andreas Behrendt, and Volker Wulfmeyer

Despite significant advancements in atmospheric observation techniques, the thermodynamic structure of the atmospheric boundary layer (ABL) remains largely unexplored due to the scarcity of suitable high-resolution remote sensing measurements. Over the past six years, the Atmospheric Raman Temperature and Humidity Sounder (ARTHUS), an automated profiler based on the Raman lidar technique (Lange et al., 2019), has participated in several ground- and ship-based measurement campaigns (Stevens et al., 2021; Flamant et al., 2021). These campaigns have demonstrated ARTHUS's capability to resolve critical atmospheric features, such as turbulent fluctuations and their statistics with high temporal and spatial resolution.

In combination with Doppler lidars, ARTHUS enables profiling of sensible and latent heat fluxes within the convective ABL, thereby supporting the investigation of flux-gradient relationships (Wulfmeyer et al. 2016, Behrendt et al., 2020). These capabilities make ARTHUS a powerful tool for advancing process studies of land-atmosphere interactions, enhancing weather and climate monitoring, validating atmospheric models, and improving data assimilation techniques. We present examples from several field campaigns with respect to the observation of diurnal cycles of profiles of mean and turbulent variables.

An eye-safe Nd:YAG laser with 20 W at 355-nm is used as transmitter. A 40-cm receiving telescope collects backscattered light providing independent measurements of temperature (T), water vapor mixing ratio (WVMR), CO2 concentration, particle extinction coefficient, and particle backscatter coefficient.

ARTHUS has proven its reliability during extended operations at the Land Atmosphere Feedback Observatory (LAFO) at the University of Hohenheim and across various field campaigns under diverse atmospheric conditions. As part of the Land-Atmosphere Feedback Initiative (LAFI, Wulfmeyer et al. 2024), ARTHUS will extend its capabilities to include scanning measurements from the surface through the ABL, capturing three-dimensional turbulent structures with a focus on entrainment processes. The campaign will take place between March and August 2025 at the LAFO site. For the first time, ARTHUS will deliver comprehensive maps of T, WVMR, and CO₂, especially near the surface and canopy but also up to the top of the ABL offering unprecedented insights into land-atmosphere feedback. At the conference, highlights of the first LAFI measurements will be shown.

References:

Lange et al. 2019, https://doi.org/10.1029/2019GL085774

Stevens et. al. 2021, https://doi.org/10.5194/essd-2021-18

Flamant et al. 2021, https://doi.org/10.1007/s42865-021-00037-6

Behrendt et al. 2020, https://doi.org/10.5194/amt-13-3221-2020

Wulfmeyer et al. 2016, https://doi.org/10.1175/JAS-D-14-0392.1

Wulfmeyer et al. 2024, https://doi.org/10.5194/egusphere-egu24-10102

How to cite: Lange Vega, D., Behrendt, A., and Wulfmeyer, V.: Scanning Measurements With an Automated Temperature and Moisture Lidar in the Atmospheric Boundary Layer, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7552, https://doi.org/10.5194/egusphere-egu25-7552, 2025.

EGU25-8390 | Orals | GI4.3

New operational perspective to identify aerosol in real-time with a pioneering algorithm (CONIOPOL) based on CL61 data 

Quentin Laffineur, Alexander Mangold, Karen De Causmaecker, and Andy Delcloo

In recent years, there has been an increase in the intensity and frequency of smoke plume events over North America (sometimes reaching Europe) and dust plume events reaching Europe from Africa. As these can potentially affect surface air quality, environmental agencies are increasingly interested in being able to identify the nature of aerosol plumes, monitor it in real time and determine whether its interaction with the atmospheric boundary layer will impact surface air quality. The automatic LIDAR-ceilometer (ALC) primarily designed for cloud base height detection has greatly improved over the last years and now provides vertical profiles of backscatter from aerosols and clouds. Recently, a new type of ALC with a depolarization function (VAISALA CL61) is commercially available for distinguishing cloud phase (which is useful for weather forecasting) and also makes it possible to support the type identification of aerosols.

At the Royal Meteorological Institute of Belgium (RMI), we have been developing a new pioneering algorithm (CONIOPOL: CONIOlogy + POLarization) based only on CL61 measurements (backscatter and depolarization profiles) to provide in real-time automatic identification of cloud phase, precipitation type and aerosol type. CONIOPOL cannot provide an independent and unambiguous identification of the aerosol type because the CL61 operates with a single wavelength. Although, CONIOPOL is a very useful operational support allowing a quick identification in real time of the type of aerosols in combination with forecasts and backward trajectories models.

The effectiveness and robustness of CONIOPOL will be demonstrated in different ways, through case studies comparing its output with CAMS forecast and air quality measurements, through statistical analysis of CONIOPOL output and by a comparison analysis between CONIOPOL output and CAMS forecasts. In addition to its operational use, it is capable of assembling a climatology of cloud phase, precipitation type and aerosol type. Further, it can contribute to the validation of EarthCARE (ESA) space-borne products.

How to cite: Laffineur, Q., Mangold, A., De Causmaecker, K., and Delcloo, A.: New operational perspective to identify aerosol in real-time with a pioneering algorithm (CONIOPOL) based on CL61 data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8390, https://doi.org/10.5194/egusphere-egu25-8390, 2025.

EGU25-8397 | Posters on site | GI4.3

A Study Mass Extinction Efficiency (MEE) Calculation and Variability Analysis by Aerosol Source Identification: Application of Horizontal Scanning Lidar and HYSPLIT Model 

Jihyun Yoon, Juseon Shin, Sohee Joo, Gahyeon Park, Dukhyeon Kim, and Youngmin Noh

South Korea faces complex air quality challenges arising from domestic emission sources driven by industrialization and urbanization, as well as seasonally influenced long-range transport pollutants from overseas. In particular, springtime dust storms and wintertime heating emissions both domestic and foreign converge to create a multifaceted air pollution environment. To effectively understand and manage these issues, accurately determining the Mass Extinction Efficiency (MEE) based on optical observations is essential. In this study, we refined MEE calculations by integrating LiDAR-based observations with ground-level measurements, analyzed variability as a function of aerosol origin, and simultaneously assessed the potential for indirect evaluation of atmospheric composition. Using a horizontal SCANNING LiDAR, we derived high-resolution, two-dimensional extinction coefficients near the surface and combined these data with hourly Particulate Matter (PM) observations from the AirKorea monitoring network. Employing the Ångström exponent to differentiate coarse mode particles (Ångström exponent ≈ 0) from fine mode particles (Ångström exponent ≈ 3), we calculated extinction coefficients for total, coarse, and fine aerosols. We then derived MEE values through three approaches: total extinction coefficient relative to PM10, coarse extinction coefficient relative to (PM10 – PM2.5), and fine extinction coefficient relative to PM2.5. To analyze aerosol origins, we used the HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) model of NOAA(National Oceanic and Atmospheric Administration), which allowed us to evaluate mesoscale and regional source contributions and investigate their impact on MEE variability. Data from December 2021 to the present revealed substantial variations in MEE values depending on aerosol source regions and compositions. By offering a refined analytical framework tailored to South Korea’s unique climatic and geographical characteristics, this study provides valuable insights for improved air quality monitoring and predictive modeling.

"This research was supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry & Technology Institute(KEITI) funded by the Ministry of Environment(MOE)"

How to cite: Yoon, J., Shin, J., Joo, S., Park, G., Kim, D., and Noh, Y.: A Study Mass Extinction Efficiency (MEE) Calculation and Variability Analysis by Aerosol Source Identification: Application of Horizontal Scanning Lidar and HYSPLIT Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8397, https://doi.org/10.5194/egusphere-egu25-8397, 2025.

EGU25-8530 | Orals | GI4.3

 Improvement of DQ-1/ACDL in Global Thin Cirrus Cloud Detection 

Sijie Chen, Bo Li, and Kai Zhang

Lidar is an essential and unique tool in the current integrated spaceborne remote sensing observation system. From CALIPSO-CloudSat in the A-Train constellation to China’s Daqi-1 (DQ-1) and the latest EarthCARE mission, lidar’s ability to detect thin cirrus and low clouds with fine vertical resolution has significant implications. The effective combination of lidar and CPR provides a complete cloud vertical structure for related studies and an accurate validation for passive remote sensors.

Launched successfully on April 16, 2022, the DQ-1 satellite carries the Aerosol Carbon Detection Lidar (ACDL), a three-wavelength  (532, 1064, and 1572 nm) lidar for comprehensive measurements of atmosphere composition. is technically a combination of two lidars with different mechanisms: a high-spectral-resolution lidar (HSRL) measuring clouds and aerosols and an integrated-path differential absorption (IPDA) lidar measuring carbon dioxide. The mechanism of HSRL allows the separation of aerosol contribution from the molecular backscatter, therefore removing the lidar ratio assumption in the traditional Mie-scattering lidar like CALIOP. Initial validation results indicate an accuracy better than 20% for a strong signal backscatter profile with 24 m vertical resolution. The cloud-top and base height, phase, and classification products have been processed accordingly.

Positioned time-wise between CALIPSO and EarthCARE missions, DQ-1 fills a critical gap in the observation and cross-validation. This report contains results from a one-year-long comparison between DQ-1/ACDL and CALIPSO/CALIOP from June 2022 to June 2023, till the end of CALIPSO operation. The analysis includes case studies from different latitudes and scenarios, and overall gridded global thin cirrus cloud distributions. The results show good consistency between the two systems, with DQ-1/ACDL demonstrating better coherence and performance. Depending on data availability, the report might also include preliminary comparisons with EarthCARE/ATLID data. The report will highlight key improvements of the DQ-1/ACDL system in thin cirrus cloud detection, for better monitoring and valuable insights of cloud properties, atmospheric dynamics, and climate modeling.

How to cite: Chen, S., Li, B., and Zhang, K.:  Improvement of DQ-1/ACDL in Global Thin Cirrus Cloud Detection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8530, https://doi.org/10.5194/egusphere-egu25-8530, 2025.

The Cloud and Aerosol Lidar for Global Scale Observations of the Ocean-Land-Atmosphere System (CALIGOLA) is an advanced multi-purpose space lidar mission with a focus on atmospheric and oceanic observation aimed at characterizing the Ocean-Earth-Atmosphere system and the mutual interactions within it. This mission has been conceived by the Italian Space Agency (ASI) with the aim to provide the international scientific community with an unprecedented dataset of geophysical parameters capable of increasing scientific knowledge in the areas of atmospheric, aquatic, terrestrial, cryospheric and hydrological sciences. The Italian Space Agency is partnering with NASA on this exciting new space lidar mission. The mission is planned to be launched in the time frame 2031-2032, with an expected lifetime of 3-5.

Exploiting the three Nd:YAG laser emissions at 354.7, 532 and 1064 nm and the elastic (Rayleigh-Mie), depolarized, Raman and fluorescent lidar echoes from atmospheric and ocean constituents, CALIGOLA will carry out multi-wavelength profile measurements of the backscatter, extinction and fluorescent coefficient and the depolarization ratio of atmospheric and ocean particles. These measurements will enable determinations of the microphysical and dimensional properties of atmospheric aerosols and clouds and their typing. Measurements of ocean optical properties will document phytoplankton seasonal and inter-annual dynamics and will improve understanding on marine biogeochemistry, the global carbon cycle, and responses of plankton ecosystems to climate variability. One specific measurement channel at 685 nm will be dedicated to fluorescence measurements from atmospheric aerosols and marine chlorophyll, for the purpose of aerosol typing and characterization of phytoplankton nutrient stress and primary production. CALIGOLA will provide accurate measurements of small-scale variability in earth surface elevation, primarily associated with variations in the ice and snow, terrain, and terrestrial vegetation height (e.g., forest canopies).

Phase A studies, commissioned by the Italian Space Agency to Leonardo S.p.A. and focusing of the technological feasibility of the laser source and the receiver, were conducted from October 2022, while Phase A/B1 activities for the payload, platform, and end-to-end system will start in January-February 2025. Scientific studies in support of the mission are ongoing, commissioned by the Italian Space Agency to University of Basilicata (KO: November 2021) and ISMAR-CNR (KO: September 2023). In September 2023, NASA-LARC initiated a pre-formulation study to assess the feasibility of a possible contribution to the CALIGOLA mission focused on development of the detection system and sampling chain and the implementation of data down link capabilities. The pre-formulation study ended in September 2024, the Mission Concept Review was successfully completed, and a phase A/formulation study has been finalized in preparation for a System Requirements Review, which should start shortly. This presentation will provide details on current status and future steps of this groundbreaking multidisciplinary lidar mission.

How to cite: Di Girolamo, P. and the CALIGOLA Team: The Cloud and Aerosol Lidar for Global Scale Observations (CALIGOLA): Overview of the current status and future steps of a groundbreaking multidisciplinary Mission, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8567, https://doi.org/10.5194/egusphere-egu25-8567, 2025.

EGU25-8872 | ECS | Posters on site | GI4.3

CO2 Measurements with Raman Lidar in the Lower Troposphere  

Moritz Schumacher, Diego Lange, Andreas Behrendt, and Volker Wulfmeyer

Carbon dioxide is the most important greenhouse gas caused by emissions from human activities. Nevertheless, little is known about its distribution in the atmposphere. Thus, continuous CO2 measurements not only on the ground but also in higher altitudes are key to improve our understanding of radiative forcing. Therefore, ground-based lidar systems with their ability of range-resolved CO2 measurements are particularly interesting. In the recent two years, we have developed and incorporated a new channel to our ground-based Raman lidar system ARTHUS ("Atmospheric Raman Temperature and HUmidity Sounder") [1] and successfully collected more then 70 days of CO2 profiles at the “Land-Atmosphere Feedback Observatory” (LAFO), in Stuttgart, Germany [2]. We utilize the 2ν2 CO2 Raman line, which is well separated from Raman lines of other atmosphere gases, especially O2. With the current setup, we profile CO2, temperature and humidity as well as particle extinction and particle backscatter coefficients in five receiver channels. The first CO2measurements in 2023 with a preliminary calibration where already presented at the EGU24 [3]. Since then, the laser power has been doubled while still being an eye-safe system. With some other improvements in addition, the integration times needed at night and for a resolution of 300 m are for example 1.5 hours for an uncertainty of 1.5 ppm and 2 hours for an uncertainty of 2 ppm at altitudes of 500 m and 1 km, respectively.

We are currently (January 2025) adding a 2-mirror scanner to the system. With this, we will much better calibrate our CO2 mixing ratio with low-level scans near our ground-based in-situ sensors located at the LAFO site. The scanning measuements of the CO2 concentration will provide insights in its distribution around the surface sensors and enable us to identify and quantify local carbon sources and sinks. We will present the recent approaches and first scanning measurements at the EGU25.

References: 

[1] Lange, D. et al.: Compact Operational Tropospheric Water Vapor and Temperature Raman Lidar with Turbulence Resolution. Geophys. Res. Lett. (2019). DOI: 10.1029/2019GL085774 

[2] Späth, F., S. Morandage, A. Behrendt, T. Streck, and V. Wulfmeyer, 2021: The Land-Atmosphere Feedback Observatory (LAFO). EGU21-7693 (2021). DOI: 10.5194/egusphere-egu21-7693 

[3] Schumacher, M., D. Lange, A. Behrendt, V. Wulfmeyer, 2024: Measurements of CO2Profiles in the Lower Troposphere with the new Raman Lidar Channel of ARTHUS. EGU24-9219 (2024). DOI: 10.5194/egusphere-egu24-9219 

How to cite: Schumacher, M., Lange, D., Behrendt, A., and Wulfmeyer, V.: CO2 Measurements with Raman Lidar in the Lower Troposphere , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8872, https://doi.org/10.5194/egusphere-egu25-8872, 2025.

EGU25-9052 | ECS | Posters on site | GI4.3

Evaluating the MONARCH Model with Lidar Data: A Step Toward Improving Global Dust Surface Concentrations 

Carlotta Gilè, Emanuele Emili, Jeronimo Escribano, Luka Ilic, Oriol Jorba Casellas, and Carlos Perez Garcia Pando

The Barcelona Dust Regional Center (BDRC) provides daily forecasts of dust optical depth and dust surface concentrations, as part and coordination entity of the Northern Africa, Middle East and Europe (NAMEE) node of the World Meteorological Organization Sand and Dust Storm Warning Advisory and Assessment System (WMO SDS-WAS). Dust optical depth forecasts from the NAMEE SDS-WAS ensemble show a relatively good agreement, while the forecasts of dust surface concentrations show larger variability between models. Moreover, the consistency between dust optical depth, as an integrated column quantity, and surface concentration forecasts remains challenging. 

Since July 2024, vertical profiles of dust concentrations from the Multiscale Online Nonhydrostatic AtmospheRe Chemistry (MONARCH) model of the SDS-WAS ensemble have been made public on the BDRC website. This study presents the first evaluation of this new forecast product through comparisons with lidar observations, focusing on vertical profiles of total and dust extinction coefficients. Specifically, we used lidar measurements from the NASA Micro-Pulse Lidar Network (MPLNET) in the Mediterranean and North Africa area. While the comparison of the total extinction coefficient between MONARCH (550 nm) and MPLNET (532 nm) can be performed directly but is affected by unaccounted aerosols (e.g. sea salts, anthropogenic aerosols), the extraction of dust extinction coefficient from MPLNET products required additional processing. To this purpose, the POLIPHON algorithm was exploited to obtain the lidar-derived dust component from the total aerosol load and enable a fair intercomparison with modeled dust profiles. Initial descriptive and quantitative results confirm the model’s reliability in forecasting and predicting dust vertical profile characteristics.

Building on this evaluation, we explore the potential of leveraging lidar data to improve the dust ground concentration estimates of the MONARCH model forecasts. The proposed approach explores empirical adjustments of the model's surface concentration using lidar observations and validates these improvements against independent ground-based PM10 measurements collected by the European Environment Agency (EEA). The analysis is performed for three European sites, namely Tenerife, Barcelona, and El Arenosillo, for the period from July 2024 to January 2025.

The expanded aim of this work is to assess the feasibility of utilizing next-generation space-borne lidar systems, such as EarthCARE (Cloud, Aerosol, and Radiation Explorer), to enhance global dust surface concentration estimations from model forecasts.

This study highlights the synergy between observations and modeling, demonstrating how lidar observations could be exploited for correcting and improving model performance at both regional and global scales.

How to cite: Gilè, C., Emili, E., Escribano, J., Ilic, L., Jorba Casellas, O., and Perez Garcia Pando, C.: Evaluating the MONARCH Model with Lidar Data: A Step Toward Improving Global Dust Surface Concentrations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9052, https://doi.org/10.5194/egusphere-egu25-9052, 2025.

EGU25-10120 | ECS | Orals | GI4.3

Comparison of fresh and aged smoke particles simultaneously observed at the ACTRIS Potenza observatory  

Benedetto De Rosa, Nikolaos Papagiannopoulos, Michail Mytilinaios, Aldo Amodeo, Giuseppe D'Amico, Marco Rosoldi, Donato Summa, Ilaria Gandolfi, Christina–Anna Papanikolaou, Pilar Gumà-Claramunt, Teresa Laurita, Francesco Cardellicchio, Igor Veselovskii, Paolo Di Girolamo, and Lucia Mona

This study presents a detailed analysis of the optical and microphysical properties of biomass burning aerosols from two distinct smoke plumes observed on 16 July 2024 at the CIAO atmospheric observatory in Potenza, Italy. The lower layer corresponds to a local wildfire, while the upper layer correspond to  a long-range transported plume from Canada. The objective is to highlight significant differences in their characteristics and atmospheric impacts.

The local fire was characterized not only with lidar measurements, but with all the remote sensing instruments present in the observatory. The fire, ignited around 16:00 UTC approximately 2 km from the observatory, was detected within an hour. Ceilometer lidar and radar data showed that wildfire particles ascended to 3 km, where elevated humidity facilitated the formation of condensation nuclei, confirmed by a radiometer-observed peak in liquid water content. The ACSM (Aerosol Chemical Speciation Monitor) and aethalometer measurements show a significant peak around 20:00 UTC, which coincides with the deposition of the particles. The inversion results from lidar measurements revealed a low contribution of black carbon and fine-mode particles, consistent with incomplete combustion typical of small-scale fires. Furthermore, a strong dependence on humidity variations was observed, emphasizing the dynamic interaction between local fires and atmospheric conditions.

In contrast, the Canadian wildfire plume, transported at altitudes between 5.5 and 6.5 km, exhibited different characteristics. Due the complete combustion particles have a higher absorption properties. The lidar ratio at 532 nm exceeded that at 355 nm, similar with previous observations of aged wildfire plumes. During long-range transport, aging processes such as coagulation significantly altered the particles, increasing their effective radius. Microphysical analysis indicated the presence of larger, more absorbent particles compared to the local plume.

This study underscores the importance of integrating remote sensing and in-situ measurements to capture the lifecycle of wildfire events. The results reveal a great variability in smoke plume properties, which must be accounted for in radiative transfer models to accurately assess their atmospheric and climatic impacts.

How to cite: De Rosa, B., Papagiannopoulos, N., Mytilinaios, M., Amodeo, A., D'Amico, G., Rosoldi, M., Summa, D., Gandolfi, I., Papanikolaou, C., Gumà-Claramunt, P., Laurita, T., Cardellicchio, F., Veselovskii, I., Di Girolamo, P., and Mona, L.: Comparison of fresh and aged smoke particles simultaneously observed at the ACTRIS Potenza observatory , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10120, https://doi.org/10.5194/egusphere-egu25-10120, 2025.

EGU25-10454 | ECS | Orals | GI4.3

Raman lidar water vapor observations to assess the uncertainty of MLS and ERA5 at the upper troposhere 

Dunya Alraddawi, Philippe Keckhut, Florian Mandija, Guillaume Payen, Jean Charles Dupont, Christophe Pietras, Abdenour Irbah, Alain Sarkissian, Alain Hauchecorne, and Jacques Porteneuve

Water vapor information in the upper troposphere (UT) is crucial for understanding the thermodynamic conditions leading to the formation of cirrus clouds and persistent contrails. Both phenomena significantly contribute to aviation-induced radiative forcing, driving global mitigation efforts. Raman lidars provide high-resolution humidity profiles, describing altitudes prone to ice supersaturation—conditions that are challenging to detect and accurately represent in current models.

In this study, Raman lidar Water Vapor Mixing Ratio (WVMR) measurements from various sites in France were used to evaluate the performance of the ERA5 model in assessing humidity at typical aircraft altitudes. Additionally, the uncertainties in Microwave Limb Sounder (MLS) WVMR measurements at the same altitudes were assessed. Raman lidar profiles were aggregated into pseudo-monthly datasets to facilitate comparison with the limited number of MLS overpasses at each site, enabling validation of spatio-temporal pseudo-monthly lidar-matched MLS and ERA5 WVMR profiles.

The MLS dataset offers one of the longest records of WVMR, making it a valuable resource for trend assessment. This investigation enables the validated use of these datasets for studying UT humidity trends and variability on seasonal and annual scales over the past decade.

How to cite: Alraddawi, D., Keckhut, P., Mandija, F., Payen, G., Dupont, J. C., Pietras, C., Irbah, A., Sarkissian, A., Hauchecorne, A., and Porteneuve, J.: Raman lidar water vapor observations to assess the uncertainty of MLS and ERA5 at the upper troposhere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10454, https://doi.org/10.5194/egusphere-egu25-10454, 2025.

EGU25-10784 | Posters on site | GI4.3

Real-Time Monitoring of Air Pollution and Detection of Illegal Emissions Using Advanced Scanning LiDAR Technology 

Seong-min Kim, Kwanchul Kim, Gahye Lee, Jeong-min Park, Sea-ho Oh, Min-kyung Sung, Sangcheol Kim, Youndae Jung, Ilkwon Yang, Byung-Jin Choi, Sungchul Choi, and Changgi Choi

Air pollution is a persistent environmental and public health challenge, particularly in industrial areas characterized by diverse and diffuse emission sources. This study demonstrates the application of an advanced scanning LiDAR system for real-time monitoring of particulate matter (PM2.5, PM10) and the detection of illegal emissions in Gyeonggi Province, South Korea. The system employs advanced remote sensing technology, enabling 360° atmospheric scans within a 5 km radius at 30-minute intervals, with a spatial resolution of 30 meters.

During its deployment in the Sihwa National Industrial Complex, home to over 978 industrial facilities, the LiDAR system identified 192 potential illegal emission sources. Subsequent investigations confirmed 22 violations of environmental regulations, resulting in regulatory actions such as facility shutdowns and legal proceedings. The deployment led to a measurable improvement in air quality, evidenced by a reduction of 2.4 μg/m³ in PM2.5 levels during the operational period.

The integration of LiDAR data with complementary environmental datasets enabled precise spatiotemporal analyses, enhancing the efficiency of regulatory enforcement and fostering effective inter-agency collaboration. The results underscore the system’s potential to overcome limitations of conventional point-source monitoring, offering an innovative tool for large-scale industrial air pollution management.

This study highlights the scalability and precision of scanning LiDAR technology as a critical asset for real-time air quality monitoring and regulatory compliance. The findings advocate for broader adoption of this technology in industrial settings globally, emphasizing its ability to address complex environmental challenges and promote sustainable industrial practices.

Acknowledgement: This research was supported by a grant (2023-MOIS-20024324) of Ministry-Cooperation R&D Program of Disaster-Safety funded by Ministry of Interior and Safety (MOIS, Korea) and Climate & Environment Division Scientific Environment Surveillance Team in Gyeonggi-do Province, Korea.

How to cite: Kim, S., Kim, K., Lee, G., Park, J., Oh, S., Sung, M., Kim, S., Jung, Y., Yang, I., Choi, B.-J., Choi, S., and Choi, C.: Real-Time Monitoring of Air Pollution and Detection of Illegal Emissions Using Advanced Scanning LiDAR Technology, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10784, https://doi.org/10.5194/egusphere-egu25-10784, 2025.

EGU25-10819 | Posters on site | GI4.3

Advanced Scanning LiDAR for Real-Time Detection of Wildfires and Industrial Fires 

Kwanchul Kim, Seong-min Kim, Gahye Lee, Jeong-Min Park, Sea-ho Oh, Min-Kyung Sung, Youngmin Noh, Kwonho Lee, Young J. Kim, Woosuk Choi, Sungchul Choi, Changgi Choi, Chun-Sang Hong, Sangcheol Kim, Youndae Jung, Ilkwon Yang, and Byung-Jin Choi

This study introduces the development and application of the advanced scanning LiDAR system, SMART LiDAR MK-II(Samwoo TCS co., Ltd), designed for the early detection of wildfires and industrial fires. Traditional fire detection methods face limitations due to diverse atmospheric conditions, topographical factors, and variability in fire and smoke characteristics. To address these challenges, monitoring systems with spatial resolutions below 30 meters are essential. The SMART LiDAR MK-II employs dual wavelengths (532 nm and 1064 nm) and provides 360° observations with an angular resolution of approximately 3° within a 30-minute interval, enabling the real-time detection of smoke and particulate matter under various environmental conditions.

 

The system was validated through field deployment in the Sihwa Industrial Complex, South Korea, during a fire at an automotive painting factory on July 22, 2024. Positioned at a monitoring height of 55 meters and approximately 20 meters from the fire source, the SMART LiDAR MK-II detected smoke with peak PM10 and PM2.5 concentrations of 724 µg/m³ and 334 µg/m³, respectively. The smoke plume was observed dispersing over 5 km northward, influenced by prevailing winds. Furthermore, the system successfully captured the temporal reduction in particulate matter concentrations following fire suppression, demonstrating its capability to monitor emission dynamics and dispersion patterns.

 

Currently, SMART LiDAR MK-II is undergoing rigorous waterproof and dustproof testing to ensure operational reliability under diverse conditions, with commercialization in progress. This cutting-edge technology represents a significant advancement in LiDAR-based fire detection, offering high spatial resolution, sensitivity, and reliability for real-time monitoring of smoke emissions and atmospheric impacts. The results highlight the transformative potential of SMART LiDAR MK-II to enhance global fire detection and environmental monitoring capabilities.

 

Acknowledgment: This research was supported by a grant (2023-MOIS-20024324) from the Ministry-Cooperation R&D Program of Disaster-Safety funded by the Ministry of Interior and Safety (MOIS, Korea).

How to cite: Kim, K., Kim, S., Lee, G., Park, J.-M., Oh, S., Sung, M.-K., Noh, Y., Lee, K., Kim, Y. J., Choi, W., Choi, S., Choi, C., Hong, C.-S., Kim, S., Jung, Y., Yang, I., and Choi, B.-J.: Advanced Scanning LiDAR for Real-Time Detection of Wildfires and Industrial Fires, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10819, https://doi.org/10.5194/egusphere-egu25-10819, 2025.

EGU25-11218 | ECS | Posters on site | GI4.3

Relationships Between Surface Fluxes and Boundary Layer Dynamics: Statistics at the Land-Atmosphere Feedback Observatory (LAFO) 

Syed Saqlain Abbas, Andreas Behrendt, Oliver Branch, and Volker Wulfmeyer

We studied the convective boundary layer (CBL) processes and surface fluxes long-term statistics by using a combination of two Doppler lidars (DLs) and an eddy-covariance station (EC) at the Land-Atmosphere Feedback Observatory (LAFO), Stuttgart, Germany (Abbas et al., 2024). At LAFO (Späth et al, 2023), one DL is continuously operated in vertical pointing mode, while the second is in six-beam scanning mode, both providing high-resolution data with resolutions of 1 s and 30 m. From this combination of DLs, we derived the profiles of vertical wind variance (Lenschow et al, 2000; Wulfmeyer et al, 2024), horizontal wind variance and turbulent kinetic energy (TKE) as well as CBL depth 𝑧𝑖 (Bonin et al., 2017; Bonin et al., 2018). The surface turbulent fluxes are acquired from an EC station in the agricultural fields of our university ~500 m away from the DLs. Daytime statistics are derived from 20 convective days from May to July 2021 with cloud cover < 40%. In this data set, we found a maximum of the CBL height averaged over all these days ⟨𝑧𝑖⟩ of (1.53 ±0.07) km at 13:30 UTC, which is about 2 hours after local noon. We found counter-clockwise hysteresis patterns between the CBL height and the surface fluxes. In the development phase, these relationships were approximately linear. In the early afternoon, the relationships reached a peak phase with both large fluxes and high values of ⟨𝑧𝑖⟩. At 12:00 UTC, just after local noon, the maximum values of vertical, horizontal, and total TKE were 0.55 m2s-2, 1.26 m2s-2 and 1.71 m2s-2 at heights of (0.30±0.06)⟨𝑧𝑖⟩ , (0.56±0.06)⟨𝑧𝑖⟩, and (0.40±0.06)⟨𝑧𝑖⟩, respectively. In the decay phase in the later afternoon, the relationships show non-linear patterns with larger values of ⟨𝑧𝑖⟩ for the same surface fluxes than in the morning. Furthermore, we analyzed relationships between the vertical and horizontal wind components and total TKE. Also, here, we found non-linear patterns in the three CBL phases.


Abbas, S. S., et al., 2024, https://doi.org/10.5194/egusphere-2024-3878
Späth et al., 2023, https://doi.org/10.5194/gi-12-25-2023
Lenschow et. al., 2000, https://doi.org/10.1175/1520-0426(2000)017<1330:MSTFOM>2.0.CO;2
Wulfmeyer et al., 2024, https://doi.org/10.5194/amt-17-1175-2024
Bonin et. al., 2017, https://doi.org/10.5194/amt-10-3021-2017
Bonin et. al., 2018, https://doi.org/10.1175/JTECH-D-17-0159.1

How to cite: Abbas, S. S., Behrendt, A., Branch, O., and Wulfmeyer, V.: Relationships Between Surface Fluxes and Boundary Layer Dynamics: Statistics at the Land-Atmosphere Feedback Observatory (LAFO), EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11218, https://doi.org/10.5194/egusphere-egu25-11218, 2025.

EGU25-11468 | ECS | Posters on site | GI4.3

Network Doppler Lidar for simultaneous multi-parameter observations 

Jan Froh, Josef Höffner, Alsu Mauer, Thorben Mense, Ronald Eixmann, Gerd Baumgarten, Alexander Munk, Sarah Scheuer, and Michael Strotkamp

We present the development progress of our compact multi-field-of-view lidar units for investigating small- to large-scale processes in the atmosphere. Matched narrowband laser and receiver enable precise daylight aerosol measurements with high aerosol visibility and high Doppler wind sensitivity in the troposphere/stratosphere and above. We present recent results with focus on extended measurement capabilities of our transportable systems.

Daylight capable Doppler lidars are complex systems particularly as lidar arrays require compact units with automated functionality. To study the 3-dimensional structure of small- to large-scale atmospheric processes we developed a universal Doppler lidar platform with multiple fields of view. All required technologies are included for studying Mie scattering (aerosols), Rayleigh scattering (air molecules), and resonance fluorescence (potassium atoms) from the troposphere (5 km) to the thermosphere (100 km). We developed unique frequency scanning laser and filter techniques that enable multiple observations (wind, temperature, aerosols, metal density). The combination of narrowband emitter and receiver allow a spectral high resolved characterization of the backscattered Doppler signals with a high wind sensitivity and aerosol visibility. Our current developments focus on enhancing lidar measurement capabilities of multiple parameters together with transferring the technology into industry (Project LidarCUBE) and demonstration of lidar array with enhanced daylight capability (EULIAA – European Lidar Array for Atmospheric Climate Monitoring). We will show recent results of our unique lidar technique with focus on aerosol measurements and more.

How to cite: Froh, J., Höffner, J., Mauer, A., Mense, T., Eixmann, R., Baumgarten, G., Munk, A., Scheuer, S., and Strotkamp, M.: Network Doppler Lidar for simultaneous multi-parameter observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11468, https://doi.org/10.5194/egusphere-egu25-11468, 2025.

EGU25-11819 | Posters on site | GI4.3

Estimation of optical and microphysical characteristics of contrails using Lidar at SIRTA observatory, Paris 

Cheikh Dione, Jean-Charles Dupont, Karine Caillault, Nicolas Gourgue, Christophe Pietras, and Martial Haeffelin

Contrails are local and thin anthropogenic clouds that are difficult to predict by numerical weather forecasting models. Given their local radiative impact, it is urgent to properly document their characteristics in order to improve their parametrization in weather models and evaluate their contribution to global warming. In the framework of the Climaviation project (Funded by the French Direction Générale de l’Aviation Civile (DGAC)), this study aims to quantify the optical, geometrical and microphysical characteristics of contrails at the SIRTA observatory in Palaiseau, France. We used a co-localised instrumental synergy composed of the Lidar IPRAL (a multichannel raman Lidar), a total sky camera, and aircraft flight altitudes to detect the occurrence of contrails over the site during the 2018-2023 period. Based on three (3) case studies, the particular and molecular integration methods are applied on the Lidar backscatter, to estimate the optical depth of contrails. Vertical profiles of temperature and relative humidity from Trappes radiosoundings are used to characterize the atmospheric conditions classified into three (3) categories of contrail evolution (non-persistent, persistent, and spreading). The results show that the optical thickness of contrails can reach 0.3 for contrails formed in a thick persistent layer. It is lower for contrails developing in a non-persistent layer. During daytime, the contrails contribute to reducing the surface downwelling and upwelling measured shortwave radiation in the order of 218 and 50 W m-2 respectively. Their impact on longwave radiation is relatively negligible.

How to cite: Dione, C., Dupont, J.-C., Caillault, K., Gourgue, N., Pietras, C., and Haeffelin, M.: Estimation of optical and microphysical characteristics of contrails using Lidar at SIRTA observatory, Paris, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11819, https://doi.org/10.5194/egusphere-egu25-11819, 2025.

EGU25-12416 | Orals | GI4.3

Building a Long-Term Cloud Record from Spaceborne Lidars: Bridging CALIOP to ATLID 

Artem Feofilov, Hélène Chepfer, Vincent Noël, and Marius Dahuron

Clouds exert multifaceted radiative effects on Earth's energy budget, serving as both insulators and reflectors of incoming solar radiation while also trapping outgoing infrared radiation. Consequently, clouds contribute to both surface cooling and warming processes, profoundly influencing regional and global climate dynamics. Despite their crucial role in Earth's energy balance, uncertainties persist regarding their feedback mechanisms.

A comprehensive understanding of clouds, including their spatial coverage, vertical distribution, and optical properties, is imperative for accurate climate prediction. Satellite-based observations, particularly those from active sounders, have offered continuous monitoring of clouds with high vertical and horizontal resolution since 2006. However, comparing cloud data from different spaceborne lidars presents challenges due to variations in wavelength, pulse energy, detector type, and local observation times.

This study discusses a methodology aimed at reconciling cloud data derived from several disparate spaceborne lidar platforms: CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation), which operated from 2006 to 2023; ALADIN/Aeolus (Atmospheric Laser Doppler Instrument), which operated from 2018 to 2023; IceSat-2, operational since 2018; and ATLID/EarthCARE (ATmospheric LIDar), launched last year.

For historical reasons, we use the Scattering Ratio at 532 nm (SR532) as a baseline for defining clouds across all lidars. The numerator contains the Attenuated Total Backscatter at 532 nm (ATB532), while the denominator includes a calculated Attenuated Molecular Backscatter at 532 nm (AMB532), assuming a cloud-free atmospheric profile. For measurements at other wavelengths, we convert the retrieved optical properties to SR532 and ATB532 to enable direct comparison. We demonstrate that this approach facilitates the retrieval of comparable cloud data for CALIOP and ALADIN using real measurements and for CALIOP and ATLID using synthetic measurements.

For lidars overlapping in time, the aforementioned cloud detection parameters can be fine-tuned to ensure a seamless transition between datasets. Collocated data are analyzed with respect to cloud fraction at different latitudes, altitudes, and seasons, and any differences are explored and corrected for, potentially accounting for instrument sensitivity or noise. However, when instruments do not overlap in time, an additional inter-calibrational procedure is necessary. We show how IceSat-2 can serve as a reference to align CALIOP and ATLID cloud datasets.

How to cite: Feofilov, A., Chepfer, H., Noël, V., and Dahuron, M.: Building a Long-Term Cloud Record from Spaceborne Lidars: Bridging CALIOP to ATLID, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12416, https://doi.org/10.5194/egusphere-egu25-12416, 2025.

EGU25-12490 | Orals | GI4.3

 d13C carbon isotopic composition of CO2 in the atmosphere by Lidar 

Fabien Gibert, Dimitri Edouart, Didier Mondelain, Thibault Delahaye, Claire Cénac, and Camille Yver

Our understanding of the global carbon cycle needs for new observations of CO2 concentration at different space and time scales but also would benefit from observations of additional tracers of intra-atmospheric or surface-atmosphere exchanges to characterize sources and sinks. Lidar is a well-known promising technology for this research as it can provide, at the same time, structure of the atmosphere, dynamics and composition of several trace gas concentration. In this framework, a coherent differential absorption lidar (CDIAL) has been developed at LMD to measure simultaneously and separately 12CO2 and 13CO2 isotopic composition of CO2in the atmosphere. It also provides the wind speed along the line of sight of the laser with an additional Doppler ability. This paper investigates the methodology of three wavelengths DIAL in the spectral domain of 2-µm to obtain range-resolved CO2 isotopic ratio d13C. The set-up of the lidar as well as the signal processing is described in details. First atmospheric measurements along three days are achieved in the surface layer above the suburban area of Ecole Polytechnique campus, Palaiseau, France. Typical performances of the instrument (median values along 70h of measurement) with 10 min of time averaging show: (1) a precision around 0.6% for 1.2 km range resolution for 12CO2 mixing ratio (2) a precision around 3.2% for 1.6 km range resolution for 13CO2 mixing ratio. In situ co-located gas analyser measurements are used to correct for biases that are explained neither by the spectroscopic database accuracy nor the signal processing and will need further investigation. Nevertheless, this preliminary study enables to make a useful state of the art for current lidar ability to provide d13C measurements in the atmosphere with respect to geophysical expected anomalies and to predict the necessary performances of a future optimized instrument.

How to cite: Gibert, F., Edouart, D., Mondelain, D., Delahaye, T., Cénac, C., and Yver, C.:  d13C carbon isotopic composition of CO2 in the atmosphere by Lidar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12490, https://doi.org/10.5194/egusphere-egu25-12490, 2025.

EGU25-12573 | ECS | Orals | GI4.3

Calibration of water vapour Raman lidar using GNSS precipitable water vapour and reanalysis model data 

Arlett Díaz Zurita, Daniel Pérez Ramírez, David Neil Whiteman, Onel Rodríguez Navarro, José Antonio Bravo Aranda, María José Granados Muñoz, Juan Luis Guerrero Rascado, Jesus Abril Gago, Sol Fernández Carvelo, Ana del Águila Pérez, Manuel Antón Martínez, Javier Vaquero Martínez, Alexander Haefele, Giovanni Martucci, Inmaculada Foyo Moreno, José Antonio Benavent Oltra, Lucas Alados Arboledas, and Francisco Navas Guzmán

Water vapour is a crucial and highly variable greenhouse gas in the Earth's atmosphere, which can significantly influence radiative balance, energy transport, and photochemical processes. It can also affect the radiative budget indirectly through cloud formation and by altering the size, shape, and chemical composition of aerosol particles. Accurate and systematic observations are essential for understanding its impacts and improving climate projections. Raman lidar technique is widely used for obtaining water vapour mixing ratio (WVMR) profiles with high vertical and temporal resolution. It relies on Raman scattering from water vapour and nitrogen molecules and is usually calibrated by reference to one or more external measurements of water vapour.

This study presents a hybrid methodology for obtaining high temporal resolution calibration constants for Raman lidar measurements, and posteriorly retrieves high accuracy WVMR profiles. It combines correlative measurements of precipitable water vapour (PWV) for calibrating lidar measurements with Numerical Weather Prediction (NWP) data to reconstruct the profile within the incomplete lidar overlap region. This methodology is applied to the MULHACEN Raman lidar system, operational at UGR station of the University of Granada (Spain) for the long period of 2009-2022. The hybrid method was optimized for the station by selecting Global Navigation Satellite System (GNSS) PWV data as the most appropriate due to its better agreement with correlative radiosondes (R2 of 0.95). Furthermore, the ERA5 model was selected as the most appropriate for reconstructing the incomplete lidar overlap region due to its better temporal and spatial resolution and its accuracy when evaluated against radiosonde data. The advantages of the hybrid calibration methodology are evaluated compared to traditional radiosonde-based methods or PWV data assuming a constant WVMR in the incomplete overlap region. Although all methods generally provide good calibration constants, the hybrid approach presented the best performance, as quantified by an R2 of 0.85, a slope of 0.97, and an intercept of -0.05 g/kg, particularly under conditions where atmospheric layers are not well-mixed. Comparison with radiosonde data revealed excellent agreement, with a mean bias error of -0.11 ± 0.38 g/kg and a standard deviation of 1.04 ± 0.35 g/kg across the entire period and vertical range (0 – 6.0 km agl). The most important result of this study is the ability to continuously evaluate calibration constants during 14 years of MULHACEN operation. The posterior application of the hybrid methodology to all MULHACEN measurements enabled the generation of a comprehensive long time database of WVMR profiles.

How to cite: Díaz Zurita, A., Pérez Ramírez, D., Neil Whiteman, D., Rodríguez Navarro, O., Bravo Aranda, J. A., Granados Muñoz, M. J., Guerrero Rascado, J. L., Abril Gago, J., Fernández Carvelo, S., del Águila Pérez, A., Antón Martínez, M., Vaquero Martínez, J., Haefele, A., Martucci, G., Foyo Moreno, I., Benavent Oltra, J. A., Alados Arboledas, L., and Navas Guzmán, F.: Calibration of water vapour Raman lidar using GNSS precipitable water vapour and reanalysis model data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12573, https://doi.org/10.5194/egusphere-egu25-12573, 2025.

We present a Doppler lidar designed to detect the molecular spectrum characteristics, which are attributed to the Rayleigh-Brillouin scattering, in the atmospheric boundary layer. The suggested system is a continuous-wave, infrared Doppler lidar based on a bi-static transceiver and a coherent in-phase/quadrature detection scheme. For the detection of the features of the Rayleigh-Brillouin spectrum we use fiber-coupled, balanced photodetectors and a digitizer with a 1.6 GHz bandwidth. This broad bandwidth is necessary for the detection of Doppler shifts not only at frequencies of atmospheric winds, but also of the ones corresponding to molecular and acoustic speed that extend over several hundred megahertz. We demonstrate that using this configuration it is possible to detect the molecular Rayleigh-Brillouin spectrum over 30-minute time periods. The observational range of this system is focused on the lower part of the atmosphere (< 200 m) and the objective is to investigate if the resolved features of the Rayleigh-Brillouin spectrum can be related to the temperature, which could lead to the development of a novel vertical profiler of atmospheric temperature.

How to cite: Angelou, N. and Mann, J.: On the measurement of the Rayleigh-Brillouin spectrum and atmospheric temperature using a coherent Doppler lidar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12657, https://doi.org/10.5194/egusphere-egu25-12657, 2025.

EGU25-12951 | Posters on site | GI4.3

Gravity waves observed by lidar at the center and edge of the Southern polar vortex 

Natalie Kaifler and Bernd Kaifler

Our Rayleigh lidar systems provide temperature profiles up to 100 km altitude at both a site at southern hemisphere mid-latitudes and at South Pole. Very strong orographic gravity waves dominate in the lee of the Southern Andes in winter, a region proximate to the polar vortex edge where strong winds prevail. In contrast, despite being situated within the stable polar vortex core, continuous but weaker gravity waves are observed above Amundsen-Scott station at South Pole. Potential sources for these waves include catabatic winds flowing across the Transantarctic Mountains – which also give rise to polar stratospheric clouds-, polar vortex dynamics, or lateral progagation from mid-latitudes. We present examples of gravity wave measurements and statistical analyses derived from our multi-year, ongoing datasets.

How to cite: Kaifler, N. and Kaifler, B.: Gravity waves observed by lidar at the center and edge of the Southern polar vortex, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12951, https://doi.org/10.5194/egusphere-egu25-12951, 2025.

EGU25-14705 | ECS | Orals | GI4.3

The calibration and validation of XCO2 measured by Lidar onboard DQ-1 

Lu Zhang and Xifeng Cao Cao

Atmospheric carbon dioxide (CO2) is the primary anthropogenic driver of climate change, accounting for more than half of the total effective radiative forcing (ERF). The accurate monitoring of carbon dioxide is essential to study the global carbon cycle and radiation budget on Earth.The Aerosol and Carbon Detection Lidar (ACDL) instrument, as the first space-borne integrated path differential absorption (IPDA) light detection and ranging (Lidar) for XCO2, was successfully launched in April 2022 onboard the DaQi-1 (DQ-1) satellite.During the two years of on-orbit operation, we constantly updated the processing methods, including the spectral broadening of CO2 caused by water vapor, etc. Finally, we calibrated and validated  the CO2 retrieved by DQ-1 usingTCCON and COCOON, and the results showed that the deviation reached the satellite design demand (1ppm).

How to cite: Zhang, L. and Cao, X. C.: The calibration and validation of XCO2 measured by Lidar onboard DQ-1, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14705, https://doi.org/10.5194/egusphere-egu25-14705, 2025.

EGU25-15242 | ECS | Posters on site | GI4.3

A field intercomparison of inter-instrument variability of six co-located Vaisala CL61 lidar-ceilometers 

Dana Looschelders, Andreas Christen, Sue Grimmond, Simone Kotthaus, Jean-Charles Dupont, Daniel Fenner, Martial Haeffelin, and William Morrison

With the advances in ground-based remote sensing technology, measurement networks of automatic aerosol lidar-ceilometers are developing rapidly across Europe and worldwide. Characterising inter-instrument variability of sensors is crucial to assessing uncertainties in observational campaigns, networks, and for data assimilation. It allows the determination of thresholds that need to be exceeded for the detection of meaningful atmospheric differences between observations obtained at different locations (e.g. urban vs rural).

We co-locate six Vaisala CL61 automatic lidar-ceilometers at the SIRTA atmospheric observatory (Palaiseau, France) for a period of ten days to quantify instrument-related differences in several observed variables: profiles of attenuated backscatter and the linear depolarisation ratio (LDR), as well as derived cloud variables, such as cloud base height (CBH) and cloud cover fraction (CCF), and mixed-layer height. Analysing intervals between 5 and 60 min, median absolute differences between sensors are used to quantify inter-instrument uncertainties. For backscatter and LDR, we differentiate between conditions with rain, clear sky, and clouds, respectively.

The agreement between instruments is capable of resolving climatological differences in mesoscale conditions (5 - 50 km, e.g. across cities) for both profile variables and derived cloud variables and layer heights. However, differences exist and can be linked to signal-to-noise ratio (SNR) and atmospheric conditions. The median absolute inter-sensor differences for 15 min aggregation intervals (AD50) are 1.9 % for total CCF (excluding clear sky and fully overcast conditions) and 7.3 m for CBH. Cloud variables agree better for boundary layer clouds where the first (of five) cloud layer < 4 km agl. The mixed-layer height AD50 is 0 m. Median differences smaller than two instrument range gates (9.6 m) highlight the close inter-instrument agreement.

How to cite: Looschelders, D., Christen, A., Grimmond, S., Kotthaus, S., Dupont, J.-C., Fenner, D., Haeffelin, M., and Morrison, W.: A field intercomparison of inter-instrument variability of six co-located Vaisala CL61 lidar-ceilometers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15242, https://doi.org/10.5194/egusphere-egu25-15242, 2025.

EGU25-15290 | ECS | Orals | GI4.3

AIRflows - a novel airborne Doppler lidar for high resolution wind measurements 

Philipp Gasch, Andreas Wieser, Thomas Feuerle, Franziska Winter, and Christoph Bollig

Wind is a core state variable of the atmosphere. Extending the capabilities of ground-based measurement systems, airborne Doppler lidar (ADL) onboard research aircraft allows for targeted and spatially resolved wind measurements, which are crucial for localized severe weather events or in inaccessible regions such as over water and complex terrain.

A novel ADL system – AIRflows (‘AIRborne fixed-beam lidar fowind measurements‘)  – has been developed by the Karlsruhe Institute of Technology (KIT) in collaboration with scientific and industrial partners during the last two years.
Up to now, ADL systems use a single Doppler lidar attached to a scanner to provide radial velocity measurements under multiple viewing angles. Multiple viewing angles are needed to reconstruct the 3D wind from the unidirectional radial velocity measurements. Due to cost and size reductions of Doppler lidar units over the recent years, it has now become possible to construct an ADL system that uses multiple lidars with fixed-direction beams, instead of a single lidar with a scanning beam. The simultaneous availability of multiple viewing angles brings advantages: Simulation results have demonstrated that a multi-lidar system can achieve approximately one order of magnitude improved spatial wind measurement resolution as well as higher accuracy, compared to existing scanning systems.

This contribution presents the novel AIRflows system developed by KIT. AIRflows implements the novel fixed-beam, multi-lidar concept onboard the TU Braunschweig Cessna F406 research aircraft. The system uses five modified Doppler lidar modules manufactured by Abacus Laser, one pointing nadir and the other four pointing forward, aft, left and right at an elevation of 30° from nadir.
The first flights deploying AIRflows have been successfully completed during summer 2024. Initial analysis demonstrates wind profiles at 100 m spatial resolution, allowing to resolve fine-scale 3D winds inside the PBL for the first time. As part of the tests, flights to the Alps were conducted in preparation for the upcoming international TEAMx campaign. AIRflows measurements across Alpine valleys and crests provide previously unattainable insight into vertical wind and valley circulations in complex terrain. Similarly, AIRflows measurements across a wind farm in the North Sea provide novel vertically resolved insight into wind farm wake behavior.

Overall, AIRflows revolutionizes the field of airborne wind measurements by providing an order of magnitude improved spatial resolution as well as higher measurement accuracy, compared to previously existing ADL.

How to cite: Gasch, P., Wieser, A., Feuerle, T., Winter, F., and Bollig, C.: AIRflows - a novel airborne Doppler lidar for high resolution wind measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15290, https://doi.org/10.5194/egusphere-egu25-15290, 2025.

EGU25-15418 | ECS | Posters on site | GI4.3

Estimation of the Optical properties of Arctic Cirrus Clouds: Insights fromLIDAR measurements and Monte Carlo simulations 

Gopika Gupta, Peter Voleger, Thomas Kuhn, and Janos Stenszky

Cirrus clouds play a critical role in Earth's energy balance by influencing radiative
processes, reflecting incoming solar radiation, and trapping outgoing infrared radiation. In the
Arctic, extreme conditions limit the observational networks and hinder direct measurements.
However, among various remote sensing tools, LIght Detection And Ranging (LIDAR)
emerges as one of a reliable tool for long-term monitoring of cirrus cloud optical properties
over the Arctic region. The extinction coefficient, derived from LIDAR measurements and
essential for evaluating the radiative effects of cirrus clouds, is strongly impacted by the
Multiple Scattering Factor (MSF). In this regard, the present study aims to estimate the MSF
by simulating LIDAR signals using the Monte Carlo method. The input parameters for the
Monte Carlo simulations include the geometry of the atmosphere and optical properties
(including extinction and Mueller matrix). Furthermore, the Mueller matrix is estimated based
on the size distribution and particle shape information acquired through the in-situ measurement
from the Balloon-borne Ice Cloud Particle Imager (B-ICI) instrument. The MSF contribution,
at least in part, depends on the characteristics of the LIDAR, particularly its Field of View. As
a result, new simulations are required, and previous results from older studies cannot be directly
applied.
The photon backscatter information obtained from the Analog and Photon
counting channels of the ground-based LIDAR instrument installed at IRF, Kiruna (68ºN,
20ºE), is utilised to estimate the cirrus cloud's optical properties. To address the instrument’s
non-linear behaviour at higher signal intensities, a glueing procedure is performed to merge the
Analog and the Photon counting signal. The resulting glued signal undergoes multiple
corrections, including background noise subtraction, signal-to-noise ratio enhancement, and
range corrections. The Dynamic Wavelet Covariance Transform (DWCT) technique is
deployed to the corrected LIDAR signal to estimate the cloud top and base altitude information.
Subsequently, an inversion technique incorporating MSF, such as the Sassen method, is chosen
for the current analysis.
The estimated cirrus cloud optical properties using the ground-based LIDAR will
subsequently be validated against EarthCARE’s ATmospheric LIDar (ATLID) satellite
observations. This study enhances the accuracy of cirrus cloud parameterisation, contributing
to improved climate models and a deeper understanding of Arctic cloud-radiative interactions.

How to cite: Gupta, G., Voleger, P., Kuhn, T., and Stenszky, J.: Estimation of the Optical properties of Arctic Cirrus Clouds: Insights fromLIDAR measurements and Monte Carlo simulations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15418, https://doi.org/10.5194/egusphere-egu25-15418, 2025.

In August 2022, China successfully launched the Terrestrial Ecosystem Carbon Inventory Satellite (TECIS). The primary payload of this satellite is an onboard multi-beam lidar system, which is capable of observing aerosol optical parameters on a global scale. This pioneering study used the Fernald forward integration method to retrieve aerosol optical parameters based on the Level 2 data of the TECIS, including the aerosol depolarization ratio, aerosol backscatter coefficient, aerosol extinction coefficient, and aerosol optical depth (AOD). The validation of the TECIS-retrieved aerosol
optical parameters was conducted using CALIPSO Level 1 and Level 2 data, with relative errors within 30%. A comparison of the AOD retrieved from the TECIS with the AERONET and MODIS AOD products yielded correlation coefficients greater than 0.7 and 0.6, respectively. The relative error
of aerosol optical parameter profiles compared with ground-based measurements for CALIPSO was within 40%. Additionally, the correlation coefficients R2 with MODIS and AERONET AOD were approximately between 0.5 and 0.7, indicating the high accuracy of TECIS retrievals. Utilizing the TECIS retrieval results, combined with ground air quality monitoring data and HYSPLIT outcomes, a typical dust transport event was analyzed from 2 to 7 April 2023. The results indicate that dust was transported from the Taklamakan Desert in Xinjiang, China, to Henan and Anhui provinces, with a gradual decrease in the aerosol depolarization ratio and backscatter coefficient during the transport process, causing varying degrees of pollution in the downstream regions. This research verifies the accuracy of the retrieval algorithm through multi-source data comparison and demonstrates the potential application of the TECIS in the field of aerosol science for the first time. It enables the fine-scale regional monitoring of atmospheric aerosols and provides reliable data support for the three-dimensional distribution of global aerosols and related scientific applications.

How to cite: Chen, B.: The First Validation of Aerosol Optical Parameters Retrieved from the Terrestrial Ecosystem Carbon Inventory Satellite (TECIS) and Its Application, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15492, https://doi.org/10.5194/egusphere-egu25-15492, 2025.

EGU25-16068 | ECS | Orals | GI4.3

Comprehensive Study of Cloud Characteristics over a High Altitude Station - Leh, India using Ground-Based Lidar and Satellite Observations 

Ruchita Shah, Som Sharma, Dharmendra Kamat, Shantikumar Ningombam, Dorje Angchuk, and Rohit Srivastava

A rise of approximately 1°C in global average temperature is influencing sea surface temperature, sea-level, intensity of storms, frequency and severity of hydro-meteorological extreme events. Such effects are comparatively more pronounced in tropical and sub-tropical zones, wherein Leh-Ladakh region of Indian subcontinent, is peculiar and characterized by extreme weather conditions. The present work unravels the cloud characteristics over the Leh region using ground-based ceilometer lidar (3255 m above mean sea level), remote-sensing, and reanalysis data sets for one-year (September 2022–August 2023). Variations in cloud base height (CBH) was observed with lidar, enabling the measurement of CBH up to three distinct layers, designated as CBH1, CBH2, and CBH3, respectively. This study reveals distinct seasonal and altitudinal variations in CBH, with cloud occurrence frequencies peaking during the pre-monsoon (67.94%) and monsoon (98%) seasons, reflecting the onset and active phases of the Indian summer monsoon. Month of July was recorded with the highest prevalence of multi-layered clouds (84.03%), which includes triple-layered clouds (CBH3, 42.13%) dominating over double-layered (CBH2, 25.98%) and single-layered (CBH1, 15.92%) clouds. Seasonal analysis showed a dominance of mid-level clouds (~3–6 km, 77.53%), while high-level clouds (~6–18 km, 4.43%) were less frequent. Altostratus and altocumulus clouds were particularly prominent across all seasons, with their variability linked to topographic and climatic factors. The ceilometer's high-resolution measurements captured the temporal dynamics of CBH, which aligned with satellite and reanalysis data, demonstrating the value of ground-based instruments in complementing remote sensing technologies. These findings provide valuable insights into cloud dynamics and their role in extreme weather events such as cloudbursts and intense rainfall, which are increasingly frequent in the Himalayan region. By improving our understanding of cloud–precipitation interactions, this study offers critical information for enhancing weather forecasting, informing rainfall prediction models, and supporting climate adaptation strategies in climatically vulnerable high-altitude regions.   

How to cite: Shah, R., Sharma, S., Kamat, D., Ningombam, S., Angchuk, D., and Srivastava, R.: Comprehensive Study of Cloud Characteristics over a High Altitude Station - Leh, India using Ground-Based Lidar and Satellite Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16068, https://doi.org/10.5194/egusphere-egu25-16068, 2025.

EGU25-16402 | Posters on site | GI4.3

1.65 µm CH4 ground-based differential absorption lidar measurements in the atmosphere 

Dimitri Edouart, Fabien Gibert, and Claire Cénac

Methane (CH4) is the second anthropogenic greenhouse gas (GHG) in the atmosphere that contributes to the global warming after CO2. If the methane emissions have a unique sink by OH oxidation, the various different sources, both anthropogenic (around 2/3) and natural, make complex the understanding of its atmospheric concentration. On the anthropogenic side (mainly gas exploitation and burning) it is fundamental to have a tool to verify inventories at different scales (from local methanizer to megacity) and prevent production network leakage in the atmosphere. As for surface-atmosphere exchanges of CO2, it is fundamental to study at different scales the spatial pattern and magnitude of the natural CH4 sources (biogenic anaerobic degradation of organic matter in wetlands, landfill and waste, livestock, rice cultivation, thermite, geological sources) and to understand their evolution with the global warming.

Lidar has an important role to play in such topic as it can make: (i) a 3D mapping of CH4 concentration in anthropogenic plumes, (ii) vertical profiles to study transport processes in the atmosphere, (iii) even measure direct flux and (iv) provide CH4 Earth global measurements from a space platform as it will be for MERLIN CH4 integrated path differential absorption lidar CNES/DLR ongoing mission.

A new ground-based Differential Absorption Lidar (DIAL) for atmospheric methane (CH4) profiling has been developed at LMD. The lidar emitter relies on a new hybrid fibered/bulk Er:YAG laser that delivers dual On/Off 8 mJ/ 300 ns pulses at a repetition frequency of 1 kHz in the methane line triplet at 1645.55 nm and out of at 1645.3 nm. It is associated with a direct detection receiver with a 50cm diameter telescope, a 2-nm linewidth interference optical filter, a near infrared photomultiplier (PMT) and a data acquisition and real time signal processing system working both in analogic and photon counting mode depending the application. First horizontal and vertical measurements in the atmosphere have been achieved and compared with in situ sensor and will be presented at the conference.

How to cite: Edouart, D., Gibert, F., and Cénac, C.: 1.65 µm CH4 ground-based differential absorption lidar measurements in the atmosphere, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16402, https://doi.org/10.5194/egusphere-egu25-16402, 2025.

EGU25-16832 | ECS | Orals | GI4.3

Integration of Doppler Wind Lidars in E-Profile wind profiling network 

Eric Sauvageat, Rolf Rüfenacht, Maxime Hervo, Myles Turp, Markus Kayser, Ronny Leinweber, Volker Lehmann, Steven Knoop, Alexander Gohm, and Alexander Haefele

E-Profile is the EUMETNET Programme coordinating the measurements of vertical profiles of wind, aerosols and clouds from radars and lidars in Europe. The E-Profile wind network provides near real-time vertical profiles of wind from weather radars and dedicated wind profilers with the main goal to promote the usability of these data for operational meteorology and provide expertise to both the data provider and the end-user.

Ground-based scanning Doppler Wind Lidars (DWLs) are capable of measuring wind profiles in the atmospheric boundary layer (ABL) at a high spatial and temporal resolution and they have the potential to improve the short-term wind forecast. With the availability of commercial DWLs in the last decade, many meteorological services and scientific institutions are now operating such instruments or are planning to do so in the future in Europe.

To extend the benefit of these observations and promote data sharing, these instruments have recently been integrated in E-Profile wind profiling network. Using an open-source code developed at the Deutscher Wetterdienst (DWD), instrument’s data from different manufacturers are processed in a harmonized way to provide 10 minutes averaged wind profiles in the ABL. Data are converted to BUFR and distributed in near real-time on the Global Telecommunication System (GTS), making them available globally for data assimilation. At the moment, 12 DWLs from 4 European countries are being processed operationally and more instruments are expected to join the network in 2025.

Here, we present the integration of DWL into the E-Profile wind network, its associated challenges and the requirements for the scan strategies. We also show comparisons at different sites against other wind profiling instruments (e.g. radar wind profilers) and against model data. Finally, we also discuss the future improvements to the network.

How to cite: Sauvageat, E., Rüfenacht, R., Hervo, M., Turp, M., Kayser, M., Leinweber, R., Lehmann, V., Knoop, S., Gohm, A., and Haefele, A.: Integration of Doppler Wind Lidars in E-Profile wind profiling network, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16832, https://doi.org/10.5194/egusphere-egu25-16832, 2025.

EGU25-16880 | ECS | Posters on site | GI4.3

The desert dust impact on the Boundary Layer in the Atlantic 

Ioanna Tsikoudi, Eleni Marinou, Maria Tombrou, Eleni Giannakaki, Emmanouil Proestakis, Konstantinos Rizos, and Vassilis Amiridis

The study investigates the dynamics of the Boundary Layer (BL) over the Atlantic Ocean, with a focus on the region surrounding Cabo Verde, using a combination of ground-based PollyXT lidar, satellite lidar data from Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO), radiosondes, and European Centre for Medium-Range Weather Forecasts (ECMWF) model output. The comparison of CALIPSO lidar profiles with ECMWF reanalysis revealed strong correlations for BL top over open ocean regions but less agreement in dust-affected areas closer to the African continent. In these regions, satellite lidar indicated higher BL tops than those estimated by ECMWF, likely due to the existence of high of aerosol concentrations, which play a crucial role in shaping dynamics. Observations in Cabo Verde highlight distinctive Marine Atmospheric Boundary Layer (MABL) characteristics, such as limited diurnal evolution, but also show the potential for BL heights to reach up to 1 km, driven by factors like strong winds that increase mechanical turbulence. Additionally, this study illustrates the challenges in accurately determining the BL height using lidar and radiosondes, examining cases with strong inversions that prevent vertical mixing, but also weaker inversions that allow for the penetration of dust particles within BL. Integrating multiple observational sources and techniques is essential for validating remote sensing data and enhancing BL characterizations. The findings underscore the complex interactions between marine and dust-laden air masses over the Atlantic, which are essential for understanding the dynamic processes in aerosol-cloud interactions.

How to cite: Tsikoudi, I., Marinou, E., Tombrou, M., Giannakaki, E., Proestakis, E., Rizos, K., and Amiridis, V.: The desert dust impact on the Boundary Layer in the Atlantic, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16880, https://doi.org/10.5194/egusphere-egu25-16880, 2025.

EGU25-17781 | ECS | Orals | GI4.3

Using the ESA eVe reference lidar system for the cal/val of lidar instruments onboard ESA satellite missions 

Peristera Paschou, Eleni Marinou, Kallopi Artemis Voudouri, Nikolaos Siomos, Antonis Gkikas, Jonas von Bismarck, Thorsten Fehr, and Vassilis Amiridis

The eVe lidar is ESA’s ground reference lidar system for the calibration and validation (cal/val) of ESA satellite missions. eVe is a combined linear/circular polarization lidar with Raman capabilities operating at 355 nm and deriving the profiles of the optical properties of aerosols and thin clouds, namely the particle backscatter and extinction coefficients, the lidar ratio, and the linear and circular depolarization ratios. The system is implemented in a dual-laser/dual-telescope configuration and it can be rotated to perform lidar measurements using different pointing geometries. As such, eVe can simultaneously reproduce the operation of any lidar system that uses linearly (e.g traditional polarization lidars; ATLID onboard EarthCARE mission) or circularly (e.g. ALADIN lidar onboard Aeolus mission) polarized emission.

The eVe lidar has been deployed in ASKOS, the ground-based component of the Joint Aeolus Tropical Atlantic Campaign in Cabo Verde (2021 and 2022), for performing targeted circular polarization lidar measurements for the validation of the Aeolus aerosol products (i.e. the Aeolus L2A products). The eVe-Aeolus comparisons reveal that the Aeolus co-polar backscatter coefficient is the most accurate L2A product followed by the noisier particle extinction coefficient with the larger discrepancies for the Aeolus profiles to be observed in lower altitudes where the aerosol load is larger. The Aeolus co-polar lidar ratio is the noisiest L2A product with the largest discrepancies from the corresponding eVe profiles. Currently the eVe lidar is under upgrade with main components of enabling the profiling of water vapor mixing ratio and extending the retrieval of the extinction coefficient towards daytime conditions, aiming to further enhance its measuring capabilities as well as to meet the requirements for the cal/val of the ATLID lidar products onboard EarthCARE mission which is currently in orbit. After the upgrade, eVe lidar will perform targeted measurements during the nearest EarthCARE overpasses from eVe’s location for the evaluation of the ATLID L2A products.

Acknowledgements:

This research is financially supported by the PANGEA4CalVal project (Grant Agreement 101079201) funded by the European Union and the “Best practice protocol for validation of Aerosol, Cloud, and Precipitation Profiles” ESA project (ACPV; Contract no. 4000140645/23/I-NS). The ASKOS campaign was funded by an ESA project (Contract no. 4000131861/20/NL/IA) and the acquired dataset can be accessed via https://evdc.esa.int/publications/askos-campaign-dataset/. The eVe lidar upgrade and the deployment for the cal/val of EarthCARE products are funded by an ESA project (Contract no. 4000146416/24/NL/FFi).

How to cite: Paschou, P., Marinou, E., Voudouri, K. A., Siomos, N., Gkikas, A., von Bismarck, J., Fehr, T., and Amiridis, V.: Using the ESA eVe reference lidar system for the cal/val of lidar instruments onboard ESA satellite missions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17781, https://doi.org/10.5194/egusphere-egu25-17781, 2025.

EGU25-18284 | ECS | Orals | GI4.3

Assessment of horizontally-oriented ice crystals with a combination of multiangle polarization lidar and cloud Doppler radar 

Zhaolong Wu, Patric Seifert, Yun He, Holger Baars, Haoran Li, Cristofer Jimenez, Chengcai Li, and Albert Ansmann

The orientation of ice crystals plays a significant role in determining their radiative and precipitating effects, horizontally oriented ice crystals (HOICs) reflect up to ~40 % more short-wave radiation back to space than randomly oriented ice crystals (ROICs). This study for the first time introduces an automatic pixel-by-pixel algorithm for HOIC identification using a combination of ground-based zenith- and 15-degree off-zenith-pointing polarization lidars. The lidar observations provided high-resolution cloud phase information. The data were collected in Beijing over 354 days in 2022. A case study from 13 October 2022 is presented to demonstrate the effectiveness and feasibility of the detection method. The synergy of lidars and collocated Ka-band cloud radar, radiosonde, and ERA5 data provide phenomenological insights into HOIC events. While cloud radar Doppler velocity data allowed the estimation of ice crystal size, Reynolds numbers, and turbulent eddy dissipation rates, corresponding environmental and radar-detected variables are also provided. HOICs were present accompanying with weak horizontal wind of 0–20 ms−1 and relatively high temperature between −8 °C to −22 °C. Compared to the ROICs, HOICs exhibited larger reflectivity, spectral width, turbulent eddy dissipation rate, and a median Doppler velocity of about 0.8 ms−1. Ice crystal diameter (1029 µm to 1756 µm for 5th and 95th percentiles) and Reynolds numbers (28 to 88 for 5th and 95th percentiles) are also estimated with the help of cloud radar Doppler velocity using an aerodynamic model. One interesting finding is that the previously found switch-off region of the specular reflection in the region of cloud base shows a higher turbulence eddy dissipation rate, probably caused by the latent heat released due to the sublimation of ice crystals in cloud-base region. The newly derived properties of HOICs have the potential to aid to derive the likelihood of their occurrence in output from general circulation models (GCMs) of the atmosphere.

How to cite: Wu, Z., Seifert, P., He, Y., Baars, H., Li, H., Jimenez, C., Li, C., and Ansmann, A.: Assessment of horizontally-oriented ice crystals with a combination of multiangle polarization lidar and cloud Doppler radar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18284, https://doi.org/10.5194/egusphere-egu25-18284, 2025.

EGU25-18566 | Posters on site | GI4.3

Enhancing lidar aerosol typing schemes: a lidar/photometer synergy 

Nikolaos Papagiannopoulos, Michail Mytilinaios, Aldo Amodeo, Giuseppe D'Amico, Pilar Gumà-Claramunt, Christina Anna Papanikolaou, and Lucia Mona

In this study we present a synergistic approach between lidar and photometer to separate volcanic ash and desert dust and, ultimately, to enhance lidar-based aerosol typing schemes. Typically, the lidar depolarization ratio measurements can be used to distinguish dust and ash with ash depolarization ratio reaching higher values. However, the variability of aerosol depolarization ratio makes it difficult to use it in automatic typing techniques. The imaginary part of refractive index when using in situ data shows stronger absorption than mineral dust; therefore, here, we make use of microphysical AERONET data to define the two aerosol classes (i.e., ash/dust). Then, trivariate Mahalanobis distance is estimated based on the real and imaginary parts of the refractive index and the single scattering albedo for any given AERONET measurement and the type is assigned. This information is then passed on in lidar aerosol typing algorithms and the aerosol type is allocated in the vertical dimension. The methodology is applied to the Potenza ACTRIS site in Italy during an intense desert dust event where an AERONET photometer and an ACTRIS lidar are collocated.

How to cite: Papagiannopoulos, N., Mytilinaios, M., Amodeo, A., D'Amico, G., Gumà-Claramunt, P., Papanikolaou, C. A., and Mona, L.: Enhancing lidar aerosol typing schemes: a lidar/photometer synergy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18566, https://doi.org/10.5194/egusphere-egu25-18566, 2025.

EGU25-19403 | Orals | GI4.3 | Highlight

Forecasting Climate Adaptation Through Cirrus Cloud Radiative Forcing Analysis Using 20 Years of MPLNET Lidar Measurements 

Simone Lolli, Andreu Salcedo-Bosch, Jasper R. Lewis, Erica K. Dolinar, James R. Campbell, and Ellsworth J. Welton

Cirrus clouds play a critical role in Earth's radiation budget and are key to understanding and forecasting climate adaptation in response to global warming. Leveraging 20 years of high-resolution lidar data from NASA's MPLNET network, we analyze and forecast cirrus cloud radiative forcing with the aim of projecting how the climate system will adapt to changing atmospheric conditions. Using ensemble learning methods, we simulate the monthly radiative impacts of cirrus clouds, emphasizing their variability and feedback mechanisms. The study also integrates future climate scenarios under shared socio-economic pathways ( CMIP6SSP2-4.5 and SSP5-8.5) to explore potential shifts in regional climate patterns driven by cirrus cloud interactions. Results highlight how increased temperatures and altered precipitation regimes may influence the climate's adaptive processes, particularly in regions currently sensitive to radiative forcing fluctuations. This research underscores the importance of long-term lidar data for advancing climate adaptation modeling and identifying critical atmospheric feedbacks.

[1] Lolli, S., 2023. Machine Learning Techniques for Vertical Lidar-Based Detection, Characterization, and Classification of Aerosols and Clouds: A Comprehensive Survey. Remote Sensing15(17), p.4318.

How to cite: Lolli, S., Salcedo-Bosch, A., Lewis, J. R., Dolinar, E. K., Campbell, J. R., and Welton, E. J.: Forecasting Climate Adaptation Through Cirrus Cloud Radiative Forcing Analysis Using 20 Years of MPLNET Lidar Measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19403, https://doi.org/10.5194/egusphere-egu25-19403, 2025.

EGU25-19850 | Orals | GI4.3

Estimating Planetary Boundary Layer Height Using CALIPSO Lidar Data: A Machine Learning Approach 

Francesc Rocadenbosch, Andreu Salcedo-Bosch, and Simone Lolli

The planetary boundary layer height (PBLH) is a critical atmospheric parameter influencing air quality, pollutant dispersion, and weather forecasting. Traditional methods for PBLH retrieval rely on radiosondes and ground-based sensors, but their spatial and temporal coverage is limited. In this study, we present a novel application of Random Forest (RF) machine learning to estimate PBLH using lidar measurements from the CALIPSO satellite's Level 1 data spanning a decade. Our RF model is trained with an extensive dataset of radiosonde-derived PBLH values coinciding with CALIPSO overpasses. This approach leverages CALIOP's lidar backscatter profiles to achieve robust performance (R² = 0.6, RMSE = 333.59 m) across a range of atmospheric conditions, including cloudy and dust-laden scenarios, without requiring atmospheric typing or ancillary data. The results surpass state-of-the-art methods in global applicability and accuracy, offering improved spatial and temporal resolution of PBLH estimates. We also discuss the model's performance variations between day- and nighttime scenarios and highlight challenges, such as data bias and surface reflection contamination, which inform future model refinements. This study underscores the potential of integrating machine learning and lidar remote sensing for advancing atmospheric science [1-2].

 

REFERENCES

[1] S. Lolli, W. Y. Khor, M. M. Z. Matjafri, and H. S. Lim, "Monsoon season quantitative assessment of biomass burning clear-sky aerosol radiative effect at surface by ground-based lidar observations in Pulau Pinang, Malaysia in 2014," Remote Sensing, vol. 11, no. 22, 2019.

[2] C. Sivaraman, S. McFarlane, E. Chapman, M. Jensen, Toto, S. Liu, and M. Fischer, Planetary Boundary Layer Height (PBL) Value Added Product (VAP): Radiosonde Retrievals, Tech. Rep., DOE Office of Science Atmospheric Radiation Measurement (ARM) Program, United States, Aug. 2013.

ACKNOWLEDGEMENTS
This research is part of the project PID2021-126436OB-C21 funded by Ministerio de Ciencia e Investigación (MCIN)/Agencia Estatal de Investigación (AEI)/ 10.13039/501100011033 y FEDER “Una manera de hacer Europa” and part of the PRIN 2022 PNRR, Project P20224AT3W funded by Ministero dell’Universit`a e della Ricerca. The European Commission collaborated under projects H2020 ATMO-ACCESS (GA-101008004) and H2020 ACTRIS-IMP (GA-871115).

How to cite: Rocadenbosch, F., Salcedo-Bosch, A., and Lolli, S.: Estimating Planetary Boundary Layer Height Using CALIPSO Lidar Data: A Machine Learning Approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19850, https://doi.org/10.5194/egusphere-egu25-19850, 2025.

EGU25-20478 | ECS | Orals | GI4.3

Proof-of-Concept of a Short-Range High Spectral Resolution Lidar using a Compact High Repetition Rate Fiber Laser 

Manuela Hoyos Restrepo, Romain Ceolato, and Yoshitaka Jin

In recent years, several climate and air quality applications have required to understand the impact of aerosols close to their source, leading to the development of novel Short-Range Elastic Backscatter Lidars (SR-EBLs), which enable measuring the radiative properties of aerosols at high spatiotemporal resolutions (<10cm, 1s) in the short-range (3 to 500m). However, the elastic lidar equation is an ill-posed problem, having one equation for two atmospheric variables: the backscatter β(r) and extinction α(r) coefficients. Solving this equation requires assuming a value for the lidar ratio, i.e., a linear relationship between β and α, reducing the accuracy of the retrievals. Advanced lidar techniques, like the High Spectral Resolution Lidar (HSRL), measure molecular and particle scattering separately. Having a direct measurement of the molecular component allows for solving the lidar problem without assumptions about the lidar ratio. However, the existing atmospheric HSRLs cannot perform short-range measurements because i) they are usually blind in the first hundredths of meters (overlap restrictions), and ii) they prioritize spectral performance using ultranarrow band (and thus long-pulse) lasers, resulting in an insufficient spatiotemporal resolution.

This work presents a proof-of-concept of a Short-Range High Spectral Resolution Lidar (SR-HSRL) optimized for aerosol characterization in the first kilometer of the atmosphere. This SR-HSRL uses a compact high-repetition rate fiber laser source with a 300 MHz linewidth and 5 ns pulse length. Since these two parameters are inversely proportional, and both are required for performing SR-HSRL measurements, a compromise had to be found to optimize the overall performance. The main challenge was to prove that, despite its relatively large linewidth, this laser has a satisfactory spectral performance so that it can be used for future implementations of the short-range HSRL. We chose this model after evaluating several laser sources because it has the right compromise between pulse length, linewidth, spectral stability, and size. The laser housing is 270 x 270 x 40 mm and weighs 2.9 kg, making it ideal for future integration on a portable short-range HSRL system.

In the receiver part, a 10:90 beam splitter transmits 10% of the backscattered light to the total channel and reflects 90% of it to the HSR channel. A 40-cm-long iodine cell is used as the spectral filter for separating the Mie and Rayleigh aerosol components. We used two thermoelectrically cooled SiPM Multi-Pixel Photon Counter (MPPC) sensors and a 160MHz analog-to-digital converter to measure the signals. The spatiotemporal resolution, limited by the acquisition system, is 7.5 m and 1 s.

To test the lidar, a two-day measurement campaign was performed at NIES in Tsukuba, Japan, in July 2024. We demonstrate that, despite having a relatively large laser linewidth, we can successfully remove the Mie aerosol component, retrieving aerosol backscatter coefficient profiles from as low as 80 m. We also compare the HSRL retrieval method to a non-conventional forward Fernald inversion method previously reported for SR-EBL. We found that the forward method normally sub-estimates β (up to 30% discrepancy) in aerosol layers and overestimates it in cloud zones (60 to >100% difference).

How to cite: Hoyos Restrepo, M., Ceolato, R., and Jin, Y.: Proof-of-Concept of a Short-Range High Spectral Resolution Lidar using a Compact High Repetition Rate Fiber Laser, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20478, https://doi.org/10.5194/egusphere-egu25-20478, 2025.

EGU25-21151 | Orals | GI4.3

Simulation and assessment of spaceborne hybrid Doppler wind lidar 

Songhua Wu, Guangyao Dai, Wenrui Long, Kangwen Sun, Xiaochun Zhai, Na Xu, and Xiuqing Hu

Accurately measuring wind field is crucial for studying the dynamical structure and evolutionary characteristics of the atmosphere, as well as heat-momentum-matter exchange and balance. According to the World Meteorological Organization (WMO), global observation of the 3D wind field is the primary factor for improving the accuracy of numerical weather prediction. Due to the absence of aeronautical data, meteorological observation and forecasting capabilities are notably deficient in sparsely populated areas, the southern hemisphere, the polar regions, and the vast oceans. Spaceborne Doppler wind lidar has become an important instrument for observing the vertical profile of the global wind field, with the successful operation of Aeolus. The third generation of FengYun polar-orbiting meteorological satellites are initially designed to develop a dual-system Doppler wind measurement lidar technology programme that integrates direct and coherent detection lidar, making full use of the observational advantages of the two methods to detect the global wind field with high resolution. Incoherent detection is used in the middle and upper troposphere and lower stratosphere, where molecules scatter strongly. Coherent detection is used for the observation of the middle and lower troposphere and boundary layer. This research analyses the key parameters of the spaceborne hybrid wind lidar for future satellite missions. The incoherent detection module operates at 355 nm and uses the dual-edge detection technique based on Fabry?Pérot etalon. And the coherent detection module uses heterodyne detection technique operating at 1064 nm. This paper presents a simulation model for wind measurement lidar that realizes gridded atmospheric parameters, scanning observation, and forward-inversion simulation. And a method for detecting horizontal wind field based on dual-beam observation was developed to ensure the response of the lidar for wind speed detection in both meridional wind component and zonal wind component.

How to cite: Wu, S., Dai, G., Long, W., Sun, K., Zhai, X., Xu, N., and Hu, X.: Simulation and assessment of spaceborne hybrid Doppler wind lidar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21151, https://doi.org/10.5194/egusphere-egu25-21151, 2025.

EGU25-21533 | Posters on site | GI4.3

Cloud Condensation Nuclei (CCN) and Ice Nucleating Particles (INP) conversion factors based on Thessaloniki AERONET station 

Eleni Giannakaki, Karageorgopoulou Archontoula, Georgoulias Aristeidis, and Koutounidis Ioannis

Several studies [1,2] have shown the potential of polarization lidar to provide vertical profiles of aerosol parameters from which cloud condensation nuclei (CCN) and ice-nucleating particles (INP) number concentrations can be retrieved. The results are based on reliable of conversion factors between aerosol optical thickness and column-integrated particle size distribution based on Aerosol Robotic Network (AERONET) photometer observations. A crucial point regarding the efficacy of aerosol particles to act as CCN or INP depends on aerosol type.

AERONET Inversion Data (Level 1.5) for Thessaloniki station were analyzed over the period 2006-2021. Following ‎[1,2], the Ångström exponent was used to separate the particles into pollution (AE > 1.6) and dust (AE < 0.5) dominated cases. To obtain a better classification of aerosols we utilize aerosol typing from CALIPSO. Only cases which are classified as either purely dust or polluted continental aerosols within 100km from Thessaloniki are selected. The Aerosol Optical Depth (AOD) at 440 nm and the Ångström exponent (AE) 440-870 were used to calculate the AOD at 532 nm, while the AOD at 1020 nm and the AE between 870-1020 nm were used to estimate the AOD at 1064 nm. The particle volume size distribution is derived for 22 discrete radius points, spaced logarithmically at equidistant intervals. The particle number concentration (n) for each radius interval is calculated by dividing the volume concentration by the particle volume and multiplying by the spectral integral width of 0.2716. The column value of n60 is the sum of number concentrations for radius classes 2 to 22 (>57 nm), while n100 is the sum for radius classes 4 to 22 (>98 nm). The INP-relevant column n250 is the sum of intervals 8–22 plus the mean of intervals 7 and 8, while n290 the sum of 8-22. To obtain particle extinction coefficient σ (or sigma) and n60, the AOD at 532 nm and the column n60 are divided by 1000 m. For urban particles, n60 (reservoir of CCN) and n250 (reservoir of INP) were used, while n100 (CCN) and n250 (INP) were used for dust particles. Following CALIPSO aerosol typing dust conversion factors was found equal to c100= 24.3±7.0 Mm cm-3, xd=0.78 ± 0.13 and c250= 0.30±0.03 Mm cm-3, while for polluted continental particles, were c60= 31.4 ± 9.0 Mm cm-3, xc= 0.94 ± 0.12 and c290= 0.089±0.002 Mm cm-3.

 

References:

[1] Mamouri, R.E. and Ansmann, A. Potential of polarization lidar to provide profiles of CCN- and INP-relevant aerosol parameters. Atmos. Chem. Phys. 2016, 16, 5905–5931. doi:10.5194/acp-16-5905-2016

[2] Georgoulias, A.; Marinou, E.; Tsekeri, A.; Proestakis, E.; Akritidis, D.; Alexandri, G.; Zanis, P.; Balis, D.; Marenco, F.; Tesche, M. and Amiridis, V. A First Case Study of CCN Concentrations from Spaceborne Lidar Observations. Remote Sens. 2020, 12, 1557. doi:10.3390/rs12101557

 

Acknowledgments: The research work was supported by the Hellenic Foundation for Research and Innovation (H.F.R.I.) under the “Basic Research Financing (Horizontal support for all Sciences), National Recovery and Resilience Plan (Greece 2.0)” (Project Number: 015144).

How to cite: Giannakaki, E., Archontoula, K., Aristeidis, G., and Ioannis, K.: Cloud Condensation Nuclei (CCN) and Ice Nucleating Particles (INP) conversion factors based on Thessaloniki AERONET station, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21533, https://doi.org/10.5194/egusphere-egu25-21533, 2025.

EGU25-21736 | Orals | GI4.3

Simultaneous observations of meteoric Ca and Ca+ by employing the Ti:sapphire-laser-based resonance-scattering Ca/Ca+ lidar 

Masayuki Katsuragawa, Mitsumu K. Ejiri, Ayaka Hashimoto, Sota Kobayashi, Sayako Miyoshi, Hikaru Miyagi, Chiaki Ohae, and Takuji Nakamura3

The upper atmosphere located at an altitude of 80 - 120 km above the ground is a crucial region for comprehensively understanding the behavior of Earth's entire atmosphere, because it is the region where the atmosphere transitions from neutral to ionospheric. In this transitional region, meteoroids are continually supplying metallic atoms and ions. The resonant-scattering lidar, which emits laser beams from the ground and then detect on the ground again how much atoms and ions cause resonant scattering of the laser radiations, is one of the significant measurement methods of observing such transitional region. While Fe and Na are selected as the major targets, we have focused on Ca and have developed a specific lidar system to detect it. This is because Ca has uniquely preferable resonance transitions for neutral atoms and ions (Ca: 422.7918 nm and Ca+: 393.4770 nm) for performing lidar measurements from the ground. The core of the developed resonant-scattering Ca/Ca+ lidar system is the injection-locked Ti:sapphire solid-state laser, which has the remarkable ability to simultaneously emit the two laser beams from a single resonator at a variety of combinations of two wavelengths, including the above resonant transitions of neutral Ca and Ca+.
    Here, we report on the first results of the long-term observations, where the developed resonant-scattering Ca/Ca+ lidar system was operated for an entire night. The averaged laser power, time resolution, and altitude resolution of the Ca/Ca+ lidar system are set to 0.2 W, 30 s, and 15 m, respectively, for Ca, and 0.4 W, 30 s, and 30 m , respectively, for Ca+ in this operation. Both neutral Ca and Ca ions distributed in the identical spatio-temporal regions could be measured in detail over an entire night. It was clearly observed that the neutral Ca and Ca ions had almost the same spatio-temporal structures with complex time and space dependences in the main layer at an altitude of 80 - 100 km, and Ca ions also had an additional high-density thin layer with a few kilometers deep at the highest altitude in the main layer. This high-density layer of Ca ions, which was not seen with the neutral Ca, suggests that it is to be related to the sporadic E layer. In our presentation, we will also report on the progress of this ongoing project.

How to cite: Katsuragawa, M., Ejiri, M. K., Hashimoto, A., Kobayashi, S., Miyoshi, S., Miyagi, H., Ohae, C., and Nakamura3, T.: Simultaneous observations of meteoric Ca and Ca+ by employing the Ti:sapphire-laser-based resonance-scattering Ca/Ca+ lidar, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21736, https://doi.org/10.5194/egusphere-egu25-21736, 2025.

EGU25-6148 | Posters on site | GI4.5

HALO airborne measurements; PERCUSION’s contribution to EarthCARE validation 

Silke Gross, Florian Ewald, Martin Wirth, André Ehrlich, Lutz Hirsch, Konstantin Krüger, Anna Luebke, Bernhard Mayer, Sophie Rosenburg, Lea Volkmer, Manfred Wendisch, Julia Windmiller, and Bjorn Stevens

In May 2024 the EarthCARE satellite mission EarthCARE was launched. For the first time, the satellite combines a high spectral resolution lidar and a cloud radar with doppler capability as key instruments on one single platform. In addition, it is equipped with a multi spectral imager and a broadband radiometer. This unique combination makes EarthCARE the most complex satellite mission to study aerosol, clouds, precipitation, and radiation. To fully use these new and advanced data for science applications, a careful validation of the measurements and data products is required. We have implemented an EarthCARE-like payload onboard the German research aircraft HALO (High Altitude and LOng range) to prepare and validate the EarthCARE data. This instrumentation was flown during PERCUSION (Persistent EarthCARE underflight studies of the ITCZ and organized convection) as a contribution to ORCESTRA (Organized Convection and EarthCARE Studies over the Tropical Atlantic).

ORCESTRA is a network of different campaigns conducted to better understand the organized tropical convection at the mesoscale, e.g. including the interaction of convective organization with tropical waves and air-sea interaction, and the impact of convective organization on the Earth’s climate and radiation budget. In addition, ORCESTRA helps to validate satellite remote sensing (especially EarthCARE). To achieve these objectives, ORCESTRA combines several sub-campaigns taking place on the Cape Verde Islands and Barbados in August and September 2024.

One of the campaigns within ORCESTRA is the PERCUSION campaign. PERCUSION aims to test factors hypothesized to influence the organization of deep maritime convection in the tropics and the influence of convective organization on its larger-scale environment. One focus of PERCUSION was to establish confidence in the EarthCARE measurements and products. For this purpose, we conducted one EarthCARE underpass within each research flight HALO measurements were performed during the EarthCARE commissioning phase in August 2024 out of Sal, Cape Verde, and out of Barbados in September 2024. In addition, we performed flights out of Oberpfaffenhofen, Germany in November 2024 for validation of conditions that could not be captured in the two first campaign parts. Altogether, 33 EarthCARE underpasses were carried out in different aerosol and cloud situations. Some of the flights were coordinated with in-situ measurements onboard other aircrafts (e.g. the French ATR42), with shipborne measurements onboard the German research vessel METEOR, or with ground-based radar and lidar measurements at Mindelo (Cape Verde), Barbados, and the ACTRIS stations Antikythera, Leipzig, Lindenberg and Munich. Four underpasses under NASA’s PACE mission were also performed.

In our presentation we will give an overview of ORCESTRA with the main focus on PERCUSION. We will present the HALO PERCUSION measurements and will show first comparisons of HALO lidar and radar and EarthCARE lidar and radar measurements.

How to cite: Gross, S., Ewald, F., Wirth, M., Ehrlich, A., Hirsch, L., Krüger, K., Luebke, A., Mayer, B., Rosenburg, S., Volkmer, L., Wendisch, M., Windmiller, J., and Stevens, B.: HALO airborne measurements; PERCUSION’s contribution to EarthCARE validation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6148, https://doi.org/10.5194/egusphere-egu25-6148, 2025.

EGU25-7050 | Orals | GI4.5

Spectroradiometric and Stray light characterization of the Pushbroom Imager for Cloud and Aerosol Research and Development (PICARD) Airborne Imager 

Alok Shrestha, Tom Ellis, Roseanne Domingues, Gary Hoffmann, Haiping Su, James Jacobson, Kerry Meyer, Julia Barsi, and Steven Platnick

The PICARD (Pushbroom Imager for Cloud and Aerosol Research and Development) instrument, developed by the NASA Ames Research Center in partnership with Brandywine Photonics, LLC, is an airborne imager consisting of dual Offner spectrometers and an all-reflective telescope with a 50° full field-of-view (FOV). The instrument operates over a wavelength range of 400 – 2400 nm in more than 200 bands. PICARD has already flown multiple engineering flights on NASA ER-2 high altitude aircraft, the most recent during 2023 Western Diversity Time Series (WDTS) spring campaign where near co-incident measurements with spaceborne sensors such as MODIS and VIIRS were obtained including those over railroad valley (RRV) calibration site.  In addition, PICARD has recently flown during the 2024 Plankton, Aerosol, Cloud, Ocean Ecosystem Postlaunch Airborne eXperiment (PACE-PAX) field campaign to gather data for the validation of the recently launched PACE mission. A recent analysis comparing PICARD measurements with RadCalNet dataset from RRV revealed excellent agreement for most of the bands except in the UV and blue region, where PICARD generally under reported. To better characterize these bands and improve this under reporting, detailed PICARD spectroradiometric characterization measurements were collected at Goddard Laser for Absolute Measurement of Radiance (GLAMR) laboratory at Goddard Space Flight Center (GSFC) in February 2024. The initial analysis of this characterization suggested that this under-report during flight is due to a stray light sensitivity inherent in the low signal-to-noise (SNR) bands of array spectroradiometers. Correcting for the GLAMR measured stray light reconciles the under report. In addition, poor SNR bands in SWIR atmospheric absorptions are recovered when corrected for stray light. In this presentation, we will share findings from our recent PICARD spectroradiometric characterization over GLAMR including updated results comparing PICARD flight radiances with RadCalNet at RRV.

How to cite: Shrestha, A., Ellis, T., Domingues, R., Hoffmann, G., Su, H., Jacobson, J., Meyer, K., Barsi, J., and Platnick, S.: Spectroradiometric and Stray light characterization of the Pushbroom Imager for Cloud and Aerosol Research and Development (PICARD) Airborne Imager, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7050, https://doi.org/10.5194/egusphere-egu25-7050, 2025.

EGU25-7774 | Posters on site | GI4.5

In-Situ Hyperspectral Absorption and Backscattering Sensors for Ocean Color and Biogeochemistry Research 

Kirby Simon, Wayne Slade, Christopher Strait, Alberto Tonizzo, Michael Twardowski, Thomas Leeuw, Chuck Pottsmith, Ravi Chandrasiri, and Ole Mikkelsen

Accurate measurements of in-water inherent optical properties (IOPs) such as absorption and backscattering, along with coincident in-situ and satellite-measured radiometry, are key to refining and calibrating algorithms used by hyperspectral satellite missions such as NASA PACE to derive ocean color data products. The accuracy of hyperspectral ocean color products, such as phytoplankton community composition, is therefore linked to the accuracy of in-situ IOP measurements. However, current instrumentation for in-situ absorption and backscattering measurements has been limited to either single- or multi-spectral wavelengths or to hyperspectral wavelengths that do not entirely meet the wavelength range and resolution requirements of PACE and other hyperspectral remote sensing missions. Advancements in instrumentation are therefore necessary to expand the range, resolution, and sensitivity of in-situ absorption and backscattering measurements to support these missions and the development and distribution of accurate ocean color data products. Additionally, advancements in hyperspectral absorption and backscattering sensors can offer new insights into studying particulate and dissolved materials in the ocean in support of biogeochemistry research.

We have recently developed and commercialized submersible hyperspectral absorption (Hyper-a) and backscattering (Hyper-bb) instruments to meet the needs of current (e.g., PACE) and future (e.g., GLIMR, SBG) hyperspectral remote sensing missions. The Hyper-bb is a single-angle backscatter sensor that utilizes a broadband LED source, scanning linear variable filter assembly, and sensitive photomultiplier tube detector. The Hyper-a is an absorption sensor that utilizes a xenon flash lamp, dual spectrometers (signal and reference), and a pump-through Lambertian integrating cavity that reduces measurement uncertainty due to scattering errors characteristic in a reflective tube design. Both sensors are designed to enable user calibration, reducing cost and downtime typically associated with sending the instrument back for factory calibration.

We will present details related to the development of these two hyperspectral instruments as well as their engineering specifications and recent test results from laboratory studies and field work.

How to cite: Simon, K., Slade, W., Strait, C., Tonizzo, A., Twardowski, M., Leeuw, T., Pottsmith, C., Chandrasiri, R., and Mikkelsen, O.: In-Situ Hyperspectral Absorption and Backscattering Sensors for Ocean Color and Biogeochemistry Research, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7774, https://doi.org/10.5194/egusphere-egu25-7774, 2025.

EGU25-7777 | Orals | GI4.5

Simultaneous aerosol and ocean retrievals from PACE multi-angle polarimeters: data products and validation 

Meng Gao, Kirk Knobelspiesse, Bryan Franz, Peng-wang Zhai, Kamal Aryal, Andrew Sayer, Amir Ibrahim, and Jeremy Werdell

The NASA Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) mission, successfully launched on February 8, 2024, with aims to advance our understanding of global ocean ecology, biogeochemistry, atmospheric aerosols, and clouds. PACE features cutting-edge instruments, including the Ocean Color Instrument (OCI), a hyperspectral scanning radiometer, and two Multi-Angle Polarimeters (MAPs): the UMBC Hyper-Angular Rainbow Polarimeter (HARP2) and the SRON Spectro-Polarimeter for Planetary EXploration one (SPEXone). These instruments offer valuable data for simultaneous retrievals of aerosol, cloud, and surface properties.

This talk will focus on simultaneous aerosol and ocean retrievals derived from PACE MAP measurements, emphasizing data products, uncertainties, and validation. The retrieved products encompass aerosol properties such as complex refractive index, effective radius and variance, layer height, optical depth, and single-scattering albedo, as well as oceanic and surface properties. To streamline operational processing, we have incorporated deep neural network-based radiative transfer models into the PACE polarimetric retrieval algorithms via the FastMAPOL framework. Preliminary validation against in-situ measurements will be presented, along with potential applications of MAP data, including the study of ocean color bidirectional reflectance signals and multi-angle cloud masking.

How to cite: Gao, M., Knobelspiesse, K., Franz, B., Zhai, P., Aryal, K., Sayer, A., Ibrahim, A., and Werdell, J.: Simultaneous aerosol and ocean retrievals from PACE multi-angle polarimeters: data products and validation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7777, https://doi.org/10.5194/egusphere-egu25-7777, 2025.

EGU25-7979 | Posters on site | GI4.5

Heat-island-effect of ship-based bulk measurements for evaporation duct estimation 

Xiaofeng Zhao, Yuxing Wang, Pinglv Yang, Yibin Chen, and chunshan Wei

Because the evaporation duct profile is difficult to measure, different empirical surface layer models have been developed to compute the average refractivity profile near the ocean surface using four bulk measurements: pressure, temperature, humidity, wind speed at a single height (e.g., the ship’s bridge), and sea surface temperature (SST). Although these parameters can be conveniently measured using standard equipment, the measurement accuracy is usually influenced by inherent factors, such as the movement of the ship or the heat island effect. To analyze the heat island effect of ship-based bulk measurements for evaporation duct estimation, an open cruise observation over the Tropical Eastern Indian Ocean from 23 Aug 2024 to 14 Oct 2024 is used. The ship weather station measurements and the corresponding evaporation duct profiles, computed by the NPS evaporation duct model, are compared with 48 low-altitude rocketsonde profiles, which sample a high vertical resolution of air temperature, air humidity, air pressure, and wind parameters. The sensors for air temperature, humidity, pressure, and wind vector are deployed at 13.4 m above the mean sea level, and the SST is measured by an infrared thermometer. The results show that the mean air temperature and relative humidity of the ship measurements are 1.03 K and 4.07% higher than the rocketsonde measurements at the same altitude (i.e., 13.4 m), and the evaporation duct height and strength computed from the ship-based measurements are 1.98 m and 10.07 M-units lower than those from the rocketsonde measurements.

How to cite: Zhao, X., Wang, Y., Yang, P., Chen, Y., and Wei, C.: Heat-island-effect of ship-based bulk measurements for evaporation duct estimation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7979, https://doi.org/10.5194/egusphere-egu25-7979, 2025.

EGU25-8293 | Posters on site | GI4.5

Radiometric Calibration using Artificial Intelligence: Constituting Uniform Observing Systems for Infrared Satellites 

Boyang Chen, Aiqun Wu, Wen Hui, Peng Rao, Xuang Feng, Fansheng Chen, Changpei Han, Qichao Ying, Yapeng Wu, Miao Liu, Damian Moss, and Zhenxing Qian
Radiometric Calibration (RC) is a critical process in aerospace infrared remote sensing that establishes the relationship between the radiation energy of observed objects and the Digital Number (DN) output from sensors, which is fundamental for ensuring high-precision applications of infrared remote sensing data. At present, Source-Based RC (SBRC) is the predominant method, relying on a variety of Radiometric Sources (RS) including in-orbit blackbodies, or natural targets such as lakes, oceans. This approach, while effective, imposes constraints on remote sensing systems such as space & weight allocation for RS and additional observation time for RC. Moreover, the reliance on physical calibration sources can introduce uncertainties due to factors such as imperfect emissivity of in-orbit blackbodies, lack of data consistency due to varied RS types, and variations in environmental conditions. In this paper, we propose a novel RC method named Artificial Intelligence Radiometric Calibration (AIRC), which directly generates RC coefficients for the in-orbit remote sensing satellites using the physical and environmental parameters of the sensor. We first theoretically prove that RC coefficients can be derived as functions of the sensor states. Next, we propose our Neural Networks for infrared Radiometric Calibration (RCNN), to learn this relationship based on historical high-accuracy calibration data, enabling a shift from Reference Traceability (RT) to States Traceability (ST). Then, to verify the feasibility of the proposed scheme, we train and test an Multi-layered Perceptron (MLP) as a simple implementation of RCNN based on our long-term well-curated RC data from our FengYun-4A Avanced Geosynchronous Radiation Imager (FY-4A AGRI), and the experiments show that the proposed method achieves high-accuracy RC comparable with the official RC method applied on FY-4A AGRI that uses an in-orbit blackbody. Our study showcases how to conduct RC using the “reason (the states of sensor) - results (calibration coefficient)” logic, as supplement to the existing “result (observation to RS) - reason (calibration coefficient)” logic, which promotes constituting a uniform observing system for cross-platform infrared satellites.

How to cite: Chen, B., Wu, A., Hui, W., Rao, P., Feng, X., Chen, F., Han, C., Ying, Q., Wu, Y., Liu, M., Moss, D., and Qian, Z.: Radiometric Calibration using Artificial Intelligence: Constituting Uniform Observing Systems for Infrared Satellites, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8293, https://doi.org/10.5194/egusphere-egu25-8293, 2025.

EGU25-8313 | Posters on site | GI4.5

Advanced cloud products from NASA’s PACE mission 

Bastiaan van Diedenhoven, Chamara Rajapakshe, Andrzej Wasilewski, Andrew Sayer, Brian Cairns, Otto Hasekamp, Kirk Knobelspiesse, Mikhail Alexandrov, Daniel Miller, Kenneth Sinclair, Brent McBride, and Vanderlei Martins

The sensitivities of cloud properties to changes in the climate and to anthropogenic aerosol emissions are crucial for understanding Earth’s climate but remain highly uncertain. Global cloud observations from satellites are needed to advance our knowledge on processes related to the formation and evolution of clouds and precipitation. While long term satellite data records of cloud microphysical properties exist, largely obtained by multi-spectral imagers, they are known to be substantially biased or failing in particular situations, such as in regions of broken and/or mixed-phase clouds. The cloud products provided by NASA’s Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) mission, which was launched on 8 February 2024, have several advantages over past missions. PACE caries the Ocean Color Instrument (OCI), which is a multi-spectral imager, the Hyper-angular Rainbow Polarimeter (HARP-2) and the Spectropolarimeter for Planetary Exploration (SPEXone). Advanced, pixel-level cloud microphysical products are produced from the polarimeters, including cloud top phase and full droplet size distributions, while collocated retrievals are provided by OCI using more traditional methods. Instrument-synergy products include liquid water path and droplet number concentrations. We present first global advanced cloud products from PACE. We present validation using airborne campaigns that indicates that the polarimetry products are much less affected by the presence of broken and mixed-phase clouds than OCI observations, consistent with previous studies using simulations and observations. These observations provide new insights on the microphysical properties of global clouds, including their drop size distribution width and bi-modality which may be linked to precipitation formation. Furthermore, we show that the polarimeter retrievals along with OCI’s unique combination of three commonly-used shortwave infrared wavelength bands allows to assess some of the biases in traditional bi-spectral retrievals in unprecedented detail and on a global scale. We show that the biases in bi-spectral results depend on cloud structure and on the wavelength used for the droplet size retrievals. The PACE data provides crucial information to reduce biases in traditional bi-spectral cloud retrievals by essentially all multi-spectral imagers in the program of record that result from, e.g., sub-pixel cloudiness, mixed-phase cases and 3D radiative transfer effects. We make recommendations on how biases in bi-spectral results may be mitigated.

How to cite: van Diedenhoven, B., Rajapakshe, C., Wasilewski, A., Sayer, A., Cairns, B., Hasekamp, O., Knobelspiesse, K., Alexandrov, M., Miller, D., Sinclair, K., McBride, B., and Martins, V.: Advanced cloud products from NASA’s PACE mission, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8313, https://doi.org/10.5194/egusphere-egu25-8313, 2025.

EGU25-9811 | Orals | GI4.5

ACROSS Mediterranean activities for EarthCARE validation and exploitation 

Eleni Marinou and the ACROSS team

The ESA-JAXA EarthCARE satellite mission, launched in May 2024, delivers vertical profiles of aerosols, clouds, and precipitation properties together with radiative fluxes, utilizing an instrumental suite of a high spectral resolution lidar (ATLID), a Doppler cloud radar (CPR), a multi-spectral imager (MSI), and a broadband radiometer (BBR). The simultaneous measurements will be utilized to improve our understanding of aerosol-cloud interactions (ACI) and their radiative effects and to assess the representation of clouds, precipitation, aerosols, radiative fluxes, and heating rates in weather and climate models [1]. Due to the multi-sensor complexity/diversity and the innovation of its standalone and synergistic products, the EarthCARE mission has several validation challenges and strong sub-orbital synergies are needed to address Cal/Val and science objectives.

The Mediterranean basin provides a complex aerosol-cloud environment for the exploitation EarthCARE's capabilities. For the validation of the EarthCARE products in the Mediterranean, the ACROSS validation activity will be implemented, which would increase synergies towards achieving the following objectives: (i) validate EarthCARE aerosol and cloud products using state-of-the-art ground-based and airborne facilities, (ii) implement science studies targeting radiative closures, ACI, and data assimilation experiments, (iii) and provide information for harmonizing and bridging past and future missions, to deliver Climate Data Records on aerosols and clouds.

The rationale for ACROSS is based on lessons learned from the JATAC campaign in the Atlantic [2]. Following the JATAC example, we target to implement 3 Intensive Observational Periods, including large-scale field experiments in the Mediterranean. The suborbital component follows the ASKOS [3] example. It includes (i) ACTRΙS Aerosol and Cloud remote sensing facilities and high-precision radiation measurements (Potenza site in Italy, Limassol Cyprus, as well as Pyrgos, Thessaloniki, and PANGEA sites in Greece), (ii) radiation measurements for closure studies, (iii) UAV and aircraft in-situ flights collocated with the remote sensing measurements. ACROSS activities will be clustered with the ARCHIMEDES experimental activities in the Mediterranean, foreseen between late 2026 and late 2027. ACROSS seeks synergies with airborne activities. To this end, the first synergistic measurements were collected during the PERCUSION campaign in November 2024, during which HALO underpass two EarthCARE tracks close to the Thessaloniki and PANGEA sites. More airborne activities are envisioned in the Mediterranean area for Spring/September 2025/2026.

ACROSS is a collaborative effort between NOA, DLR, the University of Nova Gorica, CyI, INOE, FMI, CNR-IMAA, PMOD, ERATOSTHENES CoE, CUT, and TROPOS. ACROSS is supported by ACTRIS RI and the dataset collected will support assimilation experiments and science activities in the framework of the PANGEA4CalVal, ATMO-ACCESS, and CERTAINTY EC projects and collaborations within.

References:

[1] Wehr T. et al., https://doi.org/10.5194/amt-16-3581-2023, 2023.

[2] Fehr, T., et al., https://doi.org/10.5194/egusphere-egu23-7249, 2023. 

[3] Marinou, E. Et al., https://doi.org/10.3390/environsciproc2023026200, 2023.

Acknowledgments: This research was financially supported by the PANGEA4CalVal project (Grant Agreement 101079201) funded by the European Union, and the CERTAINTY project (Grant Agreement 101137680) funded by the Horizon Europe program. Part of the wok was financed through the Core Program within the Romanian National Research Development and Innovation Plan 2022-2027, carried out with the support of MCID, project no. PN 23 05.

How to cite: Marinou, E. and the ACROSS team: ACROSS Mediterranean activities for EarthCARE validation and exploitation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9811, https://doi.org/10.5194/egusphere-egu25-9811, 2025.

EGU25-11760 | ECS | Orals | GI4.5

Aerosol Validation in NASA's PACE mission: Deployment of the SPEX Airborne Polarimeter in the PACE-PAX Field campaign 

Brecht Simon, Jasper Mens, Martijn Smit, Guangliang Fu, Jeroen Rietjens, Martin Grim, Tim Vonsée, Jelle Talsma, Rob Wolfs, Otto Hasekamp, and Bastiaan van Diedenhoven

The Plankton, Aerosol, Cloud, Ocean Ecosystem Postlaunch Airborne eXperiment (PACE-PAX) is a multi-platform, multi-instrument field campaign designed to validate NASA’s PACE mission. Two research aircraft participated in this month-long campaign: the CIRPAS Twin Otter, conducting in situ observations of aerosols and clouds, and NASA’s high-altitude research aircraft ER-2, equipped with remote sensing instruments. Among these instruments is SPEX airborne, an airborne proxy for the Dutch SPEXone instrument onboard PACE. SPEX airborne, like SPEXone, is a multi-angle spectropolarimeter for wavelengths between 400 and 780 nm, designed to characterize aerosols in the Earth’s atmosphere. It has nine viewing angles (nadir, ±14°, ±28°, ±42°, and ±56°) and an across-track swath of about 2.1 km at nadir at nominal ER-2 flight altitudes. SPEX airborne radiance and polarization data are formatted identically to SPEXone data, enabling the use of the same RemoTAP algorithm to retrieve aerosol properties such as aerosol optical depth, size distributions, refractive index, layer height, and composition. During multiple flights, totaling over 80 flight hours, the ER-2 frequently flew under PACE and ESA’s EarthCARE satellite, as well as over the Twin Otter, calibration sites, and aerosol ground stations, facilitating extensive data comparisons. In this presentation, we present preliminary validation of publicly released SPEX airborne level-1 data and collocate these with SPEXone observations. Additionally, we present validation of SPEX airborne aerosol retrievals against AERONET stations and other instruments deployed during PACE-PAX. The RemoTAP aerosol retrievals from SPEX airborne data emphasize the key role of PACE-PAX in confirming aerosol properties derived from SPEXone.

How to cite: Simon, B., Mens, J., Smit, M., Fu, G., Rietjens, J., Grim, M., Vonsée, T., Talsma, J., Wolfs, R., Hasekamp, O., and van Diedenhoven, B.: Aerosol Validation in NASA's PACE mission: Deployment of the SPEX Airborne Polarimeter in the PACE-PAX Field campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11760, https://doi.org/10.5194/egusphere-egu25-11760, 2025.

EGU25-12925 | ECS | Posters on site | GI4.5

From PACE to PLACE: Results from the First Months of Land Data Products 

Skye Caplan, Antonio Mannino, Morgaine McKibben, Fred Huemmrich, Kirk Knobelspiesse, Jeremy Werdell, Meng Gao, Otto Hasekamp, and Guangliang Fu

Although “land” is not included the acronym for NASA’s Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) satellite, the mission is actively supporting terrestrial science. Two new global, daily product suites were recently released using land data from PACE’s Ocean Color Instrument (OCI). The first, termed SFREFL, is a hyperspectral collection of surface reflectances from the ultraviolet into the shortwave infrared. SFREFL currently employs L2gen for atmospheric correction, ensuring continuity with heritage missions processed by the Ocean Biology Processing Group. ISOFIT is also being considered for use as a standard surface reflectance algorithm. Both algorithms make PACE terrestrial data directly applicable to future hyperspectral missions like SBG, and ease collaboration with current missions producing similar products. The second suite, LANDVI, includes 10 vegetation indices: 6 multispectral (NDVI, EVI, NDWI, NDII, CCI, and NDSI) and 4 which are hyperspectral-enabled, or narrowband (PRI, Car, CIRE, and mARI). Narrowband indices leverage OCI’s unique capabilities to provide previously uncharacterized insights into the status of terrestrial ecosystems across the globe. Having been in production for several months, preliminary results from both SFREFL and LANDVI will be presented here. The integration of these terrestrial products as outputs from PACE positions the mission as pivotal for global environmental monitoring and establishes it as an important part of the terrestrial hyperspectral data record.

How to cite: Caplan, S., Mannino, A., McKibben, M., Huemmrich, F., Knobelspiesse, K., Werdell, J., Gao, M., Hasekamp, O., and Fu, G.: From PACE to PLACE: Results from the First Months of Land Data Products, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12925, https://doi.org/10.5194/egusphere-egu25-12925, 2025.

EGU25-12978 | Orals | GI4.5

NASA’s PACE Mission Status Updates: Advancing Science and Data Products 

Amir Ibrahim, Jeremy Werdell, Ivona Cetinic, Bryan Franz, Brian Cairns, Susanne Craig, Otto Hasekamp, Antonio Mannino, Vanderlei Martin, Gerhard Meister, and Andrew Sayer

Following its launch from Kennedy Space Center in February 2024, NASA’s Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) mission has been revolutionizing our understanding of Earth’s systems. The observatory hosts three cutting-edge instruments: the Ocean Color Instrument (OCI), a hyperspectral radiometer, and two multi-angular polarimeters, SpexOne and HARP2. Together, these instruments are collecting unprecedented data on our living oceans, atmospheric aerosols and clouds, and land.

PACE extends NASA’s legacy of over 20 years of global satellite observation while initiating an advanced suite of climate-relevant data records. For the first time, daily global measurements are enabling improved predictions of fisheries dynamics, the emergence of harmful algal blooms, and other critical factors impacting commercial and recreational industries. Furthermore, PACE provides key insights into cloud properties and aerosols—tiny airborne particles that influence air quality and regulate Earth's energy balance by absorbing and reflecting sunlight.

Since its launch, the PACE science team, in collaboration with the broader scientific community, has focused on implementing, testing, and validating mission data products. Performance assessments through the PACE Validation Science Team (PVST) and field campaigns, such as the Post-launch Airborne eXperiment (PACE-PAX), have been pivotal in refining data quality and enhancing the mission’s scientific outcomes.

This presentation provides an overview of the current status of PACE science products, highlighting key achievements, ongoing validation efforts, and future goals aimed at maximizing the mission’s contributions to Earth science.

How to cite: Ibrahim, A., Werdell, J., Cetinic, I., Franz, B., Cairns, B., Craig, S., Hasekamp, O., Mannino, A., Martin, V., Meister, G., and Sayer, A.: NASA’s PACE Mission Status Updates: Advancing Science and Data Products, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12978, https://doi.org/10.5194/egusphere-egu25-12978, 2025.

EGU25-13069 | Posters on site | GI4.5

PACE Mission validation with the PACE-PAX field campaign 

Ivona Cetinic, Kirk Knobelspiesse, Brian Cairns, and Jeremy Werdell

NASA's Plankton, Aerosol, Clouds, and Ocean Ecosystems (PACE) Mission, launched a year ago, provides data on ocean color, aerosols, clouds, and land surfaces through its three advanced sensors. Some of these data products rely on established "heritage" algorithms, ensuring continuity with previous and ongoing missions, while others are novel, leveraging recent algorithmic advancements and PACE's unique measurement capabilities. To validate PACE's data products, the PACE Postlaunch Airborne eXperiment (PACE-PAX) was conducted in September 2024 in California. This campaign featured coordinated operations involving multiple aircraft, ocean vessels, and surface-based instruments, particularly timed with PACE satellite overpasses. Additionally, PACE-PAX supported similar activities for ESA's EarthCARE (Cloud, Aerosol, and Radiation Explorer) Mission. This presentation highlights the campaign's achievements, discusses the current status of the data, and outlines future plans for utilizing this valuable dataset.

How to cite: Cetinic, I., Knobelspiesse, K., Cairns, B., and Werdell, J.: PACE Mission validation with the PACE-PAX field campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13069, https://doi.org/10.5194/egusphere-egu25-13069, 2025.

EGU25-13336 | ECS | Posters on site | GI4.5

PACE Applications Program: Putting PACE remote sensing data to work for societal benefit across the Earth System  

S. Morgaine McKibben and Skye Caplan

Launched in February 2024 and serving data to the public as of April 2024, the NASA Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) satellite provides a novel set of hyperspectral and polarimetric Earth observation (EO) capabilities across aquatic, terrestrial, and atmospheric domains-- an interdisciplinary span not matched by other EO missions. With these observations, PACE data can support multiple applications areas such as water resource management, public health and air quality, climate science, terrestrial and agricultural, post-disaster monitoring, and more. The PACE Applications Program has the primary goal of fostering and accelerating the translation of PACE’s advanced data into actionable applications that benefit society. To achieve this, we support bridging of researchers and applied end users through programming such as the PACE Community of Practice, Early Adopters Program, and information-sharing and co-production activities such as workshops and focus sessions. In this presentation we describe the interdisciplinary applications capabilities of PACE and opportunities for you to engage with our program.

How to cite: McKibben, S. M. and Caplan, S.: PACE Applications Program: Putting PACE remote sensing data to work for societal benefit across the Earth System , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13336, https://doi.org/10.5194/egusphere-egu25-13336, 2025.

EGU25-14131 | Orals | GI4.5

First comparison between EarthCARE’s CPR and airborne W-band cloud radar observations during ECALOT campaign 

Paloma Borque, Cuong Nguyen, Zhipeng Qu, Pavlos Kollias, Bernat Puigdomenech, Keyvan Ranjbar, Kenny Bala, Natalia Bliankinshtein, Leonid Nichman, Sudesh Boodoo, and Norman Donaldson

Improving future climate predictions requires enhancing the current meteorological numerical models for which a better understanding of the roles that clouds and aerosols (and their interactions) play in Earth’s weather and climate is crucial.  Along these lines, the European Space Agency (ESA) and the Japan Aerospace Exploration Agency (JAXA) successfully launched the Earth Cloud, Aerosol, and Radiation Explorer (EarthCARE) satellite in May 2024. This satellite mission aims to advance the studies of global aerosol and cloud properties via novel active and passive spaceborne observations.  EarthCARE carries four instruments: the ATmospheric LIDar (ATLID), the Cloud Profiling Radar (CPR), the Multi-Spectral Imager (MSI), and the Broadband Radiometer (BBR).  Of particular interest to this work are the CPR observations providing significant observations of clouds’ vertical structure, including the first ever in-cloud Doppler Velocity profiles from space.

As part of ESA’s global calibration/validation initiative, the EarthCARE Commissioning Calibration/Validation Campaign in Ottawa (ECALOT) took place in Canada from October 2024 to January 2025.  ECALOT collected essential airborne and surface observations to calibrate and validate key EarthCARE products. These include CPR and ATLID Level 1 and Level 2 products, composite and synergy products, as well as EarthCARE’s scene construction algorithm and radiation products.  ECALOT successfully observed fall and winter weather conditions with dedicated flights targeted to sample relevant weather underflying the EarthCARE path.  The National Research Council Canada’s (NRC) Convair-580 aircraft, equipped with W- and X- band radars (NAWX), 355nm Lidars, and a full array of state-of-the-art in-situ cloud microphysics and aerosol probes, provided critical independent observations to support EarthCARE validation efforts.  These observations were complemented by surface-based sites deployed by Environment and Climate Change Canada and McGill University near Ottawa airport and two Climate Sentinels network stations operated by McGill University and Université du Québec à Montréal in the Montreal region.

In this presentation, we will provide an initial evaluation of EarthCARE’s CPR performance during the ECALOT campaign.  A comprehensive analysis of the cloud vertical structure as seen by the CPR and NAWX observations and an intercomparison of vertical cross sections of reflectivity and Doppler velocity will be presented.  In addition, an assessment of the behavior of CPR under stratiform and convective conditions will be provided.

How to cite: Borque, P., Nguyen, C., Qu, Z., Kollias, P., Puigdomenech, B., Ranjbar, K., Bala, K., Bliankinshtein, N., Nichman, L., Boodoo, S., and Donaldson, N.: First comparison between EarthCARE’s CPR and airborne W-band cloud radar observations during ECALOT campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14131, https://doi.org/10.5194/egusphere-egu25-14131, 2025.

EGU25-14414 | Posters on site | GI4.5

PACE Observatory validation plan, data sources, and results  

Inia M Soto Ramos, James Allen, Ivona Cetinić, Amir Ibrahim, Christopher W. Proctor, Kirk D. Knobelspiesse, and Jeremy Werdell

The success of Earth Science space-borne missions relies on the availability of optical field measurements, as well as a solid validation plan to assess and verify the in-orbit quality of the data products. Since the late 1990s, NASA’s SeaBASS has served the ocean color community as the primary repository for in situ radiometric and pigment observations, facilitating robust product validation across multiple missions. The PACE science data validation program is responsible for making sure data products meet mission-specified requirements and for assessing uncertainties across various water types, cloud conditions, and aerosol distributions. In addition to SeaBASS, the PACE validation plan includes 24 PACE Validation Science Teams and a targeted field campaign called PACE-PAX. Nonetheless, an ongoing challenge remains the limited number of matchups between in situ and satellite measurements due to cloud cover, data quality issues, and other constraints. Here, we discuss the limitations and challenges of ocean color validation and present the current PACE validation plan, data sources, and early validation results. 

How to cite: Soto Ramos, I. M., Allen, J., Cetinić, I., Ibrahim, A., Proctor, C. W., Knobelspiesse, K. D., and Werdell, J.: PACE Observatory validation plan, data sources, and results , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14414, https://doi.org/10.5194/egusphere-egu25-14414, 2025.

EGU25-14437 | ECS | Posters on site | GI4.5

The First Year of the Hyper-Angular Rainbow Polarimeter (HARP2) on the NASA PACE mission: Performance, Science, and Synergy 

Brent McBride, J. Vanderlei Martins, Xiaoguang Xu, Anin Puthukkudy, Roberto Fernandez-Borda, Noah Sienkiewicz, Rachel Smith, Meng Gao, Bastiaan van Diedenhoven, Snorre Stamnes, Kirk Knobelspiesse, Andrew Sayer, Chamara Rajapakshe, Bryan Franz, Frederick Patt, Carissa Arillo, Brian Cairns, Jeremy Werdell, and Lorraine Remer

Over the past year, the Hyper-Angular Rainbow Polarimeter (HARP2) multi-angle imaging polarimeter instrument on the NASA Plankton Aerosol Cloud ocean Ecosystem (PACE) mission observed the entire Earth every two days. HARP2 measures total and polarized radiances over four spectral channels (440/550/670/870 nm), at up to 90 distinct viewing directions, and over a 114° field-of-view (1550 km cross-track swath). This large volume of daily information requires new approaches to on-orbit operations, data processing, calibration, and science. In this work, we celebrate and recap the first year of HARP2 on PACE – from pre-launch to on-orbit calibration (solar/lunar/vicarious), exciting new and synergistic science products for cloud, aerosol, and ocean properties, and co-located intercomparisons with OCI, SPEXone, and AirHARP2 underflights during the recent NASA PACE-PAX field campaign. We close with a look ahead to HARP2 as a pathfinder for upcoming polarimetry missions.

How to cite: McBride, B., Martins, J. V., Xu, X., Puthukkudy, A., Fernandez-Borda, R., Sienkiewicz, N., Smith, R., Gao, M., van Diedenhoven, B., Stamnes, S., Knobelspiesse, K., Sayer, A., Rajapakshe, C., Franz, B., Patt, F., Arillo, C., Cairns, B., Werdell, J., and Remer, L.: The First Year of the Hyper-Angular Rainbow Polarimeter (HARP2) on the NASA PACE mission: Performance, Science, and Synergy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14437, https://doi.org/10.5194/egusphere-egu25-14437, 2025.

EGU25-15557 | Posters on site | GI4.5

Validation of Aerosol Products from Polarimetric Sensors – Application to PARASOL and 3MI 

Bertrand Fougnie, Soheila Jafariserajehlou, and David Huerta Valcarce

With the launch of EPS-SG in 2025, a new era for a long-term operational Near-Real-Time provision of aerosol product is starting. If most of the potential for such a new remote sensing polarimetry has been demonstrated since 1996 with the 3 POLDER and PARASOL missions, the recent advance in term of retrieval but also analysis and exploitation of the data reveal more and more the potential. Indeed, polarimeters allow the observation of aerosols with a significantly improved information content which will feed the retrieval. On top of the aerosol optical thickness classically retrieved, an additional set of parameters characterizing the aerosol properties can now be derived. This specificity of polarimeters requires a more demanding effort in term of validation. We will overview the different aspects to be considered for the validation, describe the methodology for most of the parameters, and focus on some examples.   

How to cite: Fougnie, B., Jafariserajehlou, S., and Huerta Valcarce, D.: Validation of Aerosol Products from Polarimetric Sensors – Application to PARASOL and 3MI, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15557, https://doi.org/10.5194/egusphere-egu25-15557, 2025.

EGU25-20586 | ECS | Orals | GI4.5

Liquid Water Cloud Retrievals from HARP2 and AirHARP2 Measurements from the PACE-PAX Validation Campaign 

Rachel Smith, Xiaoguang Xu, Brent McBride, and Vanderlei Martins

The Hyper Angular Rainbow Polarimeter 2 (HARP2), developed at UMBC, is a state-of-the-art wide field-of-view polarimeter capable of measuring total and polarized radiances with fine angular resolution (≥2 degrees) and high polarization accuracy in four spectral channels (440, 550, 670, 870 nm). HARP2 was successfully launched in February 2024 aboard NASA’s Plankton Aerosol Cloud and ocean Ecosystem (PACE) satellite and has since been collecting critical science data on Earth’s atmospheric, oceanic, and surface properties. In September 2024, UMBC’s AirHARP2, an advanced airborne polarimeter closely resembling the orbital HARP2, participated in the PACE Postlaunch Airborne eXperiment (PAX). This campaign provides a unique opportunity to validate radiometric and polarimetric measurements and derived science products from the PACE satellite by conducting direct cross-platform comparisons using co-located scenes. This study focuses on the retrieval comparisons of liquid water cloud microphysical properties from HARP2 and AirHARP2 during PACE-PAX using a novel look-up-table retrieval algorithm that leverages the geometric features of the polarized cloudbow to infer the cloud droplet size distribution. The retrievals will be performed using a novel look-up-table retrieval algorithm that uses the geometric parameters of the polarized cloudbow to retrieve the cloud droplet size distribution. With AirHARP2’s Level-1C grid resolution (~120 m) approximately 42 times finer than HARP2’s (~5 km), we will also examine the impact of spatial resolution on retrieval performance. The results will be further validated by cross-comparisons with official cloud products from the Ocean Color Instrument, the primary instrument aboard PACE.

How to cite: Smith, R., Xu, X., McBride, B., and Martins, V.: Liquid Water Cloud Retrievals from HARP2 and AirHARP2 Measurements from the PACE-PAX Validation Campaign, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20586, https://doi.org/10.5194/egusphere-egu25-20586, 2025.

EGU25-20694 | Posters on site | GI4.5

System Vicarious Calibration of the PACE Ocean Color Instrument 

Robert Frouin, Jing Tan, Andrew Barnard, Alexander Bailess, Emmanuel Boss, Nils Haëntjens, Andrew Banks, Paul Chamberlain, and Matthew Mazloff

System vicarious calibration (SVC) of satellite ocean-color sensors involves comparing retrievals of water-leaving radiance (Lw) with in-situ measurements at the time of overpass and adjusting the calibration coefficients to ensure agreement between retrieved and measured quantities. This approach is designed to reduce uncertainties associated with purely radiometric calibration techniques, which lack the accuracy required for science applications, and to minimize biases introduced by atmospheric correction. For the recently launched PACE Ocean Color Instrument (OCI), the methodology utilizes hyperspectral Lw measurements from HyperNav radiometer systems deployed at various locations (Crete, Moorea, Puerto Rico, Hawaii) and from the Marine Optical Buoy (MOBY) near Lanai. Match-ups are rigorously selected based on criteria for atmospheric, surface, water, and geometry conditions. Top-of-atmosphere (TOA) radiance derived from onboard calibration techniques is compared to TOA radiance calculated from in-situ Lw measurements, resulting in calibration adjustment gains. The application of these adjusted gains to OCI imagery in diverse oceanic regions demonstrates more realistic values for water reflectance, enhancing the accuracy of retrieved ocean color data for scientific analyses.

How to cite: Frouin, R., Tan, J., Barnard, A., Bailess, A., Boss, E., Haëntjens, N., Banks, A., Chamberlain, P., and Mazloff, M.: System Vicarious Calibration of the PACE Ocean Color Instrument, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20694, https://doi.org/10.5194/egusphere-egu25-20694, 2025.

Long-term, global ocean-color observations are needed for biogeochemistry and climate applications and require integration across multiple satellite sensors. This study proposes a methodology for cross-calibrating polar-orbiting ocean-color sensors using a geostationary reference sensor. The geostationary sensor serves as an intermediary, offering numerous coincidences in time and geometry with polar-orbiting sensors, particularly over oceanic regions where radiance levels are typical for ocean-color remote sensing. The methodology is applied to cross-calibrate current ocean-color sensors, including the recently launched OCI, using AHI, a sensor expected to remain stable over short cross-calibration intervals. Accuracy is evaluated based on radiometric noise, acquisition time differences, solar and viewing geometry variations, and spectral band mismatch uncertainties. Cross-calibration coefficients derived from suitable imagery provide a foundation for consistent, normalized calibration of polar-orbiting sensors, enabling the generation of reliable long-term ocean-color products from multiple satellites.

How to cite: Tan, J. and Frouin, R.: Cross-Calibration of Polar-Orbiting Satellite Ocean-Color Sensors Using a Geostationary Reference Sensor, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20712, https://doi.org/10.5194/egusphere-egu25-20712, 2025.

The Global Navigation Satellite System radio occultation (GNSS-RO) technique has been demonstrated to significantly enhance our understanding of the free atmosphere, with particular emphasis on the Upper Troposphere and Lower Stratosphere. We present improved estimations of global three-dimensional wind fields derived from low-pass filtered monthly mean geopotential height data. Geostrophic, gradient, and equatorial balance winds were estimated to provide foundational wind estimates, consistent with methodologies employed in previous studies. To advance beyond the traditional reliance on geostrophic and gradient wind, higher-order terms in the horizontal momentum equations, specifically advection and curvature, were considered. Newly derived wind fields were systematically evaluated against original winds from the European Center for Medium-Range Weather Forecast (ECMWF) Reanalysis 5 (ERA5), using a best-estimate algorithm. Building upon this methodology, the application of the best-estimate algorithm revealed that geostrophic winds incorporating advection were most applicable in the troposphere, while gradient winds with advection showed superior estimates in the stratosphere. Thus, the tropopause acts as a physical boundary delineating the domains of applicability for geostrophic and gradient-based wind approximations. Compared to their fundamental formulations, advection significantly improved both geostrophic and gradient wind estimates relative to the original ERA5 winds. In tropical regions, equatorial balance winds considering curvature provided the most accurate estimates across the entire vertical extent. Our findings emphasize the significant potential of GNSS-RO geopotential height data to move beyond the limitations of traditional geostrophic and gradient wind approximations. The results pave the way for creating a comprehensive global three-dimensional wind field climatology by leveraging the unique advantages of GNSS-RO, such as long-term consistency, high vertical resolution, and global coverage. This dataset will be a valuable resource for the scientific community, supporting climate monitoring and enhancing the understanding of atmospheric dynamics, particularly in the stratosphere, where data assimilation in reanalyses remains limited.

How to cite: Unegg, J.: Beyond Geostrophic and Gradient Wind: Enhancing Radio Occultation Wind Field Estimation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-869, https://doi.org/10.5194/egusphere-egu25-869, 2025.

EGU25-926 | ECS | Orals | G5.1

3-D water vapor field retrieval by GNSS tomography for InSAR observation correctionapplied to deformations of Piton de la Fournaise in Réunion Island 

Hugo Gerville, Joël Van Baelen, Laurent Morel, Fabien Albino, Frédéric Durand, Aline Peltier, and Patrice Boissier

On one hand, current processing of GNSS signals has the ability to provide the amount of
water vapor between the satellite and the ground. This information is of major interest
because these observations have good temporal resolution and are insensitive to weather
conditions. Furthermore, when the station network is dense enough, it is possible to retrieve
the 3-D water vapor field through GNSS tomography.
Although this method has already proven effective, this presentation will first detail new
approaches development to adapt to the Reunion Island context and particularly over the
Piton de la Fournaise. Indeed, this area has a dense distribution of stations while the rest of
the island shows a weaker distribution. Hence, a classic grid mesh is therefore not suited for
this situation and we developed a Voronoï adaptive mesh scheme to better account for the
irregular network geometry. Likewise, the inversion scheme used is being upgraded to a
Single Value Decomposition (SVD) approach shown to be more effective in the literature.
On the other hand, InSAR technique consists of measuring ground deformation by difference
between two radar measurements of satellite/ground distance. However, these two
measurements are not carried out at the same time and, thus, the water vapor field which
impact such observations is different for each measurement, notably in tropical regions
where water vapor variability is very important.
Hence, a second aspect of our work will be to apply the improved 3-D water vapor retrieval
obtained with the new approaches defined above in order to propose a better correction
scheme for InSAR retrieval of slow ground deformation signals at Piton de la Fournaise, a
precursor sign of possible volcanic activity.

How to cite: Gerville, H., Van Baelen, J., Morel, L., Albino, F., Durand, F., Peltier, A., and Boissier, P.: 3-D water vapor field retrieval by GNSS tomography for InSAR observation correctionapplied to deformations of Piton de la Fournaise in Réunion Island, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-926, https://doi.org/10.5194/egusphere-egu25-926, 2025.

EGU25-965 | ECS | Posters on site | G5.1

Assessment of GNSS-based PWV against radiosonde observation and reanalysis datasets in Antarctica 

Bilal Mutlu and Serdar Erol

Global warming phenomena lead to melting glaciers, rising sea levels, droughts, and irregular seasonal patterns, especially in polar regions. Besides, water vapor plays a significant role in these processes, contributing to about 60% of the natural greenhouse effect. Increasing temperature raises the atmosphere's capacity for water vapor, creating a positive feedback loop that aggravates global warming and extreme weather events. In polar regions, global warming is causing increased annual rainfall. Despite low overall precipitation, this phenomenon accelerates the melting of snow and ice, impacting local ecosystems. Future projections indicate that precipitation along Antarctica's coastline is expected to increase over the next 80 years. This increase may enhance surface melting through various processes. Consequently, monitoring atmospheric water vapor is crucial for understanding global climate dynamics and weather patterns. However, due to the harsh conditions in the polar regions, there is a shortage of conventional measurements, which makes global atmospheric reanalysis models crucial. The specific humidity and air pressure from the reanalysis models can be used to calculate Precipitable Water Vapor (PWV) (measured in meters), which is one of the most commonly used parameters for measuring atmospheric water vapor. Nevertheless, biases and discrepancies in the models may influence the data, particularly in polar regions where observations are scarce. In addition, the estimation of meteorological parameters can be acquired not only based on meteorological station data but also with the help of geodetic satellite data. Global Navigation Satellite Systems (GNSS) signals are subject to tropospheric refraction as they pass through the Earth's atmosphere, and the resulting zenith delays are divided into two components: hydrostatic (ZHD) and wet delay (ZWD). Moreover, the ZWD can be utilized to compute the PWV by multiplying a conversion factor. PWV can also be obtained by using air temperature and dew point temperature data from radiosonde observations at specific pressure levels. In this study, it is aimed to investigate and compare PWV values produced from GNSS-based, radiosonde-based, and global meteorological reanalysis models. Within the scope of the study, International GNSS Service (IGS) stations, which are located in the Antarctica continent, were used to calculate GNSS-based PWV. Besides, the radiosonde dataset retrieved from the Integrated Global Radiosonde Archive version 2.2 (IGRA 2.2) was used to obtain radiosonde-based PWV. As reanalysis datasets, the most recent reanalysis from the European Centre for Medium-Range Weather Forecasts (ECMWF), and the National Aeronautics and Space Administration (NASA) were used. The fifth-generation reanalysis product from the ECMWF called ERA-5 and the second-generation version of NASA’s Modern-Era Retrospective analysis for Research and Applications called MERRA-2 data were used to obtain reanalysis based PWV. As a result of the study, root mean square errors (RMSE) and correlation values of GNSS-based PWV compared to radiosonde-based and reanalysis-based PWV were investigated for each IGS station. Besides, it was evaluated whether the GNSS technique could be used as an alternative to other methods in studies related to the troposphere and meteorology in the Antarctic continent.

How to cite: Mutlu, B. and Erol, S.: Assessment of GNSS-based PWV against radiosonde observation and reanalysis datasets in Antarctica, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-965, https://doi.org/10.5194/egusphere-egu25-965, 2025.

A three-dimensional water vapor density field has advantages in monitoring atmospheric water vapor, especially for reflecting the vertical motion. The existing multi-source tomography models are around a fusion of single-source remote-sensing signal and Global Navigation Satellite System (GNSS) data. However, different remote-sensing data have advantages and disadvantages regarding spatiotemporal resolution and accuracy. When only single-source remote-sensing data is integrated for tomography, the model's available scenarios are severely limited by weather conditions. Therefore, we construct a tomography model by fusing multi-band spaceborne remote-sensing data and high-precision ground GNSS data, the former includes near-infrared MODIS image, long-wave infrared FengYun-4A image, and morphed integrated microwave image MIMIC. The equations system of the tomographic model is solved based on different strategies of weight determination using the weighted least square algorithm. In addition, to consider the dynamic variations of tropopause height in the research area, the tropopause detection products of Fengyun-4B with high spatial coverage are used to determine the boundary of the tomographic region, and the constraints of model is built by historical GNSS occultation observations. To verify our method, the proposed model is validated by water vapor density from reanalysis and radiosonde data, respectively. The results show that the reasonable prior weights are essential when using multi-source data to perform tightly coupled tomography, the RMSEs of water vapor density are less than 2 g/m3 in most epochs. Compared to the tomographic model based on only GNSS data, the accuracy improvement of the tomographic model fusing multi-band remote sensing data is higher than that of any tomographic model using single-source remote-sensing data. Also, the proposed tomography model can better compensate for the shortcomings of poor time continuity of integrated individual remote-sensing data to expand the application scenarios of the fusion tomographic model.

Acknowledgments: This work was supported by Natural Science Foundation of China (42192534 and 42388102).

How to cite: Xu, T. and Li, S.: Atmospheric Water Vapor Tomography based on GNSS and Multi-band Remote Sensing Measurements Combination, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2480, https://doi.org/10.5194/egusphere-egu25-2480, 2025.

EGU25-5428 | ECS | Orals | G5.1

Extraction and Application of Subcarrier Phase Measurements in GNSS-R Altimetry 

Yunqiao He, Fan Gao, Xinyue Meng, and Tianhe Xu

Subcarrier modulated signals, such as BDS-3 B2 and Galileo E5, are widely used to improve the spectral compatibility and ranging accuracy of Global Navigation Satellite Systems (GNSS). However, designing signal processing and observation extraction techniques for subcarrier modulated signals is still challenging for the navigation community. In GNSS-R application, GNSS-R phase altimetry is proposed to provide sea surface height information as an economical and accurate technology to solve the resolution problem. However, phase unwrapping and phase integer ambiguity pose significant challenges for the application of GNSS-R phase altimetry. To overcome these obstacles, the utilization of subcarrier modulated signals is noticed for the first time, presenting a novel opportunity for GNSS-R phase altimetry due to the substantial subcarrier wavelength of 19.5 meters. In the work, we developed a subcarrier modulated signal processing strategy that can track both the upper and lower band signals. By combining the two signals, we construct virtual signals whose phase matches the subcarrier phase. These virtual signals undergo processing using long-time coherent integration and sliding filtering to enhance the signal-to-noise ratio and minimize errors. Subsequently, subcarrier phase measurements are extracted from these virtual signals. To validate the effectiveness, subcarrier phase measurements are applied to a GNSS-R altimetry station and drone platform. When compared with accurate in-situ SSH results, it is evident that the phase is much easier to unwrap and the phase integer ambiguity is easier to fix. Furthermore, the accuracy can achieve centimeter-level precision.

How to cite: He, Y., Gao, F., Meng, X., and Xu, T.: Extraction and Application of Subcarrier Phase Measurements in GNSS-R Altimetry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5428, https://doi.org/10.5194/egusphere-egu25-5428, 2025.

Chile's diverse climate spans a remarkable range, from the hyper-arid desert in the north to a Mediterranean climate in the center, temperate humid conditions in the south, and polar tundra in Patagonia. This climatic gradient provides a unique opportunity to study the synchronized variability of tropospheric water vapor (TWV) and precipitation processes. In recent years, GNSS has emerged as a powerful satellite-based tool capable of capturing not only tectonic deformation but also meteorological processes. One of the key parameters derived from GNSS processing is Zenith Total Delay (ZTD), which represents the delay in GNSS signal propagation caused by the troposphere. ZTD is composed of the hydrostatic and wet delays, with the wet delay closely linked to TWV, making it an essential metric for studying atmospheric water vapor dynamics. We use GNSS ZTD observations, spanning between 15 and 28 years, to analyze the intra-seasonal and interannual probability density functions (PDFs) of TWV. Additionally, we examine the co-variability between daily average TWV and accumulated precipitation to establish links between TWV peaks and precipitation events.

Our results reveal significant differences in TWP PDFs across Chile, ranging from log-normal to normal and inverse log-normal distributions. Notably, the relationship between TWV and precipitation is stronger in central, southern, and Patagonian regions, suggesting regional variability in underlying atmospheric processes. Potential mechanisms driving these differences, such as climatic controls and local meteorological dynamics, are discussed in detail.

These findings provide a benchmark for evaluating the representativeness of general circulation models (GCMs) by comparing observed and modeled TWV distributions. Furthermore, they lay the groundwork for future research into the TWV-precipitation relationship at daily and sub-daily timescales, critical for improving weather forecasts and understanding hydrological processes.

How to cite: Valenzuela, R. and Jara, J.: GNSS-derived tropospheric water vapor and precipitation co-variability along continental Chile, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7362, https://doi.org/10.5194/egusphere-egu25-7362, 2025.

Tropospheric delay is one of the main sources of error affecting high-precision positioning and navigation and is a key parameter for detecting water vapour in the Global Navigation Satellite System (GNSS).

This delay is typically divided into wet and hydrostatic components. ZTD is described as the sum of the Zenith Hydrostatic Delay (ZHD) and the Zenith Wet Delay (ZWD) and can be combined with surface pressure and temperature to estimate the integrated content of water vapour above GNSS station.

In climate change context, the precipitable water vapour (PW) is key parameter of atmospheric process and dynamics and its variation is very high in space and time. Its accuracy is paramount for any geodetic or climatic study.

In recent years, data from atmospheric reanalysis products such as ERA-Interim, ERA5 (the fifth generation of reanalysis from the European Centre for Medium-Range Weather Forecasts) have been widely used to obtain information on tropospheric delay and water vapour   (Li et al., 2015; Zhou et al., 2020...)

The main objective of this study is to compute precipitable water vapour from ERA5 reanalysis for four stations in Algeria, which have different types of climate. We opt for using integration method for different level of pressure with ERA5.

The values of water vapour are also compared with radiosondes profiles and GNSS data. The results of this work shows good agreement with a correlation that is not less than not 0.95 and 0.70 compared as radiosondes profiles (Namaoui et al., 2022). The first results are encouraging, in particular for meteorological applications with good hope to introduce another dataset as GNSS to more understand the variation and behaviour of water vapour over a long period of observation.

How to cite: Houaria, N.: Evaluation of atmospheric water vapour based on ERA5 Reanalysis Products and GNSS Observations in Algeria., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8874, https://doi.org/10.5194/egusphere-egu25-8874, 2025.

EGU25-8951 | ECS | Posters on site | G5.1

A Ground-based GNSS-R Marine Environment Dynamic Monitoring Station 

Xinyue Meng, Fan Gao, Tianhe Xu, and Nazi Wang

Global navigation satellite system-reflectometry (GNSS-R) is considered a promising technology for monitoring marine environments. However, there is still a lack of GNSS-R stations that provide comprehensive data. For this reason, a stationary marine information dynamic monitoring platform using GNSS-R method was constructed in Weihai City, Shandong Province, China. This station consists of two antennas, an intermediate frequency (IF) data collector, a wind sensor and a laptop computer with GPUs. The up-looking antenna is used for direct signal receiving and the down-looking antenna serves for reflected signals. The wind sensor records wind speed and wind direction simultaneously at 1Hz. The collector can export IF data with 62MHz sampling rate which covers signals including GPS L1/L5, BDS B1I/B1C/B2a and Galileo E1/ E5a. The laptop with self-developed software defined receiver (SDR) is employed for processing large amounts of IF data and outputting sea surface height observations based on dual-antennas method in real-time. In the preliminary study, the results based on code-delay method show that the accuracy of BDS B2a can realize centimeter altimetry after post-processing while the accuracy of GPS L5 is approximately in the decimeter range due to the limited number of satellites within the visible range. Additionally, these observations can be also used to retrieve wind speed. We look forward to more research on GNSS-R in the future, for which we can provide data collected by this GNSS-R station.

How to cite: Meng, X., Gao, F., Xu, T., and Wang, N.: A Ground-based GNSS-R Marine Environment Dynamic Monitoring Station, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8951, https://doi.org/10.5194/egusphere-egu25-8951, 2025.

EGU25-8993 | ECS | Posters on site | G5.1

Stacking machine learning model for vertical interpolation of precipitable water vapor using GNSS networks and radio occultation data 

Jiaqi Shi, Min Li, Wenwen Li, Kefei Zhang, and Andrea Steiner

This study proposes a stacking machine learning (SML) model for the vertical interpolation of precipitable water vapor (PWV), addressing the issue of missing near-surface water vapor information in radio occultation (RO) profiles, where measurements do not reach the surface. The model integrates data from over 1500 ground-based Global Navigation Satellite System (GNSS) stations and more than 300,000 profiles from the Constellation Observing System for Meteorology, Ionosphere, and Climate-2 (COSMIC-2), and is trained and validated in two regions of the Northern Hemisphere. Results show that in the North American region, the SML model reduces the root-mean-square error (RMSE) of PWV estimates by over 33% compared to conventional models. In China and Southeast Asia, the RMSE reduction is about 42%, demonstrating notable improvements over conventional model approaches. External validation with radiosondes shows close agreement between the SML-interpolated RO-PWV and radiosonde-PWV. Additionally, the SML-interpolated RO-PWV exhibits high consistency with PWV estimates from RO profiles of the Meteorological Operational satellites (Metop by ROMSAF), which contain complete (background) near-surface information. The SML model performs reliably across various terrains and climatic conditions. This study also preliminarily explores the model performance for extreme weather conditions, providing insights for future enhancements. The new SML model provides a high-accuracy and effective solution for PWV estimation and contributes to advancements in water vapor monitoring, weather forecasting, and atmospheric science research.

How to cite: Shi, J., Li, M., Li, W., Zhang, K., and Steiner, A.: Stacking machine learning model for vertical interpolation of precipitable water vapor using GNSS networks and radio occultation data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8993, https://doi.org/10.5194/egusphere-egu25-8993, 2025.

EGU25-9979 | Posters on site | G5.1

Consistency and Homogeneity of ZTD Estimates from IGS Repro3 

Hugo Breton, Olivier Bock, and Samuel Nahmani

In 2019-2020, the International GNSS Service (IGS) coordinated its third reanalysis of the complete history of GNSS data collected by the IGS global network since 1994. Ten analysis centers (ACs) participated in this so-called “Repro3” effort, using the latest models and methodologies. Several of them provided, among other products, zenith tropospheric delay (ZTD) estimates.

In this study, we analyze the quality of ZTD estimates from four ACs (COD, GFZ, GRG, and TUG) along three different aspects: 1) the number and size of ZTD outliers, 2) the mean ZTD differences (or biases), and the standard deviation of ZTD differences between ACs as well as with respect to the ERA5 reanalysis, and 3) the homogeneity of the ZTD time series at individual sites. Overall statistics and case studies are presented for 200 sites.

We find an overall agreement between ACs at the sub-millimeter (bias) and sub-centimeter (standard deviation) level. However, a notable number of outliers and inhomogeneities are observed at individual sites. These are attributed to differences in metadata, particularly antenna information, and, to a lesser extent, to differences in processing strategies and software-specific features (e.g., outlier editing). Controlling the quality of metadata and optimizing the processing strategy are two major pathways for improving the quality of GNSS ZTD estimates for use in climate analysis.

This work is part of the activities of a Joint Working Group of the IAG Inter-Commission Committee on “Geodesy for Climate Research” (ICCC), in cooperation with the IGS ACs.

How to cite: Breton, H., Bock, O., and Nahmani, S.: Consistency and Homogeneity of ZTD Estimates from IGS Repro3, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9979, https://doi.org/10.5194/egusphere-egu25-9979, 2025.

EGU25-10034 | ECS | Posters on site | G5.1

Polarimetric GNSS-Reflectometry data over sea ice during the MOSAiC expedition 

Baojian Liu, Ruibo Lei, Wei Wan, Junming Xia, Maximilian Semmling, Jie Zhang, Yue Xu, Yueqiang Sun, Hongjie Xie, and Gunnar Spreen

Global Navigation Satellite System Reflectometry (GNSS-R) has long been explored for retrieving sea ice properties, but in-situ validation in the central Arctic during the freezing season is rare, limiting its application. The primary objective of this study is to advance the current understanding of multi-polarization GNSS-R remote sensing for sea ice. This paper presents observations from the full-polarization GNSS-R(FpolGNSSR) prototype  during the MOSAiC expedition. FpolGNSSR, with four polarization channels and high antenna gain (11.3 dB), aims to assess the impact of sea-ice thickness and permittivity on GNSS-R data, with observations from October 2019 to January 2020, the onset period of ice growth. A four-layer model simulates reflectivity, and the sensitivity of multi-polarization GNSS-R to sea ice is qualitatively analyzed. Subsequently, a simplified model reveals a linear relationship between reflectivity and ice thickness, with regression showing a correlation of 0.74 (P<0.01). The optimal RMSE of sea ice thickness retrieval is 0.13 m for first-year ice in freezing season (0.3–1.0 m thick). 

How to cite: Liu, B., Lei, R., Wan, W., Xia, J., Semmling, M., Zhang, J., Xu, Y., Sun, Y., Xie, H., and Spreen, G.: Polarimetric GNSS-Reflectometry data over sea ice during the MOSAiC expedition, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10034, https://doi.org/10.5194/egusphere-egu25-10034, 2025.

EGU25-10048 | ECS | Orals | G5.1

High-resolution zenith delay and tropospheric gradient fields track precipitation during heavy local-scale rainfall events  

Andreas Kvas, Stephanie Haas, Jürgen Fuchsberger, and Gottfried Kirchengast

Global Navigation Satellite System (GNSS) meteorology has proven to be a useful tool for the study of weather phenomena and climate change. The sensitivity of GNSS signals to the distribution of water vapor and liquid water in the atmosphere has led to numerous applications of tropospheric delay data products, ranging from the evaluation of numerical weather prediction (NWP) models via data assimilation into NWP models, to the observation-driven analysis of rainfall events. In this study, we investigate the behavior of non-hydrostatic zenith delay (ZWD), integrated water vapor (IWV), and tropospheric gradients before, during, and after heavy short-duration local-scale convective precipitation events. The study area located in the WegenerNet 3D Open-Air Laboratory for Climate Change Research Feldbach Region (WEGN3D Open-Air Lab) is situated in the Alpine forelands of southeastern Austria and covers an extent of about 22 km by 16 km. The WEGN3D Open-Air Lab consists of a six-station GNSS network with baselines between 5 km and 10 km, 156 closely spaced meteorological stations, an X-band precipitation radar, and a microwave and broadband infrared radiometer for tropospheric profiling and cloud structure observations, respectively.  We generate non-hydrostatic zenith delay maps for the study region with a temporal resolution of 150 seconds by combining estimated ZWD and tropospheric gradients. These high-resolution ZWD maps are then used to derive IWV maps using surface meteorological measurements and tropospheric profile statistics. We further exploit the approximate relationship between the spatial derivatives of ZWD with tropospheric gradients to compute gradient fields for the entire ZWD map domain.  We compare the spatial patterns of these high-resolution datasets with X-band radar-derived precipitation during heavy convective precipitation events with small spatial extent and high spatial variability. In line with previous studies, we find that the location of precipitation cells is well reflected in the ZWD, IWV, and gradient maps before, during, and after the event, even for very localized, short-lived precipitation events with an extent of only a few kilometers. This shows that GNSS meteorology can provide insights into heavy precipitation events approaching the microscale.

How to cite: Kvas, A., Haas, S., Fuchsberger, J., and Kirchengast, G.: High-resolution zenith delay and tropospheric gradient fields track precipitation during heavy local-scale rainfall events , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10048, https://doi.org/10.5194/egusphere-egu25-10048, 2025.

EGU25-10658 | ECS | Orals | G5.1

Impact of assimilating GNSS Tropospheric Gradients along with Zenith Total Delays for Severe Weather Prediction 

Rohith Muraleedharan Thundathil, Florian Zus, Thomas Schwitalla, Matthias Aichinger-Rosenberger, Galina Dick, and Jens Wickert

The Global Navigation Satellite System (GNSS) tropospheric gradients offer valuable information about how moisture is distributed in the atmosphere. These gradients are determined by studying variations in how the atmosphere refracts signals, which are measured based on delays from satellites positioned at different angles. Zus et al. (2023) developed a tropospheric gradient operator that has been added to the Weather Research and Forecasting (WRF) model. Thundathil et al. (2024) conducted several impact experiments showing promising improvements using this operator.

We are currently integrating data from MPG-NET, a multi-purpose GNSS station network in the Swiss Alps (Aichinger-Rosenberger, Matthias, et al., 2023), and data from the Swabian MOSES (Modular Observation Solutions for Earth Systems) field campaign of 2023, which focused on extreme hydro-meteorological events in southwestern Germany. As part of this work, we are simulating the occurrence of hailstorm activity in July 2023. We plan to present initial results from the assimilation of ZTD and gradients for this event.

References:

Zus, F., Thundathil, R., Dick, G., & Wickert, J. (2023). Fast Observation Operator for Global Navigation Satellite System Tropospheric Gradients. Remote Sensing15(21), 5114.

Thundathil, R., Zus, F., Dick, G., & Wickert, J. (2024). Assimilation of GNSS tropospheric gradients into the Weather Research and Forecasting (WRF) model version 4.4. 1. Geoscientific Model Development17(9), 3599-3616.

Aichinger-Rosenberger, M., Wolf, A., Senn, C., Hohensinn, R., Glaner, M. F., Moeller, G., ... & Rothacher, M. (2023). MPG-NET: A low-cost, multi-purpose GNSS co-location station network for environmental monitoring. Measurement216, 112981.

How to cite: Thundathil, R. M., Zus, F., Schwitalla, T., Aichinger-Rosenberger, M., Dick, G., and Wickert, J.: Impact of assimilating GNSS Tropospheric Gradients along with Zenith Total Delays for Severe Weather Prediction, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10658, https://doi.org/10.5194/egusphere-egu25-10658, 2025.

EGU25-10677 | ECS | Posters on site | G5.1

Comparisons between GAMIT-derived Zenith Tropospheric Delay (ZTD) values from AWS and GNSS met sensor values 

Drishti Agarwal, Somnath Mahato, Pramod Balasaheb Gandugade, Balasubramanian Nagarajan, and Onkar Dikshit

Precise estimation of Zenith Tropospheric Delay (ZTD) is crucial for improving the accuracy of data from Continuously Operating Reference Stations (CORS), particularly in applications requiring high-precision GNSS positioning. This study focuses on evaluating various ZTD models to identify the most accurate approach for mitigating atmospheric delays in CORS data. The research compares ZTD values derived from Automatic Weather Stations (AWS), GNSS meteorological sensors, and temperature-pressure-humidity-based models calculated using the GAMIT software with reference values obtained from co-located weather stations and global atmospheric models.

The methodology involves processing GNSS observations from selected CORS sites using multiple ZTD estimation models, including empirical approaches. The accuracy of these models is assessed using key performance metrics such as root mean square error (RMSE), mean bias, and correlation with actual weather conditions.

Preliminary results indicate that empirical models show better consistency in stable atmospheric conditions. Additionally, comparisons between GAMIT-derived ZTD values and those from AWS and GNSS met sensors reveal insights into the reliability and precision of each data source under different atmospheric conditions.

The study highlights that precise ZTD estimation is essential for reducing atmospheric errors in CORS data, thereby enhancing GNSS-based applications such as geodesy, surveying, and real-time positioning. The research concludes that combining inputs from various meteorological data sources offers the best accuracy across diverse CORS networks, particularly in regions with varying climatic conditions and atmospheric dynamics.

How to cite: Agarwal, D., Mahato, S., Gandugade, P. B., Nagarajan, B., and Dikshit, O.: Comparisons between GAMIT-derived Zenith Tropospheric Delay (ZTD) values from AWS and GNSS met sensor values, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10677, https://doi.org/10.5194/egusphere-egu25-10677, 2025.

EGU25-11277 | Posters on site | G5.1

Ground-GNSS ZTD trends for climate models 

Marcelo C. Santos, Rosa Pacione, Kyriakos Balidakis, Sharyl Byrant, Galina Dick, Riley Hughes, Jonathan Jones, Hanes Keernik, Anna Klos, Yidong Lou, Haroldo Marques, Samuel Nahmani, Thalia Nikolaidou, Kalev Rannat, Raul Valenzuela, Zhang Weixing, Yibin Yao, and Peng Yuan

GNSS Zenith Total Delay (ZTD) estimates are quantities of great interest by climate modellers since atmospheric water vapour is the major greenhouse gas. Therefore, the importance of its accurate, long-term monitoring and evaluation of trends and variability, potentially serving as independent benchmarks to climatological models, both on longer trends derived from GNSS, but also shorter trends, which could be used for assimilation and validation of climate models. ZTD estimates are determined on a regular basis by several processing centers as well as by demand. It has also been demonstrated that series of ZTD estimates can be used for quality control purposes. At the same time, GNSS reached the “maturity age” of 30 years when climate normals of ZTD and gradients can be derived. But what would be the best ZTD series to serve the climate community? What series would offer the most realistic trends? This poster discusses an on-going investigation under the auspices of the International Association of Geodesy, through a joint working group nested within the Inter-Commission Committee on Geodesy for Climate Research. In a previous study, we made use of the ZTD series derived by the third reprocessing campaign (REPRO3), based on a variety of processing modes and models. But this study was partial as the ZTD times series estimated by the Analysis Centers were not covering the same periods. This time, ZTD time series are generated using dedicated PPP scientific software suites. The generated trends are to be compared and analysed.

How to cite: C. Santos, M., Pacione, R., Balidakis, K., Byrant, S., Dick, G., Hughes, R., Jones, J., Keernik, H., Klos, A., Lou, Y., Marques, H., Nahmani, S., Nikolaidou, T., Rannat, K., Valenzuela, R., Weixing, Z., Yao, Y., and Yuan, P.: Ground-GNSS ZTD trends for climate models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11277, https://doi.org/10.5194/egusphere-egu25-11277, 2025.

EGU25-12037 | ECS | Orals | G5.1

From ground- to space-based GNSS tomography - initial results and concepts 

Adam Cegła, Sebastian Makuch, Witold Rohm, Gregor Moeller, Estera Trzcina, Paweł Hordyniec, Samia Gurmani, and Natalia Hanna

Monitoring the Earth's atmosphere is a fundamental activity aimed at understanding its structure and the processes occurring within it. These efforts contribute significantly to improving the quality of numerical weather models and forecasts.

In recent years, GNSS (Global Navigation Satellite System) observations have emerged as one of the primary sources of information about the troposphere, the lowest layer of the atmosphere. The use of electromagnetic wave properties, which respond to changing atmospheric conditions, is gaining recognition due to its stability, availability in all weather conditions, and the density of observations. GNSS observations are increasingly considered a viable alternative to traditional weather stations, radiosondes, and microwave satellites. However, their application is limited by challenges in deploying receivers in aquatic or mountainous regions. Furthermore, the effectiveness of ground-based GNSS observations is hindered by poor vertical resolution.

An alternative to ground-based GNSS observations is their space-based counterpart—radio occultations (RO). These observations, which are independent of ground infrastructure, serve as an ideal complement to traditional ground-based methods. However, their horizontal and temporal resolution is very limited. Their exclusive use in experiments, such as ROMEX, may not demonstrate their full potential, which can be better realized through integration with other tools, particularly GNSS tomography.

Recent studies have shown that integrating ground-based and space-based GNSS observations in a tomographic solution improves solution quality by approximately 10% on average and reduces total solution errors by about 5%. In regions without GNSS ground stations, the error reduction can reach as much as 30%.

Therefore, in this study, we extend this research by testing the feasibility of using a modified INTOMO (INtegrated TOMOgraphy) software with space-based observations only. The program employs 3D ray tracing to simulate RO ray paths between Low Earth Orbit (LEO) and Global Positioning System (GPS) satellites, along with a Kalman filter to calculate the variability of the system of equations. The observation errors are assessed using a pre-defined formula based on RO geometries.

The results presented in this study are derived from the initial phase of research conducted over five days in sea and water-land areas using RO observations from publicly available UCAR services as well as ROMEX data. Each day represents different atmospheric conditions, ranging from sunny weather to tropical cyclones. Additionally, we estimate the errors in the tomographic solution and validate our results using the European Centre for Medium-Range Weather Forecasts (ECMWF) ERA5 and Weather Research and Forecasting (WRF) models and RO processing package (ROPP), with the GPT2 model serving as the a priori data input for tomography. 

How to cite: Cegła, A., Makuch, S., Rohm, W., Moeller, G., Trzcina, E., Hordyniec, P., Gurmani, S., and Hanna, N.: From ground- to space-based GNSS tomography - initial results and concepts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12037, https://doi.org/10.5194/egusphere-egu25-12037, 2025.

EGU25-12098 | Posters on site | G5.1

GNSS for Weather Forecast and Climate Research at GFZ 

Galina Dick, Florian Zus, Rohith Thundathil, Aurélie Panetier, and Jens Wickert

Global Navigation Satellite System (GNSS) is an established atmospheric observing system for atmospheric water vapour with high spatiotemporal resolution. Water vapour is under-sampled in the current meteorological and climate-observing systems, and thus obtaining and exploiting more high-quality humidity observations is essential.

 

The operational GNSS data processing at GFZ provides all tropospheric products, zenith total delays (ZTD), precipitable water vapour (PWV), slant total delays (STD) and tropospheric gradients in the framework of different meteorological projects like e.g. E-GVAP ("The EUMETNET EIG GNSS Water Vapour Programme", http://egvap.dmi). E-GVAP is in charge of the collection and quality control of operational GNSS tropospheric products for numerical weather prediction. GFZ is one of the E-GVAP Analysis Centres and processes about 600 GNSS stations in near real-time. The tropospheric products provided by GFZ are used by European weather services for operational forecasts.

 

GFZ contributes to climate research within the Global Climate Observing System (GCOS) Reference Upper Air Network (GRUAN). Established in 2006, GRUAN, is an international reference observing network of sites measuring essential climate variables above the Earth's surface. Currently, this network comprises 33 reference sites worldwide, designed to detect long-term trends of key climate variables such as temperature and humidity. GFZ hosts a central processing facility for the GNSS data and is responsible for the installation of GNSS hardware, data transfer, processing and archiving, as well as derivation of GNSS-PWV products according to the GRUAN requirements. A complementary small scale regional climate station network is the Austrian WegenerNet, which provides since 2007 measurements of hydrometeorological variables with very high spatial and temporal resolution. GNSS-PWV measurements have been included as a priority one measurement of the essential climate variable water vapour to both GRUAN and WegenerNet climate station networks.

GNSS-derived tropospheric products and results of selected validation studies will be presented.

How to cite: Dick, G., Zus, F., Thundathil, R., Panetier, A., and Wickert, J.: GNSS for Weather Forecast and Climate Research at GFZ, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12098, https://doi.org/10.5194/egusphere-egu25-12098, 2025.

EGU25-14650 | Posters on site | G5.1

A ground-based GNSS-R station for soil moisture monitoring  

Fan Gao, Cheng Qian, Xiao Li, Jiqiang Wei, Jilei Mao, Xinyue Meng, Nazi Wang, Yue Zhu, and Yunqiao He

GNSS-R is an emerging technology for remote sensing of soil moisture with the advantages of high tempo spatial resolutions at low cost. Most of the current research has been carried out on the basis of space borne observations, and a large number of results have been obtained. Due to the high altitude of satellites, the Fresnel reflection zone is usually a few kilometers in diameter, which does not meet the requirements of fine agriculture. Ground-based and UAV-borne GNSS-R, due to their low altitude, can provide effective observations to address above problem. We have built a ground-based GNSS-R observatory at the Experimental Farm of Weihai Academy of Agricultural Sciences, Shandong Province China. The site is equipped with mainly high gain a downward facing left-handed circularly polarized antenna, an upward facing right-handed circularly polarized antenna, an IF signal collector and a computer platform for running the SDR. Currently the main observables that can be output include: SNR, Power Ratio, DDM, etc. The retrievals were evaluated by the in-suit measurements from TDR and the results show that the accuracy of the solutions can reach 3%. In addition, a UAV-based GNSS-R setups are also built and effective measurements were obtained.

How to cite: Gao, F., Qian, C., Li, X., Wei, J., Mao, J., Meng, X., Wang, N., Zhu, Y., and He, Y.: A ground-based GNSS-R station for soil moisture monitoring , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14650, https://doi.org/10.5194/egusphere-egu25-14650, 2025.

EGU25-14987 | ECS | Orals | G5.1

Advancing Sea Ice Thickness Retrieval with Spire GNSS-R Observations 

Seho Kim, Nereida Rodriguez-Alvarez, Xavier Bosch-Lluis, and Kamal Oudrhiri

Monitoring sea ice thickness (SIT) is essential for understanding the role of polar sea ice in the Earth system and addressing the challenges posed by its rapid changes. Arctic sea ice regulates global temperatures, supports ecosystems, and drives ocean circulation. Its decline disrupts ecosystems, intensifies coastal hazards, and impacts indigenous communities. Similarly, Antarctic Sea ice influences ocean stratification, buffers ice shelves from disintegration, sustains marine food webs, and affects human activities such as shipping and fisheries. Comprehensive SIT monitoring in both polar regions is vital for advancing climate science and assessing polar ecosystem health.

This study develops novel algorithms for SIT retrieval using dual-polarimetric and multi-incidence angle GNSS-R data from the Spire Global Inc. constellation. Spire’s GNSS-R receivers collect forward-scattered reflections over ice surfaces in grazing-angle configurations with right-hand circular polarization (RHCP) antennas and near-nadir configurations with left-hand circular polarization (LHCP) antennas. These datasets are utilized in a multi-parameter optimization framework based on a sea ice coherent reflection model to characterize SIT in the critical range of 0.5 m to 1.5 m, where existing remote sensing techniques show significant relative errors. The proposed two-layer model leverages the sensitivity of GNSS-R reflectivity to variations in sea ice dielectric properties, salinity, and density and was validated with data from the Soil Moisture Active Passive (SMAP) mission in its reflectometer configuration (SMAP-R). The algorithms address the measurement gap between thin and thick ice while enhancing spatial and temporal resolution, enabling weekly coverage of the Arctic and Antarctic Oceans. These advancements provide critical insights into SIT dynamics across both regions, addressing gaps in existing techniques.

This research highlights the potential of GNSS-R technology in sea ice monitoring, contributing to the development of robust SIT retrieval algorithms. By advancing SIT retrieval capabilities, this work lays the foundation for improving climate models, informing navigation and resource management, and aiding in the conservation of fragile polar ecosystems facing environmental changes.

© 2025 California Institute of Technology. Government sponsorship acknowledged.

How to cite: Kim, S., Rodriguez-Alvarez, N., Bosch-Lluis, X., and Oudrhiri, K.: Advancing Sea Ice Thickness Retrieval with Spire GNSS-R Observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14987, https://doi.org/10.5194/egusphere-egu25-14987, 2025.

EGU25-15298 | ECS | Posters on site | G5.1

Synergy of GNSS Tomography and Radio Occultation: Methods for Assimilating Refined Water Vapor Fields 

Natalia Hanna, Samia Gurmani, Estera Trzcina, Witold Rohm, Adam Cegła, Paweł Hordyniec, Sebastian Makuch, Gregor Möller, Maciej Kryza, and Robert Weber

Global Navigation Satellite Systems (GNSS) tomography is a rapidly developing method in meteorology that provides 3D grid-based information about water vapour distribution in the lower troposphere. The standard tomographic solutions are derived by processing signal delays between satellites and ground-based GNSS receiver networks. As the technique has advanced, additional observational data sources have been integrated into the process, enhancing its accuracy and applicability.

Low Earth orbit (LEO) satellites can provide signal delays similar to those from ground-based networks by tracking GNSS signals. This technique is known as GNSS radio occultation (RO) and relies on radio transmissions from GNSS satellites, where signals pass through the atmosphere and undergo refraction. The degree of refraction is influenced by atmospheric temperature and water vapor concentration. With the exponential increase in the number of LEOs satellites over the past 30 years, this technique has been a cornerstone for atmospheric measurements. It is widely used in meteorological offices as a tool for weather forecasting and shows strong potential for improving tomographic applications. 

The Weather Research and Forecasting (WRF) Model, equipped with its tomographic operator tomoref, facilitates the integration of tomographic products into meteorological fields. In recent years, several studies have explored available practices for tomographic data assimilation. In this work, we present two variants for assimilating combined RO and tomographic solutions. 

In the first approach, radio occultation-derived wet refractivity profiles from the UCAR COSMIC program were incorporated into the tomographic solution using the ATom tomographic software, enhanced with its RO extension. The 3DVar assimilation of tomographic wet refractivity fields into the WRF Data Assimilation system was performed for both combined and ground-based solutions at selected epochs when radio occultation events occurred within the defined domain. The model’s performance was further validated by comparing it to a solution that assimilated conventional GNSS observations. For ground-based stations, GNSS signal delays, expressed as Zenith Total Delays (ZTDs), were assimilated using the gpsztd operator, while space-derived total refractivity profiles were incorporated using the gpsref operator. The resulting meteorological parameters were then compared to external data sources, including radiosondes, meteorological sites, and ERA5 data.

As part of the ongoing OPUS NCN project, an alternative approach to observation integration is being developed. This integrated tomographic solution combines ground-based GNSS observations with RO excess phase data from SPIRE Global within a unified tomography model on the phase observation level. Since RO events are often unevenly distributed across space and time, the combined tomographic observations address these limitations by filling data gaps with ground-based observations. The resulting wet refractivity fields are then assimilated using a variational approach, incorporating the tomographic data into the model over a broader assimilation window. With further fine-tuning, the presented methodology for assimilating tomographic products demonstrates significant potential for future testing in meteorological centres.

How to cite: Hanna, N., Gurmani, S., Trzcina, E., Rohm, W., Cegła, A., Hordyniec, P., Makuch, S., Möller, G., Kryza, M., and Weber, R.: Synergy of GNSS Tomography and Radio Occultation: Methods for Assimilating Refined Water Vapor Fields, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15298, https://doi.org/10.5194/egusphere-egu25-15298, 2025.

EGU25-15408 | Posters on site | G5.1

New horizon of tropospheric studies using the next generation GNSS, Network of Satellite Constellations and AI 

Witold Rohm, Paweł Hordyniec, Jan Kapłon, Estera Trzcina, Saeid Haji-Aghajany, Peng Sun, Longijang Li, and Kefei Zhang

We present a collaborative research project between Polish and Chinese scientists, supported by national research funding agencies, to advance GNSS remote sensing (RS) for atmospheric studies. Recent advancements in space technologies, artificial intelligence (AI), and information and communication technologies (ICT) have significantly enhanced our ability to observe, model, and predict atmospheric processes. AI-powered GNSS RS offers robust capabilities for acquiring essential atmospheric parameters, such as water vapor content and profiles, rain rates, wind speeds, and cloud composition.

This project focuses on bridging mathematical models, physical processes, and space- and ground-based observations to achieve the following objectives:

  • Data Fusion: Standardize and integrate GNSS RS measurements from ground- and space-based platforms.
  • Innovative Methods: Exploit advanced observation techniques, including signal polarimetry and reflectometry.
  • Network Integration: Harness the potential of multi-constellation satellite networks, including GNSS, LEO satellites, and Starlink-like constellations, for atmospheric studies.
  • AI-Driven Modeling: Develop seamless connections between GNSS observations and weather and climate models using AI and Digital Twin technologies to investigate interactive atmospheric mechanisms.

This research is supported by NCN project UMO-2023/48/Q/ST10/00278, fostering Polish-Chinese scientific collaboration.

How to cite: Rohm, W., Hordyniec, P., Kapłon, J., Trzcina, E., Haji-Aghajany, S., Sun, P., Li, L., and Zhang, K.: New horizon of tropospheric studies using the next generation GNSS, Network of Satellite Constellations and AI, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15408, https://doi.org/10.5194/egusphere-egu25-15408, 2025.

EGU25-15774 | ECS | Posters on site | G5.1

Investigation on systematic deviations of absolute and double differential partial wet delay between GNSS, PS-InSAR, and ERA-5 model observations 

Alfredo Zárate, Andreas Schenk, Bettina Kamm, and Michael Mayer

Interferometric Synthetic Aperture Radar (InSAR) data stacks offer a means to derive integrated water vapor (IWV) from phase delay observations along the satellite line of sight with high spatial resolution. Since interferometric observations are differential in both space and time, they capture relative IWV changes but lack absolute values, which is the variable integration constant. Existing approaches to obtain absolute IWV from InSAR are typically validated against GNSS observations, weather models, or other remote sensing datasets. However, these validations primarily assess the integration methods rather than the observed interferometric phase delay representing partial wet delay.

In this study we investigate the reverse approach by comparing native differential partial wet delay observations from Persistent Scatterer InSAR (PSI), mapped to zenith wet delay (ZWD), with forward-modeled double differential ZWD (DsDt ZWD) derived from GNSS and ERA-5 data. The analysis focuses on a region in Central Europe spanning the France-Germany-Switzerland border from March 2015 to July 2019.

The methodology incorporates data from 4.2 million persistent scatterer (PS) points, ERA-5 ZWD interpolated to these locations, and hourly tropospheric wet delay data from 16 GNSS stations. Temporal and spatial differences were computed to generate synthetic DsDt ZWD data stacks, enabling direct comparison of GNSS and ERA-5 ZWD. Analyses were conducted in single differential (temporal) and double differential (temporal and spatial) domains, with evaluations performed at GNSS stations using statistical metrics such as the coefficient of determination (R²) and the Kling-Gupta Efficiency (KGE) index. Seasonal variability was also assessed. Additionally, the study examines how local distances around GNSS stations affect the correlation (R² and KGE) between GNSS-InSAR and GNSS-ERA data, evaluating their impact on measurement consistency.

Results reveal valuable insights into the performance of InSAR, GNSS, and ERA-5 ZWD. In the single differential domain, the variance of Dt ZPWD from InSAR aligns closely with GNSS and ERA-5 data. While scatter plots confirm a linear relationship between GNSS and ERA-5, GNSS vs. InSAR trends appear nonlinear. Applying double differences significantly enhances the correlation between GNSS and InSAR, surpassing that of GNSS and ERA-5. The KGE index highlights improved GNSS-InSAR performance, particularly in correlation (R) and variability ratio (Alpha). Seasonal analyses show that GNSS-InSAR excels during summer, with mean R² values twice those of GNSS-ERA, whereas GNSS-ERA performs better in winter. Regional variability is observed, with higher differences in R² and KGE values at stations in the Rhine Valley.

In conclusion, this study demonstrates the capability of PS-InSAR to provide high-resolution, accurate differential ZWD estimates, particularly during summer. PS-InSAR shows a stronger correlation with GNSS data in the double differential domain compared to ERA-5, underscoring the value of high-resolution ZWD data. Systematic variations in GNSS-InSAR correlation, identified as potential quality indicators for GNSS ZWD products, further highlight the importance of integrating multi-source geodetic data to enhance ZWD monitoring.

How to cite: Zárate, A., Schenk, A., Kamm, B., and Mayer, M.: Investigation on systematic deviations of absolute and double differential partial wet delay between GNSS, PS-InSAR, and ERA-5 model observations, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15774, https://doi.org/10.5194/egusphere-egu25-15774, 2025.

EGU25-15927 | ECS | Posters on site | G5.1

Near Real-Time Tropospheric Delay Assessment Through theVariometric Approach: A Comparative Study of Two-Variable and Separate-Variable Functional Models for ZTD Estimation 

Rachele Fratini, Alessandra Maria De Pace, Augusto Mazzoni, and Mattia Crespi

The variometric approach leverages the use of dual-frequency combinations of time-single differences of GNSS phase observations. Successfully applied in GNSS seismology (VADASE, [1,2]) and GNSS ionospheric seismology (VARION, [3]), this methodology is explored in this study for its potential in near real-time tropospheric delay tracking. Its application to weather forecasting could significantly improve current tools, allowing for a timely detection of severe weather events through real-time tropospheric delay monitoring. This research investigates the retrieval of absolute ZTD trends from variometric zenith tropospheric delay (VZTD) estimates, derived through two different approaches. The first strategy employs a two-unknown weighted least-squares-based functional model to estimate VZTD and receiver clock offset (VCLKR). Reseach shows that this approach may lead to potential ill-conditioning of the design matrix in the least-squares process, possibly due to the correlation between the estimated parameters. To address this issue, a second approach is introduced that utilizes a dedicated functional model to separate the estimation of the two parameters. The comparative analysis of VZTD estimates on permanent station data highlights significant discrepancies between the two approaches, with pronounced differences in the magnitude of the retrieved absolute ZTD trends. This study provides evidence of the sensitivity of the two-variable estimation approach to the correlation between VZTD and VCLKR. Separate variable estimation offers improved results, with the ZTD trend being more consistent with the reference Precise Point Positioning (PPP) estimates. This analysis demonstrates that separating the estimation of VZTD and VCLKR parameters enhances the reliability of absolute ZTD estimates through the variometric approach.

[1] Benedetti, Elisa, et al. ”Global Navigation Satellite Systems seismology for the 2012 M w 6.1 Emilia earthquake: Exploiting the VADASE algorithm.” Seismological Research Letters 85.3 (2014):649-656
[2] Colosimo, Gabriele, et al. ”Realˆatime GPS seismology with a stand−alone receiver: A preliminary feasibility demonstration” Journal of Geophysical Research: Solid Earth 116.B11 (2011).
[3] Savastano, Giorgio, et al. ”Real−time detection of tsunami ionospheric disturbances with a stand-alone GNSS receiver: A preliminary feasibility demonstration.” Scientific reports 7.1 (2017): 46607

How to cite: Fratini, R., De Pace, A. M., Mazzoni, A., and Crespi, M.: Near Real-Time Tropospheric Delay Assessment Through theVariometric Approach: A Comparative Study of Two-Variable and Separate-Variable Functional Models for ZTD Estimation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15927, https://doi.org/10.5194/egusphere-egu25-15927, 2025.

EGU25-16138 | ECS | Posters on site | G5.1

Optimizing GNSS Tomographic Node Distribution Using Signal Geometry for Enhanced Tropospheric Sensing 

Estera Trzcina, Witold Rohm, and Kamil Smolak

Global Navigation Satellite Systems (GNSS) are a powerful tool for high-resolution tropospheric sensing, offering valuable data for weather forecasting and climate monitoring. One of the key techniques for estimating three-dimensional fields of humidity-related parameters in the troposphere using GNSS data is tomography. Recent studies revealed its potential for application in data assimilation into numerical weather prediction models. However, the accuracy of the tomographic models depends heavily on the approach to the distribution of the tomographic nodes. Traditionally, the nodes are placed on a regular grid, without accounting for the uneven distribution of GNSS signal information in the troposphere, which often leads to suboptimal results.

 

In this study, we propose a novel approach to optimize the spatial arrangement of tomographic nodes, based on the geometry of the GNSS signals and the non-uniformity of the information they provide. The proposed algorithm is based on four steps to define the optimal arrangement of the tomographic nodes: 1) selecting the most valuable GNSS signals in terms of geometry (those that cross with other signals), 2) identification of the intersection spots, 3) cluster analysis of the defined intersections using DBSCAN algorithm, 4) introducing regularly-distributed nodes in the locations with lower-density of the GNSS signals to increase stability of the model. The final solution is performed using a node-based parameterization approach with interpolation of wet refractivity based on natural cubic splines. To evaluate the effectiveness of the optimized node distribution, we compare the performance of our approach with that of three conventional parameterization methods (both voxel-based and node-based with trilinear and spline-based interpolation), using cross-validation based on outputs from the Weather Research and Forecasting (WRF) model and radiosonde observations. The methodology was tested in an urban area, using zenith tropospheric delay estimates from a dense network of 16 low-cost multi-GNSS receivers located in Wrocław, Poland, with an average inter-receiver distance of 3 km.

 

The results show that the optimized node placement improves the accuracy of wet refractivity estimation, with a reduction in RMSE of 0.5–2 ppm, especially in the altitude range of 0.5–2.0 km. The proposed solution gave the best results compared to the other parameterization approaches (both voxel-based and node-based). The largest impact was noticed in the areas where the highest number of the GNSS signals’ intersections occurred. This study highlights the importance of considering the geometry of GNSS signals when designing tomographic networks and suggests that optimizing node distribution is a promising avenue for future research in GNSS-based tropospheric sensing.

How to cite: Trzcina, E., Rohm, W., and Smolak, K.: Optimizing GNSS Tomographic Node Distribution Using Signal Geometry for Enhanced Tropospheric Sensing, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16138, https://doi.org/10.5194/egusphere-egu25-16138, 2025.

Neutral atmospheric bending angles derived from GNSS Radio Occultation (GNSS-RO) data are essential for estimating atmospheric properties such as temperature, humidity, and pressure. The region of interest for atmospheric properties extends up to 80 km, where ionospheric effects remain and require ionospheric corrections for accurate RO bending angle retrievals. First-order ionospheric terms are typically removed using a linear combination of L1 and L2 bending angles. However, this approach leaves behind higher-order terms, known as residual ionospheric errors (RIEs), which introduce systematic biases into the RO data.

Healy and Culverwell (2015) demonstrated that RIEs are theoretically proportional to the square of the difference between L1 and L2 bending angles, scaled by a coefficient, kappa, which varies with ionospheric conditions. Kappa correction is a convenient method to estimate RIEs directly from bending angle data without relying on external ionospheric data such as electron density profiles. Angling et al. (2018) proposed a simple linear model to estimate kappa as a function of altitude, F10.7, and solar zenith angle. They used the NeQuick model to generate electron density profiles and derived the linear model for kappa estimation. However, since NeQuick is a monthly median ionospheric electron density model, it has limitations in representing real-world ionospheric variability, leading to discrepancies between the kappa values from the NeQuick-based model and those estimated from actual data. Therefore, a more realistic derivation of kappa using actual RO data is needed to develop an improved kappa model.

This study aims to enhance kappa correction by using real electron density profiles derived from GNSS-RO data. A double Chapman layer is fitted to electron density profiles from COSMIC-II data, incorporating the characteristics of the E and F layers to provide continuous representations of the real electron density profiles. Ray-tracing simulations are conducted to obtain L1 and L2 ionospheric bending angles, which are then used to derive kappa values. These kappa values are analyzed under various ionospheric conditions, characterized by user-end parameters such as F10.7, local time, geomagnetic latitude, and altitude.

To examine more accurately the numerical relationship between kappa and these parameters, kappa data is classified by F10.7 to represent different solar activity conditions (e.g., solar minimum and maximum), and is also divided by local time (e.g., noon, midnight, and transition periods). Kappa values for each class are then fitted to the remaining parameters. The findings suggest that kappa values from the model proposed by Angling et al. (2018) differ from those estimated using observational data in this study. By directly deriving kappa values from real data and applying separate fits for different classes of solar activity and local time periods, the modeling accuracy can be enhanced. This study shows the necessity of tailored kappa corrections for different ionospheric conditions, improving techniques for correction of RIEs in GNSS-RO data. 

References

Healy,S.B., & Culverwell,I.D. (2015). A modification to the standard ionospheric correction method used in GPS radio occultation. Atmospheric Measurement Techniques, 8(8), 3385–3393.https://doi.org/10.5194/amt-8-3385-2015

Angling,M.J., Elvidge S., & Healy,S.B. (2018). Improved model for correcting the ionospheric impact on bending angle in radio occultation measurements. Atmospheric Measurement Techniques, 11(4), 2213–2224.https://doi.org/10.5194/amt-11-2213-2018

How to cite: Park, J., Chang, J., Sun, K., and Lee, J.: Residual Ionospheric Error Correction in GNSS Radio Occultation Bending Angles: Parametric Analysis using Electron Density Profiles Derived from COSMIC-II Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18658, https://doi.org/10.5194/egusphere-egu25-18658, 2025.

EGU25-19045 | ECS | Orals | G5.1

AI for GNSS Reflectometry: Setting a New Benchmark for Earth Surface and Atmospheric Monitoring 

Milad Asgarimehr, Daixin Zhao, Tianqi Xiao, Hamed Izadgoshasb, and Jens Wickert

GNSS Reflectometry (GNSS-R) satellite constellations offer unprecedentedly large datasets. This creates a unique opportunity to harness the power of AI for Earth system monitoring using GNSS-R. By using these vast datasets, AI models can “learn” effectively and adaptively. The AI for GNSS-R (AI4GNSS-R) project unlocks the potential of deep learning to produce high-quality and innovative data products.

Previously, we introduced CyGNSSnet, a deep learning model based on a CNN-LSTM architecture, which achieved an RMSE of 1.36 m/s—representing a substantial 28% improvement over the officially operational retrieval algorithm. Building on this success, we now present an advanced version of the model that incorporates external precipitation data through data fusion. This enhanced approach achieves an RMSE of 1.57 m/s for rain-affected data, significantly improving wind speed predictions under extreme weather conditions. For land monitoring, we demonstrate the retrieval of Vegetation Water Content (VWC) from GNSS-R data. Using architectures such as LeNet, our models achieve RMSEs below 0.6 kg/m² compared to SMAP VWC data, validating GNSS-R's capability for  global vegetation moisture monitoring. A highlight of our research is the development of a GNSS-R general foundation model using self-supervised learning. This model facilitates the fusion of multimodal data and enables scalable and accurate retrieval of variety of parameters such as wind speed, soil moisture, and VWC with limited labeled data. Our findings emphasize the scalability, adaptability, and applicability of next-generation AI models for GNSS-R. These advancements establish a new benchmark for the achievable quality and extends application spectrum of spaceborne GNSS-R.

How to cite: Asgarimehr, M., Zhao, D., Xiao, T., Izadgoshasb, H., and Wickert, J.: AI for GNSS Reflectometry: Setting a New Benchmark for Earth Surface and Atmospheric Monitoring, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19045, https://doi.org/10.5194/egusphere-egu25-19045, 2025.

EGU25-20963 | ECS | Posters on site | G5.1

Evaluating the Performance of Numerical Weather Prediction Models for Precipitation and Temperature in Luxembourg and the Greater Region: Insights from WRF and WRFDA 3D-Var 

Haseeb Ur Rehman, Felicia Norma Teferle, Addisu Hunegnaw, Guy Schumann, Jens Wickert, Florian Zus, and Rohith Muraleedharan Thundathil

Compared to alluvial floods, flash or pluvial floods are difficult to predict because they result from intense and brief periods of extreme precipitation. Luxembourg has a history of being impacted by floods, with notable occurrences in January 2011, May 2016, December 2017, January 2018, February 2019, and February 2020. However, July 2021 stands out as the most severe flood year on record in the region. In this study we aim to develop, a high-resolution numerical weather predicRon (NWP) model for effective local heavy rainfall prediction in a nowcasting scenario and provide real-time for flood simulation. The modeling relies on the Weather Research and ForecasRng (WRF) model, which incorporates local Global Navigation Satellite System (GNSS) zenith total delays and precipitation observations to simulate small-scale, high-intensity convective precipitation. As part of this, we will also test run the LISFlood flood model in an operational inundation forecast mode, meaning that the flood model will be run with the WRF precipitation forecasts as inputs. The WRF model was configured for the Greater Region, utilizing a horizontal grid resolution of 12 km and incorporating high-resolution static datasets. Meteorological data, i.e., June 20 -July 20, 2021, from the Global Forecast System (GFS) were employed in the model setup as initial boundary condition. Zenith Total Delay (ZTD) data collected from various GNSS stations (245) across Germany and Luxembourg were assimilated into the model. Additionally, observational datasets, including Surface Synoptic Observations (SYNOP), Upper Air Data, Radiosonde measurements (TEMP), and Tropospheric Airborne Meteorological Data Reporting (TAMDAR) were assimilated. Following this integration, an sensitivity analysis of various meteorological parameters such as precipitation, surface temperature (T2), and relative humidity was performed.

How to cite: Rehman, H. U., Teferle, F. N., Hunegnaw, A., Schumann, G., Wickert, J., Zus, F., and Muraleedharan Thundathil, R.: Evaluating the Performance of Numerical Weather Prediction Models for Precipitation and Temperature in Luxembourg and the Greater Region: Insights from WRF and WRFDA 3D-Var, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20963, https://doi.org/10.5194/egusphere-egu25-20963, 2025.

EGU25-2295 | Orals | ESSI3.2

Data Lifecycle Management for Field Campaigns: Welcome to the Earth Observing Laboratory Field Catalog and Archive 

Jacquelyn C. Witte and the Data Management and Services Team

The NSF NCAR Earth Observing Laboratory (EOL) has supported over 600 national and international field campaigns which represent half a century of field-based observational science. Our mission is to provide responsive, high quality data services to researchers in field campaigns including pre-field phase planning, real-time decision-making tools, and long-term data curation to support the complete project life cycle. Such support includes (1) serving as the online hub for field campaign operations with access to real-time mission coordination displays and communication tools, (2) ensuring a secure, easily accessible archive of campaign observations, and (3) providing long-term stewardship and curation of observational datasets. All datasets in the EOL’s Field Data Archive are publicly accessible and findable at https://data.eol.ucar.edu/.  

 

EOL data management services are continuously evolving as we pursue FAIR and TRUSTed principles based on industry standards, user feedback and the desire to increase data discovery and accessibility to the broader scientific community. The management of our field campaign data is an iterative, human-driven and agile process. Thus, to address challenges arising from data preparation, preservation, and provenance metadata as the volume and variety of our data grows, EOL has developed tools and workflows that track and maintain the collection of data. In this presentation we will introduce highlights and functionalities of the Field Catalog and the Field Data Archive that together provide end-to-end customized data management services for field campaigns.

How to cite: Witte, J. C. and the Data Management and Services Team: Data Lifecycle Management for Field Campaigns: Welcome to the Earth Observing Laboratory Field Catalog and Archive, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2295, https://doi.org/10.5194/egusphere-egu25-2295, 2025.

EGU25-2803 | Orals | ESSI3.2

GOYAS: A FAIR-by-Design System for Innovative remote-sensing data products 

Fernando Aguilar Gómez, Verónica González-Gambau, Cristina González-Haro, Aina García-Espriu, Eva Flo, Estrella Olmedo, Isabel Caballero, Evgeniia Makarova, Marcos Portabella, Daniel García-Díaz, and Isabel Afán

The Geospatial Open Science Yielding Applications (GOYAS) project, under the umbrella of the Horizon Europe project “OSCARS”, proposes a new approach for open science and open data in remote-sensing, integrating FAIR principles (Findable, Accessible, Interoperable, and Reusable) from the initial design phase. GOYAS provides innovative and/or experimental Earth Observation (EO) data and open science practices to address diverse environmental challenges, delivering advanced geospatial products that are tailored to meet the needs of multiple stakeholders, including researchers, decision-makers, and environmental managers.

GOYAS focuses on generating innovative and accessible remote sensing products for a variety of applications: monitoring water quality parameters, such as turbidity or chlorophyll-a; deriving high-resolution bathymetric maps over coastal regions based on optical instruments; assessing oceanographic variables like sea surface temperature and salinity; improving ocean and atmosphere forecasting capabilities with enhanced sea-surface wind & stress products; and supporting ecosystem monitoring and management in protected areas such as Doñana National Park. These products are generated through the integration of multi-source EO data, including Copernicus Sentinel satellites and complementary datasets, with advanced processing pipelines built on machine learning algorithms and geospatial standards.

A core strength of the GOYAS project lies in its FAIR-by-design system architecture, which prioritizes:

  • Findability: Metadata-rich datasets indexed through open repositories and geospatial catalogues to enhance discoverability.

  • Accessibility: FAIR-compliant platforms with user-friendly interfaces that provide seamless access to data products, ensuring usability across diverse technical expertise levels. GOYAS aims at facilitating the access providing data in common formats and contextualizing them with proper metadata.

  • Interoperability: Adoption of open geospatial standards (e.g., OGC, INSPIRE) to ensure compatibility with existing systems and facilitate data exchange, specially under the context of Research Infrastructure hubs like ENVRI.

  • Reusability: Comprehensive documentation and adherence to open licenses that allow users to adapt and build upon project outputs.

Key innovations include the automated processing of remote-sensing data to extract actionable insights and the application of machine learning to improve the accuracy and reliability of derived parameters. For example, GOYAS employs advanced spectral analysis techniques to calculate shallow bathymetry with sub-meter precision in coastal environments, as well as algorithms for near-real-time detection of water quality anomalies in inland waters.

The system also provides support for the monitoring and management of sensitive ecosystems. In Doñana National Park, GOYAS enables the identification of changes in hydrological regimes or vegetation health through the integration of long-term EO datasets with local ecological studies. Similar applications extend to marine protected areas, where GOYAS aids in monitoring oceanographic dynamics and ecosystem responses to climate change.

This presentation will detail the design, architecture, implementation, and outcomes of the GOYAS project, emphasizing its alignment with FAIR principles and its transformative potential for environmental monitoring. By fostering interoperability and collaboration across disciplines, GOYAS serves as a model for how open science and advanced remote sensing can drive innovation, sustainability, and informed decision-making in geospatial research.

How to cite: Aguilar Gómez, F., González-Gambau, V., González-Haro, C., García-Espriu, A., Flo, E., Olmedo, E., Caballero, I., Makarova, E., Portabella, M., García-Díaz, D., and Afán, I.: GOYAS: A FAIR-by-Design System for Innovative remote-sensing data products, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2803, https://doi.org/10.5194/egusphere-egu25-2803, 2025.

EGU25-4203 | ECS | Orals | ESSI3.2

Escaping from the 1600s: Advancing FAIR scientific knowledge with reborn articles 

Lauren Snyder, Hadi Ghaemi, Ricardo Perez-Alvarez, and Markus Stocker

Text-based literature remains the primary expression of scientific knowledge. Since the first scientific article published in 1665, we have managed the switch from physically printed articles to PDFs, but nothing more. While PDF publications can be easily shared electronically, they remain unstructured text-based documents that machines cannot easily interpret (i.e., they are not machine-reusable). This limits our ability to use digital support tools to efficiently extract and organize knowledge from scientific articles. Rather, to reuse most scientific results (e.g., for synthesis research), we must first extract them from articles and organize them into databases, which is time consuming and prone to error. 

Here, we present reborn articles, which offer a novel approach to producing scientific knowledge. By integrating with programming languages commonly used for data analysis, like R and Python, reborn articles allow researchers to produce scientific results in a machine-reusable format from the outset. This means subsequent data users can download the results of a reborn article as a CSV file with just a click of a button and bypass post-publication data extraction. To support the production, publication, and reuse of reborn article data, we developed ORKG reborn, a FAIR knowledge online infrastructure. 

Using an ecological dataset, we showcase the production of a reborn article, and its impact on knowledge integration and synthesis. Building on the author’s original data analyses conducted in R, we developed an accompanying R script to produce machine-reusable descriptions of the original statistical models that were automatically harvested by ORKG reborn, eliminating manual data entry. We envision that the use of programming languages, like R, to facilitate the production of machine-reusable scientific knowledge could feasibly be streamlined into existing FAIR data management requirements that are already implemented by many academic publishers. Broad adoption of the approach across research communities could transform the way we share and synthesize scientific knowledge. 

How to cite: Snyder, L., Ghaemi, H., Perez-Alvarez, R., and Stocker, M.: Escaping from the 1600s: Advancing FAIR scientific knowledge with reborn articles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4203, https://doi.org/10.5194/egusphere-egu25-4203, 2025.

EGU25-9401 | Orals | ESSI3.2

Scalable Solutions for Urban Data Spaces: Insight from the USAGE blueprint 

Piotr Zaborowski, Francesca Noardo, Giacomo Martiano, and Danny Vandenbroucke

The USAGE objective is to identify, implement, and demonstrate an architecture and solutions for a data space supporting the European Green Deal priorities. It implements the methodology based on the data USAGE data space framework built around specific use cases in the context of local and European policies and guidelines as well as digitalization agendas. Use cases, considered the primary value proposition for the data uptake, are developed and maintained in the USAGE framework. They cover  urgent municipalities scenarios like heat islands, clean energy, qir quality and mobility. Target requirements are translated into data and service requirements expressed in the ISO catalog-based model tailored to the specific data quality measures for the Decision Ready Information. Implementation of the value chain goes across various data inputs including satelite and airborne images, local sensors and citizen science data, surface and urban models producing intermediary and end user products and services. Disciplined and tool-supported collection of the data and application assets consistent with the INSPIRE-compliant schemas and data requirements model which allows them to leverage the solutions' potential and implement the value proposition for their providers. Profiled models create the frames of the data value chain, documenting processing steps from the data requirements through BPMN data flow models linking to the used and produced assets. In addition, licensing schema, including the constraints model, allows for data sovereignty and trust among the data space actors.

The outcome blueprint for the urban data space goes beyond the USAGE pilots to test scalable solutions based on adopting the proposed set of standards coming mainly from ISO, OGC, W3C, OASC and their extensions. It is built in the European initiatives and legal references (i.e., the European strategy for data, the European interoperability framework, the European interoperability reference architecture), and reviewed several projects and initiatives results contributing to shaping data spaces: Open DEI design principles, the International Data Spaces Association (IDSA) reference architecture, Gaia-X architecture, Data Spaces Business Alliance (DSBA) documents, the Data Spaces Support Centre (DSSC) results, Data Space for Smart and Sustainable Cities and Communities (DS4SSCC) outcomes, and the GREAT project Technical Blueprint. Presentation goes across the best practices and guidances extracted from the implementation of the FAIR dataspace and considerations given defined frameworks.

How to cite: Zaborowski, P., Noardo, F., Martiano, G., and Vandenbroucke, D.: Scalable Solutions for Urban Data Spaces: Insight from the USAGE blueprint, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9401, https://doi.org/10.5194/egusphere-egu25-9401, 2025.

EGU25-9739 | Posters on site | ESSI3.2

Reducing the Pain of Data Discovery in Earth System Science 

Aenne Loehden, Claudia Martens, and Andrea Lammert

Ontologies offer significant potential for advancing Earth System Science (ESS) by improving the discoverability and usability of complex datasets and tools. This poster builds on last year’s comic, which illustrated the foundational benefits of ontologies, and presents the first steps in implementing generic tools from already existing terminology services designed to enhance data findability and data comprehension. These tools enable scientists to easily search for appropriate data and retrieve information about data from specific repositories, thus supporting the FAIR (Findable, Accessible, Interoperable, and Reusable) principles in ESS.

Key aspects of terminologies include the clear and consistent description of scientific terms, their relationships, and the unambiguous identification of terms to prevent inconsistencies. By using terminologies we can ensure that terms are defined in a way that is both standardized and interoperable across different datasets and research communities. Concrete examples will be drawn from the World Data Center for Climate (WDCC), where first steps have been taken to implement generic tools and extend the application of terminologies, and to thus enhance data discoverability and facilitate better searchability of climate-related information.

How to cite: Loehden, A., Martens, C., and Lammert, A.: Reducing the Pain of Data Discovery in Earth System Science, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9739, https://doi.org/10.5194/egusphere-egu25-9739, 2025.

EGU25-10627 | Orals | ESSI3.2

FAIR EU soil vocabularies: an overview of joint efforts from some EU Soil Mission projects 

Mickaël Beaufils, Paul van Genuchten, Fenny van Egmond, and Kathi Schleidt

Vocabularies or thesauri, lists of terms with their definitions and unique ID, like a dictionary of a language, play a critical role in the domain of soil science, providing a standardized framework for accurately documenting and communicating soil characteristics. In soil science, the use of precise and consistent terminology ensures the effective exchange of data, promoting interoperability among researchers, practitioners, and decision-makers. A well-structured vocabulary, part of soil classification or soil description standards, facilitates the classification of soil properties, such as texture, structure, fertility, and organic content, allowing combining data from different sources but described in a similar way. And thereby enabling reliable comparison and interpretation across different regions and time periods. Furthermore, these vocabularies enable and support the development of standardized databases, soil datasets and soil monitoring systems, which are essential for environmental management, land use planning, and agricultural practices. Inaccurate or ambiguous soil descriptions can lead to misinformed decisions, making the establishment of clear, universally accepted vocabularies crucial for advancing soil science, conservation efforts, and sustainable land management practices. Such practices would greatly enhance the FAIRness of the data being managed, ensuring data conservation over time.

Soil vocabularies come from many sources, some national or regional, some from international organizations such as the Food and Agriculture Organization of the United Nations (FAO) or the International Union of Soil Sciences (IUSS), e.g. World Reference Base for Soil Resources (WRB) or FAO Guidelines on Soil Description. Several initiatives worked on the identification and provision of agreed vocabularies in order to ensure the interoperability of their results at different scales (national, EU, international). This includes work by standard setting organizations (eg. ISO TC190), legislation (eg. EU INSPIRE Directive) and of course numerous collaborative projects, such as SIEUSOIL, EJP SOIL, ISLANDR, SoilWise, SPADES, Soil Mission Support and MARVIC. At present, many existing vocabularies have not been exposed in a referenceable and machine-readable manner, and instead remain “trapped” within PDF documents. Extracting the relevant concepts and exposing them in both human and machine readable forms on persistent URIs would be a valuable step towards soil data harmonization.

The European Mission: A Soil Deal for Europe, with currently about 50 research projects and a network of 100 living-labs and lighthouses, offers an interesting environment and opportunity for the co-creation of a harmonised framework for soil vocabulary description. Due to the diversity of Soil Mission Projects, gaps in existing vocabularies can be identified and experience can be gained in how to best present vocabularies for both data annotation as well as data discovery.

In this presentation we will share the current status on this topic, offering a non-exhaustive yet hopefully informative overview on existing materials (vocabularies and associated technologies to share them), on-going work and key challenges for achieving better soil data interoperability.

This study was made possible through funding from the EU's Horizon Europe program, specifically the ISLANDR and SoilWise projects.

How to cite: Beaufils, M., van Genuchten, P., van Egmond, F., and Schleidt, K.: FAIR EU soil vocabularies: an overview of joint efforts from some EU Soil Mission projects, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10627, https://doi.org/10.5194/egusphere-egu25-10627, 2025.

EGU25-11467 | ECS | Posters on site | ESSI3.2

Advancing FAIR geochemical data: 25 Years of GEOROC database service 

Leander Kallas, Marthe Klöcking, Kirsten Elger, Bärbel Sarbas, Adrian Sturm, Stefan Möller-McNett, Matthias Willbold, and Gerhard Wörner

The GEOROC synthesis database, a pioneering open-access resource for geochemical and isotopic data, marks 25 years of service to the geoscience community. Over its history, GEOROC has compiled data from more than 22,750 publications in the field of geochemistry, and provides free access to over 39 million individual data values, primarily on igneous and metamorphic rocks, minerals and their inclusions. As a cornerstone for interdisciplinary research, GEOROC is complementary to other geochemical synthesis databases like PetDB, AstroMat and GeoReM, in facilitating reuse of data for innovative studies that leverage data analytics and machine-learning approaches across geoscientific disciplines and beyond.

The Digital Geochemical Data Infrastructure (DIGIS) project for GEOROC 2.0 is providing an up-to-date IT infrastructure that aligns GEOROC with the FAIR principles. Data findability and accessibility are ensured through the newly developed API and the improved GEOROC web interface that allows users to retrieve a variety of distinct data products and services, including a fully customizable search functionality. Interoperability is achieved via implementation of a feature-based data model compatible with the OGC Observations and Measurements standard and controlled, machine-readable vocabularies that harmonize geospatial, analytical and sample-related metadata, and enabling seamless integration in multiple databases and portals (e.g., EarthChem). Reusability is further supported by archiving time-stamped GEOROC data products in the DIGIS Data Repository, hosted by GFZ Data Services, where datasets with digital object identifiers (DOIs) are archived for the long-term. Additionally, researchers are encouraged to directly submit new or already “published” datasets to this domain repository—through standardized (meta-)data templates, ensuring high-quality data submissions that facilitate data quality assessment and reuse.

In collaboration with national and global initiatives, such as OneGeochemistry and NFDI4Earth, the DIGIS project further promotes practical approaches to the FAIR principles for geochemistry by developing unified controlled vocabularies for geochemical data and their metadata (e.g., analytical methods, sample description, location). These vocabularies also integrate external standards, such as the International Mineralogical Association’s "List of Minerals" and MinDat’s "Subdivisions of Rocks," alongside newly developed (and published) frameworks for categories such as geological setting and analytical methods (collaboration with EarthChem). By harmonizing metadata across geospatial, analytical and sample-related categories, these efforts ensure consistency, improve data quality assessment and control and enhance interoperability across data systems, including but not limited to GEOROC, PetDB, and AusGeochem. Such advancements expand the potential applications of geochemical data, fostering innovation in fields such as environmental science, remote sensing, archaeology and geohealth.

With 25 years of experience and ongoing innovation through the DIGIS project, the GEOROC database exemplifies how operationalizing the FAIR principles enhances its value as a critical resource for the geoscience community. By providing both FAIR and open data, GEOROC empowers researchers to conduct reproducible, impactful studies and fosters interdisciplinary collaboration, driving innovation and advancing progress across the geosciences.

How to cite: Kallas, L., Klöcking, M., Elger, K., Sarbas, B., Sturm, A., Möller-McNett, S., Willbold, M., and Wörner, G.: Advancing FAIR geochemical data: 25 Years of GEOROC database service, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11467, https://doi.org/10.5194/egusphere-egu25-11467, 2025.

EGU25-14320 | ECS | Orals | ESSI3.2

EarthBank by AuScope: Building FAIR research data infrastructure for the global geochemical community 

Angus Nixon, Bryant Ware, Brent McInnes, Fabian Kohlmann, Moritz Theile, Wayne Noble, Yoann Gréau, Hayden Dalton, Halimulati Ananuer, Malcolm McMillan, and Ashley Savelkouls

The geochemical community increasingly generates and requires large volumes of analytical data from a wide array of acquisition methods, analytical scales, and sample types in order to address broad research applications. Resulting datasets are commonly collected and reported through non-standardised protocols and reporting formats, if indeed standards are applied at all, which inhibits easy sharing of data during collaborative research projects or repurposing of legacy data. Existing repository services do not presently satisfy requirements for Findable, Accessible, Interoperable and Reusable (FAIR) data, and especially contain significant flaws as to the reuse and interoperability of geochemical data. Generalist repositories such as Zenodo or Figshare do not provide consistent data structures or curation, hence data held within these services is highly variable with regard to format, parameters reported and potentially quality. While domain repositories commonly do implement internally consistent data formats and a level of curation, data within repositories is gathered from published sources which may be incomplete or unstructured, and hence often lack the complete information (metadata) required to appropriately describe the data and allow it to be confidently reused. 


To truly unlock the potential of the ever expanding wealth of geochemical data and meet FAIR requirements, improvements to the data infrastructure landscape are clearly required. The AuScope Geochemistry Network (AGN) is an Australian-based collaboration of geoscientists producing bespoke data resources and infrastructure for the international community to capture, normalise, and share geochemical data resources. These resources include best practice data reporting schema and vocabularies for a variety of data types, produced through collaborations with expert advisory groups and, where available, following or expanding on existing international community recommendations. These data resources have been implemented to the EarthBank platform (formerly AusGeochem), an open web service designed by the AGN to capture, share, store and evaluate geochemical data and metadata. Unlike many other services, researchers are able to upload data prior to publication which can assist both in allowing researchers to compare their data with other existing resources prior to submission, but importantly also improves the likelihood of capturing the full data and metadata associated with analyses required for reuse. Once data is uploaded to this service it may be associated with a dataset DOI to support data access requirements for publication, in order to streamline the publication process and provide a domain specific repository for supplemental data. Data models for U/Pb, fission track, (U-Th-Sm)/He, 40Ar/39Ar and inorganic major and trace geochemistry data types are presently implemented within EarthBank, allowing users to freely upload generated research data for these systems, or explore and integrate existing datasets. Best practice templates for upload are openly available through the EarthBank platform, and vocabularies are openly discoverable through the Research Vocabularies Australia (RVA) service. These resources may be used not only to upload data, but also to develop cross-walks for machine-to-machine interoperability with other repository services to build a global FAIR compliant infrastructure required to maximise data access and improve research outcomes.

How to cite: Nixon, A., Ware, B., McInnes, B., Kohlmann, F., Theile, M., Noble, W., Gréau, Y., Dalton, H., Ananuer, H., McMillan, M., and Savelkouls, A.: EarthBank by AuScope: Building FAIR research data infrastructure for the global geochemical community, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14320, https://doi.org/10.5194/egusphere-egu25-14320, 2025.

EGU25-14828 | Orals | ESSI3.2

Uplifting and streamlining FAIR data implementation for Australia’s climate modelling outputs 

Kelsey Druken, Clare Richards, Romain Beucher, Johanna Basevi, Chris Bull, Claire Carouge, Martin Dix, Aidan Heerdegen, Paul Leopardi, Davide Marchegiani, Heidi Nettelbeck, Anton Steketee, Charles Turner, Marc White, and Spencer Wong

Australia’s Climate Simulator (ACCESS-NRI) is a national research infrastructure established to support the Australian Community Climate and Earth System Simulator (ACCESS) modelling system. Since its launch in 2022, ACCESS-NRI has focused on modernising climate modelling software and data practices for ACCESS. Guided by the needs of our community, our goal is to make the modelling framework and data outputs more FAIR (Findable, Accessible, Interoperable, and Reusable) and easier to use.  

One of the key challenges in achieving FAIR for ACCESS data is the reliance on often optional post-processing steps to meet most of the FAIR guidelines. While ACCESS model outputs generally follow community standards (e.g., CF-Conventions), their implementation can be inconsistent across modelling components (e.g., atmosphere, ocean, and land models) as well as among individual data generators. As a result, using direct model output data frequently requires users to have previous knowledge and understanding of the specific climate models and leads to significant overheads for compatibility with data discovery and evaluation tools (e.g., Intake, ESMValTool). 

As a new infrastructure dedicated to Australian climate software and data, ACCESS-NRI has a unique opportunity to uplift and directly embed FAIR practices into the climate modelling software components we maintain and support. Building on successes and lessons learned from participation in global intercomparison activities such as CMIP6, ACCESS-NRI is working to apply similar data standardisation practices for the lower-level model outputs in a way that enhances consistency and usability. The effort involves close collaboration with the research community, identifying gaps and commonalities to establish a data specification that can be versioned and linked to future ACCESS model releases. This includes minimum and recommended requirements for file and dataset metadata such as: controlled vocabularies, file and variable naming conventions, provenance statements, and other critical elements to ensure data consistency and usability across all ACCESS components.    

By embedding FAIR principles directly into the ACCESS modelling system, ACCESS-NRI is not only addressing current challenges but is also future-proofing Australia’s climate modelling capabilities to meet the evolving needs of the research community. This approach will make data and tools more accessible, reduce research overheads, and enhance the adaptability of the infrastructure to future changes and new technologies. 

How to cite: Druken, K., Richards, C., Beucher, R., Basevi, J., Bull, C., Carouge, C., Dix, M., Heerdegen, A., Leopardi, P., Marchegiani, D., Nettelbeck, H., Steketee, A., Turner, C., White, M., and Wong, S.: Uplifting and streamlining FAIR data implementation for Australia’s climate modelling outputs, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14828, https://doi.org/10.5194/egusphere-egu25-14828, 2025.

EGU25-16485 | Orals | ESSI3.2

Improving the accessibility of ECMWF open weather forecast data and charts: maintenance challenges 

Milana Vuckovic, Emma Pidduck, Cihan Sahin, and Iain Russell

ECMWF's move towards an extensive free and open data policy is approaching its final phase, extending its user base far beyond operational forecasters in Member and Co-operating States and other licensed customers. Beginning in 2020, the first phase saw the opening of hundreds of web forecast charts (www.charts.ecmwf.int) and made archived data available under a Creative Commons (CC BY 4.0) open licence. This transition continued in January 2022 with the introduction of a free and open subset of real-time forecast data, with ongoing updates incorporating new parameters and datasets. Notably, the latest updates in 2024 included increasing the resolution from 0.4° to 0.25° and including the new Artificial Intelligence Forecasting System (AIFS) forecast data.
This phased move towards free and open data supports the UN EW4All initiative and also aims to support creativity, innovation and reproducibility in scientific research and weather applications. However, this can not be achieved by only opening the real time and archived data. The users need to be able to find and easily use the data and integrate it into their own research work or application workflows.
To address this, additional efforts are underway to improve the data's FAIR (Findable, Accessible, Interoperable and Reusable) attributes. Key developments include the creation of open source Python libraries for data downloading, processing and visualisation under the EarthKit umbrella, alongside the introduction of a set of Jupyter notebooks, each of which is reproducing one open weather forecast chart - from the downloading the data to processing and visualisation.
However, the tools and data constantly change, and keeping up with these changes in the example Jupyter notebooks presents a significant challenge if not designed with the maintenance in mind.
This talk will provide an overview of the open forecast web charts and the use of Jupyter notebooks for their reproduction, followed by an exploration of the maintenance challenges and future plans.

How to cite: Vuckovic, M., Pidduck, E., Sahin, C., and Russell, I.: Improving the accessibility of ECMWF open weather forecast data and charts: maintenance challenges, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16485, https://doi.org/10.5194/egusphere-egu25-16485, 2025.

EGU25-19266 | Posters on site | ESSI3.2

Establishing FAIRness through all-actor approaches to data pipelines: Frameworks for successful development of data standards and pipelines at the UK’s National Centre for Atmospheric Sciences 

Graham Parton, Barbara Brooks, Wendy Garland, Joshua Hampton, David Hooper, Nicholas Marsden, Hannah Price, Hugo Ricketts, Dave Spronson, Ag Stephens, and Chris Walden

The FAIR data principles are a common theme in many discussions and focus of work within research data management. Such work often focuses on particular parts of the data management lifecycle, for example: FAIR through data management planning, FAIR through data discovery and, more recently, areas of FAIR as applied to software and machine learning. 

However, whilst there are many successful attempts at enhancing metadata and data FAIRness for specific parts of the data lifecycle, there may be issues that only arise when considering the overall interconnections between the various stages and the associated actors. For example, a domain may follow common file and metadata conventions for data interoperability, such as CF conventions, enabling research to take place utilising multiple data sources, but pertinent metadata to long-term curation or wider end-usability may not be presented or indeed captured at source. This can have ongoing issues around the level that wider (true?) FAIRness that can be reached and present additional overheads for other actors wishing to handle such data resources, such as manual effort needed for full long-term curation or missed opportunities for data re-use in other spheres.

Recognising these issues and, crucially,  the interplay between all actors along the data lifecycle, the UK’s National Centre for Atmospheric Science (NCAS) have developed the frameworks to ensure all actors’ needs are considered. These are succinctly captured in the ‘NCAS Data Pyramid’, where each corner represents a given actor (data provider, long-term archive, those creating tools aiding data flows and utilisation, end-user community), whilst the sides explore the interconnections between these actors. All parts of the pyramid (corners and sides) provide a range of use-cases and requirements that need to be supported. This approach has enabled NCAS to then develop a range of data standards to enhance data FAIRness for surface and remote sensing data (including from ships and aircraft), imagery data and, in due course, laboratory data.

Furthermore, to aid establishing new data standards NCAS has developed data standards development framework, utilising the ‘Scope -> Define -> Develop -> Sustain’ data standard lifecycle:

  • Scope: Identify community groups. Assess their needs. Determine the scope for the standard.
  • Define the standard by: ensuring all stakeholder needs are covered; defining user-focused data products that it will deliver; and the underpinning standards to be drawn on for wider interoperability. 
  • Develop: provider tools (including checkers for compliance); data delivery pipelines (including those workflows to capture internal/external metadata required for data use/contextualisation of data (e.g. project info); develop end-user data exploitation(visualisation) tools
  • Sustain: having developed standards and workflows have a governance structure to maintain and manage future iterations of the standards development cycle. This must ensure that it refers back to the community groups (as in step 1). 

The approach also keeps wider inter-standards interoperability a key focus throughout. The success of this approach is demonstrated through the establishment of data pipelines aiding data to flow with associated metadata from provider to end-user and has seen wider adoption of NCAS data standards within the wider atmospheric community.

How to cite: Parton, G., Brooks, B., Garland, W., Hampton, J., Hooper, D., Marsden, N., Price, H., Ricketts, H., Spronson, D., Stephens, A., and Walden, C.: Establishing FAIRness through all-actor approaches to data pipelines: Frameworks for successful development of data standards and pipelines at the UK’s National Centre for Atmospheric Sciences, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19266, https://doi.org/10.5194/egusphere-egu25-19266, 2025.

EGU25-19487 | Orals | ESSI3.2 | Highlight

Challenges and opportunities in implementing open and FAIR data in Intergovernmental Panel on Climate Change (IPCC) Seventh Assessment Report (AR7)  

Xiaoshi Xing, Gian Carlo Delgado Ramos, Azra Alikadic, April Lamb, Martina Stockhause, Lina E. Sitz, and Adam Milward

Intergovernmental Panel on Climate Change (IPCC) authors of assessment reports (ARs) and special reports (SRs) use a huge volume of input data, generate a great deal of intermediate data in the process, and produce a large amount of final data for figures and annexes in the published reports. In previous assessment cycles before the Sixth Assessment Report (AR6), only a limited amount of IPCC data were archived and made publicly available. There was  great progress in the AR6, but many critical data sets were still not properly curated. This resulted in a data rescue effort during the transition from AR6 to AR7, supported by the IPCC and government fundings. The challenges encountered during the data rescue effort included missing or lost data after the report publication, missing data licensing agreements, version control issues, and missing data quality assurance/quality control (QA/QC) so that some data did not match the published figures. Addressing these issues demanded significantly more resources than the regular process to track, retrieve, archive, and resolve the legal and technical issues.

In the Seventh Assessment Report (AR7), IPCC progressively promotes the FAIR data principles (Findable, Accessible, Interoperable, and Reusable) through the IPCC Task Group on Data Support for Climate Change Assessments (TG-Data) and the Data Distribution Centre (DDC) (1, 2). The Working Group Technical Support Units (TSUs) have also designated data specialists in the TG-Data (3). This provides opportunities to support authors in implementing open and FAIR data in IPCC AR7. For example, in Chapter 2 of the Special Report on Climate Change and Cities (SRCities), there is an area of focus on “Data, information, tools accessibility/availability/usability/transparency" (4). By collaborating the TSUs and DDC can provide a coordinated approach that supports authors with training and tools on data workflow, metadata schema, data provenance, licensing and citation, persistent identifiers, etc., to improve the data curation process and to avoid the issues encountered in previous cycles.

References:

  • 1. Intergovernmental Panel on Climate Change. (2023). TG-Data Recommendations for AR7 (1.0). Zenodo. https://doi.org/10.5281/zenodo.10059282
  • 2. Stockhause M, Huard D, Al Khourdajie A, Gutiérrez JM, Kawamiya M, Klutse NAB, Krey V, Milward D, Okem AE, Pirani A, Sitz LA, Solman SA, Spinuso A, Xing X. (2024).  Implementing FAIR data principles in the IPCC seventh assessment cycle: Lessons learned and future prospects. PLOS Climate 3(12): e0000533. https://doi.org/10.1371/journal.pclm.0000533
  • 3. https://www.ipcc.ch/data/ (2025)
  • 4. IPCC Special Report on Climate Change and Cities (SRCities) report outline. (2024). https://www.ipcc.ch/site/assets/uploads/2024/08/IPCC-61_decisions-adopted-by-the-Panel.pdf

How to cite: Xing, X., Delgado Ramos, G. C., Alikadic, A., Lamb, A., Stockhause, M., Sitz, L. E., and Milward, A.: Challenges and opportunities in implementing open and FAIR data in Intergovernmental Panel on Climate Change (IPCC) Seventh Assessment Report (AR7) , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19487, https://doi.org/10.5194/egusphere-egu25-19487, 2025.

EGU25-19699 | Orals | ESSI3.2

Building an EOSC based virtual research environment to support the adoption of FAIR and Open Science practices in Climate Change Adaptation communities 

Raúl Palma, Malgorzata Wolniewicz, Adam Rynkiewicz, José Manuel Gómez, Andres Garcia Silva, Daniel Garijo, Esteban Gonzalez Guardia, and Anne Fouilloux

During the last years, Open Science has been gaining increasing attention from research communities and policy makers because of the benefits it can provide not only to scientists, but also to society in general, as it can accelerate the production of science and the quality of results. Open science is a policy priority for the European Commission (EC) and the standard method of working under its research and innovation funding programmes. Thus, the EC initiated the European Open Science Cloud (EOSC) initiative, which aims to create a virtual environment for sharing and accessing research data across borders and scientific disciplines, aligning with Open Science and FAIR principles. EOSC specified a layered approach with a set of core services at its center, a federated data layer, a rich set of exchange services to expand the capabilities offered to researchers across disciplines, plus a set of thematic/discipline-specific services. To fully realise EOSC’s vision, it is envisioned as a federation of distributed systems, combined into a system of systems, consisting of multiple Nodes’. At the end of last year, the first of such nodes (EOSC EU node) was launched featuring the core services enabling scientific research infrastructures to federate and a set of common exchange “horizontal services” for end-users to benefit from. 

Based on the integration of thematic, horizontal, and core resources, the goal is that EOSC enables the creation of thematic execution environments/VREs. A VRE is an online support system for researchers,  encompassing online tools, network resources and technologies interoperating with each other to ease/enhance the research process within and across institutional boundaries, facilitating collaboration, data management, analysis, and other research-related activities in one online space.

To build an EOSC-based VRE, we have leveraged and integrated different core and exchange services. At the center of the proposed VRE are RO-Crate based research objects (providing an implementation of the FAIR digital object), as well as the associated technological support (provided by ROHub platform), to manage the research lifecycle and the associated scientific resources used and produced. The VRE leverages data cubes services for efficient and scalable structured data access and discovery, AI-based text mining services  that extract machine-readable metadata from scientific resources supporting recommendations and comprehension analysis, and FAIR assessment tools supporting researchers in the FAIRification of their outcomes. Additionally, the VRE relies on EOSC services for authentication and authorization to enable seamless access to different services, the computing platforms to execute computational methods, and data repositories to store and/or share their data in their personal/community workspaces or general repositories. The VRE also connects DMP platforms to enable the creation of machine-actionable plans, and with the scientific knowledge graph to enable the discovery of resources by different communities. In the FAIR2Adapt project, such environment is being enhanced with a set of added-value services (e.g., search and discovery using NL questions, multilingual semantic enrichment, sentence detection, FAIRness-aware search and recommendations, and multilingual generative question answering) and adapted to boost FAIR adoption in Climate Change Adaptation communities and research.

How to cite: Palma, R., Wolniewicz, M., Rynkiewicz, A., Manuel Gómez, J., Garcia Silva, A., Garijo, D., Gonzalez Guardia, E., and Fouilloux, A.: Building an EOSC based virtual research environment to support the adoption of FAIR and Open Science practices in Climate Change Adaptation communities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19699, https://doi.org/10.5194/egusphere-egu25-19699, 2025.

Assessing the status and trends of water quality in inland water bodies requires access to reliable water quality monitoring data and associated metadata such as the monitoring locations, sampling methods, monitoring equipment and analytical methods. Many environmental agencies and research organizations collect water quality monitoring data, but unlike in other environmental domains and due to a lack of common best practices and standards, most organizations use their own data models, formats and controlled vocabularies to store and share these data. As a result, large-scale water quality analyses with a transboundary, continental or global scope require significant efforts to collect the necessary monitoring data from different sources and to harmonize the different data structures. Several international initiatives such as the UNEP Global Environment Monitoring System for Freshwater (GEMS/Water)1 or research activities such as the Global River Water Quality Archive (GRQA)2 have compiled global water quality datasets to facilitate large-scale hydrological studies, all facing the same challenges and often duplicating data processing efforts.
Over the last 20 years, the observing community has developed data models and semantic ontologies such as the OGC Observations, Measurements, and Samples (OMS)3 standard or the OGC/W3C Semantic Sensor Network (SSN)4 ontology to describe observations and associated metadata. These form the basis of several standards for the exchange of hydrological observation data such as the WaterML 2.0 family of standards. However, water quality specific aspects such as the description of sampling activities and associated metadata have not yet been included in these water specific standards. 
To address this issue, several government agencies and research organizations have started a Water Quality Interoperability Experiment (WQIE) within the Open Geospatial Consortium (OGC) in 2022. Several use cases for the exchange of water quality monitoring data of physical and chemical parameters monitored in surface and groundwater bodies using in-situ (sensor) or ex-situ (laboratory) monitoring were developed and described as object diagrams in UML based on the OMS conceptual model. Based on this exercise, a physical data model was developed by extending the OGC SensorThingsAPI (STA)5 with a plugin for the open source FROST server6. Several WQIE participants deployed pilot instances of water quality enabled FROST servers, making their water quality data publicly available. A web client was developed to facilitate access to the various STA endpoints and to enable data visualisation7
This presentation will give an overview of the developments of the OGC Water Quality Interoperability Experiment, highlighting achievements, outstanding challenges and future development plans. 

References:

1 https://www.unep.org/explore-topics/water/monitoring-water-quality

2 Virro, H., Amatulli, G., Kmoch, A., Shen, L., and Uuemaa, E.: GRQA: Global River Water Quality Archive, Earth Syst. Sci. Data, 13, 5483–5507, https://doi.org/10.5194/essd-13-5483-2021, 2021.

3 https://docs.ogc.org/as/20-082r4/20-082r4.html

4 https://www.w3.org/TR/vocab-ssn/

5 https://www.ogc.org/publications/standard/sensorthings/

6 https://github.com/hylkevds/FROST-Server.Plugin.WaterQualityIE/tree/main

7 https://api4inspire.k8s.ilt-dmz.iosb.fraunhofer.de/servlet/is/226/ 

How to cite: Heinle, M. and Saile, P.: A step towards FAIR water quality data – lessons learned from the OGC Water Quality Interoperability Experiment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19719, https://doi.org/10.5194/egusphere-egu25-19719, 2025.

Since their development, the FAIR principles have been met with broad acceptance in the scientific community. Tools based on various approaches are available to assess the FAIRness of individual data sets. These range from qualitative assessments based on questionnaires to automated quantitative measurements of fairness. As the FAIR principles are rather vaguely formulated, these approaches are based on individual, often differing, interpretations of the FAIR principles. In addition, the authors of the FAIR principles explicitly recognize the different implementations of FAIR within the various specialist communities. This makes it necessary to develop community-specific metrics and tests and to adapt FAIR assessment tools accordingly.

This diversity of methods for assessing FAIR is encouraging, as it sheds light on a variety of aspects of FAIR. However, this also sometimes leads to different, divergent results from these tools, which is difficult for users to work with. In addition, the measurement of FAIRness of individual datasets is heavily dependent on various technical implementations on the part of the data providers and their service providers. Numerous, possibly unintentional restrictions on the accessibility of datasets can influence or falsify FAIR measurements. 

In this presentation, we would like to report on our experiences with the applied FAIR assessment within this context. We will report on the further development of F-UJI, in particular our experiences with discipline-specific FAIR metrics and their implementation. Furthermore, we will discuss the limitations of FAIR measurements and try to delineate FAIR from aspects of data quality and accessibility and how to derive informative holistic assessments of datasets that include all these aspects in the future.

How to cite: Huber, R.: Opportunities and limitations of applied FAIR evaluation of data sets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20064, https://doi.org/10.5194/egusphere-egu25-20064, 2025.

EGU25-20123 | Orals | ESSI3.2

Automatic annotation following the I-ADOPT framework 

José Manuel Gómez Pérez and Andrés García

The fulfillment of the FAIR principles is a central requirement in modern research. Data findability and reusability are highly dependent on the quality and interoperability of their metadata. Among other attributes in earth and environmental sciences, FAIR metadata should ensure consistent and uniquely referenceable naming of geoscientific variables that support machine-interpretable semantic annotations. But in practice, most terminologies used to describe datasets and observed variables vary wildly in their granularity, quality, governance and interconnectivity which, in turn, limits their interoperability. The RDA endorsed I-ADOPT Framework addresses this issue by breaking down descriptions of observed variables into five well-defined atomic components ObjectofInterest, Property, Matrix, Constraint and Context anticipating their annotation with generic terms from FAIR semantic artefacts. As of today, the I-ADOPT decomposition is still a highly manual process that requires semantic and domain skills. Here, we propose the application of Large Language Models (LLM) to transform scientific terms into I-ADOPT-aligned descriptions. This model will enable the transformation into machine-interpretable representations by simply using natural language descriptions of observational research provided by domain experts. We will leverage the existing set of high-quality, human-made formalizations of I-ADOPT variables to adjust the LLM for this task. We will consider LLM in zero-shot scenarios where the LLM is used in its pretrained version and in-context learning where the LLM sees some examples of the task. We will also consider training specialist LLM where the LLM is further fine-tuned for this task, although the success of this approach depends on the amount of training data available. For developing this model and a first demonstrator, we will build on our previous experience in developing the I-ADOPT Framework, in transfer learning and fine-tuning neural networks, FAIR data stewardship, research data infrastructures and research software engineering. Our project will be further linked to several other ongoing activities and initiatives both on a national and also European level, which allows us to directly evaluate the performance of our LLM by potential end-users and communities. Such a service will be integrated into platforms like RoHub to help scientists make research datasets FAIR.

How to cite: Gómez Pérez, J. M. and García, A.: Automatic annotation following the I-ADOPT framework, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20123, https://doi.org/10.5194/egusphere-egu25-20123, 2025.

EGU25-20132 | Orals | ESSI3.2

How domain repositories support reusable data: metadata tools from GFZ Data Services 

Marcel Meistring, Holger Ehrmann, Jana Franz, Simone Frenzel, Ali Mohammed, and Kirsten Elger

The availability of reusable data and their associated metadata is increasingly demanded to address global societal challenges. Research data repositories and databases are the primary access points for geosciences data, and especially domain repositories are known to publish well documented and reusable data. This is due to a thorough data and metadata curation provided by the repository staff that usually includes domain scientists. Overall, the documented publication of a complex data set via a domain repository often takes time and additional preparation by the scientists, but the results clearly show a significant increase of the metadata and data quality, including the provision of cross-references to other publications, datasets, code and originating physical samples.

The largest challenge for domain repositories is to provide incentives to the researchers that reduce their workload and in the same time ensure a high quality of metadata and data documentation already at an early stage of a planned data publication. This challenge is especially high in repositories with a focus on the highly variable and usually small data from so-called “long-tail communities”. GFZ Data Services is a domain repository for DOI-referenced geosciences data and scientific software, hosted at the GFZ Helmholtz Centre for Geosciences. The repository has both a focus on the curation of long-tail data, and offers data publication services for international projects and services in the geosciences. To support researchers with the provision of descriptive metadata and receive structured data documentation, GFZ Data Services has developed an online metadata editor and data description templates. This presentation will focus on these support tools and demonstrate how both help the researchers and in the same time reduce the data curation workload.

A major focus will lay on our new metadata editor that is currently jointly developed between the University of Applied Sciences Potsdam and GFZ Data Services. The new metadata editor will enhance the support of users in data entry, so that the manual curation effort by the GFZ Data Services is reduced, and the metadata quality is improved at the same time. Technically, it has a responsive design and offers a dark mode. New facets include the ability to retrieve specific information, e.g., affiliations from the ROR API via a dropdown menu. Keywords are made uniquely identifiable through the automatic storage of schema names and uniform resource identifiers of the specific terms. All integrated thesauri can be updated via API calls. Real time validation of the input fields prevents the submission of incomplete or incorrect entries, so that significantly less work is required in data curation. The integrated help guide supports users to fill in the input fields.

The data description templates collect additional technical description in a structured form and are essential for data reuse. They are available in “commented” and “usable” versions and ensure that the descriptions meet our requirements (for many researchers the data documentation is new), offer clear instructions and even reduce the workload of the curators, because the descriptions are already provided at a very high level of content.

How to cite: Meistring, M., Ehrmann, H., Franz, J., Frenzel, S., Mohammed, A., and Elger, K.: How domain repositories support reusable data: metadata tools from GFZ Data Services, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20132, https://doi.org/10.5194/egusphere-egu25-20132, 2025.

The Intergovernmental Panel on Climate Change (IPCC) Data Distribution Centre (DDC) serves as a critical registry for climate change data, providing a shared infrastructure to ensure data quality and accessibility for the scientific community. Managing data to support IPCC reports presents challenges due to its multidisciplinary nature and diverse sources.

Key to this effort is the curation of metadata, particularly developing a metadata schema that enables data to be FAIR (Findable, Accessible, Interoperable, and Reusable). This presentation examines the IPCC's experience over the past four years in curating and preserving digital objects, focusing on the implementation of FAIR and open data principles. We will explore the successes and setbacks of the AR6 experience, with particular attention to the development and application of a metadata schema. Finally, we will offer recommendations for consolidating and expanding this approach for AR7 to enhance transparency, reproducibility, and reusability of assessment outcomes.

This initiative aims to increase the transparency of IPCC's work, improve the reproducibility and reusability of assessment outcomes, optimize the utilization of the IPCC DDC's services, and promote compliance with open science best practices.

How to cite: Milward, D., Milward, A., and Xing, X.: Managing a FAIR Climate Change Data Catalogue: Lessons Learned from IPCC AR6 and Recommendations for AR7, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20454, https://doi.org/10.5194/egusphere-egu25-20454, 2025.

EGU25-20583 | Orals | ESSI3.2

International Earth, space, and environmental coordination of data and software management efforts 

Shelley Stall, Danie Kinkade, Natalie Raia, Lesley Wyborn, and Pedro Corrêa

The international Earth, space, environmental sciences informatics community has recently formed a new Research Data Alliance Community of Practice. Here we are focused on improving data and software management and sharing practices that result in our researchers having access to community informatics resources that support their research.  This community of practice will provide a place for teams and organizations in the Earth, space, and environmental research ecosystem to coordinate on common challenges, share information, review and consider RDA recommendations, seek leading practices, and work towards finding approaches to discipline-specific challenges and issues around data and software management and sharing. The international Earth, space, and environmental community is broad and includes researchers, data managers, data curators, institutions, instrument creators and manufacturers, software developers, tools, repositories, journal editors and more. 

An RDA community of practice is where those with common interests can collaborate on complex challenges that need multiple stakeholders to work through the layers of a solution. It is a place where projects can be highlighted and shared for the benefit of building collaboration and connection.     

Join us for this session and learn more about how we envision supporting the many global data and software management efforts.

How to cite: Stall, S., Kinkade, D., Raia, N., Wyborn, L., and Corrêa, P.: International Earth, space, and environmental coordination of data and software management efforts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20583, https://doi.org/10.5194/egusphere-egu25-20583, 2025.

EGU25-21162 | Posters on site | ESSI3.2

Implementing FAIR Principles for Earth System Data: Insights from the European Eddy-Rich Earth-System Models (EERIE) project 

Heinrich Widmann, Chathurika Wickramage, and Fabian Wachsmann

We attempt to make EERIE data FAIR (Findable, Accessible, Interoperable, and Reusable) to enhance its scientific impact and utility. These principles of FAIRness ensure global access, integration, and reuse by researchers and decision-makers, thereby promoting collaboration and innovation.

Findability is enhanced through persistent identifiers such as DOIs and PIDs, ensuring data remains reliably locatable. Metadata standards, including CF conventions and CMIP standard names, ensure precise and efficient searchability. We enhance findability through data catalogs produced in the EERIE and nextGEMS projects, as well as platforms like World Data Center for Climate (WDCC) and DOKU. The WDCC ensures long-term storage with a focus on FAIRness, quality control, and DOI assignment following CF standards. Our EERIE data is also archived on DOKU with PIDs to ensure discoverability.

Accessibility is ensured by providing data through open protocols with clear terms of use. While accessibility does not always mean free access, it guarantees transparency and ease of use. Open-access repositories such as EERIE Cloud, Earth System Grid Federation (ESGF), and, WDCC combination with standardized formats such as NetCDF and Zarr, ensure broad accessibility. Additionally, tools like Zarr provide API access via HTTP, facilitating seamless and efficient data retrieval.

Interoperability is fundamental for integrating datasets across disciplines and platforms. The EERIE project supports this by linking datasets through initiatives such as EERIE Cloud, FREVA and by using standards such as CF conventions to ensure compatibility, facilitating multidisciplinary research.

Reusability is supported through detailed metadata, clear licensing models like CC-BY and CC0, and strong version control practices (e.g, v20240304). Documentation platforms such as easy.gems.dkrz.de assist users to understand and reproduce results. The maintenance of high data quality and the emphasis on archival and replication further enhance the long-term scientific use of these datasets.

Despite these efforts, the implementation of the FAIR data principles in a comprehensive manner poses significant challenges. In the EERIE project, for instance, we work with vast amounts of data, and standardizing it (e.g., CMORizing) can be complex. Obtaining CF-compliant names for all variables is particularly difficult, as there is often no one-to-one documentation from modeling groups. In some cases, this requires manually analyzing code to determine the correct definitions for certain variables.

For climate science, the application of FAIR principles is transformative. These efforts promote global collaboration, enhance the transparency of climate models, and equip policymakers with reliable data to address critical challenges such as climate adaptation and mitigation. Initiatives like EERIE cloud, ESGF and advancements in data processing, such as kerchunking massive datasets, further enhance the FAIRness of climate data, driving innovation and impact.

How to cite: Widmann, H., Wickramage, C., and Wachsmann, F.: Implementing FAIR Principles for Earth System Data: Insights from the European Eddy-Rich Earth-System Models (EERIE) project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21162, https://doi.org/10.5194/egusphere-egu25-21162, 2025.

EGU25-21472 | Orals | ESSI3.2

Community Support and Engagement for FAIR Science in Climate Change Adaptation 

Erik Schultes and Barbara Magagna

Global climate change requires urgent and actionable adaptation planning.

Current Climate Change Adaptation (CCA) strategies often lack the necessary data and other relevant information to be scientifically competent. These limitations can complicate effective action and evaluation locally, and in combination with other regions. The recently awarded FAIR2Adapt Project aims to establish a comprehensive FAIR and open data framework for CCA and to demonstrate the impact of FAIR data on CCA strategies. By making CCA data FAIR, FAIR2Adapt will accelerate adaptation actions that are tailored to local needs.

Next to the technical development of FAIR data and services, a key issue in the effective uptake  of FAIR is the transfer of knowledge regarding FAIR practices, and in many cases hands-on skills related to the design, creation and governance of domain-relevant FAIR Enabling Resources.  Beginning in February 2025, the FAIR2Adapt, stakeholders (including members of it’s six use cases) will participate in FAIR awareness and training based on the GO FAIR Foundation’s FAIR Capacity Building Programme [https://zenodo.org/records/14187859]. This will include general FAIR Awareness workshops, training on the creation of FAIR Implementation Profiles and community-specific metadata and vocabulary in Metadata for Machine workshops. In addition to this, special attention will be given to the identification and prioritization of user requirements (both the technical approach in FAIR2Adapt as well as the case studies). Having both the technical expertise and building up the salient knowledge and skills, the FAIR2Adapt community will be well positioned to co-design, implement and share CCA related data and services that can accelerate meaningful and customized CCA. In this presentation, we will report the first draft user requirements for FAIR2Adapt and the emerging list of CCA community-specific FAIR Enabling Resources.  

 

How to cite: Schultes, E. and Magagna, B.: Community Support and Engagement for FAIR Science in Climate Change Adaptation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21472, https://doi.org/10.5194/egusphere-egu25-21472, 2025.

EGU25-21516 | Orals | ESSI3.2

Advancing Data Infrastructure for Chemical Risk Assessment and Exposome Research: The GENASIS Platform in the Context of FAIR Principles 

Katarína Řiháčková, Jana Borůvková, Zdenka Bednářová, Richard Hůlek, and Jana Klánová

Excellence in exposome research and chemical risk assessment (CRA) relies on robust capacities, innovative technologies, and skilled human resources. Research infrastructures are vital in providing access to these resources and driving innovation. Over recent decades, Europe has developed numerous research infrastructures, including EIRENE RI (Research Infrastructure for Environmental Exposure Assessment in Europe), the first EU research infrastructure dedicated to the human exposome. EIRENE RI aims to integrate interdisciplinary data, offering harmonized workflows and services to users across various sectors. Other initiatives, such as the Partnership for the Assessment of Risks from Chemicals (PARC), work on advancing harmonization and innovation in CRA.

A robust data infrastructure aligned with FAIR data and Open Science principles is essential for these research infrastructures. Mapping and evaluating the current data landscape is a critical step toward enhancing FAIR implementation and machine actionability. This contribution highlights existing strategies for harmonizing and managing global data on chemical occurrences developed through two decades, using the use case of the GENASIS information system.

GENASIS information is a platform originally developed for storing, harmonizing, and visualizing global environmental monitoring data. Over time, it has expanded to include data on chemical occurrences in indoor environments, consumer products, and human matrices. Today, it hosts over 3 million harmonized records on more than 800 chemicals, described with rich metadata, and it is continuously expanding. This enables the identification of gaps, locality comparisons, and evaluation of global trends in chemical concentrations in the environemnt and humans. GENASIS also serves as a model and sister database for the Global Monitoring Plan Data Warehouse of the Stockholm Convention and supports the United Nations Environment Programme in managing environmental and human monitoring data to evaluate the effectiveness of global treaties on chemical pollutants. GENASIS’ ongoing development and associated services contribute to the European Open Science Cloud (EOSC) in the Czech Republic, EIRENE RI and PARC initiatives.

This contribution evaluates GENASIS in terms of FAIR principles, detailing its current status, roadmap for further FAIR implementation, efforts to enhance machine actionability, and challenges encountered. The discussion is framed within the broader context of initiatives such as PARC, EIRENE RI, and EOSC CZ, emphasizing their role in advancing exposome research and CRA in Europe.

Acknowledgement: This project was supported from the European Union’s Horizon 2020 research and innovation programme under grant agreement No 857560 (CETOCOEN Excellence), and from the Horizon Europe programme under grant agreements No 101057014 (PARC) and 101079789 (EIRENE PPP). Views and opinions expressed are however those of the author(s) only and do not necessarily reflect those of the European Union, European Health and Digital Executive Agency (HADEA) or European Research Executive Agency (REA). Neither the European Union nor the granting authorities can be held responsible for any use that may be made of the information it contains. Authors thank the RECETOX Research Infrastructure (No LM2023069) financed by the Ministry of Education, Youth and Sports.

How to cite: Řiháčková, K., Borůvková, J., Bednářová, Z., Hůlek, R., and Klánová, J.: Advancing Data Infrastructure for Chemical Risk Assessment and Exposome Research: The GENASIS Platform in the Context of FAIR Principles, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21516, https://doi.org/10.5194/egusphere-egu25-21516, 2025.

EGU25-21605 | Orals | ESSI3.2

Status, issues and challenges with FAIRness of seismological waveform data and beyond 

Florian Haslinger, Lesley Wyborn, Rob Casey, Helle Pederson, Elisabetta D’Anastasio, Javier Quinteros, Jonathan Hanson, and Jerry Carter

Driven by the scientific need for global exchange of data to study earthquakes and related phenomena, community standards and best practices have evolved in seismology for decades. These developments are largely driven by operational and scientific requirements coming directly from the community of academic research and seismological monitoring, and have resulted in standardised data formats, data models and services for data access and exchange.

Initial developments, promotion and further evolution of these standards are coordinated mainly within the International Federation of Digital Seismic Networks (FDSN, https://fdsn.org), a commission of IASPEI (International Association of Seismology and Physics of the Earth's Interior, httwww.iaspei.org) that is one of eight associations of the IUGG (International Union of Geodesy and Geophysics, https://iugg.org).   

With the introduction of the FAIR (Findable, Accessible, Interoperable, Reusable) principles in 2016 and the subsequent appearance of FAIR assessment methods and tools it became clear that these seismological community standards only cover parts of the FAIR principles. Interoperability remains challenging, for example, due to the lack of community standardised FAIR vocabularies, and the lack of a harmonised and consistently applied data license policy impacts Reproducibility.

The emergence of new data types and the drastic increase in data volumes due to new measurement techniques require updates and evolution of the existing community standards, highlighting another general challenge:  Who are the recognised and appropriate governance bodies for curation and further development of 'relevant community standards' (as required by the FAIR principles)?

In this presentation we describe the current status of FAIRness for seismological waveform data and beyond, also looking towards seismology in general, geodesy and some other fields of geophysics. Based on our assessment of current challenges we discuss open questions and possible ways forward. We look at FAIR-relevant development and governance of standards, the potential role of existing international organisations like FDSN, IASPEI and IUGG, and the possibility and need to coordinate across domains for harmonisation as well as demarcation.   

How to cite: Haslinger, F., Wyborn, L., Casey, R., Pederson, H., D’Anastasio, E., Quinteros, J., Hanson, J., and Carter, J.: Status, issues and challenges with FAIRness of seismological waveform data and beyond, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21605, https://doi.org/10.5194/egusphere-egu25-21605, 2025.

Integrating High-Performance Computing (HPC) and cloud computing in climate sciences is difficult, due to intricate hardware/software, compatibility, performance and reproducibility issues. Here, we address these challenges in a user-friendly way by leveraging the Conda ecosystem and containers.

Containerization allows to match or exceed native performance on HPC while ensuring bit-for-bit reproducibility for deterministic algorithms and similar processor architectures. This approach simplifies deploying climate models across different platforms; for example, CESM 2.2.2 (Community Earth System Model) provides on various clusters throughputs in simulated years per computational day within +/- 1% of bare-metal performance for simulations spanning thousands of processors.

Exclusively using generic Conda packages for MPI (Message Passing Interface) applications was challenging in HPC. Although OpenMPI included UCX (Universal Communication X) and OFI (Open Fabric Interface), it lacked UCC (Unified Collective Communication) and wasn't optimized by default for high-performance networks like InfiniBand, RoCE (Remote Direct Memory Access over Converged Ethernet) and HPE (Hewlett Packard Enterprise) Slingshot-11, often defaulting to TCP/IP (Transmission Control Protocol/Internet Protocol) or failing. 
 
After updating Conda-Forge’s OpenMPI and MPICH feedstocks, we are adding MVAPICH and ParaStationMPI support to PnetCDF, HDF5, NetCDF-C, NetCDF-Fortran and ESMF (Earth System Modeling Framework) libraries critical for modellers, alongside libFabric and openPMIx (Process Management Interface - Exascale). This incidentally exposed ABI (Application Binary Interface) compatibility issues. Now, MPI toolchains featuring major UCX/OFI/PMIx versions ensure consistent operation across different hosts without affecting numerical results. Using the same Conda environment inside a container, and no hardware-specific optimization, preserves bitwise reproducibility. OMB (Ohio State University Micro-Benchmark) tests for latency, bandwidth and other metrics help confirm if optimal performance can be achieved or not. 

Such developments enable climate scientists to focus on addressing scientific questions rather than sorting out software dependencies and technical problems. One can write code on a laptop then effortlessly scale to cloud or supercomputers, and seamlessly run climate simulations somewhere then continue these wherever compute resources are available without worrying about discontinuities. This also releases expensive HPC resources for production instead of wasting them for training, learning, development or testing which can be performed comfortably elsewhere, without job scheduling constraints, in the very same software environment.

Conda has primarily been developed with a focus on compatibility which limits its suitability in highly performance-sensitive applications where locally optimized builds of specific key components are paramount, typically in climate modeling. Additionally, instead of relying on local engineers to install and maintain host software, Conda users can benefit from the work of thousands of open-source contributors who continuously update and test the entire ecosystem.

This strategy fits the session's theme by providing a framework where cloud resources can be utilized for big data without compromising the performance or rigor of HPC environments. Conda and container technologies ought to change how climate scientists approach software management, focusing on ease of use, scalability and reproducibility, thereby potentially altering practices within the field to improve usage of computational resources and leverage community efforts to remain at the forefront.

How to cite: Iaquinta, J., Fouilloux, A., and Ragan-Kelley, B.: Climate Modeling with Conda and Containers to Improve Computational Resource Usage while Achieving Native Performance and Reproducibility, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2605, https://doi.org/10.5194/egusphere-egu25-2605, 2025.

EGU25-6798 | Orals | ESSI2.15

Advancing Geophysical Data Analysis: HEALML for Efficient Sphere-Based Statistics on Pangeo-EOSC 

Jean-Marc Delouis, Erwan Allys, Justus Mangin, Louise Mousset, and Tina Odaka

A significant challenge in data integration and ML methodologies on cloud infrastructures is accurately determining correlated statistics. Initially, aligning data to a consistent pixel grid is essential, motivating the use of Discrete Global Grid Systems (DGGS). In geophysical studies, data reside on a sphere, and approximating with tangent planes can distort results. Our solution is the HEALPix pixelization as our DGGS framework, standardizing data on a common grid for consistent statistical analysis. HEALPix's unique features, such as its iso-latitude layout and uniform pixel areas, enable the use of spin-weighted spherical harmonics in managing vector fields. This enables the accurate calculation of  correlation statistics, such as between velocity and scalar fields on the sphere, while minimizing biases due to spherical approximations. By utilizing the HEALPix framework, known in cosmology, with TensorFlow or PyTorch as backends, we created the: HEALML library. This library facilitates gradient computations of all derived statistics for AI optimization, and has been validated on the Pangeo-EOSC platform. This library parallelizes the computation of localized spherical harmonics and includes features like scattering covariance calculations, allowing the extraction of more complex nonlinear statistics beyond the power spectrum. We compare these results to traditional 2D planar methods, demonstrating the advantages of sphere-based statistics on platforms like Pangeo-EOSC. Furthermore, we demonstrate: HEALML's ability to emulate using a substantially smaller dataset. This demonstration emphasizes the ways in which incorporating spherical statistical methods into Pangeo-EOSC fosters innovative and efficient statistical analysis within geophysical research.

How to cite: Delouis, J.-M., Allys, E., Mangin, J., Mousset, L., and Odaka, T.: Advancing Geophysical Data Analysis: HEALML for Efficient Sphere-Based Statistics on Pangeo-EOSC, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6798, https://doi.org/10.5194/egusphere-egu25-6798, 2025.

EGU25-8127 | ECS | Posters on site | ESSI2.15

Seamless Upscaling Research from Cloud to HPC using eWaterCycle 

Mark Melotto, Rolf Hut, and Bart Schilperoort

The eWaterCycle platform provides hydrologists with a platform that allows them to work with each other's models and data without having to become a computer scientist in the process. The eWaterCycle platform supports existing hydrological models and makes them available for scientists using the BMI model interface as a communication layer. Models run in containers for reproducibility and dependency control. Popular hydrological models are readily available (PCRGLobWB, WFLOW, HBV, etc.). Scientists develop their analyses or experiments in the widely known JupyterHub environment. 

While in theory eWaterCycle can be installed and run on any hardware, in practice most users interact with it on the SURF Research Cloud, a cloud computing infrastructure available to the Dutch academic ecosystem. Until recently upscaling from Cloud to HPC infrastructure for larger model runs required extensive knowledge of the HPC system. Here we will present our work on building a seamless workflow that allows scientists to upscale their cloud based work to the Snellius supercomputer and the Spider grid computer without having to worry about technical issues like mounting points for (large) datasets and container engines.

Our workflow opens up the possibility for more scientists to benefit from HPC and Grid resources while focussing on their domain science. We present the workflow in such a format that it should be easily portable to other hybrid cloud - HPC infrastructures, including the DestinE systems.

How to cite: Melotto, M., Hut, R., and Schilperoort, B.: Seamless Upscaling Research from Cloud to HPC using eWaterCycle, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8127, https://doi.org/10.5194/egusphere-egu25-8127, 2025.

We present recent progress around the EERIE cloud data server (https://eerie.cloud.dkrz.de) and its software stack “cloudify”. The EERIE cloud provides efficient open access to prominent climate datasets stored on disk at the German Climate Computing Center (DKRZ).

A new kerchunk-plugin enables data access to raw model output as-is to enable verifiable data transfer with better latency. STAC (Spatio Temporal Assets Catalog) catalogs are deployed and displayed through the EERIE cloud to make the provided DKRZ datasets findable and accessible. Two in-browser apps can be started, pre-configured for each dataset, by just clicking buttons: (1) the data visualization app “gridlook” as well as a (2) jupyterlite for interactive analysis and monitoring. 

We leverage the python package xpublish, a plugin for Pangeo's central analysis package Xarray. Its main feature is to provide ESM output by mapping any input data to virtual zarr datasets. Users can retrieve these datasets as if they were cloud-native and cloud-optimized.

How to cite: Wachsmann, F.: The EERIE cloud: Apps and Catalogs for Cloudified Earth System Model Output, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8591, https://doi.org/10.5194/egusphere-egu25-8591, 2025.

EGU25-8754 | ECS | Orals | ESSI2.15

Leveraging Cloud, Earth Observation and In-Situ Sensors for Agri-Environmental Monitoring and Policy Decision-Making  

Georgios Charvalis, Panagiota Louka, Vassileios Gkoles,  Thanasis Manos, Nikos Kalatzis, Dionysios Solomos, Anastasios Trypitsidis, and Odysseas Sekkas

Cloud infrastructures play a significant role in delivering secure, scalable and efficient data processing for Earth Observation (EO) and agricultural management applications. As part of the ScaleAgData project, we present a hierarchical Agri-Environmental Monitoring Tool running on a private cloud infrastructure. The system combines data from EO, in-situ sensors and farm management information systems (FMIS), including parcel calendars, to provide farmers and policymakers multi-scale insights.  

The solution is cloud-based and designed with an underlying architecture that ensures both scalability and interoperability, leveraging OGC-compliant data formats where applicable. EO and in-situ data streams can be processed and analyzed efficiently with the help of containerized apps and microservices to facilitate modular development and simplify deployment. By using a web-based dashboard with hierarchical design, stakeholders can navigate from overviews at the municipal level to individual parcels. Aggregated summaries that comply with Common Agricultural Policy (CAP) criteria are useful to policymakers and farmers can get comprehensive parcel-level metrics to optimize irrigation, pesticide use and other agro-related activities.  

Specifically, the tool combines EO data to derive vegetation indices (e.g., NDVI, EVI) and other parameters requiring advanced processing for crop type classification. Furthermore, these datasets are enriched with in-situ sensor measurements (e.g. soil moisture, weather data) and farm logs managed within FMIS (irrigation schedule, pesticide usage). Parcel-level data (L1) is processed to generate statistics, which are then calibrated with nearby parcels data with similar properties and crop type(L2), serving as control level, and finally extrapolated to the municipal level (L3) using spatial averaging techniques  to provide indicators related to irrigation water, pesticide, fertilizer usage, etc.  Farm calendars stored within FMIS provide a reliable source of ground-truth data, enhancing the tool’s ability to validate aggregated metrics. The aggregation at L2 and L3 allows for the identification of regional trends and patterns in agricultural practices, empowering policymakers and stakeholders to implement targeted interventions at both levels, thereby promoting sustainable agriculture.   

This work showcases the potential of private cloud infrastructures to enhance agri-environmental monitoring by processing and integrating heterogeneous data streams (EO, in-situ sensors and farm log data) into a unified system. The system is being applied in diverse agricultural regions of Greece (Crete, Thessaly, Macedonia) with ongoing validation efforts aimed at refining its accuracy and adaptability. Future work includes the integration of cloud-based machine learning models and EO-derived evapotranspiration data to enhance the efficiency of extrapolating parcel-level (L1) and regional (L2) metrics into policy-level indicators (L3). Additionally, alternative aggregation methods, such as model-based approaches, spatial regression, and interpolation techniques like Kriging, will be tested to improve the accuracy and reliability of aggregated insights. 

How to cite: Charvalis, G., Louka, P., Gkoles, V., Manos,  ., Kalatzis, N., Solomos, D., Trypitsidis, A., and Sekkas, O.: Leveraging Cloud, Earth Observation and In-Situ Sensors for Agri-Environmental Monitoring and Policy Decision-Making , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8754, https://doi.org/10.5194/egusphere-egu25-8754, 2025.

EGU25-9432 | Posters on site | ESSI2.15

Co-Creating Cloud-Based Tools for Urban Climate-Resilience: The CLIMRES Project 

Claudio Pisa, Marica Antonacci, Vasileios Baousis, Sotirios Aspragkathos, Iasonas Sotiropoulos, and Stamatia Rizou

Europe faces a growing frequency of extreme weather events, from heatwaves and floods to wildfires and earthquakes, increasingly threatening urban environments. Unusually warm winters are becoming progressively common, destabilizing ecosystems and altering traditional weather dynamics. 

Addressing these crucial changes, the CLIMRES project aims to foster a “Leadership for Climate-Resilient Buildings” by identifying and categorizing vulnerabilities within the built environment and assessing their effects within urban systems. This effort integrates diverse data sources, including Copernicus services, IoT networks, and municipal datasets, and considers hazard warnings and weather forecasts. Moreover, a liaison with the Destination Earth initiative enhances the project with the capacity to leverage extreme weather predictions and future climate models. 

CLIMRES aims to deliver vulnerability assessment and impact evaluation methodologies, along with a “hub of measures” inventory for cost-effective building design and materials against climate risks, as well as decision support tools, to aid building owners, policymakers and stakeholders in planning effective interventions and to address vulnerabilities, targeting three levels of decision making at strategic, tactical and operational levels. The project deploys cloud technologies like OpenStack and Kubernetes to host an interoperable platform for vulnerability analysis, data harmonization, and decision-making. Its solutions will be tested and validated on 3 Large Scale Pilots in Spain, Greece, Italy, and Slovenia, addressing hazards such as heatwaves, flooding, fires, and earthquakes. A multi-hazard replication pilot in France will further evaluate the scalability and versatility of these approaches across diverse contexts. 

Insights from these pilots will feed into a replication roadmap and a capacity-building program designed to train future leaders in climate-resilient urban development. By fostering co-creation with local stakeholders and communities, CLIMRES ensures its innovative solutions are practical, cost-effective, and replicable, targeting Technology Readiness Levels (TRL) 6-8. 

CLIMRES aims to bridge innovation with actionable solutions, equipping building owners, policymakers, and communities with the tools needed to enhance urban climate resilience. This presentation highlights the project’s interdisciplinary approach, outputs and technological underpinnings, offering insights into scalable solutions for climate adaptation in urban settings. 

How to cite: Pisa, C., Antonacci, M., Baousis, V., Aspragkathos, S., Sotiropoulos, I., and Rizou, S.: Co-Creating Cloud-Based Tools for Urban Climate-Resilience: The CLIMRES Project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9432, https://doi.org/10.5194/egusphere-egu25-9432, 2025.

EGU25-10683 | Orals | ESSI2.15

Copernicus data and services uptake with EO4EU platform: an AI-augmented ecosystem for Earth Observation data accessibility and exploitation. 

Federico Fornari, Vasileios Baousis, Mohanad Albughdadi, Marica Antonacci, Tolga Kaprol, Claudio Pisa, Charalampos Andreou, Kakia Panagidi, and Stathes Hadjiefthymiades

The Copernicus program has fostered Earth Observation (EO) and Earth Modeling by offering extensive data and services to European Citizens. Sentinel satellites’ data is accessible  through platforms like the Copernicus Open Access Hub and the Copernicus Data Space Ecosystem, which provide a wide range of information on land, ocean and atmospheric conditions. Complementing these resources, six specialized Copernicus services deliver data in domains such as the atmosphere, marine environment, land monitoring, climate change, security and emergency response. To streamline access and usability, cloud-based Copernicus Data and Information Access Services (DIAS) offer centralised platforms equipped with cloud infrastructure and processing tools. Building on these efforts, the Copernicus Data Space Ecosystem (https://dataspace.copernicus.eu/) enhances existing DIAS services with advanced functionalities like improved search capabilities, virtualizations and APIs. Meanwhile, the Destination Earth (DestinE) initiative led by ECMWF, EUMETSAT and ESA, aims to develop high-precision digital Earth models - or digital twins - that simulate natural and human activities. These models mainly focus on weather-induced extremes and climate change adaptation, generating valuable Earth Modeling data. Furthermore, European Data Spaces integrate datasets across diverse domains, including agriculture, health, energy, and environmental monitoring, creating opportunities to combine these resources with Copernicus and DestinE data through advanced technologies like artificial intelligence (AI) and machine learning (ML). This integration paves the way for innovative solutions and public-facing products and services. Despite the volume and richness of Copernicus and related EO data, its accessibility remains limited, with most users being experts or scientists. For broader industry adoption and the development of impactful applications that benefit society and the enviroment, significant barriers must be addressed. EO data is often fragmented, complex, and difficult to process, requiring domain expertise for tasks such as data discovery, pre-processing, storage, and conversion into formats suitable for analytics and Geographic Information Systems (GIS).

The EO4EU platform (https://www.eo4eu.eu/), showcased in this presentation, introduces a multi-cloud ecosystem designed for holistic management of EO data. Its primary objective is to bridge the gap between domain experts and end users, leveraging technological advancements to broaden the adoption of EO data across diverse markets. By enhancing the accessibility and usability of EO data, EO4EU supports market growth through advanced data modeling, dynamic annotation, and state-of-the-art processing, powered by European cloud infrastructures such as WEkEO/DIAS and CINECA. EO4EU provides a suite of innovative tools and methodologies to assist a wide range of users, from professionals and domain experts to general citizens, in benefiting from EO data. Its key features include:

  • Knowledge Graph-based Decision Making: Facilitates insightful feature extraction from diverse repositories, enabling a more comprehensive understanding of datasets.
  • AI/ML Marketplace: A centralized hub for AI & ML models, algorithms, techniques, and metadata.
  • Big Data Processing Engines: Optimized for cloud environments to efficiently manage large-scale datasets.
  • User-friendly Interfaces: GUI, CLI, APIs, and immersive VR experiences, targeting both technical and non-technical users.
  • Workflow Engine: Simplifies the definition and execution of recurring tasks for EO data retrieval and processing.

How to cite: Fornari, F., Baousis, V., Albughdadi, M., Antonacci, M., Kaprol, T., Pisa, C., Andreou, C., Panagidi, K., and Hadjiefthymiades, S.: Copernicus data and services uptake with EO4EU platform: an AI-augmented ecosystem for Earth Observation data accessibility and exploitation., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10683, https://doi.org/10.5194/egusphere-egu25-10683, 2025.

EGU25-10977 | Posters on site | ESSI2.15

Cloud-Powered Earth Observation Tools for Urban Resilience: The BUILDSPACE Project 

Marica Antonacci, Vasileios Baousis, Claudio Pisa, Stamatia Rizou, and Iasonas Sotiropoulos

The BUILDSPACE project harnesses the transformative potential of cloud computing to evolve urban development and resilience practices. By integrating advanced Earth Observation (EO) data with state-of-the-art satellite and cloud technologies, BUILDSPACE addresses critical urban challenges, including climate adaptation, energy efficiency, and disaster resilience, while contributing to the European Green Deal’s objectives of sustainability and carbon neutrality. 

Central to BUILDSPACE are five innovative services designed to support urban decision-making. At the building scale, the project facilitates the generation and visualization of detailed digital twins through interactive displays, virtual reality (VR), and augmented reality (AR) interfaces. These digital twins enable precise simulations for energy optimization, operational efficiency, and climate impact assessment. At the city scale, BUILDSPACE provides tools to address climate scenarios, such as urban heat islands and flooding, empowering municipalities and urban planners with actionable insights through interactive, map-based platforms. 

The project’s technical foundation lies in a robust, cloud-native architecture built on Kubernetes and OpenStack, combined with a DevOps methodology to streamline both infrastructure services and application deployment. Kubernetes orchestrates containerised workloads, enabling efficient automated deployment, scaling and management of applications, while OpenStack provides a flexible infrastructure for managing compute, storage, and networking resources. Through the DevOps approach, we ensure continuous integration and delivery (CI/CD), fostering rapid development cycles and operational agility. By adopting open-source cloud platforms, the project ensures interoperability, reproducibility and automation across diverse environments, driving consistency and efficiency throughout the lifecycle of both infrastructure and applications. 

The project’s services are being validated across four European cities representing diverse climatic conditions, namely Warsaw, Riga, Piraeus and Ljubljana. These validations focus on two scenarios: construction companies monitoring building processes with advanced digital tools, and municipalities analysing the impacts of climate change on urban infrastructure. 

By advancing from TRL 5-6 to TRL 7-8, BUILDSPACE aims to deliver market-ready solutions that align with the European GNSS and Copernicus initiatives and to synchronise with the advances, concerning Digital Twin technologies and data federation mechanisms, of the Destination Earth initiative, while paving the way for a broader adoption of cloud technologies in EO-based urban resilience applications. 

How to cite: Antonacci, M., Baousis, V., Pisa, C., Rizou, S., and Sotiropoulos, I.: Cloud-Powered Earth Observation Tools for Urban Resilience: The BUILDSPACE Project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10977, https://doi.org/10.5194/egusphere-egu25-10977, 2025.

EGU25-11810 | Orals | ESSI2.15

DeployAI Earth Observation Services: Enabling Environmental Insights on the European AI-on-Demand Platform 

Antonis Troumpoukis, Mohanad Albughdadi, Martin Welß, Vasileios Baousis, and Iraklis Klampanos

The DeployAI project [1] designs and delivers a fully operational European AI-on-Demand Platform (AIoDP) to empower the European industry with access to cutting-edge AI technology, and to promote trustworthy, ethical, and transparent European AI solutions, with a focus on SMEs and the public sector. To achieve this, the platform enables the development and deployment of AI solutions through the following core solutions: (i) AI Builder [2], which allows the assembling of reusable AI modules into AI pipelines; (ii) seamless access to Cloud and HPC infrastructures (e.g., MeluXina and LUMI); (iii) a marketplace for the listing and distribution of ready-to-use AI products; (iv) an expansive and growing library of diverse AI-driven use cases.

As part of its domain-driven solutions, AIoDP seeks to empower Environmental Scientists, AI Engineers, Developers, Researchers, and SMEs via the DeployAI Earth Observation Services. These services will accelerate the development of AI-driven environmental applications, by providing pre-trained models that simplify satellite imagery processing, land usage classification, and image segmentation. Key models available as modules within the DeployAI’s AI Builder include:

  • Leaf Area Index (LAI) Model: Enables precise monitoring of vegetation health and ecological dynamics by calculating leaf area per unit ground [3]. 
  • Object Detection Model: Identifies specific objects in high-resolution satellite images, supporting applications such as  infrastructure monitoring, pollution tracking, and deforestation assessment [4].
  • Segment Anything Model (SAM): Simplifies analysis across diverse environmental applications through the capabilities of SAM that allows flexible, prompt-based image segmentation for new datasets, with zero-shot and few-shot learning [5].

These models, along with the broader functionalities of AI Builder, enable users to create custom AI pipelines that address their specific environmental challenges in several environmental areas, including vegetation health monitoring, water balance analysis, climate modeling, urban planning, traffic management, pollution monitoring, and infrastructure maintenance. Users can leverage the visual pipeline editor to easily assemble pipelines from reusable AI modules without needing to write code. Once created, these pipelines can be deployed as AI applications on various execution environments. DeployAI facilitates seamless transitions between these environments by providing connectors to a host of target infrastructures, including Cloud platforms and HPC systems. This empowers users to leverage the most suitable computational resources for their specific needs.

By providing a user-friendly platform with access to cutting-edge AI technology and Cloud/HPC resources, DeployAI empowers users to address critical environmental challenges and unlock new possibilities for sustainable development.

[1] https://deployaiproject.eu
[2] https://gitlab.eclipse.org/eclipse/graphene
[3] https://github.com/DeployAI-Environmental-Services/depai-lai
[4] https://github.com/DeployAI-Environmental-Services/depai-yolov8-obb
[5] https://github.com/DeployAI-Environmental-Services/depai-sam-interactive

This work has received funding from the European Union’s Digital Europe Programme (DIGITAL) under grant agreement No 101146490.

How to cite: Troumpoukis, A., Albughdadi, M., Welß, M., Baousis, V., and Klampanos, I.: DeployAI Earth Observation Services: Enabling Environmental Insights on the European AI-on-Demand Platform, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11810, https://doi.org/10.5194/egusphere-egu25-11810, 2025.

EGU25-12070 | ECS | Orals | ESSI2.15

Performance Benchmarking and Energy monitoring for Climate Modelling 

Sergi Palomas, Mario Acosta, Gladys Utrera, Okke Lennart, Daniel Beltran, Miguel Castrillo, Niclas Schroeter, and Ralf Mueller

The computational intensity of climate models makes them among the most energy-demanding applications in High-Performance Computing (HPC), resulting in significant computational costs and carbon emissions. Addressing the dual challenge of improving climate predictions —by running higher resolution, more accurate and complex models— and ensuring sustainability requires innovative tools to evaluate both computational efficiency and energy consumption across diverse HPC architectures. To address this, and in the context of the Center of Excellence in Simulation of Weather and Climate in Europe (ESiWACE), we have extended the High-Performance Climate and Weather Benchmark (HPCW) framework to incorporate a standardised set of Climate Performance Metrics for Intercomparison Projects (CPMIPs) and energy consumption monitoring.

HPCW, originally designed to maintain a set of relevant and realistic, near-operational weather forecast workloads to benchmark HPC sites, can provide insights beyond generic benchmarks like High-Performance Linpack (HPL) or High-Performance Conjugate Gradients (HPCG) by focusing on domain-specific workloads.

The inclusion of CPMIPs into HPCW brings a widely accepted set of metrics specifically tailored to the particularities of climate workflows. These metrics, already recognized by the scientific community, are key to better understanding climate model performance and allow us to keep the results from the framework relevant for research and operational runs, as well as improving our capacity for multi-model multi-platform performance comparisons.

By integrating energy monitoring, HPCW enables users to evaluate how critical computational kernels in climate models perform in terms of energy consumption. Our review of energy profiling tools across EuroHPC pre-exascale systems, including MareNostrum 5, LUMI, and Leonardo, highlights a fragmented landscape. Current tools offer varying granularity and portability, but limitations such as system configurations, administrative restrictions, and hardware compatibility often hinder their application. Low-level interfaces like Running Average Power Limit (RAPL) and Performance Application Programming Interface (PAPI) counters offer precise energy measurements but are constrained by accessibility issues.

These advancements aim to improve the allocation of climate experiments, such as those conducted for the Intergovernmental Panel on Climate Change (IPCC) in Coupled Model Intercomparison Projects (CMIPs), to the most suitable HPC resources, while also identifying architectural bottlenecks before running production experiments. Additionally, by enhancing energy consumption quantification, this work contributes to ongoing efforts to measure and reduce the carbon footprint of the climate research community. Furthermore, these analyses are expected to be particularly valuable for climate researchers, especially in the context of upcoming large-scale initiatives like CMIP7, enabling them to make informed resource requests and facilitate robust multi-platform comparisons of climate model performance which were not possible in the past. We anticipate that HPC vendors can also benefit from the outcomes of our work in optimising the systems for climate modelling workloads. By combining performance and energy metrics within a unified framework, we provide critical insights that align computational advancements with sustainability goals, ensuring efficient and environmentally conscious use of HPC resources for climate research.

How to cite: Palomas, S., Acosta, M., Utrera, G., Lennart, O., Beltran, D., Castrillo, M., Schroeter, N., and Mueller, R.: Performance Benchmarking and Energy monitoring for Climate Modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12070, https://doi.org/10.5194/egusphere-egu25-12070, 2025.

EGU25-12918 | ECS | Orals | ESSI2.15

Enhancing Pangeo-Fish with HEALPix Convolution: Impact Evaluation and Benefits 

Etienne Cap, Tina Odaka, Jean-Marc Delouis, Justus Magin, and Mathieu Woillez

The Pangeo-Fish project processes biologging data to analyze fish movement and migration patterns.  While SciPy’s convolution methods are robust, they are not optimized for handling spherical datasets inherent to Earth system science. To address this limitation, we propose the integration of HEALPix convolution, a method designed for spherical operations, into Pangeo-Fish.

HEALPix convolution offers distinct advantages for geophysical data analysis, particularly when dealing with spherical datasets in Earth system science. It uses the HEALPix pixelization as a core Discrete Global Grid System (DGGS), which ensures equally-sized pixels globally, removing distortions common in flat projections. This consistency is crucial for maintaining the physical relevance of convolutions across locations. Additionally, HEALPix’s dyadic property supports flexible, multiscale resolution adjustments, allowing for downscaling while preserving accuracy. Such scalability is essential for studying oceanic environments where areas of interest, like coastal zones and basins, are often resolution-dependent.

Our approach evaluates the performance of HEALPix convolution in comparison to traditional SciPy methods, focusing on its ability to enhance the accuracy of habitat mapping and migration pathway modeling for fish. 

This integration is particularly relevant within the Global Fish Tracking System (GFTS), which operates under the European Union’s Destination Earth (DestinE) initiative. GFTS utilizes datasets from Copernicus Marine Services and the European Tracking Network (ETN) to model fish habitats, spawning grounds, and migration swimways. HEALPix convolution strengthens the pangeo-fish’s capacity for studying Species such as tuna and eel that exhibit large-scale, transoceanic migrations.    

In conclusion, this work highlights the transformative potential of HEALPix convolution in spherical data processing. By integrating this innovative method, Pangeo-Fish can provide more accurate, scalable, and actionable insights into fish behaviors and habitats, contributing to sustainable management practices and conservation strategies globally.

 

How to cite: Cap, E., Odaka, T., Delouis, J.-M., Magin, J., and Woillez, M.: Enhancing Pangeo-Fish with HEALPix Convolution: Impact Evaluation and Benefits, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12918, https://doi.org/10.5194/egusphere-egu25-12918, 2025.

EGU25-13725 | Posters on site | ESSI2.15

Cloud-based platform for the management of hydrogeological risks in the Po Basin  

Marco Zazzeri and the PARACELSO team

In recent years, technological advances in the use of geospatial data (such as satellite images, anthropogenic and/or environmental raster and vector open data, etc.) for hydrogeological risk assessment, combined with advanced analysis techniques (e.g., machine learning), have become increasingly valuable. These technologies can be utilized by local and national authorities for land planning and emergency management to better understand the dynamics associated with climate change. This understanding can help guide actions aimed at safeguarding not only environmental resources but also socio-economic assets and citizens’ lives.

In pursuit of this goal, a partnership has been established between the Po River Basin District Authority (AdBPo), the Italian Space Agency (ASI), and academic and research institutions such as the University of Bologna (UNIBO), the University of Modena and Reggio Emilia (UNIMORE), the University of Padova (UNIPD), and the Institute of Environmental Geology and Geoengineering of the National Research Council of Italy (CNR-IGAG). The aim is to implement a downstream service for monitoring landscape evolution related to fluvial systems (geomorphological classification), and slope dynamics (including landslides and rock glaciers) and to quantitatively evaluate the exposed assets.

The PARACELSO project (Predictive Analysis, MonitoRing, and mAnagement of Climate change Effects Leveraging Satellite Observations) aims to develop a modular and interoperable cloud-based platform that supports the analysis of natural phenomena (such as fluvial hydrodynamics, landslides, and rock glaciers) using satellite images provided by:

  • DIAS platforms deployed by the Copernicus Programme (e.g., Sentinel 1-2);
  • ASI missions such as CosmoSkyMed, PRISMA, and SAOCOM.

Furthermore, a methodology integrating Earth Observation and geospatial data analysis has been implemented using open-source libraries.

To facilitate this, the MarghERita supercomputer, named in honor of the scientist Margherita Hack, has been made available by the Emilia-Romagna region. It is used both to store the downloaded satellite images and to run the algorithms developed in the project for studying the temporal evolution of river and slope systems. Finally, it enables the sharing and visualization of processed data.

The project has received funding from ASI through the “I4DP_PA (Innovation for Downstream Preparation for Public Administrations)” Call for Ideas.

How to cite: Zazzeri, M. and the PARACELSO team: Cloud-based platform for the management of hydrogeological risks in the Po Basin , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13725, https://doi.org/10.5194/egusphere-egu25-13725, 2025.

EGU25-13873 | Orals | ESSI2.15

UXarray: Extending Xarray for Enhanced Support of Unstructured Grids 

John Clyne, Hongyu Chen, Philip Chmielowiec, Orhan Eroglu, Cecile Hannay, Robert Jacob, Rajeev Jain, Brian Medeiros, Paul Ullrich, and Colin Zarzycki

Over the past decade, weather and climate models have rapidly adopted unstructured meshes to better leverage high-performance computing systems and approach kilometer-scale resolutions. Output from this new generation of models presents many challenges for their subsequent analysis, largely due to a lack of community tools supporting unstructured grid data. Last year, we introduced UXarray, a class extension of Xarray that provides native support for unstructured meshes. UXarray readily runs in a Jupyter Notebook and offers parallelized execution through its compatibility with Dask, demonstrating its flexibility as both a tool for lightweight exploration and communication, and for supporting intensive calculations applied to vast data volumes. Over the past year, UXarray has matured significantly and is now capable of supporting many real-world analysis workflows applied to outputs from a growing number of high-resolution models and dynamical cores, including ICOsahedral Non-hydrostatic (ICON) atmosphere model, the Finite-Element/volumE Sea ice-Ocean Model (FESOM), NSF NCAR’s Model for Prediction Across Scales (MPAS), and the U.S. DOE’s Energy Exascale Earth System Model (E3SM). This presentation will provide an overview of the UXarray’s current capabilities, which include extensive support for plotting and many foundational analysis operators; demonstrate examples in Jupyter Notebooks; present plans for the future;  and discuss ways for Pangeo and the broader earth system science community to help guide new developments. 

How to cite: Clyne, J., Chen, H., Chmielowiec, P., Eroglu, O., Hannay, C., Jacob, R., Jain, R., Medeiros, B., Ullrich, P., and Zarzycki, C.: UXarray: Extending Xarray for Enhanced Support of Unstructured Grids, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13873, https://doi.org/10.5194/egusphere-egu25-13873, 2025.

EGU25-14306 | ECS | Orals | ESSI2.15

Navigating New Grids: Evaluating DGGS Configurations for Marine Spatial Analysis 

Kayziel Martinez, Alexander Kmoch, Lőrinc Mészáros, Andrew Nelson, and Evelyn Uuemaa

Accurate and efficient spatial analysis is crucial for the mapping and sustainable management of marine environments, where large-scale and diverse datasets present significant analytical challenges. Traditional latitude-longitude methods, while widely used, often encounter limitations in data integration and handling distortion caused by Earth’s curvature. Discrete Global Grid Systems (DGGS) have emerged as a promising solution, offering a hierarchical, global, and equal-area framework for geospatial analysis. Despite their potential, the performance in marine spatial analysis remains underexplored.

This study evaluates the impact and suitability of DGGS-based spatial analysis by comparing its performance with the traditional latitude-longitude approaches. Using marine datasets representing point and raster data formats, the workflow begins with quantization, converting the data into DGGS cells.The implementation utilizes open-source Python tools from the Pangeo ecosystem, including xarray-xdggrid, to enable seamless integration and efficient analysis of large geospatial datasets. Three DGGS configurations – ISEA7H, HEALPIX, and ISEA3H are compared alongside traditional latitude-longitude grid for computational efficiency (processing time and memory usage) and their ability to preserve spatial patterns. Spatial analysis methods include density estimation, nearest neighbor evaluation, and clustering for point data, as well as zonal statistics, spatial autocorrelation, and resampling for raster data.

To further illustrate the application of DGGS-based methods, the study includes a case study on estuary characterization. This characterization relies on spatial analysis methods, integrating physical oceanographic parameters from Delft3D-FM, biogeochemical and optical data products, and in-situ point measurements from the Copernicus Marine Environment Monitoring Service (CMEMS). Representing these diverse datasets within the DGGS framework highlights its ability to manage varying data types and scales, offering insights into estuarine environments and demonstrating its scalability for addressing complex marine spatial challenges.

Results indicate that DGGS frameworks deliver comparable computational performance while offering consistent spatial representation. Configuration-specific trade-offs influence their effectiveness, emphasizing the importance of aligning DGGS configurations with specific analytical tasks and applications. Findings suggest that DGGS-based methods offer a promising alternative to traditional analysis techniques, providing greater flexibility in adapting to datasets, scale, and resolution. This contributes to more efficient mapping, sustainable marine environmental management, and advancing geospatial applications through open-source tools from the Pangeo ecosystem.

How to cite: Martinez, K., Kmoch, A., Mészáros, L., Nelson, A., and Uuemaa, E.: Navigating New Grids: Evaluating DGGS Configurations for Marine Spatial Analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14306, https://doi.org/10.5194/egusphere-egu25-14306, 2025.

EGU25-14400 | ECS | Orals | ESSI2.15

A community oriented approach to enabling open science with Earth science data at scale 

Max Jones, Aimee Barciauskas, Jonas Sølvsteen, Brian Freitag, Yuvi Panda, Kyle Barron, Julia Signell, Alex Mandel, Chuck Daniels, Nathan Zimmerman, Sean Harkins, Henry Rodman, Zac Deziel, Slesa Adhikari, Anthony Boyd, Alexandra Kirk, David Bitner, and Vincent Sarago

To enable wider participation in open science with geospatial data at scale, we need to reduce the effort and custom approaches required for setting up scalable scientific data analysis environments and computing workflows. We have made great strides in this pursuit by evolving and promoting community-developed open source frameworks, tools, and libraries for cloud-native data access and analysis, making them the default for scientists on the public cloud and local systems.

Many of our achievements have been supported by the NASA Visualization, Exploration, and Data Analysis (VEDA) project which seeks to proliferate cloud-native approaches for open science on Earth science data from NASA’s rich archives and many other providers. Our presentation highlights how we have engaged with communities like Pangeo, OpenScapes, Earth Science Information Partners, and the Cloud Native Geospatial Forum to build joint initiatives, target development, and ensure uptake of new solutions. We present key results from working groups, community showcases, and hackdays and hackweeks organized by VEDA team members, as well as specific contributions to the open source ecosystem, including the eoAPI platform for quickly and easily deploying an open-source Earth Observation stack, JupyterHub fancy profiles (with BinderHub) for seamless environment building, and Lonboard for fast, interactive vector visualization.

How to cite: Jones, M., Barciauskas, A., Sølvsteen, J., Freitag, B., Panda, Y., Barron, K., Signell, J., Mandel, A., Daniels, C., Zimmerman, N., Harkins, S., Rodman, H., Deziel, Z., Adhikari, S., Boyd, A., Kirk, A., Bitner, D., and Sarago, V.: A community oriented approach to enabling open science with Earth science data at scale, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14400, https://doi.org/10.5194/egusphere-egu25-14400, 2025.

EGU25-14610 | Orals | ESSI2.15

Weather Data Streaming with Kerchunk: Strengthening Early Warning Systems  

Nishadh Kalladath, Masilin Gudoshava, Shruti Nath, Jason Kinyua, Fenwick Cooper, Hannah Kimani, David Koros, Christine Maswi, Zacharia Mwai, Asaminew Teshome, Samrawit Abebe, Isaac Obai, Jesse Mason, Ahmed Amdihun, and Tim Palmer

The Ensemble Prediction System (EPS) provided by global weather forecast centres generates vast amounts of data that is crucial for early warnings of extreme weather and climate. However, regional and national meteorological services often face challenges in processing this data efficiently, particularly during regional downscaling and post-processing. Conventional methods of downloading and storing GRIB-format data have become increasingly inefficient and unsustainable. The Strengthening Early Warning Systems for Anticipatory Actions (SEWAA) project aims to address these challenges by exploring the use of cloud native operations and GenAI-cGAN driven post-processing systems.   

Kerchunk provides a groundbreaking solution for real-time weather data streaming, catering to the transition towards open and free to use cloud-based object storage from global weather forecasting centres. Kerchunk, in conjunction with GRIB index files, enables efficient, real-time access to weather data, fostering more sustainable workflows in weather and climate services, thus strengthening early warning systems.  

This study developed a workflow for streaming forecast data using Kerchunk with two primary objectives:  

1. Using GRIB index files to reduce redundant readings and generate Kerchunk reference files.  

2. Through streaming-like access, convert the reference files into virtual Zarr datasets and utilise Dask compute for scalable data handling   

The methodology utilised recent improvements in the Kerchunk library that integrate GRIB scanning with its index files. This allowed the system to sample subsets of the GRIB corpus instead of processing entire Forecast Model Run Collections (FMRC), significantly optimising performance.  

The workflow was implemented using cloud-based compute operations via Coiled python library and its service on the Google Cloud Platform. Dask cluster, managed through Coiled, enabled the creation of Zarr virtual datasets for analysis and visualisation. This streaming approach efficiently loads weather data into memory on demand, avoiding unnecessary data downloads and duplication.   

We validated the solution with NOAA GFS/GEFS datasets stored in AWS S3 bucket as open datasets. The optimised workflow demonstrated remarkable efficiency, requiring only <5% of the original GRIB data to be read, with the rest replaced by index files as input for reference file creation. This is followed by the step of Kerchunk reference files to virtual Zarr conversion by Dask clusters to process on a regional scale, such as East Africa’s in minutes supporting near real-time applications across spatial and temporal scales.  

This approach significantly enhances post processing workflows for EPS weather forecast, bolstering early warning systems and anticipatory action. Future work will focus on using the method to scaling training datasets and improving the cost efficiency of cGAN training to advance operational early warning systems. This innovative solution directly addresses the challenges faced by meteorological services in processing massive weather datasets, providing a scalable, cost-effective, development foundation for applying GenAI based post-processing and improving early warning systems. 

How to cite: Kalladath, N., Gudoshava, M., Nath, S., Kinyua, J., Cooper, F., Kimani, H., Koros, D., Maswi, C., Mwai, Z., Teshome, A., Abebe, S., Obai, I., Mason, J., Amdihun, A., and Palmer, T.: Weather Data Streaming with Kerchunk: Strengthening Early Warning Systems , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14610, https://doi.org/10.5194/egusphere-egu25-14610, 2025.

EGU25-15406 | Orals | ESSI2.15

Platform Engineering for Earth Observation: A Unified Approach to HPC and Cloud Systems 

Armagan Karatosun and Vasileios Baousis

The growing volume of Earth Observation (EO) and Earth modeling data makes it increasingly impractical to download and analyze it locally. Furthermore, as cloud-native data formats and AI/ML-driven models gain popularity, the community requires powerful computing and storage solutions to efficiently process and analyze EO data. High-performance computing (HPC) and cloud infrastructures can help accomplish this, but both bring significant challenges in maintaining those resources, putting additional workloads on the scientists and developers.

In this paper, we will present our solution, which uses cloud-native technologies and a “Control Plane” approach to seamlessly interact with HPC scheduling endpoints like SLURM and PBS, as well as cloud infrastructure resources, allowing HPC jobs to be submitted and monitored directly from a Kubernetes-based infrastructure. In contrast to traditional IT architecture, Platform Engineering is concerned with lowering operational complexity by introducing control planes to provide self-service capabilities. By abstracting away the complexities of the underlying infrastructure, this method gives teams a customized, scalable, and dependable environment to suit their unique requirements. We will thoroughly analyze existing technologies, including their methodologies, strengths, limits, and potential as universal solutions. Furthermore, we will assess their adaptation to various cloud and HPC infrastructures, providing insights into their suitability for larger applications. 

We will conclude our discussion with practical examples showing how the technical benefits of these two computing paradigms, combined with the Platform Engineering approach, may be effectively used in real-world EO data processing scenarios.

How to cite: Karatosun, A. and Baousis, V.: Platform Engineering for Earth Observation: A Unified Approach to HPC and Cloud Systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15406, https://doi.org/10.5194/egusphere-egu25-15406, 2025.

High-resolution regional climate model datasets, such as those produced within the Coordinated Regional Downscaling Experiment (CORDEX) framework, are critical for understanding climate change impacts at local and regional scales. These datasets, with their high spatial and temporal resolution, provide detailed insights into region-specific climate phenomena, including urban heat islands, mountainous climates, and extreme weather events. However, their accessibility and usability are often constrained by technical challenges such as fragmented data storage, inconsistent formats, and limited interoperability.

To address these barriers, we are developing the Climate Service Database (CSD) - a centralized data warehouse designed to streamline the temporal and spatial aggregation of CORDEX datasets for climate service applications. The CSD ingests raw CORDEX datasets and applies automated extraction, transformation, and loading (ETL) workflows to produce analysis-ready datasets tailored to user needs. By leveraging cloud-based infrastructure and adhering to Climate and Forecast (CF) conventions, the CSD ensures consistent, interoperable data products that are optimized for scalable access and analysis.

A core functionality of the CSD is its ability to aggregate datasets at multiple spatial and temporal scales, ranging from daily extremes to decadal averages, and across diverse spatial resolutions (e.g., countries, administrative regions, or watersheds). This capability enables the generation of climate indicators (e.g., hot summer days, heavy precipitation events) that are directly relevant for local decision-making and impact assessments. By providing data in cloud-optimized, analysis-ready formats (ARCO) and offering Software as a Service (SaaS), the CSD significantly lowers the technical barriers for researchers, businesses, and policymakers seeking to access user-tailored climate service datasets.

By centralizing and optimizing the processing of regional climate model datasets, the CSD fosters collaboration across research institutions, public agencies, and climate-tech startups. It enables users to efficiently access consistent and up-to-date data while eliminating the redundancies of localized data storage and processing. This approach also opens new opportunities for applying AI-driven analytics and machine learning models to CORDEX data, paving the way for innovative climate services and applications.

Through its focus on regional climate model datasets, the CSD exemplifies how modern data infrastructures can enhance the usability of high-resolution climate data, empowering stakeholders to develop robust, data-driven adaptation and mitigation strategies in response to the challenges of climate change.

How to cite: Buntemeyer, L.: Advancing Regional Climate Data Accessibility through a Cloud-native Climate Service Database, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16230, https://doi.org/10.5194/egusphere-egu25-16230, 2025.

EGU25-17137 | Orals | ESSI2.15

The Sentinels EOPF Toolkit: Community Notebooks and Plug-ins for using Copernicus Sentinel Data in Zarr format 

Dr. Julia Wagemann, Sabrina Szeto, Emmanuel Mathot, and James Banting

Zarr is a key component of the Pangeo ecosystem and instrumental for effectively accessing and processing multi-dimensional Earth data in cloud-based systems. More and more leading satellite data providers are exploring the transition of their data archives to a cloud environment. 

As part of the ESA Copernicus Earth Observation Processor Framework (EOPF), ESA is in the process of providing access to “live” sample data from the Copernicus Sentinel missions -1, -2 and -3 in the new Zarr data format. This set of reprocessed data allows users to try out accessing and processing data in the new format and experiencing the benefits thereof with their own workflows.

To help Sentinel data users to experience and adopt the new data format, a set of resources called the Sentinels EOPF Toolkit is being developed. Development Seed, SparkGeo and thriveGEO, together with a group of champion users (early-adopters), are creating a set of Jupyter Notebooks, plug-ins and libraries that showcase the use of Sentinel data in Zarr for applications across multiple domains for different user communities, including users of Python, Julia, R and QGIS.

This presentation will give a demo of the first set of notebooks and plugins of the Sentinels EOPF toolkit that were developed and that facilitate the adoption of the Zarr data format for Copernicus Sentinel data users. Additionally, we will give an overview of toolkit developments and community activities that are planned throughout the project period.

How to cite: Wagemann, Dr. J., Szeto, S., Mathot, E., and Banting, J.: The Sentinels EOPF Toolkit: Community Notebooks and Plug-ins for using Copernicus Sentinel Data in Zarr format, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17137, https://doi.org/10.5194/egusphere-egu25-17137, 2025.

EGU25-18285 | ECS | Posters on site | ESSI2.15

Regridding Satellite and Model Data to DGGS (HEALPix) Using the Pangeo Ecosystem 

Justus Magin, Jean-Marc Delouis, Lionel Zawadski, Julien Petiton, Max Jones, and Tina Odaka

Regridding data from diverse sources, such as satellite observations and numerical models, is a critical task in Earth system sciences. Proper interpolation methods are essential to ensure data fidelity when combining or comparing datasets on different grids. This becomes especially relevant in the context of emerging grid systems like Discrete Global Grid Systems (DGGS), specifically HEALPix.

DGGS are spatial reference systems designed to partition the Earth’s surface into a hierarchy of equal-area cells. Unlike traditional latitude-longitude grids, DGGS uses tessellations, such as hexagons, to represent the Earth’s curved surface with minimal distortion. This grid system is particularly suited for handling global-scale geospatial data by providing uniform coverage and resolution, enabling efficient storage, processing, and analysis.

HEALPix (Hierarchical Equal Area isoLatitude Pixelation) is a specific implementation of DGGS widely used in astronomy and Earth sciences. HEALPix divides the sphere into equal-area cells following an iso-latitude structure, making it computationally efficient for operations such as spherical harmonics and multi-resolution analysis. Originally developed for astrophysical applications, it has become increasingly popular in the Earth sciences for representing satellite data, model outputs, and other geospatial datasets in a way that preserves area integrity and facilitates seamless multi-resolution data integration.

By leveraging these grid systems, particularly HEALPix, we can achieve a more accurate and efficient representation of geospatial data.

The Pangeo ecosystem includes an array of powerful regridding tools, each tailored to specific grid types and applications. However, navigating this ecosystem to identify the most suitable tool and workflow can be challenging.

In this presentation, we will show an overview of regridding solutions within Pangeo, highlighting their capabilities and limitations, as well as  their application. We will also demonstrate a practical regridding workflow using model outputs or simulated satellite data such as the Odysea dataset (Aviso+ Altimetry. (n.d.). Simulated Level-2 Odysea Dataset. Retrieved from https://www.aviso.altimetry.fr/en/data/products/value-added-products/simulated-level-2-odysea-dataset.html on January 14, 2025), to the HEALPix grid. This workflow will make use of recent advances in technology to make it reproducible to make it efficient and reproducible, such as virtualizarr for fast metadata access and dask for scalable operations, with the output saved as chunked zarr files for seamless integration with downstream analysis.

How to cite: Magin, J., Delouis, J.-M., Zawadski, L., Petiton, J., Jones, M., and Odaka, T.: Regridding Satellite and Model Data to DGGS (HEALPix) Using the Pangeo Ecosystem, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18285, https://doi.org/10.5194/egusphere-egu25-18285, 2025.

EGU25-18336 | Posters on site | ESSI2.15

Advancing Earth System Science through collaboration: An overview of ECMWF Special Projects 

Milana Vuckovic and Becky Hemingway

ECMWF has been providing resources on its operational high-performance computing (HPC) and cloud facilities (European Weather Cloud) to researchers and institutions through the Special Projects framework. This framework has been established almost 50 years ago as part of the creation of ECMWF. ECMWF's HPC facility is specifically designed to support both operational time-critical production of global weather forecasts and typical research workflows, therefore through Special Projects, researchers can get access not only to a top high-performance computing and cloud facility and one of the largest meteorological archives in the world, but also full user support.
Special Projects are defined as experiments or investigations of a scientific or technical nature, undertaken by one or more ECMWF Member States, likely to be of interest to general scientific community. The main aim of this initiative is to facilitate collaboration, enabling the development of innovative methodologies and tools for numerical weather prediction, climate and environmental modelling, and other disciplines within Earth System Sciences. All Special Project applications undergo a review process by ECMWF and its Scientific Advisory Committee (SAC), as well as ECMWF Member State's meteorological services and are ranked primarily by their scientific quality.
This poster will describe the Special Projects framework and showcase three recent Special Projects that illustrate collaborative nature of the initiative using ECMWF's HPC and European Weather Cloud facilities, including validating ICON model on ECMWF systems, the development of next-generation European Earth System Model (EC-EARTH4) and mapping the yet uncharted continuum of cyclone dynamics for the Euro Atlantic domain.
Through these examples, the poster will demonstrate how ECMWF Special Projects foster international collaboration, resource sharing, and innovation, enabling advancement in Earth System Science. 

How to cite: Vuckovic, M. and Hemingway, B.: Advancing Earth System Science through collaboration: An overview of ECMWF Special Projects, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18336, https://doi.org/10.5194/egusphere-egu25-18336, 2025.

EGU25-20590 | Posters on site | ESSI2.15

Dhemeter: Data Hub for Environmental and METEorological Resources 

Cédric Pénard, Nathan Amsellem, Boris Gratadoux, Bastien Barthet, Jean Christophe Pere, Johannes Staufer, Laure Chaumat, and Alexia Mondot

Dhemeter is a weather and environmental data aggregator. It is developed using a microservices architecture to handle a wide variety of data from various providers, such as NOAA, ECMWF, Eumetsat, Météo-France, DWD, and Copernicus. The implementation of aggregation, concatenation, and consistency functionalities has been successfully executed for meteorological data. This versatile tool accommodates numerical model data, in-situ observations, remote sensing data, and reanalyses, allowing for online data retrieval from multiple sources.

Key features of the aggregator include:

  • Concatenation of Multiple Data Sources: Users can combine data according to selected categories such as Observations, Forecasts, and Reanalyses.
  • Standardization of Physical Data: This involves spatial and temporal interpolation as well as geographical selections to ensure uniformity.
  • Storage of Resulting Data Structures: The data is stored in a pivot format that facilitates access and distribution of scientific data, specifically in the NetCDF format.

The microservices architecture of the aggregator allows for the extensibility of the offered data catalog, and an API is available for users to make direct queries to chosen data sources.

In the short to medium term, the goal is to enhance the tool further, evolving it into a comprehensive data distribution and aggregation system that centralizes and simplifies access to various types of data, including meteorological, oceanographic, and air quality data.

Dhemeter focuses on ease of use, extensibility, scalability, and customization, offering users capabilities for data fusion and harmonization.

How to cite: Pénard, C., Amsellem, N., Gratadoux, B., Barthet, B., Pere, J. C., Staufer, J., Chaumat, L., and Mondot, A.: Dhemeter: Data Hub for Environmental and METEorological Resources, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20590, https://doi.org/10.5194/egusphere-egu25-20590, 2025.

EGU25-20676 | Orals | ESSI2.15

Integrated geospatial Python libraries for efficient analysis of modern elevation measurements 

Scott Henderson, David Shean, Jack Hayes, and Shashank Bhushan

NASA established the Surface Topography and Vegetation (STV) Incubation program to develop and mature the next-generation measurement approaches to precisely map Earth’s changing surface and overlying vegetation structure, and prepare for a dedicated satellite mission within the next decade. Over the past two decades, large archives of 3D surface elevation measurements by airborne and satellite instruments including LiDAR, altimeters, Synthetic Aperture Radar, and stereo optical imagery have been systematically collected, though not always in a coordinated way. Yet, many of these datasets are fortuitously acquired over the same location within a short temporal window (e.g., <1-14 days) and many are now publicly available and hosted on the cloud. In theory, this is a great opportunity to synthesize myriad elevation measurements for STV researchers, but in practice merging these datasets accurately for scientific analysis requires dealing with numerous data formats, complex 4D coordinate reference systems, and securing access to significant computational resources.

We are developing an open-source Python library to identify, curate, and efficiently process coincident elevation measurements spanning the last several decades. This work would not be possible without well-integrated geospatial libraries (e.g. Geopandas, Xarray, Dask), as well as emerging cloud-native data and metadata formats such as Cloud-Optimized Geotiff and STAC-GeoParquet. We will describe our work to-date and reflect on the process of collaborative development across libraries, on our increasing reliance on Cloud resources, and current and future research directions.

How to cite: Henderson, S., Shean, D., Hayes, J., and Bhushan, S.: Integrated geospatial Python libraries for efficient analysis of modern elevation measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20676, https://doi.org/10.5194/egusphere-egu25-20676, 2025.

EGU25-21202 | Orals | ESSI2.15

From SAFE to Zarr: The EOPF Sample Service Initiative 

Christian Briese, Christoph Reimer, Christian Briese, Christoph Reck, Dimitrios Papadakis, Michele Claus, Gunnar Brandt, Anne Fouilloux, and Tina Odaka

Over the past decade, the operational Copernicus Sentinels Data Processors have generated vast amounts of Earth observation data, supporting various scientific and commercial applications. However, the current format used by ESA to provide Copernicus data, known as SAFE (Standard Archive Format for Europe), has become outdated. To address this, ESA has initiated the transition to a new Zarr-based data format. The Earth Observation Processing Framework (EOPF) Sample Service is ESA’s official initiative to support this transition by providing early access to the new format for users. This shift is essential for creating a cloud-native and interoperable solution that enhances data accessibility and integration with modern processing frameworks. The primary goal is to standardize data formats across Sentinel missions, enable scalable processing on cloud platforms, and ensure compatibility with contemporary data science tools. This initiative is crucial for minimizing disruption and ensuring continuity for users, applications, and services built around existing data formats.

The EOPF Sample Service comprises several key components. The EOPF Core Platform re-formats ingested SAFE data products into the new cloud-optimized EOPF Zarr data products and provides data access via STAC API and S3 API. To ensure timely conversion, the platform utilizes Argo Events and the Copernicus Data Space Ecosystem's subscription service. This platform is maintained by experts from EODC and DLR. The EOPF User Platform offers additional user services, including JupyterHub (BinderHub), Dask, and a STAC Browser, which are essential for supporting user adoption by lowering the entrance barrier to cloud applications and data discovery capabilities. The service is designed to make use of advanced technologies such as Kubernetes for container orchestration and Dask for parallel computing. User and identity management is achieved in cooperation with the Copernicus Data Space Ecosystem.

User adoption is further facilitated through Jupyter Notebooks designed by experts within the consortium, including members from the Pangeo community. These notebooks showcase the use of the new format within the community and are continuously improved by incorporating user feedback. In addition, enhancements are made to widely-used software tools like GDAL to support the new format, with practical demonstrations available through Jupyter Notebooks. The consortium selected by ESA to carry out this implementation includes experts from Brockmann Consult, DLR, Ifremer, EURAC, Evenflow, Simula, and EODC, each contributing their specialized knowledge in Earth observation, data management, and user engagement.

This contribution aims to present the EOPF Sample Service initiative and the current status of its implementation. The first Jupyter Notebooks demonstrating the new format will also be showcased, providing users with an intuitive and user-friendly interface for accessing and processing sample data in the new EOPF format.

How to cite: Briese, C., Reimer, C., Briese, C., Reck, C., Papadakis, D., Claus, M., Brandt, G., Fouilloux, A., and Odaka, T.: From SAFE to Zarr: The EOPF Sample Service Initiative, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21202, https://doi.org/10.5194/egusphere-egu25-21202, 2025.

EGU25-21279 | Orals | ESSI2.15

Advancing Cloud-Native Data Analysis and Publishing with Pangeo Tools in EarthCODE 

Deyan Samardzhiev, Anne Fouilloux, Tina Odaka, and Benjamin Ragan-Kelley

EarthCODE (Earth Science Collaborative Open Development Environment) is a platform that leverages cloud-native tools to empower Earth system researchers in accessing, analyzing, and sharing data across distributed infrastructures, such as the Copernicus Data Space Ecosystem and Deep Earth System Data Laboratory (DeepESDL). By integrating Pangeo ecosystem tools—including Xarray, Dask, and Jupyter—EarthCODE supports scalable, FAIR-aligned workflows tailored to the challenges of Earth system science.

EarthCODE streamlines cloud-based data analysis and publishing by enabling collaborative research through interoperable workflows for analyzing complex datasets, including satellite observations, climate models, and in-situ measurements. Researchers can publish their analyses and workflows as reusable, executable resources in EarthCODE’s science catalog, fostering alignment with open science principles.

Through its integration of Pangeo tools, EarthCODE offers an intuitive environment for reproducibility, scalability, and collaboration, bridging the gap between data analysis and actionable insights. This presentation will demonstrate EarthCODE’s capabilities, including live, executable Jupyter notebooks that highlight its potential for sharing workflows and engaging diverse user groups. EarthCODE exemplifies the transformative power of cloud-native research, promoting open science and advancing the accessibility of Earth system data.

How to cite: Samardzhiev, D., Fouilloux, A., Odaka, T., and Ragan-Kelley, B.: Advancing Cloud-Native Data Analysis and Publishing with Pangeo Tools in EarthCODE, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21279, https://doi.org/10.5194/egusphere-egu25-21279, 2025.

EGU25-21603 | ECS | Orals | ESSI2.15 | Highlight

The Pangeo Ecosystem Supporting Climate Change Adaptation: The FAIR2Adapt RiOMar Case Study 

Even Moa Myklebust, Ola Formo Kihle, and Justus Magin

The RiOMar (River dominated Ocean Margins) case study, part of the FAIR2Adapt (FAIR to Adapt to Climate Change) project (EU funded project grant agreement No 101188256), focuses on supporting science-based climate change adaptation strategies for coastal water quality and marine ecosystem management. The case study uses large environmental datasets, such as sea temperature, salinity, and other marine parameters, to assess and model the impacts of climate change on coastal ecosystems. As part of the FAIR2Adapt project, which aims to enhance the shareability, accessibility, interoperability, and reusability of environmental data through the FAIR (Findable, Accessible, Interoperable, and Reusable) principles, the RiOMar case study emphasizes the use of cutting-edge data processing and analysis methods to support adaptive strategies for climate resilience.

In this presentation, we present our approach to reading the RiOMar large environmental datasets in netCDF format, creating VirtualZarr archives for efficient data handling, transforming them into a Discrete Global Grid System (DGGS) using the Healpix grid.Leveraging the Pangeo ecosystem, we use tools such as Kerchunk to create simpler access to multiple data sources, parallelize dataset processing using Dask or Cube, enabling scalable analysis of these complex, multi-dimensional data. We will show a comparison of performance between traditional cube-based approaches and Dask, highlighting the advantages of parallelized processing. Furthermore, we will showcase how to interactively visualize these datasets using tools like XDGGs and Lonboard, facilitating seamless exploration and analysis of the underlying environmental patterns. This work underscores the potential of open-source tools, scalable computing techniques, and the Pangeo ecosystem to enhance the accessibility and usability of large geospatial datasets in climate adaptation research.

How to cite: Moa Myklebust, E., Formo Kihle, O., and Magin, J.: The Pangeo Ecosystem Supporting Climate Change Adaptation: The FAIR2Adapt RiOMar Case Study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21603, https://doi.org/10.5194/egusphere-egu25-21603, 2025.

EGU25-1294 | Posters on site | ESSI2.13

A new sub-chunking strategy for fast netCDF-4 access in local, remote and cloud infrastructures.  

Flavien Gouillon, Cédric Penard, Xavier Delaunay, and Sylvain Herlédan

NetCDF (Network Common Data Form) is a self-describing, portable and platform-independent format for array-oriented scientific data which has become a community standard for sharing measurements and analysis results in the fields of oceanography, meteorology but also in the space domain.

The volume of scientific data is continuously increasing at a very fast rate. Object storage, a new paradigm that appeared with cloud infrastructures, can help with data storage and parallel access issues, but NetCDF may not be able to get the most out of this technology without some tweaks and fine tuning.

The availability of ample network bandwidth within cloud infrastructures allows for the utilization of large amounts of data. Processing data       where the data is located is preferable as it can result in substantial resource savings. But for some use cases downloading data from the cloud is required (e.g. processing also involving confidential data) and results still have to be fetched once processing tasks have been executed on the cloud.

Networks      exhibit significant variations in capacity and quality (ranging from fiber-optic and copper connections to satellite connections with poor reception in degraded conditions on boats, among other scenarios). Therefore, it is crucial for formats and software libraries to be specifically designed to optimize access to      data by minimizing the transfer to only what is strictly necessary.

In this context, a new approach has emerged in the form of a library that indexes the content of netCDF-4 datasets. This indexing enables the retrieval of sub-chunks, which are pieces of data smaller than a chunk, without the need to reformat the existing files. This approach targets access patterns such as time series in netCDF-4 datasets formatted with large chunks.

This report provides a performance assessment of netCDF-4 datasets for varied use cases. This assessment executes these use cases under various conditions, including POSIX and S3 local filesystems, as well as a simulated degraded network connection. The results of this assessment may provide guidance on the most suitable and most efficient library for reading netCDF data in different situations.

How to cite: Gouillon, F., Penard, C., Delaunay, X., and Herlédan, S.: A new sub-chunking strategy for fast netCDF-4 access in local, remote and cloud infrastructures. , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1294, https://doi.org/10.5194/egusphere-egu25-1294, 2025.

EGU25-4155 | Orals | ESSI2.13

How open software, data and platforms are transforming Earth observation data science 

Wolfgang Wagner, Matthias Schramm, Martin Schobben, Christoph Reimer, and Christian Briese

One of the most time-consuming and cumbersome tasks in Earth observation data science is finding, accessing and pre-processing geoscientific data generated by satellites, ground-based networks, and Earth system models. While the much increased availability of free and open Earth observation datasets has made this task easier in principle, scientific standards have evolved according to data availability, now emphasizing research that integrates multiple data sources, analyses longer time series, and covers larger study areas. As a result of this “rebound effect”, scientists and students may find themselves spending even more of their time on data handling and management than in the past. Fortunately, cloud platform services such as Google Earth Engine can save significant time and effort. However, until recently, there were no standardized methods for users to interact with these platforms, meaning that code written for one service could not easily be transferred to another (Schramm et al., 2021). This created a dilemma for many geoscientists: should they use proprietary cloud platforms to save time and resources at the risk of lock-in effects, or rely on publicly-funded collaborative scientific infrastructures, which require more effort for data handling? In this contribution, we argue that this dilemma is about to become obsolete thanks to rapid advancements in open source tools that allow building open, reproducible, and scalable workflows. These tools facilitate access to and integration of data from various platforms and data spaces, paving the way for the “Web of FAIR data and services” as envisioned by the European Open Science Cloud (Burgelman, 2021). We will illustrate this through distributed workflows that connect Austrian infrastructures with European platforms like the Copernicus Data Space Ecosystem and the DestinE Data Lake (Wagner et al., 2023). These workflows can be built using Pangeo-supported software libraries such as Dask, Jupyter, Xarray, or Zarr (Reimer et al., 2023). Beyond advancing scientific research, these workflows are also valuable assets for university education and training. For instance, at TU Wien, Jupyter notebooks are increasingly used in exercises involving Earth observation and climate data, and as templates for student projects and theses. Building on these educational resources, we are working on an Earth Observation Data Science Cookbook to be published on the Project Pythia website, a hub for education and training in the geoscientific Python community.

References

Burgelman (2021) Politics and Open Science: How the European Open Science Cloud Became Reality (the Untold Story). Data Intelligence 3, 5–19. https://doi.org/10.1162/dint_a_00069

Reimer et al. (2023) Multi-cloud processing with Dask: Demonstrating the capabilities of DestinE Data Lake (DEDL), Conference on Big Data from Space (BiDS’23), Vienna, Austria. https://doi.org/0.2760/46796

Schramm et al. (2021) The openEO API–Harmonising the Use of Earth Observation Cloud Services Using Virtual Data Cube Functionalities. Remote Sensing 13, 1125. https://doi.org/10.3390/rs13061125

Wagner et al. (2023) Federating scientific infrastructure and services for cross-domain applications of Earth observation and climate data, Conference on Big Data from Space (BiDS’23), Vienna, Austria. https://doi.org/10.34726/5309

How to cite: Wagner, W., Schramm, M., Schobben, M., Reimer, C., and Briese, C.: How open software, data and platforms are transforming Earth observation data science, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4155, https://doi.org/10.5194/egusphere-egu25-4155, 2025.

EGU25-4277 | Posters on site | ESSI2.13

BEACON Binary Format (BBF) - Optimizing data storage and access to large data collections 

Tjerk Krijger, Peter Thijsse, Robin Kooyman, and Dick Schaap

As part of European projects, such as EOSC related Blue-Cloud2026, EOSC-FUTURE and FAIR-EASE, MARIS has developed and demonstrated a software system called BEACON with a unique indexing system that can, on the fly with high performance, extract data subsets based on the user’s request from millions of heterogeneous observational data files. The system returns one single harmonised file as output, regardless of whether the input contains many different data types or dimensions. 

Since in many cases the original data collections that are imported in a BEACON installment contain millions of files (e.g. Euro-Argo, SeaDataNet, ERA5, World Ocean Database), it is hard to achieve fast responses. Next to this, these large collections also require a large storage capacity. To mitigate these issues, we wanted to optimize the internal file format that is used within BEACON. With the aim of reducing the data storage size and speeding up the data transfer, while guaranteeing that the information of the original data files is maintained. As a result, the BEACON software has included a unique file format called the “BEACON Binary Format (BBF)” that meets these requirements. 

The BBF is a binary data format that allows for storing multi-dimensional data as apache arrow arrays with zero deserialization costs. This means that computers can read the data stored on disk, as if it were computer memory, significantly reducing computational access time by eliminating the cost for a computer to translate what’s on disk, to computer memory.

Together with making the entire data format “non-blocking”, which means that all computer cores can access the file at the same time and simultaneously use the jump table to read millions of datasets in parallel. This enables a level of performance which reaches speeds of multiple GB/s, making the hardware the bottleneck instead of the software.

Furthermore, the format takes a unique approach to compressing data by adjusting the way it compresses and decompresses on a per dataset level. This means that every dataset is compressed in a slightly different manner, making it much more effective in terms of size reduction and time to decompress the data which can get close to the effective memory speed of a computer.

It does this while retaining full data integrity. No data is ever lost within this format, nor is any data adjusted. If one were to import a NetCDF file into BBF, one could fully rebuild the original NetCDF file from the BBF file itself. In the presentation the added benefits of using the BBF will be highlighted by comparing and benchmarking it to traditional formats such as NetCDF, CSV, ASCII, etc.

In January 2025, BEACON 1.0.0 was made publicly available as an open-source software, allowing everyone to set-up their own BEACON node to enhance the access to their data, while at the same time being able to reduce the storage size of their entire data collection without losing any information. More technical details, example applications and general information on BEACON can be found on the website https://beacon.maris.nl/.

How to cite: Krijger, T., Thijsse, P., Kooyman, R., and Schaap, D.: BEACON Binary Format (BBF) - Optimizing data storage and access to large data collections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4277, https://doi.org/10.5194/egusphere-egu25-4277, 2025.

EGU25-5977 | Orals | ESSI2.13

A comparative study of algorithms for lossy compression of 2-d meteorological gridded fields 

Uwe Ehret, Jieyu Chen, and Sebastian Lerch

Meteorological observations (e.g. from weather radar) and the output of meteorological models (e.g. from reanalyses or forecasts) are often stored and used in the form of time series of 2-d spatial gridded fields. With increasing spatial and temporal resolution of these products, and with the transition from providing single deterministic fields to providing ensembles, their size has dramatically increased, which makes use, transfer and archiving a challenge. Efficient compression of such fields - lossy or lossless - is required to solve this problem.

The goal of this work was therefore to apply several lossy compression algorithms for 2d spatial gridded meteorological fields, and to compare them in terms of compression rate and information loss compared to the original fields. We used five years of hourly observations of rainfall and 2m air temperature on a 250 x 400 km region over central Germany on a 1x1 km grid for our analysis.

In particular, we applied block averaging as a simple benchmark method, Principal Component Analysis, Autoencoder Neural Network (Hinton and Salakhutdinov, 2006) and the Ramer-Douglas-Peucker algorithm (Ramer, 1972; Douglas and Peucker, 1973) known from image compression. Each method was applied for various compression levels, expressed as the number of objects of the compressed representation, and then the (dis-)similarity of the original field and the fields reconstructed from the compressed fields was measured by Mean Absolute Error, Mean Square Error, and the Image Quality Index (Wang and Bovik, 2002). First results indicate that even for spatially heterogeneous fields like rainfall, very high compression can be achieved with small error.

 

References

Douglas, D., Peucker, T.: Algorithms for the reduction of the number of points required to represent a digitized line or its caricature. In: The Canadian Cartographer. Bd. 10, Nr. 2, 1973, ISSN 0008-3127, S. 112–122, 1973.

Hinton, G. E., & Salakhutdinov, R. R.: Reducing the dimensionality of data with neural networks. science, 313(5786), 504-507, 2006.

Ramer, U.: An iterative procedure for the polygonal approximation of plane curves, Computer Graphics and Image Processing, 1, 244-256, http://dx.doi.org/10.1016/S0146-664X(72)80017-0, 1972.

Zhou Wang, and A. C. Bovik: A universal image quality index, IEEE Signal Processing Letters, 9, 81-84, 10.1109/97.995823, 2002.

How to cite: Ehret, U., Chen, J., and Lerch, S.: A comparative study of algorithms for lossy compression of 2-d meteorological gridded fields, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5977, https://doi.org/10.5194/egusphere-egu25-5977, 2025.

EGU25-7371 | ECS | Orals | ESSI2.13

Evaluating Advanced Scientific Compressors on Climate Datasets 

Robert Underwood, Jinyang Liu, Kai Zhao, Sheng Di, and Franck Cappello

    As climate and weather scientists strive to increase accuracy and understanding of our world, models of weather and climate have increased in their resolution to square kilometers scale and become more complex increasing their demands for data storage. A recent study SCREAM run at 3.5km resolution produced nearly 4.5TB of data per simulated day, and the recent CMIP6 simulations produced nearly 28PB of data. At the same time, storage and power capacity at facilities conducting climate experiments are not increasing at the same rate as the volume of climate and weather datasets leading to a pressing challenge to reduce data volumes. While some in the weather and climate community have adopted lossless compression, these techniques frequently produce compression ratios on the order of 1.3$\times$, which are insufficient to alleviate storage constraints on facilities. Therefore, additional techniques, such as science-preserving lossy compression that can achieve higher compression ratios, are necessary to overcome these challenges.

    While data compression is an important topic for climate and weather applications, many of the current assessments of the effectiveness of climate and weather datasets do not consider the state of the art in compressor design and instead, asses scientific compressors that are 3-11 years old, substantially behind the state of the art. In this report: 

 

  •  We assess the current state of the art in advanced scientific lossy compressors against the state of the art in quality assessment criteria proposed for the ERA5 dataset to assess the current gaps between needed performance requirements and the capabilities of the current compressors.
  • We present new capabilities that allow us to build an automated, user-friendly, and extensible pipeline for quickly finding compressor configurations that maximize compression ratios while preserving scientific integrity of the data using codes developed as part of the NSF FZ project.
  • We demonstrate a number of capabilities that facilitate use within in the weather and climate community including NetCDF, HDF5, and GRIB file format support; support for innovation via Python, R, and Julia as well as low level languages such as C/C++; and the implementations of commonly used climate quality metrics including dSSIM, and the ability to extend to add new metrics in high-level languages
  • Utilizing this pipeline, We find that with advanced scientific compressors, it is possible to achieve a 6.4x improvement or more in compression ratio over previously evaluated compressors

How to cite: Underwood, R., Liu, J., Zhao, K., Di, S., and Cappello, F.: Evaluating Advanced Scientific Compressors on Climate Datasets, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7371, https://doi.org/10.5194/egusphere-egu25-7371, 2025.

EGU25-11118 | Orals | ESSI2.13

Too Big to Handle? Hexagonizing LIDAR and Satellite Data in Geoscience Applications 

Bo Møller Stensgaard, Casper Bramm, Marie Katrine Traun, and Søren Lund Jensen

The exponential growth of LIDAR and satellite data in geoscience presents both opportunities and challenges for users. Traditional data handling methods often struggle with the sheer volume and complexity of these datasets, hindering easy accessibility, efficient analysis and decision-making processes. This presentation introduces the Scandinavian Highlands HEX-Responder platform and database structure, a cutting-edge solution that leverages the power of hexagonal discrete global grid system, Uber H3, and developed processes to revolutionize geospatial data management, fast responsive visualization and analysis.

We will showcase real-world applications, highlighting the platform's potential to accelerate scientific discovery and improve decision-making processes using satellite and remote sensing data.

The platform’s approach offers several advantages over conventional methods:

  • Efficient data organization and retrieval
  • Improved advanced spatial data analyses opportunities
  • Seamless integration of multi-scale and multi-dimensional data without losing information
  • Enhanced, responsive and fast visualisation capabilities

Our ELT (extract, load, transform) and subsequent visualisation procedure can be applied to any big raster data formats. First, the raw raster data is transformed into optimised parquet files through chunked reading and compression based on a low-resolution H3 hexagon cell index (hexagonization), enabling rapid data import to a column-oriented database management system for big data storage, processing and analytics. The H3 cell organisation is preserved in the database through partitioned fetching for visualisation on the platform. This method allows for horizontal scaling and accurate multi-resolution aggregation, preserving data integrity across scales and significantly overcomes typical computational memory limitations.

The platform's capabilities are exemplified by its approach to LIDAR and satellite emissivity data processing using the H3 grid. High-resolution LIDAR data is efficiently gridded and visualized to H3 resolution level 15 hexagons (0.9m2 hexagon cells). The gridding preserves all original pixel raster points while providing aggregated views for seamless zooming.

Another prime example of the capabilities is the handling of NASA’s ASTER Global Emissivity Data (100m resolution). Here, our pipeline transformed 2.1 terabytes of extracted raw CSV-data derived from NASA’s emissivity data into a compressed format based on the H3 index occupying only 593 gigabytes in the database.

This approach not only saves data storage space but also dramatically improves data accessibility and processing speed for the users, allowing users to work in a responsive environment with this massive dataset in ways previously not possible. Each hexagon represents an opportunity to store unlimited amount, types and categories of pre-processed data for more integrative analyses and data insight.

By hexagonizing LIDAR and satellite data, the HEX-Responder platform enables users to explore massive datasets with ease and efficiency in a responsive environment. The integrated procedures allow for detailed information maintenance and retrieval, paving the way for advanced predictive modelling in geoscience applications using earth observation data in a new way.  

How to cite: Stensgaard, B. M., Bramm, C., Traun, M. K., and Jensen, S. L.: Too Big to Handle? Hexagonizing LIDAR and Satellite Data in Geoscience Applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11118, https://doi.org/10.5194/egusphere-egu25-11118, 2025.

EGU25-12760 | ECS | Posters on site | ESSI2.13

Tree-Based Adaptive Data Reduction Techniques for Scientific Simulation Data 

Niklas Böing, Johannes Holke, Achim Basermann, Gregor Gassner, and Hendrik Fuchs

Large-scale Earth system model simulations produce huge amounts of data. Due to limited I/O bandwidth and available storage space this data often needs to be reduced before written to disk or stored permanently. Error-bounded lossy compression is an effective approach to tackle the trade-off between accuracy and storage space.

We are exploring and discussing lossless as well as error-bounded lossy compression based on tree-based adaptive mesh refinement/coarsening (AMR) techniques. Our lossy compression schemes allow for absolute and relative error bounds. The data reduction methods are closely linked to an underlying (adaptive) mesh which easily permits error regions of different error tolerances and criteria – in particular, we allow nested domains of varying error tolerances specified by the user. Moreover, some of the compressed data structures allow for an incremental decompression in the resolution of the data which may be favorable for transmission and visualization.

We implement these techniques as the open source tool cmc, which is based on the parallel AMR library t8code. The compression tool can be linked to and used by arbitrary simulation applications or executed as a post-processing step. We show different application results of the compression in comparison to current state-of-the-art compression techniques on several benchmark data sets.

How to cite: Böing, N., Holke, J., Basermann, A., Gassner, G., and Fuchs, H.: Tree-Based Adaptive Data Reduction Techniques for Scientific Simulation Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12760, https://doi.org/10.5194/egusphere-egu25-12760, 2025.

EGU25-13394 | ECS | Orals | ESSI2.13

Challenges and perspectives of climate data compression in times of kilometre-scale models and generative machine learning 

Milan Klöwer, Tim Reichelt, Juniper Tyree, Ayoub Fatihi, and Hauke Schulz

Climate data compression urgently needs new standards. The continuously growing exascale mountain of data requires compressors that are widely used and supported, essentially hiding the compression details from many users. With the advent of AI revolutionising scientific computing, we have to set the rules of this game. Minimizing information loss, maximising compression factors, at any resolution, grid and dataset size, for all variables, with chunks and random access, while preserving all statistics and derivatives, at a reasonable speed — are squaring the compression circle. Many promising compressors are hardly used as trust among domain scientists is hard to gain: The large spectrum of research questions and applications using climate data is very difficult to satisfy simultaneously.

Here, we illustrate the motivation behind the newly defined climate data compression benchmark ClimateBenchPress, designed as a quality check in all those dimensions of the problem. Any benchmark will inevitably undersample this space, but we define datasets from atmosphere, ocean, and land as well as evaluation metrics to pass. Results are presented as score cards, highlighting strengths and weaknesses for every compressor.

The bitwise real information content shows a systematic way in case no error bounds are known. In the case of the ERA5 reanalysis, errors are estimated and allow us to categorize many variables into linear, log and beta distributions with values bounded from zero, one or both sides, respectively. This allows us to define error thresholds arising from observation and model errors directly, providing another alternative to the still predominant subjective choices. Most error-bounded compressors come with parameters that can be automatically chosen following this analysis.

Also new data formats are on the horizon: Chunking and hierarchical data structures allow and force us to adapt compressors to spatially or length-scale dependent information densities. Extreme events, maybe counterintuitively, often increase the compressibility through higher uncertainties, but lie on the edge or outside of the training data for machine learned-compressors. This again increases the need for well-tested compressors. Benchmarks like ClimateBenchPress are required to encourage new standards for safe lossy climate data compression.

How to cite: Klöwer, M., Reichelt, T., Tyree, J., Fatihi, A., and Schulz, H.: Challenges and perspectives of climate data compression in times of kilometre-scale models and generative machine learning, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13394, https://doi.org/10.5194/egusphere-egu25-13394, 2025.

EGU25-13567 | Posters on site | ESSI2.13

Tables as a way to deal with a variety of data formats and APIs in data spaces 

Joan Masó, Marta Olivé, Alba Brobia, Nuria Julia, Nuria Cartell, and Uta Wehn

The Green Deal Data Space is born in the big data paradigm where there is a variety of data formats and data models that are exposed as files or web APIs. As a result, we need to default in simple data structure that is transversal enough to be able to represent most of the more specific data models, formats and API payloads. Many data models present a structure that can be represented as tables.

TAPIS stands for "Tables from APIS". It is a JavaScript code that uses a common data model that is an array of objects with a list of properties that can contain a simple or a complex value. In TAPIS offers a series of operations that use one or more arrays of objects as inputs and produce a new array of objects as an output. There are operations that create the arrays of objects from files or API queries (a.k.a. data import), others that manipulate the objects (e.g. merge two arrays in a single one) and some operations that generate visual representations of the common data structure including tabular, a map, a graph, etc.

TAPIS is limited by its own data model. While many of the data models can be mapped to the common data model, a multidimensional data cube or a data tree cannot be represented in a single table in an efficient way. In the context of the Green Deal Data Space, most of the sensor data, statistical data, geospatial feature based data and administrative data can be considered object based data and can be used in TAPIS. TAPIS is able to connect to Sensor Things API (the sensor protocol selected in AD4GD and CitiObs), S3 buckets (the internal cloud repository used in AD4GD), GeoNetwork (the geospatial metadata catalogue selected in AD4GD and more4nature), and the OGC API features and derivates (the modern web API interfaces standardized by the OGC) but other data inputs will be incorporated, such as Citizen Science data sources and other popular APIs used in the more4nature project. More analytical functionalities are going to be incorporated in the CitiObs project. As part of the AD4GD Green Deal Information Model, there is an operation to associate semantics to each column of a table by linking it to a URI that defines the concept in an external vocabulary (as well as units of measure if appropriate). In order to be compatible with the data space architecture recommended by the International Data Space Association, we are working on supporting the catalogue of the Eclipse Data Connector, and to be able to negotiate a digital contract as a previous step to request access to the relevant data offered in the data space. To do so, we are working on incorporating the data space protocol as part of the TAPIS operations for data import. TAPIS is available as open source at https://github.com/joanma747/TAPIS.

AD4GD, CitiObs and more4nature are Horizon Europe projects co-funded by the European Union, Switzerland and the United Kingdom.

How to cite: Masó, J., Olivé, M., Brobia, A., Julia, N., Cartell, N., and Wehn, U.: Tables as a way to deal with a variety of data formats and APIs in data spaces, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13567, https://doi.org/10.5194/egusphere-egu25-13567, 2025.

Early career scientists rarely have the resources to work with earth observation data at continental to global scale. This is caused by a combination of factors: large scale data analysis often involves teamwork, connecting data scientists, code developers, IT specialists, statisticians and geoscientists. Young researchers are rarely able to coordinate such a team. Meanwhile, all scientists can have relevant ideas or pose powerful research questions that merit investigation. Copernicus Data Space Ecosystem provides a public, free platform for large-scale processing of earth observation data. It combines instant access to all Sentinel satellite imagery with cloud-based processing in the form of API requests and a powerful browser-based viewing interface. This new approach is enabled by storing the data in a different way: uncompressed formats such as JPEG2000, COG or ZARR support subsetting and querying the image rasters without first unzipping the file, thereby allowing direct streaming of only the area and bands that the user requests. Additionally, this means that most calculations and visualization tasks can be carried out on the server side, directly within the request process. The backend tasks of data storage and management are taken care of by the system, while the user can concentrate on the research itself.

Copernicus Data Space Ecosytem supports several API families. OGC API-s directly enable the creation of Open Geospatial Consortium compatible map products such as WMS, WMTS, WFS or WCS services. These can be accessed with GIS software or displayed in web map tools. OData, STAC, and OpenSearch are Catalog API-s, supporting the querying and of datasets in preparation for analysis. Sentinel Hub is an API family that can handle queries, raster operations, and raster-vector integration for deriving statistics. The main advantages of Sentinel Hub API-s are their efficient use and integration with advanced visualization in the Copernicus Browser.

OpenEO is a fully open-source data analysis framework designed specifically to support FAIR principles. It is independent from data formats with its own data cube format, and can be edited using several coding languages. openEO connects to all STAC-compliant repositories, enabling integration between Sentinel data and other sources. Processing tools include many mathematical operations, but also standard machine learning processes. The system is designed with upscaling in mind: the command structure is the same for small and large areas, with storage and asynchronous processing managed by the backend.

Both API families come with a comprehensive scheme of tutorials and documentation to allow step-by-step learning, and an online Jupyter Lab virtual machine facility. Therefore, early-career scientists with a basic understanding of programming can quickly learn to apply their domain knowledge, while creating solutions that are easy to share and replicate.

All in all, Copernicus Data Space Ecosystem is a transformative tool for earth observation, significantly lowering the bar for applying earth observation at large scale in the geosciences.

How to cite: Zlinszky, A. and Milcinski, G.: Copernicus Data Space Ecosystem empowers early-career scientists to do global scale earth observation data analysis, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15282, https://doi.org/10.5194/egusphere-egu25-15282, 2025.

EGU25-15672 | ECS | Posters on site | ESSI2.13

Scaling Down ESS Datasets: Lessons from the EERIE Project on Compression 

Oriol Tinto, Xavier Yepes, and Pierre Antoine Bretonniere

The rapid growth of Earth System Sciences (ESS) datasets, driven by high-resolution numerical modeling, has outpaced storage and data-sharing capabilities. To address these challenges, we investigated lossy compression techniques as part of the EERIE project, aiming to significantly reduce storage demands while maintaining the scientific validity of critical diagnostics.

Our study examined two key diagnostics: Sea Surface Height (SSH) variability and ocean density, essential for understanding climate dynamics. Leveraging tools such as SZ3 and enstools-compression, we achieved data volume reductions by orders of magnitude without compromising the diagnostics' accuracy. Compression-induced differences were found to be negligible compared to the inherent variability between model outputs and observational datasets, underscoring the robustness of these methods.

Additionally, our work highlighted inefficiencies in current workflows, including the prevalent use of double precision in post-processing. We proposed improvements to align data precision with the original model outputs, further optimizing storage and computation. Integrating lossy compression into existing workflows via widely used formats like NetCDF and HDF5 demonstrates a practical path forward for sustainable ESS data management.

This study showcases the transformative potential of lossy compression to make high-resolution datasets more manageable, ensuring they remain accessible and scientifically reliable for stakeholders while significantly reducing resource demands.

How to cite: Tinto, O., Yepes, X., and Bretonniere, P. A.: Scaling Down ESS Datasets: Lessons from the EERIE Project on Compression, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15672, https://doi.org/10.5194/egusphere-egu25-15672, 2025.

EGU25-15864 | Posters on site | ESSI2.13

The Sentinels EOPF Toolkit: Driving Community Adoption of the Zarr data format for Copernicus Sentinel Data 

Sabrina H. Szeto, Julia Wagemann, Emmanuel Mathot, and James Banting

The Standard Archive Format for Europe (SAFE) specification has been the established approach to publishing Copernicus Sentinel data products for over a decade. While SAFE has pushed the ecosystem forward through new ways to search and access the data, it is not ideal for processing large volumes of data using cloud computing. Over the last few years, data standards like STAC and cloud-native data formats like Zarr and COGs have revolutionised how scientific communities work with large-scale geospatial data and are becoming a key component of new data spaces, especially for cloud-based systems.

The ESA Copernicus Earth Observation Processor Framework (EOPF) will be providing access to “live” sample data from the Copernicus Sentinel missions -1, -2 and -3 in the new Zarr data format. This set of reprocessed data allows users to try out accessing and processing data in the new format and experiencing the benefits thereof with their own workflows.

This presentation introduces a community-driven toolkit that facilitates the adoption of the Zarr data format for Copernicus Sentinel data. The creation of this toolkit was driven by several motivating questions: 

  • What common challenges do users face and how can we help them overcome them? 
  • What resources would make it easier for Sentinel data users to use the new Zarr data format? 
  • How can we foster a community of users who will actively contribute to the creation of this toolkit and support each other?

The Sentinels EOPF Toolkit team, comprising Development Seed, SparkGeo and thriveGEO, together with a group of champion users (early-adopters), are creating a set of Jupyter Notebooks and plug-ins that showcase the use of Zarr format Sentinel data for applications across multiple domains. In addition, community engagement activities such as a notebook competition and social media outreach will bring Sentinel users together and spark interaction with the new data format in a creative yet supportive environment. Such community and user adoption efforts are necessary in order to overcome adoption and uptake barriers and to build up trust and excitement to try out new technologies and new developments around data spaces.

In addition to introducing the Sentinels EOPF Toolkit, this presentation will also highlight lessons learned from working closely with users on barriers they face in adopting the new Zarr format and how to address them. 

How to cite: Szeto, S. H., Wagemann, J., Mathot, E., and Banting, J.: The Sentinels EOPF Toolkit: Driving Community Adoption of the Zarr data format for Copernicus Sentinel Data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15864, https://doi.org/10.5194/egusphere-egu25-15864, 2025.

EGU25-16791 | ECS | Posters on site | ESSI2.13

Development and performance evaluation of dissolved oxygen climatology in the Northwestern Pacific 

Jae-Ho Lee, Yong Sun Kim, and Sung-Dae Kim

This study developed a monthly regional atlas for dissolved oxygen (DO) with a quarter-degree horizontal resolution and 73 vertical levels over the northwestern Pacific. We used observed profiles of 586,851 and gridded World Ocean Atlas 2023 (WOA23) with 1° resolution by adopting simple kriging horizontal interpolation and vertical stabilizing techniques to produce the new atlas. This approach efficiently mitigates artificial water masses and statistical noise. The new DO climatology provides detailed information along coasts and renders realistic oxygen distribution associated with the current system in the western North Pacific compared to WOA23. A meridional section demonstrates that the newly developed atlas does not yield artificial noise-like spikes frequently observed in WOA23 in the East Sea. This study expects that this new atlas can allow bio-geochemical numerical models to enhance diagnostic and forecasting performance.

How to cite: Lee, J.-H., Kim, Y. S., and Kim, S.-D.: Development and performance evaluation of dissolved oxygen climatology in the Northwestern Pacific, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16791, https://doi.org/10.5194/egusphere-egu25-16791, 2025.

EGU25-17102 | Posters on site | ESSI2.13

Calculation of Gridded Surface Current from Observed Lagrangian Trajectories in the East Sea 

Mi-Jin Jang, Jae-Ho Lee, and Yong Sun Kim

Surface ocean current is crucial for enhancing the safety and efficiency of maritime logistics and transportation, boosting fisheries production and management, and supporting military operations. This study analyzed 25,342 trajectories from NOAA’s Global Drifter Program (1991–2020), 12 from KIOST, and 63 from KHOA (2015–2024). The surface drifters entering the East Sea were extracted, and a five-step quality control process was implemented. Unobserved values were removed, quality control was applied based on drogue lost, abnormally speed or stuck, unrealistic acceleration. To estimated the gridded oceanic current with high-resolution, we removed the Ekman current and tides from the observed velocity and took advantage of a simple kriging approach. The validation against existing datasets confirmed that major ocean currents exhibited similar patterns compared to absolute geostrophic current from the satellite-based altimetry. The constructed dataset is expected to contribute to the accurate identification of surface current movements and the development of realistic models that incorporate regional characteristics based on data assimilation.

How to cite: Jang, M.-J., Lee, J.-H., and Kim, Y. S.: Calculation of Gridded Surface Current from Observed Lagrangian Trajectories in the East Sea, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17102, https://doi.org/10.5194/egusphere-egu25-17102, 2025.

The Copernicus Program is the largest and most successful public space program globally. It provides continuous data across various spectral ranges, with an archive exceeding 84 petabytes and a daily growth of approximately 20 TB, both of which are expected to increase further. The openness of its data has contributed to the widespread use of Earth observation and the development of commercial products utilizing open data in Europe and worldwide. The entire archive, along with cloud-based data processing capabilities, is available free of charge through the Copernicus Data Space Ecosystem initiative and continues to evolve to meet global user standards. 

This paper presents the process of creating the STAC Copernicus Data Space Ecosystem catalog—the largest and most comprehensive STAC catalog in terms of metadata globally. It details the workflow, starting from the development of a metadata model for Sentinel data, through efficient indexing based on the original metadata files accompanying the products, to result validation and backend system ingestion (via database DSN). A particular highlight is that this entire process is executed using a single tool, eometadatatool, initially developed by DLR, further enhanced, and released as open-source software by the CloudFerro team. The eometadatatool facilitates metadata extraction from the original files accompanying Copernicus program products and others (e.g., Landsat, Copernicus Contributing Missions) using a CSV file containing the metadata name, the file in which it occurs, and the path to the key within the file. Since the CDSE repository operates as an S3 resource offering users free access, the tool supports product access via S3 resources by default, configurable through environment variables. All the above characterizes eometadatatool as the most powerful stactool (a high-level command-line tool and Python library for working with STAC) package available, providing both valid STAC items and a method for uploading them to the selected backend. 

The standard specification itself has been influenced by the CDSE catalog development process, which contributed to the evolution of the standard by introducing version 1.1 and updated extensions (storage, eo, proj) that better meet user needs. The paper discusses the most significant modifications, their impact on the catalog’s functionality, and outlines the main differences. 

Particular attention is given to performance optimization due to the substantial data volume and high update frequency. The study examines the configuration and performance testing (using Locust) of the frontend layer (stac-fastapi-pgstac) and backend (pgstac). The stac-fastapi-pgstac implementation was deployed on a scalable Kubernetes cluster and underwent a product hydration process (specific to managing JSON data in pgstac), leveraging Python's native capabilities for this task. The pgstac schema was deployed on a dedicated bare-metal server with a PostgreSQL database, utilizing master-worker replication enabled through appropriate pgstac configuration. Both software tools are open source, and the achieved optimal configurations are documented and will be presented in detail. 

The presented solution empowers the community to fully utilize the new catalog, leverage its functionalities, and access open tools that enable independent construction of STAC catalogs compliant with ESA and community recommendations. 

How to cite: Niemyjski, M. and Musiał, J.: Building the Copernicus Data Space Ecosystem STAC Catalog: Methodologies, Optimizations, and Community Impact, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17171, https://doi.org/10.5194/egusphere-egu25-17171, 2025.

EGU25-17172 | ECS | Orals | ESSI2.13

Neural Embedding Compression for Earth Observation Data – an Ablation Study 

Amelie Koch, Isabelle Wittmann, Carlos Gomez, Rikard Vinge, Michael Marszalek, Conrad Albrecht, and Thomas Brunschwiler

The exponential growth of Earth Observation data presents challenges in storage, transfer, and processing across fields such as climate modeling, disaster response, and agricultural monitoring. Efficient compression algorithms—either lossless or lossy—are critical to reducing storage demands while preserving data utility for specific applications. Conventional methods, such as JPEG and WebP, rely on hand-crafted base functions and are widely used. However, Neural Compression, a data-driven approach leveraging deep neural networks, has demonstrated superior performance by generating embeddings suitable for high levels of entropy encoding, enabling more accurate reconstructions at significantly lower bit rates.

In our prior work, we developed a Neural Compression pipeline utilizing a masked auto-encoder, embedding quantization, and an entropy encoder tailored for satellite imagery [1]. Instead of reconstructing original images, we evaluated the reconstructed embeddings for downstream tasks such as image classification and semantic segmentation. In this study, we conducted an ablation analysis to quantify the contributions of individual pipeline components—encoder, quantizer, and entropy encoder—toward the overall compression rate. Our findings reveal that satellite images achieve higher compression rates compared to ImageNet samples due to their lower entropy. Furthermore, we demonstrate the advantages of learned entropy models over hand-crafted alternatives, achieving better compression rates, particularly for datasets with seasonal or geospatial coherence. Based on these insights, we provide a list of recommendations for optimizing Neural Compression pipelines to enhance their performance and efficiency.

This work was conducted under the Embed2Scale project, supported by the Swiss State Secretariat for Education, Research and Innovation (SERI contract no. 24.00116) and the European Union (Horizon Europe contract no. 101131841).

[1] C. Gomes and T. Brunschwiler, “Neural Embedding Compression for Efficient Multi-Task Earth Observation Modelling,” IGARSS 2024, Athens, Greece, 2024, pp. 8268-8273, doi: 10.1109/IGARSS53475.2024.10642535.

How to cite: Koch, A., Wittmann, I., Gomez, C., Vinge, R., Marszalek, M., Albrecht, C., and Brunschwiler, T.: Neural Embedding Compression for Earth Observation Data – an Ablation Study, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17172, https://doi.org/10.5194/egusphere-egu25-17172, 2025.

EGU25-17326 | Orals | ESSI2.13

The UK EO DataHub - a pathfinder programme to develop a data space for UK industry, public and academic sectors 

Philip Kershaw, Rhys Evans, Fede Moscato, Dave Poulter, Alex Manning, Jen Bulpett, Ed Williamson, John Remedios, Alastair Graham, Daniel Tipping, and Piotr Zaborowski

The EO DataHub is a new national data space which has been under development as part of a two-year pathfinder programme to facilitate the greater exploitation of EO data for UK industry, public sector and academia. The project has been led by the UK National Centre for Earth Observation partnered with public sector bodies, the UK Space Agency, Met Office, Satellite Applications Catapult and National Physical Laboratory and enlisting commercial suppliers for the development and delivery of the software.

The Hub joins a crowded space in this sector as it joins a growing number of similar such platforms. However, as a national platform (with government as an anchor tenant) it is seeking to provide a unique offering as a trusted source of data, integrating curated data products from the science community building on UK strengths in climate research.

The architecture can be considered as a three layer model. At the base layer, different data sources are integrated - both commercial (Airbus and Planet Labs) and academic providers - from the CEDA data archive (https://archive.ceda.ac.uk) hosted on the JASMIN supercomputer (https://jasmin.ac.uk). The data catalogue now includes high and very high resolution SAR and optical products, Sentinel, UK Climate Projections, CMIP (https://wcrp-cmip.org), CORDEX (https://cordex.org) and outputs from EOCIS (https://eocis.org) consisting of a range of satellite-derived climate data products.

The middle layer, the Hub Platform provides services and APIs including federated search which integrates the data from the various providers, image visualisation, a workflow engine, user workspaces and interactive analysis environments. These build on the work of ESA's EOEPCA (https://eoepca.org) and apply open standards from the Open Geospatial Consortium and STAC (https://stacspec.org/) for cataloguing. In providing this suite of services, the goal is to provide a toolkit to facilitate application developers and EO specialists in building new applications and tools to exploit the data. This forms the final layer in the architecture: as part of the programme, three example application scenarios have been funded, each partnered with a target set of users. These include 1) an application taking climate projections and land surface temperature datasets to provide risk assessments for land assets (led by SparkGeo); 2) a land cover application (Spyrosoft) and finally 3), rather than an application in its own right, a project to develop a client toolkit for use with Jupyter Notebooks and a plugin integrating the Hub’s functionality into the open source GIS desktop application QGIS (work led by Oxidian).

Over the course of the programme, running in parallel to the system development, a dedicated study has been undertaken to develop a model for future sustainability of the platform tackling engagement with potential users and cost models. At the beginning, a funding call seeded early pilots to investigate application scenarios that the platform could support. As this initial phase of the Hub completes, work is underway to engage with early adopters and provide training resources for new users.

How to cite: Kershaw, P., Evans, R., Moscato, F., Poulter, D., Manning, A., Bulpett, J., Williamson, E., Remedios, J., Graham, A., Tipping, D., and Zaborowski, P.: The UK EO DataHub - a pathfinder programme to develop a data space for UK industry, public and academic sectors, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17326, https://doi.org/10.5194/egusphere-egu25-17326, 2025.

EGU25-17799 | Posters on site | ESSI2.13

Data Spaces and geodata workflows for environmental protection 

Matthes Rieke, Benjamin Proß, Simon Jikra, Sotiris Aspragkathos, Iasonas Sotiropoulos, Stamatia Rizou, and Lisa Pourcher

The concept of Data Spaces has gained traction in recent years. Major representatives emerged which have the technological maturity as well as support by relevant decision and policy makers (e.g.  the International Data Spaces Association (IDSA) or Gaia-X). These follow different architectural approaches. In this session we want to illustrate the challenges of integrating the Data Space architectures with established concepts of Spatial Data Infrastructure.

During the next 4 years, the ENFORCE project (Empower citizeNs to join Forces with public authORities in proteCting the Environment) is dedicated to fostering sustainable practices and ensuring environmental regulatory compliance by integrating citizen science with innovative technologies. By employing Living Labs and citizen science methodologies, ENFORCE will create innovative tools that bridge the gap between data reporting, monitoring, and policy enforcement. The project integrates data collection (e.g. Copernicus satellite data), analysis, and stakeholder participation to meet these goals. ENFORCE will leverage geospatial intelligence and explainable AI to enhance environmental governance. These tools and strategies will be tested and refined at eight pilot sites in seven countries, supplemented by capacity-building and policy recommendation efforts.

The design and development of a geospatial information infrastructure that supports the envisioned data workflows is a key challenge addressed by ENFORCE. This infrastructure will prioritize the integration of OGC API-driven systems into the Data Space ecosystem, forming a central component of the project’s agenda. Through development of a blueprint architecture for integration, the project will identify gaps and missing components in current systems, aligning with standards such as the FAIR principles and open data. The concepts will be facilitated in an ENFORCE “Tools Plaza”, an innovative platform providing data science and analytical capabilities for environmental compliance workflows.

How to cite: Rieke, M., Proß, B., Jikra, S., Aspragkathos, S., Sotiropoulos, I., Rizou, S., and Pourcher, L.: Data Spaces and geodata workflows for environmental protection, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17799, https://doi.org/10.5194/egusphere-egu25-17799, 2025.

EGU25-19418 | Posters on site | ESSI2.13

Lossy Data Compression Exploration in an Online Laboratory and the Link to HPC Design Decisions 

Karsten Peters-von Gehlen, Juniper Tyree, Sara Faghih-Naini, Peter Dueben, Jannek Squar, and Anna Fuchs

It is apparent that the data amounts expected to be generated by current and upcoming Earth System Science research and operational activities stress the capabilities of HPC and associated data infrastructures. Individual research projects focusing on running global Earth System Models (ESMs) at spatial resolution of 5km or less can easily occupy several petabytes on disk. With multiple of such projects running on a single HPC infrastructure, the challenge of storing the data alone becomes apparent. Further, community-driven activities like model intercomparison projects – which are conducted for both conventional and high-resolution model setups – add to the aforementioned strain on storage systems. Hence, when planning for next-generation HPC systems, the storage requirements of state-of-the-art ESM-centered projects have to be clear so that systems are still fit-for-use 5 years down the road from the initial planning stage.

As computational hardware costs per performance unit (FLOP or Byte) are not decreasing anymore like they have in the past decades, HPC system key figures do not increase substantially anymore from one generation to the next. The mismatch between demands of research and what future systems can offer is therefore clear.

One apparent solution to this problem is to simply reduce the amount of data from ESM simulations stored on a system. Data compression is one candidate to achieve this. Current ESM projects already utilize application-side lossless compression techniques, which help reduce storage space. However, decompression may incur performance penalties, especially when read patterns misalign with the compression block sizes. Lossy compression offers the potential for higher compression rates, without access penalties for data retrieval. However, its suitability is highly content-dependent, raising questions about which lossy compression methods are best suited for specific datasets. On a large scale, applying lossy compression also prompts the consideration of how such data reduction could shape the design of next-generation HPC architectures.

With lossy compression not being very popular in the ESM-community so far, we present a key development of the ongoing ESiWACE3 project: an openly accessible Jupyter-based online laboratory for testing lossy compression techniques on ESM output datasets. This online tool currently comes with a set of notebooks allowing users to objectively evaluate the impact lossy compression has on analyses performed on the compressed compared to the input data. With some compressors promising compression ratios of 10x-1000x, providing such tools to ensure compression quality is essential. The motivation behind the online compression laboratory is to foster the acceptance of lossy compression techniques by conveying first-hand experience and immediate feedback of benefits or drawbacks of applying lossy compression algorithms. 

Going one step further, we illustrate the impacts that applying lossy-compression techniques on ESM data on large-scales can have on the design decisions made for upcoming HPC infrastructures. We illustrate, among others, that increased acceptance and application of lossy compression techniques enables more efficient resource utilization and allows for smarter reinvestment of funds saved from reduced storage demands, potentially leading to the acquisition of smaller systems and thus enabling increased research output per resource used.

How to cite: Peters-von Gehlen, K., Tyree, J., Faghih-Naini, S., Dueben, P., Squar, J., and Fuchs, A.: Lossy Data Compression Exploration in an Online Laboratory and the Link to HPC Design Decisions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19418, https://doi.org/10.5194/egusphere-egu25-19418, 2025.

EGU25-20188 | ECS | Posters on site | ESSI2.13

Creating TROPOMI superobservations for data assimilation and model evaluation 

Pieter Rijsdijk, Henk Eskes, Kazuyuki Miyazaki, Takashi Sekiya, and Sander Houweling

Satellite observations of tropospheric trace gases and aerosols are evolving rapidly. Recently launched instruments provide increasingly higher spatial resolutions with footprint diameters in the range of 2–8 km, with daily global coverage for polar orbiting satellites or hourly observations from geostationary orbit. Often the modelling system has a lower spatial resolution than the satellites used, with a model grid size in the range of 10–100 km. When the resolution mismatch is not properly bridged, the final analysis based on the satellite data may be degraded. Superobservations are averages of individual observations matching the resolution of the model and are functional to reduce the data load on the assimilation system. In this paper, we discuss the construction of superobservations, their kernels and uncertainty estimates. The methodology is applied to nitrogen dioxide tropospheric column measurements of the TROPOMI instrument on the Sentinel-5P satellite. In particular, the construction of realistic uncertainties for the superobservations is non-trivial and crucial to obtaining close to optimal data assimilation results. We present a detailed methodology to account for the representativity error when satellite observations are missing due to e.g. cloudiness. Furthermore, we account for systematic errors in the retrievals leading to error correlations between nearby individual observations contributing to one superobservation. Correlation information is typically missing in the retrieval products where an error estimate is provided for individual observations. The various contributions to the uncertainty are analysed: from the spectral fitting, the estimate of the stratospheric contribution to the column and the air-mass factor. The method is applied to TROPOMI data but can be generalised to other trace gases such as HCHO, CO, SO2 and other instruments such as OMI, GEMS and TEMPO. The superobservations and uncertainties are tested in the ensemble Kalman filter chemical data assimilation system developed by JAMSTEC. These are shown to improve forecasts compared to thinning or compared to assuming fully correlated or uncorrelated uncertainties within the superobservation. The use of realistic superobservations within model comparisons and data assimilation in this way aids the quantification of air pollution distributions, emissions and their impact on climate.

How to cite: Rijsdijk, P., Eskes, H., Miyazaki, K., Sekiya, T., and Houweling, S.: Creating TROPOMI superobservations for data assimilation and model evaluation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20188, https://doi.org/10.5194/egusphere-egu25-20188, 2025.

EGU25-20430 | Orals | ESSI2.13

Compression and Aggregation: a CF data model approach 

David Hassell, Sadie Bartholomew, Bryan Lawrence, and Daniel Westwood

The CF (Climate and Forecast) metadata conventions for netCDF datasets describe means of "compression-by-convention", i.e. methods for compressing and decompressing data according to algorithms that are fully described within the conventions themselves. These algorithms, which can be lossless or lossy, are not applicable to arbitrary data, rather the data have to exhibit certain characteristics to make the compression worthwhile, or even possible.

Aggregation, available in CF-1.13, provides the utility of being able to view, as a single entity, a dataset that has been partitioned across multiple other independent datasets on disk, whilst taking up very little extra space on disk since the aggregation dataset contains no copies of the data in each component dataset. Aggregation can facilitate a range of activities such as data analysis, by avoiding the computational expense of deriving the aggregation at the time of analysis; archive curation, by acting as a metadata-rich archive index; and the post-processing of model simulation outputs, by spanning multiple datasets written at run time that together constitute a more cohesive and useful product. CF aggregation currently has cf-python and xarray implementations.

The conceptual CF data model does not recognise compression nor aggregation, choosing to view all CF datasets as if they were uncompressed and containing all of their own data. As a result, the cf-python data analysis library, that is built exactly on the CF data model, also presents datasets lazily to the user in this manner, without decompressing or re-combining the data in memory until the user actually accesses the data, at which time it occurs automatically. This approach allows the user to interact with their data in an intuitive and efficient manner; and also removes the need for the user to have to assimilate large parts of the CF conventions and having to create their own code for dealing with the compression and aggregation algorithms.

We will introduce compression by ragged arrays (as used by Discrete Sampling Geometry features, such as timeseries and trajectories) and dataset aggregation, with cf-python examples to demonstrate the ease of use that arises from using the CF data model interpretation of the data.

How to cite: Hassell, D., Bartholomew, S., Lawrence, B., and Westwood, D.: Compression and Aggregation: a CF data model approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20430, https://doi.org/10.5194/egusphere-egu25-20430, 2025.

EGU25-443 | Orals | BG2.2

New standards for isotope measurements of CO2 for atmospheric and biogeoscience applications 

Joële Viallon, Robert Wielgosz, Edgar Flores, Tiphaine Choteau, and Philippe Moussay

Progress in the development of pure CO2 gas standards for δ13C, δ18O and Δ47 measurements as well as CO2 in air gas standards (with mole fractions in the range 350 µmol/mol to 800 µmol/mol) for δ13C, δ18O measurements are described. Initial results indicate the potential to produce standards with internal consistencies at the 0.005 ‰ level for δ13C and standard uncertainties of 0.015 ‰ in relation to the VPDB scale, with the magnitude of the latter principally limited by the homogeneity of primary carbonate reference materials.
An initial driver for standards development was the requirement for appropriate calibration strategies and standards [1]  to support commercially developed laser-based instruments that have grown in number over the last decade. These analysers can measure real-time isotopic ratio variations of greenhouse gases, and notably CO2, allowing their application across a wide range of scientific and technical disciplines. The development of appropriate standards and calibration methods has required the links and traceability to primary carbonate materials via the IRMS dual inlet reference method to be re-examined.
Outputs of the project so far include:
Establishment of a facility to produce stable pure CO2 gas standards in 6L cylinders at 2 bar with δ13C values from -1 ‰ to +45 ‰ vs VPDB, with internal consistency approaching the 0.005 ‰ level, and an effective calibration option for dual inlet IRMS systems as demonstrated in the international comparison CCQM-P204 completed in 2021 [2];
Studies of Δ47 values of mixtures of different pure CO2 gas, and the reproducibility and stability of these and their potential to act as reference standards for clumped isotope ratio measurements with IRMS systems;
The development and validation of a cryogenic Air Trapping system to extract CO2 from air for determination of δ13C and δ18O-CO2 with IRMS, including a correction for the N2O present in samples. The facility is currently being used for another international comparison (CCQM-P239) of CO2 in in air standards from 15 institutes containing CO2 over the range of 380 μmol mol−1 to 800 μmol mol−1 and δ13C and δ18O-CO2 values from 1 ‰ to -43 ‰ and -7 ‰ to -35 ‰, respectively. The method demonstrates excellent reproducibility, with standard deviations of 0.005% and 0.05% for δ13C  and δ18O-CO2, respectively, and will demonstrate the level of equivalence of new CO2 in  air isotope  ratio standards currently being produced.
[1] Flores, E., Viallon, J., Moussay, P., Griffith, D. W. T. & Wielgosz, R. I. Calibration strategies for FT-IR and other isotope ratio infrared spectrometer instruments for accurate δ13C and δ18O measurements of CO2 in air. Anal. Chem. 89, 3648–3655 (2017).
[2]  J Viallon et a, Final report of CCQM-P204, comparison on CO2 isotope ratios in pure CO2,  2023 Metrologia 60 08026 DOI 10.1088/0026-1394/60/1A/08026

How to cite: Viallon, J., Wielgosz, R., Flores, E., Choteau, T., and Moussay, P.: New standards for isotope measurements of CO2 for atmospheric and biogeoscience applications, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-443, https://doi.org/10.5194/egusphere-egu25-443, 2025.

Mercury (Hg) stable isotopes have become a powerful tracer for understanding Hg sources and complex biogeochemical processes in the natural environment. Anomalies of even mass number mercury isotopes (even-MIF; Δ200Hg, Δ204Hg), in particular, have enabled the differentiation of Hg chemical forms (Hg0 vs. HgII) and their depositional pathways. This is because even-MIF occurs exclusively via upper atmospheric photo-oxidation, leaving HgII with a positive Δ200Hg value and Hg0 with a negative Δ200Hg value. Over the past several years, my research group has characterized even-MIF anomalies in atmospheric samples (gaseous Hg0, precipitation), seawater, zooplankton, and fish from high (Beaufort, Chukchi Sea) and mid-latitude oceans (West to Central Pacific Ocean). Our goal was to comprehensively trace sources, oxidation/removal pathways, and fate of Hg to open ocean food web. The results depict a clear Δ200Hg dichotomy, in which all samples from mid-latitude oceans have positive Δ200Hg (reflecting HgII) and the samples from high-latitude oceans have negative Δ200Hg (reflecting Hg0). The δ202Hg, which has been used to trace Hg sources (types of anthropogenic, natural sources) across a large spatial scale, show that, while high-latitude oceans exhibit values similar to that of background Hg, mid-latitude oceans have δ202Hg consistent with anthropogenic Hg. There is also a gradual dilution of zooplankton Hg concentration and anthropogenic δ202Hg signals from West to the Central Pacific Ocean. We summarize Hg sources and oxidation pathways as such, by using an isotope mixing model: In the West and Central Pacific, 52-60% of Hg0 emitted from anthropogenic sources is first circulated to the upper atmosphere for photo-oxidation prior to oxidation and removal to the open ocean. The remainder of Hg comes from riverine Hg export. In the Arctic, >70% of Hg is oxidized near the biosphere, not in the upper atmosphere, thereby conserving the even-MIF of Hg0 even upon oxidation. We speculate that the presence of abundant halogens and sea salt aerosols (SSA) is responsible for rapid Hg0 oxidation and removal to the open ocean. Our study showcases that Hg stable isotopes can be used to differentiate sources, pathways of removal, and fate of Hg across a large spatial scale. After compiling further dataset, we identify that near-surface Hg0 oxidation mediated by halogens and SSA in the Arctic explains elevated Hg levels reported in the Arctic fish, mammals, and polar bears. The pathway of anthropogenic Hg0 emission to bioaccumulation detected in the West and Central Pacific suggests that anthropogenic Hg0 abatement from continental Asia would lower Hg levels in the adjacent marine ecosystems.

How to cite: Kwon, S. Y., Motta, L., and Lim, S. H.: Mercury stable isotopes reveal atmospheric oxidation and removal processes to high and mid-latitude oceans , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2293, https://doi.org/10.5194/egusphere-egu25-2293, 2025.

The presence of approximately 400,000 non-producing oil and gas wells (OGWs) in Canada and millions more globally poses significant environmental and safety issues. These wells leak methane (CH₄) and other pollutants, which exacerbate climate change, pose explosion hazards, contaminate drinking water, and damage plants and animals. Plugging all existing non-producing OGWs would cost several hundred billion dollars1, making this approach virtually impossible. However, since only 10% of these wells are responsible for >90% of the emissions2, a better strategy may be to identify and target high-emitting wells for more effective and economical mitigation efforts. It is therefore important to fully understand the processes governing methane leakage and their subsequent emissions through non-producing OGWs. Another important aspect of these efforts is the identification of well integrity failures, which may not necessarily cause high emissions to the atmosphere but can cause subsurface fluid migration, even for low-emitting wells. A modern OGW typically consists of a system of casings and cement, providing multiple barriers designed to prevent contamination. The surface casing vent (SCV), installed at the wellhead, is designed to vent gas from the annular space between the surface casing and the next casing string. Generally, methane emissions at the SCV are viewed as a sign of well integrity failure but could be unrelated if the casing intersects natural fluid migration pathways.

In this study, we compiled the geochemical data of 365 OGWs from Canada, with measurements made at the component level (wellhead, SCV and surrounding soil) wherever possible. By analyzing δ13C and δ2H isotopic signatures and gas compositions, we identified the origins of our samples as primary microbial, secondary microbial, thermogenic, or abiotic. These origins were only attributed to a third of the studied wells for at least one of the three components (wellhead, SCV and surrounding soil), due to the sensitivity of this approach. We found that the presence of thermogenic methane at the SCV is a good indicator of high-emitting wells, with magnitudes of emissions 100 times higher than microbial emissions. Furthermore, our analysis revealed that a considerable number of emitting wells (~23%) produce methane of microbial origin, which is higher than previously thought (8% in the only existing meta-analysis), and with emission magnitudes that exceed previous estimates by a factor of 1,000. These results suggest that non-producing OGWs could act as bridges facilitating the diffusion of subsurface microbial methane emissions into the atmosphere. Finally, we generally found similar geochemical signatures of methane in corresponding wellhead and SCVs, suggesting that the structural integrity of these wells has been compromised and they can act as one single entity.

  • 1. Raimi, D., Krupnick, A. J., Shah, J.-S. & Thompson, A. Decommissioning Orphaned and Abandoned Oil and Gas Wells: New Estimates and Cost Drivers. Environ. Sci. Technol. 55, 10224–10230 (2021).
  • 2. Williams, J. P., Regehr, A. & Kang, M. Methane Emissions from Abandoned Oil and Gas Wells in Canada and the United States. Environ. Sci. Technol. 55, 563–570 (2021).

How to cite: Micucci, G. and Kang, M.: Investigating the role of Canadian non-producing oil and gas wells in subsurface-atmosphere methane fluxes through geochemical signatures and methane origins, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3259, https://doi.org/10.5194/egusphere-egu25-3259, 2025.

EGU25-3453 | ECS | Posters on site | BG2.2

Long-term high-frequency isotope-specific monitoring of H2O, CO2, CH4 and N2O exchange between atmosphere and ecosystems 

Matthias Claß, Youri Rothfuss, Daniel Schulz, and Nicolas Brüggemann

The central goal of this project is to establish long-term isotope-specific monitoring of H2O, CO2, CH4 and N2O exchange between terrestrial ecosystems and the atmosphere with high temporal resolution at grassland, arable land and forest sites. The exchange of H2O and CO2 between ecosystem and atmosphere will be determined online with rapid (10 Hz) isotope-specific laser analyzers using the eddy covariance (EC) method. The objective of this measurement is to determine the isotopologue fluxes of the respective gases and the source/sink partitioning, i.e., evaporation and transpiration in the case of water vapor or photosynthetic uptake and ecosystem respiration in the case of CO2. Measurements will be conducted using fully automated measurement systems for a minimum of two years. In addition, a mobile automated sampling system will be developed for isotope-specific recording of CH4 and N2O ecosystem exchange using the profile method with off-line isotope analysis by isotope ratio mass spectrometry to ensure the highest possible precision of isotope measurements. The aim of the isotope-specific flux measurements is to partition the CH4 flux into CH4 production (methanogenesis, if relevant) and CH4 uptake (methane oxidation), and the N2O flux into nitrification and denitrification as sources and N2O reduction as an N2O sink. Furthermore, the measurements will permit the determination of the isotopic composition across seasons and during peak emission periods, such as fertilization or freeze-thaw events. All approaches will be evaluated for their relevance in identifying greenhouse gas source/sink processes and their potential for long-term deployment. This presentation will introduce the measurement concepts and present first results.

How to cite: Claß, M., Rothfuss, Y., Schulz, D., and Brüggemann, N.: Long-term high-frequency isotope-specific monitoring of H2O, CO2, CH4 and N2O exchange between atmosphere and ecosystems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3453, https://doi.org/10.5194/egusphere-egu25-3453, 2025.

EGU25-3476 | Orals | BG2.2

Carbonyl sulfide sulfur isotopes fractionation and leaves' internal conductance 

Alon Angert, Felix M. Spielmann, Boris Bazanov, Georg Wohlfahrt, and Alon Amrani

Carbonyl sulfide (OCS) is the major long-lived sulfur-bearing gas in the atmosphere. The main sink for COS occurs when it diffuses through the plant leaves stomata and enters the mesophyll cell, where it reacts with the enzyme carbonic anhydrase. Since CO2 enters the leaves by a similar pathway, COS has been used to estimate the rates of regional and global photosynthesis. For example, recently 1, it was suggested that the global GPP is ~30% higher than estimated so far, based on COS observations and new modeling of COS internal conductance, which relates to the diffusion into the active site in the mesophyll. Sulfur isotope analysis (34S/32S ratio, δ34S) of COS was shown 2 to be useful for improving the determination of atmospheric COS sources and sinks. The sulfur isotopic fractionation during COS uptake in plants is needed for using this tool, but so far, has only been established in the lab. In that study, the fractionation was found to be −1.6 ± 0.1‰ for C3 plants,  −5.4 ± 0.5‰  for C4 plants, and the carbonic anhydrase fractionation was estimated indirectly as −15 ± 2‰. Field studies of leaves' COS uptake enable the study of the effects of varying light conditions in the tree canopy. Here, we measured the COS fractionation during uptake in an Austrian alpine forest, using branch chambers at three height levels in a Pinus sylvestris canopy. In addition, we directly measured the fractionation of carbonic anhydrase in vitro in the lab. The isotopic analysis was conducted by pre-concentrating the air samples and subsequent δ34S analysis by gas chromatography (GC) connected to a multi-collector inductively coupled plasma mass spectrometer (MC-ICPMS). The results of this research are important for improving both leaves scale COS transport models and global budgets of COS and CO2.

 

1. Lai, J., Kooijmans, L. M., Sun, W., Lombardozzi, D., Campbell, J. E., Gu, L., ... & Sun, Y. (2024). Terrestrial photosynthesis is inferred from plant carbonyl sulfide uptake. Nature, 634, 855-861.

2. Davidson, C., Amrani, A., & Angert, A. (2021). Tropospheric carbonyl sulfide mass balance based on direct measurements of sulfur isotopes. Proceedings of the National Academy of Sciences, 118(6), e2020060118.

3. Davidson, C., Amrani, A., & Angert, A. (2022). Carbonyl sulfide sulfur isotope fractionation during uptake by C3 and C4 plants. Journal of Geophysical Research: Biogeosciences, 127(10), e2022JG007035.

How to cite: Angert, A., Spielmann, F. M., Bazanov, B., Wohlfahrt, G., and Amrani, A.: Carbonyl sulfide sulfur isotopes fractionation and leaves' internal conductance, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3476, https://doi.org/10.5194/egusphere-egu25-3476, 2025.

EGU25-3828 | Orals | BG2.2

Measurement and Full Model of Isotope Fractionation During Photodissociation and Applications in Cosmo and Geochemistry 

Mark Thiemens, Ksenia Komorova, Natalia Gelfand, Francoise Remacle, Raphy Levine, Subrata Chakraborty, Teresa Jackson, and Oleg Kostco

The application of isotope effects from photodissociation processes in nature date back to Viking and the observation of a massive 15N in the Martian atmosphere, derived from combined photolysis and gravitational escape. Large observed effects in meteorites, interstellar molecular clouds, and pre solar nebulae utilize photodissociation as a source of the wide range in isotopic composition. CO, which is isoelectronic with nitrogen, has also been widely used, but models do not agree with experiments suggesting models do not include all parameters.

We report precise novel measurements of the isotopic branching ratio in the photodissociation of N2 in the VUV at the advanced light source, Berkeley with quantitative scavenging of the nascent N atoms. We here report an integration of these measurements with state-of-the-art dynamics modeling and light shielding. The measured photodissociation enrichment in 15N with wavelength with a down trend above 90 nm is shown to arise from dynamical effects. There are two effects identified by the computations, the branching between exit channels and the more subtle role of the non-monotonic variation in the individual line widths that in the higher energies begin to significantly overlap. The widths have a significant effect on both the shielding computations at the higher energies and on the cross sections themselves. The modeling requires accurate quantum dynamical simulations using state of the art multireference potential energies and their state-dependent couplings. As the excitation energy increases, competition between different coupled exit channels, some leading to reactive N (2D) and some leading to significantly less reactive N (2P) in an isotope dependent way, modulates the selectivity for the 15N atoms. As a result, the dissociation lifetimes of initial states close in energy vary in a nonmonotonic isotopic dependent manner as a function of energy. Our work shows that modelling can interpret the novel experimental observations and account for the exceptionally high selectivity. Additional progress requires accurate high resolution UV spectra for entire UV bands, both measured and computed to complement fractionation measurements. The complexity of the non-statistical dynamics and the role of the light shielding make such high-resolution work necessary for the detailed understanding of isotope enrichment fractions in the higher energy regime for nitrogen and also for other molecules of interest in cosmochemistry such as CO. Given the massive range in isotopic composition, the interpretation of e.g the Mars atmosphere and photolysis intersection, meteoritic nitrogen may be modeled better. Samples from the earth’s interface with space where N2 photolysis occurs would be an interesting application and testing of the model.

 

How to cite: Thiemens, M., Komorova, K., Gelfand, N., Remacle, F., Levine, R., Chakraborty, S., Jackson, T., and Kostco, O.: Measurement and Full Model of Isotope Fractionation During Photodissociation and Applications in Cosmo and Geochemistry, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-3828, https://doi.org/10.5194/egusphere-egu25-3828, 2025.

EGU25-6805 | Orals | BG2.2

Isotopic fractionation of O2 during photochemical O2 consumption: A relevant process for estimating primary production in sunlit surface waters? 

Sarah G. Pati, Lara M. Brunner, Thomas B. Hofstetter, and Moritz F. Lehmann

Isotopic fractionation of O2 is an important tracer for estimating primary production in aquatic environments because it helps to disentangle the respective contributions from O2 production, consumption, and gas-exchange. Isotope-based methods for estimating primary productivity typically involve measurements of either only 18O/16O ratios or, in the case of triple oxygen isotope approaches, also 17O/16O ratios. Aerobic respiration is generally assumed to be the only process consuming O2, with a constant value for O-isotopic fractionation, expressed as ε or λ values, respectively. However, emerging evidence suggests that in the photic zone of lakes and oceans, photochemical O2 consumption can be of similar magnitude as microbial respiration and photosynthetic O2 production. To determine whether photochemical O2 consumption should be included in isotope-based assessments of primary productivity, we measured the O-isotopic fractionation (as 18O-ε and λ values) of two important photochemical O2 consumption reactions. First, we investigated the energy transfer from photochemically excited dissolved organic matter (DOM) to O2, leading to the reversible formation of singlet oxygen, which can irreversibly react with several functional groups within DOM. Under realistic conditions for sunlit surface waters, this photochemical O2 consumption reaction is associated with 18O-ε values of -25 ‰ to -30 ‰, which are larger than typical values for respiration (approx. -20 ‰). The second photochemical process investigated was the reaction between O2 and photochemically produced organic radicals, which yielded substantially smaller values for 18O-ε (0 ‰ to -15 ‰). 18O-ε values for photochemical O2 consumption may thus be distinguishable from those for respiration. Yet, the overall isotopic fractionation in sunlit surface water will depend on the relative contributions of the different photochemical O2 consumption reactions. Although some studies have measured the isotopic fractionation of photochemical O2 consumption in natural water samples, additional research is needed for properly implementing these processes into isotope-based estimations of primary production. Finally, results from triple oxygen isotopic fractionation measurements suggest an overlap of λ values in the range of 0.51-0.53 for photochemical O2 consumption (as determined in this study) and for respiration experiments from literature.

How to cite: Pati, S. G., Brunner, L. M., Hofstetter, T. B., and Lehmann, M. F.: Isotopic fractionation of O2 during photochemical O2 consumption: A relevant process for estimating primary production in sunlit surface waters?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6805, https://doi.org/10.5194/egusphere-egu25-6805, 2025.

EGU25-8718 | ECS | Posters on site | BG2.2

From Sunshine to Snowfall: Understanding concurrent CO2 and COS exchange in a Coniferous Forest 

Felix M. Spielmann, Albin Hammerle, Anna De-Vries, Alexander Platter, and Georg Wohlfahrt

The net ecosystem exchange (NEE) of CO2 can be measured using the eddy covariance (EC) technique, but separating NEE into ecosystem respiration and gross primary productivity (GPP) relies on models and tracers, making it a persistent challenge. Beyond the established nighttime and daytime flux partitioning algorithms, the trace gas carbonyl sulfide (COS) shows promise as a robust proxy for constraining GPP. Unlike CO2, which is exchanged bidirectionally by leaves and its ecosystem level exchange being influenced by soil respiration, COS generally enters leaves unidirectionally and is fully catalyzed by carbonic anhydrase. Other sources and sinks of COS within ecosystems are typically minor and negligible.

Initial laboratory studies have determined the leaf relative uptake rate (LRU) – the ratio of COS to CO2 deposition velocities (LRU = (FCOS/χCOS)/(GPP/χCO2)) – to be relatively stable around 1.7 under optimal conditions. By knowing the LRU and measuring COS fluxes alongside CO2 and COS ambient mixing ratios, GPP can be calculated. However, most laboratory measurements have been conducted under optimal conditions and further research revealed the influence of environmental factors such as drought, vapor pressure deficit (VPD) and photosynthetically active radiation (PAR) on the LRU.

Due to the high cost and sensitivity of required instruments, few studies have examined COS fluxes at the ecosystem scale, and even fewer have performed long-term monitoring. Seasonal dynamics, particularly during winter, remain largely unexplored.

To address this gap, we conducted EC measurements of COS and CO2 fluxes at a Pinus sylvestris-dominated coniferous forest in Austria to investigate environmental influences on COS fluxes and LRU dynamics. Sampling has been continuous since May 2021, except for a two-month gap during the winter of 2021/22. We present the influence of VPD, PAR, temperature and snowfall on COS fluxes and the LRU at the ecosystem level, based on 3.5 years of measurements.

How to cite: Spielmann, F. M., Hammerle, A., De-Vries, A., Platter, A., and Wohlfahrt, G.: From Sunshine to Snowfall: Understanding concurrent CO2 and COS exchange in a Coniferous Forest, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8718, https://doi.org/10.5194/egusphere-egu25-8718, 2025.

EGU25-10604 | ECS | Orals | BG2.2

Large temperature dependencies for the D, 13C and clumped kinetic isotope effects in methane oxidation by OH and Cl predicted by quantum chemical and transition state theory. 

Marie Kathrine Mikkelsen, Jacob Lynge Elholm, Kurt V. Mikkelsen, and Matthew S. Johnson

Methane emission budgets based on isotopic analysis (e.g. 13C-CH4, D-CH4, 13CH3D CH2D2, CHD3, and/or CD4) correct composition for the isotopic fractionation of atmospheric oxidation reactions. They rely on a handful of laboratory measurements obtained at only a couple of temperatures. The goal of this study is to better characterize KIEs of the reactions and especially the temperature dependence of the KIEs.

As a first step we have calculated the temperature dependent reaction rates using tunneling corrected Transition State Theory. We examine the reaction of methane with Cl and OH including all possible transition states with the isotopologues: CH4,13CH4, 14CH4, 13CDH3, CDH3, CD2H2, CD3H, and CD4. Transition State Theory has been used with M06-2X, ωB97X-D, and CAM-B3LYP level of theory, with the two basis sets 6-31++G(d,p) and 6-311++G(d,p). The KIE is calculated for all reactions and compared with literature. Results for the 13CH4 + Cl reaction show that the KIE changes with -12.0 ‰ per 100 K. Whereas for 13CH4 + OH the KIE changes by -1.14 ‰ from 300 to 200 K. For all isotopologues we predict that the KIE’s change significantly with temperature. Including this correction in isotopic mass balance top down emissions estimates will significantly change the results.

In future work we will examine the reaction path and molecular dynamics in detail. To do these calculations, we will perform ab initio multiple spawning (AIMS) trajectories interfaced with the TeraChem electronic structure program. This study will increase our understanding of the oxidation of methane and compare the quantum chemical understanding of isotope budgeting to observations.

How to cite: Mikkelsen, M. K., Elholm, J. L., Mikkelsen, K. V., and Johnson, M. S.: Large temperature dependencies for the D, 13C and clumped kinetic isotope effects in methane oxidation by OH and Cl predicted by quantum chemical and transition state theory., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10604, https://doi.org/10.5194/egusphere-egu25-10604, 2025.

EGU25-10857 | ECS | Orals | BG2.2

The role of sampling height in interpreting methane isotope ratios for source attribution and inversion modelling 

Emmal Safi, Dafina Kikaj, Thomas Röckmann, Edward Chung, Jacoline van Es, Chris Rennick, Carina van der Veen, Tim Arnold, and Bibhasvata Dasgupta

Methane (CH4) has a global warming potential 28-36 times that of carbon dioxide over a 100-year period [1]. Different sources of CH4 have distinct isotopic signatures, with CH4 from biological sources having a lighter signature than those from fossil sources [2]. Greenhouse gas (GHG) emissions are typically reported using bottom-up methods (based on data such as emission factors) that are verified using top-down methods (based on atmospheric transport models (ATMs) and observations) which infer fluxes, often through Bayesian methods [3]. Isotope ratio data are generally used in atmospheric models to understand individual contributions of various CH­4 sources, globally and regionally. However, there is uncertainty regarding isotopic signatures due to large temporal variabilities and regional specificities [4].

Methane isotope ratio source signature information is typically gained through discrete mobile measurement campaigns, with the aim of capturing the emissions directly from the sources, through downwind transection of plumes as closely as possible to the source [5]. These measurements fill databases that are used for atmospheric modelling [2,6,7].

Continuous measurements of CH4 isotope ratios are also carried out at from varying sampling heights [7,8,9] (ranging from tens to hundreds of meters) with the lower heights, closer to emissions sources, capturing more local influences and higher heights capturing more regional emissions. While they offer the advantage of being continuous, they are further away from the emission sources, therefore have larger uncertainties.

Understanding the information that can be gained from continuous CH4 isotope ratio measurements at different sampling heights and locations will be an important factor to consider when using observational data in inversion frameworks, in terms of accurately quantifying source signatures. We present results of mean isotopic signatures from continuous measurements, resolved using the Keeling approach and compare to modelled data to understand the inferred source contributions.

Continuous measurements of CH4 isotope ratios have been carried out at 10 European atmospheric GHG monitoring stations. This study focuses on two sites: Heathfield (an inland, 100 m a.g.l tall tower) and Krakow (an urban, 35 m a.g.l site). We present CH4 isotope ratio datasets from these sites and aim to use them to interpret isotopic signatures in the surrounding areas.

[1] IPCC 2021. Cambridge University Press.

[2] Sherwood et al. 2017. Earth Syst. Sci. Data. 9, 639-656.

[3] Manning et al. 2021. Atmos. Chem. Phys. 21, 12739-12755.

[4] Ramsden et al. 2022. Atmos. Chem. Phys. 22, 3911-3929.

[5] Bakkaloglu et al. 2022. Atmos. Environ. 276, 119021.

[6] Menoud et al. 2020. Tellus B. 72, 1823733.

[7] Menoud et al. 2022. Earth Syst. Sci. Data. 14, 4365-4386.

[8] Röckmann et al. 2016, Atmos. Chem. Phys. 16, 10469-10487.

[9] Rennick et al. 2021. Anal. Chem. 93, 10141-10141.

How to cite: Safi, E., Kikaj, D., Röckmann, T., Chung, E., van Es, J., Rennick, C., van der Veen, C., Arnold, T., and Dasgupta, B.: The role of sampling height in interpreting methane isotope ratios for source attribution and inversion modelling, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10857, https://doi.org/10.5194/egusphere-egu25-10857, 2025.

EGU25-11143 | Orals | BG2.2

Towards a calibration-free analysis of 15N site preference in N2O reference materials using matrix-isolation infrared spectroscopy 

Jonas Schlagin, Dennis Dinu, Klaus R. Liedl, Dominik Stolzenburg, Hinrich Grothe, and Joachim Mohn

In the global nitrous oxide (N2O) budget, various processes can influence the natural isotope abundances, often enriched with 15N with a site-specific preference δ15NSP that serves as a unique natural isotope tracer. Unlike δ18O and δ15Nbulk, δ15NSP is independent of the substrate’s isotopic signature and remains unchanged during N2O diffusion. However, while δ 15NSP can reveal mechanisms of N2O formation and reduction [1], distinguishing between production and consumption processes remains challenging due to overlapping isotopic signatures and variable fractionation factors. Current approaches, such as dual isotope plots (e.g., δ15NSP15Nbulk), help constrain dominant pathways but rely on experimental fractionation data. Which can be difficult considering that for the determination of 15NSP values with isotope ratio mass spectrometry (IRMS) methods it was shown that they are highly reliant on the choice of calibration with differences of up to 30 ‰ [2]. At the same time, laser absorption spectroscopy (LAS) of rotational-vibrational transition is prone to interferences by other trace gases, requires rigorous calibration and needs preconcentration units [3-4]. We propose using matrix-isolation Fourier-transform infrared (MI-FTIR) spectroscopy, which provides a calibration-free measurement of site-specific N2O isotopic composition by determining the absorption cross-section of the pure vibrational features of the respective isotopocules

 

[1] Toyoda, S., Yoshida, N. and Koba, K. (2017), Isotopocule analysis of biologically produced nitrous oxide in various environments. Mass. Spec. Rev., 36: 135-160

[2] Westley, M.B., Popp, B.N. and Rust, T.M. (2007), The calibration of the intramolecular nitrogen isotope distribution in nitrous oxide measured by isotope ratio mass spectrometry†. Rapid Commun. Mass Spectrom., 21: 391-405.

[3] Harris, E., Zeyer K., Kegel R., et al. (2015), Nitrous oxide and methane emissions and nitrous oxide isotopic composition from waste incineration in Switzerland. Waste Management, 35: 135-140

 

[4] Ostrom, N.E., Ostrom, P.H. (2017), Mining the isotopic complexity of nitrous oxide: a review of challenges and opportunities. Biogeochemistry, 132: 359–372.

How to cite: Schlagin, J., Dinu, D., Liedl, K. R., Stolzenburg, D., Grothe, H., and Mohn, J.: Towards a calibration-free analysis of 15N site preference in N2O reference materials using matrix-isolation infrared spectroscopy, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11143, https://doi.org/10.5194/egusphere-egu25-11143, 2025.

EGU25-11217 | ECS | Posters on site | BG2.2

Addressing discrepancies in 13CKIE and DKIE values for the CH₄-OH oxidation 

ChihChang Chen, Getachew Adnew, Carina van der Veen, and Thomas Röckmann

Methane (CH₄) plays a critical role in the global carbon cycle, with its mole fraction currently 2.5 times higher than preindustrial levels. The increasing growth rate observed globally highlights the importance of accurate partitioning the atmospheric CH4. Oxidation of CH₄ by hydroxyl radicals (OH) in the troposphere accounts for approximately 85% of the global CH₄ sink. The resulting isotopic fractionation of δ13C-CH₄ and δD-CH₄ provides a valuable tool for understanding the global CH₄ budget. However, discrepancies exist in the reported kinetic isotope effect (KIE) values for CH₄ destruction by OH with 13CKIE ranging from 1.0036 to 1.010 and DKIE ranging from 1.25 to 1.31. These uncertainties significantly limit the precision of global CH₄ budget estimation.

 

This study aims to address these discrepancies by accurately characterizing the KIE values under varying temperature and pressure conditions. During the laboratory experiments, CH₄ is subjected to chemical reactions with OH, which is generated through the photolysis of vapor-phase hydrogen peroxide using a deep-UV light source (200-380 nm). To minimize interference from O(1D) reactions, a coated glass filter is employed. The photochemical reactions take place in a 5-liter, triple-quartz-layered reactor, maintained at stable pressure and temperature, with by-products removed using a low-temperature trap. The reactor is coupled to two Isotope Ratio Mass Spectrometers (IRMS), enabling continuous measurements of δ13C, δD, and δ18O in remaining CH₄ and CO throughout the experiment. By enhancing our understanding of CH₄-OH reaction kinetics under controlled conditions, this study can improve the accuracy of global CH₄ budget assessments and refine the distribution between fossil and biogenic CH4 sources.

How to cite: Chen, C., Adnew, G., van der Veen, C., and Röckmann, T.: Addressing discrepancies in 13CKIE and DKIE values for the CH₄-OH oxidation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11217, https://doi.org/10.5194/egusphere-egu25-11217, 2025.

EGU25-11425 | Posters on site | BG2.2

Expanding Isotope Ratio Analysis of Intact Molecules to Gas Phase Using a MION-Orbitrap System 

Hans-Jürg Jost, Henning Finkenzeller, Aleksei Shcherbinin, Fariba Partovi, and Joona Mikkilä

Orbitrap mass spectrometers have proven highly effective for isotope ratio analysis in liquid chromatography (LC)-coupled workflows, offering high precision and resolution. We introduce an innovative expansion of this capability to gas-phase isotope ratio analysis of intact molecules, eliminating the need for complex sample preparation and molecular conversion required in traditional isotope ratio mass spectrometry (IRMS).

The MION-Orbitrap system is optimized for direct gas-phase sample introduction, enabling precise and accurate isotope ratio measurements for carbon (13C/12C), hydrogen (2H/1H), nitrogen (15N/14N), and sulfur (34S/32S) on intact molecular species. Its capability for online analysis of ambient air further enhances its applicability. By bypassing conventional combustion or molecular conversion steps, this approach simplifies workflows, reduces handling time, and minimizes potential isotopic fractionation.

Preliminary experiments demonstrate the feasibility of this method and first results will be presented. By preserving molecular integrity during analysis, the system opens new avenues for investigating complex organic compounds in environmental chemistry, atmospheric processes, biogeochemical cycles, and plant metabolism.

We also address some of the remaining challenges in advancing this methodology, including the need for standardized reference materials for intact molecular isotope ratio measurements and the mitigation of potential matrix effects. These efforts are critical for ensuring accuracy, reproducibility, and broader adoption of gas-phase isotope ratio analysis.

How to cite: Jost, H.-J., Finkenzeller, H., Shcherbinin, A., Partovi, F., and Mikkilä, J.: Expanding Isotope Ratio Analysis of Intact Molecules to Gas Phase Using a MION-Orbitrap System, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11425, https://doi.org/10.5194/egusphere-egu25-11425, 2025.

EGU25-12043 | ECS | Orals | BG2.2

Assessing drivers of uncertainty in simulating δ¹³C-CH4 at global scale 

Emeline Tapin, Antoine Berchet, Adrien Martinez, Malika Menoud, Xin Lan, Sylvia Michel, and Marielle Saunois

Methane (CH4), the second-largest contributor to global warming, necessitates a detailed examination of its sources and sinks to understand the recent rise in atmospheric CH4 mole fractions. Atmospheric isotopic signals, especially δ¹³C-CH4, offer critical insights for disentangling sectoral contributions and addressing these uncertainties.

This study focuses on enhancing our understanding of CH4 sources and sinks by incorporating updated δ¹³C-CH4 source signature datasets into atmospheric modeling. First, we updated these datasets to reflect the latest knowledge of methane emission processes. Next, we assessed the sensitivity of key modeling parameters such as atmospheric chemistry, the aggregation of δ¹³C-CH4 source signatures, and prior flux estimates on simulated CH4 signals and mole fractions. This analysis aims to validate the updated datasets and identify primary drivers of uncertainty in the simulations. We conducted forward modeling using the Global Circulation Model LMDZ coupled with the Community Inversion Framework (CIF), based on surface observations of methane and its isotopic signal from 1998 to 2022. These efforts lay the groundwork for improving the robustness of future isotopic inversions.

Building on these findings, our future work will focus on transitioning from forward simulations to atmospheric inversions to analyze global methane concentration trends. Initially, we will perform inversions using in-situ data from 1998 to 2022, leveraging the updated δ¹³C-CH4 source signature datasets and setups. Subsequently, we will analyze trends from 2018 to 2022 by integrating satellite observations of total methane columns with surface isotopic measurements. This approach utilizes the high-resolution, global coverage of TROPOMI (TROPOspheric Monitoring Instrument) onboard the Sentinel-5P platform, which measures column-averaged methane dry-air mole fractions X(CH4). By combining satellite and surface observations, we aim to enhance our ability to monitor methane dynamics and deepen our understanding of CH4 source and sink interactions. These advancements will provide critical insights for designing more effective climate mitigation strategies.

How to cite: Tapin, E., Berchet, A., Martinez, A., Menoud, M., Lan, X., Michel, S., and Saunois, M.: Assessing drivers of uncertainty in simulating δ¹³C-CH4 at global scale, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12043, https://doi.org/10.5194/egusphere-egu25-12043, 2025.

EGU25-12431 | ECS | Orals | BG2.2

A multiplexing set-up of aquatic biological chambers to study the isotopic fractionation of oxygen: application to the interpretation of the δ18O of O2 records found in deep ice cores. 

Nicolas Bienville, Amaelle Landais, Sarah Fiorini, Clément Piel, Joana Sauze, Frédéric Prie, Olivier Joussoud, Simon Chollet, and Samuel Abiven

Earth atmospheric dioxygen is mainly produced by biosphere photosynthesis, and biosphere respiration is also one of the main consumers of this gas. The evolution of atmospheric O2 is thus linked to global biosphere productivity.

 

In ice cores we extract air from bubbles to study the composition of the past atmosphere. However, as O2 concentration in air bubbles is affected by close off processes, it is difficult to reconstruct its variations in the past atmosphere from ice core analyses. In turn, the isotopic composition of O218O and δ 17O), is also influenced by biological processes and is less influenced by close-off processes so that this tracer should provide useful information on the past biosphere activity.

 

Quantitative interpretation of the isotopic composition of O2 in the past relies on robust estimate of oxygen fractionation coefficients associated with the relevant biological processes: photosynthesis and respiration. In the past decades, some determinations of these biological fractionation coefficients were performed in uncontrolled large-scale environments or at the scale of the micro-organisms in conditions very different from the natural environment. There are thus inconsistencies in previous determinations of the O2 fractionation coefficients limiting the interpretation of δ18O and δ 17O of O2.

 

In order to come up with coherent estimates of oxygen fractionation coefficients during biological processes, we developed closed biological chambers as a biosphere replica, with controlled environment parameters (light, temperature, CO2 concentration), which were used in combination with a newly designed optical spectrometer for continuous measurements of O2 concentration and of its isotopic composition.

 

In this presentation, we show the design and realisation of our aquatic biological chambers as well as the associated development of the multiplexing system to be able to run parallel experiments with the same environmental conditions. Then, we show the results obtained for light and dark periods, and the corresponding fractionation coefficients calculated for photosynthesis and respiration. Finally, we use the newly determined fractionation coefficients to improve interpretation of the δ18O of O2 record in air bubbles from ice cores.

How to cite: Bienville, N., Landais, A., Fiorini, S., Piel, C., Sauze, J., Prie, F., Joussoud, O., Chollet, S., and Abiven, S.: A multiplexing set-up of aquatic biological chambers to study the isotopic fractionation of oxygen: application to the interpretation of the δ18O of O2 records found in deep ice cores., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12431, https://doi.org/10.5194/egusphere-egu25-12431, 2025.

EGU25-13223 | Orals | BG2.2

Modeling the sulfur isotopic signature of marine carbonyl sulfide emissions 

Sinikka Lennartz, Alon Amrani, Yasmin Avidani, Chen Davidson, Heike Simon, and Alon Angert

Carbonyl sulfide (OCS), the most abundant sulfur-containing trace gas in Earth's atmosphere, plays a central role in stratospheric aerosol formation and can serve as a proxy for terrestrial carbon dioxide uptake. In this context, quantifying its atmospheric sources and sinks is of great interest, but especially the role of marine emissions is poorly constrained. Analysis of sulfur isotopic ratios (34S/32S; d34S) is a valuable tool to quantify the relative contributions of different sources to the atmospheric budget of OCS. However, the d34S values for marine OCS emissions are based on a data set that has so far been limited to a few measurements in coastal and shelf areas. Here, we present a first global ocean mixed-layer model of OCS sulfur isotopes, building on experimentally derived fractionation factors for the most important biogeochemical processes of marine OCS cycling, i.e. photochemical production, dark production and degradation by hydrolysis. The model is tested against incubation experiments and novel measurements along an Atlantic transect. We calculate the d34S values of marine OCS emissions, with the ultimate aim to decipher their relative contributions to the atmospheric budget. Our simulations show regional and temporal variations in the d34S values of OCS, suggesting a distinct latitudinal gradient with lower d34S in the tropics and higher d34S in high latitudes. The spatially weighted average of d34S values of OCS is used to update a global mass balance approach to infer the role of direct marine emissions of OCS in the atmospheric budget.

How to cite: Lennartz, S., Amrani, A., Avidani, Y., Davidson, C., Simon, H., and Angert, A.: Modeling the sulfur isotopic signature of marine carbonyl sulfide emissions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13223, https://doi.org/10.5194/egusphere-egu25-13223, 2025.

EGU25-13314 | Orals | BG2.2

Atlantic Meridional Transect of polyisotopic carbon dioxide: Challenges of ship-based laser spectroscopy and implications for atmosphere-biosphere exchange 

Jan Kaiser, Penelope A. Pickers, Grant L. Forster, Alina Marca, Richmal B. Paxton, and Barry McManus

During the AMT31 research cruise (Southampton–Montevideo, December 2024), we measured CO2 polyisotopologues using a tuneable infrared laser direct absorption spectrometer (Aerodyne TILDAS-FD-L2). Dried marine air from an inlet at the bow of the ship was alternated with a working reference every 2 min to correct for instrument drift.

Compared with land-based measurements, ship motion (roll, pitch, heave) was found to deteriorate isotope ratio precision by a factor of 3 to 10 (depending on the sea state). However, after averaging over hourly intervals, precisions better than 0.05 µmol mol–1 for y(CO2) and better than 0.03 ‰ for δ(13C), δ(18O) and δ(17O) were achieved. For the 17O isotope excess, Δ(17O), hourly precision was often better than 10 ppm (0.01 ‰), but unfortunately, target tank results showed unexplained day-to-day variability of the order of ±35 ppm.

Preliminary corrections for this day-to-day variability indicate that southern hemisphere δ(18O) is 1.2–1.8 ‰ higher and Δ(17O) is about 60 ppm higher than northern hemisphere marine background air. This interhemispheric Δ(17O) gradient is twice as high as predicted by atmosphere-biosphere exchange models (Koren et al., 2019) and could indicate a stronger than expected influence of the 17O-enriched stratospheric return flux in austral spring or a stronger biospheric exchange signal in boreal autumn.

How to cite: Kaiser, J., Pickers, P. A., Forster, G. L., Marca, A., Paxton, R. B., and McManus, B.: Atlantic Meridional Transect of polyisotopic carbon dioxide: Challenges of ship-based laser spectroscopy and implications for atmosphere-biosphere exchange, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13314, https://doi.org/10.5194/egusphere-egu25-13314, 2025.

EGU25-13624 | Posters on site | BG2.2

Advancing Greenhouse Gas Isotopic Measurements: Evaluating the Compatibility and Efficiency of Picarro Gas Autosampler with Picarro Isotopic Analyzers 

Keren Drori, Joyeeta Bhattacharya, Magdalena Hofmann, Jan Woźniak, and Tina Hemenway

The greenhouse gas research community faces a growing demand for automated solutions tailored to isotopic measurements of greenhouse gases (e.g., isotopic CO2/CH4). Traditional solutions often entail significant initial and maintenance costs, intricate deployment and maintenance processes, and limited fieldwork adaptability. Anticipating this challenge, the Picarro Gas Autosampler is poised to attract growing interest for its anticipated compatibility with Picarro isotopic Carbon analyzers featuring low flow rates (<50 scc/m), promising efficient isotopic measurements. This report delves into the compatibility, efficiency, and advantages of the Picarro Gas Autosampler when paired with the Picarro G2201-i analyzer. Our experiments showcase remarkable precision and accuracy in isotopic measurements of greenhouse gases. Additionally, we explore factors such as linearity in dilution factors and characterize memory effects and variability across different gas species (e.g., comparing CO2 vs CH4). Moreover, the report offers practical recommendations on methods and best practices for conducting isotopic measurements of greenhouse gases. In summary, the Picarro Gas Autosampler, when combined with the Picarro G2201-i analyzer, emerges as a compelling, cost-effective, and user-friendly solution for isotopic measurements of greenhouse gases, offering a distinct advantage over traditional alternatives.

How to cite: Drori, K., Bhattacharya, J., Hofmann, M., Woźniak, J., and Hemenway, T.: Advancing Greenhouse Gas Isotopic Measurements: Evaluating the Compatibility and Efficiency of Picarro Gas Autosampler with Picarro Isotopic Analyzers, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13624, https://doi.org/10.5194/egusphere-egu25-13624, 2025.

EGU25-13790 | ECS | Orals | BG2.2

Compositional analysis and isotope sourcing of gases generated from self-heating coal waste dump: the case study from France 

Yaroslav Bezyk, Dariusz Strąpoć, Maciej Górka, Łukasz Kruszewski, Jarosław Nęcki, Dariusz Więcław, Carina van der Veen, and Thomas Röckmann

The accumulation of organic matter in coal waste dumps can result in self-heating or spontaneous ignition, which lead to the release of various gaseous products into the atmosphere. GHGs and trace compounds emitted from self-heating coal waste dump located in the Nord-Pas-de-Calais region of Northern France were investigated under this study in September 2024. Tracking hotspot locations across coal waste dump confirmed various patterns of temperature and gaseous emissions from the investigated area. The temperature measured in boreholes drilled to the depth up to 0.6 meters on the top and slopes of the dump ranged between +51.0 and +83.1 °C. The non-uniform subsurface temperatures can be explained by the varied content of coal and carbon-containing rocks deposited at the dump, along with the diverse air inflow to the thermally active sites. The composition and source of the gaseous compounds emitted during self-heating were directly influenced by the various thermal activity stages and properties of the organic matter present in the dump.

Different generation patterns of released gases are related to the self-heating stage, including exothermic oxidation and pyrolysis. At thermally active sites (but below +68 °C) on the top of the dump (well-ventilated with free access of oxygen) the emission included CO2 12.8 vol%. Otherwise, at the sites on the wet dump slope (preventing oxygen entering), where prominent thermal activity was noted (temperature rise of about 80 ºC), the switch to pyrolysis was confirmed by showing a peak of CO2 (18.3 vol%), with a significant drop in O2 content (1.48 vol%). Apart from CO2, much higher was the concentration of CH4 reaching 4260 ppmv, and CO averaging 54 ppmv, above background H2, high levels of pyrolytic ethane 327 ppmv and propane 69 ppmv as well as C4 – C6 hydrocarbons.

The generation processes of the gases on both types of sites were confirmed by C and H isotopic analyses (CO2, CH4, C2H6, H2) and will be discussed in detail during the presentation of the paper. Recapitulating, the stable isotope tracing of the emitted gases was useful and can also be indicative for future monitoring of the thermal stage of self-heating coal waste dumps. Additionally, sulfur and nitrogen heterocyclic compounds such as furane, thiophene, and pyridine were detected in trace quantities. Although substantial amounts of gasses (mainly CO2 and CH4) escaped from the emission hotspot on the dump, their concentrations measured above the surface at sites without thermal activity were not significantly higher than local background levels. The surface flux mapping of entire dump, depth profiling of temperature and gas concentrations, their generative and degradation processes will be the main areas of future investigations.

 

This work was funded by the Polish Ministry of Science and Higher Education under Grant No. 2022/44/C/ST10/00112. The isotopic analysis has been supported by the ATMO-ACCESS (grant agreement No. ATMO-TNA-4—0000000041 and No. C1-ISOLAB/CESAR-9).

Acknowledgment for organization of and assistance during the onsite measurements and samples acquisition on the dump to Fabrice Quirin, Vincent Adam, Gaetan Bentivegna from Bureau de Recherches Géologiques et Minières, Unité Territoriale Après-Mine Nord, Billy-Montigny, France.

How to cite: Bezyk, Y., Strąpoć, D., Górka, M., Kruszewski, Ł., Nęcki, J., Więcław, D., van der Veen, C., and Röckmann, T.: Compositional analysis and isotope sourcing of gases generated from self-heating coal waste dump: the case study from France, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13790, https://doi.org/10.5194/egusphere-egu25-13790, 2025.

EGU25-14132 | ECS | Posters on site | BG2.2

Simulating Long-Term Trends and Seasonal Dynamics of Carbon Isotopes in Atmospheric CO2 Using a 3D Transport Model 

Uddalak Chakraborty, Naoko Saitoh, Prabir Patra, Naveen Chandra, Dmitry Belikov, and Marko Scholze

Carbon Dioxide (CO2), the primary anthropogenic greenhouse gas (GHG), plays a significant role in global warming. Earth’s global surface air temperate was higher by 1.09 °C in 2011–2020 than in 1850–1900. This rise is overwhelmed by 47% in atmospheric CO2 during the period (IPCC AR6, 2021). Analysis of carbon isotopes (13C and 14C) of CO2 plays a pivotal role in separating the anthropogenic and natural carbon release and uptake across land, ocean and atmosphere carbon pools. Despite their utility to understand carbon cycle dynamics, simulating the seasonal variations and long-term trends of 13C and 14C remains challenging. Bridging of the budget gaps requires robust modeling approaches to simulate the isotopic exchange fluxes since the rapid increase in fossil fuel emissions began in the 1950s.

This study has quantified the monthly exchange fluxes of 13C and 14C between the atmosphere and terrestrial biosphere, and between the atmosphere and ocean, as well as 13C and 14C emissions from fossil fuel, nuclear bomb tests, and nuclear power plants, for the period from 1940 to 2020. We have used fossil fuel emissions from GridFED (Jones et al., 2023), land biosphere fluxes are taken from LENS, LPJ and VISIT (NCAR ref., Scholze et al., 2008, Ito et al., 2007), and ocean exchange fluxes are taken from CESM2, LENS (NCAR ref., Danabasoglu et al., 2020). The Model for Interdisciplinary Research on Climate version 4 (MIROC4) atmospheric general circulation model (AGCM)-based chemistry-transport model (referred to as MIROC4-ACTM) has been used for the simulation of the prepared fluxes of 13C and 14C.

Our model simulated the observed concentrations of Δ14C at Jungfraujoch (JFJ; ICOS ref., Levin et al., 2021) and Baring Head (BHD; NIWA ref., Turnbull et al., 2007); e.g., the rise from -24.3 ‰ to 272.4 ‰ during 1950−1960, followed by a slow (near exponential) decay during 1965 to 2020. The two model cases using LENS and LPJ land model fluxes showed noticeable differences during 1970s. The model simulations of δ13C were compared with nine sites of SIO (Keeling et al., 2001); they successfully reproduced the long-term declining trend driven by the Suess Effect, which is the isotopic depletion of atmospheric CO2 caused by the combustion of δ¹³C-depleted fossil fuels. Seasonal variations were well captured, with enriched δ¹³C during photosynthetic periods (summer) and depleted δ¹³C during respiration periods (winter). In our simulations, the interhemispheric gradient in δ¹³C was evident, with stronger seasonal cycles and steeper declines in the Northern Hemisphere (e.g., Barrow, Mauna Loa) due to proximity to major anthropogenic CO2 sources, while Southern Hemisphere sites (e.g., Baring Head, South Pole) showed weaker seasonal variations, reflecting the dominance of ocean uptake and isotopic mixing. Discrepancies in Δ¹⁴C during 1955–1965 and 1980–2000 due to uncertainties in bomb-test emissions and biospheric uptake fluxes remain a challenge in accurately reproducing the observations.

How to cite: Chakraborty, U., Saitoh, N., Patra, P., Chandra, N., Belikov, D., and Scholze, M.: Simulating Long-Term Trends and Seasonal Dynamics of Carbon Isotopes in Atmospheric CO2 Using a 3D Transport Model, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14132, https://doi.org/10.5194/egusphere-egu25-14132, 2025.

EGU25-14144 | ECS | Orals | BG2.2

Source apportionment and evolution of reactive nitrogen in an East Asian mountain forest: A dual-isotope and modeling approach 

Wen-Chien Lee, Ming-Hao Huang, Wei-Chieh Huang, Jen-Ping Chen, Haojia Ren, and Hui-Ming Hung

Anthropogenic activities have led to a rapid increase of reactive nitrogen (Nr) in the Earth system, contributing to climate change, biodiversity loss, acid deposition, and air pollution. Among Nr species, particulate ammonium (pNH4+) and nitrate (pNO3) derived from ammonia (NH3) and nitrogen oxides (NOx) are key pollutants affecting air quality. However, their sources and formation pathways vary by location and remain poorly understood. This study investigates the sources and atmospheric processing of Nr in an East Asian mountain forest, using nitrogen (δ15N) and oxygen (δ18O) isotope compositions of pNH4+ and pNO3. A field campaign was conducted in Xitou, Taiwan (23.40°N, 120.47°E, 1179 m above sea level) from April 17 to 24, 2021. Size-segregated aerosol particles ranging from 0.056 to 18 µm were collected using a micro-orifice uniform deposit impactor (MOUDI) and analyzed for mass concentrations and isotopic compositions using Fourier-transform infrared spectroscopy with attenuated total reflection (FTIR-ATR) and gas chromatography-isotope ratio mass spectrometer (GC-IRMS), respectively. Additionally, a stable isotope mixing model (MixSIAR) was applied to quantify source contributions of Nr based on δ15N signatures. Xitou, located downstream of metropolitan coastal areas during the daytime, receives air pollutants transported inland by sea breezes and valley winds, combined with local emissions. During the campaign, the average mass concentrations of pNH4+ and pNO3 were 3.7 and 2.4 µg m−3, respectively. The mean δ15N values of pNH4+ (10.8 ± 2.7‰) and pNO3 (−3.0 ± 2.0‰) reflect their emission sources and isotopic fractionation during gas-particle partitioning. δ18O values of pNO3 ranged from 32.0‰ to 73.3‰, indicating distinct chemical formation pathways: pNO3 formed via O3 reactions exhibited higher δ18O values, while those formed via peroxy radicals (RO2) had lower values. Two distinct groups of pNO3 were identified based on δ15N-pNO3and δ18O-pNO3 signatures. The first group, characterized by higher δ15N (−5.6 to 0.8‰) and δ18O (55 to 83‰), likely formed in metropolitan areas via O3 oxidation before being transported to the mountain observation site. The second group, consisting of smaller particles with lower δ15N (−10.1 to −2.1‰) and δ18O (8.6 to 38‰), was likely produced locally with RO2 as the dominant oxidant. Source apportionment analysis of δ15N revealed that combustion-related sources, including fossil fuel combustion and NH3 slip, accounted for 63% of NH3 emissions, while anthropogenic NOx sources such as biomass burning, coal combustion, and mobile sources contributed approximately 68% of total NOx emissions. These findings highlight the importance of targeted emission control policies to reduce Nr pollution and mitigate its adverse environmental impacts, including air quality degradation and ecosystem harm.

How to cite: Lee, W.-C., Huang, M.-H., Huang, W.-C., Chen, J.-P., Ren, H., and Hung, H.-M.: Source apportionment and evolution of reactive nitrogen in an East Asian mountain forest: A dual-isotope and modeling approach, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14144, https://doi.org/10.5194/egusphere-egu25-14144, 2025.

EGU25-14260 | ECS | Posters on site | BG2.2

Multi-model Insights into δ13C-CH4 from Arctic Permafrost Thermokarsts 

Kevin Rozmiarek, Youmi Oh, Xiangyu Liu, Irina Overeem, Elijah Miller, Valerie Morris, Bruce Vaughn, Nicholas Hasson, Brooke Chase, Katey Walter Anthony, Qianlai Zhuang, Gregory Rieker, and Tyler Jones

Methane is experiencing an accelerating increase in the atmosphere globally. Of the tools researchers have to diagnosis and determine the cause of rapidly changing sources and sinks of methane, its carbon isotope composition, δ13C-CH4, is a promising option to reduce uncertainty and provide constraints on methane atmospheric inversions. A building consensus in literature points towards wetland emissions as the driving force behind increase emissions, yet our ability to be prescriptive of the wetland δ13C-CH4 flux remains uncertain. Of wetlands, northern permafrost and its thaw features add additional complexities just as they add a large potential carbon stock for future methane release. Early models attempting to determine the δ13C-CH4 of permafrost thaw predict that these landscapes will be isotopic endmembers, more depleted than any source on the planet. How does this prediction hold up against observations when downscaled to the site level?

We present an intercomparison between observations and two isotope-enabled methane production models targeting the thaw feature Big Trail Lake outside Fairbanks, Alaska. We compare the isotope-enabled version of the terrestrial ecosystem model–methane dynamics module (isoTEM) to the Arctic Lake Biogeochemistry Model (ALBM) with an added isotope mass balance. We benchmark both model runs against methane eddy-flux data and flask-collected methane isotope measurements onsite. Through this multi-model-observation intercomparison, we evaluate model mismatch of δ13C-CH4 flux at Big Trail Lake and evaluate how model physics can be improved to better capture permafrost thaw δ13C-CH4 flux for use in constraining atmospheric inversions.

How to cite: Rozmiarek, K., Oh, Y., Liu, X., Overeem, I., Miller, E., Morris, V., Vaughn, B., Hasson, N., Chase, B., Walter Anthony, K., Zhuang, Q., Rieker, G., and Jones, T.: Multi-model Insights into δ13C-CH4 from Arctic Permafrost Thermokarsts, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14260, https://doi.org/10.5194/egusphere-egu25-14260, 2025.

EGU25-15335 | Orals | BG2.2

New experiments and quantum-molecular mechanics model of isotopic fractionation in formaldehyde photolysis explains atmospheric dD-H2 anomaly  and shows extreme isotopic fractionation in CO 

Matthew Johnson, Luisa Pennacchio, Zacharias Liasi, Andreas Erbs Hillers-Bendtsen, Thomas Röckmann, and Kurt Valentin Mikkelsen

Formaldehyde is a short-lived intermediate formed by the oxidation of virtually every VOC in the atmosphere. It is the source of half of atmospheric hydrogen, and a large source of CO and CO2, and plays a role in particle growth. Efforts to better understand the remarkable transformations of formaldehyde are hindered due to lack of knowledge of some of the basic processes in formaldehyde photolysis. Here, we present a combined quantum and molecular mechanics, Rice–Ramsperger–Kassel–Marcus (RRKM) and experiment-based model that significantly advances our ability to describe photolytic kinetic isotope effects and their pressure dependencies. RRKM theory was used to calculate the decomposition rates of the S0, S1 and T1 states using CCSD(T)/aug-cc-pVTZ, ωB97X-D/aug-cc-pVTZ and CASPT2/aug-cc-pVTZ levels of theory. Experimental internal conversion and intersystem crossing rates were used and modified with the density of states of the isotopologues based on Fermi’s ‘Golden Rule’. The following isotopologues of formaldehyde were investigated: HCHO, DCHO, DCDO, D13CHO, H13CHO, HCH17O, HCH18O, HC13H17O and HC13H18O. The method and mechanism were validated by comparison to all existing and newly obtained experimental data. The model was able to accurately replicate the experimental pressure trends of the kinetic isotope effects (KIEs) and was in excellent agreement. The model was used to predict the KIEs and the molecular hydrogen yields of the deuterated species at varying altitudes.

How to cite: Johnson, M., Pennacchio, L., Liasi, Z., Erbs Hillers-Bendtsen, A., Röckmann, T., and Mikkelsen, K. V.: New experiments and quantum-molecular mechanics model of isotopic fractionation in formaldehyde photolysis explains atmospheric dD-H2 anomaly  and shows extreme isotopic fractionation in CO, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15335, https://doi.org/10.5194/egusphere-egu25-15335, 2025.

EGU25-15597 | Posters on site | BG2.2

Temporal Variations and Influencing Factors on Atmospheric CO2 in Urban Environments: A Stable Isotope Perspective 

Sergio Gurrieri and Roberto M.R. Di Martino

Volcanoes are primary geological sources of carbon dioxide (CO2), while the combustion of fossil fuels significantly contributes to raise the CO2 concentration in the atmosphere, particularly within densely populated urban areas. Previous investigations have identified distinct sources of CO2 at the district scale in urban environments and that the short term evolutions in atmospheric CO2 concentration are influenced by meteorological parameters.

This study presents continuous monitoring of stable isotope compositions and CO2 concentrations in the urban environment of Palermo over a yearly period from 2023 to 2024. A laser-based isotope mass spectrophotometer was employed for measurements, detecting various isotopologues of CO2 (e.g., COO, 13COO, and C18OO isotopologues) through mid-infrared range laser absorption. The instrument calculated the 13C/12C ratio, 18O/16O ratio, and overall CO2 concentration. Measurements were conducted outside the Istituto Nazionale di Geofisica e Vulcanologia (INGV) laboratory at an elevation of 16.30 meters above the ground floor, referenced hourly, and calibrated daily using a known stable isotope composition standard of pure CO2.

Environmental parameters, including air temperature, atmospheric pressure, relative humidity, solar radiation and wind speed and direction, were recorded at a 5-minute sampling frequency. These data were utilized for processing the atmospheric CO2 dataset. The correlation between stable isotopic ratios and CO2 concentration, analyzed through the "Keeling plot" approach, enabled the determination of the isotopic signature of the predominant source of atmospheric CO2 in the Palermo urban zone.

The results indicated that wind speed and atmospheric pressure exerted opposing effects on atmospheric CO2 concentration. Elevated CO2 levels coincided with periods of high atmospheric pressure and low wind speed, while reduced CO2 concentrations were associated with increased air turbulence during windy periods. However, meteorological variables partly explain the variability in atmospheric CO2, considering contributions from various CO2 sources. The δ13C-CO2 measurements aligned with CO2 derived from fossil fuel combustion, attributed to urban vehicular mobility and residential heating, particularly during winter periods.

Analysis indicates that CO₂ levels in medium-sized urban areas like Palermo exhibit distinct seasonal and daily variations. Seasonal shifts primarily reflects CO2 emissions from hydrocarbon combustion during winter which was unbalanced by CO₂ uptake during productivity season (spring and summer). On the weekly timescale, CO₂ variations reflect population behaviors. CO2 concentrations are lowest during weekends and holiday periods contrasting raises of CO2 concentration on weekdays and in periods of atmospheric stability, especially in winter. Urban-scale observations, where the majority of greenhouse gases are emitted, allow for tracking high-frequency variations driven by environmental conditions and changes in human activities. Monitoring CO₂ in urban areas offers crucial insights for assessing the effectiveness of climate change mitigation measures.

How to cite: Gurrieri, S. and Di Martino, R. M. R.: Temporal Variations and Influencing Factors on Atmospheric CO2 in Urban Environments: A Stable Isotope Perspective, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15597, https://doi.org/10.5194/egusphere-egu25-15597, 2025.

EGU25-16221 | Posters on site | BG2.2

An absolute reference frame for nitrous oxide position-specific and clumped isotopic measurements 

Paul Magyar, Nico Kueter, Naizhong Zhang, Noémy Chénier, Lukas Emmenegger, Béla Tuzson, and Joachim Mohn

Stable isotopes are a powerful tool for constraining the sources and sinks of nitrous oxide (N2O), essential for identifying and mitigating the climate and air quality impacts of N2O emissions. Site preference (SP), the position-specific N stable isotope incorporation in N2O (14N15N16O vs 15N14N16O), has proven especially useful. Measurements of the clumped isotopologues 14N15N18O, 15N14N18O, and 15N15N16O are emerging as new constraints on the processes of N2O formation and destruction. An advantage of clumped and position-specific isotopic systems over conventional stable isotopes is the existence of an absolute reference frame: under equilibrium conditions, isotopes are randomly distributed among molecules at high temperatures, and deviations from this random distribution at lower temperatures can be both predicted by thermodynamic modelling and measured.

We use quantum cascade laser adsorption spectroscopy to measure the seven-dimensional stable isotopic composition of N2O (δ15N, δ18O, ∆17O, SP, ∆14N15N18O, ∆15N14N18O, and ∆15N15N16O). This spectroscopic approach provides key benefits for standardization studies, including the ability to measure each isotopologue directly without the need for the fragmentation and rearrangement corrections required by mass spectrometric methods. In addition, the ability to measure a sample in replicate (n = 3) in <30 min with precision better than ±0.3‰ for all isotopologues increases the throughput of N2O clumped isotope measurements and improves greatly on previous analytical approaches.

We present results for N2O equilibrated over g-alumina, which has been identified as a catalyst for the N-O isotope exchange equilibria, at temperatures between 170 °C and 230 °C. This range of temperatures represents an optimum where the kinetics of isotope exchange reactions outpace N2O thermal decomposition but proceed fast enough for readily repeatable experiments. Additionally, this range of temperatures is associated with a predicted variation in SP of 4.6‰, suitable for evaluating the temperature dependency of reactions among N2O isotopologues. We find the catalytic activity of g-alumina to be sensitive to its conditions of activation and to the N2O/catalyst ratio. We report equilibration and analyses of gases of a wide variety of starting isotopic compositions to demonstrate the equilibrium nature of these reactions by the principle of bracketing, to document the kinetics of isotope exchange for each isotopologue, and to establish a set of reference gases suitable for robust two-point calibration in all isotopic dimensions.

How to cite: Magyar, P., Kueter, N., Zhang, N., Chénier, N., Emmenegger, L., Tuzson, B., and Mohn, J.: An absolute reference frame for nitrous oxide position-specific and clumped isotopic measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16221, https://doi.org/10.5194/egusphere-egu25-16221, 2025.

EGU25-16416 | ECS | Posters on site | BG2.2

A comprehensive carbon isotopic analysis of seasonal carbon dioxide variability from an urban environment in Hungary 

Balázs Áron Baráth, Tamás Varga, István Major, Sándor Bán, Zoltán Barcza, László Haszpra, Thomas Röckmann, Jacoline van Es, Carina van der Veen, and Mihály Molnár

Urban areas as important sources of industrial and transport emissions, have a key impact on the atmospheric greenhouse gas trends. In order to study these emissions we collected atmospheric air samples at the HUN-REN Institute for Nuclear Research (ATOMKI) of Debrecen, Hungary, in three different seasons (winter, spring and summer). Sampling was done to reflect differences between weekdays and weekends and between morning and afternoons. For this study we collected at least 23 samples each season. We compared carbon dioxide (CO2) concentration and radiocarbon (14C) results with observations from the Hungarian ICOS (Integrated Carbon Observation System) regional background station. Within the project, stable isotope analysis was performed at Utrecht University while CO2 mole fraction and 14C were measured at ATOMKI.

The results show that depleted δ13C and Δ14C values observed during morning hours -especially winter- may indicate fossil fuel emission sources.  On the other hand, summer shows enriched isotopic values because of the stronger biogenic uptake. We analyzed strong correlations between δ¹³C and Δ¹⁴C values in winter, compared to weaker correlations in spring, suggesting that isotopic signals may be influenced by different processes depending on the season. The findings provide important information in the field of carbon isotopic measurements that could simplify distinguishing between CO2 sources or understanding seasonal shifts between biogenic and anthropogenic sources.

Project number C2295145 has been implemented with the support provided by the Ministry of Culture and Innovation of Hungary from the National Research, Development and Innovation Fund, financed under the KDP-2023 finding scheme.

How to cite: Baráth, B. Á., Varga, T., Major, I., Bán, S., Barcza, Z., Haszpra, L., Röckmann, T., van Es, J., van der Veen, C., and Molnár, M.: A comprehensive carbon isotopic analysis of seasonal carbon dioxide variability from an urban environment in Hungary, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16416, https://doi.org/10.5194/egusphere-egu25-16416, 2025.

EGU25-16768 | ECS | Posters on site | BG2.2

Numerical simulation of the impact of atmospheric OH variability on the global mean δ13C(CH4) trend. 

Anna-Leah Nickl, Patrick Jöckel, Franziska Winterstein, and Anja Schmidt

The hydroxyl radical (OH) serves as a primary sink for CH4 in the atmosphere and plays an important role in interpreting the global CH4 budget. Changes in the OH trend have recently been proposed as a potential explanation for the renewed increase of CH4 and the simultaneous decrease in δ13C(CH4) since 2007. In this work, we introduce comprehensive numerical sensitivity simulations to explore the impact of temporal OH variations on the globally averaged CH4 mixing ratio and δ13C(CH4) signature. We apply the state-of-the-art global chemistry-climate model EMAC and use a simplified approach to simulate methane loss. Our simulations apply different OH fields, including climatologically described and transient OH fields, and assume moderate changes in the CH4 tropospheric lifetime. We also consider methane isotopologues and the kinetic isotope effects in physical and chemical processes. The setup uses recent CH4 emission inventories and accounts for regional differences in the isotopic signatures of individual emission source categories. Our results suggest that the influence of an OH reduction on the global δ13C(CH4) is rather small and does not explain the observed trend in CH4. Additionally, we examine the impact of the latitudinal OH distribution on the relative contribution of different emission source categories to the global CH4 rise and the global mean surface δ13C(CH4).

How to cite: Nickl, A.-L., Jöckel, P., Winterstein, F., and Schmidt, A.: Numerical simulation of the impact of atmospheric OH variability on the global mean δ13C(CH4) trend., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16768, https://doi.org/10.5194/egusphere-egu25-16768, 2025.

EGU25-17262 | ECS | Orals | BG2.2

Modelling the triple-isotopic composition of dissolved oxygen using a 3D Earth System Model of intermediate complexity 

Emeline Clermont, Ji-Woong Yang, and Didier M. Roche

Marine photosynthesis (or gross primary productivity, GPP) is one of the main mechanisms for carbon fixation and global oxygen formation, contributing around half of the oxygen produced on Earth and sustaining aquatic ecosystem. Understanding the mechanisms that regulate GPP is essential for gaining insights into biological oxygen and carbon cycles. The combined study of GPP with net primary productivity (NPP) and net community productivity (NCP) will greatly improve our understanding of the interactions between biological processes, linking photosynthesis, respiration and the carbon cycle.

The triple isotopic composition of dissolved oxygen has been proposed as a tracer of gross oxygen productivity in aquatic ecosystem (Luz & Barkan, 2000).  The reasoning behind this is that the ∆17O of dissolved O2 is determined by two main end-members: the marine photosynthesis (∆17O ~ 249 ppm) and the atmospheric O2 (∆17O ~ 8 ppm), as ∆17O is not much affected by other processes that fractionate oxygen in a mass-dependent manner. However, subsequent studies have highlighted potential sources of uncertainty or bias in this proxy. Uncertainties about fractionation factors and transport parameters call the tracer into question (Levine et al., 2009; Nicholson et al., 2014; Li et al., 2022).

To address this issue, we have recently implemented the triple isotopic composition (δ17O and δ18O) of dissolved O2 into the 3D Earth System Model of intermediate complexity, iLOVECLIM. We will present our preliminary results of model comparing them with observation and discussing sensitivity experiments; we further compare our results to previous findings that used 1D or 2D modeling approaches.

How to cite: Clermont, E., Yang, J.-W., and Roche, D. M.: Modelling the triple-isotopic composition of dissolved oxygen using a 3D Earth System Model of intermediate complexity, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17262, https://doi.org/10.5194/egusphere-egu25-17262, 2025.

EGU25-17599 | Posters on site | BG2.2

In-situ atmospheric measurements of CO2 polyisotopologues at Weybourne Atmospheric Observatory in the United Kingdom 

Penelope Pickers, Grant Forster, Jan Kaiser, Alina Marca, Andrew Manning, Richmal Paxton, and Tim Arnold

The δ18O signature of atmospheric CO2 can be used as a tracer for estimating gross primary production (GPP), however, this method requires having detailed knowledge of δ18O signatures of numerous water reservoirs and isotopic fractionation associated with transfer processes, which are highly variable due to the complexity of the hydrological cycle. Simultaneous measurements of δ18O-CO2 and δ17O-CO2 can simplify this requirement, since variations in δ17O are, for most processes, strongly correlated with variations in δ18O. Thus, it is possible to combine measurements of δ18O-CO2 and δ17O-CO2 into a tracer that removes the mass-dependent fractionations related to the hydrological cycle, known as the ‘triple oxygen isotope excess’ (Δ17O). Variability in Δ17O only depends weakly on the oxygen isotope signatures of soil and leaf water and should therefore in principle be a more direct tracer for GPP than variations in δ18O alone.

We present a 2.5-year record (2021-2024) of atmospheric δ13C-CO2, δ18O-CO2, δ17O-CO2, Δ17O, and CO2 mole fraction measurements at Weybourne Atmospheric Observatory on the north Norfolk coast in the UK (52º 57’ N, 1º 07’ E). Measurements are made in-situ every 4 minutes using a tuneable infrared laser direct adsorption spectroscopy (TILDAS) dual-laser analyser from Aerodyne Research Inc. We present observed atmospheric variability in Δ17O on seasonal, diurnal, and synoptic timescales, and report the measurement system short-term repeatability and reproducibility.

How to cite: Pickers, P., Forster, G., Kaiser, J., Marca, A., Manning, A., Paxton, R., and Arnold, T.: In-situ atmospheric measurements of CO2 polyisotopologues at Weybourne Atmospheric Observatory in the United Kingdom, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17599, https://doi.org/10.5194/egusphere-egu25-17599, 2025.

EGU25-17839 | Orals | BG2.2

High precision QCL based direct detection of stable isotopes and tracers in bio-geoscience 

Jonas Bruckhuisen, Morten Hundt, Jiri Hlubucek, Etienne Smith, and Oleg Aseev

To study the geochemical cycles of important greenhouse gases, it is helpful to go beyond measuring their concentrations. Measurements of isotopic ratios can help identify emission sources and study biological and chemical processes. This can include laboratory incubation experiments in soil, agricultural and grass lands, wastewater, and other microbial active aqueous solutions.

The abundances of the 15N and 18O isotopes can be compared to the main isotope 14N14N16O, revealing the distinct isotopic signatures. As a linear molecule with two nitrogen atoms, N2O has two structural isomers of identical mass, which cannot be distinguished by mass spectroscopy. Therefore, a geometry sensitive laser spectroscopy-based approach is required.

The new MGAi-N2O from MIRO Analytical simplifies the monitoring of N2O isotopic composition by enabling simultaneous online measurements of up to 5 major isotopologues of N2O at high measurement rates, while providing excellent stability and precision at a fraction of the cost of isotope mass spectrometers. 

In our presentation we will demonstrate the simultaneous measurement of 5 isotopologues of N2O including 17O using our recently launched MGAi-N2O analyzer. Measurements of different samples, showing high stability and precision, illustrate the potential but also the limitations of this novel analyzer. In addition to continuous flow, a batch sampling mode option will be introduced and characterized.  Recent improvements in the measurement of novel tracers such as OCS and HONO, combined with up to 9 other gases in a single instrument, will also be presented.

How to cite: Bruckhuisen, J., Hundt, M., Hlubucek, J., Smith, E., and Aseev, O.: High precision QCL based direct detection of stable isotopes and tracers in bio-geoscience, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17839, https://doi.org/10.5194/egusphere-egu25-17839, 2025.

EGU25-18216 | Posters on site | BG2.2

Semi-automated separation of methane from ambient air for analysis of Δ13CH3D and Δ12CH2D2 

Tim Arnold, Sara Defratyka, Andrew Gartside, Freya Wilson, Chris Rennick, Matthieu Clog, and Ed Chung

Bulk isotope ratios (δ13C-CH4 and δD-CH4) are used as tracers to help determine the contribution of methane (CH4) sources and sinks to the atmospheric burden. The multiply substituted (clumped) isotopologues are now potentially available as additional tracers to improve these distinctions in the global understanding of the CH4 budget. Measurement of Δ13CH3D and Δ12CH2D2, however, is more challenging than measurements of bulk isotopes and requires more advanced instrumentation. Our ongoing project, POLYGRAM (www.polygram.ac.uk), is developing the sampling strategy, sample preparation, mass spectrometry, and modelling work to begin monitoring these new isotopologue ratios.

Use of a custom-built automated preconcentrator is a key step in our approach during sample preparation, as HR-IRMS requires ultra-pure CH4 samples to measure the multiply substituted isotopologues. For ambient air studies we obtain 150 ml samples (1 bar) containing around 1% amount fraction of CH4, which can then be easily transported and further purified for final analysis. Importantly this separation technique is automated, free of liquid cryogen, and requires minimal manual intervention. We have also developed the system to be flexible and allow for preparation from any natural sources containing less than 1% CH4. We will present the validation of the method as well as a discussion to support the motivation for future development of monitoring Δ13CH3D and Δ12CH2D2 in the global atmosphere.

How to cite: Arnold, T., Defratyka, S., Gartside, A., Wilson, F., Rennick, C., Clog, M., and Chung, E.: Semi-automated separation of methane from ambient air for analysis of Δ13CH3D and Δ12CH2D2, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18216, https://doi.org/10.5194/egusphere-egu25-18216, 2025.

EGU25-18701 | Posters on site | BG2.2

Facilitating the development of a global measurement infrastructure for the measurement of stable isotope ratios for greenhouse gases source apportionment 

Christoph Nehrbass-Ahles and Abneesh Srivastava and the CCQM GAWG/IRWG Joint Task Group on Stable Isotope Ratio Metrology for Atmospheric Source Apportionment (CCQM-GAWG-IRWG-TG-ISOTOP)

Recent progress in the field of laser spectroscopy has transformed the measurement of major greenhouse gases in the atmosphere, enabling real-time, in-situ field measurements of carbon dioxide (CO2) and methane (CH4) stable isotope ratios. These advancements provide critical insights into sources and sinks at local, regional, and global scales. These new measurement capabilities have generated an urgent demand for commutable isotopic gas reference materials for CO2 and CH4 at ambient amount fractions in air. Achieving the level of uncertainty required for such reference materials to effectively support climate mitigation efforts remains challenging. Furthermore, the reliance on individual calibration procedures by end-users has resulted in inconsistent data and hindered comparability across datasets. Addressing these challenges requires the development of new reference materials, improved validation protocols, and standardised calibration guidelines. This effort is essential to ensure traceability for field-deployable spectroscopic methods and traditional offline flask sampling techniques using mass spectrometry. The Metrology for Climate Action workshop, co-hosted by BIPM and WMO in 2022, underscored the critical need for an improved metrological support infrastructure to advance global comparability of greenhouse gas stable isotope ratio measurements. National Metrology Institutes (NMIs), Designated Institutes (DIs), and the WMO's Central Calibration Laboratory (CCL) were identified as key contributors in expanding the global network of certified reference material suppliers. This collaboration is crucial for providing the atmospheric measurement community with access to traceable isotopic greenhouse gas reference materials, thereby supporting the verification of emissions measurements. To address these demands, a new CCQM GAWG/IRWG joint Isotope Ratio Task Group was established in April 2023. This task group coordinates efforts among NMIs, DIs, and intergovernmental organisations to facilitate the development of a robust metrological support infrastructure for the accurate measurement of stable isotope ratios for atmospheric greenhouse gases and related applications. As part of its foundational activities, the task group recently submitted a comprehensive paper entitled “Developing Calibration and Measurement Capabilities for Atmospheric Methane Stable Isotope Ratios at NMIs/DIs: Metrology for Global Comparability.” This collaborative effort brought together experts from NMIs, DIs, academia, and intergovernmental organizations to provide key recommendations for advancing the measurement of CH4 stable isotope ratios. The paper also reviews the various elements that make up Calibration and Measurement Capabilities (CMC) to aid NMIs and DIs in developing their capabilities to support the atmospheric community's need for reliable stable isotope ratio measurements of CH4. This presentation will summarise the task group’s objectives, progress, and key recommendations. Additionally, it will provide a preliminary result from a global survey that is conducted in the first quarter of 2025, mapping the global capabilities for the measurement stable isotope ratio of CH4. Through fostering collaboration among diverse stakeholders, the task group aims to enhance global greenhouse gas data comparability and support effective climate action. We invite experts and organisations with a shared interest in this field to join us in this critical endeavour.

How to cite: Nehrbass-Ahles, C. and Srivastava, A. and the CCQM GAWG/IRWG Joint Task Group on Stable Isotope Ratio Metrology for Atmospheric Source Apportionment (CCQM-GAWG-IRWG-TG-ISOTOP): Facilitating the development of a global measurement infrastructure for the measurement of stable isotope ratios for greenhouse gases source apportionment, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18701, https://doi.org/10.5194/egusphere-egu25-18701, 2025.

EGU25-19640 | ECS | Posters on site | BG2.2

Ship-borne atmospheric measurements during MOSAiC contribute to detect CH4 sources and transport pathways in the Arctic  

Sam Sellmaier, Ellen Damm, Torsten Sachs, Benjamin Kirbus, Inge Wiekenkamp, Annette Rinke, Falk Pätzold, Daiki Nomura, Astrid Lampert, and Markus Rex

The Arctic region plays a crucial role in the global methane (CH4) budget, as it is anticipated to contain substantial CH4 sources, such as (subsea) permafrost. The sparse network of land-based meteorological observation stations in the Arctic results in significant data gaps, particularly for marine sea-ice covered regions. Ship-based measurements can complement the land-based data enhancing our process understanding of the CH4 cycling in the Arctic including source-sink dynamics.

This study presents ship-borne observations of CH4 concentration and 𝜹13C-CH4 values continuously recorded in air near the ocean/ sea-ice surface with a Picarro G2132-i Isotope Analyzer during Leg 4 (June/July 2020) and Leg 5 (August/September 2020) of the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition in the Central Arctic. Three approaches to filter contamination by local pollution sources on both time series were compared. Finally, the Pollution Detection Algorithm was applied to the raw data. A comparison with recordings from the closest land stations and their seasonal patterns suggests that the ship-borne data is more closely linked to dynamic changes in methane sources, sinks, and transport processes, rather than being solely driven by seasonality. To unravel underlying processes, which may contribute to variations in the ship-borne data, we employed a two-step approach. First, we defined air mass source areas and transport pathways within the Arctic Ocean boundary layer using five-day backward trajectories modelled with the LAGRANTO analysis tool and ERA5 wind field data. Second, we linked the observed variations to the air mass source regions by utilizing Keeling plot analysis and 𝜹13C-CH4 fingerprints.

Our analysis reveals that variations in the time series are related both to specific geographical source areas and to seasonally different distinct CH4 source strengths within certain source areas. The findings highlight the importance of considering air mass source areas and seasons to understand variations in CH4 concentration and 𝜹13C-CH4 values in the Arctic. The study highlights the need for further collection of ship-borne measurements of CH4 concentration and 𝜹13C-CH4 data to enhance process understanding and modelling approaches.

How to cite: Sellmaier, S., Damm, E., Sachs, T., Kirbus, B., Wiekenkamp, I., Rinke, A., Pätzold, F., Nomura, D., Lampert, A., and Rex, M.: Ship-borne atmospheric measurements during MOSAiC contribute to detect CH4 sources and transport pathways in the Arctic , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19640, https://doi.org/10.5194/egusphere-egu25-19640, 2025.

EGU25-19970 | ECS | Orals | BG2.2

Continuous methane (CH4) isotope measurements in Lindenberg, Germany 

Jacoline van Es, Carina van der Veen, Stephan Henne, and Thomas Rockmann

Methane (CH4) plays a crucial role in the Earth’s radiative balance because it is a potent greenhouse gas with a shorter lifetime compared to CO2. Mitigating CH4 emissions can potentially mitigate climate change over a short period [1]. Mitigating CH4 requires a solid understanding of the emissions, in particular, which source emits the CH4. Isotopic analysis can aid in source partitioning, as different production processes produce CH4 with subtle but significant differences in isotopic composition [3], enabling the differentiation of multiple sources.
CH4 isotopic source signatures are typically obtained through mobile where sources are sampled as close to the emission point as possible [2]. While these  campaigns are valuable, they only capture for a short duration and miss many smaller and unknown emissions. In contrast, continuous CH4 measurements cover longer periods and can detect inaccessible or unknown sources. However, the downside is that identifying the exact source can be more challenging as the source origin is not always known.
Researchers at Utrecht University developed an isotope ratio mass spectrometer (IRMS) system that measures CH4 mole fraction, δD and δ13C at high
precision with a 40-minute resolution. This system was deployed from 15 April 2022 till 8 January 2023 at a tall tower in Lindenberg, Germany. Measurements were initialised at 40 m.a.g.l and later continued 98 m.a.g.l. The station is part of the Integrated Carbon Observation System (ICOS), providing mole fraction measurements of CO, CO2, and CH4. CH4 isotopic data were also compared with simulations from EMPA. These simulations include the CH4 emissions for each category, allowing us to assign an isotopic source signature to each emissions category, and thereby simulating a CH4 isotopic source signature. For the isotopic measurements, we observed 169 peaks shorter than 24 hours.
This corresponds to 67% of the deployment days. Most source signatures indicate a microbial fermentation source (δ13C : [-55‰, -62‰], δD : [-260 ‰, -360 ‰]). Additionally, we identified 19 multi-day elevations, lasting up to 20 days. Eight of these multi-day elevations displayed isotopic signatures similar to those of the diurnal peaks, while the remaining multi-day peaks showed distinctly different source signatures from one another and the diurnal elevations.

How to cite: van Es, J., van der Veen, C., Henne, S., and Rockmann, T.: Continuous methane (CH4) isotope measurements in Lindenberg, Germany, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19970, https://doi.org/10.5194/egusphere-egu25-19970, 2025.

EGU25-20440 | ECS | Orals | BG2.2

In-situ stable carbon isotope measurements with laser ablation and on-chip laser absorption spectroscopy  

Ragnar Seton, Jana Jágerská, and Jan Viljanen

Measuring stable carbon isotope ratios is a powerful method to study both the environment and ecosystems. The isotope ratios can be used as evidence of geological development or in climate sciences to study system interactions where it provides crucial insights about the ecosystem gas exchange. Mass spectrometry has remained the golden standard for stable carbon isotope analysis in solids and Isotope Ratio Mass Spectrometry (IRMS) has been applied in numerous use cases due to its precision and selectivity. However, the demand for on-site and in-situ capable carbon isotope monitoring methods is increasing. 

In this work, we present an in-situ-capable, all-optical method for stable carbon isotope ratio measurements in solid samples that combines laser ablation and on-chip tunable diode laser absorption spectroscopy (TDLAS). Laser ablation is used to transform the samples from solid to gas phase. The gas is then transported with a carrier flow through a microfluidic system, passing a particle filter and into the µl detector volume. The small sample volume is enabled by a suspended nanophotonic waveguide-based TLDAS sensor which was recently demonstrated for isotope-specific CO2 detection with a 20 ppb detection limit and isotope ratio accuracy of 0.2 ‰. Thus, the combination of an on-chip CO2 detector and laser ablation enables the construction of a compact and portable, all-optical sensor for stable carbon isotope ratio measurements. 

The presented measurement technology generates a paradigm shift in studies integrating the ecological, biological, and geochemical processes. This approach has high sample throughput with ~1 min measurement time due to the minimal requirement of sample treatment, enabling measurement of large sample sets. In addition, the measurement system can be applied to both solid and liquid samples enabling rapid, on-site screening of ecosystem carbon cycle. 

How to cite: Seton, R., Jágerská, J., and Viljanen, J.: In-situ stable carbon isotope measurements with laser ablation and on-chip laser absorption spectroscopy , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20440, https://doi.org/10.5194/egusphere-egu25-20440, 2025.

EGU25-20522 | Posters on site | BG2.2

Improvements in ambient CH4 isotope ratio measurements – the isoMET project 

Javis Nwaboh, Joachim Mohn, Mehr Fatima, Dafina Kikaj, and Volker Ebert

Atmospheric observations provide a reality check on the true efficacy of climate change mitigation policy. Methane (CH4) is a potent greenhouse gas (GHG) with multiple complex sources. Stable isotope ratio measurements for CH4 provide the fingerprints necessary to verify emissions by source type. The isoMET project focuses on improving ambient air CH4 isotope ratio monitoring capabilities both in the laboratory and field. This project also targets improvements in the quality of CH4 isotopic source signature information as well as modelling necessary to make top-down emissions estimates with sectorial attribution.

Here, we present a new metrological infrastructure, developed within the isoMET project, for a dataset for CH4 isotope source signature measurements. In addition, information on new state-of-the-art CH4 calibration reference materials, developed in the project, will be provided. Latest results from the project on analytical advances in high-resolution mass spectrometry and laser spectroscopy for doubly substituted isotopic species of CH4 (13CH3D, 12CH2D2) will be shown. In addition, we present results on laboratory and field intercomparison, demonstrating the capability of e.g. optical isotope ratio measurements (OIRS) for δ13C, δ2H, Δ13CH3D and Δ12CH2D2 measurements in CH4. Finally, the use of atmospheric chemistry transport modelling to direct the measurement strategy for optimal emissions estimation will be demonstrated.

References

[1] isoMET project available at: https://www.npl.co.uk/21grd04-isomet

[2] J. A. Nwaboh, J. Mohn, F. Mehr, T. Arnold, V. Ebert, CCQM GAWG-IRWG Workshop on Carbon Dioxide and Methane Stable Isotope Ratio Measurements, LATU (Uruguay), 2023

[3] Mehr Fatima, Javis Nwaboh, Joachim Mohn, Tim Arnold, and Volker Ebert, EGU 2024, EGU24-20560, https://doi.org/10.5194/egusphere-egu24-20560

Acknowledgements: The project 21GRD04 isoMET project has received funding from the European Partnership on Metrology, co-financed from the European Union’s Horizon Europe Research and Innovation Programme and by the Participating States.  Empa has received funding from the Swiss State Secretaritat for Education, Research and Innovation (SERI).

 

How to cite: Nwaboh, J., Mohn, J., Fatima, M., Kikaj, D., and Ebert, V.: Improvements in ambient CH4 isotope ratio measurements – the isoMET project, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20522, https://doi.org/10.5194/egusphere-egu25-20522, 2025.

AS6 – Short Courses & EDI

EGU25-725 | ECS | Orals | EOS4.6

Breaking the Ice Between Machine Learning Experts and Cryosphere Scientists - The ML4Cryo Research Community 

Kim Bente, Julia Kaltenborn, and Andrew McDonald

Recently, Machine Learning (ML) has emerged as a powerful tool within cryospheric sciences, offering innovative and effective solutions for observing, modelling, and understanding Earth's frozen regions. However, the ML and cryosphere communities have traditionally been poles apart, each shaped by distinct research motivations, publishing paradigms, and evaluation criteria. These research silos can lead to common pitfalls of interdisciplinary research, such as "helicopter science", insights getting lost in translation, or the continued use of outdated (ML) methods. To fully harness the compelling opportunities for impactful research at the intersection of these two fields, machine learning practitioners and domain scientists must join forces. 

To address this gap between machine learning and cryosphere research, we established ML4Cryo (Machine Learning for the Cryosphere, see https://ml4cryo.github.io/), a global research community that leverages collective expertise across diverse fields such as deep learning, physics-informed ML, remote sensing, and both terrestrial and marine cryospheric domains. Our goal is not only to advance scientific discovery but also to foster application-driven advances in machine learning research. ML4Cryo aims to empower researchers by initiating conversations and collaborations, enabling machine learning specialists to learn about the most pressing challenges within the cryosphere, while cryosphere researchers can learn about the state-of-the-art models developed by the ML community. Contributing to ML4Cryo’s mission, our platform serves as a community-driven hub to share and discover ideas, recent publications, tools, software, datasets, knowledge resources, funding opportunities, best practices, as well as relevant conferences and events. We invite you to join ML4Cryo, where the synergy between machine learning and cryospheric science paves the way for impactful and rewarding research.

How to cite: Bente, K., Kaltenborn, J., and McDonald, A.: Breaking the Ice Between Machine Learning Experts and Cryosphere Scientists - The ML4Cryo Research Community, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-725, https://doi.org/10.5194/egusphere-egu25-725, 2025.

EGU25-4377 | ECS | Posters on site | EOS4.6

A global dataset for lake physical variables from satellite measurements 

Marina Amadori, Monica Pinardi, Claudia Giardino, Mariano Bresciani, Rossana Caroni, Anna Joelle Greife, Stefan Simis, Jean-Francois Crétaux, Laura Carrea, Herve Yesou, Claude Duguay, Clément Albergel, and Alice Andral

Lakes are responding rapidly to climate change and in coming decades global warming is project to have more persistent and stronger effects on hydrology, nutrient cycling, and biodiversity. Factors driving lake condition vary widely across space and time, and lakes, in turn, play an important role in local and global climate regulation, with positive and negative feedback depending on the catchment. Understanding the complex behaviour of lakes in a changing environment is essential to effective water resource management and mitigation of climate change effects.

To support the comprehension of this topic at a global scale, satellite technologies provide a unique source of data. Remote sensing can indeed enable long-term monitoring of freshwaters, supporting water managers' decisions providing data, and filling knowledge gaps to a better understanding of the regional and local areas most affected and threatened by health status degradation. With this aim, space agencies and the remote sensing community have joined the efforts to provide global, stable, consistent, and long-term products openly available and easily accessible to different kinds of users.

In this contribution, we present the latest release of the dataset from the Lakes_cci project (funded by the European Space Agency), which provides the most complete collection of the Essential Climate Variable LAKES consisting of six thematic products (lake water extent and level, lake ice cover and thickness, lake surface water temperature, lake water-leaving reflectance). The dataset spans the time range 1992 to 2022 and includes over 2000 relatively large lakes, which represent a small fraction of the number of lakes worldwide but a significant portion of the global freshwater surface. An overview of the current version (V2.1) of the dataset and the improvements in quality and usability of the next version (V3) of the dataset will be presented, together with a set of tools and a dashboard for visualisation and download of the data.

With this contribution, we aim to discuss how this kind of product can be useful to the several research communities involved, their limits, potential improvements and chances to further joint research also respect to the research community's expectations and needs.  

How to cite: Amadori, M., Pinardi, M., Giardino, C., Bresciani, M., Caroni, R., Greife, A. J., Simis, S., Crétaux, J.-F., Carrea, L., Yesou, H., Duguay, C., Albergel, C., and Andral, A.: A global dataset for lake physical variables from satellite measurements, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4377, https://doi.org/10.5194/egusphere-egu25-4377, 2025.

EGU25-4414 | ECS | Posters on site | EOS4.6

User-centred design for environmental data services   

Poppy Townsend, Jesse Alexander, Louise Darroch, David Green, Monica Hanley, Nourhan Heysham, Matthew McCormack, Oluwaseni Osunkoya, David Poulter, Shwetha Raveendran, Paulius Tvaranavicius, Carl Watson, and Thomas Zwagerman

To create tailored tools and solutions that improve our ability to mitigate and respond to environmental challenges, we need to understand how to efficiently communicate complex information to the intended audience.  One of the core aims of the UK’s Environmental Data Service is to better engage with users and ensure their needs are central to everything we do.  
 
How we design, maintain and share our services hasn’t traditionally been prioritised with user feedback in mind. Many of our teams and systems are now having to change the way we work and learn new skills. There was no central location to share good practice about user-centred design of tools/services specifically for environmental sciences. We wanted to create guidance for our staff and others who develop and maintain data services for environmental science.  

We have created a ‘user-centred design toolkit for environmental services’ with the aim of supporting data, software and design experts to create user-friendly and effective environmental data services. This toolkit provides a range of resources, case studies and guidance needed to collaborate with users, gather insights, and co-design solutions that work. The toolkit has been shaped by collaborations across all environmental science domains, with a range of experts in user design, data management, communications and engagement, and software engineering.  

The toolkit is still in early development. We are looking to share our progress so far, understand if this is something the wider community would like to contribute to or partake in a community of practice.  

How to cite: Townsend, P., Alexander, J., Darroch, L., Green, D., Hanley, M., Heysham, N., McCormack, M., Osunkoya, O., Poulter, D., Raveendran, S., Tvaranavicius, P., Watson, C., and Zwagerman, T.: User-centred design for environmental data services  , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4414, https://doi.org/10.5194/egusphere-egu25-4414, 2025.

EGU25-4541 | ECS | Posters on site | EOS4.6

For a FAIR publishing environment: Geomorphica, the Diamond Open-Access Journal for Geomorphology 

Melanie Stammler, Katy Burrows, Bastian Grimm, Caio Breda, Larry Syu-Heng Lai, Matthieu Giaime, Roberto Fernández, and Alice Lefebvre

Scientific data needs to be Findable, Accessible, Interoperable, and Reusable (FAIR). Scientific publications should also follow these accessibility principles. Diamond Open Access publishing represents an approach where articles are free for all to read, without journal subscription, and free to publish, without article processing fees for authors, who also retain the copyright of their work. Thus, it strongly contributes to FAIR, open and transparent scientific publishing - promoting inclusivity and eliminating barriers.

Geomorphica (http://geomorphica.org) is a community-led and -driven scientific journal that fosters academic discourse and research advances in the field of geomorphology. It is hosted by Penn State University Libraries, supported by the International Association of Geomorphology and a proud part of the family of Diamond Open-Access journals in the Geosciences. 

Geomorphica is run by over 30 volunteers that embody the editorial, equity diversity and inclusion, communications, and ethics teams and contribute to all functions including administration, managing, editing, reviewing, typesetting, and visual branding. Geomorphica has been open for submission since June 2023 and welcomes manuscripts related (but not limited) to landscapes and landforms, Earth’s and planetary near-surface processes, and the mechanisms, dynamics and timescales pertaining to these processes. 

Here, we introduce our diverse team of volunteers, give an update on the number of manuscripts we have handled so far, and share our experiences related to setting up and running a Diamond Open Access journal. Further, we exemplify what FAIR can stand for in scientific publishing, showcasing how Geomorphica is addressing the principle. We welcome feedback from the broader community to help us continually improve Geomorphica and look forward to your involvement with the initiative.

How to cite: Stammler, M., Burrows, K., Grimm, B., Breda, C., Lai, L. S.-H., Giaime, M., Fernández, R., and Lefebvre, A.: For a FAIR publishing environment: Geomorphica, the Diamond Open-Access Journal for Geomorphology, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4541, https://doi.org/10.5194/egusphere-egu25-4541, 2025.

EGU25-4635 | Orals | EOS4.6

Developing AIDMAP: A roadmap to interactive community-based data compilation for magnetic data in Antarctica. 

Alan Aitken, Joerg Ebbing, Max Lowe, Mareen Loesing, Wolfgang Szwillus, Lu Li, and Eagles Graeme

Antarctica poses a unique challenge for data compilation and sharing, due to the sourcing of data from many national programs and a diversity of surveys and data access protocols. Coordinated by the Scientific Committee on Antarctic Research, the Antarctic Digital Magnetic Anomaly Project (ADMAP) has made huge progress to collate coordinate and disseminate the magnetic data of Antarctica. ADMAP’s first iteration was produced in 2001, and the second iteration was released in 2018. The community is looking now towards the next iteration to support ongoing research in Antarctica. We present here a roadmap for this data compilation, with a focus on the ability for researchers to access a live and interactive resource, to add new data when it is available, and for this to be realised in the compilation soon after data submission. For this it is necessary to ease the burden of data processing, to define a consistent approach to the data handling, and to accelerate the timeline from data-submission to incorporation into the compilation. The approach therefore is founded on an automated data-processing workflow that can accommodate the wide variety of data submitted (variable spacings, heights and times of collection), can tolerate incremental updates to the main product within a reasonable compute load, and can achieve results within a reasonable tolerance without requiring manual intervention. This presentation focuses on the intended approach to compilation and the expected outcomes, based on a test-case.

How to cite: Aitken, A., Ebbing, J., Lowe, M., Loesing, M., Szwillus, W., Li, L., and Graeme, E.: Developing AIDMAP: A roadmap to interactive community-based data compilation for magnetic data in Antarctica., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4635, https://doi.org/10.5194/egusphere-egu25-4635, 2025.

EGU25-8347 | Orals | EOS4.6

The evolution of the Polar-AOD network: towards a comprehensive repository supporting efforts for integrated polar observing systems 

Simone Pulimeno, Mauro Mazzola, Angelo Lupi, Giulio Verazzo, Alice Cavaliere, Claudia Frangipani, Robert Stone, and Vito Vitale

Atmospheric aerosols play a crucial role in Earth's atmospheric environment and are among its most variable components. In polar regions, aerosols originate from both natural and anthropogenic sources. In the Arctic, the majority of the aerosol mass consists of oceanic sea-salt, mineral dust, non-sea-salt sulphate, and products of biomass burning (Tomasi et al. 2015). In contrast, anthropogenic aerosols are dominated by black carbon (BC) and nitrate, which are signatures of traffic and industrial emissions (Quinn et al. 2007). Polar aerosols can have significant regional effects by interacting with incoming solar radiation and by altering the albedo of the surface-atmosphere system (IPCC 2023). To address and study these effects, the Polar-AOD project was proposed for the first time in 1999 by Claudio Tomasi from the National Research Council of Italy. This initiative aims to characterize the means, variability, and trends of aerosol properties in polar regions. Its primary goal is to connect observational stations measuring aerosol properties along the atmospheric vertical column. These observations provide critical data to quantify aerosol physical and radiative properties at high latitudes, including seasonal background concentrations derived from aerosol optical depth (AOD) measurements, spectral characterizations, and the influence of natural and anthropogenic processes on the radiative balance of the surface and atmosphere. This project fosters collaboration among scientists in the field of photometry at both poles. It also incorporates the stellar and lunar photometry data, which help to address historical gaps in AOD climatologies during the polar night. By filling these gaps, the Polar-AOD project contributes to a comprehensive understanding of aerosol behavior and its impacts on the polar regions. To support this effort, a new web platform has been recently developed to store and share data and metadata from photometric measurements, forming a polar AOD archive. This archive, managed by CNR through GeoNetwork, enables the organization and search of spatially referenced resources while allowing each scientific group to manage its own data, choosing to share metadata only or both data and metadata for specific sites or campaigns within the Polar-AOD network. The new data portal will be presented, along with the maps of the stations and instruments, and the Polar-AOD metadata catalogue.

Bibliography

Intergovernmental Panel on Climate Change (IPCC) (2023). Climate Change 2021 – The Physical Science Basis: Working Group I Contribution to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change. Cambridge University Press, Cambridge

Quinn, P. K. et al. (2007), Arctic haze: current trends and knowledge gaps, Tellus B, 59(1):99–114. https://onlinelibrary.wiley.com/doi/pdf/10.1111/j.1600-0889.2006.00238

Tomasi, C. et al. (2015), Aerosol remote sensing in polar regions. Earth-Science Reviews, 140:108–157, 0012-8252, http://dx.doi.org/10.1016/j.earscirev.2014.11.001

How to cite: Pulimeno, S., Mazzola, M., Lupi, A., Verazzo, G., Cavaliere, A., Frangipani, C., Stone, R., and Vitale, V.: The evolution of the Polar-AOD network: towards a comprehensive repository supporting efforts for integrated polar observing systems, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8347, https://doi.org/10.5194/egusphere-egu25-8347, 2025.

EGU25-8669 | Posters on site | EOS4.6

An immersive virtual approach to enhance visibility of global stratotype and reference sections of the Paleogene 

Simonetta Monechi, Laia Alegret, Aitor Payros, Claudia Agnini, Gabriele Scaduto, and Bruno Fanini

Access to geological reference sections can have limitations related to geo-political reasons, travel restrictions during global pandemics, weather conditions or time and funding for travelling, among other limiting factors. In addition, the quality of outcrops and their access often deteriorate due to weathering or vegetation cover, making it difficult and even impossible to use them in scientific research and public outreach. The rapid development of three-dimensional digital models has changed this scenario, deeply contributing to innovative information technologies and scientific research in geoscience.

In order to enhance and give visibility to Paleogene global reference sections such as the Global Stratotype section and point (GSSP) that officially marks the base of standard geological units (stages and ages), as well as globally significant geo-heritage sites, the International Subcommission on Paleogene Stratigraphy (ISPS) has focused on the acquisition and digitization of geological outcrops. The results are publicly available on the ISPS website https://www.paleogene.org/, and will be populated with additional information in the future.

Data acquisition used photogrammetry and Lidar modeling techniques with mobile phones. The models were enhanced to create an immersive virtual experience of the geosites. The utilization of ATON, an open-source framework developed by the Institute of Heritage Science of the Italian National Research Council (CNR ISPC), allows the exploration of large, massive 3D datasets using HMDs (i.e. Oculus Quest) directly through a web browser. Such a modular framework offers advanced functionalities like visual immersive analytics and integration with complex multimedia content. Users virtually immerse in the outcrop enabling real-time querying of all geometries, annotations and measurement functionalities (e.g. examining 3D fossils and other material or associated information).

This digital approach offers a unique opportunity for saving temporary outcrops, geological features or fossils in virtual environments, and it will contribute to facilitate examination of the most relevant outcrops of the Paleogene by scientists, and to promote and disseminate geo-education.

How to cite: Monechi, S., Alegret, L., Payros, A., Agnini, C., Scaduto, G., and Fanini, B.: An immersive virtual approach to enhance visibility of global stratotype and reference sections of the Paleogene, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-8669, https://doi.org/10.5194/egusphere-egu25-8669, 2025.

EGU25-9230 | Posters on site | EOS4.6

The Hellenic DataBase of Active Faults (HeDBAF): a new, national geodatabase of active faults for the broader Greek territory 

Dimitris Galanakis, Sotiris Sboras, Dimitris Sakellariou, Spyros Pavlides, Kyriaki Iordanidou, Charalambos Georgiou, Athanasios Ganas, Ioannis Koukouvelas, Charalambos Kranis, Spyros Lalechos, Theodora Rondoyanni, and Efthimios Lekkas and the EPPO Seismotectonics Committee

A new geospatial database started to realize since 2021 including parametric and descriptive information about the active faults in the broader Aegean region (Eastern Mediterranean). The Hellenic DataBase of Active Faults (HeDBAF) is a national ongoing product developed under the auspices of the EPPO (Earthquake Planning & Protection Organisation) and the supervision of its Seismotectonics Committee. The responsibility of implementation, management and hosting is held by the Hellenic Survey of Geology & Mineral Exploration (HSGME).

Active fault databases for broader Greece already existed since about 2010. Besides the fact that these databases were materialized by small groups of researchers, their objectives were also rather narrow, offering data and information for particular purposes. The HeDBAF adopts conceptual approaches and characteristics from other time-proven national databases of the world (e.g. INGV’s DISS, IGME’s QAFI, etc.). It is a multi-layered tool that hosts all available literature data (e.g. scientific articles, technical/project reports, thematic maps, etc.), targeting various groups of end-users: the primary target group is the scientific community which often needs medium- to small-scale information for geodynamic interpretations, large-scale data for local seismotectonic analyses, and appropriate parametric information for numerical modelling. The next target group is the engineers who need large-scale detailed surveying of the fault traces and ground ruptures, and fault models for the prediction of ground motion in the context of Seismic Hazard Assessment. Administration, government, security bodies and local authorities can benefit from this geodatabase as a decision-making tool for safety and rescue planning. Last, but not least, a broad range of citizens will be able to access principal theoretical and parametric information about active faults in areas they are interested in.

Until today, two main fault datasets have started to develop: i) the Fault Traces, and ii) the Fault Zones datasets. The former focuses on the mapping accuracy of faults, targeting on large- to medium-scale data (> 1:50,000). Faults originating from smaller scale maps are reassessed (if possible) using hi-resolution topographic data. Primary co-seismic ground ruptures are distinguished from geologically detected fault traces to better understand the surficial rupturing process for fault rupture hazard purposes. The Fault Zones dataset involves fault segmentation and earthquake rupture scenarios which are crucial for Seismic Hazard Assessment (SHA). Thus, the fault zones are represented by medium- to small-scale lineaments which also facilitate the visualization of large tectonic structures in small-scale maps. The HeDBAF, as a very young effort still misses both fault occurrences and associated information. However, the geodatabase is continuously updateable and upgradeable showing frequent improvements and enrichments.

How to cite: Galanakis, D., Sboras, S., Sakellariou, D., Pavlides, S., Iordanidou, K., Georgiou, C., Ganas, A., Koukouvelas, I., Kranis, C., Lalechos, S., Rondoyanni, T., and Lekkas, E. and the EPPO Seismotectonics Committee: The Hellenic DataBase of Active Faults (HeDBAF): a new, national geodatabase of active faults for the broader Greek territory, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9230, https://doi.org/10.5194/egusphere-egu25-9230, 2025.

CSV and Excel formats are among the most common storage formats for data sharing, especially in scientific and government contexts. Chaves-Fraga notes that a significant amount of public data is published in tabular formats such as CSV and Excel, which can hinder data accessibility and interoperability due to their lack of standardized metadata (Chaves-Fraga,  2020). This is in line with the findings of Burg et al. (2019). They highlight that although CSV files are widely used due to their simplicity, they often lack the necessary metadata to ensure data quality and provenance, which are crucial for compliance with the FAIR principles. Furthermore, Kaur et al. (2021) highlight that many health information systems allow data to be exported in CSV format, which is accessible but does not provide the semantic interoperability needed for effective data sharing and reuse. Furthermore, the limitations of CSV and Excel formats are compounded when datasets are converted to SQLite databases.

The NFS group (NuoroForestrySchool.io) has developed an open source Python-based application (https://gitlab.com/NuoroForestrySchool/nfs-data-documentation-procedure) that facilitates the organization of the data a researcher is willing to share. 

The application is designed to be used as a command line tool or through a graphical interface. It reads as input a spreadsheet file with one sheet for each table, plus an application-specific sheet defining the database schema, the data dictionary, the DataCite metadata, and other specific metadata (extended title, abstract/summary). The output of the procedure is represented by a SQLite file containing all the data and metadata, as well as an image of the graphical ERD-like schema, and a formal pdf document presenting the contents of the database. The SQLite file is a metadata-rich SQL-based database, taking full advantage of relational features and thus improving data accessibility, interoperability, and reusability by humans and machines.

The use of the procedure is demonstrated by processing a simple but significant use case.

LITERATURE

Chaves-Fraga, David, Edna Ruckhaus, Freddy Priyatna, Maria-Esther Vidal, e Oscar Corcho. 2021. «Enhancing virtual ontology based access over tabular data with Morph-CSV». A cura di Axel-Cyrille Ngonga Ngomo, Muhammad Saleem, Ruben Verborgh, Muhammad Saleem, Ruben Verborgh, Muhammad Intizar Ali, e Olaf Hartig. Semantic Web 12 (6): 869–902. https://doi.org/10.3233/SW-210432.
Kaur, Jasleen, Jasmine Kaur, Shruti Kapoor, e Harpreet Singh. 2021. «Design & Development of Customizable Web API for Interoperability of Antimicrobial Resistance Data». Scientific Reports 11 (1): 11226. https://doi.org/10.1038/s41598-021-90601-z.
Van Den Burg, G. J. J., A. Nazábal, e C. Sutton. 2019. «Wrangling Messy CSV Files by Detecting Row and Type Patterns». Data Mining and Knowledge Discovery 33 (6): 1799–1820. https://doi.org/10.1007/s10618-019-00646-y.

How to cite: Scotti, R., Giadrossich, F., and Casalta Badetti, A.: NFS-FAIR-DDP  the data documentation procedure developed by NuoroForestrySchool as   open source tool to upgrade entry level data sharing by exploiting the SQL standard, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9663, https://doi.org/10.5194/egusphere-egu25-9663, 2025.

The Science Explorer (SciX) digital library is a cutting-edge solution designed to address the growing complexity of accessing, evaluating, and synthesizing the expanding body of literature in Earth and environmental sciences. While the Earth System itself remains as intricate as ever, the challenge today lies in navigating an increasingly vast and diverse array of research and data. SciX responds to this need by providing a centralized, open-access platform that enhances the discovery and integration of scientific literature, all while adhering to the FAIR principles—Findable, Accessible, Interoperable, and Reusable.

In this session, we will showcase how SciX empowers researchers to efficiently explore a vast repository of scholarly publications relevant to the Earth and environmental sciences. Leveraging Artificial Intelligence (AI) and Machine Learning (ML) technologies, SciX optimizes literature search and discovery, enabling users to easily locate, evaluate, and engage with the most pertinent scientific papers and resources. Features like personalized searches, citation exports, and tailored alerts allow researchers to stay at the forefront of their fields.

We will also highlight the powerful bibliometric tools within SciX, including parameterized search and advanced visualization capabilities. These bibliometric visualizations help researchers uncover connections between authors, citations, and emerging research trends, enabling the identification of potential collaborators across disciplines and fostering a broader, more integrated approach to scientific inquiry. By mapping key contributors and intellectual networks, SciX facilitates cross-disciplinary collaboration, enhancing the impact of research across the Earth System.

At the heart of SciX is a commitment to open science and continuous user engagement. The platform evolves based on user-driven feedback, ensuring that it meets the evolving needs of the scientific community. This presentation will demonstrate how SciX is shaping the future of literature review, collaboration, and interdisciplinary research in Earth and environmental sciences.

Attendees will leave with practical insights into how SciX can streamline their literature review process, promote collaboration across scientific disciplines, and help tackle the challenges of today’s rapidly expanding research landscape.

How to cite: Kurtz, M., Myers, B., and Kelbert, A.: Enhancing Geoscience Collaboration and Discovery: Leveraging the Science Explorer (SciX) for Efficient Literature Review and Interdisciplinary Research, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10379, https://doi.org/10.5194/egusphere-egu25-10379, 2025.

EGU25-12152 | Posters on site | EOS4.6

GeoFutures: bridging the gap between geoscience and (dis)engaged audiences for the 21st century 

Thomas Harvey, Emelia Spofforth-Jones, Elisha McCowan, and Natasha Stephen

'GeoFutures' is the Geological Society of London’s flagship conference series focussing on 21st century geoscience and solutions that geoscientists can offer to global challenges. The series cycles through the Society’s five strategic science themes, with the inaugural 2023 meeting centred on the theme of 'Digital Geoscience' and the 2024 meeting focussed on the theme of ‘Planetary Geoscience’.

Both meetings have sought to foster collaboration within and out of the geoscience community by bringing together researchers, engineers, citizen scientists, policymakers, funders and representatives from government agencies. We actively seek to encourage attendance by groups and individuals who do not traditionally attend scientific meetings. The series aims to cultivate networks and research partnerships, as well as to spark innovative ideas to shape the response of geoscientists to future issues.

In addition to the disciplinary topics, sessions have focussed on the application of breakthrough technologies and methods, as well as considering how geoscientists might apply these to scientific and societal problems both current and future. Fundamental to this is consideration of how best to ensure that subsequent generations of geoscientists and geoscience facilities are adequately prepared, as well as the importance of communicating geoscience issues and solutions to the public effectively. A large part of both conversations involves promoting open data and science, and collaboration between the many varied interested parties.

In 2025, the series turns to the Society’s ‘Climate and Ecology’ theme, integrating themes from a series of talks and discussions, around the UK, related to climate and ecological research and issues. On a continuing basis, we aim to demonstrate that bringing together contributors and organisations from diverse sectors at novel, discipline-specific meetings is an effective measure to support the UK and wider international geoscience communities to tackle current and future challenges.

How to cite: Harvey, T., Spofforth-Jones, E., McCowan, E., and Stephen, N.: GeoFutures: bridging the gap between geoscience and (dis)engaged audiences for the 21st century, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12152, https://doi.org/10.5194/egusphere-egu25-12152, 2025.

EGU25-13606 | ECS | Posters on site | EOS4.6

SubMachine ORFEUS integration: Web-based tools for exploring seismic tomography models 

Maria Tsekhmistrenko, Kasra Hosseini, Karin Sigloch, Grace Shephard, Mathew Domeier, and Kara Matthews

SubMachine is a collection of web-based tools for the interactive visualisation, analysis, and quantitative comparison of global-scale datasets of the Earth's interior [1]. It focuses on making regional and global seismic tomography models easily accessible to the wider solid Earth community to facilitate collaborative exploration. Over 30 tomography models can be visualised and explored—individually, side-by-side, or through statistical and averaging tools. SubMachine also serves diverse non-tomographic datasets, including plate reconstruction models, normal mode observations, global crustal structure, shear wave splitting, geoid, marine gravity, vertical gravity gradients, and global topography in adjustable degrees of spherical harmonic resolution.

To ensure continuity beyond the DEEP TIME ERC project [2], SubMachine is transitioning to a new home within ORFEUS (Observatories and Research Facilities for European Seismology, http://orfeus-eu.org/). This transition secures SubMachine’s long-term sustainability and further integrates it into the broader seismological research infrastructure.

In preparation for this move, SubMachine has undergone significant modernization. The entire platform has been migrated to Python 3.12. The transition from Basemap to Cartopy enhances long-term stability, though some projections may experience slower performance. New features include cross-sections through vote maps [3]. These advancements, along with various performance improvements, position SubMachine as a more robust and sustainable resource for the geoscience community.

[1] Hosseini, K., Matthews, K. J., Sigloch, K., Shephard, G. E., Domeier, M., & Tsekhmistrenko, M. (2018). SubMachine: Web-Based Tools for Exploring Seismic Tomography and Other Models of Earth's Deep Interior. Geochemistry, Geophysics, Geosystems, 19(5), 1464-1483.

[2] https://cordis.europa.eu/project/id/833275

[3] Shephard, G. E., Matthews, K. J., Hosseini, K., & Domeier, M. (2017). On the consistency of seismically imaged lower mantle slabs. Scientific reports, 7(1), 10976.

How to cite: Tsekhmistrenko, M., Hosseini, K., Sigloch, K., Shephard, G., Domeier, M., and Matthews, K.: SubMachine ORFEUS integration: Web-based tools for exploring seismic tomography models, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13606, https://doi.org/10.5194/egusphere-egu25-13606, 2025.

EGU25-14319 | Posters on site | EOS4.6

The TERN Australia Soil and Herbarium Collection, a national ecological treasure 

Katie Irvine, Sally O'Neill, Andrew Tokmakoff, Donna Lewis, and Ben Sparrow

TERN (Terrestrial Ecosystem Research Network) is Australia’s field-based ecological observatory; national research infrastructure for collecting, recording and sharing data and samples using highly instrumented monitoring sites, field surveys and remote-sensing techniques such as drones and satellites. TERN’s freely available long term monitoring data and samples are used by researchers, government decision makers and industry in Australia and internationally.

The TERN Australia Soil and Vegetation Collection is a purpose-built treasure trove for scientists, bringing together more than 150,000 soil samples, soil metagenomic samples, plant voucher specimens, plant samples and plant genetic material. Beginning in 2012, the TERN field monitoring program has data and samples from 1000 long-term ecological monitoring sites across the continent. The TERN Collection was recently added to Index Herbariorum, the global network of herbaria.

Unlike most soil and plant collections around the world, each sample in the TERN Collection is associated with comprehensive, highly detailed environmental information about the 100m x 100m survey sites where it was collected. All other specimens sampled at each site are also available, enabling complex research, discovery and understanding such as on relationships between soils, plants, carbon and environmental conditions. Botanists, ecologists, taxonomists and agricultural scientists are frequent users of this collection, and the samples can also be useful to microbiologists for a range of human and environmental health applications. The repository is openly available to interested researchers globally.

This state-of-the-art repository is contributing to important research critical to solving real-world problems, particularly in the areas of climate science, earth observation, conservation, and sustainability.

How to cite: Irvine, K., O'Neill, S., Tokmakoff, A., Lewis, D., and Sparrow, B.: The TERN Australia Soil and Herbarium Collection, a national ecological treasure, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14319, https://doi.org/10.5194/egusphere-egu25-14319, 2025.

EGU25-15003 | ECS | Orals | EOS4.6

Exploring Lossy Data Compression in an Online Laboratory for Climate Science and Meteorology 

Juniper Tyree, Sara Faghih-Naini, Peter Dueben, Karsten Peters-von Gehlen, and Heikki Järvinen

While the output volumes from high-resolution weather and climate models are increasing exponentially, data storage, access, and analysis methods have not kept up. Data compression is a vital tool to keep up with this increase in data production. As lossless compression is no longer sufficient to produce the required compression ratios, lossy compression should be applied instead. However, information loss sounds scary. While mounting research shows that model and measurement data contains “false information” (e.g. noise or uncertainty from measurements or numerical inaccuracies) that can be removed for better compression without degrading the data quality, a convincing argument for lossy data compression can only be made by domain scientists themselves by trying it out for themselves.

Interactive code notebooks (e.g. Jupyter) have become popular for sharing and communicating computational experiments, analyses, and visualizations. While sharing the notebooks is easy, running them requires hosting a JupyterLab server and installing all Python and system libraries required for the notebook. This initial setup cost hinders quickly experimenting with a shared notebook and testing, e.g. a practical example of lossy data compression for oneself.

As part of the EuroHPC ESiWACE, Phase 3, Centre of Excellence (https://www.esiwace.eu/), we have been developing an Online Laboratory for Climate Science and Meteorology (https://lab.climet.eu), a JupyterLab instance that runs serverless just within your web browser and comes with many libraries pre-installed. With the online lab, which builds on the Pyodide and JupyterLite community projects, running and exploring a shared notebook can start within a minute. We use the online laboratory to provide domain scientists with an online compression laboratory, https://compression.lab.climet.eu, to reduce the barrier to experimenting with the effect of lossy compression on their own data. The lab also supports URL schemas to preload other third-party notebooks (and repositories) hosted via Git, as Gists, or behind any URL, so that sharing a ready-to-run notebook is as easy as sharing, e.g., https://lab.climet.eu/v0.2/github/juntyr/climet-lab-demo/v0.2.0/demo.ipynb. We are also working on quickly turning existing static-documentation example-notebooks into interactive documentation that invites immediate further exploration.

In this session, we want to showcase the online laboratory and the services it can provide to the earth science community by live demonstrating its applications in the compression laboratory and others. We also hope to gather feedback on the future direction of its development and collaborations with other open science tools to serve our communities best.

How to cite: Tyree, J., Faghih-Naini, S., Dueben, P., Peters-von Gehlen, K., and Järvinen, H.: Exploring Lossy Data Compression in an Online Laboratory for Climate Science and Meteorology, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15003, https://doi.org/10.5194/egusphere-egu25-15003, 2025.

EGU25-16049 | Posters on site | EOS4.6

Slinging Earth & (exo)Planets Structure and Dynamics into Diamond Open Access 

Stefano Maffei, Maelis Arnould, Mandy Bethkenhagen, Thibault Duretz, Mohamed Gouiza, Lorraine Hwang, and Iris van Zelst

The past decade has seen the consolidation of open access practices in scientific publishing, with funding bodies, international agencies and academic institutions requiring free access to not only scientific papers but also other output such as datasets and computer codes. The transition to open access practices has led multiple academic publishers to offer Gold Open Access (GOA) schemes, under which scientific papers are free-to-read. Compared to the traditional publication models, GOA comes at a much higher cost for authors. These practices have had a documented negative impact on the scientific publishing landscape, from the rise of predatory journals to the broadening of the economic divide between academic institutions.

Partly in response, different fields of Earth Sciences have seen the rise of several community-led Diamond Open Access journals (DOAJ). These journals are free-to-publish and free-to-read. The aim is to remove financial barriers to scientific publishing by making peer-reviewed articles available at no cost to both authors and readers, thus offering a platform for true open science. DOAJs are created and maintained by the very same scientific community they aim to serve, thus removing economical and business considerations that drive a large fraction of the modern publishing landscape. These community-led journals offer a high-quality alternative to classical for-profit scientific journals.

We are pleased to announce a new DOAJ initiative called Geodynamica. Coordinated by a core committee of seven scientists, Geodynamica aims at promoting academic discourse and disseminating research pertaining to the quantitative study of Earth and (exo-)planetary internal structure, dynamics, and evolution from observational to modelling perspectives.

Geodynamica, which is expected to launch in early 2025, enjoys the support of eScholarship (University of California), and hugely benefits from the experience of existing community-led journals within the geoscience field, such as Volcanica, Tektonika and Seismica, as well as the help of a pre-launch editorial team composed of a dozen of established volunteer scientists. 

In this contribution, we will provide the vision behind this initiative, report on the structure of this journal, its scope, and the remarkable community effort that will make this new DOAJ a reality.

How to cite: Maffei, S., Arnould, M., Bethkenhagen, M., Duretz, T., Gouiza, M., Hwang, L., and van Zelst, I.: Slinging Earth & (exo)Planets Structure and Dynamics into Diamond Open Access, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16049, https://doi.org/10.5194/egusphere-egu25-16049, 2025.

EGU25-16104 | ECS | Posters on site | EOS4.6

Planetary Research: Advancing Accessibility and Inclusivity through Diamond Open Access Publishing  

Adrien Broquet, Liliane M. L. Burkhard, and Mark A. Wieczorek and the The Planetary Research journal team

The planetary science community is launching a new journal, Planetary Research, as an alternative to traditional publishing models that profit from publicly funded research. This initiative aims to address accessibility and inclusivity challenges in scientific publishing by adopting the diamond open access model, ensuring no fees for authors or readers. Unlike gold, green, and hybrid open access journals, which impose significant financial barriers on authors through article processing charges or hinder the availability of their research outputs via subscriptions, diamond open access relies on minimal operational costs, achieved through free and open-source software for editorial and archival tasks and volunteer contributions.   

Scheduled to launch in January 2026, Planetary Research will be governed transparently by members of the planetary science community, providing opportunities for researchers at all career stages to contribute to its development and operations. An open call for editorial board and steering committee members will be announced at the 2025 Lunar and Planetary Science Conference. The journal will cover the full scope of planetary science, including extrasolar systems, exoplanets, spacecraft and Earth-based observatory data, laboratory studies of extraterrestrial materials, theoretical and numerical modeling, and terrestrial analog research. Original research will be published as long-format articles or short letters. Peer reviews as well as assessments and recommendations by the editorial team will be linked to the published article on the journal website   

By eliminating financial barriers, the journal aims to democratize access and dissemination of scientific knowledge, promote inclusivity, and foster collaboration. To ensure sustainability, Planetary Research will leverage volunteer-driven editorial processes, open-source platforms for managing both the peer review process and journal website, as well as low-cost infrastructure for web hosting and digital object identifiers (DOIs). Geoscience diamond open access journals typically report annual operational costs of approximately USD 1000, demonstrating the feasibility of this model. We are currently assessing funding possibilities to cover these operational costs and ensure the perenniality of the journal. The journal will also prioritize outreach to both the scientific community and the general public with the creation of a volunteer-driven media team, emphasizing the societal value of open access to planetary research as community participation is central to Planetary Research. Everyone is welcome to join our pre-launch discussions that are hosted on an online forum accessible via the pre-launch website (https://planetary-research-journal.online/). This open forum will remain active post-launch, allowing members to engage with the steering committee, editorial board, and media team, in order to adapt and evolve the journal in response to community needs. By embracing the principles of accessibility, inclusivity, and transparency, Planetary Research seeks to set a new standard in scientific publishing, ensuring that the benefits of planetary science are freely available to all. 

How to cite: Broquet, A., Burkhard, L. M. L., and Wieczorek, M. A. and the The Planetary Research journal team: Planetary Research: Advancing Accessibility and Inclusivity through Diamond Open Access Publishing , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-16104, https://doi.org/10.5194/egusphere-egu25-16104, 2025.

EGU25-18390 | ECS | Posters on site | EOS4.6

Toward Long-Term Data Stewardship: Merging The Speleothem Database SISAL into Neotoma, the Palaeoecological “Database of Databases” 

Laura Endres, Nikita Kaushal, Simon Goring, Socorro Dominguez, Franziska Lechleitner, Heather Stoll, and John W. Williams

Over the past few years, SISAL has released several versions of a global speleothem database as a community effort. The latest version, SISALv3, features 800+ records from both hemispheres, multiple proxies (stable isotopes (δ18O,δ13C) and trace elements (Mg/Ca, Sr/Ca, Ba/Ca, U/Ca, P/Ca and Sr isotopes)), and extensive metadata about cave sites and specimens. A major strength of the SISAL database is that it is a high-quality dataset with multiple manual and auto quality control checks performed by members and experts of the speleothem community, becoming de facto the gold standard for speleothem data. In the past few years, the database has been increasingly used in studies improving speleothem proxy understanding, as well as for global analysis of key past climate intervals and global climate patterns.

However, SISAL is organized only as a temporary working group within the Past Global Changes network (PAGES) and is scheduled to wind down after its current phase. This poses an essential question for this community-led effort: how can we place ourselves so that the carefully created database can be maintained and grow beyond the intended life cycle of the original working group?

To increase the visibility and ease of access to this data, accelerate database updates, and enable long-term data stewardship in a community of similar paleo datasets, SISAL has recently decided to join Neotoma as a constituent database, through a data migration that has been supported by the ETH Open Research Data program. Neotoma, a “database of databases” within the palaeoecological and paleoenvironmental sciences, provides a structure for on-going community data stewardship as well as a strong backend for SISAL data through standardisation of data entry, quality-check workflows. The SISAL team plans to maintain the popular SISAL web app for finding and downloading data, currently linked to SISALv3, and in the future plans to update the web app to dynamically link to SISAL-Neotoma holdings. This SISAL-Neotoma partnership also helps connect speleothem isotope data to data from other proxy communities, such as pollen or biomarkers, which can lead to further synergies to be exploited in the future.

How to cite: Endres, L., Kaushal, N., Goring, S., Dominguez, S., Lechleitner, F., Stoll, H., and Williams, J. W.: Toward Long-Term Data Stewardship: Merging The Speleothem Database SISAL into Neotoma, the Palaeoecological “Database of Databases”, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18390, https://doi.org/10.5194/egusphere-egu25-18390, 2025.

EGU25-18663 | ECS | Orals | EOS4.6

Enhancing Open EO Knowledge preservation through the integration of the GEO Knowledge Hub and Zenodo  

Felipe Carlos, Kalamkas Yessimkhanova, Paola de Salvo, and Lionel Menard

Reusable and actionable Earth Observation (EO) Data and Knowledge are crucial for tackling global issues. In recent years, the adoption of Open Science practices in the scientific community has increased the availability of Open EO Data and Open EO Knowledge. This movement created an ecosystem in which existing research outcomes, tools, data, and knowledge are reused as the basis for new research activities and projects. 

The Group on Earth Observation (GEO) is a global effort of countries, civil society organizations, and the private sector to empower users to access and use EO Data and Knowledge as the foundation for policymaking toward a more sustainable and resilient world. Over the past years, as one way to support its goal, GEO has been developing the GEO Infrastructure, a comprehensive set of services supporting the Open Data and Open Knowledge activities within the GEO Community. This infrastructure includes the GEOSS Platform, which provides an easy way to access Open EO Data from multiple sources. It also has the GEO Knowledge Hub (GKH), a digital repository empowering user to share and preserve Open EO Knowledge. 

 The GKH uses the Knowledge Package as its sharing unit, which is an implementation of a Research Compendium that allows users to centralize, preserve, and describe resources used to compose their research. Each resource in a Knowledge Package can have its metadata, files, and Digital Object Identifier (DOI). As the goal of the GKH is to preserve and centralize Open EO Knowledge, creating a Knowledge Package and uploading resources to it is always recommended. However, the resources used to develop research are sometimes spread across multiple platforms. In alignment with the GEO Data Sharing and Data Management Principles, the GKH also handles this case by allowing users to provide as much metadata as possible about resources and links to access it. 

Zenodo, the universal repository on which various research projects and other initiatives are based, is a common source for those remote resources. Therefore, we developed this integration in this work to facilitate the composition of Knowledge Packages using resources in Zenodo.  

This integration allows users to import a Zenodo record, such as a Dataset, as part of their Knowledge Package. Once imported, the record is visible within the package with its own page, presenting the metadata and files from Zenodo. To avoid duplications and optimize storage usage, GKH only imports metadata from Zenodo. The files are listed in GKH as remote content. Also, the Zenodo metadata in GKH is automatically synchronized when new updates are available in Zenodo. 

To test this integration, we partnered with EuroGEO, a European initiative to create a regional GEO community for Europe. We used this integration in various EU-funded projects, creating packages with a mix of content available in GKH and Zenodo. 

In this session, we are going to share our path to this integration, lessons learned, and the impact in the GEO community. 

How to cite: Carlos, F., Yessimkhanova, K., de Salvo, P., and Menard, L.: Enhancing Open EO Knowledge preservation through the integration of the GEO Knowledge Hub and Zenodo , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18663, https://doi.org/10.5194/egusphere-egu25-18663, 2025.

EGU25-18716 | Orals | EOS4.6

Opening up historical atmospheric electricity data with Citizen Science  

Keri Nicoll, Hripsime Mkrtchyan, and R. Giles Harrison

Many paper archives of environmental data have yet to be made available digitally. One example is an extensive series of atmospheric electricity observations made at UK sites during the majority of the twentieth century, which contains almost continuous measurements at hourly resolution. Renewed interest in atmospheric electricity due to its relationship to climate variables and local air pollution has made digitising this archive a priority. Due to the number of handwritten individual observations to be transcribed, a citizen science keying project has been implemented on the Zooniverse platform: see https://rdg.ac/electricity . Through press and news articles, over 500 citizen scientists have now been recruited to contribute to this task. We have also evaluated which of these profile-raising activities have been most effective for drawing volunteers to the project. One advantage of having multiple individuals take part is that ambiguous handwritten entries can be recovered effectively and accurately, through combining the judgements of different transcribers. A further key aspect of engagement has been putting our contributors in touch with how the original data looks, and to some extent “feels”, as it provides an entry point for digital era humans into how past environmental data was recorded, in pen and ink. Since citizen science project are undertaken entirely by volunteers, we also discuss the challenges with maintaining engagement with the community of volunteers, which is essential for the successful completion of data transcribing projects to yield the associated scientific advancement. 

How to cite: Nicoll, K., Mkrtchyan, H., and Harrison, R. G.: Opening up historical atmospheric electricity data with Citizen Science , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18716, https://doi.org/10.5194/egusphere-egu25-18716, 2025.

EGU25-19107 | ECS | Posters on site | EOS4.6

Navigating the Jungle of CMIP Data as a First-Time User: Key Challenges and Future Directions  

Lina Teckentrup, James O. Pope, Feba Francis, Julia K. Green, Stuart Jenkins, Stella Jes Varghese, Sian Kou-Giesbrecht, Christine Leclerc, Gaurav Madan, Kelvin Ng, Abhnil Prasad, Indrani Roy, Serena Schroeter, Susanna Winkelbauer, and Alexander J. Winkler

Output generated by the different phases of the Coupled Model Intercomparison Project (CMIP) has underpinned countless scientific projects and serves as the foundation of the United Nations climate change reports. While initially CMIP was largely driven by the scientific curiosity in the broader climate modeling community, CMIP output has also become a crucial data source for disciplines more tangentially related to physical climate science such as the economic modelling community. The upcoming CMIP phase 7 is expected to produce the largest amount of CMIP-related data to date. However, with an increasing number of modelling systems, represented realms, model complexity, variable names, experiments, and different grid types, the initial exposure to CMIP output has undoubtedly become an overwhelming experience for first-time users. For this presentation, we would like to start a conversation with users who are in or have recent experience of being in the early stages of employing CMIP outputs for their research, and together identify:

  • Key barriers and challenges experienced when first using CMIP data
  • Additional documentation/tools needed to facilitate the use of CMIP data
  • Key pieces of advice for new CMIP users

How to cite: Teckentrup, L., Pope, J. O., Francis, F., Green, J. K., Jenkins, S., Varghese, S. J., Kou-Giesbrecht, S., Leclerc, C., Madan, G., Ng, K., Prasad, A., Roy, I., Schroeter, S., Winkelbauer, S., and Winkler, A. J.: Navigating the Jungle of CMIP Data as a First-Time User: Key Challenges and Future Directions , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19107, https://doi.org/10.5194/egusphere-egu25-19107, 2025.

EGU25-19248 | Orals | EOS4.6

How can climate adaptation platforms engage and learn from each other? 

Rosie Witton and Sukaina Bharwani

In 2022, the European Union (EU) launched the Mission on Adaptation to Climate Change, to foster the climate resilience of regions, cities, citizens, and companies in Europe. The EU funded project, Adaptation AGORA, brings together 13 partners from eight EU countries and the UK to support communities and citizens to accelerate their transformation to a climate resilient future. More specifically, Adaptation AGORA has used a transdisciplinary co-creation approach to facilitate the development of a digital toolbox of innovative mechanisms and transdisciplinary approaches for inclusive climate governance that fosters citizen and community engagement, known as the online climate adaptation platform, the Agora Community Hub, as well as two digital academies focussing on accessing and using climate data and monitoring climate risks, and climate change disinformation. 

However, the proliferation of portals and platforms sharing information online is expanding daily. This does not always result in a coordinated or systematic effort, which means knowledge is often fragmented and siloed leading to redundancy and/or replication. In an era when planning must accelerate to implementation and concerted climate action, we need faster ways to learn lessons from one another on knowledge sharing and exchange. To support knowledge sharing and exchange between climate adaptation platforms, the Adaptation AGORA project has started this webinar series to engage climate adaptation platforms, encourage collaboration between platforms, and increase learning. The webinar series has focused on: EU funded projects and climate adaptation platforms; connecting knowledge to policy and practice; and has an upcoming webinar on monitoring the impact of climate adaptation platforms. 

This EGU session would be interactive, highlighting the AGORA project as well as other climate adaptation platforms available, and then engaging with the audience to discuss enablers and barriers of and how to build alliances with other climate adaptation platforms. The session aims to:  

  • Highlight the AGORA project and its related platforms, focusing on how other climate adaptation platforms can interact with the Agora Community Hub. 
  • Share and exchange information on enablers and barriers to exchanging with climate adaptation platforms. 
  • Explore potential synergies, opportunities and foster collaboration between climate adaptation platforms. 
  • Engage and foster a dialogue between climate adaptation platforms in line with the AGORA project webinar series. 

Anticipated outcomes include the identification and exploration of available climate adaptation platforms, identification of enablers and barriers to engaging with climate adaptation platforms to limit silos, and discussions around future synergies and collaborations between climate adaptation platforms. A summary and findings will be disseminated through an online feature. 

How to cite: Witton, R. and Bharwani, S.: How can climate adaptation platforms engage and learn from each other?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19248, https://doi.org/10.5194/egusphere-egu25-19248, 2025.

EGU25-19351 | Orals | EOS4.6

Transparency in open science outputs -: Ensuring Transparency, Reproducibility, and Credit for All Supporting Research Contributions 

James Ayliffe, Deborah Agarwal, Justin Buck, Joan Damerow, Graham Parton, Shelley Stall, Martina Stockhause, and Lesley Wyborn

An ongoing challenge relevant to most research disciplines is the difficulty in citing 100+ digital objects such as datasets, software, samples, and images. Journals require authors to place citations over some set limit into supplemental information, where individual citations are not properly indexed, not linked to the manuscript, nor tracked accurately. Citing these research products is critical to enable transparent and reproducible research and for researchers, institutions, and project managers to trace citation, get appropriate credit, and report impact to funders. 

 

Open Science practices encourage providing proper attribution for the digital objects that support research findings and outcomes. Journals commonly redirect authors with many digital object citations to move those to the supplemental information where they are not indexed.  This means: 

  • Creators of these digital objects do not get attribution and credit for their contribution to the scholarly literature 
  • Funders cannot measure use, impact and derived value from these digital objects
  • Machine-actionable transparency is not possible. And over time, the supplement has a high probability of not being maintained by the publisher.  

We need to develop a scalable citation implementation strategy to enable open transparent and traceable research, which allows integration into common citation/impact metrics

 

The findings of the Research Data Alliance (RDA) Complex Citations Working Group have produced key requirements (R1 - R10) for Complex Citation Objects (CCOs) to achieve our goals. In summary: 

  • CCOs capture enough detail to ensure proper credit, traceability, and transparency of cited materials (R1), supporting machine-actionable attribution for each referenced object (R2).
  • CCOs do not accrue credit themselves but simply list data and digital identifiers that require citation tracking (R3).
  • CCOs are stable, identifiable, versioned, resolvable, and persistent (R4, R5).
  • CCOs use standardized structures, limited to two PID graph levels, with a strong preference to utilize persistent identifiers (R6, R6.1, R7).
  • CCOs remain open, accessible, and flexible for various use cases, with an open license, and sufficient metadata (R8-R10).

 

The full recommendations were published ahead of a presentation at the last RDA plenary session (Agarwal et al. 2024). The recommendations were based on use cases that identified the roles and responsibilities of the Complex Citation Workflow Actors necessary for the Complex Citation Objects (CCOs) to be used in practice.

 

The Complex Citations Working Group is moving to a new phase where the recommendations need to be tested, evaluated and proven. To this end we are keen to inspire collaboration through new use cases, pilot implementations, to include repositories, journals, indexers and researchers to develop a new project and entrain more communities to take this work forward.

 

Reference: 

Agarwal, D., Ayliffe, J., J. H. Buck, J., Damerow, J., Parton, G., Stall, S., Stockhause, M., & Wyborn, L. (2024). Complex Citation Working Group Recommendation (Version 1). Zenodo. https://doi.org/10.5281/zenodo.14106603

How to cite: Ayliffe, J., Agarwal, D., Buck, J., Damerow, J., Parton, G., Stall, S., Stockhause, M., and Wyborn, L.: Transparency in open science outputs -: Ensuring Transparency, Reproducibility, and Credit for All Supporting Research Contributions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19351, https://doi.org/10.5194/egusphere-egu25-19351, 2025.

EGU25-19987 | Posters on site | EOS4.6

Tektonika: breaking barriers in scientific publishing one manuscript at a time 

Lucia Perez-Diaz, Kim Welford, and Moh Gouiza and the the Tektonika Executive Editor team

Science, without effective dissemination, has a very short life and little impact. Yet, most scientific research is hidden away behind exclusive and expensive paywalls imposed by traditional publishers. Tektonika is an Earth Science community-led diamond open-access journal (DOAJ: free for authors, free for readers) publishing peer reviewed research in tectonics and structural geology. It is a grass-roots initiative driven by the enthusiasm and devotion of a wide and diverse spectrum of Earth Scientists from around the globe, intended to help shape a new landscape for publishing in the geosciences. 

Since its debut at EGU2022, Tektonika has experienced steady growth, fueled by a consistent stream of manuscript submissions.  Tektonika’s success reflects broader trends among community-driven DOAJs, demonstrating their ability not only to survive but to flourish. The strong support of the Earth Science community has been instrumental—from authors entrusting their work to the journal, to individuals amplifying its reach via social media, and volunteers contributing to editorial tasks, peer review, and the formatting of accepted articles. Tektonika stands as a testament to the power of collective effort in transforming scientific publishing.

How to cite: Perez-Diaz, L., Welford, K., and Gouiza, M. and the the Tektonika Executive Editor team: Tektonika: breaking barriers in scientific publishing one manuscript at a time, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19987, https://doi.org/10.5194/egusphere-egu25-19987, 2025.

EGU25-20355 | ECS | Posters on site | EOS4.6

A database for igneous rocks of the Newfoundland Appalachians 

Chaoyang Wang, Tao Wang, and Yi Ding

Databases are playing an increasingly pivotal role in the field of Earth Sciences. We present a comprehensive database of igneous rocks from the Newfoundland Appalachians (https://dde.igeodata.org/subject/detail.html?id=67). The database consists of a set of 15,110 high-quality data. Each dataset includes detailed information on geographic location (latitudes and longitudes), geological background, petrology, geochronology, major and trace elements, isotopes, and references. The data were collected from published papers, publicly available databases, geological survey reports, and academic dissertations. The database offers several advantages: (1) A systematic and complementary data model aligned with the knowledge systems of igneous rock. (2) A broad range of high-quality data collected over 50 years, and derived from diverse sources; (3) A platform for efficient searchability and usability. This database will help achieve a wide range of scientific research objectives related to igneous rocks in the Newfoundland Appalachians and the tectonic evolution of the Newfoundland island.

How to cite: Wang, C., Wang, T., and Ding, Y.: A database for igneous rocks of the Newfoundland Appalachians, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20355, https://doi.org/10.5194/egusphere-egu25-20355, 2025.

The Earth, space, and environmental sciences community, through a grant from the Belmont Forum, has developed a suite of open science materials to get you and your teams started on your Open Science Journey.  The development team includes members from Australia, Brazil, France, Japan, and the United States, coordinated by the AGU. This talk will share the materials and a bit of the background. Included are topics such as your Digital Presence, Data Documentation and Citation, Software Documentation and Citation, materials for working openly as a team, and how to integrate data and software management into your research lifecycle.  

How to cite: Stall, S. and Specht, A.: Your Open Science Journey:  Earth, space, and environmental science educational materials supporting researchers and their teams., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20599, https://doi.org/10.5194/egusphere-egu25-20599, 2025.

EGU25-2164 | ECS | PICO | EOS1.6

Communicating uncertainty in extreme event attribution to the media 

Johanna Knauf, Theresa Zimmermann, Jonas Schröter, Miriam Tivig, and Frank Kreienkamp

This work examines the extent and form in which uncertainty of Extreme Event Attribution (EEA) results is best communicated to stakeholders. To achieve this, we develop communication materials in both text and graphics and test them for accuracy and accessibility through guided interviews with scientists and stakeholders.

Extreme weather events pose significant challenges for human civilization. Climate change can influence both the intensity and probability of specific extreme weather events, such as heatwaves or heavy rainfall. EEA has become an established tool to answer public questions about the contribution of climate change to such events. However, the results of EEA studies are often accompanied by considerable uncertainties. Communication of results, including an accessible representation of uncertainty, is therefore a fundamental necessity in this field of research, extending beyond the general effort to make scientific findings accessible to the public. Media representatives, who often bridge the gap between attribution scientists and the public, are therefore key stakeholders in this research.

We present the current state of research on communicating uncertainties in this field and outline our iterative approach to working with attribution scientists and media representatives alike to determine what should be communicated and how to communicate it effectively. Finally, we evaluate which communication materials are both relevant and accessible, and we reflect on the lessons learned for future communication efforts concerning EEA results.

This study is part of ClimXchange, which aims to enhance the usability of climate science for societal stakeholders. ClimXchange is embedded within the ClimXtreme research consortium, funded by the German Federal Ministry of Education and Research (BMBF), which focuses on extreme weather events in the context of climate change.

How to cite: Knauf, J., Zimmermann, T., Schröter, J., Tivig, M., and Kreienkamp, F.: Communicating uncertainty in extreme event attribution to the media, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-2164, https://doi.org/10.5194/egusphere-egu25-2164, 2025.

EGU25-4471 | PICO | EOS1.6

Communicating uncertainty in weather forecasts: the role of forecast changes 

Gabriele Messori, Stephen Jewson, and Sebastian Scher

Skilful weather forecasts help users make sound decisions when faced with potentially hazardous climatic conditions. However, this beneficial result may be reduced or negated in the absence of an effective communication of forecast uncertainty. On average, forecast skill improves for shorter lead times, which implies that we expect differences between successive forecasts. While there is a vast literature on the communication and visualisation of weather forecast uncertainty, little attention has been dedicated to communicating forecast changes to non-specialist audiences. Nonetheless, this is a key dimension of forecast uncertainty, and there are several user cases in which providing information about possible future changes in weather forecasts can improve their use.

An illustrative example is the situation in which a user has to decide whether to act now or wait for the next forecast. This can be as simple as a professional deciding whether to drive or not to a client on a day for which extremely heavy rainfall is forecasted, potentially leading to flash flooding. Cancelling well-ahead of time makes rescheduling easier, yet the forecast has a larger chance of being wrong. Cancelling on short notice minimises the chance of a false alarm, but poses greater logistical challenges for both the professional and the client. Something as simple as knowing how often the later forecast is better – for example knowing that 9 times out of 10 a heavy rainfall forecast issued one day ahead is better than one issued 5 days ahead – can qualitatively help the non-specialist users in this fictitious example to make a more informed decision.

In this contribution, we consider a variety of cases in which information on forecast changes may be of value. We then present a set of easily interpretable metrics making information on such changes accessible to non-specialist users.

How to cite: Messori, G., Jewson, S., and Scher, S.: Communicating uncertainty in weather forecasts: the role of forecast changes, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-4471, https://doi.org/10.5194/egusphere-egu25-4471, 2025.

Whether its memories of a cold, frosty Christmas or an August bank holiday beach trip interrupted by rain, many cultural, sporting, and social events in the United Kingdom have strong associations with particular weather conditions. As the average global temperature increases, the impacts of a changing climate are likely to be felt across many aspects of British life, including in the public’s experiences of these popular events. Several recent works conducted by the UK Met Office have sought to make the local day-to-day impacts of climate change more understandable for the public by exploring likely climatic conditions of popular events by the 2050s. These works have received strong engagement from the public, demonstrating the demand for relevant and understandable climate information.

We serve this demand by using the 2018 UK Climate Projections (UKCP18) and HadUK-Grid observations data to evaluate how climate change will affect the climatology of a diverse range of British social, cultural, and sporting events. To explore and communicate the uncertainties in UKCP18 due to inherent model biases, several bias correction methods are applied to the data and the resulting data is analysed together to give an improved uncertainty range. The research will focus on assessing changes to temperature variables at global warming levels of 1.5°C and 3.0°C to illustrate these two future scenarios and the uncertainty within each scenario.

We will show that some events are likely to have a significantly altered climatology which is likely to substantially change the nature of these events or force them to change when they occur during the year to give the best chance of having favourable climatic conditions. By assessing the impact of climate change on popular British events such as the London Marathon and Glastonbury Festival the findings of this research will prove useful in communicating the impacts of climate change in a way which will resonate with the British public.

How to cite: Woods, L., Pope, J., and Fung, F.: Impacting on our Lives: Using British sports and culture to explain uncertainty in climate projections, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9081, https://doi.org/10.5194/egusphere-egu25-9081, 2025.

Flood frequency analysis is a cornerstone of hydrologic studies, providing a probabilistic framework to relate the magnitude of extreme events to their frequency of occurrence. This methodology is critical for designing flood-related infrastructure, conducting economic evaluations of flood control projects, and delineating floodplains. However, its utility depends heavily on data quality, model selection, and parameter estimation, each of which introduces uncertainties that become especially significant for rare events.

This presentation will address key sources of uncertainty, including model choice, parameter inference methods, and sample size limitations. Strategies for incorporating these uncertainties into engineering practice are discussed, with an emphasis on probabilistic representations and innovative design approaches. An exceptional flood, a "black swan" event, is used to illustrate the paradox of increased uncertainty despite improved information. This case underscores the importance of expanding flood analyses through historical records, regionalization, and causal modeling, particularly in the context of a changing climate.

The presentation will be designed to foster cross-discipline exchange in the quantification of uncertainty in Earth Sciences.

How to cite: Viglione, A.: Flood Frequency Hydrology: Navigating Uncertainty in Flood Design, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11466, https://doi.org/10.5194/egusphere-egu25-11466, 2025.

EGU25-13135 | PICO | EOS1.6

Visualization of uncertainties in 2D images 

Peter Dietrich, Husain Najafi, Michael Pelzer, and Solmaz Mohadjer

Two-dimensional (2D) images are often used to communicate the results of scientific investigations and predictions. Examples are weather maps, earthquake hazard maps and MRI slices. In contrast to statistical analyses of individual variables or time series, there are currently no established methods for visualizing the uncertainties in the 2D images. However, this would be necessary to make the information in the 2D images clear to scientists as well as to the non-expert public audiences in order to avoid misinterpretation and over-interpretation.

In this study, we demonstrate the challenges and approaches to uncertainty visualization using the case study of drought forecasting, which is relevant for climate adaptations and mitigations. A drought is a deviation (anomaly) from the parameter value expected from long-term data. In our case, the parameter under consideration is soil moisture, which is an important parameter for various environmental processes. The soil moisture can be used in combination with soil type to estimate the amount of water available to plants in the topsoil. If the amount of water available to plants according to the so-called percentile approach deviates significantly from the value expected from long-term data, this is referred to as an agricultural drought.

The drought forecast is based on ensemble modelling. This means that the results of various weather forecast models are used to predict the development of soil moisture for the period of the weather forecast. For each weather model used, a possible soil moisture development is predicted. Each of these is used for a drought forecast. The result of the ensemble modelling is therefore several forecasts, which can differ significantly. Due to the use of different weather models and the consideration of uncertainties in the models, the result of ensemble modelling is therefore a large number of drought forecast maps. When visualising the results, often only a map of the mean values resulting from the predictions is shown. If only the mean value is displayed, however, the information about a possible difference and thus the uncertainty of the predictions is lost. In other words: If individual cases from the ensemble predict the possibility of drought, this will not be clearly visible in the mean value map.

In this presentation, we will demonstrate and discuss different approaches to visualize the uncertainty in the prediction.

How to cite: Dietrich, P., Najafi, H., Pelzer, M., and Mohadjer, S.: Visualization of uncertainties in 2D images, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13135, https://doi.org/10.5194/egusphere-egu25-13135, 2025.

EGU25-13260 | PICO | EOS1.6

Non-expert understanding of hazard maps: Insights from an online survey 

Peter Dietrich, Michelle Dietrich, Michael Pelzer, and Solmaz Mohadjer

Uncertainties are an unavoidable part of scientific research. Practical limits with regard to the number, accuracy and precision of available observations as well as limitations in terms of methodological accuracy and modelling contribute to the fact that even the most elaborate and meticulous forecasts can never be deterministic and no completely reliable and accurate predictions for decision-making can be achieved. In concrete applications, a sufficient understanding of the accuracy and reliability of scientifically based predictions is important, for example in disaster prevention or resource planning. For example, natural hazard maps are primarily intended for those who have the necessary expertise to understand them. However, they are also used in their unaltered form by non-experts for decision-making, many of whom are unfamiliar with the scientific background and implications of the map.

We address this problem using an earthquake hazard map which can be relevant to non-expert audiences when seeking advice on purchasing a house or obtaining insurance. In order to understand how non-experts perceive a scientifically compiled earthquake hazard map, we conducted an online survey with 229 participants. This was done as part of the 2024 Science & Innovation Days (a public engagement event) in Tübingen, Germany. Participants were asked about their first impression of the map in terms of information content, any need for further explanation and possible actions to take. Other questions assessed participants’ previous experiences and self-assessment of hazard perceptions.

In this presentation, we will discuss the survey results and share lessons learned when communicating information that contains uncertainty with non-expert audiences.

How to cite: Dietrich, P., Dietrich, M., Pelzer, M., and Mohadjer, S.: Non-expert understanding of hazard maps: Insights from an online survey, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13260, https://doi.org/10.5194/egusphere-egu25-13260, 2025.

Working with environmental data means dealing with complex processes, limited data (in space and/or time) and the impossibility of setting up controlled experiments, leading to uncertain predictions of system behaviour.

In the field of statistical hydrology, many efforts have been made during the last decades to provide methods to quantify uncertainty, but the common practice of infrastructure design has not yet incorporated them. This may be due to several reasons, including the complexity of the methods, which are often difficult to apply in most everyday cases, and regulations that "favour" well-established requirements.

Here we present the "uncertainty compliant design flood estimator" (UNCODE) method, which accounts for aleatory uncertainty in the estimation of the design flood value. The method provides a corrected design value and is easy to use for practical purposes as simplified formulae are provided to quantify the correction factor. However, in addition to its practical application, it can also be used to compare different models with different levels of uncertainty and to highlight the "cost" of uncertainty.

Finally, its mathematical formulation allows a direct link to be made between the classical approach to hydrological design, based on a fixed hazard level (or return period), and a risk-based design approach, which is widely recognised as a more flexible method but is not usually included in regulations.

How to cite: Ganora, D.: Uncertainty in flood frequency analysis and its implications for infrastructure design, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-15189, https://doi.org/10.5194/egusphere-egu25-15189, 2025.

EGU25-17779 | ECS | PICO | EOS1.6

Non-Expert Understanding of Hazard Maps: An Eye-Tracking Study  

Solmaz Mohadjer, Gökce Ergün, Sebastian G. Mutz, Max Schneider, Tom Schürmann, Michael Pelzer, and Peter Dietrich

Maps are the most commonly used means of visualizing and communicating natural hazard information to support decisions about risk mitigation. They are a product of hazard assessment studies which involve different input parameters with uncertainties relevant to decision making. This process is further complicated by the subjective uncertainties that arise in the audience when confronted with the visualization of hazard information. 

Natural hazard maps are primarily designed to be used by experts, but they are also used in their unaltered form to communicate with non-experts, many of whom are unfamiliar with the map’s scientific background and implications. Previous studies focus mainly on evaluating such maps with expert groups (e.g., directly involved stakeholders and authorities), with less attention on non-experts (e.g., the public audiences) who are confronted with these maps before purchasing a house, getting insurance or making other critical decisions. 

To address this gap, our study investigates how well hazard maps are understood and interpreted by non-expert audiences. We tested two earthquake hazard maps of Germany that differ in color palettes (rainbow vs. colorblind-friendly and perception-optimized yellow-orange-red-brown color palettes) and data classification schemes (algorithmic Fisher vs. quasi-logarithmic classification schemes). We showed both maps to 20 non-expert participants during the 2024 Science & Innovation Days (a public engagement event) in Tübingen, Germany. Participants answered map-reading and hazard perception questions (e.g., participants were asked to read off the hazard level for a given city, and to compare hazard levels between for a pair of cities) while their eye movements were monitored with eye-tracking software. 

To identify if either map improved map reading and hazard perception, participants’ responses were scored, analyzed and compared using a two-sample Mann–Whitney U and Fisher’s Exact tests. In general, the differences detected in participants’ responses were not statistically significant, perhaps due to the small sample size. Still, we observed that nearly all participants who used the redesigned map (8 out of 9) correctly read the hazard level for a city while only 33% (3 out of 9 participants) who used the rainbow color map responded correctly.

Eye-tracking data were used to analyze focus-metrics. Composite heatmaps accumulating the duration of eye fixations of all participants indicate that their eye movements were focused more on the high hazard zones and the corresponding values shown on map legend when answering questions using a hazard map redesigned to use best practices for hazard perception.

To quantify these differences, the ratio of fixations on high-hazard zones to total fixations on the map were calculated for both map versions. The data were tested for normality and the statistical significance of the differences were evaluated using Independent Samples t-tests for equal variances. While the results were not statistically significant, participants viewing the redesigned map showed a greater number of fixations on high-hazard zones compared to the participants viewing the original map, with a moderate effect size. We note tendencies in the data that encourage the repetition of the experiment with a larger sample size.

How to cite: Mohadjer, S., Ergün, G., Mutz, S. G., Schneider, M., Schürmann, T., Pelzer, M., and Dietrich, P.: Non-Expert Understanding of Hazard Maps: An Eye-Tracking Study , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-17779, https://doi.org/10.5194/egusphere-egu25-17779, 2025.

A presentation of emerging themes and lessons learnt from examples of best practice in uncertainty quantification and communication relevant to climate services.  Drawn from existing literature and reports, and from a community engagement workshop.

  • Consider the climate risks that are of most concern to the audience. 
  • Use language the audience is familiar with (don’t say uncertainty).
  • The precision of uncertainty information should be relevant to the situation.
  • Understand existing narratives about climate uncertainty.
  • Use communication about uncertainty to build trust.
  • Be aware of deep uncertainty.

Standardised approaches to uncertainty communication should consider not only the climate science component, but also the complexities regarding socio-economic vulnerability.

Climateurope2, is a Horizon Europe project with a consortium of 33 parties from 13 countries that includes intergovernmental institutions such as the World Meteorological Organisation, social sciences, humanities and STEM expertise, assurance providers, SMEs, and standardisation bodies. Together we are building a community of practice for the standardisation and support of climate services.

How to cite: Pascoe, C., Dankers, R., Domingo, X., and Pagé, C.: Don't say uncertainty: preliminary best practices and emerging themes for uncertainty quantification and communication in climate services from the Climateurope2 project., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18364, https://doi.org/10.5194/egusphere-egu25-18364, 2025.

The recent COVID-19 pandemic highlighted the need to effectively communicate forecasts and their uncertainty. This is especially important if the aim is to minimize the risk of misinformation and poorly-informed decision-making. Both the IPCC and the Sendai Framework for Disaster Risk Reduction have identified risk communication, complexity and uncertainty as major challenges to decision-making, and call for better understanding of how existing risk communication practices are perceived by those affected and those making decisions.

Despite these calls, many geoscientists, especially early career researchers, lack opportunities to discuss scientific uncertainty and explore ways to communicate uncertainty to different audiences, including the non-scientific publics. To address this demand, we organize the international training school “Understanding the Unknowns: Communicating Uncertainty as a Driving Force for Geosciences”, which is co-sponsored by the EGU and set to take place at the University of Tübingen in Germany from March 17 to 19, 2025. This in-person, three-day training school aims to equip Early Career Researchers with knowledge and skills needed to effectively account for and communicate uncertainty in geosciences with their peers as well as public audiences.

Some of the biggest challenges of training programs on uncertainty relate to the interdisciplinary nature of the concept: understanding and effectively communicating uncertainties requires knowledge and skill sets typically taught and researched across a range of diverse fields. Highlighting this interdisciplinary background, we combine insights from geoscientific uncertainty assessment and outputs (e.g., maps, interpretations, models, simulations, time series) with approaches from (visual) rhetoric, science communication, presentation research, and multimedia competence. 

Building on existing good practice, the training strives to equip geoscientists with the tools and skills they need to communicate uncertainty, help reduce misinformation, and enhance future decision-making. This will be done collaboratively through an interdisciplinary partnership between the Department of Geosciences, the Research Center for Science Communication at the Department of General Rhetoric, and Global Awareness Education at the University of Tübingen. The new approaches and exercises developed for this training will not only be practically applied in the training school, but also reflected and evaluated, including a pre-workshop survey addressing expectations and needs identified by the participants and a concluding qualitative evaluation.

In this presentation, we will discuss our multifaceted practices and strategies applied to foster skills in communicating uncertainty in geosciences, present the results of the accompanying survey and evaluation used in this training, and conclude with lessons learned and best practices recommended to further develop similar opportunities in the future.

How to cite: Pelzer, M., Dietrich, P., and Mohadjer, S.: Fostering Skills in Communicating Uncertainty in the Geosciences: a review of concepts, strategies and approaches applied in the training school “Understanding the Unknowns: Communicating Uncertainty as a Driving Force for Geosciences”, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18655, https://doi.org/10.5194/egusphere-egu25-18655, 2025.

Sub-seasonal weather forecasting is notoriously difficult, particularly for the extra-tropics. Predictions must be probabilistic, and from weeks 3 or 4 onwards forecast distributions are often very close to model-climate distributions. Together, these facts make conveying a meaningful forecast to customers extremely difficult, and those forecasts are then very vulnerable to misinterpretation. Standard map-based graphical output can show little more than whether the forecast mean is for average, or above average or below average conditions – ostensibly a 3-category classification. And indeed “average” in this scheme can be interpreted variously as a genuine forecast of average, or a “no-signal” prediction, which cannot both be right.

So ECMWF is working towards a new two-layer brand of map-based sub-seasonal forecast products, that succinctly represent both the mean anomaly and the forecast uncertainty. We plan to call these “quantile-based weekly guidance maps”. The overarching aim has been to exploit much better than hitherto the information content of the sub-seasonal forecast system in a compact format. Once these first go public they will be classed as an “experimental product”. We hope for wide-ranging uptake, providing greater outreach for our forecasts than hitherto, to benefit multiple sectors of society.

The new graphical output can be summarised in a 3-by-3 matrix form where one dimension represents the mean anomaly and the other relative spread. So for example a mean anomaly around zero can either represent a high confidence, narrow distribution forecast of average conditions (a true forecast of “average”), or more commonly a no-signal forecast where forecast and climate distributions are much the same (= “we don’t know”), or less often an odd scenario in which forecast spread exceeds climate spread (= “very uncertain indeed”). The graphical versions of the new system, and the 9 classes, will be demonstrated using real ECMWF forecast examples. These will highlight how translating appropriately chosen mathematical metrics into suitable graphics, and on into plain language text, can lie at the heart of successful uncertainty communication. Clear documentation for users is another key requirement.

How to cite: Hewson, T.: Making Uncertainty in Sub-seasonal Weather Forecasts Intelligible, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-19375, https://doi.org/10.5194/egusphere-egu25-19375, 2025.

EGU25-21809 | ECS | PICO | EOS1.6

Immersed in Uncertainty: Discussing Uncertainty in Science in a Planetarium 

Jakub Stepanovic, Sandy Claes, and Jan Sermeus
Uncertainty is an inherent part of the nature of science (NoS), and its communication is essential to maintain scientific transparency and credibility. Yet, current teaching on the topic is insufficient, leaving many with naïve views of NoS. Following calls to integrate uncertainty as a core component of science education and support NoS instruction with real-world examples, we designed an interactive learning experience conveying uncertainties in planetary science stemming from missing data and using artificial intelligence for a planetarium lecture. We were particularly interested in how interaction in the immersive planetarium settings impacts the audience's engagement with the lecture and, thus, uncertainty in science. The experience was presented to adolescents and adults attending the planetarium, and we collected feedback from 343 participants. Here, we share insights from the development, discuss interactive methods that significantly improved the audience's engagement, and share the participants' perspectives on uncertainty in science. We conclude by examining the pillars of NoS to clarify and define the presence of uncertainty and provide considerations for science communicators and educators. 

How to cite: Stepanovic, J., Claes, S., and Sermeus, J.: Immersed in Uncertainty: Discussing Uncertainty in Science in a Planetarium, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-21809, https://doi.org/10.5194/egusphere-egu25-21809, 2025.

EGU25-1469 | Orals | EOS3.1

Cata de Ciencia: Bridging the Gender Gap in STEM Through Community Engagement and Visibility 

Carme Huguet and Soraya Polanco Palomar

Cata de Ciencia: Bridging the Gender Gap in STEM Through Community Engagement and Visibility

The persistent gender gap in Science, Technology, Engineering, and Mathematics (STEM) has hindered diversity and innovation for decades. Women and girls are consistently underrepresented in these fields, limiting their career trajectories and obstructing the development of inclusive, diverse solutions for global challenges. Increasing the visibility of female role models has been identified as a critical strategy to address this disparity (e.g. Carter et al., 2018; Halili & Martin, 2019). However, studies show that women in STEM are often more vulnerable to stereotypes and biases, particularly when presenting their work in public forums (e.g. Carter et al., 2018; McKinnon & O’Connell, 2020). Cata de Ciencia aims to foster a supportive environment to promote women in STEM by showcasing their achievements and engaging a diverse local audience. This initiative combines public science communication with gender equity goals. Monthly events held in Segovia, Spain, feature presentations by local women scientists, followed by interactive discussions with the audience in an informal setting accompanied by wine and tapas. The format promotes accessibility, relatability, and inclusivity, addressing the stereotype that scientific excellence is exclusive to men or specific cultures (Carter et al., 2018; McKinnon & O’Connell, 2020). The project pursues two main objectives: increasing the visibility of women in STEM within the region of Castilla y León and promoting the dissemination of science to the public in a welcoming, interactive format. 

References
Carter, A. J., Croft, A., Lukas, D., & Sandstrom, G. M. (2018). Women’s visibility in academic seminars: Women ask fewer questions than men. PloS one, 13(9), e0202743.
Halili, M. A., & Martin, J. L. (2019). How to Make the Invisible Women of STEM Visible. Australian Journal of Chemistry, 73(3), 75-77.
McKinnon, M., & O’Connell, C. (2020). Perceptions of stereotypes applied to women who publicly communicate their STEM work. Humanities and Social Sciences Communications, 7(1).

How to cite: Huguet, C. and Polanco Palomar, S.: Cata de Ciencia: Bridging the Gender Gap in STEM Through Community Engagement and Visibility, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-1469, https://doi.org/10.5194/egusphere-egu25-1469, 2025.

EGU25-5760 | Posters on site | EOS3.1

The evolving diversity of the geodynamics community: Ada Lovelace workshop participants from 1987 to 2024 

Juliane Dannberg, Iris van Zelst, Anne Glerum, Adina Pusok, Fabio Crameri, and Cedric Thieulot

STEM fields in Europe and across the globe are not balanced in terms of gender, ethnic and racial groups, sexual orientation and other aspects of diversity (e.g. Fry et al. 2021, Freeman 2018). For example, in 2018, women made up over 40% of European academic staff, but in 2019 only 26.2% of full professors were women, less than 25% were heads of institutes, and only 31.1% board members (EC She figures 2021). This under-representation has caused academic institutions to implement new hiring practices, unconscious bias training, and intervention programs (e.g. Palid et al. 2023), as science and innovation thrive on diversity in expertise and experience. However, diversity varies across fields, and understanding field specific data is critical to propose and evaluate effective measures. Here, we wish to look inward and assess our own scientific discipline of computational geodynamics. We specifically use a recurring international conference in our fieldnow called the Ada Lovelace Workshop on Modelling Mantle and Lithosphere Dynamicsas a proxy for our field. This conference series has taken place in various European countries at a roughly two-year interval since 1987. 

For all listed attendees, we have collected gender, year of highest degree obtained, primary country and institute of affiliation at the time of the conference, presentation type and organisational role in the conference based on information available online, such as the workshop program booklets and institute, ORCID, Google Scholar and social media profiles. Using this dataset, we analysed the diversity in gender, career stage and country of affiliation of each conference overall, of the local and science organization committees and of the invited speakers. Based on the available data, we cannot make any inferences about other aspects of diversity. 

We show that over the last 38 years, the participation of women has increased from about 10% to about 35%. The percentage of women attendees has increased across all career stages, but fluctuates for established scientists. The number of invited woman speakers has also increased: whereas between 2000 and 2010, three out of the five conferences did not have any woman invitee, from 2015 to 2024, consistently more than 25% of the invited speakers were women. The number of primary countries of affiliation has approximately doubled over three decades. As expected, the majority of attendees work in Europe and a substantial fraction of participants is from North America, but contributions from scientists in Asia and Africa have increased. Given the rate over the last four decades, we project that gender equality in participants will be reached in 2040.

 

European Commission RTD, She figures 2021Gender in research and innovation: Statistics and indicators, 2021, https://data.europa.eu/doi/10.2777/06090.

Freeman, J. (2018). LGBTQ scientists are still left out. Nature 559, 27-28.

Fry, R., Kennedy, B., & Funk, C. (2021). STEM jobs see uneven progress in increasing gender, racial and ethnic diversity. Pew Research Center1.

Palid, O., Cashdollar, S., Deangelo, S., Chu, C., & Bates, M. (2023). Inclusion in practice: A systematic review of diversity-focused STEM programming in the United States. Int. J. STEM Educ., 10(1), 2.

How to cite: Dannberg, J., van Zelst, I., Glerum, A., Pusok, A., Crameri, F., and Thieulot, C.: The evolving diversity of the geodynamics community: Ada Lovelace workshop participants from 1987 to 2024, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-5760, https://doi.org/10.5194/egusphere-egu25-5760, 2025.

EGU25-6072 | Orals | EOS3.1

Autistic Voices in Geoscience: Lessons to enhance inclusive practice 

Adam Jeffery, Steven Rogers, Kelly Jeffery, Mark Lucherini, Julie Hulme, Martin Griffin, Elizabeth Derbyshire, Kristopher Wisniewski, Jamie Pringle, Catherine Hallam, Isobel Stemp, Lisa Lau, and Liam Bullock

Autism is a lifelong developmental condition which impacts how individuals communicate and interact with the world around them and is simultaneously recognised broadly as a form of neurodivergence and protected legally as a disability (e.g. U.K. Equality Act 2010). Autism frequently remains under-represented and un-disclosed in academia, despite it having no impact on intelligence. In fact, many autistic traits such as problem-solving skills and thinking ‘outside the box’ should be conducive to success in academia.

The field of Geoscience is currently facing significant scrutiny for a lack of diversity. This study contributes to this by investigating the experiences of geoscience students in U.K. higher education, using a novel qualitative methodology designed to be inclusive for autistic participants. Forty self-identified autistic geoscience students took part in semi-structured asynchronous discussions over a period of one month, sharing their self-perceptions, experiences of learning in geoscience, university life, support in higher education, and other issues that they wished to discuss.

Data were analysed using reflexive thematic analysis, generating three themes: (1) Being me; (2) Interacting with the world around me; (3) Facilitating change. Participants stressed the need to recognise the diversity of autistic experiences, and suggested a number of recommendations that would improve their learning and wider higher education experiences, including training to enhance the fundamental understanding of autistic people. The outcomes of this study can help provide actionable recommendations for educators and institutions to better address the challenges faced by autistic learners. This will ultimately facilitate better inclusivity in geoscience-based higher education and lead to improved success and well-being for autistic people in the geosciences.

How to cite: Jeffery, A., Rogers, S., Jeffery, K., Lucherini, M., Hulme, J., Griffin, M., Derbyshire, E., Wisniewski, K., Pringle, J., Hallam, C., Stemp, I., Lau, L., and Bullock, L.: Autistic Voices in Geoscience: Lessons to enhance inclusive practice, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6072, https://doi.org/10.5194/egusphere-egu25-6072, 2025.

No geoscientist is an island. It is not good practice for a geoscientist to act in isolation; rather, geoscientists need to be part of a welcoming community to thrive.  How a professional geoscientist interacts with other geoscientists, non-geoscientists and society is essential for building a culture and environment of conscious inclusion by celebrating the diversity of one and all.  This means proactively creating environments where geoscientists and others can collaborate and feel comfortable communicating openly. Recognizing and understanding how unconscious bias and privileges can create divisions and foster negative professional (toxic) environments.  The presentation will look beyond professional bodies’ codes of conduct, and it will introduce what Equity, Diversity, and Inclusion and Accessibility (EDIA) means. These concepts are vital to consider from the attraction, retention, and progression of professional geoscientists and the reputation of the communities we represent. Several self-awareness exercises will also be shared to explore potential, implicit bias.

 

How to cite: Griffin, M.: Embedding Equity, Diversity, Inclusion and Accessibility (EDIA) within a Professional Geoscientist’s Lifestyle, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6886, https://doi.org/10.5194/egusphere-egu25-6886, 2025.

EGU25-6932 | Posters on site | EOS3.1

Status and Progress of Equality, Diversity and Inclusivity at EGU General Assemblies 

Johanna Stadmark, Alberto Montanari, and Lisa Wingate

The EGU recognises the importance of equality, diversity, and inclusion as a crucial foundation for scientific research. The increasing diversity of our membership in all its facets fosters collaborative research and discovery that benefits humanity and our planet and contributes to reaching the goal of addressing global challenges.

The EGU EDI Committee, since its foundation in 2021, is actively promoting diversity in the EGU initiatives and community. The aim of the EDI Committee is to promote equality, diversity and inclusivity with a broad vision and a global approach, by working with sister associations.

The EDI Committee tasks currently include: (1) Promoting the EGU vision of EDI via an integrated, co-ordinated and constructive approach; (2) 
Raising awareness of the value of EDI within the scientific community; (3) Organising sessions and meetings dedicated to EDI issues as part of the EGU General Assembly, and at other conferences and meetings organised by EGU and its sibling societies; (4) Representing EGU on relevant initiatives focusing on EDI in the geosciences; (5) Providing constructive suggestions and ideas to the EGU Council to promote EDI within the organisation, and the geosciences in general.

The most recent achievements of EDI@EGU are the Champion(s) for Equality, Diversity and Inclusion Award that is bestowed to recognize excellent contributions to put into exemplary practice the principles of EDI. Furthermore, a new travel support scheme to promote diversity at the EGU General assemblies, is first activated in 2025.

The above actions resulted in a more diverse attendance at EGU General Assemblies along the years. The total number of presenters has increased over the time period 2015-2024, and this increase was observed throughout all career stages. The proportion of women presenters has increased from 2015 to 2024.

In the hybrid meeting in 2024 approximately 90% of the participants attended in Vienna. A slightly higher proportion of the oldest (>75 years) and youngest (18-25 years) participants attended online. While there were no differences in how women and men participated (online or physically), there are differences connected to the country affiliations. The great majority of participants from countries in most of western Europe, Asia and North America attended in Vienna, while more participants from other continents attended online.

We aim to analyse the changes in demographics with regards to gender, career stage as well as to geographical distribution of the presenters and participants also in coming years to better understand the potential impacts of meetings organized online or physically, or as a combination of both these modes.

How to cite: Stadmark, J., Montanari, A., and Wingate, L.: Status and Progress of Equality, Diversity and Inclusivity at EGU General Assemblies, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6932, https://doi.org/10.5194/egusphere-egu25-6932, 2025.

EGU25-6963 | ECS | Posters on site | EOS3.1

A new hybrid video & seminar series: Season 3 of Science Sisters is on its way!  

Marina Cano Amoros and Iris van Zelst

Science Sisters is a YouTube video and seminar series hosted by Dr. Iris van Zelst. Lighthearted in tone, it explores different career paths, academic life, and science communication in the planetary and geosciences. The guests on the show represent a range of role models to celebrate the diversity of people working in STEM. They are interviewed by Iris on their personal experiences on different topics. Past seasons have included topics like ethical fieldwork, switching careers, science communication, postdoc life, leadership, women in science, job applications, postdoc hopping, outreach, publishing, feeling incompetent, astronaut training, toxic academia, and how to build a research group.

We are now proud to announce that the production of season 3 of Science Sisters has wrapped and post-production, such as the editing of the videos, is in full swing. Anticipated to launch in fall 2025, the new season of Science Sisters will consist of the traditional interview videos and a hybrid online seminar where a viewing party of the episode is combined with an after-show discussion between Iris, the guest, and any research groups and individuals interested in joining.

This hybrid form of Science Sisters has proven to kickstart conversations in institutes and increase the cohesion within institutes by creating a more understanding atmosphere. Early career scientists in particular say that Science Sisters is extremely useful to learn about life as a researcher and they enjoy the chatty, entertaining quality of the interviews.

In season 3, the main topics across our 7 episode series are:

• PhD life

• Failure (and how to deal with it)

• Working at NASA

• Motivation (or lack thereof)

• Science management

• Lab work

• Academic motherhood

Of course, each episode also features individual experiences of (non-)academic career paths to show the diversity of ways in which people can interface with science and work in academia.

Using the hybrid form of videos and online webinars, Science Sisters therefore continues to contribute to promoting and supporting inclusivity in the planetary and geosciences. 

How to cite: Cano Amoros, M. and van Zelst, I.: A new hybrid video & seminar series: Season 3 of Science Sisters is on its way! , EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-6963, https://doi.org/10.5194/egusphere-egu25-6963, 2025.

For many geoscientists, participating in conferences are vital for their career as they provide access to state-of-the-art knowledge in their research field but also provide opportunities to share their own results whilst expanding their research network.

However, the opportunity to attend large geoscience conferences for many researchers often comes at a significant financial burden. In particular, researchers that have caring responsibilities, disabilities or experience temporary unemployment often find it a financial challenge to cover the extra costs incurred for conference participation from research project budgets or from their affiliated research institutions. This not only places a strain on those geoscientists already facing financial hardship, but it also leads to the exclusion of researchers from career-defining meetings.

In 2025, the EGU launched a new EDI Participation Support Scheme for EGU members with the aim of addressing this inequity. This support scheme aims to provide financial assistance to scientists in the Earth, planetary, and space sciences who encounter significant EDI-related financial barriers that prevent them from participating to the EGU General Assembly because of caregiving responsibilities, disability and special needs as well as temporary geoscience career transitions. In this presentation, we will provide valuable information about this new support scheme and encourage the community to raise awareness of these financial burdens with their colleagues, research institutions and research funders.

How to cite: Wingate, L., Hart, J., Turton, J., and Jacobs, P.: Tackling EDI-related financial barriers that reduce inclusivity at geoscience conferences with the EGU EDI Participation Support Scheme, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7140, https://doi.org/10.5194/egusphere-egu25-7140, 2025.

EGU25-7701 | Orals | EOS3.1

Inclusive scientific meetings need alternative modes of participation 

Jens Klump, Vanessa Moss, Rika Kobayashi, Lesley Wyborn, Stefanie Kethers, and Coralie Siegel

Major sporting events, like the Summer Olympics or the FIFA World Cup, attract a global audience of billions of spectators. While many agree that watching the Olympic Games in one of its venues is the best way to experience the event, less than one per mille of the billions worldwide audience can attend in person. The majority watch such events at public events, at home with families and friends, or by themselves on their mobile devices. All these different modes of watching the Olympics allow a global audience access to a major sporting event.

International research meetings were forced into mainly online modes by the COVID-19 pandemic during 2020-2022. While the availability of online formats was initially high, it has since dropped, and only a small fraction of meeting organisers have made efforts to develop new formats that offer value to online participants. At the same time, the poor quality of virtual options and the “rush back to normal” contributed to a drop in virtual participant numbers. This is a missed opportunity; it disregards the high environmental costs of large international meetings and favours those who can afford the high costs and time commitment of international travel and are, therefore, already advantaged. For many in the Global South, attending international conferences offered as in-person-only events is almost impossible, widening the gap in their ability to participate in global science.

While technologies for alternative modes of participation exist, many organisers of conferences cite the excessive cost and a lack of interest as barriers. Financial modelling by a major conference provider showed that offering alternative participation modes adds approximately five to ten per cent to the cost of running a conference, which can be easily offset by attracting additional participants. However, conflicting aims exist between conference organisers wanting to offer alternative participation modes but also having to be financially sustainable, as well as conference venues and tourism boards, who want to maximise the number of participants on-site. It has been reported that tourism boards and conference venues use subsidies and overpriced equipment to discourage alternatives to on-site participation.

For their 2024 Annual Scientific Meeting, the Astronomical Society of Australia organised an “online-first” conference with a location-specific “Hub Day” during the week to offer space for in-person interactions. As this example shows, there are many opportunities to innovate by blending in-person, hybrid, and online formats and adopting new technologies (see, e.g., https://thefutureofmeetings.wordpress.com), including local or regional hubs where participants can gather to discuss and network. Alternative modes are already being used successfully by communities in other areas of society to bring people together and the scientific community is lagging behind. We could draw inspiration from completely different types of events, like games, international sports or cultural events. This presentation is about how we can make research meetings more accessible, inclusive, and sustainable by being more creative about modes of participation and thinking outside the box. 

How to cite: Klump, J., Moss, V., Kobayashi, R., Wyborn, L., Kethers, S., and Siegel, C.: Inclusive scientific meetings need alternative modes of participation, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-7701, https://doi.org/10.5194/egusphere-egu25-7701, 2025.

EGU25-9552 | ECS | Posters on site | EOS3.1

Positive and Negative Academic Workplace Behaviors:  Experiences Gathered at a Scientific Conference 

Nahid Atashi, Anni Hartikainen, Laura Salo, Ilona Ylivinkka, Muhammad Shahzaib, Miikka Dal Maso, and Katja Anniina Lauri

We organized an informal equality, diversity and inclusion (EDI) themed reception for the attendees of the European Aerosol Conference (EAC) 2024 to encourage reflection and sharing of both positive and negative behaviors observed in academic workspaces. 

The event was held in a private venue near the conference site. The three-hour event featured a combination of short talks, a presentation on current and past EDI initiatives within the Finnish aerosol science community, and informal discussions in small groups. The relaxed setting fostered open dialogue and active participation. 

During the event, attendees were invited to anonymously write about their personal experiences at their workspace on sticky notes and attach them to a poster displayed throughout the reception. This interactive approach provided a safe space for participants to voice their thoughts and experiences, which remained visible for collective reflection until the event concluded. 

The collected messages were categorized into two main themes. Positive Aspects included respect and inclusion, supportive environments, social connections, and practical guidance. Negative Aspects highlighted challenges such as discrimination, exclusion, judgment, and unproductive atmospheres. Combined insights collected within this activity provide a clear understanding of workplace dynamics, offering valuable perspectives for promoting equity and addressing areas of concern within academic environments.

How to cite: Atashi, N., Hartikainen, A., Salo, L., Ylivinkka, I., Shahzaib, M., Dal Maso, M., and Lauri, K. A.: Positive and Negative Academic Workplace Behaviors:  Experiences Gathered at a Scientific Conference, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-9552, https://doi.org/10.5194/egusphere-egu25-9552, 2025.

Transition services are essential for supporting students with intellectual disabilities (ID) as they prepare for independent adult lives. While special education teachers in both the United States and Korea acknowledge the importance of providing these systematic services, their actual implementation varies widely due to differing teacher backgrounds and numerous barriers. This study examines these barriers through the lens of Windschitl's framework, which categorizes dilemmas into four types: conceptual, pedagogical, cultural, and political. These dilemmas serve as a foundation for understanding why teachers struggle to implement transition services, even when they recognize their significance.

Focusing on the Korean context, this study explored the experiences of special school teachers working with students with ID and identified additional dilemmas beyond those categorized by Windschitl. To achieve this, qualitative in-depth interviews were conducted with 35 special school teachers currently implementing transition services. Using the constant comparative method, the data was analyzed to uncover key categories, their properties, and how these elements interconnect.

The findings revealed that Korean teachers viewed transition services as vital for equipping students with ID with the skills necessary for employment, societal integration, and independence. However, despite understanding their importance, teachers reported low implementation levels due to various challenges. These included limited resources, insufficient professional development, lack of collaboration among stakeholders, and inadequate institutional support.

Rather than placing blame on teachers for the low implementation of transition services, the study emphasizes the need to create supportive environments. Collaborative efforts among school administrators, parents, policymakers, and disability organizations are critical to fostering conditions where teachers can succeed. Furthermore, investing in professional training and strengthening educational and social infrastructure would significantly enhance teachers’ capacity to provide effective transition services.

By addressing these systemic issues, this study underscores the importance of supporting special educators in their efforts to improve outcomes for students with ID, ultimately enabling them to transition successfully into adulthood.

How to cite: park, Y.: Exploring Barriers and Dilemmas in Transition Services: Insights from Korean Special Education Teachers for Students with Intellectual Disabilities, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10224, https://doi.org/10.5194/egusphere-egu25-10224, 2025.

EGU25-10372 | Posters on site | EOS3.1

Inclusive excellence at the ERC: demographic data on external reviewers and eligibility extensions 

Claudia Jesus-Rydin, Luis Fariña-Busto, Maria Ruiz, Benoit Le Noir de Carlan, and Eystein Jansen

The European Research Council (ERC), Europe’s premier funding agency for frontier research, views equality of opportunities as an essential priority and a vital mission to ensure fairness in the review process. The ERC monitors various demographic data yearly on every call and has taken actions to tackle imbalances and potential implicit and explicit biases.

Demographic gender and geographical distribution data on external reviewers is presented. External reviewers are experts who support ERC evaluation panels by externally reviewing proposals in their fields of specialization. The analysis focuses on the rates of nomination and invitation of these experts, as well as rates of acceptance and completion of the reviews. The data is presented by call and by scientific domain. In the current framework programme (Horizon Europe, 2021-2027), 24% of nominated external reviewers were women, 75% were men and 1% are non-binary. Acceptance and completion rates for men and women are similar.

Furthermore, data on requests of the eligibility window extensions are included. During the grants’ application process, the ERC allows potential grantees to extend the eligibility window, both for Consolidator and Starting Grants. These extensions are conditional on certain circumstances (e.g. parental leave, long-term illness, or clinical training). These circumstances and conditions constantly evolve. In this way, to better comprehend and monitor these requests, the ERC recently started an in-depth analysis of such data, gathered between 2021 and 2024. The data are disaggregated by year, gender, and by grant type. The analysis shows that there is a clear disparity between women researchers and men researchers when requesting extensions; both in terms of numbers and circumstances.

The ERC knows that work to ensure inclusive excellence and equality of opportunities is never-ending. This presentation analyses the institutional efforts, procedures and critically discusses the results.

How to cite: Jesus-Rydin, C., Fariña-Busto, L., Ruiz, M., Le Noir de Carlan, B., and Jansen, E.: Inclusive excellence at the ERC: demographic data on external reviewers and eligibility extensions, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-10372, https://doi.org/10.5194/egusphere-egu25-10372, 2025.

EGU25-11159 | ECS | Orals | EOS3.1

The Citation Gap: An overview of academic output in the field of Natural Hazards and Climate Extremes analysed through Google Scholar data 

Shakti Raj Shrestha, Leonardo Olivetti, Shivang Pandey, Koffi Worou, and Elena Rafetti

There has been a significant increase in both the number of publications and number of citations in the last decade partly fueled by the increased exposure to research papers and such as Google Scholar, Web of Science, ResearchGate, etc. The large data set of scientific literature and respective authors in these platforms can be utilized to get a broad overview of academic discourse. This project aims to investigate the state of academia in the field of Natural Hazards and Climate Extremes using Google Scholar data. A comprehensive set of relevant tags (such as earthquake, volcano, natural hazards, climate extremes etc.) were used to filter the researchers. Additionally, a threshold of 500 citations or more was applied to focus on the most influential academics in this field. We limited the analysis to the period 1990-2023 and subsequently stratified the obtained results by gender (as perceived by the authors) and country of affiliation of the researchers. Data for number of publications was also collected for each of the researchers.

Among 2612 researchers identified, 77.2% are male, 22.6% female, and 0.2% could not be categorized into male or female. Male researchers, on average, received a larger median number of citations compared to women even though the gender citation gap in percentage has been decreasing over the last decade. Notably, regression analysis showed that, there is limited difference in number of citations per publication between the two genders. The data also shows that 78.5% of citations are attributed to researchers in high-income countries, 14.4% for those in middle-income countries, and 7.1% for those in low-income countries despite researchers in low- and middle-income countries publishing more papers per year, on average, than their counter parts in high-income countries. The researchers from high-income countries also get larger number of citations per author, on average, even when controlling for number of publications. However, the citation gap between high-income and low- and middle-income countries has narrowed in recent years. Interestingly, the observed citation gap between researchers is more pronounced due to income group than gender. In conclusion, even though disasters affect poor countries and women disproportionately, the fact that the field of natural hazards and climate extremes is largely high-income country and male-dominated raises fundamental questions on teh epistemology and legitimacy of the scientific knowledge that has been generated. 

How to cite: Shrestha, S. R., Olivetti, L., Pandey, S., Worou, K., and Rafetti, E.: The Citation Gap: An overview of academic output in the field of Natural Hazards and Climate Extremes analysed through Google Scholar data, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-11159, https://doi.org/10.5194/egusphere-egu25-11159, 2025.

EGU25-12317 | Orals | EOS3.1

Equity in Geoscience Publishing: Indigenous Data Governance and Tackling Parachute Science 

Tanya Dzekon, Matt Giampoala, Paige Wooden, and Mia Ricci

Addressing under-representation and inequity in geoscience requires action from all participants of the scientific ecosystem. The collaborative and global nature of our science impels us to create systemic changes to better include historically marginalized voices. This work includes correcting the power imbalances that exist within scholarly publishing through equity-focused policy changes and through collaborations with communities. We will highlight AGU Publications’ recently launched Inclusion in Global Research Policy (an authorship policy to improve equity and transparency in international research collaborations and to help address the issue of parachute science), as well as work to create Guidelines for the Governance of Indigenous Data in Scientific Publishing (a partnership between the Collaboratory for Indigenous Data Governance, ENRICH, Te Kotahi Research Institute, the American Geophysical Union, the National Information Standards Organization, and AGU).

How to cite: Dzekon, T., Giampoala, M., Wooden, P., and Ricci, M.: Equity in Geoscience Publishing: Indigenous Data Governance and Tackling Parachute Science, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-12317, https://doi.org/10.5194/egusphere-egu25-12317, 2025.

EGU25-13088 | ECS | Orals | EOS3.1

Practical implementation of diversity and inclusion measures in large EU Horizon projects: lessons learned from Geo-INQUIRE. 

Elif Türker, Iris Christadler, Fabrice Cotton, Alice-Agnes Gabriel, Fatemeh Jalayer, Mateus Litwin-Prestes, Angelo Strollo, Stefanie Weege, Elisabeth Kohler, Mariusz Majdański, and Laura Sandri

Geo-INQUIRE, an EU Horizon project starting in 2022, brings together 51 partners, including high-level research institutes, universities and European consortia from different EU countries. The project aims to improve access to selected key data, products and services to monitor and model the dynamic processes within the geosphere at new levels of spatial and temporal detail and accuracy. With 150 Virtual Access (VA) and Transnational Access (TA) facilities, together with tailored mentoring programs, including workshops (both online and face-to-face), trainings and seminars, Geo-INQUIRE has brought together over 2,300 researchers in the past two years, offering 20 training events and 7 workshops attended by participants from over 70 countries. While in total 44% of these participants have been female, this number reflects the project’s ongoing commitment to gender balance, inclusion and diversity, but also acknowledges that further progress is still desired.

Despite the projects complexity due to high number of partner institutions, several strategies have been implemented to foster inclusion. These include the unique establishment of an independent advisory committee (EDIP), assigning an EDIP member (by rotation) as ex-officio member of Transnational Activity Review Panel (TARP), thinking of strategies to reduce unconscious bias in review of TA applications, setting targets for female participation and researchers from Horizon’s widening countries, offering travel support and affordable accommodation to reduce financial barriers, recording of online training events to enable access and maximise flexibility. Additionally, novel recruitment practices, supportive workplace policies and efforts to increase female representation in leadership roles have been introduced. Geo-INQUIRE also fosters inclusion across a wide range of career backgrounds (including less conventional career paths) and brings together researchers from diverse scientific disciplines—such as solid earth, marine science, and carbon capture and storage - as well as those with technical expertise in IT. Strategies such as seminars have proven effective in bridging these gaps and reducing barriers between different fields. We will present examples of these actions, discuss lessons learned and propose example guidelines for promoting diversity in large-scale research projects.

How to cite: Türker, E., Christadler, I., Cotton, F., Gabriel, A.-A., Jalayer, F., Litwin-Prestes, M., Strollo, A., Weege, S., Kohler, E., Majdański, M., and Sandri, L.: Practical implementation of diversity and inclusion measures in large EU Horizon projects: lessons learned from Geo-INQUIRE., EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-13088, https://doi.org/10.5194/egusphere-egu25-13088, 2025.

The geosciences are at a pivotal moment as institutions, organizations, and individuals confront long-standing inequities to create a more inclusive and representative future. As a geoscientist actively engaged in equity, diversity, and inclusion (EDI) initiatives, I have witnessed both the barriers and breakthroughs shaping this transformation. Notably, the geosciences have some of the poorest metrics for diversity, equity, and inclusion (DEI) in STEM disciplines. Guided by the principle, “What gets measured, gets done,” my work has focused on quantifying EDI impacts to drive meaningful progress.
Drawing on my role as an executive member of the Canadian Geophysical Union’s EDI Committee, I will present key findings from a comprehensive EDI report on representation statistics from Canadian Geophysical Union conferences since 2018. As a director on the board of Women Geoscientists in Canada, a prominent organization supporting women in technical roles, I will highlight the challenges and successes in addressing gender imbalance and improving diversity within the mining industry.
Lastly as a federal research scientist working on critical mineral exploration and green energy transitions, I will explore how EDI efforts can advance community engagement, inclusive excellence, interdisciplinary collaboration, ethical fieldwork, and environmental justice. By sharing these experiences across government, industry, and academia, this presentation will offer actionable strategies to address barriers and inspire collaboration for a more equitable future in Canadian geosciences.

How to cite: Dave, R.: Advancing Equity in Geosciences: Insights and Actions from the Canadian EDI Landscape, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-14621, https://doi.org/10.5194/egusphere-egu25-14621, 2025.

EGU25-18414 | Posters on site | EOS3.1

An EDI time capsule from the 2023 Karthaus Summer School: Where do we want the glaciological community to be in 50 years? 

Lena Nicola, Rebekka Frøystad, Antonio Juarez-Martinez, Maxence Menthon, Ana Carolina Moraes Luzardi, Katherine Turner, Sally F. Wilson, and Benjamin Keisling and the Karthaus 2023 EDI team

Despite the increased awareness towards Equality, Diversity, and Inclusion (EDI), the glaciological community still experiences and perpetuates numerous examples of inappropriate and discriminatory behavior, adding to the systemic inequalities embedded in the scientific community. What are the EDI challenges we currently face within the glaciological research community? How can we overcome them? Where do we want our research community to be in fifty years? These questions were used as a starting point for a first-of-its-kind workshop at the 2023 Karthaus Summer School on Ice Sheets and Glaciers in the Climate System. Drawing on the outcomes of that workshop, we discuss the answers and challenges to addressing these questions, in the form of both actionable steps forward and imaginative visions of the future. We identified common threads from the workshop responses and distilled them into collective visions for the future. Having consulted additional literature, while formulating suggestions for improvement, stating our own commitment, and highlighting existing initiatives, contributions to this “time capsule” exercise were sorted into three main challenges we want and need to face: making glaciology more accessible, equitable, and responsible (Nicola et al, in review).

How to cite: Nicola, L., Frøystad, R., Juarez-Martinez, A., Menthon, M., Moraes Luzardi, A. C., Turner, K., Wilson, S. F., and Keisling, B. and the Karthaus 2023 EDI team: An EDI time capsule from the 2023 Karthaus Summer School: Where do we want the glaciological community to be in 50 years?, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-18414, https://doi.org/10.5194/egusphere-egu25-18414, 2025.

EGU25-20423 | Orals | EOS3.1

Working towards more equitable  recomendations and nomination letters: Equitable Letters for Space and Physics 

Alexa Halford, Angeline Burrell, John Coxon, McArthur Jones, Kate Zawdie, and Julie Barnam

Equitable Letters in Space and Physics (ELSP) is an organization that aims to encourage merit-based recommendations and nominations in the space physics community by providing resources and reviews. Recommendation and award nomination letters are a known source of bias that affect education and job opportunities, career progression, and recognition for scientists from underrepresented backgrounds.  ELSP was founded to combat this bias within the current system by providing a proof-reading service that focuses on identifying phrasing and structure within letters that unintentionally undermines the purpose of the missive.  If you are writing a recommendation letter for someone you know professionally, you can send it to us and we will send it out to our reviewers. They will provide recommendations on how you can make your letter more equitable and less biased, using a combination of the techniques and resources described on our site, with the aim to make unbiased recommendation letters more accessible to all. If you are interested in being a reviewer or having your writing reviewed, please reach out to us.

How to cite: Halford, A., Burrell, A., Coxon, J., Jones, M., Zawdie, K., and Barnam, J.: Working towards more equitable  recomendations and nomination letters: Equitable Letters for Space and Physics, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20423, https://doi.org/10.5194/egusphere-egu25-20423, 2025.

EGU25-20788 * | Orals | EOS3.1 | Highlight

Failure to Act:  Universities’ Promising EDI Template Withering on the Vine 

Holly Stein and Judith Hannah

The triumphant implementation of equity, diversity, and inclusivity (EDI) programs in academia after more than a decade of increasing pressure and promise has brought hope to many but, unfortunately, justice to few. Enough time has passed to reveal the fraught inner workings of academia and their ability to make effective change, even as universities might be expected to lead with exemplary behavior. Sadly, the reverse is true. Failure of universities to act or react appropriately has seriously crippled EDI efforts in many academic settings. University administrators and even university presidents have lost their employment for taking EDI seriously. Those facts severely degrade the EDI landscape in academia going forward.

Stepping back and turning a scientific lens on the university environment, what are the flaws in implementation? They are rooted in human behavior and decision-making in adversarial surroundings, the recipe for fear. One might line up the course of action in three steps: (1) identifying the issues, (2) building a structure and path toward solution, and (3) establishing a university-sanctioned outcome that removes perpetual perpetrators and enables, even celebrates, those with the courage to speak up. A power relationship is almost always part of the play. Alas, though the first step is generally mastered, the second step is better known as “protecting the university at all costs”, and completion of the third step is dead rare. Rather, the rare settlement involves a victim signing away their right to talk to the press, so as not to damage the university’s reputation. This obvious three-act opera loses footing in the second act. The outcome is driven by “what is the easiest path for the university” and is too rarely driven by doing the right thing. The EDI system at most universities presents the ultimate conflict-of-interest: university lawyers are paid by the university or its governing body and thus, are indebted to them for employment and the outcomes of EDI decisions they make.

Failure to Act is a three-act play that explores the darker workings behind the academic scenery.  Can we change the storyline so that students and faculty will believe that the system works for them, should they ever need it? That is far from the standard we have now, even as sometimes generous funding has been diverted to build up EDI programming in academia. 

How to cite: Stein, H. and Hannah, J.: Failure to Act:  Universities’ Promising EDI Template Withering on the Vine, EGU General Assembly 2025, Vienna, Austria, 27 Apr–2 May 2025, EGU25-20788, https://doi.org/10.5194/egusphere-egu25-20788, 2025.

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